FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Abeykoon, AMM Hu, HF Wu, LJ Zhu, YM Billinge, SJL AF Abeykoon, A. M. Milinda Hu, Hefei Wu, Lijun Zhu, Yimei Billinge, Simon J. L. TI Calibration and data collection protocols for reliable lattice parameter values in electron pair distribution function studies SO JOURNAL OF APPLIED CRYSTALLOGRAPHY LA English DT Article DE electron pair distribution function; calibration; data collection; nanomaterials ID AMORPHOUS MATERIALS; GOLD NANOPARTICLE; DIFFRACTION; NANOCRYSTALS; REFINEMENT; MICROSCOPY; SIZE; PDF AB Different protocols for calibrating electron pair distribution function (ePDF) measurements are explored and described for quantitative studies on nanomaterials. It is found that the most accurate approach to determine the camera length is to use a standard calibration sample of Au nanoparticles from the National Institute of Standards and Technology. Different protocols for data collection are also explored, as are possible operational errors, to find the best approaches for accurate data collection for quantitative ePDF studies. C1 [Abeykoon, A. M. Milinda; Hu, Hefei; Wu, Lijun; Zhu, Yimei; Billinge, Simon J. L.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Billinge, Simon J. L.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. RP Abeykoon, AMM (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. EM aabeykoon@bnl.gov FU US Department of Energy, Office of Science, Office of Basic Energy Sciences (DOE-BES) [DE-AC02-98CH10886]; DOE-BES [DE-AC02-98CH10886] FX This work was carried out as part of the Flucteam project at BNL supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences (DOE-BES), through account DE-AC02-98CH10886. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the DOE-BES under contract No. DE-AC02-98CH10886. NR 37 TC 4 Z9 4 U1 3 U2 17 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 1600-5767 J9 J APPL CRYSTALLOGR JI J. Appl. Crystallogr. PD FEB PY 2015 VL 48 BP 244 EP 251 DI 10.1107/S1600576715000412 PN 1 PG 8 WC Chemistry, Multidisciplinary; Crystallography SC Chemistry; Crystallography GA CA8ZU UT WOS:000349210700031 ER PT J AU Konnecke, M Akeroyd, FA Bernstein, HJ Brewster, AS Campbell, SI Clausen, B Cottrell, S Hoffmann, JU Jemian, PR Mannicke, D Osborn, R Peterson, PF Richter, T Suzuki, J Watts, B Wintersberger, E Wuttke, J AF Koennecke, Mark Akeroyd, Frederick A. Bernstein, Herbert J. Brewster, Aaron S. Campbell, Stuart I. Clausen, Bjoern Cottrell, Stephen Hoffmann, Jens Uwe Jemian, Pete R. Maennicke, David Osborn, Raymond Peterson, Peter F. Richter, Tobias Suzuki, Jiro Watts, Benjamin Wintersberger, Eugen Wuttke, Joachim TI The NeXus data format SO JOURNAL OF APPLIED CRYSTALLOGRAPHY LA English DT Software Review DE NeXus data format; data exchange; data archiving; platform-independent; HDF5 AB NeXus is an effort by an international group of scientists to define a common data exchange and archival format for neutron, X-ray and muon experiments. NeXus is built on top of the scientific data format HDF5 and adds domain-specific rules for organizing data within HDF5 files, in addition to a dictionary of well defined domain-specific field names. The NeXus data format has two purposes. First, it defines a format that can serve as a container for all relevant data associated with a beamline. This is a very important use case. Second, it defines standards in the form of application definitions for the exchange of data between applications. NeXus provides structures for raw experimental data as well as for processed data. C1 [Koennecke, Mark] Paul Scherrer Inst, Lab Dev & Methods, CH-5232 Villigen, Switzerland. [Akeroyd, Frederick A.; Cottrell, Stephen] Rutherford Appleton Lab, ISIS Facil, STFC, Didcot OX11 0QX, Oxon, England. [Bernstein, Herbert J.] Dowling Coll, ImgCIF, Shirley, NY 11769 USA. [Brewster, Aaron S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Campbell, Stuart I.; Peterson, Peter F.] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. [Clausen, Bjoern] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Hoffmann, Jens Uwe] Helmholtz Zentrum Berlin Mat & Energie Gmb, D-14109 Berlin, Germany. [Jemian, Pete R.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Maennicke, David] Australian Nucl Sci & Technol Org, Menai, NSW 2234, Australia. [Osborn, Raymond] Argonne Natl Lab, Argonne, IL 60439 USA. [Richter, Tobias] Diamond Light Source, Didcot OX11 0DE, Oxon, England. [Suzuki, Jiro] KEK, Tsukuba, Ibaraki 3050801, Japan. [Watts, Benjamin] Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland. [Wintersberger, Eugen] Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany. [Wuttke, Joachim] Forschungszentrum Julich, JCNS, MLZ, D-85747 Garching, Germany. RP Konnecke, M (reprint author), Paul Scherrer Inst, Lab Dev & Methods, CH-5232 Villigen, Switzerland. EM mark.koennecke@psi.ch RI Campbell, Stuart/A-8485-2010; Clausen, Bjorn/B-3618-2015; OI Campbell, Stuart/0000-0001-7079-0878; Clausen, Bjorn/0000-0003-3906-846X; Wuttke, Joachim/0000-0002-4028-1447 FU DOE; NIH; NSF in the USA; Scientific User Facilities Division; Materials Science and Engineering Division, Basic Energy Sciences, Office of Science, US Department of Energy; European Commission FX The NIAC acknowledges the support of all the institutions contributing to NeXus and their respective funding agencies, most notably the DOE, NIH and NSF in the USA. Work at DOE National Laboratories was supported by the Scientific User Facilities Division and the Materials Science and Engineering Division, Basic Energy Sciences, Office of Science, US Department of Energy. The development of the mu SR NeXus data format was partly funded by the European Commission within the sixth Framework Programme. NR 13 TC 8 Z9 8 U1 1 U2 8 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 1600-5767 J9 J APPL CRYSTALLOGR JI J. Appl. Crystallogr. PD FEB PY 2015 VL 48 BP 301 EP 305 DI 10.1107/S1600576714027575 PN 1 PG 5 WC Chemistry, Multidisciplinary; Crystallography SC Chemistry; Crystallography GA CA8ZU UT WOS:000349210700039 ER PT J AU Popa, NC Balzar, D Vogel, SC AF Popa, N. C. Balzar, D. Vogel, S. C. TI Elastic macro strain and stress determination by powder diffraction: spherical harmonics analysis starting from the Voigt model (vol 47, pg 154, 2014) SO JOURNAL OF APPLIED CRYSTALLOGRAPHY LA English DT Correction DE strain; stress; textured polycrystals; powder diffraction; spherical harmonics AB Corrections to the paper by are provided. C1 [Popa, N. C.] Natl Inst Mat Phys, Magurele 077125, Ilfov, Romania. [Balzar, D.] Univ Denver, Dept Phys & Astron, Denver, CO 80208 USA. [Vogel, S. C.] Los Alamos Natl Lab, Los Alamos Neutron Scattering Ctr, Los Alamos, NM 87545 USA. RP Balzar, D (reprint author), Univ Denver, Dept Phys & Astron, 2112 East Wesley Ave, Denver, CO 80208 USA. EM balzar@du.edu NR 4 TC 0 Z9 0 U1 3 U2 3 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0021-8898 EI 1600-5767 J9 J APPL CRYSTALLOGR JI J. Appl. Crystallogr. PD FEB PY 2015 VL 48 BP 311 EP 311 DI 10.1107/S1600576714026673 PN 1 PG 1 WC Chemistry, Multidisciplinary; Crystallography SC Chemistry; Crystallography GA CA8ZU UT WOS:000349210700042 ER PT J AU Regenauer-Lieb, K Bunger, A Chua, HT Dyskin, A Fusseis, F Gaede, O Jeffrey, R Karrech, A Kohl, T Liu, J Lyakhovsky, V Pasternak, E Podgorney, R Poulet, T Rahman, S Schrank, C Trefry, M Veveakis, M Wu, BS Yuen, DA Wellmann, F Zhang, X AF Regenauer-Lieb, Klaus Bunger, Andrew Chua, Hui Tong Dyskin, Arcady Fusseis, Florian Gaede, Oliver Jeffrey, Rob Karrech, Ali Kohl, Thomas Liu, Jie Lyakhovsky, Vladimir Pasternak, Elena Podgorney, Robert Poulet, Thomas Rahman, Sheik Schrank, Christoph Trefry, Mike Veveakis, Manolis Wu, Bisheng Yuen, David A. Wellmann, Florian Zhang, Xi TI Deep geothermal: The 'Moon Landing' mission in the unconventional energy and minerals space SO JOURNAL OF EARTH SCIENCE LA English DT Article DE geothermal energy; enhanced geothermal systems; fracture mechanics; creep; dissolution; precipitation ID THERMO-PORO-MECHANICS; CREEP; RESERVOIRS; FRACTURE AB Deep geothermal from the hot crystalline basement has remained an unsolved frontier for the geothermal industry for the past 30 years. This poses the challenge for developing a new unconventional geomechanics approach to stimulate such reservoirs. While a number of new unconventional brittle techniques are still available to improve stimulation on short time scales, the astonishing richness of failure modes of longer time scales in hot rocks has so far been overlooked. These failure modes represent a series of microscopic processes: brittle microfracturing prevails at low temperatures and fairly high deviatoric stresses, while upon increasing temperature and decreasing applied stress or longer time scales, the failure modes switch to transgranular and intergranular creep fractures. Accordingly, fluids play an active role and create their own pathways through facilitating shear localization by a process of time-dependent dissolution and precipitation creep, rather than being a passive constituent by simply following brittle fractures that are generated inside a shear zone caused by other localization mechanisms. We lay out a new theoretical approach for the design of new strategies to utilize, enhance and maintain the natural permeability in the deeper and hotter domain of geothermal reservoirs. The advantage of the approach is that, rather than engineering an entirely new EGS reservoir, we acknowledge a suite of creep-assisted geological processes that are driven by the current tectonic stress field. Such processes are particularly supported by higher temperatures potentially allowing in the future to target commercially viable combinations of temperatures and flow rates. C1 [Regenauer-Lieb, Klaus; Chua, Hui Tong; Dyskin, Arcady; Gaede, Oliver; Karrech, Ali; Liu, Jie; Pasternak, Elena; Schrank, Christoph] Univ New S Wales, Sch Petr Engn, Sydney, NSW 2052, Australia. [Regenauer-Lieb, Klaus; Jeffrey, Rob; Poulet, Thomas; Veveakis, Manolis; Wu, Bisheng; Zhang, Xi] CSIRO, Earth Sci & Resource Engn, Kensington, WA 6151, Australia. [Regenauer-Lieb, Klaus; Rahman, Sheik] Univ Western Australia, Sch Earth & Environm, Perth, WA 6000, Australia. [Bunger, Andrew] Univ Pittsburgh, Dept Civil & Environm Engn, Pittsburgh, PA USA. [Bunger, Andrew] Univ Pittsburgh, Dept Chem & Petr Engn, Pittsburgh, PA 15261 USA. [Fusseis, Florian] Univ Edinburgh, Sch Geosci, Edinburgh, Midlothian, Scotland. [Gaede, Oliver; Schrank, Christoph] Queensland Univ Technol, Fac Sci & Engn, Sch Earth Environm & Biol Sci, Brisbane, Qld 4001, Australia. [Kohl, Thomas] Karlsruhe Inst Technol, D-76021 Karlsruhe, Germany. [Liu, Jie] Sun Yat Sen Univ, Sch Earth Sci & Geol Engn, Guangzhou 510275, Guangdong, Peoples R China. [Lyakhovsky, Vladimir] Geol Survey Israel, IL-95501 Jerusalem, Israel. [Podgorney, Robert] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Yuen, David A.] China Univ Geosci, Sch Environm Studies, Wuhan 430074, Peoples R China. [Trefry, Mike] CSIRO, Land & Water, Floreat Pk, WA 6014, Australia. [Wellmann, Florian] Rhein Westfal TH Aachen, Aachen Inst Adv Study Computat Engn Sci AICES, D-52062 Aachen, Germany. [Yuen, David A.] Univ Minnesota, Dept Earth Sci, Minneapolis, MN 55455 USA. [Yuen, David A.] Univ Minnesota, Minnesota Supercomp Inst, Minneapolis, MN 55455 USA. RP Regenauer-Lieb, K (reprint author), Univ New S Wales, Sch Petr Engn, Sydney, NSW 2052, Australia. EM klaus@unsw.edu.au RI Chua, HT/B-1317-2008; Kohl, Thomas/M-5704-2013; Fusseis, Florian/M-5321-2016; Wellmann, Florian/N-5041-2016; OI Chua, HT/0000-0001-7923-6857; Fusseis, Florian/0000-0002-3104-8109; Wellmann, Florian/0000-0003-2552-1876; Gaede, Oliver/0000-0002-1684-2873; Regenauer-Lieb, Klaus/0000-0002-2198-5895 NR 36 TC 1 Z9 1 U1 3 U2 23 PU CHINA UNIV GEOSCIENCES PI BEIJING PA 29 XUEYUAN RD, BEIJING, 100083, PEOPLES R CHINA SN 1674-487X EI 1867-111X J9 J EARTH SCI-CHINA JI J. Earth Sci. PD FEB PY 2015 VL 26 IS 1 BP 2 EP 10 DI 10.1007/s12583-015-0515-1 PG 9 WC Geosciences, Multidisciplinary SC Geology GA CA6HS UT WOS:000349012500002 ER PT J AU Khan, A Naz, BS Bowling, LC AF Khan, Asif Naz, Bibi S. Bowling, Laura C. TI Separating snow, clean and debris covered ice in the Upper Indus Basin, Hindukush-Karakoram-Himalayas, using Landsat images between 1998 and 2002 SO JOURNAL OF HYDROLOGY LA English DT Article DE ELA; AAR; Glacier inventory; Upper Indus Basin; Snow and glaciers ID EQUILIBRIUM-LINE ALTITUDES; GLACIAL MASS-BALANCE; RISING RIVER FLOWS; BALTORO GLACIER; SPATIAL-DISTRIBUTION; METEOROLOGICAL DATA; NORTHERN PAKISTAN; INVENTORY; ELEVATION; CLIMATE AB The Hindukush Karakoram Himalayan mountains contain some of the largest glaciers of the world, and supply melt water from perennial snow and glaciers to the Upper Indus Basin (UIB) upstream of Tarbela dam, which constitutes greater than 80% of the annual flows, and caters to the needs of millions of people in the Indus Basin. It is therefore important to study the response of perennial snow and glaciers in the UIB under changing climatic conditions, using improved hydrological modeling, glacier mass balance, and observations of glacier responses. However, the available glacier inventories and datasets only provide total perennial-snow and glacier cover areas, despite the fact that snow, clean ice and debris covered ice have different melt rates and densities. This distinction is vital for improved hydrological modeling and mass balance studies. This study, therefore, presents a separated perennial snow and glacier inventory (perennial snow-cover on steep slopes, perennial snow-covered ice, clean and debris covered ice) based on a semi-automated method that combines Landsat images and surface slope information in a supervised maximum likelihood classification to map distinct glacier zones, followed by manual post processing. The accuracy of the presented inventory falls well within the accuracy limits of available snow and glacier inventory products. For the entire UIB, estimates of perennial and/or seasonal snow on steep slopes, snow-covered ice, clean and debris covered ice zones are 7238 +/- 724, 5226 +/- 522, 4695 +/- 469 and 2126 +/- 212 km(2) respectively. Thus total snow and glacier cover is 19,285 +/- 1928 km(2), out of which 12,075 +/- 1207 km(2) is glacier cover (excluding steep slope snow-cover). Equilibrium Line Altitude (ELA) estimates based on the Snow Line Elevation (SLE) in various watersheds range between 4800 and 5500 m, while the Accumulation Area Ratio (AAR) ranges between 7% and 80%. 0 degrees C isotherms during peak ablation months (July and August) range between similar to 5500 and 6200 m in various watersheds. These outputs can be used as input to hydrological models, to estimate spatially-variable degree day factors for hydrological modeling, to separate glacier and snow-melt contributions in river flows, and to study glacier mass balance, and glacier responses to changing climate. (C) 2014 Elsevier B.V. All rights reserved. C1 [Khan, Asif] Univ Cambridge, Dept Engn, Cambridge CB3 1PZ, England. [Naz, Bibi S.; Bowling, Laura C.] Purdue Univ, Dept Agron, W Lafayette, IN 47907 USA. [Naz, Bibi S.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Khan, A (reprint author), Univ Cambridge, Dept Engn, Trumpington St, Cambridge CB3 1PZ, England. EM engrasif_civil@yahoo.com RI Bowling, Laura/B-6963-2013; OI Bowling, Laura/0000-0002-1439-3154; Khan, Asif/0000-0002-3724-1508; Naz, Bibi/0000-0001-9888-1384 NR 114 TC 7 Z9 7 U1 4 U2 20 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-1694 EI 1879-2707 J9 J HYDROL JI J. Hydrol. PD FEB PY 2015 VL 521 BP 46 EP 64 DI 10.1016/j.jhydrol.2014.11.048 PG 19 WC Engineering, Civil; Geosciences, Multidisciplinary; Water Resources SC Engineering; Geology; Water Resources GA CA4MZ UT WOS:000348879900004 ER PT J AU McCloy, J Washton, N Gassman, P Marcial, J Weaver, J Kukkadapu, R AF McCloy, John Washton, Nancy Gassman, Paul Marcial, Jose Weaver, Jamie Kukkadapu, Ravi TI Nepheline crystallization in boron-rich alumino-silicate glasses as investigated by multi-nuclear NMR, Raman, & Mossbauer spectroscopies SO JOURNAL OF NON-CRYSTALLINE SOLIDS LA English DT Article DE Nuclear waste glass; Alumino-boro-silicate; NMR; Mossbauer; Nepheline ID ALKALI BOROSILICATE GLASSES; HIGH-RESOLUTION B-11; AL-27 MAS NMR; NUCLEAR-WASTE GLASS; CRYSTAL-CHEMISTRY; SILICATE-GLASSES; MINERAL GLASSES; STRUCTURAL BEHAVIOR; MODULATED STRUCTURE; CHEMICAL-SHIFT AB A spectroscopic study was conducted on six simulant nuclear waste glasses using multi-nuclear NMR, Raman, and MOssbauer spectroscopies exploring the role of Si, Al, B, Na, and Fe in the glass network with the goal of understanding melt structure precursors to deleterious nepheline crystal formation. NMR showed two sites each for Al, Si, and Na in the samples which crystallized significant amounts of nepheline, and B speciation changed, typically resulting in more B(IV) after crystallization. Raman spectroscopy suggested that some of the glass structure is composed of metaborate chains or rings, thus significant numbers of non-bridging oxygen and a separation of the borate from the alumino-silicate network. Mossbauer, combined with Fe redox chemical measurements, showed Fe playing a minor role in these glasses, mostly as Fe3+, but iron oxide spinel forms with nepheline in all cases. A model of the glass network and allocation of non-bridging oxygens (NB0s) was computed using experimental B(IV) fractions which predicted a large amount of NBO consistent with Raman spectra of metaborate features. (C) 2014 Elsevier B.V. All rights reserved. C1 [McCloy, John] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. [McCloy, John; Marcial, Jose] Washington State Univ, Mat Sci & Engn Program, Pullman, WA 99164 USA. [Washton, Nancy; Kukkadapu, Ravi] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Gassman, Paul] Pacific NW Natl Lab, Richland, WA 99352 USA. [Weaver, Jamie] Washington State Univ, Dept Chem, Pullman, WA 99164 USA. RP McCloy, J (reprint author), Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. EM john.mccloy@wsu.edu RI Marcial, Jose/I-9627-2016; OI Marcial, Jose/0000-0001-6156-5310; McCloy, John/0000-0001-7476-7771 FU Department of Energy (DOE)'s Waste Treatment & Immobilization Plant Federal Project Office [DE-EM0002904]; Battelle Memorial Institute for the U.S. DOE [DE-AC05-76RL01830]; DOE's Office of Biological and Environmental Research FX This work was supported by the Department of Energy (DOE)'s Waste Treatment & Immobilization Plant Federal Project Office contract number DE-EM0002904 under the direction of Dr. Albert A. Kruger at DOE. A portion of the research was performed at Pacific Northwest National Laboratory (PNNL), operated by Battelle Memorial Institute for the U.S. DOE under contract DE-AC05-76RL01830. A portion of this research was performed using the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research and located at PNNL. NR 112 TC 4 Z9 5 U1 12 U2 48 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3093 EI 1873-4812 J9 J NON-CRYST SOLIDS JI J. Non-Cryst. Solids PD FEB 1 PY 2015 VL 409 BP 149 EP 165 DI 10.1016/j.jnoncrysol.2014.11.013 PG 17 WC Materials Science, Ceramics; Materials Science, Multidisciplinary SC Materials Science GA CA4PU UT WOS:000348888000020 ER PT J AU Terrani, KA Kiggans, JO Silva, CM Shih, C Katoh, Y Snead, LL AF Terrani, K. A. Kiggans, J. O. Silva, C. M. Shih, C. Katoh, Y. Snead, L. L. TI Progress on matrix SiC processing and properties for fully ceramic microencapsulated fuel form SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID SILICON-CARBIDE; THERMAL-CONDUCTIVITY; NEUTRON-IRRADIATION; HTR FUEL; COMPOSITES; TEMPERATURE; FABRICATION; STABILITY AB The consolidation mechanism and resulting properties of the silicon carbide (SiC) matrix of fully ceramic microencapsulated (FCM) fuel form are discussed. The matrix is produced via the nano-infiltration transient eutectic-forming (NITE) process. Coefficient of thermal expansion, thermal conductivity, and strength characteristics of this SiC matrix have been characterized in the unirradiated state. An ad hoc methodology for estimation of thermal conductivity of the neutron-irradiated NITE-SiC matrix is also provided to aid fuel performance modeling efforts specific to this concept. Finally, specific processing methods developed for production of an optimal and reliable fuel form using this process are summarized. These various sections collectively report the progress made to date on production of optimal FCM fuel form to enable its application in light water and advanced reactors. (C) 2014 Elsevier B. V. All rights reserved. C1 [Terrani, K. A.; Kiggans, J. O.; Silva, C. M.; Shih, C.; Katoh, Y.; Snead, L. L.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Terrani, KA (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM terranika@ornl.gov RI kiggans, james/E-1588-2017 OI kiggans, james/0000-0001-5056-665X FU Advanced Fuels Campaign of the Fuel Cycle R&D program in the Office of Nuclear Energy; US Department of Energy FX B. Slone, S. Jurek, W. Porter, T. Geer, J. Su, M. Trammell, and J. Pryor contributed to the experimental investigations. T. Koyanagi provided useful comments on the manuscript. The work presented in this paper was supported by the Advanced Fuels Campaign of the Fuel Cycle R&D program in the Office of Nuclear Energy, US Department of Energy. NR 36 TC 5 Z9 6 U1 2 U2 15 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD FEB PY 2015 VL 457 BP 9 EP 17 DI 10.1016/j.jnucmat.2014.10.034 PG 9 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA CA8KO UT WOS:000349169100002 ER PT J AU Judge, CD Gauquelin, N Walters, L Wright, M Cole, JI Madden, J Botton, GA Griffiths, M AF Judge, Colin D. Gauquelin, Nicolas Walters, Lori Wright, Mike Cole, James I. Madden, James Botton, Gianluigi A. Griffiths, Malcolm TI Intergranular fracture in irradiated Inconel X-750 containing very high concentrations of helium and hydrogen SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID ALLOYS; NICKEL AB In recent years, it has been observed that Inconel X-750 spacers in CANDU reactors exhibits lower ductility with reduced load carrying capacity following irradiation in a reactor environment. The fracture behaviour of ex-service material was also found to be entirely intergranular at high doses. The thermalized flux spectrum in a CANDU reactor leads to transmutation of Ni-58 to Ni-59. The Ni-59 itself has unusually high thermal neutron reaction cross-sections of the type: (n, gamma), (n, p), and (n, alpha). The latter two reactions, in particular, contribute to a significant enhancement of the atomic displacements in addition to creating high concentrations of hydrogen and helium within the material. Microstructural examinations by transmission electron microscopy (TEM) have confirmed the presence of helium bubbles in the matrix and aligned along grain boundaries and matrix-precipitate interfaces. Helium bubble size and density are found to be highly dependent on the irradiation temperature and material microstructure; the bubbles are larger within grain boundary precipitates. TEM specimens extracted from fracture surfaces and crack tips provide information that is consistent with crack propagation along grain boundaries due to the presence of He bubbles. (C) 2014 Published by Elsevier B.V. C1 [Judge, Colin D.; Walters, Lori; Wright, Mike; Griffiths, Malcolm] Atom Energy Canada Ltd, Chalk River, ON K0J 1J0, Canada. [Gauquelin, Nicolas; Botton, Gianluigi A.] McMaster Univ, Hamilton, ON, Canada. [Cole, James I.; Madden, James] Idaho Natl Lab, Idaho Falls, ID USA. RP Judge, CD (reprint author), Atom Energy Canada Ltd, Chalk River, ON K0J 1J0, Canada. EM judgec@aecl.ca OI Cole, James/0000-0003-1178-5846 FU CANDU Owners Group (COG); NSERC; McMaster University FX The authors would like to thank D. Lewis, R. Beier, and C. LeMoine for their assistance sectioning spacers in the Atomic Energy of Canada Limited hot cells. The author would also like to thank the technical staff at Idaho National Laboratory and the Center of Advanced Energy Studies in Idaho Falls, and the technical staff at the Canadian Centre of Electron Microscopy at McMaster University for their technical assistance and guidance during this investigation. G. A. Botton and N. Gauquelin are grateful to ORF-RE "Nuclear Ontario'' project for partial funding of this work. The CCEM is a national facility supported by NSERC and McMaster University.; This work was performed under a Collaborative Research and Development Agreement (CRADA) No. 11-CR-16 between Battelle Energy Alliance (through the Advanced Test Reactor National Scientific User Facility) and Atomic Energy of Canada Limited. The authors would also like to thank the CANDU Owners Group (COG) for financial support for some of this work, and permission to use the data. NR 21 TC 5 Z9 5 U1 2 U2 19 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD FEB PY 2015 VL 457 BP 165 EP 172 DI 10.1016/j.jnucmat.2014.10.008 PG 8 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA CA8KO UT WOS:000349169100022 ER PT J AU Westphal, BR Price, JC Bateman, KJ Marsden, KC AF Westphal, B. R. Price, J. C. Bateman, K. J. Marsden, K. C. TI Zirconium determination by cooling curve analysis during the pyroprocessing of used nuclear fuel SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID U-ZR; URANIUM; SYSTEM; ALLOYS AB An alternative method to sampling and chemical analyses has been developed to monitor the concentration of zirconium in real-time during the casting of uranium products from the pyroprocessing of used nuclear fuel. The method utilizes the solidification characteristics of the uranium products to determine zirconium levels based on standard cooling curve analyses and established binary phase diagram data. Numerous uranium products have been analyzed for their zirconium content and compared against measured zirconium data. From this data, the following equation was derived for the zirconium content of uranium products: Zr = 0:14M + 131.56 - 12.63(348.65 - 0.16LT)(1/2) where M is the mass (kg) of the ingot and LT is the liquidus temperature (K) found by cooling curve analyses. Based on this equation, a reasonable fit of calculated to measured zirconium content was established considering the errors in the system. (C) 2014 Elsevier B.V. All rights reserved. C1 [Westphal, B. R.; Price, J. C.; Bateman, K. J.; Marsden, K. C.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Westphal, BR (reprint author), Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. EM brian.westphal@inl.gov FU U.S. Department of Energy, Office of Nuclear Energy, Science, and Technology, under DOE-NE Idaho Operations Office [DE-AC07-05ID14517] FX The authors would like to acknowledge the Fuel Conditioning Facility operations personnel for their recent contributions and the Analytical Laboratory staff for chemical services. This work was supported by the U.S. Department of Energy, Office of Nuclear Energy, Science, and Technology, under DOE-NE Idaho Operations Office Contract DE-AC07-05ID14517. NR 16 TC 1 Z9 1 U1 0 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD FEB PY 2015 VL 457 BP 241 EP 245 DI 10.1016/j.jnucmat.2014.11.091 PG 5 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA CA8KO UT WOS:000349169100032 ER PT J AU Matthews, C Schwen, D Klein, AC AF Matthews, Christopher Schwen, Daniel Klein, Andrew C. TI Radiation re-solution of fission gas in non-oxide nuclear fuel SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID MOLECULAR-DYNAMICS; SWELLING ANALYSIS; URANIUM-DIOXIDE; OXIDE FUELS; LMFBR FUELS; UO2; IRRADIATION; BUBBLES; BEHAVIOR; RELEASE AB Renewed interest in fast nuclear reactors is creating a need for better understanding of fission gas bubble behavior in non-oxide fuels to support very long fuel lifetimes. Collisions between fission fragments and their subsequent cascades can knock fission gas atoms out of bubbles and back into the fuel lattice. We showed that these collisions can be treated as using the so-called "homogenous" atom-by-atom re-solution theory and calculated using the Binary Collision Approximation code 3DOT. The calculations showed that there is a decrease in the re-solution parameter as bubble radius increases until about 50 nm, at which the re-solution parameter stays nearly constant. Furthermore, our model shows ion cascades created in the fuel result in many more implanted fission gas atoms than collisions directly with fission fragments. This calculated re-solution parameter can be used to find a re-solution rate for future bubble simulations. (C) 2014 Elsevier B.V. All rights reserved. C1 [Matthews, Christopher; Klein, Andrew C.] Oregon State Univ, Corvallis, OR 97331 USA. [Schwen, Daniel] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Matthews, C (reprint author), Oregon State Univ, 3451 SW Jefferson Way, Corvallis, OR 97331 USA. EM matthchr@engr.orst.edu OI Schwen, Daniel/0000-0002-8958-4748 FU DOE Office of Nuclear Energy's Nuclear Energy University Programs FX This research was performed entirely at Oregon State University using funding received from the DOE Office of Nuclear Energy's Nuclear Energy University Programs. NR 40 TC 0 Z9 0 U1 1 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD FEB PY 2015 VL 457 BP 273 EP 278 DI 10.1016/j.jnucmat.2014.11.108 PG 6 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA CA8KO UT WOS:000349169100037 ER PT J AU Kaspar, TC Bowden, ME Wang, CM Shutthanandan, V Overman, NR van Ginhoven, RM Wirth, BD Kurtz, RJ AF Kaspar, T. C. Bowden, M. E. Wang, C. M. Shutthanandan, V. Overman, N. R. van Ginhoven, R. M. Wirth, B. D. Kurtz, R. J. TI Epitaxial Fe/Y2O3 interfaces as a model system for oxide-dispersion-strengthened ferritic alloys SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID YTTRIA-STABILIZED ZIRCONIA; PULSED-LASER DEPOSITION; THIN-FILMS; ODS STEELS; NANOCLUSTERS AB The fundamental mechanisms underlying the superior radiation tolerance properties of oxide-dispersion-strengthened ferritic steels and nanostructured ferritic alloys are poorly understood. Thin film heterostructures of Fe/Y2O3 can serve as a model system for fundamental studies of radiation damage. Epitaxial thin films of Y2O3 were deposited by pulsed laser deposition on 8% Y:ZrO2 (YSZ) substrates with (1 0 0), (1 1 0), and (1 1 1) orientation. Metallic Fe was subsequently deposited by molecular beam epitaxy. Characterization by X-ray diffraction and Rutherford backscattering spectrometry in the channeling geometry revealed a degree of epitaxial or axiotaxial orientation for Fe(2 1 1) deposited on Y2O3(1 1 0)/YSZ(1 1 0). In contrast, Fe on Y2O3(1 1 1)/YSZ(1 1 1) was fully polycrystalline, and Fe on Y2O3(1 0 0)/YSZ(1 0 0) exhibited out-of-plane texture in the [1 1 0] direction with little or no preferential in-plane orientation. Scanning transmission electron microscopy imaging of Fe(2 1 1)/Y2O3(1 1 0)/YSZ(1 1 0) revealed a strongly islanded morphology for the Fe film, with no epitaxial grains visible in the cross-sectional sample. Well-ordered Fe grains with no orientation to the underlying Y2O3 were observed. Well-ordered crystallites of Fe with both epitaxial and non-epitaxial orientations on Y2O3 are a promising model system for fundamental studies of radiation damage phenomena. This is illustrated with preliminary results of He bubble formation following implantation with a helium ion microscope. He bubble formation is shown to preferentially occur at the Fe/Y2O3 interface. (C) 2014 Elsevier B.V. All rights reserved. C1 [Kaspar, T. C.] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99354 USA. [Bowden, M. E.; Wang, C. M.; Shutthanandan, V.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA. [Overman, N. R.; van Ginhoven, R. M.; Kurtz, R. J.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99354 USA. [Wirth, B. D.] Univ Tennessee, Dept Nucl Engn, Knoxville, TN 37996 USA. RP Kaspar, TC (reprint author), Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99354 USA. EM tiffany.kaspar@pnnl.gov RI Wirth, Brian/O-4878-2015 OI Wirth, Brian/0000-0002-0395-0285 FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; US DOE Office of Biological and Environmental Research FX This work was supported by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. The experiments were carried out at the Environmental Molecular Sciences Laboratory (EMSL), a National Scientific User Facility located at Pacific Northwest National Laboratory (PNNL) and supported by the US DOE Office of Biological and Environmental Research. PNNL is a multiprogram national laboratory operated for DOE by Battelle. NR 21 TC 4 Z9 4 U1 4 U2 38 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD FEB PY 2015 VL 457 BP 352 EP 361 DI 10.1016/j.jnucmat.2014.11.046 PG 10 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA CA8KO UT WOS:000349169100046 ER PT J AU Swab, JJ Tice, J Wereszczak, AA Kraft, RH AF Swab, Jeffrey J. Tice, Jason Wereszczak, Andrew A. Kraft, Reuben H. TI Fracture Toughness of Advanced Structural Ceramics: Applying ASTM C1421 SO JOURNAL OF THE AMERICAN CERAMIC SOCIETY LA English DT Article ID TOUGHENED SILICON-NITRIDE; SUBCRITICAL CRACK-GROWTH; EDGE-PRECRACKED-BEAM; R-CURVE BEHAVIOR; SURFACE-CRACK; FLEXURE METHOD; RESISTANCE; ALUMINA; SHAPE; SIZE AB The three methods of determining the quasi-static Mode I fracture toughness (K-Ic) (surface crack in flexureSC, single-edge precracked beamPB, and chevron-notched beamVB) found in ASTM C1421 were applied to a variety of advanced ceramic materials. All three methods produced valid and comparable K-Ic values for the Al2O3, SiC, Si3N4, and SiAlON ceramics examined. However, not all methods could successfully be applied to B4C, ZrO2, and WC ceramics due to a variety of material factors. The coarse-grained microstructure of one B4C hindered the ability to observe and measure the precracks generated in the SC and PB methods while the transformation toughening in the ZrO2 prevented the formation of the SC and PB precracks and thus made it impossible to use either method on this ceramic. The high strength and elastic modulus of the WC made it impossible to achieve stable crack growth using the VB method because the specimen stored a tremendous amount of energy prior to fracture. Even though these methods have passed the rigors of the standardization process there are still some issues to be resolved when the methods are applied to certain classes of ceramics. It is recommended that, when appropriate, at least two of these methods be employed to determine the K-Ic, especially when a new or unfamiliar ceramic is being evaluated. C1 [Swab, Jeffrey J.; Tice, Jason; Kraft, Reuben H.] Army Res Lab, Aberdeen Proving Ground, MD 21005 USA. [Wereszczak, Andrew A.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Tice, Jason] Univ Maryland Baltimore Cty, Baltimore, MD 21228 USA. [Tice, Jason; Kraft, Reuben H.] Harford Community Coll, Bel Air, MD USA. RP Swab, JJ (reprint author), Army Res Lab, Aberdeen Proving Ground, MD 21005 USA. EM jeffrey.j.swab.civ@mail.mil RI Wereszczak, Andrew/I-7310-2016 OI Wereszczak, Andrew/0000-0002-8344-092X FU US Army Research Laboratory (USARL) FX Work performed while an undergraduate student at the University of Maryland Baltimore County and with support by an appointment to the Research Participation Program at the US Army Research Laboratory (USARL) administered by the Oak Ridge Institute for Science and Education through an interagency agreement between USARL and the US Department of Energy. NR 31 TC 1 Z9 1 U1 1 U2 30 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0002-7820 EI 1551-2916 J9 J AM CERAM SOC JI J. Am. Ceram. Soc. PD FEB PY 2015 VL 98 IS 2 BP 607 EP 615 DI 10.1111/jace.13293 PG 9 WC Materials Science, Ceramics SC Materials Science GA CA1HC UT WOS:000348662400040 ER PT J AU Foley, BM Brown-Shaklee, HJ Campion, MJ Medlin, DL Clem, PG Ihlefeld, JF Hopkins, PE AF Foley, Brian M. Brown-Shaklee, Harlan J. Campion, Michael J. Medlin, Douglas L. Clem, Paul G. Ihlefeld, Jon F. Hopkins, Patrick E. TI Glass-Like Thermal Conductivity of (010)-Textured Lanthanum-Doped Strontium Niobate Synthesized with Wet Chemical Deposition SO JOURNAL OF THE AMERICAN CERAMIC SOCIETY LA English DT Article ID PICOSECOND LIGHT-PULSES; THERMOELECTRIC-MATERIALS; PHONON-SCATTERING; THIN-FILMS; GRAIN-SIZE; SR2NB2O7; GENERATION; CRYSTALS; PHASE AB We have measured the cross-plane thermal conductivity () of (010)-textured, undoped, and lanthanum-doped strontium niobate (Sr2-xLaxNb2O7-) thin films via time-domain thermoreflectance. The thin films were deposited on (001)-oriented SrTiO3 substrates via the highly-scalable technique of chemical solution deposition. We find that both film thickness and lanthanum doping have little effect on , suggesting that there is a more dominant phonon scattering mechanism present in the system; namely the weak interlayer-bonding along the b-axis in the Sr2Nb2O7 parent structure. Furthermore, we compare our experimental results with two variations of the minimum-limit model for and discuss the nature of transport in material systems with weakly-bonded layers. The low cross-plane of these scalably-fabricated films is comparable to that of similarly layered niobate structures grown epitaxially. C1 [Foley, Brian M.; Hopkins, Patrick E.] Univ Virginia, Dept Mech & Aerosp Engn, Charlottesville, VA 22904 USA. [Brown-Shaklee, Harlan J.; Campion, Michael J.; Clem, Paul G.; Ihlefeld, Jon F.] Sandia Natl Labs, Elect Opt & Nano Mat Dept, Albuquerque, NM 87185 USA. [Medlin, Douglas L.] Sandia Natl Labs, Dept Mat Phys, Livermore, CA 94550 USA. RP Foley, BM (reprint author), Univ Virginia, Dept Mech & Aerosp Engn, Charlottesville, VA 22904 USA. EM bmf4su@virginia.edu FU ARCS Foundation Metro Washington Chapter; Army Research Office [W911NF-13-1-0378]; NSF EAGER program [CBET-1339436]; Laboratory Directed Research and Development (LDRD) program at Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; U.S. Department of Commerce Economic Development Administration [01-79-14214] FX B.M.F. is grateful for support from the ARCS Foundation Metro Washington Chapter. P.E.H. is appreciative for funding through the Army Research Office (W911NF-13-1-0378) and the NSF EAGER program (CBET-1339436). This work was performed in part at the Center for Atomic, Molecular, and Optical Science (CAMOS) at the University of Virginia. This work was supported, in part, by the Laboratory Directed Research and Development (LDRD) program at Sandia National Laboratories (H.B-S., M.J.C., D.L.M., P.G.C, J.F.I., P.E.H.). Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. This project was supported by Financial Assistance Award No. 01-79-14214, awarded by U.S. Department of Commerce Economic Development Administration, to the University of Virginia (P.E.H, B.M.F). The content is solely the responsibility of the authors and does not necessarily represent the official views of the U.S. Department of Commerce Economic Development Administration. NR 48 TC 2 Z9 2 U1 5 U2 34 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0002-7820 EI 1551-2916 J9 J AM CERAM SOC JI J. Am. Ceram. Soc. PD FEB PY 2015 VL 98 IS 2 BP 624 EP 628 DI 10.1111/jace.13318 PG 5 WC Materials Science, Ceramics SC Materials Science GA CA1HC UT WOS:000348662400042 ER PT J AU Zelenyuk, A Imre, D Wilson, J Zhang, ZY Wang, J Mueller, K AF Zelenyuk, Alla Imre, Dan Wilson, Jacqueline Zhang, Zhiyuan Wang, Jun Mueller, Klaus TI Airborne Single Particle Mass Spectrometers (SPLAT II & miniSPLAT) and New Software for Data Visualization and Analysis in a Geo-Spatial Context SO JOURNAL OF THE AMERICAN SOCIETY FOR MASS SPECTROMETRY LA English DT Article DE Single particle mass spectrometer; Aerosol composition; Aerosol size; Cloud condensation nuclei ID CLOUD CONDENSATION NUCLEI; INDIVIDUAL ORGANIC PARTICLES; IN-SITU CHARACTERIZATION; HIGH-DIMENSIONAL DATA; AEROSOL-PARTICLES; LASER-ABLATION; ATMOSPHERIC AEROSOLS; AERODYNAMIC LENSES; NOZZLE EXPANSIONS; SIZE AB Understanding the effect of aerosols on climate requires knowledge of the size and chemical composition of individual aerosol particles-two fundamental properties that determine an aerosol's optical properties and ability to serve as cloud condensation or ice nuclei. Here we present our aircraft-compatible single particle mass spectrometers, SPLAT II and its new, miniaturized version, miniSPLAT that measure in-situ and in real-time the size and chemical composition of individual aerosol particles with extremely high sensitivity, temporal resolution, and sizing precision on the order of a monolayer. Although miniSPLAT's size, weight, and power consumption are significantly smaller, its performance is on par with SPLAT II. Both instruments operate in dual data acquisition mode to measure, in addition to single particle size and composition, particle number concentrations, size distributions, density, and asphericity with high temporal resolution. We also present ND-Scope, our newly developed interactive visual analytics software package. ND-Scope is designed to explore and visualize the vast amount of complex, multidimensional data acquired by our single particle mass spectrometers, along with other aerosol and cloud characterization instruments on-board aircraft. We demonstrate that ND-Scope makes it possible to visualize the relationships between different observables and to view the data in a geo-spatial context, using the interactive and fully coupled Google Earth and Parallel Coordinates displays. Here we illustrate the utility of ND-Scope to visualize the spatial distribution of atmospheric particles of different compositions, and explore the relationship between individual particle compositions and their activity as cloud condensation nuclei. C1 [Zelenyuk, Alla; Wilson, Jacqueline] Pacific NW Natl Lab, Richland, WA 99354 USA. [Imre, Dan] Imre Consulting, Richland, WA 99352 USA. [Zhang, Zhiyuan; Wang, Jun; Mueller, Klaus] SUNY Stony Brook, Stony Brook, NY 11790 USA. RP Zelenyuk, A (reprint author), Pacific NW Natl Lab, Richland, WA 99354 USA. EM alla.zelenyuk-imre@pnnl.gov FU US Department of Energy (DOE) Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; US DOE Office of Biological and Environmental Research (OBER); Atmospheric Radiation Measurement (ARM); Program Climate Research Facility; Atmospheric Research Systems Program (ASR); US National Science Foundation [IIS-1117132]; MSIP (Ministry of Science, ICT and Future Planning), Korea under "IT Consilience Creative Program (ITCCP)" [NIPA-2013-H0203-13-1001]; DOE OBER Environmental Science Division; DOE OBER; Pacific Northwest National Laboratory FX This work was supported by the US Department of Energy (DOE) Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences (development of SPLAT II, miniSPLAT, and ND-Scope), the US DOE Office of Biological and Environmental Research (OBER), Atmospheric Radiation Measurement (ARM), Program Climate Research Facility, and Atmospheric Research Systems Program (ASR) (development of the aircraft deployment module and participation in ISDAC and TCAP field campaigns). Additional support was provided by the US National Science Foundation (ZZ & KM, grant IIS-1117132). Klaus Mueller was partially supported by the MSIP (Ministry of Science, ICT and Future Planning), Korea, under the "IT Consilience Creative Program (ITCCP)" (NIPA-2013-H0203-13-1001) supervised by NIPA (National IT Industry Promotion Agency) Some of the data were obtained from the ARM program archive, sponsored by the DOE OBER Environmental Science Division. A portion of the research was performed using EMSL, a DOE Office of Science User Facility sponsored by the DOE OBER and located at Pacific Northwest National Laboratory. NR 65 TC 7 Z9 7 U1 0 U2 27 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1044-0305 EI 1879-1123 J9 J AM SOC MASS SPECTR JI J. Am. Soc. Mass Spectrom. PD FEB PY 2015 VL 26 IS 2 BP 257 EP 270 DI 10.1007/s13361-014-1043-4 PG 14 WC Biochemical Research Methods; Chemistry, Analytical; Chemistry, Physical; Spectroscopy SC Biochemistry & Molecular Biology; Chemistry; Spectroscopy GA CA9EH UT WOS:000349223000008 PM 25563475 ER PT J AU Kamada, T Tsujii, H Blakely, EA Debus, J De Neve, W Durante, M Jakel, O Mayer, R Orecchia, R Potter, R Vatnitsky, S Chu, WT AF Kamada, Tadashi Tsujii, Hirohiko Blakely, Eleanor A. Debus, Juergen De Neve, Wilfried Durante, Marco Jaekel, Oliver Mayer, Ramona Orecchia, Roberto Poetter, Richard Vatnitsky, Stanislav Chu, William T. TI Carbon ion radiotherapy in Japan: an assessment of 20 years of clinical experience SO LANCET ONCOLOGY LA English DT Review ID PROTON-BEAM THERAPY; PARTICLE RADIATION-THERAPY; LOCALIZED PROSTATE-CANCER; HEAVY CHARGED-PARTICLES; 2ND MALIGNANCIES; PHOTON RADIATION; CERVICAL-CANCER; PHASE-I/II; GLIOMAS; CHEMOTHERAPY AB Charged particle therapy is generally regarded as cutting-edge technology in oncology. Many proton therapy centres are active in the USA, Europe, and Asia, but only a few centres use heavy ions, even though these ions are much more effective than x-rays owing to the special radiobiological properties of densely ionising radiation. The National Institute of Radiological Sciences (NIRS) Chiba, Japan, has been treating cancer with high-energy carbon ions since 1994. So far, more than 8000 patients have had this treatment at NIRS, and the centre thus has by far the greatest experience in carbon ion treatment worldwide. A panel of radiation oncologists, radiobiologists, and medical physicists from the USA and Europe recently completed peer review of the carbon ion therapy at NIRS. The review panel had access to the latest developments in treatment planning and beam delivery and to all updated clinical data produced at NIRS. A detailed comparison with the most advanced results obtained with x-rays or protons in Europe and the USA was then possible. In addition to those tumours for which carbon ions are known to produce excellent results, such as bone and soft-tissue sarcoma of the skull base, head and neck, and pelvis, promising data were obtained for other tumours, such as locally recurrent rectal cancer and pancreatic cancer. The most serious impediment to the worldwide spread of heavy ion therapy centres is the high initial capital cost. The 20 years of clinical experience at NIRS can help guide strategic decisions on the design and construction of new heavy ion therapy centres. C1 [Kamada, Tadashi; Tsujii, Hirohiko] Natl Inst Radiol Sci, Chiba 260, Japan. [Blakely, Eleanor A.; Chu, William T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Debus, Juergen; Jaekel, Oliver] Heidelberg Univ, Heidelberg, Germany. [Debus, Juergen; Jaekel, Oliver] Heidelberg Ion Therapy Ctr, Heidelberg, Germany. [De Neve, Wilfried] Univ Ghent, B-9000 Ghent, Belgium. [Durante, Marco] GSI Helmholtz Ctr Heavy Ion Res, Darmstadt, Germany. [Durante, Marco] Tech Univ Darmstadt, Darmstadt, Germany. [Mayer, Ramona; Vatnitsky, Stanislav] MedAustron, Wiener Neustadt, Austria. [Orecchia, Roberto] CNAO Fdn, Pavia, Italy. [Orecchia, Roberto] European Inst Oncol, Milan, Italy. [Poetter, Richard] Med Univ Vienna, Vienna, Austria. RP Durante, M (reprint author), GSI Helmholtzzentrum Schwerionenforsch, Dept Biophys, Planckstr 1, D-64291 Darmstadt, Germany. EM m.durante@gsi.de NR 51 TC 63 Z9 67 U1 8 U2 39 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 1470-2045 EI 1474-5488 J9 LANCET ONCOL JI Lancet Oncol. PD FEB PY 2015 VL 16 IS 2 BP E93 EP E100 PG 8 WC Oncology SC Oncology GA CA3YR UT WOS:000348841700016 PM 25638685 ER PT J AU Dahari, H Shteingart, S Gafanovich, I Cotler, SJ D'Amato, M Pohl, RT Weiss, G Ashkenazi, YJ Tichler, T Goldin, E Lurie, Y AF Dahari, Harel Shteingart, Shimon Gafanovich, Inna Cotler, Scott J. D'Amato, Massimo Pohl, Ralf T. Weiss, Gali Ashkenazi, Yaakov J. Tichler, Thomas Goldin, Eran Lurie, Yoav TI Sustained virological response with intravenous silibinin: individualized IFN-free therapy via real-time modelling of HCV kinetics SO LIVER INTERNATIONAL LA English DT Article DE hepatitis C; individualized therapy; interferon-free treatment; mathematical modelling; silibinin; sustained virological response; viral kinetics ID HEPATITIS-C-VIRUS; LIVER GRAFT REINFECTION; VITAMIN-D; ANTIVIRAL AGENT; INFECTION; MONOTHERAPY; SILYMARIN; TRANSPLANTATION; NONRESPONDERS; HEPATOCYTES AB Background & AimsIntravenous silibinin (SIL) is a potent antiviral agent against hepatitis C virus (HCV) genotype-1. In this proof of concept case-study we tested: (i) whether interferon-alfa (IFN)-free treatment with SIL plus ribavirin (RBV) can achieve sustained virological response (SVR); (ii) whether SIL is safe and feasible for prolonged duration of treatment and (iii) whether mathematical modelling of early on-treatment HCV kinetics can guide duration of therapy to achieve SVR. MethodsA 44year-old female HCV-(genotype-1)-infected patient who developed severe psychiatric adverse events to a previous course of pegIFN+RBV, initiated combination treatment with 1200mg/day of SIL, 1200mg/day of RBV and 6000u/day vitamin D. Blood samples were collected frequently till week 4, thereafter every 1-12weeks until the end of therapy. The standard biphasic mathematical model with time-varying SIL effectiveness was used to predict the duration of therapy to achieve SVR. ResultsBased on modelling the observed viral kinetics during the first 3weeks of treatment, SVR was predicted to be achieved within 34weeks of therapy. Provided with this information, the patient agreed to complete 34weeks of treatment. IFN-free treatment with SIL+RBV was feasible, safe and achieved SVR (week-33). ConclusionsWe report, for the first time, the use of real-time mathematical modelling of HCV kinetics to individualize duration of IFN-free therapy and to empower a patient to participate in shared decision making regarding length of treatment. SIL-based individualized therapy provides a treatment option for patients who do not respond to or cannot receive other HCV agents and should be further validated. C1 [Dahari, Harel; Cotler, Scott J.] Loyola Univ, Med Ctr, Dept Med, Program Expt & Theoret Modeling,Div Hepatol, Maywood, IL 60153 USA. [Dahari, Harel] Los Alamos Natl Lab, Los Alamos, NM USA. [Shteingart, Shimon; Goldin, Eran] Sharee Zedek Med Ctr, Inst Digest Dis, Jerusalem, Israel. [Gafanovich, Inna; Lurie, Yoav] Sharee Zedek Med Ctr, Liver Unit, Inst Digest Dis, Jerusalem, Israel. [D'Amato, Massimo; Pohl, Ralf T.] Rottapharm Madaus, Monza, Italy. [Weiss, Gali] Sharee Zedek Med Ctr, Nursing Div, Jerusalem, Israel. [Ashkenazi, Yaakov J.; Tichler, Thomas] Sharee Zedek Med Ctr, Jerusalem, Israel. RP Lurie, Y (reprint author), Sharee Zedek Med Ctr, Liver Unit, Inst Digest Dis, Jerusalem, Israel. EM yoav@szmc.org.il FU NIH [R01-AI078881, P20-GM103452]; U.S. Department of Energy [DE-AC52-06NA25396] FX NIH grants R01-AI078881 and P20-GM103452 and the U.S. Department of Energy contract DE-AC52-06NA25396. SIL was provided by Rottapharm vertical bar Madaus. NR 32 TC 7 Z9 7 U1 1 U2 5 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1478-3223 EI 1478-3231 J9 LIVER INT JI Liver Int. PD FEB PY 2015 VL 35 IS 2 BP 289 EP 294 DI 10.1111/liv.12692 PG 6 WC Gastroenterology & Hepatology SC Gastroenterology & Hepatology GA CA2BR UT WOS:000348714500001 PM 25251042 ER PT J AU Vishnivetskaya, TA Hamilton-Brehm, SD Podar, M Mosher, JJ Palumbo, AV Phelps, TJ Keller, M Elkins, JG AF Vishnivetskaya, Tatiana A. Hamilton-Brehm, Scott D. Podar, Mircea Mosher, Jennifer J. Palumbo, Anthony V. Phelps, Tommy J. Keller, Martin Elkins, James G. TI Community Analysis of Plant Biomass-Degrading Microorganisms from Obsidian Pool, Yellowstone National Park SO MICROBIAL ECOLOGY LA English DT Article DE Thermophiles; Plant biomass utilization; Bioenergy; Microbial communities; Yellowstone National Park; Extremophiles ID FREE QUANTITATIVE PROTEOMICS; CALDICELLULOSIRUPTOR-OBSIDIANSIS; SP NOV.; THERMOPHILIC DECONSTRUCTION; MICROBIAL COMMUNITIES; GLYCOSIDE HYDROLASES; HOT-SPRINGS; BACTERIUM; DIVERSITY; HYDROGEN AB The conversion of lignocellulosic biomass into biofuels can potentially be improved by employing robust microorganisms and enzymes that efficiently deconstruct plant polysaccharides at elevated temperatures. Many of the geothermal features of Yellowstone National Park (YNP) are surrounded by vegetation providing a source of allochthonic material to support heterotrophic microbial communities adapted to utilize plant biomass as a primary carbon and energy source. In this study, a well-known hot spring environment, Obsidian Pool (OBP), was examined for potential biomass-active microorganisms using cultivation-independent and enrichment techniques. Analysis of 33,684 archaeal and 43,784 bacterial quality-filtered 16S rRNA gene pyrosequences revealed that archaeal diversity in the main pool was higher than bacterial; however, in the vegetated area, overall bacterial diversity was significantly higher. Of notable interest was a flooded depression adjacent to OBP supporting a stand of Juncus tweedyi, a heat-tolerant rush commonly found growing near geothermal features in YNP. The microbial community from heated sediments surrounding the plants was enriched in members of the Firmicutes including potentially (hemi)cellulolytic bacteria from the genera Clostridium, Anaerobacter, Caloramator, Caldicellulosiruptor, and Thermoanaerobacter. Enrichment cultures containing model and real biomass substrates were established at a wide range of temperatures (55-85 A degrees C). Microbial activity was observed up to 80 A degrees C on all substrates including Avicel, xylan, switchgrass, and Populus sp. Independent of substrate, Caloramator was enriched at lower (< 65 A degrees C) temperatures while highly active cellulolytic bacteria Caldicellulosiruptor were dominant at high (> 65 A degrees C) temperatures. C1 [Vishnivetskaya, Tatiana A.; Hamilton-Brehm, Scott D.; Podar, Mircea; Mosher, Jennifer J.; Palumbo, Anthony V.; Phelps, Tommy J.; Keller, Martin; Elkins, James G.] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Biosci Div, Oak Ridge, TN 37831 USA. RP Elkins, JG (reprint author), Oak Ridge Natl Lab, BioEnergy Sci Ctr, Biosci Div, Oak Ridge, TN 37831 USA. EM elkinsjg@ornl.gov RI Elkins, James/A-6199-2011; Palumbo, Anthony/A-4764-2011; OI Elkins, James/0000-0002-8052-5688; Palumbo, Anthony/0000-0002-1102-3975; Mosher, Jennifer/0000-0001-6976-2036; Podar, Mircea/0000-0003-2776-0205; Vishnivetskaya, Tatiana/0000-0002-0660-023X FU BioEnergy Science Center (BESC), a U.S. Department of Energy Bioenergy Research Center; Office of Biological and Environmental Research in the DOE Office of Science, Oak Ridge National Laboratory; U.S. Department of Energy [DE-AC05-00OR22725] FX We thank the National Park Service and especially Christie Hendrix for coordinating and allowing sampling under permit #YELL-2008-SCI-5714. Heidi Anderson at the Yellowstone Center for Resources helped with plant species identification. We kindly thank Zamin Koo Yang for the assistance with pyrosequencing and Xiangping Yin for ICP analysis. Christopher W. Schadt provided helpful comments on the manuscript. This work was supported by the BioEnergy Science Center (BESC), which is a U.S. Department of Energy Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science, Oak Ridge National Laboratory. Oak Ridge National Laboratory is managed by UT-Battelle, LLC, for the U.S. Department of Energy under contract DE-AC05-00OR22725. NR 64 TC 2 Z9 2 U1 1 U2 25 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0095-3628 EI 1432-184X J9 MICROB ECOL JI Microb. Ecol. PD FEB PY 2015 VL 69 IS 2 BP 333 EP 345 DI 10.1007/s00248-014-0500-8 PG 13 WC Ecology; Marine & Freshwater Biology; Microbiology SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Microbiology GA CA6JD UT WOS:000349017600010 PM 25319238 ER PT J AU Be, NA Thissen, JB Fofanov, VY Allen, JE Rojas, M Golovko, G Fofanov, Y Koshinsky, H Jaing, CJ AF Be, Nicholas A. Thissen, James B. Fofanov, Viacheslav Y. Allen, Jonathan E. Rojas, Mark Golovko, George Fofanov, Yuriy Koshinsky, Heather Jaing, Crystal J. TI Metagenomic Analysis of the Airborne Environment in Urban Spaces SO MICROBIAL ECOLOGY LA English DT Article DE Aerosol microbiology; Urban air; Airborne bacteria; Metagenomics; Microbiome ID WHOLE GENOME AMPLIFICATION; BACILLUS-THURINGIENSIS; OUTDOOR AIR; COMMUNITIES; BACTERIA; DNA; MICROORGANISMS; DISPERSAL; DIVERSITY; FUNGI AB The organisms in aerosol microenvironments, especially densely populated urban areas, are relevant to maintenance of public health and detection of potential epidemic or biothreat agents. To examine aerosolized microorganisms in this environment, we performed sequencing on the material from an urban aerosol surveillance program. Whole metagenome sequencing was applied to DNA extracted from air filters obtained during periods from each of the four seasons. The composition of bacteria, plants, fungi, invertebrates, and viruses demonstrated distinct temporal shifts. Bacillus thuringiensis serovar kurstaki was detected in samples known to be exposed to aerosolized spores, illustrating the potential utility of this approach for identification of intentionally introduced microbial agents. Together, these data demonstrate the temporally dependent metagenomic complexity of urban aerosols and the potential of genomic analytical techniques for biosurveillance and monitoring of threats to public health. C1 [Be, Nicholas A.; Thissen, James B.; Jaing, Crystal J.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94551 USA. [Fofanov, Viacheslav Y.; Koshinsky, Heather] Eureka Genom, Hercules, CA USA. [Allen, Jonathan E.] Lawrence Livermore Natl Lab, Computat Global Secur Directorates, Livermore, CA 94551 USA. [Rojas, Mark; Golovko, George; Fofanov, Yuriy] Univ Texas Med Branch, Sealy Ctr Struct Biol & Mol Biophys, Galveston, TX 77555 USA. RP Jaing, CJ (reprint author), Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94551 USA. EM jaing2@llnl.gov FU Department of Homeland Security; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was funded by the Department of Homeland Security and performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. Maria Shin from Eureka Genomics is acknowledged for preparing sequencing libraries and generating the sequence data. Marilyn Ramsey, Anne Marie Erler, Gloria Murphy, Michael Dillon, Staci Kane, and Thomas Bunt from the LLNL environmental monitoring laboratory are acknowledged for their contribution toward collection and preparation of samples for this study. NR 38 TC 5 Z9 5 U1 16 U2 71 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0095-3628 EI 1432-184X J9 MICROB ECOL JI Microb. Ecol. PD FEB PY 2015 VL 69 IS 2 BP 346 EP 355 DI 10.1007/s00248-014-0517-z PG 10 WC Ecology; Marine & Freshwater Biology; Microbiology SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Microbiology GA CA6JD UT WOS:000349017600011 PM 25351142 ER PT J AU Khan, AI Chatterjee, K Wang, B Drapcho, S You, L Serrao, C Bakaul, SR Ramesh, R Salahuddin, S AF Khan, Asif Islam Chatterjee, Korok Wang, Brian Drapcho, Steven You, Long Serrao, Claudy Bakaul, Saidur Rahman Ramesh, Ramamoorthy Salahuddin, Sayeef TI Negative capacitance in a ferroelectric capacitor SO NATURE MATERIALS LA English DT Article ID 2-DIMENSIONAL ELECTRON; ROOM-TEMPERATURE; FILMS; POLARIZATION; TRANSISTORS; SILICON; DEVICES; BATIO3; TIME AB The Boltzmann distribution of electrons poses a fundamental barrier to lowering energy dissipation in conventional electronics, often termed as Boltzmann Tyranny(1-5). Negative capacitance in ferroelectric materials, which stems from the stored energy of a phase transition, could provide a solution, but a direct measurement of negative capacitance has so far been elusive(1-3). Here, we report the observation of negative capacitance in a thin, epitaxial ferroelectric film. When a voltage pulse is applied, the voltage across the ferroelectric capacitor is found to be decreasing with time-in exactly the opposite direction to which voltage for a regular capacitor should change. Analysis of this 'inductance'-like behaviour from a capacitor presents an unprecedented insight into the intrinsic energy profile of the ferroelectric material and could pave the way for completely new applications. C1 [Khan, Asif Islam; Chatterjee, Korok; Wang, Brian; You, Long; Serrao, Claudy; Bakaul, Saidur Rahman; Salahuddin, Sayeef] Univ Calif Berkeley, Dept Elect Engn & Comp Engn, Berkeley, CA 94720 USA. [Drapcho, Steven; Ramesh, Ramamoorthy] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Ramesh, Ramamoorthy] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94270 USA. [Ramesh, Ramamoorthy; Salahuddin, Sayeef] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94270 USA. RP Salahuddin, S (reprint author), Univ Calif Berkeley, Dept Elect Engn & Comp Engn, Berkeley, CA 94720 USA. EM sayeef@berkeley.edu OI , claudy/0000-0003-4737-0693 FU Office of Naval Research (ONR); Center for Low Energy Systems Technology (LEAST), one of the six SRC STARnet Centers - MARCO; DARPA; NSF E3S Center at Berkeley FX This work was supported in part by the Office of Naval Research (ONR), the Center for Low Energy Systems Technology (LEAST), one of the six SRC STARnet Centers, sponsored by MARCO and DARPA and the NSF E3S Center at Berkeley. A. I. K. acknowledges the Qualcomm Innovation Fellowship 2012-2013. NR 28 TC 56 Z9 56 U1 23 U2 186 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1476-1122 EI 1476-4660 J9 NAT MATER JI Nat. Mater. PD FEB PY 2015 VL 14 IS 2 BP 182 EP 186 DI 10.1038/NMAT4148 PG 5 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA CA0IE UT WOS:000348600200015 PM 25502099 ER PT J AU Kwon, SG Krylova, G Phillips, PJ Klie, RF Chattopadhyay, S Shibata, T Bunel, EE Liu, YZ Prakapenka, VB Lee, B Shevchenko, EV AF Kwon, Soon Gu Krylova, Galyna Phillips, Patrick J. Klie, Robert F. Chattopadhyay, Soma Shibata, Tomohiro Bunel, Emilio E. Liu, Yuzi Prakapenka, Vitali B. Lee, Byeongdu Shevchenko, Elena V. TI Heterogeneous nucleation and shape transformation of multicomponent metallic nanostructures SO NATURE MATERIALS LA English DT Article ID SEEDED GROWTH; BIMETALLIC NANODENDRITES; NANOROD HETEROSTRUCTURES; COLLOIDAL NANOCRYSTALS; NANOPARTICLES; HYDROGENATION; STRAIN; SCALE; RODS; SIZE AB To be able to control the functions of engineered multicomponent nanomaterials, a detailed understanding of heterogeneous nucleation at the nanoscale is essential. Here, by using in situ synchrotron X-ray scattering, we show that in the heterogeneous nucleation and growth of Au on Pt or Pt-alloy seeds the heteroepitaxial growth of the Au shell exerts high stress (similar to 2 GPa) on the seed by forming a core/shell structure in the early stage of the reaction. The development of lattice strain and subsequent strain relaxation, which we show using atomic-resolution transmission electron microscopy to occur through the slip of {111} layers, induces morphological changes from a core/shell to a dumbbell structure, and governs the nucleation and growth kinetics. We also propose a thermodynamic model for the nucleation and growth of dumbbell metallic heteronanostructures. C1 [Kwon, Soon Gu; Krylova, Galyna; Liu, Yuzi; Shevchenko, Elena V.] Argonne Natl Lab, Nanosci & Technol Div, Argonne, IL 60439 USA. [Phillips, Patrick J.; Klie, Robert F.] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. [Chattopadhyay, Soma; Shibata, Tomohiro] Argonne Natl Lab, MRCAT, CSRRI IIT, Argonne, IL 60439 USA. [Chattopadhyay, Soma; Shibata, Tomohiro] IIT, Adv Mat Grp, Dept Phys, Chicago, IL 60616 USA. [Bunel, Emilio E.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Prakapenka, Vitali B.] Univ Chicago, Ctr Adv Radiat Sources, Argonne, IL 60439 USA. [Lee, Byeongdu] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Lee, B (reprint author), Argonne Natl Lab, Adv Photon Source, 9700 S Cass Ave, Argonne, IL 60439 USA. EM blee@aps.anl.gov; eshevchenko@anl.gov RI Kwon, Soon Gu/E-3123-2015; Liu, Yuzi/C-6849-2011; OI Lee, Byeongdu/0000-0003-2514-8805 FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; MRCAT host institutions; National Science Foundation [DMR-0959470]; IC Research Resources Center; National Science Foundation-Earth Sciences [EAR-0622171]; Department of Energy-Geosciences [DE-FG02-94ER14466] FX Use of the Center for Nanoscale Materials and Advanced Photon Source was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. MRCAT is funded by MRCAT host institutions. The authors thank C. Marshall for fruitful discussion and help in tests of catalytic activity. S. C. and T. S. would like to thank V. Zyryanov for help with experiments and C. Segre for beam-time allocation. P.J.P. and R. F. K. acknowledge support from the National Science Foundation (DMR-0959470) for the acquisition of the UIC JEOL JEMARM200CF. Support from the UIC Research Resources Center is also acknowledged. The work at GeoSoilEnviroCARS was supported by the National Science Foundation-Earth Sciences (EAR-0622171) and Department of Energy-Geosciences (DE-FG02-94ER14466). NR 49 TC 30 Z9 30 U1 18 U2 165 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1476-1122 EI 1476-4660 J9 NAT MATER JI Nat. Mater. PD FEB PY 2015 VL 14 IS 2 BP 215 EP 223 DI 10.1038/NMAT4115 PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA CA0IE UT WOS:000348600200022 PM 25362354 ER PT J AU Bunkoczi, G Mccoy, AJ Echols, N Grosse-Kunstleve, RW Adams, PD Holton, JM Read, RJ Terwilliger, TC AF Bunkoczi, Gabor Mccoy, Airlie J. Echols, Nathaniel Grosse-Kunstleve, Ralf W. Adams, Paul D. Holton, James M. Read, Randy J. Terwilliger, Thomas C. TI Macromolecular X-ray structure determination using weak, single-wavelength anomalous data SO NATURE METHODS LA English DT Article ID CRYSTAL-STRUCTURE; MAXIMUM-LIKELIHOOD; DENSITY MODIFICATION; RESOLUTION REVEALS; ATOMIC MODELS; PROTEIN; DIFFRACTION; REFINEMENT; SULFUR; PHENIX AB We describe a likelihood-based method for determining the substructure of anomalously scattering atoms in macromolecular crystals that allows successful structure determination by single-wavelength anomalous diffraction (SAD) X-ray analysis with weak anomalous signal. With the use of partial models and electron density maps in searches for anomalously scattering atoms, testing of alternative values of parameters and parallelized automated model-building, this method has the potential to extend the applicability of the SAD method in challenging cases. C1 [Bunkoczi, Gabor; Mccoy, Airlie J.; Read, Randy J.] Univ Cambridge, Cambridge Inst Med Res, Dept Haematol, Cambridge, England. [Echols, Nathaniel; Adams, Paul D.; Holton, James M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Holton, James M.] Univ Calif San Francisco, Dept Biochem & Biophys, San Francisco, CA 94143 USA. [Terwilliger, Thomas C.] Los Alamos Natl Lab, Los Alamos, NM USA. RP Read, RJ (reprint author), Univ Cambridge, Cambridge Inst Med Res, Dept Haematol, Cambridge, England. EM rjr27@cam.ac.uk; terwilliger@lanl.gov RI Terwilliger, Thomas/K-4109-2012; Read, Randy/L-1418-2013; Adams, Paul/A-1977-2013 OI Terwilliger, Thomas/0000-0001-6384-0320; Read, Randy/0000-0001-8273-0047; Adams, Paul/0000-0001-9333-8219 FU US National Institutes of Health [P01GM063210, GM073210]; Wellcome Trust (Principal Research Fellowship) [082961/Z/07/Z]; US Department of Energy [DE-AC02-05CH11231] FX We thank Q. Liu, W. Henderickson and colleagues for generously providing the CysZ sulfur SAD data sets. Support received from the US National Institutes of Health (grant P01GM063210 to P.D.A., T.C.T. and R.J.R. and grant GM073210 to J.M.H.) and the Wellcome Trust (Principal Research Fellowship to R.J.R., grant 082961/Z/07/Z) is gratefully acknowledged. This work was partially supported by the US Department of Energy under contract DE-AC02-05CH11231. NR 47 TC 10 Z9 10 U1 1 U2 11 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1548-7091 EI 1548-7105 J9 NAT METHODS JI Nat. Methods PD FEB PY 2015 VL 12 IS 2 BP 127 EP U157 DI 10.1038/nmeth.3212 PG 9 WC Biochemical Research Methods SC Biochemistry & Molecular Biology GA CA4GL UT WOS:000348862500013 PM 25532136 ER PT J AU Hartmann, H Adams, HD Anderegg, WRL Jansen, S Zeppel, MJB AF Hartmann, Henrik Adams, Henry D. Anderegg, William R. L. Jansen, Steven Zeppel, Melanie J. B. TI Research frontiers in drought-induced tree mortality: crossing scales and disciplines SO NEW PHYTOLOGIST LA English DT Editorial Material DE biotic agents; carbon availability; desiccation; global warming; interdisciplinary; plant-water relations; remote sensing; stress ID FOREST DIE-OFF; CARBOHYDRATE DYNAMICS; CARBON METABOLISM; SEEDLINGS; TEMPERATURE; MECHANISMS; STRESS; STRATEGIES; STARVATION; SAPLINGS C1 [Hartmann, Henrik] Max Planck Inst Biogeochem, Dept Biogeochem Proc, D-07745 Jena, Germany. [Adams, Henry D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Anderegg, William R. L.] Princeton Univ, Princeton Environm Inst, Princeton, NJ 08544 USA. [Jansen, Steven] Univ Ulm, Inst Systemat Bot & Ecol, D-89081 Ulm, Germany. [Zeppel, Melanie J. B.] Macquarie Univ, Dept Biol Sci, Sydney, NSW 2109, Australia. RP Hartmann, H (reprint author), Max Planck Inst Biogeochem, Dept Biogeochem Proc, Hans Knoll Str 10, D-07745 Jena, Germany. EM hhart@bgc-jena.mpg.de RI Hartmann, Henrik/C-5632-2015; Jansen, Steven/A-9868-2012; OI Hartmann, Henrik/0000-0002-9926-5484; Jansen, Steven/0000-0002-4476-5334; Zeppel, Melanie/0000-0002-5510-0936 NR 39 TC 32 Z9 32 U1 4 U2 82 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0028-646X EI 1469-8137 J9 NEW PHYTOL JI New Phytol. PD FEB PY 2015 VL 205 IS 3 BP 965 EP 969 DI 10.1111/nph.13246 PG 5 WC Plant Sciences SC Plant Sciences GA CA2HX UT WOS:000348730600006 PM 25580653 ER PT J AU Field, KG Remec, I Le Pape, Y AF Field, K. G. Remec, I. Le Pape, Y. TI Radiation effects in concrete for nuclear power plants - Part I: Quantification of radiation exposure and radiation effects SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article ID IRRADIATED CRYSTALLINE QUARTZ; HIGH-STRENGTH CONCRETE; HIGH-TEMPERATURE; GAMMA-RADIATION; AMORPHIZATION; CERAMICS; DAMAGE; SCATTERING; SILICA AB A large fraction of light water reactor (LWR) construction utilizes concrete, including safety-related structures such as the biological shielding and containment building. Concrete is an inherently complex material, with the properties of concrete structures changing over their lifetime due to the intrinsic nature of concrete and influences from local environment. As concrete structures within LWRs age, the total neutron fluence exposure of the components, in particular the biological shield, can increase to levels where deleterious effects are introduced as a result of neutron irradiation. This work summarizes the current state of the art on irradiated concrete, including a review of the current literature and estimates the total neutron fluence expected in biological shields in typical LWR configurations. It was found a first-order mechanism for loss of mechanical properties of irradiated concrete is due to radiation-induced swelling of aggregates, which leads to volumetric expansion of the concrete. This phenomena is estimated to occur near the end of life of biological shield components in LWRs based on calculations of estimated peak neutron fluence in the shield after 80 years of operation. (C) 2014 Elsevier B.V. All rights reserved. C1 [Field, K. G.; Remec, I.; Le Pape, Y.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Field, KG (reprint author), Oak Ridge Natl Lab, One Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM fieldkg@ornl.gov FU U.S. Department of Energy [DE-AC05-000R22725]; Department of Energy Light Water Reactor Sustainability Program FX The authors would like to thank Dr. D. Naus, Dr. T.M. Rosseel and Dr. J.T. Busby for their thoughtful discussions on the presented topics. This research is sponsored by the Department of Energy Light Water Reactor Sustainability Program. This manuscript has been authored by the Oak Ridge National Laboratory, managed by UT-Battelle LLC under Contract No. DE-AC05-000R22725 with the U.S. Department of Energy. The publisher, by accepting the article for publication, acknowledges that the U.S. Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for U.S. Government purposes. NR 98 TC 13 Z9 13 U1 3 U2 31 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 EI 1872-759X J9 NUCL ENG DES JI Nucl. Eng. Des. PD FEB PY 2015 VL 282 BP 126 EP 143 DI 10.1016/j.nucengdes.2014.10.003 PG 18 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CA5PY UT WOS:000348961500013 ER PT J AU Le Pape, Y Field, KG Remec, I AF Le Pape, Y. Field, K. G. Remec, I. TI Radiation effects in concrete for nuclear power plants, Part II: Perspective from micromechanical modeling SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article ID HYDRATING CEMENT PASTE; THERMAL-EXPANSION; AUTOGENOUS-SHRINKAGE; GAMMA-IRRADIATION; ELASTIC-MODULI; QUARTZ; AMORPHIZATION; INCLUSION; ROCK AB The need to understand and characterize the effects of neutron irradiation on concrete has become urgent because of the possible extension of service life of many nuclear power generating stations. Current knowledge is primarily based on a collection of data obtained in test reactors. These data are inherently difficult to interpret because materials and testing conditions are inconsistent. A micromechanical approach based on the Hashin composite sphere model is presented to derive a first-order separation of the effects of radiation on cement paste and aggregate, and, also, on their interaction. Although the scarcity of available data limits the validation of the model, it appears that, without negating a possible gamma-ray induced effect, the neutron-induced damage and swelling of aggregate plays a predominant role on the overall concrete expansion and the damage of the cement paste. The radiation-induced volumetric expansion (RIVE) effects can also be aided by temperature elevation and shrinkage in the cement paste. (C) 2014 Elsevier B.V. All rights reserved. C1 [Le Pape, Y.; Field, K. G.; Remec, I.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Le Pape, Y (reprint author), Oak Ridge Natl Lab, One Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM lepapeym@ornl.gov OI Le Pape, Yann/0000-0001-5410-6546 FU DOE; U.S. Department of Energy [DE-AC05-000R22725] FX The authors would like to thank Pr. Ippei Maruyama, Dr. D. Naus, Dr. T.M. Rosseel and Dr. J.T. Busby for their thoughtful discussions on the presented topics. This research is sponsored by the DOE Light Water Reactor Sustainability Program. This manuscript has been authored by the Oak Ridge National Laboratory, managed by UT-Battelle LLC under Contract No. DE-AC05-000R22725 with the U.S. Department of Energy. The publisher, by accepting the article for publication, acknowledges that the U.S. Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for U.S. Government purposes. NR 67 TC 12 Z9 12 U1 2 U2 13 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 EI 1872-759X J9 NUCL ENG DES JI Nucl. Eng. Des. PD FEB PY 2015 VL 282 BP 144 EP 157 DI 10.1016/j.nucengdes.2014.10.014 PG 14 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CA5PY UT WOS:000348961500014 ER PT J AU Cai, HS Fu, GY AF Cai, Huishan Fu, Guoyong TI Influence of resistive internal kink on runaway current profile SO NUCLEAR FUSION LA English DT Letter DE runaway current; resistive kink; disruption ID DISRUPTIONS AB An extended magnetohydrodynamic model including the effect of runaway current is developed and implemented in the M3D code. Based on this model, a simulation has been carried out to investigate the linear stability and the nonlinear evolution of the n = 1 resistive kink mode in the presence of runaway current. It is found that sawteeth oscillation is suppressed in a runaway plasma. The nonlinear evolution of the n = 1 mode only leads to a single sawtooth crash before reaching a new steady state axi-symmetric equilibrium with flattened current profile in the plasma core and q(0) > 1. C1 [Cai, Huishan] Univ Sci & Technol China, Dept Modern Phys, CAS Key Lab Geospace Environm, Hefei 230026, Peoples R China. [Fu, Guoyong] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. RP Cai, HS (reprint author), Univ Sci & Technol China, Dept Modern Phys, CAS Key Lab Geospace Environm, Hefei 230026, Peoples R China. EM hscai@mail.ustc.edu.cn FU US Department of Energy [DE-AC02-09CH11466]; National Magnetic Confinement Fusion Science Program; National Science Foundation of China [2014GB106004, 2013GB111000, 11375189, 11075161, 11275260] FX One of the authors (GYF) gratefully thank Drs Henry Strauss, Per Helander and Richard Hawryluk for stimulating discussions on the runaway problem. In particular he thanks Dr Strauss for suggesting this work. This work is supported by US Department of Energy under DE-AC02-09CH11466, National Magnetic Confinement Fusion Science Program and National Science Foundation of China under Grants Nos 2014GB106004, 2013GB111000, 11375189, 11075161 and 11275260. The simulations were carried out using the supercomputers at NERSC. NR 14 TC 3 Z9 4 U1 2 U2 20 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD FEB PY 2015 VL 55 IS 2 AR 022001 DI 10.1088/0029-5515/55/2/022001 PG 5 WC Physics, Fluids & Plasmas SC Physics GA CA3ZE UT WOS:000348843100001 ER PT J AU Ding, R Pitts, RA Borodin, D Carpentier, S Ding, F Gong, XZ Guo, HY Kirschner, A Kocan, M Li, JG Luo, GN Mao, HM Qian, JP Stangeby, PC Wampler, WR Wang, HQ Wang, WZ AF Ding, R. Pitts, R. A. Borodin, D. Carpentier, S. Ding, F. Gong, X. Z. Guo, H. Y. Kirschner, A. Kocan, M. Li, J. G. Luo, G. -N. Mao, H. M. Qian, J. P. Stangeby, P. C. Wampler, W. R. Wang, H. Q. Wang, W. Z. TI Material migration studies with an ITER first wall panel proxy on EAST SO NUCLEAR FUSION LA English DT Article DE material migration; erosion and deposition; ITER first wall ID CHEMICAL EROSION; CARBON; JET; DEPOSITION; DEUTERIUM; PHYSICS AB The ITER beryllium (Be) first wall (FW) panels are shaped to protect leading edges between neighbouring panels arising from assembly tolerances. This departure from a perfectly cylindrical surface automatically leads to magnetically shadowed regions where eroded Be can be re-deposited, together with co-deposition of tritium fuel. To provide a benchmark for a series of erosion/re-deposition simulation studies performed for the ITER FW panels, dedicated experiments have been performed on the EAST tokamak using a specially designed, instrumented test limiter acting as a proxy for the FW panel geometry. Carbon coated molybdenum plates forming the limiter front surface were exposed to the outer midplane boundary plasma of helium discharges using the new Material and Plasma Evaluation System (MAPES). Net erosion and deposition patterns are estimated using ion beam analysis to measure the carbon layer thickness variation across the surface after exposure. The highest erosion of about 0.8 mu m is found near the midplane, where the surface is closest to the plasma separatrix. No net deposition above the measurement detection limit was found on the proxy wall element, even in shadowed regions. The measured 2D surface erosion distribution has been modelled with the 3D Monte Carlo code ERO, using the local plasma parameter measurements together with a diffusive transport assumption. Excellent agreement between the experimentally observed net erosion and the modelled erosion profile has been obtained. C1 [Ding, R.; Ding, F.; Gong, X. Z.; Guo, H. Y.; Li, J. G.; Luo, G. -N.; Mao, H. M.; Qian, J. P.; Wang, H. Q.; Wang, W. Z.] Chinese Acad Sci, Inst Plasma Phys, Hefei 230031, Anhui, Peoples R China. [Pitts, R. A.; Carpentier, S.; Kocan, M.] ITER Org, F-613067 St Paul Les Durance, France. [Borodin, D.; Kirschner, A.] Forschungszentrum Julich, Assoc EURATOM FZJ, Trilateral Euregio Cluster, Inst Energy & Climate Research Plasma Phys, D-52425 Julich, Germany. [Wampler, W. R.] Sandia Natl Labs, Radiation Solid Interact Dept 1111, Albuquerque, NM 87185 USA. [Stangeby, P. C.] Univ Toronto, Inst Aerosp Studies, Toronto, ON M3H 5T6, Canada. RP Ding, R (reprint author), Chinese Acad Sci, Inst Plasma Phys, POB 1126, Hefei 230031, Anhui, Peoples R China. EM rding@ipp.ac.cn OI Kirschner, Andreas/0000-0002-3213-3225 FU National Magnetic Confinement Fusion Science Programme of China [2013GB107004, 2013GB105001, 2013GB105002, 2013GB105003]; National Natural Science Foundation of China [11375010, 11005125, 11205198]; Sino-German Center for Research Promotion [GZ769]; US Department of Energy Office of Science Fusion Energy Sciences Program [DE-AC04-94AL85000] FX The views and opinions expressed herein do not necessarily reflect those of the ITER Organization. This work has been supported by the National Magnetic Confinement Fusion Science Programme of China under contract Nos 2013GB107004, 2013GB105001, 2013GB105002, 2013GB105003, the National Natural Science Foundation of China under Contract Nos 11375010, 11005125, 11205198, and the Sino-German Center for Research Promotion under Contract No. GZ769. Sandia National Laboratories is a multi-programme laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy Office of Science Fusion Energy Sciences Program under contract DE-AC04-94AL85000. NR 21 TC 2 Z9 2 U1 4 U2 24 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD FEB PY 2015 VL 55 IS 2 AR 023013 DI 10.1088/0029-5515/55/2/023013 PG 10 WC Physics, Fluids & Plasmas SC Physics GA CA3ZE UT WOS:000348843100014 ER PT J AU Jackson, GL Luce, TC Solomon, WM Turco, F Buttery, RJ Hyatt, AW deGrassie, JS Doyle, EJ Ferron, JR La Haye, RJ Politzer, PA AF Jackson, G. L. Luce, T. C. Solomon, W. M. Turco, F. Buttery, R. J. Hyatt, A. W. deGrassie, J. S. Doyle, E. J. Ferron, J. R. La Haye, R. J. Politzer, P. A. TI Long-pulse stability limits of the ITER baseline scenario SO NUCLEAR FUSION LA English DT Article DE tokamaks; spherical tokamaks; plasma heating by microwaves; ECR; ICR; ICP; helicons; MHD modes; kinetic modes ID TEARING MODES; TOKAMAK; COLLISIONALITY; PLASMAS AB DIII-D has made significant progress in developing the techniques required to operate ITER, and in understanding their impact on performance when integrated into operational scenarios at ITER-relevant parameters. Long duration plasmas, stable to m/n = 2/1 tearing modes, with an ITER-similar shape and I-p/aB(T), have been demonstrated in DIII-D, that evolve to stationary conditions. The operating region most likely to reach stable conditions has normalized pressure, beta(N) approximate to 1.9-2.1 (compared to the ITER baseline design of 1.6-1.8), and a Greenwald normalized density fraction, f(GW) 0.42-0.70 (the ITER design is f(GW) approximate to 0.8). The evolution of the current profile, using internal inductance (l(i)) as an indicator, is found to produce a smaller fraction of stable pulses when li is increased above approximate to 1.1 at the beginning of beta(N) flattop. Stable discharges with co-neutral beam injection are generally accompanied with a benign n = 2 magnetohydrodynamic mode. However if this mode exceeds approximate to 10 G, the onset of a m/n = 2/1 tearing mode occurs with a loss of confinement. In addition, stable operation with low applied external torque, at or below the extrapolated value expected for ITER has also been demonstrated. With electron cyclotron injection, the operating region of stable discharges has been further extended at ITER equivalent levels of torque and to edge-localized mode (ELM) free discharges at higher torque but with the addition of an n = 3 magnetic perturbation from the DIII-D internal coil set. The characterization of the ITER baseline scenario evolution for long pulse duration, extension to more ITER-relevant values of torque and electron heating, and suppression of ELMs have significantly advanced the physics basis of this scenario, although significant effort remains in the simultaneous integration of all these requirements. C1 [Jackson, G. L.; Luce, T. C.; Buttery, R. J.; Hyatt, A. W.; deGrassie, J. S.; Ferron, J. R.; La Haye, R. J.; Politzer, P. A.] Gen Atom Co, San Diego, CA 92186 USA. [Solomon, W. M.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Turco, F.] Columbia Univ, New York, NY 10027 USA. [Doyle, E. J.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. RP Jackson, GL (reprint author), Gen Atom Co, POB 85608, San Diego, CA 92186 USA. EM jackson@fusion.gat.com OI Solomon, Wayne/0000-0002-0902-9876 FU US Department of Energy [DE-FC02-04ER54698, DE-AC02-09CH11466, DE-FG02-04ER54761, DE-FG02-08ER54984] FX This work was supported by the US Department of Energy under DE-FC02-04ER54698, DE-AC02-09CH11466, DE-FG02-04ER54761 and DE-FG02-08ER54984. DIII-D data shown in this paper can be obtained in digital format by following the links at https://fusion.gat.com/global/D3D_DMP. NR 25 TC 2 Z9 2 U1 1 U2 13 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD FEB PY 2015 VL 55 IS 2 AR 023004 DI 10.1088/0029-5515/55/2/023004 PG 8 WC Physics, Fluids & Plasmas SC Physics GA CA3ZE UT WOS:000348843100005 ER PT J AU Klimek, I Cecconello, M Gorelenkova, M Keeling, D Meakins, A Jones, O Akers, R Lupelli, I Turnyanskiy, M Ericsson, G AF Klimek, I. Cecconello, M. Gorelenkova, M. Keeling, D. Meakins, A. Jones, O. Akers, R. Lupelli, I. Turnyanskiy, M. Ericsson, G. CA MAST Team TI TRANSP modelling of total and local neutron emission on MAST SO NUCLEAR FUSION LA English DT Article DE neutron measurements; TRANSP/NUBEAM simulations; fishbone ID SPHERICAL TOKAMAK AB The results of TRANSP simulations of neutron count rate profiles measured by a collimated neutron flux monitor-neutron camera (NC)-for different plasma scenarios on MAST are reported. In addition, the effect of various plasma parameters on neutron emission is studied by means of TRANSP simulation. The fast ion redistribution and losses due to fishbone modes, which belong to a wider category of energetic particle modes, are observed by the NC and modelled in TRANSP. C1 [Klimek, I.; Cecconello, M.; Ericsson, G.] Uppsala Univ, Dept Phys & Astron, SE-75120 Uppsala, Sweden. [Gorelenkova, M.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Keeling, D.; Meakins, A.; Jones, O.; Akers, R.; Lupelli, I.; MAST Team] CCFE, Culham Sci Ctr, Abingdon OX14 3DB, Oxon, England. [Jones, O.] Univ Durham, Dept Phys, Durham DH1 3LE, England. [Turnyanskiy, M.] EFDA CSU Garching, ITER Phys Dept, D-85748 Garching, Germany. RP Klimek, I (reprint author), Uppsala Univ, Dept Phys & Astron, SE-75120 Uppsala, Sweden. EM iwona.klimek@physics.uu.se OI Lupelli, Ivan/0000-0001-5053-1502 FU European Union's Horizon research and innovation programme [633053]; Swedish Research Council; RCUK Energy Programme [EP/I501045] FX This project has received funding from the European Union's Horizon 2020 research and innovation programme under grant agreement number 633053, from the Swedish Research Council and from the RCUK Energy Programme [grant number EP/I501045]. The views and opinions expressed herein do not necessarily reflect those of the European Commission. NR 31 TC 4 Z9 4 U1 0 U2 11 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD FEB PY 2015 VL 55 IS 2 AR 023003 DI 10.1088/0029-5515/55/2/023003 PG 12 WC Physics, Fluids & Plasmas SC Physics GA CA3ZE UT WOS:000348843100004 ER PT J AU Lazerson, SA AF Lazerson, S. A. CA DIII-D Team TI Three-dimensional equilibrium reconstruction on the DIII-D device SO NUCLEAR FUSION LA English DT Article DE fusion; reconstruction; equilibrium; tokamak; diagnostics; magnetics ID D TOKAMAK; MAGNETIC-FIELDS; SYSTEM; STELLARATORS; PARAMETERS; STABILITY; PLASMAS AB The presence of toroidal variation in diagnostic measurements indicates that the two-dimensional (2D) symmetry of tokamak equilibria can be violated when resonant magnetic perturbations (RMPs) are applied to suppress edge localized modes. While tokamak control is still possible with a 2D model, questions arise regarding the applicability of 2D equilibria when performing detailed analysis. In particular, questions regarding edge physics would benefit from equilibrium calculations which are consistent with measurements indicating toroidal variations. The ability to fit three-dimensional (3D) equilibria to diagnostic measurements has long been a challenge for stellarators, non-axisymmetric devices with an inherently 3D field structure. The STELLOPT code provides a solution to such a challenge by fitting 3D VMEC equilibria to magnetic, Thomson, motional Stark effect (MSE) and charge-exchange diagnostics. The plasma of the DIII-D tokamak with applied n = 3 RMP is reconstructed with STELLOPT (shot number 142603). The reconstruction is governed by fit to magnetic diagnostics, measured vacuum coil currents, Thomson scattering, charge-exchange spectroscopy and MSE polarimetry. The reconstructed equilibria possess features where pressure gradients become vanishingly small at low-order rationals. Such features can be associated with the applied RMP spectrum, indicating mode penetration for this shot. Boundary displacements on the order of 0.5 cm peak-to-peak were present. This suggests that while the 3D effect was small relative to the plasma minor radius, resonant mode penetration occurred, indicating the ability of 3D reconstructions to resolve small key features in the plasma. C1 [Lazerson, S. A.; DIII-D Team] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. RP Lazerson, SA (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. EM lazerson@pppl.gov RI Lazerson, Samuel/E-4816-2014 OI Lazerson, Samuel/0000-0001-8002-0121 FU US Department of Energy [09CH11466] FX The author would thank D. Gates, A. Turnbull, R. Nazikian, T. Strait and N. Ferraro for their valuable discussions on equilibrium and the DIII-D device. The author would also like to thank S. Hirshman for access to the VMEC code. A special thanks to all the diagnosticians at DIII-D for their help in sorting out the locations of all the diagnostics. This manuscript has been authored by Princeton University under Contract Number DE-AC02-09CH11466 with the US Department of Energy. The publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 32 TC 5 Z9 5 U1 1 U2 14 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD FEB PY 2015 VL 55 IS 2 AR 023009 DI 10.1088/0029-5515/55/2/023009 PG 14 WC Physics, Fluids & Plasmas SC Physics GA CA3ZE UT WOS:000348843100010 ER PT J AU Mazzitelli, G Hirooka, Y Hu, JS Mirnov, SV Nygren, R Shimada, M Ono, M Tabares, FL AF Mazzitelli, G. Hirooka, Y. Hu, J. S. Mirnov, S. V. Nygren, R. Shimada, M. Ono, M. Tabares, F. L. TI Conference Report on the 3rd International Symposium on Lithium Application for Fusion Devices SO NUCLEAR FUSION LA English DT Article DE conference report; lithium; liquid metal AB The third International Symposium on Lithium Application for Fusion Device (ISLA-2013) was held on 9-11 October 2013 at ENEA Frascati Centre with growing participation and interest from the community working on more general aspect of liquid metal research for fusion energy development. ISLA-2013 has been confirmed to be the largest and the most important meeting dedicated to liquid metal application for the magnetic fusion research. Overall, 45 presentation plus 5 posters were given, representing 28 institutions from 11 countries. The latest experimental results from nine magnetic fusion devices were presented in 16 presentations from NSTX (PPPL, USA), FTU (ENEA, Italy), T-11M (Trinity, RF), T-10 (Kurchatov Institute, RF), TJ-II (CIEMAT, Spain), EAST(ASIPP, China), HT-7 (ASIPP, China), RFX (Padova, Italy), KTM (NNC RK, Kazakhstan). Sessions were devoted to the following: (I) lithium in magnetic confinement experiments (facility overviews), (II) lithium in magnetic confinement experiments (topical issues), (III) special session on liquid lithium technology, (IV) lithium laboratory test stands, (V) Lithium theory/modelling/comments, (VI) innovative lithium applications and (VII) special Session on lithium-safety and lithium handling. There was a wide participation from the fusion technology communities, including IFMIF and TBM communities providing productive exchange with the physics oriented magnetic confinement liquid metal research groups. This international workshop will continue on a biennial basis (alternating with the Plasma-Surface Interactions (PSI) Conference) and the next workshop will be held at CIEMAT, Madrid, Spain, in 2015. C1 [Mazzitelli, G.] Assoc EURATOM ENEA Fus, Ctr Ric Frascati, I-00044 Frascati, Italy. [Hirooka, Y.] Natl Inst Fus Sci, Toki, Gifu 5095292, Japan. [Hirooka, Y.] Grad Univ Adv Studies, Toki, Gifu 5095292, Japan. [Hu, J. S.] Chinese Acad Sci, Inst Plasma Phys, Hefei 230031, Anhui, Peoples R China. [Mirnov, S. V.] TRINITI, Troitsk 142190, Moscow Reg, Russia. [Mirnov, S. V.] NRNU MEPhI, Moscow 115409, Russia. [Nygren, R.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Shimada, M.] IFERC Obuchi, JAEA Int Fus Res Ctr, Rokkasho, Aomori, Japan. [Ono, M.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Tabares, F. L.] As EURATOM CIEMAT, Natl Inst Fus, Madrid 28040, Spain. RP Mazzitelli, G (reprint author), Assoc EURATOM ENEA Fus, Ctr Ric Frascati, CP 65, I-00044 Frascati, Italy. EM guiseppe.mazzitelli@enea.it OI Tabares, Francisco/0000-0001-7045-8672 NR 3 TC 3 Z9 3 U1 3 U2 16 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD FEB PY 2015 VL 55 IS 2 AR 027001 DI 10.1088/0029-5515/55/2/027001 PG 9 WC Physics, Fluids & Plasmas SC Physics GA CA3ZE UT WOS:000348843100020 ER PT J AU Wade, MR Nazikian, R deGrassie, JS Evans, TE Ferraro, NM Moyer, RA Orlov, DM Buttery, RJ Fenstermacher, ME Garofalo, AM Lanctot, MA McKee, GR Osborne, TH Shafer, MA Solomon, WM Snyder, PB Suttrop, W Wingen, A Unterberg, EA Zeng, L AF Wade, M. R. Nazikian, R. deGrassie, J. S. Evans, T. E. Ferraro, N. M. Moyer, R. A. Orlov, D. M. Buttery, R. J. Fenstermacher, M. E. Garofalo, A. M. Lanctot, M. A. McKee, G. R. Osborne, T. H. Shafer, M. A. Solomon, W. M. Snyder, P. B. Suttrop, W. Wingen, A. Unterberg, E. A. Zeng, L. TI Advances in the physics understanding of ELM suppression using resonant magnetic perturbations in DIII-D SO NUCLEAR FUSION LA English DT Article DE DIII-D; resonant magnetic perturbation; ELM control; MHD plasma response; non-axisymmetric fields ID OPERATION; MODES; STABILITY; TOKAMAKS; PLASMAS; REGIME AB Recent experiments on DIII-D have increased confidence in the ability to suppress edge-localized modes (ELMs) using edge-resonant magnetic perturbations (RMPs) in ITER, including an improved physics basis for the edge response to RMPs as well as expansion of RMP ELM suppression to more ITER-like conditions. Complete ELM suppression has been achieved utilizing n = 3 RMPs in the ITER baseline scenario. In addition, RMP ELM suppression has been expanded to include plasmas with helium concentrations near 25% and the use of n = 2 RMPs. Analysis of the kinetic profile response suggests that ELM suppression is correlated with the co-alignment of the omega(perpendicular to e) = 0 location, an n = 3 rational surface, and the top of the pedestal. Modelling predicts that such a co-alignment could potentially lead to island (or island chain) formation just inside the top of the pedestal, inhibiting the growth of the pedestal and thereby maintaining the ELM-free state. Detailed analysis of data obtained during toroidal phase variations of the applied n = 3 RMPs have provided further evidence of an island-like structure at the top of the pedestal. In addition, nearly matched discharges with co-neutral-beam-injection (co-NBI) and counter-NBI have demonstrated the importance of the presence of the omega(perpendicular to e) = 0 location for ELM suppression. In the counter-NBI cases, the toroidal rotation profile is such that there is no omega(perpendicular to e) = 0 location and ELMs are not suppressed in conditions in which ELM suppression is generally observed with co-NBI. C1 [Wade, M. R.; deGrassie, J. S.; Evans, T. E.; Ferraro, N. M.; Buttery, R. J.; Garofalo, A. M.; Lanctot, M. A.; Osborne, T. H.; Snyder, P. B.] Gen Atom Co, San Diego, CA 92186 USA. [Nazikian, R.; Solomon, W. M.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Moyer, R. A.; Orlov, D. M.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Fenstermacher, M. E.] Lawrence Livermore Natl Lab, Lawrence, CA 94550 USA. [McKee, G. R.] Univ Wisconsin, Madison, WI 53706 USA. [Shafer, M. A.; Wingen, A.; Unterberg, E. A.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Suttrop, W.] IPP Garching, Garching, Germany. [Zeng, L.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. RP Wade, MR (reprint author), Gen Atom Co, San Diego, CA 92186 USA. EM wade@fusion.gat.com RI Orlov, Dmitriy/D-2406-2016; Unterberg, Ezekial/F-5240-2016; Lanctot, Matthew J/O-4979-2016; OI Shafer, Morgan/0000-0001-9808-6305; Orlov, Dmitriy/0000-0002-2230-457X; Unterberg, Ezekial/0000-0003-1353-8865; Lanctot, Matthew J/0000-0002-7396-3372; Wingen, Andreas/0000-0001-8855-1349; Solomon, Wayne/0000-0002-0902-9876 FU US Department of Energy [DE-AC02-09CH11466, DE-AC05-00O422725, DE-AC52-07NA27344, DE-FC02-04ER54698, DE-FG02-07ER54917, DE-FG02-08ER35984, DE-FG02-89ER53296] FX This work was supported by the US Department of Energy under DE-AC02-09CH11466, DE-AC05-00O422725, DE-AC52-07NA27344, DE-FC02-04ER54698, DE-FG02-07ER54917, DE-FG02-08ER35984, DE-FG02-89ER53296. DIII-D data shown in this paper can be obtained in digital format by following the links at https://fusion.gat.com/global/D3D_DMP. NR 40 TC 18 Z9 18 U1 4 U2 30 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD FEB PY 2015 VL 55 IS 2 AR 023002 DI 10.1088/0029-5515/55/2/023002 PG 18 WC Physics, Fluids & Plasmas SC Physics GA CA3ZE UT WOS:000348843100003 ER PT J AU Troia, MJ Gido, KB AF Troia, Matthew J. Gido, Keith B. TI Functional strategies drive community assembly of stream fishes along environmental gradients and across spatial scales SO OECOLOGIA LA English DT Article DE Environmental filtering; Feeding; Locomotion; Prairie streams; Reproductive life history ID LIFE-HISTORY STRATEGIES; PHYLOGENETIC STRUCTURE; TRAIT DISPERSION; PRAIRIE STREAMS; ECOLOGY; PATTERNS; VARIABILITY; FRAMEWORK; FOREST; CONVERGENCE AB Trade-offs among functional traits produce multi-trait strategies that shape species' interactions with the environment and drive the assembly of local communities from regional species pools. Stream fish communities vary along stream size gradients and among hierarchically structured habitat patches, but little is known about how the dispersion of strategies varies along environmental gradients and across spatial scales. We used null models to quantify the dispersion of reproductive life history, feeding, and locomotion strategies in communities sampled at three spatial scales in a prairie stream network in Kansas, USA. Strategies were generally underdispersed at all spatial scales, corroborating the longstanding notion of abiotic filtering in stream fish communities. We tested for variation in strategy dispersion along a gradient of stream size and between headwater streams draining different ecoregions. Reproductive life history strategies became increasingly underdispersed moving from downstream to upstream, suggesting that abiotic filtering is stronger in headwaters. This pattern was stronger among reaches compared to mesohabitats, supporting the premise that differences in hydrologic regime among reaches filter reproductive life history strategies. Feeding strategies became increasingly underdispersed moving from upstream to downstream, indicating that environmental filters associated with stream size affect the dispersion of feeding and reproductive life history in opposing ways. Weak differences in strategy dispersion were detected between ecoregions, suggesting that different abiotic filters or strategies drive community differences between ecoregions. Given the pervasiveness of multi-trait strategies in plant and animal communities, we conclude that the assessment of strategy dispersion offers a comprehensive approach for elucidating mechanisms of community assembly. C1 [Troia, Matthew J.; Gido, Keith B.] Kansas State Univ, Div Biol, Manhattan, KS 66506 USA. RP Troia, MJ (reprint author), Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37830 USA. EM troiamj@ornl.gov FU Kansas Department of Wildlife, Parks and Tourism; National Science Foundation FX We thank Kevin Kirkbride, Josh Perkin, Dustin Shaw, Trevor Starks, and James Whitney for field assistance and numerous property owners for providing private land access to sampling locations. We thank Tony Joern, Walter Dodds, Melinda Daniels, Jamie Kneitel and two anonymous reviewers for comments that greatly improved this manuscript. This research was funded by the Kansas Department of Wildlife, Parks and Tourism and the National Science Foundation Experimental Program to Stimulate Competitive Research. NR 66 TC 7 Z9 7 U1 6 U2 45 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0029-8549 EI 1432-1939 J9 OECOLOGIA JI Oecologia PD FEB PY 2015 VL 177 IS 2 BP 545 EP 559 DI 10.1007/s00442-014-3178-1 PG 15 WC Ecology SC Environmental Sciences & Ecology GA CA5XK UT WOS:000348981500022 PM 25502608 ER PT J AU Liu, C Yeager, JD Ramos, KJ AF Liu, C. Yeager, J. D. Ramos, K. J. TI Bonding energy of Sylgard on fused quartz: an experimental investigation SO PHILOSOPHICAL MAGAZINE LA English DT Article DE interfacial debonding; bulge test; digital image correlation (DIC); bonding energy; Sylgard ID BLISTER TEST; INTERFACIAL FRACTURE; SHEAR COEFFICIENT; HIGH EXPLOSIVES; ADHESION; TOUGHNESS; FILMS; SYSTEM; HMX AB The bonding energy between the polymer Sylgard and fused quartz is determined experimentally using a miniature bulge test combined with three-dimensional digital image correlation (3D-DIC). Based on the experimental observation, Mindlin plate theory is used to compute the bonding energy (adhesive energy or surface energy) between the Sylgard and the fused quartz. The experimental results demonstrate that the combination of the miniature bulge test and the 3D-DIC provides a viable tool to directly measure interfacial and bonding properties. C1 [Liu, C.; Yeager, J. D.; Ramos, K. J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Liu, C (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM cliu@lanl.gov OI Yeager, John/0000-0002-3121-6053 FU DoD/DOE Munitions Program (JMP); High Explosive Science and Engineering of Science Campaign 2 FX This study was supported by the Joint DoD/DOE Munitions Program (JMP) and the High Explosive Science and Engineering of Science Campaign 2. NR 36 TC 1 Z9 1 U1 0 U2 11 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 1478-6435 EI 1478-6443 J9 PHILOS MAG JI Philos. Mag. PD FEB 1 PY 2015 VL 95 IS 4 BP 346 EP 366 DI 10.1080/14786435.2015.1006292 PG 21 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering; Physics, Applied; Physics, Condensed Matter SC Materials Science; Metallurgy & Metallurgical Engineering; Physics GA CB1NA UT WOS:000349393400002 ER PT J AU Sun, YW Carrigan, CR Hao, Y AF Sun, Yunwei Carrigan, Charles R. Hao, Yue TI Radioxenon Production and Transport from an Underground Nuclear Detonation to Ground Surface SO PURE AND APPLIED GEOPHYSICS LA English DT Article DE Reactive transport; decay; ingrowth; first-order reaction; isotopic ratio ID TEST-BAN TREATY; REACTIVE TRANSPORT; EQUATIONS; SYSTEM; CHAINS; TESTS; WATER AB Radioxenon isotopes are considered as possible indicators for detecting and discriminating underground nuclear explosions. To monitor and sample the release of radioxenon isotopes, both independent and chain-reaction yields need to be considered together with multiphase transport in geological systems from the detonation point to the ground surface. For the sake of simplicity, modeling of radioxenon isotopic radioactivities has typically been focused either on chain reactions in a batch reactor without considering multiphase transport or on radionuclide transport with simplified reactions. Although numerical methods are available for integrating coupled differential equations of complex decay networks, the stiffness of ordinary differential equations due to greatly differing decay rates may require substantial additional effort to obtain solutions for the fully coupled system. For this reason, closed-form solutions for sequential reactions and numerical solutions for multiparent converging and multidaughter branching reactions were previously developed and used to simulate xenon isotopic radioactivities in the batch reactor mode. In this paper, we develop a fully coupled numerical model, which involves tracking 24 components (i.e., 22 radionuclide components plus air and water) in two phases to enhance model predictability of simultaneously simulating xenon isotopic transport and fully coupled chain reactions. To validate the numerical model and verify the corresponding computer code, we derived closed-form solutions for first-order xenon reactions in a batch reactor mode and for single-gas phase transport coupled with the xenon reactions in a one-dimensional column. Finally, cylindrical 3-D simulations of two-phase flow within a dual permeability fracture-matrix medium, simulating the geohydrologic regime of an underground nuclear explosion, indicate the existence of both a strong temporal and spatial dependence of xenon isotopic ratios sampled at the surface. In the example presented here, temporally evolving subsurface xenon isotopic ratios are found to migrate across the discrimination line delineating civilian nuclear activities from an underground nuclear explosion in the KALINOWSKI Multi-Isotope Ratio Chart. C1 [Sun, Yunwei; Carrigan, Charles R.; Hao, Yue] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Sun, YW (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM sun4@llnl.gov RI Sun, Yunwei/C-9751-2010 FU Office of Proliferation Detection, U.S. Department of Energy; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; [DE-AC52-06NA25946] FX The authors wish to thank Martin B. Kalinowski at Carl Friedrich von Weizsacker Center for Science and Peace Research (ZNF) and Carol A. Velsko at Lawrence Livermore National Laboratory for providing and interpreting data of fission product decay chains. The authors also thank Nathan G. Wimer and Steven A. Kreek at Lawrence Livermore National Laboratory, two anonymous reviewers, for their careful review and helpful comments that led to an improved manuscript. This research was funded by the Office of Proliferation Detection (NA-221), U.S. Department of Energy and performed under award number DE-AC52-06NA25946 and the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. The authors also wish to express their gratitude to the National Nuclear Security Administration, Office of Defense Nuclear Nonproliferation Research and Development (DNN R&D) and the Comprehensive Inspection Technologies working group, a multi-institutional and interdisciplinary group of scientists and engineers. NR 39 TC 2 Z9 2 U1 0 U2 7 PU SPRINGER BASEL AG PI BASEL PA PICASSOPLATZ 4, BASEL, 4052, SWITZERLAND SN 0033-4553 EI 1420-9136 J9 PURE APPL GEOPHYS JI Pure Appl. Geophys. PD FEB PY 2015 VL 172 IS 2 BP 243 EP 265 DI 10.1007/s00024-014-0863-2 PG 23 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CA3DT UT WOS:000348787100004 ER PT J AU Junek, WN Kvaerna, T Pirli, M Schweitzer, J Harris, DB Dodge, DA Woods, MT AF Junek, William N. Kvaerna, Tormod Pirli, Myrto Schweitzer, Johannes Harris, David B. Dodge, Douglas A. Woods, Mark T. TI Inferring Aftershock Sequence Properties and Tectonic Structure Using Empirical Signal Detectors SO PURE AND APPLIED GEOPHYSICS LA English DT Article DE Correlation detectors; Subspace detectors; Aftershock sequence; Tectonics; Seismicity ID WAVE-FORM CORRELATION; MAGNITUDE; SVALBARD; ENVIRONMENT; EVENTS; SWARMS AB Seismotectonic studies of the 2008 Storfjorden aftershock sequence were limited to data acquired by the permanent, but sparse, regional seismic network in the Svalbard archipelago. Storfjorden's remote location and harsh polar environment inhibited deployment of temporary seismometers that would have improved observations of sequence events. The lack of good station coverage prevented the detection and computation of hypocenter locations of many low magnitude events (mb < 2.5) in the NORSAR analyst-reviewed bulletin. As a result, the fine structure of the sequence's space-time distribution was not captured. In this study, an autonomous event detection and clustering framework is employed to build a more complete catalog of Storfjorden events using data from the Spitsbergen (SPITS) array. The new catalog allows the spatiotemporal distribution of seismicity within the fjord to be studied in greater detail. Information regarding the location of active event clusters provides a means of inferring the tectonic structure within the fault zone. The distribution of active clusters and moment tensor solutions for the Storfjorden sequence suggests there are at least two different structures within the fjord: a NE-SW trending linear feature with oblique-normal to strike-slip faulting and E-W trending normal faults. C1 [Junek, William N.; Woods, Mark T.] Patrick AF Base, AF Tech Applicat Ctr, Brevard, FL USA. [Kvaerna, Tormod; Pirli, Myrto; Schweitzer, Johannes] NORSAR, Kjeller, Norway. [Harris, David B.] Deschutes Signal Proc, Maupin, OR USA. [Dodge, Douglas A.] Lawrence Livermore Natl Lab, Livermore, CA USA. RP Junek, WN (reprint author), Patrick AF Base, AF Tech Applicat Ctr, Brevard, FL USA. EM william.junek@us.af.mil OI Kvaerna, Tormod/0000-0003-4435-257X NR 19 TC 4 Z9 4 U1 0 U2 9 PU SPRINGER BASEL AG PI BASEL PA PICASSOPLATZ 4, BASEL, 4052, SWITZERLAND SN 0033-4553 EI 1420-9136 J9 PURE APPL GEOPHYS JI Pure Appl. Geophys. PD FEB PY 2015 VL 172 IS 2 BP 359 EP 373 DI 10.1007/s00024-014-0938-0 PG 15 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CA3DT UT WOS:000348787100010 ER PT J AU Hsiao, YC Wu, T Zang, HD Li, MX Hu, B AF Hsiao, Yu-Che Wu, Ting Zang, Huidong Li, Mingxing Hu, Bin TI Addressing dynamic photovoltaic processes at electrode:active layer and donor:acceptor interfaces in organic solar cells under device-operating conditions SO SCIENCE CHINA-CHEMISTRY LA English DT Article DE electrode interface; donor-acceptor interface; dielectric layer; charge transfer states ID OPEN-CIRCUIT VOLTAGE; MAGNETIC-FIELD; HIGH-PERFORMANCE; WORK-FUNCTION; CHARGE COLLECTION; POLYMER; EFFICIENCY; RECOMBINATION; OXIDE; TRANSPORT AB This article presents our experimental studies to unravel the dynamic photovoltaic processes occurring at donor:acceptor (D:A) and electrode:active layer (E:A) interfaces under device-operating conditions by using two unique magneto-optical measurements, namely photo-induced capacitance and magnetic field effect measurement. First, we have found that a higher surface polarization of dielectric thin film can decrease the surface charge accumulation at E:A interface. The photo-induced capacitance results indicate that dielectric thin film plays a crucial role in the charge collection in generating photocurrent in organic solar cells. Second, our experimental results from magnetic field effect show that the binding energies of charge transfer (CT) states at D:A interface can be evaluated by using the critical bias required to completely dissociate the CT states. This is the first experimental demonstration that the binding energies of CT states can be measured under deviceoperating conditions. Furthermore, we use our measurement of magnetic field effect to investigate the most popular organic photovoltaic solar cells, organometal halide perovskite photovoltaic devices. The results of magneto-photoluminescence show that the photogenerated electrons and holes are inevitably recombined into electron-hole pairs through a spin-dependent process in the perovskites. Therefore, using spin polarizations can present a new design to control the photovoltaic loss in perovskites-based photovoltaic devices. Also, we found that introducing D:A interface can largely affect the bulk charge dissociation and recombination in perovskite solar cells. This indicates that the interfacial and bulk photovoltaic processes are internally coupled in developing photovoltaic actions in perovskite devices. Clearly, these magneto-optical measurements show a great potential to unravel the deeper photovoltaic processes occurring at D:A and E:A interfaces in both organic bulk-heterojunction and perovskite solar cells under device-operating conditions. C1 [Hsiao, Yu-Che; Wu, Ting; Li, Mingxing; Hu, Bin] Beijing Jiaotong Univ, Inst Optoelect Technol, Beijing 100044, Peoples R China. [Hsiao, Yu-Che; Hu, Bin] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Zang, Huidong] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Hu, B (reprint author), Beijing Jiaotong Univ, Inst Optoelect Technol, Beijing 100044, Peoples R China. EM bhu@utk.edu FU National Science Foundation of the United States [ECCS-1102011, ECCS-0644945, CBET-1438181]; Sustainable Energy Education and Research Center; Center for Materials Processing at the University of Tennessee; Division of Scientific User Facilities, U.S. Department of Energy [CNMS2012-106, CNMS2012-107, CNMS-2012-108]; National Natural Science Foundation of China [21161160445, 61077020] FX This work was supported by the National Science Foundation of the United States (ECCS-1102011, ECCS-0644945, and CBET-1438181). The authors also acknowledge the support from Sustainable Energy Education and Research Center and Center for Materials Processing at the University of Tennessee. This research was partially conducted at the Center for Nanophase Materials Sciences based on user project (CNMS2012-106, CNMS2012-107, CNMS-2012-108), which is sponsored at Oak Ridge National Laboratory by the Division of Scientific User Facilities, U.S. Department of Energy. The authors at the University of Tennessee also acknowledge the project support from the National Natural Science Foundation of China (21161160445, 61077020). NR 55 TC 2 Z9 2 U1 3 U2 37 PU SCIENCE PRESS PI BEIJING PA 16 DONGHUANGCHENGGEN NORTH ST, BEIJING 100717, PEOPLES R CHINA SN 1674-7291 EI 1869-1870 J9 SCI CHINA CHEM JI Sci. China-Chem. PD FEB PY 2015 VL 58 IS 2 SI SI BP 239 EP 247 DI 10.1007/s11426-014-5280-y PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA CA6EI UT WOS:000349001500009 ER PT J AU Blair, J Mebane, DS AF Blair, Joshua Mebane, David S. TI A Bayesian approach to electrical conductivity relaxation and isotope exchange/secondary ion mass spectrometry SO SOLID STATE IONICS LA English DT Article DE Electrical conductivity relaxation; Mixed ionic-electronic conductor; Isotope exchange depth profiling; Parameter estimation ID OPTIMAL EXPERIMENTAL-DESIGN; CHEMICAL DIFFUSION-COEFFICIENT; SURFACE EXCHANGE COEFFICIENTS; OXYGEN SELF-DIFFUSION; SENSITIVITY-ANALYSIS; STABILIZED ZIRCONIA; THIN-FILM; IMPEDANCE; IDENTIFICATION; MODELS AB A Bayesian method for interpretation of electrical conductivity relaxation and isotope exchange/secondary ion mass spectrometry data is presented and demonstrated on data appearing in the literature. The new method enables quantification of uncertainty due to data fitting in estimates for the effective surface exchange coefficient k(+) and the effective diffusion coefficient D+. The standard infinite series solutions to the semi-infinite diffusion problem with linearized chemical kinetics at the boundary are utilized, although the Bayesian technique does not depend on the existence of analytical solutions. The methodology is demonstrated in the analysis of data appearing in the literature, both for isotope exchange/secondary ion mass spectrometry and electrical conductivity relaxation. In particular, the utility of the technique in definitively resolving questions of parameter identifiability is demonstrated in a comparison of two literature studies on the same bulk material that lead to widely different estimated parameters using the standard nonlinear least squares fit. (C) 2014 Elsevier B.V. All rights reserved. C1 Natl Energy Technol Lab, Morgantown, WV USA. W Virginia Univ, Dept Mech & Aerosp Engn, Morgantown, WV 26506 USA. RP Mebane, DS (reprint author), POB 6106,ESB 333, Morgantown, WV 26506 USA. EM david.mebane@mail.wvu.edu FU National Energy Technology Laboratory's ongoing research in solid oxide fuel cells under the RES contract [DE-FE0004000] FX The assistance of Harry Abernathy, Kirk Gerdes and Roger De Souza is gratefully acknowledged. This technical effort was performed in support of the National Energy Technology Laboratory's ongoing research in solid oxide fuel cells under the RES contract DE-FE0004000. NR 25 TC 4 Z9 4 U1 2 U2 7 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-2738 EI 1872-7689 J9 SOLID STATE IONICS JI Solid State Ion. PD FEB PY 2015 VL 270 BP 47 EP 53 DI 10.1016/j.ssi.2014.12.009 PG 7 WC Chemistry, Physical; Physics, Condensed Matter SC Chemistry; Physics GA CA9XG UT WOS:000349277500007 ER PT J AU Newsom, RK Berg, LK Shaw, WJ Fischer, ML AF Newsom, Rob K. Berg, Larry K. Shaw, William J. Fischer, Marc L. TI Turbine-scale wind field measurements using dual-Doppler lidar SO WIND ENERGY LA English DT Article DE Doppler lidar; dual-Doppler; wind measurement ID COHERENT LASER-RADAR; LOW-LEVEL JET; BOUNDARY-LAYER; SINGLE-DOPPLER; PART I; RETRIEVAL; TURBULENCE; CASES-99; SYSTEM; MUSCAT AB Spatially resolved measurements of microscale winds are retrieved using scanning dual-Doppler lidar and then compared with independent in situ wind measurements. Data for this study were obtained during a month-long field campaign conducted at a site in north-central Oklahoma in November of 2010. Observational platforms include one instrumented 60m meteorological tower and two scanning coherent Doppler lidars. The lidars were configured to perform coordinated dual-Doppler scans surrounding the 60m tower, and the resulting radial velocity observations were processed to retrieve the three-component velocity vector field on surfaces defined by the intersecting scan planes. The dual-Doppler analysis method is described, and three-dimensional visualizations of the retrieved fields are presented. The retrieved winds are compared with sonic anemometer (SA) measurements at the 60m level on the tower. The Pearson correlation coefficient between the retrievals and the SA wind speeds was greater than 0.97, and the wind direction difference was very small (<0.1(o)), suggesting that the dual-Doppler technique can be used to examine fine-scale variations in the flow. However, the mean percent difference between the SA and dual-Doppler wind speed was approximately 15%, with the SA consistently measuring larger wind speeds. To identify the source of the discrepancy, a multi-instrument intercomparison study was performed involving lidar wind speeds derived from standard velocity-azimuth display (VAD) analysis of plan position indicator scan data, a nearby 915MHz radar wind profiler (RWP) and radiosondes. The lidar VAD, RWP and radiosondes wind speeds were found to agree to within 3%. By contrast, SA wind speeds were found to be approximately 14% larger than the lidar VAD wind speeds. These results suggest that the SA produced wind speeds that were too large. Copyright (c) 2013 John Wiley & Sons, Ltd. C1 [Newsom, Rob K.; Berg, Larry K.; Shaw, William J.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Fischer, Marc L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Newsom, RK (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM rob.newsom@pnnl.gov RI Berg, Larry/A-7468-2016; OI Berg, Larry/0000-0002-3362-9492; Shaw, William/0000-0002-9979-1089 FU DOEs Office of Biological and Environmental Research [DE-AC02-05CH11231] FX The research described in this paper was conducted under the Laboratory Directed Research and Development Program at Pacific Northwest National Laboratory (PNNL) and made use of DOEs ARM Climate Research Facility. The authors wish to express their thanks to Guy Pearson and Justin Eacock at Halo Photonics and the staff at the ARM SGP site. MLF also acknowledges support for analysis from the Atmospheric System Research Program, DOEs Office of Biological and Environmental Research, under contract DE-AC02-05CH11231. NR 34 TC 13 Z9 13 U1 4 U2 17 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1095-4244 EI 1099-1824 J9 WIND ENERGY JI Wind Energy PD FEB PY 2015 VL 18 IS 2 BP 219 EP 235 DI 10.1002/we.1691 PG 17 WC Energy & Fuels; Engineering, Mechanical SC Energy & Fuels; Engineering GA CA4CI UT WOS:000348851500003 ER PT J AU Kusnick, J Adams, DE Griffith, DT AF Kusnick, Josh Adams, Douglas E. Griffith, D. Todd TI Wind turbine rotor imbalance detection using nacelle and blade measurements SO WIND ENERGY LA English DT Article DE wind energy; wind turbine imbalance; condition monitoring; structural dynamics; pitch control; structural health monitoring AB Wind power is the world's fastest growing renewable energy source, but operations and maintenance costs are still a major obstacle toward reliability and widescale adoption of wind power, accounting for a large part of the cost of energy for offshore installations. Structural health monitoring systems have been proposed for implementing condition-based maintenance. The wind energy industry currently uses condition monitoring systems that are mostly adapted from roating machinery in other power generation industries. However, these systems have had limited effectiveness on wind turbines because of their atypical operating conditions, which are characterized by low and variable rotational speed, rapidly varying torque, extremely large rotors and stochastic loading from the wind. Although existing systems primarily take measurements from the nacelle, valuable information can be extracted from the structural dynamic response of the rotor blades to mitigate potentially damaging loading conditions. One such condition is rotor imbalance, which not only reduces the aerodynamic efficiency of the turbine and therefore its power output but can also lead to very large increases in loading on the drivetrain, blades and tower. The National Renewable Energy Laboratory's fast software was used to model both mass and aerodynamic imbalance in a 5MW offshore wind turbine. It is shown that a combination of blade and nacelle measurements, most of which can be obtained from standard instrumentation already found on utility-scale wind turbines, can be formulated into an algorithm used to detect and locate imbalance. The method described herein allows for imbalance detection that is potentially more sensitive than existing on-line systems, while taking advantage of sensors that are already in place on many utility-scale wind turbines. Copyright (c) 2014 John Wiley & Sons, Ltd. C1 [Kusnick, Josh] Purdue Univ, Sch Mech Engn, W Lafayette, IN 47907 USA. [Adams, Douglas E.] Vanderbilt Univ, Nashville, TN 37235 USA. [Griffith, D. Todd] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Kusnick, J (reprint author), Purdue Univ, Sch Mech Engn, W Lafayette, IN 47907 USA. EM jkusnick@purdue.edu RI Lin, Zhao/C-8319-2011 OI Lin, Zhao/0000-0002-6131-9723 FU Sandia National Laboratories [1067259]; US Department of Energy FX The authors would like to acknowledge Sandia National Laboratories (Contract Agreement 1067259) and the US Department of Energy for their support of this paper and their continuing support of the wind energy research efforts being performed at Vanderbilt University. NR 12 TC 3 Z9 3 U1 2 U2 20 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1095-4244 EI 1099-1824 J9 WIND ENERGY JI Wind Energy PD FEB PY 2015 VL 18 IS 2 BP 267 EP 276 DI 10.1002/we.1696 PG 10 WC Energy & Fuels; Engineering, Mechanical SC Energy & Fuels; Engineering GA CA4CI UT WOS:000348851500006 ER PT J AU Pace, A Johnson, K Wright, A AF Pace, A. Johnson, K. Wright, A. TI Preventing wind turbine overspeed in highly turbulent wind events using disturbance accommodating control and light detection and ranging SO WIND ENERGY LA English DT Article DE LIDAR; extreme events; rotor overspeed AB Light detection and ranging (LIDAR) systems can be used to provide wind inflow information to a wind turbine controller before the wind reaches the turbine. Both fatigue and extreme load reduction are possible as a result; in this research, we propose a LIDAR-based controller designed to prevent emergency shutdowns caused by rotor overspeed. This switching controller consists of a disturbance accommodating control (DAC)-based baseline controller and a different DAC linearized about a reduced generator speed for extreme events, also referred to as an extreme event controller. Switching between the controllers was performed using linear interpolation over various transition times, depending on how early the extreme event could be detected. If a gust of wind is detected using LIDAR measurements evaluated by a one-sided cumulative summation algorithm, a relatively long transition time can be used. Switching can also be based on a large output estimation error, epsilon(y), in which case the transition time is shorter. Once the extreme event passed, control is switched from the extreme event controller back to the baseline DAC. This switching controller resulted in fewer overspeeds when compared with the modified baseline controller, which is a gain scheduled DAC. By preventing overspeeds, the switching controller increased the mean power the wind turbine generated over a simulated 10min period. Copyright (c) 2014 John Wiley & Sons, Ltd. C1 [Pace, A.; Johnson, K.] Colorado Sch Mines, Golden, CO 80401 USA. [Johnson, K.; Wright, A.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Johnson, K (reprint author), Colorado Sch Mines, 1500 Illinois St, Golden, CO 80401 USA. EM kjohnson@mines.edu FU NREL FX The authors would like to thank NREL for providing the research funding, Michigan Aerospace Corporation for collaboration and Eric Simley for providing the LIDAR module used in FAST. NR 33 TC 2 Z9 2 U1 1 U2 8 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1095-4244 EI 1099-1824 J9 WIND ENERGY JI Wind Energy PD FEB PY 2015 VL 18 IS 2 BP 351 EP 368 DI 10.1002/we.1705 PG 18 WC Energy & Fuels; Engineering, Mechanical SC Energy & Fuels; Engineering GA CA4CI UT WOS:000348851500011 ER PT J AU Pierson, BD Griffin, HC Flaska, M Katalenich, JA Kitchen, BB Pozzi, SA AF Pierson, Bruce D. Griffin, Henry C. Flaska, Marek Katalenich, Jeff A. Kitchen, Brian B. Pozzi, Sara A. TI Benchmarking the repeatability of a pneumatic cyclic neutron activation analysis facility using O-16(n,p)N-16 for nuclear forensics SO APPLIED RADIATION AND ISOTOPES LA English DT Article DE Fusion neutron; Cyclic neutron activation analysis; Short-lived; Half-life; List-mode data acquisition; Dead-time; Pulse pile-up; Nitrogen-16 ID HALF-LIFE; 16N AB A target was prepared for cyclic neutron activation analysis by heat sealing lithium-carbonate in polyethylene. The target was cyclically irradiated 50 times using a Thermo-Scientific accelerator based deuterium-tritium fusion neutron generator. During counting periods, gamma-rays emitted by N-16 were detected using three high-purity germanium detectors acquiring data in list-mode. Total counts acquired in each spectrum were compared between the three detectors to examine variability in geometric positioning of the target and variability of the generator intensity throughout the experiment. These two effects were determined to be the primary sources of variation in the measured counts. Variation in target positioning and generator intensity were found to increase the standard deviation by 34% and 33%, respectively. Transit times to the detector were found to be slower and more variable than transit to the generator but were well below the half second threshold needed to measure short-lived radionuclides with half-lives on the order of seconds. The standard deviation in irradiation time was found to be less than 1 milliseconds. The impact on statistical variability in the measured counts was negligible relative to the two primary sources of variation. Spectra acquired from each cycle were summed together. The sum of the peak areas from the 6.1 MeV gamma-ray and its corresponding single and double escape peaks were used to measure the half-life of N-16. The result of 7.108(15) seconds derived from data suggests that the currently published value of 7.13(2) seconds has minimal systematic bias induced by background. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Pierson, Bruce D.; Griffin, Henry C.; Flaska, Marek; Kitchen, Brian B.; Pozzi, Sara A.] Univ Michigan, Dept Nucl Engn & Radiol Sci, Ann Arbor, MI 48109 USA. [Katalenich, Jeff A.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Pierson, BD (reprint author), Univ Michigan, Dept Nucl Engn & Radiol Sci, 2355 Bonisteel Blvd, Ann Arbor, MI 48109 USA. EM bpnuke@umich.edu FU U.S. Department of Homeland Security [2012-DN-130-NF0001] FX This material is based upon work supported by the U.S. Department of Homeland Security under Grant Award 2012-DN-130-NF0001. The views and conclusions contained in this paper are those of the authors and should not be interpreted as representing the official policies, either expressed or implied, of the U.S. Department of Homeland Security. NR 23 TC 1 Z9 1 U1 0 U2 9 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0969-8043 J9 APPL RADIAT ISOTOPES JI Appl. Radiat. Isot. PD FEB PY 2015 VL 96 BP 20 EP 26 DI 10.1016/j.apradiso.2014.11.010 PG 7 WC Chemistry, Inorganic & Nuclear; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging SC Chemistry; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging GA CA2PD UT WOS:000348749100004 PM 25479431 ER PT J AU Roberts, AD Geddes, CGR Matlis, N Nakamura, K O'Neil, JP Shaw, BH Steinke, S van Tilborg, J Leemans, WP AF Roberts, A. D. Geddes, C. G. R. Matlis, N. Nakamura, K. O'Neil, J. P. Shaw, B. H. Steinke, S. van Tilborg, J. Leemans, W. P. TI Measured bremsstrahlung photonuclear production of Mo-99 (Tc-99m) with 34 MeV to 1.7 GeV electrons SO APPLIED RADIATION AND ISOTOPES LA English DT Article DE Tc-99m; Mo-99; Bremsstrahlung production AB Mo-99 photonuclear yield was measured using high-energy electrons from Laser Plasma Accelerators and natural molybdenum. Spectroscopically resolved electron beams allow comparisons to Monte Carlo calculations using known Mo-100(gamma,n)Mo-99 cross sections. Yields are consistent with published low-energy data, and higher energy data are well predicted from the calculations. The measured yield is (15 +/- 2) x 10(-5) atoms/electron (0.92 +/- 0.11 GBq/1.1 mu A) for 25 mm targets at 33.7 MeV, rising to (1391 +/- 20) x 10(-5) atoms/electron (87 +/- 2 GBq/mu A) for 54 mm/ 1.7 GeV, with peak power-normalized yield at 150.MeV. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Roberts, A. D.] Minnesota State Univ, Dept Phys & Astron, Mankato, MN 56001 USA. [Geddes, C. G. R.; Matlis, N.; Nakamura, K.; O'Neil, J. P.; Shaw, B. H.; Steinke, S.; van Tilborg, J.; Leemans, W. P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Roberts, AD (reprint author), Minnesota State Univ, Dept Phys & Astron, Mankato, MN 56001 USA. EM andrew.roberts@mnsu.edu RI Steinke, Sven/D-8086-2011 OI Steinke, Sven/0000-0003-0507-698X FU Minnesota State University, Mankato; U.S. Department of Energy [DE-AC02-05CH11231] FX The corresponding author was supported through grant funding from Minnesota State University, Mankato. The authors gratefully acknowledge the assistance of Cs. Toth, D.E. Mittelberger, R. Donahue, and A. Smith of LBNL. This work was performed at Lawrence Berkeley National Laboratory under Contract no. DE-AC02-05CH11231 with the U.S. Department of Energy. NR 41 TC 3 Z9 3 U1 0 U2 12 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0969-8043 J9 APPL RADIAT ISOTOPES JI Appl. Radiat. Isot. PD FEB PY 2015 VL 96 BP 122 EP 128 DI 10.1016/j.apradiso.2014.11.008 PG 7 WC Chemistry, Inorganic & Nuclear; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging SC Chemistry; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging GA CA2PD UT WOS:000348749100016 PM 25484305 ER PT J AU Li, GL Abbott, JKC Brasfield, JD Liu, PZ Dale, A Duscher, G Rack, PD Feigerle, CS AF Li, Guoliang Abbott, Julia K. C. Brasfield, John D. Liu, Peizhi Dale, Alexis Duscher, Gerd Rack, Philip D. Feigerle, Charles S. TI Structure characterization and strain relief analysis in CVD growth of boron phosphide on silicon carbide SO APPLIED SURFACE SCIENCE LA English DT Article DE Boron phosphide; Defect; Strain relief; CVD; Neutron detection ID HETEROEPITAXIAL GROWTH; CRYSTAL-GROWTH AB Boron phosphide (BP) is a material of interest for development of a high-efficiency solid-state thermal neutron detector. For a thick film-based device, microstructure evolution is key to the engineering of material synthesis. Here, we report epitaxial BP films grown on silicon carbide with vicinal steps and provide a detailed analysis of the microstructure evolution and strain relief. The BP film is epitaxial in the near-interface region but deviates from epitaxial growth as the film develops. Defects such as coherent and incoherent twin boundaries, dislocation loops, stacking faults concentrate in the near-interface region and segment this region into small domains. The formation of defects in this region do not fully release the strain originated from the lattice mismatch. Large grains emerge above the near-interface region and grain boundaries become the main defects in the upper part of the BP film. (C) 2014 Elsevier B.V. All rights reserved. C1 [Li, Guoliang; Liu, Peizhi; Duscher, Gerd; Rack, Philip D.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Abbott, Julia K. C.; Brasfield, John D.; Dale, Alexis; Feigerle, Charles S.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Duscher, Gerd] Oak Ridge Natl Lab, Div Engn & Mat Sci, Oak Ridge, TN 37831 USA. [Rack, Philip D.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Feigerle, CS (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. EM cfeigerl@tennessee.edu RI Liu, Peizhi/K-6442-2013; Li, Guoliang/M-6614-2014; Duscher, Gerd/G-1730-2014; OI Liu, Peizhi/0000-0001-9638-2960; Li, Guoliang/0000-0003-3798-8422; Duscher, Gerd/0000-0002-2039-548X; Rack, Philip/0000-0002-9964-3254 FU U.S. Department of Energy (DOE), NNSA [NA-221]; Office of Nuclear Proliferation Detection FX The research is supported by the U.S. Department of Energy (DOE), NNSA, NA-221, Office of Nuclear Proliferation Detection. We thank joint Institute for Advanced Materials (JIAM) at the University of Tennessee and DOE-Basic Energy Sciences (BES) for microscope access. NR 13 TC 6 Z9 6 U1 3 U2 40 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0169-4332 EI 1873-5584 J9 APPL SURF SCI JI Appl. Surf. Sci. PD FEB 1 PY 2015 VL 327 BP 7 EP 12 DI 10.1016/j.apsusc.2014.11.037 PG 6 WC Chemistry, Physical; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA AZ8GQ UT WOS:000348453800002 ER PT J AU Yue, MY Zhou, BM Jiao, KY Qian, XM Xu, ZW Teng, KY Zhao, LH Wang, JJ Jiao, YN AF Yue, Mengyao Zhou, Baoming Jiao, Kunyan Qian, Xiaoming Xu, Zhiwei Teng, Kunyue Zhao, Lihuan Wang, Jiajun Jiao, Yanan TI Switchable hydrophobic/hydrophilic surface of electrospun poly (L-lactide) membranes obtained by CF4 microwave plasma treatment SO APPLIED SURFACE SCIENCE LA English DT Article DE CF4 plasma; Hydrophobic/hydrophilic surface; Poly (lactic acid); Tunable wettability; Electrospinning membrane ID POLYLACTIC ACID; EXCIMER-LASER; AR-PLASMA; FILMS; BIOPOLYMERS; NANOFIBERS; SCAFFOLDS; HYDROPHOBICITY; DISCHARGE; ADHESION AB A switchable surface that promotes either hydrophobic or hydrophilic wettability of poly (L-lactide) (PLLA) microfibrous membranes is obtained by CF4 microwave plasma treatment in this paper. The results indicated that both etching and grafting process occurred during the CF4 plasma treatment and these two factors synergistically affected the final surface wettability of PLLA membranes. When plasma treatment was taken under a relatively low power, the surface wettability of PLLA membranes turned from hydrophobic to hydrophilic. Especially when CF4 plasma treatment was taken under 100 W for 10 min and 150 W for 5 min, the water contact angle sharply decreased from 116 +/- 3.0 degrees to similar to 0 degrees. According to Field-emission scanning electron microscopy (FESEM) results, the PLLA fibers were notably etched by CF4 plasma treatment. Combined with the X-ray photoelectron spectroscopy (XPS) measurements, only a few fluorine-containing groups were grafted onto the surface, so the etching effect directly affected the surface wettability of PLLA membranes in low plasma power condition. However, with the plasma power increasing to 200 W, the PLLA membrane surface turned to hydrophobic again. In contrast, the morphology changes of PLLA fiber surfaces were not obvious while a large number of fluorine-containing groups grafted onto the surface. So the grafting effect gradually became the major factor for the final surface wettability. (C) 2014 Elsevier B.V. All rights reserved. C1 [Yue, Mengyao; Zhou, Baoming; Jiao, Kunyan; Qian, Xiaoming; Xu, Zhiwei; Teng, Kunyue; Zhao, Lihuan; Jiao, Yanan] Tianjin Polytech Univ, Minist Educ, Key Lab Adv Braided Composites, Tianjin 300387, Peoples R China. [Wang, Jiajun] Brookhaven Natl Lab, Photon Sci Directorate, Upton, NY 11973 USA. RP Xu, ZW (reprint author), Tianjin Polytech Univ, Minist Educ, Key Lab Adv Braided Composites, Tianjin 300387, Peoples R China. EM xuzhiwei@tjpu.edu.cn; jjwang@bnl.gov RI Xu, Zhiwei/A-1313-2015 OI Xu, Zhiwei/0000-0002-8067-5344 FU Petrochemical Joint Funds of National Natural Science Fund Committee - China National Petroleum Corporation [U1362108]; China Postdoctoral Science Foundation [2014T70217] FX The work was funded by the Petrochemical Joint Funds of National Natural Science Fund Committee - China National Petroleum Corporation (U1362108) and China Postdoctoral Science Foundation (2014T70217). NR 48 TC 11 Z9 11 U1 11 U2 57 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0169-4332 EI 1873-5584 J9 APPL SURF SCI JI Appl. Surf. Sci. PD FEB 1 PY 2015 VL 327 BP 93 EP 99 DI 10.1016/j.apsusc.2014.11.149 PG 7 WC Chemistry, Physical; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA AZ8GQ UT WOS:000348453800013 ER PT J AU Ruggles, A Kelman, J AF Ruggles, Adam Kelman, James TI Unsteady vortex breakdown in an atmospheric swirl stabilised combustor. Part 1: Chamber behaviour SO COMBUSTION AND FLAME LA English DT Article DE Gas turbine combustor; Combustion instabilities; Vortex breakdown; Swirling flows; High speed diagnostics; SPIV ID TURBINE MODEL COMBUSTOR; LARGE-EDDY SIMULATION; LEAN-PREMIXED COMBUSTOR; HEAT RELEASE; ACOUSTIC ANALYSIS; DUMP COMBUSTOR; FLAME DYNAMICS; FLOW; INSTABILITY; MECHANISMS AB This paper presents the behaviour of three very different and unique flame and flow structures within an atmospheric swirl-stabilised dump combustor supplied with a lean premixed mixture of methane and air. The reactant flow was artificially perturbed with frequencies of 100 Hz, 200 Hz, and 400 Hz. Phase average behaviour and temporal dynamics were characterised using phase locked high speed CH chemiluminescence and high speed stereo particle imaging. The interaction between the flame and flow field, in particular the internal recirculation zone of the vortex breakdown, was determined to be responsible for differences observed in behaviour at the three forcing frequencies. The 100 Hz perturbation frequency displayed simple oscillatory motion. Higher perturbation frequencies of 200 Hz and 400 Hz gave rise to a second toroidal vortex ring which formed within the internal recirculation zone adjacent to the inner shear layer. This caused additional out of phase modulation of the heat release rate and flame area. Twin counter rotating vorticity structures attached to the annulus were formed as a result of the chamber geometry. The oscillating inlet flow and oscillating reversed flow region of the inner recirculation zone caused oscillations in vorticity magnitude which were responsible for flame wrinkling and stretch effects upon the flame front. Vorticity within the shear layers was found to be the source of harmonic frequency generation of the imposed perturbation frequencies. The data is presented in detail to facilitate CFD model comparisons, particularly LES. Published by Elsevier Inc. C1 [Ruggles, Adam] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94550 USA. [Ruggles, Adam; Kelman, James] Cranfield Univ, Cranfield MK43 0AL, Beds, England. RP Ruggles, A (reprint author), Sandia Natl Labs, Combust Res Facil, 7011 East Ave, Livermore, CA 94550 USA. EM ajruggl@sandia.gov FU EPSRC FX This work was funded by the EPSRC and conducted at Cranfield University, UK. Many insightful discussions were had with Sandia National Laboratory scientists, Robert Barlow in particular. NR 61 TC 3 Z9 3 U1 1 U2 10 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0010-2180 EI 1556-2921 J9 COMBUST FLAME JI Combust. Flame PD FEB PY 2015 VL 162 IS 2 BP 388 EP 407 DI 10.1016/j.combustflame.2014.07.016 PG 20 WC Thermodynamics; Energy & Fuels; Engineering, Multidisciplinary; Engineering, Chemical; Engineering, Mechanical SC Thermodynamics; Energy & Fuels; Engineering GA AZ7QB UT WOS:000348411900009 ER PT J AU Bane, SPM Ziegler, JL Shepherd, JE AF Bane, Sally P. M. Ziegler, Jack L. Shepherd, Joseph E. TI Investigation of the effect of electrode geometry on spark ignition SO COMBUSTION AND FLAME LA English DT Article DE Spark ignition; Flames; Electrode ID FLAME KERNEL; NONEQUILIBRIUM PLASMA; NANOSECOND DISCHARGE; METHANE/AIR MIXTURES; GAS TEMPERATURE; AIR MIXTURES; COMBUSTION; SIMULATION; ENERGY; MECHANISM AB High-speed schlieren visualization and numerical simulations are used to study the fluid mechanics following a spark discharge and the effect on the ignition process in a hydrogen-air mixture. A two-dimensional axisymmetric model of spark discharge in air and spark ignition was developed using the non-reactive and reactive Navier-Stokes equations including mass and heat diffusion. The numerical method employs structured adaptive mesh refinement software to produce highly-resolved simulations, which is critical for accurate resolution of all the physical scales of the complex fluid mechanics and chemistry. The simulations were performed with three different electrode geometries to investigate the effect of the geometry on the fluid mechanics of the evolving spark kernel and on flame formation. The computational results were compared with high-speed schlieren visualization of spark and ignition kernels. It was shown that the spark channel emits a blast wave that is spherical near the electrode surfaces and cylindrical near the center of the spark gap, and thus is highly influenced by the electrode geometry. The ensuing competition between spherical and cylindrical expansion in the spark gap and the boundary layer on the electrode surface both generate vorticity, resulting in the toroidal shape of the hot gas kernel and enhanced mixing. The temperature and rate of cooling of the hot kernel and mixing region are significantly. effected by the electrode geometry and will have a critical impact on ignition. In the flanged electrode configuration the viscous effects generate a multidimensional flow field and lead to a curved flame front, a result not seen in previous work. Also, the high level of confinement by the flanges results in higher gas temperatures, suggesting that a lower ignition energy would be required. The results of this work provide new insights on the roles of the various physical phenomena in spark kernel formation and ignition, in particular the important effects of viscosity, pressure gradients, electrode geometry, and hot gas confinement. (C) 2014 The Combustion Institute. Published by Elsevier Inc. All rights reserved. C1 [Bane, Sally P. M.] Purdue Univ, Sch Aeronaut & Astronaut, W Lafayette, IN 47907 USA. [Ziegler, Jack L.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. [Shepherd, Joseph E.] CALTECH, Grad Aerosp Labs, Pasadena, CA 91125 USA. RP Bane, SPM (reprint author), Purdue Univ, Sch Aeronaut & Astronaut, 701 W Stadium Ave, W Lafayette, IN 47907 USA. EM sbane@purdue.edu RI Shepherd, Joseph/B-5997-2014 OI Shepherd, Joseph/0000-0003-3181-9310 FU Boeing Company through a Strategic Research and Development Relationship Agreement [CT-BA-GTA-1]; Department of Energy Computational Science Graduate Fellowship program (DOE CSGF) FX Sally Bane was supported by The Boeing Company through a Strategic Research and Development Relationship Agreement CT-BA-GTA-1. Jack Ziegler was supported by the Department of Energy Computational Science Graduate Fellowship program (DOE CSGF). NR 45 TC 4 Z9 4 U1 4 U2 27 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0010-2180 EI 1556-2921 J9 COMBUST FLAME JI Combust. Flame PD FEB PY 2015 VL 162 IS 2 BP 462 EP 469 DI 10.1016/j.combustflame.2014.07.017 PG 8 WC Thermodynamics; Energy & Fuels; Engineering, Multidisciplinary; Engineering, Chemical; Engineering, Mechanical SC Thermodynamics; Energy & Fuels; Engineering GA AZ7QB UT WOS:000348411900014 ER PT J AU Long, PE Williams, KH Davis, JA Fox, PM Wilkins, MJ Yabusaki, SB Fang, YL Waichler, SR Berman, ESF Gupta, M Chandler, DP Murray, C Peacock, AD Giloteaux, L Handley, KM Lovley, DR Banfield, JF AF Long, Philip E. Williams, Kenneth H. Davis, James A. Fox, Patricia M. Wilkins, Michael J. Yabusaki, Steven B. Fang, Yilin Waichler, Scott R. Berman, Elena S. F. Gupta, Manish Chandler, Darrell P. Murray, Chris Peacock, Aaron D. Giloteaux, Ludovic Handley, Kim M. Lovley, Derek R. Banfield, Jillian F. TI Bicarbonate impact on U(VI) bioreduction in a shallow alluvial aquifer SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID IN-SITU BIOREMEDIATION; URANIUM-CONTAMINATED GROUNDWATER; MICROBIAL COMMUNITY STRUCTURE; STABLE-ISOTOPE VARIATIONS; COLUMN ANALOG EXPERIMENT; BIOSTIMULATION EXPERIMENT; DESULFOTOMACULUM-REDUCENS; METAL REDUCTION; SEDIMENTS; MODEL AB Field-scale biostimulation and desorption tracer experiments conducted in a uranium (U) contaminated, shallow alluvial aquifer have provided insight into the coupling of microbiology, biogeochemistry, and hydrogeology that control U mobility in the subsurface. Initial experiments successfully tested the concept that Fe-reducing bacteria such as Geobacter sp. could enzymatically reduce soluble U(VI) to insoluble U(IV) during in situ electron donor amendment (Anderson et al., 2003; Williams et al., 2011). In parallel, in situ desorption tracer tests using bicarbonate amendment demonstrated rate-limited U(VI) desorption (Fox et al., 2012). These results and prior laboratory studies underscored the importance of enzymatic U(VI)reduction and suggested the ability to combine desorption and bioreduction of U(VI). Here we report the results of a new field experiment in which bicarbonate-promoted uranium desorption and acetate amendment were combined and compared to an acetate amendment-only experiment in the same experimental plot. Results confirm that bicarbonate amendment to alluvial aquifer sediments desorbs U(VI) and increases the abundance of Ca-uranyl-carbonato complexes. At the same time, the rate of acetate-promoted enzymatic U(VI) reduction was greater in the presence of added bicarbonate in spite of the increased dominance of Ca-uranyl-carbonato aqueous complexes. A model-simulated peak rate of U(VI) reduction was similar to 3.8 times higher during acetate-bicarbonate treatment than under acetate-only conditions. Lack of consistent differences in microbial community structure between acetate-bicarbonate and acetate-only treatments suggest that a significantly higher rate of U(VI) reduction in the bicarbonate-impacted sediment may be due to a higher intrinsic rate of microbial reduction induced by elevated concentrations of the bicarbonate oxyanion. The findings indicate that bicarbonate amendment may be useful in improving the engineered bioremediation of uranium in aquifers. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Long, Philip E.; Williams, Kenneth H.; Davis, James A.; Fox, Patricia M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Wilkins, Michael J.; Yabusaki, Steven B.; Fang, Yilin; Waichler, Scott R.; Murray, Chris] Pacific NW Natl Lab, Richland, WA 99352 USA. [Berman, Elena S. F.; Gupta, Manish] Los Gatos Res, Mountain View, CA 94041 USA. [Chandler, Darrell P.] Akonni Biosyst Inc, Frederick, MD 21701 USA. [Peacock, Aaron D.] Haley & Aldrich Inc, Greenville, SC 29601 USA. [Giloteaux, Ludovic] Cornell Univ, Dept Mol Biol & Genet, Ithaca, NY 14853 USA. [Handley, Kim M.; Banfield, Jillian F.] Univ Calif Berkeley, Berkeley, CA USA. [Lovley, Derek R.] Univ Massachusetts, Dept Microbiol, Amherst, MA 01003 USA. RP Long, PE (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM pelong@lbl.gov RI Fox, Patricia/I-2208-2014; Davis, James/G-2788-2015; Williams, Kenneth/O-5181-2014; Fang, Yilin/J-5137-2015; Giloteaux, Ludovic/L-6986-2015; Wilkins, Michael/A-9358-2013; Long, Philip/F-5728-2013 OI Fox, Patricia/0000-0002-5264-1876; Handley, Kim/0000-0003-0531-3009; Williams, Kenneth/0000-0002-3568-1155; Long, Philip/0000-0003-4152-5682 FU Office of Science, Biological and Environmental Research, Subsurface Biogeochemistry Program of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Director, Office of Science, Biological and Environmental Research, Subsurface Biogeochemistry Program of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We thank the entire Rifle, Colorado Integrated Field Challenge (IFRC) team for their contributions to the Super 8 Experiment, including the U.S. Department of Energy, Grand Junction Office for their excellent field support. We also thank Jason Greenwood for assistance with Fig. 1, Roelof Versteeg for help with uploading data to Pangaea, and anonymous Reviewer #2 for extensive, detailed and very helpful comments that significantly improved the manuscript. NR 77 TC 16 Z9 16 U1 4 U2 53 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD FEB 1 PY 2015 VL 150 BP 106 EP 124 DI 10.1016/j.gca.2014.11.013 PG 19 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AZ9DH UT WOS:000348511300007 ER PT J AU Deditius, AP Smith, FN Utsunomiya, S Ewing, RC AF Deditius, Artur P. Smith, Frances N. (Skomurski) Utsunomiya, Satoshi Ewing, Rodney C. TI Role of vein-phases in nanoscale sequestration of U, Nb, Ti, and Pb during the alteration of pyrochlore SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID NUCLEAR-WASTE GLASSES; GROUP MINERALS; HYDROTHERMAL ALTERATION; GEOCHEMICAL ALTERATION; RADIATION-DAMAGE; HETEROGENEOUS REDUCTION; CRYSTALLINE PYROCHLORE; GRENVILLE PROVINCE; AQUEOUS ALTERATION; DOPED ZIRCONOLITE AB Grains of pyrochlore and secondary phases from tailings of Silver Crater Mine in Bancroft, Ontario (Canada) have been studied to understand the alteration processes, redox conditions, and retention of pyrochlore-derived species (U, Ti, Nb, Pb, Ta, REE) in near-field environments. Alteration processes are documented by the formation of two types of co-existing secondary veins associated with primary apatite and calcite: (i) amorphous Fe-rich veins, 46-75 wt.% of FeO, and similar to 500 ppm of UO2, and (ii) crystalline calcite-rich veins, found in fractures and penetrating the pyrochlore. Based on electron microprobe analysis (EMPA), the chemical composition of the pyrochlore is: (Ca(0.84)U(0.35)Fe(0.20)Na(0.09)Pb(0.04)Ln(0.04)Mn(0.03)Sr(0.01)Th(0.01) Mg-0.01)(1.62)(Nb1.00Ti0.87Ta0.10Si0.02)(2.0)O6.5F0.14. Elemental mapping revealed that migration of liberated U, Pb, Nb, Ta, Ti, and REE, is confined to the secondary veins of Fe-rich and calcite-rich compositions. Transmission electron microscopy (TEM), high-angle annular dark-field scanning TEM (HAADF-STEM), energy dispersive spectroscopy (EDS), and electron energy loss spectroscopy (EELS) results showed that pyrochlore contains nanoparticulate inclusions of uraninite, galena, and magnetite, while secondary veins host betafite, magnetite, Pb-0, cerusite, and 10 angstrom mica nanoparticles (NPs). Randomly oriented uraninite NPs, 15 nm in size, concentrate around pores, 50-100 nm in size, in the pyrochlore. In the Fe-rich veins, HAADF-STEM images revealed that U, Pb, Nb, and Ti were sequestered in the form of spherical betafite NPs, <800 nm in size, with composition: (Ca1.1Fe0.35Pb0.28U0.09)(1.83)(Ti1.56Nb0.44)(2.0)O-6.1. The association of betafite NPs, magnetite, and Pb-0 NPs in Fe-rich and calcite-rich veins indicates reducing conditions during alteration of pyrochlore and immobilization of pyrochlore derived elements. This observation combined with identification of nanoscale galena and magnetite in pyrochlore, and the association of Pb-0 and Fe3O4 in veins, indicate relatively low fS(2) and fO(2) conditions during pyrochlore alteration. In spite of prolonged exposure (>= 20 years) to atmospheric conditions, pyrochlore and betafite NPs retained <25 wt.% and <6 wt.% of UO2, respectively; and no secondary uranyl phases were observed. The alteration of pyrochlore most likely began with metamictization, followed by volume swelling, fracturing and surface interactions with fluids that caused mobilization of major and minor elements. The occurrence of amorphous Fe-rich material on the surface of the pyrochlore suggests that amorphous gels could form in Fe-rich environments as an alteration product of crystalline waste forms. The nano-geochemical complexity of the samples investigated here suggests that there is a significant nano-scale component to the sequestration of actinides during the alteration of natural and likely synthetic materials. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Deditius, Artur P.] Murdoch Univ, Sch Engn & Informat Technol, Murdoch, WA 6150, Australia. [Deditius, Artur P.] Graz Univ Technol, Inst Appl Geosci, A-8010 Graz, Austria. [Smith, Frances N. (Skomurski)] Pacific NW Natl Lab, Nucl Chem & Engn Grp, Richland, WA 99352 USA. [Utsunomiya, Satoshi] Kyushu Univ, Dept Chem, Higashi Ku, Fukuoka 8128581, Japan. [Ewing, Rodney C.] Stanford Univ, Dept Geol & Environm Sci, Stanford, CA 94305 USA. RP Deditius, AP (reprint author), Murdoch Univ, Sch Engn & Informat Technol, Murdoch, WA 6150, Australia. EM A.Deditius@murdoch.edu.au; frances.smith@pnnl.gov; utsunomiya.satoshi.998@m.kyushu-u.ac.jp; rewing1@stanford.edu RI U-ID, Kyushu/C-5291-2016 FU U.S. Department of Energy Office of Science, Office of Basic Energy Sciences Energy Frontier Research Centers program [DE-SC0001089]; JSPS [24540516, 20840035, 24340132]; EMPA analyses [EAR-9911352] FX The authors are indebted to three anonymous reviewers and Associate Editor Chris Kim for their insightful comments that greatly improved the manuscript. R.C.E. was supported by the U.S. Department of Energy Office of Science, Office of Basic Energy Sciences Energy Frontier Research Centers program under Award Number DE-SC0001089. S.U. is thankful to JSPS KAKENHI Grant Numbers 24540516, 20840035 and 24340132; the EMPA analyses were supported by #EAR-9911352. The authors are grateful to Carl Henderson for help with EMPA analyses conducted at the Electron Microbeam Analysis Laboratory (EMAL) at the University of Michigan. NR 79 TC 2 Z9 2 U1 7 U2 47 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD FEB 1 PY 2015 VL 150 BP 226 EP 252 DI 10.1016/j.gca.2014.11.024 PG 27 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AZ9DH UT WOS:000348511300014 ER PT J AU Medina, R Elkhoury, JE Morris, JP Prioul, R Desroches, J Detwiler, RL AF Medina, R. Elkhoury, J. E. Morris, J. P. Prioul, R. Desroches, J. Detwiler, R. L. TI Flow of concentrated suspensions through fractures: small variations in solid concentration cause significant in-plane velocity variations SO GEOFLUIDS LA English DT Article DE fracture; granular; non-Newtonian; rheology; suspension ID 2-DIMENSIONAL CHANNEL FLOW; FLUID-FLOW; TRANSPORT; SYSTEMS; MOTION AB Flow of high-concentration suspensions through fractures is important to a range of natural and induced subsurface processes where fractures provide the primary permeability (e.g., mud volcanoes, sand intrusion, and hydraulic fracturing). For these flows, the simple linear relationship between pressure gradient and flow rate, which applies for viscous-dominated flows of Newtonian fluids, breaks down. We present results from experiments in which a high concentration (50% by volume) of granular solids suspended in a non-Newtonian carrier fluid (0.75% guar gum in water) flowed through a parallel-plate fracture. Digital imaging and particle-image-velocimetry analysis provided detailed two-dimensional maps of velocities within the fracture. Results demonstrate development of a strongly heterogeneous velocity field within the fracture. Surprisingly, we observed the highest velocities along the no-flow boundaries of the fracture and the lowest velocities along the centerline of the fracture. Depth-averaged simulations using a recently developed model of the rheology of concentrated suspensions of monodisperse solids in Newtonian carrier fluids reproduced experimental observations of pressure gradient versus flow rate. Results from additional simulations suggest that small (3%) variations in solid concentration within the fracture can lead to significant (factor of two) velocity variations within the fracture yet negligible changes in observed pressure gradients. Furthermore, the variations in solid concentration persist over the length of the fracture, suggesting that such heterogeneities may play a significant role in the transport of concentrated suspensions. Our results suggest that a simple fracture-averaged conductivity does not adequately represent the transport of suspended solids through fractures, which has direct implications for subsurface suspension flows where small concentration variations are likely. C1 [Medina, R.; Elkhoury, J. E.; Detwiler, R. L.] Univ Calif Irvine, Dept Civil & Environm Engn, Irvine, CA 92617 USA. [Elkhoury, J. E.; Morris, J. P.; Prioul, R.] Schlumberger Doll Res Ctr, Cambridge, MA USA. [Morris, J. P.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Desroches, J.] Serv Petroliers Schlumberger, Paris, France. RP Detwiler, RL (reprint author), Univ Calif Irvine, Dept Civil & Environm Engn, 844C Engn Tower, Irvine, CA 92617 USA. EM detwiler@uci.edu RI Detwiler, Russell/C-3228-2008; OI Detwiler, Russell/0000-0002-7693-9271; Desroches, Jean/0000-0001-6002-8388 FU Schlumberger FX The authors would like to thank Schlumberger for sponsoring this research and Luke Shannon for his assistance with developing the experimental system. NR 31 TC 2 Z9 2 U1 6 U2 18 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1468-8115 EI 1468-8123 J9 GEOFLUIDS JI Geofluids PD FEB PY 2015 VL 15 IS 1-2 SI SI BP 24 EP 36 DI 10.1111/gfl.12109 PG 13 WC Geochemistry & Geophysics; Geology SC Geochemistry & Geophysics; Geology GA AZ9BC UT WOS:000348505200003 ER PT J AU Rutqvist, J AF Rutqvist, J. TI Fractured rock stress-permeability relationships from in situ data and effects of temperature and chemical-mechanical couplings SO GEOFLUIDS LA English DT Article DE chemical and mechanical coupling; fractured rock; in situ experiments; permeabilty and stress; temperature ID EXCAVATION DAMAGED ZONE; NEAR-FIELD SAFETY; NORMAL STIFFNESS; YUCCA MOUNTAIN; FLUID-FLOW; SLUG TESTS; WELL TESTS; GRANITE; REPOSITORY; INJECTION AB The purpose of this paper is to (i) review field data on stress-induced permeability changes in fractured rock; (ii) describe estimation of fractured rock stress-permeability relationships through model calibration against such field data; and (iii) discuss observations of temperature and chemically mediated fracture closure and its effect on fractured rock permeability. The field data that are reviewed include in situ block experiments, excavation-induced changes in permeability around tunnels, borehole injection experiments, depth (and stress) dependent permeability, and permeability changes associated with a large-scale rock-mass heating experiment. Data show how the stress-permeability relationship of fractured rock very much depends on local in situ conditions, such as fracture shear offset and fracture infilling by mineral precipitation. Field and laboratory experiments involving temperature have shown significant temperature-driven fracture closure even under constant stress. Such temperature-driven fracture closure has been described as thermal overclosure and relates to better fitting of opposing fracture surfaces at high temperatures, or is attributed to chemically mediated fracture closure related to pressure solution (and compaction) of stressed fracture surface asperities. Back-calculated stress-permeability relationships from field data may implicitly account for such effects, but the relative contribution of purely thermal-mechanical and chemically mediated changes is difficult to isolate. Therefore, it is concluded that further laboratory and in situ experiments are needed to increase the knowledge of the true mechanisms behind thermally driven fracture closure, and to further assess the importance of chemical-mechanical coupling for the long-term evolution of fractured rock permeability. C1 Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Rutqvist, J (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM Jrutqvist@lbl.gov RI Rutqvist, Jonny/F-4957-2015 OI Rutqvist, Jonny/0000-0002-7949-9785 FU Swedish Radiation Safety Authority (SSM) [DE-AC02-05CH11231] FX This paper was prepared with funds from the Swedish Radiation Safety Authority (SSM) to the Lawrence Berkeley National Laboratory through the U.S. Department of Energy Contract No. DE-AC02-05CH11231. Technical review comments of the initial manuscript by Victor Vilarrasa and editorial review by Dan Hawkes of the Lawrence Berkeley National Laboratory are greatly appreciated. Technical and editorial reviews for the journal publication by Steven Micklethwaite, University of Western Australia, and by Steve Ingebritsen, U.S. Geological Survey, substantially improved the manuscript and are greatly appreciated by the author. NR 80 TC 14 Z9 15 U1 3 U2 45 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1468-8115 EI 1468-8123 J9 GEOFLUIDS JI Geofluids PD FEB PY 2015 VL 15 IS 1-2 SI SI BP 48 EP 66 DI 10.1111/gfl.12089 PG 19 WC Geochemistry & Geophysics; Geology SC Geochemistry & Geophysics; Geology GA AZ9BC UT WOS:000348505200005 ER PT J AU Burns, ER Williams, CF Ingebritsen, SE Voss, CI Spane, FA Deangelo, J AF Burns, E. R. Williams, C. F. Ingebritsen, S. E. Voss, C. I. Spane, F. A. Deangelo, J. TI Understanding heat and groundwater flow through continental flood basalt provinces: insights gained from alternative models of permeability/depth relationships for the Columbia Plateau, USA SO GEOFLUIDS LA English DT Article DE advection; advective heat transport; anisotropy; conduction-dominated; flood basalts; heat flow; hydrothermal alteration; permeability; regional groundwater flow ID SPRING-DOMINATED STREAMS; MOUNTAINOUS TERRAIN; OREGON CASCADES; SYSTEMS; CONSTRAINTS; STRATIGRAPHY; VOLCANO; HAWAII; WATER; HOLE AB Heat-flow mapping of the western USA has identified an apparent low-heat-flow anomaly coincident with the Columbia Plateau Regional Aquifer System, a thick sequence of basalt aquifers within the Columbia River Basalt Group (CRBG). A heat and mass transport model (SUTRA) was used to evaluate the potential impact of groundwater flow on heat flow along two different regional groundwater flow paths. Limitedin situ permeability (k) data from the CRBG are compatible with a steep permeability decrease (approximately 3.5 orders of magnitude) at 600-900m depth and approximately 40 degrees C. Numerical simulations incorporating this permeability decrease demonstrate that regional groundwater flow can explain lower-than-expected heat flow in these highly anisotropic (k(x)/k(z)similar to 10(4)) continental flood basalts. Simulation results indicate that the abrupt reduction in permeability at approximately 600m depth results in an equivalently abrupt transition from a shallow region where heat flow is affected by groundwater flow to a deeper region of conduction-dominated heat flow. Most existing heat-flow measurements within the CRBG are from shallower than 600m depth or near regional groundwater discharge zones, so that heat-flow maps generated using these data are likely influenced by groundwater flow. Substantialkdecreases at similar temperatures have also been observed in the volcanic rocks of the adjacent Cascade Range volcanic arc and at Kilauea Volcano, Hawaii, where they result from low-temperature hydrothermal alteration. C1 [Burns, E. R.] US Geol Survey, Portland, OR 97201 USA. [Williams, C. F.; Ingebritsen, S. E.; Voss, C. I.; Deangelo, J.] US Geol Survey, Menlo Pk, CA 94025 USA. [Spane, F. A.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Burns, ER (reprint author), US Geol Survey, 2130 SW 5th Ave, Portland, OR 97201 USA. EM eburns@usgs.gov OI Burns, Erick/0000-0002-1747-0506 FU US Department of Energy - Geothermal Technologies Program; USGS Energy Resources Program FX Dave Norman, Jeff Bowman, and Jessica Czajkowski (all from the Washington State Department of Natural Resources) provided new data to augment the USGS geothermal data base. Alden Provost (USGS Reston) provided the new version of SUTRA for use in this study, altering the code to ensure matrix singularities did not occur in the deep (heat conduction only) part of the domain. He was also a wonderful resource when considering how to best apply the new general head boundary conditions. Jonathan Haynes (USGS Oregon Water Science Center) provided geologic model GIS support and figure preparation. Many thanks to reviewers, Ingrid Stober, Ying Fan, and one anonymous reviewer, and editors Mark Person and Tom Gleeson, for the obvious care and many excellent comments and suggestions that resulted in significant improvement of the original manuscript. Funding for this project was provided by the US Department of Energy - Geothermal Technologies Program and the USGS Energy Resources Program. NR 57 TC 3 Z9 3 U1 1 U2 13 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1468-8115 EI 1468-8123 J9 GEOFLUIDS JI Geofluids PD FEB PY 2015 VL 15 IS 1-2 SI SI BP 120 EP 138 DI 10.1111/gfl.12095 PG 19 WC Geochemistry & Geophysics; Geology SC Geochemistry & Geophysics; Geology GA AZ9BC UT WOS:000348505200009 ER PT J AU Howald, T Person, M Campbell, A Lueth, V Hofstra, A Sweetkind, D Gable, CW Banerjee, A Luijendijk, E Crossey, L Karlstrom, K Kelley, S Phillips, FM AF Howald, T. Person, M. Campbell, A. Lueth, V. Hofstra, A. Sweetkind, D. Gable, C. W. Banerjee, A. Luijendijk, E. Crossey, L. Karlstrom, K. Kelley, S. Phillips, F. M. TI Evidence for long timescale (> 10(3) years) changes in hydrothermal activity induced by seismic events SO GEOFLUIDS LA English DT Article DE fault; hydrothermal; oxygen isotope; permeability; sinter ID OXYGEN-ISOTOPE FRACTIONATION; YELLOWSTONE-NATIONAL-PARK; SILICEOUS SINTER DEPOSIT; NORTH-CENTRAL NEVADA; CHI-CHI EARTHQUAKE; FLUID-FLOW; GROUNDWATER-FLOW; UNITED-STATES; TEMPERATURE-CHANGES; GEOTHERMAL SYSTEMS AB The pollen C-14 age and oxygen isotopic composition of siliceous sinter deposits from the former Beowawe geyser field reveal evidence of two hydrothermal discharge events that followed relatively low-magnitude (10(-11)m(2)) following each earthquake. However, the timescale for onset of thermal convection implied by an overturned temperature profile in a geothermal well 300m from the Malpais fault is much shorter: 200-1000years. We speculate that individual segments of the Malpais fault become clogged on shorter timescales and that upward flow of groundwater subsequently follows new routes to the surface. C1 [Howald, T.; Person, M.; Campbell, A.; Phillips, F. M.] New Mexico Inst Min & Technol, Socorro, NM 87801 USA. [Lueth, V.; Kelley, S.] New Mexico Bur Geol & Mineral Resources, Socorro, NM USA. [Hofstra, A.; Sweetkind, D.] US Geol Survey, Denver, CO 80225 USA. [Gable, C. W.] Los Alamos Natl Lab, Los Alamos, NM USA. [Banerjee, A.] Indian Stat Inst, Kolkata, India. [Luijendijk, E.] Univ Gottingen, D-37073 Gottingen, Germany. [Crossey, L.; Karlstrom, K.] Univ New Mexico, Albuquerque, NM 87131 USA. RP Person, M (reprint author), New Mexico Inst Min & Technol, Socorro, NM 87801 USA. EM mpersonaustinperson@gmail.com RI Banerjee, Amlan/P-9658-2016; OI Banerjee, Amlan/0000-0002-2065-1391; Gable, Carl/0000-0001-7063-0815; Crossey, Laura/0000-0001-6237-8023 FU NSF [NSF-EAR 0809644]; National Science Foundation (EPSCoR) [IIA-1301346] FX We thank Andy Manning of the USGS and two anonymous reviewers for their constructive criticism of an earlier draft of this manuscript. This work was supported by a NSF grant to Mark Person and Albert Hofstra (NSF-EAR 0809644). We also acknowledge support under a National Science Foundation (EPSCoR) under Grant No. IIA-1301346 to Mark Person and Laura Crossey. NR 86 TC 3 Z9 3 U1 1 U2 10 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1468-8115 EI 1468-8123 J9 GEOFLUIDS JI Geofluids PD FEB PY 2015 VL 15 IS 1-2 SI SI BP 252 EP 268 DI 10.1111/gfl.12113 PG 17 WC Geochemistry & Geophysics; Geology SC Geochemistry & Geophysics; Geology GA AZ9BC UT WOS:000348505200016 ER PT J AU Arribas, AP Shang, F Krishnamurthy, M Shenai, K AF Arribas, Alejandro Pozo Shang, Fei Krishnamurthy, Mahesh Shenai, Krishna TI Simple and Accurate Circuit Simulation Model for SiC Power MOSFETs SO IEEE TRANSACTIONS ON ELECTRON DEVICES LA English DT Article DE Circuit model; dc-dc converter; efficiency; power MOSFET; Schottky diode; silicon carbide (SiC); synchronous operation AB Simple and accurate circuit simulation models for high-voltage silicon carbide power MOSFETs and Schottky barrier diodes are presented and validated. The models are physics-based and consist of minimal number of model parameters that can be easily extracted from simple static I-V and C-V measurements. The models are used in a buck-boost bidirectional dc-dc converter, with and without an antiparallel Schottky diode. The efficiency of the converter was analyzed for synchronous and nonsynchronous operation of the switches. An optimal selection of the antiparallel Schottky diode is proposed to minimize the cost of the converter without compromising its efficiency. C1 [Arribas, Alejandro Pozo; Shang, Fei; Krishnamurthy, Mahesh] IIT, Dept Elect & Comp Engn, Chicago, IL 60616 USA. [Shenai, Krishna] Argonne Natl Lab, Argonne, IL 60439 USA. RP Arribas, AP (reprint author), IIT, Dept Elect & Comp Engn, Chicago, IL 60616 USA. EM apozoarr@hawk.iit.edu; fshang2@hawk.iit.edu; kmahesh@ece.iit.edu; kshenai@yahoo.com FU U.S. Government FX The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the government. NR 16 TC 2 Z9 2 U1 1 U2 11 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0018-9383 EI 1557-9646 J9 IEEE T ELECTRON DEV JI IEEE Trans. Electron Devices PD FEB PY 2015 VL 62 IS 2 BP 449 EP 457 DI 10.1109/TED.2014.2384277 PG 9 WC Engineering, Electrical & Electronic; Physics, Applied SC Engineering; Physics GA AZ7FZ UT WOS:000348386100027 ER PT J AU Tsai, CL Burkinshaw, BJ Strynadka, NCJ Tainer, JA AF Tsai, Chi-Lin Burkinshaw, Brianne J. Strynadka, Natalie C. J. Tainer, John A. TI The Salmonella Type III Secretion System Virulence Effector Forms a New Hexameric Chaperone Assembly for Export of Effector/Chaperone Complexes SO JOURNAL OF BACTERIOLOGY LA English DT Editorial Material ID ENTEROPATHOGENIC ESCHERICHIA-COLI; IV PILUS STRUCTURE; PROTEIN EXPORT; NEEDLE LENGTH; ATPASE; OLIGOMERIZATION; CONFORMATIONS; ARCHITECTURE; INJECTISOME; APPARATUS AB Bacteria hijack eukaryotic cells by injecting virulence effectors into host cytosol with a type III secretion system (T3SS). Effectors are targeted with their cognate chaperones to hexameric T3SS ATPase at the bacterial membrane's cytosolic face. In this issue of the Journal of Bacteriology, Roblin et al. (P. Roblin, F. Dewitte, V. Villeret, E. G. Biondi, and C. Bompard, J Bacteriol 197:688-698, 2015, http://dx.doi.org/10.1128/JB.02294-14) show that the T3SS chaperone SigE of Salmonella can form hexameric rings rather than dimers when bound to its cognate effector, SopB, implying a novel multimeric association for chaperone/effector complexes with their ATPase. C1 [Tsai, Chi-Lin; Tainer, John A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Burkinshaw, Brianne J.; Strynadka, Natalie C. J.] Univ British Columbia, Dept Biochem & Mol Biol, Vancouver, BC V5Z 1M9, Canada. [Burkinshaw, Brianne J.; Strynadka, Natalie C. J.] Univ British Columbia, Ctr Blood Res, Vancouver, BC V5Z 1M9, Canada. RP Strynadka, NCJ (reprint author), Univ British Columbia, Dept Biochem & Mol Biol, Vancouver, BC V5Z 1M9, Canada. EM ncjs@mail.ubc.ca; JATainer@lbl.gov OI Tsai, Chi-Lin/0000-0002-0365-2405 FU Canadian Institutes of Health Research; NIGMS NIH HHS [R01 GM105404, R01GM105404] NR 33 TC 1 Z9 1 U1 1 U2 19 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0021-9193 EI 1098-5530 J9 J BACTERIOL JI J. Bacteriol. PD FEB PY 2015 VL 197 IS 4 BP 672 EP 675 DI 10.1128/JB.02524-14 PG 4 WC Microbiology SC Microbiology GA AZ5RN UT WOS:000348277600002 PM 25488302 ER PT J AU Drury, JL Jang, Y Taylor-Pashow, KML Elvington, M Hobbs, DT Wataha, JC AF Drury, Jeanie L. Jang, Yoonji Taylor-Pashow, Kathryn M. L. Elvington, Mark Hobbs, David T. Wataha, John C. TI In vitro biological response of micro- and nano-sized monosodium titanates and titanate-metal compounds SO JOURNAL OF BIOMEDICAL MATERIALS RESEARCH PART B-APPLIED BIOMATERIALS LA English DT Article DE titanium oxide; biocompatibility; metal ions; nanoparticles ID TITANIUM-DIOXIDE NANOPARTICLES; SURFACE; CELLS AB Previous studies report that microsized monosodium titanates (MSTs) deliver metal ions and species to mammalian cells and bacteria with cell-specific and metal-specific effects. In this study, we explored the use of MST and a new synthesized nanosized monosodium titanate (nMST) to deliver gold(III), cisplatin, or platinum(IV) to two human cell lines with different population doubling times, in vitro. The effect was measured using a fluorescent mitochondrial activity assay (CellTiter-Blue((R)) Assay). This fluorescence assay was implemented to mitigate optical density measurement errors owing to particulate titanate interference and allowed for the studies to be extended to higher titanate concentrations than previously possible. Overall, native MST significantly (p<0.05) decreased mitochondrial activity of both cell types by 50% at concentrations of >50 mg/L. Native nMST significantly suppressed the rapidly dividing cell line (by 50%) over untreated cultures, but had no effect on the more slowly dividing cells. For both cell types, increased titanate concentrations resulted in increased effects from delivered metals. However, there was no difference in the effect of metal delivered from micro- versus nano-sized MST. (c) 2014 Wiley Periodicals, Inc. J Biomed Mater Res Part B: Appl Biomater, 103B: 254-260, 2015. C1 [Drury, Jeanie L.; Jang, Yoonji; Wataha, John C.] Univ Washington, Sch Dent, Dept Restorat Dent, Seattle, WA 98195 USA. [Taylor-Pashow, Kathryn M. L.; Elvington, Mark; Hobbs, David T.] US DOE, Savannah River Natl Lab, Aiken, SC 29808 USA. RP Drury, JL (reprint author), Univ Washington, Sch Dent, Dept Restorat Dent, Seattle, WA 98195 USA. EM jldrury@u.washington.edu FU Savannah River National Laboratory, Department of Energy [AC71713O]; Spencer Endowment at the University of Washington, School of Dentistry FX Contract grant sponsor: Savannah River National Laboratory, Department of Energy; contract grant number: AC71713O; Contract grant sponsor: The Spencer Endowment at the University of Washington, School of Dentistry NR 20 TC 2 Z9 2 U1 2 U2 10 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1552-4973 EI 1552-4981 J9 J BIOMED MATER RES B JI J. Biomed. Mater. Res. Part B PD FEB PY 2015 VL 103 IS 2 BP 254 EP 260 DI 10.1002/jbm.b.33194 PG 7 WC Engineering, Biomedical; Materials Science, Biomaterials SC Engineering; Materials Science GA AZ7TD UT WOS:000348419700002 PM 24819184 ER PT J AU Vartanian, KB Mitchell, HD Stevens, SL Conrad, VK McDermott, JE Stenzel-Poore, MP AF Vartanian, Keri B. Mitchell, Hugh D. Stevens, Susan L. Conrad, Valerie K. McDermott, Jason E. Stenzel-Poore, Mary P. TI CpG preconditioning regulates miRNA expression that modulates genomic reprogramming associated with neuroprotection against ischemic injury SO JOURNAL OF CEREBRAL BLOOD FLOW AND METABOLISM LA English DT Article DE microRNA; neuroprotection; preconditioning; reprogramming; stroke ID CEREBRAL-ISCHEMIA; HYPOXIA-ISCHEMIA; GENE-EXPRESSION; CELL-DEATH; KAPPA-B; STROKE; BRAIN; TOLERANCE; HIBERNATION; PROTECTS AB Cytosine-phosphate-guanine (CpG) preconditioning reprograms the genomic response to stroke to protect the brain against ischemic injury. The mechanisms underlying genomic reprogramming are incompletely understood. MicroRNAs (miRNAs) regulate gene expression; however, their role in modulating gene responses produced by CpG preconditioning is unknown. We evaluated brain miRNA expression in response to CpG preconditioning before and after stroke using microarray. Importantly, we have data from previous gene microarrays under the same conditions, which allowed integration of miRNA and gene expression data to specifically identify regulated miRNA gene targets. CpG preconditioning did not significantly alter miRNA expression before stroke, indicating that miRNA regulation is not critical for the initiation of preconditioning-induced neuroprotection. However, after stroke, differentially regulated miRNAs between CpG- and saline-treated animals associated with the upregulation of several neuroprotective genes, implicating these miRNAs in genomic reprogramming that increases neuroprotection. Statistical analysis revealed that the miRNA targets were enriched in the gene population regulated in the setting of stroke, implying that miRNAs likely orchestrate this gene expression. These data suggest that miRNAs regulate endogenous responses to stroke and that manipulation of these miRNAs may have the potential to acutely activate novel neuroprotective processes that reduce damage. C1 [Vartanian, Keri B.; Stevens, Susan L.; Conrad, Valerie K.; Stenzel-Poore, Mary P.] Oregon Hlth & Sci Univ, Dept Mol Microbiol & Immunol, Portland, OR 97239 USA. [Mitchell, Hugh D.; McDermott, Jason E.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Stenzel-Poore, MP (reprint author), Oregon Hlth & Sci Univ, Dept Mol Microbiol & Immunol, Portland, OR 97239 USA. EM poorem@ohsu.edu FU NINDS [NS062381]; Collins Medical Trust; [DE-AC05-76RLO-1830] FX This work was supported by funds from NINDS NS062381 and Collins Medical Trust. Portions of this work were undertaken at PNNL, which is operated by Battelle Memorial Institute under contract DE-AC05-76RLO-1830. NR 38 TC 0 Z9 0 U1 3 U2 6 PU NATURE PUBLISHING GROUP PI NEW YORK PA 75 VARICK ST, 9TH FLR, NEW YORK, NY 10013-1917 USA SN 0271-678X EI 1559-7016 J9 J CEREBR BLOOD F MET JI J. Cereb. Blood Flow Metab. PD FEB PY 2015 VL 35 IS 2 BP 257 EP 266 DI 10.1038/jcbfm.2014.193 PG 10 WC Endocrinology & Metabolism; Hematology; Neurosciences SC Endocrinology & Metabolism; Hematology; Neurosciences & Neurology GA CA2QS UT WOS:000348753100013 PM 25388675 ER PT J AU Brown, RA Borst, M AF Brown, Robert A. Borst, Michael TI Evaluation of Surface and Subsurface Processes in Permeable Pavement Infiltration Trenches SO JOURNAL OF HYDROLOGIC ENGINEERING LA English DT Article DE Permeable pavement; Clogging; Pressure transducer; Stormwater control measure; SCM; Green infrastructure; Long-term performance; Infiltration ID STORM-WATER; LOW IMPACT; SYSTEMS; BIORETENTION; TEMPERATURE; PERFORMANCE AB The hydrologic performance of permeable pavement systems can be affected by clogging at the pavement surface and/or clogging at the interface where the subsurface storage layer meets the underlying soil. The objective of this paper was to evaluate changes in infiltration and exfiltration using three pressure transducers installed in piezometers along the length of two, 2.47-m wide, permeable pavement strips. Each system was retrofitted in the parking lane of a curb-and-gutter system in Louisville, Kentucky. The strips received run-on from a drainage area about 20-25 times larger than the paver area. Below each permeable pavement strip (16.8-m and 36.6-m long) was a deep (3.0 m) and narrow (0.6 m) infiltration trench. Piezometers were installed at the bottom of the trench about 1 m from the uphill edge, and at roughly one-third and two-thirds along the permeable paver strips, to measure the rise and fall of water for 13 months. Initially, infiltrating run-on was localized near the uphill edge. During periods with intense runoff, the localized inflow accumulated in the trench faster than it could move laterally creating a measureable subsurface gradient between piezometers. Runoff transported solids to the uphill edge where a portion was filtered and accumulated between the paver blocks. With time, surface clogging progressed along the paver strip past the next piezometer. The localized infiltration caused the subsurface water level gradient between piezometers to reverse. After each event, the exfiltration rate per wetted surface area was calculated for fixed 0.15-m intervals. The exfiltration rate decreased drastically after the first few events. The primary cause of the initial exfiltration rate decline was attributed to infiltrating water rinsing the fine solids attached to the washed aggregate and depositing them at the bottom of the trench. Silt and clay-sized particles (particle size smaller than 75 mu m) accounted for about 1.7-1.8% of the washed aggregate mass. This large source of fine-grained particles from construction materials can be eliminated if cleaner aggregate is available and used. A continued and significant decrease in exfiltration rate with age was measured during year 1 of use. To optimize the design of these systems, a lifecycle analysis incorporating exfiltration rate decline with age should be included. Another item to consider during the design process is the variability of urban soils. Although these sites are across the street from one another, exfiltration rates were markedly different. Installation should be targeted in soils with larger hydraulic conductivities to improve hydrologic performance, so more preconstruction soil borings and soil tests are necessary to characterize the in situ soils. (C) 2014 American Society of Civil Engineers. C1 [Brown, Robert A.] US EPA, Oak Ridge Inst Sci & Educ, Edison, NJ 08837 USA. [Borst, Michael] US EPA, Edison, NJ 08837 USA. RP Brown, RA (reprint author), US EPA, Oak Ridge Inst Sci & Educ, 2890 Woodbridge Ave,MS 104, Edison, NJ 08837 USA. EM Brown.Robert-A@epa.gov; borst.mike@epa.gov FU Research Participation Program at the National Risk Management Research Laboratory FX The research reported in this paper is the result of a collaborative effort among many parties. It was supported in part by an appointment to the Research Participation Program at the National Risk Management Research Laboratory administered by the Oak Ridge Institute for Science and Education (ORISE) through an interagency agreement between the U.S. DOE and U.S. EPA. The writers would like to thank the following parties for their assistance with this project: (1) Louisville and Jefferson County MSD, (2) URS Corporation, (3) University of Louisville Center for Infrastructure Research, and (4) PARS Environmental. The writers would also like to thank Amirhossein Ehsaei, Hamidreza Kazemi, and Joshua Rivard at the CIR for conducting surface infiltration measurements, and providing field assessment documentation. NR 27 TC 1 Z9 1 U1 7 U2 53 PU ASCE-AMER SOC CIVIL ENGINEERS PI RESTON PA 1801 ALEXANDER BELL DR, RESTON, VA 20191-4400 USA SN 1084-0699 EI 1943-5584 J9 J HYDROL ENG JI J. Hydrol. Eng. PD FEB PY 2015 VL 20 IS 2 DI 10.1061/(ASCE)HE.1943-5584.0001016 PG 12 WC Engineering, Civil; Environmental Sciences; Water Resources SC Engineering; Environmental Sciences & Ecology; Water Resources GA AZ1ZN UT WOS:000348034000007 ER PT J AU Besara, T Ramirez, D Sun, J Whalen, JB Tokumoto, TD McGill, SA Singh, DJ Siegrist, T AF Besara, T. Ramirez, D. Sun, J. Whalen, J. B. Tokumoto, T. D. McGill, S. A. Singh, D. J. Siegrist, T. TI Ba2TeO: A new layered oxytelluride SO JOURNAL OF SOLID STATE CHEMISTRY LA English DT Article DE Oxytelluride; Single crystal growth; Single crystal x-ray diffraction; Layered structure; Semiconductor ID TRANSPARENT OXIDE SEMICONDUCTORS; P-TYPE CONDUCTIVITY; CRYSTAL-STRUCTURE; ELECTRONIC-STRUCTURES; OPTOELECTRONIC PROPERTIES; OPTICAL-PROPERTIES; OXYCHALCOGENIDE SEMICONDUCTORS; PHYSICAL-PROPERTIES; DEVICE APPLICATION; SE AB Single crystals of the new semiconducting oxytelluride phase, Ba2TeO, were synthesized from barium oxide powder and elemental tellurium in a molten barium metal flux. Ba2TeO crystallizes in tetragonal symmetry with space group P4/nmm (#129), a = 5.0337(1) angstrom, c = 9.9437(4) angstrom, Z = 2. The crystals were characterized by single crystal x-ray diffraction, heat capacity and optical measurements. The optical measurements along with electronic band structure calculations indicate semiconductor behavior with a band gap of 2.93 eV. Resistivity measurements show that Ba2TeO is highly insulating. (C) 2014 Elsevier Inc. All rights reserved. C1 [Besara, T.; Ramirez, D.; Sun, J.; Whalen, J. B.; Tokumoto, T. D.; McGill, S. A.; Siegrist, T.] Condensed Matter Sci Dept, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. [Ramirez, D.; Sun, J.; Siegrist, T.] Florida State Univ, Florida Agr & Mech Univ, Coll Engn, Dept Chem & Biomed Engn, Tallahassee, FL 32310 USA. [Sun, J.; Singh, D. J.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Whalen, J. B.] Specialized Crystal Proc Inc, Tallahassee, FL 32301 USA. RP Besara, T (reprint author), Condensed Matter Sci Dept, Natl High Magnet Field Lab, 1800 E Paul Dirac Dr, Tallahassee, FL 32310 USA. OI Besara, Tiglet/0000-0002-2143-2254 FU U.S. Department of Energy, Basic Energy Science, Materials Sciences and Engineering Division [DE-SC0008832]; Florida State University; Leon County Research and Development Authority; U.S. Department of Energy, Basic Energy Science, Materials Sciences and Engineering Division, through the ORNL GOI program; National Science Foundation Cooperative Agreement [DMR-1157490]; State of Florida; U.S. Department of Energy FX This work is supported by the U.S. Department of Energy, Basic Energy Science, Materials Sciences and Engineering Division, under award DE-SC0008832. J.B.W. acknowledges support by the State of Florida, Florida State University, and the Leon County Research and Development Authority. Work at the Oak Ridge National Laboratory was supported by the U.S. Department of Energy, Basic Energy Science, Materials Sciences and Engineering Division. J.S. acknowledges a graduate student fellowship, funded by the U.S. Department of Energy, Basic Energy Science, Materials Sciences and Engineering Division, through the ORNL GOI program. A portion of this work was performed at the National High Magnetic Field Laboratory, which is supported by the National Science Foundation Cooperative Agreement # DMR-1157490, the State of Florida, and the U.S. Department of Energy. NR 56 TC 2 Z9 2 U1 2 U2 24 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0022-4596 EI 1095-726X J9 J SOLID STATE CHEM JI J. Solid State Chem. PD FEB PY 2015 VL 222 BP 60 EP 65 DI 10.1016/j.jssc.2014.11.003 PG 6 WC Chemistry, Inorganic & Nuclear; Chemistry, Physical SC Chemistry GA CA0WH UT WOS:000348633800009 ER PT J AU Hammerstrom, TG Horton, LB Swick, MC Joachimiak, A Osipiuk, J Koehler, TM AF Hammerstrom, Troy G. Horton, Lori B. Swick, Michelle C. Joachimiak, Andrzej Osipiuk, Jerzy Koehler, Theresa M. TI Crystal structure of Bacillus anthracis virulence regulator AtxA and effects of phosphorylated histidines on multimerization and activity SO MOLECULAR MICROBIOLOGY LA English DT Article ID GROUP-A STREPTOCOCCUS; ANTITERMINATOR PROTEIN GLCT; PROTECTIVE ANTIGEN GENE; TRANSCRIPTIONAL ANTITERMINATOR; ESCHERICHIA-COLI; TOXIN GENES; EXPRESSION; SUBTILIS; MGA; DNA AB The Bacillus anthracis virulence regulator AtxA controls transcription of the anthrax toxin genes and capsule biosynthetic operon. AtxA activity is elevated during growth in media containing glucose and CO2/bicarbonate, and there is a positive correlation between the CO2/bicarbonate signal, AtxA activity and homomultimerization. AtxA activity is also affected by phosphorylation at specific histidines. We show that AtxA crystallizes as a dimer. Distinct folds associated with predicted DNA-binding domains (HTH1 and HTH2) and phosphoenolpyruvate: carbohydrate phosphotransferase system-regulated domains (PRD1 and PRD2) are apparent. We tested AtxA variants containing single and double phosphomimetic (HisAsp) and phosphoablative (HisAla) amino acid changes for activity in B.anthracis cultures and for protein-protein interactions in cell lysates. Reduced activity of AtxA H199A, lack of multimerization and activity of AtxAH379D variants, and predicted structural changes associated with phosphorylation support a model for control of AtxA function. We propose that (i) in the AtxA dimer, phosphorylation of H199 in PRD1 affects HTH2 positioning, influencing DNA-binding; and (ii) phosphorylation of H379 in PRD2 disrupts dimer formation. The AtxA structure is the first reported high-resolution full-length structure of a PRD-containing regulator, and can serve as a model for proteins of this family, especially those that link virulence to bacterial metabolism. C1 [Hammerstrom, Troy G.; Horton, Lori B.; Swick, Michelle C.; Koehler, Theresa M.] Univ Texas Hlth Sci Ctr Houston, Dept Microbiol & Mol Genet, Houston, TX 77030 USA. [Joachimiak, Andrzej; Osipiuk, Jerzy] Argonne Natl Lab, Ctr Struct Genom Infect Dis, Argonne, IL 60439 USA. [Joachimiak, Andrzej; Osipiuk, Jerzy] Argonne Natl Lab, Struct Biol Ctr, Biosci Div, Argonne, IL 60439 USA. RP Koehler, TM (reprint author), Univ Texas Hlth Sci Ctr Houston, Dept Microbiol & Mol Genet, Houston, TX 77030 USA. EM josipiuk@anl.gov; Theresa.M.Koehler@uth.tmc.edu FU U.S. Department of Energy, Office of Biological and Environmental Research [DE-AC02-06CH11357]; NIAID, NIH, Department of Health and Human Services [HHSN272200700058C, HHSN272201200026C]; National Institute of Allergy and Infectious Diseases [R01 AI033537]; Keck Center Computational and Structural Biology in Biodefense Training Program of the Gulf Coast Consortia (NIH Grant) [1 T32 AI065396] FX Argonne is operated by UChicago Argonne, LLC, for the U.S. Department of Energy, Office of Biological and Environmental Research under contract DE-AC02-06CH11357. Work by A.J. and J.O. was supported by grants from the NIAID, NIH, Department of Health and Human Services, Contracts HHSN272200700058C and HHSN272201200026C. Work by T.M.K., T.G.H, L.B.H. and M.C.S. was supported by Award Number R01 AI033537 from the National Institute of Allergy and Infectious Diseases to T.M.K. T.G.H. was also supported during a portion of this work by a training fellowship from the Keck Center Computational and Structural Biology in Biodefense Training Program of the Gulf Coast Consortia (NIH Grant No. 1 T32 AI065396). The content of this publication is solely the responsibility of the authors and does not necessarily represent the official views of the National Allergy and Infectious Diseases or the National Institutes of Health. NR 71 TC 12 Z9 12 U1 0 U2 3 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0950-382X EI 1365-2958 J9 MOL MICROBIOL JI Mol. Microbiol. PD FEB PY 2015 VL 95 IS 3 BP 426 EP 441 DI 10.1111/mmi.12867 PG 16 WC Biochemistry & Molecular Biology; Microbiology SC Biochemistry & Molecular Biology; Microbiology GA AZ9XM UT WOS:000348567600004 PM 25402841 ER PT J AU Zhu, XJ Liu, J Zhang, WJ AF Zhu, Xuejun Liu, Joyce Zhang, Wenjun TI De novo biosynthesis of terminal alkyne-labeled natural products SO NATURE CHEMICAL BIOLOGY LA English DT Article ID CYANOBACTERIUM LYNGBYA-MAJUSCULA; CARRIER-PROTEIN DESATURASE; FATTY-ACID SYNTHESIS; ANTIMYCIN BIOSYNTHESIS; ESCHERICHIA-COLI; CHEMISTRY; DIVERSIFICATION; POLYKETIDES; FERREDOXIN; DIVERSITY AB The terminal alkyne is a functionality widely used in organic synthesis, pharmaceutical science, material science and bioorthogonal chemistry. This functionality is also found in acetylenic natural products, but the underlying biosynthetic pathways for its formation are not well understood. Here we report the characterization of what is to our knowledge the first carrier protein-dependent terminal alkyne biosynthetic machinery in microbes. We further demonstrate that this enzymatic machinery can be exploited for the in situ generation and incorporation of terminal alkynes into two natural product scaffolds in Escherichia coli. These results highlight the prospect for tagging major classes of natural products, including polyketides and polyketide/nonribosomal peptide hybrids, using biosynthetic pathway engineering. C1 [Zhu, Xuejun; Zhang, Wenjun] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Zhu, Xuejun; Liu, Joyce; Zhang, Wenjun] Univ Calif Berkeley, Energy Biosci Inst, Berkeley, CA 94720 USA. [Liu, Joyce] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Zhang, Wenjun] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Zhang, WJ (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. EM wjzhang@berkeley.edu RI kandula, sivakumar/D-4090-2015 FU Pew Scholars Program; University of California FX This research was financially supported by the Pew Scholars Program and University of California Cancer Research Coordinating Committee funds. We thank I. Abe (University of Tokyo) for providing hspks1, S. Bauer (University of California-Berkeley) for assisting with LC/HRMS analysis, J. Pelton (University of California-Berkeley) for helping with NMR spectroscopic analysis, J. Chung (University of California-Berkeley) for helping with compound purification and L. Zhang (University of California-Berkeley) for providing scACP. NR 42 TC 27 Z9 27 U1 4 U2 61 PU NATURE PUBLISHING GROUP PI NEW YORK PA 75 VARICK ST, 9TH FLR, NEW YORK, NY 10013-1917 USA SN 1552-4450 EI 1552-4469 J9 NAT CHEM BIOL JI Nat. Chem. Biol. PD FEB PY 2015 VL 11 IS 2 BP 115 EP U51 DI 10.1038/NCHEMBIO.1718 PG 8 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA AZ6WN UT WOS:000348358800008 PM 25531891 ER PT J AU Yang, SH Ramirez-Cuesta, AJ Newby, R Garcia-Sakai, V Manuel, P Callear, SK Campbell, SI Tang, CC Schroder, M AF Yang, Sihai Ramirez-Cuesta, Anibal J. Newby, Ruth Garcia-Sakai, Victoria Manuel, Pascal Callear, Samantha K. Campbell, Stuart I. Tang, Chiu C. Schroeder, Martin TI Supramolecular binding and separation of hydrocarbons within a functionalized porous metal-organic framework SO Nature Chemistry LA English DT Article ID SELECTIVE ADSORPTION; NEUTRON-SCATTERING; GAS-ADSORPTION; CARBON-DIOXIDE; ETHYLENE; SITES; DIFFUSION; ZEOLITES; ETHANE; COMBINATION AB Supramolecular interactions are fundamental to host-guest binding in many chemical and biological processes. Direct visualization of such supramolecular interactions within host-guest systems is extremely challenging, but crucial to understanding their function. We report a comprehensive study that combines neutron scattering, synchrotron X-ray and neutron diffraction, and computational modelling to define the detailed binding at a molecular level of acetylene, ethylene and ethane within the porous host NOTT-300. This study reveals simultaneous and cooperative hydrogen-bonding, pi center dot center dot center dot pi stacking interactions and intermolecular dipole interactions in the binding of acetylene and ethylene to give up to 12 individual weak supramolecular interactions aligned within the host to form an optimal geometry for the selective binding of hydrocarbons. We also report the cooperative binding of a mixture of acetylene and ethylene within the porous host, together with the corresponding breakthrough experiments and analysis of adsorption isotherms of gas mixtures. C1 [Yang, Sihai; Newby, Ruth; Schroeder, Martin] Univ Nottingham, Sch Chem, Nottingham NG7 2RD, England. [Ramirez-Cuesta, Anibal J.] Oak Ridge Natl Lab, Neutron Sci Directorate, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Garcia-Sakai, Victoria; Manuel, Pascal; Callear, Samantha K.] STFC Rutherford Appleton Lab, ISIS Neutron Facil, Chilton OX11 0QX, Oxon, England. [Campbell, Stuart I.] Oak Ridge Natl Lab, Neutron Sci Directorate, Neutron Data Anal & Visualizat Div NDAV, Oak Ridge, TN 37831 USA. [Tang, Chiu C.] Diamond Light Source, Didcot OX11 0DE, Oxon, England. RP Yang, SH (reprint author), Univ Nottingham, Sch Chem, Univ Pk, Nottingham NG7 2RD, England. EM sihai.yang@nottingham.ac.uk; m.schroder@nottingham.ac.uk RI Schroder, Martin/I-5432-2013; Ramirez-Cuesta, Timmy/A-4296-2010; Campbell, Stuart/A-8485-2010 OI Schroder, Martin/0000-0001-6992-0700; Ramirez-Cuesta, Timmy/0000-0003-1231-0068; Campbell, Stuart/0000-0001-7079-0878 FU Nottingham Research Fellowship; Leverhulme Trust Early Career Research Fellowship; European Research Council Advanced Grant; Engineering and Physical Sciences Research Council Programme Grant; Office of Science of the US Department of Energy [DE-AC05-00OR22725] FX S.Y. acknowledges receipt of a Nottingham Research Fellowship and a Leverhulme Trust Early Career Research Fellowship, and M.S. the receipt of a European Research Council Advanced Grant and an Engineering and Physical Sciences Research Council Programme Grant. We are especially grateful to STFC and the ISIS Neutron Facility for access to Beamlines TOSCA, WISH, IRIS and the SCARF supercomputer resources, and to Diamond Light Source for access to Beamline I11. We thank C. Goodway and M. Kibble of the user support group at ISIS and J. Potter at Diamond for the technical help with the beamlines. We also thank J. Ke for helpful discussions on the implementation of IAST. This research used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC05-00OR22725. NR 30 TC 54 Z9 54 U1 27 U2 192 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1755-4330 EI 1755-4349 J9 NAT CHEM JI Nat. Chem. PD FEB PY 2015 VL 7 IS 2 BP 121 EP 129 DI 10.1038/nchem.2114 PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA CA0IA UT WOS:000348599600010 ER PT J AU Que, EL Bleher, R Duncan, FE Kong, BY Gleber, SC Vogt, S Chen, S Garwin, SA Bayer, AR Dravid, VP Woodruff, TK O'Halloran, TV AF Que, Emily L. Bleher, Reiner Duncan, Francesca E. Kong, Betty Y. Gleber, Sophie C. Vogt, Stefan Chen, Si Garwin, Seth A. Bayer, Amanda R. Dravid, Vinayak P. Woodruff, Teresa K. O'Halloran, Thomas V. TI Quantitative mapping of zinc fluxes in the mammalian egg reveals the origin of fertilization-induced zinc sparks SO Nature Chemistry LA English DT Article ID CELLS; BIOLOGY; SPERM; TRANSITION; CHEMISTRY; OOCYTES; COPPER; TRAFFICKING; TRANSPORTER; POTENTIALS AB Fertilization of a mammalian egg initiates a series of 'zinc sparks' that are necessary to induce the egg-to-embryo transition. Despite the importance of these zinc-efflux events little is known about their origin. To understand the molecular mechanism of the zinc spark we combined four physical approaches that resolve zinc distributions in single cells: a chemical probe for dynamic live-cell fluorescence imaging and a combination of scanning transmission electron microscopy with energy-dispersive spectroscopy, X-ray fluorescence microscopy and three-dimensional elemental tomography for high-resolution elemental mapping. We show that the zinc spark arises from a system of thousands of zinc-loaded vesicles, each of which contains, on average, 10(6) zinc atoms. These vesicles undergo dynamic movement during oocyte maturation and exocytosis at the time of fertilization. The discovery of these vesicles and the demonstration that zinc sparks originate from them provides a quantitative framework for understanding how zinc fluxes regulate cellular processes. C1 [Que, Emily L.; Bleher, Reiner; Garwin, Seth A.; Bayer, Amanda R.; Woodruff, Teresa K.; O'Halloran, Thomas V.] Northwestern Univ, Chem Life Proc Inst, Evanston, IL 60208 USA. [Bleher, Reiner; Dravid, Vinayak P.] Northwestern Univ, Atom & Nanoscale Characterizat Expt Ctr, Evanston, IL 60208 USA. [Duncan, Francesca E.; Kong, Betty Y.; Woodruff, Teresa K.] Northwestern Univ, Feinberg Sch Med, Dept Obstet & Gynecol, Chicago, IL 60611 USA. [Gleber, Sophie C.; Vogt, Stefan; Chen, Si] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Garwin, Seth A.; Bayer, Amanda R.; Dravid, Vinayak P.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Dravid, Vinayak P.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Woodruff, Teresa K.; O'Halloran, Thomas V.] Northwestern Univ, Dept Mol Biosci, Evanston, IL 60208 USA. RP Woodruff, TK (reprint author), Northwestern Univ, Chem Life Proc Inst, Evanston, IL 60208 USA. EM tkw@northwestern.edu; t-ohalloran@northwestern.edu RI Dravid, Vinayak/B-6688-2009; Vogt, Stefan/B-9547-2009; Vogt, Stefan/J-7937-2013 OI Vogt, Stefan/0000-0002-8034-5513; Vogt, Stefan/0000-0002-8034-5513 FU Argonne National Laboratory [DE-AC02-06CH11357]; Medical Research Award from the W. M. Keck Foundation; SPARK Award from the Chicago Biomedical Consortium; National Institutes of Health [P01 HD021921, GM38784, U54HD076188, T32GM105538] FX The authors thank members of the O'Halloran, Woodruff and Dravid labs for scientific discussions and advice. We thank E. W. Roth for the preparation of electron microscopy samples and J-H. Chung and J. Shangguan for help with chemical syntheses. Equipment and experimental guidance were provided by the following core facilities at Northwestern University: the Integrated Molecular Structure Education and Research Center, the Biological Imaging Facility, the Quantitative Bioelemental Imaging Center, the Electron Probe Instrumentation Centre and the Keck Biophysics Facility. This research used resources of the Advanced Photon Source, a US Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under contract no. DE-AC02-06CH11357. This work was supported by a Medical Research Award from the W. M. Keck Foundation, a SPARK Award from the Chicago Biomedical Consortium and the National Institutes of Health (P01 HD021921, GM38784, U54HD076188 and T32GM105538). NR 55 TC 31 Z9 31 U1 5 U2 55 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1755-4330 EI 1755-4349 J9 NAT CHEM JI Nat. Chem. PD FEB PY 2015 VL 7 IS 2 BP 130 EP 139 DI 10.1038/NCHEM.2133 PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA CA0IA UT WOS:000348599600011 PM 25615666 ER PT J AU Lalkovski, S Kondev, FG AF Lalkovski, S. Kondev, F. G. TI Nuclear Data Sheets for A=112 SO NUCLEAR DATA SHEETS LA English DT Article ID NEUTRON-RICH NUCLEI; HIGH-SPIN STATES; INELASTIC PROTON-SCATTERING; CAPTURE GAMMA-RAYS; EVEN TIN ISOTOPES; A-SIMILAR-TO-100 FISSION FRAGMENTS; OCTUPOLE COUPLED STATES; MASS CADMIUM ISOTOPES; MEV POLARIZED PROTONS; ION-INDUCED FISSION AB Evaluated nuclear structure and decay data for all nuclei within the A=112 mass chain are presented. The experimental data are evaluated and best values for level and gamma ray energies, quantum numbers, lifetimes, gamma ray intensities, and other nuclear properties are recommended. Inconsistencies and discrepancies that exist in the literature are noted. This work supersedes the earlier evaluation by D.De Frenne and E.Jacobs (1996De55), published in Nuclear Data Sheets 79, 639 (1996). C1 [Lalkovski, S.] Univ Sofia, Fac Phys, Sofia 1164, Bulgaria. [Kondev, F. G.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. RP Lalkovski, S (reprint author), Univ Sofia, Fac Phys, 5 James Bourchier Blvd, Sofia 1164, Bulgaria. FU U.S. Department of Energy, Office of Science [DE-AC02-06CH11357]; U.S. Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357]; Nuclear Data Section, IAEA [15994/R0] FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics under contract No. DE-AC02-06CH11357. SL acknowledges support from the Nuclear Data Section, IAEA under contract 15994/R0. NR 403 TC 2 Z9 2 U1 0 U2 3 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD FEB PY 2015 VL 124 BP 157 EP 412 DI 10.1016/j.nds.2014.12.046 PG 256 WC Physics, Nuclear SC Physics GA AZ6NI UT WOS:000348335900002 ER PT J AU Lyons, JA Marcum, WR Morrell, S Dehart, M AF Lyons, Jennifer A. Marcum, Wade R. Morrell, Sean Dehart, Mark TI REACTOR PHYSICS SCOPING AND CHARACTERIZATION STUDY ON IMPLEMENTATION OF TRIGA FUEL IN THE ADVANCED TEST REACTOR SO NUCLEAR TECHNOLOGY LA English DT Article DE reactor physics; core design; Advanced Test Reactor AB The Advanced Test Reactor (ATR) is conducting scoping studies for the conversion of its fuel from a highly enriched uranium (HEU) composition to a low-enriched uranium (LEU) composition, through the Reduced Enrichment for Research and Test Reactors Program, within the Global Threat Reduction Initiative. These studies have considered a wide variety of LEU plate-type fuels to replace the current HEU fuel. Continuing to investigate potential alternatives to the present HEU fuel form, this study presents a preliminary reactor physics scoping and feasibility analysis of TRIGA fuel within the current ATR fuel element envelope and compares it to the functional requirements delineated by the Naval Reactors Program, which includes >4.8 x 10(14) fissions/s.g(-1) of U-235 in test positions, a fast to thermal neutron flux ratio that has a <5% deviation from its current value, a desired steady cycle power within the corner lobes, and an operational cycle length of 56 days at 120 MW. Other design parameters outside those put forth by the Naval Reactors Program that are investigated herein include axial and radial power profiles, effective delayed neutron fraction, and mean neutron generation time. The result of this study demonstrates potential promise for implementation of TRIGA fuel in the ATR from a reactor physics perspective; discussion of observations and limitations are provided herein. C1 [Lyons, Jennifer A.] Pacific Northwest Natl Lab, Richland, WA 99354 USA. [Marcum, Wade R.] Oregon State Univ, Dept Nucl Engn, Corvallis, OR 97331 USA. [Morrell, Sean; Dehart, Mark] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Marcum, WR (reprint author), Oregon State Univ, Dept Nucl Engn, 116 Radiat Ctr, Corvallis, OR 97331 USA. EM wade.marcum@oregonstate.edu NR 37 TC 0 Z9 0 U1 1 U2 4 PU AMER NUCLEAR SOC PI LA GRANGE PK PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA SN 0029-5450 EI 1943-7471 J9 NUCL TECHNOL JI Nucl. Technol. PD FEB PY 2015 VL 189 IS 2 BP 202 EP 217 PG 16 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CA0WA UT WOS:000348633100009 ER PT J AU Plucinski, KJ Sabov, M Fedorchuk, AO Barchiy, I Lakshminarayana, G Filep, M AF Plucinski, K. J. Sabov, M. Fedorchuk, A. O. Barchiy, I. Lakshminarayana, G. Filep, M. TI UV laser induced second order optical effects in the Tl4PbTe3, Tl4SnSe3 and Tl4PbSe3 single crystals SO OPTICAL AND QUANTUM ELECTRONICS LA English DT Article DE Optoelectronic materials; Electrooptical effect; DFT simulations ID 2ND-HARMONIC GENERATION; ZNO FILMS; ELECTROOPTICS; ABSORPTION; GLASSES AB In this work, following the crystallochemical analysis and electronic structural parameters of and single crystals, we predicted and experimentally demonstrated the second harmonic generation (SHG) and electrooptics effects for them. Photoinduced changes were performed by using the 7 ns UV nitrogen laser at wavelength 337 nm. The parameters of the SHG were determined through probing in to the reflected regime at wavelength of the 532 nm. The dependence of the output SHG versus photoinducing power density is studied. Explanation of the observed effect is given within a framework of the quantum chemical DFT simulations. C1 [Plucinski, K. J.] Mil Univ Technol, Dept Elect, PL-00908 Warsaw, Poland. [Sabov, M.; Barchiy, I.; Filep, M.] Uzhgorod State Univ, Dept Phys, UA-294000 Uzhgorod, Ukraine. [Fedorchuk, A. O.] Lviv Natl Univ Vet Med & Biotechnol, Dept Inorgan & Organ Chem, UA-79010 Lvov, Ukraine. [Lakshminarayana, G.] Los Alamos Natl Lab, Mat Sci & Technol Div MST 7, Los Alamos, NM 87545 USA. [Fedorchuk, A. O.] Natl Acad Sci Ukraine, Dept Phys Chem Fossil Fuels InPOCC, UA-79053 Lvov, Ukraine. RP Fedorchuk, AO (reprint author), Lviv Natl Univ Vet Med & Biotechnol, Dept Inorgan & Organ Chem, Pekarska St 50, UA-79010 Lvov, Ukraine. EM ft.1958@yahoo.co.uk RI Sabov, Marjan/J-8608-2015 NR 18 TC 0 Z9 0 U1 1 U2 16 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0306-8919 EI 1572-817X J9 OPT QUANT ELECTRON JI Opt. Quantum Electron. PD FEB PY 2015 VL 47 IS 2 BP 185 EP 192 DI 10.1007/s11082-014-9899-x PG 8 WC Engineering, Electrical & Electronic; Optics SC Engineering; Optics GA AZ6UZ UT WOS:000348357300008 ER PT J AU Imam, S Fitzgerald, CM Cook, EM Donohue, TJ Noguera, DR AF Imam, Saheed Fitzgerald, Colin M. Cook, Emily M. Donohue, Timothy J. Noguera, Daniel R. TI Quantifying the effects of light intensity on bioproduction and maintenance energy during photosynthetic growth of Rhodobacter sphaeroides SO PHOTOSYNTHESIS RESEARCH LA English DT Article DE Photosynthesis; Maintenance energy; Rhodobacter sphaeroides; Metabolic modeling; Bioenergetics; Hydrogen ID SCALE METABOLIC RECONSTRUCTION; RHODOPSEUDOMONAS-CAPSULATA; HYDROGEN-PRODUCTION; GENOME; MEMBRANE; BACTERIUM; MODELS; BACTERIOCHLOROPHYLL; DIFFERENTIATION; OPTIMALITY AB Obtaining a better understanding of the physiology and bioenergetics of photosynthetic microbes is an important step toward optimizing these systems for light energy capture or production of valuable commodities. In this work, we analyzed the effect of light intensity on bioproduction, biomass formation, and maintenance energy during photoheterotrophic growth of Rhodobacter sphaeroides. Using data obtained from steady-state bioreactors operated at varying dilution rates and light intensities, we found that irradiance had a significant impact on biomass yield and composition, with significant changes in photopigment, phospholipid, and biopolymer storage contents. We also observed a linear relationship between incident light intensity and H-2 production rate between 3 and 10 W m(-2), with saturation observed at 100 W m(-2). The light conversion efficiency to H-2 was also higher at lower light intensities. Photosynthetic maintenance energy requirements were also significantly affected by light intensity, with links to differences in biomass composition and the need to maintain redox homeostasis. Inclusion of the measured condition-dependent biomass and maintenance energy parameters and the measured photon uptake rate into a genome-scale metabolic model for R. sphaeroides (iRsp1140) significantly improved its predictive performance. We discuss how our analyses provide new insights into the light-dependent changes in bioenergetic requirements and physiology during photosynthetic growth of R. sphaeroides and potentially other photosynthetic organisms. C1 [Imam, Saheed] Univ Wisconsin, Program Cellular & Mol Biol, Madison, WI USA. [Imam, Saheed; Donohue, Timothy J.] Univ Wisconsin Madison, Wisconsin Energy Inst, Dept Bacteriol, Madison, WI 53726 USA. [Imam, Saheed; Fitzgerald, Colin M.; Donohue, Timothy J.; Noguera, Daniel R.] Univ Wisconsin, DOE Great Lakes Bioenergy Res Ctr, Madison, WI USA. [Fitzgerald, Colin M.; Cook, Emily M.; Noguera, Daniel R.] Univ Wisconsin, Dept Civil & Environm Engn, Madison, WI 53706 USA. RP Noguera, DR (reprint author), Univ Wisconsin, Dept Civil & Environm Engn, Madison, WI 53706 USA. EM noguera@engr.wisc.edu OI Donohue, Timothy/0000-0001-8738-2467 FU Department of Energy, Office of Science, Great Lakes Bioenergy Research Center [DE-FC02-07ER64494]; Genomics:GTL Program [DE-FG02-04ER25627]; Genomics: SciDAC Program [DE-FG02-04ER25627]; University of Wisconsin-Madison Bacteriology Department FX This work was funded in part by the Department of Energy, Office of Science, Great Lakes Bioenergy Research Center (DE-FC02-07ER64494), and the Genomics:GTL and SciDAC Programs (DE-FG02-04ER25627). SI was supported during part of this work by a William H. Peterson Predoctoral Fellowship from the University of Wisconsin-Madison Bacteriology Department. NR 54 TC 3 Z9 3 U1 0 U2 34 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0166-8595 EI 1573-5079 J9 PHOTOSYNTH RES JI Photosynth. Res. PD FEB PY 2015 VL 123 IS 2 BP 167 EP 182 DI 10.1007/s11120-014-0061-1 PG 16 WC Plant Sciences SC Plant Sciences GA AZ7DM UT WOS:000348378700006 PM 25428581 ER PT J AU Rappaport, F Malnoe, A Govindjee AF Rappaport, Fabrice Malnoe, Alizee Govindjee TI Gordon research conference on photosynthesis: from evolution of fundamental mechanisms to radical re-engineering SO PHOTOSYNTHESIS RESEARCH LA English DT Article DE Ute Ambruster; Han Bao; Gordon research conference; Arthur Grossman; David M. Kramer; Nicoletta Liguori; Photosynthesis; Fabrice Rappaport; Anat Shperberg-Avni; Colin A. Wraight AB We provide here a News Report on the 2014 Gordon Research Conference on Photosynthesis, with the subtitle "From Evolution of Fundamental Mechanisms to Radical Re-Engineering." It was held at Mount Snow Resort, West Dover, Vermont, during August 10-15, 2014. After the formal sessions ended, four young scientists (Ute Ambruster of USA; Han Bao of USA; Nicoletta Liguori of the Netherlands; and Anat Shperberg-Avni of Israel) were recognized for their research; they each received a book from one of us (G) in memory of Colin A. Wraight (1945-2014), a brilliant and admired scientist who had been very active in the bioenergetics field in general and in past Gordon Conferences in particular, having chaired the 1988 Gordon Conference on Photosynthesis. (See an article on Wraight by one of us (Govindjee) at http://www.life.illinois.edu/plantbio/Features/ColinWraight/ColinWraight.html.) C1 [Rappaport, Fabrice] Univ Paris 06, Inst Biol Phys Chim, CNRS, UMR 7141, F-75005 Paris, France. [Malnoe, Alizee] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Govindjee] Univ Illinois, Dept Biochem, Dept Plant Biol, Urbana, IL 61801 USA. [Govindjee] Univ Illinois, Ctr Biophys & Quantitat Biol, Urbana, IL 61801 USA. RP Rappaport, F (reprint author), Univ Paris 06, Inst Biol Phys Chim, CNRS, UMR 7141, 13 Rue Pierre & Marie Curie, F-75005 Paris, France. EM fabrice.rappaport@ibpc.fr; alizee.malnoe@berkeley.edu; gov@illinois.edu NR 4 TC 2 Z9 2 U1 1 U2 11 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0166-8595 EI 1573-5079 J9 PHOTOSYNTH RES JI Photosynth. Res. PD FEB PY 2015 VL 123 IS 2 BP 213 EP 223 DI 10.1007/s11120-014-0058-9 PG 11 WC Plant Sciences SC Plant Sciences GA AZ7DM UT WOS:000348378700009 PM 25425217 ER PT J AU Zhang, XB Gou, MY Guo, CR Yang, HJ Liu, CJ AF Zhang, Xuebin Gou, Mingyue Guo, Chunrong Yang, Huijun Liu, Chang-Jun TI Down-Regulation of Kelch Domain-Containing F-Box Protein in Arabidopsis Enhances the Production of (Poly)phenols and Tolerance to Ultraviolet Radiation SO PLANT PHYSIOLOGY LA English DT Article ID PHENYLALANINE AMMONIA-LYASE; PHENYLPROPANOID BIOSYNTHESIS; TRANSGENIC TOBACCO; GENE FAMILY; FLAVONOID BIOSYNTHESIS; FUNCTIONAL-ANALYSIS; REPEAT SUPERFAMILY; CINNAMIC ACID; HUMAN HEALTH; B RADIATION AB Phenylpropanoid biosynthesis in plants engenders myriad phenolics with diverse biological functions. Phenylalanine ammonialyase (PAL) is the first committed enzyme in the pathway, directing primary metabolic flux into a phenylpropanoid branch. Previously, we demonstrated that the Arabidopsis (Arabidopsis thaliana) Kelch domain-containing F-box proteins, AtKFB01, AtKFB20, and AtKFB50, function as the negative regulators controlling phenylpropanoid biosynthesis via mediating PAL's ubiquitination and subsequent degradation. Here, we reveal that Arabidopsis KFB39, a close homolog of AtKFB50, also interacts physically with PAL isozymes and modulates PAL stability and activity. Disturbing the expression of KFB39 reciprocally affects the accumulation/deposition of a set of phenylpropanoid end products, suggesting that KFB39 is an additional posttranslational regulator responsible for the turnover of PAL and negatively controlling phenylpropanoid biosynthesis. Furthermore, we discover that exposure of Arabidopsis to ultraviolet (UV)-B radiation suppresses the expression of all four KFB genes while inducing the transcription of PAL isogenes; these data suggest that Arabidopsis consolidates both transcriptional and posttranslational regulation mechanisms to maximize its responses to UV light stress. Simultaneous down-regulation of all four identified KFBs significantly enhances the production of (poly)phenols and the plant's tolerance to UV irradiation. This study offers a biotechnological approach for engineering the production of useful phenolic chemicals and for increasing a plant's resistance to environmental stress. C1 [Zhang, Xuebin; Gou, Mingyue; Yang, Huijun; Liu, Chang-Jun] Brookhaven Natl Lab, Biol Environm & Climate Sci Dept, Upton, NY 11973 USA. [Guo, Chunrong] Shanxi Agr Univ, Coll Art & Sci, Taigu 030801, Shanxi, Peoples R China. [Yang, Huijun] SUNY Stony Brook, Dept Biochem & Cell Biol, Stony Brook, NY 11972 USA. RP Liu, CJ (reprint author), Brookhaven Natl Lab, Biol Environm & Climate Sci Dept, Upton, NY 11973 USA. EM cliu@bnl.gov RI zhang, xuebin/K-3361-2015 FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy [DEAC0298CH10886]; National Science Foundation [MCB-1051675]; Office of Basic Energy Sciences, U.S. Department of Energy [DEAC0298CH10886] FX This work was supported by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy (grant no. DEAC0298CH10886 to C.-J.L.); H.Y. was supported by the National Science Foundation (grant no. MCB-1051675 to C.-J.L.). The use of the confocal microscope in the Center for Functional Nanomaterials, Brookhaven National Laboratory was supported by the Office of Basic Energy Sciences, U.S. Department of Energy (contract no. DEAC0298CH10886). NR 65 TC 8 Z9 8 U1 3 U2 25 PU AMER SOC PLANT BIOLOGISTS PI ROCKVILLE PA 15501 MONONA DRIVE, ROCKVILLE, MD 20855 USA SN 0032-0889 EI 1532-2548 J9 PLANT PHYSIOL JI Plant Physiol. PD FEB PY 2015 VL 167 IS 2 BP 337 EP U548 DI 10.1104/pp.114.249136 PG 18 WC Plant Sciences SC Plant Sciences GA CA1DH UT WOS:000348652700005 PM 25502410 ER PT J AU Urano, D Czarnecki, O Wang, XP Jones, AM Chen, JG AF Urano, Daisuke Czarnecki, Olaf Wang, Xiaoping Jones, Alan M. Chen, Jin-Gui TI Arabidopsis Receptor of Activated C Kinase1 Phosphorylation by WITH NO LYSINE8 KINASE1[OPEN] SO PLANT PHYSIOLOGY LA English DT Article ID HETEROTRIMERIC G-PROTEIN; INTRACELLULAR RECEPTOR; PHASEOLUS-VULGARIS; FLOWERING TIME; CELL-DIVISION; BETA-SUBUNIT; RACK1; THALIANA; GENE; IDENTIFICATION AB Receptor of activated C kinase1 (RACK1) is a versatile scaffold protein that binds to numerous proteins to regulate diverse cellular pathways in mammals. In Arabidopsis (Arabidopsis thaliana), RACK1 has been shown to regulate plant hormone signaling, stress responses, and multiple processes of growth and development. However, little is known about the molecular mechanism underlying these regulations. Here, we show that an atypical serine (Ser)/threonine (Thr) protein kinase, WITH NO LYSINE8 (WNK8), phosphorylates RACK1. WNK8 physically interacted with and phosphorylated RACK1 proteins at two residues: Ser-122 and Thr-162. Genetic epistasis analysis of rack1 wnk8 double mutants indicated that RACK1 acts downstream of WNK8 in the glucose responsiveness and flowering pathways. The phosphorylation-dead form, RACK1A(S122A/T162A), but not the phosphomimetic form, RACK1A(S122D/T162E), rescued the rack1a null mutant, implying that phosphorylation at Ser-122 and Thr-162 negatively regulates RACK1A function. The transcript of RACK1A(S122D/T162E) accumulated at similar levels as those of RACK1(S122A/T162A). However, although the steady-state level of the RACK1A(S122A/T162A) protein was similar to wild-type RACK1A protein, the RACK1A(S122D/T162E) protein was nearly undetectable, suggesting that phosphorylation affects the stability of RACK1A proteins. Taken together, these results suggest that RACK1 is phosphorylated by WNK8 and that phosphorylation negatively regulates RACK1 function by influencing its protein stability. C1 [Urano, Daisuke; Jones, Alan M.] Univ N Carolina, Dept Biol, Chapel Hill, NC 27599 USA. [Jones, Alan M.] Univ N Carolina, Dept Pharmacol, Chapel Hill, NC 27599 USA. [Czarnecki, Olaf; Wang, Xiaoping; Chen, Jin-Gui] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Wang, Xiaoping] NE Normal Univ, Key Lab Mol Epigenet, Minist Educ, Changchun 130024, Peoples R China. [Wang, Xiaoping] NE Normal Univ, Inst Cytol & Genet, Changchun 130024, Peoples R China. RP Jones, AM (reprint author), Univ N Carolina, Dept Biol, Chapel Hill, NC 27599 USA. EM alan_jones@unc.edu; chenj@ornl.gov RI Chen, Jin-Gui/A-4773-2011 OI Chen, Jin-Gui/0000-0002-1752-4201 FU National Institute of General Medical Sciences [R01GM065989]; U.S. Department of Energy [DE-FG02-05er15671]; National Science Foundation [MCB-0723515, MCB-0718202]; Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; Oak Ridge National Laboratory (U.S. Department of Energy) [DE-AC05-00OR22725]; Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy [E-FG02-05er15671]; China Scholarship Council FX This work was supported by the National Institute of General Medical Sciences (grant no. R01GM065989), the U.S. Department of Energy (grant no. DE-FG02-05er15671), the National Science Foundation (grant nos. MCB-0723515 and MCB-0718202 to A.M.J.), the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory (to J.-G.C.), the Oak Ridge National Laboratory (managed by UT-Battelle, LLC for the U.S. Department of Energy under contract no. DE-AC05-00OR22725), the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy (technical support through grant no. DE-FG02-05er15671 to A.M.J.), and the China Scholarship Council (scholarship to X.W.). NR 49 TC 7 Z9 7 U1 2 U2 9 PU AMER SOC PLANT BIOLOGISTS PI ROCKVILLE PA 15501 MONONA DRIVE, ROCKVILLE, MD 20855 USA SN 0032-0889 EI 1532-2548 J9 PLANT PHYSIOL JI Plant Physiol. PD FEB PY 2015 VL 167 IS 2 BP 507 EP U349 DI 10.1104/pp.114.247460 PG 14 WC Plant Sciences SC Plant Sciences GA CA1DH UT WOS:000348652700016 PM 25489024 ER PT J AU Wu, C Xiong, W Dai, JB Wu, QY AF Wu, Chao Xiong, Wei Dai, Junbiao Wu, Qingyu TI Genome-Based Metabolic Mapping and C-13 Flux Analysis Reveal Systematic Properties of an Oleaginous Microalga Chlorella protothecoides SO PLANT PHYSIOLOGY LA English DT Article ID CITRATE SYNTHASE ACTIVITY; CHLAMYDOMONAS-REINHARDTII; BIODIESEL PRODUCTION; MASS-SPECTROMETRY; BALANCE ANALYSIS; PHOTOAUTOTROPHIC METABOLISM; GREEN-ALGAE; NETWORK; PHOTOSYNTHESIS; GROWTH AB Integrated and genome-based flux balance analysis, metabolomics, and C-13-label profiling of phototrophic and heterotrophic metabolism in Chlorella protothecoides, an oleaginous green alga for biofuel. The green alga Chlorella protothecoides, capable of autotrophic and heterotrophic growth with rapid lipid synthesis, is a promising candidate for biofuel production. Based on the newly available genome knowledge of the alga, we reconstructed the compartmentalized metabolic network consisting of 272 metabolic reactions, 270 enzymes, and 461 encoding genes and simulated the growth in different cultivation conditions with flux balance analysis. Phenotype-phase plane analysis shows conditions achieving theoretical maximum of the biomass and corresponding fatty acid-producing rate for phototrophic cells (the ratio of photon uptake rate to CO2 uptake rate equals 8.4) and heterotrophic ones (the glucose uptake rate to O-2 consumption rate reaches 2.4), respectively. Isotope-assisted liquid chromatography-mass spectrometry/mass spectrometry reveals higher metabolite concentrations in the glycolytic pathway and the tricarboxylic acid cycle in heterotrophic cells compared with autotrophic cells. We also observed enhanced levels of ATP, nicotinamide adenine dinucleotide (phosphate), reduced, acetyl-Coenzyme A, and malonyl-Coenzyme A in heterotrophic cells consistently, consistent with a strong activity of lipid synthesis. To profile the flux map in experimental conditions, we applied nonstationary C-13 metabolic flux analysis as a complementing strategy to flux balance analysis. The result reveals negligible photorespiratory fluxes and a metabolically low active tricarboxylic acid cycle in phototrophic C. protothecoides. In comparison, high throughput of amphibolic reactions and the tricarboxylic acid cycle with no glyoxylate shunt activities were measured for heterotrophic cells. Taken together, the metabolic network modeling assisted by experimental metabolomics and C-13 labeling better our understanding on global metabolism of oleaginous alga, paving the way to the systematic engineering of the microalga for biofuel production. C1 [Wu, Chao; Xiong, Wei; Dai, Junbiao; Wu, Qingyu] Tsinghua Univ, Sch Life Sci, Minist Educ, Key Lab Bioinformat, Beijing 100084, Peoples R China. [Xiong, Wei] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA. RP Wu, QY (reprint author), Tsinghua Univ, Sch Life Sci, Minist Educ, Key Lab Bioinformat, Beijing 100084, Peoples R China. EM jbdai@biomed.tsinghua.edu.cn; qingyu@tsinghua.edu.cn FU National Natural Science Foundation of China [31370282, 41030210]; Chinese Ministry of Science and Technology [2011BAD14B05, 2014AA02200]; Tsinghua University Initiative Scientific Research Program [2012Z08128]; National Renewable Energy Laboratory Director's Postdoctorate Fellowship FX This work was supported by National Natural Science Foundation of China (project nos. 31370282 and 41030210), Chinese Ministry of Science and Technology (project nos. 2011BAD14B05 and 2014AA02200 to Q.W.), the Tsinghua University Initiative Scientific Research Program (grant no. 2012Z08128 to J.D.), and the National Renewable Energy Laboratory Director's Postdoctorate Fellowship (to W.X.). NR 63 TC 12 Z9 12 U1 8 U2 62 PU AMER SOC PLANT BIOLOGISTS PI ROCKVILLE PA 15501 MONONA DRIVE, ROCKVILLE, MD 20855 USA SN 0032-0889 EI 1532-2548 J9 PLANT PHYSIOL JI Plant Physiol. PD FEB PY 2015 VL 167 IS 2 BP 586 EP 599 DI 10.1104/pp.114.250688 PG 14 WC Plant Sciences SC Plant Sciences GA CA1DH UT WOS:000348652700022 PM 25511434 ER PT J AU Baalrud, SD Lafleur, T Fox, W Germaschewski, K AF Baalrud, Scott D. Lafleur, Trevor Fox, William Germaschewski, Kai TI Instability-enhanced friction in the presheath of two-ion-species plasmas SO PLASMA SOURCES SCIENCE & TECHNOLOGY LA English DT Article DE two-stream instability; sheath; Bohm criterion ID BOHM CRITERION; CROSS-SECTIONS; SHEATH AB The speed at which ions enter a sheath is a fundamental property of a plasma that also provides a useful boundary condition in modeling. A recent theory proposed that this can be significantly influenced by an instability-enhanced friction force arising from two-stream instabilities in the presheath when multiple ion species are present. Although experiments appeared to confirm this theory, recent particle simulations have brought it into question. We reconcile this controversy using direct numerical solutions of the dispersion relation, which show that there is a dependence on the electron-ion temperature ratio that was not considered previously. In addition, particle-in-cell simulations are used to show that ion-ion two-stream instabilities can arise near the sheath edge and generate an enhanced ion-ion friction force. Only by accounting for the instability-enhanced friction force can theory predict the simulated ion speeds at the sheath edge. C1 [Baalrud, Scott D.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Lafleur, Trevor] Univ Paris Sud, Univ Paris 06, Sorbonne Univ, Lab Phys Plasmas,CNRS,Ecole Polytech, F-91128 Palaiseau, France. [Lafleur, Trevor] Off Natl Etud & Rech Aerosp, F-91120 Palaiseau, France. [Fox, William] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Germaschewski, Kai] Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA. RP Baalrud, SD (reprint author), Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. FU University of Iowa; DOE [ER55093] FX This research was supported in part by the University of Iowa and an appointment to the US DOE Fusion Energy Postdoctoral Research Program administered by ORISE (S.D.B.). KG was supported in part by DOE grant ER55093. TL would like to thank Dr Jean-Paul Booth for access to computational resources. NR 33 TC 5 Z9 5 U1 1 U2 15 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0963-0252 EI 1361-6595 J9 PLASMA SOURCES SCI T JI Plasma Sources Sci. Technol. PD FEB PY 2015 VL 24 IS 1 AR 015034 DI 10.1088/0963-0252/24/1/015034 PG 8 WC Physics, Fluids & Plasmas SC Physics GA AZ5ZW UT WOS:000348298200035 ER PT J AU Vinokur, JM Korman, TP Sawaya, MR Collazo, M Cascio, D Bowie, JU AF Vinokur, Jeffrey M. Korman, Tyler P. Sawaya, Michael R. Collazo, Michael Cascio, Duillio Bowie, James U. TI Structural analysis of mevalonate-3-kinase provides insight into the mechanisms of isoprenoid pathway decarboxylases SO PROTEIN SCIENCE LA English DT Article DE mevalonate diphosphate decarboxylase; mevalonate pyrophosphate decarboxylase; mevalonate pathway; mevalonate-3-kinase; mevalonate kinase; GHMP kinase; statin; cholesterol ID DIPHOSPHATE DECARBOXYLASE; 5-DIPHOSPHATE DECARBOXYLASE; CRYSTAL-STRUCTURES; TRANSITION-STATE; BIOSYNTHESIS; KINASE; IDENTIFICATION; INHIBITION; SEQUENCE; BINDING AB In animals, cholesterol is made from 5-carbon building blocks produced by the mevalonate pathway. Drugs that inhibit the mevalonate pathway such as atorvastatin (lipitor) have led to successful treatments for high cholesterol in humans. Another potential target for the inhibition of cholesterol synthesis is mevalonate diphosphate decarboxylase (MDD), which catalyzes the phosphorylation of (R)-mevalonate diphosphate, followed by decarboxylation to yield isopentenyl pyrophosphate. We recently discovered an MDD homolog, mevalonate-3-kinase (M3K) from Thermoplasma acidophilum, which catalyzes the identical phosphorylation of (R)-mevalonate, but without concomitant decarboxylation. Thus, M3K catalyzes half the reaction of the decarboxylase, allowing us to separate features of the active site that are required for decarboxylation from features required for phosphorylation. Here we determine the crystal structure of M3K in the apo form, and with bound substrates, and compare it to MDD structures. Structural and mutagenic analysis reveals modifications that allow M3K to bind mevalonate rather than mevalonate diphosphate. Comparison to homologous MDD structures show that both enzymes employ analogous Arg or Lys residues to catalyze phosphate transfer. However, an invariant active site Asp/Lys pair of MDD previously thought to play a role in phosphorylation is missing in M3K with no functional replacement. Thus, we suggest that the invariant Asp/Lys pair in MDD may be critical for decarboxylation rather than phosphorylation. C1 [Vinokur, Jeffrey M.; Korman, Tyler P.; Sawaya, Michael R.; Collazo, Michael; Cascio, Duillio; Bowie, James U.] Univ Calif Los Angeles, UCLA DOE Inst Genom & Prote, Inst Mol Biol, Dept Chem & Biochem, Los Angeles, CA 90095 USA. RP Bowie, JU (reprint author), Univ Calif Los Angeles, 659 Boyer Hall,611 Charles E Young Dr East, Los Angeles, CA 90095 USA. EM bowie@mbi.ucla.edu OI Sawaya, Michael/0000-0003-0874-9043 FU DOE [DE-FC02-02ER63421, DE-AC02-06CH11357]; NSF Graduate Research Fellowship [DGE-1144087]; NIH CBI Training Program [NIGMS 5T32GM008496]; NCRR [5P41RR015301-10]; NIH [P41 GM103403] FX Grant sponsor: DOE; Grant numbers: DE-FC02-02ER63421, DE-AC02-06CH11357; Grant sponsor: NSF Graduate Research Fellowship; Grant number: DGE-1144087; Grant sponsor: NIH CBI Training Program; Grant number: NIGMS 5T32GM008496; Grant sponsor: NCRR; Grant number: 5P41RR015301-10; Grant sponsor: NIH; Grant number: P41 GM103403. NR 57 TC 4 Z9 4 U1 0 U2 8 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0961-8368 EI 1469-896X J9 PROTEIN SCI JI Protein Sci. PD FEB PY 2015 VL 24 IS 2 BP 212 EP 220 DI 10.1002/pro.2607 PG 9 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CA1HK UT WOS:000348663200006 PM 25422158 ER PT J AU Weerth, RS Michalska, K Bingman, CA Yennamalli, RM Li, H Jedrzejczak, R Wang, FB Babnigg, G Joachimiak, A Thomas, MG Phillips, GN AF Weerth, R. Sophia Michalska, Karolina Bingman, Craig A. Yennamalli, Ragothaman M. Li, Hui Jedrzejczak, Robert Wang, Fengbin Babnigg, Gyorgy Joachimiak, Andrzej Thomas, Michael G. Phillips, George N., Jr. TI Structure of a cupin protein Plu4264 from Photorhabdus luminescens subsp laumondii TTO1 at 1.35 angstrom resolution SO PROTEINS-STRUCTURE FUNCTION AND BIOINFORMATICS LA English DT Article DE cupin; X-ray; structural genomics; natural product; manganese-bound ID PURIFICATION; MODEL; CRYSTALLOGRAPHY; VALIDATION AB Proteins belonging to the cupin superfamily have a wide range of catalytic and noncatalytic functions. Cupin proteins commonly have the capacity to bind a metal ion with the metal frequently determining the function of the protein. We have been investigating the function of homologous cupin proteins that are conserved in more than 40 species of bacteria. To gain insights into the potential function of these proteins we have solved the structure of Plu4264 from Photorhabdus luminescens TTO1 at a resolution of 1.35 angstrom and identified manganese as the likely natural metal ligand of the protein. Proteins 2015; 83:383-388. (c) 2014 Wiley Periodicals, Inc. C1 [Weerth, R. Sophia; Thomas, Michael G.] Univ Wisconsin, Dept Bacteriol, Madison, WI 53706 USA. [Michalska, Karolina; Babnigg, Gyorgy; Joachimiak, Andrzej] Argonne Natl Lab, Biosci Div, Midwest Ctr Struct Genom, Argonne, IL 60439 USA. [Michalska, Karolina; Li, Hui; Jedrzejczak, Robert; Babnigg, Gyorgy; Joachimiak, Andrzej] Argonne Natl Lab, Biosci Div, Struct Biol Ctr, Argonne, IL 60439 USA. [Bingman, Craig A.] Univ Wisconsin, Dept Biochem, Madison, WI 53705 USA. [Yennamalli, Ragothaman M.; Wang, Fengbin; Phillips, George N., Jr.] Rice Univ, Biosci Rice, Houston, TX 77005 USA. RP Phillips, GN (reprint author), Rice Univ, Biosci Rice, 6100 Main St, Houston, TX 77005 USA. EM georgep@rice.edu FU National Institutes of Health [GM098248, GM094585]; U.S. Department of Energy, Office of Biological and Environmental Research [DE-AC02-06CH11357] FX Grant sponsor: National Institutes of Health; grant numbers: GM098248; GM094585; Grant sponsor: U.S. Department of Energy, Office of Biological and Environmental Research; grant number: DE-AC02-06CH11357. NR 22 TC 0 Z9 0 U1 1 U2 5 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0887-3585 EI 1097-0134 J9 PROTEINS JI Proteins PD FEB PY 2015 VL 83 IS 2 BP 383 EP 388 DI 10.1002/prot.24705 PG 6 WC Biochemistry & Molecular Biology; Biophysics SC Biochemistry & Molecular Biology; Biophysics GA CA2FN UT WOS:000348724500015 PM 25354690 ER PT J AU Kim, J Haberkorn, N Nazaretski, E de Paula, R Tan, T Xi, XX Tajima, T Movshovich, R Civale, L AF Kim, Jeehoon Haberkorn, N. Nazaretski, E. de Paula, R. Tan, Teng Xi, X. X. Tajima, T. Movshovich, R. Civale, L. TI Strong magnetic field dependence of critical current densities and vortex activation energies in an anisotropic clean MgB2 thin film SO SOLID STATE COMMUNICATIONS LA English DT Article DE Superconducting materials; Films; Magnetic penetration depth; Vortex pinning ID HIGH-TEMPERATURE SUPERCONDUCTORS; PINNING MECHANISMS AB We report the influence of two-band superconductivity on the flux creep and the critical current densities of a MgB2 thin film. The small magnetic penetration depth of lambda=50 +/- 10 nm at T=4 K is related to a clean pi-band. We find a high self-field critical current density J(C), which is strongly reduced with applied magnetic field, and attribute this to suppression of the superconductivity in the pi-band. The temperature dependence of the creep rate S (T) at low magnetic field can be explained by a simple Anderson-Kim mechanism. The system shows high pinning energies at low field that are strongly suppressed by high field. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Kim, Jeehoon] CALDES, Inst Basic Sci, Pohang, South Korea. [Kim, Jeehoon] Pohang Univ Sci & Technol, Dept Phys, Pohang, South Korea. [Haberkorn, N.] Ctr Atom Bariloche, RA-8400 San Carlos De Bariloche, Rio Negro, Argentina. [Nazaretski, E.] Brookhaven Natl Lab, Upton, NY 11973 USA. [de Paula, R.; Tajima, T.; Movshovich, R.; Civale, L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Tan, Teng; Xi, X. X.] Temple Univ, Dept Phys, Philadelphia, PA 19122 USA. RP Kim, J (reprint author), Pohang Univ Sci & Technol, Dept Phys, Pohang, South Korea. EM jeehoon@postech.ac.kr; haberkornn@yahoo.com.ar; enazasetski@bnl.gov; nataliad@lanl.gov; ttan@temple.edu; xiaoxing@temple.edu; tajima@lanl.gov; roman@lanl.gov; lcivale@lanl.gov FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; Institute for Basic Science [IBS-R015-D1]; USA Department of Energy [DE-SC0004410] FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, and was supported by Institute for Basic Science by Project Code (IBS-R015-D1). N.H. is a member of CONICET (Argentina). The work at Temple University was supported by the USA Department of Energy under Grant No. DE-SC0004410. NR 43 TC 0 Z9 0 U1 3 U2 21 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0038-1098 EI 1879-2766 J9 SOLID STATE COMMUN JI Solid State Commun. PD FEB PY 2015 VL 204 BP 56 EP 60 DI 10.1016/j.ssc.2014.11.015 PG 5 WC Physics, Condensed Matter SC Physics GA CA3YU UT WOS:000348842000013 ER PT J AU McClanahan, R De Leon, PL AF McClanahan, Richard De Leon, Phillip L. TI Reducing computation in an i-vector speaker recognition system using a tree-structured universal background model SO SPEECH COMMUNICATION LA English DT Article DE Speaker recognition; Clustering methods; Tree graphs ID VERIFICATION; EXTRACTION; MEMORY AB The majority of state-of-the-art speaker recognition systems (SR) utilize speaker models that are derived from an adapted universal background model (UBM) in the form of a Gaussian mixture model (GMM). This is true for GMM supervector systems, joint factor analysis systems, and most recently i-vector systems. In all of these systems, the posterior probabilities and sufficient statistics calculations represent a computational bottleneck in both enrollment and testing. We propose a multi-layered hash system, employing a tree-structured GMM UBM which uses Runnalls' Gaussian mixture reduction technique, in order to reduce the number of these calculations. With this tree-structured hash, we can trade-off reduction in computation with a corresponding degradation of equal error rate (EER). As an example, we reduce this computation by a factor of 15x while incurring less than 10% relative degradation of EER (or 0.3% absolute EER) when evaluated with NIST 2010 speaker recognition evaluation (SRE) telephone data. (C) 2014 Elsevier B.V. All rights reserved. C1 [McClanahan, Richard; De Leon, Phillip L.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [McClanahan, Richard; De Leon, Phillip L.] New Mexico State Univ, Las Cruces, NM 88003 USA. RP McClanahan, R (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM rmcclan@sandia.gov; pdeleon@nmsu.edu NR 28 TC 1 Z9 1 U1 0 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-6393 EI 1872-7182 J9 SPEECH COMMUN JI Speech Commun. PD FEB PY 2015 VL 66 BP 36 EP 46 DI 10.1016/j.specom.2014.07.003 PG 11 WC Acoustics; Computer Science, Interdisciplinary Applications SC Acoustics; Computer Science GA AZ5LE UT WOS:000348261700003 ER PT J AU Paul, P Bhattacharyya, D Turton, R Zitney, SE AF Paul, Prokash Bhattacharyya, Debangsu Turton, Richard Zitney, Stephen E. TI Sensor Network Design for Maximizing Process Efficiency: An Algorithm and Its Application SO AICHE JOURNAL LA English DT Article DE sensor placement; estimator-based control system; efficiency maximization; parallel computation; integrated gasification combined cycle; acid gas removal unit ID CHEMICAL-PLANTS; DATA RECONCILIATION; LINEAR-PROCESSES; FAULT-DIAGNOSIS; RELIABILITY CRITERIA; COMPREHENSIVE DESIGN; MILP FORMULATION; SYSTEMS; SELECTION; ACCURACY AB Sensor network design (SND) is a constrained optimization problem requiring systematic and effective solution algorithms for determining where best to locate sensors. A SND algorithm is developed for maximizing plant efficiency for an estimator-based control system while simultaneously satisfying accuracy requirements for the desired process measurements. The SND problem formulation leads to a mixed integer nonlinear programming (MINLP) optimization that is difficult to solve for large-scale system applications. Therefore, a sequential approach is developed to solve the MINLP problem, where the integer problem for sensor selection is solved using the genetic algorithm while the nonlinear programming problem including convergence of the tear stream in the estimator-based control system is solved using the direct substitution method. The SND algorithm is then successfully applied to a large scale, highly integrated chemical process. (c) 2014 American Institute of Chemical Engineers AIChE J, 61: 464-476, 2015 C1 [Paul, Prokash; Bhattacharyya, Debangsu; Turton, Richard] W Virginia Univ, Dept Chem Engn, Morgantown, WV 26506 USA. [Zitney, Stephen E.] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. RP Bhattacharyya, D (reprint author), W Virginia Univ, Dept Chem Engn, Morgantown, WV 26506 USA. EM Debangsu.Bhattacharyya@mail.wvu.edu FU RES [DE-FE0004000] FX As part of the National Energy Technology Laboratory's Regional University Alliance (NETL-RUA), a collaborative initiative of the NETL, this technical effort was performed under the RES contract DE-FE0004000. NR 50 TC 3 Z9 3 U1 1 U2 11 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0001-1541 EI 1547-5905 J9 AICHE J JI AICHE J. PD FEB PY 2015 VL 61 IS 2 BP 464 EP 476 DI 10.1002/aic.14649 PG 13 WC Engineering, Chemical SC Engineering GA AZ1ZG UT WOS:000348033200008 ER PT J AU Peng, X Lin, LC Sun, WZ Smit, B AF Peng, Xuan Lin, Li-Chiang Sun, Weizhen Smit, Berend TI Water Adsorption in Metal-Organic Frameworks with Open-Metal Sites SO AICHE JOURNAL LA English DT Article DE adsorption; molecular simulation; water; metal; organic frameworks ID ZEOLITIC IMIDAZOLATE FRAMEWORKS; ELECTRONIC-STRUCTURE CALCULATIONS; CARBON-DIOXIDE; MOLECULAR-DYNAMICS; FORCE-FIELD; COORDINATION POLYMER; HYDROGEN ADSORPTION; POTENTIAL FUNCTIONS; LIQUID WATER; CO2 CAPTURE AB H2O adsorptions inside porous materials, including silica zeolites, zeolite imidazolate frameworks, and metal-organic frameworks (MOFs) using molecular simulations with different water models are investigated. Due to the existence of coordinately unsaturated metal sites, the predicted adsorption properties in M-MOF-74 (M=Mg, Ni, Co, Zn) and Cu-BTC are found to be greatly sensitive to the adopted H2O models. Surprisingly, the analysis of the orientations of H2O minimum energy configuration in these materials show that three-site H2O models predict an unusual perpendicular angle of H2O plane with respect to the Metal-O-4 plane, whereas those models with more than three sites give a more parallel angle that is in better agreement with the one obtained from density functional theory (DFT) calculations. In addition, the use of these commonly used models estimates the binding energies with the values lower than the ones computed by DFT ranging from 15 to 40%. To correct adsorption energies, simple approach to adjust metal-O(H2O) sigma parameters to reproduce the DFT-calculated binding energies is used. With the refined parameters, the computed water isotherms inside Mg-MOF-74 and Cu-BTC are in reasonable agreement with experimental data, and provide significant improvement compared to the predictions made by the original models. Further, a detailed inspection on the water configurations at higher-pressure region was also made, and observed that there is an interesting two-layer water network formed using three- and four-site models. (c) 2014 American Institute of Chemical Engineers AIChE J, 61: 677-687, 2015 C1 [Peng, Xuan] Beijing Univ Chem Technol, Dept Automat, Coll Informat Sci & Technol, Beijing 100029, Peoples R China. [Peng, Xuan; Lin, Li-Chiang; Sun, Weizhen; Smit, Berend] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Sun, Weizhen] E China Univ Sci & Technol, State Key Lab Chem Engn, Shanghai 200237, Peoples R China. [Sun, Weizhen] E China Univ Sci & Technol, Key Lab Adv Control & Optimizat Chem Proc, Shanghai 200237, Peoples R China. [Smit, Berend] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Smit, Berend] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Smit, B (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. RI Smit, Berend/B-7580-2009; EFRC, CGS/I-6680-2012; Stangl, Kristin/D-1502-2015; Lin, Li-Chiang/J-8120-2014; OI Smit, Berend/0000-0003-4653-8562; Lin, Li-Chiang/0000-0002-2821-9501 FU Open Project of State Key Laboratory of Chemical Engineering [SKL-Che-12C01]; China Scholarship Council; Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001015] FX XP was supported by the Open Project of State Key Laboratory of Chemical Engineering (SKL-Che-12C01). XP and WZS were supported by the China Scholarship Council. LCL and BS were supported as part of the Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0001015. NR 57 TC 4 Z9 4 U1 25 U2 189 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0001-1541 EI 1547-5905 J9 AICHE J JI AICHE J. PD FEB PY 2015 VL 61 IS 2 BP 677 EP 687 DI 10.1002/aic.14707 PG 11 WC Engineering, Chemical SC Engineering GA AZ1ZG UT WOS:000348033200025 ER PT J AU Lundquist, JK Bariteau, L AF Lundquist, J. K. Bariteau, L. TI Dissipation of Turbulence in the Wake of a Wind Turbine SO BOUNDARY-LAYER METEOROLOGY LA English DT Article DE Dissipation rate; Tethered lifting system; Turbulent kinetic energy; Wind energy; Wind turbines ID BOUNDARY-LAYER PROFILES; SURFACE-LAYER; ENERGY-DISSIPATION; MEASUREMENT SYSTEM; FLUX MEASUREMENTS; DOPPLER LIDAR; MODEL; FARMS; TEMPERATURE; ENVIRONMENT AB The wake of a wind turbine is characterized by increased turbulence and decreased wind speed. Turbines are generally deployed in large groups in wind farms, and so the behaviour of an individual wake as it merges with other wakes and propagates downwind is critical in assessing wind-farm power production. This evolution depends on the rate of turbulence dissipation in the wind-turbine wake, which has not been previously quantified in field-scale measurements. In situ measurements of winds and turbulence dissipation from the wake region of a multi-MW turbine were collected using a tethered lifting system (TLS) carrying a payload of high-rate turbulence probes. Ambient flow measurements were provided from sonic anemometers on a meteorological tower located near the turbine. Good agreement between the tower measurements and the TLS measurements was established for a case without a wind-turbine wake. When an operating wind turbine is located between the tower and the TLS so that the wake propagates to the TLS, the TLS measures dissipation rates one to two orders of magnitude higher in the wake than outside of the wake. These data, collected between two and three rotor diameters downwind of the turbine, document the significant enhancement of turbulent kinetic energy dissipation rate within the wind-turbine wake. These wake measurements suggest that it may be useful to pursue modelling approaches that account for enhanced dissipation. Comparisons of wake and non-wake dissipation rates to mean wind speed, wind-speed variance, and turbulence intensity are presented to facilitate the inclusion of these measurements in wake modelling schemes. C1 [Lundquist, J. K.] Univ Colorado, Dept Atmospher & Ocean Sci, Boulder, CO 80309 USA. [Lundquist, J. K.] Natl Renewable Energy Lab, Natl Wind Technol Ctr, Golden, CO 80401 USA. [Bariteau, L.] NOAA, Earth Syst Res Lab, Boulder, CO 80305 USA. [Bariteau, L.] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. RP Lundquist, JK (reprint author), Univ Colorado, Dept Atmospher & Ocean Sci, Boulder, CO 80309 USA. EM julie.lundquist@colorado.edu OI LUNDQUIST, JULIE/0000-0001-5490-2702 FU Colorado Research and Education in Wind FX This work was supported by a seed grant from Colorado Research and Education in Wind submitted by Prof. J. K. Lundquist and Dr. Yannick Meillier with cooperation from NREL. NREL is a National Laboratory of the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, operated by the Alliance for Sustainable Energy, LLC. The authors thank NREL staff Dr. Andrew Clifton, Mr. Michael Stewart, Mr. Jeroen van Dam, and University of Colorado at Boulder researchers and students Michael Rhodes, Matthew Aitken, Brian Vanderwende, Ryan King, Clara St. Martin, and Josh Aikens for their considerable efforts in collecting these data, and Michael Rhodes for assistance with the figures. The authors also acknowledge Dr. Chris Fairall, Dr. Branko Kosovic, and Dr. Andrew Clifton for helpful discussions, as well as the helpful comments of three anonymous reviewers. NR 54 TC 3 Z9 3 U1 1 U2 23 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0006-8314 EI 1573-1472 J9 BOUND-LAY METEOROL JI Bound.-Layer Meteor. PD FEB PY 2015 VL 154 IS 2 BP 229 EP 241 DI 10.1007/s10546-014-9978-3 PG 13 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA AZ6WK UT WOS:000348358500004 ER PT J AU Payne, MA Miller, JB Gellman, AJ AF Payne, Matthew A. Miller, James B. Gellman, Andrew J. TI High-throughput characterization of early oxidation across AlxFeyNi1-x-y composition space SO CORROSION SCIENCE LA English DT Article DE Aluminium; Iron; Nickel; Raman spectroscopy; XPS; Oxidation ID HIGH-TEMPERATURE OXIDATION; X-RAY-DIFFRACTION; ALUMINUM-ALLOYS; IRON-OXIDES; AL ALLOYS; FE-AL; BEHAVIOR; RAMAN; SCALES; ELECTROCATALYSTS AB Improving our fundamental understanding of the oxidation of multicomponent alumina-forming alloys is crucial to their ongoing development. In this work, high-throughput methods were developed to study oxidation of AlxFeyNi1-x-y alloys in dry air at 427 degrees C using composition spread alloy films as combinatorial libraries (x = 0 -> 1, y = 0 -> [1-x]). The results divide the AlxFeyNi1-x-y composition space into four regions of phenomenologically distinct oxidation behaviour. The boundary defining the critical Al concentration, N-Al* (x, y), for establishment of a passivating Al2O3 scale was determined across the entire continuous AlxFeyNi1-x-y composition space. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Gellman, Andrew J.] Carnegie Mellon Univ, Dept Chem Engn, Pittsburgh, PA 15213 USA. DOE Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. RP Gellman, AJ (reprint author), Carnegie Mellon Univ, Dept Chem Engn, 5000 Forbes Ave, Pittsburgh, PA 15213 USA. EM gellman@cmu.edu RI Gellman, Andrew/M-2487-2014 OI Gellman, Andrew/0000-0001-6618-7427 FU Cross-Cutting Technologies Program at the National Energy Technology Laboratory; Carnegie Mellon University by NETL through the RES Contract [DE-FE000400] FX This work was funded by the Cross-Cutting Technologies Program at the National Energy Technology Laboratory, managed by Susan Maley (Technology Manager) and Charles Miller (Technical Monitor). The Research was executed through NETL Office of Research and Development's Innovative Process Technologies (IPT) Field Work Proposal. This work was financially supported at the Carnegie Mellon University by NETL through the RES Contract No. DE-FE000400. NR 51 TC 8 Z9 8 U1 5 U2 22 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0010-938X EI 1879-0496 J9 CORROS SCI JI Corrosion Sci. PD FEB PY 2015 VL 91 BP 46 EP 57 DI 10.1016/j.corsci.2014.10.034 PG 12 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AZ5MJ UT WOS:000348264700005 ER PT J AU Neal-Kluever, A Cooper, J Zebovitz, TC Butts, KM AF Neal-Kluever, April Cooper, Jessica Zebovitz, Thomas C. Butts, Kyla M. TI Ten-year retrospective assessment of the performance of the Food Contact Notification (FCN) programme SO FOOD ADDITIVES AND CONTAMINANTS PART A-CHEMISTRY ANALYSIS CONTROL EXPOSURE & RISK ASSESSMENT LA English DT Article DE regulatory toxicology; regulatory chemistry; safety assessment; health policy; food contact AB The Food Contact Notification (FCN) programme was authorised by the US Food and Drug Administration (USFDA) Modernization Act of 1997. Manufacturers may file FCNs for food contact substances (FCSs) not already authorised or pre-sanctioned by the USFDA by demonstrating a reasonable certainty of no harm for their intended uses. The Division of Food Contact Notifications (DFCN) 10-year Retrospective Assessment Group was formed to collect and develop metrics associated with the first decade of the FCN Programme and determine the extent selected aspects of the review process contributed to the effective FCN. Comparative analysis of 924 FCNs revealed that 76% become effective, 23% were withdrawn and 1% received a not accepted status. The focus of the Group was to identify factors impacting the likelihood of an FCN becoming effective. C1 [Neal-Kluever, April; Cooper, Jessica; Zebovitz, Thomas C.] US FDA, Ctr Food Safety & Appl Nutr, Div Food Contact Notificat, College Pk, MD USA. [Butts, Kyla M.] ORISE, Oak Ridge, TN USA. RP Neal-Kluever, A (reprint author), US FDA, Ctr Food Safety & Appl Nutr, Div Food Contact Notificat, College Pk, MD USA. EM April.kluever@fda.hhs.gov NR 1 TC 0 Z9 0 U1 0 U2 2 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 1944-0049 EI 1944-0057 J9 FOOD ADDIT CONTAM A JI Food Addit. Contam. Part A-Chem. PD FEB 1 PY 2015 VL 32 IS 2 BP 261 EP 270 DI 10.1080/19440049.2014.994112 PG 10 WC Chemistry, Applied; Food Science & Technology; Toxicology SC Chemistry; Food Science & Technology; Toxicology GA CA1FN UT WOS:000348658300014 PM 25529924 ER PT J AU Lunden, MM Delp, WW Singer, BC AF Lunden, M. M. Delp, W. W. Singer, B. C. TI Capture efficiency of cooking-related fine and ultrafine particles by residential exhaust hoods SO INDOOR AIR LA English DT Article DE Cooker hood; Extractor fan; Kitchen ventilation; PM; 2; 5; Range hood ID KITCHEN RANGE HOODS; INDOOR SOURCES; GAS; EMISSIONS; EXPOSURE; RATES; FLOW AB Effective exhaust hoods can mitigate the indoor air quality impacts of pollutant emissions from residential cooking. This study reports capture efficiencies (CE) measured for cooking-generated particles for scripted cooking procedures in a 121-m(3) chamber with kitchenette. CEs also were measured for burner produced CO2 during cooking and separately for pots and pans containing water. The study used four exhaust hoods previously tested by Delp and Singer (Environ. Sci. Technol., 2012, 46, 6167-6173). For pan-frying a hamburger over medium heat on the back burner, CEs for particles were similar to those for burner produced CO2 and mostly above 80%. For stir-frying green beans in a wok (high heat, front burner), CEs for burner CO2 during cooking varied by hood and airflow: CEs were 34-38% for low (51-68l/s) and 54-72% for high (109-138l/s) settings. CEs for 0.3-2.0m particles during front burner stir-frying were 3-11% on low and 16-70% on high settings. Results indicate that CEs measured for burner CO2 are not predictive of CEs of cooking-generated particles under all conditions, but they may be suitable to identify devices with CEs above 80% both for burner combustion products and for cooking-related particles. C1 [Lunden, M. M.; Delp, W. W.; Singer, B. C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Indoor Environm Grp, Berkeley, CA 94720 USA. [Lunden, M. M.; Delp, W. W.; Singer, B. C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Residential Bldg Syst Grp, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Lunden, M. M.] Aclima Inc, San Francisco, CA USA. RP Singer, BC (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd,MS90-3058, Berkeley, CA 94720 USA. EM bcsinger@lbl.gov FU California Energy Commission PIER-Environmental Program [500-09-024]; U.S. Department of Energy Building America Program [DE-AC02-05CH11231]; U.S. Department of Housing and Urban Development, Office of Healthy Homes and Lead Hazard Control [I-PHI-01070]; U.S. Environmental Protection Agency Indoor Environments Division [DW-89-92322201-0] FX Funding was provided by the California Energy Commission PIER-Environmental Program via Contract 500-09-024; the U.S. Department of Energy Building America Program via Contract DE-AC02-05CH11231; the U.S. Department of Housing and Urban Development, Office of Healthy Homes and Lead Hazard Control via Agreement I-PHI-01070; and the U.S. Environmental Protection Agency Indoor Environments Division via Agreement DW-89-92322201-0. We thank Tosh Hotchi and Doug Sullivan for chamber set-up and Marcella Barrios and Omsri Bharat for carefully conducting the cooking experiments. NR 29 TC 6 Z9 7 U1 13 U2 38 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0905-6947 EI 1600-0668 J9 INDOOR AIR JI Indoor Air PD FEB PY 2015 VL 25 IS 1 BP 45 EP 58 DI 10.1111/ina.12118 PG 14 WC Construction & Building Technology; Engineering, Environmental; Public, Environmental & Occupational Health SC Construction & Building Technology; Engineering; Public, Environmental & Occupational Health GA AZ3GM UT WOS:000348115500006 PM 24750219 ER PT J AU Dutton, SM Mendell, MJ Chan, WR Barrios, M Sidheswaran, MA Sullivan, DP Eliseeva, EA Fisk, WJ AF Dutton, S. M. Mendell, M. J. Chan, W. R. Barrios, M. Sidheswaran, M. A. Sullivan, D. P. Eliseeva, E. A. Fisk, W. J. TI Evaluation of the indoor air quality minimum ventilation rate procedure for use in California retail buildings SO INDOOR AIR LA English DT Article DE Indoor Air Quality Procedure; Occupant exposure; Retail store; Ventilation rates; Indoor contaminants; Ventilation standards AB This research assesses benefits of adding to California Title-24 ventilation rate (VR) standards a performance-based option, similar to the American Society of Heating, Refrigerating, and Air Conditioning Engineers Indoor Air Quality Procedure' (IAQP) for retail spaces. Ventilation rates and concentrations of contaminants of concern (CoC) were measured in 13 stores. Mass balance models were used to estimate IAQP-based' VRs that would maintain concentrations of all CoCs below health- or odor-based reference concentration limits. An intervention study in a big box' store assessed how the current VR, the Title 24-prescribed VR, and the IAQP-based VR (0.24, 0.69, and 1.51 air changes per hour) influenced measured IAQ and perceived of IAQ. Neither current VRs nor Title 24-prescribed VRs would maintain all CoCs below reference limits in 12 of 13 stores. In the big box store, the IAQP-based VR kept all CoCs below limits. More than 80% of subjects reported acceptable air quality at all three VRs. In 11 of 13 buildings, saving energy through lower VRs while maintaining acceptable IAQ would require source reduction or gas-phase air cleaning for CoCs. In only one of the 13 retail stores surveyed, application of the IAQP would have allowed reduced VRs without additional contaminant-reduction strategies. C1 [Dutton, S. M.; Mendell, M. J.; Chan, W. R.; Barrios, M.; Sidheswaran, M. A.; Sullivan, D. P.; Eliseeva, E. A.; Fisk, W. J.] Lawrence Berkeley Natl Lab, Berkeley, CA 94704 USA. RP Dutton, SM (reprint author), Lawrence Berkeley Natl Lab, 1 Cyclotron Rd MS90R3058D, Berkeley, CA 94704 USA. EM smdutton@lbl.gov FU California Energy Commission [500-09-049, DE-AC03-05CH11231] FX The research reported here was supported by the California Energy Commission Public Interest Energy Research Program, Energy-Related Environmental Research Program, award number 500-09-049 under contract DE-AC03-05CH11231 between the U.S. Department of Energy and the University of California. The authors thank: Marla Mueller for program management; Sebastian Cohn for assistance with measurements and sample analysis; Marion Russell for assistance with sample analysis; staff at the big box building for their assistance with the intervention study; and members of the project advisory committee for their reviews of a draft of this document. NR 34 TC 4 Z9 4 U1 2 U2 12 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0905-6947 EI 1600-0668 J9 INDOOR AIR JI Indoor Air PD FEB PY 2015 VL 25 IS 1 BP 93 EP 104 DI 10.1111/ina.12125 PG 12 WC Construction & Building Technology; Engineering, Environmental; Public, Environmental & Occupational Health SC Construction & Building Technology; Engineering; Public, Environmental & Occupational Health GA AZ3GM UT WOS:000348115500010 PM 24809924 ER PT J AU Svahn, SL Grahnemo, L Palsdottir, V Nookaew, I Wendt, K Gabrielsson, B Schele, E Benrick, A Andersson, N Nilsson, S Johansson, ME Jansson, JO AF Svahn, Sara L. Grahnemo, Louise Palsdottir, Vilborg Nookaew, Intawat Wendt, Karl Gabrielsson, Britt Schele, Erik Benrick, Anna Andersson, Niklas Nilsson, Staffan Johansson, Maria E. Jansson, John-Olov TI Dietary Polyunsaturated Fatty Acids Increase Survival and Decrease Bacterial Load during Septic Staphylococcus aureus Infection and Improve Neutrophil Function in Mice SO INFECTION AND IMMUNITY LA English DT Article ID HEMATOPOIETIC STEM-CELLS; SEPSIS; APOPTOSIS; GLUTAMINE; EPIDEMIOLOGY; INFLAMMATION; CHALLENGES; RESISTANCE; MORTALITY; MONOCYTES AB Severe infection, including sepsis, is an increasing clinical problem that causes prolonged morbidity and substantial mortality. At present, antibiotics are essentially the only pharmacological treatment for sepsis. The incidence of resistance to antibiotics is increasing; therefore, it is critical to find new therapies for sepsis. Staphylococcus aureus is a major cause of septic mortality. Neutrophils play an important role in the defense against bacterial infections. We have shown that a diet with high levels of dietary saturated fatty acids decreases survival in septic mice, but the mechanisms behind this remain elusive. The aim of the present study was to investigate how the differences in dietary fat composition affect survival and bacterial load after experimental septic infection and neutrophil function in uninfected mice. We found that, after S. aureus infection, mice fed a polyunsaturated high-fat diet (HFD-P) for 8 weeks had increased survival and decreased bacterial load during sepsis compared with mice fed a saturated high-fat diet (HFD-S), similar to mice fed a low-fat diet (LFD). Uninfected mice fed HFD-P had a higher frequency of neutrophils in bone marrow than mice fed HFD-S. In addition, mice fed HFD-P had a higher frequency of neutrophils recruited to the site of inflammation in response to peritoneal injection of thioglycolate than mice fed HFD-S. Differences between the proportion of dietary protein and carbohydrate did not affect septic survival at all. In conclusion, polyunsaturated dietary fat increased both survival and efficiency of bacterial clearance during septic S. aureus infection. Moreover, this diet increased the frequency and chemotaxis of neutrophils, key components of the immune response to S. aureus infections. C1 [Svahn, Sara L.; Palsdottir, Vilborg; Wendt, Karl; Schele, Erik; Benrick, Anna; Andersson, Niklas; Johansson, Maria E.; Jansson, John-Olov] Univ Gothenburg, Dept Physiol, Inst Neurosci & Physiol, Sahlgrenska Acad, Gothenburg, Sweden. [Grahnemo, Louise] Univ Gothenburg, Dept Rheumatol & Inflammat Res, Inst Med, Sahlgrenska Acad, Gothenburg, Sweden. [Nookaew, Intawat] Oak Ridge Natl Lab, Biosci Div, Comparat Genom Grp, Oak Ridge, TN USA. [Nookaew, Intawat; Gabrielsson, Britt] Chalmers, Dept Chem & Biol Engn, S-41296 Gothenburg, Sweden. [Nilsson, Staffan] Chalmers, Dept Math Stat, S-41296 Gothenburg, Sweden. RP Johansson, ME (reprint author), Univ Gothenburg, Dept Physiol, Inst Neurosci & Physiol, Sahlgrenska Acad, Gothenburg, Sweden. EM maria.e.johansson@neuro.gu.se RI Gabrielsson, Britt/B-9870-2011; OI Gabrielsson, Britt/0000-0003-4318-8704; Grahnemo, Louise/0000-0001-5276-6612 FU Swedish Research Council [K2013-54X-09894-19-3]; European Framework Programme [FP7-KBBE-2010-4-266408] FX This work was supported by the Swedish Research Council (no. K2013-54X-09894-19-3) and European Framework Programme 7 funding (Full4Health; contract no. FP7-KBBE-2010-4-266408). NR 32 TC 10 Z9 10 U1 2 U2 8 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0019-9567 EI 1098-5522 J9 INFECT IMMUN JI Infect. Immun. PD FEB PY 2015 VL 83 IS 2 BP 514 EP 521 DI 10.1128/IAI.02349-14 PG 8 WC Immunology; Infectious Diseases SC Immunology; Infectious Diseases GA AZ0ST UT WOS:000347955700007 PM 25404025 ER PT J AU Hardt, DJ James, RA Gut, CP McInturf, SM Sweeney, LM Erickson, RP Gargas, ML AF Hardt, Daniel J. James, R. Arden Gut, Chester P., Jr. McInturf, Shawn M. Sweeney, Lisa M. Erickson, Richard P. Gargas, Michael L. TI Evaluation of submarine atmospheres: effects of carbon monoxide, carbon dioxide and oxygen on general toxicology, neurobehavioral performance, reproduction and development in rats. I. Subacute exposures SO INHALATION TOXICOLOGY LA English DT Article DE Carbon dioxide; carbon monoxide; hematology; hypoxia; inhalation; mixtures; neurobehavioral; reproductive toxicity ID PRENATAL EXPOSURE; CIGARETTE-SMOKE; INTERMITTENT HYPOXIA; AVOIDANCE-BEHAVIOR; GUINEA-PIG; WATER-MAZE; FETAL; PREGNANCY; INHALATION; TOXICITY AB The inhalation toxicity of submarine contaminants is of concern to ensure the health of men and women aboard submarines during operational deployments. Due to a lack of adequate prior studies, potential general, neurobehavioral, reproductive and developmental toxicity was evaluated in male and female rats exposed to mixtures of three critical submarine atmospheric components: carbon monoxide (CO) and carbon dioxide (CO2; levels elevated above ambient), and oxygen (O2; levels decreased below ambient). In a 14-day, 23 h/day, whole-body inhalation study of exposure to clean air (0.4ppm CO, 0.1% CO2 and 20.6% O-2), low-dose, mid-dose and high-dose gas mixtures (high dose of 88.4 ppm CO, 2.5% CO2 and 15.0% O-2), no adverse effects on survival, body weight or histopathology were observed. Reproductive, developmental and neurobehavioral performance were evaluated after a 28-day exposure in similar atmospheres. No adverse effects on estrus phase, mating, gestation or parturition were observed. No developmental or functional deficits were observed in either exposed parents or offspring related to motor activity, exploratory behavior or higher-level cognitive functions (learning and memory). Only minimal effects were discovered in parent-offspring emotionality tests. While statistically significant increases in hematological parameters were observed in the offspring of exposed parents compared to controls, these parameters remained within normal clinical ranges for blood cells and components and were not considered adverse. In summary, subacute exposures to elevated concentrations of the submarine atmosphere gases did not affect the ability of rats to reproduce and did not appear to have any significant adverse health effects. C1 [Hardt, Daniel J.; Erickson, Richard P.; Gargas, Michael L.] Naval Med Res Unit Dayton NAMRU D, Wright Patterson AFB, OH USA. [James, R. Arden; Gut, Chester P., Jr.; McInturf, Shawn M.] CAMRIS, Wright Patterson AFB, OH USA. [Gut, Chester P., Jr.] Oak Ridge Inst Sci & Educ, Wright Patterson AFB, OH USA. [Sweeney, Lisa M.] Henry M Jackson Fdn Advancement Mil Med, Wright Patterson AFB, OH USA. RP Sweeney, LM (reprint author), Naval Med Res Unit Dayton, 2729 R St, Wright Patterson AFB, OH 45433 USA. EM Lisa.sweeney.3.ctr@us.af.mil FU Office of Naval Research [61064] FX There are no conflicts of interest to declare. This effort was supported by the Office of Naval Research under Work Unit Number 61064. The views expressed in this article are those of the author and do not necessarily reflect the official policy or position of the Department of the Navy, Department of Defense, nor the US Government. The authors are military service members, employees or contract employees of the US Government. This work was prepared as part of their official duties. Title 17 U.S.C. 105 provides that "Copyright protection under this title is not available for any work of the United States Government". Title 17 U.S.C. 101 defines the US Government work as a work prepared by a military service member or employee of the US Government as part of that person's official duties. NR 64 TC 1 Z9 1 U1 1 U2 5 PU INFORMA HEALTHCARE PI LONDON PA TELEPHONE HOUSE, 69-77 PAUL STREET, LONDON EC2A 4LQ, ENGLAND SN 0895-8378 EI 1091-7691 J9 INHAL TOXICOL JI Inhal. Toxicol. PD FEB PY 2015 VL 27 IS 2 BP 83 EP 99 DI 10.3109/08958378.2014.995386 PG 17 WC Toxicology SC Toxicology GA AZ3QR UT WOS:000348142300001 PM 25600219 ER PT J AU Fantke, P Jolliet, O Evans, JS Apte, JS Cohen, AJ Hanninen, OO Hurley, F Jantunen, MJ Jerrett, M Levy, JI Loh, MM Marshall, JD Miller, BG Preiss, P Spadaro, JV Tainio, M Tuomisto, JT Weschler, CJ McKone, TE AF Fantke, Peter Jolliet, Olivier Evans, John S. Apte, Joshua S. Cohen, Aaron J. Hanninen, Otto O. Hurley, Fintan Jantunen, Matti J. Jerrett, Michael Levy, Jonathan I. Loh, Miranda M. Marshall, Julian D. Miller, Brian G. Preiss, Philipp Spadaro, Joseph V. Tainio, Marko Tuomisto, Jouni T. Weschler, Charles J. McKone, Thomas E. TI Health effects of fine particulate matter in life cycle impact assessment: findings from the Basel Guidance Workshop SO INTERNATIONAL JOURNAL OF LIFE CYCLE ASSESSMENT LA English DT Article DE Air pollution; Exposure-response function; Fine particulate matter; Global guidance; Human health effects; Intake fraction; Life cycle impact assessment (LCIA) ID LONG-TERM EXPOSURE; AIR-POLLUTANT EXPOSURE; INTAKE FRACTIONS; GLOBAL BURDEN; CARDIOVASCULAR-DISEASE; ULTRAFINE PARTICLES; UNITED-STATES; RESPIRATORY-INFECTIONS; SYSTEMATIC ANALYSIS; POWER-PLANTS AB Purpose Fine particulate matter (PM2.5) is considered to be one of the most important environmental factors contributing to the global human disease burden. However, due to the lack of broad consensus and harmonization in the life cycle assessment (LCA) community, there is no clear guidance on how to consistently include health effects from PM2.5 exposure in LCA practice. As a consequence, different models are currently used to assess life cycle impacts for PM2.5, sometimes leading to inconsistent results. In a global effort initiated by the United Nations Environment Programme (UNEP)/Society for Environmental Toxicology and Chemistry (SETAC) Life Cycle Initiative, respiratory inorganics' impacts expressed as health effects from PM2.5 exposure were selected as one of the initial impact categories to undergo review with the goal of providing global guidance for implementation in life cycle impact assessment (LCIA). The goal of this paper is to summarize the current knowledge and practice for assessing health effects from PM2.5 exposure and to provide recommendations for their consistent integration into LCIA. Methods A task force on human health impacts was convened to build the framework for consistently quantifying health effects from PM2.(5) exposure and for recommending PM2.5 characterization factors. In an initial Guidance Workshop, existing literature was reviewed and input from a broad range of internationally recognized experts was obtained and discussed. Workshop objectives were to identify the main scientific questions and challenges for quantifying health effects from PM2.5 exposure and to provide initial guidance to the impact quantification process. Results and discussion A set of 10 recommendations was developed addressing (a) the general framework for assessing PM2.5-related health effects, (b) approaches and data to estimate human exposure to PM2.5 using intake fractions, and (c) approaches and data to characterize exposure-response functions (ERFs) for PM2.5 and to quantify severity of the diseases attributed to PM2.5 exposure. Despite these advances, a number of complex issues, such as those related to nonlinearity of the ERF and the possible need to provide different ERFs for use in different geographical regions, require further analysis. Conclusions and outlook Questions of how to refine and improve the overall framework were analyzed. Data and models were proposed for harmonizing various elements of the health impact pathways for PM2.5. Within the next two years, our goal is to build a global guidance framework and to determine characterization factors that are more reliable for incorporating the health effects from exposure to PM2.5 into LCIA. Ideally, this will allow quantification of the impacts of both indoor and outdoor exposures to PM2.5. C1 [Fantke, Peter] Tech Univ Denmark, Dept Engn Management, Quantitat Sustainabil Assessment Div, DK-2800 Lyngby, Denmark. [Jolliet, Olivier] Univ Michigan, Sch Publ Hlth, Ann Arbor, MI 48109 USA. [Evans, John S.] Harvard Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02115 USA. [Evans, John S.] Cyprus Univ Technol, Cyprus Int Inst Environm & Publ Hlth, CY-3041 Limassol, Cyprus. [Apte, Joshua S.] Univ Calif Berkeley, Energy & Resources Grp, Berkeley, CA 94720 USA. [Cohen, Aaron J.] Hlth Effects Inst, Boston, MA 02110 USA. [Hanninen, Otto O.; Jantunen, Matti J.; Tuomisto, Jouni T.] Natl Inst Hlth & Welf, Kuopio 70701, Finland. [Hurley, Fintan; Miller, Brian G.] Inst Occupat Med, Edinburgh EH14 4AP, Midlothian, Scotland. [Jerrett, Michael; McKone, Thomas E.] Univ Calif Berkeley, Sch Publ Hlth, Berkeley, CA 94720 USA. [Levy, Jonathan I.] Boston Univ, Sch Publ Hlth, Boston, MA 02118 USA. [Loh, Miranda M.] Univ Arizona, Mel & Enid Zuckerman Coll Publ Hlth, Tucson, AZ 85724 USA. [Marshall, Julian D.] Univ Minnesota, Dept Civil Engn, Minneapolis, MN 55455 USA. [Preiss, Philipp] Econcept AG, CH-8002 Zurich, Switzerland. [Spadaro, Joseph V.] Basque Ctr Climate Change, Bilbao Bizkaia 48008, Spain. [Tainio, Marko] Polish Acad Sci, Syst Res Inst, PL-01447 Warsaw, Poland. [Tainio, Marko] Univ Cambridge, UKCRC Ctr Diet & Act Res, Cambridge, England. [Weschler, Charles J.] Rutgers State Univ, Environm & Occupat Hlth Sci Inst, Piscataway, NJ 08854 USA. [Weschler, Charles J.] Tech Univ Denmark, Int Ctr Indoor Environm & Energy, DK-2800 Lyngby, Denmark. [McKone, Thomas E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Fantke, P (reprint author), Tech Univ Denmark, Dept Engn Management, Quantitat Sustainabil Assessment Div, Prod Torvet 424, DK-2800 Lyngby, Denmark. EM pefan@dtu.dk RI QSA, DTU/J-4787-2014; Spadaro, Joseph/F-2938-2012; Fantke, Peter/N-2704-2015; Apte, Joshua/K-2570-2014; Levy, Jon/B-4542-2011; Weschler, Charles/A-9788-2009; OI Fantke, Peter/0000-0001-7148-6982; Apte, Joshua/0000-0002-2796-3478; Levy, Jon/0000-0002-1116-4006; Weschler, Charles/0000-0002-9097-5850; Tainio, Marko/0000-0002-0973-2342; Hanninen, Otto/0000-0002-4868-4822 NR 86 TC 13 Z9 13 U1 1 U2 49 PU SPRINGER HEIDELBERG PI HEIDELBERG PA TIERGARTENSTRASSE 17, D-69121 HEIDELBERG, GERMANY SN 0948-3349 EI 1614-7502 J9 INT J LIFE CYCLE ASS JI Int. J. Life Cycle Assess. PD FEB PY 2015 VL 20 IS 2 BP 276 EP 288 DI 10.1007/s11367-014-0822-2 PG 13 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AZ3OZ UT WOS:000348138000011 ER PT J AU Holmes, DE Giloteaux, L Chaurasia, AK Williams, KH Luef, B Wilkins, MJ Wrighton, KC Thompson, CA Comolli, LR Lovley, DR AF Holmes, Dawn E. Giloteaux, Ludovic Chaurasia, Akhilesh K. Williams, Kenneth H. Luef, Birgit Wilkins, Michael J. Wrighton, Kelly C. Thompson, Courtney A. Comolli, Luis R. Lovley, Derek R. TI Evidence of Geobacter-associated phage in a uranium-contaminated aquifer SO ISME JOURNAL LA English DT Article ID IN-SITU; MARINE VIRUSES; VIRAL LYSIS; QUANTIFYING EXPRESSION; MICROBIAL COMMUNITIES; SUBSURFACE SEDIMENTS; MOLECULAR ANALYSIS; ORGANIC-MATTER; SP-NOV.; BIOREMEDIATION AB Geobacter species may be important agents in the bioremediation of organic and metal contaminants in the subsurface, but as yet unknown factors limit the in situ growth of subsurface Geobacter well below rates predicted by analysis of gene expression or in silico metabolic modeling. Analysis of the genomes of five different Geobacter species recovered from contaminated subsurface sites indicated that each of the isolates had been infected with phage. Geobacter-associated phage sequences were also detected by metagenomic and proteomic analysis of samples from a uranium-contaminated aquifer undergoing in situ bioremediation, and phage particles were detected by microscopic analysis in groundwater collected from sediment enrichment cultures. Transcript abundance for genes from the Geobacter-associated phage structural proteins, tail tube Gp19 and baseplate J, increased in the groundwater in response to the growth of Geobacter species when acetate was added, and then declined as the number of Geobacter decreased. Western blot analysis of a Geobacter-associated tail tube protein Gp19 in the groundwater demonstrated that its abundance tracked with the abundance of Geobacter species. These results suggest that the enhanced growth of Geobacter species in the subsurface associated with in situ uranium bioremediation increased the abundance and activity of Geobacter-associated phage and show that future studies should focus on how these phages might be influencing the ecology of this site. C1 [Holmes, Dawn E.; Giloteaux, Ludovic; Chaurasia, Akhilesh K.; Thompson, Courtney A.; Lovley, Derek R.] Univ Massachusetts, Dept Microbiol, Amherst, MA 01003 USA. [Holmes, Dawn E.] Western New England Univ, Springfield, MA USA. [Williams, Kenneth H.; Luef, Birgit; Comolli, Luis R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Luef, Birgit; Wrighton, Kelly C.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Wilkins, Michael J.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Holmes, DE (reprint author), Univ Massachusetts, Dept Microbiol, 203 N Morrill Sci Ctr IVN, Amherst, MA 01003 USA. EM dholmes@microbio.umass.edu RI Williams, Kenneth/O-5181-2014; Giloteaux, Ludovic/L-6986-2015; Wilkins, Michael/A-9358-2013 OI Williams, Kenneth/0000-0002-3568-1155; FU Office of Science (BER), US Department of Energy [DE-SC0006790]; Integrated Field Research Challenge Site (IFRC) at Rifle, CO, USA; Lawrence Berkeley National Laboratory's Sustainable Systems Scientific Focus Area; US Department of Energy (DOE), Office of Science (BER) [DE-AC02-05CH11231]; Subsurface Biogeochemistry Program (SBR) [DE-SC0004733]; Office of Basic Energy Sciences of the US Department of Energy [DE-AC02- 05CH11231] FX Research at the University of Massachusetts was funded by the Office of Science (BER), US Department of Energy, Award No. DE-SC0006790. Additional support for field research was equally supported through the Integrated Field Research Challenge Site (IFRC) at Rifle, CO, USA, and the Lawrence Berkeley National Laboratory's Sustainable Systems Scientific Focus Area. Research at the Lawrence Berkeley National Laboratory was supported by the US Department of Energy (DOE), Office of Science (BER) under contract DE-AC02-05CH11231, the Subsurface Biogeochemistry Program (SBR) Grant Number DE-SC0004733, and by the Office of Basic Energy Sciences of the US Department of Energy under Contract No. DE-AC02-05CH11231. We thank Jillian Banfield for allowing us to analyze metagenomic and proteomic data generated by her laboratory at the University of California, Berkeley. NR 62 TC 4 Z9 4 U1 0 U2 41 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1751-7362 EI 1751-7370 J9 ISME J JI ISME J. PD FEB PY 2015 VL 9 IS 2 BP 333 EP 346 DI 10.1038/ismej.2014.128 PG 14 WC Ecology; Microbiology SC Environmental Sciences & Ecology; Microbiology GA AZ4SQ UT WOS:000348213600006 PM 25083935 ER PT J AU Youssef, NH Rinke, C Stepanauskas, R Farag, I Woyke, T Elshahed, MS AF Youssef, Noha H. Rinke, Christian Stepanauskas, Ramunas Farag, Ibrahim Woyke, Tanja Elshahed, Mostafa S. TI Insights into the metabolism, lifestyle and putative evolutionary history of the novel archaeal phylum 'Diapherotrites' SO ISME JOURNAL LA English DT Article ID ACID-MINE DRAINAGE; HORIZONTAL GENE-TRANSFER; MICROBIAL COMMUNITIES; SP-NOV.; HYPERTHERMOPHILIC ARCHAEA; GENOME SEQUENCE; SOLAR SALTERN; PHYLOGENETIC CHARACTERIZATION; SALINITY GRADIENT; MARINE-SEDIMENTS AB The archaeal phylum 'Diapherotrites' was recently proposed based on phylogenomic analysis of genomes recovered from an underground water seep in an abandoned gold mine (Homestake mine in Lead, SD, USA). Here we present a detailed analysis of the metabolic capabilities and genomic features of three single amplified genomes (SAGs) belonging to the 'Diapherotrites'. The most complete of the SAGs, Candidatus 'Iainarchaeum andersonii' (Cand. IA), had a small genome (similar to 1.24 Mb), short average gene length (822 bp), one ribosomal RNA operon, high coding density (similar to 90.4%), high percentage of overlapping genes (27.6%) and low incidence of gene duplication (2.16%). Cand. IA genome possesses limited catabolic capacities that, nevertheless, could theoretically support a free-living lifestyle by channeling a narrow range of substrates such as ribose, polyhydroxybutyrate and several amino acids to acetyl-coenzyme A. On the other hand, Cand. IA possesses relatively well-developed anabolic capabilities, although it remains auxotrophic for several amino acids and cofactors. Phylogenetic analysis suggests that the majority of Cand. IA anabolic genes were acquired from bacterial donors via horizontal gene transfer. We thus propose that members of the 'Diapherotrites' have evolved from an obligate symbiotic ancestor by acquiring anabolic genes from bacteria that enabled independent biosynthesis of biological molecules previously acquired from symbiotic hosts. 'Diapherotrites' 16S rRNA genes exhibit multiple mismatches with the majority of archaeal 16S rRNA primers, a fact that could be responsible for their observed rarity in amplicon-generated data sets. The limited substrate range, complex growth requirements and slow growth rate predicted could be responsible for its refraction to isolation. C1 [Youssef, Noha H.; Farag, Ibrahim; Elshahed, Mostafa S.] Oklahoma State Univ, Dept Microbiol & Mol Genet, Stillwater, OK 74074 USA. [Rinke, Christian; Woyke, Tanja] DOE Joint Genome Inst, Walnut Creek, CA USA. [Stepanauskas, Ramunas] Bigelow Lab Ocean Sci, E Boothbay, ME USA. RP Youssef, NH (reprint author), Oklahoma State Univ, Dept Microbiol & Mol Genet, 1110S Innovat Way Dr, Stillwater, OK 74074 USA. EM noha@okstate.edu OI Rinke, Christian/0000-0003-4632-1187; Farag, Ibrahim/0000-0002-5732-4108; Stepanauskas, Ramunas/0000-0003-4458-3108 FU National Science Foundation Microbial Observatories Program [EF0801858] FX This work was supported by the National Science Foundation Microbial Observatories Program (Grant EF0801858). NR 104 TC 6 Z9 6 U1 2 U2 27 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1751-7362 EI 1751-7370 J9 ISME J JI ISME J. PD FEB PY 2015 VL 9 IS 2 BP 447 EP 460 DI 10.1038/ismej.2014.141 PG 14 WC Ecology; Microbiology SC Environmental Sciences & Ecology; Microbiology GA AZ4SQ UT WOS:000348213600015 PM 25083931 ER PT J AU Woebken, D Burow, LC Behnam, F Mayali, X Schintlmeister, A Fleming, ED Prufert-Bebout, L Singer, SW Cortes, AL Hoehler, TM Pett-Ridge, J Spormann, AM Wagner, M Weber, PK Bebout, BM AF Woebken, Dagmar Burow, Luke C. Behnam, Faris Mayali, Xavier Schintlmeister, Arno Fleming, Erich D. Prufert-Bebout, Leslie Singer, Steven W. Lopez Cortes, Alejandro Hoehler, Tori M. Pett-Ridge, Jennifer Spormann, Alfred M. Wagner, Michael Weber, Peter K. Bebout, Brad M. TI Revisiting N-2 fixation in Guerrero Negro intertidal microbial mats with a functional single-cell approach SO ISME JOURNAL LA English DT Article ID SULFATE-REDUCING BACTERIA; IN-SITU HYBRIDIZATION; NITROGEN-FIXATION; CYANOBACTERIAL MATS; OLIGONUCLEOTIDE MICROARRAY; COMMUNITY STRUCTURE; BAJA-CALIFORNIA; GENE-EXPRESSION; LYNGBYA-SP; MARINE AB Photosynthetic microbial mats are complex, stratified ecosystems in which high rates of primary production create a demand for nitrogen, met partially by N-2 fixation. Dinitrogenase reductase (nifH) genes and transcripts from Cyanobacteria and heterotrophic bacteria (for example, Deltaproteobacteria) were detected in these mats, yet their contribution to N-2 fixation is poorly understood. We used a combined approach of manipulation experiments with inhibitors, nifH sequencing and single-cell isotope analysis to investigate the active diazotrophic community in intertidal microbial mats at Laguna Ojo de Liebre near Guerrero Negro, Mexico. Acetylene reduction assays with specific metabolic inhibitors suggested that both sulfate reducers and members of the Cyanobacteria contributed to N-2 fixation, whereas N-15(2) tracer experiments at the bulk level only supported a contribution of Cyanobacteria. Cyanobacterial and nifH Cluster III (including deltaproteobacterial sulfate reducers) sequences dominated the nifH gene pool, whereas the nifH transcript pool was dominated by sequences related to Lyngbya spp. Single-cell isotope analysis of N-15(2)-incubated mat samples via high-resolution secondary ion mass spectrometry (NanoSIMS) revealed that Cyanobacteria were enriched in N-15, with the highest enrichment being detected in Lyngbya spp. filaments (on average 4.4 at% N-15), whereas the Deltaproteobacteria (identified by CARD-FISH) were not significantly enriched. We investigated the potential dilution effect from CARD-FISH on the isotopic composition and concluded that the dilution bias was not substantial enough to influence our conclusions. Our combined data provide evidence that members of the Cyanobacteria, especially Lyngbya spp., actively contributed to N-2 fixation in the intertidal mats, whereas support for significant N-2 fixation activity of the targeted deltaproteobacterial sulfate reducers could not be found. C1 [Woebken, Dagmar; Burow, Luke C.; Spormann, Alfred M.] Stanford Univ, Dept Chem Engn, Stanford, CA 94305 USA. [Woebken, Dagmar; Burow, Luke C.; Spormann, Alfred M.] Stanford Univ, Dept Civil & Environm Engn, Stanford, CA 94305 USA. [Woebken, Dagmar; Burow, Luke C.; Fleming, Erich D.; Prufert-Bebout, Leslie; Hoehler, Tori M.; Bebout, Brad M.] NASA, Exobiol Branch, Ames Res Ctr, Moffett Field, CA USA. [Woebken, Dagmar; Behnam, Faris; Wagner, Michael] Univ Vienna, Dept Microbiol & Ecosyst Sci, Div Microbial Ecol, A-1090 Vienna, Austria. [Mayali, Xavier; Pett-Ridge, Jennifer; Weber, Peter K.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA USA. [Schintlmeister, Arno; Wagner, Michael] Univ Vienna, Large Instrument Facil Adv Isotope Res, A-1090 Vienna, Austria. [Singer, Steven W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Lopez Cortes, Alejandro] Northwestern Ctr Biol Res CIBNOR, Lab Geomicrobiol & Biotechnol, La Paz, Mexico. RP Woebken, D (reprint author), Univ Vienna, Dept Microbiol & Ecosyst Sci, Div Microbial Ecol, Waehringer Guertel 18, A-1090 Vienna, Austria. EM dwoebken@gmail.com; brad.m.bebout@nasa.gov RI Woebken, Dagmar/A-4447-2013; Wagner, Michael/A-7801-2011; OI Wagner, Michael/0000-0002-9778-7684; Woebken, Dagmar/0000-0002-1314-9926 FU National Commission of Aquaculture and Fishery of the Ministry of Agriculture, Livestock, Rural Development, Fisheries and Food (Mexico) [DAPA/2/080310/734]; DOE [DE-AC52-07NA27344, DE-AC02-05CH11231]; U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, Genomic Sciences Program [SCW1039]; German Research Foundation (Deutsche Forschungsgemeinschaft); Austrian Science Fund (FWF) [P 25700-B20]; European Research Council [294343] FX We thank Angela Detweiler, Jan Dolinsek, Mike Kubo and Christina Ramon for their excellent technical assistance, Jose Q Garcia-Maldonado for his assistance in the field, Andrew McDowell at UC Berkeley for IRMS analyses, and Stephanie A Eichorst for helpful comments on the manuscript. We are grateful for access to the field site and for the logistical support provided by Exportadora de Sal, S.A. de C.V. This work was performed under Fishery Permit DAPA/2/080310/734 granted by the National Commission of Aquaculture and Fishery of the Ministry of Agriculture, Livestock, Rural Development, Fisheries and Food (Mexico). Work at LLNL was performed under the auspices of the DOE under contract DE-AC52-07NA27344. Work at LBNL was performed under the auspices of the DOE under contract DE-AC02-05CH11231. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, Genomic Sciences Program, under contract number SCW1039. This work was further financially supported by the German Research Foundation (Deutsche Forschungsgemeinschaft) (to DW) and the Austrian Science Fund (FWF) (P 25700-B20 to DW). FB and MW were supported by the European Research Council (Advanced Grant Nitrification Reloaded (NITRI-CARE) 294343). NR 53 TC 13 Z9 13 U1 11 U2 54 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1751-7362 EI 1751-7370 J9 ISME J JI ISME J. PD FEB PY 2015 VL 9 IS 2 BP 485 EP 496 DI 10.1038/ismej.2014.144 PG 12 WC Ecology; Microbiology SC Environmental Sciences & Ecology; Microbiology GA AZ4SQ UT WOS:000348213600018 PM 25303712 ER PT J AU Davis, RW Carvalho, BJ Jones, HDT Singh, S AF Davis, Ryan W. Carvalho, Benjamin J. Jones, Howland D. T. Singh, Seema TI The role of photo-osmotic adaptation in semi-continuous culture and lipid particle release from Dunaliella viridis SO JOURNAL OF APPLIED PHYCOLOGY LA English DT Article DE Microalgae; Dunaliella viridis; Algae bioproducts; Semi-continuous culture; Photo-osmotic adaptation; Lipid microparticles; Algal milking ID GLYCEROL-3-PHOSPHATE DEHYDROGENASE EC-1.1.1.8; UNICELLULAR GREEN-ALGA; PARTIAL-PURIFICATION; HALOPHILIC ALGA; CHLOROPHYLL EQUATIONS; RAMAN-SPECTROSCOPY; ETHANOL SOLVENTS; HYPERTONIC SHOCK; INTRACELLULAR PH; SALINA AB Although great efforts have been made to elucidate the phenotypic responses of alga to varying levels of nutrients, osmotic environments, and photosynthetically active radiation intensities, the role of interactions among these variables is largely nebulous. Here, we describe a general method for establishing and maintaining semi-continuous cultures of the halophilic microalgal production strain, Dunaliella viridis, that is independent of variations in salinity and illumination intensity. Using this method, the cultures were evaluated to elucidate the overlapping roles of photosynthetic and osmotic adaptation on the accumulation and compositional variation of the biomass, photosynthetic productivity, and physiological biomarkers, as well as spectroscopic and morphological details at the single-cell level. Correlation matrices defining the relationships among the observables and based on variation of the illumination intensity and salinity were constructed for predicting bioproduct yields for varying culture conditions. Following maintenance of stable cultures for 6-week intervals, phenotypic responses to photo-osmotic drift were explored using a combination of single-cell hyperspectral fluorescence imaging and flow cytometry. In addition to morphological changes, release of lipid microparticles from the cells that is disproportionate to cell lysis was observed under hypotonic drift, indicating the existence of a reversible membrane permeation mechanism in Dunaliella. This phenomenon introduces the potential for low-cost strategies for recovering lipids and pigments from the microalgae by minimizing the requirement for energy intensive harvesting and dewatering of the biomass. The results should be applicable to outdoor culture, where seasonal changes resulting in variable solar flux and precipitation and evaporation rates are anticipated. C1 [Davis, Ryan W.; Carvalho, Benjamin J.; Singh, Seema] Sandia Natl Labs, Livermore, CA 94551 USA. [Jones, Howland D. T.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Singh, S (reprint author), Sandia Natl Labs, Livermore, CA 94551 USA. EM seesing@sandia.gov FU United States Department of Energy [DE-ACO4-94AL85000]; Sandia National Laboratories' Laboratory Directed Research and Development FX Sandia is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy under Contract DE-ACO4-94AL85000. Support is acknowledged from Sandia National Laboratories' Laboratory Directed Research and Development projects titled, "From algae to oilgae: In situ studies of the factors controlling growth and oil production in microalgae," Seema Singh (PI) and "Self-deconstructing algal biomass for transportation fuels," Ryan W. Davis (PI). NR 75 TC 3 Z9 3 U1 3 U2 34 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0921-8971 EI 1573-5176 J9 J APPL PHYCOL JI J. Appl. Phycol. PD FEB PY 2015 VL 27 IS 1 BP 109 EP 123 DI 10.1007/s10811-014-0331-5 PG 15 WC Biotechnology & Applied Microbiology; Marine & Freshwater Biology SC Biotechnology & Applied Microbiology; Marine & Freshwater Biology GA AZ3OU UT WOS:000348137600009 ER PT J AU Turner, DZ AF Turner, D. Z. TI Peridynamics-Based Digital Image Correlation Algorithm Suitable for Cracks and Other Discontinuities SO JOURNAL OF ENGINEERING MECHANICS LA English DT Article DE Digital image correlation; Peridynamics; Experimental fracture mechanics; Nonlocal methods; Damage ID ELASTICITY THEORY; MECHANICS AB This work presents a novel approach to circumventing the difficulties associated with using digital image correlation (DIC) for problems that involve discontinuities like fracture and fragmentation. The proposed method provides a simple means to combine traditional DIC approaches with peridynamics to achieve full-field displacements, even in the vicinity of cracks. In regions where DIC is accurate and effective, the displacement field is determined using a traditional approach. In discontinuous regions, the displacement field is solved for using peridynamics. This study shows that this method can be used successfully for investigating damage in materials such as nuclear graphite and fiberRC (FRC). It also shows that the proposed method alleviates nonphysical strains in the vicinity of cracks, common to alternative approaches, which detrimentally degrade the quality of postprocessed quantities of interest such as fracture toughness. (C) 2014 American Society of Civil Engineers. C1 [Turner, D. Z.] Univ Stellenbosch, Dept Civil Engn, ZA-7602 Stellenbosch, South Africa. [Turner, D. Z.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Turner, DZ (reprint author), Univ Stellenbosch, Dept Civil Engn, ZA-7602 Stellenbosch, South Africa. EM dzturne@sandia.gov FU Institute for Structural Engineering at Stellenbosch University; U.S. DOE's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the Institute for Structural Engineering at Stellenbosch University. Their support is gratefully acknowledged. The author thanks Professor Billy Boshoff for providing the images used for the examples related to FRC. The author also thanks Dr. Thorsten Becker for the data related to nuclear graphite and many helpful discussions on this topic. Lastly, Johan Conradie and Matt Molteno are thanked for their assistance in obtaining the experimental results for nuclear graphite. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. DOE's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 15 TC 0 Z9 0 U1 2 U2 16 PU ASCE-AMER SOC CIVIL ENGINEERS PI RESTON PA 1801 ALEXANDER BELL DR, RESTON, VA 20191-4400 USA SN 0733-9399 EI 1943-7889 J9 J ENG MECH JI J. Eng. Mech. PD FEB PY 2015 VL 141 IS 2 AR 04014115 DI 10.1061/(ASCE)EM.19437889.0000831 PG 10 WC Engineering, Mechanical SC Engineering GA AZ4PB UT WOS:000348203700011 ER PT J AU Agbaglah, G Thoraval, MJ Thoroddsen, ST Zhang, LV Fezzaa, K Deegan, RD AF Agbaglah, G. Thoraval, M. -J Thoroddsen, S. T. Zhang, L. V. Fezzaa, K. Deegan, R. D. TI Drop impact into a deep pool: vortex shedding and jet formation SO JOURNAL OF FLUID MECHANICS LA English DT Article DE breakup/coalescence; drops; drops and bubbles ID SINGLE DROP; ADAPTIVE SOLVER; CROWN FORMATION; EJECTA SHEET; LIQUID-FILMS; SURFACES; ENTRAINMENT; ENTRAPMENT; SPLASH; WAVES AB One of the simplest splashing scenarios results from the impact of a single drop on a deep pool. The traditional understanding of this process is that the impact generates an axisymmetric sheet-like jet that later breaks up into secondary droplets. Recently it was shown that even this simplest of scenarios is more complicated than expected because multiple jets can be generated from a single impact event and there are transitions in the multiplicity of jets as the experimental parameters are varied. Here, we use experiments and numerical simulations of a single drop impacting on a deep pool to examine the transition from impacts that produce a single jet to those that produce two jets. Using high-speed X-ray imaging methods we show that vortex separation within the drop leads to the formation of a second jet long after the formation of the ejecta sheet. Using numerical simulations we develop a phase diagram for this transition and show that the capillary number is the most appropriate order parameter for the transition. C1 [Agbaglah, G.; Zhang, L. V.; Deegan, R. D.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Agbaglah, G.; Zhang, L. V.; Deegan, R. D.] Univ Michigan, Ctr Study Complex Syst, Ann Arbor, MI 48109 USA. [Thoraval, M. -J; Thoroddsen, S. T.] KAUST, Div Phys Sci & Engn, Thuwal 239556900, Saudi Arabia. [Thoraval, M. -J; Thoroddsen, S. T.] KAUST, Clean Combust Res Ctr, Thuwal 239556900, Saudi Arabia. [Thoraval, M. -J] Univ Twente, Mesa Inst, Fac Sci & Technol, Phys Fluids Grp, NL-7500 AE Enschede, Netherlands. [Fezzaa, K.] Xray Sci Div, Argonne Natl Lab, Argonne, IL 60439 USA. RP Agbaglah, G (reprint author), Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. EM agbagla@umich.edu RI Thoraval, Marie-Jean/A-7255-2010; OI Thoraval, Marie-Jean/0000-0002-6590-0603; Thoroddsen, Sigurdur T/0000-0001-6997-4311 FU McDonnell Foundation FX The authors thank the James S. McDonnell Foundation for support through a 21st Century Science Initiative in Studying Complex Systems Research Award, S. Weiss and J. Soundar Jerome for valuable discussions, and Claudio Falcon for assistance with the experiments. NR 33 TC 11 Z9 11 U1 4 U2 50 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0022-1120 EI 1469-7645 J9 J FLUID MECH JI J. Fluid Mech. PD FEB PY 2015 VL 764 AR R1 DI 10.1017/jfm.2014.723 PG 12 WC Mechanics; Physics, Fluids & Plasmas SC Mechanics; Physics GA AZ3LK UT WOS:000348128700001 ER PT J AU Briceno, RA Davoudi, Z Luu, TC AF Briceno, Raul A. Davoudi, Zohreh Luu, Thomas C. TI Nuclear reactions from lattice QCD SO JOURNAL OF PHYSICS G-NUCLEAR AND PARTICLE PHYSICS LA English DT Review DE lattice quantum chromodynamics; nuclear reactions; scattering; resonances ID EFFECTIVE-FIELD THEORY; CHIRAL PERTURBATION-THEORY; CORE-SHELL-MODEL; TWISTED BOUNDARY-CONDITIONS; SHORT-RANGE INTERACTIONS; FINITE-VOLUME; MATRIX-ELEMENTS; PHASE-SHIFTS; FORM-FACTORS; HADRON INTERACTIONS AB One of the overarching goals of nuclear physics is to rigorously compute properties of hadronic systems directly from the fundamental theory of strong interactions, quantum chromodynamics (QCD). In particular, the hope is to perform reliable calculations of nuclear reactions which will impact our understanding of environments that occur during big bang nucleosynthesis, the evolution of stars and supernovae, and within nuclear reactors and high energy/density facilities. Such calculations, being truly ab initio, would include all two-nucleon and three-nucleon (and higher) interactions in a consistent manner. Currently, lattice quantum chromodynamics (LQCD) provides the only reliable option for performing calculations of some of the low-energy hadronic observables. With the aim of bridging the gap between LQCD and nuclear many-body physics, the Institute for Nuclear Theory held a workshop on Nuclear Reactions from LQCD on March 2013. In this review article, we report on the topics discussed in this workshop and the path planned to move forward in the upcoming years. C1 [Briceno, Raul A.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Davoudi, Zohreh] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Davoudi, Zohreh] Univ Washington, Inst Nucl Theory, Seattle, WA 98195 USA. [Luu, Thomas C.] Forschungszentrum Julich, Inst Adv Simulat, Inst Kernphys, D-52425 Julich, Germany. [Luu, Thomas C.] Forschungszentrum Julich, Julich Ctr Hadron Phys, D-52425 Julich, Germany. RP Briceno, RA (reprint author), Thomas Jefferson Natl Accelerator Facil, 12000 Jefferson Ave, Newport News, VA 23606 USA. EM rbriceno@jlab.org; davoudi@uw.edu; t.luu@fz-juelich.de OI Briceno, Raul/0000-0003-1109-1473 FU U.S. Department of Energy under Jefferson Science Associates, LLC [DE-AC05-06OR23177]; DOE [DE-FG02-97ER41014, DE-FG02-00ER41132] FX We gratefully acknowledge discussions with, and supports from, Martin Savage and David Kaplan. We would like to thank all the participants of the workshop for their contributions, and for promoting inspiring discussions, and the help from the extremely kind staff of the Institute for Nuclear Theory. We appreciate useful discussions with Jozef Dudek, Peng Guo, Maxwell Hansen, Dean Lee and Achim Schwenk and their permission to use the corresponding figures. We also would like to thank Achim Schwenk and Michael Wagman for comments on the initial draft of this review. RB acknowledges support from the U.S. Department of Energy contract DE-AC05-06OR23177, under which Jefferson Science Associates, LLC, manages and operates the Jefferson Laboratory. ZD was supported in part by DOE grant No. DE-FG02-97ER41014 and by DOE grant No. DE-FG02-00ER41132. NR 317 TC 11 Z9 11 U1 3 U2 15 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0954-3899 EI 1361-6471 J9 J PHYS G NUCL PARTIC JI J. Phys. G-Nucl. Part. Phys. PD FEB PY 2015 VL 42 IS 2 AR 023101 DI 10.1088/0954-3899/42/2/023101 PG 35 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA AZ3MA UT WOS:000348130400001 ER PT J AU Wood, DL Li, JL Daniel, C AF Wood, David L., III Li, Jianlin Daniel, Claus TI Prospects for reducing the processing cost of lithium ion batteries SO JOURNAL OF POWER SOURCES LA English DT Article DE Lithium-ion battery; Cost reduction study; Electrode processing; Aqueous colloidal chemistry; Thick electrodes; Formation cycle ID SOLID-ELECTROLYTE INTERPHASE; LICOO2 CATHODES; CELL PERFORMANCE; ELECTROCHEMICAL PERFORMANCE; DISPERSION HOMOGENEITY; LIFEPO4 CATHODES; OPTIMIZATION; GRAPHITE; BINDER; INTERCALATION AB A detailed processing cost breakdown is given for lithium-ion battery (LIB) electrodes, which focuses on: 1) elimination of toxic, costly N-methylpyrrolidone (NMP) dispersion chemistry; 2) doubling the thicknesses of the anode and cathode to raise energy density; and 3) reduction of the anode electrolyte wetting and SEI-layer formation time. These processing cost reduction technologies generically adaptable to any anode or cathode cell chemistry and are being implemented at ORNL This paper shows step by step how these cost savings can be realized in existing or new LIB manufacturing plants using a baseline case of thin (power) electrodes produced with NMP processing and a standard 10-14-day wetting and formation process. In particular, it is shown that aqueous electrode processing can cut the electrode processing cost and energy consumption by an order of magnitude. Doubling the thickness of the electrodes allows for using half of the inactive current collectors and separators, contributing even further to the processing cost savings. Finally wetting and RI-layer formation cost savings are discussed in the context of a protocol with significantly reduced time. These three benefits collectively offer the possibility of reducing LIB pack cost from $502.8 kW h(-1)-usable to $370.3 kW h(-1)-usable, a savings of $132.5/kWh (or 26.4%). (C) 2014 The Authors. Published by Elsevier B.V. C1 [Wood, David L., III; Li, Jianlin; Daniel, Claus] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. RP Wood, DL (reprint author), Oak Ridge Natl Lab, Energy & Transportat Sci Div, One Bethel Valley Rd,POB 2008, Oak Ridge, TN 37831 USA. EM wooddl@ornl.gov RI Daniel, Claus/A-2060-2008; OI Daniel, Claus/0000-0002-0571-6054; Wood, David/0000-0002-2471-4214; Li, Jianlin/0000-0002-8710-9847 FU U.S. Department of Energy (DOE) [DE-AC05-00OR22725]; Office of Energy Efficiency and Renewable Energy (EERE) Vehicle Technologies Office (VTO) (Program Manager: David Howell) Applied Battery Research subprogram (Program Manager: Peter Faguy) FX This research at Oak Ridge National Laboratory, managed by UT Battelle, LLC, for the U.S. Department of Energy (DOE) under contract DE-AC05-00OR22725, was sponsored by the Office of Energy Efficiency and Renewable Energy (EERE) Vehicle Technologies Office (VTO) (Program Manager: David Howell) Applied Battery Research subprogram (Program Manager: Peter Faguy). The authors would also like to thank Gabriel Veith, Andrew Payzant, Peter Faguy, and Jack Deppe for helpful technical discussions in finalizing the manuscript. NR 45 TC 50 Z9 50 U1 40 U2 125 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD FEB 1 PY 2015 VL 275 BP 234 EP 242 PG 9 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA AZ2UT UT WOS:000348088400031 ER PT J AU Paxton, WA Zhong, Z Tsakalakos, T AF Paxton, William A. Zhong, Zhong Tsakalakos, Thomas TI Tracking inhomogeneity in high-capacity lithium iron phosphate batteries SO JOURNAL OF POWER SOURCES LA English DT Article DE Inhomogeneity; X-ray diffraction; Lithium iron phosphate; Heterogeneous electrode; Characterization; In-situ ID LIFEPO4; TRANSFORMATION; VISUALIZATION; DYNAMICS; CATHODE AB Energy-dispersive x-ray diffraction (EDXRD) is one of the few techniques that can internally probe a sealed battery under operating conditions. In this paper, we use EDXRD with ultrahigh energy synchrotron radiation to track inhomogeneity in a cycled high-capacity lithium iron phosphate cell under in-situ and operando conditions. A sequence of depth-profile x-ray diffraction spectra are collected with 40 gm resolution as the cell is discharged. Additionally, nine different locations of the cell are tracked independently throughout a second discharge process. In each case, a two-peak reference intensity ratio analysis (RIR) was used on the LiFePO4 311 and the FePO4 020 reflections to estimate the relative phase abundance of the lithiated and non-lithiated phases. The data provide a first-time look at the dynamics of electrochemical inhomogeneity in a real-world battery. We observe a strong correlation between inhomogeneity and overpotential in the galvanic response of the cell. Additionally, the data closely follow the behavior that is predicted by the resistive-reactant model originally proposed by Thomas-Alyea. Despite a non-linear response in the independently measured locations, the behavior of the ensemble is strikingly linear. This suggests that effects of inhomogeneity can be elusive and highlights the power of the EDXRD technique. (C) 2014 Elsevier B.V. All rights reserved. C1 [Paxton, William A.; Tsakalakos, Thomas] Rutgers State Univ, Piscataway, NJ 08854 USA. [Zhong, Zhong] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Paxton, WA (reprint author), Rutgers State Univ, Dept Mat Sci & Engn, 607 Taylor Rd, Piscataway, NJ 08854 USA. EM will.paxton@rutgers.edu OI Paxton, William/0000-0001-5899-9038 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX The authors gratefully acknowledge Ankur Choksi, and Bart Visser for their support in the laboratory. The authors also acknowledge General Electric for the use of use of their battery cycler and their efforts in improving the beamline. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 31 TC 9 Z9 9 U1 6 U2 46 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD FEB 1 PY 2015 VL 275 BP 429 EP 434 DI 10.1016/j.jpowsour.2014.11.035 PG 6 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA AZ2UT UT WOS:000348088400054 ER PT J AU Piper, DM Son, SB Travis, JJ Lee, Y Han, SS Kim, SC Oh, KH George, SM Lee, SH Ban, CM AF Piper, Daniela Molina Son, Seoung-Bum Travis, Jonathan J. Lee, Younghee Han, Sang Sub Kim, Seul Cham Oh, Kyu Hwan George, Steven M. Lee, Se-Hee Ban, Chunmei TI Mitigating irreversible capacity losses from carbon agents via surface modification SO JOURNAL OF POWER SOURCES LA English DT Article DE Lithium-ion battery; Atomic layer deposition; Molecular layer deposition; Irreversible capacity loss ID ATOMIC LAYER DEPOSITION; LITHIUM-ION BATTERIES; LECLANCHE TYPE BATTERIES; COMPOSITE ELECTRODES; LI INSERTION; CATHODES; BEHAVIOR; BLACK; STABILITY; ANODE AB Greatly improved cycling performance has been demonstrated with conformally coated lithium-ion electrodes by atomic layer deposition (ALD) and molecular layer deposition (MLD) techniques. This paper reports the impact of coating on the electrode additives towards mitigating undesired parasitic reactions during cycling. The ALD and MLD coatings with conformality and atomic scale thickness control effectively stabilize the surface of the electrode components, and the current collector, resulting in the increase of coulombic efficiency throughout cycling. The organic fragment integrated into the recently developed MLD process allows the coating to possess excellent mechanical properties and enhanced ionic conductivity, which significantly reduces cell polarizations throughout cycling. This work validates the importance of ALD and MLD as surface modifiers and further demonstrates their versatility and compatibility with lithium-ion battery technology. (C) 2014 Elsevier B.V. All rights reserved. C1 [Piper, Daniela Molina; George, Steven M.; Lee, Se-Hee] Univ Colorado, Dept Mech Engn, Boulder, CO 80309 USA. [Piper, Daniela Molina; Son, Seoung-Bum; Ban, Chunmei] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Travis, Jonathan J.; Lee, Younghee; George, Steven M.] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. [Han, Sang Sub; Kim, Seul Cham; Oh, Kyu Hwan] Seoul Natl Univ, Dept Mat Sci & Engn, Seoul 151742, South Korea. RP Ban, CM (reprint author), Natl Renewable Energy Lab, 1617 Cole Blvd, Golden, CO 80401 USA. EM chunmei.ban@nrel.gov RI Lee, Sehee/A-5989-2011; Lee, Younghee/C-1793-2015; George, Steven/O-2163-2013; Son, Seoung-Bum/C-6783-2014 OI George, Steven/0000-0003-0253-9184; FU Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies for the U.S. Department of Energy under [DE-AC-36-08GO28308, NFT-8-88527-01]; Fundamental R&D Program for Technology of World Premier Materials; Ministry of Knowledge Economy, Republic of Korea [10037919]; NREL Lab Directed Research and Development (LDRD) program FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies for the U.S. Department of Energy under Contract No. DE-AC-36-08GO28308, subcontract No. NFT-8-88527-01 under the Batteries for Advanced Transportation Technologies (BATT) Program, and by a grant from the Fundamental R&D Program for Technology of World Premier Materials funded by the Ministry of Knowledge Economy, Republic of Korea (10037919). We would also like to acknowledge the financial support from NREL Lab Directed Research and Development (LDRD) program. NR 33 TC 4 Z9 4 U1 7 U2 45 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD FEB 1 PY 2015 VL 275 BP 605 EP 611 DI 10.1016/j.jpowsour.2014.11.032 PG 7 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA AZ2UT UT WOS:000348088400074 ER PT J AU Poineau, F German, KE Burton-Pye, BP Weck, PF Kim, E Kriyzhovets, O Safonov, A Ilin, V Francesconi, LC Sattelberger, AP Czerwinski, KR AF Poineau, Frederic German, Konstantin E. Burton-Pye, Benjamin P. Weck, Philippe F. Kim, Eunja Kriyzhovets, Olga Safonov, Aleksey Ilin, Viktor Francesconi, Lynn C. Sattelberger, Alfred P. Czerwinski, Kenneth R. TI Speciation of technetium peroxo complexes in sulfuric acid revisited SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article DE Technetium; Peroxo complexes; Speciation; Sulfuric acid AB The reaction of Tc(+7) with H2O2 has been studied in H2SO4 and the speciation of technetium performed by UV-visible and 99-Tc NMR spectroscopy. UV-visible measurements show that for H2SO4 a parts per thousand yen 9 M and H2O2 = 0.17 M, TcO3(OH)(H2O)(2) reacts immediately and blue solutions are obtained, while no reaction occurs for H2SO4 < 9 M. The spectra of the blue solutions exhibit bands centered around 520 and 650 nm which are attributed to Tc(+7) peroxo species. Studies in 6 M H2SO4 show that TcO4 (-) begins to react for H2O2 = 2.12 M and red solutions are obtained. The UV-visible spectra of the red species are identical to the one obtained from the reaction of TcO4 (-) with H2O2 in HNO3 and consistent with the presence of TcO(O-2)(2)(H2O)(OH). The 99-Tc NMR spectrum of the red solution exhibits a broad signal centered at +5.5 ppm vs TcO4 (-) and is consistent with the presence of a low symmetry Tc(+7) molecule. C1 [Poineau, Frederic; Czerwinski, Kenneth R.] Univ Nevada, Dept Chem, Las Vegas, NV 89154 USA. [German, Konstantin E.; Safonov, Aleksey; Ilin, Viktor] Russian Acad Sci, AN Frumkin Inst Phys Chem & Electrochem, Moscow, Russia. [Burton-Pye, Benjamin P.; Francesconi, Lynn C.] CUNY Hunter Coll, Dept Chem, New York, NY 10021 USA. [Weck, Philippe F.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Kim, Eunja] Univ Nevada, Dept Phys & Astron, Las Vegas, NV 89154 USA. [Kriyzhovets, Olga; Ilin, Viktor] Med Inst REAVIZ, Moscow Branch, Moscow, Russia. [Sattelberger, Alfred P.] Argonne Natl Lab, Energy Engn & Syst Anal Directorate, Lemont, IL USA. RP Poineau, F (reprint author), Univ Nevada, Dept Chem, Las Vegas, NV 89154 USA. EM poineauf@unlv.nevada.edu RI Safonov, Alexey/C-2582-2014; German, Konstantin/B-7694-2011; OI Safonov, Alexey/0000-0001-6920-4659; German, Konstantin/0000-0003-2368-4081; , Philippe/0000-0002-7610-2893 FU U.S. Department of Energy, Office of Nuclear Energy, NEUP grant through INL/BEA [321 LLC, 00129169, DE-AC07-05ID14517]; National Science Foundation [NSF-CHE 0750118, NSF-CHE-0959617]; U. S Department of Energy [DE-FG02-09ER16097, DE-SC0002456]; National Center for Research Resources (NCRR), a component of the National Institutes of Health (NIH) [RR003037]; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Funding for this research was provided by the U.S. Department of Energy, Office of Nuclear Energy, NEUP grant through INL/BEA, 321 LLC, 00129169, agreement number DE-AC07-05ID14517. Further supports were provided by the National Science Foundation (Grant NSF-CHE 0750118 and Grant NSF-CHE-0959617 for purchase of the 400 MHz NMR spectrometer at Hunter College) and the U. S Department of Energy, Grant DE-FG02-09ER16097 (Heavy Element Chemistry, Office of Science) and Grant DE-SC0002456 (Biological and Environmental Research, Office of Science). Infrastructure at Hunter College is partially supported by Grant RR003037 from the National Center for Research Resources (NCRR), a component of the National Institutes of Health (NIH). Sandia National Laboratories is a multiprogram laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. The authors thank Trevor Low and Julie Bertoia for outstanding health physics support. NR 11 TC 2 Z9 2 U1 1 U2 15 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD FEB PY 2015 VL 303 IS 2 BP 1163 EP 1167 DI 10.1007/s10967-014-3434-1 PG 5 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA AZ4LJ UT WOS:000348192200017 ER PT J AU Rudolph, D Forsberg, U Golubev, P Sarmiento, LG Yakushev, A Andersson, LL Di Nitto, A Dullmann, CE Gates, JM Gregorich, KE Gross, CJ Herzberg, RD Hessberger, FP Khuyagbaatar, J Kratz, JV Rykaczewski, K Schadel, M Aberg, S Ackermann, D Block, M Brand, H Carlsson, BG Cox, D Derkx, X Eberhardt, K Even, J Fahlander, C Gerl, J Jager, E Kindler, B Krier, J Kojouharov, I Kurz, N Lommel, B Mistry, A Mokry, C Nitsche, H Omtvedt, JP Papadakis, P Ragnarsson, I Runke, J Schaffner, H Schausten, B Thorle-Pospiech, P Torres, T Traut, T Trautmann, N Turler, A Ward, A Ward, DE Wiehl, N AF Rudolph, D. Forsberg, U. Golubev, P. Sarmiento, L. G. Yakushev, A. Andersson, L-L. Di Nitto, A. Dullmann, Ch. E. Gates, J. M. Gregorich, K. E. Gross, C. J. Herzberg, R-D. Hessberger, F. P. Khuyagbaatar, J. Kratz, J. V. Rykaczewski, K. Schaedel, M. Aberg, S. Ackermann, D. Block, M. Brand, H. Carlsson, B. G. Cox, D. Derkx, X. Eberhardt, K. Even, J. Fahlander, C. Gerl, J. Jaeger, E. Kindler, B. Krier, J. Kojouharov, I. Kurz, N. Lommel, B. Mistry, A. Mokry, C. Nitsche, H. Omtvedt, J. P. Papadakis, P. Ragnarsson, I. Runke, J. Schaffner, H. Schausten, B. Thoerle-Pospiech, P. Torres, T. Traut, T. Trautmann, N. Tuerler, A. Ward, A. Ward, D. E. Wiehl, N. TI Selected spectroscopic results on element 115 decay chains SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article DE Superheavy elements; Nuclear spectroscopy; Nuclear structure ID HEAVIEST NUCLEI; CA-48-INDUCED REACTIONS; SUPERHEAVY ELEMENTS; ENERGIES; SPECTRA; MASSES; TASCA; GSI AB Thirty correlated alpha-decay chains were observed in an experiment studying the fusion-evaporation reaction Ca-48 + Am-243 at the GSI Helmholtzzentrum fur Schwerionenforschung. The decay characteristics of the majority of these 30 chains are consistent with previous observations and interpretations of such chains to originate from isotopes of element Z = 115. High-resolution alpha-photon coincidence spectroscopy in conjunction with comprehensive Monte-Carlo simulations allow to propose excitation schemes of atomic nuclei of the heaviest elements, thereby probing nuclear structure models near the 'Island of Stability' with unprecedented experimental precision. C1 [Rudolph, D.; Forsberg, U.; Golubev, P.; Sarmiento, L. G.; Aberg, S.; Carlsson, B. G.; Fahlander, C.; Ragnarsson, I.; Ward, D. E.] Lund Univ, S-22100 Lund, Sweden. [Yakushev, A.; Dullmann, Ch. E.; Hessberger, F. P.; Schaedel, M.; Ackermann, D.; Block, M.; Brand, H.; Gerl, J.; Jaeger, E.; Kindler, B.; Krier, J.; Kojouharov, I.; Kurz, N.; Lommel, B.; Runke, J.; Schaffner, H.; Schausten, B.; Torres, T.] GSI Helmholtzzentrum Schwerionenforsch GmbH, D-64291 Darmstadt, Germany. [Andersson, L-L.; Dullmann, Ch. E.; Hessberger, F. P.; Khuyagbaatar, J.; Derkx, X.; Eberhardt, K.; Even, J.; Mokry, C.; Thoerle-Pospiech, P.; Wiehl, N.] Helmholtz Inst Mainz, D-55099 Mainz, Germany. [Di Nitto, A.; Dullmann, Ch. E.; Kratz, J. V.; Derkx, X.; Eberhardt, K.; Mokry, C.; Thoerle-Pospiech, P.; Traut, T.; Trautmann, N.; Wiehl, N.] Johannes Gutenberg Univ Mainz, D-55099 Mainz, Germany. [Gates, J. M.; Gregorich, K. E.; Nitsche, H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Gross, C. J.; Rykaczewski, K.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Herzberg, R-D.; Cox, D.; Mistry, A.; Papadakis, P.; Ward, A.] Univ Liverpool, Liverpool L69 7ZE, Merseyside, England. [Schaedel, M.] Japan Atom Energy Agcy, Adv Sci Res Ctr, Tokai, Ibaraki, Japan. [Omtvedt, J. P.] Univ Oslo, N-0315 Oslo, Norway. [Tuerler, A.] Paul Scherrer Inst, CH-5232 Villigen, Switzerland. [Tuerler, A.] Univ Bern, CH-5232 Villigen, Switzerland. RP Rudolph, D (reprint author), Lund Univ, S-22100 Lund, Sweden. EM Dirk.Rudolph@nuclear.lu.se RI Block, Michael/I-2782-2015; Di Nitto, Antonio/C-5069-2011; Even, Julia/K-1186-2016; Turler, Andreas/D-3913-2014; OI Block, Michael/0000-0001-9282-8347; Di Nitto, Antonio/0000-0002-9319-366X; Even, Julia/0000-0002-6314-9094; Turler, Andreas/0000-0002-4274-1056; Ward, Andrew/0000-0002-6288-7327; Cox, Daniel/0000-0002-2790-8348; Papadakis, Philippos/0000-0001-7509-4257 FU European Community FP7-Capacities ENSAR [262010]; Royal Physiographic Society in Lund; Euroball Owners Committee; Swedish Research Council; German BMBF; Office of Nuclear Physics, U.S. Department of Energy; UK Science and Technology Facilities Council FX The authors would like to thank the ion-source and accelerator staff at GSI. This work is supported by the European Community FP7-Capacities ENSAR No. 262010, the Royal Physiographic Society in Lund, the Euroball Owners Committee, the Swedish Research Council, the German BMBF, the Office of Nuclear Physics, U.S. Department of Energy, and the UK Science and Technology Facilities Council. NR 39 TC 3 Z9 3 U1 1 U2 21 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD FEB PY 2015 VL 303 IS 2 BP 1185 EP 1190 DI 10.1007/s10967-014-3445-y PG 6 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA AZ4LJ UT WOS:000348192200021 ER PT J AU Gharibyan, N Moody, KJ Despotopulos, JD Grant, PM Shaughnessy, DA AF Gharibyan, Narek Moody, Kenton J. Despotopulos, John D. Grant, Patrick M. Shaughnessy, Dawn A. TI First fission yield measurements at the National Ignition Facility: 14-MeV neutron fission of U-238 SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article DE 14-MeV neutrons; Fission yields; U-238; TOAD; NIF AB The use of the Solid Radiochemistry diagnostic platform at the National Ignition Facility (NIF) has allowed the development and implementation of the Target Option Activation Device assembly for fielding materials of interest inside the NIF chamber during high yield neutron shots. Preliminary studies with ultra-depleted uranium have allowed for the measurements of fission yields of U-238. Radiochemical procedures were utilized for the separation of fission and reaction products from the target material to provide higher sensitivity measurements. Cumulative fission mass-yields for 32 different isobars, 72 a parts per thousand currency sign A a parts per thousand currency sign 153, were measured from experiments fielded on two separate NIF shots. C1 [Gharibyan, Narek; Moody, Kenton J.; Despotopulos, John D.; Grant, Patrick M.; Shaughnessy, Dawn A.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Despotopulos, John D.] Univ Nevada, Las Vegas, NV 89154 USA. RP Gharibyan, N (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave,L-236, Livermore, CA 94551 USA. EM gharibyan1@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The authors would like to thank the NIF engineers Kenn Knittel and Bahram Talison, who were instrumental in the design process and in fielding the TOAD assembly. We also thank the staff of the Nuclear Counting Facility at Lawrence Livermore National Laboratory, including B. Bandong, P. Torretto and T. Wooddy. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 8 TC 3 Z9 3 U1 3 U2 19 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD FEB PY 2015 VL 303 IS 2 BP 1335 EP 1338 DI 10.1007/s10967-014-3474-6 PG 4 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA AZ4LJ UT WOS:000348192200051 ER PT J AU Kuang, WH Liu, Y Dou, YY Chi, WF Chen, GS Gao, CF Yang, TR Liu, JY Zhang, RH AF Kuang, Wenhui Liu, Yue Dou, Yinyin Chi, Wenfeng Chen, Guangsheng Gao, Chengfeng Yang, Tianrong Liu, Jiyuan Zhang, Renhua TI What are hot and what are not in an urban landscape: quantifying and explaining the land surface temperature pattern in Beijing, China SO LANDSCAPE ECOLOGY LA English DT Article DE Urban heat island; Land surface temperature; Urban landscape; Land-use/land-cover; MODIS; Portable infrared thermometer ID TANGSHAN METROPOLITAN-AREA; HEAT-ISLAND; ECOLOGICAL-SYSTEMS; DRIVING FORCES; VARIABILITY; IMPACTS; GROWTH; CONFIGURATION; ENVIRONMENT; EMISSIVITY AB Understanding how landscape components affect the urban heat islands is crucial for urban ecological planning and sustainable development. The purpose of this study was to quantify the spatial pattern of land surface temperatures (LSTs) and associated heat fluxes in relation to land-cover types in Beijing, China, using portable infrared thermometers, thermal infrared imagers, and the moderate resolution imaging spectroradiometer. The spatial differences and the relationships between LSTs and the hierarchical landscape structure were analyzed with in situ observations of surface radiation and heat fluxes. Large LST differences were found among various land-use/land-cover types, urban structures, and building materials. Within the urban area, the mean LST of urban impervious surfaces was about 6-12 A degrees C higher than that of the urban green space. LSTs of built-up areas were on average 3-6 A degrees C higher than LSTs of rural areas. The observations for surface radiation and heat fluxes indicated that the differences were caused by different fractions of sensible heat or latent heat flux in net radiation. LSTs decreased with increasing elevation and normalized difference vegetation index. Variations in building materials and urban structure significantly influenced the spatial pattern of LSTs in urban areas. By contrast, elevation and vegetation cover are the major determinants of the LST pattern in rural areas. To alleviate urban heat island intensity, urban planners and policy makers should pay special attention to the selection of appropriate building materials, the reasonable arrangement of urban structures, and the rational design of landscape components. C1 [Kuang, Wenhui; Liu, Yue; Chi, Wenfeng; Yang, Tianrong; Liu, Jiyuan; Zhang, Renhua] Chinese Acad Sci, Inst Geog Sci & Nat Resources Res, Key Lab Land Surface Pattern & Simulat, Beijing 100101, Peoples R China. [Dou, Yinyin] Beijing Normal Univ, State Key Lab Earth Surface Proc & Resource Ecol, Beijing 100875, Peoples R China. [Chi, Wenfeng] Univ Chinese Acad Sci, Coll Resources & Environm, Beijing 100049, Peoples R China. [Chen, Guangsheng] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Gao, Chengfeng] Southwest Univ Sci & Technol, Mianyang 621010, Peoples R China. RP Kuang, WH (reprint author), Chinese Acad Sci, Inst Geog Sci & Nat Resources Res, Key Lab Land Surface Pattern & Simulat, Beijing 100101, Peoples R China. EM kuangwh@igsnrr.ac.cn FU National Natural Science Foundation of China [41371408]; National Basic Research Program of China [2014CB954302, 2010CB950900]; National Key Technology RD Program [2012BAJ15B02] FX We thank the National Natural Science Foundation of China (41371408), the National Basic Research Program of China (2014CB954302; 2010CB950900), and National Key Technology R&D Program (2012BAJ15B02) for financial support. We also thank Dr. Shaomin Liu of Beijing Normal University for providing the radiation and energy fluxes data from the Daxing Station, and Dr. Jianguo Wu for constructive comments/suggestions for this paper. NR 63 TC 7 Z9 9 U1 10 U2 66 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0921-2973 EI 1572-9761 J9 LANDSCAPE ECOL JI Landsc. Ecol. PD FEB PY 2015 VL 30 IS 2 BP 357 EP 373 DI 10.1007/s10980-014-0128-6 PG 17 WC Ecology; Geography, Physical; Geosciences, Multidisciplinary SC Environmental Sciences & Ecology; Physical Geography; Geology GA AZ3ML UT WOS:000348131500013 ER PT J AU Webb, JD Seki, T Goldston, JF Pruski, M Crudden, CM AF Webb, Jonathan D. Seki, Tomohiro Goldston, Jennifer F. Pruski, Marek Crudden, Cathleen M. TI Selective functionalization of the mesopores of SBA-15 SO MICROPOROUS AND MESOPOROUS MATERIALS LA English DT Article DE Mesoporous silica; SBA-15; Silylation; Surface functionalization; Selective grafting; Solid state NMR ID SOLID-STATE NMR; DRUG-DELIVERY; SILICA NANOPARTICLES; ORGANOMETALLIC CATALYSTS; ELECTROLESS DEPOSITION; INTERFACIAL REACTIONS; CARRIER SYSTEM; MCM-41; ENANTIOSELECTIVITY; MOLECULES AB A method has been developed that permits the highly selective functionalization of the interior and exterior surfaces of the ubiquitous mesoporous material, SBA-15. The key step is reloading the as-synthesized material with structure-directing agent, Pluronic (R) P123, prior to selective functionalization of the external surface with a silylating agent. This new approach represents a significant improvement over literature procedures. Results from physisorption analyses as well as solid-state NMR permit a detailed, quantitative assessment of functionalized SBA-15. This work also provides insight into the stability of the silyl layer during extraction procedures - an issue often neglected in other studies but of significant importance as decomposition of this layer could result in the introduction of new silanols and reduce the effectiveness of any selective grafting procedure. (C) 2014 Elsevier Inc. All rights reserved. C1 [Webb, Jonathan D.; Seki, Tomohiro; Crudden, Cathleen M.] Queens Univ, Dept Chem, Kingston, ON K7L 3N6, Canada. [Goldston, Jennifer F.; Pruski, Marek] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. [Goldston, Jennifer F.; Pruski, Marek] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Crudden, Cathleen M.] Nagoya Univ, Inst Transformat Biomol WPI ITbM, Nagoya, Aichi 4648601, Japan. RP Crudden, CM (reprint author), Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. EM mpruski@iastate.edu; cathleen.crudden@chem.queensu.ca FU Natural Sciences and Engineering Research Council of Canada (NSERC); Canada Foundation for Innovation (CFI); NSERC; U. E. Carmichael and Queen's University; Queen's University; U.S. Department of Energy, Office of Basic Energy Sciences (BES), Division of Chemical Sciences, Geosciences, and Biosciences through the Ames Laboratory; Iowa State University [DE-AC02-07CH11358] FX CMC thanks the Natural Sciences and Engineering Research Council of Canada (NSERC) for funding in terms of Discovery, Discovery Accelerator and RTI grants. CMC also acknowledges the Canada Foundation for Innovation (CFI) for infrastructure funding. JDW acknowledges NSERC for a Canada PGSD fellowship. TS acknowledges U. E. Carmichael and Queen's University for a Duncan and Urlla Carmichael Fellowship. JDW and TS acknowledge Queen's University for Queen's Graduate Awards. This research was also supported by the U.S. Department of Energy, Office of Basic Energy Sciences (BES), Division of Chemical Sciences, Geosciences, and Biosciences through the Ames Laboratory (JFG and MP). The Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. NR 56 TC 3 Z9 3 U1 2 U2 48 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1387-1811 EI 1873-3093 J9 MICROPOR MESOPOR MAT JI Microporous Mesoporous Mat. PD FEB PY 2015 VL 203 BP 123 EP 131 DI 10.1016/j.micromeso.2014.10.032 PG 9 WC Chemistry, Applied; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AY5DI UT WOS:000347593000015 ER PT J AU Fowler, JS Logan, J Volkow, ND Shumay, E McCall-Perez, F Jayne, M Wang, GJ Alexoff, DL Apelskog-Torees, K Hubbard, B Carter, P King, P Fahn, S Gilmor, M Telang, F Shea, C Xu, YW Muench, L AF Fowler, Joanna S. Logan, Jean Volkow, Nora D. Shumay, Elena McCall-Perez, Fred Jayne, Millard Wang, Gene-Jack Alexoff, David L. Apelskog-Torees, Karen Hubbard, Barbara Carter, Pauline King, Payton Fahn, Stanley Gilmor, Michelle Telang, Frank Shea, Colleen Xu, Youwen Muench, Lisa TI Evidence that Formulations of the Selective MAO-B Inhibitor, Selegiline, which Bypass First-Pass Metabolism, also Inhibit MAO-A in the Human Brain SO NEUROPSYCHOPHARMACOLOGY LA English DT Article ID TYRAMINE PRESSOR SENSITIVITY; MONOAMINE-OXIDASE INHIBITORS; MAJOR DEPRESSIVE DISORDER; HIGH-DOSE SELEGILINE; TRANSDERMAL SYSTEM; L-DEPRENYL; DOPAMINE TRANSPORTER; DOUBLE-BLIND; HEALTHY-SUBJECTS; EFFICACY AB Selegiline (L-deprenyl) is a selective, irreversible inhibitor of monoamine oxidase B (MAO-B) at the conventional dose (10 mg/day oral) that is used in the treatment of Parkinson's disease. However, controlled studies have demonstrated antidepressant activity for high doses of oral selegiline and for transdermal selegiline suggesting that when plasma levels of selegiline are elevated, brain MAO-A might also be inhibited. Zydis selegiline (Zelapar) is an orally disintegrating formulation of selegiline, which is absorbed through the buccal mucosa producing higher plasma levels of selegiline and reduced amphetamine metabolites compared with equal doses of conventional selegiline. Although there is indirect evidence that Zydis selegiline at high doses loses its selectivity for MAO-B, there is no direct evidence that it also inhibits brain MAO-A in humans. We measured brain MAO-A in 18 healthy men after a 28-day treatment with Zydis selegiline (2.5, 5.0, or I 0 mg/day) and in 3 subjects receiving the selegiline transdermal system (Emsam patch, 6 mg/day) using positron emission tomography and the MAO-A radiotracer [C-11]clorgyline. We also measured dopamine transporter (DAT) availability in three subjects from the 10 mg group. The I 0 mg Zydis selegiline dose significantly inhibited MAO-A (36.9 +/- 19.7%, range 11-70%, p<0.007)) but not DAT; and while Emsam also inhibited MAO-A (33.2 +/- 28.9 (range 9-68%) the difference did not reach significance (p=0.10)) presumably because of the small sample size. Our results provide the first direct evidence of brain MAO-A inhibition in humans by formulations of selegiline, which are currently postulated but not verified to target brain MAO-A in addition to MAO-B. C1 [Fowler, Joanna S.; Alexoff, David L.; Hubbard, Barbara; Carter, Pauline; King, Payton; Shea, Colleen; Xu, Youwen] Brookhaven Natl Lab, Biol Environm & Climate Sci Dept, Upton, NY 11973 USA. [Logan, Jean] NYU, Dept Radiol, Langone Med Ctr, New York, NY 10016 USA. [Volkow, Nora D.] NIDA, NIH, Bethesda, MD 20892 USA. [Volkow, Nora D.; Shumay, Elena; Jayne, Millard; Wang, Gene-Jack; Apelskog-Torees, Karen; Telang, Frank; Muench, Lisa] NIAAA, NIH, Bethesda, MD USA. [McCall-Perez, Fred] Targeted Med Pharma Inc, Los Angeles, CA USA. [Fahn, Stanley] Columbia Univ, Dept Neurol, Med Ctr, New York, NY USA. [Gilmor, Michelle] Novartis Pharmaceut, E Hanover, NJ USA. RP Fowler, JS (reprint author), Brookhaven Natl Lab, Dept Biosci, Bldg 555, Upton, NY 11973 USA. EM fowler@bnl.gov OI Logan, Jean/0000-0002-6993-9994 FU Valeant Pharmaceuticals International FX This study was funded by Valeant Pharmaceuticals International. The authors disclose no other conflict of interest that might potentially bias this work. NR 45 TC 10 Z9 11 U1 5 U2 24 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0893-133X EI 1740-634X J9 NEUROPSYCHOPHARMACOL JI Neuropsychopharmacology PD FEB PY 2015 VL 40 IS 3 BP 650 EP 657 DI 10.1038/npp.2014.214 PG 8 WC Neurosciences; Pharmacology & Pharmacy; Psychiatry SC Neurosciences & Neurology; Pharmacology & Pharmacy; Psychiatry GA AY6ET UT WOS:000347660900013 PM 25249059 ER PT J AU Razzaghi, H Marcinkevage, J Peterson, C AF Razzaghi, Hilda Marcinkevage, Jessica Peterson, Cora TI Prevalence of undiagnosed diabetes among non-pregnant women of reproductive age in the United States, 1999-2010 SO PRIMARY CARE DIABETES LA English DT Article DE Diabetes mellitus/diagnosis; Diabetes mellitus/epidemiology; Pregnancy complications ID PREGNANCY; OUTCOMES; FETAL AB Undiagnosed diabetes has particularly harmful consequences among women of reproductive age. We assessed the prevalence of undiagnosed diabetes among non-pregnant women of reproductive age. In our data 30 women had A1C >= 6.5 and 28 had FPG >= 126 mg/dl values suggesting approximately 300,000 women of reproductive age nationwide may have undiagnosed diabetes. (c) 2013 Primary Care Diabetes Europe. Published by Elsevier Ltd. All rights reserved. C1 [Razzaghi, Hilda; Marcinkevage, Jessica; Peterson, Cora] Ctr Dis Control & Prevent, Natl Ctr Birth Defects & Dev Disabil, Atlanta, GA 30333 USA. [Razzaghi, Hilda] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. [Marcinkevage, Jessica] Emory Univ, Laney Grad Sch, Nutr & Hlth Sci Program, Atlanta, GA 30322 USA. RP Razzaghi, H (reprint author), Ctr Dis Control & Prevent, Natl Ctr Birth Defects & Dev Disabil, 1600 Clifton Rd NE,MS E-86, Atlanta, GA 30333 USA. EM hir2@cdc.gov OI Peterson, Cora/0000-0001-7955-0977 FU Intramural CDC HHS [CC999999]; NIDDK NIH HHS [T32 DK007734] NR 12 TC 1 Z9 1 U1 0 U2 2 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1751-9918 EI 1878-0210 J9 PRIM CARE DIABETES JI Prim. Care Diabetes PD FEB PY 2015 VL 9 IS 1 BP 71 EP 73 DI 10.1016/j.pcd.2013.10.004 PG 3 WC Endocrinology & Metabolism; Primary Health Care SC Endocrinology & Metabolism; General & Internal Medicine GA AZ5MR UT WOS:000348265500011 PM 24216319 ER PT J AU Heatwole, E Parker, G Holmes, M Dickson, P AF Heatwole, Eric Parker, Gary Holmes, Matt Dickson, Peter TI Grit-mediated frictional ignition of a polymer-bonded explosive during oblique impacts: Probability calculations for safety engineering SO RELIABILITY ENGINEERING & SYSTEM SAFETY LA English DT Article DE Friction; Hot spots; PBX 9501; Explosives; Skid test; Oblique impact ID INITIATION AB Frictional heating of high-melting-point grit particles during oblique impacts of consolidated explosives is considered to be the major source of ignition in accidents involving dropped explosives. It has been shown in other work that the lower temperature melting point of two frictionally interacting surfaces will cap the maximum temperature reached, which provides a simple way to mitigate the danger in facilities by implementing surfaces with melting points below the ignition temperature of the explosive. However, a recent series of skid testing experiments has shown that ignition can occur on low-melting-point surfaces with a high concentration of grit particles, most likely due to a grit-grit collision mechanism. For risk-based safety engineering purposes, the authors present a method to estimate the probability of grit contact and/or grit-grit collision during an oblique impact. These expressions are applied to potentially high-consequence oblique impact scenarios in order to give the probability of striking one or more grit particles (for high-melting-point surfaces), or the probability of one or more grit-grit collisions occurring (for low-melting-point surfaces). The probability is dependent on a variety of factors, many of which can be controlled for mitigation to achieve acceptable risk levels for safe explosives handling operations. (C) 2014 Published by Elsevier Ltd. C1 [Heatwole, Eric; Parker, Gary; Holmes, Matt; Dickson, Peter] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Heatwole, E (reprint author), Los Alamos Natl Lab, WX-6, Los Alamos, NM 87545 USA. EM heatwole@lanl.gov; gparker@lanl.gov; mholmes@lanl.gov; dickson@lanl.gov NR 12 TC 0 Z9 0 U1 1 U2 12 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0951-8320 EI 1879-0836 J9 RELIAB ENG SYST SAFE JI Reliab. Eng. Syst. Saf. PD FEB PY 2015 VL 134 BP 10 EP 18 DI 10.1016/j.ress.2014.09.023 PG 9 WC Engineering, Industrial; Operations Research & Management Science SC Engineering; Operations Research & Management Science GA AY6FR UT WOS:000347663200002 ER PT J AU Varley, JB Schleife, A AF Varley, Joel B. Schleife, Andre TI Bethe-Salpeter calculation of optical-absorption spectra of In2O3 and Ga2O3 SO SEMICONDUCTOR SCIENCE AND TECHNOLOGY LA English DT Article DE optical properties; excitonic effects; first-principles calculations ID TRANSPARENT CONDUCTING OXIDES; SINGLE-CRYSTALS; 1ST PRINCIPLES; BETA-GA2O3; SEMICONDUCTORS; EDGE; SNO2 AB Transparent conducting oxides keep attracting strong scientific interest not only due to their promising potential for 'transparent electronics' applications but also due to their intriguing optical absorption characteristics. Materials such as In2O3 and Ga2O3 have complicated unit cells and, consequently, are interesting systems for studying the physics of excitons and anisotropy of optical absorption. Since currently no experimental data is available, for instance, for their dielectric functions across a large photon-energy range, we employ modern first-principles computational approaches based on many-body perturbation theory to provide theoreticalspectroscopy results. Using the Bethe-Salpeter framework, we compute dielectric functions and we compare to spectra computed without excitonic effects. We find that the electron-hole interaction strongly modifies the spectra and we discuss the anisotropy of optical absorption that we find for Ga2O3 in relation to existing theoretical and experimental data. C1 [Varley, Joel B.] Lawrence Livermore Natl Lab, Condensed Matter & Mat Div, Livermore, CA 94550 USA. [Schleife, Andre] Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USA. RP Varley, JB (reprint author), Lawrence Livermore Natl Lab, Condensed Matter & Mat Div, Livermore, CA 94550 USA. EM varley2@llnl.gov; schleife@illinois.edu FU National Science Foundation [OCI-0725070, ACI-1238993]; state of Illinois; US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We acknowledge fruitful discussions with O Bierwagen, C Cobet, K Irmscher, Z Galazka, M Mohamed, and C G Van de Walle. This research is part of the Blue Waters sustained-petascale computing project, which is supported by the National Science Foundation (awards OCI-0725070 and ACI-1238993) and the state of Illinois. Blue Waters is a joint effort of the University of Illinois at Urbana-Champaign and its National Center for Supercomputing Applications. Part of this work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 51 TC 8 Z9 8 U1 3 U2 45 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0268-1242 EI 1361-6641 J9 SEMICOND SCI TECH JI Semicond. Sci. Technol. PD FEB PY 2015 VL 30 IS 2 SI SI AR 024010 DI 10.1088/0268-1242/30/2/024010 PG 5 WC Engineering, Electrical & Electronic; Materials Science, Multidisciplinary; Physics, Condensed Matter SC Engineering; Materials Science; Physics GA AZ3IQ UT WOS:000348121200011 ER PT J AU Dong, YJ Brooks, JD Chen, TL Mullins, DR Cox, DF AF Dong, Yujung Brooks, John D. Chen, Tsung-Liang Mullins, David R. Cox, David F. TI Methylene migration and coupling on a non-reducible metal oxide: The reaction of dichloromethane on stoichiometric alpha-Cr2O3(0001) SO SURFACE SCIENCE LA English DT Article DE Temperature programmed desorption; XPS; Density functional calculations ID SUPPORTED CHROMIUM-OXIDE; TOTAL-ENERGY CALCULATIONS; CARBON BOND FORMATION; AUGMENTED-WAVE METHOD; SURFACE-CHEMISTRY; DISSOCIATIVE ADSORPTION; THIN-FILMS; BASIS-SET; OXYGEN; DEHYDROGENATION AB The reaction of CH2Cl2 over the nearly-stoichiometric alpha-Cr2O3(0001) surface produces gas phase ethylene, methane and surface chlorine adatoms. The reaction is initiated by the decomposition of CH2Cl2 into surface methylene and chlorine. Photoemission indicates that surface cations are the preferred binding sites for both methylene and chlorine adatoms. Two reaction channels are observed for methylene coupling to ethylene in temperature-programmed desorption (TPD). A desorption-limited, low-temperature route is attributed to two methylenes bound at a single site. The majority of ethylene is produced by a reaction-limited process involving surface migration (diffusion) of methylene as the rate-limiting step. DFT calculations indicate the surface diffusion mechanism is mediated by surface oxygen anions. The source of hydrogen for methane formation is adsorbed background water. Chlorine adatoms produced by the dissociation of CH2Cl2 deactivate the surface by simple site-blocking of surface Cr3+ sites. A comparison of experiment and theory shows that DEL provides a better description of the surface chemistry of the carbene intermediate than DFT+U using reported parameters for a best representation of the bulk electronic properties of alpha-Cr2O3. (C) 2014 Elsevier B.V. All rights reserved. C1 [Dong, Yujung; Brooks, John D.; Cox, David F.] Virginia Polytech Inst & State Univ, Dept Chem Engn, Blacksburg, VA 24061 USA. [Chen, Tsung-Liang; Mullins, David R.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Cox, DF (reprint author), Virginia Polytech Inst & State Univ, Dept Chem Engn, Blacksburg, VA 24061 USA. EM dfcox@vt.edu FU Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy [DE-FG02-97ER14751]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX YD, JDB and DFC gratefully acknowledge financial support by the Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy through Grant DE-FG02-97ER14751. The efforts of TLC and DRM are sponsored by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. The authors also acknowledge Advanced Research Computing at Virginia Tech for providing computational resources and technical support that have contributed to the results reported within this paper. NR 67 TC 3 Z9 3 U1 1 U2 33 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0039-6028 EI 1879-2758 J9 SURF SCI JI Surf. Sci. PD FEB PY 2015 VL 632 BP 28 EP 38 DI 10.1016/j.susc.2014.09.008 PG 11 WC Chemistry, Physical; Physics, Condensed Matter SC Chemistry; Physics GA AY5IJ UT WOS:000347605600005 ER PT J AU Colakerol, L Piper, LFJ Fedorov, A Chen, T Moustakas, TD Smith, KE AF Colakerol, L. Piper, L. F. J. Fedorov, A. Chen, T. Moustakas, T. D. Smith, K. E. TI Potassium and ion beam induced electron accumulation in InN SO SURFACE SCIENCE LA English DT Article DE Angle resolved photoemission; Alkali-metal; Charge accumulation; Molecular beam epitaxy; InN surface ID ROOM-TEMPERATURE; INTERFACE FORMATION; SCHOTTKY-BARRIER; SURFACE; INAS(110); BAND; PHOTOLUMINESCENCE; NANOWIRES; LAYER; MBE AB "We present angle resolved photoemission study of quantized electron accumulation subbands obtained from both clean and potassium deposited InN(000 (1) over bar) surfaces. Shifting of the quantized accumulation states toward higher binding energies upon low energy N-2(+) ion bombardment or a small amount of potassium adsorption is explained by the modification of the In-adlayer induced surface states. N-2(+) ion bombardment leads to a higher density of donor-type surface states by creating nitrogen vacancies near the surface. On the other hand, a small amount of K adsorbates initially donate their free electron to InN and result in more pronounced downward band bending. Eventually, further K adsorption leads to passivation of surface states and reduction of the surface electron accumulation. With the increase of the electron density, enhanced many-body interactions of electrons within the electron accumulation layer are observed." (C) 2014 Elsevier B.V. All rights reserved. C1 [Colakerol, L.; Piper, L. F. J.; Smith, K. E.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Colakerol, L.] Gebze Inst Technol, Dept Phys, TR-41400 Kocaeli, Turkey. [Piper, L. F. J.] Binghamton Univ, Dept Phys Appl Phys & Astron, Binghamton, NY 13902 USA. [Fedorov, A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Chen, T.; Moustakas, T. D.] Boston Univ, Dept Elect & Comp Engn, Boston, MA 02215 USA. [Smith, K. E.] Univ Auckland, Sch Chem Sci, Auckland 1142, New Zealand. [Smith, K. E.] Univ Auckland, MacDiarmid Inst Adv Mat & Nanotechnol, Auckland 1142, New Zealand. RP Smith, KE (reprint author), Boston Univ, Dept Phys, Boston, MA 02215 USA. EM ksmith@bu.edu RI Moustakas, Theodore/D-9249-2016; Piper, Louis/C-2960-2011 OI Moustakas, Theodore/0000-0001-8556-884X; Piper, Louis/0000-0002-3421-3210 FU DOE [RF-06-PRD-001]; NSF [DMR-0311792] FX This work was supported in part by the DOE under RF-06-PRD-001 and by the NSF under grant no. DMR-0311792. NR 36 TC 1 Z9 1 U1 2 U2 23 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0039-6028 EI 1879-2758 J9 SURF SCI JI Surf. Sci. PD FEB PY 2015 VL 632 BP 154 EP 157 DI 10.1016/j.susc.2014.10.004 PG 4 WC Chemistry, Physical; Physics, Condensed Matter SC Chemistry; Physics GA AY5IJ UT WOS:000347605600022 ER PT J AU Ilton, ES Droubay, TC Chaka, AM Kovarik, L Varga, T Arey, BW Kerisit, SN AF Ilton, Eugene S. Droubay, Timothy C. Chaka, Anne M. Kovarik, Libor Varga, Tamas Arey, Bruce W. Kerisit, Sebastien N. TI Epitaxial single-crystal thin films of MnxTi1 (-) O-x(2) (- delta) grown on (rutile)TiO2 substrates with pulsed laser deposition: Experiment and theory SO SURFACE SCIENCE LA English DT Article DE Thin films; Pulsed laser deposition; Ab initio thermodynamics; Rutile; Manganese ID MOLECULAR-BEAM EPITAXY; DOPED TIO2; TITANIUM-DIOXIDE; PHOTOCATALYTIC ACTIVITY; ELECTRONIC-STRUCTURES; VACANCY FORMATION; RUTILE TIO2; MANGANESE; NITROGEN; OXIDES AB Epitaxial rutile-structured single-crystal MnxTi1 - xO2 (- delta) films were synthesized on rutile- (110) and -(001) substrates using pulsed laser deposition. The films were characterized by reflection high-energy electron diffraction (RHEED), X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS), and aberration-corrected transmission electron microscopy (ACTEM). Under the present conditions, 400 degrees C and PO2 = 20 mTorr, single crystal epitaxial thin films were grown for x = 0.13, where x is the nominal average mole fraction of Mn. In fact, arbitrarily thick films could be grown with near invariant Mn/Ti concentration profiles from the substrate/film interface to the film surface. In contrast, at x = 0.25, Mn became enriched towards the surface and a secondary nano-scale phase formed which appeared to maintain the basic rutile structure but with enhanced z-contrast in the tunnels, or interstitial sites. Ab initio thermodynamic calculations provided quantitative estimates for the destabilizing effect of expanding the beta-MnO2 lattice parameters to those of TiO2-rutile, the stabilizing effect of diluting Mn with increasing Ti concentration, and competing reaction pathways for surface oxide formation. (C) 2014 Elsevier B.V. All rights reserved. C1 [Ilton, Eugene S.; Droubay, Timothy C.; Chaka, Anne M.; Kovarik, Libor; Varga, Tamas; Arey, Bruce W.; Kerisit, Sebastien N.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Ilton, ES (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99352 USA. EM Eugene.Ilton@PNNL.gov RI Droubay, Tim/D-5395-2016; Kovarik, Libor/L-7139-2016 OI Droubay, Tim/0000-0002-8821-0322; FU PNNL Laboratory Directed Research and Development Program; U.S. Department of Energy's Office of Biological and Environmental Research FX This work was funded by the PNNL Laboratory Directed Research and Development Program. The research was performed using EMSL, a national scientific user facility sponsored by the U.S. Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). PNNL is a multiprogram national laboratory operated for DOE by Battelle. NR 50 TC 2 Z9 2 U1 3 U2 34 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0039-6028 EI 1879-2758 J9 SURF SCI JI Surf. Sci. PD FEB PY 2015 VL 632 BP 185 EP 194 DI 10.1016/j.susc.2014.10.013 PG 10 WC Chemistry, Physical; Physics, Condensed Matter SC Chemistry; Physics GA AY5IJ UT WOS:000347605600027 ER PT J AU Droubay, TC Kong, L Chambers, SA Hess, WP AF Droubay, T. C. Kong, L. Chambers, S. A. Hess, W. P. TI Work function reduction by BaO: Growth of crystalline barium oxide on Ag(001) and Ag(111) surfaces SO SURFACE SCIENCE LA English DT Article DE Work function; Epitaxy; X-ray photoemission spectroscopy ID THETA-AL2O3/NIAL(100) ULTRATHIN FILMS; AB-INITIO CALCULATIONS; THIN-FILMS; OXIDATION; CATHODE; OXYGEN; DEPOSITION; MECHANISM; PT(111); SILVER AB Ultrathin films of barium oxide were grown on Ag(001) and Ag(111) using the evaporation of Ba metal in an O-2 atmosphere by molecular beam epitaxy. Ultraviolet photoemission spectroscopy reveals that films consisting of predominantly BaO or BaO2 result in Ag(001) work function reductions of 1.74 eV and 0.64 eV, respectively. On the Ag(001) surface, Ba oxide growth is initiated by two-dimensional nucleation of epitaxial BaO, followed by a transition to three-dimensional dual-phase nucleation of epitaxial BaO and BaO2. Three-dimensional islands of primarily BaO2(111) nucleate epitaxially on the Ag(111) substrate leaving large patches of Ag uncovered. We find no indication of chemical reaction or charge transfer between the films and the Ag substrates. These data suggest that the origin of the observed work function reduction is largely due to a combination of BaO surface relaxation and an electrostatic compressive effect. (C) 2014 Elsevier B.V. All rights reserved. C1 [Droubay, T. C.; Kong, L.; Chambers, S. A.; Hess, W. P.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP Droubay, TC (reprint author), Pacific NW Natl Lab, Div Phys Sci, POB 999 MS K8-87, Richland, WA 99352 USA. EM Tim.Droubay@pnnl.gov RI Droubay, Tim/D-5395-2016 OI Droubay, Tim/0000-0002-8821-0322 FU U.S. Department of Energy [DE-AC05-76RL01830]; Department of Energy's Office of Biological and Environmental Research FX The research described here is part of the Chemical Imaging Initiative at Pacific Northwest National Laboratory (PNNL). It was conducted under the Laboratory Directed Research and Development Program at PNNL, a multi-program national laboratory operated by Battelle for the U.S. Department of Energy under Contract DE-AC05-76RL01830. The work was performed at EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at PNNL. NR 32 TC 1 Z9 1 U1 5 U2 23 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0039-6028 EI 1879-2758 J9 SURF SCI JI Surf. Sci. PD FEB PY 2015 VL 632 BP 201 EP 206 DI 10.1016/j.susc.2014.07.010 PG 6 WC Chemistry, Physical; Physics, Condensed Matter SC Chemistry; Physics GA AY5IJ UT WOS:000347605600029 ER PT J AU Simeone, RM Devine, OJ Marcinkevage, JA Gilboa, SM Razzaghi, H Bardenheier, BH Sharma, AJ Honein, MA AF Simeone, Regina M. Devine, Owen J. Marcinkevage, Jessica A. Gilboa, Suzanne M. Razzaghi, Hilda Bardenheier, Barbara H. Sharma, Andrea J. Honein, Margaret A. TI Diabetes and Congenital Heart Defects A Systematic Review, Meta-Analysis, and Modeling Project SO AMERICAN JOURNAL OF PREVENTIVE MEDICINE LA English DT Article ID INDEPENDENT RISK-FACTOR; BIRTH-DEFECTS; PRECONCEPTION CARE; UNITED-STATES; CARDIOVASCULAR MALFORMATIONS; METROPOLITAN ATLANTA; US POPULATION; OBESE WOMEN; PREVALENCE; MELLITUS AB Context: Maternal pregestational diabetes (PGDM) is a risk factor for development of congenital heart defects (CHDs). Glycemic control before pregnancy reduces the risk of CHDs. A meta-analysis was used to estimate summary ORs and mathematical modeling was used to estimate population attributable fractions (PAFs) and the annual number of CHDs in the U.S. potentially preventable by establishing glycemic control before pregnancy. Evidence acquisition: A systematic search of the literature through December 2012 was conducted in 2012 and 2013. Case-control or cohort studies were included. Data were abstracted from 12 studies for a meta-analysis of all CHDs. Evidence synthesis: Summary estimates of the association between PGDM and CHDs and 95% credible intervals (95% CrIs) were developed using Bayesian random-effects meta-analyses for all CHDs and specific CHD subtypes. Posterior estimates of this association were combined with estimates of CHD prevalence to produce estimates of PAFs and annual prevented cases. Ninety-five percent uncertainty intervals (95% UIs) for estimates of the annual number of preventable cases were developed using Monte Carlo simulation. Analyses were conducted in 2013. The summary OR estimate for the association between PGDM and CHDs was 3.8 (95% CrI=3.0, 4.9). Approximately 2670 (95% UI=1795, 3795) cases of CHDs could potentially be prevented annually if all women in the U.S. with PGDM achieved glycemic control before pregnancy. Conclusions: Estimates from this analysis suggest that preconception care of women with PGDM could have a measureable impact by reducing the number of infants born with CHDs. Published by Elsevier Inc. on behalf of American Journal of Preventive Medicine C1 [Simeone, Regina M.; Devine, Owen J.; Marcinkevage, Jessica A.; Gilboa, Suzanne M.; Razzaghi, Hilda; Honein, Margaret A.] CDC, Natl Ctr Birth Defects & Dev Disabil, Atlanta, GA 30333 USA. [Bardenheier, Barbara H.; Sharma, Andrea J.] CDC, Natl Ctr Chron Dis Prevent & Hlth Promot, Atlanta, GA 30333 USA. [Sharma, Andrea J.] US Publ Hlth Serv Commissioned Corps, Atlanta, GA USA. [Simeone, Regina M.; Marcinkevage, Jessica A.; Razzaghi, Hilda] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. RP Simeone, RM (reprint author), CDC, Natl Ctr Birth Defects & Dev Disabil, 1600 Clifton Rd NE,Mail Stop E-86, Atlanta, GA 30333 USA. EM rsimeone@cdc.gov OI Sharma, Andrea/0000-0003-0385-0011 FU U.S. Department of Energy; CDC FX The authors gratefully acknowledge librarians, Christy Cechman, MLIS, of the American Public University System, and Gail Bang, MLIS, of the CDC Public Health Library and Information Center, who conducted the literature searches; Jaynia Anderson, MPH, a graduate student from Emory University's Rollins School of Public Health, who assisted with the collection and maintenance of the manuscripts; and Amy Cordero, MPA, who developed the original search strategy for this project. This research (J.A.M., H.R., R.M.S.) was supported in part by an appointment to the Research Participation Program at CDC administered by the Oak Ridge Institute for Science and Education through an interagency agreement between the U.S. Department of Energy and CDC. NR 65 TC 9 Z9 9 U1 0 U2 7 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0749-3797 EI 1873-2607 J9 AM J PREV MED JI Am. J. Prev. Med. PD FEB PY 2015 VL 48 IS 2 BP 195 EP 204 DI 10.1016/j.amepre.2014.09.002 PG 10 WC Public, Environmental & Occupational Health; Medicine, General & Internal SC Public, Environmental & Occupational Health; General & Internal Medicine GA AZ2YY UT WOS:000348096300012 PM 25326416 ER PT J AU Wang, DP Dorosky, RJ Han, CS Lo, CC Dichosa, AEK Chain, PS Yu, JM Pierson, LS Pierson, EA AF Wang, Dongping Dorosky, Robert J. Han, Cliff S. Lo, Chien-chi Dichosa, Armand E. K. Chain, Patrick S. Yu, Jun Myoung Pierson, Leland S., III Pierson, Elizabeth A. TI Adaptation Genomics of a Small-Colony Variant in a Pseudomonas chlororaphis 30-84 Biofilm SO APPLIED AND ENVIRONMENTAL MICROBIOLOGY LA English DT Article ID HIGHLY ADHERENT; PHENAZINE BIOSYNTHESIS; EXPRESSION ANALYSIS; BACTERIAL UPTAKE; AERUGINOSA PA14; GENE-EXPRESSION; CYSTIC-FIBROSIS; RESISTANCE; ACID; OXYR AB The rhizosphere-colonizing bacterium Pseudomonas chlororaphis 30-84 is an effective biological control agent against take-all disease of wheat. In this study, we characterize a small-colony variant (SCV) isolated from a P. chlororaphis 30-84 biofilm. The SCV exhibited pleiotropic phenotypes, including small cell size, slow growth and motility, low levels of phenazine production, and increased biofilm formation and resistance to antimicrobials. To better understand the genetic alterations underlying these phenotypes, RNA and whole-genome sequencing analyses were conducted comparing an SCV to the wild-type strain. Of the genome's 5,971 genes, transcriptomic profiling indicated that 1,098 (18.4%) have undergone substantial reprograming of gene expression in the SCV. Whole-genome sequence analysis revealed multiple alterations in the SCV, including mutations in yfiR (cyclic- di-GMP production), fusA (elongation factor), and cyoE (heme synthesis) and a 70-kb deletion. Genetic analysis revealed that the yfiR locus plays a major role in controlling SCV phenotypes, including colony size, growth, motility, and biofilm formation. Moreover, a point mutation in the fusA gene contributed to kanamycin resistance. Interestingly, the SCV can partially switch back to wild-type morphologies under specific conditions. Our data also support the idea that phenotypic switching in P. chlororaphis is not due to simple genetic reversions but may involve multiple secondary mutations. The emergence of these highly adherent and antibiotic-resistant SCVs within the biofilm might play key roles in P. chlororaphis natural persistence. C1 [Wang, Dongping; Han, Cliff S.; Lo, Chien-chi; Dichosa, Armand E. K.; Chain, Patrick S.] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87544 USA. [Dorosky, Robert J.; Yu, Jun Myoung; Pierson, Leland S., III; Pierson, Elizabeth A.] Texas A&M Univ, Dept Plant Pathol & Microbiol, College Stn, TX 77843 USA. [Pierson, Elizabeth A.] Texas A&M Univ, Dept Hort Sci, College Stn, TX 77843 USA. RP Wang, DP (reprint author), Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87544 USA. EM dwang22@lanl.gov; eapierson@tamu.edu OI Chain, Patrick/0000-0003-3949-3634; Dichosa, Armand/0000-0003-0640-6629 FU Laboratory Directed Research and Development (LDRD) program at Los Alamos National Laboratory; USDA NIFA NRI Competitive Grants [2008-35319-21879] FX This project was supported by the Laboratory Directed Research and Development (LDRD) program at Los Alamos National Laboratory and USDA NIFA NRI Competitive Grants project no. 2008-35319-21879. NR 42 TC 3 Z9 3 U1 1 U2 15 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0099-2240 EI 1098-5336 J9 APPL ENVIRON MICROB JI Appl. Environ. Microbiol. PD FEB PY 2015 VL 81 IS 3 BP 890 EP 899 DI 10.1128/AEM.02617-14 PG 10 WC Biotechnology & Applied Microbiology; Microbiology SC Biotechnology & Applied Microbiology; Microbiology GA AZ0CU UT WOS:000347914800010 PM 25416762 ER PT J AU Yang, XR Li, H Nie, SA Su, JQ Weng, BS Zhu, GB Yao, HY Gilbert, JA Zhu, YG AF Yang, Xiao-Ru Li, Hu Nie, San-An Su, Jian-Qiang Weng, Bo-Sen Zhu, Gui-Bing Yao, Huai-Ying Gilbert, Jack A. Zhu, Yong-Guan TI Potential Contribution of Anammox to Nitrogen Loss from Paddy Soils in Southern China SO APPLIED AND ENVIRONMENTAL MICROBIOLOGY LA English DT Article ID ANAEROBIC AMMONIUM OXIDATION; 16S RIBOSOMAL-RNA; CANDIDATUS BROCADIA FULGIDA; IN-SITU DETECTION; OXIDIZING BACTERIA; NITRATE REDUCTION; N-2 PRODUCTION; AGRICULTURAL SOILS; ESTUARINE SEDIMENT; MARINE-SEDIMENTS AB The anaerobic oxidation of ammonium (anammox) process has been observed in diverse terrestrial ecosystems, while the contribution of anammox to N-2 production in paddy soils is not well documented. In this study, the anammox activity and the abundance and diversity of anammox bacteria were investigated to assess the anammox potential of 12 typical paddy soils collected in southern China. Anammox bacteria related to "Candidatus Brocadia" and "Candidatus Kuenenia" and two novel unidentified clusters were detected, with "Candidatus Brocadia" comprising 50% of the anammox population. The prevalence of the anammox was confirmed by the quantitative PCR results based on hydrazine synthase (hzsB) genes, which showed that the abundance ranged from 1.16 x 10(4) to 9.65 x 10(4) copies per gram of dry weight. The anammox rates measured by the isotope-pairing technique ranged from 0.27 to 5.25 nmol N per gram of soil per hour in these paddy soils, which contributed 0.6 to 15% to soil N-2 production. It is estimated that a total loss of 2.50 x 10(6) Mg N per year is linked to anammox in the paddy fields in southern China, which implied that ca. 10% of the applied ammonia fertilizers is lost via the anammox process. Anammox activity was significantly correlated with the abundance of hzsB genes, soil nitrate concentration, and C/N ratio. Additionally, ammonia concentration and pH were found to be significantly correlated with the anammox bacterial structure. C1 [Yang, Xiao-Ru; Li, Hu; Nie, San-An; Su, Jian-Qiang; Weng, Bo-Sen; Yao, Huai-Ying; Zhu, Yong-Guan] Chinese Acad Sci, Inst Urban Environm, Key Lab Urban Environm & Hlth, Xiamen, Peoples R China. [Li, Hu; Nie, San-An] Univ Chinese Acad Sci, Beijing, Peoples R China. [Zhu, Gui-Bing] Chinese Acad Sci, Ecoenvironm Sci Res Ctr, State Key Lab Environm Aquat Qual, Beijing, Peoples R China. [Gilbert, Jack A.] Argonne Natl Lab, Inst Genom & Syst Biol, Lemont, IL USA. [Gilbert, Jack A.] Univ Chicago, Dept Ecol & Evolut, Chicago, IL 60637 USA. RP Zhu, YG (reprint author), Chinese Acad Sci, Inst Urban Environm, Key Lab Urban Environm & Hlth, Xiamen, Peoples R China. EM ygzhu@iue.ac.cn RI Zhu, Yong-Guan/A-1412-2009; Zhu, Guibing/C-2905-2013; CAS, KLUEH/G-8978-2016; Su, Jian Qiang/C-2388-2009; SPRP, XDB150200/N-7373-2016 OI Zhu, Yong-Guan/0000-0003-3861-8482; Zhu, Guibing/0000-0001-7227-8157; Su, Jian Qiang/0000-0003-1875-249X; FU Natural Science Foundation of China [41090282]; Strategic Priority Research Program of Chinese Academy of Sciences [XDB15020300, XDB15020400]; International Science & Technology Cooperation Program of China [2011DFB91710]; U.S. Department of Energy [DE-AC02-06CH11357] FX This study was financially supported by the Natural Science Foundation of China (41090282), the Strategic Priority Research Program of Chinese Academy of Sciences (XDB15020300 and XDB15020400), and the International Science & Technology Cooperation Program of China (2011DFB91710). This work was supported in part by the U.S. Department of Energy under contract DE-AC02-06CH11357. NR 54 TC 14 Z9 16 U1 18 U2 90 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0099-2240 EI 1098-5336 J9 APPL ENVIRON MICROB JI Appl. Environ. Microbiol. PD FEB PY 2015 VL 81 IS 3 BP 938 EP 947 DI 10.1128/AEM.02664-14 PG 10 WC Biotechnology & Applied Microbiology; Microbiology SC Biotechnology & Applied Microbiology; Microbiology GA AZ0CU UT WOS:000347914800015 PM 25416768 ER PT J AU Jacobs, AC Fair, JM Zuk, M AF Jacobs, Anne C. Fair, Jeanne M. Zuk, Marlene TI Parasite infection, but not immune response, influences paternity in western bluebirds SO BEHAVIORAL ECOLOGY AND SOCIOBIOLOGY LA English DT Article DE Avian malaria; Extra-pair paternity; Immunity; Mate choice; Sialia mexicana ID EXTRA-PAIR PATERNITY; SOCIALLY MONOGAMOUS BIRD; ASH-THROATED FLYCATCHERS; MALE EASTERN BLUEBIRDS; TITS PARUS-CAERULEUS; MALARIA PARASITES; REPRODUCTIVE SUCCESS; SEXUAL SELECTION; ECOLOGICAL IMMUNOLOGY; TERRITORIAL BEHAVIOR AB Parasites can impose heavy costs on their hosts, and females may benefit from selecting mates that are parasite resistant and/or have a stronger immune response. Trade-offs between immune response and sexual signaling have been proposed as a mechanism to ensure signal honesty. Much of the work on sexual signaling and immune response does not consider parasites directly and thus cannot confirm whether a stronger immune response necessarily results in lower parasite burdens. Also, immunity is costly, and these costs can lower the overall fitness of individuals with too strong of an immune response. Males with immune responses of intermediate strength are therefore expected to be preferred by females and have the highest reproductive success. We tested whether immune response and blood parasite loads relate to sexual signaling and mating preferences in western bluebirds (Sialia mexicana). Immunity did not predict male reproductive success when considering either within- or extra-pair offspring, although a stronger immune response was correlated with lower parasite loads. However, uninfected males were more likely to sire extra-pair offspring than males infected with avian malaria. Thus, females were more likely to mate with uninfected males but not necessarily males with a stronger immune response. Our results may indicate that females select parasite-resistant males as mates to gain resistance genes for their offspring or that infected males are less likely to pursue extra-pair copulations. C1 [Jacobs, Anne C.] Univ Calif Riverside, Dept Biol, Riverside, CA 92521 USA. [Fair, Jeanne M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Zuk, Marlene] Univ Minnesota, Dept Ecol Evolut & Behav, St Paul, MN 55108 USA. [Jacobs, Anne C.] Allegheny Coll, Dept Biol, Meadville, PA 16335 USA. RP Jacobs, AC (reprint author), Allegheny Coll, Dept Biol, Meadville, PA 16335 USA. EM ajacobs@allegheny.edu FU University of California, Riverside; Los Alamos National Security, LLC under US Department of Energy [DE-AC52-06NA25396]; Sigma Xi; Los Angeles Audubon's Society; National Science Foundation Doctoral Dissertation Improvement Grant FX We are grateful to K. Burnett, C. Hathcock, D. Keller, L. Maestas, R. Robinson, L. Reader, and C. Lemanski for assistance in the field. We thank B. Faircloth, J. Burnette, L. Enders, L. Nunney, and A. Cortez for invaluable advice and assistance regarding the molecular analyses. We thank Y. Shou, K. McCabe, E. Hong-Geller, and the Bradbury lab for assistance with the immune assays and M. Venesky for help with the statistical analyses. This project was funded by the University of California, Riverside and Los Alamos National Security, LLC, operator of the Los Alamos National Laboratory under contract no. DE-AC52-06NA25396 with the US Department of Energy. Additional funding for molecular work was provided by a Sigma Xi Grant-in-Aid-of-Research, a Ralph Schreiber Memorial Award from the Los Angeles Audubon's Society, and a National Science Foundation Doctoral Dissertation Improvement Grant awarded to ACJ. NR 76 TC 2 Z9 3 U1 13 U2 76 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0340-5443 EI 1432-0762 J9 BEHAV ECOL SOCIOBIOL JI Behav. Ecol. Sociobiol. PD FEB PY 2015 VL 69 IS 2 BP 193 EP 203 DI 10.1007/s00265-014-1832-6 PG 11 WC Behavioral Sciences; Ecology; Zoology SC Behavioral Sciences; Environmental Sciences & Ecology; Zoology GA AY8QM UT WOS:000347818500003 ER PT J AU Kent, AD Liebrock, LM Neil, JC AF Kent, Alexander D. Liebrock, Lone M. Neil, Joshua C. TI Authentication graphs: Analyzing user behavior within an enterprise network SO COMPUTERS & SECURITY LA English DT Article DE User authentication; Network authentication; Graph analysis; Intrusion detection; Cyber security; Enterprise security ID ALGORITHMS; MODEL AB User authentication over the network builds a foundation of trust within large-scale computer networks. The collection of this network authentication activity provides valuable insight into user behavior within an enterprise network. Representing this authentication data as a set of user-specific graphs and graph features, including time-constrained attributes, enables novel and comprehensive analysis opportunities. We show graph-based approaches to user classification and intrusion detection with practical results. We also show a method for assessing network authentication trust risk and cyber attack mitigation within an enterprise network using bipartite authentication graphs. We demonstrate the value of these graph-based approaches on a real-world authentication data set collected from an enterprise network. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Kent, Alexander D.; Neil, Joshua C.] Los Alamos Natl Lab, Los Alamos, NM USA. [Liebrock, Lone M.] New Mexico Inst Min & Technol, Socorro, NM 87801 USA. RP Kent, AD (reprint author), Los Alamos Natl Lab, Los Alamos, NM USA. EM alex@lanl.gov; liebrock@cs.nmt.edu; jneil@lanl.gov FU U.S. Department of Energy [DE-AC52-06NA25396] FX A number of people contributed to the success of this research. First, we would like to thank Aric Hagberg for pointing out the simplicity of arc traversal over vertex traversal for our time-constrained breadth-first search algorithm. We appreciate Subhashish Mazumdar's help in reviewing and validating the time-constrained algorithm. Finally, we are grateful for the reviews and suggestions from Aric, Pieter Swart, Nathan Lemons, Mike Fisk, and Feng Pan. This work was funded, in part, by the U.S. Department of Energy under contract DE-AC52-06NA25396. NR 41 TC 7 Z9 7 U1 0 U2 11 PU ELSEVIER ADVANCED TECHNOLOGY PI OXFORD PA OXFORD FULFILLMENT CENTRE THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0167-4048 EI 1872-6208 J9 COMPUT SECUR JI Comput. Secur. PD FEB PY 2015 VL 48 BP 150 EP 166 DI 10.1016/j.cose.2014.09.001 PG 17 WC Computer Science, Information Systems SC Computer Science GA AY7UD UT WOS:000347763300010 ER PT J AU Liu, G Tomsovic, K AF Liu, G. Tomsovic, K. TI Robust unit commitment considering uncertain demand response SO ELECTRIC POWER SYSTEMS RESEARCH LA English DT Article DE Unit commitment; Price elasticity; Demand response; Uncertainty; Robust optimization; Locational Marginal Price (LMP) ID WIND POWER-GENERATION; ENERGY/RESERVE ELECTRICITY MARKETS; PROBABILISTIC SPINNING RESERVE; ECONOMIC-DISPATCH; OPTIMIZATION; SECURITY; ENERGY; JOINT; SCUC AB Although price responsive demand response has been widely accepted as playing an important role in the reliable and economic operation of power system, the real response from demand side can be highly uncertain due to limited understanding of consumers' response to pricing signals. To model the behavior of consumers, the price elasticity of demand has been explored and utilized in both research and real practice. However, the price elasticity of demand is not precisely known and may vary greatly with operating conditions and types of customers. To accommodate the uncertainty of demand response, alternative unit commitment methods robust to the uncertainty of the demand response require investigation. In this paper, a robust unit commitment model to minimize the generalized social cost is proposed for the optimal unit commitment decision taking into account uncertainty of the price elasticity of demand. By optimizing the worst case under proper robust level, the unit commitment solution of the proposed model is robust against all possible realizations of the modeled uncertain demand response. Numerical simulations on the IEEE Reliability Test System show the effectiveness of the method. Compared to unit commitment with deterministic price elasticity of demand, the proposed robust model can reduce the average Locational Marginal Prices (LMPs) as well as the price volatility. (C) 2014 Elsevier B.V. All rights reserved. C1 [Liu, G.] Oak Ridge Natl Lab, Power & Energy Syst Grp, Oak Ridge, TN 37831 USA. [Tomsovic, K.] Univ Tennessee, Dept Elect Engn & Comp Sci, Knoxville, TN 37996 USA. RP Liu, G (reprint author), Oak Ridge Natl Lab, Power & Energy Syst Grp, One Bethel Valley Rd,POB 2008,MS-6070, Oak Ridge, TN 37831 USA. EM liug@ornl.gov; tomsovic@utk.edu FU Office of Electricity Delivery & Energy Reliability, U.S. Department of Energy [DE-AC05-000R22725]; National Science Foundation; Department of Energy under NSF [EEC-1041877]; CURENT Industry Partnership Program FX This work was sponsored by the Office of Electricity Delivery & Energy Reliability, U.S. Department of Energy under Contract No. DE-AC05-000R22725 with UT-Battelle and conducted at ORNL and UT Knoxville. This work also made use of Engineering Research Center Shared Facilities supported by the Engineering Research Center Program of the National Science Foundation and the Department of Energy under NSF Award Number EEC-1041877 and the CURENT Industry Partnership Program. NR 43 TC 4 Z9 6 U1 4 U2 21 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0378-7796 EI 1873-2046 J9 ELECTR POW SYST RES JI Electr. Power Syst. Res. PD FEB PY 2015 VL 119 BP 126 EP 137 DI 10.1016/j.epsr.2014.09.006 PG 12 WC Engineering, Electrical & Electronic SC Engineering GA AY7RM UT WOS:000347756700015 ER PT J AU Mousavian, S Valenzuela, J Wang, JH AF Mousavian, Seyedamirabbas Valenzuela, Jorge Wang, Jianhui TI A two-phase investment model for optimal allocation of phasor measurement units considering transmission switching SO ELECTRIC POWER SYSTEMS RESEARCH LA English DT Article DE Phasor measurement unit; Optimal placement; Network observability; Transmission switching; Integer linear programming; Two-phase investment model ID POWER-SYSTEM OBSERVABILITY; OPTIMAL PMU PLACEMENT; ALGORITHM; SEARCH; FLOW AB Ensuring the reliability of an electrical power system requires a wide-area monitoring and full observability of the state variables. Phasor measurement units (PMUs) collect in real time synchronized phasors of voltages and currents which are used for the observability of the power grid. Due to the considerable cost of installing PMUs, it is not possible to equip all buses with PMUs. In this paper, we propose an integer linear programming model to determine the optimal PMU placement plan in two investment phases. In the first phase, PMUs are installed to achieve full observability of the power grid whereas additional PMUs are installed in the second phase to guarantee the N-1 observability of the power grid. The proposed model also accounts for transmission switching and single contingencies such as failure of a PMU or a transmission line. Results are provided on several IEEE test systems which show that our proposed approach is a promising enhancement to the methods available for the optimal placement of PMUs. (C) 2014 Elsevier B.V. All rights reserved. C1 [Mousavian, Seyedamirabbas] Clarkson Univ, Sch Business, Potsdam, NY 13699 USA. [Valenzuela, Jorge] Auburn Univ, Dept Ind & Syst Engn, Auburn, AL 36849 USA. [Wang, Jianhui] Argonne Natl Lab, Argonne, IL 60439 USA. RP Mousavian, S (reprint author), Clarkson Univ, Sch Business, Potsdam, NY 13699 USA. EM amir@clarkson.edu NR 24 TC 2 Z9 2 U1 0 U2 3 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0378-7796 EI 1873-2046 J9 ELECTR POW SYST RES JI Electr. Power Syst. Res. PD FEB PY 2015 VL 119 BP 492 EP 498 DI 10.1016/j.epsr.2014.10.025 PG 7 WC Engineering, Electrical & Electronic SC Engineering GA AY7RM UT WOS:000347756700055 ER PT J AU Shah, N Sathaye, N Phadke, A Letschert, V AF Shah, Nihar Sathaye, Nakul Phadke, Amol Letschert, Virginie TI Efficiency improvement opportunities for ceiling fans SO ENERGY EFFICIENCY LA English DT Article DE Ceiling fan; Energy efficiency; Standards; Labeling; Incentives; Market transformation AB Ceiling fans contribute significantly to residential electricity consumption, especially in developing countries with warm climates. This paper provides an analysis of costs and benefits of several options to improve the efficiency of ceiling fans to assess the global potential for electricity savings and green house gas (GHG) emission reductions. Ceiling fan efficiency can be cost-effectively improved by at least 50 % using commercially available technology. If these efficiency improvements are implemented in all ceiling fans sold by 2020, 70 TWh/year could be saved and 25 million metric tons of carbon dioxide equivalent (CO2-e) emissions per year could be avoided, globally. We assess how policies and programs such as standards, labels, and financial incentives can be used to accelerate the adoption of efficient ceiling fans in order to realize potential savings. C1 [Shah, Nihar; Sathaye, Nakul; Phadke, Amol; Letschert, Virginie] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Energy Anal Dept, Berkeley, CA 94720 USA. RP Shah, N (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Energy Anal Dept, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM nkshah@lbl.gov FU Bureau of Oceans and International Environmental and Scientific Affairs, US Department of State; SEAD initiative through the US Department of Energy [DE-AC02-05CH11231] FX This work was funded by the Bureau of Oceans and International Environmental and Scientific Affairs, US Department of State, and administered by the US Department of Energy in support of the SEAD initiative through the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 27 TC 0 Z9 0 U1 0 U2 10 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 1570-646X EI 1570-6478 J9 ENERG EFFIC JI Energy Effic. PD FEB PY 2015 VL 8 IS 1 BP 37 EP 50 DI 10.1007/s12053-014-9274-6 PG 14 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels; Environmental Studies SC Science & Technology - Other Topics; Energy & Fuels; Environmental Sciences & Ecology GA AY4NA UT WOS:000347554100003 ER PT J AU Evans, JM Jenkins, RA Ilgner, RH Knapp, CF Zhang, QG Patwardhan, AR AF Evans, Joyce M. Jenkins, Roger A. Ilgner, Ralph H. Knapp, Charles F. Zhang, Qingguang Patwardhan, Abhijit R. TI Acute cardiovascular autonomic responses to inhaled particulates SO EUROPEAN JOURNAL OF APPLIED PHYSIOLOGY LA English DT Article DE Autonomic control; Baroreflex; Blood pressure variability; Cooking oil; ETS; Gender; Heart rate variability; Wood smoke ID ENVIRONMENTAL TOBACCO-SMOKE; HEART-RATE-VARIABILITY; CIGARETTE-SMOKING; AIR-POLLUTION; EXPOSURE; DISEASE; VASOCONSTRICTION; ADULTS; BAROREFLEX AB Harmful effects of inhaled particulates have been established in epidemiologic studies of ambient air pollution. In particular, heart rate variability responses to high levels of environmental tobacco smoke (ETS), similar to responses observed during direct smoking, have been reported. We sought to determine whether such responses could be observed at lower particulate concentrations. We monitored cardiovascular responses of non-smoking 21 women and 19 men to work-place-relevant levels of: ETS, cooking oil fumes (Coil), wood smoke (WS), and water vapor as sham control. Responses, tested on three consecutive days (random order of aerosol presentation), were averaged for each subject. Low frequency spectral powers of heart rate and blood pressure rose during recovery from exposure to particulate, but not to sham exposures. At breathing frequencies, spectral power of men's systolic pressure doubled, and baroreflex effectiveness increased, following ETS exposure. An index of sympathetic control of heart rate was more pronounced in men than women, in response to ETS and Coil, compared to WS and sham. When measured under controlled conditions, autonomic activities in non-smoking men and women exposed to low level, short term, particulate concentrations were similar to those observed during longer term, higher level exposures to ETS and to direct smoking. These increased indexes of sympathetic control of heart rate and peripheral vasomotion followed introduction of particulates by about 15 min. Finally, coupling of heart rate and systolic pressure indicated an increase in baroreflex activity in the response to breathing ETS that was less effective in men than women. C1 [Evans, Joyce M.; Knapp, Charles F.; Zhang, Qingguang; Patwardhan, Abhijit R.] Univ Kentucky, Dept Biomed Engn, Lexington, KY 40506 USA. [Jenkins, Roger A.; Ilgner, Ralph H.] Oak Ridge Natl Lab, Oak Ridge, TN USA. RP Evans, JM (reprint author), Univ Kentucky, Dept Biomed Engn, 143 Graham Ave, Lexington, KY 40506 USA. EM jevans1@uky.edu OI Zhang, Qingguang/0000-0003-4500-813X FU Philip Morris External Research Program; US Department of Energy [ERD0302351]; U.S. Government [DE-AC05-00OR22725] FX M. Mahadevappa, for assistance in conduct of studies and data archiving, C. Ferguson, G.E. Baxter and A. Jayanthi, for data analysis and figure preparation, P. Amick of Amick Research for help with questionnaire development and subject recruitment, E. Hartman, for data acquisition hardware and software development. This work was funded by a Philip Morris External Research Program Grant to the University of Kentucky. Oak Ridge National Laboratory's participation was via subcontract No. ERD0302351 with the US Department of Energy. This manuscript has been authored by a contractor of the U.S. Government under contract DE-AC05-00OR22725. Accordingly, the U.S. Government retains a paid-up, nonexclusive, irrevocable, worldwide license to publish or reproduce the published form of this contribution, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, or allow others to do so, for U.S. Government purposes. NR 33 TC 1 Z9 1 U1 1 U2 9 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1439-6319 EI 1439-6327 J9 EUR J APPL PHYSIOL JI Eur. J. Appl. Physiol. PD FEB PY 2015 VL 115 IS 2 BP 257 EP 268 DI 10.1007/s00421-014-2998-3 PG 12 WC Physiology; Sport Sciences SC Physiology; Sport Sciences GA AY7FD UT WOS:000347725800004 PM 25272970 ER PT J AU Gagne, RB Hogan, JD Pracheil, BM Mcintyre, PB Hain, EF Gilliam, JF Blum, MJ AF Gagne, Roderick B. Hogan, J. Derek Pracheil, Brenda M. Mcintyre, Peter B. Hain, Ernie F. Gilliam, James F. Blum, Michael J. TI Spread of an introduced parasite across the Hawaiian archipelago independent of its introduced host SO FRESHWATER BIOLOGY LA English DT Article DE Awaous stamineus; biological invasions; enemy addition; parasite; Camallanus cotti ID CAMALLANUS-COTTI NEMATODA; FRESH-WATER FISHES; GENETIC DIVERSITY; LAND-USE; CONSEQUENCES; INVASIONS; COMMUNITIES; INFECTIONS; SELECTION; ECOSYSTEM AB Co-introductions of non-native parasites with non-native hosts can be a major driver of disease emergence in native species, but the conditions that promote the establishment and spread of non-native parasites remain poorly understood. Here, we characterise the infection of a native host species by a non-native parasite relative to the distribution and density of the original non-native host species and a suite of organismal and environmental factors that have been associated with parasitism, but not commonly considered within a single system. We examined the native Hawaiian goby Awaous stamineus across 23 catchments on five islands for infection by the non-native nematode parasite Camallanus cotti. We used model selection to test whether parasite infection was associated with the genetic diversity, size and population density of native hosts, the distribution and density of non-native hosts, land use and water quality. We found that the distribution of non-native C.cotti parasites has become decoupled from the non-native hosts that were primary vectors of introduction to the Hawaiian Islands. Although no single intrinsic or extrinsic factor was identified that best explains parasitism of A.stamineus by C.cotti, native host size, population density and water quality were consistently identified as influencing parasite intensity and prevalence. The introduction of non-native species can indirectly influence native species through infection of co-introduced parasites. Here, we show that the effects of enemy addition' can extend beyond the range of non-native hosts through the independent spread of non-native parasites. This suggests that control of non-native hosts is not sufficient to halt the spread of introduced parasites. Designing importation regulations to prevent host-parasite co-introductions can promote native species conservation, even in remote areas that may not seem susceptible to human influence. C1 [Gagne, Roderick B.; Hogan, J. Derek; Blum, Michael J.] Tulane Univ, Dept Ecol & Evolutionary Biol, New Orleans, LA 70810 USA. [Hogan, J. Derek] Texas A&M Corpus Christi, Dept Life Sci, Corpus Christi, TX USA. [Hogan, J. Derek; Pracheil, Brenda M.; Mcintyre, Peter B.] Univ Wisconsin, Ctr Limnol, Madison, WI 53706 USA. [Pracheil, Brenda M.] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Hain, Ernie F.; Gilliam, James F.] N Carolina State Univ, Dept Biol, Raleigh, NC 27695 USA. RP Gagne, RB (reprint author), Tulane Univ, 400 Lindy Boggs, New Orleans, LA 70810 USA. EM rgagne@tulane.edu FU US Department of Defense Strategic Environmental Research Development Program (SERDP) [RC-1646] FX We thank C. Criscione for laboratory training assistance, E. Childress, J. Fenner, G. Glotzbecker, T. Haas, B. Lamphere, D.P. Lindstrom, K. Moody, D. Oele, T. Rayner, J. Rossa, R.P. Walter for field assistance, J. Thore and E. Hamann for laboratory analyses, N. Keutler and P. Crump for assistance with statistical analysis and two anonymous reviewers that provided useful comments that greatly improved this manuscript. This study was funded by the US Department of Defense Strategic Environmental Research Development Program (SERDP) through project RC-1646. NR 66 TC 7 Z9 7 U1 4 U2 29 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0046-5070 EI 1365-2427 J9 FRESHWATER BIOL JI Freshw. Biol. PD FEB PY 2015 VL 60 IS 2 BP 311 EP 322 DI 10.1111/fwb.12491 PG 12 WC Marine & Freshwater Biology SC Marine & Freshwater Biology GA AY6XP UT WOS:000347706400007 ER PT J AU Pezzini, P Celestin, S Tucker, D AF Pezzini, Paolo Celestin, Sue Tucker, David TI Control Impacts of Cold-Air Bypass on Pressurized Fuel Cell Turbine Hybrids SO JOURNAL OF FUEL CELL SCIENCE AND TECHNOLOGY LA English DT Article AB A pressure drop analysis for a direct-fired fuel cell turbine hybrid power system was evaluated using a hardware-based simulation of an integrated gasifier/fuel cell/turbine hybrid cycle, implemented through the hybrid performance (Hyper) project at the National Energy Technology Laboratory, U.S. Department of Energy (NETL). The Hyper facility is designed to explore dynamic operation of hybrid systems and quantitatively characterize such transient behavior. It is possible to model, test, and evaluate the effects of different parameters on the design and operation of a gasifier/fuel cell/gas turbine hybrid system and provide means of evaluating risk mitigation strategies. The cold-air bypass in the Hyper facility directs compressor discharge flow to the turbine inlet duct, bypassing the fuel cell, and exhaust gas recuperators in the system. This valve reduces turbine inlet temperature while reducing cathode airflow, but significantly improves compressor surge margin. Regardless of the reduced turbine inlet temperature as the valve opens, a peak in turbine efficiency is observed during characterization of the valve at the middle of the operating range. A detailed experimental analysis shows the unusual behavior during steady state and transient operation, which is considered a key point for future control strategies in terms of turbine efficiency optimization and cathode airflow control. C1 [Pezzini, Paolo] Univ Genoa, Thermochem Power Grp TPG DIME, I-16100 Genoa, Italy. [Celestin, Sue] Northeastern Univ, Dept Chem Engn, Boston, MA 02115 USA. [Tucker, David] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. RP Tucker, D (reprint author), US DOE, Natl Energy Technol Lab, 3610 Collins Ferry Rd 26505, Morgantown, WV 26507 USA. EM david.tucker@netl.doe.gov FU U.S. Department of Energy Crosscutting Research program FX This work was funded by the U.S. Department of Energy Crosscutting Research program, administered through the National Energy Technology Laboratory. Student support was provided through the U.S. Department of Energy, Mickey Leland Program. This work was also developed in collaboration with both Woodward Industrial Controls (Woodward), the Thermochemical Power Group of the University of Genoa (Italy). NR 8 TC 3 Z9 3 U1 2 U2 4 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 1550-624X EI 1551-6989 J9 J FUEL CELL SCI TECH JI J. Fuel Cell Sci. Technol. PD FEB PY 2015 VL 12 IS 1 AR 011006 DI 10.1115/1.4029083 PG 8 GA AZ2GA UT WOS:000348051300006 ER PT J AU Zhou, N Yang, C Tucker, D AF Zhou, Nana Yang, Chen Tucker, David TI Evaluation of Cathode Air Flow Transients in a SOFC/GT Hybrid System Using Hardware in the Loop Simulation SO JOURNAL OF FUEL CELL SCIENCE AND TECHNOLOGY LA English DT Article ID OXIDE FUEL-CELL; THERMAL MANAGEMENT; POWER AB Thermal management in the fuel cell component of a direct fired solid oxide fuel cell gas turbine (SOFC/GT) hybrid power system can be improved by effective management and control of the cathode airflow. The disturbances of the cathode airflow were accomplished by diverting air around the fuel cell system through the manipulation of a hot-air bypass valve in open loop experiments, using a hardware-based simulation facility designed and built by the U.S. Department of Energy, National Energy Technology Laboratory (NETL). The dynamic responses of the fuel cell component and hardware component of the hybrid system were studied in this paper. C1 [Zhou, Nana; Yang, Chen] Chongqing Univ, Coll Power Engn, Chongqing 400044, Peoples R China. [Tucker, David] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. RP Zhou, N (reprint author), Chongqing Univ, Coll Power Engn, 174 Shazhengjie, Chongqing 400044, Peoples R China. EM zhounana.cqu@gmail.com; yxtyc@cqu.edu.cn; David.Tucker@netl.doe.gov FU Crosscutting Research program; U.S. Department of Energy Crosscutting Research program FX This work was funded by the Crosscutting Research program implemented through the U.S. Department of Energy, National Energy Technology Laboratory (NETL). The authors would like to acknowledge Paolo Pezzini and Nor Farida Harun for their effort in operating the HyPer facility. Also, the authors would like to express the gratitude to the China Scholarship Council (CSC). This work was funded by the U.S. Department of Energy Crosscutting Research program, administered through the National Energy Technology Laboratory. NR 14 TC 2 Z9 2 U1 1 U2 9 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 1550-624X EI 1551-6989 J9 J FUEL CELL SCI TECH JI J. Fuel Cell Sci. Technol. PD FEB PY 2015 VL 12 IS 1 AR 011003 DI 10.1115/1.4028950 PG 7 GA AZ2GA UT WOS:000348051300003 ER PT J AU Abbink, P Maxfield, LF Ng'ang'a, D Borducchi, EN Iampietro, MJ Bricault, CA Teigler, JE Blackmore, S Parenteau, L Wagh, K Handley, SA Zhao, GY Virgin, HW Korber, B Barouch, DH AF Abbink, Peter Maxfield, Lori F. Ng'ang'a, David Borducchi, Erica N. Iampietro, M. Justin Bricault, Christine A. Teigler, Jeffrey E. Blackmore, Stephen Parenteau, Lily Wagh, Kshitij Handley, Scott A. Zhao, Guoyan Virgin, Herbert W. Korber, Bette Barouch, Dan H. TI Construction and Evaluation of Novel Rhesus Monkey Adenovirus Vaccine Vectors SO JOURNAL OF VIROLOGY LA English DT Article ID HIV-1 ENV VACCINE; NEUTRALIZING ANTIBODIES; CHIMPANZEE ADENOVIRUS; CYTOKINE RESPONSES; IPCAVD 001; SPECIES D; VIRUS; IMMUNOGENICITY; IMMUNITY; GENE AB Adenovirus vectors are widely used as vaccine candidates for a variety of pathogens, including HIV-1. To date, human and chimpanzee adenoviruses have been explored in detail as vaccine vectors. The phylogeny of human and chimpanzee adenoviruses is overlapping, and preexisting humoral and cellular immunity to both are exhibited in human populations worldwide. More distantly related adenoviruses may therefore offer advantages as vaccine vectors. Here we describe the primary isolation and vectorization of three novel adenoviruses from rhesus monkeys. The seroprevalence of these novel rhesus monkey adenovirus vectors was extremely low in sub-Saharan Africa human populations, and these vectors proved to have immunogenicity comparable to that of human and chimpanzee adenovirus vaccine vectors in mice. These rhesus monkey adenoviruses phylogenetically clustered with the poorly described adenovirus species G and robustly stimulated innate immune responses. These novel adenoviruses represent a new class of candidate vaccine vectors. IMPORTANCE Although there have been substantial efforts in the development of vaccine vectors from human and chimpanzee adenoviruses, far less is known about rhesus monkey adenoviruses. In this report, we describe the isolation and vectorization of three novel rhesus monkey adenoviruses. These vectors exhibit virologic and immunologic characteristics that make them attractive as potential candidate vaccine vectors for both HIV-1 and other pathogens. C1 [Abbink, Peter; Maxfield, Lori F.; Ng'ang'a, David; Borducchi, Erica N.; Iampietro, M. Justin; Bricault, Christine A.; Teigler, Jeffrey E.; Blackmore, Stephen; Parenteau, Lily; Barouch, Dan H.] Harvard Univ, Beth Israel Deaconess Med Ctr, Sch Med, Ctr Virol & Vaccine Res, Boston, MA 02215 USA. [Barouch, Dan H.] Ragon Inst MGH MIT & Harvard, Boston, MA USA. [Wagh, Kshitij; Korber, Bette] Los Alamos Natl Lab, Los Alamos, NM USA. [Wagh, Kshitij; Korber, Bette] New Mexico Consortium, Los Alamos, NM USA. [Handley, Scott A.; Zhao, Guoyan; Virgin, Herbert W.] Washington Univ, Sch Med, Dept Pathol & Immunol, St Louis, MO USA. RP Barouch, DH (reprint author), Harvard Univ, Beth Israel Deaconess Med Ctr, Sch Med, Ctr Virol & Vaccine Res, Boston, MA 02215 USA. EM dbarouch@bidmc.harvard.edu OI Korber, Bette/0000-0002-2026-5757 FU Bill and Melinda Gates Foundation [OPP1040741]; Ragon Institute of MGH; MIT; Harvard; [OD011170]; [AI078526]; [AI084794]; [AI096040] FX We acknowledge support from grants OD011170, AI078526, AI084794, and AI096040; Bill and Melinda Gates Foundation grant OPP1040741; and the Ragon Institute of MGH, MIT, and Harvard. NR 48 TC 7 Z9 8 U1 3 U2 8 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0022-538X EI 1098-5514 J9 J VIROL JI J. Virol. PD FEB PY 2015 VL 89 IS 3 BP 1512 EP 1522 DI 10.1128/JVI.02950-14 PG 11 WC Virology SC Virology GA AY8QJ UT WOS:000347818100004 PM 25410856 ER PT J AU Bailey, DH Borwein, D Borwein, JM AF Bailey, David H. Borwein, David Borwein, Jonathan M. TI On Eulerian log-gamma integrals and Tornheim-Witten zeta functions SO RAMANUJAN JOURNAL LA English DT Article DE Gamma function; Log gamma function; Riemann zeta function; Tornheim-Weitten zeta function; Integration ID DOUBLE SUMS AB Stimulated by earlier work by Moll and his coworkers (Amdeberhan et al., Proc. Am. Math. Soc., 139(2): 535-545, 2010), we evaluate various basic log Gamma integrals in terms of partial derivatives of Tornheim-Witten zeta functions and their extensions arising from evaluations of Fourier series. In particular, we fully evaluate LG(n) = integral(1)(0) log(n) Gamma(x) dx for 1 <= n <= 4 and make some comments regarding the general case. The subsidiary computational challenges are substantial, interesting and significant in their own right. C1 [Bailey, David H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Borwein, David] Univ Western Ontario, Dept Math, London, ON N6A 5B7, Canada. [Borwein, Jonathan M.] Univ Newcastle, Sch Math & Phys Sci, Ctr Comp Assisted Res Math & Its Applicat CARMA, Callaghan, NSW 2308, Australia. [Borwein, Jonathan M.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. RP Bailey, DH (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM DHBailey@lbl.gov; dborwein@uwo.ca; jonathan.borwein@newcastle.edu.au OI Borwein, Jonathan/0000-0002-1263-0646 FU Office of Computational and Technology Research, Division of Mathematical, Information, and Computational Sciences of the US Department of Energy [DE-AC02-05CH11231]; Australian Research Council; University of Newcastle FX D.H. Bailey was supported in part by the Director, Office of Computational and Technology Research, Division of Mathematical, Information, and Computational Sciences of the US Department of Energy, under contract number DE-AC02-05CH11231.; J.M. Borwein was supported in part by the Australian Research Council and the University of Newcastle. NR 17 TC 3 Z9 3 U1 0 U2 0 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 1382-4090 EI 1572-9303 J9 RAMANUJAN J JI Ramanujan J. PD FEB PY 2015 VL 36 IS 1-2 BP 43 EP 68 DI 10.1007/s11139-012-9427-1 PG 26 WC Mathematics SC Mathematics GA AY6UT UT WOS:000347701700003 ER PT J AU Leng, GY Tang, QH Huang, MY Leung, LYR AF Leng, Guoyong Tang, Qiuhong Huang, Maoyi Leung, Lai-yung Ruby TI A comparative analysis of the impacts of climate change and irrigation on land surface and subsurface hydrology in the North China Plain SO REGIONAL ENVIRONMENTAL CHANGE LA English DT Article DE Climate change; Irrigation; Land surface/subsurface hydrology; North China Plain ID US HIGH-PLAINS; GROUNDWATER EXPLOITATION; DISTRICT SPAIN; CENTRAL VALLEY; UNITED-STATES; WATER CYCLE; SUSTAINABILITY; VARIABILITY; SALT; PRECIPITATION AB Few studies have investigated the similar/different characteristics of regional environmental changes induced by climate change and human activities (e.g., irrigation, groundwater pumping). In this study, three climate change scenarios and one irrigation scenario were simulated using the Community Land Model 4.0 to investigate and compare the water-related environmental changes induced by climate change and irrigation in the North China Plain (NCP). Compared to future change climate scenarios, extensive groundwater-fed irrigation in the NCP could have similar magnitude of effects on land surface fluxes and states, but with much larger effects on subsurface water fluxes/states. For example, it was found that groundwater-fed irrigation has led to the decrease of annual mean water table depth by 1 m in major agricultural areas of the NCP while climate change has negligible impacts on water table depth. That is, human water use tends to dominate the subsurface water balance in the NCP. Moreover, climate change and irrigation exhibited different effects on the vertical profile of soil column. That is, irrigation appears to have much larger effects on the top layer soil moisture (SM) whereas increase in precipitation associated with climate change exerts more influence on lower layer SM. Through indentifying the similar/different characteristics between climate change and irrigation, our results highlight the importance of exactly accounting for the effects of human water use and could provide guidance for determining effective measures for adapting to environmental changes induced by climate change and human water use for this region. C1 [Leng, Guoyong; Tang, Qiuhong] Chinese Acad Sci, Inst Geog Sci & Nat Resources Res, Beijing 100101, Peoples R China. [Leng, Guoyong] Univ Chinese Acad Sci, Beijing 100049, Peoples R China. [Huang, Maoyi; Leung, Lai-yung Ruby] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. RP Leng, GY (reprint author), Chinese Acad Sci, Inst Geog Sci & Nat Resources Res, Beijing 100101, Peoples R China. EM lenggy.11b@igsnrr.ac.cn RI Huang, Maoyi/I-8599-2012; OI Huang, Maoyi/0000-0001-9154-9485; Tang, Qiuhong/0000-0002-0886-6699 FU National Natural Science Foundation of China [41171031]; National Basic Research Program of China [2012CB955403]; Hundred Talents Program of the Chinese Academy of Sciences; U.S. Department of Energy Regional and Global Climate Modeling Program through the U.S. Department of Energy; U.S. Department of Energy Regional and Global Climate Modeling Program through the China Ministry of Science and Technology; US DOE by Battelle Memorial Institute [DE-AC05-76RL01830] FX This work was supported by the National Natural Science Foundation of China (Grant No. 41171031), National Basic Research Program of China (Grant No. 2012CB955403), and Hundred Talents Program of the Chinese Academy of Sciences. M. Huang and L. R. Leung are supported by the U.S. Department of Energy Regional and Global Climate Modeling Program through the bilateral agreement between U.S. Department of Energy and China Ministry of Science and Technology on regional climate research. PNNL is operated for the US DOE by Battelle Memorial Institute under Contract DE-AC05-76RL01830. The authors thank two anonymous reviewers for their valuable comments that were helpful in improving this manuscript. NR 48 TC 5 Z9 6 U1 8 U2 40 PU SPRINGER HEIDELBERG PI HEIDELBERG PA TIERGARTENSTRASSE 17, D-69121 HEIDELBERG, GERMANY SN 1436-3798 EI 1436-378X J9 REG ENVIRON CHANGE JI Reg. Envir. Chang. PD FEB PY 2015 VL 15 IS 2 BP 251 EP 263 DI 10.1007/s10113-014-0640-x PG 13 WC Environmental Sciences; Environmental Studies SC Environmental Sciences & Ecology GA AY6XE UT WOS:000347705300004 ER PT J AU Dubey, A Weide, K Lee, D Bachan, J Daley, C Olofin, S Taylor, N Rich, PM Reid, LB AF Dubey, Anshu Weide, Klaus Lee, Dongwook Bachan, John Daley, Christopher Olofin, Samuel Taylor, Noel Rich, Paul M. Reid, Lynn B. TI Ongoing verification of a multiphysics community code: FLASH SO SOFTWARE-PRACTICE & EXPERIENCE LA English DT Article DE multiple platforms; parallel computing; regression testing; verification AB When developing a complex, multi-authored code, daily testing on multiple platforms and under a variety of conditions is essential. It is therefore necessary to have a regression test suite that is easily administered and configured, as well as a way to easily view and interpret the test suite results. We describe the methodology for verification of FLASH, a highly capable multiphysics scientific application code with a wide user base. The methodology uses a combination of unit and regression tests and an in-house testing software that is optimized for operation under limited resources. Although our practical implementations do not always comply with theoretical regression-testing research, our methodology provides a comprehensive verification of a large scientific code under resource constraints.Copyright (c) 2013 John Wiley & Sons, Ltd. C1 [Dubey, Anshu; Weide, Klaus; Lee, Dongwook; Bachan, John; Daley, Christopher; Olofin, Samuel; Taylor, Noel] Univ Chicago, Flash Ctr Computat Sci, Chicago, IL 60637 USA. [Dubey, Anshu] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. [Rich, Paul M.] Argonne Natl Lab, ALCF, Argonne, IL 60439 USA. [Reid, Lynn B.] Univ Western Australia, Crawley, WA, Australia. RP Dubey, A (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. EM adubey@lbl.gov OI Weide, Klaus/0000-0001-9869-9750 FU US DOE NNSA ASC at the ASC/Alliance Center for Astrophysical Thermonuclear Flashes [B523820] FX The development of the FLASH code has been supported in part by the US DOE NNSA ASC, first at the ASC/Alliance Center for Astrophysical Thermonuclear Flashes under grant B523820, and later, through the Argonne Institute for Computing in Science under field work proposal 57789 at the Flash Center for Computational Science at the University of Chicago. NR 0 TC 1 Z9 1 U1 0 U2 0 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0038-0644 EI 1097-024X J9 SOFTWARE PRACT EXPER JI Softw.-Pract. Exp. PD FEB PY 2015 VL 45 IS 2 BP 233 EP 244 DI 10.1002/spe.2220 PG 12 WC Computer Science, Software Engineering SC Computer Science GA AY4FJ UT WOS:000347533400005 ER PT J AU Kanevce, A Repins, I Wei, SH AF Kanevce, Ana Repins, Ingrid Wei, Su-Huai TI Impact of bulk properties and local secondary phases on the Cu-2(Zn,Sn)Se-4 solar cells open-circuit voltage SO SOLAR ENERGY MATERIALS AND SOLAR CELLS LA English DT Article DE Numerical simulations; CZTSe solar cells; Device performance ID THIN-FILM PHOTOVOLTAICS; GRAIN-BOUNDARY; EFFICIENCY; PERFORMANCE; INTERFACE; GROWTH; ZNO AB As the development of kesterite solar cells accelerates, the bottlenecks in device performance need to be identified and ways for their circumvention defined and developed. In this work, we use 2-dimensional (2D) numerical simulations to explore possible reasons for low open-circuit voltage (V-oc) in Cu-2(Zn,Sn) Se-4 (CZTSe) solar cells. High defect density in the CZTSe absorber and at the CZTSe/CdS interface can be significant reasons for V-oc deficit, but they do not explain all of the losses observed experimentally. Local deviation from stoichiometry could create secondary phases with a lower band gap compared to the absorber. These secondary phases can be severely harmful to V-oc if located in the vicinity of the heterointerface and along the grain boundaries. (C) 2014 Elsevier B.V. All rights reserved. C1 [Kanevce, Ana; Repins, Ingrid; Wei, Su-Huai] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Kanevce, A (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM Ana.Kanevce@nrel.gov FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory FX This work was supported by the U.S. Department of Energy under Contract no. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. This paper is subject to government rights. NR 54 TC 18 Z9 18 U1 4 U2 35 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0248 EI 1879-3398 J9 SOL ENERG MAT SOL C JI Sol. Energy Mater. Sol. Cells PD FEB PY 2015 VL 133 BP 119 EP 125 DI 10.1016/j.solmat.2014.10.042 PG 7 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA AZ1RH UT WOS:000348015100019 ER PT J AU Sharma, V Erdemir, A Aswath, PB AF Sharma, Vibhu Erdemir, Ali Aswath, Pranesh B. TI An analytical study Of tribofilms generated by the interaction of ashless antiwear additives with ZDDP using XANES and nano-indentation SO TRIBOLOGY INTERNATIONAL LA English DT Article DE Wear; Ashless antiwear additives; XANES; Nanoindentation ID RAY-ABSORPTION-SPECTROSCOPY; THIOPHOSPHATE OIL ADDITIVES; SI L-EDGE; ZINC DIALKYLDITHIOPHOSPHATE; TRIBOLOGICAL PROPERTIES; FLUORINATED ZDDP; LIQUID PARAFFIN; IONIC LIQUIDS; FILMS; MECHANISM AB Mixtures of zinc dialkyl dithiophosphates (ZDDP) and ashless fluorothiophosphates and thiophosphates were examined under tribological conditions. The tribofilms were studied using nano-indentation, electron microscopy and X-ray absorption near edge structure spectroscopy. With the addition of ashless fluorothiophosphates and thiophosphates, there is significant reduction in wear at identical phosphorous levels. Tribofilms formed with mixtures of ZDDP and ashless antiwear additives had stable pad-like structures, while those from ZDDP alone were more heterogeneous. When ZDDP alone is used, S L-edge indicates a preponderance of sulfates at the surface of the tribofilms, while in the presence of a mixture of antiwear additives a mixture of sulfates and sulfides was observed. In all the cases, the phosphates formed were short chain polyphosphates of Zn. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Sharma, Vibhu] Univ Texas Arlington, Arlington, TX 76019 USA. [Erdemir, Ali] Argonne Natl Lab, Argonne, IL 60439 USA. [Aswath, Pranesh B.] Univ Texas Arlington, Coll Engn, Arlington, TX 76019 USA. RP Aswath, PB (reprint author), Univ Texas Arlington, Coll Engn, Arlington, TX 76019 USA. EM Aswath@uta.edu RI Aswath, Pranesh/A-7184-2009 OI Aswath, Pranesh/0000-0003-2885-1918 FU Materials Science and Engineering Department; NSERC; NRC; CIHR; University of Saskatchewan; [DE-AC02-06CH11357] FX Support provided by the Materials Science and Engineering Department and use of the characterization facilities at the Center for Characterization of Materials and Biology at The University of Texas at Arlington is gratefully acknowledged. The XANES experiments were performed at Canadian Light Source, which is supported by NSERC, NRC, CIHR, and the University of Saskatchewan. Tribology experiments were performed at Argonne National Laboratory, which is a U.S. Department of Energy Office of Science laboratory, and operated under Contract No. DE-AC02-06CH11357. NR 60 TC 8 Z9 9 U1 3 U2 17 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0301-679X EI 1879-2464 J9 TRIBOL INT JI Tribol. Int. PD FEB PY 2015 VL 82 BP 43 EP 57 DI 10.1016/j.triboint.2014.09.019 PN A PG 15 WC Engineering, Mechanical SC Engineering GA AY7QC UT WOS:000347753200005 ER PT J AU Werth, D Chen, KF AF Werth, David Chen, Kuo-Fu TI The Application of a Statistical Downscaling Process to Derive 21st Century River Flow Predictions Using a Global Climate Simulation SO WATER RESOURCES MANAGEMENT LA English DT Article DE Climate downscaling; Hydrology; Climate modeling; Climate change; Watershed modeling ID LOCAL CLIMATE; MODELS; CALIFORNIA AB The ability of water managers to maintain adequate supplies in coming decades depends, in part, on future weather conditions, as climate change has the potential to alter river flows from their current values, possibly rendering them unable to meet demand. Reliable climate projections are therefore critical to predicting the future water supply for the United States, but the resolution of the global climate models (GCMs) often used for climate forecasting is too coarse to resolve the changes that can affect hydrology, and hence water supply, at regional to local scales. We therefore apply a statistical downscaling technique that involves a correction of the cumulative distribution functions of the GCM-derived temperature and precipitation for the 20th century, and the application of the same correction to 21st century GCM projections. This is done for three meteorological stations located within the Coosa River basin in northern Georgia, and is used with a surface hydrology model to calculate future river flow statistics for the upper Coosa River. Results are compared to historical Coosa River flow and to flows calculated with the original, unscaled GCM results to determine the impact of potential changes in meteorology on future flows. C1 [Werth, David; Chen, Kuo-Fu] Savannah River Natl Lab, Aiken, SC 29808 USA. RP Werth, D (reprint author), Savannah River Natl Lab, Bldg 773-A, Aiken, SC 29808 USA. EM david.werth@srnl.doe.gov FU Savannah River National Laboratory's Laboratory Directed Research and Development (LDRD) Strategic Initiative program FX "We acknowledge the support of the Savannah River National Laboratory's Laboratory Directed Research and Development (LDRD) Strategic Initiative program, which provided funding for this research." NR 41 TC 0 Z9 0 U1 2 U2 19 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0920-4741 EI 1573-1650 J9 WATER RESOUR MANAG JI Water Resour. Manag. PD FEB PY 2015 VL 29 IS 3 BP 849 EP 861 DI 10.1007/s11269-014-0847-0 PG 13 WC Engineering, Civil; Water Resources SC Engineering; Water Resources GA AY8AN UT WOS:000347776900012 ER PT J AU Jacobs, AC Fair, JM Zuk, M AF Jacobs, Anne C. Fair, Jeanne M. Zuk, Marlene TI Coloration, Paternity, and Assortative Mating in Western Bluebirds SO ETHOLOGY LA English DT Article DE extra-pair paternity; mate choice; Sialia mexicana; structural coloration; melanin ID STRUCTURAL PLUMAGE COLORATION; MALE EASTERN BLUEBIRDS; EXTRA-PAIR PATERNITY; SEXUAL SELECTION; SIALIA-SIALIS; MOUNTAIN BLUEBIRD; PARENTAL EFFORT; FEMALE CHOICE; EVOLUTION; SUCCESS AB Coloration in birds can act as an important sexual signal in males, yet in many species, both sexes display bright colors. Social selection may account for this pattern, with more brightly colored individuals pairing together on the best territories. Mutual mate choice may also explain this, as males investing a great deal of parental care in the offspring should be choosy about their social mates. It is less clear whether this pattern of mate choice can apply to extra-pair partners as well. We examined western bluebirds (Sialia mexicana) to determine whether more colorful individuals tended to pair with one another, both in social pairs and between females and their extra-pair partners. Both male and female western bluebirds display both UV-blue structural plumage and a melanin-based chestnut breast patch, although females are duller than males. Social pairs mated assortatively with regard to UV-blue brightness, but not chestnut coloration. There was no evidence that extra-pair partners mated assortatively, but males with brighter UV-blue coloration had fewer extra-pair offspring in their nests. Older males were more successful at siring extra-pair offspring, despite displaying no differences in coloration compared to younger males. Coloration did not play a role in determining extra-pair male success. These results suggest that coloration plays a role in the formation of social pairs, but not mate choice for extra-pair partners. C1 [Jacobs, Anne C.] Univ Calif Riverside, Dept Biol, Riverside, CA 92521 USA. [Fair, Jeanne M.] Los Alamos Natl Lab, Los Alamos, NM USA. [Zuk, Marlene] Univ Minnesota, Dept Ecol Evolut & Behav, St Paul, MN 55108 USA. RP Jacobs, AC (reprint author), Allegheny Coll, Dept Biol, Meadville, PA 16335 USA. EM ajacobs@allegheny.edu FU Los Alamos National Laboratory [DE-AC52-06NA25396]; US Department of Energy; University of California, Riverside; Sigma Xi Grant-in-Aid of Research; Schreiber Award from the Los Angeles Audubon Society; Doctoral Dissertation Improvement Grant from the National Science Foundation [IOS-1210532] FX We thank K. Burnett, C. Hathcock, D. Keller, C. Lemanski, L. Maestas, L. Reader, and R. Robinson for their assistance in the field, B. Faircloth, L. Enders, and L. Nunney for help with the molecular methods, and three anonymous reviewers for their suggestions on the manuscript. We would also like to thank the Los Alamos Fire Department and all the firefighters who battled the Las Conchas blaze in 2011 and saved our field sites and our laboratory space from the flames. This work was supported by the Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396 with the US Department of Energy, the University of California, Riverside, a Sigma Xi Grant-in-Aid of Research, a Schreiber Award from the Los Angeles Audubon Society awarded to ACJ, and a Doctoral Dissertation Improvement Grant from the National Science Foundation (Grant # IOS-1210532). NR 56 TC 1 Z9 1 U1 11 U2 73 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0179-1613 EI 1439-0310 J9 ETHOLOGY JI Ethology PD FEB PY 2015 VL 121 IS 2 BP 176 EP 186 DI 10.1111/eth.12327 PG 11 WC Psychology, Biological; Behavioral Sciences; Zoology SC Psychology; Behavioral Sciences; Zoology GA AY4KE UT WOS:000347545900008 ER PT J AU Stickle, AM Schultz, PH Crawford, DA AF Stickle, A. M. Schultz, P. H. Crawford, D. A. TI Subsurface failure in spherical bodies: A formation scenario for linear troughs on Vesta's surface SO ICARUS LA English DT Article DE Asteroid Vesta; Impact processes; Cratering ID ASTEROID 4 VESTA; COLLISIONAL EVOLUTION; IMPACT FRAGMENTATION; DAWN MISSION; PARENT BODY; DISRUPTION; FRACTURE; GRAVITY; CORE; HOWARDITE AB Many asteroids in the Solar System exhibit unusual, linear features on their surface. The Dawn mission recently observed two sets of linear features on the surface of the asteroid 4 Vesta. Geologic observations indicate that these features are related to the two large impact basins at the south pole of Vesta, though no specific mechanism of origin has been determined. Further, the orientation of the features is offset from the center of the basins. Experimental and numerical results reveal that the offset angle is a natural consequence of oblique impacts into a spherical target. Here we demonstrate that a set of shear planes develops in the subsurface of the body opposite to the point of first contact. These subsurface failure zones then propagate to the surface under combined tensile-shear stress fields after the impact to create sets of approximately linear faults on the surface. Comparison between the orientation of damage structures in the laboratory and failure regions within Vesta can be used to constrain impact parameters (e.g., the approximate impact point and likely impact trajectory). (C) 2014 Elsevier Inc. All rights reserved. C1 [Stickle, A. M.; Schultz, P. H.] Brown Univ, Dept Earth Environm & Planetary Sci, Providence, RI 02912 USA. [Crawford, D. A.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Stickle, AM (reprint author), Johns Hopkins Univ, Appl Phys Lab, Johns Hopkins Rd, Laurel, MD 20723 USA. EM angela_stickle@alumni.brown.edu RI Stickle, Angela/F-4568-2015 OI Stickle, Angela/0000-0002-7602-9120 FU NASA Planetary Geology and Geophysics program [NNX 08AM45G]; United States Department of Energy [DE-AC04-94AL85000] FX AMS was funded by the NASA Planetary Geology and Geophysics program, Grant NNX 08AM45G, for this research. AMS thanks Amy Barr, Karen Fischer, Greg Hirth, and John Spray for helpful reviews that strengthened the manuscript. D.A. Crawford acknowledges that Sandia is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy under Contract DE-AC04-94AL85000. The authors would also like to thank two anonymous reviewers for their comments to help finalize this manuscript. NR 89 TC 1 Z9 1 U1 2 U2 3 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0019-1035 EI 1090-2643 J9 ICARUS JI Icarus PD FEB PY 2015 VL 247 BP 18 EP 34 DI 10.1016/j.icarus.2014.10.002 PG 17 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AX1ER UT WOS:000346691400002 ER PT J AU Cullinan, T Kalay, I Kalay, YE Kramer, M Napolitano, R AF Cullinan, Tim Kalay, Ilkay Kalay, Y. Eren Kramer, Matt Napolitano, Ralph TI Kinetics and Mechanisms of Isothermal Devitrification in Amorphous Cu50Zr50 SO METALLURGICAL AND MATERIALS TRANSACTIONS A-PHYSICAL METALLURGY AND MATERIALS SCIENCE LA English DT Article ID CU-ZR; METALLIC GLASSES; THERMAL-STABILITY; INTERMETALLIC PHASE; COPPER-ZIRCONIUM; ALLOY SYSTEM; CRYSTALLIZATION; BEHAVIOR; AT.PERCENT; CU70ZR30 AB The crystallization kinetics and microstructural dynamics associated with devitrifying a melt-spun Cu50Zr50 metallic glass were investigated using isothermal treatments, in situ high-energy synchrotron X-ray diffraction, conventional and high-resolution transmission electron microscopy, and differential scanning calorimetry. The analysis of isothermal transformations allows us to more clearly unravel the complex interplay between nucleation and growth of competing stable and metastable phases. The isothermal devitrification response was found to involve the Cu10Zr7, CuZr2, and CuZr phases, consistent with previously reported constant heating rate experiments, but here we have resolved the phase evolution and structural characteristics of the transformation, including the very early stages of crystallization. At 671 K (398 A degrees C), the isothermal transformation starts with the formation of the Cu10Zr7 phase, which grows in a generally equiaxed morphology. At a size of approximately 100 nm, the growth of the Cu10Zr7 particles is interrupted by the precipitation of a thin layer of the CuZr2 phase, upon which the metastable CuZr (B2) grows epitaxially. Crystallization kinetics are quantified here though in situ measurements (HEXRD, DSC) and ex situ microstructural analysis (TEM, HRTEM). Finally, the influences of chemical partitioning, diffusion, and crystallographic orientation on this sequence are examined. C1 [Cullinan, Tim; Kramer, Matt; Napolitano, Ralph] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Cullinan, Tim; Kramer, Matt; Napolitano, Ralph] US DOE, Ames Lab, Ames, IA 50011 USA. [Kalay, Ilkay] Cankaya Univ, Dept Mat Sci & Engn, TR-06810 Ankara, Turkey. [Kalay, Y. Eren] Middle E Tech Univ, Dept Met & Mat Engn, TR-06790 Ankara, Turkey. RP Napolitano, R (reprint author), Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. EM ren1@iastate.edu FU U.S. Department of Energy, Office of Basic Energy Science, the Division of Materials Sciences and Engineering; U.S. Department of Energy [DE-AC02-07CH11358]; Advanced Photon Source, Argonne National Laboratory [DE-AC02-06CH11357] FX This study was supported by the U.S. Department of Energy, Office of Basic Energy Science, the Division of Materials Sciences and Engineering. The research was performed at the Ames Laboratory. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. Synchrotron experiments were performed at the Advanced Photon Source, Argonne National Laboratory, under Grant No. DE-AC02-06CH11357. The authors thank Will Landau (Department of Statistics, Iowa State University) for assisting with the development of the "direct" JMAK fitting procedure. NR 39 TC 2 Z9 2 U1 2 U2 28 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1073-5623 EI 1543-1940 J9 METALL MATER TRANS A JI Metall. Mater. Trans. A-Phys. Metall. Mater. Sci. PD FEB PY 2015 VL 46A IS 2 BP 600 EP 613 DI 10.1007/s11661-014-2661-y PG 14 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AY0RD UT WOS:000347303400007 ER PT J AU Elliott, DC Biller, P Ross, AB Schmidt, AJ Jones, SB AF Elliott, Douglas C. Biller, Patrick Ross, Andrew B. Schmidt, Andrew J. Jones, Susanne B. TI Hydrothermal liquefaction of biomass: Developments from batch to continuous process SO BIORESOURCE TECHNOLOGY LA English DT Review DE Hydrothermal; Liquefaction; Biomass; Algae; Lignocellulosic ID MICROALGAE CULTIVATION; SUPERCRITICAL WATER; NANNOCHLOROPSIS SP; ALGAE FEEDSTOCKS; HIGH-TEMPERATURE; WOODY BIOMASS; BIO-OIL; GASIFICATION; CONVERSION; TECHNOLOGIES AB This review describes the recent results in hydrothermal liquefaction (HTL) of biomass in continuous-flow processing systems. Although much has been published about batch reactor tests of biomass HTL, there is only limited information yet available on continuous-flow tests, which can provide a more reasonable basis for process design and scale-up for commercialization. High-moisture biomass feedstocks are the most likely to be used in HTL. These materials are described and results of their processing are discussed. Engineered systems for HTL are described; however, they are of limited size and do not yet approach a demonstration scale of operation. With the results available, process models have been developed, and mass and energy balances determined. From these models, process costs have been calculated and provide some optimism as to the commercial likelihood of the technology. (C) 2014 The Authors. Published by Elsevier Ltd. This is an open access article under the CC BY license C1 [Elliott, Douglas C.; Schmidt, Andrew J.; Jones, Susanne B.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Biller, Patrick; Ross, Andrew B.] Univ Leeds, Energy Res Inst, Leeds LS2 9JT, W Yorkshire, England. RP Elliott, DC (reprint author), Pacific NW Natl Lab, POB 999, Richland, WA 99352 USA. FU U.S. Department of Energy [DE-AC05-76RL01830]; Department of Energy Bioenergy Technologies Office; EPSRC [EP/I014365/1, EP/L504993/1] FX The manuscript preparation work at PNNL was supported by the U.S. Department of Energy under Contract No. DE-AC05-76RL01830 at the Pacific Northwest National Laboratory. The PNNL authors gratefully acknowledge the support of the Department of Energy Bioenergy Technologies Office. The researchers at the University of Leeds would like to thank the EPSRC for financial support (EP/I014365/1, EP/L504993/1) for the manuscript preparation work. NR 58 TC 82 Z9 83 U1 27 U2 211 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0960-8524 EI 1873-2976 J9 BIORESOURCE TECHNOL JI Bioresour. Technol. PD FEB PY 2015 VL 178 BP 147 EP 156 DI 10.1016/j.biortech.2014.09.132 PG 10 WC Agricultural Engineering; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA AX8HM UT WOS:000347150700019 PM 25451780 ER PT J AU Eremenko, V Upadhyay, NJ Thompson, IJ Elster, C Nunes, FM Arbanas, G Escher, JE Hlophe, L AF Eremenko, V. Upadhyay, N. J. Thompson, I. J. Elster, Ch. Nunes, F. M. Arbanas, G. Escher, J. E. Hlophe, L. CA TORUS Collaboration TI Coulomb wave functions in momentum space SO COMPUTER PHYSICS COMMUNICATIONS LA English DT Article DE Momentum-space partial-wave Coulomb functions ID COMPLEX AB An algorithm to calculate non-relativistic partial-wave Coulomb functions in momentum space is presented. The arguments are the Sommerfeld parameter eta, the angular momentum l, the asymptotic momentum q and the 'running' momentum p, where both momenta are real. Since the partial-wave Coulomb functions exhibit singular behavior when p -> q, different representations of the Legendre functions of the 2nd kind need to be implemented in computing the functions for the values of p close to the singularity and far away from it. The code for the momentum-space Coulomb wave functions is applicable for values of vertical bar eta vertical bar in the range of 10(-1) to 10, and thus is particularly suited for momentum space calculations of nuclear reactions. Program Summary Program title: libcwfn Catalogue identifier: AEUQ_v1_0 Program summary URL: http://cpc.cs.qub.ac.uk/summaries/AEUQ_v1_0.html Program obtainable from: CPC Program Library, Queen's University, Belfast, N. Ireland Licensing provisions: Standard CPC licence, http://cpc.cs.qub.ac.uk/licence/licence.html No. of lines in distributed program, including test data, etc.: 864503 No. of bytes in distributed program, including test data, etc.: 7178021 Distribution format: tar.gz Programming language: Fortran 90, Fortran 77, Python, make (GNU Make dialect), GNU Bash shell interpreter (available as /bin/bash). Computer: Apple Powermac (Intel Xeon), ASUS K53U (AMD E-350 (Dual Core)), DELL Precision T3500 (Intel Xeon), NERSC Carver (Intel Nehalem Quad Core). Operating system: Linux, Windows (using Cygwin). RAM: less than 512 Mbytes Classification: 17.8, 17.13, 17.16. Nature of problem: The calculation of partial wave Coulomb functions with integer land all other arguments real. Solution method: Computing the value of the function using explicit formulae and algorithms. Running time: Less than 10(-3) s. (C) 2014 Elsevier B.V. All rights reserved. C1 [Eremenko, V.; Elster, Ch.; Hlophe, L.] Ohio Univ, Inst Nucl & Particle Phys, Athens, OH 45701 USA. [Eremenko, V.; Elster, Ch.; Hlophe, L.] Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. [Upadhyay, N. J.; Nunes, F. M.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Upadhyay, N. J.; Nunes, F. M.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Thompson, I. J.; Escher, J. E.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Arbanas, G.] Oak Ridge Natl Lab, Reactor & Nucl Syst Div, Oak Ridge, TN 37831 USA. [Eremenko, V.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow 119991, Russia. RP Eremenko, V (reprint author), Ohio Univ, Inst Nucl & Particle Phys, Athens, OH 45701 USA. EM eremenko@ohio.edu; njupadhyay@gmail.com; elster@ohio.edu RI Elster, Charlotte/N-9845-2015 FU US Department of Energy, Office of Science of Nuclear Physics [DE-SC0004084, DE-SC0004087, DE-FG02-93ER40756]; Ohio University [DE-FG52-08NA28552]; Michigan State University; Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; U.T. Battelle LLC [DE-AC-0500OR22725]; National Science Foundation [PHY-080026]; Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX The TORUS Collaboration acknowledges the insight of Prof. Akram Mukhamedzhanov in respect to this project. Eremenko and Upadhyay are grateful to Prof. Akram Mukhamedzhanov and Dr. Ahdior Sattarov for providing invaluable guidance in the early stages of this work. The authors are also grateful to Prof. Jeff Tostevin for many useful discussions. This material is based on work in part supported by the US Department of Energy, Office of Science of Nuclear Physics under contracts DE-SC0004084 and DE-SC0004087 (TORUS Collaboration), DE-FG02-93ER40756 with Ohio University, contract DE-FG52-08NA28552 with Michigan State University, and by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344, and the U.T. Battelle LLC Contract DE-AC-0500OR22725. F.M. Nunes also acknowledges support from the National Science Foundation under grant PHY-080026. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 19 TC 2 Z9 2 U1 2 U2 19 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0010-4655 EI 1879-2944 J9 COMPUT PHYS COMMUN JI Comput. Phys. Commun. PD FEB PY 2015 VL 187 BP 195 EP 203 DI 10.1016/j.cpc.2014.10.002 PG 9 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AX5GH UT WOS:000346954200021 ER PT J AU Efroymson, RA Dale, VH AF Efroymson, Rebecca A. Dale, Virginia H. TI Environmental indicators for sustainable production of algal biofuels SO ECOLOGICAL INDICATORS LA English DT Article DE Algae; Bioenergy; Biofuel; Biodiversity; Greenhouse gas emissions; Indicator; Productivity; Sustainability; Water ID LIFE-CYCLE ENERGY; BLUE-GREEN-ALGAE; FRESH-WATER; BIODIESEL PRODUCTION; BIOMASS PRODUCTION; ETHANOL-PRODUCTION; ORGANIC-COMPOUNDS; UNITED-STATES; AIR-QUALITY; TRADE-OFFS AB For analyzing sustainability of algal biofuels, we identify 16 environmental indicators that fall into six categories: soil quality, water quality and quantity, air quality, greenhouse gas emissions, biodiversity, and productivity. Indicators are selected to be practical, widely applicable, predictable in response, anticipatory of future changes, independent of scale, and responsive to management. Major differences between algae and terrestrial plant feedstocks, as well as their supply chains for biofuel, are highlighted, for they influence the choice of appropriate sustainability indicators. Algae strain selection characteristics do not generally affect which indicators are selected. The use of water instead of soil as the growth medium for algae determines the higher priority of water- over soil-related indicators. The proposed set of environmental indicators provides an initial checklist for measures of algal biofuel sustainability but may need to be modified for particular contexts depending on data availability, goals of stakeholders, and financial constraints. Use of these indicators entails defining sustainability goals and targets in relation to stakeholder values in a particular context and can lead to improved management practices. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Efroymson, Rebecca A.; Dale, Virginia H.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Efroymson, RA (reprint author), Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. EM efroymsonra@ornl.gov; dalevh@ornl.gov OI Efroymson, Rebecca/0000-0002-3190-880X FU DOE [DE-AC05-00OR22725]; U.S. Department of Energy (DOE) under the Bioenergy Technologies Office (BETO) FX Tanya Kuritz, Esther Parish, and Kristen Johnson provided helpful reviews of earlier drafts. We thank Matt Langholtz, Jeri Sullivan, Kitt Bagwell, Tanya Kuritz, Gary Saylor, Ed Frank, and Mark Wignosta for useful discussions. We thank Kristen Johnson and Dan Fishman of DOE for insights and project sponsorship. This research was supported by the U.S. Department of Energy (DOE) under the Bioenergy Technologies Office (BETO). Oak Ridge National Laboratory is managed by UT-Battelle, LLC, for DOE under contract DE-AC05-00OR22725. NR 110 TC 7 Z9 7 U1 2 U2 105 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1470-160X EI 1872-7034 J9 ECOL INDIC JI Ecol. Indic. PD FEB PY 2015 VL 49 BP 1 EP 13 DI 10.1016/j.ecolind.2014.09.028 PG 13 WC Biodiversity Conservation; Environmental Sciences SC Biodiversity & Conservation; Environmental Sciences & Ecology GA AX5GK UT WOS:000346954500001 ER PT J AU Pryor, KH AF Pryor, Kathryn H. TI RADIATION SAFETY OF SEALED RADIOACTIVE SOURCES SO HEALTH PHYSICS LA English DT Article DE National Council on Radiation Protection and Measurements; exposure, radiation; radioactive materials; occupational safety AB Sealed radioactive sources are used in a wide variety of occupational settings and under differing regulatory/licensing structures. The definition of a sealed radioactive source varies between U.S. regulatory authorities and standard-setting organizations. Potential problems with sealed sources cover a range of risks and impacts. The loss of control of high activity sealed sources can result in very high or even fatal doses to members of the public who come in contact with them. Sources that are not adequately sealed and that fail can cause spread of contamination and potential intake of radioactive material. There is also the possibility that sealed sources may be (or threaten to be) used for terrorist purposes and disruptive opportunities. Until fairly recently, generally licensed sealed sources and devices received little, if any, regulatory oversight and were often forgotten, lost or unaccounted for. Nonetheless, generally licensed devices can contain fairly significant quantities of radioactive material, and there is some potential for exposure if a device is treated in a way for which it was never designed. Industrial radiographers use and handle high activity and/or high dose-rate sealed sources in the field with a high degree of independence and minimal regulatory oversight. Failure to follow operational procedures and properly handle radiography sources can and has resulted in serious injuries and death. Industrial radiographers have experienced a disproportionately large fraction of incidents that have resulted in unintended exposure to radiation. Sources do not have to contain significant quantities of radioactive material to cause problems in the event of their failure. A loss of integrity can cause the spread of contamination and potential exposure to workers and members of the public. The National Council on Radiation Protection and Measurements has previously provided recommendations on select aspects of sealed source programs. Future efforts to provide recommendations for sealed source programs are discussed. C1 Pacific NW Natl Lab, Radiat Protect Div, Richland, WA 99352 USA. RP Pryor, KH (reprint author), Pacific NW Natl Lab, Radiat Protect Div, POB 999,MSIN J2-40,902 Battelle Blvd, Richland, WA 99352 USA. EM kathy.pryor@pnnl.gov NR 10 TC 1 Z9 1 U1 1 U2 6 PU LIPPINCOTT WILLIAMS & WILKINS PI PHILADELPHIA PA TWO COMMERCE SQ, 2001 MARKET ST, PHILADELPHIA, PA 19103 USA SN 0017-9078 EI 1538-5159 J9 HEALTH PHYS JI Health Phys. PD FEB PY 2015 VL 108 IS 2 BP 172 EP 177 DI 10.1097/HP.0000000000000225 PG 6 WC Environmental Sciences; Public, Environmental & Occupational Health; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging SC Environmental Sciences & Ecology; Public, Environmental & Occupational Health; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging GA AX6YN UT WOS:000347064100014 PM 25551499 ER PT J AU Hoover, MD Myers, DS Cash, LJ Guilmette, RA Kreyling, WG Oberdorster, G Smith, R Cassata, JR Boecker, BB Grissom, MP AF Hoover, Mark D. Myers, David S. Cash, Leigh J. Guilmette, Raymond A. Kreyling, Wolfgang G. Oberdoerster, Guenter Smith, Rachel Cassata, James R. Boecker, Bruce B. Grissom, Michael P. TI APPLICATION OF AN INFORMATICS-BASED DECISION-MAKING FRAMEWORK AND PROCESS TO THE ASSESSMENT OF RADIATION SAFETY IN NANOTECHNOLOGY SO HEALTH PHYSICS LA English DT Article DE National Council on Radiation Protection and Measurements; occupational safety; radiation protection; risk analysis ID FILTERING FACEPIECE RESPIRATORS; FILTRATION PERFORMANCE; GOLD NANOPARTICLES; RAT; DIOXIDE; SIZE AB The National Council on Radiation Protection and Measurements (NCRP) established NCRP Scientific Committee 2-6 to develop a report on the current state of knowledge and guidance for radiation safety programs involved with nanotechnology. Nanotechnology is the understanding and control of matter at the nanoscale, at dimensions between similar to 1 and 100 nm, where unique phenomena enable novel applications. While the full report is in preparation, this paper presents and applies an informatics-based decision-making framework and process through which the radiation protection community can anticipate that nano-enabled applications, processes, nanomaterials, and nanoparticles are likely to become present or are already present in radiation-related activities; recognize specific situations where environmental and worker safety, health, well-being, and productivity may be affected by nano-related activities; evaluate how radiation protection practices may need to be altered to improve protection; control information, interpretations, assumptions, and conclusions to implement scientifically sound decisions and actions; and confirm that desired protection outcomes have been achieved. This generally applicable framework and supporting process can be continuously applied to achieve health and safety at the convergence of nanotechnology and radiation-related activities. C1 [Hoover, Mark D.] NIOSH, Morgantown, WV 26505 USA. [Cash, Leigh J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Guilmette, Raymond A.] Ray Guilmette & Associates LLC, Perry, ME 04667 USA. [Guilmette, Raymond A.; Boecker, Bruce B.] Lovelace Resp Res Inst, Albuquerque, NM 87108 USA. [Kreyling, Wolfgang G.] Helmholtz Zentrum Munchen, D-85764 Neuherberg, Germany. [Oberdoerster, Guenter] Univ Rochester, Dept Environm Med, Rochester, NY 14627 USA. [Smith, Rachel] Publ Hlth England, Ctr Radiat Chem & Environm Hazards, Chilton OX11 0RQ, Oxon, England. [Cassata, James R.] Natl Council Radiat Protect & Measurements, Bethesda, MD 20814 USA. [Grissom, Michael P.] MPG HP Inc, Riverside, CA 92508 USA. RP Hoover, MD (reprint author), NIOSH, 1095 Willowdale Rd, Morgantown, WV 26505 USA. EM mhoover1@cdc.gov OI Kreyling, Wolfgang/0000-0002-0702-6567 FU NCRP FX The authors gratefully acknowledge John Boice and NCRP for creating and supporting Scientific Committee 2-6. Appreciation is also expressed to Stephanie Mathews, Ilise Feitshans, John Iskander, and Stacey Harper for their valuable coauthor contributions on the Encyclopedia of Toxicology chapter on communications concepts and their useful discussions and input on application of the communications concepts to broader applications such as the emerging confluence of nanotechnology and radiation safety. The findings and conclusions in this presentation are those of the authors and do not necessarily represent the views of their respective organizations. This presentation has been assigned document number LA-UR-14-28101. The authors gratefully acknowledge the support of their respective organizations. NR 44 TC 5 Z9 6 U1 0 U2 12 PU LIPPINCOTT WILLIAMS & WILKINS PI PHILADELPHIA PA TWO COMMERCE SQ, 2001 MARKET ST, PHILADELPHIA, PA 19103 USA SN 0017-9078 EI 1538-5159 J9 HEALTH PHYS JI Health Phys. PD FEB PY 2015 VL 108 IS 2 BP 179 EP 194 DI 10.1097/HP.0000000000000250 PG 16 WC Environmental Sciences; Public, Environmental & Occupational Health; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging SC Environmental Sciences & Ecology; Public, Environmental & Occupational Health; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging GA AX6YN UT WOS:000347064100016 PM 25551501 ER PT J AU Bouville, A Toohey, RE Boice, JD Beck, HL Dauer, LT Eckerman, KF Hagemeyer, D Leggett, RW Mumma, MT Napier, B Pryor, KH Rosenstein, M Schauer, DA Sherbini, S Stram, DO Thompson, JL Till, JE Yoder, C Zeitlin, C AF Bouville, Andre Toohey, Richard E. Boice, John D., Jr. Beck, Harold L. Dauer, Larry T. Eckerman, Keith F. Hagemeyer, Derek Leggett, Richard W. Mumma, Michael T. Napier, Bruce Pryor, Kathy H. Rosenstein, Marvin Schauer, David A. Sherbini, Sami Stram, Daniel O. Thompson, James L. Till, John E. Yoder, Craig Zeitlin, Cary TI DOSE RECONSTRUCTION FOR THE MILLION WORKER STUDY: STATUS AND GUIDELINES SO HEALTH PHYSICS LA English DT Article DE National Council on Radiation Protection and Measurements; dose assessment; exposure, occupational; radiation risk ID FILM DOSIMETER RESPONSE; US RADIOLOGIC TECHNOLOGISTS; RADIATION WORKERS; MILITARY PARTICIPANTS; MORTALITY; COHORT; UNCERTAINTY; PLUTONIUM; METHODOLOGY; EXPOSURES AB The primary aim of the epidemiologic study of one million U.S. radiation workers and veterans [the Million Worker Study (MWS)] is to provide scientifically valid information on the level of radiation risk when exposures are received gradually over time and not within seconds, as was the case for Japanese atomic bomb survivors. The primary outcome of the epidemiologic study is cancer mortality, but other causes of death such as cardiovascular disease and cerebrovascular disease will be evaluated. The success of the study is tied to the validity of the dose reconstruction approaches to provide realistic estimates of organ-specific radiation absorbed doses that are as accurate and precise as possible and to properly evaluate their accompanying uncertainties. The dosimetry aspects for the MWS are challenging in that they address diverse exposure scenarios for diverse occupational groups being studied over a period of up to 70 y. The dosimetric issues differ among the varied exposed populations that are considered: atomic veterans, U.S. Department of Energy workers exposed to both penetrating radiation and intakes of radionuclides, nuclear power plant workers, medical radiation workers, and industrial radiographers. While a major source of radiation exposure to the study population comes from external gamma-or x-ray sources, for some of the study groups, there is a meaningful component of radionuclide intakes that requires internal radiation dosimetry assessments. Scientific Committee 6-9 has been established by the National Council on Radiation Protection and Measurements (NCRP) to produce a report on the comprehensive organ dose assessment (including uncertainty analysis) for the MWS. The NCRP dosimetry report will cover the specifics of practical dose reconstruction for the ongoing epidemiologic studies with uncertainty analysis discussions and will be a specific application of the guidance provided in NCRP Report Nos. 158, 163, 164, and 171. The main role of the Committee is to provide guidelines to the various groups of dosimetrists involved in the MWS to ensure that certain dosimetry criteria are considered: calculation of annual absorbed doses in the organs of interest, separation of low and high linear-energy transfer components, evaluation of uncertainties, and quality assurance and quality control. It is recognized that the MWS and its approaches to dosimetry are a work in progress and that there will be flexibility and changes in direction as new information is obtained with regard to both dosimetry and the epidemiologic features of the study components. This paper focuses on the description of the various components of the MWS, the available dosimetry results, and the challenges that have been encountered. It is expected that the Committee will complete its report in 2016. C1 [Bouville, Andre] NCI, Rockville, MD 20850 USA. [Toohey, Richard E.] MH Chew & Associates, Oak Ridge, TN USA. [Boice, John D., Jr.; Schauer, David A.] Natl Council Radiat Protect & Measurements, Bethesda, MD USA. [Beck, Harold L.] US DOE, New York, NY USA. [Dauer, Larry T.] Mem Sloan Kettering Canc Ctr, New York, NY 10021 USA. [Eckerman, Keith F.; Leggett, Richard W.] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Hagemeyer, Derek] Oak Ridge Associated Univ, Oak Ridge, TN USA. [Mumma, Michael T.] Int Epidemiol Inst, Rockville, MD USA. [Napier, Bruce; Pryor, Kathy H.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Sherbini, Sami] US Nucl Regulatory Commiss, Washington, DC 20555 USA. [Stram, Daniel O.] Univ So Calif, Los Angeles, CA USA. [Thompson, James L.] US Nucl Regulatory Commiss, Arlington, TX USA. [Till, John E.] Risk Assessment Corp, Neeses, SC USA. [Yoder, Craig] Landauer Inc, Glenwood, IL USA. [Zeitlin, Cary] SW Res Inst, Boulder, CO USA. RP Bouville, A (reprint author), NCI, 9609 Med Ctr Dr,Room 7E590,MSC 9778, Rockville, MD 20850 USA. EM andre.bouville@nih.gov OI Dauer, Lawrence/0000-0002-5629-8462 FU U.S. Department of Energy [DE-SC0008944]; U.S. Nuclear Regulatory Commission; U.S. Environmental Protection Agency; National Aeronautics and Space Administration; National Cancer Institute [U01 CA137026]; Vanderbilt-Ingram Cancer Center [404-357-9682] FX This research was supported in part by contracts and grants from the U.S. Department of Energy (Grant No. DE-SC0008944 awarded to NCRP), which included interagency support from the U.S. Nuclear Regulatory Commission, the U.S. Environmental Protection Agency and the National Aeronautics and Space Administration; the National Cancer Institute (Grant No. U01 CA137026); and a Discovery Grant from the Vanderbilt-Ingram Cancer Center (Center no. 404-357-9682). We also acknowledge Paul Blake, Director, Chief, Nuclear Test Personnel Review, Defense Threat Reduction Agency, Department of Defense and his staff for their technical support of the atomic veterans project. Similarly, Han Kang and Tim Bullman, Environmental Epidemiology Service, U.S. Department of Veterans Affairs, were instrumental in providing support and assistance throughout the conduct of the atomic veteran study. NR 56 TC 13 Z9 13 U1 2 U2 13 PU LIPPINCOTT WILLIAMS & WILKINS PI PHILADELPHIA PA TWO COMMERCE SQ, 2001 MARKET ST, PHILADELPHIA, PA 19103 USA SN 0017-9078 EI 1538-5159 J9 HEALTH PHYS JI Health Phys. PD FEB PY 2015 VL 108 IS 2 BP 206 EP 220 DI 10.1097/HP.0000000000000231 PG 15 WC Environmental Sciences; Public, Environmental & Occupational Health; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging SC Environmental Sciences & Ecology; Public, Environmental & Occupational Health; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging GA AX6YN UT WOS:000347064100019 PM 25551504 ER PT J AU Kim, SJ Zou, L Jones, BG AF Kim, Seung Jun Zou, Ling Jones, Barclay G. TI An experimental study on sub-cooled flow boiling CHF of R134a at low pressure condition with atmospheric pressure (AP) plasma assisted surface modification SO INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER LA English DT Article DE Sub-cooled flow boiling; CHF; Surface wettability; Surface modification ID CRITICAL HEAT-FLUX; POLYMER SURFACES; BURNOUT; ENHANCEMENT; NANOFLUIDS; WATER; POOL AB In this study, sub-cooled flow boiling critical heat flux tests at low pressure were conducted in a rectangular flow channel with one uniformly heated surface, using simulant fluid R-134a as coolant. The experiments were conducted under the following conditions: (1) inlet pressure (P) of 400-800 kPa, (2) mass flux (G) of 124-248 kg/m(2) s, (3) inlet sub-cooling enthalpy (Delta H-i) of 12-26 kJ/ kg. Parametric trends of macroscopic system parameters (G,P,Delta H-i) were examined by changing inlet conditions. Those trends were found to be generally consistent with previous understandings of CHF behavior at low pressure condition (i.e. reduced pressure less than 0.2). A fluid-to-fluid scaling model was utilized to convert the test data obtained with the simulant fluid (R-134a) into the prototypical fluid (water). The comparison between the converted CHF of equivalent water and CHF look-up table with same operation conditions were conducted, which showed good agreement. Furthermore, the effect of surface wettability on CHF was also investigated by applying atmospheric pressure plasma (AP-plasma) treatment to modify the surface characteristic. With AP-plasma treatment, the change of microscopic surface characteristic was measured in terms of static contact angle. The static contact angle was reduced from 80 degrees on original non-treated surface to 15 degrees on treated surface. An enhancement of 18% on CHF values under flow boiling conditions were observed on AP-plasma treated surfaces compared to those on non-treated heating surfaces. Published by Elsevier Ltd. C1 [Kim, Seung Jun] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Zou, Ling] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Jones, Barclay G.] Univ Illinois, Dept Nucl Plasma & Radiol Engn, Urbana, IL 61801 USA. RP Kim, SJ (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM skim@lanl.gov RI Zou, Ling/D-7577-2016; OI Zou, Ling/0000-0003-0664-0474; Kim, Seung Jun/0000-0002-6913-6358 NR 31 TC 0 Z9 0 U1 1 U2 9 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0017-9310 EI 1879-2189 J9 INT J HEAT MASS TRAN JI Int. J. Heat Mass Transf. PD FEB PY 2015 VL 81 BP 362 EP 372 DI 10.1016/j.ijheatmasstransfer.2014.10.032 PG 11 WC Thermodynamics; Engineering, Mechanical; Mechanics SC Thermodynamics; Engineering; Mechanics GA AX5FE UT WOS:000346951400039 ER PT J AU Konomi, B Karagiannis, G Lin, G AF Konomi, Bledar Karagiannis, Georgios Lin, Guang TI On the Bayesian treed multivariate Gaussian process with linear model of coregionalization SO JOURNAL OF STATISTICAL PLANNING AND INFERENCE LA English DT Article DE Multivariate Gaussian process; Linear model of coregionalization; Bayesian treed Gaussian process; Markov chain Monte Carlo ID ADAPTIVE DESIGN; UNCERTAINTY; INFERENCE AB The Bayesian treed multivariate Gaussian process (BTMGP) and Bayesian treed Gaussian process (BTGP) provide straightforward mechanisms for emulating non-stationary multivariate computer codes that alleviate computational demands by fitting models locally. Here, we show that the existing BTMGP performs acceptably when the output variables are dependent but unsatisfactory when they are independent while the BTGP performs contrariwise. We develop the BTMGP with linear model of coregionalization (LMC) cross-covariance, an extension of the BTMGP, that gives satisfactory fitting compared to the other two emulators regardless of whether the output variables are locally dependent. The proposed BTMGP is able to locally model more complex and realistic cross-covariance functions. The conditional representation of LMC in combination with the right choice of the prior distributions allow us to improve the MCMC mixing and invert smaller matrices in the Bayesian inference. We illustrate our empirical results and the performance of the proposed method through artificial examples, and one application to the multiphase flow in a full scale regenerator of a carbon capture unit. (c) 2014 Elsevier B.V. All rights reserved. C1 [Konomi, Bledar; Karagiannis, Georgios; Lin, Guang] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Konomi, B (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM alex.konomi@uc.edu FU Department of Energy Carbon Capture Simulation Initiative; US Department of Energy [DE-AC05-76RL01830] FX The research at Pacific Northwest National Laboratory (PNNL) was supported by the Department of Energy Carbon Capture Simulation Initiative. PNNL is operated by Battelle for the US Department of Energy under Contract DE-AC05-76RL01830. The authors thank Dr. Avik Sarkar and Dr. Xin Sun for helping with the computer simulations in carbon capture regenerator. NR 35 TC 1 Z9 1 U1 1 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-3758 EI 1873-1171 J9 J STAT PLAN INFER JI J. Stat. Plan. Infer. PD FEB-MAR PY 2015 VL 157 BP 1 EP 15 DI 10.1016/j.jspi.2014.08.010 PG 15 WC Statistics & Probability SC Mathematics GA AX8BA UT WOS:000347134200001 ER PT J AU Janish, MT Mook, WM Carter, CB AF Janish, Matthew T. Mook, William M. Carter, C. Barry TI Nucleation of fcc Ta when heating thin films SO SCRIPTA MATERIALIA LA English DT Article DE Focused ion beam (FIB); High-resolution electron microscopy (HREM); Transmission electron microscopy (TEM); Crystal structure; Tantalum ID ULTRAFINE-GRAINED MATERIALS; TANTALUM FILMS; SPECIAL-ISSUE; COATINGS; SYSTEM; BETA AB Thin tantalum films have been studied during in situ heating in a transmission electron microscope. Diffraction patterns from the as-deposited films were typical of amorphous materials. Crystalline grains were observed to form when the specimen was annealed in situ at 450 degrees C. Particular attention was addressed to the formation and growth of grains with the face-centered cubic (fcc) crystal structure. These observations are discussed in relation to prior work on the formation of fcc Ta by deformation and during thin film deposition. (C) 2014 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Janish, Matthew T.; Carter, C. Barry] Univ Connecticut, Dept Mat Sci & Engn, Storrs, CT 06269 USA. [Mook, William M.; Carter, C. Barry] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. [Carter, C. Barry] Univ Connecticut, Dept Chem & Biomol Engn, Storrs, CT 06269 USA. [Carter, C. Barry] Univ Connecticut, Inst Mat Sci, Storrs, CT 06269 USA. RP Janish, MT (reprint author), Univ Connecticut, Dept Mat Sci & Engn, 97 North Eagleville Rd, Storrs, CT 06269 USA. RI Janish, Matthew/M-8625-2016; OI Carter, C Barry/0000-0003-4251-9102 FU Department of Education; US Department of Energy [DEAC04-94AL85000] FX M.T.J. would like to acknowledge a GAANN Fellowship from the Department of Education. The authors thank Katie Jungjohann for access to the F30 in CINT. This work was performed at Sandia National Laboratories in CINT, the Center for Integrated Nanotechnologies. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the US Department of Energy under contract DEAC04-94AL85000. NR 25 TC 0 Z9 0 U1 3 U2 20 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6462 J9 SCRIPTA MATER JI Scr. Mater. PD FEB PY 2015 VL 96 BP 21 EP 24 DI 10.1016/j.scriptamat.2014.10.010 PG 4 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA AX8BD UT WOS:000347134500006 ER PT J AU Yu, Q Jiang, YY Wang, J AF Yu, Qin Jiang, Yanyao Wang, Jian TI Cyclic deformation and fatigue damage in single-crystal magnesium under fully reversed strain-controlled tension-compression in the [10(1)over-bar0] direction SO SCRIPTA MATERIALIA LA English DT Article DE Magnesium single crystal; Cyclic deformation; Twinning-detwinning; Fatigue ID BEHAVIOR; ALLOYS; CRACK; PROPAGATION; PLASTICITY; FRACTURE; SLIP AB Cyclic deformation and the resulting fatigue are experimentally investigated in single-crystal magnesium subjected to fully reversed strain-controlled tension-compression in the [1 0 (1) over bar 0] direction at room temperature. Plastic instability is found near the end of the first detwinning reversal. Twin twin boundaries and secondary twins are induced by interaction of primary {1 0 (1) over bar 2} twins. Microcracks are developed at primary twin boundaries and twin twin interaction sites. Final fracture is most likely caused by cleavage-cracking on the {1 0 (1) over bar 1}-{1 0 (1) over bar 2} double twin and shearing fracture on the basal plane. Published by Elsevier Ltd. on behalf of Acta Materialia Inc. C1 [Yu, Qin; Jiang, Yanyao] Univ Nevada, Dept Mech Engn, Reno, NV 89557 USA. [Yu, Qin; Wang, Jian] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. RP Jiang, YY (reprint author), Univ Nevada, Dept Mech Engn, Reno, NV 89557 USA. EM yjiang@unr.edu; wangj6@lanl.gov RI Jiang, Yanyao/H-1816-2012; Wang, Jian/F-2669-2012 OI Jiang, Yanyao/0000-0002-1977-4669; Wang, Jian/0000-0001-5130-300X FU Office of Basic Energy Sciences under US DOE [FWP 06SCPE401, W-7405-ENG-36]; Los Alamos National Laboratory Directed Research and Development ER grant [20140450ER] FX The Office of Basic Energy Sciences, Project FWP 06SCPE401 under US DOE Contract No. W-7405-ENG-36, supported this work. Q.Y. and J.W. were supported by the Office of Basic Energy Sciences, Project FWP 06SCPE401, under US DOE Contract No W-7405-ENG-36. The authors thank Dr. Carlos N. Tome at Los Alamos National Laboratory for valuable discussions. J.W. is also grateful for support from Los Alamos National Laboratory Directed Research and Development ER grant 20140450ER. NR 34 TC 7 Z9 7 U1 1 U2 27 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6462 J9 SCRIPTA MATER JI Scr. Mater. PD FEB PY 2015 VL 96 BP 41 EP 44 DI 10.1016/j.scriptamat.2014.10.020 PG 4 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA AX8BD UT WOS:000347134500011 ER PT J AU Singh, A Datta, S Sachdeva, A Maslanka, S Dykes, J Skinner, G Burr, D Whiting, RC Sharma, SK AF Singh, Ajay Datta, Shomik Sachdeva, Amita Maslanka, Susan Dykes, Janet Skinner, Guy Burr, Donald Whiting, Richard C. Sharma, Shashi K. TI EVALUATION OF AN ENZYME-LINKED IMMUNOSORBENT ASSAY (ELISA) KIT FOR THE DETECTION OF BOTULINUM NEUROTOXINS A, B, E, AND F IN SELECTED FOOD MATRICES SO HEALTH SECURITY LA English DT Article ID CLOSTRIDIUM-BOTULINUM; TOXINS; TECHNOLOGIES AB The mouse bioassay (MBA) is the only accepted standard method for detection of botulinum neurotoxins (BoNTs) in foods. The ELISA method has several advantages over the MBA and is therefore widely used for in vitro detection of BoNTs. The US Food and Drug Administration (FDA) and the Centers for Disease Control and Prevention (CDC) conducted a precollaborative study to evaluate the applicability of Botulinum Toxin ELISA kits for the detection of BoNT serotypes A, B, E, and F in a variety of food matrices. In this study, food samples (eg, broccoli, salami, smoked salmon, green beans, orange juice, tomato juice, low-fat plain yogurt, whole milk, liquid infant formula milk, and liquid eggs) were spiked with high, medium, and low concentration BoNT serotypes A, B, E, and F. Samples (unspiked and spiked) were tested at both laboratories by the ELISA kits. All food samples were positive for BoNTs by ELISA in both laboratories at medium and high spiking levels; a positive ELISA result in low spiked samples was both serotype and laboratory dependent. Overall, the ELISA method appears to be an effective preliminary screening method for BoNT detection in food matrices. C1 [Singh, Ajay; Datta, Shomik; Sachdeva, Amita] US FDA, Off Regulatory Sci, Ctr Food Safety & Appl Nutr, College Pk, MD USA. [Singh, Ajay; Datta, Shomik; Sachdeva, Amita; Maslanka, Susan; Dykes, Janet; Skinner, Guy; Burr, Donald; Whiting, Richard C.; Sharma, Shashi K.] US Dept Energy Inst, Oak Ridge Inst Sci & Educ, Washington, DC USA. [Datta, Shomik] Vorsight LLC, Arlington, VA USA. [Sachdeva, Amita] Emergent Biosolut, Gaithersburg, MD USA. [Maslanka, Susan; Dykes, Janet] Ctr Dis Control & Prevent, CDC, Natl Botulism Lab Team, Atlanta, GA USA. [Skinner, Guy] US FDA, Inst Food Safety & Hlth, Ctr Food Safety & Appl Nutr, Bedford Pk, IL USA. [Burr, Donald] US FDA, Off Regulatory Affairs, Off Regulatory Sci, Rockville, MD USA. [Whiting, Richard C.] Exponent, Chem Regulat & Food Safety, Bowie, MD USA. [Sharma, Shashi K.] US FDA, Special Pathogen Team, Off Regulatory Sci, Ctr Food Safety & Appl Nutr, College Pk, MD USA. RP Sharma, SK (reprint author), FDA CFSAN, Div Microbiol, Off Regulatory Sci, Room 4E023,5100 Paint Branch Pkwy,HFS-711, College Pk, MD 20740 USA. EM Shashi.Sharma@fda.hhs.gov NR 16 TC 1 Z9 1 U1 3 U2 6 PU MARY ANN LIEBERT, INC PI NEW ROCHELLE PA 140 HUGUENOT STREET, 3RD FL, NEW ROCHELLE, NY 10801 USA SN 2326-5094 EI 2326-5108 J9 HEALTH SECUR JI Health Secur. PD FEB 1 PY 2015 VL 13 IS 1 BP 37 EP 44 DI 10.1089/hs.2014.0075 PG 8 WC Public, Environmental & Occupational Health SC Public, Environmental & Occupational Health GA DD0FT UT WOS:000369596500004 PM 25812427 ER PT J AU Kawano, T Brown, DA AF Kawano, Toshihiko Brown, David A. TI Neutron elastic scattering angular distribution in the resolved and unresolved resonance regions SO JOURNAL OF NUCLEAR SCIENCE AND TECHNOLOGY LA English DT Article DE nuclear data; elastic scattering; angular distribution; neutron resonance; nickel-58; iron-56; zirconium-90; Reich-Moore; multi-level Breit-Wigner ID CROSS-SECTIONS; NUCLEAR-DATA; SCIENCE; MODEL AB We derive a simple relationship between observed total cross sections and elastic scattering angular distributions for neutron-induced reactions in the fast energy range by combining resonance theory and the optical model (OM). This relationship enables us to estimate the anisotropy in the scattering angular distribution when experimental total cross-section data are available. We apply this method to the angular distributions of Ni-58 and Fe-56 and compare with the evaluated values which are based on the experimental data. We also explore the method with Zr-90 for which the multi-level Breit-Wigner resonance parameters are given. C1 [Kawano, Toshihiko] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Brown, David A.] Brookhaven Natl Lab, Natl Nucl Data Ctr, Upton, NY 11973 USA. RP Kawano, T (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM kawano@lanl.gov FU National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; Office of Nuclear Physics of the U.S. Department of Energy [DE-AC02-98CH10886]; Office of Science of the U.S. Department of Energy [DE-AC02-98CH10886]; Brookhaven Science Associates, LLC. FX We would like to thank all the participants of Subgroup 35 "Scattering Angular Distribution in the Fast Energy Range," in Working Party on International Nuclear Data Evaluation Co-operation (WPEC), under the OECD Nuclear Energy Agency. This work was carried out under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. The work at Brookhaven National Laboratory was sponsored by the Office of Nuclear Physics, Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-98CH10886 with Brookhaven Science Associates, LLC. NR 25 TC 0 Z9 0 U1 2 U2 4 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 0022-3131 EI 1881-1248 J9 J NUCL SCI TECHNOL JI J. Nucl. Sci. Technol. PD FEB 1 PY 2015 VL 52 IS 2 BP 274 EP 281 DI 10.1080/00223131.2014.945977 PG 8 WC Nuclear Science & Technology SC Nuclear Science & Technology GA AY4FB UT WOS:000347532500013 ER PT J AU Parrish, K Singh, R Chien, SC AF Parrish, Kristen Singh, Reshma Chien, Szu-Cheng TI The role of international institutional partnerships in delivering low-energy building design: A case study SO SUSTAINABLE CITIES AND SOCIETY LA English DT Article DE International partnerships; High-performance buildings; Design process ID TRENDS AB This paper explores the role of international partnerships to facilitate low-energy building design, construction, and operations. We briefly discuss multiple collaboration models and the levels of impact they support. We present a case study of one collaborative partnership model, the Scientific Planning Support (SPS) team. Staff from the Lawrence Berkeley National Laboratory, the Austrian Institute of Technology, and Nanyang Technological University formed the SPS team to provide design assistance and process support during the design phase of a low-energy building project. Specifically, the SPS team worked on the CleanTech Two project, a tenanted laboratory and office building that seeks Green Mark Platinum, the highest green building certification in Singapore. The SPS team hosted design charrettes, helped to develop design alternatives, and provided suggestions on the design process in support of this aggressive energy target. This paper describes these efforts and discusses how teams like the SPS team and other partnership schemes can be leveraged to achieve high performance, low-energy buildings at an international scale. Specifically, it discusses how international institutional partnerships build capacity for low-energy design, challenge the status quo for building design, and create new resources in support of energy savings on the order of 40%. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Parrish, Kristen] Arizona State Univ, Sch Sustainable Engn & Built Environm, Tempe, AZ 85287 USA. [Singh, Reshma] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Chien, Szu-Cheng] Nanyang Technol Univ, Energy Res Inst, Singapore 637141, Singapore. [Parrish, Kristen] LBNL, Berkeley, CA USA. RP Parrish, K (reprint author), Arizona State Univ, Sch Sustainable Engn & Built Environm, POB 870204, Tempe, AZ 85287 USA. EM Kristen.Parrish@asu.edu; ReshmaSingh@lbl.gov; scchien@ntu.edu.sg FU JTC Corporation, Singapore [JTC C11502011] FX This work was supported by JTC Corporation, Singapore under Contract No. JTC C11502011. This support is gratefully acknowledged. Any opinions, findings, conclusions, or recommendations expressed in this paper are those of the writers and do not necessarily reflect the views of the JTC Corporation. NR 25 TC 1 Z9 1 U1 2 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2210-6715 J9 SUSTAIN CITIES SOC JI Sust. Cities Soc. PD FEB PY 2015 VL 14 BP 383 EP 389 DI 10.1016/j.scs.2014.05.007 PG 7 WC Construction & Building Technology; GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels SC Construction & Building Technology; Science & Technology - Other Topics; Energy & Fuels GA CZ8XY UT WOS:000367383600040 ER PT J AU Scott, F Li, MY Williams, DL Conejeros, R Hodge, DB Aroca, G AF Scott, Felipe Li, Muyang Williams, Daniel L. Conejeros, Raul Hodge, David B. Aroca, German TI Corn stover semi-mechanistic enzymatic hydrolysis model with tight parameter confidence intervals for model-based process design and optimization SO BIORESOURCE TECHNOLOGY LA English DT Article DE Lignocellulose; Enzymatic hydrolysis; Kinetic model; High-solids saccharification; Biofuels ID PRACTICAL IDENTIFIABILITY ANALYSIS; LIGNOCELLULOSIC BIOMASS; CELLULOSE HYDROLYSIS; PRETREATMENT; UNCERTAINTY; INHIBITION; CELLULASES; SOLIDS; SACCHARIFICATION; LIKELIHOOD AB Uncertainty associated to the estimated values of the parameters in a model is a key piece of information for decision makers and model users. However, this information is typically not reported or the confidence intervals are too large to be useful. A semi-mechanistic model for the enzymatic saccharification of dilute acid pretreated corn stover is proposed in this work, the model is a modification of an existing one providing a statistically significant improved fit towards a set of experimental data that includes varying initial solid loadings (10-25% w/w) and the use of the pretreatment liquor and washed solids with or without supplementation of key inhibitors. A subset of 8 out of 17 parameters was identified, showing sufficiently tight confidence intervals to be used in uncertainty propagation and model analysis, without requiring interval truncation via expert judgment. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Scott, Felipe; Conejeros, Raul; Aroca, German] Pontificia Univ Catolica Valparaiso, Sch Biochem Engn, Valparaiso, Chile. [Scott, Felipe; Conejeros, Raul; Aroca, German] Bioenercel SA Barrio Univ, Concepcion, Chile. [Li, Muyang; Williams, Daniel L.; Hodge, David B.] Michigan State Univ, DOE Great Lakes Bioenergy Res Ctr, E Lansing, MI USA. [Li, Muyang; Hodge, David B.] Michigan State Univ, Dept Agr & Biosyst Engn, E Lansing, MI 48824 USA. [Williams, Daniel L.; Hodge, David B.] Michigan State Univ, Dept Chem Engn & Mat Sci, E Lansing, MI 48824 USA. [Hodge, David B.] Lulea Univ Technol, Div Chem Engn, S-95187 Lulea, Sweden. RP Scott, F (reprint author), Pontificia Univ Catolica Valparaiso, Sch Biochem Engn, Av Brasil 2147, Valparaiso, Chile. EM felipe.scott.c@mail.pucv.cl RI Conejeros, Raul/A-2466-2011; Scott, Felipe/K-4193-2016; Aroca, German/L-1319-2016 OI Scott, Felipe/0000-0003-2041-4641; Aroca, German/0000-0003-1376-7940 FU CONICYT's scholarship program (Comision Nacional de Investigacion Cientifica y Tecnologica, Chile); National Science Foundation United States (NSF) [CBET 1336622]; Innova Chile Project Technological Consortium Bioenercel S.A [208-7320] FX Financial support granted to F. Scott by CONICYT's scholarship program (Comision Nacional de Investigacion Cientifica y Tecnologica, Chile) is gratefully acknowledged. Muyang Li was supported in part by a grant from the National Science Foundation United States (NSF CBET 1336622). This work was funded by Innova Chile Project 208-7320 Technological Consortium Bioenercel S.A. NR 35 TC 2 Z9 2 U1 2 U2 32 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0960-8524 EI 1873-2976 J9 BIORESOURCE TECHNOL JI Bioresour. Technol. PD FEB PY 2015 VL 177 BP 255 EP 265 DI 10.1016/j.biortech.2014.11.062 PG 11 WC Agricultural Engineering; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA AX0MT UT WOS:000346647100034 PM 25496946 ER PT J AU Roy, UN Bolotnikov, AE Camarda, GS Cui, Y Hossain, A Lee, K Lee, W Tappero, R Yang, G Cui, Y Burger, A James, RB AF Roy, U. N. Bolotnikov, A. E. Camarda, G. S. Cui, Y. Hossain, A. Lee, K. Lee, W. Tappero, R. Yang, Ge Cui, Y. Burger, A. James, R. B. TI Compositional homogeneity and X-ray topographic analyses of CdTexSe1-x grown by the vertical Bridgman technique SO JOURNAL OF CRYSTAL GROWTH LA English DT Article DE Characterization; Defects; Te-inclusions; Subgrain boundary; CdTeSe; Semiconducting II-VI materials ID CADMIUM ZINC TELLURIDE; TE-RICH SOLUTION; GRADIENT FREEZE; CDTE; DETECTORS; CRYSTALS; SEGREGATION AB We grew CdTexSe1-x crystals with nominal Se concentrations of 5%, 7%, and 10% by the vertical Bridgman technique, and evaluated their compositional homogeneity and structural quality at the NSLS' X-ray fluorescence and white beam X-ray topography beam lines. Both X-ray fluorescence and photoluminescence mapping revealed very high compositional homogeneity of the CdTexSe1-x crystals. We noted that those crystals with higher concentrations of Se were more prone to twinning than those with a lower content. The crystals were fairly free from strains and contained low concentrations of sub-grain boundaries and their networks. Published by Elsevier B.V. C1 [Roy, U. N.; Bolotnikov, A. E.; Camarda, G. S.; Cui, Y.; Hossain, A.; Lee, K.; Lee, W.; Tappero, R.; Yang, Ge; James, R. B.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Lee, K.; Lee, W.] Korea Univ, Seoul 136103, South Korea. [Cui, Y.; Burger, A.] Fisk Univ, Nashville, TN USA. RP Roy, UN (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM uroy@bnl.gov FU U.S. Department of Energy, Office of Defense Nuclear Nonproliferation Research and development, DNN RD; U.S. Department of Energy [DE-AC02-98CH10886] FX The authors would like to thank Richard Greene for fabricating the ampoule lowering mechanism. This work was supported by the U.S. Department of Energy, Office of Defense Nuclear Nonproliferation Research and development, DNN R&D. The manuscript has been authored by Brookhaven Science Associates, LLC under Contract No DE-AC02-98CH10886 with the U.S. Department of Energy. NR 24 TC 1 Z9 1 U1 2 U2 13 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-0248 EI 1873-5002 J9 J CRYST GROWTH JI J. Cryst. Growth PD FEB 1 PY 2015 VL 411 BP 34 EP 37 DI 10.1016/j.jcrysgro.2014.10.057 PG 4 WC Crystallography; Materials Science, Multidisciplinary; Physics, Applied SC Crystallography; Materials Science; Physics GA AX3RW UT WOS:000346857500007 ER PT J AU Subramaniyan, A Perkins, JD O'Hayre, RP Ginley, DS Lany, S Zakutayev, A AF Subramaniyan, Archana Perkins, John D. O'Hayre, Ryan P. Ginley, David S. Lany, Stephan Zakutayev, Andriy TI Non-equilibrium synthesis, structure, and opto-electronic properties of Cu2-2x Zn (x) O alloys SO JOURNAL OF MATERIALS SCIENCE LA English DT Article ID CU2O THIN-FILMS; CUPROUS-OXIDE; DEFECTS; DENSITY; GROWTH; STATES; NI AB Alloying in traditional semiconductors is a well-established method to tune the electronic structure and the materials properties, but this technique is less common for oxides. Here, we present results on the non-equilibrium alloying of the prototypical semiconductor Cu2O with ZnO synthesized via high-throughput RF magnetron sputtering. It is demonstrated that the Zn solid solubility in Cu2O structure can be increased up to 17 at.% in the substrate temperature range 210-270 A degrees C; this upper bound estimate of the solubility limit is much higher than that at equilibrium (sub atomic percent range). The preferential orientation in the film changes from (200) to (111) with increasing Zn concentration, but the lattice parameter and the grain size (80-180 nm) remains constant. Incorporation of Zn into Cu2O increases the optical absorption fourfold at the band gap (2.1 eV) and reduces the p-type electrical conductivity by an order of magnitude. The ability to synthesize phase pure Cu2-2x Zn (x) O alloys with Zn solid solubility in excess of the thermodynamic limit with tunable structural and optoelectronic properties demonstrates the potential of non-equilibrium growth to overcome the solubility limits in oxide thin films and the promise of such alloys for optoelectronic applications. C1 [Subramaniyan, Archana; Perkins, John D.; Ginley, David S.; Lany, Stephan; Zakutayev, Andriy] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Subramaniyan, Archana; O'Hayre, Ryan P.] Colorado Sch Mines, Dept Met & Mat Engn MME, Golden, CO 80401 USA. RP Zakutayev, A (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM asubrama@mymail.mines.edu; john.perkins@nrel.gov; rohayre@mines.edu; David.Ginley@nrel.gov; Stephan.Lany@nrel.gov; Andriy.Zakutayev@nrel.gov OI Lany, Stephan/0000-0002-8127-8885; Zakutayev, Andriy/0000-0002-3054-5525 FU U.S. Department of Energy, office of Energy Efficiency and Renewable Energy [DE-AC36-08GO28308] FX This work was funded by U.S. Department of Energy, office of Energy Efficiency and Renewable Energy under Contract No. DE-AC36-08GO28308 to National Renewable Energy Laboratory, as a part of a Next Generation PV II Project within the SunShot initiative. Thanks to Anna Duda for depositing Au contacts for Seebeck coefficient measurement. Thanks also go to Chris Caskey and Adam Welch for performing few of the XRF measurements. NR 31 TC 7 Z9 7 U1 0 U2 23 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0022-2461 EI 1573-4803 J9 J MATER SCI JI J. Mater. Sci. PD FEB PY 2015 VL 50 IS 3 BP 1350 EP 1357 DI 10.1007/s10853-014-8695-0 PG 8 WC Materials Science, Multidisciplinary SC Materials Science GA AX2MJ UT WOS:000346777800035 ER PT J AU Liu, C Cady, CM Lovato, ML Orler, EB AF Liu, C. Cady, C. M. Lovato, M. L. Orler, E. B. TI Uniaxial tension of thin rubber liner sheets and hyperelastic model investigation SO JOURNAL OF MATERIALS SCIENCE LA English DT Article ID DIGITAL-IMAGE-CORRELATION; DEFORMATION; SOLIDS; FIELD AB Uniaxial tension tests were performed on two different thin rubber liner sheets, the silica-filled and the Kevlar-filled EPDM rubber, for the purpose of establishing the constitutive relations via different hyperelasticity models. Due to the fact that the rubber liner sheet can sustain large amount of deformation, over 700 % engineering strain, we used the non-contact, optical technique of digital image correlation to measure local deformation over the sample surface. Three different hyperelastic models were considered for analyzing the experimental measurement, one is the neo-Hookean including the generalized neo-Hookean (GNH), the second is the Rivlin-type models including the special case of Mooney-Rivlin model, and the third is the Ogden model. Model parameters were determined by fitting the hyperelastic model to the experimental data. It was found that the Rivlin model up to the second order and the Ogden model capture the constitutive behavior of both the silica-filled and the Kevlar-filled rubber sheets quite well, while the GNH model can only describe the stress-stretch relation of the Kevlar-filled rubber sheet. C1 [Liu, C.; Cady, C. M.; Lovato, M. L.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. [Orler, E. B.] Virginia Polytech Inst & State Univ, Dept Chem, Blacksburg, VA 24061 USA. RP Liu, C (reprint author), Los Alamos Natl Lab, Mat Sci & Technol Div, POB 1663, Los Alamos, NM 87545 USA. EM cliu@lanl.gov FU National Nuclear Security Administration (NNSA) of the U.S. Department of Energy [DE-AC52-06NA25396]; Joint DoD/DOE Munitions Program (JMP) FX Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration (NNSA) of the U.S. Department of Energy under contract DE-AC52-06NA25396. This study was supported by the Joint DoD/DOE Munitions Program (JMP). NR 10 TC 1 Z9 1 U1 2 U2 19 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0022-2461 EI 1573-4803 J9 J MATER SCI JI J. Mater. Sci. PD FEB PY 2015 VL 50 IS 3 BP 1401 EP 1411 DI 10.1007/s10853-014-8700-7 PG 11 WC Materials Science, Multidisciplinary SC Materials Science GA AX2MJ UT WOS:000346777800040 ER PT J AU Politakos, N Liontos, G Kortaberria, G Messman, JM Calvo, J Moya, SE Mays, JW Avgeropoulos, A AF Politakos, Nikolaos Liontos, George Kortaberria, Galder Messman, Jamie M. Calvo, Javier Moya, Sergio E. Mays, Jimmy W. Avgeropoulos, Apostolos TI Comparing Linear and Cyclic Synthetic Homopolypeptides: Synthesis and Molecular Characterization SO JOURNAL OF POLYMER SCIENCE PART A-POLYMER CHEMISTRY LA English DT Article DE gel permeation chromatography (GPC); mass spectrometry; NMR; peptides; ring-opening polymerization ID ACID-N-CARBOXYANHYDRIDES; HIGH-VACUUM TECHNIQUES; COIL BLOCK-COPOLYMERS; POLY(GAMMA-BENZYL L-GLUTAMATE); ANIONIC-POLYMERIZATION; DIBLOCK COPOLYMERS; POLYPEPTIDE BLOCK; AMINO-ACIDS; A-COMPONENT; B-COMPONENT AB The synthesis and molecular characterization of a linear and a cyclic homopolypeptide of protected l-tyrosine are reported. In this work, the successful synthesis of polypeptides exhibiting the desired linear and cyclic structures through various characterization methods such as high temperature gel permeation chromatography, Fourier transform infrared spectroscopy, proton and carbon nuclear magnetic resonance spectroscopy, mass spectrometry, dynamic light scattering, differential scanning calorimetry, and thermogravimetric analysis was verified. The results are very promising especially if such cyclic materials will be potentially used as carriers for drug delivery, either through conjugation with specific ligands or directly through the functional hydroxyl groups of the monomeric units of poly(l-Tyr) after deprotection. (c) 2014 Wiley Periodicals, Inc. J. Polym. Sci., Part A: Polym. Chem. 2015, 53, 393-404 C1 [Politakos, Nikolaos; Kortaberria, Galder] Euskal Herriko Unibertsitatea, Univ Pais Vasco, Dept Ingn Quim & M Ambiente, Mat Technol Grp,Polytech Sch, San Sebastian 20018, Spain. [Politakos, Nikolaos; Calvo, Javier; Moya, Sergio E.] CIC biomaGUNE, San Sebastian 20009, Spain. [Politakos, Nikolaos; Liontos, George; Avgeropoulos, Apostolos] Univ Ioannina, Dept Mat Sci Engn, GR-45110 Ioannina, Greece. [Messman, Jamie M.; Mays, Jimmy W.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Avgeropoulos, A (reprint author), Univ Ioannina, Dept Mat Sci Engn, Univ Campus Dourouti, GR-45110 Ioannina, Greece. EM aavger@cc.uoi.gr RI Kortaberria, Galder/H-4600-2015; Moya, Sergio/I-1446-2015; biomaGUNE, CIC/J-9136-2014; Avgeropoulos, Apostolos/I-5772-2012; OI Kortaberria, Galder/0000-0002-0433-7693; biomaGUNE, CIC/0000-0001-7690-0660; Kortaberria, Galder/0000-0003-3890-7946 FU Basque Country Government [NanoIker IE11-304, SAIOTEK2012 S-PE12UN106, IT776-13]; Ministry of Education and Innovation [MAT2012-31675]; Office of Basic Energy Sciences, U.S. Department of Energy at Oak Ridge National Laboratory FX Financial support from the Basque Country Government (NanoIker IE11-304, SAIOTEK2012 S-PE12UN106, Grupos Consolidados IT776-13) and from the Ministry of Education and Innovation (MAT2012-31675) is gratefully acknowledged. A portion of this research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Office of Basic Energy Sciences, U.S. Department of Energy. Technical and human support provided by SGIker (UPV/EHU, MICINN, GV/EJ, ERDF and ESF) is also acknowledged. NR 61 TC 1 Z9 1 U1 2 U2 39 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0887-624X EI 1099-0518 J9 J POLYM SCI POL CHEM JI J. Polym. Sci. Pol. Chem. PD FEB 1 PY 2015 VL 53 IS 3 BP 393 EP 404 DI 10.1002/pola.27434 PG 12 WC Polymer Science SC Polymer Science GA AX2JC UT WOS:000346768400001 ER PT J AU Kirk, M Iddins, CJ AF Kirk, Mark Iddins, Carol J. TI Resources for Toxicologic and Radiologic Information and Assistance SO EMERGENCY MEDICINE CLINICS OF NORTH AMERICA LA English DT Article DE Resources; Chemical; Radiological; Nuclear detonation; Competencies; Risk assessment ID DECONTAMINATION; EXPOSURE AB Most approaches toward chemical and radiological/nuclear (CRN) incidents focus on the clinical skills of the first receiver. These skills are certainly important and are addressed throughout this article. Information management skills are often overlooked. Emergency physicians must competently amass information elements most critical to know during a crisis, choosing an appropriate resource to rapidly find reliable information. During large-scale CRN incidents, the emergency physician needs to use information for: planning, incident management, toxicant management, disposition/definitive care, and recovery management. Information management and synthesis are crucial throughout the phases of the disaster cycle: planning, response, mitigation, and recovery. C1 [Kirk, Mark] US Dept Homeland Secur, Chem Def Program, Hlth Threats Resilience Div, Off Hlth Affairs, Washington, DC USA. [Iddins, Carol J.] US DOE, Radiat Emergency Assistance Ctr, ORISE, ORAU, Oak Ridge, TN 37831 USA. RP Iddins, CJ (reprint author), US DOE, Radiat Emergency Assistance Ctr, ORISE, ORAU, Training Site,POB 117,MS 39, Oak Ridge, TN 37831 USA. EM carol.iddins@orau.org NR 19 TC 0 Z9 0 U1 1 U2 7 PU W B SAUNDERS CO-ELSEVIER INC PI PHILADELPHIA PA 1600 JOHN F KENNEDY BOULEVARD, STE 1800, PHILADELPHIA, PA 19103-2899 USA SN 0733-8627 EI 1558-0539 J9 EMERG MED CLIN N AM JI Emerg. Med. Clin. N. Am. PD FEB PY 2015 VL 33 IS 1 BP 69 EP + DI 10.1016/j.emc.2014.09.007 PG 21 WC Emergency Medicine SC Emergency Medicine GA AW6PS UT WOS:000346391800007 PM 25455663 ER PT J AU Kazzi, Z Buzzell, J Bertelli, L Christensen, D AF Kazzi, Ziad Buzzell, Jennifer Bertelli, Luiz Christensen, Doran TI Emergency Department Management of Patients Internally Contaminated with Radioactive Material SO EMERGENCY MEDICINE CLINICS OF NORTH AMERICA LA English DT Article DE Radioactive terrorism; Contamination; Radioactive elements; Radiation dosage; Chelation therapy ID UNITED-STATES; GOIANIA; RESIDENTS; ACCIDENT; INCIDENT AB After a radiation emergency that involves the dispersal of radioactive material, patients can become externally and internally contaminated with 1 or more radionuclides. Internal contamination can lead to the delivery of harmful ionizing radiation doses to various organs and tissues or the whole body. The clinical consequences can range from acute radiation syndrome to the long-term development of cancer. Estimating the amount of radioactive material absorbed into the body can guide the management of patients. Treatment includes, in addition to supportive care and long term monitoring, certain medical countermeasures like Prussian blue, calcium diethylenetriamine pentaacetic acid (DTPA) and zinc DTPA. C1 [Kazzi, Ziad; Buzzell, Jennifer] Ctr Dis Control & Prevent, Natl Ctr Environm Hlth, Atlanta, GA 30341 USA. [Kazzi, Ziad] Emory Univ, Dept Emergency Med, Atlanta, GA 30322 USA. [Bertelli, Luiz] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Christensen, Doran] Radiat Emergency Assistance Ctr, Oak Ridge, TN 37831 USA. RP Kazzi, Z (reprint author), 4770 Buford Highway Norhteast,MS F59, Atlanta, GA 30341 USA. EM ZKAZZI@emory.edu NR 55 TC 2 Z9 2 U1 2 U2 12 PU W B SAUNDERS CO-ELSEVIER INC PI PHILADELPHIA PA 1600 JOHN F KENNEDY BOULEVARD, STE 1800, PHILADELPHIA, PA 19103-2899 USA SN 0733-8627 EI 1558-0539 J9 EMERG MED CLIN N AM JI Emerg. Med. Clin. N. Am. PD FEB PY 2015 VL 33 IS 1 BP 179 EP + DI 10.1016/j.emc.2014.09.008 PG 19 WC Emergency Medicine SC Emergency Medicine GA AW6PS UT WOS:000346391800012 PM 25455668 ER PT J AU Lu, F Morzfeld, M Tu, XM Chorin, AJ AF Lu, Fei Morzfeld, Matthias Tu, Xuemin Chorin, Alexandre J. TI Limitations of polynomial chaos expansions in the Bayesian solution of inverse problems SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Polynomial chaos expansion; Bayesian inverse problem; Monte Carlo sampling ID UNCERTAINTY QUANTIFICATION; DATA ASSIMILATION; PARTICLE FILTERS; INFERENCE; EQUATIONS AB Polynomial chaos expansions are used to reduce the computational cost in the Bayesian solutions of inverse problems by creating a surrogate posterior that can be evaluated inexpensively. We show, by analysis and example, that when the data contain significant information beyond what is assumed in the prior, the surrogate posterior can be very different from the posterior, and the resulting estimates become inaccurate. One can improve the accuracy by adaptively increasing the order of the polynomial chaos, but the cost may increase too fast for this to be cost effective compared to Monte Carlo sampling without a surrogate posterior. (C) 2014 Elsevier Inc. All rights reserved. C1 [Lu, Fei; Morzfeld, Matthias; Chorin, Alexandre J.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Lu, Fei; Morzfeld, Matthias; Chorin, Alexandre J.] Univ Calif Berkeley, Dept Math, Berkeley, CA 94720 USA. [Tu, Xuemin] Univ Kansas, Dept Math, Lawrence, KS 66045 USA. RP Morzfeld, M (reprint author), Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM mmo@math.lbl.gov FU Office of Science, Computational and Technology Research, U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [DMS-1217065, DMS-1419069, DMS-1115759] FX This work was supported in part by the Director, Office of Science, Computational and Technology Research, U.S. Department of Energy under Contract No. DE-AC02-05CH11231, and by the National Science Foundation under grants DMS-1217065, DMS-1419069, and DMS-1115759. NR 32 TC 3 Z9 3 U1 0 U2 13 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD FEB 1 PY 2015 VL 282 BP 138 EP 147 DI 10.1016/j.jcp.2014.11.010 PG 10 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AW7FS UT WOS:000346430700010 ER PT J AU Norman, MR AF Norman, Matthew R. TI Hermite WENO limiting for multi-moment finite-volume methods using the ADER-DT time discretization for 1-D systems of conservation laws SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE ADER; WENO; Hermite WENO; Differential transform; Finite-volume ID ESSENTIALLY NONOSCILLATORY SCHEMES; HAMILTON-JACOBI EQUATIONS; EFFICIENT IMPLEMENTATION; SOURCE TERMS; MESHES; ORDER AB New Hermite Weighted Essentially Non-Oscillatory (HWENO) interpolants are developed and investigated within the Multi-Moment Finite-Volume (MMFV) formulation using the ADER-DT time discretization. Whereas traditional WENO methods interpolate pointwise, function-based WENO methods explicitly form a non-oscillatory, high-order polynomial over the cell in question. This study chooses a function-based approach and details how fast convergence to optimal weights for smooth flow is ensured. Methods of sixth-, eighth-, and tenth-order accuracy are developed. These are compared against traditional single-moment WENO methods of fifth-, seventh-, ninth-, and eleventh-order accuracy to compare against more familiar methods from literature. The new HWENO methods improve upon existing HWENO methods (1) by giving a better resolution of unreinforced contact discontinuities and (2) by only needing a single HWENO polynomial to update both the cell mean value and cell mean derivative. Test cases to validate and assess these methods include 1-D linear transport, the 1-D inviscid Burger's equation, and the 1-D inviscid Euler equations. Smooth and non-smooth flows are used for evaluation. These HWENO methods performed better than comparable literature-standard WENO methods for all regimes of discontinuity and smoothness in all tests herein. They exhibit improved optimal accuracy due to the use of derivatives, and they collapse to solutions similar to typical WENO methods when limiting is required. The study concludes that the new HWENO methods are robust and effective when used in the ADER-DT MMFV framework. These results are intended to demonstrate capability rather than exhaust all possible implementations. Published by Elsevier Inc. C1 Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Norman, MR (reprint author), Oak Ridge Natl Lab, POB 2008 MS6016, Oak Ridge, TN 37831 USA. EM normanmr@ornl.gov FU Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725] FX This research used resources of the National Center for Computational Sciences at Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. NR 22 TC 1 Z9 1 U1 0 U2 4 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD FEB 1 PY 2015 VL 282 BP 381 EP 396 DI 10.1016/j.jcp.2014.11.017 PG 16 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AW7FS UT WOS:000346430700024 ER PT J AU Batygin, YK AF Batygin, Yuri k. TI Dynamics of intense particle beam in axial-symmetric magnetic field SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Beam; Emittance; Acceptance; Solenoid; Aberration; Space charge ID LINEAR ACCELERATORS AB Axial-symmetric magnetic field is often used in focusing of particle beams. Most existing ion Low Energy Beam Transport lines are based on solenoid focusing. Modern accelerator projects utilize superconducting solenoids in combination with superconducting accelerating cavities for acceleration of high-intensity particle beams. Present article discusses conditions for matched beam in axial-symmetric magnetic field. Analysis allows us to minimize power consumption of solenoids and beam emittance growth due to nonlinear space charge, lens aberrations, and maximize acceptance of the channel. Expressions for maximum beam current in focusing structure, beam emittance growth due to spherical aberrations and non-linear space charge forces are derived. (C) 2014 Elsevier B.V. All rights reserved. C1 Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Batygin, YK (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM batygin@lanl.gov NR 15 TC 0 Z9 0 U1 1 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD FEB 1 PY 2015 VL 772 BP 93 EP 102 DI 10.1016/j.nima.2014.10.034 PG 10 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AX0KU UT WOS:000346642200014 ER PT J AU Zhu, GD Neises, T Turchi, C Bedilion, R AF Zhu, Guangdong Neises, Ty Turchi, Craig Bedilion, Robin TI Thermodynamic evaluation of solar integration into a natural gas combined cycle power plant SO RENEWABLE ENERGY LA English DT Article DE Concentrating solar power; Integrated solar combined cycle; Solar hybridization; Thermodynamic analysis ID PERFORMANCE AB The term integrated solar combined-cycle (ISCC) has been used to define the combination of solar thermal energy into a natural gas combined-cycle (NGCC) power plant. Based on a detailed thermodynamic cycle model for a reference ISCC plant, the impact of solar addition is thoroughly evaluated for a wide range of input parameters such as solar thermal input and ambient temperature. It is shown that solar hybridization into an NGCC plant may give rise to a substantial benefit from a thermodynamic point of view. The work here also indicates that a significant solar contribution may be achieved in an ISCC plant, thus implying substantial fuel savings and environmental benefits. (C) 2014 Published by Elsevier Ltd. C1 [Zhu, Guangdong; Neises, Ty; Turchi, Craig] NREL, Concentrating Solar Power Program, Golden, CO 80401 USA. [Bedilion, Robin] Elect Power Res Inst, Palo Alto, CA 94304 USA. RP Zhu, GD (reprint author), NREL, Concentrating Solar Power Program, Golden, CO 80401 USA. EM guangdong.zhu@nrel.gov FU U.S. Department of Energy [DE-A06-08-GO28308] FX The work at NREL was supported by the U.S. Department of Energy under Contract No. DE-A06-08-GO28308. The authors wish to thank Robin Bedilion and Cara Libby from EPRI for their kindest support on the original ISCC model. The authors greatly benefitted from discussions with June Chen at GE Global Research. Special thanks go to Mike Erbes at Enginomix for his support on the IPSEpro modeling. NR 14 TC 12 Z9 13 U1 3 U2 14 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0960-1481 J9 RENEW ENERG JI Renew. Energy PD FEB PY 2015 VL 74 BP 815 EP 824 DI 10.1016/j.renene.2014.08.073 PG 10 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels SC Science & Technology - Other Topics; Energy & Fuels GA AU9YK UT WOS:000345947700088 ER PT J AU Richardson, M Sankaranarayanan, SKRS Bhethanabotla, VR AF Richardson, Mandek Sankaranarayanan, Subramanian K. R. S. Bhethanabotla, Venkat R. TI Low Insertion Loss and Highly Sensitive SH-SAW Sensors Based on 36 degrees YX LiTaO3 Through the Incorporation of Filled Microcavities SO IEEE SENSORS JOURNAL LA English DT Article DE ANSYS; biosensors; finite element modeling (FEM); frequency response; insertion loss (IL) piezoelectric materials; surface acoustic waves (SAW) ID ACOUSTIC-WAVE BIOSENSOR; NANOCRYSTALLINE DIAMOND; ZNO/LITAO3 STRUCTURES; ALUMINUM NITRIDE; DEVICES; IMMUNOSENSORS; ZNO/QUARTZ; FILM AB Reduction in power consumption and improvement in mass sensitivity are important considerations for surface acoustic wave (SAW) devices used in various sensing applications. Detection of minute quantities of a particular species (clinical sensing) and power requirements (wireless sensing) are two key metrics that must be optimized. In this paper, a 3-D finite element model (FEM) was employed to compare insertion loss (IL) and mass sensitivity of SAW sensors having microcavities filled with ZnO and nanocrystalline diamond to a standard two-port SAW design. Initial simulation results show that ZnO filled cavities (depth = 5 mu m) were most effective at reducing power loss Delta IL = (6.03 dB) by increasing particle displacement (acousto-electric to mechanical transduction) at the output transducer. A 100-pg/cm(2) load was applied to the sensing area of each device to evaluate mass sensitivity. Our simulations suggest that ZnO filled cavities with shallow depth (2.5 mu m) have the greatest sensitivity. The FEM simulations are used to understand the acoustic wave propagation in microcavity-based SAW sensors. The observed enhancement in mass sensitivity and power transfer is attributed to waveguiding effects and constructive interference of the scattered acoustic waves from the microcavities. Devices fabricated with microcavities similar to 1 mu m deep decreased IL by 3.306 dB compared with a standard SAW device. Additional simulations were conducted for each device configuration using the same depth in order to make a direct comparison between measured and simulated results. Our findings offer encouraging prospects for designing low IL highly sensitive microcavity-based SAW biosensors. C1 [Richardson, Mandek; Bhethanabotla, Venkat R.] Univ S Florida, Dept Chem & Biomed Engn, Tampa, FL 33620 USA. [Sankaranarayanan, Subramanian K. R. S.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Richardson, M (reprint author), Univ S Florida, Dept Chem & Biomed Engn, Tampa, FL 33620 USA. EM mbrichar@mail.usf.edu; skrssank@anl.gov; bhethana@usf.edu FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX The authors would like to thank Research Computing, within USF Information Technology, University of South Florida for use of software and access to high performance computing resources. Use of the Center for Nanoscale Materials was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 36 TC 6 Z9 6 U1 6 U2 34 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1530-437X EI 1558-1748 J9 IEEE SENS J JI IEEE Sens. J. PD FEB PY 2015 VL 15 IS 2 BP 787 EP 796 DI 10.1109/JSEN.2014.2353794 PG 10 WC Engineering, Electrical & Electronic; Instruments & Instrumentation; Physics, Applied SC Engineering; Instruments & Instrumentation; Physics GA AU9IQ UT WOS:000345905900002 ER PT J AU Lindner, B Petridis, L Langan, P Smith, JC AF Lindner, Benjamin Petridis, Loukas Langan, Paul Smith, Jeremy C. TI Determination of Cellulose Crystallinity from Powder Diffraction Diagrams SO BIOPOLYMERS LA English DT Article DE molecular modeling; X-ray scattering; finite crystallites; noncrystallinity ID NEUTRON FIBER DIFFRACTION; HYDROGEN-BONDING SYSTEM; X-RAY DIFFRACTOGRAMS; ENZYMATIC-HYDROLYSIS; CELL WALL; MICROFIBRIL; SIMULATION; INDEX; SIZE AB One-dimensional (1D) (spherically averaged) powder diffraction diagrams are commonly used to determine the degree of cellulose crystallinity in biomass samples. Here, it is shown using molecular modeling how disorder in cellulose fibrils can lead to considerable uncertainty in conclusions drawn concerning crystallinity based on 1D powder diffraction data alone. For example, cellulose microfibrils that contain both crystalline and noncrystalline segments can lead to powder diffraction diagrams lacking identifiable peaks, while microfibrils without any crystalline segments can lead to such peaks. This leads to false positives, that is, assigning disordered cellulose as crystalline, and false negatives, that is, categorizing fibrils with crystalline segments as amorphous. The reliable determination of the fraction of crystallinity in any given biomass sample will require a more sophisticated approach combining detailed experiment and simulation. (c) 2014 Wiley Periodicals, Inc. Biopolymers 103: 67-73, 2015. C1 [Lindner, Benjamin; Petridis, Loukas; Smith, Jeremy C.] Oak Ridge Natl Lab, UT ORNL Ctr Mol Biophys, Biosci Div, Oak Ridge, TN 37830 USA. [Smith, Jeremy C.] Univ Tennessee, Dept Biochem & Cellular & Mol Biol, Knoxville, TN 37996 USA. [Langan, Paul] Oak Ridge Natl Lab, Biol & Soft Matter Div, CSMB, Oak Ridge, TN 37831 USA. RP Smith, JC (reprint author), Oak Ridge Natl Lab, UT ORNL Ctr Mol Biophys, Biosci Div, 1 Bethel Valley Rd,Bldg 6011, Oak Ridge, TN 37830 USA. EM smithjc@ornl.gov RI smith, jeremy/B-7287-2012; Petridis, Loukas/B-3457-2009; Langan, Paul/N-5237-2015 OI smith, jeremy/0000-0002-2978-3227; Petridis, Loukas/0000-0001-8569-060X; Langan, Paul/0000-0002-0247-3122 FU Genomic Science Program, Office of Biological and Environmental Research, U. S. Department of Energy [FWP ERKP752] FX Contract grant sponsor: Genomic Science Program, Office of Biological and Environmental Research, U. S. Department of Energy; Contract grant number: FWP ERKP752 NR 25 TC 5 Z9 5 U1 1 U2 50 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0006-3525 EI 1097-0282 J9 BIOPOLYMERS JI Biopolymers PD FEB PY 2015 VL 103 IS 2 BP 67 EP 73 DI 10.1002/bip.22555 PG 7 WC Biochemistry & Molecular Biology; Biophysics SC Biochemistry & Molecular Biology; Biophysics GA AU3LS UT WOS:000345515300001 PM 25269646 ER PT J AU Ong, SP Cholia, S Jain, A Brafman, M Gunter, D Ceder, G Persson, KA AF Ong, Shyue Ping Cholia, Shreyas Jain, Anubhav Brafman, Miriam Gunter, Dan Ceder, Gerbrand Persson, Kristin A. TI The Materials Application Programming Interface (API): A simple, flexible and efficient API for materials data based on REpresentational State Transfer (REST) principles SO COMPUTATIONAL MATERIALS SCIENCE LA English DT Article DE Materials Project; Application Programming Interface; High-throughput; Materials genome; Rest; Representational state transfer ID CATHODES; PYTHON; ION AB In this paper, we describe the Materials Application Programming Interface (API), a simple, flexible and efficient interface to programmatically query and interact with the Materials Project database based on the REpresentational State Transfer (REST) pattern for the web. Since its creation in Aug 2012, the Materials API has been the Materials Project's de facto platform for data access, supporting not only the Materials Project's many collaborative efforts but also enabling new applications and analyses. We will highlight some of these analyses enabled by the Materials API, particularly those requiring consolidation of data on a large number of materials, such as data mining of structural and property trends, and generation of phase diagrams. We will conclude with a discussion of the role of the API in building a community that is developing novel applications and analyses based on Materials Project data. (C) 2014 Elsevier B.V. All rights reserved. C1 [Ong, Shyue Ping] Univ Calif San Diego, Dept NanoEngn, La Jolla, CA 92093 USA. [Cholia, Shreyas; Jain, Anubhav; Brafman, Miriam; Gunter, Dan; Persson, Kristin A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Ceder, Gerbrand] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. RP Ong, SP (reprint author), Univ Calif San Diego, Dept NanoEngn, 9500 Gilman Dr,Mail Code 0448, La Jolla, CA 92093 USA. EM ongsp@ucsd.edu; scholia@lbl.gov; ajain@lbl.gov; mbrafman@lbl.gov; dkgunter@lbl.gov; gceder@mit.edu; kapersson@lbl.gov RI Ong, Shyue Ping/D-7573-2014 OI Ong, Shyue Ping/0000-0001-5726-2587 FU Department of Energy's Basic Energy Sciences program [EDCBEE]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Department of Energy's Basic Energy Sciences program under Grant No. EDCBEE. We also thank the National Energy Research Scientific Computing Center (NERSC), a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, for providing invaluable computing resources and IT support for this project. NR 37 TC 29 Z9 29 U1 7 U2 41 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0256 EI 1879-0801 J9 COMP MATER SCI JI Comput. Mater. Sci. PD FEB 1 PY 2015 VL 97 BP 209 EP 215 DI 10.1016/j.commatsci.2014.10.037 PG 7 WC Materials Science, Multidisciplinary SC Materials Science GA AU3JF UT WOS:000345508100029 ER PT J AU Stacchiola, D Sterrer, M Senanayake, SD Liu, P AF Stacchiola, Dario Sterrer, Martin Senanayake, Sanjaya D. Liu, Ping TI Oxides in Catalysis Preface SO CATALYSIS TODAY LA English DT Editorial Material C1 [Stacchiola, Dario; Senanayake, Sanjaya D.; Liu, Ping] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Sterrer, Martin] Fritz Haber Inst, Dept Chem Phys, Berlin, Germany. RP Stacchiola, D (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM djs@bnl.gov; sterrer@fhl-berlin.mpg.de; ssenanay@bnl.gov; pingliu3@bnl.gov RI Stacchiola, Dario/B-1918-2009 OI Stacchiola, Dario/0000-0001-5494-3205 NR 0 TC 0 Z9 0 U1 2 U2 16 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0920-5861 EI 1873-4308 J9 CATAL TODAY JI Catal. Today PD FEB 1 PY 2015 VL 240 BP 183 EP 183 DI 10.1016/j.cattod.2014.10.024 PN B PG 1 WC Chemistry, Applied; Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA AT7NJ UT WOS:000345124200001 ER PT J AU Mudiyanselage, K Baber, AE Liu, ZY Senanayake, SD Stacchiola, DJ AF Mudiyanselage, Kumudu Baber, Ashleigh E. Liu, Zongyuan Senanayake, Sanjaya D. Stacchiola, Dario J. TI Isolation and characterization of formates on CeOx-CuyO/Cu(111) SO CATALYSIS TODAY LA English DT Article DE Formate; IRRAS; Cu(111); Ceria ID WATER-GAS SHIFT; FORMIC-ACID ADSORPTION; SCANNING-TUNNELING-MICROSCOPY; METHANOL SYNTHESIS; CU(110) SURFACES; SPECTROSCOPIC IDENTIFICATION; PHOTOELECTRON DIFFRACTION; IN-SITU; OXYGEN; DECOMPOSITION AB Formate species have been proposed to be either critical intermediates or spectators in the water-gas shift (WGS) and methanol synthesis processes. CeOx-CuyO/Cu(1 1 1) has been shown to be a very active inverse catalyst for the WGS reaction. We present here the study of formate species obtained from the deprotonation of formic acid (HCOOH) on the inverse catalysts. Exposure of CeOx-CuyO/Cu(1 1 1) to HCOOH at 300K leads to the formation of formates on both ceria and Cu sites. The formates isolated on CeOx-CuyO/Cu( 1 1 1) systems cannot be hydrogenated even at a pressure of 200 Torr H-2 at 300-350 K. The formate species localized on ceria sites are thermally more stable than those on Cu sites, and the thermal decomposition of all of the formates occurs by dehydrogenation releasing CO2 and H-2. Evidence of reverse spillover of formates from the oxide to the metal was observed on CeO2-x/Cu(1 1 1) inverse catalysts. (C) 2014 Elsevier B.V. All rights reserved. C1 [Mudiyanselage, Kumudu; Baber, Ashleigh E.; Senanayake, Sanjaya D.; Stacchiola, Dario J.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Mudiyanselage, Kumudu] BMCC CUNY, Dept Sci, New York, NY 10007 USA. [Liu, Zongyuan] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. RP Stacchiola, DJ (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM djs@bnl.gov RI Stacchiola, Dario/B-1918-2009; Mudiyanselage, Kumudu/B-2277-2013; OI Stacchiola, Dario/0000-0001-5494-3205; Mudiyanselage, Kumudu/0000-0002-3539-632X; Senanayake , Sanjaya /0000-0003-3991-4232 FU U.S. Department of Energy, Office of Science [DE-ACO2-98CH10886]; Division of Chemical Sciences, Geosciences, and Biosciences within the Office of Basic Energy Sciences FX The work at BNL was carried out under Contract No. DE-ACO2-98CH10886 with the U.S. Department of Energy, Office of Science, and supported by its Division of Chemical Sciences, Geosciences, and Biosciences within the Office of Basic Energy Sciences. NR 62 TC 5 Z9 5 U1 7 U2 57 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0920-5861 EI 1873-4308 J9 CATAL TODAY JI Catal. Today PD FEB 1 PY 2015 VL 240 BP 190 EP 200 DI 10.1016/j.cattod.2014.06.001 PN B PG 11 WC Chemistry, Applied; Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA AT7NJ UT WOS:000345124200003 ER PT J AU Rodriguez, JA Si, R Evans, J Xu, WQ Hanson, JC Tao, J Zhu, YM AF Rodriguez, Jose A. Si, Rui Evans, Jaime Xu, Wenqian Hanson, Jonathan C. Tao, Jing Zhu, Yimei TI Active gold-ceria and gold-ceria/titania catalysts for CO oxidation: From single-crystal model catalysts to powder catalysts SO CATALYSIS TODAY LA English DT Article DE Gold; Ceria; Titania; CO oxidation; X-ray diffraction; X-ray absorption; Active site ID WATER-GAS SHIFT; LOW-TEMPERATURE OXIDATION; CARBON-MONOXIDE; IN-SITU; TITANIA CATALYSTS; AU; NANOPARTICLES; OXIDE; AU/CEOX/TIO2(110); IDENTIFICATION AB CO oxidation was studied on model and powder catalysts of Au-CeO2 and Au-CeOx/TiO2. Phenomena observed in Au-CeO2(1 1 1) and Au-CeO2/TiO2(11 0) provided useful concepts for designing and preparing highly active and stable Au-CeOx/TiO2 powder catalysts for CO oxidation. Small particles of Au dispersed on CeO2(1 1 1) displayed high catalytic activity, making Au-CeO2(1 1 1) a better CO oxidation catalyst than Au-TiO2(11 0) or Au-MgO(1 00). An excellent support for gold was found after depositing nanoparticles of ceria on TiO2(1 1 0). The CeO, nanoparticles act as nucleation centers for gold, improving dispersion of the supported metal and helping in the creation of reaction sites efficient for the adsorption of CO and the dissociation of the O-2 molecule. High-surface area catalysts were prepared by depositing gold on ceria nanorods and CeOx/TiO2 powders. The samples were tested for the low-temperature (10-70 degrees C) oxygenrich (1%CO/4%O-2/He) CO oxidation reaction after pre-oxidation (20%O-2/He, 300 degrees C) and pre-reduction (5%H-2/He, 300 degrees C) treatments. Synchrotron-based operando X-ray diffraction (XRD) and X-ray absorption (XAS) spectroscopy were used to study the Au-CeO2 and Au-CeOx/TiO2 catalysts under reaction conditions. Our operando findings indicate that the most active phase of these catalysts for low-temperature CO oxidation consist of small particles of metallic Au dispersed on CeO2 or CeOx/TiO2. (C) 2014 Elsevier By. All rights reserved. C1 [Rodriguez, Jose A.; Si, Rui; Xu, Wenqian; Hanson, Jonathan C.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Evans, Jaime] Cent Univ Venezuela, Fac Ciencias, Caracas 1020, Venezuela. [Tao, Jing; Zhu, Yimei] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Rodriguez, JA (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM rodrigez@bnl.gov RI Hanson, jonathan/E-3517-2010 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-ACO2-98CH10886]; INTEVEP; IDB for research; Universidad Central de Venezuela FX This research was carried out in part at the National Synchrotron Light Source and the Center for Functional Nanomaterials at Brookhaven National Laboratory, which are supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under contract DE-ACO2-98CH10886. I.E. thanks INTEVEP and IDB for research grants that made possible part of the work done at the Universidad Central de Venezuela. NR 43 TC 15 Z9 15 U1 12 U2 150 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0920-5861 EI 1873-4308 J9 CATAL TODAY JI Catal. Today PD FEB 1 PY 2015 VL 240 BP 229 EP 235 DI 10.1016/j.cattod.2014.06.033 PN B PG 7 WC Chemistry, Applied; Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA AT7NJ UT WOS:000345124200008 ER PT J AU Goldberg, RN Schliesser, J Mittal, A Decker, SR Santos, AFLOM Freitas, VLS Urbas, A Lang, BE Heiss, C da Silva, MDMCR Woodfield, BF Katahira, R Wang, W Johnson, DK AF Goldberg, Robert N. Schliesser, Jacob Mittal, Ashutosh Decker, Stephen R. Santos, Ana Filipa L. O. M. Freitas, Vera L. S. Urbas, Aaron Lang, Brian E. Heiss, Christian da Silva, Maria D. M. C. Ribeiro Woodfield, Brian F. Katahira, Rui Wang, Wei Johnson, David K. TI A thermodynamic investigation of the cellulose allomorphs: Cellulose(am), cellulose I beta(cr), cellulose II(cr), and cellulose III(cr) SO JOURNAL OF CHEMICAL THERMODYNAMICS LA English DT Article DE Cadoxen; Calorimetry; Cellulose amorphous; Cellulose I; Cellulose II; Cellulose III; Enthalpy; Entropy; Gibbs free energy; Heat capacity; NMR ID DIFFERENTIAL SCANNING CALORIMETRY; NEUTRON FIBER DIFFRACTION; SYNCHROTRON X-RAY; NUCLEAR-MAGNETIC-RESONANCE; HEAT-CAPACITY MEASUREMENTS; HYDROGEN-BONDING SYSTEM; CRYSTAL-STRUCTURE; MICROCRYSTALLINE CELLULOSE; GLASSY STATE; WATER AB The thermochemistry of samples of amorphous cellulose, cellulose I, cellulose II, and cellulose III was studied by using oxygen bomb calorimetry, solution calorimetry in which the solvent was cadoxen (a cadmium ethylenediamine solvent), and with a Physical Property Measurement System (PPMS) in zero magnetic field to measure standard massic heat capacities C-p,C-w degrees over the temperature range T = (2 to 302) K. The samples used in this study were prepared so as to have different values of crystallinity indexes CI and were characterized by X-ray diffraction, by Karl Fischer moisture determination, and by using gel permeation chromatography to determine the weight average degree of polymerization DPw. NMR measurements on solutions containing the samples dissolved in cadoxen were also performed in an attempt to resolve the issue of the equivalency or non-equivalency of the nuclei in the different forms of cellulose that were dissolved in cadoxen. While large differences in the NMR spectra for the various cellulose samples in cadoxen were not observed, one cannot be absolutely certain that these cellulose samples are chemically equivalent in cadoxen. Equations were derived which allow one to adjust measured property values of cellulose samples having a mass fraction of water w(H2O) to a reference value of the mass fraction of water w(ref). The measured thermodynamic properties (standard massic enthalpy of combustion Delta H-c(w)degrees, standard massic enthalpy of solution Delta H-sol(w)degrees, and C-p,C-w degrees) were used in conjunction with the measured CI values to calculate values of the changes in the standard massic enthalpies of reaction Delta H-r(w)degrees*, the standard massic entropies of reaction Delta S-r(w)degrees*, the standard massic Gibbs free energies of reaction Delta(r)G(w)degrees*, and the standard massic heat capacity Delta C-r(p,w)degrees, for the interconversion reactions of the pure (CI = 100) cellulose allomorphs, i.e., cellulose(am), cellulose I(cr), cellulose II(cr), and cellulose II(cr), at the temperature T = 298.15 K, the pressure p degrees = 0.1 MPa, and w(H2O) = 0.073. The "*"' denotes that the thermodynamic property pertains to pure cellulose allomorphs. Values of standard massic enthalpy differences Delta H-T(0)w degrees, standard massic entropy differences Delta S-T(0)w degrees, and the standard massic thermal function Phi(w)degrees = Delta S-T(0)w degrees - Delta H-T(0)w degrees/T were calculated from the measured heat capacities for the cellulose samples and for the pure cellulose allomorphs. The extensive literature pertinent to the thermodynamic properties of cellulose has been summarized and, in many cases, property values have been calculated or recalculated from previously reported data. The thermodynamic property data show that cellulose(am) is the least stable of the cellulose allomorphs considered in this study. However, due to the uncertainties in the measured property values, it is not possible to use these values to order the relative stabilities of the cellulose (I, II, and III) crystalline allomorphs with a reasonable degree of certainty. Nevertheless, based on chemical reactivity information, the qualitative order of stability for these three allomorphs is cellulose III(cr) > cellulose II(cr) > cellulose I beta(cr) at T = 298.15 K. However, as evidenced by the fact that cellulose I(cr) can be reformed by the application of heat and water to a sample of cellulose III(cr), the differences in the stabilities of these three allomorphs appear to be small and may be temperature dependent. Standard thermodynamic formation properties as well as property values for the conversion reactions of the cellulose allomorphs to alpha-D-glucose(cr) have been calculated on the assumption that S-w degrees -> 0 as T -> 0. The values for the standard massic Gibbs free energy of reaction Delta(r)G(w)degrees for the conversion of the cellulose allomorphs to alpha-D-glucose(cr), with the exception of anhydrous cellulose(am), all have positive values and thus are thermodynamically not favored for mass fractions of water w(H2O) < 0.073. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Goldberg, Robert N.; Urbas, Aaron; Lang, Brian E.] Natl Inst Stand & Technol, Biosyst & Biomat Div, Gaithersburg, MD 20899 USA. [Schliesser, Jacob; Woodfield, Brian F.] Brigham Young Univ, Dept Chem & Biochem, Provo, UT 84602 USA. [Mittal, Ashutosh; Decker, Stephen R.; Katahira, Rui; Wang, Wei; Johnson, David K.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Santos, Ana Filipa L. O. M.; Freitas, Vera L. S.; da Silva, Maria D. M. C. Ribeiro] Univ Porto, Fac Sci, Ctr Invest Quim, Dept Chem & Biochem, P-4169007 Oporto, Portugal. [Heiss, Christian] Univ Georgia, Complex Carbohydrate Res Ctr, Athens, GA 30602 USA. RP Goldberg, RN (reprint author), Natl Inst Stand & Technol, Biosyst & Biomat Div, Gaithersburg, MD 20899 USA. EM robert.goldberg@nist.gov; jacob_schliesser@me.com; ashutosh.mittal@nrel.gov; steve.decker@nrel.gov; ana.santos@fc.up.pt; vera.freitas@fc.up.pt; aaron.urbas@nist.gov; brian.lang@nist.gov; cheiss@ccrc.uga.edu; mdsilva@fc.up.pt; brian_woodfield@byu.edu; rui.katahira@nist.gov; wei.wang@nrel.gov; david.johnson@nrel.gov RI Ribeiro da Silva, Maria/N-4255-2013; Freitas, Vera/M-9108-2013 OI Ribeiro da Silva, Maria/0000-0003-0482-0308; Freitas, Vera/0000-0002-3670-2595 FU Fundacao para a Ciencia e Tecnologia (FCT), Lisbon, Portugal; FEDER; Centro de Investigacao em Quimica da Universidade do Porto [PEst-C/QUI/UI0081/2013]; FCT; European Social Fund (ESF) under the Community [SFRH/BPD/41601/2007, SFRH/BPD/78552/2011]; US Department of Energy [DE-AC36- 08GO28308]; National Renewable Energy Laboratory [AEV-2-22205-01]; DOE Office of Energy Efficiency and Renewable Energy, Bioenergy Technologies Office FX We thank Professor Julie Boerio-Goates for providing her fit for the heat capacity of hexagonal ice, Drs. Bruce Coxon and Katrice Lippa for their consultations on the NMR experiments, Drs. Gregg Beckham and Mike Crowley for their helpful discussions and comments on the manuscript, and Drs. Vytas Reipa and Alfons Weber for their help with the foreign language publications. Thanks are also due to Fundacao para a Ciencia e Tecnologia (FCT), Lisbon, Portugal and to FEDER for financial support given to Centro de Investigacao em Quimica da Universidade do Porto (PEst-C/QUI/UI0081/2013). A.F.L.O.M.S and V.L.S.F. thank FCT and The European Social Fund (ESF) under the Community Support Framework (CSF) for the award of the post-doctoral grants SFRH/BPD/41601/2007 and SFRH/BPD/78552/2011, respectively. This work was supported, in part, by the US Department of Energy under contract No. DE-AC36- 08GO28308 and sub-contract No. AEV-2-22205-01 with the National Renewable Energy Laboratory. Funding for the aforementioned contracts was provided by the DOE Office of Energy Efficiency and Renewable Energy, Bioenergy Technologies Office. NR 115 TC 11 Z9 11 U1 5 U2 57 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0021-9614 EI 1096-3626 J9 J CHEM THERMODYN JI J. Chem. Thermodyn. PD FEB PY 2015 VL 81 BP 184 EP 226 DI 10.1016/j.jct.2014.09.006 PG 43 WC Thermodynamics; Chemistry, Physical SC Thermodynamics; Chemistry GA AT9NL UT WOS:000345253800022 ER PT J AU Patra, A Balasubrahmaniyam, M Laha, R Malar, P Osipowicz, T Manivannan, A Kasiviswanathan, S AF Patra, Anuradha Balasubrahmaniyam, M. Laha, Ranjit Malar, P. Osipowicz, T. Manivannan, A. Kasiviswanathan, S. TI Localized Surface Plasmon Resonance in Au Nanoparticles Embedded dc Sputtered ZnO Thin Films SO JOURNAL OF NANOSCIENCE AND NANOTECHNOLOGY LA English DT Article DE Surface Plasmon Resonance; Optical Absorption; Gold Nanoparticles; ZnO Thin Films; Window Coatings ID RUTHERFORD BACKSCATTERING SPECTROMETRY AB The plasmonic behavior of metallic nanoparticles is explicitly dependent on their shape, size and the surrounding dielectric space. This study encompasses the influence of ZnO matrix, morphology of Au nanoparticles (AuNPs) and their organization on the optical behavior of ZnO/AuNPs-ZnO/ZnO/GP structures (GP: glass plate). These structures have been grown by a multiple-step physical process, which includes dc sputtering, thermal evaporation and thermal annealing. Different analytical techniques such as scanning electron microscopy, glancing angle X-ray diffraction, Rutherford backscattering spectrometry and optical absorption have been used to study the structures. In-situ rapid thermal treatment during dc sputtering of ZnO film has been found to induce subtle changes in the morphology of AuNPs, thereby altering the profile of the plasmon band in the absorption spectra. The results have been contrasted with a recent study on the spectral response of dc magnetron sputtered ZnO films embedded with AuNPs. Initial simulation results indicate that AuNPs ZnO/Au/GP structure reflects/absorbs UV and infrared radiations, and therefore can serve as window coatings. C1 [Patra, Anuradha; Balasubrahmaniyam, M.; Laha, Ranjit; Kasiviswanathan, S.] Indian Inst Technol, Dept Phys, Madras 600036, Tamil Nadu, India. [Malar, P.; Osipowicz, T.] Natl Univ Singapore, Ctr Ion Beam Applicat, Singapore 119260, Singapore. [Manivannan, A.] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. RP Kasiviswanathan, S (reprint author), Indian Inst Technol, Dept Phys, Madras 600036, Tamil Nadu, India. RI Osipowicz, Thomas/G-1365-2012 NR 24 TC 2 Z9 2 U1 0 U2 37 PU AMER SCIENTIFIC PUBLISHERS PI VALENCIA PA 26650 THE OLD RD, STE 208, VALENCIA, CA 91381-0751 USA SN 1533-4880 EI 1533-4899 J9 J NANOSCI NANOTECHNO JI J. Nanosci. Nanotechnol. PD FEB PY 2015 VL 15 IS 2 BP 1805 EP 1814 DI 10.1166/jnn.2015.9045 PG 10 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AT6NB UT WOS:000345054100139 PM 26353736 ER PT J AU Bolon, AM Sisneros, TA Schubert, AB Clausen, B Brown, DW Gentleman, MM AF Bolon, Amy M. Sisneros, Thomas A. Schubert, Amanda B. Clausen, Bjorn Brown, Donald W. Gentleman, Molly M. TI Comparison of neutron diffraction and Raman spectroscopic studies of the ferroelastic behavior of ceria-stabilized zirconia at elevated temperatures SO JOURNAL OF THE EUROPEAN CERAMIC SOCIETY LA English DT Article DE Ferroelastic switching; Raman spectroscopy; Thermal barrier coatings ID THERMAL BARRIER COATINGS; TETRAGONAL ZIRCONIA; TRANSFORMATION; POLYCRYSTALS; TOUGHNESS; MECHANISM; EVOLUTION; CERAMICS; SYSTEM AB Measurements of coercive stress for ferroelastic switching were made for 18-mol% ceria-stabilized zirconia under compressive loading using both neutron diffraction and Raman spectroscopy to validate the accuracy of those made by Raman against standard neutron diffraction measurements. Good agreement was observed between the two techniques and as a result, Raman scattering was identified as an effective technique for measuring coercive stresses in ferroelastic ceramics. In addition to absolute measurements in coercive stress, it was confirmed that coercive stress remains invariant in neutron diffraction measurements ranging from room temperature to 1200 degrees C. This suggests measurements of coercive stress measured using Raman spectroscopic techniques at room temperature are relevant to toughening mechanisms active at turbine operating conditions. Published by Elsevier Ltd. C1 [Bolon, Amy M.; Schubert, Amanda B.; Gentleman, Molly M.] Texas A&M Univ, Dept Mech Engn, TAMU 3123, College Stn, TX 77843 USA. [Sisneros, Thomas A.; Clausen, Bjorn; Brown, Donald W.] Los Alamos Neutron Sci Ctr, Los Alamos, NM USA. RP Gentleman, MM (reprint author), SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11794 USA. EM tsisneros@lanl.gov; Amanda.schubert@stonybrook.edu; clausen@lanl.gov; dbrown@lanl.gov; molly.gentleman@stonybrook.edu RI Clausen, Bjorn/B-3618-2015 OI Clausen, Bjorn/0000-0003-3906-846X NR 23 TC 0 Z9 0 U1 3 U2 33 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0955-2219 EI 1873-619X J9 J EUR CERAM SOC JI J. Eur. Ceram. Soc. PD FEB PY 2015 VL 35 IS 2 BP 623 EP 629 DI 10.1016/j.jeurceramsoc.2014.09.013 PG 7 WC Materials Science, Ceramics SC Materials Science GA AT8SG UT WOS:000345201700020 ER PT J AU Surowiec, M Custelcean, R Surowiec, K Bartsch, RA AF Surowiec, Malgorzata Custelcean, Radu Surowiec, Kazimierz Bartsch, Richard A. TI Alkali metal cation complexation by 1,3-alternate, mono-ionisable calix[4]arene-benzocrown-6 compounds SO SUPRAMOLECULAR CHEMISTRY LA English DT Article DE calixcrown ligand; caesium-selective extractant; alkali metal cation extraction; crown ether ID EXTRACTION; CESIUM AB Alkali metal cation extraction behaviour for two series of 1,3-alternate, mono-ionisable calix[4]arene-benzocrown-6 compounds is examined. In Series 1, the proton-ionisable group (PIG) is a substituent on the benzo group of the polyether ring that directs it away from the crown ether cavity. In Series 2, the PIG is attached to one para position in the calixarene framework, thereby positioning it over the crown ether ring. Competitive solvent extraction of alkali metal cations from aqueous solutions into chloroform shows high Cs+ efficiency and selectivity. Single-species extraction pH profiles of Cs+ for Series 1 and 2 ligands with the same PIG are very similar. Thus, association of Cs+ with the calixcrown ring is more important than the position of the PIG relative to the crown ether cavity. Solid-state structures of two unionised ligands from Series 2 are presented. Also described is a crystal containing two different ionised ligand-Cs+ complexes. C1 [Surowiec, Malgorzata; Surowiec, Kazimierz; Bartsch, Richard A.] Texas Tech Univ, Dept Chem & Biochem, Lubbock, TX 79409 USA. [Custelcean, Radu] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Bartsch, RA (reprint author), Texas Tech Univ, Dept Chem & Biochem, Lubbock, TX 79409 USA. EM richard.bartsch@ttu.edu RI Custelcean, Radu/C-1037-2009 OI Custelcean, Radu/0000-0002-0727-7972 FU Office of Biological and Environmental Research of the US Department of Energy [FG02-03ER63676]; Environmental Management Science Program of the Offices of Science and Environmental Management of the US Department of Energy [DE-AC5-00R22725] FX This research was supported at TTU by the Office of Biological and Environmental Research of the US Department of Energy [grant number FG02-03ER63676]. The research contribution of RC at ORNL was supported by the Environmental Management Science Program of the Offices of Science and Environmental Management of the US Department of Energy (contract number DE-AC5-00R22725). NR 14 TC 1 Z9 1 U1 3 U2 41 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 1061-0278 EI 1029-0478 J9 SUPRAMOL CHEM JI Supramol. Chem. PD FEB 1 PY 2015 VL 27 IS 1-2 BP 59 EP 64 DI 10.1080/10610278.2014.904869 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA AT7SQ UT WOS:000345138000009 ER PT J AU Auvray, X Partridge, W Choi, JS Pihl, J Coehlo, F Yezerets, A Kamasamudram, K Currier, N Olsson, L AF Auvray, Xavier Partridge, William Choi, Jae-Soon Pihl, Josh Coehlo, Filipa Yezerets, Aleksey Kamasamudram, Krishna Currier, Neal Olsson, Louise TI Kinetic modeling of NH3-SCR over a supported Cu zeolite catalyst using axial species distribution measurements SO APPLIED CATALYSIS B-ENVIRONMENTAL LA English DT Article DE NH3 SCR; Kinetic modeling; Spatial distribution measurements; Cu zeolites; Spaci-MS ID STORAGE-REDUCTION CATALYST; NOX STORAGE; NH3 SCR; CU-ZSM-5; AMMONIA; ADSORPTION; FE; REGENERATION; OXIDATION; FE-ZSM5 AB In this study, a kinetic model is developed for NH3-SCR over a honeycomb-monolith-supported Cu-zeolites using intra-catalyst axial species distribution measurements. An ammonia TPD experiment, together with micro calorimetry data were used for tuning the ammonia adsorption and desorption properties. The spatial distribution for NO oxidation, NH3 oxidation and NH3 "Standard" SCR were modeled between 200 and 400 degrees C. Four-step protocol measurements were employed in order to validate the transient functions of the model. The resulting kinetic model provides good spatiotemporal simulation of the SCR reaction and component reactions throughout the monolith catalyst system. (C) 2014 Elsevier B.V. All rights reserved. C1 [Auvray, Xavier; Coehlo, Filipa; Olsson, Louise] Chalmers, Competence Ctr Catalysis, S-41296 Gothenburg, Sweden. [Partridge, William; Choi, Jae-Soon; Pihl, Josh] Oak Ridge Natl Lab, Fuels Engines & Emiss Res Ctr, Oak Ridge, TN 37831 USA. [Yezerets, Aleksey; Kamasamudram, Krishna; Currier, Neal] Cummins Inc, Columbus, IN 47201 USA. RP Olsson, L (reprint author), Chalmers, Competence Ctr Catalysis, S-41296 Gothenburg, Sweden. EM louise.olsson@chalmers.se OI Choi, Jae-Soon/0000-0002-8162-4207 FU U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Office; Swedish Foundation for Strategic Research [F06-0006]; U.S. Department of Energy [DE-AC05-00OR22725] FX This work is a collaboration between Oak Ridge National Laboratory, Competence Centre for Catalysis at Chalmers University and Cummins Inc. This research was sponsored by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Office, with Ken Howden and Gurpreet Singh as the Program Managers and the Swedish Foundation for Strategic Research (F06-0006).; Notice: This manuscript has been authored by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 37 TC 6 Z9 6 U1 6 U2 105 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0926-3373 EI 1873-3883 J9 APPL CATAL B-ENVIRON JI Appl. Catal. B-Environ. PD FEB PY 2015 VL 163 BP 393 EP 403 DI 10.1016/j.apcatb.2014.08.003 PG 11 WC Chemistry, Physical; Engineering, Environmental; Engineering, Chemical SC Chemistry; Engineering GA AR5GG UT WOS:000343612500044 ER PT J AU Olalla, C Deline, C Clement, D Levron, Y Rodriguez, M Maksimovic, D AF Olalla, Carlos Deline, Christopher Clement, Daniel Levron, Yoash Rodriguez, Miguel Maksimovic, Dragan TI Performance of Power-Limited Differential Power Processing Architectures in Mismatched PV Systems SO IEEE TRANSACTIONS ON POWER ELECTRONICS LA English DT Article DE Aging; dc-dc converters; differential power processing (DPP); equalization; mismatch; partial shading; photovoltaic modules; submodule-integrated converters (subMICs) ID PHOTOVOLTAIC APPLICATIONS; CONVERTERS; MODULE AB Differential power processing (DPP) architectures employ distributed, low power processing, submodule-integrated converters to mitigate mismatches in photovoltaic (PV) power systems, while introducing no insertion losses. This paper evaluates the effects of the simple voltage-balancing DPP control approach on the submodule-level maximum power point (MPP) efficiency. It is shown that the submodule MPP efficiency of voltage-balancing DPP converters exceeds 98% in the presence of worst-case MPP voltage variations due to irradiance or temperature mismatches. Furthermore, the effects of reduced converter power rating in the isolated-portDPP architecture are investigated by long-term, high-granularity simulations of five representative PV system scenarios. For partially shaded systems, it is shown that the isolated-port DPP architecture offers about two times larger energy yield improvements compared to full power processing (FPP) module-level converters, and that it outperforms module-level FPP approaches even when the power rating of DPP converters is only 20-30% of the PV system peak power. In the cases of aging-related mismatches, more than 90% of the energy yield improvements are obtained with DPP converters rated at only 10% of the PV peak power. C1 [Olalla, Carlos] Univ Rovira & Virgili, Dept Elect Elect & Automat Control Engn, E-43007 Tarragona, Spain. [Deline, Christopher] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Clement, Daniel; Levron, Yoash; Rodriguez, Miguel; Maksimovic, Dragan] Univ Colorado, Dept Elect Comp & Energy Engn, Boulder, CO 80309 USA. RP Olalla, C (reprint author), Univ Rovira & Virgili, Dept Elect Elect & Automat Control Engn, E-43007 Tarragona, Spain. EM carlos.olalla@urv.cat; chris.deline@nrel.gov; Daniel.Clement@colorado.edu; yoashlevron@gmail.com; miguel.rodriguez@colorado.edu; maksimov@colorado.edu RI Olalla, Carlos/A-8571-2012 OI Olalla, Carlos/0000-0001-8333-9840 FU Advanced Research Projects Agency-Energy, an agency of the United States Government, U.S. Department of Energy [DE-AR0000216]; Generalitat de Catalunya, Beatriu de Pinos programme [BP-B00047] FX This work was supported in part by the Advanced Research Projects Agency-Energy, an agency of the United States Government, U.S. Department of Energy, under Award DE-AR0000216. The work of C. Olalla was supported in part by the Generalitat de Catalunya, Beatriu de Pinos programme under Award BP-B00047. Recommended for publication by Associate Editor C. A. Canesin. NR 27 TC 26 Z9 26 U1 0 U2 16 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8993 EI 1941-0107 J9 IEEE T POWER ELECTR JI IEEE Trans. Power Electron. PD FEB PY 2015 VL 30 IS 2 BP 618 EP 631 DI 10.1109/TPEL.2014.2312980 PG 14 WC Engineering, Electrical & Electronic SC Engineering GA AQ8AA UT WOS:000343041300012 ER PT J AU Chapman, JA Mascher, M Buluc, A Barry, K Georganas, E Session, A Strnadova, V Jenkins, J Sehgal, S Oliker, L Schmutz, J Yelick, KA Scholz, U Waugh, R Poland, JA Muehlbauer, GJ Stein, N Rokhsar, DS AF Chapman, Jarrod A. Mascher, Martin Buluc, Aydin Barry, Kerrie Georganas, Evangelos Session, Adam Strnadova, Veronika Jenkins, Jerry Sehgal, Sunish Oliker, Leonid Schmutz, Jeremy Yelick, Katherine A. Scholz, Uwe Waugh, Robbie Poland, Jesse A. Muehlbauer, Gary J. Stein, Nils Rokhsar, Daniel S. TI A whole-genome shotgun approach for assembling and anchoring the hexaploid bread wheat genome SO GENOME BIOLOGY LA English DT Article ID COPY NUMBER VARIATION; AEGILOPS-TAUSCHII; PHYSICAL MAP; SEQUENCING DATA; DRAFT GENOME; HIGH-DENSITY; BARLEY; NUCLEOTIDE; DIVERSITY; EVOLUTION AB Polyploid species have long been thought to be recalcitrant to whole-genome assembly. By combining high-throughput sequencing, recent developments in parallel computing, and genetic mapping, we derive, de novo, a sequence assembly representing 9.1 Gbp of the highly repetitive 16 Gbp genome of hexaploid wheat, Triticum aestivum, and assign 7.1 Gb of this assembly to chromosomal locations. The genome representation and accuracy of our assembly is comparable or even exceeds that of a chromosome-by-chromosome shotgun assembly. Our assembly and mapping strategy uses only short read sequencing technology and is applicable to any species where it is possible to construct a mapping population. C1 [Chapman, Jarrod A.; Barry, Kerrie; Jenkins, Jerry; Schmutz, Jeremy; Rokhsar, Daniel S.] Joint Genome Inst, Dept Energy, Walnut Creek, CA 94598 USA. [Mascher, Martin; Scholz, Uwe; Stein, Nils] Leibniz Inst Plant Genet, D-06466 Stadt Seeland, Germany. [Mascher, Martin; Scholz, Uwe; Stein, Nils] Crop Plant Res IPK Gatersleben, D-06466 Stadt Seeland, Germany. [Buluc, Aydin; Barry, Kerrie; Georganas, Evangelos; Oliker, Leonid; Yelick, Katherine A.] Computat Res Div, Berkeley, CA 94720 USA. [Buluc, Aydin; Georganas, Evangelos; Oliker, Leonid; Yelick, Katherine A.] NERSC, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Georganas, Evangelos; Yelick, Katherine A.] Univ Calif Berkeley, Div Comp Sci, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. [Session, Adam; Rokhsar, Daniel S.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Strnadova, Veronika] Univ Calif Santa Barbara, Dept Comp Sci, Santa Barbara, CA 93106 USA. [Schmutz, Jeremy] HudsonAlpha Inst Biotechnol, Huntsville, AL 35806 USA. [Sehgal, Sunish] Kansas State Univ, Dept Plant Pathol, Manhattan, KS 66506 USA. [Waugh, Robbie] Univ Dundee & James Hutton Inst, Div Plant Sci, Dundee DD2 5DA, Scotland. [Muehlbauer, Gary J.] Univ Minnesota, Dept Agron & Plant Genet, St Paul, MN 55108 USA. [Muehlbauer, Gary J.] Univ Minnesota, Dept Plant Biol, St Paul, MN 55108 USA. RP Rokhsar, DS (reprint author), Joint Genome Inst, Dept Energy, 2800 Mitchell Dr, Walnut Creek, CA 94598 USA. EM dsrokhsar@gmail.com OI Scholz, Uwe/0000-0001-6113-3518; Poland, Jesse/0000-0002-7856-1399 FU Office of Science of the US Department of Energy [DE-AC02-05CH11231]; Triticeae Coordinated Agricultural Project, US Department of Agriculture/National Institute for Food and Agriculture [2011-68002-30029]; Kansas Wheat Commission; Kansas Wheat Alliance; Bill and Melinda Gates Foundation; US National Science Foundation; USAID; Scottish Government Rural and Environment Science and Analytical Services Division; BBSRC grant [BB/I00663X/1]; Bundesministerium fur Bildung und Forschung Plant program [TRITEX 0315954, NUGGET 0315957A]; US DOE [DE-SC0008700]; NHGRI Berkeley Training Grant in Genomics FX The work performed by the US Department of Energy Joint Genome Institute is supported by the Office of Science of the US Department of Energy under contract number DE-AC02- 05CH11231. The authors would also like to acknowledge the support given by funds received from the Triticeae Coordinated Agricultural Project, US Department of Agriculture/National Institute for Food and Agriculture grant number 2011-68002-30029 to GJM and JAP, the Kansas Wheat Commission, Kansas Wheat Alliance, The Bill and Melinda Gates Foundation, US National Science Foundation, and USAID to JAP, the Scottish Government Rural and Environment Science and Analytical Services Division and BBSRC grant number BB/I00663X/1 to RW, and the Bundesministerium fur Bildung und Forschung Plant2030 program (TRITEX 0315954, NUGGET 0315957A) to NS and US Research at the Computational Research Division/Lawrence Berkeley National Laboratory is supported in part by the Department of Energy, Office of Science, contract number DE-AC02-05CH11231. This work used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy under contract DE-AC02-05CH11231. EG acknowledges the support of the US DOE grant DE-SC0008700. AS acknowledges support from the NHGRI Berkeley Training Grant in Genomics. We thank Lisa Borello for helpful comments on the manuscript. We are grateful to Doreen Stengel, Daniel Arend and Matthias Lange for help with data submission. We thank the International Wheat Genome Sequencing Consortium for making their chromosome-by-chromosome shotgun assemblies available prior to publication. NR 69 TC 45 Z9 47 U1 4 U2 40 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1465-6906 EI 1474-760X J9 GENOME BIOL JI Genome Biol. PD JAN 31 PY 2015 VL 16 AR UNSP 26 DI 10.1186/s13059-015-0582-8 PG 17 WC Biotechnology & Applied Microbiology; Genetics & Heredity SC Biotechnology & Applied Microbiology; Genetics & Heredity GA CE4RQ UT WOS:000351818200001 PM 25637298 ER PT J AU Kong, T Bud'ko, SL Canfield, PC AF Kong, Tai Bud'ko, Sergey L. Canfield, Paul C. TI Anisotropic H-c2, thermodynamic and transport measurements, and pressure dependence of T-c in K2Cr3As3 single crystals SO PHYSICAL REVIEW B LA English DT Article ID SUPERCONDUCTORS; FIELD AB We present a detailed study of single crystalline K2Cr3As3 and analyze its thermodynamic and transport properties, anisotropic H-c2(T), and initial pressure dependence of T-c. In zero field, the temperature-dependent resistivity is metallic. Deviation from a linear temperature dependence is evident below100Kand a T-3 dependence is roughly followed from just above T-c (similar to 10 K) to similar to 40 K. Anisotropic H-c2(T) data were measured up to 140 kOe with field applied along and perpendicular to the rodlike crystals. For the applied field perpendicular to the rod, H-c2(T) is linear with a slope similar to-70 kOe/K. For field applied along the rod, the slope is about -120 kOe/K below 70 kOe. Above 70 kOe, the magnitude of the slope decreases to similar to-70 kOe/K. The electronic specific heat coefficient gamma, just above T-c, is 73 mJ/mol K-2; the Debye temperature Theta(D) is 220 K. The specific heat jump at the superconducting transition Delta C similar to 2.2 gamma T-c. Finally, for hydrostatic pressures up to similar to 7 kbar, T-c decreases under pressure linearly at a rate of -0.034K/kbar. C1 [Kong, Tai] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Kong, T (reprint author), Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. OI Kong, Tai/0000-0002-5064-3464 FU US Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; US DOE [DE-AC02-07CH11358] FX We would like to thank U. S. Kaluarachchi, A. E. Bohmer, D. K. Finnemore, V. G. Kogan, and V. Taufour for useful discussions. This work was supported by the US Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. The research was performed at the Ames Laboratory, which is operated for the US DOE by Iowa State University under Contract NO. DE-AC02-07CH11358. NR 15 TC 29 Z9 29 U1 7 U2 39 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 30 PY 2015 VL 91 IS 2 AR 020507 DI 10.1103/PhysRevB.91.020507 PG 5 WC Physics, Condensed Matter SC Physics GA CD6RR UT WOS:000351217400002 ER PT J AU Ovchinnikov, YN Varlamov, AA AF Ovchinnikov, Yu. N. Varlamov, A. A. TI Phase slips in a current-biased narrow superconducting strip SO PHYSICAL REVIEW B LA English DT Article ID GINZBURG-LANDAU EQUATIONS AB The theory of current transport in a narrow superconducting strip is revisited taking the effect of thermal fluctuations into account. The value of voltage drop across the sample is found as a function of temperature (close to the transition temperature, T - T-c << T-c) and bias current J < J(c) (J(c) is the critical current calculated in the framework of the BCS approximation, neglecting thermal fluctuations). It is shown that careful analysis of vortices crossing the strip results in considerable increase of the activation energy. C1 [Ovchinnikov, Yu. N.] Max Plank Inst Phys Complex Syst, D-01187 Dresden, Germany. [Ovchinnikov, Yu. N.] RAS, Landau Inst Theoret Phys, Chernogolovka 142432, Moscow District, Russia. [Varlamov, A. A.] CNR SPIN, I-00133 Rome, Italy. [Varlamov, A. A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60639 USA. RP Ovchinnikov, YN (reprint author), Max Plank Inst Phys Complex Syst, D-01187 Dresden, Germany. FU FP7-IRSES program SIMTECH [236947]; U.S. Department of Energy, Office of Science, Office of Advanced Scientific Computing Research and Materials Sciences and Engineering Division, Scientific Discovery through Advanced Computing program FX The authors acknowledge financial support from the FP7-IRSES program SIMTECH, Grant No. 236947. A.V. was partially supported by the U.S. Department of Energy, Office of Science, Office of Advanced Scientific Computing Research and Materials Sciences and Engineering Division, Scientific Discovery through Advanced Computing program. A. V. is grateful to I. Aronson, A. Bezryadin, and A. Glatz for valuable discussions. NR 15 TC 2 Z9 2 U1 0 U2 26 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 30 PY 2015 VL 91 IS 1 AR 014514 DI 10.1103/PhysRevB.91.014514 PG 9 WC Physics, Condensed Matter SC Physics GA CD6RL UT WOS:000351216700005 ER PT J AU Quintero, PA Rajan, D Peprah, MK Brinzari, TV Fishman, RS Talham, DR Meisel, MW AF Quintero, P. A. Rajan, D. Peprah, M. K. Brinzari, T. V. Fishman, R. S. Talham, D. R. Meisel, M. W. TI Pressure-induced enhancement of the magnetic anisotropy in Mn(N(CN)(2))(2) SO PHYSICAL REVIEW B LA English DT Article ID DICYANAMIDE ANION; WEAK FERROMAGNET; EXCHANGE BIAS; BEHAVIOR AB Using dc and ac magnetometry, the pressure dependence of the magnetization of the three- dimensional antiferromagnetic coordination polymer Mn(N(CN)(2))(2) was studied up to 12 kbar and down to 8 K. The antiferromagnetic transition temperature, T-N, increases dramatically with applied pressure (P), where a change from T-N(P = ambient) = 16.0 K to T-N(P = 12.1 kbar) = 23.5 K was observed. In addition, a marked difference in the magnetic behavior is observed above and below 7.1 kbar. Specifically, for P < 7.1 kbar, the differences between the field-cooled and zero-field-cooled magnetizations, the coercive field, and the remanent magnetization decrease with increasing pressure. However, for P > 7.1 kbar, the behavior is inverted. Additionally, for P > 8.6 kbar, minor hysteresis loops are observed. All of these effects are evidence of the increase of the superexchange interaction and the appearance of an enhanced exchange anisotropy with applied pressure. C1 [Quintero, P. A.; Peprah, M. K.; Brinzari, T. V.; Meisel, M. W.] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. [Quintero, P. A.; Peprah, M. K.; Brinzari, T. V.; Meisel, M. W.] Univ Florida, Natl High Magnet Field Lab, Gainesville, FL 32611 USA. [Rajan, D.; Talham, D. R.] Univ Florida, Dept Chem, Gainesville, FL 32611 USA. [Fishman, R. S.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Quintero, PA (reprint author), Univ Florida, Dept Phys, Gainesville, FL 32611 USA. FU NSF [DMR-1202033, DMR-1405439, DMR-1157490]; Office of Science, Materials Sciences and Engineering Division, Office of Basic Energy Sciences, US Department of Energy FX This work is supported, in part, by NSF Grants No. DMR-1202033 (M.W.M.), No. DMR-1405439 (D.R.T.), and No. DMR-1157490 (NHMFL). Research by R.S.F. is sponsored by the Office of Science, Materials Sciences and Engineering Division, Office of Basic Energy Sciences, US Department of Energy. We gratefully acknowledge enlightening conversations with Jamie L. Manson and Janice L. Musfeldt. NR 28 TC 5 Z9 5 U1 4 U2 36 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 30 PY 2015 VL 91 IS 1 AR 014439 DI 10.1103/PhysRevB.91.014439 PG 7 WC Physics, Condensed Matter SC Physics GA CD6RL UT WOS:000351216700003 ER PT J AU Vlasko-Vlasov, V Koshelev, A Glatz, A Phillips, C Welp, U Kwok, W AF Vlasko-Vlasov, V. Koshelev, A. Glatz, A. Phillips, C. Welp, U. Kwok, W. TI Flux cutting in high-T-c superconductors SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTORS; CRITICAL-STATE MODEL; II SUPERCONDUCTORS; MAGNETIC-FIELD; LAYERED SUPERCONDUCTORS; HARD SUPERCONDUCTORS; TRANSPORT CURRENTS; MEISSNER HOLES; VORTEX SHAKING; LINE AB We performed a magneto-optical study of flux distributions in yttrium barium copper oxide (YBCO) crystal under various applied crossed field orientations to elucidate the complex nature of magnetic flux cutting in superconductors. Our work reveals unusual vortex patterns induced by the interplay between flux cutting and vortex pinning. We observe strong flux penetration anisotropy of the normal flux B-perpendicular to in the presence of an in-plane field H-parallel to and associate the modified flux dynamics with the staircase structure of tilted vortices in YBCO and the flux-cutting process. We demonstrate that flux cutting can effectively delay vortex entry in the direction transverse to H-parallel to. Finally, we elucidate details of the vortex cutting and reconnection process using time-dependent Ginzburg-Landau simulations. C1 [Vlasko-Vlasov, V.; Koshelev, A.; Glatz, A.; Phillips, C.; Welp, U.; Kwok, W.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Vlasko-Vlasov, V (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. FU U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division and Office of Advanced Scientific Computing Research, Scientific Discovery through Advanced Computing (SciDAC) program FX This work was supported by the U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division and Office of Advanced Scientific Computing Research, Scientific Discovery through Advanced Computing (SciDAC) program. NR 68 TC 7 Z9 7 U1 2 U2 32 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 30 PY 2015 VL 91 IS 1 DI 10.1103/PhysRevB.91.014516 PG 16 WC Physics, Condensed Matter SC Physics GA CD6RL UT WOS:000351216700007 ER PT J AU Siriwardane, R Tian, HJ Fisher, J AF Siriwardane, Ranjani Tian, Hanjing Fisher, James TI Production of pure hydrogen and synthesis gas with Cu-Fe oxygen carriers using combined processes of chemical looping combustion and methane decomposition/reforming SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Review DE Hydrogen production; Synthesis gas production; CuO-Fe2O3 oxides; Chemical looping; Methane reforming ID PARTIAL OXIDATION; CO2 CAPTURE; SYSTEM; GASIFICATION; GENERATION; UNIT; COAL AB Two processes for production of synthesis gas and pure hydrogen from methane using chemical looping were investigated using CuO-Fe2O3-alumina oxygen carriers. In the first process, CuO-Fe2O3 was initially reduced with methane and the reduced oxygen carrier was used as a catalyst for decomposition of methane to produce hydrogen; then the carbon formed during the methane decomposition was gasified with steam to produce synthesis gas. Methane chemical looping combustion with CuO-Fe2O3 oxygen carrier provides the heat for both the methane decomposition and carbon gasification reaction. In the second process, the reduced Cu-Fe oxygen carrier was used as a methane steam reforming catalyst to produce synthesis gas from steam and methane. Heat for the reforming reaction is provided by the methane chemical looping combustion reaction of the Cu-Fe oxygen carrier. Multiple-cycle tests of those process steps have been experimentally evaluated in a bench-scale flow reactor. Both processes use the same CuO-Fe2O3 oxide system, as an oxygen carrier for chemical looping combustion reactions and as a catalyst for methane decomposition and methane steam reforming reactions. Copyright (C) 2014, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Siriwardane, Ranjani; Tian, Hanjing; Fisher, James] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. [Tian, Hanjing] W Virginia Univ, Dept Chem Engn, Morgantown, WV 26505 USA. RP Siriwardane, R (reprint author), US DOE, Natl Energy Technol Lab, 3610 Collins Ferry Rd,POB 880, Morgantown, WV 26507 USA. EM ranjani.siriwardane@netl.doe.gov; Hanjing.tian@netl.doe.gov; James.fisher@netl.doe.gov NR 31 TC 15 Z9 15 U1 16 U2 84 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 EI 1879-3487 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD JAN 30 PY 2015 VL 40 IS 4 BP 1698 EP 1708 DI 10.1016/j.ijhydene.2014.11.090 PG 11 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA CA9UR UT WOS:000349270800008 ER PT J AU Zhou, NN Yang, C Tucker, D Pezzini, P Traverso, A AF Zhou, Nana Yang, Chen Tucker, David Pezzini, Paolo Traverso, Alberto TI Transfer function development for control of cathode airflow transients in fuel cell gas turbine hybrid systems SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Solid oxide fuel cell; Gas turbine; Hybrid system; Hardware-in-the-loop simulation; Transients; Transfer function ID PERFORMANCE; OPERATION AB Direct-fired fuel cell gas turbine hybrid power system responses to open-loop transients were evaluated using a hardware-based simulation of an integrated solid oxide fuel cell gas turbine (SOFC/GT) hybrid system, implemented through the Hybrid Performance (Hyper) facility at the U.S. Department of Energy, National Energy Technology Laboratory (NETL). A disturbance in the cathode inlet air mass flow was performed by manipulating a hot-air bypass valve implemented in the hardware component. Two tests were performed; the fuel cell stack subsystem numerical simulation model was both decoupled and fully coupled with the gas turbine hardware component. The dynamic responses of the entire SOFC/GT hybrid system were studied in this paper. The reduction of cathode airflow resulted in a sharp decrease and partial recovery of the fuel cell thermal effluent in 10 s. In contrast, the turbine rotational speed did not exhibit a similar trend. The transfer functions of several important variables in the fuel cell stack subsystem and gas turbine subsystem were developed to be used in the future control method development. The importance of the cathode airflow regulation was quantified through transfer functions. The management of cathode airflow was also suggested to be a potential strategy to increase the life of fuel cells by reducing the thermal impact of operational transients on the fuel cell subsystem. Copyright (C) 2014, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Zhou, Nana; Yang, Chen] Minist Educ, Key Lab Low Grade Energy Utilizat Technol & Syst, Chongqing 400030, Peoples R China. [Zhou, Nana; Yang, Chen] Chongqing Univ, Coll Power Engn, Chongqing 400030, Peoples R China. [Tucker, David; Pezzini, Paolo] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. [Traverso, Alberto] Univ Genoa, TPG DIME, I-16145 Genoa, Italy. RP Zhou, NN (reprint author), Chongqing Univ, Coll Power Engn, Chongqing 400030, Peoples R China. EM zhounana.cqu@gmail.com FU Crosscutting Research program implemented through the U.S. Department of Energy FX This work was funded by the Crosscutting Research program implemented through the U.S. Department of Energy, administered through the National Energy Technology Laboratory (NETL). The authors would like to express the gratitude to Nor Farida Harun for her effort in execution maintenance of the HyPer facility. NR 30 TC 5 Z9 5 U1 2 U2 10 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 EI 1879-3487 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD JAN 30 PY 2015 VL 40 IS 4 BP 1967 EP 1979 DI 10.1016/j.ijhydene.2014.11.107 PG 13 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA CA9UR UT WOS:000349270800038 ER PT J AU Wang, JJA Ren, F Tan, T Liu, K AF Wang, John Jy-An Ren, Fei Tan, Tin Liu, Ken TI The development of in situ fracture toughness evaluation techniques in hydrogen environment SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Welding; Hydrogen; Embrittlement; Fracture toughness; In situ testing; Torsion test AB Fracture toughness and fatigue properties of pipeline steels play a critical role in developing advanced high-pressure hydrogen infrastructure for alternative fuel pipelines program. The reliability of structure components, particularly resistance to damage and failure in the intended service environment, is highly dependent on the selected materials. An effective surveillance program is also necessary to monitor the material degradation during the course of service. Steels have been proven to be desirable for hydrogen infrastructure. However, hydrogen embrittlement is an important factor that limits steel performance under high-pressure hydrogen conditions. Furthermore, many conventional fracture testing techniques are difficult to be realized under the presence of hydrogen, in addition to the inherent specimen size effect. Thus it is desired to develop novel in situ fracture toughness evaluation techniques to study the fracture behavior of structural materials in hydrogen environments. In this study, a torsional fixture was developed to utilize Spiral Notch Torsion Test (SNTT) methodology. A fatigue pre-crack procedure of SNTT approach was also developed and demonstrated for weldment. The in situ testing results indicated that the exposure to H-2 significantly reduces the fracture toughness of 4340 high strength steels by up to 50 percent. Moreover, in-air simulated heat-affected zone specimen by Gleeble demonstrated a significant fracture toughness reduction of 75 percent in samples which illustrated the effect of welding on the fracture toughness. Copyright (C) 2014, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Wang, John Jy-An; Ren, Fei; Tan, Tin; Liu, Ken] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Wang, JJA (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM wangja@ornl.gov OI Wang, Jy-An/0000-0003-2402-3832 FU U.S. Department of Energy (DOE) [DE-AC05-00OR22725]; Oak Ridge National Laboratory Seed Money Program FX This project is sponsored by U.S. Department of Energy (DOE) and Oak Ridge National Laboratory Seed Money Program. Oak Ridge National Laboratory is managed by UT-Battelle, LLC for the U.S. Department of Energy under Contract DE-AC05-00OR22725. The authors also acknowledge Larry Anovitz, Hanbing Xu, Hao Jiang, Thomas Cox, Wei Zhang, and Zhili Feng for their contributions during the program development. NR 25 TC 4 Z9 4 U1 2 U2 21 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 EI 1879-3487 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD JAN 30 PY 2015 VL 40 IS 4 BP 2013 EP 2024 DI 10.1016/j.ijhydene.2014.11.147 PG 12 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA CA9UR UT WOS:000349270800042 ER PT J AU Nie, WY Tsai, HH Asadpour, R Blancon, JC Neukirch, AJ Gupta, G Crochet, JJ Chhowalla, M Tretiak, S Alam, MA Wang, HL Mohite, AD AF Nie, Wanyi Tsai, Hsinhan Asadpour, Reza Blancon, Jean-Christophe Neukirch, Amanda J. Gupta, Gautam Crochet, Jared J. Chhowalla, Manish Tretiak, Sergei Alam, Muhammad A. Wang, Hsing-Lin Mohite, Aditya D. TI High-efficiency solution-processed perovskite solar cells with millimeter-scale grains SO SCIENCE LA English DT Article ID HALIDE PEROVSKITES; DEPOSITION; RECOMBINATION; TEMPERATURE; HYSTERESIS; MORPHOLOGY; LENGTHS AB State-of-the-art photovoltaics use high-purity, large-area, wafer-scale single-crystalline semiconductors grown by sophisticated, high-temperature crystal growth processes. We demonstrate a solution-based hot-casting technique to grow continuous, pinhole-free thin films of organometallic perovskites with millimeter-scale crystalline grains. We fabricated planar solar cells with efficiencies approaching 18%, with little cell-to-cell variability. The devices show hysteresis-free photovoltaic response, which had been a fundamental bottleneck for the stable operation of perovskite devices. Characterization and modeling attribute the improved performance to reduced bulk defects and improved charge carrier mobility in large-grain devices. We anticipate that this technique will lead the field toward synthesis of wafer-scale crystalline perovskites, necessary for the fabrication of high-efficiency solar cells, and will be applicable to several other material systems plagued by polydispersity, defects, and grain boundary recombination in solution-processed thin films. C1 [Nie, Wanyi; Gupta, Gautam; Mohite, Aditya D.] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. [Tsai, Hsinhan; Blancon, Jean-Christophe; Crochet, Jared J.; Wang, Hsing-Lin] Los Alamos Natl Lab, Phys Chem & Appl Spect Div, Los Alamos, NM 87545 USA. [Asadpour, Reza; Alam, Muhammad A.] Purdue Univ, Sch Elect & Comp Engn, W Lafayette, IN 47907 USA. [Neukirch, Amanda J.; Tretiak, Sergei] Los Alamos Natl Lab, Theoret Chem & Mol Phys Div, Los Alamos, NM 87545 USA. [Neukirch, Amanda J.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Chhowalla, Manish] Rutgers State Univ, Piscataway, NJ 08854 USA. RP Mohite, AD (reprint author), Los Alamos Natl Lab, Mat Phys & Applicat Div, POB 1663, Los Alamos, NM 87545 USA. EM hwang@lanl.gov; amohite@lanl.gov RI Tretiak, Sergei/B-5556-2009; OI Tretiak, Sergei/0000-0001-5547-3647; Blancon, Jean-Christophe/0000-0002-3833-5792; Crochet, Jared/0000-0002-9570-2173 FU U.S. Department of Energy, Office of Basic Energy Sciences [08SPCE973]; LANL LORD program [XW11]; U.S. Department of Energy under DOE [DE-EE0004946] FX Work at Los Alamos National Laboratuy (LANL) was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Work Proposal 08SPCE973 (W.N., G.G., and. A.D.M.) and by We LANL LORD program XW11 (A.D.M., H.-L.W., and S.T.). This work was done in part at the Center for Integrated Nanotechnologies, an Office of Science User Facility. Work at Purdue University was supported by the U.S. Department of Energy under DOE Cooperative Agreement no. DE-EE0004946 ("PVMI Bay Area PV Consortium"). We thank C. Sheehan for the high-resolution cross-sectional SEM images. A.J.N. and S.T. thank C. Katan, J. Even, L. Pedesseatl, and M. Kepenekian for useful discussions as well as starting coordinates for bulk peeovskites. Author contributions: A.D.M. conceived the idea, designed and supervised experiments, analyzed data, and wrote the manuscript. H.-L.W. and H.T. designed the synthesis chemistry for perovskite thin-film growth and analyzed data. W.N. developed the hot-casting, slow-quenching method for large-area crystal growth along with H. I. and also performed device fabrication and solar cell testing, x-ray diffraction and analyzed the data. J.-C.B. performed optical spectroscopy measurements, analyzed the data under the supervision of J.J.C. R.A. performed device modeling simulations. conceived the device modeling, superyised the device modeling, analyzed crystal growth mechanisms, and co-wrote the paper. A.J.N. performed OFT calculations under the guida.nce of SI., who designed the OFT calculations, analyzed the data, and provided guidance to the project. G.G. and M.C. conceived the XRD measurements and analyzed the data, co-designed the experiments, and contributed to the organization of the manuscript. All authors have read the manuscript and agree to its contents. NR 31 TC 682 Z9 694 U1 232 U2 1248 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JAN 30 PY 2015 VL 347 IS 6221 BP 522 EP 525 DI 10.1126/science.aaa0472 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CA0YK UT WOS:000348639300046 PM 25635093 ER PT J AU Guo, YZ Kalathur, RC Liu, Q Kloss, B Bruni, R Ginter, C Kloppmann, E Rost, B Hendrickson, WA AF Guo, Youzhong Kalathur, Ravi C. Liu, Qun Kloss, Brian Bruni, Renato Ginter, Christopher Kloppmann, Edda Rost, Burkhard Hendrickson, Wayne A. TI Structure and activity of tryptophan-rich TSPO proteins SO SCIENCE LA English DT Article ID MITOCHONDRIAL TRANSLOCATOR PROTEIN; BENZODIAZEPINE-RECEPTOR; 18 KDA; PROTOPORPHYRIN-IX; IN-VIVO; BINDING-AFFINITY; PET RADIOLIGAND; STEROIDOGENESIS; BIOSYNTHESIS; PORPHYRINS AB Translocator proteins (TSPOs) bind steroids and porphyrins, and they are implicated in many human diseases, for which they serve as biomarkers and therapeutic targets. TSPOs have tryptophan-rich sequences that are highly conserved from bacteria to mammals. Here we report crystal structures for Bacillus cereus TSPO (BcTSPO) down to 1.7 angstrom resolution, including a complex with the benzodiazepine-like inhibitor PK11195. We also describe BcTSPO-mediated protoporphyrin IX (PpIX) reactions, including catalytic degradation to a previously undescribed heme derivative. We used structure-inspired mutations to investigate reaction mechanisms, and we showed that TSPOs from Xenopus and man have similar PpIX-directed activities. Although TSPOs have been regarded as transporters, the catalytic activity in PpIX degradation suggests physiological importance for TSPOs in protection against oxidative stress. C1 [Guo, Youzhong; Hendrickson, Wayne A.] Columbia Univ, Dept Biochem & Mol Biophys, New York, NY 10032 USA. [Kalathur, Ravi C.; Liu, Qun; Kloss, Brian; Bruni, Renato; Ginter, Christopher; Kloppmann, Edda; Rost, Burkhard; Hendrickson, Wayne A.] New York Consortium Membrane Prot Struct NYCOMPS, New York Struct Biol Ctr, New York, NY 10027 USA. [Liu, Qun; Hendrickson, Wayne A.] Brookhaven Natl Lab, New York Struct Biol Ctr, Upton, NY 11973 USA. [Kloppmann, Edda; Rost, Burkhard] Tech Univ Munich, Dept Informat Bioinformat & Computat Biol, D-85748 Garching, Germany. [Hendrickson, Wayne A.] Columbia Univ, Dept Physiol & Cellular Biophys, New York, NY 10032 USA. RP Hendrickson, WA (reprint author), Columbia Univ, Dept Biochem & Mol Biophys, 630 W 168th St, New York, NY 10032 USA. EM wayne@xtl.cumc.columbia.edu RI Kalathur, Ravi/L-7696-2016 OI Kalathur, Ravi/0000-0003-1669-9277 FU NIH [GM095315, GM107462] FX We thank members of the Hendrickson laboratory, especially J. Lidestri for LCP instrumentation, O. Clarke for thought-provoking discussion, K. Hu from Stuyvesant High School for help in collecting fluorescence data, and O. Clarke and J. Qin for help in crystallographic computing. We also thank J. Schwanof and R. Abramowitz at National Synchrotron Light Source (NSLS) beamlines X4A and X4C for help in measuring diffraction data, M. L. Hackert of the University of Texas at Austin for insightful suggestions related to phycocyanobilin, A. Palmer of Columbia University for advice on spectroscopic interpretation, and S. Ferguson-Miller of Michigan State University for sharing coordinates ahead of publication. This work was supported in part by NIH grant GM095315 and GM107462 to W.A.H. X4 beamlines were supported by the New York Structural Biology Center at the NSLS of Brookhaven National Laboratory, a U.S. Department of Energy facility. The crystallographic data reported here are deposited in the Protein Data Bank with identification codes listed in table S2. Y.G. and W.A.H. designed research, analyzed data, and wrote the paper; Y.G. performed experiments; E.K. and B.R. performed bioinformatics analyses; B.K. and R.B. performed expression tests; R.C.K. and R.B. overexpressed eukaryotic proteins; Q.L. participated in diffraction analysis; and C.G. participated in the design of activity assays. NR 33 TC 48 Z9 49 U1 4 U2 43 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JAN 30 PY 2015 VL 347 IS 6221 BP 551 EP 555 DI 10.1126/science.aaa1534 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CA0YK UT WOS:000348639300054 PM 25635100 ER PT J AU Li, YL Jiang, Z Lin, XM Wen, HD Walko, DA Deshmukh, SA Subbaraman, R Sankaranarayanan, SKRS Gray, SK Ho, P AF Li, Yuelin Jiang, Zhang Lin, Xiao-Min Wen, Haidan Walko, Donald A. Deshmukh, Sanket A. Subbaraman, Ram Sankaranarayanan, Subramanian K. R. S. Gray, Stephen K. Ho, Phay TI Femtosecond Laser Pulse Driven Melting in Gold Nanorod Aqueous Colloidal Suspension: Identification of a Transition from Stretched to Exponential Kinetics SO SCIENTIFIC REPORTS LA English DT Article ID NANOPARTICLES; BEAM; MECHANISM; DIFFUSION; DYNAMICS; ENERGY AB Many potential industrial, medical, and environmental applications of metal nanorods rely on the physics and resultant kinetics and dynamics of the interaction of these particles with light. We report a surprising kinetics transition in the global melting of femtosecond laser-driven gold nanorod aqueous colloidal suspension. At low laser intensity, the melting exhibits a stretched exponential kinetics, which abruptly transforms into a compressed exponential kinetics when the laser intensity is raised. It is found the relative formation and reduction rate of intermediate shapes play a key role in the transition. Supported by both molecular dynamics simulations and a kinetic model, the behavior is traced back to the persistent heterogeneous nature of the shape dependence of the energy uptake, dissipation and melting of individual nanoparticles. These results could have significant implications for various applications such as water purification and electrolytes for energy storage that involve heat transport between metal nanorod ensembles and surrounding solvents. C1 [Li, Yuelin; Jiang, Zhang; Wen, Haidan; Walko, Donald A.; Ho, Phay] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Lin, Xiao-Min; Deshmukh, Sanket A.; Sankaranarayanan, Subramanian K. R. S.; Gray, Stephen K.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Subbaraman, Ram] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Li, YL (reprint author), Argonne Natl Lab, Adv Photon Source, 9700 S Cass Ave, Argonne, IL 60439 USA. EM ylli@aps.anl.gov; ssankaranarayanan@anl.gov RI Jiang, Zhang/A-3297-2012 OI Jiang, Zhang/0000-0003-3503-8909 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facilities [DE-AC02-06CH11357] FX This work was performed, in part, at the Advanced Photon Source, the Center for Nanoscale Materials, and Argonne Leadership Computing Facility, all U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facilities, under Contract No. DE-AC02-06CH11357. The authors thank Jan Ilavsky and Byeongdu Lee for insightful discussion and Harold Gibson for technical help. NR 35 TC 2 Z9 2 U1 3 U2 37 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 30 PY 2015 VL 5 AR 8146 DI 10.1038/srep08146 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CA0AN UT WOS:000348576600013 PM 25634673 ER PT J AU Yu, JJ Liberton, M Cliften, PF Head, RD Jacobs, JM Smith, RD Koppenaal, DW Brand, JJ Pakrasi, HB AF Yu, Jingjie Liberton, Michelle Cliften, Paul F. Head, Richard D. Jacobs, Jon M. Smith, Richard D. Koppenaal, David W. Brand, Jerry J. Pakrasi, Himadri B. TI Synechococcus elongatus UTEX 2973, a fast growing cyanobacterial chassis for biosynthesis using light and CO2 SO SCIENTIFIC REPORTS LA English DT Article ID BLUE-GREEN ALGAE; MASS-SPECTROMETRY; SYNTHETIC BIOLOGY; CARBON-DIOXIDE; GROWTH; PROTEOME; CHROMATOGRAPHY; REDUCTION; PCC-7942; PCC-6301 AB Photosynthetic microbes are of emerging interest as production organisms in biotechnology because they can grow autotrophically using sunlight, an abundant energy source, and CO2, a greenhouse gas. Important traits for such microbes are fast growth and amenability to genetic manipulation. Here we describe Synechococcus elongatus UTEX 2973, a unicellular cyanobacterium capable of rapid autotrophic growth, comparable to heterotrophic industrial hosts such as yeast. Synechococcus UTEX 2973 can be readily transformed for facile generation of desired knockout and knock-in mutations. Genome sequencing coupled with global proteomics studies revealed that Synechococcus UTEX 2973 is a close relative of the widely studied cyanobacterium Synechococcus elongatus PCC 7942, an organism that grows more than two times slower. A small number of nucleotide changes are the only significant differences between the genomes of these two cyanobacterial strains. Thus, our study has unraveled genetic determinants necessary for rapid growth of cyanobacterial strains of significant industrial potential. C1 [Yu, Jingjie; Liberton, Michelle; Pakrasi, Himadri B.] Washington Univ, Dept Biol, St Louis, MO 63130 USA. [Cliften, Paul F.; Head, Richard D.] Washington Univ Sch Med, Genome Technol Access Ctr, St Louis, MO 63110 USA. [Jacobs, Jon M.; Smith, Richard D.; Koppenaal, David W.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Brand, Jerry J.] Univ Texas Austin, Culture Collect Algae, Austin, TX 78712 USA. RP Pakrasi, HB (reprint author), Washington Univ, Dept Biol, Campus Box 1137, St Louis, MO 63130 USA. EM pakrasi@wustl.edu RI Smith, Richard/J-3664-2012 OI Smith, Richard/0000-0002-2381-2349 FU U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research; Photosynthetic Antenna Research Center (PARC); Energy Frontier Research Center -e U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC 0001035]; Battelle for the U.S. Department of Energy [DE-AC05-76RLO 1830]; National Science Foundation [DBI-1201881] FX We thank all members of the Pakrasi lab for helpful discussions, and Howard Berg at the Integrated Microscopy Facility of Donald Danforth Plant Science Center for TEM assistance. Work at Washington University was primarily supported by U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research. The electron microscopy study was supported as part of the Photosynthetic Antenna Research Center (PARC), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC 0001035. LC-MS/MS proteomics work was performed in the Environmental Molecular Sciences Laboratory, a U.S. Department of Energy Office of Biological and Environmental Research national scientific user facility located at Pacific Northwest National Laboratory in Richland, Washington. Pacific Northwest National Laboratory is operated by Battelle for the U.S. Department of Energy under Contract No. DE-AC05-76RLO 1830. Work at University of Texas at Austin was supported by the National Science Foundation under Award number DBI-1201881. NR 44 TC 13 Z9 14 U1 10 U2 40 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 30 PY 2015 VL 5 AR 8132 DI 10.1038/srep08132 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CA0AL UT WOS:000348576400001 PM 25633131 ER PT J AU Kalay, Z Ben-Naim, E AF Kalay, Z. Ben-Naim, E. TI Fragmentation of random trees SO JOURNAL OF PHYSICS A-MATHEMATICAL AND THEORETICAL LA English DT Article DE fragmentation; trees; networks ID RANDOM NETWORKS; KINETICS; DELETION; MODEL AB We study fragmentation of a random recursive tree into a forest by repeated removal of nodes. The initial tree consists of N nodes and it is generated by sequential addition of nodes with each new node attaching to a randomly-selected existing node. As nodes are removed from the tree, one at a time, the tree dissolves into an ensemble of separate trees, namely, a forest. We study statistical properties of trees and nodes in this heterogeneous forest, and find that the fraction of remaining nodes m characterizes the system in the limit N -> infinity. We obtain analytically the size density phi(s) of trees of size s. The size density has power-law tail phi(s) similar to s(-alpha) with exponent alpha = 1 + 1/m. Therefore, the tail becomes steeper as further nodes are removed, and the fragmentation process is unusual in that exponent alpha increases continuously with time. We also extend our analysis to the case where nodes are added as well as removed, and obtain the asymptotic size density for growing trees. C1 [Kalay, Z.] Kyoto Univ, Inst Integrated Cell Mat Sci WPI iCeMS, Sakura Ku, Kyoto 6068501, Japan. [Ben-Naim, E.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Ben-Naim, E.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. RP Kalay, Z (reprint author), Kyoto Univ, Inst Integrated Cell Mat Sci WPI iCeMS, Sakura Ku, Yoshida Ushinomiya Cho, Kyoto 6068501, Japan. EM ebn@lanl.gov RI Ben-Naim, Eli/C-7542-2009 OI Ben-Naim, Eli/0000-0002-2444-7304 FU World Premier International Research Center (WPI) Initiative of the Ministry of Education, Culture, Sports, Science and Technology (MEXT) of Japan; US-DOE [DE-AC52-06NA25396] FX We acknowledge support by the World Premier International Research Center (WPI) Initiative of the Ministry of Education, Culture, Sports, Science and Technology (MEXT) of Japan, and by the US-DOE (grant DE-AC52-06NA25396). NR 54 TC 2 Z9 2 U1 0 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1751-8113 EI 1751-8121 J9 J PHYS A-MATH THEOR JI J. Phys. A-Math. Theor. PD JAN 30 PY 2015 VL 48 IS 4 AR 045001 DI 10.1088/1751-8113/48/4/045001 PG 15 WC Physics, Multidisciplinary; Physics, Mathematical SC Physics GA AY9CO UT WOS:000347847500002 ER PT J AU Lanata, N Yao, YX Wang, CZ Ho, KM Kotliar, G AF Lanata, Nicola Yao, Yongxin Wang, Cai-Zhuang Ho, Kai-Ming Kotliar, Gabriel TI Phase Diagram and Electronic Structure of Praseodymium and Plutonium SO PHYSICAL REVIEW X LA English DT Article ID MEAN-FIELD THEORY; STRONGLY CORRELATED SYSTEMS; ABSORPTION BRANCHING RATIO; SLAVE-BOSON APPROACH; LDA PLUS DMFT; TRANSITION-METALS; CRYSTAL-STRUCTURE; DELTA-PLUTONIUM; ALPHA-PU; VALENCE AB We develop a new implementation of the Gutzwiller approximation in combination with the local density approximation, which enables us to study complex 4f and 5f systems beyond the reach of previous approaches. We calculate from first principles the zero-temperature phase diagram and electronic structure of Pr and Pu, finding good agreement with the experiments. Our study of Pr indicates that its pressure-induced volume-collapse transition would not occur without change of lattice structure-contrarily to Ce. Our study of Pu shows that the most important effect originating the differentiation between the equilibrium densities of its allotropes is the competition between the Peierls effect and the Madelung interaction and not the dependence of the electron correlations on the lattice structure. C1 [Lanata, Nicola; Kotliar, Gabriel] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08856 USA. [Yao, Yongxin; Wang, Cai-Zhuang; Ho, Kai-Ming] US DOE, Ames Lab, Ames, IA 50011 USA. [Yao, Yongxin; Wang, Cai-Zhuang; Ho, Kai-Ming] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Lanata, N (reprint author), Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08856 USA. EM lanata@physics.rutgers.edu; ykent@iastate.edu FU U. S. Department of Energy (DOE), Office of Basic Energy Sciences [DE-FG02-99ER45761]; U. S. DOE, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; Iowa State University [DE-AC02-07CH11358] FX We thank XiaoYu Deng, Kristjan Haule, Xi Dai, Hugo U. R. Strand, and Michele Fabrizio for useful discussions. N. L. and G. K. were supported by the U. S. Department of Energy (DOE), Office of Basic Energy Sciences under Grant No. DE-FG02-99ER45761. Research at Ames Laboratory was supported by the U. S. DOE, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. Ames Laboratory is operated for the U. S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. NR 102 TC 12 Z9 12 U1 3 U2 33 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2160-3308 J9 PHYS REV X JI Phys. Rev. X PD JAN 29 PY 2015 VL 5 IS 1 AR 011008 DI 10.1103/PhysRevX.5.011008 PG 28 WC Physics, Multidisciplinary SC Physics GA CL5BO UT WOS:000356975000002 ER PT J AU Pruttivarasin, T Ramm, M Porsev, SG Tupitsyn, II Safronova, MS Hohensee, MA Haffner, H AF Pruttivarasin, T. Ramm, M. Porsev, S. G. Tupitsyn, I. I. Safronova, M. S. Hohensee, M. A. Haeffner, H. TI Michelson-Morley analogue for electrons using trapped ions to test Lorentz symmetry SO NATURE LA English DT Article ID INERTIAL MASS; ANISOTROPY; ATOMS; CPT AB All evidence so far suggests that the absolute spatial orientation of an experiment never affects its outcome. This is reflected in the standard model of particle physics by requiring all particles and fields to be invariant under Lorentz transformations. The best-known tests of this important cornerstone of physics are Michelson-Morley-type experiments verifying the isotropy of the speed of light(1-3). For matter, Hughes-Drever-type experiments(4-11) test whether the kinetic energy of particles is independent of the direction of their velocity, that is, whether their dispersion relations are isotropic. To provide more guidance for physics beyond the standard model, refined experimental verifications of Lorentz symmetry are desirable. Here we search for violation of Lorentz symmetry for electrons by performing an electronic analogue of a Michelson-Morley experiment. We split an electron wave packet bound inside a calcium ion into two parts with different orientations and recombine them after a time evolution of 95 milliseconds. As the Earth rotates, the absolute spatial orientation of the two parts of the wave packet changes, and anisotropies in the electron dispersion will modify the phase of the interference signal. To remove noise, we prepare a pair of calcium ions in a superposition of two decoherence-free states, thereby rejecting magnetic field fluctuations common to both ions(12). After a 23-hour measurement, we find a limit of h x 11 millihertz (h is Planck's constant) on the energy variations, verifying the isotropy of the electron's dispersion relation at the level of one part in 10(18), a 100-fold improvement on previous work(9). Alternatively, we can interpret our result as testing the rotational invariance of the Coulomb potential. Assuming that Lorentz symmetry holds for electrons and that the photon dispersion relation governs the Coulomb force, we obtain a fivefold-improved limit on anisotropies in the speed of light(2,3). Our result probes Lorentz symmetry violation at levels comparable to the ratio between the electroweak and Planck energy scales(13). Our experiment demonstrates the potential of quantum information techniques in the search for physics beyond the standard model. C1 [Pruttivarasin, T.; Ramm, M.; Hohensee, M. A.; Haeffner, H.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Pruttivarasin, T.] RIKEN, Quantum Metrol Lab, Wako, Saitama 3510198, Japan. [Porsev, S. G.; Safronova, M. S.] Univ Delaware, Dept Phys & Astron, Newark, DC 19716 USA. [Porsev, S. G.] Petersburg Nucl Phys Inst, Gatchina 188300, Leningrad Distr, Russia. [Tupitsyn, I. I.] St Petersburg State Univ, Dept Phys, St Petersburg 198504, Russia. [Safronova, M. S.] NIST, Joint Quantum Inst, College Pk, MD 20742 USA. [Safronova, M. S.] Univ Maryland, College Pk, MD 20742 USA. [Hohensee, M. A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Pruttivarasin, T (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM thaned.pruttivarasin@riken.jp; hhaeffner@berkeley.edu RI Haeffner, Hartmut/D-8046-2012; Tupitsyn, Ilya/J-6611-2013 OI Haeffner, Hartmut/0000-0002-5113-9622; Tupitsyn, Ilya/0000-0001-9237-5667 FU NSF CAREER programme grant [PHY 0955650]; NSF [PHY 1212442, PHY 1404156]; US Department of Energy, Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was supported by the NSF CAREER programme grant no. PHY 0955650 and NSF grants no. PHY 1212442 and no. PHY 1404156, and was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. We thank H. Muller for critical reading of the manuscript. NR 41 TC 24 Z9 24 U1 2 U2 20 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD JAN 29 PY 2015 VL 517 IS 7536 BP 592 EP U357 DI 10.1038/nature14091 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CA2ZL UT WOS:000348775000038 PM 25631446 ER PT J AU Karwat, DMA Wooldridge, MS Klippenstein, SJ Davis, MJ AF Karwat, Darshan M. A. Wooldridge, Margaret S. Klippenstein, Stephen J. Davis, Michael J. TI Effects of New Ab Initio Rate Coefficients on Predictions of Species Formed during n-Butanol Ignition and Pyrolysis SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID VARIATIONAL TRANSITION-STATE; HYDROGEN-ABSTRACTION; COMBUSTION CHEMISTRY; RATE CONSTANTS; KINETICS; OXIDATION; 1-BUTANOL; HYDROXYBUTYL; PRESSURE; RADICALS AB Experimental, time-resolved species profiles provide critical tests in developing accurate combustion models for biofuels such as n-butanol. A number of such species profiles measured by Karwat et al. [Karwat, D. M. A.; et al. J. Phys. Chem. A 2011, 115, 4909] were discordant with predictions from a well-tested chemical kinetic mechanism developed by Black et al. [Black, G.; et al. Combust. Flame 2010, 157, 363]. Since then, significant theoretical and experimental efforts have focused on determining the rate coefficients of primary n-butanol consumption pathways in combustion environments, including H atom abstraction reactions from n-butanol by key radicals such as HO2 and OH, as well as the decomposition of the radicals formed by these H atom abstractions. These reactions not only determine the overall reactivity of n-butanol, but also significantly affect the concentrations of intermediate species formed during n-butanol ignition. In this paper we explore the effect of incorporating new ab initio predictions into the Black et al. mechanism on predictions of ignition delay time and species time histories for the experimental conditions studied by Karwat et al. The revised predictions for the intermediate species time histories are in much improved agreement with the measurements, but some discrepancies persist. A rate of production analysis comparing the effects of various modifications to the Black et al. mechanism shows significant changes in the predicted consumption pathways of n-butanol, and of the hydroxybutyl and butoxy radicals formed by H atom abstraction from n-butanol. The predictions from the newly revised mechanism are in very good agreement with the low-pressure n-butanol pyrolysis product species measurements of Stranic et al. [Stranic, I.; et al. Combust. Flame 2012, 159, 3242] for all but one species. Importantly, the changes to the Black et al. mechanism show that concentrations of small products from n-butanol pyrolysis are sensitive to different reactions than those presented by Stranic et al. C1 [Karwat, Darshan M. A.; Wooldridge, Margaret S.] Univ Michigan, Dept Mech Engn, Ann Arbor, MI 48109 USA. [Wooldridge, Margaret S.] Univ Michigan, Dept Aerosp Engn, Ann Arbor, MI 48109 USA. [Klippenstein, Stephen J.; Davis, Michael J.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Karwat, DMA (reprint author), Univ Michigan, Dept Mech Engn, Ann Arbor, MI 48109 USA. EM dippind@umich.edu OI Klippenstein, Stephen/0000-0001-6297-9187 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; Combustion Energy Frontier Research Center [DE-SC0001198]; [DE-SC0002645]; [DE-AC02-06CH11357] FX This material is based on work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences. The work at the University of Michigan was supported under Contract No. DE-SC0002645. The work at Argonne was supported under Contract No. DE-AC02-06CH11357, with the work of S.J.K. performed under the auspices of the Combustion Energy Frontier Research Center under Award No. DE-SC0001198. NR 31 TC 2 Z9 2 U1 7 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JAN 29 PY 2015 VL 119 IS 4 BP 543 EP 551 DI 10.1021/jp509279d PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CA2QL UT WOS:000348752400001 PM 25560388 ER PT J AU Srinivasan, SG van Duin, ACT Ganesh, P AF Srinivasan, Sriram Goverapet van Duin, Adri C. T. Ganesh, P. TI Development of a ReaxFF Potential for Carbon Condensed Phases and Its Application to the Thermal Fragmentation of a Large Fullerene SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID CHEMICAL MOLECULAR-DYNAMICS; REACTIVE FORCE-FIELD; ELECTRONEGATIVITY EQUALIZATION METHOD; AUGMENTED-WAVE METHOD; HOT GIANT ROAD; C-2 FRAGMENTATION; DISSOCIATION-ENERGIES; C-70 CLUSTERS; C-60; DENSITY AB In this article, we report the development of a ReaxFF reactive potential that can accurately describe the chemistry and dynamics of carbon condensed phases. Density functional theory (DFT)-based calculations were performed to obtain the equation of state for graphite and diamond and the formation energies of defects in graphene and amorphous phases from fullerenes. The DFT data were used to reparametrize ReaxFF(CHO), resulting in a new potential called Reax(FFC-2013). ReaxFF(C-2013) accurately predicts the atomization energy of graphite and closely reproduces the DFT-based energy difference between graphite and diamond, and the barrier for transition from graphite to diamond. ReaxFF(C-2013) also accurately predicts the DFT-based energy barrier for Stone-Wales transformation in a C-60(Ih) fullerene through the concerted rotation of a C-2 unit. Later, MD simulations of a C-180 fullerene using ReaxFF(C-2013) suggested that the thermal fragmentation of these giant fullerenes is an exponential function of time. An Arrhenius-type equation was fit to the decay rate, giving an activation energy of 7.66 eV for the loss of carbon atoms from the fullerene. Although the decay of the molecule occurs primarily via the loss of C-2 units, we observed that, with an increase in temperature, the probability of loss of larger fragments increases. The ReaxFF(C-2013) potential developed in this work, and the results obtained on fullerene fragmentation, provide an important step toward the full computational chemical modeling of coal pyrolysis, soot incandescence, high temperature erosion of graphitic rocket nozzles, and ablation of carbon-based spacecraft materials during atmospheric reentry. C1 [Srinivasan, Sriram Goverapet; van Duin, Adri C. T.] Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16802 USA. [Ganesh, P.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP van Duin, ACT (reprint author), Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16802 USA. EM acv13@psu.edu RI Ganesh, Panchapakesan/E-3435-2012; Goverapet Srinivasan, Sriram/L-9681-2016 OI Ganesh, Panchapakesan/0000-0002-7170-2902; Goverapet Srinivasan, Sriram/0000-0003-3984-1547 FU Air Force Office of Scientific Research (AFOSR) [FA9550-10-1-0563]; US Department of Energy, Office of Science, Office of Basic Energy Sciences; Center for Nanophase Materials Sciences - Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX The molecular dynamics simulations and their analysis were supported by Air Force Office of Scientific Research (AFOSR) under Grant No. FA9550-10-1-0563. The views and conclusions contained herein are those of the authors and should not be interpreted as necessarily representing the official policies or endorsements, either expressed or implied, of the AFOSR or the U.S. Government. A.C.T.vD. also acknowledges the support of the Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences for the ReaxFF force field development work. P.G. acknowledges support from the Center for Nanophase Materials Sciences, which is sponsored at the Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy for the DFT-calculations. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 68 TC 22 Z9 23 U1 10 U2 74 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JAN 29 PY 2015 VL 119 IS 4 BP 571 EP 580 DI 10.1021/jp510274e PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CA2QL UT WOS:000348752400004 PM 25562718 ER PT J AU Ong, MT Verners, O Draeger, EW van Duin, ACT Lordi, V Pask, JE AF Ong, Mitchell T. Verners, Osvalds Draeger, Erik W. van Duin, Adri C. T. Lordi, Vincenzo Pask, John E. TI Lithium Ion Solvation and Diffusion in Bulk Organic Electrolytes from First-Principles and Classical Reactive Molecular Dynamics SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID TOTAL-ENERGY CALCULATIONS; BINARY SOLVENT SYSTEMS; AUGMENTED-WAVE METHOD; ETHYLENE CARBONATE; PROPYLENE CARBONATE; LI-ION; DIMETHYL CARBONATE; FORCE-FIELD; BASIS-SET; BATTERIES AB Lithium-ion battery performance is strongly influenced by the ionic conductivity of the electrolyte, which depends on the speed at which Li ions migrate across the cell and relates to their solvation structure. The choice of solvent can greatly impact both solvation and diffusivity of Li ions. We use first principles molecular dynamics to examine the solvation and diffusion of Li ions in the bulk organic solvents ethylene carbonate (EC), ethyl methyl carbonate (EMC), and a mixture of EC/EMC. We find that Li ions are solvated by either carbonyl or ether oxygen atoms of the solvents and sometimes by the PF6- anion. Li+ prefers a tetrahedrally-coordinated first solvation shell regardless of which species are involved, with the specific preferred solvation structure dependent on the organic solvent. In addition, we calculate Li diffusion coefficients in each electrolyte, finding slightly larger diffusivities in the linear carbonate EMC compared to the cyclic carbonate EC. The magnitude of the diffusion coefficient correlates with the strength of Li+ solvation. Corresponding analysis for the PF6- anion shows greater diffusivity associated with a weakly-bound, poorly defined first solvation shell. These results may be used to aid in the design of new electrolytes to improve Li-ion battery performance. C1 [Ong, Mitchell T.; Lordi, Vincenzo] Lawrence Livermore Natl Lab, Div Mat Sci, Livermore, CA 94550 USA. [Draeger, Erik W.] Lawrence Livermore Natl Lab, Ctr Appl Sci Comp, Livermore, CA 94550 USA. [Pask, John E.] Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94550 USA. [Verners, Osvalds; van Duin, Adri C. T.] Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16801 USA. RP Ong, MT (reprint author), Lawrence Livermore Natl Lab, Div Mat Sci, Livermore, CA 94550 USA. EM ong7@llnl.gov; lordi2@llnl.gov OI Lordi, Vincenzo/0000-0003-2415-4656 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Scientific Discovery through Advanced Computing (SciDAC) program - U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research and Basic Energy Sciences; U.S. Army Research Laboratory through the Collaborative Research Alliance (CRA) for Multi Scale Multidisciplinary Modeling of Electronic Materials (MSME); Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences FX M.T.O. acknowledges Brandon Wood, Kyle Caspersen, Eric Schwegler, Tingting Qi, and Md Mahbubul Islam for useful comments and discussions regarding content presented in this article. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. Support for this work was provided through Scientific Discovery through Advanced Computing (SciDAC) program funded by the U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research and Basic Energy Sciences. O.V. and A.C.T.v.D. acknowledge funding from a grant from the U.S. Army Research Laboratory through the Collaborative Research Alliance (CRA) for Multi Scale Multidisciplinary Modeling of Electronic Materials (MSME) for ReaxFF molecular dynamics validation and from the Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences for the ReaxFF force field development. NR 53 TC 16 Z9 16 U1 11 U2 59 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JAN 29 PY 2015 VL 119 IS 4 BP 1535 EP 1545 DI 10.1021/jp508184f PG 11 WC Chemistry, Physical SC Chemistry GA CA2QY UT WOS:000348753600030 PM 25523643 ER PT J AU Vo, QN Hawkins, CA Dang, LX Nilsson, M Nguyen, HD AF Vo, Quynh N. Hawkins, Cory A. Dang, Liem X. Nilsson, Mikael Nguyen, Hung D. TI Computational Study of Molecular Structure and Self-Association of Tri-n-butyl Phosphates in n-Dodecane SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID DYNAMICS SIMULATIONS; TRIBUTYL-PHOSPHATE; FORCE-FIELD; DIFFUSION-COEFFICIENT; EFFICIENT GENERATION; URANYL-NITRATE; AM1-BCC MODEL; LIQUID-VAPOR; SYSTEM-SIZE; WATER AB Tri-n-butyl phosphate (TBP) is an important extractant used in the solvent extraction process for recovering uranium and plutonium from used nuclear fuel. An atomistic molecular dynamics study was used to understand the fundamental molecular-level behavior of extracting agents in solution. Atomistic parametrization was carried out using the AMBER force field to model the TBP molecule and n-dodecane molecule, a commonly used organic solvent. Validation of the optimized force field was accomplished through various thermophysical properties of pure TBP and pure n-dodecane in the bulk liquid phase. The mass density, dipole moment, self-diffusion coefficient, and heat of vaporization were calculated from our simulations and compared favorably with experimental values. The molecular structure of TBPs in n-dodecane at a dilute TBP concentration was examined based on radial distribution functions. 1D and 2D potential mean force studies were carried out to establish the criteria for identifying TBP aggregates. The dimerization constant of TBP in the TBP/n-dodecane mixture was also obtained and matched the experimental value. C1 [Vo, Quynh N.; Hawkins, Cory A.; Nilsson, Mikael; Nguyen, Hung D.] Univ Calif Irvine, Dept Chem Engn & Mat Sci, Irvine, CA 92697 USA. [Dang, Liem X.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP Nguyen, HD (reprint author), Univ Calif Irvine, Dept Chem Engn & Mat Sci, Irvine, CA 92697 USA. EM hdn@uci.edu FU U.S. Department of Energy through the Nuclear Energy University Program, NEUP [120569]; National Science Foundation [DGE-1321846]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences FX We would like to give special thanks to Phil Dennison (UCI NMR Facility Director) for helping with the NMR experiments and the High Performance Computing (HPC) Cluster at UCI for computational resources. The authors wish to thank the U.S. Department of Energy for funding the work through the Nuclear Energy University Program, NEUP Contract No. 120569. Q.N.V. acknowledges support from a Graduate Research Fellowship from the National Science Foundation (DGE-1321846). The U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences funded the work performed by L.X.D. NR 53 TC 7 Z9 7 U1 4 U2 24 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JAN 29 PY 2015 VL 119 IS 4 BP 1588 EP 1597 DI 10.1021/jp510365c PG 10 WC Chemistry, Physical SC Chemistry GA CA2QY UT WOS:000348753600035 PM 25564136 ER PT J AU Hong, WT Stoerzinger, KA Moritz, B Devereaux, TP Yang, WL Shao-Horn, Y AF Hong, Wesley T. Stoerzinger, Kelsey A. Moritz, Brian Devereaux, Thomas P. Yang, Wanli Shao-Horn, Yang TI Probing LaMO3 Metal and Oxygen Partial Density of States Using X-ray Emission, Absorption, and Photoelectron Spectroscopy SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID LEVEL PHOTOEMISSION SPECTRA; FIELD-EFFECT TRANSISTOR; ELECTRONIC-STRUCTURE; TRANSITION-METAL; BAND-STRUCTURE; PEROVSKITE STRUCTURE; EXCITATION-SPECTRA; EDGE SPECTROSCOPY; CHEMICAL-STATES; VALENCE STATES AB We examined the electronic structure in LaMO3 perovskite oxides (M = Cr, Mn, Fe, Co, Ni) by combining information from X-ray emission, absorption, and photoelectron spectroscopy. Through first-principles density functional theory simulations, we identified complementary hybridization features present in the transition metal and oxygen X-ray emission spectra. We then developed a method for the self-consistent alignment of the emission data onto a common energy scale using these features, providing a valuable supplementary technique to photoelectron spectroscopy for studying the partial density of states in perovskites. The combined information from X-ray emission and absorption was used to explore trends in electronic structure characteristics under the Zaanen-Sawatzky-Allen frameworknamely the extent of metal-oxygen hybridization, band gap, and charge-transfer gap. We further established a method that allows for the experimental determination of the occupied and unoccupied band positions relative to the oxide Fermi level, as well as on an absolute energy scale. C1 [Hong, Wesley T.; Stoerzinger, Kelsey A.; Shao-Horn, Yang] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. [Shao-Horn, Yang] MIT, Dept Mech Engn, Cambridge, MA 02139 USA. [Moritz, Brian; Devereaux, Thomas P.] SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, Menlo Pk, CA 94025 USA. [Moritz, Brian] Univ N Dakota, Dept Phys & Astrophys, Grand Forks, ND 58202 USA. [Yang, Wanli] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Hong, WT (reprint author), MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. EM whong@mit.edu; shaohorn@mit.edu RI Yang, Wanli/D-7183-2011; Moritz, Brian/D-7505-2015; OI Yang, Wanli/0000-0003-0666-8063; Moritz, Brian/0000-0002-3747-8484; Stoerzinger, Kelsey/0000-0002-3431-8290 FU U.S. Department of Energy [SISGR DE-SC0002633]; Skoltech-MIT Center for Electro-chemical Energy; National Science Foundation [DMR-0819762]; National Science Foundation Graduate Research Fellowship [1122374]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-76SF00515] FX The authors thank Alexis Grimaud for assistance with sample preparation, and Paul Olalde-Velasco and Ruimin Qiao for guidance with the XES and XAS measurements. This work was supported in part by the U.S. Department of Energy (SISGR DE-SC0002633) and the Skoltech-MIT Center for Electro-chemical Energy. This work made use of the MRSEC Shared Experimental Facilities at MIT, supported by the National Science Foundation under award number DMR-0819762. K.A.S. was supported in part by the National Science Foundation Graduate Research Fellowship under Grant No. 1122374. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The work at SLAC National Accelerator Laboratory was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Contract No. DE-AC02-76SF00515. NR 83 TC 4 Z9 4 U1 5 U2 34 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 29 PY 2015 VL 119 IS 4 BP 2063 EP 2072 DI 10.1021/jp511931y PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CA2QR UT WOS:000348753000052 ER PT J AU Li, J Sham, TK Ye, YF Zhu, JF Guo, JH AF Li, Jun Sham, Tsun-Kong Ye, Yifan Zhu, Junfa Guo, Jinghua TI Structural and Optical Interplay of Palladium-Modified TiO2 Nanoheterostructure SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID X-RAY-ABSORPTION; CANADIAN-LIGHT-SOURCE; NANOTUBE ARRAYS; L-EDGE; HYDROGEN GENERATION; POLARIZATION DEPENDENCE; CHARGE REDISTRIBUTION; PHASE-TRANSFORMATION; PD NANOPARTICLES; SPECTROSCOPY AB The electronic structure and optical properties of Pd-modified TiO2 nanotubes (NTs) with a vertically aligned nanotubular structure grown by a two-step electrochemical anodization method have been studied using X-ray spectroscopy. X-ray absorption near-edge structure (XANES) at the Ti L-3,L-2- and O K-edges was used to investigate the TiO2 NTs before and after Pd modification. It was found that Pd nanoparticles (NPs) are uniformly coated on the NT surface. The Pd L-3-edge of the deposited Pd NPs shows a more intense whiteline and a blue shift for the Pd L-3-edge absorption threshold relative to Pd metal, indicating charge depletion from the Pd 4d orbital as a result NP formation. The lattice of Pd is slightly contracted upon NP formation, although it remains fcc as revealed by extended X-ray absorption fine structure (EXAFS) analysis at the Pd K-edge. X-ray-excited optical luminescence (XEOL) together with XANES with element and site specificity was used to study the optical luminescence from TiO2 NTs. It was found that the defect-originated XEOL intensity dropped noticeably in the Pd NP-coated NTs, suggesting a Pd NP-TiO2-interaction-mediated reduction in the radiative recombination of electrons and holes. Further evidence is provided by Ti 2p resonant inelastic X-ray scattering (RIXS), in which no low-energy loss features (d-d transitions) were observed. The implications of these results are discussed. C1 [Li, Jun; Sham, Tsun-Kong] Univ Western Ontario, Dept Chem, London, ON N6A 5B7, Canada. [Ye, Yifan; Guo, Jinghua] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Ye, Yifan; Zhu, Junfa] Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230029, Anhui, Peoples R China. [Ye, Yifan; Zhu, Junfa] Univ Sci & Technol China, Collaborat Innovat Ctr Suzhou Nano Sci & Technol, Hefei 230029, Anhui, Peoples R China. RP Sham, TK (reprint author), Univ Western Ontario, Dept Chem, 1151 Richmond St, London, ON N6A 5B7, Canada. EM tsham@uwo.ca RI Zhu, Junfa/E-4020-2010; Li, Jun/I-8384-2012 OI Zhu, Junfa/0000-0003-0888-4261; Li, Jun/0000-0002-1958-5665 FU NSERC; CRC; CFI; OIT; NRC; CIHR; University of Saskatchewan; CLS Graduate Student Travel Support Program; Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; National Natural Science Foundation of China [U1232102] FX Research at the University of Western Ontario is supported by NSERC, CRC (TKS), CFI, and OIT. The work at Canadian Light Source (CLS) is supported by CFI, NSERC, NRC, CIHR, and the University of Saskatchewan. J.L. acknowledges the receipt of support from the CLS Graduate Student Travel Support Program. The work at the Advanced Light Source is supported by the Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. J.F.Z. thanks the financial support from the National Natural Science Foundation of China (U1232102). We thank Dr. Tim Goldhawk and Dr. Todd Simpson of the Nanofabrication Laboratory at University of Western Ontario for SEM characterization, and we thank Dr. Grace Yau in the Department of Earth Science, University of Western Ontario, for XRD characterization. We also thank Dr. Yongfeng Hu for technical support at the SXRMB, Dr. Ning Chen for technical support at the FDCMA beamline, and Dr. Tom Regier for technical support at the SGM beamline, all at Canadian Light Source, as well as Dr. Wanli Yang for technical support at beamline 8.0.1, Advanced Light Source. NR 57 TC 3 Z9 3 U1 3 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 29 PY 2015 VL 119 IS 4 BP 2222 EP 2230 DI 10.1021/jp511080q PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CA2QR UT WOS:000348753000068 ER PT J AU Gong, K Martin, JE Shea-Rohwer, LE Lu, P Kelley, DF AF Gong, Ke Martin, James E. Shea-Rohwer, Lauren E. Lu, Ping Kelley, David F. TI Radiative Lifetimes of Zincblende CdSe/CdS Quantum Dots SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ABSORPTION CROSS-SECTION; OPTICAL-PROPERTIES; SEMICONDUCTOR NANOCRYSTALS; CDTE NANOCRYSTALS; EXCITON-STATES; BAND OFFSETS; SIZE; SPECTROSCOPY; DEPENDENCE; NANORODS AB Recent synthetic advances have made available very monodisperse zincblende CdSe/CdS quantum dots having near-unity photoluminescence quantum yields. Because of the absence of nonradiative decay pathways, accurate values of the radiative lifetimes can be obtained from time-resolved PL measurements. Radiative lifetimes can also be obtained from the Einstein relations, using the static absorption spectra and the relative thermal populations in the angular momentum sublevels. One of the inputs into these calculations is the shell thickness, and it is useful to be able to determine shell thickness from spectroscopic measurements. We use an empirically corrected effective mass model to produce a map of exciton wavelength as a function of core size and shell thickness. These calculations use an elastic continuum model and the known lattice and elastic constants to include the effect of lattice strain on the band gap energy. The map is in agreement with the known CdSe sizing curve and with the shell thicknesses of zincblende core/shell particles obtained from TEM images. If seleniumsulfur diffusion is included and lattice strain is omitted from the calculation then the resulting map is appropriate for wurtzite CdSe/CdS quantum dots synthesized at high temperatures, and this map is very similar to one previously reported ( J. Am. Chem. Soc. 2009, 131, 14299). Radiative lifetimes determined from time-resolved measurements are compared to values obtained from the Einstein relations, and found to be in excellent agreement. For a specific core size (2.64 nm diameter, in the present case), radiative lifetimes are found to decrease with increasing shell thickness. This is similar to the size dependence of one-component CdSe quantum dots and in contrast to the size dependence in type-II quantum dots. C1 [Gong, Ke; Kelley, David F.] Univ Calif Merced, Merced, CA 95343 USA. [Martin, James E.; Shea-Rohwer, Lauren E.; Lu, Ping] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Kelley, DF (reprint author), Univ Calif Merced, 5200 North Lake Rd, Merced, CA 95343 USA. EM dfkelley@ucmerced.edu FU Sandia National Laboratories Solid-State-Lighting Science Energy Frontier Research Center - U.S. Department of Energy, Office of Basic Energy Sciences; Laboratory Research and Development Program; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported through the Sandia National Laboratories Solid-State-Lighting Science Energy Frontier Research Center, funded by the U.S. Department of Energy, Office of Basic Energy Sciences. Funding at Sandia was also provided by the Laboratory Research and Development Program. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 36 TC 12 Z9 12 U1 6 U2 58 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 29 PY 2015 VL 119 IS 4 BP 2231 EP 2238 DI 10.1021/jp5118932 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CA2QR UT WOS:000348753000069 ER PT J AU Tawfik, AN Magdy, N AF Tawfik, Abdel Nasser Magdy, Niseem TI SU(3) Polyakov linear-sigma model in magnetic fields: Thermodynamics, higher-order moments, chiral phase structure, and meson masses SO PHYSICAL REVIEW C LA English DT Article ID JONA-LASINIO MODEL; TEMPERATURE CONFINEMENT TRANSITIONS; CONSTANT ELECTROMAGNETIC-FIELD; FINITE-TEMPERATURE; SYMMETRY-BREAKING; QUARK; QCD; LOOP AB Effects of an external magnetic field on various properties of quantum chromodynamics (QCD) matter under extreme conditions of temperature and density (chemical potential) have been analyzed. To this end, we use SU(3) Polyakov linear-sigma model and assume that the external magnetic field (eB) adds some restrictions to the quarks' energy due to the existence of free charges in the plasma phase. In doing this, we apply the Landau theory of quantization, which assumes that the cyclotron orbits of charged particles in a magnetic field should be quantized. This requires an additional temperature to drive the system through the chiral phase transition. Accordingly, the dependence of the critical temperature of chiral and confinement phase transitions on the magnetic field is characterized. Based on this, we have studied the thermal evolution of thermodynamic quantities (energy density and trace anomaly) and the first four higher-order moment of particle multiplicity. Having all these calculations, we have studied the effects of the magnetic field on the chiral phase transition. We found that both critical temperature T-c and critical chemical potential increase with increasing magnetic field, eB. Last but not least, the magnetic effects of the thermal evolution of four scalar and four pseudoscalar meson states are studied. We concluded that the meson masses decrease as the temperature increases up to T-c. Then, the vacuum effect becomes dominant and rapidly increases with the temperature T. At low T, the scalar meson masses normalized to the lowest Matsubara frequency rapidly decrease as T increases. Then, starting from T-c, we find that the thermal dependence almost vanishes. Furthermore, the meson masses increase with increasing magnetic field. This gives a characteristic phase diagram of T vs external magnetic field eB. At high T, we find that the masses of almost all meson states become temperature independent. It is worthwhile to highlight that the various meson states likely have different critical temperatures. C1 [Tawfik, Abdel Nasser] Modern Univ Technol & Informat MTI, Egyptian Ctr Theoret Phys, Cairo 11571, Egypt. [Tawfik, Abdel Nasser; Magdy, Niseem] World Lab Cosmol & Particle Phys WLCAPP, Cairo, Egypt. [Magdy, Niseem] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Tawfik, AN (reprint author), Modern Univ Technol & Informat MTI, Egyptian Ctr Theoret Phys, Cairo 11571, Egypt. RI Tawfik, Abdel Nasser/M-6220-2013 OI Tawfik, Abdel Nasser/0000-0002-1679-0225 FU World Laboratory for Cosmology and Particle Physics (WLCAPP) FX This work is supported by the World Laboratory for Cosmology and Particle Physics (WLCAPP), http://wlcapp.net/. A.T. would like to thank Abdel Magied Diab for the constructive discussion about the implementation of an external magnetic field in the sigma model. NR 80 TC 3 Z9 3 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JAN 29 PY 2015 VL 91 IS 1 AR 015206 DI 10.1103/PhysRevC.91.015206 PG 18 WC Physics, Nuclear SC Physics GA CA1NG UT WOS:000348678600003 ER PT J AU Keller, L White, JS Frontzek, M Babkevich, P Susner, MA Sims, ZC Sefat, AS Ronnow, HM Ruegg, C AF Keller, L. White, J. S. Frontzek, M. Babkevich, P. Susner, M. A. Sims, Z. C. Sefat, A. S. Ronnow, H. M. Rueegg, Ch. TI Pressure dependence of the magnetic order in CrAs: A neutron diffraction investigation SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTIVITY AB The suppression of magnetic order with pressure concomitant with the appearance of pressure-induced superconductivity was recently discovered in CrAs. Here we present a neutron diffraction study of the pressure evolution of the helimagnetic ground state towards and in the vicinity of the superconducting phase. Neutron diffraction on polycrystalline CrAs was employed from zero pressure to 0.65 GPa and at various temperatures. The helimagnetic long-range order is sustained under pressure and the magnetic propagation vector does not show any considerable change. The average ordered magnetic moment is reduced from 1.73(2) mu(B) at ambient pressure to 0.4(1) mu(B) close to the critical pressure P-c approximate to 0.7 GPa, at which magnetic order is completely suppressed. The width of the magnetic Bragg peaks strongly depends on temperature and pressure, showing a maximum in the region of the onset of superconductivity. We interpret this as associated with competing ground states in the vicinity of the superconducting phase. C1 [Keller, L.; White, J. S.; Frontzek, M.; Rueegg, Ch.] Paul Scherrer Inst, Lab Neutron Scattering & Imaging, CH-5232 Villigen, Switzerland. [Babkevich, P.; Ronnow, H. M.] Ecole Polytech Fed Lausanne, Lab Quantum Magnetism, CH-1015 Lausanne, Switzerland. [Susner, M. A.; Sims, Z. C.; Sefat, A. S.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Ronnow, H. M.] RIKEN, CEMS, Wako, Saitama 3510198, Japan. [Rueegg, Ch.] Univ Geneva, Dept Quantum Matter Phys, CH-1211 Geneva, Switzerland. RP Keller, L (reprint author), Paul Scherrer Inst, Lab Neutron Scattering & Imaging, CH-5232 Villigen, Switzerland. EM lukas.keller@psi.ch RI Ruegg, Christian/A-3476-2012; White, Jonathan/G-2742-2010; Susner, Michael/G-3275-2015; Sefat, Athena/R-5457-2016; Susner, Michael/B-1666-2013; Frontzek, Matthias/C-5146-2012; EPFL, Physics/O-6514-2016 OI Ruegg, Christian/0000-0003-0139-7786; White, Jonathan/0000-0001-7738-0150; Susner, Michael/0000-0002-1211-8749; Sefat, Athena/0000-0002-5596-3504; Susner, Michael/0000-0002-1211-8749; Frontzek, Matthias/0000-0001-8704-8928; FU Swiss National Science Foundation; Sinergia network MPBH; European Research Council project CONQUEST; U.S. Department of Energy, Office of Science Basic Energy Sciences, Materials Science and Engineering Division; LDRD program FX Part of this work was performed at the Swiss Spallation Neutron Source SINQ, Paul Scherrer Institut, Villigen, Switzerland. The work in Switzerland was supported by the Swiss National Science Foundation, its Sinergia network MPBH, and the European Research Council project CONQUEST. The work at Oak Ridge National Laboratory was supported by the U.S. Department of Energy, Office of Science Basic Energy Sciences, Materials Science and Engineering Division (Z.C.S. and A.S.); also partially by the LDRD program (M.A.S.). The authors thank R. Khasanov and H. Luetkens for helpful discussions. NR 14 TC 8 Z9 8 U1 8 U2 51 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 29 PY 2015 VL 91 IS 2 AR 020409 DI 10.1103/PhysRevB.91.020409 PG 5 WC Physics, Condensed Matter SC Physics GA CA1MR UT WOS:000348677100001 ER PT J AU Deng, ZD Carlson, TJ Li, H Xiao, J Myjak, MJ Lu, J Martinez, JJ Woodley, CM Weiland, MA Eppard, MB AF Deng, Z. D. Carlson, T. J. Li, H. Xiao, J. Myjak, M. J. Lu, J. Martinez, J. J. Woodley, C. M. Weiland, M. A. Eppard, M. B. TI An injectable acoustic transmitter for juvenile salmon SO SCIENTIFIC REPORTS LA English DT Article ID CHINOOK SALMON; TELEMETRY SYSTEM; SURVIVAL; PASSAGE; INSTRUMENTATION; MANAGEMENT; TRACKING; GROWTH; DESIGN; OCEAN AB Salmon recovery and the potential detrimental effects of dams on fish have been attracting national attention due to the environmental and economic implications. In recent years acoustic telemetry has been the primary method for studying salmon passage. However, the size of the existing transmitters limits the minimum size of fish that can be studied, introducing a bias to the study results. We developed the first acoustic fish transmitter that can be implanted by injection instead of surgery. The new injectable transmitter lasts four times longer and weighs 30% less than other transmitters. Because the new transmitter costs significantly less to use and may substantially reduce adverse effects of implantation and tag burden, it will allow for study of migration behavior and survival of species and sizes of fish that have never been studied before. The new technology will lead to critical information needed for salmon recovery and the development of fish-friendly hydroelectric systems. C1 [Deng, Z. D.; Carlson, T. J.; Li, H.; Xiao, J.; Myjak, M. J.; Lu, J.; Martinez, J. J.; Woodley, C. M.; Weiland, M. A.; Eppard, M. B.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Deng, ZD (reprint author), Pacific NW Natl Lab, POB 999, Richland, WA 99352 USA. EM zhiqun.deng@pnnl.gov RI Deng, Daniel/A-9536-2011; OI Deng, Daniel/0000-0002-8300-8766; Myjak, Mitchell/0000-0002-3807-3542 FU U.S. Army Corps of Engineers, Portland District FX This study was funded by the U.S. Army Corps of Engineers, Portland District. It was conducted at Pacific Northwest National Laboratory (PNNL), operated in Richland, Washington, by Battelle for the U.S. Department of Energy. Numerous PNNL staff from the Ecology Group, Hydrology Group, and Marine Sciences Laboratory contributed to developing and proving this technology. NR 24 TC 13 Z9 13 U1 0 U2 20 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 29 PY 2015 VL 5 AR 8111 DI 10.1038/srep08111 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AZ8ZQ UT WOS:000348501100002 PM 25630763 ER PT J AU Blake, JA Christie, KR Dolan, ME Drabkin, HJ Hill, DP Ni, L Sitnikov, D Burgess, S Buza, T Gresham, C McCarthy, F Pillai, L Wang, H Carbon, S Dietze, H Lewis, SE Mungall, CJ Munoz-Torres, MC Feuermann, M Gaudet, P Basu, S Chisholm, RL Dodson, RJ Fey, P Mi, H Thomas, PD Muruganujan, A Poudel, S Hu, JC Aleksander, SA McIntosh, BK Renfro, DP Siegele, DA Attrill, H Brown, NH Tweedie, S Lomax, J Osumi-Sutherland, D Parkinson, H Roncaglia, P Lovering, RC Talmud, PJ Humphries, SE Denny, P Campbell, NH Foulger, RE Chibucos, MC Giglio, MG Chang, HY Finn, R Fraser, M Mitchell, A Nuka, G Pesseat, S Sangrador, A Scheremetjew, M Young, SY Stephan, R Harris, MA Oliver, SG Rutherford, K Wood, V Bahler, J Lock, A Kersey, PJ McDowall, MD Staines, DM Dwinell, M Shimoyama, M Laulederkind, S Hayman, GT Wang, SJ Petri, V D'Eustachio, P Matthews, L Balakrishnan, R Binkley, G Cherry, JM Costanzo, MC Demeter, J Dwight, SS Engel, SR Hitz, BC Inglis, DO Lloyd, P Miyasato, SR Paskov, K Roe, G Simison, M Nash, RS Skrzypek, MS Weng, S Wong, ED Berardini, TZ Li, D Huala, E Argasinska, J Arighi, C Auchincloss, A Axelsen, K Argoud-Puy, G Bateman, A Bely, B Blatter, MC Bonilla, C Bougueleret, L Boutet, E Breuza, L Bridge, A Britto, R Casals, C Cibrian-Uhalte, E Coudert, E Cusin, I Duek-Roggli, P Estreicher, A Famiglietti, L Gane, P Garmiri, P Gos, A Gruaz-Gumowski, N Hatton-Ellis, E Hinz, U Hulo, C Huntley, R Jungo, F Keller, G Laiho, K Lemercier, P Lieberherr, D MacDougall, A Magrane, M Martin, M Masson, P Mutowo, P O'Donovan, C Pedruzzi, I Pichler, K Poggioli, D Poux, S Rivoire, C Roechert, B Sawford, T Schneider, M Shypitsyna, A Stutz, A Sundaram, S Tognolli, M Wu, C Xenarios, I Chan, J Kishore, R Sternberg, PW Van Auken, K Muller, HM Done, J Li, Y Howe, D Westerfield, M AF Blake, J. A. Christie, K. R. Dolan, M. E. Drabkin, H. J. Hill, D. P. Ni, L. Sitnikov, D. Burgess, S. Buza, T. Gresham, C. McCarthy, F. Pillai, L. Wang, H. Carbon, S. Dietze, H. Lewis, S. E. Mungall, C. J. Munoz-Torres, M. C. Feuermann, M. Gaudet, P. Basu, S. Chisholm, R. L. Dodson, R. J. Fey, P. Mi, H. Thomas, P. D. Muruganujan, A. Poudel, S. Hu, J. C. Aleksander, S. A. McIntosh, B. K. Renfro, D. P. Siegele, D. A. Attrill, H. Brown, N. H. Tweedie, S. Lomax, J. Osumi-Sutherland, D. Parkinson, H. Roncaglia, P. Lovering, R. C. Talmud, P. J. Humphries, S. E. Denny, P. Campbell, N. H. Foulger, R. E. Chibucos, M. C. Giglio, M. Gwinn Chang, H. Y. Finn, R. Fraser, M. Mitchell, A. Nuka, G. Pesseat, S. Sangrador, A. Scheremetjew, M. Young, S. Y. Stephan, R. Harris, M. A. Oliver, S. G. Rutherford, K. Wood, V. Bahler, J. Lock, A. Kersey, P. J. McDowall, M. D. Staines, D. M. Dwinell, M. Shimoyama, M. Laulederkind, S. Hayman, G. T. Wang, S. J. Petri, V. D'Eustachio, P. Matthews, L. Balakrishnan, R. Binkley, G. Cherry, J. M. Costanzo, M. C. Demeter, J. Dwight, S. S. Engel, S. R. Hitz, B. C. Inglis, D. O. Lloyd, P. Miyasato, S. R. Paskov, K. Roe, G. Simison, M. Nash, R. S. Skrzypek, M. S. Weng, S. Wong, E. D. Berardini, T. Z. Li, D. Huala, E. Argasinska, J. Arighi, C. Auchincloss, A. Axelsen, K. Argoud-Puy, G. Bateman, A. Bely, B. Blatter, M. C. Bonilla, C. Bougueleret, L. Boutet, E. Breuza, L. Bridge, A. Britto, R. Casals, C. Cibrian-Uhalte, E. Coudert, E. Cusin, I. Duek-Roggli, P. Estreicher, A. Famiglietti, L. Gane, P. Garmiri, P. Gos, A. Gruaz-Gumowski, N. Hatton-Ellis, E. Hinz, U. Hulo, C. Huntley, R. Jungo, F. Keller, G. Laiho, K. Lemercier, P. Lieberherr, D. MacDougall, A. Magrane, M. Martin, M. Masson, P. Mutowo, P. O'Donovan, C. Pedruzzi, I. Pichler, K. Poggioli, D. Poux, S. Rivoire, C. Roechert, B. Sawford, T. Schneider, M. Shypitsyna, A. Stutz, A. Sundaram, S. Tognolli, M. Wu, C. Xenarios, I. Chan, J. Kishore, R. Sternberg, P. W. Van Auken, K. Muller, H. M. Done, J. Li, Y. Howe, D. Westerfield, M. CA Gene Ontology Consortium TI Gene Ontology Consortium: going forward SO NUCLEIC ACIDS RESEARCH LA English DT Article ID ANATOMY ONTOLOGY; ANNOTATIONS; TOOL; ENHANCEMENTS; UNIFICATION; RESOURCES; DATABASE AB The Gene Ontology (GO; ext-link-type="uri" xlink:href="http://www.geneontology.org" xlink:type="simple">http://www.geneontology.org) is a community-based bioinformatics resource that supplies information about gene product function using ontologies to represent biological knowledge. Here we describe improvements and expansions to several branches of the ontology, as well as updates that have allowed us to more efficiently disseminate the GO and capture feedback from the research community. The Gene Ontology Consortium (GOC) has expanded areas of the ontology such as cilia-related terms, cell-cycle terms and multicellular organism processes. We have also implemented new tools for generating ontology terms based on a set of logical rules making use of templates, and we have made efforts to increase our use of logical definitions. The GOC has a new and improved web site summarizing new developments and documentation, serving as a portal to GO data. Users can perform GO enrichment analysis, and search the GO for terms, annotations to gene products, and associated metadata across multiple species using the all-new AmiGO 2 browser. We encourage and welcome the input of the research community in all biological areas in our continued effort to improve the Gene Ontology. C1 [Blake, J. A.; Christie, K. R.; Dolan, M. E.; Drabkin, H. J.; Hill, D. P.; Ni, L.; Sitnikov, D.] Jackson Lab, MGI, Bar Harbor, ME 04609 USA. [Burgess, S.; Buza, T.; Gresham, C.; McCarthy, F.; Pillai, L.; Wang, H.] Mississippi State Univ, AgBase, Starkville, MS USA. [Carbon, S.; Dietze, H.; Lewis, S. E.; Mungall, C. J.; Munoz-Torres, M. C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley Bioinformat Open Source Projects, Genom Div, Berkeley, CA 94720 USA. [Feuermann, M.; Gaudet, P.] SIB, CALIPHO Grp, Geneva, Switzerland. [Basu, S.; Chisholm, R. L.; Dodson, R. J.; Fey, P.] Northwestern Univ, DictyBase, Chicago, IL 60611 USA. [Mi, H.; Thomas, P. D.; Muruganujan, A.; Poudel, S.] Univ So Calif, Dept Prevent Med, Div Bioinformat, Los Angeles, CA 90089 USA. [Hu, J. C.; Aleksander, S. A.; McIntosh, B. K.; Renfro, D. P.; Siegele, D. A.] Texas A&M Univ, Dept Biol, EcoliWiki, College Stn, TX 77843 USA. [Hu, J. C.; Aleksander, S. A.; McIntosh, B. K.; Renfro, D. P.; Siegele, D. A.] Texas A&M Univ, Dept Biochem & Biophys, EcoliWiki, College Stn, TX 77843 USA. [Attrill, H.; Brown, N. H.; Tweedie, S.] Univ Cambridge, Gurdon Inst, FlyBase, Cambridge, England. [Attrill, H.; Brown, N. H.; Tweedie, S.] Univ Cambridge, Dept Genet, Cambridge, England. [Lomax, J.; Osumi-Sutherland, D.; Parkinson, H.; Roncaglia, P.] GO EMBL EBI, Hinxton, England. [Lovering, R. C.; Talmud, P. J.; Humphries, S. E.; Denny, P.; Campbell, N. H.; Foulger, R. E.] UCL, Inst Cardiovasc Sci, London, England. [Chibucos, M. C.; Giglio, M. Gwinn] Univ Maryland, Sch Med, Inst Genome Sci, Baltimore, MD 21201 USA. [Chang, H. Y.; Finn, R.; Fraser, M.; Mitchell, A.; Nuka, G.; Pesseat, S.; Sangrador, A.; Scheremetjew, M.; Young, S. Y.] EMBL EBI, InterPro, Hinxton, England. [Stephan, R.] Collect & Refinement Physiol Data Mycobacterium, Berlin, Germany. [Harris, M. A.; Oliver, S. G.; Rutherford, K.; Wood, V.] Univ Cambridge, PomBase, Cambridge, England. [Bahler, J.; Lock, A.] UCL, PomBase, London, England. [Kersey, P. J.; McDowall, M. D.; Staines, D. M.] EMBL EBI, PomBase, Hinxton, England. [Dwinell, M.; Shimoyama, M.; Laulederkind, S.; Hayman, G. T.; Wang, S. J.; Petri, V.] Med Coll Wisconsin, RGD, Milwaukee, WI 53226 USA. [D'Eustachio, P.; Matthews, L.] NYU, Sch Med, Reactome, Dept Biochem & Mol Pharmacol, New York, NY USA. [Balakrishnan, R.; Binkley, G.; Cherry, J. M.; Costanzo, M. C.; Demeter, J.; Dwight, S. S.; Engel, S. R.; Hitz, B. C.; Inglis, D. O.; Lloyd, P.; Miyasato, S. R.; Paskov, K.; Roe, G.; Simison, M.; Nash, R. S.; Skrzypek, M. S.; Weng, S.; Wong, E. D.] Stanford Univ, Dept Genet, SGD, Stanford, CA 94305 USA. [Berardini, T. Z.; Li, D.; Huala, E.] Phoenix Bioinformat, TAIR, Redwood City, CA USA. [Argasinska, J.; Arighi, C.; Auchincloss, A.; Axelsen, K.; Argoud-Puy, G.; Bateman, A.; Bely, B.; Blatter, M. C.; Bonilla, C.; Bougueleret, L.; Boutet, E.; Breuza, L.; Bridge, A.; Britto, R.; Casals, C.; Cibrian-Uhalte, E.; Coudert, E.; Cusin, I.; Duek-Roggli, P.; Estreicher, A.; Famiglietti, L.; Gane, P.; Garmiri, P.; Gos, A.; Gruaz-Gumowski, N.; Hatton-Ellis, E.; Hinz, U.; Hulo, C.; Huntley, R.; Jungo, F.; Keller, G.; Laiho, K.; Lemercier, P.; Lieberherr, D.; MacDougall, A.; Magrane, M.; Martin, M.; Masson, P.; Mutowo, P.; O'Donovan, C.; Pedruzzi, I.; Pichler, K.; Poggioli, D.; Poux, S.; Rivoire, C.; Roechert, B.; Sawford, T.; Schneider, M.; Shypitsyna, A.; Stutz, A.; Sundaram, S.; Tognolli, M.; Wu, C.; Xenarios, I.] UniProt EMBL EBI, Hinxton, England. [Argasinska, J.; Arighi, C.; Auchincloss, A.; Axelsen, K.; Argoud-Puy, G.; Bateman, A.; Bely, B.; Blatter, M. C.; Bonilla, C.; Bougueleret, L.; Boutet, E.; Breuza, L.; Bridge, A.; Britto, R.; Casals, C.; Cibrian-Uhalte, E.; Coudert, E.; Cusin, I.; Duek-Roggli, P.; Estreicher, A.; Famiglietti, L.; Gane, P.; Garmiri, P.; Gos, A.; Gruaz-Gumowski, N.; Hatton-Ellis, E.; Hinz, U.; Hulo, C.; Huntley, R.; Jungo, F.; Keller, G.; Laiho, K.; Lemercier, P.; Lieberherr, D.; MacDougall, A.; Magrane, M.; Martin, M.; Masson, P.; Mutowo, P.; O'Donovan, C.; Pedruzzi, I.; Pichler, K.; Poggioli, D.; Poux, S.; Rivoire, C.; Roechert, B.; Sawford, T.; Schneider, M.; Shypitsyna, A.; Stutz, A.; Sundaram, S.; Tognolli, M.; Wu, C.; Xenarios, I.] SIB, Geneva, Switzerland. [Argasinska, J.; Arighi, C.; Auchincloss, A.; Axelsen, K.; Argoud-Puy, G.; Bateman, A.; Bely, B.; Blatter, M. C.; Bonilla, C.; Bougueleret, L.; Boutet, E.; Breuza, L.; Bridge, A.; Britto, R.; Casals, C.; Cibrian-Uhalte, E.; Coudert, E.; Cusin, I.; Duek-Roggli, P.; Estreicher, A.; Famiglietti, L.; Gane, P.; Garmiri, P.; Gos, A.; Gruaz-Gumowski, N.; Hatton-Ellis, E.; Hinz, U.; Hulo, C.; Huntley, R.] Prot Informat Resource, Washington, DC USA. [Chan, J.; Kishore, R.; Sternberg, P. W.; Van Auken, K.; Muller, H. M.; Done, J.; Li, Y.] CALTECH, WormBase, Pasadena, CA 91125 USA. [Howe, D.; Westerfield, M.] Univ Oregon, ZFIN, Eugene, OR 97403 USA. RP Munoz-Torres, MC (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley Bioinformat Open Source Projects, Genom Div, Berkeley, CA 94720 USA. EM McMunozT@lbl.gov RI Bahler, Jurg/B-4572-2009; Pedruzzi, Ivo/O-7423-2015; Huntley, Rachael/R-1036-2016; OI Bahler, Jurg/0000-0003-4036-1532; Bely, Benoit/0000-0002-0029-9693; Tweedie, Susan/0000-0003-1818-8243; Lomax, Jane/0000-0001-8865-4321; Roncaglia, Paola/0000-0002-2825-0621; Parkinson, Helen/0000-0003-3035-4195; Pedruzzi, Ivo/0000-0001-8561-7170; Engel, Stacia/0000-0001-5472-917X; Huntley, Rachael/0000-0001-6718-3559; McDowall, Mark/0000-0002-6666-602X; Demeter, Janos/0000-0002-7301-8055; Inglis, Diane/0000-0003-3166-4638; Siegele, Deborah/0000-0001-8935-0696; Matthews, Lisa/0000-0001-5707-3065; Pichler, Klemens/0000-0001-6099-8931; Rutherford, Kim/0000-0001-6277-726X; Foulger, Rebecca/0000-0001-8682-8754; Finn, Robert/0000-0001-8626-2148; Garmiri, Penelope/0000-0002-2283-2575; Talmud, Philippa/0000-0002-5560-1933; Bateman, Alex/0000-0002-6982-4660; Osumi-Sutherland, David/0000-0002-7073-9172; Scheremetjew, Maxim/0000-0002-7458-3072; Staines, Daniel/0000-0002-7564-9125; Lewis, Suzanna/0000-0002-8343-612X; Britto, Ramona/0000-0003-1011-5410; Mutowo, Prudence/0000-0002-4646-4172; D'Eustachio, Peter/0000-0002-5494-626X; Magrane, Michele/0000-0003-3544-996X; Kersey, Paul/0000-0002-7054-800X; Arighi, Cecilia/0000-0002-0803-4817; Hatton-Ellis, Emma/0000-0002-7262-1928; Breuza, Lionel/0000-0002-8075-8625; Martin, Maria-Jesus/0000-0001-5454-2815; Poux, Sylvain/0000-0001-7299-6685; Bridge, Alan/0000-0003-2148-9135; O'Donovan, Claire/0000-0001-8051-7429; Chibucos, Marcus/0000-0001-9586-0780 FU National Institutes of Health/National Human Genome Research Institute [HG002273] FX National Institutes of Health/National Human Genome Research Institute grant [HG002273] awarded to the PI group formed by Judith A. Blake, J. Michael Cherry, Suzanna E. Lewis, Paul W. Sternberg, and Paul D. Thomas, as well as additional funding awarded to each participating institution. For more details please visit: http://geneontology.org/page/go-consortium-contributors-list. Funding for open access charge: National Institutes of Health/National Human Genome Research Institute [HG002273]. NR 24 TC 142 Z9 144 U1 12 U2 35 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 EI 1362-4962 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD JAN 28 PY 2015 VL 43 IS D1 BP D1049 EP D1056 DI 10.1093/nar/gku1179 PG 8 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CC2YF UT WOS:000350210400154 ER PT J AU Hudson, CM Williams, KP AF Hudson, Corey M. Williams, Kelly P. TI The tmRNA website SO NUCLEIC ACIDS RESEARCH LA English DT Article ID MESSENGER-RNA; DATABASE; SMPB; RESOURCES; SEQUENCES; FAMILIES; RIBOSOME; GENOMES AB The transfer-messenger RNA (tmRNA) and its partner protein SmpB act together in resolving problems arising when translating bacterial ribosomes reach the end of mRNA with no stop codon. Their genes have been found in nearly all bacterial genomes and in some organelles. The tmRNA Website serves tmRNA sequences, alignments and feature annotations, and has recently moved to http://bioinformatics.sandia.gov/tmrna/. New features include software used to find the sequences, an update raising the number of unique tmRNA sequences from 492 to 1716, and a database of SmpB sequences which are served along with the tmRNA sequence from the same organism. C1 [Hudson, Corey M.; Williams, Kelly P.] Sandia Natl Labs, Dept Syst Biol, Livermore, CA 94551 USA. RP Williams, KP (reprint author), Sandia Natl Labs, Dept Syst Biol, Livermore, CA 94551 USA. EM kpwilli@sandia.gov FU Laboratory Directed Research and Development 108 program at Sandia National Laboratories; U.S. Department of Energy's 111 National Nuclear Security Administration [DE-AC04-94AL85000]; Laboratory Directed Research and Development program at Sandia National Laboratories FX This research was fully supported by the Laboratory Directed Research and Development 108 program at Sandia National Laboratories. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned 110 subsidiary of Lock-heed Martin Corporation, for the U.S. Department of Energy's 111 National Nuclear Security Administration under contract DE-AC04-94AL85000. Funding for open access charge: Laboratory Directed Research and Development program at Sandia National Laboratories. NR 18 TC 5 Z9 5 U1 0 U2 3 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 EI 1362-4962 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD JAN 28 PY 2015 VL 43 IS D1 BP D138 EP D140 DI 10.1093/nar/gku1109 PG 3 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CC2YF UT WOS:000350210400022 PM 25378311 ER PT J AU Hudson, CM Lau, BY Williams, KP AF Hudson, Corey M. Lau, Britney Y. Williams, Kelly P. TI Islander: a database of precisely mapped genomic islands in tRNA and tmRNA genes SO NUCLEIC ACIDS RESEARCH LA English DT Article ID NUCLEOTIDE-SEQUENCES; INTEGRATION SITES; COLI O157-H7; PROGRAM; RECOMBINASES; ANNOTATION; ELEMENTS; PROTEIN; STRAIN; DNA AB Genomic islands are mobile DNAs that are major agents of bacterial and archaeal evolution. Integration into prokaryotic chromosomes usually occurs site-specifically at tRNA or tmRNA gene (together, tDNA) targets, catalyzed by tyrosine integrases. This splits the target gene, yet sequences within the island restore the disrupted gene; the regenerated target and its displaced fragment precisely mark the endpoints of the island. We applied this principle to search for islands in genomic DNA sequences. Our algorithm identifies tDNAs, finds fragments of those tDNAs in the same replicon and removes unlikely candidate islands through a series of filters. A search for islands in 2168 whole prokaryotic genomes produced 3919 candidates. The website Islander (recently moved to http://bioinformatics.sandia.gov/islander/) presents these precisely mapped candidate islands, the gene content and the island sequence. The algorithm further insists that each island encode an integrase, and attachment site sequence identity is carefully noted; therefore, the database also serves in the study of integrase site-specificity and its evolution. C1 [Hudson, Corey M.; Lau, Britney Y.; Williams, Kelly P.] Sandia Natl Labs, Dept Syst Biol, Livermore, CA 94550 USA. RP Williams, KP (reprint author), Sandia Natl Labs, Dept Syst Biol, Livermore, CA 94550 USA. EM kpwilli@sandia.gov FU Laboratory Directed Research and Development program at Sandia National Laboratories [14-1155] FX Funding for open access charge: Laboratory Directed Research and Development program at Sandia National Laboratories, grant number 14-1155. NR 29 TC 7 Z9 7 U1 0 U2 4 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 EI 1362-4962 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD JAN 28 PY 2015 VL 43 IS D1 BP D48 EP D53 DI 10.1093/nar/gku1072 PG 6 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CC2YF UT WOS:000350210400008 PM 25378302 ER PT J AU Kibbe, WA Arze, C Felix, V Mitraka, E Bolton, E Fu, G Mungall, CJ Binder, JX Malone, J Vasant, D Parkinson, H Schriml, LM AF Kibbe, Warren A. Arze, Cesar Felix, Victor Mitraka, Elvira Bolton, Evan Fu, Gang Mungall, Christopher J. Binder, Janos X. Malone, James Vasant, Drashtti Parkinson, Helen Schriml, Lynn M. TI Disease Ontology 2015 update: an expanded and updated database of human diseases for linking biomedical knowledge through disease data SO NUCLEIC ACIDS RESEARCH LA English DT Article ID INFORMATION; SPECIFICATIONS; TERMINOLOGY; SYSTEM; MODEL AB The current version of the Human Disease Ontology (DO) ( ext-link-type="uri" xlink:href="http://www.disease-ontology.org" xlink:type="simple">http://www.disease-ontology.org) database expands the utility of the ontology for the examination and comparison of genetic variation, phenotype, protein, drug and epitope data through the lens of human disease. DO is a biomedical resource of standardized common and rare disease concepts with stable identifiers organized by disease etiology. The content of DO has had 192 revisions since 2012, including the addition of 760 terms. Thirty-two percent of all terms now include definitions. DO has expanded the number and diversity of research communities and community members by 50+ during the past two years. These community members actively submit term requests, coordinate biomedical resource disease representation and provide expert curation guidance. Since the DO 2012 NAR paper, there have been hundreds of term requests and a steady increase in the number of DO listserv members, twitter followers and DO website usage. DO is moving to a multi-editor model utilizing Prot,g, to curate DO in web ontology language. This will enable closer collaboration with the Human Phenotype Ontology, EBI's Ontology Working Group, Mouse Genome Informatics and the Monarch Initiative among others, and enhance DO's current asserted view and multiple inferred views through reasoning. C1 [Kibbe, Warren A.] NCI, Ctr Biomed Informat & Informat Technol, Rockville, MD 20850 USA. [Arze, Cesar; Felix, Victor; Mitraka, Elvira; Schriml, Lynn M.] Univ Maryland, Sch Med, Inst Genome Sci, Baltimore, MD 21201 USA. [Bolton, Evan; Fu, Gang] NIH, PubChem, Natl Ctr Biotechnol Informat, Natl Lib Med,Dept Hlth & Human Serv, Bethesda, MD 20894 USA. [Mungall, Christopher J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Genom Div, Berkeley, CA 94720 USA. [Binder, Janos X.] European Mol Biol Lab, Struct & Computat Biol Unit, D-69117 Heidelberg, Germany. [Binder, Janos X.] Univ Luxembourg, LCSB, Bioinformat Core Facil, L-4362 Luxembourg, Luxembourg. [Malone, James; Vasant, Drashtti; Parkinson, Helen] EBI, EMBL, Cambridge CB10 1SD, England. [Schriml, Lynn M.] Univ Maryland, Sch Med, Dept Epidemiol & Publ Hlth, Baltimore, MD 21201 USA. RP Schriml, LM (reprint author), Univ Maryland, Sch Med, Inst Genome Sci, Baltimore, MD 21201 USA. EM lschriml@som.umaryland.edu RI Fu, Gang/F-8837-2016; OI Fu, Gang/0000-0002-4860-8539; Mitraka, Elvira/0000-0003-0719-3485; Malone, James Robert/0000-0002-1615-2899; Parkinson, Helen/0000-0003-3035-4195; Schriml, Lynn/0000-0001-8910-9851 FU National Institutes of Health-National Center for Research Resources [R01RR025341]; EMBL Core funds; WT HIPSCI [098503/D/12/Z]; NHGRI; NHLBI; NIH Common Fund [U54-HG004028]; NIH [R24OD011883]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; University of Maryland, Institute for Genome Sciences FX National Institutes of Health-National Center for Research Resources (R01RR025341); EMBL Core funds and WT HIPSCI [098503/D/12/Z]; NHGRI, NHLBI and NIH Common Fund under U54-HG004028. NIH R24OD011883 (to C.J.M.); Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 (to C.J.M.). Funding for open access charge: University of Maryland, Institute for Genome Sciences. NR 32 TC 48 Z9 48 U1 2 U2 6 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 EI 1362-4962 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD JAN 28 PY 2015 VL 43 IS D1 BP D1071 EP D1078 DI 10.1093/nar/gku1011 PG 8 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CC2YF UT WOS:000350210400157 PM 25348409 ER PT J AU Petrov, AI Kay, SJE Gibson, R Kulesha, E Staines, D Bruford, EA Wright, MW Burge, S Finn, RD Kersey, PJ Cochrane, G Bateman, A Griffiths-Jones, S Harrow, J Chan, PP Lowe, TM Zwieb, CW Wower, J Williams, KP Hudson, CM Gutell, R Clark, MB Dinger, M Quek, XC Bujnicki, JM Chua, NH Liu, J Wang, H Skogerbo, G Zhao, Y Chen, RS Zhu, WM Cole, JR Chai, BL Huang, HD Huang, HY Cherry, JM Hatzigeorgiou, A Pruitt, KD AF Petrov, Anton I. Kay, Simon J. E. Gibson, Richard Kulesha, Eugene Staines, Dan Bruford, Elspeth A. Wright, Mathew W. Burge, Sarah Finn, Robert D. Kersey, Paul J. Cochrane, Guy Bateman, Alex Griffiths-Jones, Sam Harrow, Jennifer Chan, Patricia P. Lowe, Todd M. Zwieb, Christian W. Wower, Jacek Williams, Kelly P. Hudson, Corey M. Gutell, Robin Clark, Michael B. Dinger, Marcel Quek, Xiu Cheng Bujnicki, Janusz M. Chua, Nam-Hai Liu, Jun Wang, Huan Skogerbo, Geir Zhao, Yi Chen, Runsheng Zhu, Weimin Cole, James R. Chai, Benli Huang, Hsien-Da Huang, His-Yuan Cherry, J. Michael Hatzigeorgiou, Artemis Pruitt, Kim D. CA RNAcent Consortium TI RNAcentral: an international database of ncRNA sequences SO NUCLEIC ACIDS RESEARCH LA English DT Article ID RNA GENES; EVOLUTION; PROJECT; ARCHIVE; GENCODE; UPDATE AB The field of non-coding RNA biology has been hampered by the lack of availability of a comprehensive, up-to-date collection of accessioned RNA sequences. Here we present the first release of RNAcentral, a database that collates and integrates information from an international consortium of established RNA sequence databases. The initial release contains over 8.1 million sequences, including representatives of all major functional classes. A web portal (http://rnacentral.org) provides free access to data, search functionality, cross-references, source code and an integrated genome browser for selected species. C1 [Petrov, Anton I.; Kay, Simon J. E.; Gibson, Richard; Kulesha, Eugene; Staines, Dan; Bruford, Elspeth A.; Wright, Mathew W.; Burge, Sarah; Finn, Robert D.; Kersey, Paul J.; Cochrane, Guy; Bateman, Alex] European Bioinformat Inst, European Mol Biol Lab, Cambridge CB10 1SD, England. [Griffiths-Jones, Sam] Univ Manchester, Fac Life Sci, Manchester M13 9PT, Lancs, England. [Harrow, Jennifer] Wellcome Trust Sanger Inst, Cambridge CB10 1SD, England. [Chan, Patricia P.; Lowe, Todd M.] Univ Calif Santa Cruz, Dept Biomol Engn, Santa Cruz, CA 95064 USA. [Zwieb, Christian W.] Univ Texas Hlth Sci Ctr San Antonio, Dept Biochem, San Antonio, TX 78229 USA. [Wower, Jacek] Auburn Univ, Dept Anim Sci, Auburn, AL 36849 USA. [Williams, Kelly P.; Hudson, Corey M.] Sandia Natl Labs, Livermore, CA 94551 USA. [Gutell, Robin] Univ Texas Austin, Dept Integrat Biol, Austin, TX 78712 USA. [Clark, Michael B.] Univ Oxford, Dept Physiol Anat & Genet, MRC, Funct Genom Unit, Oxford OX1 3PT, England. [Dinger, Marcel; Quek, Xiu Cheng] St Vincents Hosp, Garvan Inst Med Res, Kinghorn Ctr Clin Genom, Darlinghurst, NSW 2010, Australia. [Bujnicki, Janusz M.] Int Inst Mol & Cell Biol Warsaw, Lab Bioinformat & Prot Engn, PL-02109 Warsaw, Poland. [Bujnicki, Janusz M.] Adam Mickiewicz Univ, Inst Mol Biol & Biotechnol, Fac Biol, Lab Bioinformat, PL-61614 Poznan, Poland. [Chua, Nam-Hai; Liu, Jun; Wang, Huan] Rockefeller Univ, Plant Mol Biol Lab, New York, NY 10065 USA. [Skogerbo, Geir; Zhao, Yi; Chen, Runsheng] Chinese Acad Sci, Inst Biophys, Lab Noncoding RNA, Beijing 100101, Peoples R China. [Skogerbo, Geir; Zhao, Yi; Chen, Runsheng] Chinese Acad Sci, Inst Comp Technol, Beijing 100190, Peoples R China. [Skogerbo, Geir; Zhao, Yi; Chen, Runsheng] Chinese Acad Med Sci, Inst Basic Med Sci, Beijing, Peoples R China. [Zhu, Weimin] Peking Union Med Coll, Sch Basic Med, Beijing 100005, Peoples R China. [Zhu, Weimin] Taicang Inst Life Sci Informat, Suzhou 215400, Peoples R China. [Cole, James R.; Chai, Benli] Michigan State Univ, E Lansing, MI 48824 USA. [Huang, Hsien-Da; Huang, His-Yuan] Natl Chiao Tung Univ, Dept Biol Sci & Technol, Inst Bioinformat & Syst Biol, Hsinchu, Taiwan. [Cherry, J. Michael] Stanford Univ, Dept Genet, Palo Alto, CA 94304 USA. [Hatzigeorgiou, Artemis] Univ Thessaly, Dept Comp & Commun Engn, Volos 38221, Greece. [Pruitt, Kim D.] Natl Lib Med, Natl Ctr Biotechnol Informat, Bethesda, MD 20894 USA. RP Petrov, AI (reprint author), European Bioinformat Inst, European Mol Biol Lab, Wellcome Trust Genome Campus, Cambridge CB10 1SD, England. EM agb@ebi.ac.uk OI Kay, Simon/0000-0001-7690-2711; Clark, Michael/0000-0002-2903-9537; Cochrane, Guy/0000-0001-7954-7057; Gibson, Richard Charles/0000-0001-5412-1965; Finn, Robert/0000-0001-8626-2148; Petrov, Anton/0000-0001-7279-2682; Wright, Matt/0000-0002-2650-2426; Bateman, Alex/0000-0002-6982-4660; Staines, Daniel/0000-0002-7564-9125; Bruford, Elspeth/0000-0002-8380-5247; Kersey, Paul/0000-0002-7054-800X FU Biotechnology and Biological Sciences Research Council (BBSRC) [BB/J019232/1, BB/J019321/1]; Intramural Research Program of the National Institutes of Health, National Library of Medicine; European Bioinformatics Institute FX Biotechnology and Biological Sciences Research Council (BBSRC) [BB/J019232/1, BB/J019321/1]; Intramural Research Program of the National Institutes of Health, National Library of Medicine. Funding for open access charge: European Bioinformatics Institute. NR 23 TC 13 Z9 13 U1 2 U2 12 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 EI 1362-4962 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD JAN 28 PY 2015 VL 43 IS D1 BP D123 EP D129 DI 10.1093/nar/gku991 PG 7 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CC2YF UT WOS:000350210400020 ER PT J AU Reddy, TBK Thomas, AD Stamatis, D Bertsch, J Isbandi, M Jansson, J Mallajosyula, J Pagani, I Lobos, EA Kyrpides, NC AF Reddy, T. B. K. Thomas, Alex D. Stamatis, Dimitri Bertsch, Jon Isbandi, Michelle Jansson, Jakob Mallajosyula, Jyothi Pagani, Ioanna Lobos, Elizabeth A. Kyrpides, Nikos C. TI The Genomes OnLine Database (GOLD) v.5: a metadata management system based on a four level (meta)genome project classification SO NUCLEIC ACIDS RESEARCH LA English DT Article ID METAGENOMIC PROJECTS; WORLD-WIDE; MONITOR; PHYLOGENY; VERSION AB The Genomes OnLine Database (GOLD; ext-link-type="uri" xlink:href="http://www.genomesonline.org" xlink:type="simple">http://www.genomesonline.org) is a comprehensive online resource to catalog and monitor genetic studies worldwide. GOLD provides up-to-date status on complete and ongoing sequencing projects along with a broad array of curated metadata. Here we report version 5 (v.5) of the database. The newly designed database schema and web user interface supports several new features including the implementation of a four level (meta)genome project classification system and a simplified intuitive web interface to access reports and launch search tools. The database currently hosts information for about 19 200 studies, 56 000 Biosamples, 56 000 sequencing projects and 39 400 analysis projects. More than just a catalog of worldwide genome projects, GOLD is a manually curated, quality-controlled metadata warehouse. The problems encountered in integrating disparate and varying quality data into GOLD are briefly highlighted. GOLD fully supports and follows the Genomic Standards Consortium (GSC) Minimum Information standards. C1 [Reddy, T. B. K.; Thomas, Alex D.; Stamatis, Dimitri; Bertsch, Jon; Isbandi, Michelle; Jansson, Jakob; Mallajosyula, Jyothi; Pagani, Ioanna; Lobos, Elizabeth A.; Kyrpides, Nikos C.] DOE Joint Genome Inst, Prokaryot Super Program, Walnut Creek, CA 94598 USA. [Kyrpides, Nikos C.] King Abdulaziz Univ, Fac Sci, Dept Biol Sci, Jeddah, Saudi Arabia. RP Reddy, TBK (reprint author), DOE Joint Genome Inst, Prokaryot Super Program, Walnut Creek, CA 94598 USA. EM tbreddy@lbl.gov; nckyrpides@lbl.gov RI Kyrpides, Nikos/A-6305-2014; Fac Sci, KAU, Biol Sci Dept/L-4228-2013; Faculty of, Sciences, KAU/E-7305-2017 OI Kyrpides, Nikos/0000-0002-6131-0462; FU US Department of Energy Office of Science, Biological and Environmental Research Program; University of California, Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; US Department of Energy FX This work was performed under the auspices of the US Department of Energy Office of Science, Biological and Environmental Research Program, and by the University of California, Lawrence Berkeley National Laboratory under contract no. DE-AC02-05CH11231. Funding for open access charge: US Department of Energy. NR 23 TC 102 Z9 105 U1 9 U2 24 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 EI 1362-4962 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD JAN 28 PY 2015 VL 43 IS D1 BP D1099 EP D1106 DI 10.1093/nar/gku950 PG 8 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CC2YF UT WOS:000350210400160 PM 25348402 ER PT J AU Movshovitz, N Nimmo, F Korycansky, DG Asphaug, E Owen, JM AF Movshovitz, N. Nimmo, F. Korycansky, D. G. Asphaug, E. Owen, J. M. TI Disruption and reaccretion of midsized moons during an outer solar system Late Heavy Bombardment SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE satellite formation; solar system formation ID CRATERING RATES; POSSIBLE ORIGIN; SATURN SYSTEM; SCALING LAWS; SATELLITES; IMPACTS; PLANETS; RINGS; TOPOGRAPHY; COLLISIONS AB We investigate the problem of satellite survival during a hypothetical Late Heavy Bombardment in the outer solar system, as predicted by the Nice model (Tsiganis, Gomes, Morbidelli,and Levison 2005, Nature 435). Using a Monte Carlo approach we calculate, for satellites of Jupiter, Saturn, and Uranus, the probability of experiencing a catastrophic collision during the Late Heavy Bombardment (LHB). We find that Mimas, Enceladus, Tethys, and Miranda experience at least one catastrophic impact in every simulation. Because reaccretion is expected to be rapid, these bodies will have emerged as scrambled mixtures of rock and ice. Tidal heating may have subsequently modified the latter three, but in the nominal LHB model Mimas should be a largely undifferentiated, homogeneous body. A differentiated Mimas would imply either that this body formed late or that the Nice model requires significant modification. C1 [Movshovitz, N.; Nimmo, F.; Korycansky, D. G.] Univ Calif Santa Cruz, Dept Earth & Planetary Sci, Santa Cruz, CA 95064 USA. [Asphaug, E.] Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ USA. [Owen, J. M.] Lawrence Livermore Natl Lab, Livermore, CA USA. RP Movshovitz, N (reprint author), Univ Calif Santa Cruz, Dept Earth & Planetary Sci, Santa Cruz, CA 95064 USA. EM nmovshov@ucsc.edu OI Movshovitz, Naor/0000-0001-5583-0042 FU OPR grant [NNX11AM57G]; PG and G grant [NNX13AR66G] FX We thank John Chambers, Fred Ciesla, Sebastien Charnoz, and Alessandro Morbidelli for useful conversations. We also thank both reviewers for their helpful comments. D.K. was supported by OPR grant NNX11AM57G. N.M. and E.A. were supported by PG and G grant NNX13AR66G. NR 40 TC 5 Z9 5 U1 1 U2 11 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JAN 28 PY 2015 VL 42 IS 2 BP 256 EP 263 DI 10.1002/2014GL062133 PG 8 WC Geosciences, Multidisciplinary SC Geology GA CB9MO UT WOS:000349956000010 ER PT J AU Maceira, M Larmat, C Porritt, RW Higdon, DM Rowe, CA Allen, RM AF Maceira, Monica Larmat, Carene Porritt, Robert W. Higdon, David M. Rowe, Charlotte A. Allen, Richard M. TI On the validation of seismic imaging methods: Finite frequency or ray theory? SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE finite frequency; ray theory; validation; seismic models; spectral element method ID SPECTRAL-ELEMENT METHOD; TRAVEL-TIMES; SENSITIVITY KERNELS; VELOCITY MODELS; FRECHET KERNELS; TOMOGRAPHY; MANTLE; RESOLUTION; PLUMES AB We investigate the merits of the more recently developed finite-frequency approach to tomography against the more traditional and approximate ray theoretical approach for state of the art seismic models developed for western North America. To this end, we employ the spectral element method to assess the agreement between observations on real data and measurements made on synthetic seismograms predicted by the models under consideration. We check for phase delay agreement as well as waveform cross-correlation values. Based on statistical analyses on S wave phase delay measurements, finite frequency shows an improvement over ray theory. Random sampling using cross-correlation values identifies regions where synthetic seismograms computed with ray theory and finite-frequency models differ the most. Our study suggests that finite-frequency approaches to seismic imaging exhibit measurable improvement for pronounced low-velocity anomalies such as mantle plumes. C1 [Maceira, Monica; Larmat, Carene; Higdon, David M.; Rowe, Charlotte A.] Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. [Porritt, Robert W.] Univ So Calif, Dept Earth Sci, Los Angeles, CA USA. [Porritt, Robert W.; Allen, Richard M.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. RP Maceira, M (reprint author), Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. EM mmaceira@lanl.gov OI Maceira, Monica/0000-0003-1248-2185; Rowe, Charlotte/0000-0001-5803-0147; Larmat, Carene S/0000-0002-3607-7558 FU U.S. Department of Energy by Los Alamos National Laboratory [DE-AC52-06NA25396/LA12-SignalPropagation-NDD2Ab]; program LFRP-Lab Fees [116467] FX Thanks to Guust Nolet and Tarje Nissen-Meyer for their thoughtful reviews that considerably improved the original manuscript. We thank Peter Loxley and Yasuyuki Kato for providing useful discussion regarding the use of statistics for the purpose of models validation. Special thanks to the Data Management Center of IRIS for making the data so easily accessible to us (data from II, IU, TA, and U.S. networks were used in this study), to CIG for developing and facilitating software, and to LANL Institutional Computing Program for providing HPC resources. We thank Wessel and Smith [1991], the developers of the Generic Mapping Tools software, which we use to create many of the illustrations of our research. This work was performed under the auspices of the U.S. Department of Energy by Los Alamos National Laboratory under contract DE-AC52-06NA25396/LA12-SignalPropagation-NDD2Ab and grant ID 116467 under research program LFRP-Lab Fees. NR 41 TC 3 Z9 3 U1 1 U2 10 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JAN 28 PY 2015 VL 42 IS 2 BP 323 EP 330 DI 10.1002/2014GL062571 PG 8 WC Geosciences, Multidisciplinary SC Geology GA CB9MO UT WOS:000349956000018 ER PT J AU Santer, BD Solomon, S Bonfils, C Zelinka, MD Painter, JF Beltran, F Fyfe, JC Johannesson, G Mears, C Ridley, DA Vernier, JP Wentz, FJ AF Santer, Benjamin D. Solomon, Susan Bonfils, Celine Zelinka, Mark D. Painter, Jeffrey F. Beltran, Francisco Fyfe, John C. Johannesson, Gardar Mears, Carl Ridley, David A. Vernier, Jean-Paul Wentz, Frank J. TI Observed multivariable signals of late 20th and early 21st century volcanic activity SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE Volcanic forcing; Climate change; Signal detection ID GLOBAL CLIMATE-CHANGE; STRATOSPHERIC AEROSOL; DECADAL CHANGES; WATER-VAPOR; TEMPERATURE; TRENDS; VARIABILITY; MODEL; ENSO AB The relatively muted warming of the surface and lower troposphere since 1998 has attracted considerable attention. One contributory factor to this warming hiatus is an increase in volcanically induced cooling over the early 21st century. Here we identify the signals of late 20th and early 21st century volcanic activity in multiple observed climate variables. Volcanic signals are statistically discernible in spatial averages of tropical and near-global SST, tropospheric temperature, net clear-sky short-wave radiation, and atmospheric water vapor. Signals of late 20th and early 21st century volcanic eruptions are also detectable in near-global averages of rainfall. In tropical average rainfall, however, only a Pinatubo-caused drying signal is identifiable. Successful volcanic signal detection is critically dependent on removal of variability induced by the El Nino-Southern Oscillation. C1 [Santer, Benjamin D.; Bonfils, Celine; Zelinka, Mark D.; Painter, Jeffrey F.; Beltran, Francisco; Johannesson, Gardar] Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA. [Solomon, Susan; Ridley, David A.] MIT, Cambridge, MA 02139 USA. [Fyfe, John C.] Environm Canada, Canadian Ctr Climate Modelling & Anal, Victoria, BC, Canada. [Mears, Carl; Wentz, Frank J.] Remote Sensing Syst, Santa Rosa, CA USA. [Vernier, Jean-Paul] NASA, Langley Res Ctr, Hampton, VA 23665 USA. RP Santer, BD (reprint author), Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA. EM santer1@llnl.gov RI Santer, Benjamin/F-9781-2011; Zelinka, Mark/C-4627-2011 OI Zelinka, Mark/0000-0002-6570-5445 FU US Department of Energy [DE-AC52-07NA27344]; DOE/OBER Early Career Research Program Award [SCW1295]; NSF [AGS-1342810] FX All observational climate data used here are in the public domain, available at the following locations: (1) http://www.remss.com/data (for TMT, TLT, and PW); (2) http://www.ncdc.noaa.gov/oa/climate/research/sst (for SST); (3) http://ceres-tool.larc.nasa.gov/ord-tool/ (for SW); and (4) http://www.esrl.noaa.gov/psd/data/gridded/data.gpcp.html (for PR). We thank Tom Wigley (University of Adelaide) for valuable comments and suggestions. At Lawrence Livermore National Laboratory, work by B.D.S., J.P., and M.Z. was performed under the auspices of the US Department of Energy under contract DE-AC52-07NA27344; C.B. was supported by the DOE/OBER Early Career Research Program Award SCW1295. S.S. was supported in part by NSF grant AGS-1342810. NR 36 TC 15 Z9 15 U1 5 U2 30 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JAN 28 PY 2015 VL 42 IS 2 BP 500 EP 509 DI 10.1002/2014GL062366 PG 10 WC Geosciences, Multidisciplinary SC Geology GA CB9MO UT WOS:000349956000040 ER PT J AU Taraphdar, S Leung, LR Hagos, S AF Taraphdar, Sourav Leung, L. Ruby Hagos, Samson TI Linkages of remote sea surface temperatures and Atlantic tropical cyclone activity mediated by the African monsoon SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE tropical cyclones; sea surface temperature; African monsoon; Mediterranean SST; African easterly wave; African easterly jet ID IDEALIZED 2-DIMENSIONAL FRAMEWORK; STRONG ASSOCIATION; SAHEL RAINFALL; EASTERLY WAVES; HURRICANES; NORTH; JET AB Warm sea surface temperatures (SSTs) in North Atlantic and Mediterranean (NAMED) can influence tropical cyclone (TC) activity in the tropical East Atlantic by modulating summer convection over western Africa. Analysis of 30years of observations demonstrates that warm NAMED SST is linked to a strengthening of the Saharan heat low and enhancement of moisture and moist static energy in the lower troposphere over West Africa, which favors a northward displacement of the monsoonal front. These processes also lead to a northward shift of the African easterly jet that introduces an anomalous positive vorticity from western Africa to the main development region (50 degrees W-20 degrees E; 10 degrees N-20 degrees N) of Atlantic TCs. By modulating multiple African monsoon processes, NAMED SST explains comparable and approximately one third of the interannual variability of Atlantic TC frequency as that explained by local wind shear and local SST, respectively, which are known key factors that influence Atlantic TC development. C1 [Taraphdar, Sourav; Leung, L. Ruby; Hagos, Samson] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. RP Leung, LR (reprint author), Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. EM ruby.Leung@pnnl.gov FU U.S. Department of Energy, Office of Science Biological and Environmental Research as part of the Regional and Global Climate Modeling Program; DOE [DE-AC05-76RLO1830] FX This research is based on work supported by the U.S. Department of Energy, Office of Science Biological and Environmental Research as part of the Regional and Global Climate Modeling Program. The Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under contract DE-AC05-76RLO1830. NR 24 TC 0 Z9 0 U1 2 U2 5 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JAN 28 PY 2015 VL 42 IS 2 BP 572 EP 578 DI 10.1002/2014GL062600 PG 7 WC Geosciences, Multidisciplinary SC Geology GA CB9MO UT WOS:000349956000048 ER PT J AU Di, ZH Duan, QY Gong, W Wang, C Gan, YJ Quan, JP Li, JD Miao, CY Ye, AZ Tong, C AF Di, Zhenhua Duan, Qingyun Gong, Wei Wang, Chen Gan, Yanjun Quan, Jiping Li, Jianduo Miao, Chiyuan Ye, Aizhong Tong, Charles TI Assessing WRF model parameter sensitivity: A case study with 5 day summer precipitation forecasting in the Greater Beijing Area SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE WRF model parameter sensitivities; global sensitivity analysis; uncertainty quantification; WRF model calibration; MOAT method ID NUMERICAL WEATHER-PREDICTION; DATA ASSIMILATION; MESOSCALE MODEL; CONVECTIVE PARAMETERIZATION; PART I; SIMULATION; CLOUDS; SYSTEM; SCHEME; TESTS AB A global sensitivity analysis method was used to identify the parameters of the Weather Research and Forecasting (WRF) model that exert the most influence on precipitation forecasting. Twenty-three adjustable parameters were selected from seven physical components of the WRF model. The sensitivity was evaluated based on skill scores calculated over nine 5 day precipitation forecasts during the summer seasons from 2008 to 2010 in the Greater Beijing Area in China. We found that eight parameters are more sensitive than others. Storm type seems to have no impact on the list of sensitive parameters but does influence the degree of sensitivity. We also examined the physical interpretation of parameter sensitivity. This analysis is useful for further optimization of the WRF model parameters to improve precipitation forecasting. C1 [Di, Zhenhua; Duan, Qingyun; Gong, Wei; Wang, Chen; Gan, Yanjun; Quan, Jiping; Li, Jianduo; Miao, Chiyuan; Ye, Aizhong] Beijing Normal Univ, Coll Global Change & Earth Syst Sci, Beijing 100875, Peoples R China. [Di, Zhenhua] Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Numer Modeling Atmospher Sci & Geop, Beijing, Peoples R China. [Wang, Chen; Tong, Charles] Lawrence Livermore Natl Lab, Livermore, CA USA. RP Di, ZH (reprint author), Beijing Normal Univ, Coll Global Change & Earth Syst Sci, Beijing 100875, Peoples R China. EM zhdi@bnu.edu.cn RI Duan, Qingyun/C-7652-2011; OI Duan, Qingyun/0000-0001-9955-1512; Miao, Chiyuan/0000-0001-6413-7020; Gan, Yanjun/0000-0001-6660-8236; ye, aizhong/0000-0002-5272-134X; Gong, Wei/0000-0003-3622-7090 FU Beijing Excellent Talent Training Project [2012D009012000001]; Fundamental Research Funds for the Central Universities of China [2012LYB40]; Natural Science Foundation of China [41305052, 41375139]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We thank S.Y. Hong of Yonsei University, S. Miao and Y. Zhang of China Meteorological Administration, and Y. Dai and L. Chen of Beijing Normal University for their expert advice. Validation data are provided by X. Zheng (E-mail: x.zheng@bnu.edu.cn). We acknowledge NCEP Reanalysis data set obtained from http://rda.ucar.edu/datasets/ds083.2/ and the CFSR data set obtained from http://nomads.ncdc.noaa.gov/modeldata/. The research was partially supported by Beijing Excellent Talent Training Project (2012D009012000001), Fundamental Research Funds for the Central Universities of China (2012LYB40), and Natural Science Foundation of China (41305052&41375139). The work of Tong is performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. NR 53 TC 4 Z9 5 U1 5 U2 22 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JAN 28 PY 2015 VL 42 IS 2 BP 579 EP 587 DI 10.1002/2014GL061623 PG 9 WC Geosciences, Multidisciplinary SC Geology GA CB9MO UT WOS:000349956000049 ER PT J AU Zhou, J Sumpter, BG Kent, PRC Huang, JS AF Zhou, Jia Sumpter, Bobby G. Kent, Paul R. C. Huang, Jingsong TI A Novel and Functional Single-Layer Sheet of ZnSe SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE Two-dimensional materials; DFT; GW approximation; BSE; photovoltaic ID INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; CADMIUM CHALCOGENIDES; CDSE NANOSHEETS; BASIS-SET; GRAPHENE; SEMICONDUCTORS; METALS; GAP AB The recently synthesized freestanding four-atom-thick double-layer sheet of ZnSe holds great promise as an ultraflexible and transparent photoelectrode material for solar water splitting. In this work, we report theoretical studies on a novel three-atom-thick single-layer sheet of ZnSe that demonstrates a strong quantum confinement effect by exhibiting a large enhancement of the band gap (2.0 eV) relative to the zinc blende (ZB) bulk phase. Theoretical optical absorbance shows that the largest absorption of this ultrathin single-layer sheet of ZnSe occurs at a wavelength similar to its four-atom-thick double-layer counterpart, suggesting a comparable behavior on incident photon-to-current conversion efficiency for solar water splitting, among a wealth of potential applications. The results presented herein for ZnSe may be generalized to other group II-VI analogues. C1 [Zhou, Jia; Sumpter, Bobby G.; Kent, Paul R. C.; Huang, Jingsong] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Sumpter, Bobby G.; Kent, Paul R. C.; Huang, Jingsong] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. RP Zhou, J (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM jiajoe@gmail.com RI Sumpter, Bobby/C-9459-2013; Kent, Paul/A-6756-2008; Huang, Jingsong/A-2789-2008 OI Sumpter, Bobby/0000-0001-6341-0355; Kent, Paul/0000-0001-5539-4017; Huang, Jingsong/0000-0001-8993-2506 FU Center for Nanophase Materials Sciences at ORNL by Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Office of Science of the U.S. Department of Energy [DE-AC05-00OR22750, DE-AC02-05CH11231] FX We thank Drs. Yu Xie and Houlong Zhuang for helpful discussions. We are also indebted to Prof. Georg Kresse for kindly providing the latest PAW potentials with norm-conserving partial waves for Zn and Se. This work was supported by the Center for Nanophase Materials Sciences, which is sponsored at ORNL by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. This work used computational resources of the Oak Ridge Leadership Computing Facility at Oak Ridge National laboratory and of the National Energy Research Scientific Computing Center, which are supported by the Office of Science of the U.S. Department of Energy under Contract Nos. DE-AC05-00OR22750 and DE-AC02-05CH11231, respectively. NR 46 TC 4 Z9 4 U1 12 U2 66 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JAN 28 PY 2015 VL 7 IS 3 BP 1458 EP 1464 DI 10.1021/am505655m PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CA1RG UT WOS:000348688700010 PM 25535766 ER PT J AU Chatman, S Zarzycki, P Rosso, KM AF Chatman, S. Zarzycki, P. Rosso, K. M. TI Spontaneous Water Oxidation at Hematite (alpha-Fe2O3) Crystal Faces SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE water-splitting; single crystal; photoelectrochemical cell; protonation; oxygen evolution reaction; alpha-Fe2O3 ID PHOTOELECTROCHEMICAL HYDROGEN-PRODUCTION; REDUCTIVE DISSOLUTION; SOLUTION INTERFACE; PROTON ADSORPTION; IRON(III) OXIDE; THIN-FILMS; SURFACE; POTENTIALS; REACTIVITY; ELECTRODES AB Hematite (alpha-Fe2O3) persists as a promising candidate for photoelectrochemical water splitting, but a slow oxygen evolution reaction (OER) at its surfaces remains a limitation. Here we extend a series of studies that examine pH-dependent surface potentials and electron-transfer properties of effectively perfect low-index crystal faces of hematite in contact with simple electrolyte. Zero-resistance amperometry (ZRA) was performed in a two electrode configuration to quantify spontaneous dark current between hematite crystal face pairs (001)/(012), (001)/(113), and (012)/(113) at pH 3. Exponentially decaying currents initially of up to 200 nA were reported between faces over 4 min experiments. Fourth-order ZRA kinetics indicated rate limitation by the OER for current that flows between (001)/(012) and (001)/(113) face pairs, with the (012) and (113) faces serving as the anodes when paired with (001). The cathodic partner reaction is reductive dissolution of the (001) face, converting surface Fe3+ to solubilized aqueous Fe2+, at a rate maintained by the OER at the anode. In contrast, OER rate limitation does not manifest for the (012)/(113) pair. The uniqueness of the (001) face is established in terms of a faster intrinsic ability to accept the protons required for the reductive dissolution reaction. OER rate limitation inversely may thus arise from sluggish kinetics of hematite surfaces to dispense with the protons that accompany the four-electron OER. The results are explained in terms of semiquantitative energy band diagrams. The finding may be useful as a consideration for tailoring the design of polycrystalline hematite photoanodes that present multiple terminations to the interface with electrolyte. C1 [Chatman, S.; Rosso, K. M.] Pacific NW Natl Lab, Phys Sci Div, Richland, WA USA. [Zarzycki, P.] Polish Acad Sci, Inst Phys Chem, Warsaw, Poland. RP Chatman, S (reprint author), CALTECH, Joint Ctr Artificial Photosynth, Pasadena, CA 91125 USA. EM chatmans@caltech.edu; Kevin.Rosso@pnnl.gov FU Geosciences Research Program in the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; DOE Office of Biological and Environmental Research at Pacific Northwest National Laboratory; Ministerstwo Nauki i Szkolnictwa Wyzszego (MNiSW) [IP2012 059872] FX This research was supported by the Geosciences Research Program in the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences. It was performed using EMSL, a national scientific user facility sponsored by the DOE Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory, which is a multiprogram national laboratory operated for DOE by Battelle. P.Z. was also supported by Ministerstwo Nauki i Szkolnictwa Wyzszego (MNiSW) Grant No. IP2012 059872. NR 66 TC 9 Z9 9 U1 11 U2 124 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JAN 28 PY 2015 VL 7 IS 3 BP 1550 EP 1559 DI 10.1021/am5067783 PG 10 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CA1RG UT WOS:000348688700021 PM 25506667 ER PT J AU Cheng, L Chen, W Kunz, M Persson, K Tamura, N Chen, GY Doeff, M AF Cheng, Lei Chen, Wei Kunz, Martin Persson, Kristin Tamura, Nobumichi Chen, Guoying Doeff, Marca TI Effect of Surface Microstructure on Electrochemical Performance of Garnet Solid Electrolytes SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE solid electrolyte; interface; lithium metal; solid state battery; heterostructures ID LITHIUM SUPERIONIC CONDUCTOR; GRAIN-BOUNDARY RESISTANCE; SODIUM-BETA ALUMINA; LI ION CONDUCTORS; STATE BATTERY; TITANIUM PHOSPHATE; LI7LA3ZR2O12; AL; STABILITY; METAL AB Cubic garnet phases based on Al-substituted Li7La3Zr2O12 (LLZO) have high ionic conductivities and exhibit good stability versus metallic lithium, making them of particular interest for use in next-generation rechargeable battery systems. However, high interfacial impedances have precluded their successful utilization in such devices until the present. Careful engineering of the surface microstructure, especially the grain boundaries, is critical to achieving low interfacial resistances and enabling long-term stable cycling with lithium metal. This study presents the fabrication of LLZO heterostructured solid electrolytes, which allowed direct correlation of surface microstructure with the electrochemical characteristics of the interface. Grain orientations and grain boundary distributions of samples with differing microstructures were mapped using high-resolution synchrotron polychromatic X-ray Laue microdiffraction. The electrochemical characteristics are strongly dependent upon surface microstructure, with small grained samples exhibiting much lower interfacial resistances and better cycling behavior than those with larger grain sizes. Low area specific resistances of 37 Omega cm(2) were achieved; low enough to ensure stable cycling with minimal polarization losses, thus removing a significant obstacle toward practical implementation of solid electrolytes in high energy density batteries. C1 [Cheng, Lei; Chen, Wei; Persson, Kristin; Chen, Guoying; Doeff, Marca] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Cheng, Lei] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Kunz, Martin; Tamura, Nobumichi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Cheng, L (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM leicheng@lbl.gov; mmdoeff@lbl.gov RI Chen, Wei/B-3045-2012; Cheng, Lei/F-9170-2014; OI Chen, Wei/0000-0002-1135-7721; Cheng, Lei/0000-0001-5498-9246; Doeff, Marca/0000-0002-2148-8047 FU Chemical Sciences, Geosciences, and Biosciences Division, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Materials Project Center (BES DOE Grant EDCBEE) FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies and the Chemical Sciences, Geosciences, and Biosciences Division, Office of Basic Energy Sciences of the U.S. Department of Energy under Contract DE-AC02-05CH11231. The Advanced Light Source is supported by the Director Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract DE-AC02-05CH11231. L.C., G.C, and M.D acknowledge illuminating discussion with Dr. Thomas Richardson. Prof. Lutgard De Jonghe is cordially acknowledged for the discussion on solid electrolytes. L.C. would like to acknowledge Dr. Miao Liu for assistance on data visualization, and Mr. James Wu and Mr. Yuyi Li for assistance with instruments. W.C. gratefully acknowledges the Materials Project Center (BES DOE Grant EDCBEE) for funding support. NR 51 TC 30 Z9 30 U1 34 U2 207 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JAN 28 PY 2015 VL 7 IS 3 BP 2073 EP 2081 DI 10.1021/am508111r PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CA1RG UT WOS:000348688700083 PM 25563572 ER PT J AU Hwang, S Kim, SM Bak, SM Cho, BW Chung, KY Lee, JY Chang, W Stach, EA AF Hwang, Sooyeon Kim, Seung Min Bak, Seong-Min Cho, Byun-Won Chung, Kyung Yoon Lee, Jeong Yong Chang, Wonyoung Stach, Eric A. TI Investigating the Local Degradation and Thermal Stability of Charged Ni-Based Cathode Materials through Real Time Electron Microscopy (vol 6, pg 15140, 2014) SO ACS APPLIED MATERIALS & INTERFACES LA English DT Correction C1 [Hwang, Sooyeon; Chung, Kyung Yoon; Lee, Jeong Yong] Korea Adv Inst Sci & Technol, Dept Mat Sci & Engn, Taejon 305701, South Korea. [Hwang, Sooyeon; Bak, Seong-Min; Cho, Byun-Won; Chang, Wonyoung] Korea Inst Sci & Technol, Ctr Energy Convergence, Seoul 136791, South Korea. [Stach, Eric A.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Kim, Seung Min] Korea Inst Sci & Technol, Carbon Convergence Mat Res Ctr, Wanju Gun 565905, South Korea. [Hwang, Sooyeon; Lee, Jeong Yong] Inst for Basic Sci Korea, Ctr Nanomat & Chem React, Taejon 305701, South Korea. RP Lee, JY (reprint author), Korea Adv Inst Sci & Technol, Dept Mat Sci & Engn, Taejon 305701, South Korea. RI Stach, Eric/D-8545-2011; Chung, Kyung Yoon/E-4646-2011; Bak, Seong Min/J-4597-2013 OI Stach, Eric/0000-0002-3366-2153; Chung, Kyung Yoon/0000-0002-1273-746X; NR 1 TC 0 Z9 0 U1 1 U2 11 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JAN 28 PY 2015 VL 7 IS 3 BP 2134 EP 2134 DI 10.1021/am508856p PG 1 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CA1RG UT WOS:000348688700090 ER PT J AU Golge, S Vlahovic, B Wojtsekhowski, B AF Golge, S. Vlahovic, B. Wojtsekhowski, B. TI High-intensity positron microprobe at the Thomas Jefferson National Accelerator Facility (vol 115, 234907, 2014) SO JOURNAL OF APPLIED PHYSICS LA English DT Correction C1 [Golge, S.; Vlahovic, B.] N Carolina Cent Univ, Durham, NC 27707 USA. [Wojtsekhowski, B.] Jefferson Lab, Newport News, VA 23606 USA. RP Golge, S (reprint author), N Carolina Cent Univ, Durham, NC 27707 USA. EM serkan.golge@nasa.gov OI Golge, Serkan/0000-0002-4236-0974 NR 1 TC 0 Z9 0 U1 0 U2 2 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JAN 28 PY 2015 VL 117 IS 4 AR 049902 DI 10.1063/1.4906775 PG 1 WC Physics, Applied SC Physics GA CA6DF UT WOS:000348998200076 ER PT J AU Gordiz, K Singh, DJ Henry, A AF Gordiz, Kiarash Singh, David J. Henry, Asegun TI Ensemble averaging vs. time averaging in molecular dynamics simulations of thermal conductivity SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID LATTICE; DECOMPOSITION; NANOWIRES; CRYSTALS; ARGON; SPACE AB In this report, we compare time averaging and ensemble averaging as two different methods for phase space sampling in molecular dynamics (MD) calculations of thermal conductivity. For the comparison, we calculate thermal conductivities of solid argon and silicon structures, using equilibrium MD. We introduce two different schemes for the ensemble averaging approach and show that both can reduce the total simulation time as compared to time averaging. It is also found that velocity rescaling is an efficient mechanism for phase space exploration. Although our methodology is tested using classical MD, the approaches used for generating independent trajectories may find their greatest utility in computationally expensive simulations such as first principles MD. For such simulations, where each time step is costly, time averaging can require long simulation times because each time step must be evaluated sequentially and therefore phase space averaging is achieved through sequential operations. On the other hand, with ensemble averaging, phase space sampling can be achieved through parallel operations, since each trajectory is independent. For this reason, particularly when using massively parallel architectures, ensemble averaging can result in much shorter simulation times (similar to 100-200X), but exhibits similar overall computational effort. (C) 2015 AIP Publishing LLC. C1 [Gordiz, Kiarash; Henry, Asegun] Georgia Inst Technol, George W Woodruff Sch Mech Engn, Atlanta, GA 30332 USA. [Singh, David J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Henry, Asegun] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA. RP Gordiz, K (reprint author), Georgia Inst Technol, George W Woodruff Sch Mech Engn, Atlanta, GA 30332 USA. EM kgordiz3@gatech.edu FU Department of Energy, BES, through the S3TEC Energy Frontier Research Center FX Work at ORNL was supported by the Department of Energy, BES, through the S3TEC Energy Frontier Research Center. NR 40 TC 6 Z9 6 U1 2 U2 16 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JAN 28 PY 2015 VL 117 IS 4 AR 045104 DI 10.1063/1.4906957 PG 8 WC Physics, Applied SC Physics GA CA6DF UT WOS:000348998200048 ER PT J AU Palla, KS Witus, LS Mackenzie, KJ Netirojjanakul, C Francis, MB AF Palla, Kanwal S. Witus, Leah S. Mackenzie, Katherine J. Netirojjanakul, Chawita Francis, Matthew B. TI Optimization and Expansion of a Site-Selective N-Methylpyridinium-4-carboxaldehyde-Mediated Transamination for Bacterially Expressed Proteins SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID N-TERMINAL MODIFICATION; PYROCOCCUS-HORIKOSHII; CHEMICAL LIGATION; ESCHERICHIA-COLI; AMINO-ACIDS; CONJUGATION; ENZYMES; SURFACE AB Site-selective bioconjugation methods are valuable because of their ability to confer new properties to proteins by the chemical attachment of specific functional groups. Well-defined bioconjugates obtained through these methods have found utility for the study of protein function and the creation of protein-based materials. We have previously reported a protein modification strategy to modify the N-terminus of peptides and proteins using N-methylpyridinium-4-carboxaldehyde benzenesulfonate (Rapoports salt, RS) as a transamination reagent, which oxidizes the N-terminal amino group to provide a uniquely reactive aldehyde or ketone. This functional handle can subsequently be modified with an alkoxyamine reagent of choice. Previous work had found glutamate terminal sequences to be highly reactive toward RS-mediated transamination. However, proteins of interest are often recombinantly expressed in E. coli, where the expression of a glutamate-terminal protein is rendered difficult because the N-terminal methionine derived from the start codon is not cleaved when Glu is in the second position. In this work, we describe a way to overcome this difficulty via the insertion of a Factor Xa proteolytic cleavage site to acquire the optimal glutamate residue at the N-terminus. Additionally, we present studies on alternative high-yielding sequences containing N-terminal residues that can be expressed directly. We have used site-directed mutagenesis to validate these findings on a model cellulase enzyme, an endoglucanase from the thermophilic Pyrococcus horikoshii. Activity assays performed with these mutants show that RS transamination and subsequent modification with alkoxyamines have no negative impact on cellulolytic ability. C1 [Palla, Kanwal S.; Witus, Leah S.; Mackenzie, Katherine J.; Netirojjanakul, Chawita; Francis, Matthew B.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Francis, Matthew B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Francis, MB (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM mbfrancis@berkeley.edu FU Energy Biosciences Institute at UC Berkeley; NSF [CHE 1059083]; NSF; Berkeley Chemical Biology Graduate Program (NRSA Training Grant) [1 T32 GMO66698]; Howard Hughes Medical Institute FX This work was funded by the Energy Biosciences Institute at UC Berkeley and the NSF (CHE 1059083). K.S.P, K.J.M., and L.S.W. were supported by a predoctoral fellowship from the NSF and from the Berkeley Chemical Biology Graduate Program (NRSA Training Grant No. 1 T32 GMO66698). C.N. was supported by a Howard Hughes Medical Institute International Student Research Fellowship. NR 34 TC 5 Z9 5 U1 2 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 28 PY 2015 VL 137 IS 3 BP 1123 EP 1129 DI 10.1021/ja509955n PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA CA1RU UT WOS:000348690100022 PM 25486267 ER PT J AU Mani, T Grills, DC Miller, JR AF Mani, Tomoyasu Grills, David C. Miller, John R. TI Vibrational Stark Effects To Identify Ion Pairing and Determine Reduction Potentials in Electrolyte-Free Environments SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID PULSE-RADIOLYSIS; SPECTROSCOPY; SOLVENTS; CATALYST; ANION AB A recently developed instrument for time-resolved infrared detection following pulse radiolysis has been used to measure the nu(C N) IR band of the radical anion of a CN-substituted fluorene in tetrahydrofuran. Specific vibrational frequencies can exhibit distinct frequency shifts due to ion pairing, which can be explained in the framework of the vibrational Stark effect. Measurements of the ratio of free ions and ion pairs in different electrolyte concentrations allowed us to obtain an association constant and free energy change for ion pairing. This new method has the potential to probe the geometry of ion pairing and allows the reduction potentials of molecules to be determined in the absence of electrolyte in an environment of low dielectric constant. C1 [Mani, Tomoyasu; Grills, David C.; Miller, John R.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Mani, T (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM tmani@bnl.gov; jrmiller@bnl.gov RI Mani, Tomoyasu/B-2241-2012; Grills, David/F-7196-2016 OI Mani, Tomoyasu/0000-0002-4125-5195; Grills, David/0000-0001-8349-9158 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98-CH10886]; Goldhaber Distinguished Fellowship from Brookhaven Science Associates FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences through Grant DE-AC02-98-CH10886, including use of the LEAF facility of the BNL Accelerator Center for Energy Research and the computer Cluster at the Center for Functional Nanomaterials. T.M. is grateful for the support by the Goldhaber Distinguished Fellowship from Brookhaven Science Associates. The authors thank Bobby H. Layne for technical assistance in LEAF experiments and Dr. Qin Wu for his assistance in quantum calculations. NR 26 TC 8 Z9 8 U1 1 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 28 PY 2015 VL 137 IS 3 BP 1136 EP 1140 DI 10.1021/ja512302c PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA CA1RU UT WOS:000348690100024 PM 25554821 ER PT J AU Colabello, DM Camino, FE Huq, A Hybertsen, M Khalifah, PG AF Colabello, Diane M. Camino, Fernando E. Huq, Ashfia Hybertsen, Mark Khalifah, Peter G. TI Charge Disproportionation in Tetragonal La2MoO5, a Small Band Gap Semiconductor Influenced by Direct Mo-Mo Bonding SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID BIOCTAHEDRAL MO-10 CLUSTERS; AUGMENTED-WAVE METHOD; CRYSTAL-STRUCTURE; ELECTRONIC-STRUCTURE; VALENCE PARAMETERS; PHYSICAL-PROPERTIES; MAGNETIC-PROPERTIES; STRUCTURAL TRENDS; RHENIUM DOUBLETS; COMPOUNDS R AB The structure of the novel compound La2MoO5 has been solved from powder X-ray and neutron diffraction data and belongs to the tetragonal space group P4/m (no. 83) with a = 12.6847(3) angstrom and c = 6.0568(2)angstrom and with Z = 8. It consists of equal proportions of bioctahedral (Mo2O10) and square prismatic (Mo2O8) dimers, both of which contain direct Mo-Mo bonds and are arranged in 1D chains. The Mo-Mo bond length in the Mo2O10 dimers is 2.684(8) angstrom, while there are two types of Mo2O8 dimers with Mo-Mo bonds lengths of 2.22(2) and 2.28(2) angstrom. Although the average Mo oxidation state in La2MoO5 is 4+, the very different Mo-Mo distances reflect the fact that the Mo2O10 dimers contain only Mo5+ (d(1)), while the prismatic Mo2O8 dimers only contain Mo3+ (d(3)), a result directly confirmed by density function theory calculations. This is due to the complete disproportionation of Mo4+, a phenomenon which has not previously been observed in solid-state compounds. La2MoO5 is diamagnetic, behavior which is not expected for a nonmetallic transition-metal oxide whose cation sites have an odd number of d-electrons. The resistivity displays the Arrhenius-type activated behavior expected for a semiconductor with a band gap of 0.5 eV, exhibiting an unusually small transport gap relative to other diamagnetic oxides. Diffuse reflectance studies indicate that La2MoO5 is a rare example of a stable oxide semiconductor with strong infrared absorbance. It is shown that the d-orbital splitting associated with the Mo2O8 and Mo2O10 dimeric units can be rationalized using simple molecular orbital bonding concepts. C1 [Colabello, Diane M.; Khalifah, Peter G.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Khalifah, Peter G.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11793 USA. [Camino, Fernando E.; Hybertsen, Mark] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11793 USA. [Huq, Ashfia] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37830 USA. RP Khalifah, PG (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. EM Peter.Khalifah@stonybrook.edu RI Huq, Ashfia/J-8772-2013; OI Huq, Ashfia/0000-0002-8445-9649; Hybertsen, Mark S/0000-0003-3596-9754 FU National Science Foundation [DMR-0955646]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357]; U.S. Department of Energy, Office of basic Energy Sciences [DE-AC02-98CH10886] FX This work was supported by the National Science Foundation grant no. DMR-0955646. The portion of this research conducted at Oak Ridge National Laboratory's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under contract no. DE-AC02-06CH11357. Research was carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of basic Energy Sciences, under contract no. DE-AC02-98CH10886. NR 74 TC 2 Z9 2 U1 7 U2 47 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 28 PY 2015 VL 137 IS 3 BP 1245 EP 1257 DI 10.1021/ja511218g PG 13 WC Chemistry, Multidisciplinary SC Chemistry GA CA1RU UT WOS:000348690100036 PM 25551640 ER PT J AU Friebel, D Louie, MW Bajdich, M Sanwald, KE Cai, Y Wise, AM Cheng, MJ Sokaras, D Weng, TC Alonso-Mori, R Davis, RC Bargar, JR Norskov, JK Nilsson, A Bell, AT AF Friebel, Daniel Louie, Mary W. Bajdich, Michal Sanwald, Kai E. Cai, Yun Wise, Anna M. Cheng, Mu-Jeng Sokaras, Dimosthenis Weng, Tsu-Chien Alonso-Mori, Roberto Davis, Ryan C. Bargar, John R. Norskov, Jens K. Nilsson, Anders Bell, Alexis T. TI Identification of Highly Active Fe Sites in (Ni,Fe)OOH for Electrocatalytic Water Splitting SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID OXYGEN EVOLUTION REACTION; ABSORPTION FINE-STRUCTURE; NICKEL-HYDROXIDE ELECTRODE; ALKALINE ELECTROLYTES; OXIDE-FILMS; ELECTROCHEMICAL-BEHAVIOR; NEUTRON-DIFFRACTION; OXIDATION CATALYSIS; COBALT OXIDES; GAMMA-FEOOH AB Highly active catalysts for the oxygen evolution reaction (OER) are required for the development of photoelectrochemical devices that generate hydrogen efficiently from water using solar energy. Here, we identify the origin of a 500-fold OER activity enhancement that can be achieved with mixed (Ni,Fe)oxyhydroxides (Ni1-xFexOOH) over their pure Ni and Fe parent compounds, resulting in one of the most active currently known OER catalysts in alkaline electrolyte. Operando X-ray absorption spectroscopy (XAS) using high energy resolution fluorescence detection (HERFD) reveals that Fe3+ in Ni1-xFexOOH occupies octahedral sites with unusually short Fe-O bond distances, induced by edge-sharing with surrounding [NiO6] octahedra. Using computational methods, we establish that this structural motif results in near optimal adsorption energies of OER intermediates and low overpotentials at Fe sites. By contrast, Ni sites in Ni1-xFexOOH are not active sites for the oxidation of water. C1 [Friebel, Daniel; Louie, Mary W.; Cai, Yun; Cheng, Mu-Jeng; Nilsson, Anders; Bell, Alexis T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. [Louie, Mary W.; Cai, Yun; Cheng, Mu-Jeng; Bell, Alexis T.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Friebel, Daniel; Bajdich, Michal; Sanwald, Kai E.; Norskov, Jens K.; Nilsson, Anders] SLAC Natl Accelerator Lab, SUNCAT Ctr Interface Sci & Catalysis, Menlo Pk, CA 94025 USA. [Sanwald, Kai E.] Tech Univ Munich, Dept Chem, D-85749 Garching, Germany. [Wise, Anna M.; Sokaras, Dimosthenis; Weng, Tsu-Chien; Davis, Ryan C.; Bargar, John R.; Nilsson, Anders] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Alonso-Mori, Roberto] SLAC Natl Accelerator Lab, Linac Coherent Lightsource, Menlo Pk, CA 94025 USA. RP Friebel, D (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, 1 Cyclotron Rd,Mail Stop 976, Berkeley, CA 94720 USA. EM dfriebel@slac.stanford.edu; alexbell@berkeley.edu RI Nilsson, Anders/E-1943-2011; Norskov, Jens/D-2539-2017; OI Nilsson, Anders/0000-0003-1968-8696; Norskov, Jens/0000-0002-4427-7728; Cheng, Mu-Jeng/0000-0002-8121-0485; Bell, Alexis/0000-0002-5738-4645 FU Office of Science of the U.S. Department of Energy [DE-SC0004993]; University of California; Ernest-Solvay-Stiftung; DOE [DE-AC02-05CH11231] FX This material is based upon work performed by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under Award Number DE-SC0004993. This research was partly carried out at the Stanford Synchrotron Radiation Lightsource, a National User Facility operated by Stanford University on behalf of the U.S. Department of Energy, Office of Basic Energy Sciences. We thank Lena Trotochaud, Harri Ali-Loytti and Lin Li for their assistance with data collection. We are grateful to Uwe Bergmann, Thomas Bligaard, Aleksandra Vojvodic and Lena Trotochaud for helpful discussions. We thank Tyler Matthews for assistance with sample preparation. M.W.L. was partially supported by the University of California President's Postdoctoral Fellowship. K.E.S. gratefully acknowledges the Ernest-Solvay-Stiftung for financial support. This research employed NERSC computational resources under DOE Contract No. DE-AC02-05CH11231. NR 72 TC 201 Z9 203 U1 123 U2 619 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 28 PY 2015 VL 137 IS 3 BP 1305 EP 1313 DI 10.1021/ja511559d PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA CA1RU UT WOS:000348690100042 PM 25562406 ER PT J AU Smith, BH Clark, MB Kuang, H Grieco, C Larsen, AV Zhu, CH Wang, C Hexemer, A Asbury, JB Janik, MJ Gomez, ED AF Smith, Brandon H. Clark, Michael B., Jr. Kuang, Hao Grieco, Christopher Larsen, Alec V. Zhu, Chenhui Wang, Cheng Hexemer, Alexander Asbury, John B. Janik, Michael J. Gomez, Enrique D. TI Controlling Polymorphism in Poly(3-Hexylthiophene) through Addition of Ferrocene for Enhanced Charge Mobilities in Thin-Film Transistors SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article DE organic field-effect transistors; charge transport; conjugated polymers; metallocenes; time-resolved infrared spectroscopy ID FIELD-EFFECT TRANSISTORS; ORGANOMETALLIC BLOCK-COPOLYMERS; MOLECULE ORGANIC SEMICONDUCTOR; LIGHT-EMITTING-DIODES; REGIOREGULAR POLY(3-HEXYLTHIOPHENE); HIGH-PERFORMANCE; PHOTOVOLTAIC MATERIALS; INFRARED-SPECTROSCOPY; CONJUGATED POLYMERS; MORPHOLOGY CONTROL AB Crystalline organic molecules often exhibit the ability to assemble into multiple crystal structures depending on the processing conditions. Exploiting this polymorphism to optimize molecular orbital overlap between adjacent molecules in the unit lattice is an effective method for improving charge transport within the material. In this study, grazing incident X-ray diffraction was employed to demonstrate the formation of tighter - stacking poly(3-hexylthiophene-2,5-diyl) polymorphs in films spin coated from ferrocene-containing solutions. As a result, the addition of ferrocene to casting solutions yields thin-film transistors which exhibit approximately three times higher source-drain currents and charge mobilities than neat polymer devices. Nevertheless, XPS depth profiling and NMR analyses of the active layer reveal that all ferrocene is removed during the spin coating process, which may be an essential factor to achieve high mobilities. Such insights gleaned from ferrocene/poly(3-hexylthiophene-2,5-diyl) mixtures can serve as a template for selection and optimization of other small molecule/polymer systems with greater baseline charge mobilities. C1 [Smith, Brandon H.; Kuang, Hao; Janik, Michael J.; Gomez, Enrique D.] Penn State Univ, Dept Chem Engn, University Pk, PA 16802 USA. [Clark, Michael B., Jr.] Dow Chem Co USA, Collegeville, PA 19426 USA. [Grieco, Christopher; Larsen, Alec V.; Asbury, John B.] Penn State Univ, Dept Chem, University Pk, PA 16802 USA. [Zhu, Chenhui; Wang, Cheng; Hexemer, Alexander] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Smith, BH (reprint author), Penn State Univ, Dept Chem Engn, University Pk, PA 16802 USA. EM edg12@psu.edu RI Wang, Cheng/A-9815-2014 FU Center for Flexible Electronics at the Pennsylvania State University; Dow Chemical Company; U.S. Department of Energy [DE-AC02-05CH11231] FX This work was funded by the Center for Flexible Electronics at the Pennsylvania State University and the Dow Chemical Company. The Advanced Light Source is an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Lawrence Berkeley National Laboratory and supported by the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The authors also gratefully acknowledge T. Le and C. Guo's assistance with GIXRD measurements, Dr. Y. Lee and P. Zhan's help with NMR measurements, Dr. Kyle Bishop for use of the DLS, and the assistance of the Pennsylvania State University Materials Characterization Laboratory and Nanofabrication Laboratory staff. NR 105 TC 7 Z9 7 U1 11 U2 67 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD JAN 28 PY 2015 VL 25 IS 4 BP 542 EP 551 DI 10.1002/adfm.201403089 PG 10 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CA4EH UT WOS:000348856500005 ER PT J AU Bjorgaard, JA Kuzmenko, V Velizhanin, KA Tretiak, S AF Bjorgaard, J. A. Kuzmenko, V. Velizhanin, K. A. Tretiak, S. TI Solvent effects in time-dependent self-consistent field methods. I. Optical response calculations SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID DENSITY-FUNCTIONAL THEORY; POLARIZABLE CONTINUUM MODEL; ELECTRONIC EXCITATION-ENERGIES; CHARGE-TRANSFER STATES; CCSD-PCM METHOD; EXCITED-STATES; SOLVATION MODELS; MOLECULAR-DYNAMICS; HARTREE-FOCK; NONEMPIRICAL CALCULATIONS AB We implement and examine three excited state solvent models in time-dependent self-consistent field methods using a consistent formalism which unambiguously shows their relationship. These are the linear response, state specific, and vertical excitation solvent models. Their effects on energies calculated with the equivalent of COSMO/CIS/AM1 are given for a set of test molecules with varying excited state charge transfer character. The resulting solvent effects are explained qualitatively using a dipole approximation. It is shown that the fundamental differences between these solvent models are reflected by the character of the calculated excitations. (C) 2015 AIP Publishing LLC. C1 [Bjorgaard, J. A.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Div Theoret, Los Alamos, NM 87545 USA. [Kuzmenko, V.] Natl Tech Univ Ukraine, KPI, UA-03056 Kiev, Ukraine. [Velizhanin, K. A.; Tretiak, S.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Tretiak, S.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. RP Bjorgaard, JA (reprint author), Los Alamos Natl Lab, Ctr Nonlinear Studies, Div Theoret, Los Alamos, NM 87545 USA. EM jbjorgaard@lanl.gov; serg@lanl.gov RI Velizhanin, Kirill/C-4835-2008; Tretiak, Sergei/B-5556-2009 OI Tretiak, Sergei/0000-0001-5547-3647 FU U.S. Department of Energy through the Los Alamos National Laboratory (LANL) LDRD Program; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396]; Center for Nonlinear Studies (CNLS); Center for Integrated Nanotechnology (CINT) at LANL FX We acknowledge support of the U.S. Department of Energy through the Los Alamos National Laboratory (LANL) LDRD Program. LANL is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. We also acknowledge support of the Center for Nonlinear Studies (CNLS) and the Center for Integrated Nanotechnology (CINT) at LANL. We would like acknowledge Giovanni Scalmani for useful comments on the manuscript. NR 93 TC 5 Z9 5 U1 2 U2 17 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JAN 28 PY 2015 VL 142 IS 4 AR 044103 DI 10.1063/1.4905828 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CA6JH UT WOS:000349018100006 PM 25637965 ER PT J AU Buckingham, GT Ormond, TK Porterfield, JP Hemberger, P Kostko, O Ahmed, M Robichaud, DJ Nimlos, MR Daily, JW Ellison, GB AF Buckingham, Grant T. Ormond, Thomas K. Porterfield, Jessica P. Hemberger, Patrick Kostko, Oleg Ahmed, Musahid Robichaud, David J. Nimlos, Mark R. Daily, John W. Ellison, G. Barney TI The thermal decomposition of the benzyl radical in a heated micro-reactor. I. Experimental findings SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID ULTRAVIOLET PHOTOELECTRON-SPECTROSCOPY; SUPERSONIC JET; GAS-PHASE; PHOTOIONIZATION; SPECTRUM; CYCLOPENTADIENYL; PHENYLCARBENE; FULVENALLENE; GENERATION; PYROLYSIS AB The pyrolysis of the benzyl radical has been studied in a set of heated micro-reactors. A combination of photoionization mass spectrometry (PIMS) and matrix isolation infrared (IR) spectroscopy has been used to identify the decomposition products. Both benzyl bromide and ethyl benzene have been used as precursors of the parent species, C6H5CH2, as well as a set of isotopically labeled radicals: C6H5CD2, C6D5CH2, and (C6H5CH2)-C-13. The combination of PIMS and IR spectroscopy has been used to identify the earliest pyrolysis products from benzyl radical as: C5H4=C=CH2, H atom, C5H4-C CH, C5H5, HCCCH2, and HC CH. Pyrolysis of the C6H5CD2, C6D5CH2, and (C6H5CH2)-C-13 benzyl radicals produces a set of methyl radicals, cyclopentadienyl radicals, and benzynes that are not predicted by a fulvenallene pathway. Explicit PIMS searches for the cycloheptatrienyl radical were unsuccessful, there is no evidence for the isomerization of benzyl and cycloheptatrienyl radicals: C6H5CH2 (sic) C7H7. These labeling studies suggest that there must be other thermal decomposition routes for the C6H5CH2 radical that differ from the fulvenallene pathway. (C) 2015 AIP Publishing LLC. C1 [Buckingham, Grant T.; Ormond, Thomas K.; Porterfield, Jessica P.; Ellison, G. Barney] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. [Buckingham, Grant T.; Ormond, Thomas K.; Robichaud, David J.; Nimlos, Mark R.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Hemberger, Patrick] Paul Scherrer Inst, Mol Dynam Grp, CH-5232 Villigen, Switzerland. [Kostko, Oleg; Ahmed, Musahid] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Daily, John W.] Univ Colorado, Dept Mech Engn, Ctr Combust & Environm Res, Boulder, CO 80309 USA. RP Buckingham, GT (reprint author), Univ Colorado, Dept Chem & Biochem, Campus Box 215, Boulder, CO 80309 USA. RI Kostko, Oleg/B-3822-2009; Ahmed, Musahid/A-8733-2009; Hemberger, Patrick/E-7909-2017 OI Kostko, Oleg/0000-0003-2068-4991; Hemberger, Patrick/0000-0002-1251-4549 FU National Science Foundation [CHE-1112466, CBET-1403979]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy through the Chemical Sciences Division [DE-AC02-05CH11231]; United States Department of Energy's Bioenergy Technology Office [DE-AC36-99GO10337]; National Renewable Energy Laboratory; Swiss Federal Office for Energy (BFE) [101969/152433] FX This paper has been strengthened by many helpful discussions with Dr. Hans Heinrich Carstensen. We would like to acknowledge support from the National Science Foundation (Nos. CHE-1112466 and CBET-1403979) for J.W.D. and G.B.E. M.A., O.K., and the Advanced Light Source are supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 through the Chemical Sciences Division. M.R.N. and D.J.R. are supported by United States Department of Energy's Bioenergy Technology Office, under Contract No. DE-AC36-99GO10337 with the National Renewable Energy Laboratory. P.H. was supported by the Swiss Federal Office for Energy (BFE Contract No. 101969/152433). Some of the experimental work was carried out at the x04db (VUV) beamline of the Swiss Light Source located at the Paul Scherrer Instititut (PSI). NR 69 TC 6 Z9 6 U1 4 U2 45 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JAN 28 PY 2015 VL 142 IS 4 AR 044307 DI 10.1063/1.4906156 PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CA6JH UT WOS:000349018100028 PM 25637987 ER PT J AU Yu, HG AF Yu, Hua-Gen TI Multi-layer Lanczos iteration approach to calculations of vibrational energies and dipole transition intensities for polyatomic molecules SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID DISCRETE VARIABLE REPRESENTATION; FILTER-DIAGONALIZATION METHOD; RESIDUE-GENERATION METHOD; SPECTRAL TRANSFORM METHOD; QUANTUM-DYNAMICS; TETRAATOMIC MOLECULES; VARIATIONAL CALCULATIONS; ROVIBRATIONAL ENERGIES; RESONANCE ENERGIES; PROPAGATION METHOD AB We report a rigorous full dimensional quantum dynamics algorithm, the multi-layer Lanczos method, for computing vibrational energies and dipole transition intensities of polyatomic molecules without any dynamics approximation. The multi-layer Lanczos method is developed by using a few advanced techniques including the guided spectral transform Lanczos method, multi-layer Lanczos iteration approach, recursive residue generation method, and dipole-wavefunction contraction. The quantum molecular Hamiltonian at the total angular momentum J = 0 is represented in a set of orthogonal polyspherical coordinates so that the large amplitude motions of vibrations are naturally described. In particular, the algorithm is general and problem-independent. An application is illustrated by calculating the infrared vibrational dipole transition spectrum of CH4 based on the ab initio T8 potential energy surface of Schwenke and Partridge [Spectrochimica Acta, Part A 57, 887 (2001)] and the low-order truncated ab initio dipole moment surfaces of Yurchenko et al. [J. Mol. Spectrosc. 291, 69 (2013)]. A comparison with experiments is made. The algorithm is also applicable for Raman polarizability active spectra. (C) 2015 AIP Publishing LLC. C1 Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Yu, HG (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM hgy@bnl.gov RI Yu, Hua-Gen/N-7339-2015 FU U.S. Department of Energy [DE-AC02-98CH10886]; Division of Chemical Sciences, Office of Basic Energy Sciences; National Energy Research Scientific Computing Center (NERSC) [AC02-05CH11231] FX This work was performed at Brookhaven National Laboratory under Contract No. DE-AC02-98CH10886 with the U.S. Department of Energy and supported by its Division of Chemical Sciences, Office of Basic Energy Sciences. It also used the resource at the National Energy Research Scientific Computing Center (NERSC) under Contract No. DE-AC02-05CH11231. The author thanks Professor Sergey Yurchenko for providing the FORTRAN code of dipole moment surfaces. NR 117 TC 4 Z9 4 U1 3 U2 17 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JAN 28 PY 2015 VL 142 IS 4 AR 044106 DI 10.1063/1.4906492 PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CA6JH UT WOS:000349018100009 PM 25637968 ER PT J AU Limmer, SJ Medlin, DL Siegal, MP Hekmaty, M Lensch-Falk, JL Erickson, K Pillars, J Yelton, WG AF Limmer, Steven J. Medlin, Douglas L. Siegal, Michael P. Hekmaty, Michelle Lensch-Falk, Jessica L. Erickson, Kristopher Pillars, Jamin Yelton, W. Graham TI Using galvanostatic electroforming of Bi1-xSbx nanowires to control composition, crystallinity, and orientation SO JOURNAL OF MATERIALS RESEARCH LA English DT Article ID THERMOELECTRIC FIGURE; HIGH-DENSITY; ARRAYS; ELECTRODEPOSITION; GROWTH; MERIT; SIZE AB Using galvanostatic pulse deposition, we studied the factors influencing the quality of electroformed Bi1-xSbx nanowires with respect to composition, crystallinity, and preferred orientation for high thermoelectric performance. Two nonaqueous baths with different Sb salts were investigated. The Sb salts used played a major role in both crystalline quality and preferred orientations. Nanowire arrays electroformed using an SbI3-based chemistry were polycrystalline with no preferred orientation, whereas arrays electroformed from an SbCl3-based chemistry were strongly crystallographically textured with the desired trigonal orientation for optimal thermoelectric performance. From the SbCl3 bath, the electroformed nanowire arrays were optimized to have nanocompositional uniformity, with a nearly constant composition along the nanowire length. Nanowires harvested from the center of the array had an average composition of Bi0.75Sb0.25. However, the nanowire compositions were slightly enriched in Sb in a small region near the edges of the array, with the composition approaching Bi0.70Sb0.30. C1 [Limmer, Steven J.; Siegal, Michael P.; Pillars, Jamin; Yelton, W. Graham] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Medlin, Douglas L.; Hekmaty, Michelle; Lensch-Falk, Jessica L.; Erickson, Kristopher] Sandia Natl Labs, Livermore, CA 94551 USA. RP Yelton, WG (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM wgyelto@sandia.gov OI Limmer, Steven/0000-0001-6588-372X FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors wish to thank Donald L. Overmyer for assistance with film deposition and x-ray diffraction. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 22 TC 2 Z9 2 U1 1 U2 11 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 EI 2044-5326 J9 J MATER RES JI J. Mater. Res. PD JAN 28 PY 2015 VL 30 IS 2 BP 164 EP 169 DI 10.1557/jmr.2014.354 PG 6 WC Materials Science, Multidisciplinary SC Materials Science GA CA8DQ UT WOS:000349147200002 ER PT J AU Rochford, C Limmer, SJ Howell, SW Beechem, TE Siegal, MP AF Rochford, C. Limmer, S. J. Howell, S. W. Beechem, T. E. Siegal, M. P. TI Planarized arrays of aligned, untangled multiwall carbon nanotubes with Ohmic back contacts SO JOURNAL OF MATERIALS RESEARCH LA English DT Article ID CHEMICAL-VAPOR-DEPOSITION; LOW-TEMPERATURE GROWTH; FIELD-EMISSION; NANOWIRE ARRAYS; TEMPLATE; DENSITY; CVD; FABRICATION; TUBE; SI AB Vertically aligned, untangled planarized arrays of multiwall carbon nanotubes (MWNTs) with Ohmic back contacts were grown in nanopore templates on arbitrary substrates. The templates were prepared by sputter depositing Nd-doped Al films onto W-coated substrates, followed by anodization to form an aluminum oxide nanopore array. The W underlayer helps eliminate the aluminum oxide barrier that typically occurs at the nanopore bottoms by instead forming a thin WO3 layer. The WO3 can be selectively etched to enable electrodeposition of Co catalysts with control over the Co site density. This led to control of the site density of MWNTs grown by thermal chemical vapor deposition, with W also serving as a back electrical contact. Ohmic contact to MWNTs was confirmed, even following ultrasonic cutting of the entire array to a uniform height. C1 [Rochford, C.; Limmer, S. J.; Howell, S. W.; Beechem, T. E.; Siegal, M. P.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Rochford, C (reprint author), Sandia Natl Labs, Albuquerque, NM 87185 USA. EM crochfo@sandia.gov OI Rochford, Caitlin/0000-0002-5070-209X; Limmer, Steven/0000-0001-6588-372X FU Laboratory Directed Research and Development program at Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors thank Lyle Brunke for assistance with sputter depositions and Anthony McDonald for assistance in Raman spectroscopy measurements. This work is supported by the Laboratory Directed Research and Development program at Sandia National Laboratories. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 30 TC 0 Z9 0 U1 0 U2 20 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 EI 2044-5326 J9 J MATER RES JI J. Mater. Res. PD JAN 28 PY 2015 VL 30 IS 2 BP 315 EP 322 DI 10.1557/jmr.2014.359 PG 8 WC Materials Science, Multidisciplinary SC Materials Science GA CA8DQ UT WOS:000349147200018 ER PT J AU Keating, T Cook, RL Hankin, AM Jau, YY Biedermann, GW Deutsch, IH AF Keating, Tyler Cook, Robert L. Hankin, Aaron M. Jau, Yuan-Yu Biedermann, Grant W. Deutsch, Ivan H. TI Robust quantum logic in neutral atoms via adiabatic Rydberg dressing SO PHYSICAL REVIEW A LA English DT Article AB We study a scheme for implementing a controlled-Z (CZ) gate between two neutral-atom qubits based on the Rydberg blockade mechanism in a manner that is robust to errors caused by atomic motion. By employing adiabatic dressing of the ground electronic state, we can protect the gate from decoherence due to random phase errors that typically arise because of atomic thermal motion. In addition, the adiabatic protocol allows for a Doppler-free configuration that involves counterpropagating lasers in a sigma(+)/sigma(-) orthogonal polarization geometry that further reduces motional errors due to Doppler shifts. The residual motional error is dominated by dipole-dipole forces acting on doubly excited Rydberg atoms when the blockade is imperfect. For reasonable parameters, with qubits encoded into the clock states of Cs-133, we predict that our protocol could produce a CZ gate in < 10 mu s with error probability on the order of 10(-3). C1 [Keating, Tyler; Cook, Robert L.; Hankin, Aaron M.; Jau, Yuan-Yu; Biedermann, Grant W.; Deutsch, Ivan H.] Univ New Mexico, Ctr Quantum Informat & Control CQuIC, Albuquerque, NM 87131 USA. [Keating, Tyler; Cook, Robert L.; Hankin, Aaron M.; Biedermann, Grant W.; Deutsch, Ivan H.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Hankin, Aaron M.; Jau, Yuan-Yu; Biedermann, Grant W.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Keating, T (reprint author), Univ New Mexico, Ctr Quantum Informat & Control CQuIC, Albuquerque, NM 87131 USA. RI Deutsch, Ivan/D-1882-2009 OI Deutsch, Ivan/0000-0002-1733-5750 FU Laboratory Directed Research and Development program at Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the Laboratory Directed Research and Development program at Sandia National Laboratories. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 27 TC 12 Z9 12 U1 3 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD JAN 28 PY 2015 VL 91 IS 1 AR 012337 DI 10.1103/PhysRevA.91.012337 PG 9 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CB0TN UT WOS:000349340300003 ER PT J AU Chen, L Zhang, L Kang, QJ Viswanathan, HS Yao, J Tao, WQ AF Chen, Li Zhang, Lei Kang, Qinjun Viswanathan, Hari S. Yao, Jun Tao, Wenquan TI Nanoscale simulation of shale transport properties using the lattice Boltzmann method: permeability and diffusivity SO SCIENTIFIC REPORTS LA English DT Article ID GAS-FLOW; POROUS-MEDIA; PORES; MODEL; MULTISCALE; KEROGEN AB Porous structures of shales are reconstructed using the markov chain monte carlo (MCMC) method based on scanning electron microscopy (SEM) images of shale samples from Sichuan Basin, China. Characterization analysis of the reconstructed shales is performed, including porosity, pore size distribution, specific surface area and pore connectivity. The lattice Boltzmann method (LBM) is adopted to simulate fluid flow and Knudsen diffusion within the reconstructed shales. Simulation results reveal that the tortuosity of the shales is much higher than that commonly employed in the Bruggeman equation, and such high tortuosity leads to extremely low intrinsic permeability. Correction of the intrinsic permeability is performed based on the dusty gas model (DGM) by considering the contribution of Knudsen diffusion to the total flow flux, resulting in apparent permeability. The correction factor over a range of Knudsen number and pressure is estimated and compared with empirical correlations in the literature. For the wide pressure range investigated, the correction factor is always greater than 1, indicating Knudsen diffusion always plays a role on shale gas transport mechanisms in the reconstructed shales. Specifically, we found that most of the values of correction factor fall in the slip and transition regime, with no Darcy flow regime observed. C1 [Chen, Li; Tao, Wenquan] Xi An Jiao Tong Univ, Sch Energy & Power Engn, Key Lab Thermofluid Sci & Engn MOE, Xian 710049, Shaanxi, Peoples R China. [Chen, Li; Kang, Qinjun; Viswanathan, Hari S.] Los Alamos Natl Lab, Earth & Environm Sci Div, Los Alamos, NM 87545 USA. [Zhang, Lei; Yao, Jun] China Univ Petr, Sch Petr Engn, Qingdao 266580, Shandong, Peoples R China. RP Kang, QJ (reprint author), China Univ Petr, Sch Petr Engn, Qingdao 266580, Shandong, Peoples R China. EM qkang@lanl.gov RI Chen, Li/P-4886-2014; Kang, Qinjun/A-2585-2010 OI Chen, Li/0000-0001-7956-3532; Kang, Qinjun/0000-0002-4754-2240 FU LANL's LDRD Program; Institutional Computing Program; National Nature Science Foundation of China [51406145, 51136004]; NNSFC international-joint key project [51320105004] FX The authors acknowledge the support of LANL's LDRD Program, Institutional Computing Program, National Nature Science Foundation of China (51406145 and 51136004) and NNSFC international-joint key project (51320105004). Li Chen appreciates the helpful discussions with Doctor H. Sun from China University of Petroleum, Qingdao. NR 42 TC 27 Z9 27 U1 28 U2 135 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 28 PY 2015 VL 5 AR 8089 DI 10.1038/srep08089 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AZ8AG UT WOS:000348436500003 PM 25627247 ER PT J AU Uysal, A Zhou, H Feng, G Lee, SS Li, S Cummings, PT Fulvio, PF Dai, S McDonough, JK Gogotsi, Y Fenter, P AF Uysal, Ahmet Zhou, Hua Feng, Guang Lee, Sang Soo Li, Song Cummings, Peter T. Fulvio, Pasquale F. Dai, Sheng McDonough, John K. Gogotsi, Yury Fenter, Paul TI Interfacial ionic 'liquids': connecting static and dynamic structures SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE ionic liquid; supercapacitor; electric double layer; epitaxial graphene; x-ray reflectivity; RTIL; interfacial structure ID ELECTRIC DOUBLE-LAYER; X-RAY REFLECTIVITY; ROOM-TEMPERATURE; DIFFERENTIAL CAPACITANCE; MOLECULAR-DYNAMICS; HYSTERESIS; SURFACE; METAL; WATER; SUPERCAPACITORS AB It is well known that room temperature ionic liquids (RTILs) often adopt a charge-separated layered structure, i.e. with alternating cation- and anion-rich layers, at electrified interfaces. However, the dynamic response of the layered structure to temporal variations in applied potential is not well understood. We used in situ, real-time x-ray reflectivity to study the potential-dependent electric double layer (EDL) structure of an imidazolium-based RTIL on charged epitaxial graphene during potential cycling as a function of temperature. The results suggest that the graphene-RTIL interfacial structure is bistable in which the EDL structure at any intermediate potential can be described by the combination of two extreme-potential structures whose proportions vary depending on the polarity and magnitude of the applied potential. This picture is supported by the EDL structures obtained by fully atomistic molecular dynamics simulations at various static potentials. The potential-driven transition between the two structures is characterized by an increasing width but with an approximately fixed hysteresis magnitude as a function of temperature. The results are consistent with the coexistence of distinct anion-and cation-adsorbed structures separated by an energy barrier (similar to 0.15 eV). C1 [Uysal, Ahmet; Lee, Sang Soo; Fenter, Paul] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Zhou, Hua] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Feng, Guang; Li, Song; Cummings, Peter T.] Vanderbilt Univ, Dept Chem & Biomol Engn, Nashville, TN 37235 USA. [Fulvio, Pasquale F.; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [McDonough, John K.; Gogotsi, Yury] Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. [McDonough, John K.; Gogotsi, Yury; Fenter, Paul] Drexel Univ, AJ Drexel Nanomat Inst, Philadelphia, PA 19104 USA. RP Feng, G (reprint author), Vanderbilt Univ, Dept Chem & Biomol Engn, Nashville, TN 37235 USA. EM ahmet@anl.gov; gfeng@hust.edu.cn; pfenter@anl.gov RI Dai, Sheng/K-8411-2015; Feng, Guang/D-8989-2011; OI Dai, Sheng/0000-0002-8046-3931; Feng, Guang/0000-0001-6659-9181 FU Fluid Interface Reactions, Structures and Transport (FIRST) Center; Energy Frontier Research Center - US Department of Energy, Office of Science, Office of Basic Energy Sciences; DOE-SC-BES [DE-AC02-06CH11357]; DOE-SC [DE-AC02-05CH11231]; Palmetto cluster at Clemson University FX We thank Tim T Fister, Francesco Bellucci and Nouamane Laanait for technical and intellectual support at various stages of the experiments. We also thank Brian Skinner for valuable discussions. This work was supported as part of the Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences. Use of the beamlines 6ID, 12ID and 33ID at the Advanced Photon Source was supported by DOE-SC-BES under Contract DE-AC02-06CH11357 to UChicago Argonne, LLC as operator of Argonne National Laboratory. This research used computational resources of the National Energy Research Scientific Computing Center, which is supported by DOE-SC under Contract No DE-AC02-05CH11231, and the Palmetto cluster at Clemson University. NR 55 TC 18 Z9 18 U1 11 U2 130 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD JAN 28 PY 2015 VL 27 IS 3 AR 032101 DI 10.1088/0953-8984/27/3/032101 PG 9 WC Physics, Condensed Matter SC Physics GA AZ8WX UT WOS:000348493400001 PM 25475119 ER PT J AU Abdel-Naby, SA Pindzola, MS Colgan, J AF Abdel-Naby, Shahin A. Pindzola, M. S. Colgan, J. TI Differential cross section for the double photoionization of Mg SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article DE photoionization; differential; correlations ID PHOTO-DOUBLE IONIZATION; HELIUM; SINGLE; GAMMA AB The time-dependent close-coupling (TDCC) method is used to calculate the energy and angle triple differential cross section for the double photoionization of Mg(3s(2)) at a photon energy of 55.49 eV to compare with recent converged close-coupling (CCC) calculations and in support of recent experiments at ELETTRA. Comparisons are made between the TDCC, CCC, and experimental results for equal energy sharing at scattering angles of 0 degrees, 30 degrees, and 60 degrees, and for unequal energy sharing at 0 degrees and 30 degrees. Comparisons are made between the TDCC and CCC results for equal and unequal energy sharing at 90 degrees. In addition, TDCC, CCC, and experimental results are compared for complex scattering amplitudes and the TDCC method is used to calculate single energy differential cross sections at photon energies of 30, 35, 40, 45, and 55.49 eV. Although there are scattering angles in the triple differential cross sections at 55.49 eV at which the TDCC, CCC, and experimental results are quite different, the overall agreement between the theories and experiment is reasonable for such small cross sections. C1 [Abdel-Naby, Shahin A.; Pindzola, M. S.] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. [Abdel-Naby, Shahin A.] Beni Suef Univ, Dept Phys, Bani Suwayf, Egypt. [Colgan, J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Abdel-Naby, SA (reprint author), Auburn Univ, Dept Phys, Auburn, AL 36849 USA. EM abdelsh@auburn.edu FU US Department of Energy; US National Science Foundation FX We would like to thank A Kheifets and L Avaldi for sending their theoretical results and experimental measurements. This work was supported in part by grants from the US Department of Energy and the US National Science Foundation. Computational work was carried out at the National Energy Research Scientific Computing Center in Oakland, California, and the National Institute for Computational Sciences in Oak Ridge, Tennessee. NR 33 TC 1 Z9 1 U1 1 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 EI 1361-6455 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD JAN 28 PY 2015 VL 48 IS 2 AR 025204 DI 10.1088/0953-4075/48/2/025204 PG 8 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA AX7PU UT WOS:000347108300009 ER PT J AU Kraft, ML Frisz, JF Klitzing, HA Wilson, RL Yeager, A Lizunov, V Zimmerberg, JJ Weber, PK AF Kraft, Mary L. Frisz, Jessica F. Klitzing, Haley A. Wilson, Robert L. Yeager, Ashley Lizunov, Vladimir Zimmerberg, Joshua J. Weber, Peter K. TI Investigating the Mechanisms of Non-Random Sphingolipid Organization in the Plasma Membranes of Fibroblast Cells SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Kraft, Mary L.; Yeager, Ashley] Univ Illinois, Chem & Biomol Engr, Urbana, IL 61801 USA. [Frisz, Jessica F.; Klitzing, Haley A.; Wilson, Robert L.] Univ Illinois, Chem, Urbana, IL 61801 USA. [Lizunov, Vladimir; Zimmerberg, Joshua J.] Eunice Kennedy Shriver Natl Inst Child Hlth & Hum, Program Phys Biol, Bethesda, MD USA. [Weber, Peter K.] Lawrence Livermore Natl Lab, Glenn T Seaborg Inst, Livermore, CA USA. NR 0 TC 0 Z9 0 U1 1 U2 1 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 4-Subg BP 1A EP 1A PG 1 WC Biophysics SC Biophysics GA CO9DB UT WOS:000359471700005 ER PT J AU Kent, MS Akgun, B Nanda, H Pirrone, GF Engen, J AF Kent, Michael S. Akgun, Bulent Nanda, Hirsh Pirrone, Gregory F. Engen, John TI Combining Neutron Reflectivity and Hydrogen Deuterium Exchange Mass Spectrometry to Resolve Structural details of Membrane Associated Proteins SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Kent, Michael S.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Akgun, Bulent] Bogazici Univ, Chem, TR-80815 Bebek, Turkey. [Nanda, Hirsh] Natl Inst Stand & Technol, Gaithersburg, MD 20899 USA. [Pirrone, Gregory F.; Engen, John] Northeastern Univ, Boston, MA 02115 USA. RI Akgun, Bulent/H-3798-2011 NR 0 TC 0 Z9 0 U1 3 U2 4 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 77-Plat BP 16A EP 16A PG 1 WC Biophysics SC Biophysics GA CO9DB UT WOS:000359471700078 ER PT J AU Chapman, EG Costantino, DA Rabe, JL Moon, SL Nix, JC Wilusz, J Kieft, JS AF Chapman, Erich G. Costantino, David A. Rabe, Jennifer L. Moon, Stephanie L. Nix, Jay C. Wilusz, Jeffrey Kieft, Jeffrey S. TI How Flaviviruses use a Unique 'Slipknot-Like' Structure to Mechanically Confound a Cellular Exonuclease and Produce Pathogenic RNA SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Chapman, Erich G.; Rabe, Jennifer L.] Univ Colorado, Sch Med, Biochem & Mol Genet, Aurora, CO USA. [Costantino, David A.; Kieft, Jeffrey S.] HHMI, Biochem & Mol Genet, Aurora, CO USA. [Costantino, David A.; Kieft, Jeffrey S.] Univ Colorado, Sch Med, Aurora, CO USA. [Moon, Stephanie L.; Wilusz, Jeffrey] Colorado State Univ, Dept Microbiol Immunol & Pathol, Ft Collins, CO 80523 USA. [Nix, Jay C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Mol Biol Consortium, Berkeley, CA 94720 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 129-Plat BP 27A EP 27A PG 1 WC Biophysics SC Biophysics GA CO9DB UT WOS:000359471700130 ER PT J AU Nickels, JD Ohl, M Cheng, XL Stanley, C Heberle, F Standaert, R Katsaras, J AF Nickels, Jonathan D. Ohl, Michael Cheng, Xiaolin Stanley, Christopher Heberle, Frederick Standaert, Robert Katsaras, John TI Experiment and Simulation Reveal the Bending Properties of Nanoscopic Lipid Domains SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Nickels, Jonathan D.; Cheng, Xiaolin; Standaert, Robert; Katsaras, John] Univ Tennessee, Oak Ridge Natl Lab, Oak Ridge, TN USA. [Ohl, Michael] Julich Ctr Neutron Sci, Oak Ridge Natl Lab, Oak Ridge, TN USA. [Stanley, Christopher; Heberle, Frederick] Oak Ridge Natl Lab, Oak Ridge, TN USA. RI Standaert, Robert/D-9467-2013; Nickels, Jonathan/I-1913-2012 OI Standaert, Robert/0000-0002-5684-1322; Nickels, Jonathan/0000-0001-8351-7846 NR 0 TC 1 Z9 1 U1 0 U2 1 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 152-Plat BP 31A EP 31A PG 1 WC Biophysics SC Biophysics GA CO9DB UT WOS:000359471700153 ER PT J AU Swingle, KL Adams, PG Montano, GA AF Swingle, Kirstie L. Adams, Peter G. Montano, Gabriel A. TI Using Lipopolysaccharides to Create 3-D Multicomponent Biomimetic Membranes on Solid Supports SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Swingle, Kirstie L.; Adams, Peter G.; Montano, Gabriel A.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Albuquerque, NM USA. NR 0 TC 0 Z9 0 U1 2 U2 2 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 156-Plat BP 32A EP 32A PG 1 WC Biophysics SC Biophysics GA CO9DB UT WOS:000359471700157 ER PT J AU Meddens, MBM Liu, S James, CD Lidke, KA AF Meddens, Marjolein B. M. Liu, Sheng James, Conrad D. Lidke, Keith A. TI Reflected Beam Light-Sheet Microscopy for Whole-Cell 3D Super-Resolution Imaging SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Meddens, Marjolein B. M.; Liu, Sheng; Lidke, Keith A.] Univ New Mexico, Phys & Astron, Albuquerque, NM 87131 USA. [James, Conrad D.] Sandia Natl Labs, Albuquerque, NM 87185 USA. NR 0 TC 0 Z9 0 U1 2 U2 2 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 169-Plat BP 35A EP 35A PG 1 WC Biophysics SC Biophysics GA CO9DB UT WOS:000359471700170 ER PT J AU Shrestha, U Bhowmik, D Perera, SMDC Chawla, U Struts, AV Graziano, V Qian, S Heller, WT Brown, MF Chu, XQ AF Shrestha, Utsab Bhowmik, Debsindhu Perera, Suchithranga M. D. C. Chawla, Udeep Struts, Andrey V. Graziano, Vito Qian, Shuo Heller, William T. Brown, Michael F. Chu, Xiang-Qiang TI Small Angle Neutron and X-Ray Scattering Reveal Conformational Differences in Detergents Affecting Rhodopsin Activation SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract ID DYNAMICS C1 [Shrestha, Utsab; Bhowmik, Debsindhu; Chu, Xiang-Qiang] Wayne State Univ, Dept Phys & Astron, Detroit, MI 48202 USA. [Perera, Suchithranga M. D. C.; Chawla, Udeep; Struts, Andrey V.; Brown, Michael F.] Univ Arizona, Dept Chem & Biochem, Tucson, AZ USA. [Graziano, Vito] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. [Qian, Shuo; Heller, William T.] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN USA. NR 3 TC 2 Z9 2 U1 0 U2 5 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 189-Plat BP 39A EP 39A PG 1 WC Biophysics SC Biophysics GA CO9DB UT WOS:000359471700190 ER PT J AU Jo, S Jiang, W Roux, B AF Jo, Sunhwan Jiang, Wei Roux, Benoit TI Quantifying Protein-Protein Binding Energy and Entropy using Molecular Dynamics Simulations SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Jo, Sunhwan; Jiang, Wei] Argonne Natl Lab, Leadership Comp Facil, Argonne, IL 60439 USA. [Roux, Benoit] Univ Chicago, Dept Biochem & Mol Biol, Chicago, IL 60637 USA. [Roux, Benoit] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA. NR 0 TC 0 Z9 0 U1 2 U2 2 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 199-Plat BP 41A EP 41A PG 1 WC Biophysics SC Biophysics GA CO9DB UT WOS:000359471700200 ER PT J AU Bhowmik, D Dhindsa, GK Rusek, AJ Van Delinder, K Shrestha, U Ng, JD Sharp, M Stingaciu, LR Chu, XQ AF Bhowmik, Debsindhu Dhindsa, Gurpreet Kaur Rusek, Andrew J. Van Delinder, Kurt Shrestha, Utsab Ng, Joseph D. Sharp, Melissa Stingaciu, Laura R. Chu, Xiang-qiang TI Probing the Domain Motions of an Oligomeric Protein from Deep-Sea Hyperthermophile by Neutron Spin Echo SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract ID DYNAMICS C1 [Bhowmik, Debsindhu; Dhindsa, Gurpreet Kaur; Rusek, Andrew J.; Van Delinder, Kurt; Shrestha, Utsab; Chu, Xiang-qiang] Wayne State Univ, Dept Phys & Astron, Detroit, MI 48202 USA. [Ng, Joseph D.] Univ Alabama, Dept Biol Sci, Huntsville, AL 35899 USA. [Sharp, Melissa] European Spallat Souce, Lund, Sweden. [Stingaciu, Laura R.] Oak Ridge Natl Lab, Oak Ridge, TN USA. NR 5 TC 3 Z9 3 U1 1 U2 6 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 295-Pos BP 59A EP 59A PG 1 WC Biophysics SC Biophysics GA CO9DB UT WOS:000359471700296 ER PT J AU Bhowmik, D Shrestha, U Perera, SMDC Chawla, U Mamontov, E Brown, MF Chu, XQ AF Bhowmik, Debsindhu Shrestha, Utsab Perera, Suchithranga M. D. C. Chawla, Udeep Mamontov, Eugene Brown, Michael F. Chu, Xiang-Qiang TI Rhodopsin Photoactivation Dynamics Revealed by Quasi-Elastic Neutron Scattering SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Bhowmik, Debsindhu; Shrestha, Utsab; Chu, Xiang-Qiang] Wayne State Univ, Dept Phys & Astron, Detroit, MI 48202 USA. [Perera, Suchithranga M. D. C.; Chawla, Udeep; Brown, Michael F.] Univ Arizona, Dept Chem & Biochem, Tucson, AZ USA. [Mamontov, Eugene] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN USA. RI Mamontov, Eugene/Q-1003-2015 OI Mamontov, Eugene/0000-0002-5684-2675 NR 4 TC 2 Z9 2 U1 0 U2 3 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 306-Pos BP 61A EP 61A PG 1 WC Biophysics SC Biophysics GA CO9DB UT WOS:000359471700307 ER PT J AU Lequieu, JP Freeman, GS de Pablo, JJ AF Lequieu, Joshua P. Freeman, Gordon S. de Pablo, Juan J. TI The Role of DNA Shape in Nucleosome Formation and Positioning SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Lequieu, Joshua P.; de Pablo, Juan J.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. [Freeman, Gordon S.] Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI USA. [de Pablo, Juan J.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. NR 0 TC 0 Z9 0 U1 1 U2 2 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 367-Pos BP 72A EP 72A PG 1 WC Biophysics SC Biophysics GA CO9DB UT WOS:000359471700368 ER PT J AU Heberle, FA Anghel, VNP Katsaras, J AF Heberle, Frederick A. Anghel, Vinicius N. P. Katsaras, John TI Scattering from Laterally Heterogeneous Vesicles: An Analytical form Factor for Multiple Domains SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Heberle, Frederick A.; Katsaras, John] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN USA. [Anghel, Vinicius N. P.] Atom Energy Canada Ltd, Chalk River Labs, Chalk River, ON K0J 1J0, Canada. [Katsaras, John] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 426-Pos BP 84A EP 84A PG 1 WC Biophysics SC Biophysics GA CO9DB UT WOS:000359471700427 ER PT J AU Johnson, MA Seifert, S Petrache, HI AF Johnson, Merrell A. Seifert, Soenke Petrache, Horia I. TI Cation Effects on Zwitterionic Lipid Multilayers SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Johnson, Merrell A.; Petrache, Horia I.] IUPUI, Phys, Indianapolis, IN USA. [Seifert, Soenke] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. NR 0 TC 0 Z9 0 U1 1 U2 1 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 431-Pos BP 85A EP 85A PG 1 WC Biophysics SC Biophysics GA CO9DB UT WOS:000359471700432 ER PT J AU Enoki, TA Kim, S Heberle, FA Feigenson, GW AF Enoki, Thais A. Kim, Sarah Heberle, Fred A. Feigenson, Gerald W. TI Partitioning of the Transmembrane Peptide GWALP23 between Lo and Ld Phases in Macro and Nanoscale Domains. Nanometer-Scale Domains can be Treated as a Phase SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Enoki, Thais A.] Univ Sao Paulo, Inst Phys, Sao Paulo, Brazil. [Enoki, Thais A.; Feigenson, Gerald W.] Cornell Univ, Ithaca, NY USA. [Kim, Sarah] Johns Hopkins Univ, Baltimore, MD USA. [Heberle, Fred A.] Oak Ridge Natl Lab, Oak Ridge, TN USA. RI Azevedo Enoki, Thais/D-6569-2017 OI Azevedo Enoki, Thais/0000-0003-4639-9160 NR 0 TC 0 Z9 0 U1 1 U2 2 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 438-Pos BP 86A EP 86A PG 1 WC Biophysics SC Biophysics GA CO9DB UT WOS:000359471700439 ER PT J AU Marquardt, D Van Oosten, B Heberle, FA Kucerka, N Wassall, S Standaert, R Katsaras, J Harroun, TA AF Marquardt, Drew Van Oosten, Brad Heberle, Frederick A. Kucerka, Norbert Wassall, Stephen Standaert, Robert Katsaras, John Harroun, Thad A. TI Hydrocarbon Thickness Dictates Cholesterol's Location, Orientation and Motion in a Phospholipid Bilayer SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Marquardt, Drew] Graz Univ, Div Biophys, Inst Mol Biosci, Graz, Austria. [Marquardt, Drew; Van Oosten, Brad; Harroun, Thad A.] Brock Univ, Phys, St Catharines, ON L2S 3A1, Canada. [Heberle, Frederick A.] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN USA. [Kucerka, Norbert] Joint Inst Nucl Res, Frank Lab Neutron Phys, Dubna, Russia. [Wassall, Stephen] Indiana Univ Purdue Univ, Phys, Indianapolis, IN 46202 USA. [Standaert, Robert] Oak Ridge Natl Lab, Biol & Nanoscale Syst, Oak Ridge, TN USA. [Katsaras, John] Oak Ridge Natl Lab, Neutron Sci Directorate, Oak Ridge, TN USA. [Katsaras, John] Univ Tennessee, Phys, Knoxville, TN USA. RI Standaert, Robert/D-9467-2013 OI Standaert, Robert/0000-0002-5684-1322 NR 0 TC 1 Z9 1 U1 0 U2 2 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 435-Pos BP 86A EP 86A PG 1 WC Biophysics SC Biophysics GA CO9DB UT WOS:000359471700436 ER PT J AU Gabelli, SB Boto, A Halpernin, V Bianchet, MA Farinelli, F Aripirala, S Yoder, JB Jakoncic, J Tomaselli, GF Amzel, M AF Gabelli, Sandra B. Boto, Agedi Halpernin, Victoria Bianchet, Mario A. Farinelli, Federica Aripirala, Srinivas Yoder, Jesse B. Jakoncic, Jean Tomaselli, Gordon F. Amzel, Mario TI Cardiac Sodium Channel: Activation by CaM Involves a NaV1.5-NaV1.5 Interaction SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Gabelli, Sandra B.; Boto, Agedi; Bianchet, Mario A.; Aripirala, Srinivas; Yoder, Jesse B.; Amzel, Mario] Johns Hopkins Univ, Sch Med, Biophys & Biophys Chem, Baltimore, MD USA. [Halpernin, Victoria] Johns Hopkins Univ, Sch Med, Physiol, Baltimore, MD USA. [Farinelli, Federica; Tomaselli, Gordon F.] Johns Hopkins Univ, Sch Med, Med, Baltimore, MD USA. [Jakoncic, Jean] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. RI Gabelli, Sandra/A-3705-2008 OI Gabelli, Sandra/0000-0003-1205-5204 NR 0 TC 0 Z9 0 U1 0 U2 0 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 637-Pos BP 127A EP 128A PG 2 WC Biophysics SC Biophysics GA CO9DB UT WOS:000359471700638 ER PT J AU Zielazinski, E Zerbs, S Larsen, P Collart, F Laible, PD AF Zielazinski, Eliza Zerbs, Sarah Larsen, Peter Collart, Frank Laible, Philip D. TI Methionine Importers in Soil Bacteria: Potential for Transporter-Component Crosstalk SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Zielazinski, Eliza; Zerbs, Sarah; Larsen, Peter; Collart, Frank; Laible, Philip D.] Argonne Natl Lab, Biosci Div, Lemont, IL USA. NR 0 TC 0 Z9 0 U1 2 U2 2 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 728-Pos BP 146A EP 146A PG 1 WC Biophysics SC Biophysics GA CO9DB UT WOS:000359471700729 ER PT J AU Klosowiak, J Focia, P Chakravarthy, S Freymann, D Rice, S AF Klosowiak, Julian Focia, Pamela Chakravarthy, Srinivas Freymann, Douglas Rice, Sarah TI Structures of Human Miro1 Reveal Conformational Changes SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Klosowiak, Julian] Northwestern Univ, Chicago, IL 60611 USA. [Focia, Pamela; Freymann, Douglas] Northwestern Univ, Mol Pharmacol & Biol Chem, Chicago, IL 60611 USA. [Chakravarthy, Srinivas] ArgonneNatl Lab, Biophys Collaborat Access Team, Chicago, IL USA. [Rice, Sarah] Northwestern Univ, Cell & Mol Biol, Chicago, IL 60611 USA. NR 0 TC 0 Z9 0 U1 1 U2 1 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 772-Pos BP 155A EP 155A PG 1 WC Biophysics SC Biophysics GA CO9DB UT WOS:000359471700773 ER PT J AU Guo, SR Buchsbaum, SF Meshot, ER Davenport, MW Siwy, Z Fornasiero, F AF Guo, Shirui Buchsbaum, Steven F. Meshot, Eric R. Davenport, Matthew W. Siwy, Zuzanna Fornasiero, Francesco TI Giant Conductance and Anomalous Concentration Dependence in Sub-5 nm Carbon Nanotube Nanochannels SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Guo, Shirui; Buchsbaum, Steven F.; Meshot, Eric R.; Davenport, Matthew W.; Fornasiero, Francesco] Lawrence Livermore Natl Lab, Phys & Life Sci, Livermore, CA USA. [Siwy, Zuzanna] Univ Calif Irvine, Irvine, CA USA. RI Fornasiero, Francesco/I-3802-2012 NR 0 TC 2 Z9 2 U1 2 U2 2 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 882-Pos BP 175A EP 175A PG 1 WC Biophysics SC Biophysics GA CT5KR UT WOS:000362849100092 ER PT J AU Zwolak, M Velizhanin, K Chien, CC Dubi, Y AF Zwolak, Michael Velizhanin, Kirill Chien, Chih-Chun Dubi, Yonatan TI Deconstructing Structural Transitions via Thermal Transport SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Zwolak, Michael] Oregon State Univ, Dept Phys, Corvallis, OR 97331 USA. [Velizhanin, Kirill] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM USA. [Chien, Chih-Chun] Univ Calif Merced, Dept Phys, Merced, CA USA. [Dubi, Yonatan] Ben Gurion Univ Negev, Dept Chem, Beer Sheva, Israel. NR 0 TC 0 Z9 0 U1 0 U2 1 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 885-Pos BP 176A EP 176A PG 1 WC Biophysics SC Biophysics GA CT5KR UT WOS:000362849100095 ER PT J AU Hetherington, CL Bischak, CG Stachelrodt, CE Precht, JT Wang, Z Schlom, DG Ginsberg, NS AF Hetherington, Craig L. Bischak, Connor G. Stachelrodt, Claire E. Precht, Jake T. Wang, Zhe Schlom, Darrell G. Ginsberg, Naomi S. TI Superresolution Fluorescence Microscopy within a Scanning Electron Microscope SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Hetherington, Craig L.; Bischak, Connor G.; Stachelrodt, Claire E.; Precht, Jake T.; Ginsberg, Naomi S.] Univ Calif Berkeley, Chem, Berkeley, CA USA. [Hetherington, Craig L.; Ginsberg, Naomi S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Wang, Zhe; Schlom, Darrell G.] Cornell Univ, Mat Sci & Engn, Ithaca, NY USA. NR 0 TC 0 Z9 0 U1 1 U2 4 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 958-Plat BP 190A EP 191A PG 2 WC Biophysics SC Biophysics GA CT5KR UT WOS:000362849100168 ER PT J AU Kokhan, O Ponomarenko, N Pokkuluri, PR Schiffer, M Tiede, DM AF Kokhan, Oleksandr Ponomarenko, Nina Pokkuluri, P. Raj Schiffer, Marianne Tiede, David M. TI Multimerization of Solution-State Proteins by Anionic Porphyrins SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Kokhan, Oleksandr] James Madison Univ, Dept Chem & Biochem, Harrisonburg, VA 22807 USA. [Ponomarenko, Nina; Tiede, David M.] Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL USA. [Pokkuluri, P. Raj; Schiffer, Marianne] Argonne Natl Lab, Biosci Div, Lemont, IL USA. NR 0 TC 0 Z9 0 U1 1 U2 1 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 1091-Pos BP 218A EP 218A PG 1 WC Biophysics SC Biophysics GA CT5KR UT WOS:000362849100301 ER PT J AU Vanegas, JM Anishkin, A Rogers, DM Sukharev, S Rempe, SB AF Vanegas, Juan M. Anishkin, Andriy Rogers, David M. Sukharev, Sergei Rempe, Susan B. TI Active Role of the Substrate during Catalysis by the Therapeutic Enzyme L-Asparaginase II SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Vanegas, Juan M.; Rempe, Susan B.] Sandia Natl Labs, Ctr Biol & Mat Sci, Albuquerque, NM 87185 USA. [Anishkin, Andriy; Sukharev, Sergei] Univ Maryland, Dept Biol, College Pk, MD 20742 USA. [Rogers, David M.] Univ S Florida, Dept Chem, Tampa, FL 33620 USA. NR 0 TC 0 Z9 0 U1 0 U2 1 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 1120-Pos BP 223A EP 223A PG 1 WC Biophysics SC Biophysics GA CT5KR UT WOS:000362849100330 ER PT J AU Walker, JA Takasuka, TE Deng, K Bianchetti, CM Udell, H Prom, BM Kim, H Northern, TR Fox, BG AF Walker, Johnnie A. Takasuka, Taichi E. Deng, Kai Bianchetti, Christopher M. Udell, Hannah Prom, Ben M. Kim, Hyunkee Northern, Trent R. Fox, Brian G. TI Substrate Binding Effects of Carbohydrate Binding Modules on the Catalytic Activity of a Multifunctional Cellulase SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Walker, Johnnie A.; Takasuka, Taichi E.; Bianchetti, Christopher M.; Udell, Hannah; Prom, Ben M.; Kim, Hyunkee; Fox, Brian G.] Univ Wisconsin, Madison, WI USA. [Deng, Kai; Northern, Trent R.] Lawrence Berkeley Natl Lab, Emeryville, CA USA. NR 0 TC 0 Z9 0 U1 6 U2 6 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 1131-Pos BP 225A EP 225A PG 1 WC Biophysics SC Biophysics GA CT5KR UT WOS:000362849100341 ER PT J AU Chennubhotla, CS Ramanathan, A Stanley, C AF Chennubhotla, Chakra S. Ramanathan, Arvind Stanley, Chris TI Enabling Biophysical Characterization of Intrinsically Disordered Protein Ensembles SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Chennubhotla, Chakra S.] Univ Pittsburgh, Computat Biol, Pittsburgh, PA USA. [Ramanathan, Arvind; Stanley, Chris] Oak Ridge Natl Lab, Knoxville, TN USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 1140-Pos BP 227A EP 227A PG 1 WC Biophysics SC Biophysics GA CT5KR UT WOS:000362849100350 ER PT J AU Hayes, RL Noel, JK Mandic, A Whitford, PC Sanbonmatsu, KY Mohanty, U Onuchic, JN AF Hayes, Ryan L. Noel, Jeffrey K. Mandic, Ana Whitford, Paul C. Sanbonmatsu, Karissa Y. Mohanty, Udayan Onuchic, Jose N. TI Magnesium Dependence of the RNA Free Energy Landscape SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Hayes, Ryan L.; Noel, Jeffrey K.; Onuchic, Jose N.] Rice Univ, CTBP, Houston, TX USA. [Mandic, Ana] Univ Houston, Biomed Engn, Houston, TX USA. [Whitford, Paul C.] Northeastern Univ, Phys, Boston, MA 02115 USA. [Sanbonmatsu, Karissa Y.] Los Alamos Natl Lab, Theoret Biol & Biophys, Los Alamos, NM USA. [Mohanty, Udayan] Boston Coll, Chem, Chestnut Hill, MA 02167 USA. NR 0 TC 0 Z9 0 U1 2 U2 3 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 1185-Pos BP 235A EP 235A PG 1 WC Biophysics SC Biophysics GA CT5KR UT WOS:000362849100395 ER PT J AU Petrou, VI Clarke, OB Schultz, KM Tomasek, D Kloss, B Banerjee, S Rajashankar, KR Klug, CS Shapiro, L Mancia, F AF Petrou, Vasileios I. Clarke, Oliver B. Schultz, Kathryn M. Tomasek, David Kloss, Brian Banerjee, Surajit Rajashankar, Kanagalaghatta R. Klug, Candice S. Shapiro, Lawrence Mancia, Filippo TI Crystal Structure of the Bacterial Aminoarabinose Transferase ArnT SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Petrou, Vasileios I.; Tomasek, David; Mancia, Filippo] Columbia Univ, Dept Physiol & Cellular Biophys, New York, NY USA. [Clarke, Oliver B.; Shapiro, Lawrence] Columbia Univ, Dept Biochem & Mol Biophys, New York, NY USA. [Schultz, Kathryn M.; Klug, Candice S.] Med Coll Wisconsin, Dept Biophys, Milwaukee, WI 53226 USA. [Kloss, Brian] New York Struct Biol Ctr, New York Consortium Membrane Prot Struct, New York, NY USA. [Banerjee, Surajit; Rajashankar, Kanagalaghatta R.] Cornell Univ, Dept Chem & Chem Biol, NE CAT, Adv Photon Source, Argonne, IL USA. OI Petrou, Vasileios/0000-0002-3194-9863 NR 0 TC 0 Z9 0 U1 0 U2 2 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 1280-Pos BP 253A EP 253A PG 1 WC Biophysics SC Biophysics GA CT5KR UT WOS:000362849100490 ER PT J AU Carpenter, TS Lightstone, FC AF Carpenter, Timothy S. Lightstone, Felice C. TI Simulated Closing of the NMDA Ligand-Binding Domain SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Carpenter, Timothy S.; Lightstone, Felice C.] Lawrence Livermore Natl Lab, BBTD, Livermore, CA USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 1436-Pos BP 286A EP 286A PG 1 WC Biophysics SC Biophysics GA CT5KR UT WOS:000362849100646 ER PT J AU Bautista, CAL Phillips, J Gnanakaran, S AF Bautista, Cesar A. Lopez Phillips, Joshua Gnanakaran, S. TI Mechanistic Details of Drug Translocation in MexAB-OprM Efflux Pump SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract C1 [Bautista, Cesar A. Lopez; Phillips, Joshua; Gnanakaran, S.] Los Alamos Natl Lab, Theoret Biol & Biophys, Los Alamos, NM USA. NR 0 TC 0 Z9 0 U1 1 U2 1 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 1551-Pos BP 310A EP 310A PG 1 WC Biophysics SC Biophysics GA CT5KR UT WOS:000362849100761 ER PT J AU Gurusaran, M Rai, D Qian, S Weiss, K Urban, V Li, PZ Ma, LL Narayanan, TN Ajayan, PM Sekar, K Viswanathan, S Renugopalakrishanan, V AF Gurusaran, Manickam Rai, Durgesh Qian, Shuo Weiss, Kevin Urban, Volker Li, Pingzuo Ma, Lulu Narayanan, Tharangattu N. Ajayan, Pulickel M. Sekar, Kanagaraj Viswanathan, Sowmya Renugopalakrishanan, Venkatesan TI Small Angle Neutron Scattering Studies of Glucose Oxidase Immobilized on Single Layer Graphene: Relevant to Protein Microfluidic Chip SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Gurusaran, Manickam; Sekar, Kanagaraj] Indian Inst Sci, Supercomp Educ & Res Ctr, Bangalore 560012, Karnataka, India. [Gurusaran, Manickam; Li, Pingzuo; Renugopalakrishanan, Venkatesan] Harvard Univ, Childrens Hosp, Sch Med, Ctr Life Sci, Boston, MA 02115 USA. [Rai, Durgesh; Qian, Shuo; Weiss, Kevin; Urban, Volker] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN USA. [Ma, Lulu; Ajayan, Pulickel M.] Rice Univ, Dept Mech Engn & Mat Sci, Houston, TX 77251 USA. [Narayanan, Tharangattu N.] Tata Inst Fundamental Res, Ctr Interdisciplinary Sci, Hyderabad, Andhra Pradesh, India. [Viswanathan, Sowmya] Newton Wellesley Hosp, Partners Healthcare Syst, Newton, MA USA. RI Urban, Volker/N-5361-2015 OI Urban, Volker/0000-0002-7962-3408 NR 2 TC 1 Z9 1 U1 2 U2 7 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 1645-Pos BP 327A EP 328A PG 2 WC Biophysics SC Biophysics GA CT5KU UT WOS:000362849400060 ER PT J AU Heftberger, P Kollmitzer, B Heberle, F Nickels, J Katsaras, J Pabst, G AF Heftberger, Peter Kollmitzer, Benjamin Heberle, Frederick Nickels, Jonathan Katsaras, John Pabst, Georg TI Influence of Domain Size on Structure and Elastic Fluctuations in Complex Lipid Mixtures SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Heftberger, Peter; Kollmitzer, Benjamin; Pabst, Georg] Graz Univ, NAWI Graz, BioTechMed Graz, Inst Mol Biosci,Biophys Div, Graz, Austria. [Heberle, Frederick; Nickels, Jonathan; Katsaras, John] Oak Ridge Natl Lab, Neutron Sci Directorate, Oak Ridge, TN USA. NR 1 TC 0 Z9 0 U1 1 U2 1 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 1717-Plat BP 341A EP 341A PG 1 WC Biophysics SC Biophysics GA CT5KU UT WOS:000362849400132 ER PT J AU Johnson, MA Seifert, S Firestone, MA Petrache, HI Kimble-Hill, AC AF Johnson, Merrell A. Seifert, Soenke Firestone, Millicent A. Petrache, Horia I. Kimble-Hill, Ann C. TI Phase Coexistence in Lipid Membranes Induced by Buffering Agents and Charged Lipid Headgroups SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Johnson, Merrell A.; Petrache, Horia I.] IUPUI, Dept Phys, Indianapolis, IN USA. [Seifert, Soenke] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Firestone, Millicent A.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM USA. [Kimble-Hill, Ann C.] Indiana Univ Sch Med, Dept Biochem & Mol Biol, Indianapolis, IN 46202 USA. NR 0 TC 0 Z9 0 U1 1 U2 1 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 1718-Plat BP 341A EP 341A PG 1 WC Biophysics SC Biophysics GA CT5KU UT WOS:000362849400133 ER PT J AU Taylor, VG Kondrashkina, E Bommarito, P Lund, G Cierpicki, T Tesmer, JJG AF Taylor, Veronica G. Kondrashkina, Elena Bommarito, Paige Lund, George Cierpicki, Tomasz Tesmer, John J. G. TI Structural Studies of G-Alpha-Q Signaling SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Taylor, Veronica G.] Univ Michigan, Biophys, Ann Arbor, MI 48109 USA. [Kondrashkina, Elena] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Bommarito, Paige] Univ Michigan, Inst Life Sci, Ann Arbor, MI 48109 USA. [Lund, George; Cierpicki, Tomasz] Univ Michigan, Pathol, Ann Arbor, MI 48109 USA. [Tesmer, John J. G.] Univ Michigan, Pharmacol, Ann Arbor, MI 48109 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 1728-Plat BP 343A EP 344A PG 2 WC Biophysics SC Biophysics GA CT5KU UT WOS:000362849400143 ER PT J AU Xiong, YJ Beech, BM Boschek, CB Baird, CL Bigelow, DJ McAteer, K Squier, TC AF Xiong, Yijia Beech, Brenda M. Boschek, Curt B. Baird, Cheryl L. Bigelow, Diana J. McAteer, Kathleen Squier, Thomas C. TI Controlled Activation of Protein Rotational Dynamics using Smart Hydrogel Tethering SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Xiong, Yijia; Squier, Thomas C.] Western Univ Hlth Sci, Basic Med Sci, Lebanon, OR USA. [Beech, Brenda M.; Boschek, Curt B.; Baird, Cheryl L.; Bigelow, Diana J.] Pacific NW Natl Lab, Biol Sci, Richland, WA 99352 USA. [McAteer, Kathleen] Washington State Univ Tricities, Biol Sci, Richland, WA USA. NR 0 TC 0 Z9 0 U1 3 U2 3 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 1734-Plat BP 345A EP 345A PG 1 WC Biophysics SC Biophysics GA CT5KU UT WOS:000362849400149 ER PT J AU Evilevitch, A Sae-Ueng, U Li, D Zuo, XB Huffman, J Homa, F Rau, D AF Evilevitch, Alex Sae-Ueng, Udom Li, Dong Zuo, Xiaobing Huffman, Jamie Homa, Fred Rau, Donald TI Solid-To-Fluid DNA Transition Inside HSV-1 Capsid Close to the Temperature of Infection SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Evilevitch, Alex; Sae-Ueng, Udom; Li, Dong] Carnegie Mellon Univ, Phys, Pittsburgh, PA 15213 USA. [Zuo, Xiaobing] Argonne Natl Lab, Argonne, IL 60439 USA. [Huffman, Jamie; Homa, Fred] Univ Pittsburgh, Sch Med, Pittsburgh, PA USA. [Rau, Donald] NIH, Bethesda, MD 20892 USA. NR 0 TC 0 Z9 0 U1 1 U2 2 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 1764-Plat BP 351A EP 351A PG 1 WC Biophysics SC Biophysics GA CT5KU UT WOS:000362849400179 ER PT J AU Valley, CC Arndt-Jovin, DJ Jovin, TM Steinkamp, MP Chizhik, AI Karedla, N Hlavacek, WS Wilson, BS Lidke, KA Lidke, DS AF Valley, Christopher C. Arndt-Jovin, Donna J. Jovin, Thomas M. Steinkamp, Mara P. Chizhik, Alexey I. Karedla, Narain Hlavacek, William S. Wilson, Bridget S. Lidke, Keith A. Lidke, Diane S. TI Inside-Out Signaling of Oncogenic EGFR Mutants Promotes Ligand-Independent Dimerization SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Valley, Christopher C.; Steinkamp, Mara P.; Wilson, Bridget S.; Lidke, Diane S.] Univ New Mexico, Dept Pathol, Albuquerque, NM 87131 USA. [Arndt-Jovin, Donna J.; Jovin, Thomas M.] Max Planck Inst Biophys Chem, Lab Cellular Dynam, D-37077 Gottingen, Germany. [Chizhik, Alexey I.; Karedla, Narain] Univ Gottingen, Inst Phys 3, D-37073 Gottingen, Germany. [Hlavacek, William S.] Los Alamos Natl Lab, Theoret Biol & Biophys Grp, Los Alamos, NM USA. [Lidke, Keith A.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. NR 0 TC 0 Z9 0 U1 2 U2 2 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 1762-Plat BP 351A EP 351A PG 1 WC Biophysics SC Biophysics GA CT5KU UT WOS:000362849400177 ER PT J AU Pirbadian, S Barchinger, SE Leung, KM Byun, HS Jangir, Y Bouhenni, RA Reed, SB Romine, MF Saffarini, DA Shi, L Gorby, YA Golbeck, JH El-Naggar, MY AF Pirbadian, Sahand Barchinger, Sarah E. Leung, Kar Man Byun, Hye Suk Jangir, Yamini Bouhenni, Rachida A. Reed, Samantha B. Romine, Margaret F. Saffarini, Daad A. Shi, Liang Gorby, Yuri A. Golbeck, John H. El-Naggar, Mohamed Y. TI Bacterial Nanowires of Shewanella Oneidensis MR-1 are Outer Membrane and Periplasmic Extensions of the Extracellular Electron Transport Components SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Pirbadian, Sahand; Leung, Kar Man; Byun, Hye Suk; Jangir, Yamini; El-Naggar, Mohamed Y.] Univ So Calif, Phys & Astron, Los Angeles, CA USA. [Barchinger, Sarah E.; Golbeck, John H.] Penn State Univ, Biochem & Mol Biol, University Pk, PA 16802 USA. [Bouhenni, Rachida A.; Saffarini, Daad A.] Univ Wisconsin, Biol Sci, Milwaukee, WI 53201 USA. [Reed, Samantha B.; Romine, Margaret F.; Shi, Liang] Pacific NW Natl Lab, Richland, WA 99352 USA. [Gorby, Yuri A.] Rensselaer Polytech Inst, Civil & Environm Engn, Troy, NY USA. [Golbeck, John H.] Penn State Univ, Chem, University Pk, PA 16802 USA. [El-Naggar, Mohamed Y.] Univ So Calif, Mol & Computat Biol Sect, Biol Sci, Los Angeles, CA USA. NR 0 TC 0 Z9 0 U1 8 U2 21 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 1845-Plat BP 368A EP 368A PG 1 WC Biophysics SC Biophysics GA CT5KU UT WOS:000362849400260 ER PT J AU Baker, NA Dowling, C Gosink, L Pulsipher, T Sansone, SA AF Baker, Nathan A. Dowling, Chase Gosink, Luke Pulsipher, Trenton Sansone, Susanna-Assunta TI Informatics Approaches to Data Preservation and Analysis in Protein Electrostatics SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Baker, Nathan A.; Dowling, Chase; Gosink, Luke; Pulsipher, Trenton] Pacific NW Natl Lab, Richland, WA 99352 USA. [Sansone, Susanna-Assunta] Oxford E Res Ctr, Oxford, England. RI Baker, Nathan/A-8605-2010 OI Baker, Nathan/0000-0002-5892-6506 NR 0 TC 0 Z9 0 U1 0 U2 0 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 1852-Wkshp BP 369A EP 369A PG 1 WC Biophysics SC Biophysics GA CT5KU UT WOS:000362849400267 ER PT J AU Ramanathan, A Chennubhotla, CS Agarwal, PK Stanley, CB AF Ramanathan, Arvind Chennubhotla, Chakra S. Agarwal, Pratul K. Stanley, Christopher B. TI Large-Scale Machine Learning Approaches for Molecular Biophysics SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Ramanathan, Arvind] Oak Ridge Natl Lab, Comp Sci, Oak Ridge, TN USA. [Chennubhotla, Chakra S.] Univ Pittsburgh, Dept Computat & Syst Biol, Pittsburgh, PA USA. [Agarwal, Pratul K.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN USA. [Stanley, Christopher B.] Oak Ridge Natl Lab, Div Neutron Sci, Oak Ridge, TN USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 1855-Wkshp BP 370A EP 370A PG 1 WC Biophysics SC Biophysics GA CT5KU UT WOS:000362849400270 ER PT J AU Hurley, M Germane, KL Servinsky, M Gerlach, E Sund, C AF Hurley, Margaret Germane, Katherine L. Servinsky, Matthew Gerlach, Elliot Sund, Christian TI Structure and Function of Clostridial Yter SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Hurley, Margaret] US Army Res Lab, Aberdeen Proving Ground, MD USA. [Germane, Katherine L.] Oak Ridge Associated Univ, Belcamp, MD USA. [Servinsky, Matthew; Sund, Christian] US Army Res Lab, Adelphi, MD USA. [Gerlach, Elliot] Fed Staffing Resources, Annapolis, MD USA. NR 0 TC 0 Z9 0 U1 2 U2 2 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 1883-Pos BP 375A EP 375A PG 1 WC Biophysics SC Biophysics GA CT5KU UT WOS:000362849400298 ER PT J AU Kapoor, K Duff, M Hinde, R Baudry, J Howell, E AF Kapoor, Karan Duff, Michael Hinde, Robert Baudry, Jerome Howell, Elizabeth TI Characterizing Dynamics of Anion/Pi Interactions through Molecular Dynamics Simulations SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Kapoor, Karan; Baudry, Jerome] Univ Tennessee, Oak Ridge Natl Lab, Ctr Biophys Mol, Knoxville, TN USA. [Duff, Michael; Howell, Elizabeth] Univ Tennessee, Dept Biochem Cellular & Mol Biol, Knoxville, TN USA. [Hinde, Robert] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 1905-Pos BP 379A EP 379A PG 1 WC Biophysics SC Biophysics GA CT5KU UT WOS:000362849400320 ER PT J AU Vanegas, JM Rogers, DM Kent, MS Rempe, SB AF Vanegas, Juan M. Rogers, David M. Kent, Michael S. Rempe, Susan B. TI Role of Electrostatic Interactions in the Anchoring of Dengue E Protein to Lipid Membranes SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Vanegas, Juan M.; Kent, Michael S.; Rempe, Susan B.] Sandia Natl Labs, Ctr Biol & Mat Sci, Albuquerque, NM 87185 USA. [Rogers, David M.] Univ S Florida, Dept Chem, Tampa, FL 33620 USA. NR 0 TC 0 Z9 0 U1 0 U2 4 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 2043-Pos BP 406A EP 406A PG 1 WC Biophysics SC Biophysics GA CT5KU UT WOS:000362849400458 ER PT J AU Greathouse, DV Kinnun, JJ Williams, JA Marquardt, D Klauda, JB Koeppe, RE Katsaras, J Harroun, TA Wassall, SR AF Greathouse, Denise V. Kinnun, Jacob J. Williams, Justin A. Marquardt, Drew Klauda, Jeffrey B. Koeppe, Roger E., II Katsaras, John Harroun, Thad A. Wassall, Stephen R. TI Disorderly Polyunsaturated Fatty Acids and Orderly Cholesterol: Just How do they get along in a Membrane? SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Greathouse, Denise V.; Koeppe, Roger E., II] Univ Arkansas, Dept Chem & Biochem, Fayetteville, AR 72701 USA. [Kinnun, Jacob J.; Williams, Justin A.; Wassall, Stephen R.] Indiana Univ Purdue Univ, Dept Phys, Indianapolis, IN 46205 USA. [Marquardt, Drew; Harroun, Thad A.] Brock Univ, Dept Phys, St Catharines, ON L2S 3A1, Canada. [Klauda, Jeffrey B.] Univ Maryland, Dept Chem & Biomol Engn, College Pk, MD 20742 USA. [Katsaras, John] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Katsaras, John] Univ Tennessee, Dept Phys, Knoxville, TN 37996 USA. OI Greathouse, Denise/0000-0001-7104-8499 NR 0 TC 0 Z9 0 U1 0 U2 15 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 2075-Pos BP 412A EP 412A PG 1 WC Biophysics SC Biophysics GA CT5KU UT WOS:000362849400490 ER PT J AU Noy, A AF Noy, Aleksandr TI Mimicking Biology with Nanomaterials: Carbon Nanotube Porins in Lipid Membranes SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Noy, Aleksandr] Lawrence Livermore Natl Lab, Livermore, CA USA. NR 0 TC 1 Z9 1 U1 1 U2 1 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 2227-Pos BP 443A EP 443A PG 1 WC Biophysics SC Biophysics GA CT5KU UT WOS:000362849400642 ER PT J AU Bouxsein, NF Bachand, GD AF Bouxsein, Nathan F. Bachand, George D. TI Effects of Added Divalent Counterions on the Properties and Behaviors of Microtubule Filaments SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Bouxsein, Nathan F.; Bachand, George D.] Sandia Natl Labs, Albuquerque, NM 87185 USA. NR 0 TC 0 Z9 0 U1 1 U2 1 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 2269-Pos BP 451A EP 451A PG 1 WC Biophysics SC Biophysics GA CT5KU UT WOS:000362849400684 ER PT J AU Cannon, WR Thomas, DG Baxter, DJ AF Cannon, William R. Thomas, Dennis G. Baxter, Douglas J. TI Simulating Metabolism with Statistical Thermodynamics SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Cannon, William R.; Thomas, Dennis G.] Pacific NW Natl Lab, Computat Biol & Bioinformat Grp, Richland, WA 99352 USA. [Baxter, Douglas J.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. NR 0 TC 0 Z9 0 U1 1 U2 2 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 2370-Pos BP 470A EP 470A PG 1 WC Biophysics SC Biophysics GA CT5KU UT WOS:000362849400785 ER PT J AU Adams, PG Swingle, KL Paxton, WF Nogan, JJ Lamoureux, L Firestone, MA Mukundan, H Montano, GA AF Adams, Peter G. Swingle, Kirstie L. Paxton, Walter F. Nogan, John J. Lamoureux, Loreen Firestone, Millicent A. Mukundan, Harshini Montano, Gabriel A. TI Bio-Lithography: A Novel Process for Modification and Patterning of Supported Lipid Bilayers using Lipopolysaccharide, a Biological Amphiphile SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Adams, Peter G.; Swingle, Kirstie L.; Firestone, Millicent A.; Montano, Gabriel A.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM USA. [Swingle, Kirstie L.] Univ New Mexico, Dept Biol, Albuquerque, NM 87131 USA. [Paxton, Walter F.; Nogan, John J.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. [Lamoureux, Loreen] Univ New Mexico, Ctr Biomed Engn, Albuquerque, NM 87131 USA. [Mukundan, Harshini] Los Alamos Natl Lab, Phys Chem & Appl Spect, Los Alamos, NM USA. [Mukundan, Harshini] New Mexico Consortium, Los Alamos, NM USA. NR 0 TC 0 Z9 0 U1 2 U2 2 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 2458-Pos BP 487A EP 487A PG 1 WC Biophysics SC Biophysics GA CT5KV UT WOS:000362849600066 ER PT J AU Geng, J Stannard, W Escalada, A Kim, K Thelen, MP Frolov, VA Noy, A AF Geng, Jia Stannard, Whitney Escalada, Arthur Kim, Kyunghoon Thelen, Michael P. Frolov, Vadim A. Noy, Aleksandr TI Live Cell Interactions with Biocompatible Ultra-Short Carbon Nanotube Porins SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Geng, Jia; Stannard, Whitney; Kim, Kyunghoon; Thelen, Michael P.; Noy, Aleksandr] Lawrence Livermore Natl Lab, Livermore, CA USA. [Geng, Jia; Noy, Aleksandr] Univ Calif, Merced, CA USA. [Escalada, Arthur; Frolov, Vadim A.] Univ Basque Country, Leioa, Spain. [Kim, Kyunghoon] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Frolov, Vadim A.] Basque Fdn Sci, Ikerbasque, Bilbao, Spain. RI Thelen, Michael/G-2032-2014 OI Thelen, Michael/0000-0002-2479-5480 NR 0 TC 0 Z9 0 U1 1 U2 4 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 2461-Pos BP 487A EP 488A PG 2 WC Biophysics SC Biophysics GA CT5KV UT WOS:000362849600069 ER PT J AU Perticaroli, S Nickels, JD Sokolov, AP AF Perticaroli, Stefania Nickels, Jonathan D. Sokolov, Alexei P. TI Rigidity of Poly-L-Glutamic Acid: Influence of Secondary and Supramolecular Structures SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Perticaroli, Stefania; Sokolov, Alexei P.] Univ Tennessee, Chem, Knoxville, TN USA. [Perticaroli, Stefania; Sokolov, Alexei P.] Oak Ridge Natl Lab, Joint Inst Neutron Sci, Div Chem & Mat Sci, Oak Ridge, TN USA. [Nickels, Jonathan D.] Oak Ridge Natl Lab, Joint Inst Neutron Sci, Oak Ridge, TN USA. RI Nickels, Jonathan/I-1913-2012 OI Nickels, Jonathan/0000-0001-8351-7846 NR 3 TC 0 Z9 0 U1 0 U2 1 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 2457-Pos BP 487A EP 487A PG 1 WC Biophysics SC Biophysics GA CT5KV UT WOS:000362849600065 ER PT J AU Tunuguntla, RH Belliveau, A Kim, K Geng, J Ajo-Franklin, C Noy, A AF Tunuguntla, Ramya H. Belliveau, Allison Kim, Kyunghoon Geng, Jia Ajo-Franklin, Caroline Noy, Aleksandr TI Transport Properties of Carbon Nanotube Porins in Lipid Vesicles SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Tunuguntla, Ramya H.; Geng, Jia; Noy, Aleksandr] Lawrence Livermore Natl Lab, Livermore, CA USA. [Belliveau, Allison] Northeastern Univ, Boston, MA 02115 USA. [Kim, Kyunghoon] Univ Calif Berkeley, Berkeley, CA USA. [Ajo-Franklin, Caroline] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. NR 0 TC 0 Z9 0 U1 2 U2 3 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 2464-Pos BP 488A EP 488A PG 1 WC Biophysics SC Biophysics GA CT5KV UT WOS:000362849600072 ER PT J AU Siwy, ZS Innes, L Schiel, M Vlassiouk, I Shea, KJ Theogarajan, L AF Siwy, Zuzanna S. Innes, Laura Schiel, Matthew Vlassiouk, Ivan Shea, Kenneth J. Theogarajan, Luke TI Pores with Undulating Diameter for Multipronged Characterization of Single Particles and Cells in Resistive-Pulse Technique SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Siwy, Zuzanna S.; Innes, Laura; Schiel, Matthew] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Vlassiouk, Ivan] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Shea, Kenneth J.] Univ Calif Irvine, Dept Chem, Irvine, CA 92717 USA. [Theogarajan, Luke] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 2474-Symp BP 490A EP 490A PG 1 WC Biophysics SC Biophysics GA CT5KV UT WOS:000362849600082 ER PT J AU Rajapaksha, A Stanley, CB Todd, BA AF Rajapaksha, Ajith Stanley, Christopher B. Todd, Brian A. TI Macromolecular Crowding of a Protein Complex by Small Angle Neutron Scattering and Small Angle X-Ray Scattering SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Rajapaksha, Ajith; Todd, Brian A.] Purdue Univ, Phys & Astron, W Lafayette, IN 47907 USA. [Stanley, Christopher B.] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN USA. NR 0 TC 0 Z9 0 U1 2 U2 4 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 2586-Pos BP 512A EP 512A PG 1 WC Biophysics SC Biophysics GA CT5KV UT WOS:000362849600194 ER PT J AU Palacio, LA Stanley, CB Seifert, S Lybarger, R Petrache, HI AF Palacio, Luis A. Stanley, Christopher B. Seifert, Soenke Lybarger, Ryan Petrache, Horia I. TI Small Angle Neutron and X-Ray Scattering of Plasma Glycoprotein Interactions with Lipid Membranes SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Palacio, Luis A.] Indiana Univ Purdue Univ, Dept Phys, Indianapolis, IN 46205 USA. [Stanley, Christopher B.] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN USA. [Seifert, Soenke] Argonne Natl Lab, APS, Xray Sci Div, Chem & Mat Sci, Lemont, IL USA. [Lybarger, Ryan; Petrache, Horia I.] Indiana Univ Purdue Univ, Phys, Indianapolis, IN 46202 USA. NR 0 TC 0 Z9 0 U1 1 U2 1 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 2609-Pos BP 516A EP 516A PG 1 WC Biophysics SC Biophysics GA CT5KV UT WOS:000362849600217 ER PT J AU Levendosky, R Horvath, K Chakravarthy, S Hobson, M Bowman, G AF Levendosky, Robert Horvath, Kyle Chakravarthy, Srinivas Hobson, Matt Bowman, Gregory TI Using FRET to Monitor Nucleosome Movement by the Chd1 Chromatin Remodeler SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Levendosky, Robert; Horvath, Kyle] Johns Hopkins Univ, Biol, Baltimore, MD USA. [Chakravarthy, Srinivas] Argon Natl Lab, Chicago, IL USA. [Hobson, Matt; Bowman, Gregory] Johns Hopkins Univ, Biophys, Baltimore, MD USA. NR 0 TC 0 Z9 0 U1 3 U2 5 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 2732-Pos BP 539A EP 539A PG 1 WC Biophysics SC Biophysics GA CT5KV UT WOS:000362849600340 ER PT J AU Kooijman, EE Graber, ZT Wang, WJ Kuzmenko, I Vaknin, D AF Kooijman, Edgar E. Graber, Zachary T. Wang, Wenji Kuzmenko, Ivan Vaknin, David TI Specificity and Competitive Cation Association to Phosphatidylinositol-4,5-Bisphosphate Model Membranes SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Kooijman, Edgar E.] Kent State Univ, Biol Sci, Kent, OH 44242 USA. [Graber, Zachary T.] Kent State Univ, Chem & Biochem, Kent, OH 44242 USA. [Wang, Wenji; Vaknin, David] Iowa State Univ, Ames Lab, Ames, IA USA. [Wang, Wenji; Vaknin, David] Iowa State Univ, Dept Phys, Ames, IA USA. [Kuzmenko, Ivan] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. RI Vaknin, David/B-3302-2009 OI Vaknin, David/0000-0002-0899-9248 NR 0 TC 0 Z9 0 U1 0 U2 1 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 2768-Pos BP 546A EP 546A PG 1 WC Biophysics SC Biophysics GA CT5KV UT WOS:000362849600376 ER PT J AU Henderson, JM Cao, KD Gong, ZL Tietjen, GT Heffern, CTR Kerr, D Iyengar, N Roy, I Waring, AJ Meron, M Lin, BH Satija, S Majewski, J Lee, KYC AF Henderson, J. Michael Cao, Kathleen D. Gong, Zhiliang L. Tietjen, Gregory T. Heffern, Charles T. R. Kerr, Daniel Iyengar, Nishanth Roy, Indroneil Waring, Alan J. Meron, Mati Lin, Binhua Satija, Sushil Majewski, Jaroslaw Lee, Ka Yee C. TI Activity of Antimicrobial Peptide Protegrin-1 is Tuned by Membrane Cholesterol Content SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Henderson, J. Michael; Cao, Kathleen D.; Gong, Zhiliang L.; Heffern, Charles T. R.; Iyengar, Nishanth; Lee, Ka Yee C.] Univ Chicago, Chem, Chicago, IL 60637 USA. [Tietjen, Gregory T.] Yale Univ, Sch Engn & Appl Sci, New Haven, CT USA. [Kerr, Daniel] Univ Chicago, Inst Biophys Dynam, Chicago, IL 60637 USA. [Roy, Indroneil] CUNY City Coll, Chem Engn, New York, NY 10031 USA. [Waring, Alan J.] Univ Calif Los Angeles, Los Angeles, CA USA. [Waring, Alan J.] Univ Calif Irvine, Irvine, CA USA. [Meron, Mati; Lin, Binhua] Univ Chicago, Ctr Adv Radiat Sources, Chicago, IL 60637 USA. [Satija, Sushil] NIST, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Majewski, Jaroslaw] Los Alamos Natl Lab, Los Alamos Neutron Sci Ctr, Los Alamos, NM USA. NR 0 TC 0 Z9 0 U1 2 U2 2 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 2792-Pos BP 550A EP 551A PG 2 WC Biophysics SC Biophysics GA CT5KV UT WOS:000362849600400 ER PT J AU Nguyen, PT Kimball, IH Eum, KS Cohen, BE Sack, JT Yarov-Yarovoy, V AF Nguyen, Phuong T. Kimball, Ian H. Eum, Kenneth S. Cohen, Bruce E. Sack, Jon T. Yarov-Yarovoy, Vladimir TI Understanding the State Dependence of Voltage Sensor Toxin Action on Voltage Gated Sodium Channels SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Nguyen, Phuong T.; Kimball, Ian H.; Eum, Kenneth S.; Sack, Jon T.; Yarov-Yarovoy, Vladimir] Univ Calif Davis, Davis, CA 95616 USA. [Nguyen, Phuong T.; Eum, Kenneth S.; Cohen, Bruce E.; Sack, Jon T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 2904-Pos BP 574A EP 574A PG 1 WC Biophysics SC Biophysics GA CT5KV UT WOS:000362849600512 ER PT J AU Moonshiram, D Aukauloo, A Avenier, F Southworth, S Lehmann, C Picon, A AF Moonshiram, Dooshaye Aukauloo, Ally Avenier, Frederic Southworth, Steve Lehmann, Carl Picon, Antonio TI Studying the Structural and Electronic Configurations during Photocatalytic Activation of O2 at a Diiron(II) Complex SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Moonshiram, Dooshaye; Southworth, Steve; Lehmann, Carl; Picon, Antonio] Argonne Natl Lab, Phys, Lemont, IL USA. [Aukauloo, Ally; Avenier, Frederic] Univ Paris 11, Inorgan Chem Lab, Orsay, France. RI Moonshiram, Dooshaye/J-5138-2014 OI Moonshiram, Dooshaye/0000-0002-9075-3035 NR 2 TC 0 Z9 0 U1 2 U2 3 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 3052-Pos BP 605A EP 605A PG 1 WC Biophysics SC Biophysics GA CT5KV UT WOS:000362849600660 ER PT J AU Purohit, V Moonshiram, D Yan, LF Alperovich, I Pushkar, Y AF Purohit, Vatsal Moonshiram, Dooshaye Yan, Lifen Alperovich, Igor Pushkar, Yulia TI EPR and X-Ray Spectroscopy Characterization of Reported Mono-Ruthenium Water Splitting Catalysts SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Purohit, Vatsal] Purdue Univ, Interdisplinary Life Sci Program, W Lafayette, IN 47907 USA. [Moonshiram, Dooshaye] Argonne Natl Lab, Lemont, IL USA. [Yan, Lifen; Pushkar, Yulia] Purdue Univ, Phys, W Lafayette, IN 47907 USA. [Alperovich, Igor] South Fed Univ, Res Ctr Nanoscale Struct Matter, W Lafayette, IN USA. RI Moonshiram, Dooshaye/J-5138-2014 OI Moonshiram, Dooshaye/0000-0002-9075-3035 NR 0 TC 0 Z9 0 U1 2 U2 8 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 3054-Pos BP 605A EP 605A PG 1 WC Biophysics SC Biophysics GA CT5KV UT WOS:000362849600662 ER PT J AU He, QP Aronova, MA Joy, DC Zhang, GF Leapman, RD AF He, Qianping Aronova, Maria A. Joy, David C. Zhang, Guofeng Leapman, Richard D. TI Sub-Surface Serial Block Face Scanning Electron Microscopy SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [He, Qianping; Aronova, Maria A.; Zhang, Guofeng; Leapman, Richard D.] NIBIB, NIH, Bethesda, MD USA. [Joy, David C.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Joy, David C.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN USA. NR 0 TC 0 Z9 0 U1 2 U2 3 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 3125-Pos BP 619A EP 620A PG 2 WC Biophysics SC Biophysics GA CT5KV UT WOS:000362849600733 ER PT J AU Bohon, J Muller, EM Ding, WX Gaowei, MJ Zhou, TY Smedley, J AF Bohon, Jen Muller, Erik M. Ding, Wenxiang Gaowei, Mengjia Zhou, Tianyi Smedley, John TI Transmission X-Ray Imaging Detector Captures the Last Light at NSLS SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Bohon, Jen] Case Western Reserve Univ, Ctr Synchrotron Biosci, Upton, NY USA. [Muller, Erik M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ding, Wenxiang] SUNY Stony Brook, Dept Elect & Comp Engn, Stony Brook, NY 11794 USA. [Gaowei, Mengjia; Smedley, John] Brookhaven Natl Lab, Instrumentat Div, Upton, NY 11973 USA. [Zhou, Tianyi] SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11794 USA. NR 0 TC 0 Z9 0 U1 2 U2 3 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 3129-Pos BP 620A EP 620A PG 1 WC Biophysics SC Biophysics GA CT5KV UT WOS:000362849600737 ER PT J AU Burman, SSR Pacella, MS De Yoreo, JJ Gray, JJ AF Burman, Shourya Sonkar Roy Pacella, Michael S. De Yoreo, James J. Gray, Jeffrey J. TI Characterization of Peptides Designed to Control Crystal Nucleation and Growth SO BIOPHYSICAL JOURNAL LA English DT Meeting Abstract CT 59th Annual Meeting of the Biophysical-Society CY FEB 07-11, 2015 CL Baltimore, MD SP Biophys Soc C1 [Burman, Shourya Sonkar Roy; Gray, Jeffrey J.] Johns Hopkins Univ, Chem & Biomol Engn, Baltimore, MD USA. [Pacella, Michael S.] Johns Hopkins Univ, Biomed Engn, Baltimore, MD USA. [De Yoreo, James J.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. [De Yoreo, James J.] Johns Hopkins Univ, Program Mol Biophys, Baltimore, MD USA. NR 0 TC 0 Z9 0 U1 2 U2 3 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 27 PY 2015 VL 108 IS 2 SU 1 MA 3190-Pos BP 633A EP 633A PG 1 WC Biophysics SC Biophysics GA CT5KV UT WOS:000362849600798 ER PT J AU Li, ZJ Feng, S Liu, YG Lin, WY Zhang, MH Toto, T Vogelmann, AM Endo, S AF Li, Zhijin Feng, Sha Liu, Yangang Lin, Wuyin Zhang, Minghua Toto, Tami Vogelmann, Andrew M. Endo, Satoshi TI Development of fine-resolution analyses and expanded large-scale forcing properties: 1. Methodology and evaluation SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE fine-resolution analyses; data assimilation; high-resolution observations ID COMMUNITY ATMOSPHERE MODEL; CLOUD MICROPHYSICS SCHEME; DATA ASSIMILATION SYSTEM; SINGLE-COLUMN MODELS; VARIATIONAL ANALYSIS; RESOLVING MODEL; KALMAN FILTER; RADIATION; SMOOTHER; PROGRAM AB We produce fine-resolution, three-dimensional fields of meteorological and other variables for the U.S. Department of Energy's Atmospheric Radiation Measurement (ARM) Southern Great Plains site. The Community Gridpoint Statistical Interpolation system is implemented in a multiscale data assimilation (MS-DA) framework that is used within the Weather Research and Forecasting model at a cloud-resolving resolution of 2km. The MS-DA algorithm uses existing reanalysis products and constrains fine-scale atmospheric properties by assimilating high-resolution observations. A set of experiments show that the data assimilation analysis realistically reproduces the intensity, structure, and time evolution of clouds and precipitation associated with a mesoscale convective system. Evaluations also show that the large-scale forcing derived from the fine-resolution analysis has an overall accuracy comparable to the existing ARM operational product. For enhanced applications, the fine-resolution fields are used to characterize the contribution of subgrid variability to the large-scale forcing and to derive hydrometeor forcing, which are presented in companion papers. C1 [Li, Zhijin; Feng, Sha] CALTECH, Jet Prop Lab, Pasadena, CA 91125 USA. [Li, Zhijin; Feng, Sha] Univ Calif Los Angeles, Joint Inst Reg Earth Syst Sci & Engn, Los Angeles, CA USA. [Liu, Yangang; Lin, Wuyin; Toto, Tami; Vogelmann, Andrew M.; Endo, Satoshi] Brookhaven Natl Lab, Dept Environm Sci, Upton, NY 11973 USA. [Zhang, Minghua] SUNY Stony Brook, Inst Terr & Planetary Atmospheres, Stony Brook, NY 11794 USA. RP Li, ZJ (reprint author), CALTECH, Jet Prop Lab, Pasadena, CA 91125 USA. EM Zhijin.Li@jpl.nasa.gov RI Liu, Yangang/H-6154-2011; Vogelmann, Andrew/M-8779-2014 OI Vogelmann, Andrew/0000-0003-1918-5423 FU U.S. Department of Energy Earth System Modeling (ESM) program via the FAst-physics System TEstbed and Research (FASTER) FX The research described in this publication was supported by the U.S. Department of Energy Earth System Modeling (ESM) program via the FAst-physics System TEstbed and Research (FASTER) project www.bnl.gov/faster. The research was carried out, in part, at Jet Propulsion Laboratory (JPL) California Institute of Technology, under a contract with the National Aeronautics and Space Administration (NASA). The authors thank the ARM program for providing the SGP observations. The authors are grateful to Ann Fridlind (NASA Goddard Institute for Space Studies) for numerous stimulating discussions, insightful suggestions, and strong support. The authors thank the anonymous reviewers for comments that were very helpful in improving the manuscript. NR 48 TC 4 Z9 4 U1 0 U2 9 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD JAN 27 PY 2015 VL 120 IS 2 BP 654 EP 666 DI 10.1002/2014JD022245 PG 13 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA CC1QQ UT WOS:000350117100017 ER PT J AU Feng, S Li, ZJ Liu, YG Lin, WY Zhang, MH Toto, T Vogelmann, AM Endo, S AF Feng, Sha Li, Zhijin Liu, Yangang Lin, Wuyin Zhang, Minghua Toto, Tami Vogelmann, Andrew M. Endo, Satoshi TI Development of fine-resolution analyses and expanded large-scale forcing properties: 2. Scale awareness and application to single-column model experiments SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE scale-aware forcing; subgrid-scale dynamic process; single-column model ID COMMUNITY ATMOSPHERE MODEL; CLOUD MICROPHYSICS SCHEME; RESOLVING MODEL; CLIMATE; SYSTEM; RADIATION; PROGRAM; WEATHER; TESTS; CAM3 AB Fine-resolution three-dimensional fields have been produced using the Community Gridpoint Statistical Interpolation (GSI) data assimilation system for the U.S. Department of Energy's Atmospheric Radiation Measurement Program (ARM) Southern Great Plains region. The GSI system is implemented in a multiscale data assimilation framework using the Weather Research and Forecasting model at a cloud-resolving resolution of 2km. From the fine-resolution three-dimensional fields, large-scale forcing is derived explicitly at grid-scale resolution; a subgrid-scale dynamic component is derived separately, representing subgrid-scale horizontal dynamic processes. Analyses show that the subgrid-scale dynamic component is often a major component over the large-scale forcing for grid scales larger than 200km. The single-column model (SCM) of the Community Atmospheric Model version 5 is used to examine the impact of the grid-scale and subgrid-scale dynamic components on simulated precipitation and cloud fields associated with a mesoscale convective system. It is found that grid-scale size impacts simulated precipitation, resulting in an overestimation for grid scales of about 200km but an underestimation for smaller grids. The subgrid-scale dynamic component has an appreciable impact on the simulations, suggesting that grid-scale and subgrid-scale dynamic components should be considered in the interpretation of SCM simulations. C1 [Feng, Sha; Li, Zhijin] Univ Calif Los Angeles, Joint Inst Reg Earth Syst Sci & Engn, Los Angeles, CA 90095 USA. [Feng, Sha; Li, Zhijin] CALTECH, Jet Prop Lab, Pasadena, CA USA. [Liu, Yangang; Lin, Wuyin; Toto, Tami; Vogelmann, Andrew M.; Endo, Satoshi] Brookhaven Natl Lab, Dept Environm Sci, Upton, NY 11973 USA. [Zhang, Minghua] SUNY Stony Brook, Stony Brook, NY 11794 USA. RP Feng, S (reprint author), Univ Calif Los Angeles, Joint Inst Reg Earth Syst Sci & Engn, Los Angeles, CA 90095 USA. EM sfeng@jifresse.ucla.edu RI Liu, Yangang/H-6154-2011; Vogelmann, Andrew/M-8779-2014 OI Vogelmann, Andrew/0000-0003-1918-5423 FU U.S. Department of Energy Earth System Modeling program via the FASTER project FX The research described in this publication was supported by the U.S. Department of Energy Earth System Modeling program via the FASTER project (http://www.bnl.gov/faster). This research was carried out, in part, at the Jet Propulsion Laboratory, California Institute of Technology, under a contract with the National Aeronautics and Space Administration (NASA). The authors are grateful to Ann Fridlind (NASA Goddard Institute for Space Studies) and Leo J. Donner (Geophysical Fluid Dynamics Laboratory) for stimulating the discussions and insightful suggestions. Data from the U.S. Department of Energy's SGP ARM Climate Research Facility (http://www.arm.gov/) are used in this article. The authors thank the anonymous reviewers for their comments that were very helpful in improving the manuscript. NR 28 TC 3 Z9 3 U1 0 U2 6 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD JAN 27 PY 2015 VL 120 IS 2 BP 667 EP 677 DI 10.1002/2014JD022254 PG 11 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA CC1QQ UT WOS:000350117100018 ER PT J AU Hu, L Montzka, SA Miller, JB Andrews, AE Lehman, SJ Miller, BR Thoning, K Sweeney, C Chen, HL Godwin, DS Masarie, K Bruhwiler, L Fischer, ML Biraud, SC Torn, MS Mountain, M Nehrkorn, T Eluszkiewicz, J Miller, S Draxler, RR Stein, AF Hall, BD Elkins, JW Tans, PP AF Hu, Lei Montzka, Stephen A. Miller, John B. Andrews, Aryln E. Lehman, Scott J. Miller, Benjamin R. Thoning, Kirk Sweeney, Colm Chen, Huilin Godwin, David S. Masarie, Kenneth Bruhwiler, Lori Fischer, Marc L. Biraud, Sebastien C. Torn, Margaret S. Mountain, Marikate Nehrkorn, Thomas Eluszkiewicz, Janusz Miller, Scot Draxler, Roland R. Stein, Ariel F. Hall, Bradley D. Elkins, James W. Tans, Pieter P. TI US emissions of HFC-134a derived for 2008-2012 from an extensive flask-air sampling network SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE HFC-134a; emissions; inverse modeling; atmosphere based; US ID ATMOSPHERIC OBSERVATIONS; EUROPEAN EMISSIONS; TRANSPORT MODELS; GLOBAL EMISSIONS; INVERSION METHOD; UNITED-STATES; STILT MODEL; PART 1; CO2; PERSPECTIVE AB U.S. national and regional emissions of HFC-134a are derived for 2008-2012 based on atmospheric observations from ground and aircraft sites across the U.S. and a newly developed regional inverse model. Synthetic data experiments were first conducted to optimize the model assimilation design and to assess model-data mismatch errors and prior flux error covariances computed using a maximum likelihood estimation technique. The synthetic data experiments also tested the sensitivity of derived national and regional emissions to a range of assumed prior emissions, with the goal of designing a system that was minimally reliant on the prior. We then explored the influence of additional sources of error in inversions with actual observations, such as those associated with background mole fractions and transport uncertainties. Estimated emissions of HFC-134a range from 52 to 61 Gg yr(-1) for the contiguous U.S. during 2008-2012 for inversions using air transport from Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model driven by the 12km resolution meteorogical data from North American Mesoscale Forecast System (NAM12) and all tested combinations of prior emissions and background mole fractions. Estimated emissions for 2008-2010 were 20% lower when specifying alternative transport from Stochastic Time-Inverted Lagrangian Transport (STILT) model driven by the Weather Research and Forecasting (WRF) meteorology. Our estimates (for HYSPLIT-NAM12) are consistent with annual emissions reported by U.S. Environmental Protection Agency for the full study interval. The results suggest a 10-20% drop in U.S. national HFC-134a emission in 2009 coincident with a reduction in transportation-related fossil fuel CO2 emissions, perhaps related to the economic recession. All inversions show seasonal variation in national HFC-134a emissions in all years, with summer emissions greater than winter emissions by 20-50%. C1 [Hu, Lei; Miller, John B.; Miller, Benjamin R.; Sweeney, Colm] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. [Hu, Lei; Montzka, Stephen A.; Miller, John B.; Andrews, Aryln E.; Miller, Benjamin R.; Thoning, Kirk; Sweeney, Colm; Masarie, Kenneth; Bruhwiler, Lori; Hall, Bradley D.; Elkins, James W.; Tans, Pieter P.] NOAA, Global Monitoring Div, Earth Syst Res Lab, Boulder, CO USA. [Lehman, Scott J.] Univ Colorado, Inst Arctic & Alpine Res, Boulder, CO 80309 USA. [Chen, Huilin] Univ Groningen, Ctr Isotope Res, Groningen, Netherlands. [Godwin, David S.] US EPA, Alternat & Emiss Reduct Branch, Stratospher Protect Div, Off Atmospher Programs,Off Air & Radiat, Washington, DC 20460 USA. [Fischer, Marc L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Biraud, Sebastien C.; Torn, Margaret S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Mountain, Marikate; Nehrkorn, Thomas; Eluszkiewicz, Janusz] Atmospher & Environm Res, Lexington, MA USA. [Miller, Scot] Harvard Univ, Dept Earth & Planetary Sci, Cambridge, MA 02138 USA. [Draxler, Roland R.; Stein, Ariel F.] NOAA, Air Resources Lab, College Pk, MD USA. RP Hu, L (reprint author), Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. EM lei.hu@colorado.edu; stephen.a.montzka@noaa.gov RI Andrews, Arlyn/K-3427-2012; Chen, Huilin/J-9479-2012; Stein, Ariel F/L-9724-2014; Torn, Margaret/D-2305-2015; Biraud, Sebastien/M-5267-2013; OI Chen, Huilin/0000-0002-1573-6673; Stein, Ariel F/0000-0002-9560-9198; Biraud, Sebastien/0000-0001-7697-933X; Montzka, Stephen/0000-0002-9396-0400; Nehrkorn, Thomas/0000-0003-0637-3468 FU NOAA Climate Program Office's Atmospheric Chemistry, Carbon Cycle, and Climate (AC4) program - North American Carbon Program; California Energy Commission; California Air Resources Board [DE-AC02-05CH11231]; U.S. Department of Energy, Office of Science, Atmospheric Radiation Measurement Program [DE-AC02-05CH11231]; U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231]; NOAA's Climate Program Office under the CarbonTracker-Lagrange project FX This work was performed while one of us (LH) was a National Research Council postdoctoral fellow and was funded in part by NOAA Climate Program Office's Atmospheric Chemistry, Carbon Cycle, and Climate (AC4) program in support of the North American Carbon Program. Flask sampling at the WGC and STR towers were partially supported by a California Energy Commission and the California Air Resources Board grants to LBNL under contract DE-AC02-05CH11231, while aircraft sampling above the SGP site was supported by the U.S. Department of Energy, Office of Science, Atmospheric Radiation Measurement Program and Office of Biological and Environmental Research, both underx U.S. Department of Energy contract DE-AC02-05CH11231. WRF-STILT runs were supported by NOAA's Climate Program Office under the CarbonTracker-Lagrange project. This inversion analysis was conducted using the high performance computing system in the NOAA Environmental Security Computing Center, located in Fairmont, West Virginia, USA. We thank A. Jacobson and S. Basu for useful discussions related to inversion problems. We thank C. Siso, D. Mondeel, P. M. Lang, J. Higgs, M. Crotwell, S. Wolter, D. Neff, J. Kofler, and others involved with flask analysis and the large team of collaborators associated with operation, maintenance, and logistics of NOAA's Cooperative U.S.- and global-scale Greenhouse Gas Reference flask sampling networks. Measured atmospheric mole fractions of HFC-134a and calculated footprints used in this analysis can be downloaded at NOAA/ESRL/GMD website (http://www.esrl.noaa.gov/gmd/hats/gases/HFC134a.html). NR 68 TC 4 Z9 4 U1 2 U2 16 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD JAN 27 PY 2015 VL 120 IS 2 BP 801 EP 825 DI 10.1002/2014JD022617 PG 25 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA CC1QQ UT WOS:000350117100026 ER PT J AU Hu, L Millet, DB Baasandorj, M Griffis, TJ Travis, KR Tessum, CW Marshall, JD Reinhart, WF Mikoviny, T Muller, M Wisthaler, A Graus, M Warneke, C de Gouw, J AF Hu, Lu Millet, Dylan B. Baasandorj, Munkhbayar Griffis, Timothy J. Travis, Katherine R. Tessum, Christopher W. Marshall, Julian D. Reinhart, Wesley F. Mikoviny, Tomas Mueller, Markus Wisthaler, Armin Graus, Martin Warneke, Carsten de Gouw, Joost TI Emissions of C-6-C-8 aromatic compounds in the United States: Constraints from tall tower and aircraft measurements SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE US EPA NEI08; RETRO; Bayesian inversion; benzene; toluene; xylenes ID SECONDARY ORGANIC AEROSOL; US UPPER MIDWEST; HYDROCARBON EMISSIONS; AMBIENT AIR; TRACE GASES; CHEMISTRY; BENZENE; MODEL; PHOTOOXIDATION; TOLUENE AB We present two full years of continuous C-6-C-8 aromatic compound measurements by PTR-MS at the KCMP tall tower (Minnesota, US) and employ GEOS-Chem nested grid simulations in a Bayesian inversion to interpret the data in terms of new constraints on US aromatic emissions. Based on the tall tower data, we find that the RETRO inventory (year-2000) overestimates US C-6-C-8 aromatic emissions by factors of 2.0-4.5 during 2010-2011, likely due in part to post-2000 reductions. Likewise, our implementation of the US EPA's NEI08 overestimates the toluene flux by threefold, reflecting an inventory bias in non-road emissions plus uncertainties associated with species lumping. Our annual top-down emission estimates for benzene and C-8 aromatics agree with the NEI08 bottom-up values, as does the inferred contribution from non-road sources. However, the NEI08 appears to underestimate on-road emissions of these compounds by twofold during the warm season. The implied aromatic sources upwind of North America are more than double the prior estimates, suggesting a substantial underestimate of East Asian emissions, or large increases there since 2000. Long-range transport exerts an important influence on ambient benzene over the US: on average 43% of its wintertime abundance in the US Upper Midwest is due to sources outside North America. Independent aircraft measurements show that the inventory biases found here for C-6-C-8 aromatics also apply to other parts of the US, with notable exceptions for toluene in California and Houston, Texas. Our best estimates of year-2011 contiguous US emissions are 206 (benzene), 408 (toluene), and 822 (C-8 aromatics) GgC. C1 [Hu, Lu; Millet, Dylan B.; Baasandorj, Munkhbayar; Griffis, Timothy J.; Reinhart, Wesley F.] Univ Minnesota, Dept Soil Water & Climate, St Paul, MN 55108 USA. [Hu, Lu; Travis, Katherine R.] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. [Tessum, Christopher W.; Marshall, Julian D.] Univ Minnesota, Dept Civil Environm & Geoengn, Minneapolis, MN USA. [Mikoviny, Tomas; Wisthaler, Armin] Univ Oslo, Dept Chem, Oslo, Norway. [Mikoviny, Tomas] Oak Ridge Associated Univ, Oak Ridge, TN USA. [Mueller, Markus; Wisthaler, Armin] Univ Innsbruck, Inst Ion Phys & Appl Phys, A-6020 Innsbruck, Austria. [Graus, Martin; Warneke, Carsten; de Gouw, Joost] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. [Graus, Martin; Warneke, Carsten; de Gouw, Joost] NOAA, Div Chem Sci, Earth Syst Res Lab, Boulder, CO USA. RP Millet, DB (reprint author), Univ Minnesota, Dept Soil Water & Climate, St Paul, MN 55108 USA. EM dbm@umn.edu RI Muller, Markus/L-1699-2014; de Gouw, Joost/A-9675-2008; Warneke, Carsten/E-7174-2010; Millet, Dylan/G-5832-2012; Travis, Katherine/G-1417-2016; Chem, GEOS/C-5595-2014; Manager, CSD Publications/B-2789-2015; Griffis, Timothy/A-5707-2011; Graus, Martin/E-7546-2010 OI Muller, Markus/0000-0003-4110-8950; de Gouw, Joost/0000-0002-0385-1826; Travis, Katherine/0000-0003-1628-0353; Hu, Lu/0000-0002-4892-454X; Graus, Martin/0000-0002-2025-9242 FU National Science Foundation [0937004, 1148951]; Minnesota Supercomputing Institute; University of Minnesota Doctoral Dissertation Fellowship; NASA Postdoctoral Program FX This study was supported by the National Science Foundation (grants 0937004 and 1148951), by the Minnesota Supercomputing Institute, and by a University of Minnesota Doctoral Dissertation Fellowship. We thank Tom Nelson and Minnesota Public Radio for their logistical support at the KCMP tall tower. PTR-MS measurements during DISCOVER-AQ and DC-3 were supported by the Austrian Space Applications Programme (ASAP, bmvit, FFG-ALR). TM was supported by the NASA Postdoctoral Program. We acknowledge the US Environmental Protection Agency for providing 2006 and 2010 North American emission inventories. These emission inventories are intended for research purposes and were developed for Phase 2 of the Air Quality Model Evaluation International Initiative (AQMEII) using information from the 2008-based modeling platform (http://www.epa.gov/ttn/chief/emch/index.html#2008) as a starting point. Measurements from the KCMP tall tower described here are available for download at http://www.atmoschem.umn.edu/data.htm. NR 75 TC 12 Z9 12 U1 5 U2 33 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD JAN 27 PY 2015 VL 120 IS 2 BP 826 EP 842 DI 10.1002/2014JD022627 PG 17 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA CC1QQ UT WOS:000350117100027 ER PT J AU Vogt, L Ertem, MZ Pal, R Brudvig, GW Batista, VS AF Vogt, Leslie Ertem, Mehmed Z. Pal, Rhitankar Brudvig, Gary W. Batista, Victor S. TI Computational Insights on Crystal Structures of the Oxygen-Evolving Complex of Photosystem II with Either Ca2+ or Ca2+ Substituted by Sr2+ SO BIOCHEMISTRY LA English DT Article ID SUBSTRATE WATER-MOLECULES; EFFECTIVE CORE POTENTIALS; ELECTRONIC-STRUCTURE; MANGANESE CLUSTER; OXIDATION-STATE; SPECTROSCOPY; RESOLUTION; EVOLUTION; EXCHANGE; CALCIUM AB The oxygen-evolving complex of photosystem II can function with either Ca2+ or Sr2+ as the heterocation, but the reason for different turnover rates remains unresolved despite reported X-ray crystal structures for both forms. Using quantum mechanics/molecular mechanics (QM/MM) calculations, we optimize structures with each cation in both the resting state (S-1) and in a series of reduced states (S-0, S-1, and S-2). Through comparison with experimental data, we determine that the X-ray crystal structures with either Ca2+ or Sr2+ are most consistent with the S-2 state (i.e., Mn-4[III,III,III,II] with O-4 and O-5 protonated). As expected, the QM/MM models show that Ca2+/Sr2+ substitution results in the elongation of the heterocation bonds and the displacement of terminal waters W-3 and W-4. The optimized structures also show that hydrogen-bonded W-5 is displaced in all S states with Sr2+ as the heterocation, suggesting that this water may play a critical role during water oxidation. C1 [Vogt, Leslie; Ertem, Mehmed Z.; Pal, Rhitankar; Brudvig, Gary W.; Batista, Victor S.] Yale Univ, Dept Chem, New Haven, CT 06511 USA. [Ertem, Mehmed Z.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Vogt, L (reprint author), NYU, Dept Chem, New York, NY 10003 USA. EM leslie.vogt@gmail.com; victor.batista@yale.edu FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy [DE-SC0001423]; Computational Materials and Chemical Sciences project at Brookhaven National Laboratory [DE-AC02-98CH10886]; [DE-FG02-05ER15646] FX The authors acknowledge funding from the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy grant DE-SC0001423 (V.S.B.); contract DE-AC02-98CH10886, a Computational Materials and Chemical Sciences project at Brookhaven National Laboratory (M.Z.E.); and grant DE-FG02-05ER15646 (G.W.B.). NR 45 TC 16 Z9 16 U1 3 U2 43 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD JAN 27 PY 2015 VL 54 IS 3 BP 820 EP 825 DI 10.1021/bi5011706 PG 6 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CA0PA UT WOS:000348618100017 PM 25555204 ER PT J AU Homyak, P Liu, Y Ferdous, S Liu, F Russell, TP Coughlin, EB AF Homyak, Patrick Liu, Yao Ferdous, Sunzida Liu, Feng Russell, Thomas P. Coughlin, E. Bryan TI Effect of Pendant Functionality in Thieno[3,4-b]thiophene-alt-benzodithiophene Polymers for OPVs SO CHEMISTRY OF MATERIALS LA English DT Article ID POWER CONVERSION EFFICIENCY; SOLAR-CELL PERFORMANCE; HETEROJUNCTION PHOTOVOLTAIC CELLS; COPOLYMER; RECOMBINATION; INTERLAYERS; MORPHOLOGY; TANDEM; ALKYL AB The performance of organic photovoltaics (OPVs) is heavily dependent on the structure and functionalization of the conjugated polymer used in the active absorbing layer. Using a set of materials based on poly(thieno[3,4-b]thiophene-alt-benzodithiophene) with different alkyl, aryl, perfluoroalkyl, and perfluoroaryl pendant functionalities, we have studied the correlation between absorbance, morphology, crystallinity, charge mobility, and the OPV performance in an effort to identify structure-performance relationships. The perfluorinated pendants on PTF8B and PTFPB were shown to significantly enhance the V-oc in the OPV devices (by similar to 0.2 V), but also induced the formation of larger phase separated PCBM-rich domains. PT8B and PTFPB devices reached average efficiencies of similar to 3.2%. C1 [Homyak, Patrick; Liu, Yao; Ferdous, Sunzida; Russell, Thomas P.; Coughlin, E. Bryan] Univ Massachusetts, Conte Ctr Polymer Res, Dept Polymer Sci & Engn, Amherst, MA 01003 USA. [Liu, Feng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Liu, Feng] Univ Massachusetts, Energy Frontier Res Ctr PHaSE, Amherst, MA 01003 USA. RP Russell, TP (reprint author), Univ Massachusetts, Conte Ctr Polymer Res, Dept Polymer Sci & Engn, 120 Governors Dr, Amherst, MA 01003 USA. EM Russell@mail.pse.umass.edu; Coughlin@mail.pse.umass.edu RI Liu, Feng/J-4361-2014; liu, yao/H-2534-2016 OI Liu, Feng/0000-0002-5572-8512; FU Polymer-Based Materials for Harvesting Solar Energy (PHaSE), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001087]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-76SF00515]; DOE, Office of Science; DOE, Office of Basic Energy Sciences FX This work is supported as part of Polymer-Based Materials for Harvesting Solar Energy (PHaSE), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award DE-SC0001087. Portions of this research were carried out at the Stanford Synchrotron Radiation Lightsource, a national user facility operated by Stanford University on behalf of the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract DE-AC02-76SF00515. The authors also acknowledge A. Hexemer and E. Schaible for support in ALS beamline 7.3.3. Portions of this research were carried out at the Advanced Light Source, Berkeley National Laboratory, which is supported by the DOE, Office of Science, and Office of Basic Energy Sciences. NR 45 TC 9 Z9 9 U1 1 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JAN 27 PY 2015 VL 27 IS 2 BP 443 EP 449 DI 10.1021/cm503334h PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CA0PD UT WOS:000348618400007 ER PT J AU Weidman, MC Yager, KG Tisdale, WA AF Weidman, Mark C. Yager, Kevin G. Tisdale, William A. TI Interparticle Spacing and Structural Ordering in Superlattice PbS Nanocrystal Solids Undergoing Ligand Exchange SO CHEMISTRY OF MATERIALS LA English DT Article ID QUANTUM-DOT SOLIDS; LIGHT-EMITTING-DIODES; ELECTRICAL-PROPERTIES; FILMS; PHOTOVOLTAICS; TRANSPORT AB Controlling the interparticle spacing in quantum dot (QD) solids is the most readily accessible way to control transport rates between neighboring QDs and a critical strategy for device optimization. Here, we use X-ray scattering to accurately measure the interparticle spacing in films of highly monodisperse lead sulfide (PbS) QDs that have undergone a variety of device-relevant ligand exchanges. We tabulate these values for use in simulations and to assist in data interpretation. We find that monothiol and dithiol ligand species typically result in interparticle spacings that are equal to the length of a single monothiol or dithiol ligand. Additionally, we find that spin-coating a thick film of QDs followed by a long-duration ligand exchange results in a significantly closer-packed arrangement than spin-coating many thin layers with short-duration ligand exchanges in between (layer-by-layer method). The former method preserves a remarkable degree of the superlattice order that was present in the film prior to ligand exchange, but also generates cracks due to volume loss within the solid. The similarity in interparticle spacing for many of the shortest ligands points to the importance of other factors, such as energy level matching and surface passivation in choosing the optimal ligand for a given device application. These results provide strategies for producing highly ordered QD solids with compact and functional ligands, which could lead to enhanced interdot coupling and transport phenomena. C1 [Weidman, Mark C.; Tisdale, William A.] MIT, Dept Chem Engn, Cambridge, MA 02139 USA. [Yager, Kevin G.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Tisdale, WA (reprint author), MIT, Dept Chem Engn, Cambridge, MA 02139 USA. EM tisdale@mit.edu RI Yager, Kevin/F-9804-2011; Tisdale, William/E-8466-2012; OI Yager, Kevin/0000-0001-7745-2513; Tisdale, William/0000-0002-6615-5342; , /0000-0001-6034-6458 FU MIT Energy Initiative Seed Fund Program FX MIT Energy Initiative Seed Fund Program. NR 33 TC 15 Z9 15 U1 2 U2 41 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JAN 27 PY 2015 VL 27 IS 2 BP 474 EP 482 DI 10.1021/cm503626s PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CA0PD UT WOS:000348618400011 ER PT J AU Al Saghir, K Chenu, S Veron, E Fayon, F Suchomel, M Genevois, C Porcher, F Matzen, G Massiot, D Allix, M AF Al Saghir, Kholoud Chenu, Sebastien Veron, Emmanuel Fayon, Franck Suchomel, Matthew Genevois, Cecile Porcher, Florence Matzen, Guy Massiot, Dominique Allix, Mathieu TI Transparency through Structural Disorder: A New Concept for Innovative Transparent Ceramics SO CHEMISTRY OF MATERIALS LA English DT Article ID FABRICATION; ALUMINA; FUTURE; LASERS; GLASS; NMR AB Transparent polycrystalline ceramics present significant economical and functional advantages over single crystal materials for optical, communication, and laser technologies. To date, transparency in these ceramics is ensured either by an optical isotropy (i.e., cubic symmetry) or a nanometric crystallite size, and the main challenge remains to eliminate porosity through complex high pressurehigh temperature synthesis. Here we introduce a new concept to achieve ultimate transparency reaching the theoretical limit. We use a controlled degree of chemical disorder in the structure to obtain optical isotropy at the micrometer length scale. This approach can be applied in the case of anisotropic structures and micrometer scale crystal size ceramics. We thus report Sr1+x/2Al2+xSi2-xO8 (0 < x <= 0.4) readily scalable polycrystalline ceramics elaborated by full and congruent crystallization from glass. These materials reach 90% transmittance. This innovative method should drive the development of new highly transparent materials with technologically relevant applications. C1 [Al Saghir, Kholoud; Chenu, Sebastien; Veron, Emmanuel; Fayon, Franck; Genevois, Cecile; Matzen, Guy; Massiot, Dominique; Allix, Mathieu] Univ Orleans, CNRS, CEMHTI UPR3079, F-45071 Orleans, France. [Suchomel, Matthew] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Porcher, Florence] CEA Saclay, Lab Leon Brillouin, F-91191 Gif Sur Yvette, France. RP Fayon, F (reprint author), Univ Orleans, CNRS, CEMHTI UPR3079, F-45071 Orleans, France. EM franck.fayon@cnrs-orleans.fr; mathieu.allix@cnrs-orleans.fr RI Massiot, Dominique/C-1287-2008; Fayon, Franck/C-1835-2008; VERON, Emmanuel/C-1825-2008; Allix, Mathieu/C-1679-2008; Chenu, Sebastien/A-3388-2014; OI Massiot, Dominique/0000-0003-1207-7040; Allix, Mathieu/0000-0001-9317-1316; Chenu, Sebastien/0000-0002-5648-9779; SUCHOMEL, Matthew/0000-0002-9500-5079 FU ANR [ANR-12-JS08-0002]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX The authors thank the ANR for its financial support to the project CrystOG ANR-12-JS08-0002 and both the CRMD and CRISMAT/CIMAP laboratories for TEM access. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. Neutron experiments were performed at the Laboratoire Leon Brillouin in Saday (France). DFT computations have been performed at the "Centre de Calcul Scientifique en Region Centre" facility (CCRS - Orleans, France) under the CASCIMODOT program. Domingos De Sousa Meneses is acknowledged for refractive index measurement. NR 30 TC 7 Z9 7 U1 11 U2 80 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JAN 27 PY 2015 VL 27 IS 2 BP 508 EP 514 DI 10.1021/cm5037106 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CA0PD UT WOS:000348618400014 ER PT J AU Larson, AM Moetakef, P Gaskell, K Brown, CM King, G Rodriguez, EE AF Larson, Amber M. Moetakef, Pouya Gaskell, Karen Brown, Craig M. King, Graham Rodriguez, Efrain E. TI Inducing Ferrimagnetism in Insulating Hollandite Ba1.2Mn8O16 SO CHEMISTRY OF MATERIALS LA English DT Article ID OCTAHEDRAL MOLECULAR-SIEVES; BOND-VALENCE PARAMETERS; MAGNETIC-PROPERTIES; MANGANESE OXIDES; TUNNEL STRUCTURE; KAGOME ANTIFERROMAGNET; CATION DISPLACEMENTS; CRYSTAL-STRUCTURE; OXIDATION-STATE; CHEMISTRY AB Magnetic insulators are functional materials with potential applications in spintronics and multiferroics. The hollandites A(x)M(8)O(16), which contain mixed-valent transition metals, have demonstrated ferromagnetism combined with insulating behavior and provide a new platform for exploring the effects of magnetic frustration due to their folded triangular lattice. We have tuned the hollandite BaxMn8O16 from a complex antiferromagnet with Neel temperature (T-N) = 25 K to a ferrimagnet with Curie temperature (T-C) = 180 K via partial cobalt substitution for manganese. Both BaxMn8O16 and BaxCoyMn8-yO16 were prepared by salt flux methods, and combined neutron and X-ray diffraction confirm a distorted hollandite-type structure for both oxides. X-ray photoelectron spectroscopy reveals that the Co2+ substitution drives the average Mn oxidation state from 3.7+ to nearly 4.0+, thereby changing its d-electron count. Magnetization and resistivity measurements show that the cobalt-doped hollandite is a ferrimagnetic insulator, with a high T-C of 180 K. On the basis of neutron diffraction measurements, we provide the first solution of the magnetic structure of BaxMn8O16, which consists of a complex antiferromagnet with a large magnetic unit cell. Upon substituting cobalt for manganese, the magnetic structure changes dramatically, destroying the previously large magnetic unit cell and promoting ferromagnetic alignment along the hollandite tunnel direction. The observed hysteresis at base temperature for BaxCoyMn8-yO16 is explained as arising from uncompensated spins aligned along the (200) crystallographic planes. C1 [Larson, Amber M.; Moetakef, Pouya; Gaskell, Karen; Rodriguez, Efrain E.] Univ Maryland, Dept Chem & Biochem, College Pk, MD 20742 USA. [Brown, Craig M.] NIST, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Brown, Craig M.] Univ Delaware, Dept Chem & Biomol Engn, Newark, DE 19716 USA. [King, Graham] Los Alamos Natl Lab, Lujan Neutron Scattering Ctr, Los Alamos, NM 87545 USA. RP Rodriguez, EE (reprint author), Univ Maryland, Dept Chem & Biochem, College Pk, MD 20742 USA. EM efrain@umd.edu RI King, Graham/E-3632-2010; Moetakef, Pouya/F-6353-2012; Brown, Craig/B-5430-2009 OI King, Graham/0000-0003-1886-7254; Moetakef, Pouya/0000-0003-0642-4704; Brown, Craig/0000-0002-9637-9355 FU DOE [DE-AC52-06NA25396]; Maryland NanoCenter; X-ray Crystallography Center; Surface Analysis Center; NispLab FX This work has benefited from the use of the HIPD beamline at the Lujan Center at Los Alamos Neutron Science Center. Los Alamos National Laboratory is operated by Los Alamos National Security LLC under DOE Contract DE-AC52-06NA25396. We also acknowledge the support of the National Institute of Standards and Technology, U.S. Department of Commerce, in providing the neutron research facilities used in this work. We are grateful for the collaboration of Sarah Stoll and Vidumin Dahanayake of the Georgetown University Chemistry Department in obtaining the ICP-MS measurements of our samples. We acknowledge the support of the Maryland NanoCenter, the X-ray Crystallography Center, Surface Analysis Center, and NispLab. NR 89 TC 3 Z9 3 U1 6 U2 41 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JAN 27 PY 2015 VL 27 IS 2 BP 515 EP 525 DI 10.1021/cm503801j PG 11 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CA0PD UT WOS:000348618400015 ER PT J AU Pellicione, CJ Timofeeva, EV Segre, CU AF Pellicione, Christopher J. Timofeeva, Elena V. Segre, Carlo U. TI In Situ X-ray Absorption Spectroscopy Study of the Capacity Fading Mechanism in Hybrid Sn3O2(OH)(2)/Graphite Battery Anode Nanomaterials SO CHEMISTRY OF MATERIALS LA English DT Article ID LITHIUM-ION BATTERIES; TIN OXIDE; ELECTROCHEMICAL PROPERTIES; ELECTRODE MATERIALS; COMPOSITE; SIZE; INTERCALATION; NANOCOMPOSITE; NANOPARTICLES; DIFFRACTION AB In situ X-ray absorption spectroscopy (XAS) of an electrode material under electrochemical control has enabled a detailed examination of the capacity fading mechanism during charge-discharge cycling in a hybrid nanomaterial, Sn3O2(OH)(2)/graphite, that is considered for use as a high-capacity lithium-ion battery anode. By the use of an original one-pot solvothermal synthesis technique, Sn3O2(OH)(2) nanoparticles were directly deposited on the surface of nanothin graphite and were charged/discharged in situ for several cycles while XAS spectra at the Sn K-edge were taken. Modeling of the collected extended X-ray absorption fine structure (EXAFS) spectra provides detailed information on the Sn-O, Sn-Sn, and Sn-Li coordination numbers and atomic distances for each charged and discharged electrode state. On the basis of electrochemical data and the changes in atomic arrangement deduced from the EXAFS fitting results, including the first unambiguous observation of Sn-Li near neighbors, a capacity fading mechanism is proposed that is different from widely accepted volume expansion for tin metal and tin oxides. Our experimental results suggest that atomic clusters of metallic tin surrounded by highly disordered Li2O shells are formed on first charge. The metallic tin clusters participate in lithiation and delithiation on the following charge/discharge cycles; however, because of continued segregation of tin and Li2O phases, the tin clusters eventually lose electrical contact with the rest of the electrode and become excluded from further participation in electrochemical reactions, resulting in reduced capacity of this anode material. C1 [Pellicione, Christopher J.; Segre, Carlo U.] IIT, Dept Phys, Chicago, IL 60616 USA. [Pellicione, Christopher J.; Segre, Carlo U.] IIT, CSRRI, Chicago, IL 60616 USA. [Pellicione, Christopher J.; Timofeeva, Elena V.] Argonne Natl Lab, Div Energy Syst, Lemont, IL 60439 USA. RP Pellicione, CJ (reprint author), IIT, Dept Phys, 3300 South Fed St, Chicago, IL 60616 USA. EM cpellic1@hawk.iit.edu RI Segre, Carlo/B-1548-2009; BM, MRCAT/G-7576-2011; OI Segre, Carlo/0000-0001-7664-1574; Timofeeva, Elena V./0000-0001-7839-2727 FU Department of Education GAANN Fellowship [P200A090137]; National Science Foundation [DMR-086935]; U.S. Department of Energy, Office of Basic Energy Science; U.S. Department of Energy [DE-AC02-06CH113] FX C.J.P. was supported by a Department of Education GAANN Fellowship, award no. P200A090137, and the National Science Foundation under Grant no. DMR-086935. The project is supported by U.S. Department of Energy, Office of Basic Energy Science. MRCAT operations are supported by the Department of Energy and the MRCAT member institutions. Use of the Argonne National Laboratory Advanced Photon Source and Electron Microscopy Center is supported by the U.S. Department of Energy, under Contract no. DE-AC02-06CH113. NR 47 TC 7 Z9 7 U1 3 U2 42 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JAN 27 PY 2015 VL 27 IS 2 BP 574 EP 580 DI 10.1021/cm504101h PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CA0PD UT WOS:000348618400022 ER PT J AU Wong, DHC Vitale, A Devaux, D Taylor, A Pandya, AA Hallinan, DT Thelen, JL Mecham, SJ Lux, SF Lapides, AM Resnick, PR Meyer, TJ Kostecki, RM Balsara, NP DeSimone, JM AF Wong, Dominica H. C. Vitale, Alessandra Devaux, Didier Taylor, Austria Pandya, Ashish A. Hallinan, Daniel T. Thelen, Jacob L. Mecham, Sue J. Lux, Simon F. Lapides, Alexander M. Resnick, Paul R. Meyer, Thomas J. Kostecki, Robert M. Balsara, Nitash P. DeSimone, Joseph M. TI Phase Behavior and Electrochemical Characterization of Blends of Perfluoropolyether, Poly(ethylene glycol), and a Lithium Salt SO CHEMISTRY OF MATERIALS LA English DT Article ID POLYMER ELECTROLYTES; IONIC-CONDUCTIVITY; MOLECULAR-WEIGHT; BATTERIES; PEO; LIQUID; CHALLENGES; VISCOSITY; COMPLEX AB Electrolytes consisting of low molecular weight perfluoropolyether (PFPE), poly(ethylene glycol) (PEG), and lithium bis(trifluoromethanesulfonyl)imide (LiTFSI) blends were prepared and systematically studied for salt concentration and stoichiometry effects on the materials thermal and electrochemical properties. Herein we report that the tunable ratios of PFPE and PEG allow for precise control of crystalline melting and glass transition temperature properties. These blended liquid polymer electrolytes are inherently nonflammable and remain stable in the amorphous phase from approximately 150 degrees C down to -85 degrees C. The ionic conductivity of the electrolytes are on the order of 10(-4) S/cm at 30 degrees C, which makes them suitable for rechargeable lithium batteries. C1 [Wong, Dominica H. C.; Pandya, Ashish A.; Mecham, Sue J.; Lapides, Alexander M.; Meyer, Thomas J.; DeSimone, Joseph M.] Univ N Carolina, Dept Chem, Chapel Hill, NC 27599 USA. [Vitale, Alessandra] Politecn Torino, Dept Appl Sci & Technol, I-10129 Turin, Italy. [Devaux, Didier; Hallinan, Daniel T.; Lux, Simon F.; Kostecki, Robert M.; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Taylor, Austria] Winston Salem State Univ, Dept Chem, Winston Salem, NC 27110 USA. [Resnick, Paul R.] FluoroSci LLC, Alexandria, VA 22314 USA. [Thelen, Jacob L.; Balsara, Nitash P.] Univ Calif Berkeley, Dept Chem Engn, Berkeley, CA 94720 USA. [Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [DeSimone, Joseph M.] N Carolina State Univ, Dept Chem & Biomol Engn, Raleigh, NC 27695 USA. RP Balsara, NP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM nbalsara@berkeley.edu; desimone@unc.edu OI Vitale, Alessandra/0000-0002-8682-3125 FU Office of Naval Research [N00014-10-10550]; National Science Foundation [DMR-1122483]; Natural Sciences and Engineering Research Council of Canada; Consorzio INSTM; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001011]; Office of Vehicle Technologies of the US Department of Energy [DE-AC02-05CH11231] FX The work of D.H.C.W., A.A.P., and J.M.D. was funded by the Office of Naval Research (Grant N00014-10-10550 to J.M.D.) and the National Science Foundation (DMR-1122483). D.H.C.W. also is funded by the Natural Sciences and Engineering Research Council of Canada. The work of A.V. was funded by Consorzio INSTM. A portion of this work made use of electrochemical instrumentation in the University of North Carolina (UNC) Energy Frontier Research Center (EFRC) Instrumentation Facility established by the UNC EFRC: Center for Solar Fuels, funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Award DE-SC0001011. The work of J.L.T, D.D, S.L, R.M.K., and N.P.B. is funded by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the US Department of Energy under Contract DE-AC02-05CH11231 under the Batteries for Advanced Transportation Technologies Program. The authors would also like to thank Dr. Marc ter Horst for help with the NMR experiments. NR 39 TC 9 Z9 9 U1 9 U2 80 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JAN 27 PY 2015 VL 27 IS 2 BP 597 EP 603 DI 10.1021/cm504228a PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CA0PD UT WOS:000348618400025 ER PT J AU McGuire, MA Dixit, H Cooper, VR Sales, BC AF McGuire, Michael A. Dixit, Hemant Cooper, Valentino R. Sales, Brian C. TI Coupling of Crystal Structure and Magnetism in the Layered, Ferromagnetic Insulator CrI3 SO CHEMISTRY OF MATERIALS LA English DT Article ID TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; BASIS-SET; SEMICONDUCTORS; TRICHLORIDE; TRANSITION; RESONANCE; FIELD; CRCL3; MOS2 AB We have examined the crystallographic and magnetic properties of single crystals of CrI3, an easily cleavable, layered and insulating ferromagnet with a Curie temperature of 61 K. Our X-ray diffraction studies reveal a first-order crystallographic phase transition occurring near 210-220 K upon warming, with significant thermal hysteresis. The low-temperature structure is rhombohedral (R (3) over bar, BiI3-type) and the high-temperature structure is monoclinic (C-2/m, AlCl3-type). We find evidence for coupling between the crystallographic and magnetic degrees of freedom in CrI3, observing an anomaly in the interlayer spacing at the Curie temperature and an anomaly in the magnetic susceptibility at the structural transition. First-principles calculations reveal the importance of proper treatment of the long-ranged interlayer forces, and van der Waals density functional theory does an excellent job of predicting the crystal structures and their relative stability. Calculations also suggest that the ferromagnetic order found in the bulk material may persist into monolayer form, suggesting that CrI3 and other chromium trihalides may be promising materials for spintronic and magnetoelectronic research. C1 [McGuire, Michael A.; Dixit, Hemant; Cooper, Valentino R.; Sales, Brian C.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37830 USA. RP McGuire, MA (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37830 USA. EM mcguirema@ornl.gov RI McGuire, Michael/B-5453-2009; Cooper, Valentino /A-2070-2012 OI McGuire, Michael/0000-0003-1762-9406; Cooper, Valentino /0000-0001-6714-4410 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division FX The authors thank Radu Custelcean for assistance with the single-crystal data diffraction data collection and Jiaqiang Yan and Andrew May for helpful discussions. Research was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 44 TC 14 Z9 14 U1 25 U2 75 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JAN 27 PY 2015 VL 27 IS 2 BP 612 EP 620 DI 10.1021/cm504242t PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CA0PD UT WOS:000348618400027 ER PT J AU Sharma, K Kim, YH Gabitto, J Mayes, RT Yiacoumi, S Bilheux, HZ Walker, LMH Dai, S Tsouris, C AF Sharma, K. Kim, Y. -H. Gabitto, J. Mayes, R. T. Yiacoumi, S. Bilheux, H. Z. Walker, L. M. H. Dai, S. Tsouris, C. TI Transport of Ions in Mesoporous Carbon Electrodes during Capacitive Deionization of High-Salinity Solutions SO LANGMUIR LA English DT Article ID COMPOSITE FILM ELECTRODES; AQUEOUS-SOLUTIONS; DESALINATION EFFICIENCY; AEROGEL ELECTRODES; BRACKISH-WATER; ELECTROSORPTION; NANOTUBES; MEMBRANE; FLOW; NACL AB Desalination of high-salinity solutions has been studied using a novel experimental technique and a theoretical model. Neutron imaging has been employed to visualize lithium ions in mesoporous carbon materials, which are used as electrodes in capacitive deionization (CDI) for water desalination. Experiments were conducted with a flow-through CDI cell designed for neutron imaging and with lithium-6 chloride ((LiCl)-Li-6) as the electrolyte. Sequences of neutron images have been obtained at a relatively high concentration of (LiCl)-Li-6 solution to provide information on the transport of ions within the electrodes. A new model that computes the individual ionic concentration profiles inside mesoporous carbon electrodes has been used to simulate the CDI process. Modifications have also been introduced into the simulation model to calculate results at high electrolyte concentrations. Experimental data and simulation results provide insight into why CDI is not effective for desalination of high ionic-strength solutions. The combination of experimental information, obtained through neutron imaging, with the theoretical model will help in the design of CDI devices, which can improve the process for high ionic-strength solutions. C1 [Sharma, K.; Kim, Y. -H.; Yiacoumi, S.; Tsouris, C.] Georgia Inst Technol, Atlanta, GA 30332 USA. [Gabitto, J.] Prairie View A&M Univ, Prairie View, TX 77446 USA. [Mayes, R. T.; Bilheux, H. Z.; Walker, L. M. H.; Dai, S.; Tsouris, C.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Tsouris, C (reprint author), Georgia Inst Technol, Atlanta, GA 30332 USA. EM tsourisc@ornl.gov RI Dai, Sheng/K-8411-2015; Bilheux, Hassina/H-4289-2012; Tsouris, Costas/C-2544-2016; Mayes, Richard/G-1499-2016 OI Dai, Sheng/0000-0002-8046-3931; Bilheux, Hassina/0000-0001-8574-2449; Tsouris, Costas/0000-0002-0522-1027; Mayes, Richard/0000-0002-7457-3261 FU Laboratory Director's Research and Development Seed Program of ORNL; U.S. Department of Energy [DE-AC05-0096OR22725]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; National Science Foundation [CBET-0651683] FX This research was partially supported by the Laboratory Director's Research and Development Seed Program of ORNL. ORNL is managed by UT-Battelle, LLC, under Contract DE-AC05-0096OR22725 with the U.S. Department of Energy. A portion of this research at the Oak Ridge National Laboratory's High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Partial support to S.Y., K.S., and Y.-H.K. was provided by the National Science Foundation, under Grant No. CBET-0651683. The authors are thankful to Jean Bilheux for his help with the neutron image analysis. NR 46 TC 10 Z9 10 U1 15 U2 92 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD JAN 27 PY 2015 VL 31 IS 3 BP 1038 EP 1047 DI 10.1021/la5043102 PG 10 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CA1RQ UT WOS:000348689700020 PM 25533167 ER PT J AU Liu, WJ Tilley, TD AF Liu, Wenjun Tilley, T. Don TI Sterically Controlled Functionalization of Carbon Surfaces with -C6H4CH2X (X = OSO2Me or N-3) Groups for Surface Attachment of Redox-Active Molecules SO LANGMUIR LA English DT Article ID ARYL DIAZONIUM SALTS; COVALENT ATTACHMENT; ELECTROCHEMICAL REDUCTION; CONDUCTIVE DIAMOND; ELECTRON-TRANSFER; CLICK CHEMISTRY; ORBITAL METHODS; MONOLAYERS; DENSITY; FILMS AB Glassy carbon electrodes were modified by electrochemical reduction of a diazonium molecule ((Pr3SiOCH2C6H4N2+BF4-)-Pr-i) featuring a triisopropylsilyl-protected benzylic hydroxyl group. This electrochemical process introduced a monolayer of (Pr3SiOCH2C6H4)-Pr-i- groups onto the surface of the electrode. The bulky -SiiPr(3) protecting group not only prevents the uncontrolled growth of structurally ill-defined and electronically blocking polyphenylene multilayers, but also separates the phenyl groups in the monolayer. Thus, the void spaces between these aryl units should allow a better accommodation of sizable molecules. Removal of the -SiiPr(3) protecting groups by (Bu4NF)-Bu-n exposed the reactive benzylic hydroxyl functionalities that can undergo further transformations to anchor functional molecules. As an example, redox-active ferrocene molecules were grafted onto the modified electrode via a sequence of mesylation, azidation, and copper-catalyzed [3 + 2] cycloaddition reactions. The presence of ferrocenyl groups on the surface was confirmed by X-ray photoelectron spectroscopic and electrochemical studies. The resulting ferrocene-modified glassy carbon electrode exhibits cyclic voltammograms typical of surface-bound redox active species and remarkable electrochemical stability in an acidic aqueous environment. C1 [Liu, Wenjun; Tilley, T. Don] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. [Liu, Wenjun] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Tilley, T. Don] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Chem Sci Div, Berkeley, CA 94720 USA. [Tilley, T. Don] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Tilley, TD (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. EM tdiilley@berkeley.edu FU Office of Science of the U.S. Department of Energy [DE-SC0004993] FX This material is based upon work performed by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under Award Number DE-SC0004993. Dr. Mu-Jeng Cheng was acknowledged for his help on DFT calculations. NR 44 TC 8 Z9 8 U1 1 U2 34 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD JAN 27 PY 2015 VL 31 IS 3 BP 1189 EP 1195 DI 10.1021/la503796z PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CA1RQ UT WOS:000348689700038 PM 25549529 ER PT J AU Villaluenga, I Chen, XC Devaux, D Hallinan, DT Balsara, NP AF Villaluenga, Irune Chen, Xi Chelsea Devaux, Didier Hallinan, Daniel T. Balsara, Nitash P. TI Nanoparticle-Driven Assembly of Highly Conducting Hybrid Block Copolymer Electrolytes SO MACROMOLECULES LA English DT Article ID RECHARGEABLE LITHIUM BATTERIES; POLYMER ELECTROLYTES; IONIC-CONDUCTIVITY; MOLECULAR-WEIGHT; DIBLOCK COPOLYMERS; ORDER-DISORDER; PHASE; MORPHOLOGIES; DIFFUSION; ROUTE AB Hybrid nanostructured materials comprising block copolymers, nanoparticles, and lithium salts have the potential to serve as electrolytes in non-flammable rechargeable lithium batteries. Here we show that the addition of functionalized nanoparticles, at an optimized concentration, into lamellar block copolymer electrolytes, results in an increase in ionic conductivity. This is due to the occurrence of a lamellar-to-bicontinuous phase transition, driven by the addition of nanoparticles. The magnitude of the increase in conductivity is consistent with a simple model that accounts for the morphology of the conducting channels. The conductivity of the optimized hybrid electrolyte is only 6% lower than that of an idealized nanostructured electrolyte with perfectly connected conducting pathways and no dead ends. C1 [Villaluenga, Irune; Devaux, Didier; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Villaluenga, Irune; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, JCESR, Berkeley, CA 94720 USA. [Chen, Xi Chelsea; Balsara, Nitash P.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Hallinan, Daniel T.] Florida State Univ, Dept Chem & Biomed Engn, Tallahassee, FL 32310 USA. RP Balsara, NP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM nbalsara@berkeley.edu FU Joint Center for Energy Storage Research, an Energy Innovation Hub - U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES); DOE, Office of Science, BES; Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported as part of the Joint Center for Energy Storage Research, an Energy Innovation Hub funded by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES). X-ray scattering research at the Advanced Light Source was supported by DOE, Office of Science, BES. STEM work was provided by the Electron Microscopy of Soft Matter Program from the Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The STEM experiments were performed as user projects at the National Center for Electron Microscopy, Lawrence Berkeley National Laboratory, under the same contract. We acknowledge Eric Schaible for beamline support. We would also like to thank Jacob L. Thelen for helpful comments on small-angle X-ray scattering measurements. NR 27 TC 20 Z9 20 U1 7 U2 78 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD JAN 27 PY 2015 VL 48 IS 2 BP 358 EP 364 DI 10.1021/ma502234y PG 7 WC Polymer Science SC Polymer Science GA CA0PL UT WOS:000348619200007 ER PT J AU Aad, G Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Auerbach, B Augsten, K Aurousseau, M Avolio, G Axen, B Azuelos, G Azuma, Y Baak, MA Baas, AE Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Balek, P Balli, F Banas, E Banerjee, S Bannoura, AAE Bansil, HS Barak, L Baranov, SP Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Bartsch, V Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Battistin, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Becot, C Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, K Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bessidskaia, O Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boddy, CR Boehler, M Boek, TT Bogaerts, JA Bogdanchikov, AG Bogouch, A Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boterenbrood, H Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutouil, S Boveia, A Boyd, J Boyko, IR Bozic, I Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brelier, B Brendlinger, K Brennan, AJ Brenner, R Bressler, S Bristow, K Bristow, TM Britton, D Brochu, FM Brock, I Brock, R Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Brunet, S Bruni, A Bruni, G Bruschi, M Bryngemark, L Buanes, T Buat, Q Bucci, F Buchholz, P Buckley, AG Buda, SI Budagov, IA Buehrer, F Bugge, L Bugge, MK Bulekov, O Bundock, AC Burckhart, H Burdin, S Burghgrave, B Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Buszello, CP Butler, B Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Byszewski, M Urban, SC Caforio, D Cakir, O Calafiura, P Calandri, A Calderini, G Calfayan, P Caloba, LP Calvet, D Calvet, S Toro, RC Camarda, S Cameron, D Caminada, LM Armadans, RC Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Cardarelli, R Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Cattani, G Caudron, J Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, BC Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chang, P Chapleau, B Chapman, JD Charfeddine, D Charlton, DG Chau, CC Barajas, CAC Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A Cheremushkina, E El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiefari, G Childers, JT Chilingarov, A Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Chouridou, S Chow, BKB Chromek-Burckhart, D Chu, ML Chudoba, J Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Ciftci, R Cinca, D Cindro, V Ciocio, A Citron, ZH Citterio, M Ciubancan, M Clark, A Clark, PJ Clarke, RN Cleland, W Clemens, JC Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Cogan, JG Cole, B Cole, S Colijn, AP Collot, J Colombo, T Compostella, G Muino, PC Coniavitis, E Connell, SH Connelly, IA Consonni, SM Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cooper-Smith, NJ Copic, K Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cote, D Cottin, G Cowan, G Cox, BE Cranmer, K Cree, G Crepe-Renaudin, S Crescioli, F Cribbs, WA Ortuzar, MC Cristinziani, M Croft, V Crosetti, G Donszelmann, TC Cummings, J Curatolo, M Cuthbert, C Czirr, H Czodrowski, P D'Auria, S D'Onofrio, M De Sousa, MJDS Da Via, C Dabrowski, W Dafinca, A Dai, T Dale, O Dallaire, F Dallapiccola, C Dam, M Daniells, AC Danninger, M Hoffmann, MD Dao, V Darbo, G Darmora, S Dassoulas, J Dattagupta, A Davey, W David, C Davidek, T Davies, E Davies, M Davignon, O Davison, AR Davison, P Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Castro, S De Cecco, S De Groot, N de Jong, P De la Torre, H De Lorenzi, F De Nooij, L De Pedis, D De Salvo, A De Sanctis, U De Santo, A De Regie, JBD Dearnaley, WJ Debbe, R Debenedetti, C Dechenaux, B Dedovich, DV Deigaard, I Del Peso, J Del Prete, T Deliot, F Delitzsch, CM Deliyergiyev, M Dell'Acqua, A Dell'Asta, L Dell'Orso, M Della Pietra, M della Volpe, D Delmastro, M Delsart, PA Deluca, C DeMarco, DA Demers, S Demichev, M Demilly, A Denisov, SP Derendarz, D Derkaoui, JE Derue, F Dervan, P Desch, K Deterre, C Deviveiros, PO Dewhurst, A Dhaliwal, S Di Ciaccio, A Di Ciaccio, L Di Domenico, A Di Donato, C Di Girolamo, A Di Girolamo, B Di Mattia, A Di Micco, B Di Nardo, R Di Simone, A Di Sipio, R Di Valentino, D Dias, FA Diaz, MA Diehl, EB Dietrich, J Dietzsch, TA Diglio, S Dimitrievska, A Dingfelder, J Dita, P Dita, S Dittus, F Djama, F Djobava, T Djuvsland, JI do Vale, MAB Dobos, D Doglioni, C Doherty, T Dohmae, T Dolejsi, J Dolezal, Z Dolgoshein, BA Donadelli, M Donati, S Dondero, P Donini, J Dopke, J Doria, A Dova, MT Doyle, AT Dris, M Dubbert, J Dube, S Dubreuil, E Duchovni, E Duckeck, G Ducu, OA Duda, D Dudarev, A Dudziak, F Duflot, L Duguid, L Duhrssen, M Dunford, M Yildiz, HD Duren, M Durglishvili, A Duschinger, D Dwuznik, M Dyndal, M Edson, W Edwards, NC Ehrenfeld, W Eifert, T Eigen, G Einsweiler, K Ekelof, T El Kacimi, M Ellert, M Elles, S Ellinghaus, F Elliot, AA Ellis, N Elmsheuser, J Elsing, M Emeliyanov, D Enari, Y Endner, OC Endo, M Engelmann, R Erdmann, J Ereditato, A Eriksson, D Ernis, G Ernst, J Ernst, M Ernwein, J Errede, S Ertel, E Escalier, M Esch, H Escobar, C Esposito, B Etienvre, AI Etzion, E Evans, H Ezhilov, A Fabbri, L Facini, G Fakhrutdinov, RM Falciano, S Falla, RJ Faltova, J Fang, Y Fanti, M Farbin, A Farilla, A Farooque, T Farrell, S Farrington, SM Farthouat, P Fassi, F Fassnacht, P Fassouliotis, D Favareto, A Fayard, L Federic, P Fedin, OL Fedorko, W Feigl, S Feligioni, L Feng, C Feng, EJ Feng, H Fenyuk, AB Martinez, PF Perez, SF Ferrag, S Ferrando, J Ferrari, A Ferrari, P Ferrari, R de Lima, DEF Ferrer, A Ferrere, D Ferretti, C Parodi, AF Fiascaris, M Fiedler, F Filipcic, A Filipuzzi, M Filthaut, F Fincke-Keeler, M Finelli, KD Fiolhais, MCN Fiorini, L Firan, A Fischer, A Fischer, J Fisher, WC Fitzgerald, EA Flechl, M Fleck, I Fleischmann, P Fleischmann, S Fletcher, GT Fletcher, G Flick, T Floderus, A Castillo, LRF Flowerdew, MJ Formica, A Forti, A Fournier, D Fox, H Fracchia, S Francavilla, P Franchini, M Franchino, S Francis, D Franconi, L Franklin, M Fraternali, M French, ST Friedrich, C Friedrich, F Froidevaux, D Frost, JA Fukunaga, C Torregrosa, EF Fulsom, BG Fuster, J Gabaldon, C Gabizon, O Gabrielli, A Gabrielli, A Gadatsch, S Gadomski, S Gagliardi, G Gagnon, P Galea, C Galhardo, B Gallas, EJ Gallop, BJ Gallus, P Galster, G Gan, KK Gao, J Gao, YS Walls, FMG Garberson, F Garcia, C Navarro, JEG Garcia-Sciveres, M Gardner, RW Garelli, N Garonne, V Gatti, C Gaudio, G Gaur, B Gauthier, L Gauzzi, P Gavrilenko, IL Gay, C Gaycken, G Gazis, EN Ge, P Gecse, Z Gee, CNP Geerts, DAA 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CA ATLAS Collaboration TI Search for new phenomena in events with a photon and missing transverse momentum in pp collisions at root s = 8 TeV with the ATLAS detector SO PHYSICAL REVIEW D LA English DT Article ID E(+)E(-) COLLISIONS; DARK-MATTER; SUPERGAUGE TRANSFORMATIONS; FIELD THEORY; ENERGY; MODEL; CONSTRAINTS; DIMENSIONS; PARTICLE; SQUARK AB Results of a search for new phenomena in events with an energetic photon and large missing transverse momentum with the ATLAS experiment at the LHC are reported. Data were collected in proton-proton collisions at a center-of-mass energy of 8 TeVand correspond to an integrated luminosity of 20.3 fb(-1). The observed data are well described by the expected Standard Model backgrounds. The expected (observed) upper limit on the fiducial cross section for the production of events with a photon and large missing transverse momentum is 6.1 (5.3) fb at 95% confidence level. 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[Anjos, N.; Bosman, M.; Armadans, R. Caminal; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fracchia, S.; Giangiobbe, V.; Gonzalez Parra, G.; Grinstein, S.; Rozas, A. Juste; Korolkov, I.; Le Menedeu, E.; Paz, I. Lopez; Martinez, M.; Mir, L. M.; Berlingen, J. Montejo; Pages, A. Pacheco; Aranda, C. Padilla; Rubbo, F.; Sorin, V.; Succurro, A.; Tripiana, M. F.; Tsiskaridze, S.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Anjos, N.; Bosman, M.; Armadans, R. Caminal; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fracchia, S.; Giangiobbe, V.; Gonzalez Parra, G.; Grinstein, S.; Rozas, A. Juste; Korolkov, I.; Le Menedeu, E.; Paz, I. Lopez; Martinez, M.; Mir, L. M.; Berlingen, J. Montejo; Pages, A. Pacheco; Aranda, C. Padilla; Riu, I.; Rubbo, F.; Sorin, V.; Succurro, A.; Tripiana, M. F.; Tsiskaridze, S.] Univ Autonoma Barcelona, Dept Fis, E-08193 Barcelona, Spain. [Agatonovic-Jovin, T.; Bozic, I.; Dimitrievska, A.; Krstic, J.; Marjanovic, M.; Popovic, D. S.; Sijacki, Dj.; Simic, Lj.; Milosavljevic, M. Vranjes] Univ Belgrade, Inst Phys, Belgrade, Serbia. [Mamuzic, J.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Buanes, T.; Dale, O.; Eigen, G.; Kastanas, A.; Liebig, W.; Lipniacka, A.; Latour, B. Martin Dit; Rosendahl, P. L.; Sandaker, H.; Sjursen, T. B.; Smestad, L.; Stugu, B.; Ugland, M.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Axen, B.; Barnett, R. M.; Beringer, J.; Brandt, G.; Brosamer, J.; Calafiura, P.; Caminada, L. M.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Dube, S.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Holmes, T. R.; Hurwitz, M.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Virzi, J.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Axen, B.; Barnett, R. M.; Beringer, J.; Brandt, G.; Brosamer, J.; Calafiura, P.; Caminada, L. M.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Dube, S.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Holmes, T. R.; Hurwitz, M.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Virzi, J.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Dietrich, J.; Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Herrberg-Schubert, R.; Hristova, I.; Kind, O.; Kolanoski, H.; Lacker, H.; Lohse, T.; Nikiforou, N.; Nikiforov, A.; Rehnisch, L.; Rieck, P.; Stamm, S.; Wendland, D.; zur Nedden, M.] Humboldt Univ, Dept Phys, D-10099 Berlin, Germany. [Agustoni, M.; Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Schneider, B.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Agustoni, M.; Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Schneider, B.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allbrooke, B. M. M.; Bella, L. Aperio; Bansil, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Palmer, J. D.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Alberghi, G. L.; Bellagamba, L.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Caforio, D.; Corradi, M.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, Bologna, Italy. [Alberghi, G. L.; Caforio, D.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Hageboeck, S.; Hellmich, D.; Huegging, F.; Janssen, J.; Khoriauli, G.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lenz, T.; Leyko, A. M.; Limbach, C.; Mergelmeyer, S.; Mijovic, L.; Mueller, K.; Nanava, G.; Nattermann, T.; Obermann, T.; Pohl, D.; Sarrazin, B.; Schaepe, S.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Seema, P.; Stillings, J. A.; Tannoury, N.; Therhaag, J.; Uhlenbrock, M.; Velz, T.; Vogel, A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Fitzgerald, E. A.; Sciolla, G.; Venturini, A.; Zambito, S.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Univ Fed Juiz de Fora, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Schovancova, J.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Ducu, O. A.; Jinaru, A.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; Marchand, J. F.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Battistin, M.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Franchino, S.; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jakobsen, S.; Jenni, P.; Kaneda, M.; Klioutchnikova, T.; Krasnopevtsev, D.; Krasznahorkay, A.; Lantzsch, K.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Martin, B.; Marzin, A.; Messina, A.; Meyer, J.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Schaefer, D.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Cheng, Y.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Krizka, K.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Tompkins, L.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Lu, F.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Jiang, Y.; Li, B.; Liu, B.; Liu, J. B.; Liu, M.; Peng, H.; Song, H. Y.; Xu, L.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.; Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Podlyski, F.; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Podlyski, F.; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Podlyski, F.; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Guo, J.; Hu, D.; Hughes, E. W.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, Cosenza, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Wang, H.; Ye, J.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Camarda, S.; Deterre, C.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Gomez Fajardo, L. S.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Moenig, K.; Morton, A.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Camarda, S.; Deterre, C.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Gomez Fajardo, L. S.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Moenig, K.; Morton, A.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Wang, C.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dao, V.; Di Simone, A.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Madar, R.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ronzani, M.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Vu Anh, T.; Warsinsky, M.; Weiser, C.; Zimmermann, S.] Univ Freiburg, Fak Mathemat & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; Bilbao De Mendizabal, J.; Bucci, F.; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Picazio, A.; Pohl, M.; Rosbach, K.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jezelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, High Energy Phys Inst, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. 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J. Alconada; Alonso, F.; Anduaga, X. S.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Orlando, N.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dassoulas, J.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Readioff, N. P.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. 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W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. 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G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Thompson, R. J.; Tomlinson, L.; Watts, G.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. 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E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. 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G.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Merola, L.; Patricelli, S.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Konig, A. C.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Kharlamov, A.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Beacham, J. B.; Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, K.; Boddy, C. R.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pachal, K.; Pickering, M. A.; Pinder, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Lester, C. M.; Lipeles, E.; Meyer, C.; Ospanov, R.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Mueller, J.; Prieur, D.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; Sargedas De Sousa, M. J. Da Cunha; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; Sargedas De Sousa, M. J. Da Cunha; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Nova Lisboa, Fac Ciencias & Tecnol, Dept Fis, Caparica, Portugal. [Aguilar-Saavedra, J. A.] Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Stanescu, C.; Taccini, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Taccini, C.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Firmino Da Costa, J. Goncalves Pinto; Guyot, C.; Hanna, R.; Hassani, S.; Kozanecki, W.; Laporte, J. F.; Maiani, C.; Mal, P.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Protopopescu, S.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay, Commissariat Energie Atom & Energies Alternat, DSM IRFU, Inst Recherches Lois Fondament Univers, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Hernandez, D. Paredes; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, S.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; Horton, A. J.; O'Neil, D. C.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nef, P. D.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Lee, C. A.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Carrillo-Montoya, G. D.; Hamity, G. N.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bessidskaia, O.; Clement, C.; Cribbs, W. A.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bessidskaia, O.; Clement, C.; Cribbs, W. A.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Asquith, L.; Bartsch, V.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Potter, C. T.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Aguilar-Saavedra, J. A.; Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Patel, N. D.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Ren, Z. L.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei 115, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. 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[Jezelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys, Dolgoprudnyi, Russia. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Technol State Univ, Dolgoprudnyi, Russia. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Wildt, M. A.] Univ Hamburg, Inst Experimentalphys, Hamburg, Germany. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Tartarelli, Giuseppe Francesco/A-5629-2016; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Gutierrez, Phillip/C-1161-2011; Gerbaudo, Davide/J-4536-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Martinez, Mario /I-3549-2015; Peleganchuk, Sergey/J-6722-2014; Zhou, Ning/D-1123-2017; Monzani, Simone/D-6328-2017; Garcia, Jose /H-6339-2015; Korol, Aleksandr/A-6244-2014; Capua, Marcella/A-8549-2015; Smirnova, Oxana/A-4401-2013; Livan, Michele/D-7531-2012; Villa, Mauro/C-9883-2009; White, Ryan/E-2979-2015; Joergensen, Morten/E-6847-2015; Brooks, William/C-8636-2013; Di Domenico, Antonio/G-6301-2011; Connell, Simon/F-2962-2015; Bosman, Martine/J-9917-2014; Boyko, Igor/J-3659-2013; Mitsou, Vasiliki/D-1967-2009; Carquin, Edson/G-5221-2015; Riu, Imma/L-7385-2014; Mir, Lluisa-Maria/G-7212-2015; Cavalli-Sforza, Matteo/H-7102-2015; Marti-Garcia, Salvador/F-3085-2011; Vos, Marcel/G-8123-2015; Della Pietra, Massimo/J-5008-2012; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Grancagnolo, Sergio/J-3957-2015; Doyle, Anthony/C-5889-2009; spagnolo, stefania/A-6359-2012; Tassi, Enrico/K-3958-2015; Ciubancan, Liviu Mihai/L-2412-2015; Zhukov, Konstantin/M-6027-2015; Shmeleva, Alevtina/M-6199-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; De, Kaushik/N-1953-2013; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Snesarev, Andrey/H-5090-2013; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; BESSON, NATHALIE/L-6250-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Staroba, Pavel/G-8850-2014; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Mindur, Bartosz/A-2253-2017; Fabbri, Laura/H-3442-2012 OI Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Giorgi, Filippo Maria/0000-0003-1589-2163; Coccaro, Andrea/0000-0003-2368-4559; Castro, Nuno/0000-0001-8491-4376; Veneziano, Stefano/0000-0002-2598-2659; Price, Darren/0000-0003-2750-9977; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Monzani, Simone/0000-0002-0479-2207; Korol, Aleksandr/0000-0001-8448-218X; Giordani, Mario/0000-0002-0792-6039; Capua, Marcella/0000-0002-2443-6525; Smirnova, Oxana/0000-0003-2517-531X; Livan, Michele/0000-0002-5877-0062; Villa, Mauro/0000-0002-9181-8048; White, Ryan/0000-0003-3589-5900; Joergensen, Morten/0000-0002-6790-9361; Brooks, William/0000-0001-6161-3570; Di Domenico, Antonio/0000-0001-8078-2759; Connell, Simon/0000-0001-6000-7245; Bosman, Martine/0000-0002-7290-643X; Boyko, Igor/0000-0002-3355-4662; Mitsou, Vasiliki/0000-0002-1533-8886; Carquin, Edson/0000-0002-7863-1166; Riu, Imma/0000-0002-3742-4582; Mir, Lluisa-Maria/0000-0002-4276-715X; Vos, Marcel/0000-0001-8474-5357; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Grancagnolo, Sergio/0000-0001-8490-8304; Doyle, Anthony/0000-0001-6322-6195; spagnolo, stefania/0000-0001-7482-6348; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Tikhomirov, Vladimir/0000-0002-9634-0581; Warburton, Andreas/0000-0002-2298-7315; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; De, Kaushik/0000-0002-5647-4489; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353 FU ANPCyT, Argentina FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC, and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST, and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR, and VSC CR, Czech Republic; DNRF, DNSRC, and Lundbeck Foundation, Denmark; EPLANET, ERC, and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG, and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, I-CORE, and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF, and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society, and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK), and BNL (USA) and in the Tier-2 facilities worldwide. NR 86 TC 19 Z9 19 U1 13 U2 80 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JAN 27 PY 2015 VL 91 IS 1 AR 012008 DI 10.1103/PhysRevD.91.012008 PG 25 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CA3WI UT WOS:000348834800001 ER PT J AU Kang, ZB Ma, YQ Qiu, JW Sterman, G AF Kang, Zhong-Bo Ma, Yan-Qing Qiu, Jian-Wei Sterman, George TI Heavy quarkonium production at collider energies: Partonic cross section and polarization SO PHYSICAL REVIEW D LA English DT Article ID QCD; ANNIHILATION AB We calculate the O(alpha(3)(s)) short-distance, QCD collinear-factorized coefficient functions for all partonic channels that include the production of a heavy quark pair at short distances. This provides the first power correction to the collinear-factorized inclusive hadronic production of heavy quarkonia at large transverse momentum, pT, including the full leading-order perturbative contributions to the production of heavy quark pairs in all color and spin states employed in NRQCD treatments of this process. We discuss the role of the first power correction in the production rates and the polarizations of heavy quarkonia in high-energy hadronic collisions. The consistency of QCD collinear factorization and nonrelativistic QCD factorization applied to heavy quarkonium production is also discussed. C1 [Kang, Zhong-Bo] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Ma, Yan-Qing] Univ Maryland, Maryland Ctr Fundamental Phys, College Pk, MD 20742 USA. [Ma, Yan-Qing] Peking Univ, Ctr High Energy Phys, Beijing 100871, Peoples R China. [Qiu, Jian-Wei] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Qiu, Jian-Wei; Sterman, George] SUNY Stony Brook, CN Yang Inst Theoret Phys, Stony Brook, NY 11794 USA. [Qiu, Jian-Wei; Sterman, George] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. RP Kang, ZB (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM zkang@lanl.gov; yqma@bnl.gov; jqiu@bnl.gov; sterman@insti.physics.sunysb.edu RI Kang, Zhongbo/P-3645-2014 FU U.S. Department of Energy [DE-AC02-06NA25396, DE-AC02-98CH10886, DE-FG02-93ER-40762]; National Science Foundation [PHY-0969739, PHY-1316617] FX We thank G. T. Bodwin, E. Braaten, and H. Zhang for helpful discussions. This work was supported in part by the U.S. Department of Energy under Contracts No. DE-AC02-06NA25396 and No. DE-AC02-98CH10886, and Grant No. DE-FG02-93ER-40762, and the National Science Foundation under Grants No. PHY-0969739 and No. PHY-1316617. NR 47 TC 8 Z9 8 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JAN 27 PY 2015 VL 91 IS 1 AR 014030 DI 10.1103/PhysRevD.91.014030 PG 25 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CA3WI UT WOS:000348834800003 ER PT J AU Jeong, J Aetukuri, NB Passarello, D Conradson, SD Samant, MG Parkin, SSP AF Jeong, Jaewoo Aetukuri, Nagaphani B. Passarello, Donata Conradson, Steven D. Samant, Mahesh G. Parkin, Stuart S. P. TI Giant reversible, facet-dependent, structural changes in a correlated-electron insulator induced by ionic liquid gating SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE electrolyte gating; correlated oxides; EXAFS; metal-insulator transition; vanadium dioxide ID TRANSITION; VO2; SURFACE AB The use of electric fields to alter the conductivity of correlated electron oxides is a powerful tool to probe their fundamental nature as well as for the possibility of developing novel electronic devices. Vanadium dioxide (VO2) is an archetypical correlated electron system that displays a temperature-controlled insulating to metal phase transition near room temperature. Recently, ionic liquid gating, which allows for very high electric fields, has been shown to induce a metallic state to low temperatures in the insulating phase of epitaxially grown thin films of VO2. Surprisingly, the entire film becomes electrically conducting. Here, we show, from in situ synchrotron X-ray diffraction and absorption experiments, that the whole film undergoes giant, structural changes on gating in which the lattice expands by up to similar to 3% near room temperature, in contrast to the 10 times smaller (similar to 0.3%) contraction when the system is thermally metallized. Remarkably, these structural changes are fully reversible on reverse gating. Moreover, we find these structural changes and the concomitant metallization are highly dependent on the VO2 crystal facet, which we relate to the ease of electric-field-induced motion of oxygen ions along chains of edge-sharing VO6 octahedra that exist along the (rutile) c axis. C1 [Jeong, Jaewoo; Aetukuri, Nagaphani B.; Passarello, Donata; Samant, Mahesh G.; Parkin, Stuart S. P.] Int Business Machines Almaden Res Ctr, San Jose, CA 95120 USA. [Passarello, Donata] Univ Kaiserslautern, Grad Sch Excellence Mat Sci Mainz, D-67663 Kaiserslautern, Germany. [Conradson, Steven D.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. [Parkin, Stuart S. P.] Max Planck Inst Microstruct Phys, D-06120 Halle, Germany. RP Parkin, SSP (reprint author), Int Business Machines Almaden Res Ctr, San Jose, CA 95120 USA. EM Stuart.Parkin@icloud.com FU Graduate School "Material Science in Mainz" (Deutsche Forschungsgemeinschaft) [GSC 266]; Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, DOE, under the Heavy Element Chemistry Program; Laboratory Directed Research and Development program at Los Alamos National Laboratory FX We thank Prof. Juana Acrivos for discussions and encouragement. Support for D. P. from the Graduate School "Material Science in Mainz" (Deutsche Forschungsgemeinschaft, GSC 266) is gratefully acknowledged. Portions of this research were carried out at the Stanford Synchrotron Radiation Lightsource, a Directorate of Standford Linear Accelerator Center National Accelerator Laboratory and an Office of Science User Facility operated for the US Department of Energy (DOE) Office of Science by Stanford University. S. D. C. is supported by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, DOE, under the Heavy Element Chemistry Program and the Laboratory Directed Research and Development program at Los Alamos National Laboratory. NR 24 TC 22 Z9 22 U1 5 U2 64 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JAN 27 PY 2015 VL 112 IS 4 BP 1013 EP 1018 DI 10.1073/pnas.1419051112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AZ7SB UT WOS:000348417000030 PM 25583517 ER PT J AU Wray, LA Huang, SW Xia, YQ Hasan, MZ Mathy, C Eisaki, H Hussain, Z Chuang, YD AF Wray, L. Andrew Huang, Shih-Wen Xia, Yuqi Hasan, M. Zahid Mathy, Charles Eisaki, Hiroshi Hussain, Zahid Chuang, Yi-De TI Experimental signatures of phase interference and subfemtosecond time dynamics on the incident energy axis of resonant inelastic x-ray scattering SO PHYSICAL REVIEW B LA English DT Article ID ONE-DIMENSIONAL SRCUO2; ELECTRONIC-STRUCTURE; EXCITATIONS; NIO; PHOTOEMISSION; EMISSION AB Core hole resonance is used in x-ray spectroscopy to incisively probe the local electronic states of many-body systems. Here, resonant inelastic x-ray scattering (RIXS) is studied as a function of incident photon energy on Mott insulators SrCuO2 and NiO to examine how resonance states decay into different excitation symmetries at the transition-metal M, L, and K edges. Quantum interference patterns characteristic of the two major RIXS mechanisms are identified within the data, and used to distinguish the attosecond scale scattering dynamics by which fundamental excitations of a many-body system are created. A function is proposed to experimentally evaluate whether a particular excitation has constructive or destructive interference in the RIXS cross section, and corroborates other evidence that an anomalous excitation is present at the leading edge of the Mott gap in quasi-one-dimensional SrCuO2. C1 [Wray, L. Andrew] NYU, Dept Phys, New York, NY 10003 USA. [Huang, Shih-Wen; Hussain, Zahid; Chuang, Yi-De] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Xia, Yuqi; Hasan, M. Zahid] Princeton Univ, Dept Phys, Joseph Henry Labs, Princeton, NJ 08544 USA. [Mathy, Charles] Harvard Smithsonian Ctr Astrophys, ITAMP, Cambridge, MA 02138 USA. [Eisaki, Hiroshi] Natl Inst Adv Ind Sci & Technol, Nanoelect Res Inst, Tsukuba, Ibaraki 3058568, Japan. RP Wray, LA (reprint author), NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. EM lawray@nyu.edu FU US DOE/BES Grant [DE-FG02-05ER46200]; Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231]; Argonne National Laboratory [DE-AC02-06CH11357] FX We are grateful for discussions with K. Wohlfeld, B. Moritz, T. Devereaux, K. Ishii, I. Jarrige, R. Eder, D.-H. Lee, S. Roy, and P. Shafer. M. Z. H. was supported by US DOE/BES Grant No. DE-FG02-05ER46200. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract No. DE-AC02-05CH11231. This research used resources of the Advanced Photon Source, a US Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 37 TC 3 Z9 3 U1 3 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JAN 27 PY 2015 VL 91 IS 3 AR 035131 DI 10.1103/PhysRevB.91.035131 PG 11 WC Physics, Condensed Matter SC Physics GA CA3WF UT WOS:000348834400001 ER PT J AU Baxevanis, P Huang, ZR Ruth, R Schroeder, CB AF Baxevanis, Panagiotis Huang, Zhirong Ruth, Ronald Schroeder, Carl B. TI Eigenmode analysis of a high-gain free-electron laser based on a transverse gradient undulator SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article ID AMPLIFIED SPONTANEOUS EMISSION; INITIAL-VALUE PROBLEM; OUTPUT POWER; COHERENCE; ENERGY AB The use of a transverse gradient undulator (TGU) is viewed as an attractive option for free-electron lasers (FELs) driven by beams with a large energy spread. By suitably dispersing the electron beam and tilting the undulator poles, the energy spread effect can be substantially mitigated. However, adding the dispersion typically leads to electron beams with large aspect ratios. As a result, the presence of higher-order modes in the FEL radiation can become significant. To investigate this effect, we study the eigenmode properties of a TGU-based, high-gain FEL, using both an analytically-solvable model and a variational technique. Our analysis, which includes the fundamental and the higher-order FEL eigenmodes, can provide an estimate of the mode content for the output radiation. This formalism also enables us to study the trade-off between FEL gain and transverse coherence. Numerical results are presented for a representative soft X-ray, TGU FEL example. C1 [Baxevanis, Panagiotis; Huang, Zhirong; Ruth, Ronald] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Schroeder, Carl B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Baxevanis, P (reprint author), SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. OI Schroeder, Carl/0000-0002-9610-0166 FU Office of Science, of the U.S. Department of Energy [DE-AC02-76SF00515, DE-AC02-05CH11231] FX This work was supported by the Director, Office of Science, of the U.S. Department of Energy under Contracts No. DE-AC02-76SF00515 and No. DE-AC02-05CH11231. NR 17 TC 5 Z9 5 U1 1 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD JAN 27 PY 2015 VL 18 IS 1 AR 010701 DI 10.1103/PhysRevSTAB.18.010701 PG 10 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA CA3WN UT WOS:000348835400001 ER PT J AU Walton, SK Zeissler, K Burn, DM Ladak, S Read, DE Tyliszczak, T Cohen, LF Branford, WR AF Walton, S. K. Zeissler, K. Burn, D. M. Ladak, S. Read, D. E. Tyliszczak, T. Cohen, L. F. Branford, W. R. TI Limitations in artificial spin ice path selectivity: the challenges beyond topological control SO NEW JOURNAL OF PHYSICS LA English DT Article DE artificial spin ice; domain wall; chirality; topology; vortex ID DOMAIN-WALLS; MAGNETIC MONOPOLES; PHASE-DIAGRAM; MANIPULATION; NANOWIRES; DYNAMICS; DEFECTS; SYSTEM; STRIPS AB Magnetic charge is carried through nanowire networks by domain walls, and the micromagnetic structure of a domain wall provides an opportunity to manipulate its movement. We have shown previously that magnetic monopole defects exist in artificial spin ice (ASI) and result from two bar switching at a vertex. To create and manipulate monopole defects and indeed magnetic charge in general, path selectivity of the domain wall at a vertex is required. We have recently shown that in connected ASI structures, transverse wall chirality (or topology) determines wall path direction, but a mechanism known as Walker breakdown, where a wall mutates into a wall of opposite chirality partially destroys selectivity. Recently it has been claimed that in isolated Y-shaped junctions that support vortex walls, selectivity is entirely determined by chirality (or topology), the suggestion being that vortex wall chirality is robust in the Walker breakdown process. Here we demonstrate that in Y-shaped junctions, magnetic switching in the important topologically protected regime exists only for a narrow window of field and bar geometry, and that it will be challenging to access this regime in field-driven ASI. This work has implications for the wider field of magnetic charge manipulation for high density memory storage. C1 [Walton, S. K.; Zeissler, K.; Burn, D. M.; Cohen, L. F.; Branford, W. R.] Univ London Imperial Coll Sci Technol & Med, Dept Phys, Blackett Lab, London SW7 2AZ, England. [Ladak, S.; Read, D. E.] Cardiff Univ, Sch Phys & Astron, Cardiff CF24 3AA, S Glam, Wales. [Tyliszczak, T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Walton, SK (reprint author), Univ London Imperial Coll Sci Technol & Med, Dept Phys, Blackett Lab, Prince Consort Rd, London SW7 2AZ, England. EM W.branford@imperial.ac.uk RI Read, Dan/G-5115-2011; OI Read, Dan/0000-0002-4178-4986; Ladak, Sam/0000-0002-0275-0927; Burn, David/0000-0001-7540-1616 FU Leverhulme Trust [RPG_2012-692]; UK EPSRC [ED/G004765/1]; Office of Science, Office of Basic Energy Sciences of the US Department of Energy [DE-AC02-05CH11231] FX WB acknowledges Leverhulme Trust: RPG_2012-692 and UK EPSRC grant ED/G004765/1 for funding. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences of the US Department of Energy under contract no. DE-AC02-05CH11231. NR 43 TC 8 Z9 8 U1 3 U2 37 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD JAN 27 PY 2015 VL 17 AR 013054 DI 10.1088/1367-2630/17/1/013054 PG 9 WC Physics, Multidisciplinary SC Physics GA CA2TJ UT WOS:000348760300009 ER PT J AU Strelcov, E Kumar, R Bocharova, V Sumpter, BG Tselev, A Kalinin, SV AF Strelcov, Evgheni Kumar, Rajeev Bocharova, Vera Sumpter, Bobby G. Tselev, Alexander Kalinin, Sergei V. TI Nanoscale Lubrication of Ionic Surfaces Controlled via a Strong Electric Field SO SCIENTIFIC REPORTS LA English DT Article ID ATOMIC-FORCE MICROSCOPY; SCANNING ELECTROCHEMICAL MICROSCOPE; SINGLE-CRYSTAL ELECTRODES; AQUEOUS-SOLUTIONS; WATER; FRICTION; DISSOLUTION; NANOTRIBOLOGY; CALIBRATION AB Frictional forces arise whenever objects around us are set in motion. Controlling them in a rational manner means gaining leverage over mechanical energy losses and wear. This paper presents a way of manipulating nanoscale friction by means of in situ lubrication and interfacial electrochemistry. Water lubricant is directionally condensed from the vapor phase at a moving metal-ionic crystal interface by a strong confined electric field, thereby allowing friction to be tuned up or down via an applied bias. The electric potential polarity and ionic solid solubility are shown to strongly influence friction between the atomic force microscope (AFM) tip and salt surface. An increase in friction is associated with the AFM tip digging into the surface, whereas reducing friction does not influence its topography. No current flows during friction variation, which excludes Joule heating and associated electrical energy losses. The demonstrated novel effect can be of significant technological importance for controlling friction in nano- and micro-electromechanical systems. C1 [Strelcov, Evgheni; Kumar, Rajeev; Sumpter, Bobby G.; Tselev, Alexander; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Kumar, Rajeev; Sumpter, Bobby G.] Oak Ridge Natl Lab, Div Math & Comp Sci, Oak Ridge, TN 37831 USA. [Bocharova, Vera] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Strelcov, E (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM strelcove@ornl.gov RI Strelcov, Evgheni/H-1654-2013; Tselev, Alexander/L-8579-2015; Sumpter, Bobby/C-9459-2013; Kumar, Rajeev/Q-2255-2015; Kalinin, Sergei/I-9096-2012 OI Tselev, Alexander/0000-0002-0098-6696; Sumpter, Bobby/0000-0001-6341-0355; Kumar, Rajeev/0000-0001-9494-3488; Kalinin, Sergei/0000-0001-5354-6152 FU Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Laboratory Directed Research and Development Program of Oak Ridge National Laboratory FX This research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. VB would like to acknowledge sponsorship by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U. S. Department of Energy. ES and SVK would like to thank Dr. P. Collier for fruitful discussion. ES gratefully acknowledges Mr. A. Strelkov for his help in illustrating this manuscript. NR 27 TC 5 Z9 5 U1 4 U2 48 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 27 PY 2015 VL 5 AR 8049 DI 10.1038/srep08049 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AZ6SQ UT WOS:000348350500001 PM 25623295 ER PT J AU Salloum, M James, SC Robinson, DB AF Salloum, Maher James, Scott C. Robinson, David B. TI Effects of surface thermodynamics on hydrogen isotope exchange kinetics in palladium: Particle and flow models SO CHEMICAL ENGINEERING SCIENCE LA English DT Article DE Adsorption; Hydride; Activation Barrier; Chromatography; Pressure Drop; Isotope Exchange ID GASEOUS-HYDROGEN; HYDRIDE POWDER; SEPARATION; ADSORPTION; DIFFUSION; SYSTEM; CHROMATOGRAPHY; MEMBRANES; ALLOYS; BED AB Palladium is an important material for separation of hydrogen from other gases, separation of hydrogen isotopes, and for hydrogen storage. Its main advantages are its high selectivity and rapid, highly reversible uptake and release of hydrogen at near ambient temperatures and pressures. Toward a more comprehensive understanding of its behavior, we present particle and continuum multiphysics mathematical models of the coupled reactive transport of hydrogen isotopes in the context of a single palladium sphere, and of flow in a packed palladium hydride bed. The models consider rates of chemical reactions and mass transport within a hydride bed, and incorporate a multistep reaction mechanism involving the metal bulk, metal surface, and gas phases. A unique feature in this formulation is that the chemical reaction model accounts for all absorption, adsorption, and diffusion activation energies. In particular, the adsorption energy is believed to depend strongly on the composition and atom-scale structure of the surface. We perform a parametric study to evaluate the effects of temperature, surface adsorption energy, and hydride particle radius on the isotope exchange kinetics. The models are useful in designing optimal hydride beds operating at various temperatures, with varied hydride particle size, and surface conditions. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Salloum, Maher; James, Scott C.; Robinson, David B.] Sandia Natl Labs, Livermore, CA 94550 USA. RP Salloum, M (reprint author), Sandia Natl Labs, 7011 East Ave,MS 9158, Livermore, CA 94550 USA. EM mnsallo@sandia.gov OI James, Scott/0000-0001-7955-0491 FU Laboratory Directed Research and Development program at Sandia National Laboratories, a multiprogram laboratory; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the Laboratory Directed Research and Development program at Sandia National Laboratories, a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 38 TC 1 Z9 2 U1 2 U2 37 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0009-2509 EI 1873-4405 J9 CHEM ENG SCI JI Chem. Eng. Sci. PD JAN 27 PY 2015 VL 122 BP 474 EP 490 DI 10.1016/j.ces.2014.09.001 PG 17 WC Engineering, Chemical SC Engineering GA AW1SE UT WOS:000346069300044 ER PT J AU Joseph, AI Lapidus, SH Kane, CM Holman, KT AF Joseph, Akil I. Lapidus, Saul H. Kane, Christopher M. Holman, K. Travis TI Extreme Confinement of Xenon by Cryptophane-111 in the Solid State SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE container molecules; cryptophanes; gas storage; microporous materials; xenon ID WATER-SOLUBLE CRYPTOPHANE-111; METAL-ORGANIC FRAMEWORK; NOBLE-GAS ADSORPTION; HYPERPOLARIZED XENON; MOLECULAR RECOGNITION; XE-129 NMR; CRYSTAL; HOST; COMPLEXES; SEPARATION AB Solids that sorb, capture and/or store the heavier noble gases are of interest because of their potential for transformative rare gas separation/production, storage, or recovery technologies. Herein, we report the isolation, crystal structures, and thermal stabilities of a series of xenon and krypton clathrates of (+/-)-cryptophane-111 (111). One trigonal crystal form, Xe@111 center dot y(solvent), is exceptionally stable, retaining xenon at temperatures of up to about 300 degrees C. The high kinetic stability is attributable not only to the high xenon affinity and cage-like nature of the host, but also to the crystal packing of the clathrate, wherein each window of the molecular container is blocked by the bridges of adjacent containers, effectively imprisoning the noble gas in the solid state. The results highlight the potential of discrete molecule materials exhibiting intrinsic microcavities or zero-dimensional pores. C1 [Joseph, Akil I.; Kane, Christopher M.; Holman, K. Travis] Georgetown Univ, Dept Chem, Washington, DC 20057 USA. [Lapidus, Saul H.] Argonne Natl Lab, Xray Sci Div, Lemont, IL 60439 USA. RP Holman, KT (reprint author), Georgetown Univ, Dept Chem, Washington, DC 20057 USA. EM kth7@georgetown.edu OI Holman, Kevin Travis/0000-0003-1800-300X FU U.S. National Science Foundation (NSF) [DMR-1106266, CHE-1337975]; IMI Program of the NSF [DMR 0843934]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work was supported by the U.S. National Science Foundation (NSF; DMR-1106266, CHE-1337975). C.M.K. acknowledges the IMI Program of the NSF under DMR 0843934, and we thank Leonard Barbour for hosting C.M.K. at the University of Stellenbosch. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under DE-AC02-98CH10886. NR 57 TC 5 Z9 5 U1 8 U2 42 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD JAN 26 PY 2015 VL 54 IS 5 BP 1471 EP 1475 DI 10.1002/anie.201409415 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA CA2BL UT WOS:000348713900009 PM 25504739 ER PT J AU Chamberlin, SE Nayyar, IH Kaspar, TC Sushko, PV Chambers, SA AF Chamberlin, S. E. Nayyar, I. H. Kaspar, T. C. Sushko, P. V. Chambers, S. A. TI Electronic structure and optical properties of alpha-(Fe1-xVx)(2)O-3 solid-solution thin films SO APPLIED PHYSICS LETTERS LA English DT Article ID AUGMENTED-WAVE METHOD; INSULATOR-TRANSITION; PHOTOEMISSION; ALPHA-FE2O3; ABSORPTION; OXIDES; V2O3 AB We have examined the effect of V doping on the electronic and optical properties of epitaxial hematite (alpha-Fe2O3) thin films, by employing several characterization techniques and computational modeling. The conductivity of alpha-(Fe1-xVx)(2)O-3 (0 <= x <= similar to 0.5) is enhanced by several orders of magnitude as x is increased, as evidenced by electrical resistivity measurements and x-ray photoelectron spectroscopy core-level and valence-band spectra. Optical absorption shows a reduction in the direct band gap by as much as 0.64 eV for x = 0.53 (E-g = 1.46 eV) relative to that of alpha-Fe2O3 (E-g = 2.10 eV). Detailed understanding of the character of the optical transitions in the alloys is achieved using first-principles calculations of the ground and excited states. These calculations reveal that V doping results in occupied V 3d orbitals hybridized with Fe orbitals and located at approximately mid-gap in alpha-Fe2O3. The lowest energy transitions involve charge transfer from occupied V 3d to unoccupied Fe 3d* orbitals. With a low band gap and high conductivity, alpha-(Fe1-xVx)(2)O-3 is a promising material for photovoltaic and photoelectrochemical applications. (C) 2015 AIP Publishing LLC. C1 [Chamberlin, S. E.; Nayyar, I. H.; Kaspar, T. C.; Sushko, P. V.; Chambers, S. A.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP Chambers, SA (reprint author), Pacific NW Natl Lab, Div Phys Sci, 902 Battelle Blvd, Richland, WA 99352 USA. EM sa.chambers@pnnl.gov RI Sushko, Peter/F-5171-2013; Nayyar, Iffat/B-4925-2016 OI Sushko, Peter/0000-0001-7338-4146; Nayyar, Iffat/0000-0002-0896-5259 FU U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES), Division of Chemical Sciences, Geosciences, and Biosciences; U.S. DOE, Office of Science, BES, Division of Materials Sciences and Engineering; Department of Energy's Office of Biological and Environmental Research FX S.E.C., I.H.N., and S.A.C. were supported by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES), Division of Chemical Sciences, Geosciences, and Biosciences; T.C.K. and P.V.S. were supported by the U.S. DOE, Office of Science, BES, Division of Materials Sciences and Engineering. A portion of the research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). A portion of the computation was performed using PNNL Institutional Computing at Pacific Northwest National Laboratory. PNNL is a multiprogram national laboratory operated for DOE by Battelle. I.H.N. acknowledges Niri Govind for useful discussions. NR 29 TC 2 Z9 2 U1 2 U2 37 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 26 PY 2015 VL 106 IS 4 AR 041905 DI 10.1063/1.4906597 PG 5 WC Physics, Applied SC Physics GA CA6CN UT WOS:000348996200029 ER PT J AU Choi, SG Kang, J Li, J Haneef, H Podraza, NJ Beall, C Wei, SH Christensen, ST Repins, IL AF Choi, S. G. Kang, J. Li, J. Haneef, H. Podraza, N. J. Beall, C. Wei, S. -H. Christensen, S. T. Repins, I. L. TI Optical function spectra and bandgap energy of Cu2SnSe3 SO APPLIED PHYSICS LETTERS LA English DT Article ID THIN-FILMS; SPECTROSCOPIC ELLIPSOMETRY; SEMICONDUCTOR CU2SNSE3; COEVAPORATED CU2SNSE3; SOLAR-CELLS; TEMPERATURE; GROWTH; GAP AB We present the optical function spectra of Cu2SnSe3 determined from 0.30 to 6.45 eV by spectroscopic ellipsometry (SE) at room temperature. We analyze the SE data using the Tauc-Lorentz model and obtain the direct-bandgap energy of 0.49 +/- 0.02 eV, which is much smaller than the previously known value of 0.84 eV for the monoclinic-phase Cu2SnSe3. We also perform density-functional theory calculations to obtain the complex dielectric function data, and the results show good agreement with the experimental spectrum. Finally, we discuss the electronic origin of the main optical structures. (C) 2015 AIP Publishing LLC. C1 [Choi, S. G.; Kang, J.; Beall, C.; Wei, S. -H.; Christensen, S. T.; Repins, I. L.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Li, J.; Haneef, H.; Podraza, N. J.] Univ Toledo, Dept Phys & Astron, Toledo, OH 43606 USA. [Li, J.; Haneef, H.; Podraza, N. J.] Univ Toledo, Wright Ctr Photovolta Innovat & Commercializat, Toledo, OH 43606 USA. RP Choi, SG (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM sukgeun.choi@nrel.gov FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory; University of Toledo FX This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. N.J.P. acknowledges start-up funding support provided by the University of Toledo. NR 35 TC 8 Z9 8 U1 3 U2 39 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 26 PY 2015 VL 106 IS 4 AR 043902 DI 10.1063/1.4907202 PG 5 WC Physics, Applied SC Physics GA CA6CN UT WOS:000348996200075 ER PT J AU Jiang, CS Contreras, MA Mansfield, LM Moutinho, HR Egaas, B Ramanathan, K Al-Jassim, MM AF Jiang, C. -S. Contreras, M. A. Mansfield, L. M. Moutinho, H. R. Egaas, B. Ramanathan, K. Al-Jassim, M. M. TI Nanometer-scale surface potential and resistance mapping of wide-bandgap Cu(In,Ga)Se-2 thin films SO APPLIED PHYSICS LETTERS LA English DT Article ID PROBE FORCE MICROSCOPY; SOLAR-CELLS; EFFICIENCY AB We report microscopic characterization studies of wide-bandgap Cu(In,Ga)Se-2 photovoltaic thin films using the nano-electrical probes of scanning Kelvin probe force microscopy and scanning spreading resistance microscopy. With increasing bandgap, the potential imaging shows significant increases in both the large potential features due to extended defects or defect aggregations and the potential fluctuation due to unresolvable point defects with single or a few charges. The resistance imaging shows increases in both overall resistance and resistance nonuniformity due to defects in the subsurface region. These defects are expected to affect open-circuit voltage after the surfaces are turned to junction upon device completion. (C) 2015 AIP Publishing LLC. C1 [Jiang, C. -S.; Contreras, M. A.; Mansfield, L. M.; Moutinho, H. R.; Egaas, B.; Ramanathan, K.; Al-Jassim, M. M.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Jiang, CS (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM chun.sheng.jiang@nrel.gov RI jiang, chun-sheng/F-7839-2012 FU U.S. Department of Energy [DE-AC36-08GO28308]; National Renewable Energy Laboratory FX The authors thank I. L. Repins at NREL for discussions. This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08GO28308 with the National Renewable Energy Laboratory. NR 11 TC 1 Z9 1 U1 3 U2 22 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 26 PY 2015 VL 106 IS 4 AR 043901 DI 10.1063/1.4907165 PG 5 WC Physics, Applied SC Physics GA CA6CN UT WOS:000348996200074 ER PT J AU Mitrani, JM Shneider, MN AF Mitrani, J. M. Shneider, M. N. TI Time-resolved laser-induced incandescence from multiwalled carbon nanotubes in air SO APPLIED PHYSICS LETTERS LA English DT Article ID LOW-FLUENCE LII; SOOT; DEFECTS; FLAME; PARTICLE; SIZE AB We observed temporal laser-induced incandescence (LII) signals from multiwalled carbon nanotubes (MWCNTs) suspended in ambient air. Unlike previous LII experiments with soot particles, which showed that primary particles with larger diameters cool at slower timescales relative to smaller particles, we observed that thicker MWCNTs with larger outer diameters (ODs) cool at faster timescales relative to thinner MWCNTs with smaller ODs. We suggested a simple explanation of this effect, based on the solution of one-dimensional nonstationary heat conduction equation for the initial non-uniform heating of MWCNTs with ODs greater than the skin depth. (C) 2015 AIP Publishing LLC. C1 [Mitrani, J. M.] Princeton Plasma Phys Lab, Princeton, NJ 08540 USA. [Shneider, M. N.] Princeton Univ, Dept Mech Engn, Princeton, NJ 08544 USA. RP Mitrani, JM (reprint author), Princeton Plasma Phys Lab, Princeton, NJ 08540 USA. EM jmitrani@pppl.gov FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; Program Plasma Science and Technology, at Princeton Plasma Physics Laboratory FX The authors thank Y. Raitses, B. C. Stratton, S. Patel, and A. Merzhevskiy for assistance. This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. James M. Mitrani acknowledges support through the Program Plasma Science and Technology, at Princeton Plasma Physics Laboratory. NR 25 TC 3 Z9 3 U1 1 U2 9 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 26 PY 2015 VL 106 IS 4 AR 043102 DI 10.1063/1.4907000 PG 4 WC Physics, Applied SC Physics GA CA6CN UT WOS:000348996200054 ER PT J AU Burghoff, D Yang, Y Hayton, DJ Gao, JR Reno, JL Hu, Q AF Burghoff, David Yang, Yang Hayton, Darren J. Gao, Jian-Rong Reno, John L. Hu, Qing TI Evaluating the coherence and time-domain profile of quantum cascade laser frequency combs SO OPTICS EXPRESS LA English DT Article ID TERAHERTZ; MICRORESONATOR; LOCKING; NOISE AB Recently, much attention has been focused on the generation of optical frequency combs from quantum cascade lasers. We discuss how fast detectors can be used to demonstrate the mutual coherence of such combs, and present an inequality that can be used to quantitatively evaluate their performance. We discuss several technical issues related to shifted wave interference Fourier Transform spectroscopy (SWIFTS), and show how such measurements can be used to elucidate the time-domain properties of such combs, showing that they can possess signatures of both frequency-modulation and amplitude-modulation. (C) 2015 Optical Society of America C1 [Burghoff, David; Yang, Yang; Hu, Qing] MIT, Dept Elect Engn & Comp Sci, Elect Res Lab, Cambridge, MA 02139 USA. [Hayton, Darren J.; Gao, Jian-Rong] SRON Netherlands Inst Space Res, SRON, NL-9747 AD Groningen, Netherlands. [Gao, Jian-Rong] Delft Univ Technol, Kavli Inst NanoSci, NL-2628 CJ Delft, Netherlands. [Reno, John L.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87123 USA. RP Burghoff, D (reprint author), MIT, Dept Elect Engn & Comp Sci, Elect Res Lab, Cambridge, MA 02139 USA. EM burghoff@mit.edu FU NASA; NSF; NWO; NATO; SFP; RadioNet; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX We would like to acknowledge Jeffrey Hesler of Virginia Diodes for loaning us one of their Schottky mixers. The work at MIT is supported by NASA and NSF. The work in the Netherlands was supported by NWO, NATO SFP, and RadioNet. This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 29 TC 13 Z9 13 U1 1 U2 24 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD JAN 26 PY 2015 VL 23 IS 2 BP 1190 EP 1202 DI 10.1364/OE.23.001190 PG 13 WC Optics SC Optics GA CA8JT UT WOS:000349166100059 PM 25835878 ER PT J AU Caleman, C Timneanu, N Martin, AV Jonsson, HO Aquila, A Barty, A Scott, HA White, TA Chapman, HN AF Caleman, Carl Timneanu, Nicusor Martin, Andrew V. Jonsson, H. Olof Aquila, Andrew Barty, Anton Scott, Howard A. White, Thomas A. Chapman, Henry N. TI Ultrafast self-gating Bragg diffraction of exploding nanocrystals in an X-ray laser SO OPTICS EXPRESS LA English DT Article ID FREE-ELECTRON LASER; RADIATION-DAMAGE; PLASMAS; PULSES; IONIZATION; SCATTERING; RESOLUTION; OPERATION; CRYSTALS; CODE AB In structural determination of crystalline proteins using intense femtosecond X-ray lasers, damage processes lead to loss of structural coherence during the exposure. We use a nonthermal description for the damage dynamics to calculate the ultrafast ionization and the subsequent atomic displacement. These effects degrade the Bragg diffraction on femtosecond time scales and gate the ultrafast imaging. This process is intensity and resolution dependent. At high intensities the signal is gated by the ionization affecting low resolution information first. At lower intensities, atomic displacement dominates the loss of coherence affecting high-resolution information. We find that pulse length is not a limiting factor as long as there is a high enough X-ray flux to measure a diffracted signal. (C) 2015 Optical Society of America C1 [Caleman, Carl; Martin, Andrew V.; Aquila, Andrew; Barty, Anton; White, Thomas A.; Chapman, Henry N.] DESY, Ctr Free Elect Laser Sci, DE-22607 Hamburg, Germany. [Caleman, Carl; Timneanu, Nicusor; Jonsson, H. Olof] Uppsala Univ, Dept Phys & Astron, SE-75120 Uppsala, Sweden. [Timneanu, Nicusor] Uppsala Univ, Dept Cell & Mol Biol, Biomed Ctr, SE-75124 Uppsala, Sweden. [Scott, Howard A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Chapman, Henry N.] Univ Hamburg, DE-22761 Hamburg, Germany. RP Chapman, HN (reprint author), DESY, Ctr Free Elect Laser Sci, Notkestr 85, DE-22607 Hamburg, Germany. EM henry.chapman@cfel.de RI Barty, Anton/K-5137-2014; Timneanu, Nicusor/C-7691-2012; Chapman, Henry/G-2153-2010; OI Barty, Anton/0000-0003-4751-2727; Timneanu, Nicusor/0000-0001-7328-0400; Chapman, Henry/0000-0002-4655-1743; MARTIN, ANDREW/0000-0003-3704-1829 FU Helmholtz Association through the Center for Free-Electron Laser Science at DESY; Swedish Research foundation; Rontgen Angstrom Cluster; Swedish Foundation for Strategic Research; CRETIN FX The authors thank the Helmholtz Association through the Center for Free-Electron Laser Science at DESY, Swedish Research foundation, Rontgen Angstrom Cluster, and the Swedish Foundation for Strategic Research for financial support. The Swedish National Infrastructure for Computing, UPPMAX (project S00111-71 and p2012227) and David van der Spoel are acknowledged for computational resources, and Magnus Bergh for support with CRETIN simulations. NR 63 TC 7 Z9 7 U1 0 U2 18 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD JAN 26 PY 2015 VL 23 IS 2 BP 1213 EP 1231 DI 10.1364/OE.23.001213 PG 19 WC Optics SC Optics GA CA8JT UT WOS:000349166100061 PM 25835880 ER PT J AU Soehnel, G AF Soehnel, Grant TI Time resolved photo-luminescent decay characterization of mercury cadmium telluride focal plane arrays SO OPTICS EXPRESS LA English DT Article ID HG1-XCDXTE AB The minority carrier lifetime is a measurable material property that is an indication of infrared detector device performance. To study the utility of measuring the carrier lifetime, an experiment has been constructed that can time resolve the photo-luminescent decay of a detector or wafer sample housed inside a liquid nitrogen cooled Dewar. Motorized stages allow the measurement to be scanned over the sample surface, and spatial resolutions as low as 50 mu m have been demonstrated. A carrier recombination simulation was developed to analyze the experimental data. Results from measurements performed on 4 mercury cadmium telluride focal plane arrays show strong correlation between spatial maps of the lifetime, dark current, and relative response. (C) 2015 Optical Society of America C1 Sandia Natl Labs, Albuquerque, NM 87123 USA. RP Soehnel, G (reprint author), Sandia Natl Labs, 1515 Eubank SE, Albuquerque, NM 87123 USA. EM gsoehne@sandia.gov NR 8 TC 0 Z9 0 U1 0 U2 8 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD JAN 26 PY 2015 VL 23 IS 2 BP 1256 EP 1264 DI 10.1364/OE.23.001256 PG 9 WC Optics SC Optics GA CA8JT UT WOS:000349166100065 PM 25835884 ER PT J AU Halls, BR Meyer, TR Kastengren, AL AF Halls, Benjamin R. Meyer, Terrence R. Kastengren, Alan L. TI Quantitative measurement of binary liquid distributions using multiple-tracer x-ray fluorescence and radiography SO OPTICS EXPRESS LA English DT Article ID SPRAYS; BEAMLINE AB The complex geometry and large index-of-refraction gradients that occur near the point of impingement of binary liquid jets present a challenging environment for optical interrogation. A simultaneous quadruple-tracer x-ray fluorescence and line-of-sight radiography technique is proposed as a means of distinguishing and quantifying individual liquid component distributions prior to, during, and after jet impact. Two different pairs of fluorescence tracers are seeded into each liquid stream to maximize their attenuation ratio for reabsorption correction and differentiation of the two fluids during mixing. This approach for instantaneous correction of xray fluorescence reabsorption is compared with a more time-intensive approach of using stereographic reconstruction of x-ray attenuation along multiple lines of sight. The proposed methodology addresses the need for a quantitative measurement technique capable of interrogating optically complex, near-field liquid distributions in many mixing systems of practical interest involving two or more liquid streams. (C) 2015 Optical Society of America C1 [Halls, Benjamin R.; Meyer, Terrence R.] Iowa State Univ, Dept Mech Engn, Ames, IA 50011 USA. [Kastengren, Alan L.] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Meyer, TR (reprint author), Iowa State Univ, Dept Mech Engn, Ames, IA 50011 USA. EM trm@iastate.edu FU Army Research Office; U.S. Department of Energy [DE-AC02-06CH11357] FX This work was funded, in part, by the Army Research Office (Dr. Ralph Anthenien, Program Manager). A portion of this research was performed at the 7-BM beamline of the Advanced Photon Source, Argonne National Laboratory. Use of the APS is supported by the U.S. Department of Energy under Contract No. DE-AC02-06CH11357. The authors express their gratitude to M. Johnson, C. Radke, A. Poniatowski, J. Tiarks, D. Stoecklein, and W. Lubberden of Iowa State University for their technical assistance. NR 24 TC 5 Z9 5 U1 0 U2 0 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD JAN 26 PY 2015 VL 23 IS 2 BP 1730 EP 1739 DI 10.1364/OE.23.001730 PG 10 WC Optics SC Optics GA CA8JT UT WOS:000349166100109 PM 25835928 ER PT J AU Adare, A Aidala, C Ajitanand, NN Akiba, Y Al-Bataineh, H Alexander, J Angerami, A Aoki, K Apadula, N Aramaki, Y Atomssa, ET Averbeck, R Awes, TC Azmoun, B Babintsev, V Bai, M Baksay, G Baksay, L Barish, KN Bassalleck, B Basye, AT Bathe, S Baublis, V Baumann, C Bazilevsky, A Belikov, S Belmont, R Bennett, R Bhom, JH Blau, DS Bok, JS Boyle, K Brooks, ML Buesching, H Bumazhnov, V Bunce, G Butsyk, S Campbell, S Caringi, A Chen, CH Chi, CY Chiu, M Choi, IJ Choi, JB Choudhury, RK Christiansen, P Chujo, T Chung, P Chvala, O Cianciolo, V Citron, Z Cole, BA del Valle, ZC Connors, M Csanad, M Csorgo, T Dahms, T Dairaku, S Danchev, I Das, K Datta, A David, G Dayananda, MK Denisov, A Deshpande, A Desmond, EJ Dharmawardane, KV Dietzsch, O Dion, A Donadelli, M Drapier, O Drees, A Drees, KA Durham, JM Durum, A Dutta, D D'Orazio, L Edwards, S Efremenko, YV Ellinghaus, F Engelmore, T Enokizono, A En'yo, H Esumi, S Fadem, B Fields, DE Finger, M Finger, M Fleuret, F Fokin, SL Fraenkel, Z Frantz, JE Franz, A Frawley, AD Fujiwara, K Fukao, Y Fusayasu, T Garishvili, I Glenn, A Gong, H Gonin, M Goto, Y de Cassagnac, RG Grau, N Greene, SV Grim, G Perdekamp, MG Gunji, T Gustafsson, HA Haggerty, JS Hahn, KI Hamagaki, H Hamblen, J Han, R Hanks, J Haslum, E Hayano, R He, X Heffner, M Hemmick, TK Hester, T Hill, JC Hohlmann, M Holzmann, W Homma, K Hong, B Horaguchi, T Hornback, D Huang, S Ichihara, T Ichimiya, R Ikeda, Y Imai, K Inaba, M Isenhower, D Ishihara, M Issah, M Ivanischev, D Iwanaga, Y Jacak, BV Jia, J Jiang, X Jin, J Johnson, BM Jones, T Joo, KS Jouan, D Jumper, DS Kajihara, F Kamin, J Kang, JH Kapustinsky, J Karatsu, K Kasai, M Kawall, D Kawashima, M Kazantsev, AV Kempel, T Khanzadeev, A Kijima, KM Kikuchi, J Kim, A Kim, BI Kim, DJ Kim, EJ Kim, YJ Kinney, E Kiss, A Kistenev, E Kleinjan, D Kochenda, L Komkov, B Konno, M Koster, J Kral, A Kravitz, A Kunde, GJ Kurita, K Kurosawa, M Kwon, Y Kyle, GS Lacey, R Lai, YS Lajoie, JG Lebedev, A Lee, DM Lee, J Lee, KB Lee, KS Leitch, MJ Leite, MAL Li, X Lichtenwalner, P Liebing, P Levy, LAL Liska, T Liu, H Liu, MX Love, B Lynch, D Maguire, CF Makdisi, YI Malik, MD Manko, VI Mannel, E Mao, Y Masui, H Matathias, F McCumber, M McGaughey, PL McGlinchey, D Means, N Meredith, B Miake, Y Mibe, T Mignerey, AC Miki, K Milov, A Mitchell, JT Mohanty, AK Moon, HJ Morino, Y Morreale, A Morrison, DP Moukhanova, TV Murakami, T Murata, J Nagamiya, S Nagle, JL Naglis, M Nagy, MI Nakagawa, I Nakamiya, Y Nakamura, KR Nakamura, T Nakano, K Nam, S Newby, J Nguyen, M Nihashi, M Nouicer, R Nyanin, AS Oakley, C O'Brien, E Oda, SX Ogilvie, CA Oka, M Okada, K Onuki, Y Oskarsson, A Ouchida, M Ozawa, K Pak, R Pantuev, V Papavassiliou, V Park, IH Park, SK Park, WJ Pate, SF Pei, H Peng, JC Pereira, H Peressounko, DY Petti, R Pinkenburg, C Pisani, RP Proissl, M Purschke, ML Qu, H Rak, J Ravinovich, I Read, KF Rembeczki, S Reygers, K Riabov, V Riabov, Y Richardson, E Roach, D Roche, G Rolnick, SD Rosati, M Rosen, CA Rosendahl, SSE Ruzicka, P Sahlmueller, B Saito, N Sakaguchi, T Sakashita, K Samsonov, V Sano, S Sato, T Sawada, S Sedgwick, K Seele, J Seidl, R Seto, R Sharma, D Shein, I Shibata, TA Shigaki, K Shimomura, M Shoji, K Shukla, P Sickles, A Silva, CL Silvermyr, D Silvestre, C Sim, KS Singh, BK Singh, CP Singh, V Slunecka, M Soltz, RA Sondheim, WE Sorensen, SP Sourikova, IV Stankus, PW Stenlund, E Stoll, SP Sugitate, T Sukhanov, A Sziklai, J Takagui, EM Taketani, A Tanabe, R Tanaka, Y Taneja, S Tanida, K Tannenbaum, MJ Tarafdar, S Taranenko, A Themann, H Thomas, D Thomas, TL Togawa, M Toia, A Tomasek, L Torii, H Towell, RS Tserruya, I Tsuchimoto, Y Vale, C Valle, H van Hecke, HW Vazquez-Zambrano, E Veicht, A Velkovska, J Vertesi, R Virius, M Vrba, V Vznuzdaev, E Wang, XR Watanabe, D Watanabe, K Watanabe, Y Wei, F Wei, R Wessels, J White, SN Winter, D Woody, CL Wright, RM Wysocki, M Yamaguchi, YL Yamaura, K Yang, R Yanovich, A Ying, J Yokkaichi, S You, Z Young, GR Younus, I Yushmanov, IE Zajc, WA Zhou, S AF Adare, A. Aidala, C. Ajitanand, N. N. Akiba, Y. Al-Bataineh, H. Alexander, J. Angerami, A. Aoki, K. Apadula, N. Aramaki, Y. Atomssa, E. T. Averbeck, R. Awes, T. C. Azmoun, B. Babintsev, V. Bai, M. Baksay, G. Baksay, L. Barish, K. N. Bassalleck, B. Basye, A. T. Bathe, S. Baublis, V. Baumann, C. Bazilevsky, A. Belikov, S. Belmont, R. Bennett, R. Bhom, J. H. Blau, D. S. Bok, J. S. Boyle, K. Brooks, M. L. Buesching, H. Bumazhnov, V. Bunce, G. Butsyk, S. Campbell, S. Caringi, A. Chen, C. -H. Chi, C. Y. Chiu, M. Choi, I. J. Choi, J. B. Choudhury, R. K. Christiansen, P. Chujo, T. Chung, P. Chvala, O. Cianciolo, V. Citron, Z. Cole, B. A. del Valle, Z. Conesa Connors, M. Csanad, M. Csoergo, T. Dahms, T. Dairaku, S. Danchev, I. Das, K. Datta, A. David, G. Dayananda, M. K. Denisov, A. Deshpande, A. Desmond, E. J. Dharmawardane, K. V. Dietzsch, O. Dion, A. Donadelli, M. Drapier, O. Drees, A. Drees, K. A. Durham, J. M. Durum, A. Dutta, D. D'Orazio, L. Edwards, S. Efremenko, Y. V. Ellinghaus, F. Engelmore, T. Enokizono, A. En'yo, H. Esumi, S. Fadem, B. Fields, D. E. Finger, M. Finger, M., Jr. Fleuret, F. Fokin, S. L. Fraenkel, Z. Frantz, J. E. Franz, A. Frawley, A. D. Fujiwara, K. Fukao, Y. Fusayasu, T. Garishvili, I. Glenn, A. Gong, H. Gonin, M. Goto, Y. de Cassagnac, R. Granier Grau, N. Greene, S. V. Grim, G. Perdekamp, M. Grosse Gunji, T. Gustafsson, H. -A. Haggerty, J. S. Hahn, K. I. Hamagaki, H. Hamblen, J. Han, R. Hanks, J. Haslum, E. Hayano, R. He, X. Heffner, M. Hemmick, T. K. Hester, T. Hill, J. C. Hohlmann, M. Holzmann, W. Homma, K. Hong, B. Horaguchi, T. Hornback, D. Huang, S. Ichihara, T. Ichimiya, R. Ikeda, Y. Imai, K. Inaba, M. Isenhower, D. Ishihara, M. Issah, M. Ivanischev, D. Iwanaga, Y. Jacak, B. V. Jia, J. Jiang, X. Jin, J. Johnson, B. M. Jones, T. Joo, K. S. Jouan, D. Jumper, D. S. Kajihara, F. Kamin, J. Kang, J. H. Kapustinsky, J. Karatsu, K. Kasai, M. Kawall, D. Kawashima, M. Kazantsev, A. V. Kempel, T. Khanzadeev, A. Kijima, K. M. Kikuchi, J. Kim, A. Kim, B. I. Kim, D. J. Kim, E. -J. Kim, Y. -J. Kinney, E. Kiss, A. Kistenev, E. Kleinjan, D. Kochenda, L. Komkov, B. Konno, M. Koster, J. Kral, A. Kravitz, A. Kunde, G. J. Kurita, K. Kurosawa, M. Kwon, Y. Kyle, G. S. Lacey, R. Lai, Y. S. Lajoie, J. G. Lebedev, A. Lee, D. M. Lee, J. Lee, K. B. Lee, K. S. Leitch, M. J. Leite, M. A. L. Li, X. Lichtenwalner, P. Liebing, P. Levy, L. A. Linden Liska, T. Liu, H. Liu, M. X. Love, B. Lynch, D. Maguire, C. F. Makdisi, Y. I. Malik, M. D. Manko, V. I. Mannel, E. Mao, Y. Masui, H. Matathias, F. McCumber, M. McGaughey, P. L. McGlinchey, D. Means, N. Meredith, B. Miake, Y. Mibe, T. Mignerey, A. C. Miki, K. Milov, A. Mitchell, J. T. Mohanty, A. K. Moon, H. J. Morino, Y. Morreale, A. Morrison, D. P. Moukhanova, T. V. Murakami, T. Murata, J. Nagamiya, S. Nagle, J. L. Naglis, M. Nagy, M. I. Nakagawa, I. Nakamiya, Y. Nakamura, K. R. Nakamura, T. Nakano, K. Nam, S. Newby, J. Nguyen, M. Nihashi, M. Nouicer, R. Nyanin, A. S. Oakley, C. O'Brien, E. Oda, S. X. Ogilvie, C. A. Oka, M. Okada, K. Onuki, Y. Oskarsson, A. Ouchida, M. Ozawa, K. Pak, R. Pantuev, V. Papavassiliou, V. Park, I. H. Park, S. K. Park, W. J. Pate, S. F. Pei, H. Peng, J. -C. Pereira, H. Peressounko, D. Yu. Petti, R. Pinkenburg, C. Pisani, R. P. Proissl, M. Purschke, M. L. Qu, H. Rak, J. Ravinovich, I. Read, K. F. Rembeczki, S. Reygers, K. Riabov, V. Riabov, Y. Richardson, E. Roach, D. Roche, G. Rolnick, S. D. Rosati, M. Rosen, C. A. Rosendahl, S. S. E. Ruzicka, P. Sahlmueller, B. Saito, N. Sakaguchi, T. Sakashita, K. Samsonov, V. Sano, S. Sato, T. Sawada, S. Sedgwick, K. Seele, J. Seidl, R. Seto, R. Sharma, D. Shein, I. Shibata, T. -A. Shigaki, K. Shimomura, M. Shoji, K. Shukla, P. Sickles, A. Silva, C. L. Silvermyr, D. Silvestre, C. Sim, K. S. Singh, B. K. Singh, C. P. Singh, V. Slunecka, M. Soltz, R. A. Sondheim, W. E. Sorensen, S. P. Sourikova, I. V. Stankus, P. W. Stenlund, E. Stoll, S. P. Sugitate, T. Sukhanov, A. Sziklai, J. Takagui, E. M. Taketani, A. Tanabe, R. Tanaka, Y. Taneja, S. Tanida, K. Tannenbaum, M. J. Tarafdar, S. Taranenko, A. Themann, H. Thomas, D. Thomas, T. L. Togawa, M. Toia, A. Tomasek, L. Torii, H. Towell, R. S. Tserruya, I. Tsuchimoto, Y. Vale, C. Valle, H. van Hecke, H. W. Vazquez-Zambrano, E. Veicht, A. Velkovska, J. Vertesi, R. Virius, M. Vrba, V. Vznuzdaev, E. Wang, X. R. Watanabe, D. Watanabe, K. Watanabe, Y. Wei, F. Wei, R. Wessels, J. White, S. N. Winter, D. Woody, C. L. Wright, R. M. Wysocki, M. Yamaguchi, Y. L. Yamaura, K. Yang, R. Yanovich, A. Ying, J. Yokkaichi, S. You, Z. Young, G. R. Younus, I. Yushmanov, I. E. Zajc, W. A. Zhou, S. CA PHENIX Collaboration TI Cross section for b(b)over-bar production via dielectrons in d plus Au collisions at root s(NN)=200 GeV SO PHYSICAL REVIEW C LA English DT Article ID QUARK-GLUON PLASMA; PHENIX; COLLABORATION; PERSPECTIVE; MATTER AB We report a measurement of e(+)e(-) pairs from semileptonic heavy-flavor decays in d + Au collisions at root s(NN) = 200 GeV. By exploring the mass and transverse-momentum dependence of the yield, the bottom decay contribution can be isolated from charm, and quantified by comparison to PYTHIA and MC@NLO simulations. The resulting b (b) over bar -production cross section is sigma(dAu)(b (b) over bar) = 1.37 +/- 0.28 (stat) +/- 0.46 (syst) mb, which is equivalent to a nucleon-nucleon cross section of sigma(NN)(b (b) over bar) = 3.4 +/- 0.8 (stat) +/- 1.1 ( syst) mu b. C1 [Basye, A. T.; Isenhower, D.; Jones, T.; Jumper, D. S.; Thomas, D.; Towell, R. S.; Wright, R. M.] Abilene Christian Univ, Abilene, TX 79699 USA. [Grau, N.] Augustana Coll, Dept Phys, Sioux Falls, SD 57197 USA. [Singh, B. K.; Singh, V.] Banaras Hindu Univ, Dept Phys, Varanasi 221005, Uttar Pradesh, India. [Choudhury, R. K.; Dutta, D.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Bathe, S.] CUNY, Baruch Coll, New York, NY USA. [Bai, M.; Drees, K. A.; Makdisi, Y. I.] Brookhaven Natl Lab, Collider Accelerator Dept, Upton, NY 11973 USA. [Azmoun, B.; Bazilevsky, A.; Belikov, S.; Buesching, H.; Bunce, G.; Chiu, M.; David, G.; Desmond, E. J.; Franz, A.; Grim, G.; Haggerty, J. S.; Jia, J.; Johnson, B. M.; Kistenev, E.; Lynch, D.; Milov, A.; Mitchell, J. T.; Morrison, D. P.; Nouicer, R.; O'Brien, E.; Pak, R.; Petti, R.; Pinkenburg, C.; Pisani, R. P.; Purschke, M. L.; Sakaguchi, T.; Sickles, A.; Sourikova, I. V.; Stoll, S. P.; Sukhanov, A.; Tannenbaum, M. J.; Vale, C.; White, S. N.; Woody, C. L.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Barish, K. N.; Bathe, S.; Chvala, O.; Hester, T.; Kleinjan, D.; Morreale, A.; Rolnick, S. D.; Sedgwick, K.; Seto, R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Finger, M.; Slunecka, M.] Charles Univ Prague, CR-11636 Prague, Czech Republic. [Choi, J. B.; Kim, E. -J.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Li, X.; Zhou, S.] China Inst Atom Energy, Sci & Technol Nucl Data Lab, Beijing 102413, Peoples R China. [Aramaki, Y.; Gunji, T.; Hamagaki, H.; Hayano, R.; Kajihara, F.; Morino, Y.; Oda, S. X.; Ozawa, K.; Sano, S.; Yamaguchi, Y. L.] Univ Tokyo, Grad Sch Sci, Ctr Nucl Study, Bunkyo Ku, Tokyo 1130033, Japan. [Adare, A.; Ellinghaus, F.; Kinney, E.; Levy, L. A. Linden; McGlinchey, D.; Nagle, J. L.; Rosen, C. A.; Seele, J.; Wysocki, M.] Univ Colorado, Boulder, CO 80309 USA. [Angerami, A.; Chi, C. Y.; Cole, B. A.; Engelmore, T.; Grau, N.; Hanks, J.; Holzmann, W.; Jin, J.; Kravitz, A.; Lai, Y. S.; Mannel, E.; Matathias, F.; Vazquez-Zambrano, E.; Winter, D.; Zajc, W. A.] Columbia Univ, New York, NY 10027 USA. [Angerami, A.; Chi, C. Y.; Cole, B. A.; Engelmore, T.; Grau, N.; Hanks, J.; Holzmann, W.; Jin, J.; Kravitz, A.; Lai, Y. S.; Mannel, E.; Matathias, F.; Vazquez-Zambrano, E.; Winter, D.; Zajc, W. A.] Nevis Labs, Irvington, NY 10533 USA. [Kral, A.; Liska, T.; Virius, M.] Czech Tech Univ, Prague 16636 6, Czech Republic. [Pereira, H.; Silvestre, C.] CEA Saclay, Dapnia, F-91191 Gif Sur Yvette, France. [Csanad, M.; Kiss, A.] Eotvos Lorand Univ, ELTE, H-1117 Budapest, Hungary. [Hahn, K. I.; Kim, A.; Lee, J.; Nam, S.; Park, I. H.] Ewha Womans Univ, Seoul 120750, South Korea. [Baksay, G.; Baksay, L.; Hohlmann, M.; Rembeczki, S.] Florida Inst Technol, Melbourne, FL 32901 USA. [Das, K.; Edwards, S.; Frawley, A. D.; McGlinchey, D.] Florida State Univ, Tallahassee, FL 32306 USA. [Dayananda, M. K.; He, X.; Oakley, C.; Qu, H.; Ying, J.] Georgia State Univ, Atlanta, GA 30303 USA. [Homma, K.; Horaguchi, T.; Iwanaga, Y.; Kijima, K. M.; Nakamiya, Y.; Nihashi, M.; Ouchida, M.; Shigaki, K.; Sugitate, T.; Torii, H.; Tsuchimoto, Y.; Watanabe, D.; Yamaura, K.] Hiroshima Univ, Higashihiroshima 7398526, Japan. [Babintsev, V.; Bumazhnov, V.; Denisov, A.; Durum, A.; Shein, I.; Yanovich, A.] State Res Ctr Russian Federat, IHEP Protvino, Inst High Energy Phys, Protvino, Russia. [Perdekamp, M. Grosse; Kim, Y. -J.; Koster, J.; Meredith, B.; Peng, J. -C.; Seidl, R.; Veicht, A.; Yang, R.] Univ Illinois, Urbana, IL 61801 USA. [Pantuev, V.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Ruzicka, P.; Tomasek, L.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague 18221 8, Czech Republic. [Dion, A.; Hill, J. C.; Kempel, T.; Lajoie, J. G.; Lebedev, A.; Ogilvie, C. A.; Pei, H.; Rosati, M.; Silva, C. L.; Wei, F.] Iowa State Univ, Ames, IA 50011 USA. [Imai, K.] Japan Atom Energy Agcy, Adv Sci Res Ctr, Naka, Ibaraki, Japan. [Kim, D. J.; Rak, J.] Helsinki Inst Phys, FI-40014 Jyvaskyla, Finland. [Kim, D. J.; Rak, J.] Univ Jyvaskyla, FI-40014 Jyvaskyla, Finland. [Mibe, T.; Nagamiya, S.; Saito, N.; Sawada, S.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki 3050801, Japan. [Hong, B.; Kim, B. I.; Lee, K. B.; Lee, K. S.; Park, S. K.; Park, W. J.; Sim, K. S.] Korea Univ, Seoul 136701, South Korea. [Blau, D. S.; Fokin, S. L.; Kazantsev, A. V.; Manko, V. I.; Moukhanova, T. V.; Nyanin, A. S.; Peressounko, D. Yu.; Yushmanov, I. E.] Russian Res Ctr, Kurchatov Inst, Moscow 123098, Russia. [Aoki, K.; Dairaku, S.; Imai, K.; Karatsu, K.; Murakami, T.; Nakamura, K. R.; Shoji, K.; Tanida, K.] Kyoto Univ, Kyoto 6068502, Japan. [Atomssa, E. T.; del Valle, Z. Conesa; Drapier, O.; Fleuret, F.; Gonin, M.; de Cassagnac, R. Granier] Ecole Polytech, CNRS, Lab Leprince Ringuet, IN2P3, F-91128 Palaiseau, France. [Younus, I.] Lahore Univ Management Sci, Dept Phys, Lahore 54792, Pakistan. [Glenn, A.; Heffner, M.; Newby, J.; Soltz, R. A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Brooks, M. L.; Butsyk, S.; Durham, J. M.; Grim, G.; Jiang, X.; Kapustinsky, J.; Kunde, G. J.; Lee, D. M.; Leitch, M. J.; Liu, H.; Liu, M. X.; McGaughey, P. L.; Sondheim, W. E.; van Hecke, H. W.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Roach, D.; Roche, G.] Univ Clermont Ferrand, CNRS, LPC, IN2P3, F-63177 Aubiere, France. [Christiansen, P.; Gustafsson, H. -A.; Haslum, E.; Oskarsson, A.; Rosendahl, S. S. E.; Stenlund, E.] Lund Univ, Dept Phys, SE-22100 Lund, Sweden. [D'Orazio, L.; Mignerey, A. C.] Univ Maryland, College Pk, MD 20742 USA. [Aidala, C.; Datta, A.; Kawall, D.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Aidala, C.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Baumann, C.; Reygers, K.; Sahlmueller, B.; Wessels, J.] Univ Munster, Inst Kernphys, D-48149 Munster, Germany. [Caringi, A.; Fadem, B.; Lichtenwalner, P.] Muhlenberg Coll, Allentown, PA 18104 USA. [Joo, K. S.; Moon, H. J.] Myongji Univ, Yongin 449728, Kyonggido, South Korea. [Fusayasu, T.; Tanaka, Y.] Nagasaki Inst Appl Sci, Nagasaki 8510193, Japan. [Samsonov, V.; Taranenko, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst, MEPhI, Moscow 115409, Russia. [Bassalleck, B.; Fields, D. E.; Malik, M. D.; Thomas, T. L.; Younus, I.] Univ New Mexico, Albuquerque, NM 87131 USA. [Al-Bataineh, H.; Dharmawardane, K. V.; Kyle, G. S.; Papavassiliou, V.; Pate, S. F.; Wang, X. R.] New Mexico State Univ, Las Cruces, NM 88003 USA. [Frantz, J. E.] Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. [Awes, T. C.; Cianciolo, V.; Efremenko, Y. V.; Enokizono, A.; Read, K. F.; Silvermyr, D.; Stankus, P. W.; Young, G. R.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Jouan, D.] Univ Paris 11, IPN Orsay, CNRS, IN2P3, F-91406 Orsay, France. [Han, R.; Mao, Y.; You, Z.] Peking Univ, Beijing 100871, Peoples R China. [Baublis, V.; Ivanischev, D.; Khanzadeev, A.; Kochenda, L.; Komkov, B.; Riabov, V.; Riabov, Y.; Samsonov, V.; Vznuzdaev, E.] Petersburg Nucl Phys Inst, St Petersburg 188300, Russia. [Akiba, Y.; Aoki, K.; Aramaki, Y.; Dairaku, S.; En'yo, H.; Fujiwara, K.; Fukao, Y.; Goto, Y.; Ichihara, T.; Ichimiya, R.; Imai, K.; Ishihara, M.; Karatsu, K.; Kasai, M.; Kawashima, M.; Kurita, K.; Kurosawa, M.; Mao, Y.; Miki, K.; Murata, J.; Nagamiya, S.; Nakagawa, I.; Nakamura, K. R.; Nakamura, T.; Nakano, K.; Onuki, Y.; Ouchida, M.; Sakashita, K.; Shibata, T. -A.; Shoji, K.; Taketani, A.; Tanida, K.; Watanabe, Y.; Yamaguchi, Y. L.; Yokkaichi, S.] RIKEN, Nishina Ctr Accelerator Based Sci, Wako, Saitama 3510198, Japan. [Akiba, Y.; Bathe, S.; Bunce, G.; Deshpande, A.; En'yo, H.; Goto, Y.; Ichihara, T.; Kawall, D.; Liebing, P.; Nakagawa, I.; Okada, K.; Seidl, R.; Taketani, A.; Tanida, K.; Togawa, M.; Watanabe, Y.; Yokkaichi, S.] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Kasai, M.; Kawashima, M.; Kurita, K.; Murata, J.] Rikkyo Univ, Dept Phys, Tokyo 1718501, Japan. [Dietzsch, O.; Donadelli, M.; Leite, M. A. L.; Takagui, E. M.] Univ Sao Paulo, Inst Fis, BR-05315970 Sao Paulo, Brazil. [Ajitanand, N. N.; Alexander, J.; Chung, P.; Jia, J.; Lacey, R.; Taranenko, A.; Wei, R.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Apadula, N.; Averbeck, R.; Bennett, R.; Boyle, K.; Campbell, S.; Chen, C. -H.; Citron, Z.; Connors, M.; Dahms, T.; Deshpande, A.; Dion, A.; Drees, A.; Durham, J. M.; Frantz, J. E.; Gong, H.; Hemmick, T. K.; Jacak, B. V.; Kamin, J.; McCumber, M.; Means, N.; Nguyen, M.; Pantuev, V.; Petti, R.; Proissl, M.; Sahlmueller, B.; Taneja, S.; Themann, H.; Toia, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Garishvili, I.; Hamblen, J.; Hornback, D.; Read, K. F.; Sorensen, S. P.] Univ Tennessee, Knoxville, TN 37996 USA. [Sakashita, K.; Shibata, T. -A.] Tokyo Inst Technol, Dept Phys, Tokyo 1528551, Japan. [Chujo, T.; Esumi, S.; Ikeda, Y.; Inaba, M.; Konno, M.; Masui, H.; Miake, Y.; Miki, K.; Oka, M.; Sato, T.; Shimomura, M.; Tanabe, R.; Watanabe, K.] Univ Tsukuba, Inst Phys, Tsukuba, Ibaraki 305, Japan. [Belmont, R.; Danchev, I.; Greene, S. V.; Huang, S.; Issah, M.; Love, B.; Maguire, C. F.; Richardson, E.; Valle, H.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Kikuchi, J.; Sano, S.] Waseda Univ, Adv Res Inst Sci & Engn, Shinjuku Ku, Tokyo 1620044, Japan. [Deshpande, A.; Fraenkel, Z.; Kiss, A.; Naglis, M.; Ravinovich, I.; Sharma, D.; Tserruya, I.] Weizmann Inst Sci, IL-76100 Rehovot, Israel. [Csoergo, T.; Nagy, M. I.; Sziklai, J.; Vertesi, R.] Hungarian Acad Sci, Wigner Res Ctr Phys, Inst Nucl & Particle Phys, Wigner RCP,RMKI, H-1525 Budapest, Hungary. [Bhom, J. H.; Bok, J. S.; Choi, I. J.; Kang, J. H.; Kwon, Y.] Yonsei Univ, IPAP, Seoul 120749, South Korea. RP Morrison, DP (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. EM morrison@bnl.gov; jamie.nagle@colorado.edu RI Hayano, Ryugo/F-7889-2012; HAMAGAKI, HIDEKI/G-4899-2014; Durum, Artur/C-3027-2014; Sorensen, Soren /K-1195-2016; Yokkaichi, Satoshi/C-6215-2017; Taketani, Atsushi/E-1803-2017 OI Hayano, Ryugo/0000-0002-1214-7806; Sorensen, Soren /0000-0002-5595-5643; Taketani, Atsushi/0000-0002-4776-2315 FU Office of Nuclear Physics in the Office of Science of the Department of Energy; National Science Foundation; Abilene Christian University Research Council; Research Foundation of SUNY; College of Arts and Sciences, Vanderbilt University (USA); Ministry of Education, Culture, Sports, Science, and Technology; Japan Society for the Promotion of Science (Japan); Conselho Nacional de Desenvolvimento Cientifico e Tecnologico; Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (Brazil); Natural Science Foundation of China (P. R. China); Ministry of Education, Youth and Sports (Czech Republic); Centre National de la Recherche Scientifique; Commissariat a l'Energie Atomique; Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung; Deutscher Akademischer Austausch dienst; Alexander von Humboldt Stiftung (Germany); Hungarian National Science Fund; OTKA (Hungary); Department of Atomic Energy and Department of Science and Technology (India); Israel Science Foundation (Israel); National Research Foundation; WCU program of the Ministry Education Science and Technology (Korea); Physics Department, Lahore University of Management Sciences (Pakistan); Ministry of Education and Science, Russian Academy of Sciences, Federal Agency of Atomic Energy (Russia); VR and Wallenberg Foundation (Sweden); US Civilian Research and Development Foundation for the Independent States of the Former Soviet Union; US-Hungarian Fulbright Foundation for Educational Exchange; US-Israel Binational Science Foundation FX We thank the staff of the Collider-Accelerator and Physics Departments at Brookhaven National Laboratory and the staff of the other PHENIX participating institutions for their vital contributions. We acknowledge support from the Office of Nuclear Physics in the Office of Science of the Department of Energy, the National Science Foundation, Abilene Christian University Research Council, Research Foundation of SUNY, and Dean of the College of Arts and Sciences, Vanderbilt University (USA), Ministry of Education, Culture, Sports, Science, and Technology and the Japan Society for the Promotion of Science (Japan), Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (Brazil), Natural Science Foundation of China (P. R. China), Ministry of Education, Youth and Sports (Czech Republic), Centre National de la Recherche Scientifique, Commissariat a l'Energie Atomique, and Institut National de Physique Nucleaire et de Physique des Particules (France), Bundesministerium fur Bildung und Forschung, Deutscher Akademischer Austausch dienst, and Alexander von Humboldt Stiftung (Germany), Hungarian National Science Fund, OTKA (Hungary), Department of Atomic Energy and Department of Science and Technology (India), Israel Science Foundation (Israel), National Research Foundation and WCU program of the Ministry Education Science and Technology (Korea), Physics Department, Lahore University of Management Sciences (Pakistan), Ministry of Education and Science, Russian Academy of Sciences, Federal Agency of Atomic Energy (Russia), VR and Wallenberg Foundation (Sweden), the US Civilian Research and Development Foundation for the Independent States of the Former Soviet Union, the US-Hungarian Fulbright Foundation for Educational Exchange, and the US-Israel Binational Science Foundation. NR 43 TC 8 Z9 8 U1 5 U2 33 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JAN 26 PY 2015 VL 91 IS 1 AR 014907 DI 10.1103/PhysRevC.91.014907 PG 18 WC Physics, Nuclear SC Physics GA CA1NE UT WOS:000348678400004 ER PT J AU Gross, F AF Gross, Franz TI Covariant spectator theory of np scattering: Deuteron quadrupole moment SO PHYSICAL REVIEW C LA English DT Article ID ENERGY; EQUATIONS AB The deuteron quadrupole moment is calculated using two covariant spectator theory model wave functions obtained from the 2007 high-precision fits to np scattering data. Included in the calculation are a new class of isoscalar np interaction currents automatically generated by the nuclear force model used in these fits. The prediction for model WJC-1, with larger relativistic P-state components, is 2.5% smaller than the experimental result, in common with the inability of models prior to 2014 to predict this important quantity. However, model WJC-2, with very small P-state components, gives agreement to better than 1%, similar to the results obtained recently from chiral effective field theory predictions to next-to-next-to-next-to-leading order. C1 [Gross, Franz] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Gross, Franz] Coll William & Mary, Williamsburg, VA 23185 USA. RP Gross, F (reprint author), Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. FU Jefferson Science Associates, LLC, under US DOE [DE-AC05-06OR23177] FX It is a pleasure to thank Rocco Schiavilla for stimulating conversations about the chi EFT predictions. This material is based upon work supported by the Jefferson Science Associates, LLC, under US DOE Contract No. DE-AC05-06OR23177. NR 21 TC 3 Z9 3 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JAN 26 PY 2015 VL 91 IS 1 AR 014005 DI 10.1103/PhysRevC.91.014005 PG 16 WC Physics, Nuclear SC Physics GA CA1NE UT WOS:000348678400001 ER PT J AU Buhot, J Measson, MA Gallais, Y Cazayous, M Sacuto, A Bourdarot, F Raymond, S Lapertot, G Aoki, D Regnault, LP Ivanov, A Piekarz, P Parlinski, K Legut, D Homes, CC Lejay, P Lobo, RPSM AF Buhot, J. Measson, M. A. Gallais, Y. Cazayous, M. Sacuto, A. Bourdarot, F. Raymond, S. Lapertot, G. Aoki, D. Regnault, L. P. Ivanov, A. Piekarz, P. Parlinski, K. Legut, D. Homes, C. C. Lejay, P. Lobo, R. P. S. M. TI Lattice dynamics of the heavy-fermion compound URu2Si2 SO PHYSICAL REVIEW B LA English DT Article ID HIDDEN-ORDER; SYSTEM URU2SI2; MAGNETIC EXCITATIONS; SYMMETRY-BREAKING; RAMAN-SCATTERING; SUPERCONDUCTOR URU2SI2; PHASE; TRANSITIONS; PHONONS; SAMPLES AB We report a comprehensive investigation of the lattice dynamics of URu2Si2 as a function of temperature using Raman scattering, optical conductivity, and inelastic neutron scattering measurements as well as theoretical ab initio calculations. The main effects on the optical phonon modes are related to Kondo physics. The B-1g (Gamma(3) symmetry) phonon mode slightly softens below similar to 100 K, in connection with the previously reported softening of the elastic constant, C-11-C-12, of the same symmetry, both observations suggesting a B-1g symmetry-breaking instability in the Kondo regime. Through optical conductivity, we detect clear signatures of strong electron-phonon coupling, with temperature-dependent spectral weight and Fano line shape of some phonon modes. Surprisingly, the line shapes of two phonon modes, E-u(1) and A(2u)(2), show opposite temperature dependencies. The A(2u)(2) mode loses its Fano shape below 150 K, whereas the E-u(1) mode acquires it below 100 K, in the Kondo crossover regime. This may point to momentum-dependent Kondo physics. By inelastic neutron-scattering measurements we have drawn the full dispersion of the phonon modes between 300 and 2 K. No remarkable temperature dependence has been obtained, including through the hidden order transition. Ab initio calculations with the spin-orbit coupling are in good agreement with the data except for a few low-energy branches with propagation in the (a, b) plane. C1 [Buhot, J.; Measson, M. A.; Gallais, Y.; Cazayous, M.; Sacuto, A.] Univ Paris Diderot, CNRS, Lab Mat & Phenomenes Quant, UMR 7162, F-75205 Paris 13, France. [Bourdarot, F.; Raymond, S.; Lapertot, G.; Aoki, D.; Regnault, L. P.] UJF Grenoble 1, SPSMS, UMR E CEA, INAC, F-38054 Grenoble, France. [Ivanov, A.] Inst Max Von Laue Paul Langevin, F-38042 Grenoble, France. [Piekarz, P.; Parlinski, K.] Polish Acad Sci, Inst Nucl Phys, PL-31342 Krakow, Poland. [Legut, D.] VSB Tech Univ Ostrava, Ctr IT4Innovat, Ostrava, Czech Republic. [Homes, C. C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Lejay, P.] CNRS, Inst Neel, F-38042 Grenoble 9, France. [Lejay, P.] Univ Grenoble 1, F-38042 Grenoble 9, France. [Lobo, R. P. S. M.] PSL Res Univ, LPEM, ESPCI ParisTech, F-75231 Paris 5, France. [Lobo, R. P. S. M.] CNRS, UMR 8213, F-75005 Paris, France. [Lobo, R. P. S. M.] Univ Paris 06, Sorbonne Univ, F-75005 Paris, France. RP Buhot, J (reprint author), Univ Paris Diderot, CNRS, Lab Mat & Phenomenes Quant, UMR 7162, Bat Condorcet, F-75205 Paris 13, France. EM marie_aude.measson@univ-paris-diderot.fr RI Measson, Marie-aude/E-6388-2015; Gallais, Yann/E-5240-2011; Aoki, Dai/K-3673-2012; Sacuto, Alain/L-2620-2016; OI Measson, Marie-aude/0000-0002-6495-7376; Gallais, Yann/0000-0002-0589-1522; Aoki, Dai/0000-0003-2334-8360; Sacuto, Alain/0000-0002-8351-6154; Lobo, Ricardo/0000-0003-2355-6856 FU Labex SEAM [ANR-11-IDEX-0005-02]; French Agence Nationale de la Recherche (ANR PRINCESS); US Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-98CH10886] FX This work was supported by the Labex SEAM (Grant No. ANR-11-IDEX-0005-02) and by the French Agence Nationale de la Recherche (ANR PRINCESS). C.C.H. is supported by the US Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Contract No. DE-AC02-98CH10886. The IT4Innovations National Supercomputing Center, VSB-Technical University, Ostrava, Czech Republic, is acknowledged for providing the computer facilities under Grant Reg. No. CZ.1.05/1.1.00/02.0070. We thank I. Paul, G. Knebel, C. Lacroix, and P. Oppeneer for very fruitful discussions. NR 61 TC 5 Z9 5 U1 9 U2 49 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JAN 26 PY 2015 VL 91 IS 3 AR 035129 DI 10.1103/PhysRevB.91.035129 PG 13 WC Physics, Condensed Matter SC Physics GA AZ8OU UT WOS:000348475700003 ER PT J AU Butch, NP Manley, ME Jeffries, JR Janoschek, M Huang, K Maple, MB Said, AH Leu, BM Lynn, JW AF Butch, Nicholas P. Manley, Michael E. Jeffries, Jason R. Janoschek, Marc Huang, Kevin Maple, M. Brian Said, Ayman H. Leu, Bogdan M. Lynn, Jeffrey W. TI Symmetry and correlations underlying hidden order in URu2Si2 SO PHYSICAL REVIEW B LA English DT Article ID SPIN-DENSITY-WAVE; ELECTRON SUPERCONDUCTOR URU2SI2; HEAVY-FERMION COMPOUNDS; TEMPERATURE PHASE-DIAGRAM; NEUTRON-SCATTERING; COMPOUND URU2SI2; SYSTEM URU2SI2; MAGNETIC EXCITATIONS; POSSIBLE MECHANISM; ANDERSON LATTICE AB We experimentally investigate the symmetry in the hidden order (HO) phase of intermetallic URu2Si2 by mapping the lattice and magnetic excitations via inelastic neutron and x-ray scattering measurements in the HO and high-temperature paramagnetic phases. At all temperatures, the excitations respect the zone edges of the body-centered tetragonal paramagnetic phase, showing no signs of reduced spatial symmetry, even in the HO phase. The magnetic excitations originate from transitions between hybridized bands and track the Fermi surface, whose features are corroborated by the phonon measurements. Due to a large hybridization energy scale, a full uranium moment persists in the HO phase, consistent with a lack of observed crystal-field-split states. Our results are inconsistent with local order-parameter models and the behavior of typical density waves. We suggest that an order parameter that does not break spatial symmetry would naturally explain these characteristics. C1 [Butch, Nicholas P.] Univ Maryland, Dept Phys, Ctr Nanophys & Adv Mat, College Pk, MD 20742 USA. [Butch, Nicholas P.; Lynn, Jeffrey W.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Butch, Nicholas P.; Jeffries, Jason R.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Manley, Michael E.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Janoschek, Marc] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Janoschek, Marc; Huang, Kevin; Maple, M. Brian] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Said, Ayman H.; Leu, Bogdan M.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Butch, NP (reprint author), Univ Maryland, Dept Phys, Ctr Nanophys & Adv Mat, College Pk, MD 20742 USA. EM nicholas.butch@nist.gov RI Janoschek, Marc/M-8871-2015; Manley, Michael/N-4334-2015 OI Janoschek, Marc/0000-0002-2943-0173; FU U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division FX We would like to thank J. W. Allen, P. Chandra, P. Coleman, J. A. Mydosh, P. M. Oppeneer, T. Shibauchi, F. Weber, C. M. Varma, L. A. Wray, and T. Yanagisawa for valuable discussions and F. Bourdarot for sharing his unpublished data. We are particularly grateful to J. D. Denlinger for sharing his unpublished data and insight over the course of this study. N. P. B. acknowledges support by CNAM and the LLNL PLS directorate. M. E. M. was sponsored in part by the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division. J. R. J. is partially supported by the Science Campaign. M. J. gratefully acknowledges support by the Alexander von Humboldt Foundation. Portions of this work were performed under LDRD (Tracking Code 14-ERD-041). This work utilized facilities supported in part by the National Science Foundation under Agreement No. DMR-0944772. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U. S. DOE under Contract No. DE-AC02-06CH11357. The construction of HERIX was partially supported by the NSF under Grant No. DMR-0115852. L. L. N. L. is operated by Lawrence Livermore National Security, LLC, for the DOE, NNSA under Contract No. DE-AC52-07NA27344. Crystal growth at UCSD was supported by the U. S. DOE Grant No. DE-FG02-04ER46105. NR 114 TC 11 Z9 11 U1 3 U2 32 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JAN 26 PY 2015 VL 91 IS 3 AR 035128 DI 10.1103/PhysRevB.91.035128 PG 15 WC Physics, Condensed Matter SC Physics GA AZ8OU UT WOS:000348475700002 ER PT J AU Ma, J Lee, JH Hahn, SE Hong, T Cao, HB Aczel, AA Dun, ZL Stone, MB Tian, W Qiu, Y Copley, JRD Zhou, HD Fishman, RS Matsuda, M AF Ma, J. Lee, J. H. Hahn, S. E. Hong, Tao Cao, H. B. Aczel, A. A. Dun, Z. L. Stone, M. B. Tian, W. Qiu, Y. Copley, J. R. D. Zhou, H. D. Fishman, R. S. Matsuda, M. TI Strong competition between orbital ordering and itinerancy in a frustrated spinel vanadate SO PHYSICAL REVIEW B LA English DT Article AB The crossover from localized to itinerant electron regimes in the geometrically frustrated spinel system Mn1-x CoxV2O4 is explored by neutron-scattering measurements, first-principles calculations, and spin models. At low Co doping, the orbital ordering (OO) of the localized V3+ spins suppresses magnetic frustration by triggering a tetragonal distortion. At high Co doping levels, however, electronic itinerancy melts the OO and lessens the structural and magnetic anisotropies, thus increasing the amount of geometric frustration for the V-site pyrochlore lattice. Contrary to the predicted paramagentism induced by chemical pressure, the measured noncollinear spin states in the Co-rich region of the phase diagram provide a unique platform where localized spins and electronic itinerancy compete in a geometrically frustrated spinel. C1 [Ma, J.; Hahn, S. E.; Hong, Tao; Cao, H. B.; Aczel, A. A.; Stone, M. B.; Tian, W.; Matsuda, M.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Lee, J. H.; Fishman, R. S.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Dun, Z. L.; Zhou, H. D.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Qiu, Y.; Copley, J. R. D.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Qiu, Y.] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. RP Fishman, RS (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM fishmanrs@ornl.gov; matsudam@ornl.gov RI Hong, Tao/F-8166-2010; Ma, Jie/C-1637-2013; Aczel, Adam/A-6247-2016; Cao, Huibo/A-6835-2016; Matsuda, Masaaki/A-6902-2016; Dun, Zhiling/F-5617-2016; Zhou, Haidong/O-4373-2016; Tian, Wei/C-8604-2013; Stone, Matthew/G-3275-2011 OI Hong, Tao/0000-0002-0161-8588; Aczel, Adam/0000-0003-1964-1943; Cao, Huibo/0000-0002-5970-4980; Matsuda, Masaaki/0000-0003-2209-9526; Dun, Zhiling/0000-0001-6653-3051; Tian, Wei/0000-0001-7735-3187; Hahn, Steven/0000-0002-2018-7904; Stone, Matthew/0000-0001-7884-9715 FU Scientific User Facilities Division; Materials Science and Engineering Division; Office of Basic Energy Sciences; US Department of Energy; Laboratory's Director's fund; NSF-DMR [DMR-1350002]; National Science Foundation [DMR-0944772] FX The research at HFIR and SNS, ORNL, were sponsored by the Scientific User Facilities Division (J.M., J.H.L, S.E.H., T.H., H.B.C., A.A.A., M.S., W.T., M.M.) and Materials Science and Engineering Division (J.H.L., R.F.), Office of Basic Energy Sciences, US Department of Energy. S.E.H. acknowledges support by the Laboratory's Director's fund, ORNL. Z. L. D and H. D. Z. thank the support from NSF-DMR through Award DMR-1350002. Work at NIST is supported in part by the National Science Foundation under Agreement No. DMR-0944772. The authors acknowledge valuable discussions with S. Okamoto and G. MacDougall. NR 34 TC 6 Z9 6 U1 4 U2 36 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 26 PY 2015 VL 91 IS 2 AR 020407 DI 10.1103/PhysRevB.91.020407 PG 5 WC Physics, Condensed Matter SC Physics GA AZ8OF UT WOS:000348474200002 ER PT J AU Jin, XY Kuramashi, Y Nakamura, Y Takeda, S Ukawa, A AF Jin, Xiao-Yong Kuramashi, Yoshinobu Nakamura, Yoshifumi Takeda, Shinji Ukawa, Akira TI Critical endpoint of the finite temperature phase transition for three flavor QCD SO PHYSICAL REVIEW D LA English DT Article ID HYBRID MONTE-CARLO; CHIRAL CRITICAL-POINT; LATTICE QCD; ALGORITHM; QUARKS AB We investigate the critical endpoint of finite temperature phase transition of Nf = 3 QCD at zero chemical potential. We employ the renormalization-group improved Iwasaki gauge action and non-perturbatively O(a)-improved Wilson-clover fermion action. The critical endpoint is determined by using the intersection point of kurtosis for the temporal size N-t = 4, 6, 8. Spatial sizes of N-l = 6-16 (N-t = 4), 10-24 (N-t = 6), and 12-24 (N-t = 8) are employed. We find that N-t = 4 is out of the scaling region. Using results for N-t = 6 and 8 and making linear extrapolations in 1/N-t(2), we obtain root t(0)T(E) = 0.0988(14)(9), root t(0) m(PS,E) = 0.2274(52)(108), and m(PS,E)/T-E = 2.302(62)(13), where the first error is statistical error, the second error is systematic error, and m(PS) is the pseudoscalar meson mass. If one uses 1/root t(0) = 1.347(30) GeV, as reported by Borsanyi et al., one finds T-E = 133(2)(1)(3) MeV, m(PS,E) = 306(7)(14)(7) MeV, and m(PS,E)/m(PS)(phys,sym) = 0.745(17)(35)(17), where the third error comes from the error of root t(0) and m(PS)(phys,sym) =root(m(pi)(2) + 2m(k)(2))/3. Our current estimation of root t(0) m(PS,E) in the continuum limit is about 25% smaller than the SU(3) symmetric point. C1 [Jin, Xiao-Yong; Kuramashi, Yoshinobu; Nakamura, Yoshifumi; Takeda, Shinji; Ukawa, Akira] RIKEN, Adv Inst Computat Sci, Kobe, Hyogo 6500047, Japan. [Kuramashi, Yoshinobu] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki 3058571, Japan. [Kuramashi, Yoshinobu] Univ Tsukuba, Ctr Computat Sci, Tsukuba, Ibaraki 3058577, Japan. [Nakamura, Yoshifumi] Kobe Univ, Grad Sch Syst Informat, Dept Computat Sci, Kobe, Hyogo 6578501, Japan. [Takeda, Shinji] Kanazawa Univ, Inst Phys, Kanazawa, Ishikawa 9201192, Japan. RP Jin, XY (reprint author), Argonne Natl Lab, Argonne Leadership Comp Facil, 9700 S Cass Ave, Argonne, IL 60439 USA. EM nakamura@riken.jp RI Ukawa, Akira/A-6549-2011; Nakamura, Yoshifumi/C-4630-2016; Kuramashi, Yoshinobu /C-8637-2016; Jin, Xiao-Yong/R-7694-2016 OI Jin, Xiao-Yong/0000-0002-2346-6861 FU HPCI System Research Project [hp120115]; Ministry of Education, Culture, Sports, Science and Technology [26800130] FX The Berlin QCD code [ 15] was used in this work. Our calculations were carried out on the K computer provided by the RIKEN Advanced Institute for Computational Science, HA8000 and FX10 at the University of Tokyo, HA8000-tc/HT210 and FX10 at Kyushu University, and Cray XC30 with Xeon Phi at Kyoto University. This research came about through the HPCI System Research Project (Project No. hp120115), FX10 at the University of Tokyo and Kyushu University, HA8000 at the University of Tokyo through the HPCI System Research Project (Project No. hp130092), and System E at Kyoto University through the HPCI System Research Project (Project No. hp140180). This work was supported by Large Scale Simulation Program Grants No. 12/13-13 (FY2012-2013) and No. 13/14-12 (FY2013-2014) of the High Energy Accelerator Research Organization (KEK). Part of this work was supported by the Grants-in-Aid for Scientific Research from the Ministry of Education, Culture, Sports, Science and Technology (Grant No. 26800130). NR 24 TC 9 Z9 9 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JAN 26 PY 2015 VL 91 IS 1 AR 014508 DI 10.1103/PhysRevD.91.014508 PG 17 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CA1NJ UT WOS:000348678900003 ER PT J AU Saravanan, K Jarry, A Kostecki, R Chen, GY AF Saravanan, Kuppan Jarry, Angelique Kostecki, Robert Chen, Guoying TI A study of room-temperature LixMn1.5Ni0.5O4 solid solutions SO SCIENTIFIC REPORTS LA English DT Article ID LI-ION BATTERIES; RECHARGEABLE LITHIUM BATTERIES; SYNCHROTRON X-RAY; 5 V; CATHODE MATERIALS; ELECTRODE MATERIALS; SOLUTION PHASES; OXIDE SPINEL; LINI0.5MN1.5O4; INSERTION AB Understanding the kinetic implication of solid-solution vs. biphasic reaction pathways is critical for the development of advanced intercalation electrode materials. Yet this has been a long-standing challenge in materials science due to the elusive metastable nature of solid solution phases. The present study reports the synthesis, isolation, and characterization of room-temperature LixMn1.5Ni0.5O4 solid solutions. In situ XRD studies performed on pristine and chemically-delithiated, micron-sized single crystals reveal the thermal behavior of LixMn1.5Ni0.5O4 (0 <= x <= 1) cathode material consisting of three cubic phases: LiMn1.5Ni0.5O4 (Phase I), Li0.5Mn1.5Ni0.5O4 (Phase II) and Mn1.5Ni0.5O4 (Phase III). A phase diagram capturing the structural changes as functions of both temperature and Li content was established. The work not only demonstrates the possibility of synthesizing alternative electrode materials that are metastable in nature, but also enables in-depth evaluation on the physical, electrochemical and kinetic properties of transient intermediate phases and their role in battery electrode performance. C1 [Saravanan, Kuppan; Jarry, Angelique; Kostecki, Robert; Chen, Guoying] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Chen, GY (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM gchen@lbl.gov OI kuppan, saravanan/0000-0003-4976-4514 FU Stanford Synchrotron Radiation Lightsource, a Directorate of SLAC National Accelerator Laboratory; Office of Science User Facility; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of FreedomCAR and Vehicle Technologies of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors acknowledge the support of Stanford Synchrotron Radiation Lightsource, a Directorate of SLAC National Accelerator Laboratory and an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Stanford University. We thank Drs. Marca Doeff, Feng Lin, Ryan Davis, Doug Van Campen and Chad Miller for assisting with the synchrotron experiments, and Drs. Thomas Richardson and Hugues Duncan for helpful discussion. This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of FreedomCAR and Vehicle Technologies of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 43 TC 6 Z9 6 U1 4 U2 90 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 26 PY 2015 VL 5 AR 8027 DI 10.1038/srep08027 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AZ5XM UT WOS:000348291800014 PM 25619504 ER PT J AU Yang, XF Liu, CX Fang, YL Hinkle, R Li, HY Bailey, V Bond-Lamberty, B AF Yang, Xiaofan Liu, Chongxuan Fang, Yilin Hinkle, Ross Li, Hong-Yi Bailey, Vanessa Bond-Lamberty, Ben TI Simulations of ecosystem hydrological processes using a unified multi-scale model SO ECOLOGICAL MODELLING LA English DT Article DE Multi-scale modelling; Computational fluid dynamics; Groundwater flow; Groundwater and surface water interactions ID SUBSURFACE FLOWS; SURFACE; SOILS; WETLANDS; SCALE AB This paper presents a unified multi-scale model (UMSM) that we developed to simulate hydrological processes in an ecosystem containing both surface water and groundwater. The UMSM approach modifies the Navier-Stokes equation by adding a Darcy force term to formulate a single set of equations to describe fluid momentum and uses a generalized equation to describe fluid mass balance. The advantage of the approach is that the single set of the equations can describe hydrological processes in both surface water and groundwater where different models are traditionally required to simulate fluid flow. This feature of the UMSM significantly facilitates modelling of hydrological processes in ecosystems, especially at locations where soil/sediment may be frequently inundated and drained in response to precipitation, regional hydrological and climate changes. In this paper, the UMSM was benchmarked using WASH123D, a model commonly used for simulating coupled surface water and groundwater flow. Disney Wilderness Preserve (DWP) site at the Kissimmee, Florida, where active field monitoring and measurements are ongoing to understand hydrological and biogeochemical processes, was then used as an example to illustrate the UMSM modelling approach. The simulations results demonstrated that the DWP site is subject to the frequent changes in soil saturation, the geometry and volume of surface water bodies, and groundwater and surface water exchange. All the hydrological phenomena in surface water and groundwater components including inundation and draining, river bank flow, groundwater table change, soil saturation, hydrological interactions between groundwater and surface water, and the migration of surface water and groundwater interfaces can be simultaneously simulated using the UMSM. Overall, the UMSM offers a cross-scale approach that is particularly suitable to simulate coupled surface and ground water flow in ecosystems with strong surface water and groundwater interactions. (C) 2014 Elsevier B.V. All rights reserved. C1 [Yang, Xiaofan; Liu, Chongxuan; Fang, Yilin; Li, Hong-Yi; Bailey, Vanessa; Bond-Lamberty, Ben] Pacific NW Natl Lab, Richland, WA 99352 USA. [Hinkle, Ross] Univ Cent Florida, Orlando, FL 32816 USA. RP Liu, CX (reprint author), 3335 Innovat St, Richland, WA 99354 USA. EM Chongxuan.Liu@pnnl.gov RI Bond-Lamberty, Ben/C-6058-2008; Liu, Chongxuan/C-5580-2009; Fang, Yilin/J-5137-2015; Li, Hong-Yi/C-9143-2014; Yang, Xiaofan/L-6472-2015; OI Bond-Lamberty, Ben/0000-0001-9525-4633; Li, Hong-Yi/0000-0001-5690-3610; Yang, Xiaofan/0000-0003-4514-0229; Bailey, Vanessa/0000-0002-2248-8890 FU US Department of Energy (DOE) Biological and Environmental Research (BER) Division through Terrestrial Ecosystem Science (TES) program; DOE Earth System Modelling program; Battelle Memorial Institute [DE-AC06-76RLO 1830] FX This research was supported by the US Department of Energy (DOE) Biological and Environmental Research (BER) Division through the Terrestrial Ecosystem Science (TES) program. H. Li was supported by the DOE Earth System Modelling program. Part of the research was performed at Environmental Molecular Science Laboratory (EMSL), a DOE National user facility located at Pacific Northwest National Laboratory (PNNL). PNNL is operated by Battelle Memorial Institute under subcontract DE-AC06-76RLO 1830. NR 30 TC 2 Z9 2 U1 3 U2 27 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-3800 EI 1872-7026 J9 ECOL MODEL JI Ecol. Model. PD JAN 24 PY 2015 VL 296 BP 93 EP 101 DI 10.1016/j.ecolmodel.2014.10.032 PG 9 WC Ecology SC Environmental Sciences & Ecology GA AX5FX UT WOS:000346953200008 ER PT J AU Wright, AF Modine, NA AF Wright, A. F. Modine, N. A. TI Application of the bounds-analysis approach to arsenic and gallium antisite defects in gallium arsenide SO PHYSICAL REVIEW B LA English DT Article ID 1ST-PRINCIPLES CALCULATIONS; ELECTRON-GAS; TOTAL-ENERGY; GAAS; STATE; EL2; EXPLANATION; ACCEPTOR; SILICON; POINTS AB A recently developed bounds-analysis approach has been used to interpret density-functional-theory (DFT) results for the As and Ga antisites in GaAs. The bounds analysis and subsequent processing of DFT results for the As antisite yielded levels-defined as the Fermi levels at which the defect charge state changes-in very good agreement with measurements, including the -1/0 level which is within 0.1 eV of the conduction-band edge. Good agreement was also obtained for the activation energies to transform the As-Ga from its metastable state to its stable state. For the Ga antisite, the bounds analysis revealed that the -1 and 0 charge states are hole states weakly bound to a localized -2 charge state. The calculated levels are in good agreement with measurements. C1 [Wright, A. F.; Modine, N. A.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Wright, AF (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. FU US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was performed, in part, at the Center for Integrated Nanotechnologies, a US Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. The authors wish to thank S. R. Lee and W. R. Wampler at Sandia National Laboratories for helpful discussions. NR 38 TC 6 Z9 6 U1 1 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 23 PY 2015 VL 91 IS 1 AR 014110 DI 10.1103/PhysRevB.91.014110 PG 8 WC Physics, Condensed Matter SC Physics GA CB1XQ UT WOS:000349421700001 ER PT J AU Butter, D Gaillard, MK AF Butter, Daniel Gaillard, Mary K. TI ANOMALY STRUCTURE OF REGULARIZED SUPERGRAVITY SO PHYSICAL REVIEW D LA English DT Article ID YANG-MILLS THEORIES; CHERN-SIMONS FORMS; GAUGE COUPLINGS; FIELD-THEORIES; ONE-LOOP; STRING THEORY; LINEAR MULTIPLETS; WARD IDENTITIES; CHIRAL MATTER; SIGMA-MODEL AB On-shell Pauli-Villars regularization of the one-loop divergences of supergravity theories is used to study the anomaly structure of supergravity and the cancellation of field theory anomalies under a U(1) gauge transformation and under the T-duality group of modular transformations in effective supergravity theories with three Kahler moduli T-i obtained from orbifold compactification of the weakly coupled heterotic string. This procedure requires constraints on the chiral matter representations of the gauge group that are consistent with known results from orbifold compactifications. Pauli-Villars (PV) regulator fields allow for the cancellation of all quadratic and logarithmic divergences, as well as most linear divergences. If all linear divergences were canceled, the theory would be anomaly free, with noninvariance of the action arising only from Pauli-Villars masses. However there are linear divergences associated with nonrenormalizable gravitino/gaugino interactions that cannot be canceled by PV fields. The resulting chiral anomaly forms a supermultiplet with the corresponding conformal anomaly, provided the ultraviolet cutoff has the appropriate field dependence, in which case total derivative terms, such as Gauss-Bonnet, do not drop out from the effective action. The anomalies can be partially canceled by the four-dimensional version of the Green-Schwarz mechanism, but additional counterterms, and/or a more elaborate set of Pauli-Villars fields and couplings, are needed to cancel the full anomaly, including D-term contributions to the conformal anomaly that are nonlinear in the parameters of the anomalous transformations. C1 [Butter, Daniel] Nikhef Theory Grp, NL-1098 XG Amsterdam, Netherlands. [Gaillard, Mary K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Phys, Berkeley, CA 94720 USA. [Gaillard, Mary K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. RP Butter, D (reprint author), Nikhef Theory Grp, Sci Pk 105, NL-1098 XG Amsterdam, Netherlands. FU Office of Science, Office of High Energy and Nuclear Physics, Division of High Energy Physics, of the U. S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [PHY-0457315, PHY-1002399, PHY-0098840]; Australian Research Council [DP1096372]; UWA Research Development Award; ERC [246974]; European Commission Marie Curie International Incoming Fellowship [PIIF-GA-2012-627976] FX We are happy to acknowledge the contributions of Andreas Birkedal, Choonseo Park, Matthijs Ransdorp, and Soo-Jong Rey to various early stages of this work. We thank Dan Freedman, Joel Giedt, Brent Nelson, Claudio Scrucca, Marco Serone, Tom Taylor, and Lewis Tunstall for discussions and helpful input. M. K. G. would like to thank the Kavli Institute of Physics at the University of California at Santa Barbara for hospitality during part of the completion of this work. This work was supported in part by the Director, Office of Science, Office of High Energy and Nuclear Physics, Division of High Energy Physics, of the U. S. Department of Energy under Contract No. DE-AC02-05CH11231, in part by the National Science Foundation under Grants No. PHY-0457315, No. PHY-1002399, and No. PHY-0098840, in part by the Australian Research Council (Grant No. DP1096372), in part by a UWA Research Development Award, by the ERC Advanced Grant No. 246974, "Supersymmetry: a window to non-perturbative physics" and by the European Commission Marie Curie International Incoming Fellowship Grant No. PIIF-GA-2012-627976. NR 58 TC 2 Z9 2 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JAN 23 PY 2015 VL 91 IS 2 AR 025015 DI 10.1103/PhysRevD.91.025015 PG 57 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CB2VG UT WOS:000349485800006 ER PT J AU Zhang, JJ Gao, JH Wang, XN AF Zhang, Jia Jun Gao, Jian-Hua Wang, Xin-Nian TI Higher-twist contributions to the transverse momentum broadening in semi-inclusive deep inelastic scattering off large nuclei SO PHYSICAL REVIEW D LA English DT Article ID MULTIPLE PARTON SCATTERING; ENERGY-LOSS; POWER CORRECTIONS; HADRONIC SCATTERING; QCD; DISTRIBUTIONS; OPACITY; QUARKS AB Multiple scattering leads to transverse momentum broadening of the struck quark in semi-inclusive deeply inelastic scatterings. Nuclear broadening of the transverse momentum squared at the leading twist is determined by the twist-four collinear quark-gluon correlation function of the target nucleus that is in turn related to the jet transport parameter inside the nuclear medium. The twist-six contributions to the transverse momentum broadening are calculated as power corrections similar to 1/Q(2). Such power corrections are found to have no extra nuclear enhancement beyond the twist-four matrix elements and are determined by the nuclear modification of collinear parton distribution and correlation functions. They become important for an accurate extraction of the jet transport parameter inside large nuclei and its scale evolution at intermediate values of the hard scale Q(2). C1 [Zhang, Jia Jun; Wang, Xin-Nian] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China. [Zhang, Jia Jun; Gao, Jian-Hua; Wang, Xin-Nian] Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China. [Gao, Jian-Hua] Shandong Univ, Inst Space Sci, Shandong Prov Key Lab Opt Astron & Solar Terr Env, Weihai 264209, Peoples R China. [Wang, Xin-Nian] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Nucl Sci Div, Berkeley, CA 94720 USA. RP Zhang, JJ (reprint author), Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China. RI Gao, Jianhua/O-9550-2014; OI Wang, Xin-Nian/0000-0002-9734-9967 FU Natural Science Foundation of China [11221504, 11105137, 11475104]; Chinese Ministry of Science and Technology [2014DFG02050]; Major State Basic Research Development Program in China [2014CB845406, 2014CB845404]; Office of Energy Research, Office of High Energy and Nuclear Physics, Division of Nuclear Physics, of the U.S. Department of Energy [DE-AC02-05CH11231]; CCNU-QLPL Innovation Fund [QLPL2014P01]; JET Collaboration FX We thank Dr. Hongxi Xing and Dr. Feng Yuan for helpful discussions and useful comments. This work is supported in part by Natural Science Foundation of China under Grants No. 11221504, No. 11105137 and No. 11475104, Chinese Ministry of Science and Technology under Grant No. 2014DFG02050, the Major State Basic Research Development Program in China (Grants No. 2014CB845406 and No. 2014CB845404), by the Director, Office of Energy Research, Office of High Energy and Nuclear Physics, Division of Nuclear Physics, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 and within the framework of the JET Collaboration. J.H.G. is also supported by CCNU-QLPL Innovation Fund (QLPL2014P01). NR 34 TC 2 Z9 2 U1 2 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JAN 23 PY 2015 VL 91 IS 1 AR 014026 DI 10.1103/PhysRevD.91.014026 PG 11 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CB2VB UT WOS:000349485300001 ER PT J AU Antonio, D Czaplewski, DA Guest, JR Lopez, D Arroyo, SI Zanette, DH AF Antonio, Dario Czaplewski, David A. Guest, Jeffrey R. Lopez, Daniel Arroyo, Sebastian I. Zanette, Damian H. TI Nonlinearity-Induced Synchronization Enhancement in Micromechanical Oscillators SO PHYSICAL REVIEW LETTERS LA English DT Article AB An autonomous oscillator synchronizes to an external harmonic force only when the forcing frequency lies within a certain interval-known as the synchronization range-around the oscillator's natural frequency. Under ordinary conditions, the width of the synchronization range decreases when the oscillation amplitude grows, which constrains synchronized motion of micro-and nanomechanical resonators to narrow frequency and amplitude bounds. Here, we show that nonlinearity in the oscillator can be exploited to manifest a regime where the synchronization range increases with increasing oscillation amplitude. Experimental data are provided for self-sustained micromechanical oscillators operating in this regime, and analytical results show that nonlinearities are the key determinants of this effect. Our results provide a new strategy to enhance the synchronization of micromechanical oscillators by capitalizing on their intrinsic nonlinear dynamics. C1 [Antonio, Dario; Czaplewski, David A.; Guest, Jeffrey R.; Lopez, Daniel] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Arroyo, Sebastian I.; Zanette, Damian H.] Ctr Atom Bariloche, RA-8400 San Carlos De Bariloche, Rio Negro, Argentina. [Arroyo, Sebastian I.; Zanette, Damian H.] Inst Balseiro, RA-8400 San Carlos De Bariloche, Rio Negro, Argentina. [Zanette, Damian H.] Consejo Nacl Invest Cient & Tecn, RA-1033 Buenos Aires, DF, Argentina. RP Antonio, D (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. RI Guest, Jeffrey/B-2715-2009; OI Guest, Jeffrey/0000-0002-9756-8801; Zanette, Damian/0000-0003-0681-0592 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; ANPCyT [PICT 2011-0545]; CONICET, Argentina [PIP 112-200801-76] FX Use of the Center for Nanoscale Materials at the Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. S. I. A. and D. H. Z. acknowledge financial support from ANPCyT (PICT 2011-0545) and CONICET (PIP 112-200801-76), Argentina. We thank J. Sader for helpful discussions. NR 16 TC 9 Z9 9 U1 0 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 23 PY 2015 VL 114 IS 3 AR 034103 DI 10.1103/PhysRevLett.114.034103 PG 5 WC Physics, Multidisciplinary SC Physics GA CB2WQ UT WOS:000349489600002 PM 25659001 ER PT J AU Sea, K Sohn, SH Durazo, A Sheng, YW Shaw, BF Cao, XH Taylor, AB Whitson, LJ Holloway, SP Hart, PJ Cabelli, DE Gralla, EB Valentine, JS AF Sea, Kevin Sohn, Se Hui Durazo, Armando Sheng, Yuewei Shaw, Bryan F. Cao, Xiaohang Taylor, Alexander B. Whitson, Lisa J. Holloway, Stephen P. Hart, P. John Cabelli, Diane E. Gralla, Edith Butler Valentine, Joan Selverstone TI Insights into the Role of the Unusual Disulfide Bond in Copper-Zinc Superoxide Dismutase SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article ID AMYOTROPHIC-LATERAL-SCLEROSIS; CU,ZN-SUPEROXIDE DISMUTASE; SACCHAROMYCES-CEREVISIAE; ATOMIC-RESOLUTION; PULSE-RADIOLYSIS; REDUCED FORM; METAL; AGGREGATION; YEAST; ALS AB The functional and structural significance of the intrasubunit disulfide bond in copper-zinc superoxide dismutase (SOD1) was studied by characterizing mutant forms of human SOD1 (hSOD) and yeast SOD1 lacking the disulfide bond. We determined x-ray crystal structures of metal-bound and metal-deficient hC57S SOD1. C57S hSOD1 isolated from yeast contained four zinc ions per protein dimer and was structurally very similar to wild type. The addition of copper to this four-zinc protein gave properly reconstituted 2Cu, 2Zn C57S hSOD, and its spectroscopic properties indicated that the coordination geometry of the copper was remarkably similar to that of holo wild type hSOD1. In contrast, the addition of copper and zinc ions to apo C57S human SOD1 failed to give proper reconstitution. Using pulse radiolysis, we determined SOD activities of yeast and human SOD1s lacking disulfide bonds and found that they were enzymatically active at similar to 10% of the wild type rate. These results are contrary to earlier reports that the intrasubunit disulfide bonds in SOD1 are essential for SOD activity. Kinetic studies revealed further that the yeast mutant SOD1 had less ionic attraction for superoxide, possibly explaining the lower rates. Saccharomyces cerevisiae cells lacking the sod1 gene do not grow aerobically in the absence of lysine, but expression of C57S SOD1 increased growth to 30-50% of the growth of cells expressing wild type SOD1, supporting that C57S SOD1 retained a significant amount of activity. C1 [Sea, Kevin; Sohn, Se Hui; Durazo, Armando; Sheng, Yuewei; Shaw, Bryan F.; Gralla, Edith Butler; Valentine, Joan Selverstone] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. [Sea, Kevin] Santa Rosa Jr Coll, Dept Wine Studies, Santa Rosa, CA 95401 USA. [Sohn, Se Hui] LG Chem Ltd, Taejon 305380, South Korea. [Durazo, Armando] Univ Arizona, Dept Chem & Environm Engn, Tucson, AZ 85721 USA. [Cabelli, Diane E.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Shaw, Bryan F.] Baylor Univ, Dept Chem & Biochem, Waco, TX 76798 USA. [Cao, Xiaohang; Taylor, Alexander B.; Whitson, Lisa J.; Holloway, Stephen P.; Hart, P. John] Univ Texas Hlth Sci Ctr San Antonio, Dept Biochem, San Antonio, TX 78229 USA. [Hart, P. John] South Texas Vet Hlth Care Syst, Dept Vet Affairs, San Antonio, TX 78229 USA. [Valentine, Joan Selverstone] Ewha Womans Univ, Dept Bioinspired Sci, Seoul 120750, South Korea. RP Sea, K (reprint author), Santa Rosa Jr Coll, Dept Wine Studies, 1501 Mendocino Ave, Santa Rosa, CA 95401 USA. EM kevinsea@yahoo.com; jsv@chem.ucla.edu RI Shaw, Bryan/A-7001-2008 FU National Institutes of Health [DK46828, GM28222, GM08496, NS39112]; Veterans Affairs [VA 101 BX00506]; U.S. Department of Energy Division of Chemical Sciences, Geosciences, and Biosciences [DE-AC02-98CH10886] FX This work was supported, in whole or in part, by National Institutes of Health Grants DK46828 and GM28222 (to J. S. V.), GM08496 (to K. S.), and NS39112 (to P. J. H.). This work was also supported by Veterans Affairs Grant VA 101 BX00506 (to P. J. H.) and Contract DE-AC02-98CH10886 from the U.S. Department of Energy Division of Chemical Sciences, Geosciences, and Biosciences (to Brookhaven National Laboratory). NR 63 TC 6 Z9 6 U1 3 U2 27 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD JAN 23 PY 2015 VL 290 IS 4 BP 2405 EP 2418 DI 10.1074/jbc.M114.588798 PG 14 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CA0EH UT WOS:000348588000043 PM 25433341 ER PT J AU Mahaffy, PR Webster, CR Stern, JC Brunner, AE Atreya, SK Conrad, PG Domagal-Goldman, S Eigenbrode, JL Flesch, GJ Christensen, LE Franz, HB Freissinet, C Glavin, DP Grotzinger, JP Jones, JH Leshin, LA Malespin, C McAdam, AC Ming, DW Navarro-Gonzalez, R Niles, PB Owen, T Pavlov, AA Steele, A Trainer, MG Williford, KH Wray, JJ AF Mahaffy, P. R. Webster, C. R. Stern, J. C. Brunner, A. E. Atreya, S. K. Conrad, P. G. Domagal-Goldman, S. Eigenbrode, J. L. Flesch, G. J. Christensen, L. E. Franz, H. B. Freissinet, C. Glavin, D. P. Grotzinger, J. P. Jones, J. H. Leshin, L. A. Malespin, C. McAdam, A. C. Ming, D. W. Navarro-Gonzalez, R. Niles, P. B. Owen, T. Pavlov, A. A. Steele, A. Trainer, M. G. Williford, K. H. Wray, J. J. CA Msl Sci Team TI The imprint of atmospheric evolution in the D/H of Hesperian clay minerals on Mars SO SCIENCE LA English DT Article ID MARTIAN ATMOSPHERE; TERRESTRIAL PLANETS; HYDROGEN ISOTOPES; WATER RESERVOIRS; GALE CRATER; ORIGIN; FRACTIONATION; CONSTRAINTS; DEUTERIUM; ABUNDANCE AB The deuterium-to-hydrogen (D/H) ratio in strongly bound water or hydroxyl groups in ancient martian clays retains the imprint of the water of formation of these minerals. Curiosity's Sample Analysis at Mars (SAM) experiment measured thermally evolved water and hydrogen gas released between 550 degrees and 950 degrees C from samples of Hesperian-era Gale crater smectite to determine this isotope ratio. The D/H value is 3.0 (+/- 0.2) times the ratio in standard mean ocean water. The D/H ratio in this similar to 3-billion-year-old mudstone, which is half that of the present martian atmosphere but substantially higher than that expected in very early Mars, indicates an extended history of hydrogen escape and desiccation of the planet. C1 [Mahaffy, P. R.; Stern, J. C.; Brunner, A. E.; Conrad, P. G.; Domagal-Goldman, S.; Eigenbrode, J. L.; Franz, H. B.; Freissinet, C.; Glavin, D. P.; Malespin, C.; McAdam, A. C.; Pavlov, A. A.; Trainer, M. G.] NASA, Planetary Environm Lab, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Webster, C. R.; Flesch, G. J.; Christensen, L. E.; Williford, K. H.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Brunner, A. E.] Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ 85281 USA. [Brunner, A. E.; Franz, H. B.] Univ Maryland, Ctr Res & Explorat Space Sci & Technol, College Pk, MD 20742 USA. [Atreya, S. K.] Univ Michigan, Dept Atmospher Ocean & Space Sci, Ann Arbor, MI 48109 USA. [Freissinet, C.] Oak Ridge Associated Univ, NASA, Postdoctoral Program, Oak Ridge, TN 37831 USA. [Grotzinger, J. P.] CALTECH, Div Geol & Planetary Sci, Pasadena, CA 91125 USA. [Jones, J. H.; Ming, D. W.; Niles, P. B.] NASA, Johnson Space Flight Ctr, Houston, TX 77058 USA. [Leshin, L. A.] Worcester Polytech Inst, Off President, Worcester, MA 01609 USA. [Malespin, C.] NASA, Goddard Earth Sci Technol & Res GESTAR, Univ Space Res Assoc USRA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Navarro-Gonzalez, R.] Univ Nacl Autonoma Mexico, Mexico City 04510, DF, Mexico. [Owen, T.] Univ Hawaii, Inst Astron, Honolulu, HI 96822 USA. [Steele, A.] Carnegie Inst Sci, Geophys Lab, Washington, DC 20015 USA. [Wray, J. J.] Georgia Inst Technol, Sch Earth & Atmospher Sci, Atlanta, GA 30332 USA. RP Mahaffy, PR (reprint author), NASA, Planetary Environm Lab, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. EM paul.r.mahaffy@nasa.gov RI Gonzalez, Rafael/D-1748-2009; Martin-Torres, Francisco Javier/G-6329-2015; Rodriguez-Manfredi, Jose/L-8001-2014; Glavin, Daniel/D-6194-2012; Harri, Ari-Matti/C-7142-2012; Wray, James/B-8457-2008; Zorzano, Maria-Paz/C-5784-2015; Trainer, Melissa/E-1477-2012; Lemmon, Mark/E-9983-2010; Merikallio, Sini/C-7812-2014; szopa, cyril/C-6865-2015; Ramos, Miguel/K-2230-2014; Zorzano, Maria-Paz/F-2184-2015; Dworkin, Jason/C-9417-2012 OI Martin-Torres, Francisco Javier/0000-0001-6479-2236; Rodriguez-Manfredi, Jose/0000-0003-0461-9815; Glavin, Daniel/0000-0001-7779-7765; Harri, Ari-Matti/0000-0001-8541-2802; Wray, James/0000-0001-5559-2179; Zorzano, Maria-Paz/0000-0002-4492-9650; Lemmon, Mark/0000-0002-4504-5136; Merikallio, Sini/0000-0001-7120-6127; szopa, cyril/0000-0002-0090-4056; Ramos, Miguel/0000-0003-3648-6818; Zorzano, Maria-Paz/0000-0002-4492-9650; Dworkin, Jason/0000-0002-3961-8997 FU NASA's Mars Exploration Program FX This work was supported by NASA's Mars Exploration Program. The dedicated teams that developed the SAM suite of instruments are acknowledged. All data described can be found in NASA's the Planetary Data System archive pds.nasa.gov. NR 45 TC 28 Z9 29 U1 7 U2 81 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JAN 23 PY 2015 VL 347 IS 6220 BP 412 EP 414 DI 10.1126/science.1260291 PG 3 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AZ4XZ UT WOS:000348225800040 PM 25515119 ER PT J AU Millot, M Dubrovinskaia, N Cernok, A Blaha, S Dubrovinsky, L Braun, DG Celliers, PM Collins, GW Eggert, JH Jeanloz, R AF Millot, M. Dubrovinskaia, N. Cernok, A. Blaha, S. Dubrovinsky, L. Braun, D. G. Celliers, P. M. Collins, G. W. Eggert, J. H. Jeanloz, R. TI Shock compression of stishovite and melting of silica at planetary interior conditions SO SCIENCE LA English DT Article ID SIO2; TEMPERATURES; CORES; PRESSURES; DYNAMICS; MGSIO3 AB Deep inside planets, extreme density, pressure, and temperature strongly modify the properties of the constituent materials. In particular, how much heat solids can sustain before melting under pressure is key to determining a planet's internal structure and evolution. We report laser-driven shock experiments on fused silica, alpha-quartz, and stishovite yielding equation-of-state and electronic conductivity data at unprecedented conditions and showing that the melting temperature of SiO2 rises to 8300 K at a pressure of 500 gigapascals, comparable to the core-mantle boundary conditions for a 5-Earth mass super-Earth. We show that mantle silicates and core metal have comparable melting temperatures above 500 to 700 gigapascals, which could favor long-lived magma oceans for large terrestrial planets with implications for planetary magnetic-field generation in silicate magma layers deep inside such planets. C1 [Millot, M.; Braun, D. G.; Celliers, P. M.; Collins, G. W.; Eggert, J. H.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Millot, M.; Jeanloz, R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Dubrovinskaia, N.] Univ Bayreuth, Crystallog Lab, D-95440 Bayreuth, Germany. [Cernok, A.; Blaha, S.; Dubrovinsky, L.] Univ Bayreuth, Bayer Geoinst, D-95440 Bayreuth, Germany. RP Millot, M (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM millot1@llnl.gov OI Millot, Marius/0000-0003-4414-3532 FU LLNL [DE-AC52-07NA27344]; German Research Foundation (Deutsche Forschungsgemeinschaft, DFG); Federal Ministry of Education and Research (BMBF, Germany) through DFG Heisenberg Program [DU 954-8/1]; BMBF [5K13WC3, O5K2013]; U.S. Department of Energy; University of California including UC Berkeley's Miller Institute for Basic Research in Science FX Data are available in the supplementary materials and upon request to millot1@llnl.gov. Authors gratefully acknowledge assistance of A. Correa Barrios, W. Unites, R. Wallace, C. Davis, and J. Emig, Lawrence Livermore National Laboratory (LLNL); R. Paguio, M. Farrell, and A. Nikroo, General Atomics; M. Bonino, D. Harding, and the entire Omega Laser staff at the Laboratory for Laser Energetics (LLE); H. Schulze, T. Boffa Ballaran, A. Audetat, and H. Fischer (Bayreuth University); and discussions with D. K. Spaulding, T. R. Boehly, and J. R. Rygg. Prepared by LLNL under contract DE-AC52-07NA27344. Omega shots were allocated by LLE Laboratory Basic Science program. N.D. thanks the German Research Foundation (Deutsche Forschungsgemeinschaft, DFG) and the Federal Ministry of Education and Research (BMBF, Germany) for financial support through the DFG Heisenberg Program and project no. DU 954-8/1 and the BMBF grant no. 5K13WC3 (Verbundprojekt O5K2013, Teilprojekt 2, PT-DESY). Partial support was provided by the U.S. Department of Energy and the University of California, including UC Berkeley's Miller Institute for Basic Research in Science. NR 29 TC 22 Z9 23 U1 13 U2 82 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JAN 23 PY 2015 VL 347 IS 6220 BP 418 EP 420 DI 10.1126/science.1261507 PG 3 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AZ4XZ UT WOS:000348225800042 PM 25613887 ER PT J AU Dolzhnikov, DS Zhang, H Jang, J Son, JS Panthani, MG Shibata, T Chattopadhyay, S Talapin, DV AF Dolzhnikov, Dmitriy S. Zhang, Hao Jang, Jaeyoung Son, Jae Sung Panthani, Matthew G. Shibata, Tomohiro Chattopadhyay, Soma Talapin, Dmitri V. TI Composition-matched molecular "solders" for semiconductors SO SCIENCE LA English DT Article ID FIELD-EFFECT TRANSISTORS; COLLOIDAL NANOCRYSTALS; SOLIDS; THERMOELECTRICS; REDUCTION; TRANSPORT; FILMS; PBS AB We propose a general strategy to synthesize largely unexplored soluble chalcogenidometallates of cadmium, lead, and bismuth. These compounds can be used as "solders" for semiconductors widely used in photovoltaics and thermoelectrics. The addition of solder helped to bond crystal surfaces and link nano-or mesoscale particles together. For example, CdSe nanocrystals with Na2Cd2Se3 solder was used as a soluble precursor for CdSe films with electron mobilities exceeding 300 square centimeters per volt-second. CdTe, PbTe, and Bi2Te3 powders were molded into various shapes in the presence of a small additive of composition-matched chalcogenidometallate or chalcogel, thus opening new design spaces for semiconductor technologies. C1 [Dolzhnikov, Dmitriy S.; Zhang, Hao; Jang, Jaeyoung; Son, Jae Sung; Panthani, Matthew G.; Talapin, Dmitri V.] Univ Chicago, Dept Chem, Chicago, IL 60637 USA. [Dolzhnikov, Dmitriy S.; Zhang, Hao; Jang, Jaeyoung; Son, Jae Sung; Panthani, Matthew G.; Talapin, Dmitri V.] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA. [Shibata, Tomohiro; Chattopadhyay, Soma] Argonne Natl Lab, MRCAT, Adv Photon Source, Sect 10, Argonne, IL 60439 USA. [Shibata, Tomohiro; Chattopadhyay, Soma] IIT, Dept Phys, Adv Mat Grp, Chicago, IL 60616 USA. [Talapin, Dmitri V.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Talapin, DV (reprint author), Univ Chicago, Dept Chem, 5735 S Ellis Ave, Chicago, IL 60637 USA. EM dvtalapin@uchicago.edu RI Son, Jae Sung/C-2903-2014; ID, MRCAT/G-7586-2011 FU II-VI Foundation; U.S. Department of Energy (DOE) SunShot program [DE-EE0005312]; NSF [DMR-1310398]; Keck Foundation; NSF Materials Research Science and Engineering Center Program [DMR 08-20054, DMR 14-20709]; DOE, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; DOE; MRCAT FX We thank S. Kwon and V. Zyryanov for help with EXAFS measurements and N. James for reading the manuscript. The work was supported by the II-VI Foundation, U.S. Department of Energy (DOE) SunShot program under award DE-EE0005312 and by NSF under award DMR-1310398. D.V.T. also thanks the Keck Foundation. This work used facilities supported by the NSF Materials Research Science and Engineering Center Program under awards DMR 08-20054 and DMR 14-20709. Use of the Center for Nanoscale Materials and Advanced Photon Source was supported by the DOE, Office of Science, Office of Basic Energy Sciences, under contract DE-AC02-06CH11357. MRCAT operations are supported by the DOE and MRCAT host institutions. NR 29 TC 47 Z9 47 U1 17 U2 123 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JAN 23 PY 2015 VL 347 IS 6220 BP 425 EP 428 DI 10.1126/science.1260501 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AZ4XZ UT WOS:000348225800044 PM 25569110 ER PT J AU Zhou, CZ Reichhardt, C Reichhardt, CJO Beyerlein, IJ AF Zhou, Caizhi Reichhardt, Charles Reichhardt, Cynthia J. Olson Beyerlein, Irene J. TI Dynamic Phases, Pinning, and Pattern Formation for Driven Dislocation Assemblies SO SCIENTIFIC REPORTS LA English DT Article ID FLUX-LINE-LATTICE; SUPERCONDUCTING VORTEX AVALANCHES; CHANNEL ANGULAR EXTRUSION; CRYSTAL PLASTICITY; FLOW; DEFORMATION; COPPER; SCALE; BURSTS; PASSES AB We examine driven dislocation assemblies and show that they can exhibit a set of dynamical phases remarkably similar to those of driven systems with quenched disorder such as vortices in superconductors, magnetic domain walls, and charge density wave materials. These phases include pinned-jammed, fluctuating, and dynamically ordered states, and each produces distinct dislocation patterns as well as specific features in the noise fluctuations and transport properties. Our work suggests that many of the results established for systems with quenched disorder undergoing plastic depinning transitions can be applied to dislocation systems, providing a new approach for understanding pattern formation and dynamics in these systems. C1 [Zhou, Caizhi] Missouri Univ Sci & Technol, Dept Mat Sci & Engn, Rolla, MO 65409 USA. [Zhou, Caizhi; Reichhardt, Charles; Reichhardt, Cynthia J. Olson; Beyerlein, Irene J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Reichhardt, CJO (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM cjrx@lanl.gov FU NNSA of the US DoE at LANL [DE-AC52-06NA25396]; UMRB funding FX We acknowledge helpful discussions with Karen Dahmen. This work was carried out under the auspices of the NNSA of the US DoE at LANL under Contract No. DE-AC52-06NA25396. C. Z. also received partial support from UMRB funding. NR 50 TC 2 Z9 2 U1 4 U2 17 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 23 PY 2015 VL 5 AR 8000 DI 10.1038/srep08000 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AZ5WA UT WOS:000348287600002 PM 25613839 ER PT J AU Shiau, CE Kaufman, Z Meireles, AM Talbot, WS AF Shiau, Celia E. Kaufman, Zoe Meireles, Ana M. Talbot, William S. TI Differential Requirement for irf8 in Formation of Embryonic and Adult Macrophages in Zebrafish SO PLOS ONE LA English DT Article ID CD8-ALPHA(+) DENDRITIC CELLS; SEQUENCE BINDING-PROTEIN; IN-VIVO; TRANSCRIPTION FACTORS; REGULATORY FACTOR-8; B-CELL; MICROGLIA; ICSBP; INFLAMMATION; PROGENITOR AB Interferon regulatory factor 8 (Irf8) is critical for mammalian macrophage development and innate immunity, but its role in teleost myelopoiesis remains incompletely understood. In particular, genetic tools to analyze the role of Irf8 in zebrafish macrophage development at larval and adult stages are lacking. We generated irf8 null mutants in zebrafish using TALEN-mediated targeting. Our analysis defines different requirements for irf8 at different stages. irf8 is required for formation of all macrophages during primitive and transient definitive hematopoiesis, but not during adult-phase definitive hematopoiesis starting at 5-6 days postfertilization. At early stages, irf8 mutants have excess neutrophils and excess cell death in pu.1-expressing myeloid cells. Macrophage fates were recovered in irf8 mutants after wildtype irf8 expression in neutrophil and macrophage lineages, suggesting that irf8 regulates macrophage specification and survival. In juvenile irf8 mutant fish, mature macrophages are present, but at numbers significantly reduced compared to wildtype, indicating an ongoing requirement for irf8 after embryogenesis. As development progresses, tissue macrophages become apparent in zebrafish irf8 mutants, with the possible exception of microglia. Our study defines distinct requirement for irf8 in myelopoiesis before and after transition to the adult hematopoietic system. C1 [Shiau, Celia E.; Kaufman, Zoe; Meireles, Ana M.; Talbot, William S.] Stanford Univ, Sch Med, Dept Dev Biol, Stanford, CA 94305 USA. RP Shiau, CE (reprint author), Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. EM shiauc@ornl.gov; wtalbot@stanford.edu RI Shiau, Celia/C-7679-2015 FU NIH NRSA fellowship [5F32NS067754]; ORNL Liane Russell Fellowship; Stanford Undergraduate VPUE funds; EMBO fellowship [ALTF 1125-2011]; NIH [R01 NS065787, R56 HL125040] FX C.E.S. was supported by NIH NRSA fellowship 5F32NS067754 and ORNL Liane Russell Fellowship, Z.K. was supported by Stanford Undergraduate VPUE funds, and A.M.M. was supported by EMBO fellowship ALTF 1125-2011. This work was supported by NIH grants R01 NS065787 and R56 HL125040 to W.S.T. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 43 TC 15 Z9 15 U1 0 U2 13 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JAN 23 PY 2015 VL 10 IS 1 AR UNSP e0117513 DI 10.1371/journal.pone.0117513 PG 15 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CA7UF UT WOS:000349122100063 PM 25615614 ER PT J AU Muchero, W Guo, J DiFazio, SP Chen, JG Ranjan, P Slavov, GT Gunter, LE Jawdy, S Bryan, AC Sykes, R Ziebell, A Klapste, J Porth, I Skyba, O Unda, F El-Kassaby, YA Douglas, CJ Mansfield, SD Martin, J Schackwitz, W Evans, LM Czarnecki, O Tuskan, GA AF Muchero, Wellington Guo, Jianjun DiFazio, Stephen P. Chen, Jin-Gui Ranjan, Priya Slavov, Gancho T. Gunter, Lee E. Jawdy, Sara Bryan, Anthony C. Sykes, Robert Ziebell, Angela Klapste, Jaroslav Porth, Ilga Skyba, Oleksandr Unda, Faride El-Kassaby, Yousry A. Douglas, Carl J. Mansfield, Shawn D. Martin, Joel Schackwitz, Wendy Evans, Luke M. Czarnecki, Olaf Tuskan, Gerald A. TI High-resolution genetic mapping of allelic variants associated with cell wall chemistry in Populus SO BMC GENOMICS LA English DT Article DE QTL doning; Association genetics; Cell wall recalcitrance; Lignin; Cellulose; Hemicellulose ID ETHANOL-PRODUCTION; WOOD PROPERTIES; LIGNIN; TRICHOCARPA; BIOMASS; POPLAR; ARABIDOPSIS; PYROLYSIS; PRODUCTS; CALCIUM AB Background: QTL cloning for the discovery of genes underlying polygenic traits has historically been cumbersome in long-lived perennial plants like Populus. Linkage disequilibrium-based association mapping has been proposed as a cloning tool, and recent advances in high-throughput genotyping and whole- genome resequencing enable marker saturation to levels sufficient for association mapping with no a priori candidate gene selection. Here, multiyear and multienvironment evaluation of cell wall phenotypes was conducted in an interspecific P. trichocarpa x P. deltoides pseudo-backcross mapping pedigree and two partially overlapping populations of unrelated P. trichocarpa genotypes using pyrolysis molecular beam mass spectrometry, saccharification, and/ or traditional wet chemistry. QTL mapping was conducted using a high-density genetic map with 3,568 SNP markers. As a fine-mapping approach, chromosome-wide association mapping targeting a QTL hot-spot on linkage group XIV was performed in the two P. trichocarpa populations. Both populations were genotyped using the 34 K Populus Infinium SNP array and whole- genome resequencing of one of the populations facilitated marker-saturation of candidate intervals for gene identification. Results: Five QTLs ranging in size from 0.6 to 1.8 Mb were mapped on linkage group XIV for lignin content, syringyl to guaiacyl (S/G) ratio, 5- and 6-carbon sugars using the mapping pedigree. Six candidate loci exhibiting significant associations with phenotypes were identified within QTL intervals. These associations were reproducible across multiple environments, two independent genotyping platforms, and different plant growth stages. cDNA sequencing for allelic variants of three of the six loci identified polymorphisms leading to variable length poly glutamine (PolyQ) stretch in a transcription factor annotated as an ANGUSTIFOLIA C-terminus Binding Protein (CtBP) and premature stop codons in a KANADI transcription factor as well as a protein kinase. Results from protoplast transient expression assays suggested that each of the polymorphisms conferred allelic differences in the activation of cellulose, hemicelluloses, and lignin pathway marker genes. Conclusion: This study illustrates the utility of complementary QTL and association mapping as tools for gene discovery with no a priori candidate gene selection. This proof of concept in a perennial organism opens up opportunities for discovery of novel genetic determinants of economically important but complex traits in plants. C1 [Muchero, Wellington; Guo, Jianjun; Chen, Jin-Gui; Ranjan, Priya; Gunter, Lee E.; Jawdy, Sara; Bryan, Anthony C.; Czarnecki, Olaf; Tuskan, Gerald A.] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA. [DiFazio, Stephen P.; Evans, Luke M.] W Virginia Univ, Dept Biol, Morgantown, WV 26506 USA. [Slavov, Gancho T.] Aberystwyth Univ, Inst Biol Environm & Rural Sci, Aberystwyth SY23 3EB, Dyfed, Wales. [Sykes, Robert] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA. [Klapste, Jaroslav; Porth, Ilga; El-Kassaby, Yousry A.] Univ British Columbia, Fac Forestry, Forest Sci Ctr, Dept Forest & Conservat Sci, Vancouver, BC V6T 1Z4, Canada. [Skyba, Oleksandr; Unda, Faride; Mansfield, Shawn D.] Univ British Columbia, Fac Forestry, Forest Sci Ctr, Dept Wood Sci, Vancouver, BC V6T 1Z4, Canada. [Douglas, Carl J.] Univ British Columbia, Dept Bot, Vancouver, BC V6T 1Z4, Canada. [Martin, Joel; Schackwitz, Wendy] US Dept Energy Joint Genome Inst, Walnut Creek, CA 94598 USA. [Klapste, Jaroslav] Czech Univ Life Sci, Fac Forestry & Wood Sci, Dept Genet & Physiol Forest Trees, Prague 16521 6, Czech Republic. RP Muchero, W (reprint author), Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA. EM mucherow@ornl.gov RI Chen, Jin-Gui/A-4773-2011; Klapste, Jaroslav/B-6668-2016; Porth, Ilga/N-4862-2015; El-Kassaby, Yousry/K-9856-2016; Gunter, Lee/L-3480-2016; Tuskan, Gerald/A-6225-2011 OI Chen, Jin-Gui/0000-0002-1752-4201; Klapste, Jaroslav/0000-0001-5504-3735; Porth, Ilga/0000-0002-9344-6348; El-Kassaby, Yousry/0000-0002-4887-8977; Gunter, Lee/0000-0003-1211-7532; Tuskan, Gerald/0000-0003-0106-1289 FU BioEnergy Science Center (Oak Ridge National Laboratory); US Department of Energy (DOE) Bioenergy Research Center - Office of Biological and Environmental Research in the DOE Office of Science; U.S. Dept. of Energy [DE-AC05-00OR22725]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Genome British Columbia Applied Genomics Innovation Program [103BIO]; Genome Canada Large Scale Applied Research Program [168BIO]; Natural Sciences and Engineering Research Council of Canada FX This research was supported, in part, by funding from the BioEnergy Science Center (Oak Ridge National Laboratory), a US Department of Energy (DOE) Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science. Oak Ridge National Laboratory is managed by UT-Battelle, LLC, for the U.S. Dept. of Energy under contract DE-AC05-00OR22725. The work conducted by the U.S. Department of Energy Joint Genome Institute was supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We also acknowledge financial support from the Genome British Columbia Applied Genomics Innovation Program (Project 103BIO) and the Genome Canada Large Scale Applied Research Program (Project 168BIO). Jianjun Guo was supported by a post-doctoral fellowship from the Natural Sciences and Engineering Research Council of Canada. The funding agencies had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 42 TC 13 Z9 13 U1 8 U2 47 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2164 J9 BMC GENOMICS JI BMC Genomics PD JAN 23 PY 2015 VL 16 AR 24 DI 10.1186/s12864-015-1215-z PG 14 WC Biotechnology & Applied Microbiology; Genetics & Heredity SC Biotechnology & Applied Microbiology; Genetics & Heredity GA CA5GL UT WOS:000348936800001 PM 25613058 ER PT J AU Chen, Y Di Marco, E Lykken, J Spiropulu, M Vega-Morales, R Xie, S AF Chen, Yi Di Marco, Emanuele Lykken, Joe Spiropulu, Maria Vega-Morales, Roberto Xie, Si TI 8D likelihood effective Higgs couplings extraction framework in h -> 4l SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering; Higgs physics ID STANDARD MODEL; BOSON DECAYS; LHC; LEPTONS; MASS; SPIN AB We present an overview of a comprehensive analysis framework aimed at performing direct extraction of all possible effective Higgs couplings to neutral electroweak gauge bosons in the decay to electrons and muons, the so called 'golden channel'. Our framework is based primarily on a maximum likelihood method constructed from analytic expressions of the fully differential cross sections for h -> 4l and for the dominant irreducible q (q) over bar -> 4l background, where 4l = 2e2 mu, 4e, 4 mu. Detector effects are included by an explicit convolution of these analytic expressions with the appropriate transfer function over all center of mass variables. Utilizing the full set of observables, we construct an unbinned detector-level likelihood which is continuous in the effective couplings. We consider possible ZZ, Z Upsilon, and Upsilon Upsilon couplings simultaneously, allowing for general CP odd/even admixtures. A broad overview is given of how the convolution is performed and we discuss the principles and theoretical basis of the framework. This framework can be used in a variety of ways to study Higgs couplings in the golden channel using data obtained at the LHC and other future colliders. C1 [Chen, Yi; Spiropulu, Maria; Xie, Si] CALTECH, Lauritsen Lab Phys, Pasadena, CA 92115 USA. [Di Marco, Emanuele; Lykken, Joe; Vega-Morales, Roberto] Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. [Vega-Morales, Roberto] Univ Paris 11, CNRS, UMR8627, Lab Phys Theor Orsay, F-91405 Orsay, France. [Vega-Morales, Roberto] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. RP Chen, Y (reprint author), CALTECH, Lauritsen Lab Phys, 1200 E Calif Blvd, Pasadena, CA 92115 USA. EM yi.chen@cern.ch; emanuele.di.marco@cern.ch; lykken@fnal.gov; smaria@caltech.edu; roberto.vega@th.u-psud.fr; sixie@hep.caltech.edu FU Fermi lab Graduate Student Fellowship in Theoretical Physics; ERC Advanced Grant Higgs@LHC; United States Department of Energy [DE-AC02-07CH11359]; Weston Havens Foundation; DOE [DE-FG02-92-ER-40701, DE-FG02-91ER40684]; National Science Foundation [OCI-1053575] FX The authors are grateful to Artur Apresyan, Michalis Bachtis, Adam Falkowski, Patrick Fox, Andrei Gritsan, Roni Harnik, Alex Mott, Pavel Nadolsky, Daniel Stolarski, Reisaburo Tanaka, Nhan Tran, Roberto Vega, and Felix Yu for helpful discussions as well as the ATLAS and CMS collaborations for their encouragement and interest in this work. R.V.M. is supported by the Fermi lab Graduate Student Fellowship in Theoretical Physics and the ERC Advanced Grant Higgs@LHC. Fermi lab is operated by Fermi Research Alliance, LLC, under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. Y.C. is supported by the Weston Havens Foundation and DOE grant DE-FG02-92-ER-40701. This work is also sponsored in part by the DOE grant No. DE-FG02-91ER40684. R.V.M is also grateful to the CalTech physics department for their hospitality during which much of this work was done. This work used the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by National Science Foundation grant number OCI-1053575. NR 60 TC 0 Z9 0 U1 1 U2 5 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN 23 PY 2015 IS 1 DI 10.1007/JHEP01(2015)125 PG 26 WC Physics, Particles & Fields SC Physics GA AZ8CK UT WOS:000348442300002 ER PT J AU Ding, JJ Zhang, YG Deng, Y Cong, J Lu, H Sun, X Yang, CY Yuan, T Van Nostrand, JD Li, DQ Zhou, JZ Yang, YF AF Ding, Junjun Zhang, Yuguang Deng, Ye Cong, Jing Lu, Hui Sun, Xin Yang, Caiyun Yuan, Tong Van Nostrand, Joy D. Li, Diqiang Zhou, Jizhong Yang, Yunfeng TI Integrated metagenomics and network analysis of soil microbial community of the forest timberline SO SCIENTIFIC REPORTS LA English DT Article ID CENTRAL AUSTRIAN ALPS; ORGANIC-MATTER; VEGETATION COMPOSITION; OXIDIZING BACTERIA; PLANT DIVERSITY; LOW-TEMPERATURE; TUNDRA ECOTONE; CLIMATE-CHANGE; PINUS-CEMBRA; DYNAMICS AB The forest timberline responds quickly and markedly to climate changes, rendering it a ready indicator. Climate warming has caused an upshift of the timberline worldwide. However, the impact on belowground ecosystem and biogeochemical cycles remain elusive. To understand soil microbial ecology of the timberline, we analyzed microbial communities via 16s rRNA Illumina sequencing, a microarray-based tool named GeoChip 4.0 and a random matrix theory-based association network approach. We selected 24 sampling sites at two vegetation belts forming the timberline of Shennongjia Mountain in Hubei Province of China, a region with extraordinarily rich biodiversity. We found that temperature, among all of measured environmental parameters, showed the most significant and extensive linkages with microbial biomass, microbial diversity and composition at both taxonomic and functional gene levels, and microbial association network. Therefore, temperature was the best predictor for microbial community variations in the timberline. Furthermore, abundances of nitrogen cycle and phosphorus cycle genes were concomitant with NH4+-N, NO3--N and total phosphorus, offering tangible clues to the underlying mechanisms of soil biogeochemical cycles. As the first glimpse at both taxonomic and functional compositions of soil microbial community of the timberline, our findings have major implications for predicting consequences of future timberline upshift. C1 [Ding, Junjun; Zhang, Yuguang; Cong, Jing; Lu, Hui; Li, Diqiang] Chinese Acad Forestry, Inst Forestry Ecol Environm & Protect, Beijing 100091, Peoples R China. [Ding, Junjun; Zhang, Yuguang; Cong, Jing; Lu, Hui; Li, Diqiang] Chinese Acad Forestry, Key Lab Forest Ecol & Environm State Forestry Adm, Beijing 100091, Peoples R China. [Ding, Junjun; Sun, Xin; Zhou, Jizhong; Yang, Yunfeng] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China. [Deng, Ye] Chinese Acad Sci, Ecoenvironm Sci Res Ctr, CAS Key Lab Environm Biotechnol, Beijing 100085, Peoples R China. [Deng, Ye; Yang, Caiyun; Yuan, Tong; Van Nostrand, Joy D.; Zhou, Jizhong] Univ Oklahoma, Inst Environm Genom, Norman, OK 73019 USA. [Deng, Ye; Yang, Caiyun; Yuan, Tong; Van Nostrand, Joy D.; Zhou, Jizhong] Univ Oklahoma, Dept Bot & Microbiol, Norman, OK 73019 USA. [Zhou, Jizhong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Cong, Jing] Cent S Univ, Sch Minerals Proc & Bioengn, Changsha 410083, Hunan, Peoples R China. RP Yang, YF (reprint author), Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China. EM zhangyg@caf.ac.cn; yangyf@tsinghua.edu.cn RI Van Nostrand, Joy/F-1740-2016; OI Van Nostrand, Joy/0000-0001-9548-6450; ?, ?/0000-0002-7584-0632 FU Yuguang Zhang from the public welfare project of the national scientific research institution [CAFRIFEEP201101]; Technology Program for Water Pollution Control and Treatment [2013ZX07315-001-03]; Strategic Priority Research Program of the Chinese Academy of Sciences [XDB15010102]; National Key Basic Research Program of China [2013CB956601]; National High Technology Research and Development Program of China [2012AA061401]; National Science Foundation of China [41471202, 41171201]; State Key Laboratory of Forest and Soil Ecology [LFSE2014-02]; US National Science Foundation [EF-1065844] FX This research was supported by grants to Yuguang Zhang from the public welfare project of the national scientific research institution (CAFRIFEEP201101), to Yunfeng Yang from Major Science and Technology Program for Water Pollution Control and Treatment (2013ZX07315-001-03), the Strategic Priority Research Program of the Chinese Academy of Sciences (XDB15010102), the National Key Basic Research Program of China (2013CB956601), National High Technology Research and Development Program of China (2012AA061401) and National Science Foundation of China (41471202 & 41171201), to Ye Deng from State Key Laboratory of Forest and Soil Ecology (Grant No. LFSE2014-02) and the Strategic Priority Research Program of the Chinese Academy of Sciences (Grant XDB15010302), and to Jizhong Zhou from the US National Science Foundation (EF-1065844). NR 70 TC 10 Z9 10 U1 18 U2 126 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 23 PY 2015 VL 5 AR 7994 DI 10.1038/srep07994 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AZ5UZ UT WOS:000348287500015 PM 25613225 ER PT J AU Felberg, LE Brookes, DH Head-Gordon, T Rice, JE Swope, WC AF Felberg, Lisa E. Brookes, David H. Head-Gordon, Teresa Rice, Julia E. Swope, William C. TI Role of Hydrophilicity and Length of Diblock Arms for Determining Star Polymer Physical Properties SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID ATOM FORCE-FIELD; MOLECULAR-DYNAMICS; VORONOI POLYHEDRA; GAS-PHASE; AB-INITIO; SIMULATIONS; MODEL; CONSTRUCTION; ALGORITHMS; HYDRATION AB We present a molecular simulation study of star polymers consisting of 16 diblock copolymer arms bound to a small adamantane core by varying both arm length and the outer hydrophilic block when attached to the same hydrophobic block of poly-d-valerolactone. Here we consider two biocompatible star polymers in which the hydrophilic block is composed of polyethylene glycol (PEG) or polymethyloxazoline (POXA) in addition to a polycarbonate-based polymer with a pendant hydrophilic group (PC1). We find that the different hydrophilic blocks of the star polymers show qualitatively different trends in their interactions with aqueous solvent, orientational time correlation functions, and orientational correlation between pairs of monomers of their polymeric arms in solution, in which we find that the PEG polymers are more thermosensitive compared with the POXA and PC1 star polymers over the physiological temperature range we have investigated. C1 [Felberg, Lisa E.; Head-Gordon, Teresa] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Head-Gordon, Teresa] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Brookes, David H.; Head-Gordon, Teresa] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Head-Gordon, Teresa] Lawrence Berkeley Natl Labs, Chem Sci Div, Berkeley, CA 94720 USA. [Rice, Julia E.; Swope, William C.] IBM Res, IBM Almaden Res Ctr, San Jose, CA 95120 USA. RP Head-Gordon, T (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. EM thg@berkeley.edu; swope@us.ibm.com FU Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [DGE 1106400, CHE-1265731] FX This work was supported by the Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under U.S. Department of Energy Contract No. DE-AC02-05CH11231. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. L.E.F. was supported by the National Science Foundation Graduate Research Fellowship under Grant No. DGE 1106400. We also thank the National Science Foundation grant CHE-1265731 for undergraduate training support for D.H.B. NR 37 TC 2 Z9 2 U1 1 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JAN 22 PY 2015 VL 119 IS 3 SI SI BP 944 EP 957 DI 10.1021/jp506203k PG 14 WC Chemistry, Physical SC Chemistry GA CD8FA UT WOS:000351329400031 PM 25254622 ER PT J AU Ellingson, SR Miao, YL Baudry, J Smith, JC AF Ellingson, Sally R. Miao, Yinglong Baudry, Jerome Smith, Jeremy C. TI Multi-Conformer Ensemble Docking to Difficult Protein Targets SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID RECEPTOR FLEXIBILITY; LIGAND-BINDING; DRUG DESIGN; DISCOVERY; INHIBITORS; SRC; CONFORMATIONS; PREDICTION; DYNAMICS; OVERCOME AB Large-scale ensemble docking is investigated using five proteins from the Directory Of Useful' Decoys (DUD, ducl.clocking.org) for which docking to crystal structures has proven difficult. Molecular dynamics trajectories are produced for each protein, and an ensemble of representative conformational structures extracted from the trajectories. Docking calculations are performed on these selected simulation structures and ensemble-based enrichment factors compared with those obtained using docking in crystal structures of the same protein targets or random selection of compounds. Simulation-derived snapshots are found with improved enrichment factors that increase the chemical diversity of docking hits for four of the five selected proteins. A combination of all the docking results obtained from moleCtilar dynamics simulation followed by selection of top-ranking compounds appears to be an effective strategy for increasing the number and diversity of hits when using docking to screen large libraries of chemicals against difficult protein targets. C1 [Ellingson, Sally R.] Univ Tennessee, Genome Sci & Technol, Knoxville, TN USA. [Miao, Yinglong; Baudry, Jerome; Smith, Jeremy C.] Univ Tennessee, Dept Biochem & Cellular & Mol Biol, Knoxville, TN 37996 USA. [Ellingson, Sally R.; Miao, Yinglong; Baudry, Jerome; Smith, Jeremy C.] Oak Ridge Natl Lab, UT ORNL Ctr Mol Biophys, Oak Ridge, TN USA. [Ellingson, Sally R.] Univ Kentucky, Div Biomed Informat, UK Coll Publ Hlth, Lexington, KY USA. RP Smith, JC (reprint author), Univ Tennessee, Dept Biochem & Cellular & Mol Biol, Knoxville, TN 37996 USA. EM smithjc@ornl.gov RI smith, jeremy/B-7287-2012 OI smith, jeremy/0000-0002-2978-3227 FU National Center for Computational Sciences at Oak Ridge National Laboratory; [bio026] FX We thank Loukas Petridis for helpful discussions regarding molecular docking simulations using NAMD2 and Jim Phillips (UIUC) for providing the GPU-enabled binaries of NAMD2. This work was partially funded through the National Center for Computational Sciences at Oak Ridge National Laboratory, and computing time was provided through grant number bio026. NR 40 TC 13 Z9 13 U1 3 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JAN 22 PY 2015 VL 119 IS 3 SI SI BP 1026 EP 1034 DI 10.1021/jp506511p PG 9 WC Chemistry, Physical SC Chemistry GA CD8FA UT WOS:000351329400039 PM 25198248 ER PT J AU Tang, XY Sousa, LD Jin, MJ Chundawat, SPS Chambliss, CK Lau, MW Xiao, ZY Dale, BE Balan, V AF Tang, Xiaoyu Sousa, Leonardo da Costa Jin, Mingjie Chundawat, Shishir P. S. Chambliss, Charles Kevin Lau, Ming W. Xiao, Zeyi Dale, Bruce E. Balan, Venkatesh TI Designer synthetic media for studying microbial-catalyzed biofuel production SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Synthetic hydrolysate; Lignocellulose; AFEX; Yeast fermentation inhibition; Amides inhibition; Carboxylic acids inhibition; Pretreatment decomposition products; Hydrolysate composition ID AMMONIA FIBER EXPANSION; TREATED CORN STOVER; SACCHAROMYCES-CEREVISIAE 424A(LNH-ST); TRANS-ACONITIC ACID; ACETIC-ACID; LIGNOCELLULOSIC BIOMASS; ETHANOL-PRODUCTION; XYLOSE FERMENTATION; CELLULOSIC ETHANOL; YEAST AB Background: The fermentation inhibition of yeast or bacteria by lignocellulose-derived degradation products, during hexose/pentose co-fermentation, is a major bottleneck for cost-effective lignocellulosic biorefineries. To engineer microbial strains for improved performance, it is critical to understand the mechanisms of inhibition that affect fermentative organisms in the presence of major components of a lignocellulosic hydrolysate. The development of a synthetic lignocellulosic hydrolysate (SH) media with a composition similar to the actual biomass hydrolysate will be an important advancement to facilitate these studies. In this work, we characterized the nutrients and plant-derived decomposition products present in AFEX (TM) pretreated corn stover hydrolysate (ACH). The SH was formulated based on the ACH composition and was further used to evaluate the inhibitory effects of various families of decomposition products during Saccharomyces cerevisiae 424A (LNH-ST) fermentation. Results: The ACH contained high levels of nitrogenous compounds, notably amides, pyrazines, and imidazoles. In contrast, a relatively low content of furans and aromatic and aliphatic acids were found in the ACH. Though most of the families of decomposition products were inhibitory to xylose fermentation, due to their abundance, the nitrogenous compounds showed the most inhibition. From these compounds, amides (products of the ammonolysis reaction) contributed the most to the reduction of the fermentation performance. However, this result is associated to a concentration effect, as the corresponding carboxylic acids (products of hydrolysis) promoted greater inhibition when present at the same molar concentration as the amides. Due to its complexity, the formulated SH did not perfectly match the fermentation profile of the actual hydrolysate, especially the growth curve. However, the SH formulation was effective for studying the inhibitory effect of various compounds on yeast fermentation. Conclusions: The formulation of SHs is an important advancement for future multi-omics studies and for better understanding the mechanisms of fermentation inhibition in lignocellulosic hydrolysates. The SH formulated in this work was instrumental for defining the most important inhibitors in the ACH. Major AFEX decomposition products are less inhibitory to yeast fermentation than the products of dilute acid or steam explosion pretreatments; thus, ACH is readily fermentable by yeast without any detoxification. C1 [Tang, Xiaoyu] Minist Agr, Biogas Inst, Chengdu 610041, Peoples R China. [Sousa, Leonardo da Costa; Jin, Mingjie; Chundawat, Shishir P. S.; Lau, Ming W.; Dale, Bruce E.; Balan, Venkatesh] Michigan State Univ, DOE Great Lakes Bioenergy Res Ctr, BCRL, Lansing, MI 48910 USA. [Chundawat, Shishir P. S.] Rutgers State Univ, Dept Chem & Biochem Engn, Piscataway, NJ 08854 USA. [Chambliss, Charles Kevin] Baylor Univ, Dept Chem & Biochem, Waco, TX 76798 USA. [Xiao, Zeyi] Sichuan Univ, Sch Chem Engn, Chengdu 610065, Peoples R China. RP Tang, XY (reprint author), Minist Agr, Biogas Inst, Sect 4,13 Remin South Rd, Chengdu 610041, Peoples R China. EM tangxiaoyu@caas.cn; balan@msu.edu RI da Costa Sousa, Leonardo/A-1536-2016; OI Chundawat, Shishir/0000-0003-3677-6735; Chambliss, Kevin/0000-0003-3888-6890; Jin, Mingjie/0000-0002-9493-305X FU DOE Great Lakes Bioenergy Research Center (GLBRC) [DE-FC02-07ER64494]; Fundacao para a Ciencia e a Tecnologia and European Social Fund [SFRH/BD/62517/2009]; China Scholarship Council [2009101936] FX We would like to acknowledge Novozymes and Genencor for kindly providing the enzymes used in the production of the lignocellulosic hydrolysate and oligomeric xylan. We thank Professor Nancy Ho from Purdue University for kindly providing the recombinant Saccharomyces cerevisiae 424A (LNH-ST) strain. We would like to acknowledge Professor Dan Jones for making available some of the analytical instrumentation at the MSU mass spectrometry facility for hydrolysate analysis. We also want to thank Charles Donald, Christa Gunawan, and Jeffrey Halim for their assistance in sample preparation and analysis. This work was partially funded by the DOE Great Lakes Bioenergy Research Center (GLBRC), grant number DE-FC02-07ER64494. Leonardo Sousa was funded by Fundacao para a Ciencia e a Tecnologia and European Social Fund, grant number SFRH/BD/62517/2009. Xiaoyu Tang was supported by the China Scholarship Council, grant number 2009101936. NR 48 TC 5 Z9 5 U1 7 U2 33 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD JAN 22 PY 2015 VL 8 AR 1 DI 10.1186/s13068-014-0179-6 PG 17 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA CB6BG UT WOS:000349711300001 PM 25642283 ER PT J AU Aad, G Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Almond, J Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N 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CA ATLAS Collaboration TI Measurement of the production and lepton charge asymmetry of W bosons in Pb plus Pb collisions at root s(NN)=2.76 TeV with the ATLAS detector SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID TRANSVERSE-MOMENTUM DEPENDENCE; LEAD-LEAD COLLISIONS; QUARK-GLUON PLASMA; MONTE-CARLO; QCD; COLLABORATION; PERSPECTIVE; SUPPRESSION; MATTER; MODEL AB A measurement of W boson production in lead-lead collisions at root s(NN) = 2.76 TeV is presented. It is based on the analysis of data collected with the ATLAS detector at the LHC in 2011 corresponding to an integrated luminosity of 0.14 nb(-1) and 0.15 nb(-1) in the muon and electron decay channels, respectively. The differential production yields and lepton charge asymmetry are each measured as a function of the average number of participating nucleons < N-part > and absolute pseudorapidity of the charged lepton. The results are compared to predictions based on next-to-leading-order QCD calculations. 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M.; Grafstroem, P.; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Semprini-Cesari, N.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Alberghi, G. L.; Caforio, D.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Semprini-Cesari, N.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Hageboeeck, S.; Hellmich, D.; Hillert, S.; Huegging, F.; Janssen, J.; Khoriauli, G.; Koevesarki, P.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lehmacher, M.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Loddenkoetter, T.; Mergelmeyer, S.; Mijovic, L.; Mueller, K.; Nanava, G.; Nattermann, T.; Obermann, T.; Pohl, D.; Sarrazin, B.; Schaepe, S.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Stillings, J. A.; Tannoury, N.; Therhaag, J.; Uchida, K.; Uhlenbrock, M.; Vogel, A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Fitzgerald, E. A.; Gozpinar, S.; Sciolla, G.; Venturini, A.; Zambito, S.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Amaral Coutinho, Y.; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE, EE, IF, BR-21945 Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Univ Fed Juiz de Fora, Juiz de Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Hu, X.; Klimentov, A.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Okawa, H.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Schovancova, J.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dita, P.; Dita, S.; Ducu, O. A.; Jinaru, A.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Horia Hulubei Natl Inst Phys & Nucl Engn, Bucharest 077125, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Lacey, J.; Leight, W. A.; Marchand, J. F.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Battistin, M.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Franchino, S.; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hauschild, M.; Hawkings, R. 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C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, CH-1211 Geneva 23, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Cheng, Y.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China. [Chen, S.; Li, Y.; Wang, C.] Nanjing Univ, Dept Phys, Nanjing 210008, Jiangsu, Peoples R China. [Chen, L.; Fengd, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan 250100, Shandong, Peoples R China. [Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] IN2P3, CNRS, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Guo, J.; Hu, D.; Hughes, E. W.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Wulf, E.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, I-00044 Frascati, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hoffman, J.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Lou, X.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Prokofiev, K.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dao, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Madar, R.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ronzani, M.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Picazio, A.; Pohl, M.; Rosbach, K.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Bindi, M.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. 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F.; Giulini, M.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Gandrajula, R. P.; Mallik, U.; Mandrysch, R.; Morange, N.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Topilin, N. D.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Readioff, N. P.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr; Rose, M.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Egham, Surrey, England. [Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Cooper, B. D.; Davison, A. R.; Davison, P.; Falla, R. J.; Gregersen, K.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Sircar, A.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] IN2P3, CNRS, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Blum, W.; Buescher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Goeringer, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Chen, L.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Chen, L.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] IN2P3, CNRS, Marseille, France. [Bellomo, M.; Brau, B.; Colon, G.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Mantifel, R.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Urquijo, P.; Volpi, M.] Univ Melbourne, Sch Phys, Parkville, Vic 3052, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Harper, D.; Levin, D.; Liu, L.; Long, J. D.; Lu, N.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Panikashvili, N.; Qian, J.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Xu, L.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Perini, L.; Pizio, C.; Ragusa, F.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. 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S.; Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Heller, C.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Will, J. Z.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Konig, A. C.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Burghgrave, B.; Calkins, R.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Skovpen, K. Yu; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Tannenwald, B. B.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] IN2P3, CNRS, Orsay, France. [Endo, M.; Hanagaki, K.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Gjelsten, B. K.; Gramstad, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Slater, M.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Behr, K.; Boddy, C. R.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Livermore, S. S. A.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Vickeyc, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Meyer, C.; Ospanov, R.; Saxon, J.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Do Valle Wemans, A.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Marques, C. N.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Do Valle Wemans, A.] Univ Nova Lisboa, Fac Ciencias & Tecnol, Dept Fis, Caparica, Portugal. [Do Valle Wemans, A.] Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Bohm, J.; Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Chiefari, G.; Davies, E.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Stanescu, C.; Taccini, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Taccini, C.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.; Fassi, F.; Haddad, N.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Grabas, H. M. X.; Guyot, C.; Hanna, R.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mal, P.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay Commissariat Energie Atom & Energies A, DSM IRFU Inst Rech Lois Fondamentales Univers, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Suruliz, K.; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; Godfrey, J.; O'Neil, D. C.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nef, P. D.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Carrillo-Montoya, G. D.; Chen, X.; Hamity, G. N.; Hsu, C.; Garcia, B. R. Mellado; Ruan, X.; Vickeyc, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bessidskaia, O.; Bohm, C.; Clement, C.; Cribbs, W. A.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bessidskaia, O.; Clement, C.; Cribbs, W. A.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; Cerri, A.; Barajas, C. A. Chavez; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Ren, Z. L.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Leisos, A.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.; Sidiropoulou, O.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Brelier, B.; Chau, C. C.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Ramos, J. A. Manjarres; Palacino, G.; Qureshi, A.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Quayle, W. B.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; De Sanctis, U.; Quayle, W. B.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. 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[Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Korol, A. A.; Maximov, D. A.; Rezanova, O. L.; Talyshev, A. A.; Tikhonov, Yu A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Ciubancan, Liviu Mihai/L-2412-2015; Zhukov, Konstantin/M-6027-2015; Shmeleva, Alevtina/M-6199-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; De, Kaushik/N-1953-2013; Carvalho, Joao/M-4060-2013; Riu, Imma/L-7385-2014; Cabrera Urban, Susana/H-1376-2015; Mir, Lluisa-Maria/G-7212-2015; Cavalli-Sforza, Matteo/H-7102-2015; Marti-Garcia, Salvador/F-3085-2011; Della Pietra, Massimo/J-5008-2012; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Grancagnolo, Sergio/J-3957-2015; Doyle, Anthony/C-5889-2009; spagnolo, stefania/A-6359-2012; Tassi, Enrico/K-3958-2015; Livan, Michele/D-7531-2012; Moraes, Arthur/F-6478-2010; Boyko, Igor/J-3659-2013; Mitsou, Vasiliki/D-1967-2009; Carquin, Edson/G-5221-2015; Villa, Mauro/C-9883-2009; White, Ryan/E-2979-2015; Joergensen, Morten/E-6847-2015; Brooks, William/C-8636-2013; Di Domenico, Antonio/G-6301-2011; Connell, Simon/F-2962-2015; Bosman, Martine/J-9917-2014; Garcia, Jose /H-6339-2015; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Mindur, Bartosz/A-2253-2017; Fabbri, Laura/H-3442-2012; Gutierrez, Phillip/C-1161-2011; Gerbaudo, Davide/J-4536-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Martinez, Mario /I-3549-2015; Gabrielli, Alessandro/H-4931-2012; Peleganchuk, Sergey/J-6722-2014; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Snesarev, Andrey/H-5090-2013; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Staroba, Pavel/G-8850-2014; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Smirnova, Oxana/A-4401-2013; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Wemans, Andre/A-6738-2012; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Pacheco Pages, Andres/C-5353-2011; Vranjes Milosavljevic, Marija/F-9847-2016; Perrino, Roberto/B-4633-2010 OI Ciubancan, Liviu Mihai/0000-0003-1837-2841; Tikhomirov, Vladimir/0000-0002-9634-0581; Warburton, Andreas/0000-0002-2298-7315; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; De, Kaushik/0000-0002-5647-4489; Carvalho, Joao/0000-0002-3015-7821; Riu, Imma/0000-0002-3742-4582; Mir, Lluisa-Maria/0000-0002-4276-715X; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Grancagnolo, Sergio/0000-0001-8490-8304; Doyle, Anthony/0000-0001-6322-6195; spagnolo, stefania/0000-0001-7482-6348; Livan, Michele/0000-0002-5877-0062; Moraes, Arthur/0000-0002-5157-5686; Boyko, Igor/0000-0002-3355-4662; Mitsou, Vasiliki/0000-0002-1533-8886; Carquin, Edson/0000-0002-7863-1166; Villa, Mauro/0000-0002-9181-8048; White, Ryan/0000-0003-3589-5900; Joergensen, Morten/0000-0002-6790-9361; Brooks, William/0000-0001-6161-3570; Di Domenico, Antonio/0000-0001-8078-2759; Connell, Simon/0000-0001-6000-7245; Bosman, Martine/0000-0002-7290-643X; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Gabrielli, Alessandro/0000-0001-5346-7841; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Mashinistov, Ruslan/0000-0001-7925-4676; Smirnova, Oxana/0000-0003-2517-531X; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Wemans, Andre/0000-0002-9669-9500; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Pacheco Pages, Andres/0000-0001-8210-1734; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Perrino, Roberto/0000-0002-5764-7337 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET; ERC; NSRF; European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 59 TC 5 Z9 5 U1 12 U2 87 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JAN 22 PY 2015 VL 75 IS 1 AR 23 DI 10.1140/epjc/s10052-014-3231-6 PG 30 WC Physics, Particles & Fields SC Physics GA CA6BF UT WOS:000348992600002 ER PT J AU Vlcek, L Uhlik, F Moucka, F Nezbeda, I Chialvo, AA AF Vlcek, Lukas Uhlik, Filip Moucka, Filip Nezbeda, Ivo Chialvo, Ariel A. TI Thermodynamics of Small Alkali Metal Halide Cluster Ions: Comparison of Classical Molecular Simulations with Experiment and Quantum Chemistry SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID MONTE-CARLO SIMULATIONS; POLARIZABLE FORCE-FIELD; GIBBS FREE-ENERGY; WATER CLUSTERS; GAS-PHASE; HYDRATION ENERGIES; MASS-SPECTROMETRY; COMPUTER-SIMULATIONS; DYNAMICS SIMULATIONS; AQUEOUS SOLVATION AB We evaluate the ability of selected classical molecular models to describe the thermodynamic and structural aspects of gas-phase hydration of alkali metal halide ions and the formation of small water clusters. To understand the effect of many-body interactions (polarization) and charge penetration effects on the accuracy of a force field, we perform Monte Carlo simulations with three rigid water models using different functional forms to account for these effects: (i) point charge nonpolarizable SPC/E, (ii) Drude point charge polarizable SWM4-DP, and (iii) Drude Gaussian charge polarizable BK3. Model predictions are compared with experimental Gibbs free energies and enthalpies of ion hydration, and with microscopic structural properties obtained from quantum DFT calculations. We find that all three models provide comparable predictions for pure water clusters and cation hydration but differ significantly in their description of anion hydration. None of the investigated classical force fields can consistently and quantitatively reproduce the experimental gas-phase hydration thermodynamics. The outcome of this study highlights the relation between the functional form that describes the effective intermolecular interactions and the accuracy of the resulting ion hydration properties. C1 [Vlcek, Lukas; Chialvo, Ariel A.] Oak Ridge Natl Lab, Geochem & Interfacial Sci Grp, Div Chem Sci, Oak Ridge, TN 37831 USA. [Vlcek, Lukas] Oak Ridge Natl Lab, Joint Inst Computat Sci, Oak Ridge, TN 37831 USA. [Uhlik, Filip] Charles Univ Prague, Fac Sci, Dept Phys & Macromol Chem, Prague 12843 2, Czech Republic. [Moucka, Filip; Nezbeda, Ivo] Univ JE Purkyne, Fac Sci, Usti Nad Labem 40096, Czech Republic. [Nezbeda, Ivo] Acad Sci Czech Republic, Inst Chem Proc Fundamentals, E Hala Lab Thermodynam, CR-16502 Prague 6, Czech Republic. RP Vlcek, L (reprint author), Oak Ridge Natl Lab, Geochem & Interfacial Sci Grp, Div Chem Sci, Oak Ridge, TN 37831 USA. EM vlcekl1@ornl.gov RI Moucka, Filip/M-4013-2013; Vlcek, Lukas/N-7090-2013; Uhlik, Filip/G-7395-2012; OI Moucka, Filip/0000-0002-1400-7890; Vlcek, Lukas/0000-0003-4782-7702; Uhlik, Filip/0000-0002-1628-2861; Chialvo, Ariel/0000-0002-6091-4563 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division FX This research was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. The participation of F.M. and I.N. was facilitated by the Czech-USA cooperative research program "Nonadditive interactions in aqueous solutions of electrolytes". F.U. thanks the Czech Science Foundation (P208/10/1724) and is thankful for access to the CERIT-SC computing facilities (CZ.1.05/3.2.00/08.0144) NR 85 TC 5 Z9 5 U1 9 U2 59 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JAN 22 PY 2015 VL 119 IS 3 BP 488 EP 500 DI 10.1021/jp509401d PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AZ8WG UT WOS:000348491800007 PM 25513841 ER PT J AU Clark, JM Nimlos, MR Robichaud, DJ AF Clark, Jared M. Nimlos, Mark R. Robichaud, David J. TI Bimolecular Decomposition Pathways for Carboxylic Acids of Relevance to Biofuels SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID THERMAL UNIMOLECULAR DECOMPOSITION; BETAGAMMA-UNSATURATED ACIDS; GAS-PHASE DECARBOXYLATION; RADICAL-WATER COMPLEXES; GASEOUS FORMIC ACID; ACETIC-ACID; HYDROGEN ABSTRACTION; ASYMMETRIC-SYNTHESIS; DENSITY FUNCTIONALS; KINETIC-PARAMETERS AB The bimolecular thermal reactions of carboxylic acids were studied using quantum mechanical molecular modeling. Previous work1 investigated the unimolecular decomposition of a variety of organic acids, including saturated, alpha,beta-unsaturated, and beta,gamma-unsaturated acids, and showed that the type and position of the unsaturation resulted in unique branching ratios between dehydration and decarboxylation, [H2O]/[CO2]. In this work, the effect of bimolecular chemistry (wateracid and acidacid) is considered with a representative of each acid class. In both cases, the strained 4-centered, unimolecular transition state, typical of most organic acids, is opened up to 6- or 8-centered bimolecular geometries. These larger structures lead to a reduction in the barrier heights (2045%) of the thermal decomposition pathways for organic acids and an increase in the decomposition kinetics. In some cases, they even cause a shift in the branching ratio of the corresponding product slates. C1 [Clark, Jared M.; Nimlos, Mark R.; Robichaud, David J.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. RP Robichaud, DJ (reprint author), Natl Renewable Energy Lab, Natl Bioenergy Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM david.robichaud@nrel.gov FU Department of Energy (DOE) Bioenergy Technology Office [DE-AC-08GO28308]; Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy (EERE) Postdoctoral Research Awards under EERE Biomass Program; DOE [DE-AC05-06OR23100] FX This research was conducted as part of the Computational Pyrolysis Consortium supported by the Department of Energy (DOE) Bioenergy Technology Office under contract number DE-AC-08GO28308. This research was supported in part by the Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy (EERE) Postdoctoral Research Awards under the EERE Biomass Program administered by the Oak Ridge Institute for Science and Education (ORISE) for the DOE. ORISE is managed by Oak Ridge Associated Universities (ORAU) under DOE contract number DE-AC05-06OR23100. All opinions expressed in this paper are the authors' and do not necessarily reflect the policies and views of DOE, ORAU, or ORISE. NR 59 TC 5 Z9 5 U1 2 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JAN 22 PY 2015 VL 119 IS 3 BP 501 EP 516 DI 10.1021/jp509285n PG 16 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AZ8WG UT WOS:000348491800008 PM 25513721 ER PT J AU Sampat, S Mohite, AD Crone, B Tretiak, S Malko, AV Taylor, AJ Yarotski, DA AF Sampat, Siddharth Mohite, Aditya D. Crone, Brian Tretiak, Sergei Malko, Anton V. Taylor, Antoinette J. Yarotski, Dmitry A. TI Tunable Charge Transfer Dynamics at Tetracene/LiF/C-60 Interfaces SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SOLAR-ENERGY CONVERSION; C-60 FILMS; CELLS; EXCITONS; POLYMER; FISSION; STATE AB Ultrafast optical spectroscopy was utilized to investigate charge transfer dynamics across organic semiconductor tetracene/C-60 interfaces in the presence of a LiF barrier layer. Photoinduced absorption spectra in the 1.6-2.3 eV range reveal a strong effect of the intermediate LiF barrier layer on dynamics of the charge transfer excitons (CTE) creation and recombination. Increasing thickness of the LiF film from 0 to 1 nm significantly suppresses CTE recombination while CTE generation remains practically unaltered. Further increase of LiF thickness to 2 nm prevents creation of CTE by diffusion from tetracene but does not affect direct CTE excitation by incident photons. Unlike thin films studied here, direct CTE photogeneration at the interface between thick organic films accounts for a small fraction (as compared to diffusion-induced) of total CTE population, resulting in a larger contribution of the LiF barrier to charge separation efficiency. C1 [Sampat, Siddharth; Malko, Anton V.] Univ Texas Dallas, Dept Phys, Richardson, TX 75080 USA. [Mohite, Aditya D.; Crone, Brian; Tretiak, Sergei; Taylor, Antoinette J.; Yarotski, Dmitry A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Yarotski, DA (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM dzmitry@lanl.gov RI Yarotski, Dmitry/G-4568-2010; Tretiak, Sergei/B-5556-2009 OI Tretiak, Sergei/0000-0001-5547-3647 FU Los Alamos National Laboratory Directed Research and Development program FX This work was performed in part at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences (DOE BES) user facility, and funded by the Los Alamos National Laboratory Directed Research and Development program. NR 26 TC 1 Z9 1 U1 0 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 22 PY 2015 VL 119 IS 3 BP 1286 EP 1290 DI 10.1021/jp5095905 PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AZ8WH UT WOS:000348491900003 ER PT J AU Trinh, MT Zhong, Y Chen, QS Schiros, T Jockusch, S Sfeir, MY Steigerwald, M Nuckolls, C Zhu, XY AF Trinh, M. Tuan Zhong, Yu Chen, Qishui Schiros, Theanne Jockusch, Steffen Sfeir, Matthew Y. Steigerwald, Michael Nuckolls, Colin Zhu, Xiaoyang TI Intra- to Intermolecular Singlet Fission SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID PUMP-PROBE SPECTROSCOPY; EXCITON-FISSION; SOLAR-CELLS; THIN-FILMS; ENERGY; STATE; FLUORESCENCE; CAROTENOIDS; TEMPERATURE; GENERATION AB Singlet fission, the splitting of one singlet into two triplets, can potentially increase the efficiency of optoelectronic devices beyond conventional limits. Among the singlet fission molecules discovered to date, two mechanisms have emerged: intra- or intermolecular singlet fission. Here we show a combined intra- to intermolecular singlet fission mechanism in the model system of diphenyl-dicyano-oligoene (DPDC). Excitation of DPDC to the first optically bright state leads to the ultrafast formation of an intramolecular triplet pair, which decays in 40 ps in the solution phase but can also split competitively in 30 ps into two long-lived triplets (2xT(1)) on adjacent molecules in solid films. These findings suggest a design principle for efficient singlet fission: the independent tuning of singlet-triplet pair coupling and triplet pair splitting from intra- and intermolecular interactions, respectively. C1 [Trinh, M. Tuan; Zhong, Yu; Chen, Qishui; Schiros, Theanne; Jockusch, Steffen; Steigerwald, Michael; Nuckolls, Colin; Zhu, Xiaoyang] Columbia Univ, Dept Chem, New York, NY 10027 USA. [Sfeir, Matthew Y.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Nuckolls, C (reprint author), Columbia Univ, Dept Chem, New York, NY 10027 USA. EM cn37@columbia.edu; xyzhu@columbia.edu OI Sfeir, Matthew/0000-0001-5619-5722; Zhong, Yu/0000-0001-8631-2213 FU program "Center for Re-Defining Photovoltaic Efficiency Through Molecule Scale Control", an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001085]; National Science Foundation [DMR 1321405]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work was supported before June 30, 2014, as part of the program "Center for Re-Defining Photovoltaic Efficiency Through Molecule Scale Control", an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0001085; most experimental work on DPDCn molecules and initial data analysis was carried out during this time period. After June 30, 2014, this work was supported by the National Science Foundation grant DMR 1321405 (to X.Z.); new experimental analysis presented in this manuscript and control experiments on other oligoene molecules were carried out during this time period. Research carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. X.Z. thanks Prof. Valy Vardeny for the teaching on picosecond acoustics. We thank D. Nordlund at SLAC National Accelerator Laboratory for help with synchrotron measurements. NR 57 TC 12 Z9 12 U1 11 U2 78 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 22 PY 2015 VL 119 IS 3 BP 1312 EP 1319 DI 10.1021/jp512650g PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AZ8WH UT WOS:000348491900006 ER PT J AU Zhao, ZC Xu, SC Hu, MY Bao, XH Peden, CHF Hu, JZ AF Zhao, Zhenchao Xu, Suochang Hu, Mary Y. Bao, Xinhe Peden, Charles H. F. Hu, Jianzhi TI Investigation of Aluminum Site Changes of Dehydrated Zeolite H-Beta during a Rehydration Process by High-Field Solid-State NMR SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID EXTRA-FRAMEWORK ALUMINUM; MQMAS NMR; AL-27 MAS; NONFRAMEWORK ALUMINUM; PROTON-TRANSFER; ACID SITES; SPECTROSCOPY; DEALUMINATION; MOLECULES; ZSM-5 AB Aluminum site changes of dehydrated H-Beta zeolite during a rehydration process are systematically investigated by Al-27 MAS and MQ MAS NMR at a high magnetic field up to 19.9 T. Benefiting from the high magnetic field, more detailed information is obtained from the considerably broadened and overlapped spectra of dehydrated H-Beta zeolite. Dynamic changes of aluminum sites are demonstrated during the rehydration process. In completely dehydrated H-Beta, invisible aluminums can reach 29%. The strength of quadrupole interactions for framework aluminum sites decreases gradually during the progressive water adsorption process. Extra-framework aluminum (EFAL) species, that is, penta- (34 ppm) and octahedral- (4 ppm) coordinated aluminum atoms, rise initially with increasing amount of water adsorption, and finally change into either tetra-coordinated framework or extra-framework aluminum in water saturated samples, with the remaining octahedrally coordinated aluminum lying at 0 and -4 ppm, respectively. Quantitative Al-27 MAS NMR analysis combined with 1H MAS NMR indicates that some active EFAL species formed during calcination can reinsert into the framework during this hydration process. The assignment of aluminum at 0 ppm to EFAL cation and -4 ppm to framework aluminum is clarified for H-Beta zeolite. C1 [Zhao, Zhenchao; Xu, Suochang; Hu, Mary Y.; Peden, Charles H. F.; Hu, Jianzhi] Pacific NW Natl Lab, Richland, WA 99352 USA. [Zhao, Zhenchao; Bao, Xinhe] Xiamen Univ, Collaborat Innovat Ctr Chem Energy Mat, Xiamen 361005, Peoples R China. [Xu, Suochang; Bao, Xinhe] Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China. RP Hu, JZ (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM jianzhi.hu@pnnl.gov RI li, haobo/P-5373-2014; Hu, Jian Zhi/F-7126-2012 OI li, haobo/0000-0002-9215-3754; FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences; DOE's Office of Biological and Environmental Research; DOE [DE-AC06-76RLO 1830] FX This research was supported by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences. All of the NMR experiments were performed in the Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research, and located at Pacific Northwest National Laboratory (PNNL). PNNL is a multiprogram national laboratory operated for the DOE by Battelle Memorial Institute under contract DE-AC06-76RLO 1830. NR 41 TC 7 Z9 7 U1 11 U2 74 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 22 PY 2015 VL 119 IS 3 BP 1410 EP 1417 DI 10.1021/jp509982r PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AZ8WH UT WOS:000348491900016 ER PT J AU Gupta, S Arend, N Lunkenheimer, P Loidl, A Stingaciu, L Jalarvo, N Mamontov, E Ohl, M AF Gupta, S. Arend, N. Lunkenheimer, P. Loidl, A. Stingaciu, L. Jalarvo, N. Mamontov, E. Ohl, M. TI Excess wing in glass-forming glycerol and LiCl-glycerol mixtures detected by neutron scattering SO EUROPEAN PHYSICAL JOURNAL E LA English DT Article ID GOLDSTEIN BETA-RELAXATION; SPIN-ECHO SPECTROMETER; LIGHT-SCATTERING; SUPERCOOLED LIQUIDS; PROPYLENE CARBONATE; ALPHA-RELAXATION; DIELECTRIC-SPECTROSCOPY; IONIC CONDUCTORS; DECAY FUNCTION; TRANSITION AB The relaxational dynamics in glass-forming glycerol and glycerol mixed with LiCl is investigated using different neutron scattering techniques. The performed neutron spin echo experiments, which extend up to relatively long relaxation time scales of the order of 10ns, should allow for the detection of contributions from the so-called excess wing. This phenomenon, whose microscopic origin is controversially discussed, arises in a variety of glass formers and, until now, was almost exclusively investigated by dielectric spectroscopy and light scattering. Here we show that the relaxational process causing the excess wing can also be detected by neutron scattering, which directly couples to density fluctuations. C1 [Gupta, S.; Arend, N.; Stingaciu, L.; Jalarvo, N.; Ohl, M.] Forschungszentrum Julich GmbH, Outstn SNS Oak Ridge Natl Lab ORNL, JCNS, Oak Ridge, TN 37831 USA. [Arend, N.] Forschungszentrum Julich GmbH, Outstn MLZ, JCNS, D-85747 Garching, Germany. [Lunkenheimer, P.; Loidl, A.] Univ Augsburg, Ctr Elect Correlat & Magnetism, D-86135 Augsburg, Germany. [Mamontov, E.] Oak Ridge Natl Lab, Neutron Sci Directorate, SNS, Oak Ridge, TN 37831 USA. RP Gupta, S (reprint author), Forschungszentrum Julich GmbH, Outstn SNS Oak Ridge Natl Lab ORNL, JCNS, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM s.gupta@fz-juelich.de RI Lunkenheimer, Peter/C-6196-2008; Mamontov, Eugene/Q-1003-2015; Gupta, Sudipta/I-7960-2015; Loidl, Alois/L-8199-2015; Jalarvo, Niina/Q-1320-2015; OI Lunkenheimer, Peter/0000-0002-4525-1394; Mamontov, Eugene/0000-0002-5684-2675; Loidl, Alois/0000-0002-5579-0746; Jalarvo, Niina/0000-0003-0644-6866; Stingaciu, Laura/0000-0003-2696-5233 FU Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; Deutsche Forschungsgemeinschaft via Research Unit [FOR 1394] FX We thank Prof. D. Richter, M. Monkenbusch, and R. Zorn for helpful discussions. Research conducted at ORNL's Spallation Neutron Source, was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. The work at the University of Augsburg was partly supported by the Deutsche Forschungsgemeinschaft via Research Unit FOR 1394. NR 64 TC 5 Z9 5 U1 1 U2 26 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1292-8941 EI 1292-895X J9 EUR PHYS J E JI Eur. Phys. J. E PD JAN 22 PY 2015 VL 38 IS 1 AR 1 DI 10.1140/epje/i2015-15001-0 PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Applied; Polymer Science SC Chemistry; Materials Science; Physics; Polymer Science GA AZ9XK UT WOS:000348567400001 PM 25612850 ER PT J AU Walen, H Liu, DJ Oh, J Lim, H Evans, JW Aikens, CM Kim, Y Thiel, PA AF Walen, Holly Liu, Da-Jiang Oh, Junepyo Lim, Hyunseob Evans, J. W. Aikens, Christine M. Kim, Yousoo Thiel, P. A. TI Cu2S3 complex on Cu(111) as a candidate for mass transport enhancement SO PHYSICAL REVIEW B LA English DT Article ID SCANNING TUNNELING MICROSCOPE; SURFACE SELF-DIFFUSION; METAL-SURFACES; SULFUR; APPROXIMATION; CATALYST; HYDROGEN; GROWTH; OXYGEN AB Sulfur-metal complexes, containing only a few atoms, can open new, highly efficient pathways for transport of metal atoms on surfaces. For example, they can accelerate changes in the shape and size of morphological features, such as two-dimensional nanoclusters, over time. In this study we perform STM under conditions that are designed to specifically isolate such complexes. We find a new, unexpected S-Cu complex on the Cu(111) surface, which we identify as Cu2S3. We propose that Cu2S3 enhances mass transport in this system, which contradicts a previous proposal based on Cu3S3. We analyze bonding within these Cu-S complexes, identifying a principle for stabilization of sulfur complexes on coinage metal surfaces. C1 [Walen, Holly; Thiel, P. A.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Liu, Da-Jiang; Evans, J. W.; Thiel, P. A.] US DOE, Ames Lab, Ames, IA 50011 USA. [Oh, Junepyo; Lim, Hyunseob; Kim, Yousoo] RIKEN, Surface & Interface Sci Lab, Wako, Saitama 3510198, Japan. [Evans, J. W.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Aikens, Christine M.] Kansas State Univ, Dept Chem, Manhattan, KS 66506 USA. [Thiel, P. A.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. RP Thiel, PA (reprint author), Iowa State Univ, Dept Chem, Ames, IA 50011 USA. EM pthiel@iastate.edu RI Lim, Hyunseob /K-1692-2015; Oh, Junepyo/M-3244-2016 OI Lim, Hyunseob /0000-0002-4956-4208; Oh, Junepyo/0000-0003-2452-3386 FU NSF [CHE-1111500]; Scientific Research on Priority Areas "Electron Transport Through a Linked Molecule in Nanoscale"; "Single Molecule Spectroscopy using Probe Microscope"; Ministry of Education, Culture, Sports, Science, and Technology (MEXT); Division of Chemical Sciences, Basic Energy Sciences, US Department of Energy (USDOE); National Energy Research Scientific Computing Center - Office of Science of the US Department of Energy [AC02-05CH11231]; National Science Foundation [CHE-1213771]; Henry Dreyfus Foundation FX The experimental component of this work was supported by several sources. From the U.S., it was NSF Grant CHE-1111500. From Japan, support was provided by a Grant-in- Aid for Scientific Research on Priority Areas "Electron Transport Through a Linked Molecule in Nanoscale"; and a Grant-in-Aid for Scientific Research(S) "Single Molecule Spectroscopy using Probe Microscope" from the Ministry of Education, Culture, Sports, Science, and Technology (MEXT). The theoretical analysis of kinetics was also supported by NSF Grant CHE-1111500. The DFT analysis of the energetics of chemisorbed complexes and of simulated STM images was supported by the Division of Chemical Sciences, Basic Energy Sciences, US Department of Energy (USDOE), and it utilized resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy (Contract No. DE-AC02-05CH11231). The theoretical molecular orbital analysis for gas phase species was supported by the National Science Foundation under Grant No. CHE-1213771. C.M.A. also thanks the Camille and Henry Dreyfus Foundation for a Camille Dreyfus Teacher-Scholar Award (2011-2016). We thank Kan Ueji and Hiroshi Imada for assistance with the experiments, and Gordon J. Miller for useful discussions. NR 30 TC 11 Z9 11 U1 4 U2 26 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 22 PY 2015 VL 91 IS 4 AR 045426 DI 10.1103/PhysRevB.91.045426 PG 7 WC Physics, Condensed Matter SC Physics GA CA1BT UT WOS:000348648500003 ER PT J AU Cui, YT Moore, RG Zhang, AM Tian, Y Lee, JJ Schmitt, FT Zhang, WH Li, W Yi, M Liu, ZK Hashimoto, M Zhang, Y Lu, DH Devereaux, TP Wang, LL Ma, XC Zhang, QM Xue, QK Lee, DH Shen, ZX AF Cui, Y. -T. Moore, R. G. Zhang, A. -M. Tian, Y. Lee, J. J. Schmitt, F. T. Zhang, W. -H. Li, W. Yi, M. Liu, Z. -K. Hashimoto, M. Zhang, Y. Lu, D. -H. Devereaux, T. P. Wang, L. -L. Ma, X. -C. Zhang, Q. -M. Xue, Q. -K. Lee, D. -H. Shen, Z. -X. TI Interface Ferroelectric Transition near the Gap-Opening Temperature in a Single-Unit-Cell FeSe Film Grown on Nb-Doped SrTiO3 Substrate SO PHYSICAL REVIEW LETTERS LA English DT Article ID RAMAN-SCATTERING; STRONTIUM-TITANATE; PHASE-TRANSITION; SUPERCONDUCTIVITY; SR1-XCAXTIO3; PEROVSKITE; ORIGIN AB We report findings of strong anomalies in both mutual inductance and inelastic Raman spectroscopy measurements of single-unit-cell FeSe film grown on Nb-doped SrTiO3, which occur near the temperature where the superconductinglike energy gap opens. Analysis suggests that the anomaly is associated with a broadened ferroelectric transition in a thin layer near the FeSe/SrTiO3 interface. The coincidence of the ferroelectric transition and gap-opening temperatures adds credence to the central role played by the film-substrate interaction on the strong Cooper pairing in this system. We discuss scenarios that could explain such a coincidence. C1 [Cui, Y. -T.; Moore, R. G.; Lee, J. J.; Schmitt, F. T.; Li, W.; Yi, M.; Liu, Z. -K.; Devereaux, T. P.; Shen, Z. -X.] Stanford Inst Mat & Energy Sci, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Zhang, A. -M.; Tian, Y.; Zhang, Q. -M.] Renmin Univ China, Dept Phys, Beijing 100872, Peoples R China. [Zhang, W. -H.; Wang, L. -L.; Ma, X. -C.; Xue, Q. -K.] Tsinghua Univ, Dept Phys, State Key Lab Low Dimens Quantum Phys, Beijing 100084, Peoples R China. [Hashimoto, M.; Zhang, Y.; Lu, D. -H.] Stanford Synchrotron Radiat Lightsource, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Zhang, Y.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Wang, L. -L.; Ma, X. -C.; Xue, Q. -K.] Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China. [Lee, D. -H.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Lee, D. -H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Cui, YT (reprint author), Stanford Inst Mat & Energy Sci, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. EM zxshen@stanford.edu RI Cui, Yong-Tao/G-8505-2015 OI Cui, Yong-Tao/0000-0002-8015-1049 FU Gordon and Betty Moore Foundation [GBMF3133]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science [DE-AC0205CH11231]; Ministry of Science and Technology; National Science Foundation of China FX We thank Yayu Wang for helpful discussions. The mutual inductance work is funded by the Gordon and Betty Moore Foundation through Grant No. GBMF3133 to Z.-X.S. The MBE and ARPES work is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science. ARPES measurements were performed at the Stanford Synchrotron Radiation Lightsource, a national user facility operated by Stanford University on behalf of the U. S. Department of Energy, Office of Basic Energy Sciences. D.-H. Lee is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science, under Quantum Material program DE-AC0205CH11231. L.-L. W, X.-C. M., Q.-M.Z., and Q.-K.X. are supported by Ministry of Science and Technology and National Science Foundation of China. NR 27 TC 11 Z9 12 U1 8 U2 118 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 22 PY 2015 VL 114 IS 3 AR 037002 DI 10.1103/PhysRevLett.114.037002 PG 5 WC Physics, Multidisciplinary SC Physics GA CA0AI UT WOS:000348576100017 PM 25659015 ER PT J AU Iskandar, W Matsumoto, J Leredde, A Flechard, X Gervais, B Guillous, S Hennecart, D Mery, A Rangama, J Zhou, CL Shiromaru, H Cassimi, A AF Iskandar, W. Matsumoto, J. Leredde, A. Flechard, X. Gervais, B. Guillous, S. Hennecart, D. Mery, A. Rangama, J. Zhou, C. L. Shiromaru, H. Cassimi, A. TI Interatomic Coulombic Decay as a New Source of Low Energy Electrons in Slow Ion-Dimer Collisions SO PHYSICAL REVIEW LETTERS LA English DT Article ID CLUSTERS; DNA; IMPACT; WATER AB We provide the experimental evidence that the single electron capture process in slow collisions between O3+ ions and neon dimer targets leads to an unexpected production of low-energy electrons. This production results from the interatomic Coulombic decay process, subsequent to inner-shell single electron capture from one site of the neon dimer. Although pure one-electron capture from the inner shell is expected to be negligible in the low collision energy regime investigated here, the electron production due to this process overtakes by 1 order of magnitude the emission of Auger electrons by the scattered projectiles after double-electron capture. This feature is specific to low charge states of the projectile: similar studies with Xe20+ and Ar9+ projectiles show no evidence of inner-shell single-electron capture. The dependence of the process on the projectile charge state is interpreted using simple calculations based on the classical over the barrier model. C1 [Iskandar, W.; Gervais, B.; Guillous, S.; Hennecart, D.; Mery, A.; Rangama, J.; Zhou, C. L.; Cassimi, A.] CEA CNRS ENSICAEN, CIMAP, F-14070 Caen 5, France. [Matsumoto, J.; Shiromaru, H.] Tokyo Metropolitan Univ, Dept Chem, Tokyo 1920397, Japan. [Leredde, A.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Flechard, X.] Univ Caen, ENSICAEN, LPC Caen, CNRS,IN2P3, F-14050 Caen 04, France. RP Iskandar, W (reprint author), CEA CNRS ENSICAEN, CIMAP, BP 5133, F-14070 Caen 5, France. EM iskandar@ganil.fr; flechard@lpccaen.in2p3.fr RI RANGAMA, Jimmy/O-9880-2015; OI RANGAMA, Jimmy/0000-0002-8083-6881; Iskandar, Wael/0000-0003-4604-4431 FU TMU Research Program FX We thank the CIMAP and GANIL staff for their technical support. This work was partly supported by TMU Research Program Grant. NR 22 TC 3 Z9 3 U1 2 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 22 PY 2015 VL 114 IS 3 AR 033201 DI 10.1103/PhysRevLett.114.033201 PG 5 WC Physics, Multidisciplinary SC Physics GA CA0AI UT WOS:000348576100007 PM 25658997 ER PT J AU Seder, E Biselli, A Pisano, S Niccolai, S Smith, GD Joo, K Adhikari, K Amaryan, MJ Anderson, MD Pereira, SA Avakian, H Battaglieri, M Bedlinskiy, I Bono, J Boiarinov, S Bosted, P Briscoe, W Brock, J Brooks, WK Bueltmann, S Burkert, VD Carman, DS Carlin, C Celentano, A Chandavar, S Charles, G Colaneri, L Cole, PL Contalbrigo, M Crabb, D Crede, V D'Angelo, A Dashyan, N De Vita, R De Sanctis, E Deur, A Djalali, C Doughty, D Dupre, R El Fassi, L Elouadrhiri, L Eugenio, P Fedotov, G Fegan, S Filippi, A Fleming, JA Fradi, A Garillon, B Garcon, M Gevorgyan, N Ghandilyan, Y Giovanetti, KL Girod, FX Goetz, JT Gohn, W Gothe, RW Griffioen, KA Guegan, B Guidal, M Guo, L Hafidi, K Hakobyan, H Hanretty, C Harrison, N Hattawy, M Saylor, NH Holtrop, M Hughes, SM Ilieva, Y Ireland, DG Ishkhanov, BS Isupov, EL Jo, HS Joosten, S Keith, CD Keller, D Khachatryan, G Khandaker, M Kim, A Kim, W Klein, A Klein, FJ Koirala, S Kubarovsky, V Kuhn, SE Lenisa, P Livingston, K Lu, HY MacGregor, IJD Markov, N Mayer, M McKinnon, B Meekins, DG Mineeva, T Mirazita, M Mokeev, V Montgomery, R Moody, CI Moutarde, H Movsisyan, A Camacho, CM Nadel-Turonski, P Niculescu, I Osipenko, M Ostrovidov, AI Paolone, M Pappalardo, LL Park, K Park, S Pasyuk, E Peng, P Phelps, W Pogorelko, O Price, JW Prok, Y Protopopescu, D Puckett, AJR Ripani, M Rizzo, A Rosner, G Rossi, P Roy, P Sabatie, F Salgado, C Schott, D Schumacher, RA Senderovich, I Simonyan, A Skorodumina, I Sokhan, D Sparveris, N Stepanyan, S Stoler, P Strakovsky, II Strauch, S Sytnik, V Taiuti, M Tang, W Tian, Y Ungaro, M Voskanyan, H Voutier, E Walford, NK Watts, DP Wei, X Weinstein, LB Wood, MH Zachariou, N Zana, L Zhang, J Zonta, I AF Seder, E. Biselli, A. Pisano, S. Niccolai, S. Smith, G. D. Joo, K. Adhikari, K. Amaryan, M. J. Anderson, M. D. Pereira, S. Anefalos Avakian, H. Battaglieri, M. Bedlinskiy, I. Bono, J. Boiarinov, S. Bosted, P. Briscoe, W. Brock, J. Brooks, W. K. Bueltmann, S. Burkert, V. D. Carman, D. S. Carlin, C. Celentano, A. Chandavar, S. Charles, G. Colaneri, L. Cole, P. L. Contalbrigo, M. Crabb, D. Crede, V. D'Angelo, A. Dashyan, N. De Vita, R. De Sanctis, E. Deur, A. Djalali, C. Doughty, D. Dupre, R. El Fassi, L. Elouadrhiri, L. Eugenio, P. Fedotov, G. Fegan, S. Filippi, A. Fleming, J. A. Fradi, A. Garillon, B. Garcon, M. Gevorgyan, N. Ghandilyan, Y. Giovanetti, K. L. Girod, F. X. Goetz, J. T. Gohn, W. Gothe, R. W. Griffioen, K. A. Guegan, B. Guidal, M. Guo, L. Hafidi, K. Hakobyan, H. Hanretty, C. Harrison, N. Hattawy, M. Saylor, N. Hirlinger Holtrop, M. Hughes, S. M. Ilieva, Y. Ireland, D. G. Ishkhanov, B. S. Isupov, E. L. Jo, H. S. Joosten, S. Keith, C. D. Keller, D. Khachatryan, G. Khandaker, M. Kim, A. Kim, W. Klein, A. Klein, F. J. Koirala, S. Kubarovsky, V. Kuhn, S. E. Lenisa, P. Livingston, K. Lu, H. Y. MacGregor, I. J. D. Markov, N. Mayer, M. McKinnon, B. Meekins, D. G. Mineeva, T. Mirazita, M. Mokeev, V. Montgomery, R. Moody, C. I. Moutarde, H. Movsisyan, A. Camacho, C. Munoz Nadel-Turonski, P. Niculescu, I. Osipenko, M. Ostrovidov, A. I. Paolone, M. Pappalardo, L. L. Park, K. Park, S. Pasyuk, E. Peng, P. Phelps, W. Pogorelko, O. Price, J. W. Prok, Y. Protopopescu, D. Puckett, A. J. R. Ripani, M. Rizzo, A. Rosner, G. Rossi, P. Roy, P. Sabatie, F. Salgado, C. Schott, D. Schumacher, R. A. Senderovich, I. Simonyan, A. Skorodumina, I. Sokhan, D. Sparveris, N. Stepanyan, S. Stoler, P. Strakovsky, I. I. Strauch, S. Sytnik, V. Taiuti, M. Tang, W. Tian, Y. Ungaro, M. Voskanyan, H. Voutier, E. Walford, N. K. Watts, D. P. Wei, X. Weinstein, L. B. Wood, M. H. Zachariou, N. Zana, L. Zhang, J. Zonta, I. CA CLAS Collaboration TI Longitudinal Target-Spin Asymmetries for Deeply Virtual Compton Scattering SO PHYSICAL REVIEW LETTERS LA English DT Article ID GENERALIZED PARTON DISTRIBUTIONS; ELECTRON-SCATTERING; FORM-FACTORS; NUCLEON; IMPACT; CLAS AB A measurement of the electroproduction of photons off protons in the deeply inelastic regime was performed at Jefferson Lab using a nearly 6 GeV electron beam, a longitudinally polarized proton target, and the CEBAF Large Acceptance Spectrometer. Target-spin asymmetries for ep. e'p'gamma. events, which arise from the interference of the deeply virtual Compton scattering and the Bethe-Heitler processes, were extracted over the widest kinematics in Q(2), x(B), t, and phi, for 166 four-dimensional bins. In the framework of generalized parton distributions, at leading twist the t dependence of these asymmetries provides insight into the spatial distribution of the axial charge of the proton, which appears to be concentrated in its center. These results also bring important and necessary constraints for the existing parametrizations of chiral-even generalized parton distributions. C1 [Seder, E.; Joo, K.; Gohn, W.; Harrison, N.; Markov, N.; Mineeva, T.; Puckett, A. J. R.; Ungaro, M.] Univ Connecticut, Storrs, CT 06269 USA. [Seder, E.; Garcon, M.; Girod, F. X.; Moutarde, H.; Sabatie, F.] CEA, Ctr Saclay, Irfu Serv Phys Nucl, F-91191 Gif Sur Yvette, France. [Biselli, A.] Fairfield Univ, Fairfield, CT 06824 USA. [Pisano, S.; Pereira, S. Anefalos; De Sanctis, E.; Mirazita, M.; Montgomery, R.; Rossi, P.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Pisano, S.; Niccolai, S.; Charles, G.; Dupre, R.; Fradi, A.; Garillon, B.; Guegan, B.; Guidal, M.; Hattawy, M.; Jo, H. S.; Camacho, C. Munoz] Inst Phys Nucl, F-91406 Orsay, France. [Smith, G. D.; Anderson, M. D.; Fegan, S.; Ireland, D. G.; Livingston, K.; MacGregor, I. J. D.; McKinnon, B.; Protopopescu, D.; Rosner, G.; Sokhan, D.] Univ Glasgow, Glasgow G12 8QQ, Lanark, Scotland. [Smith, G. D.; Fleming, J. A.; Hughes, S. M.; Sokhan, D.; Watts, D. P.; Zana, L.] Univ Edinburgh, Edinburgh EH9 3JZ, Midlothian, Scotland. [Adhikari, K.; Amaryan, M. J.; Bueltmann, S.; El Fassi, L.; Klein, A.; Koirala, S.; Kuhn, S. E.; Mayer, M.; Prok, Y.; Weinstein, L. B.; Zhang, J.] Old Dominion Univ, Norfolk, VA 23529 USA. [Avakian, H.; Boiarinov, S.; Bosted, P.; Brock, J.; Burkert, V. D.; Carman, D. S.; Carlin, C.; Deur, A.; Doughty, D.; Elouadrhiri, L.; Girod, F. X.; Keith, C. D.; Kubarovsky, V.; Meekins, D. G.; Mokeev, V.; Nadel-Turonski, P.; Park, K.; Pasyuk, E.; Rossi, P.; Stepanyan, S.; Ungaro, M.; Wei, X.; Zhang, J.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Battaglieri, M.; Celentano, A.; De Vita, R.; Fegan, S.; Osipenko, M.; Ripani, M.; Taiuti, M.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Bedlinskiy, I.; Pogorelko, O.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Bono, J.; Guo, L.; Phelps, W.; Schott, D.] Florida Int Univ, Miami, FL 33199 USA. [Bosted, P.; Griffioen, K. A.] Coll William & Mary, Williamsburg, VA 23187 USA. [Briscoe, W.; Schott, D.; Strakovsky, I. I.] George Washington Univ, Washington, DC 20052 USA. [Brooks, W. K.; Hakobyan, H.; Sytnik, V.] Univ Tecn Federico Santa Maria, Valparaiso, Chile. [Chandavar, S.; Goetz, J. T.; Keller, D.; Tang, W.] Ohio Univ, Athens, OH 45701 USA. [Colaneri, L.; D'Angelo, A.; Rizzo, A.; Zonta, I.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, I-00133 Rome, Italy. [Cole, P. L.; Khandaker, M.] Idaho State Univ, Pocatello, ID 83209 USA. [Contalbrigo, M.; Lenisa, P.; Movsisyan, A.; Pappalardo, L. L.] Ist Nazl Fis Nucl, Sez Ferrara, I-44100 Ferrara, Italy. [Crabb, D.; Crede, V.; Hanretty, C.; Keller, D.; Peng, P.] Univ Virginia, Charlottesville, VA 22901 USA. [Eugenio, P.; Ostrovidov, A. I.; Park, S.; Roy, P.] Florida State Univ, Tallahassee, FL 32306 USA. [D'Angelo, A.] Univ Roma Tor Vergata, I-00133 Rome, Italy. [Dashyan, N.; Gevorgyan, N.; Ghandilyan, Y.; Hakobyan, H.; Khachatryan, G.; Simonyan, A.; Voskanyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Djalali, C.; Fedotov, G.; Gothe, R. W.; Ilieva, Y.; Lu, H. Y.; Park, K.; Skorodumina, I.; Strauch, S.; Tian, Y.; Wood, M. H.; Zachariou, N.] Univ S Carolina, Columbia, SC 29208 USA. [Doughty, D.] Christopher Newport Univ, Newport News, VA 23606 USA. [Dupre, R.; Hafidi, K.; Moody, C. I.] Argonne Natl Lab, Argonne, IL 60439 USA. [Fedotov, G.; Ishkhanov, B. S.; Isupov, E. L.; Mokeev, V.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow 119234, Russia. [Filippi, A.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Giovanetti, K. L.; Niculescu, I.] James Madison Univ, Harrisonburg, VA 22807 USA. [Saylor, N. Hirlinger; Stoler, P.] Rensselaer Polytech Inst, Troy, NY 12180 USA. [Holtrop, M.] Univ New Hampshire, Durham, NH 03824 USA. [Joosten, S.; Paolone, M.; Sparveris, N.] Temple Univ, Philadelphia, PA 19122 USA. [Khandaker, M.; Salgado, C.] Norfolk State Univ, Norfolk, VA 23504 USA. [Kim, A.; Kim, W.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Klein, F. J.; Nadel-Turonski, P.; Walford, N. K.] Catholic Univ Amer, Washington, DC 20064 USA. [Pasyuk, E.; Senderovich, I.] Arizona State Univ, Tempe, AZ 85287 USA. [Price, J. W.] Calif State Univ Dominguez Hills, Carson, CA 90747 USA. [Schumacher, R. A.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Taiuti, M.] Univ Genoa, I-16146 Genoa, Italy. [Voutier, E.] Univ Grenoble Alps, CNRS, IN2P3, LPSC, Grenoble, France. [Wood, M. H.] Canisius Coll, Buffalo, NY 14208 USA. RP Niccolai, S (reprint author), Inst Phys Nucl, BP 1, F-91406 Orsay, France. EM silvia@jlab.org RI Brooks, William/C-8636-2013; MacGregor, Ian/D-4072-2011; Sabatie, Franck/K-9066-2015; Schumacher, Reinhard/K-6455-2013; Osipenko, Mikhail/N-8292-2015; Zhang, Jixie/A-1461-2016; Celentano, Andrea/J-6190-2012; D'Angelo, Annalisa/A-2439-2012 OI Brooks, William/0000-0001-6161-3570; Sabatie, Franck/0000-0001-7031-3975; Schumacher, Reinhard/0000-0002-3860-1827; Osipenko, Mikhail/0000-0001-9618-3013; Celentano, Andrea/0000-0002-7104-2983; D'Angelo, Annalisa/0000-0003-3050-4907 FU U. S. Department of Energy [DE-FG02-96ER40950, DE-AC05-06OR23177]; National Science Foundation; French Centre National de la Recherche Scientifique and Commissariat a l'Energie Atomique; French-American Cultural Exchange (FACE); Italian Istituto Nazionale di Fisica Nucleare; Chilean Comision Nacional de Investigacion Cientifica y Tecnologica (CONICYT); National Research Foundation of Korea; UK Science and Technology Facilities Council (STFC) FX We thank the staff of the Accelerator and Physics Divisions and of the Target Group at Jefferson Lab for making the experiment possible. We give special thanks to M. Guidal, F. Sabatie, S. Liuti, D. Muller, and K. Kumericki for the theoretical support. This work was supported in part by the U. S. Department of Energy (No. DE-FG02-96ER40950) and National Science Foundation, the French Centre National de la Recherche Scientifique and Commissariat a l'Energie Atomique, the French-American Cultural Exchange (FACE), the Italian Istituto Nazionale di Fisica Nucleare, the Chilean Comision Nacional de Investigacion Cientifica y Tecnologica (CONICYT), the National Research Foundation of Korea, and the UK Science and Technology Facilities Council (STFC). The Jefferson Science Associates (JSA) operates the Thomas Jefferson National Accelerator Facility for the U. S. Department of Energy under Contract No. DE-AC05-06OR23177. NR 35 TC 15 Z9 15 U1 0 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 22 PY 2015 VL 114 IS 3 AR 032001 DI 10.1103/PhysRevLett.114.032001 PG 7 WC Physics, Multidisciplinary SC Physics GA CA0AI UT WOS:000348576100006 PM 25658994 ER PT J AU Cheaito, R Gaskins, JT Caplan, ME Donovan, BF Foley, BM Giri, A Duda, JC Szwejkowski, CJ Constantin, C Brown-Shaklee, HJ Ihlefeld, JF Hopkins, PE AF Cheaito, Ramez Gaskins, John T. Caplan, Matthew E. Donovan, Brian F. Foley, Brian M. Giri, Ashutosh Duda, John C. Szwejkowski, Chester J. Constantin, Costel Brown-Shaklee, Harlan J. Ihlefeld, Jon F. Hopkins, Patrick E. TI Thermal boundary conductance accumulation and interfacial phonon transmission: Measurements and theory SO PHYSICAL REVIEW B LA English DT Article ID LATTICE-DYNAMICS; MOLECULAR-DYNAMICS; HEAT-FLOW; DOMAIN THERMOREFLECTANCE; DISPERSION CURVES; CRYSTAL DYNAMICS; MISMATCH MODEL; RESISTANCE; CONDUCTIVITY; TRANSPORT AB The advances in phonon spectroscopy in homogeneous solids have unveiled extremely useful physics regarding the contribution of phonon energies and mean-free paths to the thermal transport in solids. However, as material systems decrease to length scales less than the phonon mean-free paths, thermal transport can become much more impacted by scattering and transmission across interfaces between two materials than the intrinsic relaxation in the homogeneous solid. To elucidate the fundamental interactions driving this thermally limiting interfacial phonon scattering process, we analytically derive and experimentally measure a thermal boundary conductance accumulation function. We develop a semiclassical theory to calculate the thermal boundary conductance accumulation function across interfaces using the diffuse mismatch model, and validate this derivation by measuring the interface conductance between eight different metals on native oxide/silicon substrates and four different metals on sapphire substrates. Measurements were performed at room temperature using time-domain thermoreflectance and represent the first-reported values for interface conductance across several metal/native oxide/silicon and metal/sapphire interfaces. The various metal films provide a variable bandwidth of phonons incident on the metal/substrate interface. This method of varying phonons' cutoff frequency in the film while keeping the same substrate allows us to mimic the accumulation of thermal boundary conductance and thus provides a direct method to experimentally validate our theory. We show that the accumulation function can be written as the product of a weighted average of the interfacial phonon transmission function and the accumulation of the temperature derivative of the phonon flux incident on the interface; this provides the framework to extract an average, spectrally dependent phonon transmissivity from a series of thermal boundary conductance measurements. Our approach provides a platform for analyzing the spectral phononic contribution to interfacial thermal transport in our experimentally measured data of metal/substrate thermal boundary conductance. Based on the assumptions made in this work and the measurement results on different metals on native oxide/silicon and sapphire substrates, we demonstrate that high-frequency phonons dictate the transport across metal/Si interfaces, especially in low Debye temperature metals with low-cutoff frequencies. C1 [Cheaito, Ramez; Gaskins, John T.; Caplan, Matthew E.; Donovan, Brian F.; Foley, Brian M.; Giri, Ashutosh; Duda, John C.; Szwejkowski, Chester J.; Hopkins, Patrick E.] Univ Virginia, Dept Mech & Aerosp Engn, Charlottesville, VA 22904 USA. [Constantin, Costel] James Madison Univ, Dept Phys & Astron, Harrisonburg, VA 22807 USA. [Brown-Shaklee, Harlan J.; Ihlefeld, Jon F.] Sandia Natl Labs, Elect Opt & Nanomat Dept, Albuquerque, NM 87185 USA. RP Cheaito, R (reprint author), Seagate Technol, Bloomington, MN 55435 USA. EM phopkins@virginia.edu FU Office of Naval Research, Young Investigator Program [N00014-13-4-0528]; Commonwealth Research Commercialization Fund (CRCF) of Virginia; 4-VA mini-grant; Financial Assistance Award - U.S. Department of Commerce Economic Development Administration [01-79-14214]; U.S. Department of Energy National Nuclear Security Administration [DE-AC04-94AL85000] FX Authors acknowledge Bilal Cheaito for the useful discussion on the mean value theorem. Authors would like to thank M. Blea-Kirby from Sandia National Laboratories for her assistance in film deposition. This work was supported by the Office of Naval Research, Young Investigator Program (No. N00014-13-4-0528), Commonwealth Research Commercialization Fund (CRCF) of Virginia, and the 4-VA mini-grant for university collaboration in the Commonwealth of Virginia. This project was supported by Financial Assistance Award No. 01-79-14214, awarded by U.S. Department of Commerce Economic Development Administration, to the University of Virginia. The content is solely the responsibility of the authors and does not necessarily represent the official views of the U.S. Department of Commerce Economic Development Administration. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 113 TC 14 Z9 14 U1 13 U2 63 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JAN 22 PY 2015 VL 91 IS 3 AR 035432 DI 10.1103/PhysRevB.91.035432 PG 12 WC Physics, Condensed Matter SC Physics GA CA1BS UT WOS:000348648400002 ER PT J AU Arguello, CJ Rosenthal, EP Andrade, EF Jin, W Yeh, PC Zaki, N Jia, S Cava, RJ Fernandes, RM Millis, AJ Valla, T Osgood, RM Pasupathy, AN AF Arguello, C. J. Rosenthal, E. P. Andrade, E. F. Jin, W. Yeh, P. C. Zaki, N. Jia, S. Cava, R. J. Fernandes, R. M. Millis, A. J. Valla, T. Osgood, R. M., Jr. Pasupathy, A. N. TI Quasiparticle Interference, Quasiparticle Interactions, and the Origin of the Charge Density Wave in 2H-NbSe2 SO PHYSICAL REVIEW LETTERS LA English DT Article ID SCANNING-TUNNELING-MICROSCOPE; BI2SR2CACU2O8+DELTA; SUPERLATTICE; INSTABILITY; MECHANISM; STATES AB We show that a small number of intentionally introduced defects can be used as a spectroscopic tool to amplify quasiparticle interference in 2H-NbSe2 that we measure by scanning tunneling spectroscopic imaging. We show, from the momentum and energy dependence of the quasiparticle interference, that Fermi surface nesting is inconsequential to charge density wave formation in 2H-NbSe2. We demonstrate that, by combining quasiparticle interference data with additional knowledge of the quasiparticle band structure from angle resolved photoemission measurements, one can extract the wave vector and energy dependence of the important electronic scattering processes thereby obtaining direct information both about the fermiology and the interactions. In 2H-NbSe2, we use this combination to confirm that the important near-Fermi-surface electronic physics is dominated by the coupling of the quasiparticles to soft mode phonons at a wave vector different from the charge density wave ordering wave vector. C1 [Arguello, C. J.; Rosenthal, E. P.; Andrade, E. F.; Millis, A. J.; Pasupathy, A. N.] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Jin, W.; Yeh, P. C.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. [Zaki, N.; Osgood, R. M., Jr.] Columbia Univ, Dept Elect Engn, New York, NY 10027 USA. [Jia, S.; Cava, R. J.; Osgood, R. M., Jr.] Princeton Univ, Dept Chem, Princeton, NJ 08540 USA. [Fernandes, R. M.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Valla, T.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Arguello, CJ (reprint author), Columbia Univ, Dept Phys, 538 W 120th St, New York, NY 10027 USA. RI Fernandes, Rafael/E-9273-2010 FU National Science Foundation (NSF) [DMR-1056527]; Materials Interdisciplinary Research Team Grant [DMR-1122594]; U.S. Department of Energy [DE-FG 02-04-ER-46157, DE-SC0012336]; U.S. Department of Energy, Office of Basic Energy Sciences (DOE-BES) [DE-AC02-98CH10886]; DOE-BES [DE-FG02-98ER45706]; NSF [1066293] FX This work was supported by the National Science Foundation (NSF) under Grant No. DMR-1056527 (E. P. R., A. N. P.) and by the Materials Interdisciplinary Research Team Grant No. DMR-1122594 (A. N. P., A. J. M.). Salary support was also provided by the U.S. Department of Energy under Contracts No. DE-FG 02-04-ER-46157 (W. J., P. C. Y., N. Z., and R. M. O.). R. M. F. is supported by the U.S. Department of Energy under Award No. DE-SC0012336. ARPES research carried out at National Synchrotron Light Source, Brookhaven National Laboratory is supported by the U.S. Department of Energy, Office of Basic Energy Sciences (DOE-BES), under Contract No. DE-AC02-98CH10886. The crystal growth work at Princeton University was funded by DOE-BES Grant No. DE-FG02-98ER45706. A. J. M. acknowledges the hospitality of the Aspen Center for Physics (supported by NSF Grant No. 1066293) for hospitality during the conception and writing of this Letter. NR 32 TC 11 Z9 11 U1 8 U2 69 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 21 PY 2015 VL 114 IS 3 AR 037001 DI 10.1103/PhysRevLett.114.037001 PG 5 WC Physics, Multidisciplinary SC Physics GA CE9BG UT WOS:000352137700006 PM 25659014 ER PT J AU Bedaque, P Steiner, AW AF Bedaque, Paulo Steiner, Andrew W. TI Sound Velocity Bound and Neutron Stars SO PHYSICAL REVIEW LETTERS LA English DT Article ID EQUATION-OF-STATE; MASS-RADIUS RELATION; SYMMETRY ENERGY; CONSTRAINTS; MATTER AB It has been conjectured that the velocity of sound in any medium is smaller than the velocity of light in vacuum divided by root 3. Simple arguments support this bound in nonrelativistic and/or weakly coupled theories. The bound has been demonstrated in several classes of strongly coupled theories with gravity duals and is saturated only in conformal theories. We point out that the existence of neutron stars with masses around two solar masses combined with the knowledge of the equation of state of hadronic matter at "low" densities is in strong tension with this bound. C1 [Bedaque, Paulo] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Steiner, Andrew W.] Univ Washington, Inst Nucl Theory, Seattle, WA 98195 USA. [Steiner, Andrew W.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Steiner, Andrew W.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. RP Bedaque, P (reprint author), Univ Maryland, Dept Phys, College Pk, MD 20742 USA. OI Steiner, Andrew/0000-0003-2478-4017 FU U.S. Department of Energy Office of Science, Office of Nuclear Physics [DE-FG02-93ER-40762] FX The authors would like to thank Aleksey Cherman, Tom Cohen, Aleksi Kurkela, Shmuel Nussinov, Sanjay Reddy, and Aleksi Vuorinen for conversations on the topic. This material is based upon work supported by the U.S. Department of Energy Office of Science, Office of Nuclear Physics under Award No. DE-FG02-93ER-40762. NR 33 TC 18 Z9 18 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 21 PY 2015 VL 114 IS 3 AR 031103 DI 10.1103/PhysRevLett.114.031103 PG 5 WC Physics, Multidisciplinary SC Physics GA CE9BG UT WOS:000352137700001 PM 25658990 ER PT J AU Fuhrman, WT Leiner, J Nikolic, P Granroth, GE Stone, MB Lumsden, MD DeBeer-Schmitt, L Alekseev, PA Mignot, JM Koohpayeh, SM Cottingham, P Phelan, WA Schoop, L McQueen, TM Broholm, C AF Fuhrman, W. T. Leiner, J. Nikolic, P. Granroth, G. E. Stone, M. B. Lumsden, M. D. DeBeer-Schmitt, L. Alekseev, P. A. Mignot, J. -M. Koohpayeh, S. M. Cottingham, P. Phelan, W. Adam Schoop, L. McQueen, T. M. Broholm, C. TI Interaction Driven Subgap Spin Exciton in the Kondo Insulator SmB6 SO PHYSICAL REVIEW LETTERS LA English DT Article ID MAGNETIC EXCITATIONS; MIXED-VALENCE; SEMICONDUCTORS; LATTICE AB Using inelastic neutron scattering, we map a 14 meV coherent resonant mode in the topological Kondo insulator SmB6 and describe its relation to the low energy insulating band structure. The resonant intensity is confined to the X and R high symmetry points, repeating outside the first Brillouin zone and dispersing less than 2 meV, with a 5d-like magnetic form factor. We present a slave-boson treatment of the Anderson Hamiltonian with a third neighbor dominated hybridized band structure. This approach produces a spin exciton below the charge gap with features that are consistent with the observed neutron scattering. We find that maxima in the wave vector dependence of the inelastic neutron scattering indicate band inversion. C1 [Fuhrman, W. T.; Nikolic, P.; Koohpayeh, S. M.; Cottingham, P.; Phelan, W. Adam; Schoop, L.; McQueen, T. M.; Broholm, C.] Johns Hopkins Univ, Inst Quantum Matter, Baltimore, MD 21218 USA. [Fuhrman, W. T.; Nikolic, P.; Koohpayeh, S. M.; Cottingham, P.; Phelan, W. Adam; Schoop, L.; McQueen, T. M.; Broholm, C.] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Leiner, J.; Stone, M. B.; Lumsden, M. D.; Broholm, C.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Nikolic, P.] George Mason Univ, Sch Phys Astron & Computat Sci, Fairfax, VA 22030 USA. [Granroth, G. E.] Oak Ridge Natl Lab, Neutron Data Anal & Visualizat Div, Oak Ridge, TN 37831 USA. [DeBeer-Schmitt, L.] Oak Ridge Natl Lab, Instrument Source Div, Oak Ridge, TN 37831 USA. [Alekseev, P. A.] Natl Res Ctr, Kurchatov Inst, Moscow 123182, Russia. [Alekseev, P. A.] Natl Res Nucl Univ MEPhI, Moscow 115409, Russia. [Mignot, J. -M.] CEA Saclay, CEA CNRS, Lab Leon Brillouin, F-91191 Gif Sur Yvette, France. [Cottingham, P.; Phelan, W. Adam; McQueen, T. M.] Johns Hopkins Univ, Dept Chem, Baltimore, MD 21218 USA. [Schoop, L.] Princeton Univ, Dept Chem, Princeton, NJ 08540 USA. [McQueen, T. M.; Broholm, C.] Johns Hopkins Univ, Dept Mat Sci & Engn, Baltimore, MD 21218 USA. RP Fuhrman, WT (reprint author), Johns Hopkins Univ, Inst Quantum Matter, Baltimore, MD 21218 USA. EM wesleytf@gmail.com; leinerjc@ornl.gov RI Stone, Matthew/G-3275-2011; Schoop, Leslie/A-4627-2013; DeBeer-Schmitt, Lisa/I-3313-2015; Granroth, Garrett/G-3576-2012; Lumsden, Mark/F-5366-2012 OI Stone, Matthew/0000-0001-7884-9715; Schoop, Leslie/0000-0003-3459-4241; DeBeer-Schmitt, Lisa/0000-0001-9679-3444; Granroth, Garrett/0000-0002-7583-8778; Lumsden, Mark/0000-0002-5472-9660 FU UT-Battelle LDRD [3211-2440]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Material Sciences and Engineering [DE-FG02-08ER46544]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; RFBR [14-22-01002] FX This project was supported by UT-Battelle LDRD #3211-2440. The work at IQM was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Material Sciences and Engineering under Grant No. DE-FG02-08ER46544. Research conducted at ORNL's SNS was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. P. A. A. is grateful to RFBR Grant No. 14-22-01002 for the partial support of participation in this work. The authors thank Martin Mourigal, Yuan Wan, and Ari Turner for fruitful discussions. NR 45 TC 27 Z9 27 U1 8 U2 52 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 21 PY 2015 VL 114 IS 3 AR 036401 DI 10.1103/PhysRevLett.114.036401 PG 5 WC Physics, Multidisciplinary SC Physics GA CE9BG UT WOS:000352137700004 PM 25659009 ER PT J AU D'Ammando, F Orienti, M Finke, J Raiteri, CM Hovatta, T Larsson, J Max-Moerbeck, W Perkins, J Readhead, ACS Richards, JL Beilicke, M Benbow, W Berger, K Bird, R Bugaev, V Cardenzana, JV Cerruti, M Chen, X Ciupik, L Dickinson, HJ Eisch, JD Errando, M Falcone, A Finley, JP Fleischhack, H Fortin, P Fortson, L Furniss, A Gerard, L Gillanders, GH Griffiths, ST Grube, J Gyuk, G Hakansson, N Holder, J Humensky, TB Kar, P Kertzman, M Khassen, Y Kieda, D Krennrich, F Kumar, S Lang, MJ Maier, G McCann, A Meagher, K Moriarty, P Mukherjee, R Nieto, D de Bhroithe, AO Ong, RA Otte, AN Pohl, M Popkow, A Prokoph, H Pueschel, E Quinn, J Ragan, K Reynolds, PT Richards, GT Roache, E Rousselle, J Santander, M Sembroski, GH Smith, AW Staszak, D Telezhinsky, I Tucci, JV Tyler, J Varlotta, A Vassiliev, VV Wakely, SP Weinstein, A Welsing, R Williams, DA Zitzer, B AF D'Ammando, F. Orienti, M. Finke, J. Raiteri, C. M. Hovatta, T. Larsson, J. Max-Moerbeck, W. Perkins, J. Readhead, A. C. S. Richards, J. L. Beilicke, M. Benbow, W. Berger, K. Bird, R. Bugaev, V. Cardenzana, J. V. Cerruti, M. Chen, X. Ciupik, L. Dickinson, H. J. Eisch, J. D. Errando, M. Falcone, A. Finley, J. P. Fleischhack, H. Fortin, P. Fortson, L. Furniss, A. Gerard, L. Gillanders, G. H. Griffiths, S. T. Grube, J. Gyuk, G. Hakansson, N. Holder, J. Humensky, T. B. Kar, P. Kertzman, M. Khassen, Y. Kieda, D. Krennrich, F. Kumar, S. Lang, M. J. Maier, G. McCann, A. Meagher, K. Moriarty, P. Mukherjee, R. Nieto, D. de Bhroithe, A. O'Faolain Ong, R. A. Otte, A. N. Pohl, M. Popkow, A. Prokoph, H. Pueschel, E. Quinn, J. Ragan, K. Reynolds, P. T. Richards, G. T. Roache, E. Rousselle, J. Santander, M. Sembroski, G. H. Smith, A. W. Staszak, D. Telezhinsky, I. Tucci, J. V. Tyler, J. Varlotta, A. Vassiliev, V. V. Wakely, S. P. Weinstein, A. Welsing, R. Williams, D. A. Zitzer, B. CA VERITAS Collaboration TI The most powerful flaring activity from the NLSyl PMN J0948+0022 SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE galaxies: active-galaxies: individual: PMN J0948+0022; galaxies: nuclei; galaxies: Seyfert; gamma-rays: general ID LINE SEYFERT 1; GAMMA-RAY EMISSION; LARGE-AREA TELESCOPE; QUASAR PKS 1510-089; EXTRAGALACTIC BACKGROUND LIGHT; SPECTRUM RADIO QUASARS; GALACTIC NUCLEI; X-RAY; MULTIWAVELENGTH OBSERVATIONS; RELATIVISTIC JETS AB We report on multifrequency observations performed during 2012 December-2013 August of the first narrow-line Seyfert 1 galaxy detected in gamma-rays, PMN J0948+0022 (z = 0.5846). A y -ray flare was observed by the Large Area Telescope on board Fermi during 2012 December-2013 January, reaching a daily peak flux in the 0.1-100 GeV energy range of (155 31) x 10 8 ph cm(-2) S-1 on 2013 January 1, corresponding to an apparent isotropic luminosity of similar to 1.5 x 1048 erg s(-1). The y -ray flaring period triggered Swift and Very Energetic Radiation Imaging Telescope Array System (VERITAS) observations in addition to radio and optical monitoring by Owens Valley Radio Observatory, Monitoring Of Jets in Active galactic nuclei with VLBA Experiments, and Catalina Real-time Transient Survey. A strong flare was observed in optical, UV, and X-rays on 2012 December 30, quasi-simultaneously to the y -ray flare, reaching a record flux for this source from optical to y gamma-rays. VERITAS observations at very high energy (E > 100 GeV) during 2013 January 6-17 resulted in an upper limit of F>0.2 Trev < 4.0 x 10(-12) ph cm(-2) s(-1). We compared the spectral energy distribution (SED) of the flaring state in 2013 January with that of an intermediate state observed in 2011. The two SEDs, modelled as synchrotron emission and an external Compton scattering of seed photons from a dust torus, can be modelled by changing both the electron distribution parameters and the magnetic field. C1 [D'Ammando, F.] Univ Bologna, Dipartimento Fis & Astron, I-40127 Bologna, Italy. [D'Ammando, F.] Inaf Ist Radioastron, I-40129 Bologna, Italy. [Finke, J.] US Naval Res Lab, Washington, DC 20375 USA. [Raiteri, C. M.] INAF Osservatorio Astrofis Torino, I-10025 Pino Torinese, TO, Italy. [Hovatta, T.; Readhead, A. C. S.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Larsson, J.] KTH, Dept Phys, SE-10691 Stockholm, Sweden. [Larsson, J.] KTH, Oskar Klein Ctr, SE-10691 Stockholm, Sweden. [Max-Moerbeck, W.] Natl Radio Astron Observ NRAO, Socorro, NM 87801 USA. [Perkins, J.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Richards, J. L.; Finley, J. P.; Sembroski, G. H.; Tucci, J. V.; Varlotta, A.] Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA. [Beilicke, M.; Bugaev, V.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Benbow, W.; Cerruti, M.; Fortin, P.; Roache, E.] Harvard Smithsonian Ctr Astrophys, Fred Lawrence Whipple Observ, Amado, AZ 85645 USA. [Berger, K.; Holder, J.; Kumar, S.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [Berger, K.; Holder, J.; Kumar, S.] Univ Delaware, Bartol Res Inst, Newark, DE 19716 USA. [Bird, R.; Khassen, Y.; Pueschel, E.; Quinn, J.] Univ Coll Dublin, Sch Phys, Dublin 4, Ireland. [Cardenzana, J. V.; Dickinson, H. J.; Eisch, J. D.; Krennrich, F.; Weinstein, A.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Chen, X.; Hakansson, N.; Pohl, M.; Telezhinsky, I.] Univ Potsdam, Inst Phys & Astron, D-14476 Potsdam, Germany. [Chen, X.; Fleischhack, H.; Gerard, L.; Maier, G.; de Bhroithe, A. O'Faolain; Pohl, M.; Prokoph, H.; Telezhinsky, I.; Welsing, R.] DESY, D-15738 Zeuthen, Germany. [Ciupik, L.; Grube, J.; Gyuk, G.] Adler Planetarium & Astron Museum, Dept Astron, Chicago, IL 60605 USA. [Errando, M.; Mukherjee, R.; Santander, M.] Columbia Univ, Barnard Coll, Dept Phys & Astron, New York, NY 10027 USA. [Falcone, A.] Penn State Univ, Dept Astron & Astrophys, Davey Lab 525, University Pk, PA 16802 USA. [Fortson, L.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Furniss, A.; Williams, D. A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Furniss, A.; Williams, D. A.] Univ Calif Santa Cruz, Dept Phys, Santa Cruz, CA 95064 USA. [Gillanders, G. H.; Lang, M. J.; Moriarty, P.] Natl Univ Ireland Galway, Sch Phys, Galway, Ireland. [Griffiths, S. T.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Humensky, T. B.; Nieto, D.] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Kar, P.; Kieda, D.; Smith, A. W.] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. [Kertzman, M.] Depauw Univ, Dept Phys & Astron, Greencastle, IN 46135 USA. [McCann, A.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Meagher, K.; Otte, A. N.; Richards, G. T.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Meagher, K.; Otte, A. N.; Richards, G. T.] Georgia Inst Technol, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Ong, R. A.; Popkow, A.; Rousselle, J.; Vassiliev, V. V.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Ragan, K.; Staszak, D.; Tyler, J.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Reynolds, P. T.] Cork Inst Technol, Dept Appl Phys & Instrumentat, Cork, Ireland. [Wakely, S. P.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Zitzer, B.] Argonne Natl Lab, Argonne, IL 60439 USA. RP D'Ammando, F (reprint author), Univ Bologna, Dipartimento Fis & Astron, Viale Berti Pichat 6-2, I-40127 Bologna, Italy. EM dammando@ira.inaf.it; dammando@ira.inaf.it; dammando@ira.inaf.it; dammando@ira.inaf.it; dammando@ira.inaf.it; dammando@ira.inaf.it; dammando@ira.inaf.it RI Nieto, Daniel/J-7250-2015 OI Nieto, Daniel/0000-0003-3343-0755 FU US Department of Energy Office of Science; Smithsonian Institution; NSERC in Canada; Science Foundation Ireland [SFI 10/RFP/AST2748]; Science and Technology Facilities Council in the UK; NASA [NNX08AW31G, NNX11A043G]; NSF [AST-0808050, AST-1109911]; US National Science Foundation [AST-0909182]; Fermi Guest Investigator grants [NNX08AW56G, NNX09AU10G, NNX12AO93G] FX The VERITAS Collaboration is grateful to Trevor Weekes for his seminal contributions and leadership in the field of VHE gamma-ray astrophysics, which made this study possible. The work of the VERITAS Collaboration is supported by grants from the US Department of Energy Office of Science, the US National Science Foundation, and the Smithsonian Institution, by NSERC in Canada, by Science Foundation Ireland (SFI 10/RFP/AST2748) and by the Science and Technology Facilities Council in the UK. We acknowledge the excellent work of the technical support staff at the Fred Lawrence Whipple Observatory and at the collaborating institutions in the construction and operation of the instrument.; We thank the Swift team for making these observations possible, the duty scientists, and science planners. The OVRO 40 m monitoring programme is supported in part by NASA grants NNX08AW31G and NNX11A043G, and NSF grants AST-0808050 and AST-1109911. The CRTS survey is supported by the US National Science Foundation under grants AST-0909182. This research has made use of data from the MOJAVE data base that is maintained by the MOJAVE team (Lister et al. 2009). Data from the Steward Observatory spectropolarimetric monitoring project were used. This programme is supported by Fermi Guest Investigator grants NNX08AW56G, NNX09AU10G, and NNX12AO93G. The National Radio Astronomy Observatory is a facility of the National Science Foundation operated under cooperative agreement by Associated Universities, Inc. We thank F. Schinzel, S. Digel, P. Bruel, and the referee, Anthony M. Brown, for useful comments and suggestions. NR 88 TC 9 Z9 9 U1 1 U2 11 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD JAN 21 PY 2015 VL 446 IS 3 BP 2456 EP 2467 DI 10.1093/mnras/stu2251 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CC3TG UT WOS:000350272300020 ER PT J AU Banerji, M Jouvel, S Lin, H McMahon, RG Lahav, O Castander, FJ Abdalla, FB Bertin, E Bosman, SE Carnero, A Kind, MC da Costa, LN Gerdes, D Gschwend, J Lima, M Maia, MAG Merson, A Miller, C Ogando, R Pellegrini, P Reed, S Saglia, R Sanchez, C Allam, S Annis, J Bernstein, G Bernstein, J Bernstein, R Capozzi, DD Childress, M Cunha, CE Davis, TM DePoy, DDL Desai, S Diehl, HT Doel, P Findlay, J Finley, DA Flaugher, B Frieman, J Gaztanaga, E Glazebrook, K Gonzalez-Fernandez, C Gonzalez-Solares, E Honscheid, K Irwin, MJ Jarvis, MJ Kim, A Koposov, S Kuehn, K Kupcu-Yoldas, A Lagattuta, D Lewis, JR Lidman, C Makler, M Marriner, J Marshall, JL Miquel, R Mohr, JJ Neilsen, E Peoples, J Sako, M Sanchez, E Scarpine, V Schindler, R Schubnell, M Sevilla, I Sharp, R Soares-Santos, M Swanson, MEC Tarle, G Thaler, J Tucker, D Uddin, SA Wechsler, R Wester, W Yuan, F Zuntz, J AF Banerji, Manda Jouvel, S. Lin, H. McMahon, R. G. Lahav, O. Castander, F. J. Abdalla, F. B. Bertin, E. Bosman, S. E. Carnero, A. Kind, M. Carrasco da Costa, L. N. Gerdes, D. Gschwend, J. Lima, M. Maia, M. A. G. Merson, A. Miller, C. Ogando, R. Pellegrini, P. Reed, S. Saglia, R. Sanchez, C. Allam, S. Annis, J. Bernstein, G. Bernstein, J. Bernstein, R. Capozzi, D. D. Childress, M. Cunha, Carlos E. Davis, T. M. DePoy, D. D. L. Desai, S. Diehl, H. T. Doel, P. Findlay, J. Finley, D. A. Flaugher, B. Frieman, J. Gaztanaga, E. Glazebrook, K. Gonzalez-Fernandez, C. Gonzalez-Solares, E. Honscheid, K. Irwin, M. J. Jarvis, M. J. Kim, A. Koposov, S. Kuehn, K. Kupcu-Yoldas, A. Lagattuta, D. Lewis, J. R. Lidman, C. Makler, M. Marriner, J. Marshall, Jennifer L. Miquel, R. Mohr, Joseph J. Neilsen, E. Peoples, J. Sako, M. Sanchez, E. Scarpine, V. Schindler, R. Schubnell, M. Sevilla, I. Sharp, R. Soares-Santos, M. Swanson, M. E. C. Tarle, G. Thaler, J. Tucker, D. Uddin, S. A. Wechsler, R. Wester, W. Yuan, F. Zuntz, J. TI Combining Dark Energy Survey Science Verification data with near-infrared data from the ESO VISTA Hemisphere Survey SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE catalogues; surveys; galaxies: distances and redshifts; galaxies: photometry; quasars: general ID DIGITAL SKY SURVEY; SPECTROSCOPIC TARGET SELECTION; MASS ASSEMBLY GAMA; LARGE-AREA SURVEY; DATA-FLOW SYSTEM; VLT DEEP SURVEY; SIMILAR-TO 2; PHOTOMETRIC REDSHIFTS; STELLAR MASSES; GALAXY SAMPLE AB We present the combination of optical data from the Science Verification phase of the Dark Energy Survey (DES) with near-infrared (NIR) data from the European Southern Observatory VISTA Hemisphere Survey (VHS). The deep optical detections from DES are used to extract fluxes and associated errors from the shallower VHS data. Joint seven-band (grizYJK) photometric catalogues are produced in a single 3 sq-deg dedicated camera field centred at 02h26m-04d36m where the availability of ancillary multiwavelength photometry and spectroscopy allows us to test the data quality. Dual photometry increases the number of DES galaxies with measured VHS fluxes by a factor of similar to 4.5 relative to a simple catalogue level matching and results in a similar to 1.5 mag increase in the 80 per cent completeness limit of the NIR data. Almost 70 per cent of DES sources have useful NIR flux measurements in this initial catalogue. Photometric redshifts are estimated for a subset of galaxies with spectroscopic redshifts and initial results, although currently limited by small number statistics, indicate that the VHS data can help reduce the photometric redshift scatter at both z < 0.5 and z > 1. We present example DES VHS colour selection criteria for high-redshift luminous red galaxies (LRGs) at z similar to 0.7 as well as luminous quasars. Using spectroscopic observations in this field we show that the additional VHS fluxes enable a cleaner selection of both populations with <10 per cent contamination from galactic stars in the case of spectroscopically confirmed quasars and <0.5 per cent contamination from galactic stars in the case of spectroscopically confirmed LRGs. The combined DES+VHS data set, which will eventually cover almost 5000 sq-deg, will therefore enable a range of new science and be ideally suited for target selection for future wide-field spectroscopic surveys. C1 [Banerji, Manda; Jouvel, S.; Lahav, O.; Abdalla, F. B.; Doel, P.] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Lin, H.; Allam, S.; Annis, J.; Diehl, H. T.; Finley, D. A.; Flaugher, B.; Frieman, J.; Marriner, J.; Neilsen, E.; Peoples, J.; Scarpine, V.; Soares-Santos, M.; Tucker, D.; Wester, W.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [McMahon, R. G.; Bosman, S. E.; Merson, A.; Reed, S.; Findlay, J.; Gonzalez-Fernandez, C.; Gonzalez-Solares, E.; Irwin, M. J.; Koposov, S.; Kupcu-Yoldas, A.; Lewis, J. R.] Univ Cambridge, Inst Astron, Cambridge CB3 0HA, England. [McMahon, R. G.] Univ Cambridge, Kavli Inst Cosmol, Cambridge CB3 0HA, England. [Castander, F. J.; Gaztanaga, E.] IEEC CSIC, Inst Ciencies Espai, E-08193 Barcelona, Spain. [Bertin, E.] Univ Paris 06, Inst Astrophys Paris, F-75014 Paris, France. [Carnero, A.; da Costa, L. N.; Gschwend, J.; Maia, M. A. G.; Ogando, R.; Pellegrini, P.] Observ Nacl, BR-20921400 Rio De Janeiro, RJ, Brazil. [Carnero, A.; da Costa, L. N.; Gschwend, J.; Lima, M.; Maia, M. A. G.; Ogando, R.; Pellegrini, P.] Lab Interinst eAstron LIneA, BR-20921400 Rio De Janeiro, RJ, Brazil. [Kind, M. Carrasco] Univ Illinois, Dept Astron, Champaign, IL 61820 USA. [Gerdes, D.; Miller, C.; Schubnell, M.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Lima, M.; Tarle, G.] Univ Sao Paulo, Inst Fis, Dept Fis Matemat, BR-05314970 Sao Paulo, Brazil. [Saglia, R.; Mohr, Joseph J.] Max Planck Inst Extraterr Phys, D-85748 Garching, Germany. [Sanchez, C.; Miquel, R.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Bellaterra, Barcelona, Spain. [Allam, S.] Space Telescope Sci Inst StScI, Baltimore, MD 21218 USA. [Bernstein, G.; Sako, M.] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. [Bernstein, J.] Argonne Natl Lab, Argonne, IL 60439 USA. [Bernstein, R.] Carnegie Observ, Pasadena, CA 91101 USA. [Capozzi, D. D.] Univ Portsmouth, Inst Cosmol & Gravitat, Portsmouth PO1 3FX, Hants, England. [Childress, M.; Yuan, F.] Australian Natl Univ, Res Sch Astron & Astrophys, Canberra, ACT 2611, Australia. [Childress, M.; Davis, T. M.; Lagattuta, D.; Uddin, S. A.] ARC Ctr Excellence All Sky Astrophys CAASTRO, Sydney, NSW, Australia. [Cunha, Carlos E.; Wechsler, R.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, Stanford, CA 94305 USA. [Davis, T. M.] Univ Queensland, Sch Math & Phys, Brisbane, Qld 4072, Australia. [DePoy, D. D. L.; Marshall, Jennifer L.] Texas A&M Univ, Dep Phys & Astron, George P & Cynthia Woods Mitchell Inst Fundamenta, College Stn, TX 77843 USA. [Desai, S.; Mohr, Joseph J.] Univ Munich, Dept Phys, D-81679 Munich, Germany. [Desai, S.; Mohr, Joseph J.] Excellence Cluster Univ, D-85748 Garching, Germany. [Glazebrook, K.; Lagattuta, D.; Uddin, S. A.] Swinburne Univ Technol, Ctr Astrophys & Supercomp, Hawthorn, Vic 3122, Australia. [Honscheid, K.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Jarvis, M. J.] Univ Oxford, Dept Phys, Oxford OX1 3RH, England. [Jarvis, M. J.] Univ Western Cape, Dept Phys, ZA-7535 Bellville, South Africa. [Kim, A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Kuehn, K.; Lidman, C.] Australian Astron Observ, N Ryde, NSW 2113, Australia. [Makler, M.] Ctr Brasileiro Pesquisas Fis, ICRA, BR-22290180 Rio De Janeiro, RJ, Brazil. [Miquel, R.] Inst Catalana Recerca & Estudis Avancats, E-08010 Barcelona, Spain. [Sanchez, E.; Sevilla, I.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Schindler, R.] SL4C Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Sharp, R.] Australian Natl Univ, Res Sch Astron & Astrophys, Canberra, ACT 2611, Australia. [Swanson, M. E. C.] Natl Ctr Supercomp Applicat, Urbana, IL 61801 USA. [Thaler, J.; Yuan, F.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Zuntz, J.] Univ Manchester, Jordrell Bank Ctr Astrophys, Manchester M13 9PL, Lancs, England. RP Banerji, M (reprint author), UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. EM m.banerji@ucl.ac.uk RI Lima, Marcos/E-8378-2010; Koposov, Sergey/F-2754-2012; Gonzalez-Fernandez, Carlos/H-3569-2015; Glazebrook, Karl/N-3488-2015; Davis, Tamara/A-4280-2008; Gaztanaga, Enrique/L-4894-2014; Ogando, Ricardo/A-1747-2010; Sanchez, Eusebio/H-5228-2015; Makler, Martin/G-2639-2012; OI Koposov, Sergey/0000-0003-2644-135X; Gonzalez-Fernandez, Carlos/0000-0003-2612-0118; Glazebrook, Karl/0000-0002-3254-9044; Davis, Tamara/0000-0002-4213-8783; Gaztanaga, Enrique/0000-0001-9632-0815; Carrasco Kind, Matias/0000-0002-4802-3194; Ogando, Ricardo/0000-0003-2120-1154; Sanchez, Eusebio/0000-0002-9646-8198; Makler, Martin/0000-0003-2206-2651; McMahon, Richard/0000-0001-8447-8869; Abdalla, Filipe/0000-0003-2063-4345; Tucker, Douglas/0000-0001-7211-5729 FU OL's Advanced European Research Council Grant (TESTDE); US Department of Energy; US National Science Foundation; Ministry of Science and Education of Spain; Science and Technology Facilities Council of UK; Higher Education Funding Council for England; National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign; Kavli Institute of Cosmological Physics at the University of Chicago; Financiadora de Estudos e Projetos; Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico; Ministerio da Ciencia e Tecnologia; Deutsche Forschungsgemeinschaft; Argonne National Laboratories; University of California at Santa Cruz; University of Cambridge; Centro de Investigaciones Energeticas; Medioambientales y Tecnologicas-Madrid; University of Chicago; University College London; DES-Brazil Consortium; Eidgenossische Technische Hochschule (ETH) Zurich; Fermi National Accelerator Laboratory; University of Edinburgh; University of Illinois at Urbana-Champaign; Institut de Ciencies de l'Espai (IEEC/CSIC); Institut de Fisica d'Altes Energies; Lawrence Berkeley National Laboratory; Ludwig-Maximilians Universitat; associated Excellence Cluster Universe; University of Michigan; National Optical Astronomy Observatory; University of Nottingham; Ohio State University; University of Pennsylvania; University of Portsmouth; SLAC National Laboratory; Stanford University; University of Sussex; Texas AM University; MINECO [AYA2009-13936, AYA2012-39559, AYA2012-39620, FPA2012-39684]; FEDER funds from the European Union; VISTA Hemisphere Survey, ESO Progamme [179.A-2010]; Australian Research Council Centre of Excellence for All-sky Astrophysics (CAASTRO) [CE110001020]; Australian Research Council [FT100100595]; [179.A-2006] FX We thank the referee, Nicholas Cross, for a very useful report on this manuscript. MB acknowledges a postdoctoral fellowship via OL's Advanced European Research Council Grant (TESTDE).; Funding for the DES Projects has been provided by the US Department of Energy, the US National Science Foundation, the Ministry of Science and Education of Spain, the Science and Technology Facilities Council of UK, the Higher Education Funding Council for England, the National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign, the Kavli Institute of Cosmological Physics at the University of Chicago, Financiadora de Estudos e Projetos, Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro, Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and the Ministerio da Ciencia e Tecnologia, the Deutsche Forschungsgemeinschaft and the Collaborating Institutions in the Dark Energy Survey.; The Collaborating Institutions are Argonne National Laboratories, the University of California at Santa Cruz, the University of Cambridge, Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas-Madrid, the University of Chicago, University College London, the DES-Brazil Consortium, the Eidgenossische Technische Hochschule (ETH) Zurich, Fermi National Accelerator Laboratory, the University of Edinburgh, the University of Illinois at Urbana-Champaign, the Institut de Ciencies de l'Espai (IEEC/CSIC), the Institut de Fisica d'Altes Energies, the Lawrence Berkeley National Laboratory, the Ludwig-Maximilians Universitat and the associated Excellence Cluster Universe, the University of Michigan, the National Optical Astronomy Observatory, the University of Nottingham, The Ohio State University, the University of Pennsylvania, the University of Portsmouth, SLAC National Laboratory, Stanford University, the University of Sussex, and Texas A&M University.; The DES participants from Spanish institutions are partially supported by MINECO under grants AYA2009-13936, AYA2012-39559, AYA2012-39620, and FPA2012-39684, which include FEDER funds from the European Union.; The analysis presented here is based on observations obtained as part of the VISTA Hemisphere Survey, ESO Progamme, 179.A-2010 (PI: McMahon) and data products from observations made with ESO Telescopes at the La Silla Paranal Observatory under programme ID 179.A-2006 (PI: Jarvis).; Data for the OzDES spectroscopic survey were obtained with the Anglo-Australian Telescope (programme numbers 12B/11 and 13B/12). Parts of this research were conducted by the Australian Research Council Centre of Excellence for All-sky Astrophysics (CAASTRO), through project number CE110001020. TMD acknowledges the support of the Australian Research Council through Future Fellowship, FT100100595. NR 62 TC 11 Z9 11 U1 3 U2 11 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD JAN 21 PY 2015 VL 446 IS 3 BP 2523 EP 2539 DI 10.1093/mnras/stu2261 PG 17 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CC3TG UT WOS:000350272300025 ER PT J AU Castelli, IE Huser, F Pandey, M Li, H Thygesen, KS Seger, B Jain, A Persson, KA Ceder, G Jacobsen, KW AF Castelli, Ivano E. Huser, Falco Pandey, Mohnish Li, Hong Thygesen, Kristian S. Seger, Brian Jain, Anubhav Persson, Kristin A. Ceder, Gerbrand Jacobsen, Karsten W. TI New Light-Harvesting Materials Using Accurate and Efficient Bandgap Calculations SO ADVANCED ENERGY MATERIALS LA English DT Article DE photoelectrochemical cells; light-harvesting materials; high-throughput screening; Pourbaix diagrams; stability ID DENSITY-FUNCTIONAL THEORY; PHOTOCATALYTIC PROPERTIES; PHOTOPHYSICAL PROPERTIES; ELECTRONIC-STRUCTURES; HYDROGEN-PRODUCTION; CRYSTAL-STRUCTURES; WATER; OXIDES; CAPTURE; PBCU2O2 AB Electronic bandgap calculations are presented for 2400 experimentally known materials from the Materials Project database and the bandgaps, obtained with different types of functionals within density functional theory and (partial) self-consistent GW approximation, are compared for 20 randomly chosen compounds forming an unconventional set of ternary and quaternary materials. It is shown that the computationally cheap GLLB-SC potential gives results in good agreement (around 15%) with the more advanced and demanding eigenvalue-self-consistent GW. This allows for a high-throughput screening of materials for different applications where the bandgaps are used as descriptors for the efficiency of a photoelectrochemical device. Here, new light harvesting materials are proposed to be used in a one-photon photoelectrochemical device for water splitting by combining the estimation of the bandgaps with the stability analysis using Pourbaix diagrams and with the evaluation of the position of the band edges. Using this methodology, 25 candidate materials are obtained and 5 of them appear to have a realistic possibility of being used as photocatalyst in a one-photon water splitting device. C1 [Castelli, Ivano E.; Huser, Falco; Pandey, Mohnish; Li, Hong; Thygesen, Kristian S.; Jacobsen, Karsten W.] Tech Univ Denmark, Dept Phys, Ctr Atom Scale Mat Design, DK-2800 Lyngby, Denmark. [Seger, Brian] Tech Univ Denmark, Dept Phys, Ctr Individual Nanoparticle Funct, DK-2800 Lyngby, Denmark. [Jain, Anubhav; Persson, Kristin A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. [Ceder, Gerbrand] MIT, Cambridge, MA 02139 USA. RP Castelli, IE (reprint author), Tech Univ Denmark, Dept Phys, Ctr Atom Scale Mat Design, DK-2800 Lyngby, Denmark. EM ivca@fysik.dtu.dk RI Thygesen, Kristian /B-1062-2011; Jacobsen, Karsten/B-3602-2009; Seger, Brian/G-2433-2011; Castelli, Ivano/N-1627-2015; OI Pandey, Mohnish/0000-0002-1715-0617; Thygesen, Kristian /0000-0001-5197-214X; Jacobsen, Karsten/0000-0002-1121-2979; Seger, Brian/0000-0002-0036-095X; Castelli, Ivano/0000-0001-5880-5045; Huser, Falco Jonas/0000-0001-9645-6691 FU Catalysis for Sustainable Energy (CASE) initiative - Danish Ministry of Science, Technology and Innovation; Danish National Research Foundation [DNRF54]; Center on Nanostructuring for the Efficient Energy Conversion (CNEEC) at Stanford University, an Energy Frontier Research Center - US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001060]; Assistant Secretary for Energy Efficiency and Renewable Energy [DE-AC02-05CH11231]; Department of Energy's Basic Energy Sciences program [EDCBEE] FX The authors acknowledge support from the Catalysis for Sustainable Energy (CASE) initiative funded by the Danish Ministry of Science, Technology and Innovation, from the Danish National Research Foundation for funding The Center for Individual Nanoparticle Functionality (CINF) (DNRF54) and from the Center on Nanostructuring for the Efficient Energy Conversion (CNEEC) at Stanford University, an Energy Frontier Research Center founded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under award number DE-SC0001060. Work at the Lawrence Berkeley National Laboratory was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, under Contract No. DE-AC02-05CH11231. The Materials Project work is supported by Department of Energy's Basic Energy Sciences program under Grant No. EDCBEE. NR 60 TC 17 Z9 17 U1 10 U2 104 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD JAN 21 PY 2015 VL 5 IS 2 AR 1400915 DI 10.1002/aenm.201400915 PG 7 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA CA2YR UT WOS:000348772600006 ER PT J AU Brown, MA Gelis, AV Fortner, JA Jerden, JL Wiedmeyer, S Vandegrift, GF AF Brown, M. Alex Gelis, Artem V. Fortner, Jeffrey A. Jerden, James L. Wiedmeyer, Stan Vandegrift, George F. TI A Novel Method for Molybdenum-99/Technetium-99m Recovery via Anodic Carbonate Dissolution of Irradiated Low-Enriched Uranium Metal Foil SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID MO-99 AB A new method is presented here for digesting irradiated low-enriched uranium foil targets in alkaline carbonate media to recover 99Mo. This method consists of the electrolytic dissolution of uranium foil in a sodium bicarbonate solution, followed by the precipitation of carbonate, base-insoluble fission products, activation products, and actinides with calcium oxide; most of the molybdenum, technetium, and iodine remain in solution. An electrochemical dissolver and mixing vessel were designed, fabricated, and tested for the processing of a full-sized irradiated foil under ambient pressure and elevated temperature. Over 92% of the fission-induced Mo-99 was recovered in a product solution that was compatible with an anion-exchange column for retaining molybdenum and iodine. C1 [Brown, M. Alex; Gelis, Artem V.; Fortner, Jeffrey A.; Jerden, James L.; Wiedmeyer, Stan; Vandegrift, George F.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Gelis, AV (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM gelis@anl.gov FU U.S. Department of Energy, NNSA's Office of Defense Nuclear Nonproliferation [DE-AC02-06CH11357]; U.S. Department of Energy by UChicago Argonne, LLC. Argonne, a U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357] FX Work supported by the U.S. Department of Energy, NNSA's Office of Defense Nuclear Nonproliferation, under Contract DE-AC02-06CH11357. Argonne National Laboratory is operated for the U.S. Department of Energy by UChicago Argonne, LLC. Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract DE-AC02-06CH11357. The authors also thank the technicians, postdocs, and staff scientists of the Chemical Sciences and Engineering, Sergey Chemerisov, Roman Gromov, Vakhtang Makarashvilli, and Lohman Hafenrichter at the Argonne Linear Accelerator, and Luke Ivasca and Bill Brown at Argonne Central Shops. NR 21 TC 1 Z9 1 U1 0 U2 5 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD JAN 21 PY 2015 VL 54 IS 2 BP 712 EP 719 DI 10.1021/ie503858j PG 8 WC Engineering, Chemical SC Engineering GA AZ8RW UT WOS:000348483300018 ER PT J AU Aceves, SM Espinosa-Loza, F Elmer, JW Huber, R AF Aceves, Salvador M. Espinosa-Loza, Francisco Elmer, John W. Huber, Robert TI Comparison of Cu, Ti and Ta interlayer explosively fabricated aluminum to stainless steel transition joints for cryogenic pressurized hydrogen storage SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Cryogenic hydrogen storage; Transition joints; Explosive welding, Dissimilar metal welding ID NIOBIUM; VESSELS AB Fabrication of a bimetallic joint to facilitate a material transition from a 6061-T651 aluminum pressure vessel liner to stainless steel tubing in cryogenic pressure vessels is explored using three different dissimilar metal interlayers with an explosive welding (EXW) process. Due to difficulties in directly EXW joining aluminum (Al) 6061 to 304 stainless steel, interlayers are used to prevent interaction of the aluminum and stainless steel, thus minimizing brittle intermetallic phase formation. Titanium (Ti), copper (Cu), and tantalum (Ta) were selected as the dissimilar metal interlayer materials; each having advantages and disadvantages. Titanium is a commonly used interlayer for this joint, but can microcrack during EXW if the bonding parameters are not correct. Copper has the advantage that it is compatible with hydrogen, but is also known to form brittle intermetallics with aluminum. Tantalum is ductile and bonds well to both Al and stainless steel, and is a high temperature metal that does well to prevent interdiffusion and intermetallic phase formation. However Ta is the most expensive metal of the three. Results of the characterization of the three interlayer bonds showed that Ti produced the highest strength joints, Ta produced the most ductile joints, and Cu produced a joint that failed with low ductility at the Al/Cu interface. Based on these results, the Cu-interlayer joint is not recommended for this application, while the Ti and Ta interlayer bonds both appear to have sufficient strength and ductility for the intended use. Copyright (C) 014, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Aceves, Salvador M.; Espinosa-Loza, Francisco; Elmer, John W.; Huber, Robert] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Aceves, SM (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave,L-792, Livermore, CA 94550 USA. EM saceves@llnl.gov FU DOE, Office of Hydrogen and Fuel Cell Technologies; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This project was funded by DOE, Office of Hydrogen and Fuel Cell Technologies, Jesse Adams, Technology Development Manager. This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 16 TC 2 Z9 2 U1 6 U2 27 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 EI 1879-3487 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD JAN 21 PY 2015 VL 40 IS 3 BP 1490 EP 1503 DI 10.1016/j.ijhydene.2014.11.038 PG 14 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA CA6XF UT WOS:000349060100014 ER PT J AU Tran, TT Gooch, M Lorenz, B Litvinchuk, AP Sorolla, MG Brgoch, J Chu, PCW Guloy, AM AF Tran, T. Thao Gooch, Melissa Lorenz, Bernd Litvinchuk, Alexander P. Sorolla, Maurice G., II Brgoch, Jakoah Chu, Paul C. W. Guloy, Arnold M. TI Nb2O2F3: A Reduced Niobium (III/IV) Oxyfluoride with a Complex Structural, Magnetic, and Electronic Phase Transition SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID METAL OXIDES; INSTABILITIES; BOND; SUPERCONDUCTIVITY; COMPOUND AB A new niobium oxyfluoride, Nb2O2F3, synthesized through the reaction of Nb, SnO, and SnF2 in Sn flux, within welded Nb containers, crystallizes in a monoclinic structure (space group: I2/a; a = 5.7048(1)angstrom, b = 5.1610(1)angstrom, c = 12.2285(2)angstrom, beta = 95.751(1)degrees). It features [Nb2X10] units (X = O, F), with short (2.5739(1) angstrom) NbNb bonds, that are linked through shared O/F vertices to form a 3D structure configurationally isotypic to zeta-Nb2O5. Nb2O2F3 undergoes a structural transition at similar to 90 K to a triclinic structure (space group: P1(-); a = 5.1791(5)angstrom, b = 5.7043(6)angstrom, c = 6.8911(7)angstrom, alpha = 108.669(3)degrees, beta = 109.922(2)degrees, gamma = 90.332(3)degrees). The transition is described as a disproportionation or charge ordering of [Nb-2](7)+ dimers: (2[Nb-2]7+ -> [Nb-2](6)+ + [Nb-2](8)+), resulting in doubly (2.5000(9) angstrom) and singly bonded (2.6560(9) angstrom) Nb-2 dimers. The structural transition is accompanied by an unusual field-independent spin-gap-like magnetic transition. C1 [Tran, T. Thao; Sorolla, Maurice G., II; Brgoch, Jakoah; Guloy, Arnold M.] Univ Houston, Dept Chem, Houston, TX 77204 USA. [Gooch, Melissa; Lorenz, Bernd; Litvinchuk, Alexander P.; Chu, Paul C. W.] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Tran, T. Thao; Gooch, Melissa; Lorenz, Bernd; Litvinchuk, Alexander P.; Sorolla, Maurice G., II; Brgoch, Jakoah; Chu, Paul C. W.; Guloy, Arnold M.] Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. [Chu, Paul C. W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Guloy, AM (reprint author), Univ Houston, Dept Chem, Univ Pk, Houston, TX 77204 USA. EM aguloy@uh.edu RI Litvinchuk, Alexander/K-6991-2012 OI Litvinchuk, Alexander/0000-0002-5128-5232 FU R. A. Welch Foundation [E-1297]; State of Texas through the Texas Center for Superconductivity; US AFOSR FX This work was supported in part by the R. A. Welch Foundation (E-1297), the State of Texas through the Texas Center for Superconductivity, and the US AFOSR. We thank Dr. J. D. Korp for assistance in collecting low-temperature X-ray diffraction data. T.T.T. acknowledges Prof. P. S. Halasyamani. NR 35 TC 7 Z9 7 U1 3 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 21 PY 2015 VL 137 IS 2 BP 636 EP 639 DI 10.1021/ja511745q PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA AZ8RX UT WOS:000348483400022 PM 25581015 ER PT J AU Zhao, Y Burkert, SC Tang, YF Sorescu, DC Kapralov, AA Shurin, GV Shurin, MR Kagan, VE Star, A AF Zhao, Yong Burkert, Seth C. Tang, Yifan Sorescu, Dan C. Kapralov, Alexandr A. Shurin, Galina V. Shurin, Michael R. Kagan, Valerian E. Star, Alexander TI Nano-Gold Corking and Enzymatic Uncorking of Carbon Nanotube Cups SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID REGULATORY DENDRITIC CELLS; DRUG-DELIVERY SYSTEMS; SUPPRESSOR-CELLS; MACROMOLECULAR THERAPEUTICS; ELECTROCATALYTIC ACTIVITY; CHEMOTHERAPEUTIC-AGENTS; INTRACELLULAR DELIVERY; NITROGEN; NANOPARTICLES; CANCER AB Because of their unique stacked, cup-shaped, hollow compartments, nitrogen-doped carbon nanotube cups (NCNCs) have promising potential as nanoscale containers. Individual NCNCs are isolated from their stacked structure through acid oxidation and subsequent probe-tip sonication. The NCNCs are then effectively corked with gold nanoparticles (GNPs) by sodium citrate reduction with chloroauric acid, forming graphitic nanocapsules with significant surface-enhanced Raman signature. Mechanistically, the growth of the GNP corks starts from the nucleation and welding of gold seeds on the open rims of NCNCs enriched with nitrogen functionalities, as confirmed by density functional theory calculations. A potent oxidizing enzyme of neutrophils, myeloperoxidase (MPO), can effectively open the corked NCNCs through GNP detachment, with subsequent complete enzymatic degradation of the graphitic shells. This controlled opening and degradation was further carried out in vitro with human neutrophils. Furthermore, the GNP-corked NCNCs were demonstrated to function as novel drug delivery carriers, capable of effective (i) delivery of paclitaxel to tumor-associated myeloid-derived suppressor cells (MDSC), (ii) MPO-regulated release, and (iii) blockade of MDSC immunosuppressive potential. C1 [Zhao, Yong; Burkert, Seth C.; Tang, Yifan; Star, Alexander] Univ Pittsburgh, Dept Chem, Pittsburgh, PA 15260 USA. [Sorescu, Dan C.] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15263 USA. [Kapralov, Alexandr A.; Kagan, Valerian E.] Univ Pittsburgh, Dept Environm & Occupat Hlth, Pittsburgh, PA 15261 USA. [Shurin, Galina V.; Shurin, Michael R.] Univ Pittsburgh, Med Ctr, Dept Pathol, Pittsburgh, PA 15261 USA. [Shurin, Michael R.] Univ Pittsburgh, Med Ctr, Dept Immunol, Pittsburgh, PA 15261 USA. RP Star, A (reprint author), Univ Pittsburgh, Dept Chem, Pittsburgh, PA 15260 USA. EM astar@pitt.edu RI Tang, Yifan/F-4275-2012; Zhao, Yong/C-9160-2014; OI Zhao, Yong/0000-0003-1990-4387; Kapralov, Oleksandr/0000-0002-3006-916X FU NSF CAREER Award [0954345]; NIH [R01ES019304,, RO1 CA154369, U19 AI068021, HL114453]; NIOSH [OH008282]; Bayer Material Science Fellowship FX This work at the University of Pittsburgh was supported by an NSF CAREER Award No. 0954345, NIH R01ES019304, RO1 CA154369, U19 AI068021, HL114453, and NIOSH OH008282. We thank the Nanoscale Fabrication and Characterization Facility and the Department of Biological Sciences at the University of Pittsburgh for provision of access to the TEM and Raman instruments and acknowledge R. J. Lee's group for access to the XPS instrumentation. Y.Z. is thankful for support from a Bayer Material Science Fellowship. NR 66 TC 15 Z9 15 U1 14 U2 75 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 21 PY 2015 VL 137 IS 2 BP 675 EP 684 DI 10.1021/ja511843w PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA AZ8RX UT WOS:000348483400031 PM 25530234 ER PT J AU Zhang, J Rowland, C Liu, YZ Xiong, H Kwon, S Sheychenko, E Schaller, RD Prakapenka, VB Tkachev, S Rajh, T AF Zhang, Jun Rowland, Clare Liu, Yuzi Xiong, Hui Kwon, Soongu Sheychenko, Elena Schaller, Richard D. Prakapenka, Vitali B. Tkachev, Sergey Rajh, Tijana TI Evolution of Self-Assembled ZnTe Magic-Sized Nanoclusters SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID CDSE QUANTUM DOTS; SEMICONDUCTOR NANOCRYSTALS; ORIENTED ATTACHMENT; SHAPE-CONTROL; GROWTH; CLUSTERS; NANOPARTICLES; MONODISPERSE; MECHANISMS; NUCLEATION AB Three families of ZnTe magic-sized nanoclusters (MSNCs) were obtained exclusively using polytellurides as a tellurium precursor in a one-pot reaction by simply varying the reaction temperature and time only. Different ZnTe MSNCs exhibit different self-assembling or aggregation behavior, owing to their different structure, cluster size, and dipole-dipole interactions. The smallest family of ZnTe MSNCs (F323) does not reveal a crystalline structure and as a result assembles into lamellar triangle plates. Continuous heating of as synthesized ZnTe F323 assemblies resulted in the formation of ZnTe F398 MSNCs with wurzite structure and concomitant transformation into lamellar rectangle assemblies with the organization of nanoclusters along the < 002 > direction. Further annealing of ZnTe F398 assembled lamellar rectangles leads to full organization of MSNCs in all directions and formation of larger ZnTe F444 NCs that spontaneously form ultrathin nanowires following an oriented attachment mechanism. The key step in control over the size distribution of ZnTe ultrathin nanowires is, in fact, the growth mechanism of ZnTe F398 MSNCs; namely, the step growth mechanism enables formation of more uniform nanowires compared to those obtained by continuous growth mechanism. High yield of ZnTe nanowires is achieved as a result of the wurzite structure of F398 precursor. Transient absorption (TA) measurements show that all three families possess ultrafast dynamics of photogenerated electrons, despite their different crystalline structures. C1 [Zhang, Jun] China Univ Petr, Coll Chem Engn, State Key Lab Heavy Oil Proc, Qingdao 266580, Peoples R China. [Zhang, Jun; Rowland, Clare; Liu, Yuzi; Xiong, Hui; Kwon, Soongu; Sheychenko, Elena; Schaller, Richard D.; Rajh, Tijana] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Prakapenka, Vitali B.; Tkachev, Sergey] Univ Chicago, Ctr Adv Radiat Sources, Chicago, IL 60637 USA. RP Zhang, J (reprint author), China Univ Petr, Coll Chem Engn, State Key Lab Heavy Oil Proc, Qingdao 266580, Peoples R China. EM zhangj@upc.edu.cn; rajh@anl.gov RI Kwon, Soon Gu/E-3123-2015; Liu, Yuzi/C-6849-2011 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; National Science Foundation-Earth Sciences [EAR-1128799]; Department of Energy-GeoSciences [DE-FG02-94ER14466]; Center for Nanoscale Materials at Argonne National Laboratory through a CNM distinguished postdoctoral fellowship; National Natural Science Foundation of China [21471160]; Fundamental Research Funds for the Central Universities [14CX05037A]; Tai Shan Scholar Foundation FX Work at the Center for Nanoscale Materials was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. Part of the work was performed at GeoSoilEnviroCARS (Sector 13), Advanced Photon Source (APS), Argonne National Laboratory. GeoSoilEnviroCARS is supported by the National Science Foundation-Earth Sciences (EAR-1128799) and Department of Energy-GeoSciences (DE-FG02-94ER14466). J.Z. gratefully acknowledges the financial support from the Center for Nanoscale Materials at Argonne National Laboratory through a CNM distinguished postdoctoral fellowship, National Natural Science Foundation of China (No. 21471160), the Fundamental Research Funds for the Central Universities (14CX05037A), and Tai Shan Scholar Foundation. NR 45 TC 7 Z9 7 U1 10 U2 86 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 21 PY 2015 VL 137 IS 2 BP 742 EP 749 DI 10.1021/ja509782n PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA AZ8RX UT WOS:000348483400039 PM 25531438 ER PT J AU Bellone, DE Bours, J Menke, EH Fischer, FR AF Bellone, Donatela E. Bours, Justin Menke, Elisabeth H. Fischer, Felix R. TI Highly Selective Molybdenum ONO Pincer Complex Initiates the Living Ring-Opening Metathesis Polymerization of Strained Alkynes with Exceptionally Low Polydispersity Indices SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID TUNGSTEN ALKYLIDYNE COMPLEXES; METAL-CARBON BONDS; TRIANIONIC PINCER; ACETYLENE METATHESIS; CHEMICAL-EXCHANGE; CATALYSTS; LIGAND; IMIDAZOLIN-2-IMINATO; CYCLOOCTYNE; CLICK AB The pseudo-octahedral molybdenum benzylidyne complex [TolC Mo(ONO)(OR)]center dot KOR (R = CCH3(CF3)(2)) 1, featuring a stabilizing ONO pincer ligand, initiates the controlled living polymerization of strained dibenzocyclooctynes at T > 60 degrees C to give high molecular weight polymers with exceptionally low polydispersities (PDI similar to 1.02). Kinetic analyses reveal that the growing polymer chain attached to the propagating catalyst efficiently limits the rate of propagation with respect to the rate of initiation (k(p)/k(i) similar to 10(-3)). The reversible coordination of KOCCH3(CF3)(2) to the propagating catalyst prevents undesired chain-termination and -transfer processes. The ring-opening alkyne metathesis polymerization with 1 has all the characteristics of a living polymerization and enables, for the first time, the controlled synthesis of amphiphilic block copolymers via ROAMP. C1 [Bellone, Donatela E.; Bours, Justin; Menke, Elisabeth H.; Fischer, Felix R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Fischer, Felix R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Fischer, Felix R.] Univ Calif Berkeley, Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. [Fischer, Felix R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Fischer, FR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM ffischer@berkeley.edu FU American Chemical Society Petroleum Research Fund [52722-DNI7]; NIH [SRR023679A, S10-RR027172]; Abrahamson Foundation; German Academic Exchange Service (DAAD) FX Research was supported by the Donors of the American Chemical Society Petroleum Research Fund under Contract 52722-DNI7, Berkeley NMR Facility is supported in part by NIH Grant SRR023679A, and X-ray Facility is supported in part by NIH Shared Instrumentation Grant S10-RR027172. D.E.B. acknowledges fellowship support through the Abrahamson Foundation, E.H.M. acknowledges fellowship support through the German Academic Exchange Service (DAAD). The authors acknowledge Prof. Alex D. Bain for helpful discussions relating to the SIR experiments, Dr. Christian Canlas for support with NMR acquisition, Dr. Antonio DiPasquale for assistance with X-ray analysis, and Dr. Rita Nichiporuk for assistance with mass spectrometry. NR 52 TC 7 Z9 7 U1 2 U2 34 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 21 PY 2015 VL 137 IS 2 BP 850 EP 856 DI 10.1021/ja510919v PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA AZ8RX UT WOS:000348483400050 PM 25535767 ER PT J AU Biswas, A Chandra, S Stefanoski, S Blazquez, JS Ipus, JJ Conde, A Phan, MH Franco, V Nolas, GS Srikanth, H AF Biswas, Anis Chandra, Sayan Stefanoski, Stevce Blazquez, J. S. Ipus, J. J. Conde, A. Phan, M. H. Franco, V. Nolas, G. S. Srikanth, H. TI Enhanced cryogenic magnetocaloric effect in Eu8Ga16Ge30 clathrate nanocrystals SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID SURFACE SPIN DISORDER; THERMOELECTRIC APPLICATIONS; NANOPARTICLES AB We observe an enhanced magnetic entropy change (-Delta S-M) at cryogenic temperatures (T < 20 K) in Eu8Ga16Ge30 clathrate (type-I) nanocrystals prepared by a ball milling method. With reduction in the crystal size to 15 nm, -Delta S-M is enhanced at low temperatures, reaching the highest value (similar to 10 J/kg K) at 5K for a field change of 5 T. For all samples investigated, there is a cross-over temperature (similar to 25 K) in -Delta S-M (T) above which -Delta S-M decreases with crystal size, opposite to that observed at low temperatures. A careful analysis of the magnetic and magnetocaloric data reveals that as the crystal size decreases the magnetic interaction between Eu2+ ions on the Eu2 site governing the primary ferromagnetic transition at similar to 35K becomes gradually weaker, in effect, altering the interaction between Eu2+ ions occupying the Eu1 and Eu2 sites responsible for the secondary ferromagnetic transition at 15 K. As a result, we have observed a strong change in magnetization and the enhancement of -Delta S-M at low temperature. (C) 2015 AIP Publishing LLC. C1 [Biswas, Anis; Chandra, Sayan; Stefanoski, Stevce; Phan, M. H.; Nolas, G. S.; Srikanth, H.] Univ S Florida, Dept Phys, Tampa, FL 33620 USA. [Blazquez, J. S.; Ipus, J. J.; Conde, A.; Franco, V.] Univ Seville, ICMSE, CSIC, Dept Fis Mat Condensada, Seville 41080, Spain. RP Biswas, A (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA. EM anisbiswas@ameslab.gov; sharihar@usf.edu RI Phan, Manh-Huong/A-6709-2014; Franco, Victorino/B-8982-2008; Blazquez, Javier/C-7787-2011; Conde, Alejandro/A-8115-2013; IPUS, JHON/I-8830-2012 OI Franco, Victorino/0000-0003-3028-6815; Blazquez, Javier/0000-0003-2318-5418; Conde, Alejandro/0000-0002-1067-2754; IPUS, JHON/0000-0002-5402-6164 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-FG02-07ER46438]; U.S. Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering [DE-FG02-04ER46145]; Spanish MINECO; EU FEDER [MAT 2013-45165-P]; PAI of the Regional Government of Andalucia [P10-FQM-6462] FX A.B., S.C., M.H.P., and H.S. thank the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award No. DE-FG02-07ER46438 (magnetic measurements and analysis). S.S. and G.S.N. acknowledge the support of the U.S. Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering under Award No. DE-FG02-04ER46145 for bulk synthesis of polycrystalline Eu8Ga16Ge30. The work at Sevilla University was supported by the Spanish MINECO and EU FEDER (Project MAT 2013-45165-P) and the PAI of the Regional Government of Andalucia (Project P10-FQM-6462) for the synthesis of nanocrystalline Eu8Ga16Ge30. NR 31 TC 3 Z9 3 U1 4 U2 31 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JAN 21 PY 2015 VL 117 IS 3 AR 033903 DI 10.1063/1.4906280 PG 5 WC Physics, Applied SC Physics GA AZ6US UT WOS:000348356600010 ER PT J AU Eliseev, EA Kalinin, SV Morozovska, AN AF Eliseev, Eugene A. Kalinin, Sergei V. Morozovska, Anna N. TI Finite size effects in ferroelectric-semiconductor thin films under open-circuit electric boundary conditions SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID DOMAIN-STRUCTURE; NANOSCALE; POLARIZATION; BIFEO3 AB General features of finite size effects in the ferroelectric-semiconductor film under open-circuit electric boundary conditions are analyzed using Landau-Ginzburg-Devonshire theory and continuum media electrostatics. The temperature dependence of the film critical thickness, spontaneous polarization, and depolarization field profiles of the open-circuited films are found to be significantly different from the characteristics of short-circuited ones. In particular, we predict the re-entrant type transition boundary between the mono-domain and poly-domain ferroelectric states due to reduced internal screening efficiency and analyzed possible experimental scenarios created by this mechanism. Performed analysis is relevant for the quantitative description of free-standing ferroelectric films phase diagrams and polar properties. Also our results can be useful for the explanation of the scanning-probe microscopy experiments on free ferroelectric surfaces. (C) 2015 AIP Publishing LLC. C1 [Eliseev, Eugene A.] NAS Ukraine, Inst Problems Mat Sci, UA-03028 Kiev, Ukraine. [Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37922 USA. [Morozovska, Anna N.] NAS Ukraine, Inst Phys, UA-03028 Kiev, Ukraine. RP Morozovska, AN (reprint author), NAS Ukraine, Inst Phys, UA-03028 Kiev, Ukraine. EM anna.n.morozovska@gmail.com RI Kalinin, Sergei/I-9096-2012 OI Kalinin, Sergei/0000-0001-5354-6152 FU Center for Nanophase Materials Sciences (CNMS) [CNMS 2013-293, CNMS 2014-270]; National Academy of Sciences of Ukraine [35-02-14] FX Authors are very grateful to the constructive critical remarks from Reviewers. E.A.E. and A.N.M. acknowledge Center for Nanophase Materials Sciences (CNMS), user Project Nos. CNMS 2013-293 and CNMS 2014-270, and National Academy of Sciences of Ukraine (Grant No. 35-02-14). S.V.K. acknowledges Office of Basic Energy Sciences, U.S. Department of Energy. NR 47 TC 0 Z9 0 U1 1 U2 31 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JAN 21 PY 2015 VL 117 IS 3 AR 034102 DI 10.1063/1.4906139 PG 7 WC Physics, Applied SC Physics GA AZ6US UT WOS:000348356600012 ER PT J AU Sarker, P Al-Jassim, MM Huda, MN AF Sarker, Pranab Al-Jassim, Mowafak M. Huda, Muhammad N. TI Theoretical limits on the stability of single-phase kesterite-Cu2ZnSnS4 SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID FILM SOLAR-CELLS; GENERALIZED GRADIENT APPROXIMATION; BRILLOUIN-ZONE INTEGRATIONS; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; BASIS-SET; CU2ZNSNS4; DEFECTS; PHOTOVOLTAICS; PERFORMANCE AB The single-phase stability of Cu2ZnSnS4 (CZTS), after an intrinsic defect was incorporated in it, has been examined here for the first time based on ab initio calculations. The stability analysis of such a non-stoichiometric-defect incorporated CZTS shows that the single-phase formation is unlikely at thermodynamic equilibrium conditions. In addition, the effective growth condition of CZTS is determined and quantified for all the elements (Cu-poor, Zn-rich, Sn-poor, and S-rich) to extract maximum photovoltaic efficiency from CZTS. These conditions promote (i) spontaneous formation of Cu vacancy (V-Cu), which might benefit p-type conduction, and (ii) the co-existence of ZnS while suppressing other harmful defects and secondary phases. Further, the results presented here explain the unavailability of single-phase CZTS to date. (C) 2015 AIP Publishing LLC. C1 [Sarker, Pranab; Huda, Muhammad N.] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA. [Al-Jassim, Mowafak M.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Huda, MN (reprint author), Univ Texas Arlington, Dept Phys, POB 19059, Arlington, TX 76019 USA. EM huda@uta.edu OI Huda, Muhammad/0000-0002-2655-498X FU National Renewable Energy Laboratory [XEJ-9-99042-01]; U.S. Department of Energy [DE-AC36-08GO28308] FX The authors are greatly thankful to Prahsant Kharti for providing the most probable DFT ground state (stoichiometric) crystal structure of Cu2S, which is yet to be published. All computations were performed using the High Performance Computing Facility (HPC) at the University of Texas at Arlington and at the Texas Advanced Computing Center (TACC). The work at UTA was partially supported by National Renewable Energy Laboratory, Subcontract No. XEJ-9-99042-01. M.M.A. was supported by the U.S. Department of Energy under Contract No. DE-AC36-08GO28308 with the National Renewable Energy Laboratory. NR 74 TC 4 Z9 4 U1 3 U2 59 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JAN 21 PY 2015 VL 117 IS 3 AR 035702 DI 10.1063/1.4906065 PG 13 WC Physics, Applied SC Physics GA AZ6US UT WOS:000348356600043 ER PT J AU Dunning, TH Takeshita, TY Xu, LT AF Dunning, Thom H., Jr. Takeshita, Tyler Y. Xu, Lu T. TI Fundamental aspects of recoupled pair bonds. II. Recoupled pair bond dyads in carbon and sulfur difluoride SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID IMPROVED QUANTUM-THEORY; MANY-ELECTRON SYSTEMS; CORRELATED MOLECULAR CALCULATIONS; GAUSSIAN-BASIS SETS; WAVE-FUNCTIONS; ATOMS; SPIN; SPECTRUM AB Formation of a bond between a second ligand and a molecule with a recoupled pair bond results in a recoupled pair bond dyad. We examine the recoupled pair bond dyads in the a(3)B(1) states of CF2 and SF2, which are formed by the addition of a fluorine atom to the a(4)Sigma(-) tates of CF and SF, both of which possess recoupled pair bonds. The two dyads are very different. In SF2, the second FS-F bond is very strong (D-e = 106.3 kcal/mol), the bond length is much shorter than that in the SF(a(4)Sigma(-)) state (1.666 angstrom versus 1.882 angstrom), and the three atoms are nearly collinear (theta(e) = 162.7 degrees) with only a small barrier to linearity (0.4 kcal/mol). In CF2, the second FC-F bond is also very strong (D-e = 149.5 kcal/mol), but the bond is only slightly shorter than that in the CF(a(4)Sigma(-)) state (1.314 angstrom versus 1.327 angstrom), and the molecule is strongly bent (theta(e) = 119.0 degrees) with an 80.5 kcal/mol barrier to linearity. The a(3)B(1) states of CF2 and SF2 illustrate the fundamental differences between recoupled pair bond dyads formed from 2s and 3p lone pairs. (c) 2015 Author(s). C1 [Dunning, Thom H., Jr.; Takeshita, Tyler Y.; Xu, Lu T.] Univ Illinois, Dept Chem, Urbana, IL 61801 USA. RP Dunning, TH (reprint author), Pacific NW Natl Lab, Northwest Inst Adv Comp, Seattle, WA 98195 USA. FU Distinguished Chair for Research Excellence in Chemistry; National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign FX Support for this work was provided by funding from the Distinguished Chair for Research Excellence in Chemistry and the National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign. The authors would also like to acknowledge Dr. David L. Cooper from the University of Liverpool for his helpful insights into the CASVB program within the Molpro quantum chemistry package and Dr. David E. Woon, Dr. Beth Lindquist, and the other members of the research group for many helpful discussions. NR 33 TC 7 Z9 7 U1 3 U2 7 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JAN 21 PY 2015 VL 142 IS 3 AR 034114 DI 10.1063/1.4905272 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AZ6BJ UT WOS:000348302900014 PM 25612696 ER PT J AU Dunning, TH Xu, LT Takeshita, TY AF Dunning, Thom H., Jr. Xu, Lu T. Takeshita, Tyler Y. TI Fundamental aspects of recoupled pair bonds. I. Recoupled pair bonds in carbon and sulfur monofluoride SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID IMPROVED QUANTUM-THEORY; MANY-ELECTRON SYSTEMS; CORRELATED MOLECULAR CALCULATIONS; PHASE CONTINUITY PRINCIPLE; GENERALIZED VALENCE-BOND; COUPLED WAVE-FUNCTIONS; GAUSSIAN-BASIS SETS; P-BLOCK ELEMENTS; CONFIGURATION-INTERACTION; MICROWAVE-SPECTRUM AB The number of singly occupied orbitals in the ground-state atomic configuration of an element defines its nominal valence. For carbon and sulfur, with two singly occupied orbitals in their P-3 ground states, the nominal valence is two. However, in both cases, it is possible to form more bonds than indicated by the nominal valence-up to four bonds for carbon and six bonds for sulfur. In carbon, the electrons in the 2s lone pair can participate in bonding, and in sulfur the electrons in both the 3p and 3s lone pairs can participate. Carbon 2s and sulfur 3p recoupled pair bonds are the basis for the tetravalence of carbon and sulfur, and 3s recoupled pair bonds enable sulfur to be hexavalent. In this paper, we report generalized valence bond as well as more accurate calculations on the a(4)Sigma-states of CF and SF, which are archetypal examples of molecules that possess recoupled pair bonds. These calculations provide insights into the fundamental nature of recoupled pair bonds and illustrate the key differences between recoupled pair bonds formed with the 2s lone pair of carbon, as a representative of the early p-block elements, and recoupled pair bonds formed with the 3p lone pair of sulfur, as a representative of the late p-block elements. (c) 2015 Author(s). C1 [Dunning, Thom H., Jr.; Xu, Lu T.; Takeshita, Tyler Y.] Univ Illinois, Dept Chem, Urbana, IL 61801 USA. RP Dunning, TH (reprint author), Pacific NW Natl Lab, Northwest Inst Adv Comp, Washington, DC USA. EM thdjr@uw.edu FU Distinguished Chair for Research Excellence in Chemistry at the University of Illinois at Urbana-Champaign FX Support for this work was provided by funding from the Distinguished Chair for Research Excellence in Chemistry at the University of Illinois at Urbana-Champaign. The authors would also like to acknowledge Dr. David L. Cooper from the University of Liverpool for his helpful insights into the CASVB program within the Molpro quantum chemistry package and David E. Woon, Beth A. Lindquist, and the other members of the research group for many helpful discussions. We also thank the reviewers for their comments on the manuscript; in particular, comments from one of the reviewers led us to consider the impact of dynamical correlations on the GVB description of the states with recoupled pair bonds. NR 61 TC 7 Z9 7 U1 3 U2 8 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JAN 21 PY 2015 VL 142 IS 3 AR 034113 DI 10.1063/1.4905271 PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AZ6BJ UT WOS:000348302900013 PM 25612695 ER PT J AU Gao, Y Neuhauser, D Baer, R Rabani, E AF Gao, Yi Neuhauser, Daniel Baer, Roi Rabani, Eran TI Sublinear scaling for time-dependent stochastic density functional theory SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID AB-INITIO CALCULATION; OPTICAL-SPECTRA; REAL-TIME; SYSTEMS; ATOMS; APPROXIMATION; EXCITATIONS; ABSORPTION; MOLECULES; ENERGIES AB A stochastic approach to time-dependent density functional theory is developed for computing the absorption cross section and the random phase approximation (RPA) correlation energy. The core idea of the approach involves time-propagation of a small set of stochastic orbitals which are first projected on the occupied space and then propagated in time according to the time-dependent Kohn-Sham equations. The evolving electron density is exactly represented when the number of random orbitals is infinite, but even a small number (approximate to 16) of such orbitals is enough to obtain meaningful results for absorption spectrum and the RPA correlation energy per electron. We implement the approach for silicon nanocrystals using real-space grids and find that the overall scaling of the algorithm is sublinear with computational time and memory. (c) 2015 AIP Publishing LLC. C1 [Gao, Yi; Neuhauser, Daniel] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. [Baer, Roi] Hebrew Univ Jerusalem, Inst Chem, Fritz Haber Ctr Mol Dynam, IL-91904 Jerusalem, Israel. [Rabani, Eran] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Rabani, Eran] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Gao, Y (reprint author), Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. OI Gao, Yi/0000-0001-7045-9595 FU Israel Science Foundation-FIRST Program [1700/14]; DOE, Office of Science, Office of Basic Energy Sciences [DE-SC0001342]; National Science Foundation (NSF) [CHE-1112500] FX R.B. and ER. are supported by The Israel Science Foundation-FIRST Program (Grant No. 1700/14). Y.G. and D.N. are part of the Molecularly Engineered Energy Materials (MEEM), an Energy Frontier Research Center funded by the DOE, Office of Science, Office of Basic Energy Sciences under Award No. DE-SC0001342. D.N. also acknowledges support by the National Science Foundation (NSF), Grant No. CHE-1112500. NR 44 TC 8 Z9 8 U1 0 U2 7 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JAN 21 PY 2015 VL 142 IS 3 AR 034106 DI 10.1063/1.4905568 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AZ6BJ UT WOS:000348302900006 PM 25612688 ER PT J AU Kim, DS Smith, HL Niedziela, JL Li, CW Abernathy, DL Fultz, B AF Kim, D. S. Smith, H. L. Niedziela, J. L. Li, C. W. Abernathy, D. L. Fultz, B. TI Phonon anharmonicity in silicon from 100 to 1500 K SO PHYSICAL REVIEW B LA English DT Article ID INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; THERMAL-EXPANSION; RAMAN-SCATTERING; BASIS-SET; GERMANIUM; SI; SEMICONDUCTORS; NANOWIRES AB Inelastic neutron scattering was performed on silicon powder to measure the phonon density of states (DOS) from 100 to 1500 K. The mean fractional energy shifts with temperature of the modes were = -0.07, giving a mean isobaric Gruneisen parameter of +6.95 +/- 0.67, which is significantly different from the isothermal parameter of +0.98. These large effects are beyond the predictions from quasiharmonic models using density functional theory or experimental data, demonstrating large effects from phonon anharmonicity. At 1500 K the anharmonicity contributes 0.15k(B)/atom to the vibrational entropy, compared to 0.03k(B)/atom from quasiharmonicity. Excellent agreement was found between the entropy from phonon DOS measurements and the reference NIST-JANAF thermodynamic entropy from calorimetric measurements. C1 [Kim, D. S.; Smith, H. L.; Fultz, B.] CALTECH, Dept Appl Phys & Mat Sci, Pasadena, CA 91125 USA. [Niedziela, J. L.] Oak Ridge Natl Lab, Instrument & Source Div, Oak Ridge, TN 37831 USA. [Li, C. W.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Abernathy, D. L.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP Kim, DS (reprint author), CALTECH, Dept Appl Phys & Mat Sci, Pasadena, CA 91125 USA. EM dskim@caltech.edu RI Abernathy, Douglas/A-3038-2012; BL18, ARCS/A-3000-2012; OI Abernathy, Douglas/0000-0002-3533-003X; Kim, Dennis S/0000-0002-5707-2609 FU Scientific User Facilities Division, BES, DOE; DOE Office of Science, BES [DE-FG02-03ER46055] FX The authors thank F. H. Saadi for assisting in sample preparation and discussions. Research at Oak Ridge National Laboratory's SNS was sponsored by the Scientific User Facilities Division, BES, DOE. This work was supported by the DOE Office of Science, BES, under Contract No. DE-FG02-03ER46055. NR 51 TC 5 Z9 5 U1 2 U2 28 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 21 PY 2015 VL 91 IS 1 AR 014307 DI 10.1103/PhysRevB.91.014307 PG 6 WC Physics, Condensed Matter SC Physics GA CA2EY UT WOS:000348722900001 ER PT J AU Lischner, J Bazhirov, T MacDonald, AH Cohen, ML Louie, SG AF Lischner, Johannes Bazhirov, Timur MacDonald, Allan H. Cohen, Marvin L. Louie, Steven G. TI First-principles theory of electron-spin fluctuation coupling and superconducting instabilities in iron selenide SO PHYSICAL REVIEW B LA English DT Article AB We present first-principles calculations of the coupling of quasiparticles to spin fluctuations in iron selenide and discuss which types of superconducting instabilities this coupling gives rise to. We find that strong antiferromagnetic stripe-phase spin fluctuations lead to large coupling constants for superconducting gaps with s(+/-) symmetry, but these coupling constants are significantly reduced by other spin fluctuations with small wave vectors. An accurate description of this competition and an inclusion of band-structure and Stoner parameter renormalization effects lead to a value of the coupling constant for an s(+/-)-symmetric gap which can produce a superconducting transition temperature consistent with experimental measurements. C1 [Lischner, Johannes; Bazhirov, Timur; Cohen, Marvin L.; Louie, Steven G.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Lischner, Johannes; Bazhirov, Timur; Cohen, Marvin L.; Louie, Steven G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [MacDonald, Allan H.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. RP Lischner, J (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM jlischner@civet.berkeley.edu FU NSF [DMR10-1006184]; SciDAC Program on Excited State Phenomena (methods and software developments) and Theory Program (magnetic susceptibility calculations) - U.S. Department of Energy, the Office of Basic [DE-AC02-05CH11231] FX J.L. acknowledges valuable discussions with L. Kemper, S. Coh, H. Oh, and D. Scalapino. This work was supported by NSF Grant No. DMR10-1006184 (theoretical analysis) and by the SciDAC Program on Excited State Phenomena (methods and software developments) and Theory Program (magnetic susceptibility calculations) funded by the U.S. Department of Energy, the Office of Basic Energy Sciences, and of Advanced Scientific Computing Research, under Contract No. DE-AC02-05CH11231 at the Lawrence Berkeley National Laboratory. Computational resources have been provided by the DOE at NERSC. NR 40 TC 7 Z9 7 U1 3 U2 25 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 21 PY 2015 VL 91 IS 2 AR 020502 DI 10.1103/PhysRevB.91.020502 PG 5 WC Physics, Condensed Matter SC Physics GA CA2FM UT WOS:000348724400001 ER PT J AU Taghavi, S Wu, X Ouyang, LM Zhang, YB Stadler, A McCorkle, S Zhu, W Maslov, S Van der Lelie, D AF Taghavi, Safiyh Wu, Xiao Ouyang, Liming Zhang, Yian Biao Stadler, Andrea McCorkle, Sean Zhu, Wei Maslov, Sergei Van der Lelie, Daniel TI Transcriptional Responses to Sucrose Mimic the Plant-Associated Life Style of the Plant Growth Promoting Endophyte Enterobacter sp 638 SO PLOS ONE LA English DT Article ID ESCHERICHIA-COLI K-12; DIFFERENTIAL EXPRESSION ANALYSIS; QUORUM-SENSING SIGNAL; BINDING PROTEIN CSRA; GENE-EXPRESSION; BIOFILM FORMATION; RNA-SEQ; INDOLE-3-ACETIC-ACID BIOSYNTHESIS; PSEUDOMONAS-AERUGINOSA; SYSTEMIC RESISTANCE AB Growth in sucrose medium was previously found to trigger the expression of functions involved in the plant associated life style of the endophytic bacterium Enterobacter sp. 638. Therefore, comparative transcriptome analysis between cultures grown in sucrose or lactate medium was used to gain insights in the expression levels of bacterial functions involved in the endophytic life style of strain 638. Growth on sucrose as a carbon source resulted in major changes in cell physiology, including a shift from a planktonic life style to the formation of bacterial aggregates. This shift was accompanied by a decrease in transcription of genes involved in motility (e.g. flagella biosynthesis) and an increase in the transcription of genes involved in colonization, adhesion and biofilm formation. The transcription levels of functions previously suggested as being involved in endophytic behavior and functions responsible for plant growth promoting properties, including the synthesis of indole-acetic acid, acetoin and 2,3-butanediol, also increased significantly for cultures grown in sucrose medium. Interestingly, despite an abundance of essential nutrients transcription levels of functions related to uptake and processing of nitrogen and iron became increased for cultures grown on sucrose as sole carbon source. Transcriptome data were also used to analyze putative regulatory relationships. In addition to the small RNA csrABCD regulon, which seems to play a role in the physiological adaptation and possibly the shift between free-living and plant-associated endophytic life style of Enterobacter sp. 638, our results also pointed to the involvement of rcsAB in controlling responses by Enterobacter sp. 638 to a plant-associated life style. Targeted mutagenesis was used to confirm this role and showed that compared to wild-type Enterobacter sp. 638 a Delta rcsB mutant was affected in its plant growth promoting ability. C1 [Taghavi, Safiyh; Ouyang, Liming; Van der Lelie, Daniel] Ctr Agr & Environm Biotechnol, RTI Int, Charlotte, NC USA. [Taghavi, Safiyh; Wu, Xiao; Zhang, Yian Biao; Stadler, Andrea; McCorkle, Sean; Maslov, Sergei; Van der Lelie, Daniel] Dept Biosci, Brookhaven Natl Lab, Upton, NY USA. [Wu, Xiao; Zhu, Wei] SUNY Stony Brook, Dept Appl Math & Stat, Stony Brook, NY 11794 USA. [Ouyang, Liming] E China Univ Sci & Technol, Sch Biotechnol, State Key Lab Bioreactor Engn, Shanghai 200237, Peoples R China. RP Van der Lelie, D (reprint author), FMC Corp, Ctr Excellence Agr Biotechnol, Res Triangle Pk, Charlotte, NC 28208 USA. EM daniel.vanderlelie@FMC.com OI Maslov, Sergei/0000-0002-3701-492X FU U.S. Department of Energy, Office of Science, BER [KP1102010, DE-AC02-98CH10886]; Laboratory Directed Research and Development funds at the Brookhaven National Laboratory [LDRD09-005] FX This research was funded by the U.S. Department of Energy, Office of Science, BER, Project KP1102010 under Contract DE-AC02-98CH10886, and by Laboratory Directed Research and Development funds (LDRD09-005) at the Brookhaven National Laboratory under contract with the U.S. Department of Energy. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 63 TC 5 Z9 5 U1 4 U2 47 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JAN 21 PY 2015 VL 10 IS 1 AR e0115455 DI 10.1371/journal.pone.0115455 PG 22 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AZ4PR UT WOS:000348205300014 PM 25607953 ER PT J AU Sun, YG Wang, L Liu, YZ Ren, Y AF Sun, Yugang Wang, Lin Liu, Yuzi Ren, Yang TI Birnessite-Type MnO2 Nanosheets with Layered Structures Under High Pressure: Elimination of Crystalline Stacking Faults and Oriented Laminar Assembly SO SMALL LA English DT Article ID GRAPHENE-BASED MATERIALS; MANGANESE OXIDE; ELECTRONIC-STRUCTURE; BORON-NITRIDE; FIELD; MOS2; HETEROSTRUCTURES; NANOMATERIALS; GENERATION; GERMANANE C1 [Sun, Yugang; Liu, Yuzi] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Wang, Lin] Carnegie Inst Sci, Geophys Lab, HPSync, Argonne, IL 60439 USA. [Wang, Lin] Jilin Univ, State Key Lab Superhard Mat, Changchun 130012, Peoples R China. [Wang, Lin] Ctr High Pressure Sci & Technol Adv Res, Shanghai 201203, Peoples R China. [Ren, Yang] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. RP Sun, YG (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 South Cass Ave, Argonne, IL 60439 USA. EM ygsun@anl.gov RI Sun, Yugang /A-3683-2010; Liu, Yuzi/C-6849-2011 OI Sun, Yugang /0000-0001-6351-6977; FU Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility [DE-AC02-06CH11357]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; CIW; CDAC; UNLV; LLNL from DOE-NNSA; DOE-BES; NSF; EFree, an Energy Frontier Research Center - U.S. Department of Energy (DOE), Office of Science [DE-SC0001057]; National Natural Science Foundation of China (NSFC) [11004072]; Program for New Century Excellent Talents in University [NCET-10-0444] FX This work was performed at the Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility under contract No. DE-AC02-06CH11357. Use of Advanced Photon Source (beamline 11ID-C, 16ID-B, 16BM-D) was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract No. DE-AC02-06CH11357. HPCAT is supported by CIW, CDAC, UNLV and LLNL through funding from DOE-NNSA, DOE-BES, and NSF. Lin Wang is supported by EFree, an Energy Frontier Research Center funded by the U.S. Department of Energy (DOE), Office of Science under DE-SC0001057, the National Natural Science Foundation of China (NSFC, 11004072) and Program for New Century Excellent Talents in University (NCET-10-0444). NR 53 TC 9 Z9 9 U1 8 U2 74 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1613-6810 EI 1613-6829 J9 SMALL JI Small PD JAN 21 PY 2015 VL 11 IS 3 BP 300 EP 305 DI 10.1002/smll.201400892 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AZ3PR UT WOS:000348139800004 PM 25179122 ER PT J AU Frantti, J Fujioka, Y Puretzky, A Xie, Y Ye, ZG Parish, C Glazer, AM AF Frantti, J. Fujioka, Y. Puretzky, A. Xie, Y. Ye, Z-G Parish, C. Glazer, A. M. TI Phase transitions and thermal-stress-induced structural changes in a ferroelectric Pb(Zr0.80Ti0.20)O-3 single crystal SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE lead-zirconate-titanate; Raman scattering; phase transition ID LEAD-ZIRCONATE-TITANATE; NEUTRON-DIFFRACTION; MONOCLINIC PHASE; PBZR1-XTIXO3; PEROVSKITES; CERAMICS; PBTIO3; SERIES AB A single crystal of lead-zirconate-titanate, composition Pb(Zr0.80Ti0.20)O-3, was studied by polarized-Raman scattering as a function of temperature. Raman spectra reveal that the local structure deviates from the average structure in both ferroelectric and paraelectric phases. We show that the crystal possesses several, inequivalent complex domain boundaries which show no sign of instability even 200 K above the ferroelectric-to-paraelectric phase transition temperature T-C. Two types of boundaries are addressed. The first boundary was formed between ferroelectric domains below T-C. This boundary remained stable up to the highest measurement temperatures, and stabilized the domains so that they had the same orientation after repeated heating and cooling cycles. These domains transformed normally to the cubic paraelectric phase. Another type of boundary was formed at 673 K and exhibited no signs of instability up to 923 K. The boundary formation was reversible: it formed and vanished between 573 and 673 K during heating and cooling, respectively. A model in which the crystal is divided into thin slices with different Zr/Ti ratios is proposed. The physical mechanism behind the thermal-stress-induced structural changes is related to the different thermal expansion of the slices, which forces the domain to grow similarly after each heating and cooling cycle. The results are interesting for non-volatile memory development, as it implies that the original ferroelectric state can be restored after the material has been transformed to the paraelectric phase. It also suggests that a low-symmetry structure, stable up to high temperatures, can be prepared through controlled deposition of layers with desired compositions. C1 [Puretzky, A.; Parish, C.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Xie, Y.; Ye, Z-G] Simon Fraser Univ, Dept Chem, Burnaby, BC V5A 1S6, Canada. [Xie, Y.; Ye, Z-G] Simon Fraser Univ, LABS 4D, Burnaby, BC V5A 1S6, Canada. [Glazer, A. M.] Univ Oxford, Dept Phys, Clarendon Lab, Oxford OX1 3PU, England. RP Frantti, J (reprint author), Jaalaranta 9 B 42, Helsinki 00180, Finland. EM johannes.frantti@fre.fi RI Puretzky, Alexander/B-5567-2016; Parish, Chad/J-8381-2013 OI Puretzky, Alexander/0000-0002-9996-4429; FU Engineering and Physical Sciences Research Council [EP/G026696/1] NR 33 TC 3 Z9 3 U1 4 U2 24 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD JAN 21 PY 2015 VL 27 IS 2 AR 025901 DI 10.1088/0953-8984/27/2/025901 PG 14 WC Physics, Condensed Matter SC Physics GA AX2TP UT WOS:000346797700014 PM 25531118 ER PT J AU Ghimire, NJ Ronning, F Williams, DJ Scott, BL Luo, YK Thompson, JD Bauer, ED AF Ghimire, N. J. Ronning, F. Williams, D. J. Scott, B. L. Luo, Yongkang Thompson, J. D. Bauer, E. D. TI Investigation of the physical properties of the tetragonal CeMAl4Si2 (M = Rh, Ir, Pt) compounds SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE Ce-based intermetallic compounds; heavy-fermions; electronic anisotropy ID HEAVY-FERMION COMPOUNDS; HOMOLOGOUS SERIES; KONDO-LATTICE; SUPERCONDUCTIVITY; MAGNETISM; CRYSTAL AB The synthesis, crystal structure and physical properties studied by means of x-ray diffraction, magnetic, thermal and transport measurements of CeMAl4Si2 (M = Rh, Ir, Pt) are reported, along with the electronic structure calculations for LaMAl4Si2 (M = Rh, Ir, Pt). These materials adopt a tetragonal crystal structure (space group P4/ mmm) comprised of BaAl4 blocks, separated by MAl2 units, stacked along the c-axis. Both CeRhAl4Si2 and CeIrAl4Si2 order antiferromagnetically below T-N1 = 14 and 16 K, respectively, and undergo a second antiferromagnetic transitition at lower temperature (T-N2 = 9 and 14 K, respectively). CePtAl4Si2 orders ferromagnetically below T-C = 3 K with an ordered moment of mu(sat) = 0.8 mu(B) for a magnetic field applied perpendicular to the c-axis. Electronic structure calculations reveal quasi-2D character of the Fermi surface. C1 [Ghimire, N. J.; Ronning, F.; Williams, D. J.; Scott, B. L.; Luo, Yongkang; Thompson, J. D.; Bauer, E. D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Ghimire, NJ (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM nghimire@lanl.gov RI Scott, Brian/D-8995-2017; OI Scott, Brian/0000-0003-0468-5396; Ronning, Filip/0000-0002-2679-7957; Bauer, Eric/0000-0003-0017-1937 FU US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; US DOE, OBES, Division of Material Science and Engineering; National Nuclear Security Administration of the US Department of Energy [DE-AC52-06NA25396]; Los Alamos ADRD program FX Work at Los Alamos National Laboratory was performed under the auspices of the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering and PECASE funding from the US DOE, OBES, Division of Material Science and Engineering. The EDS measurements were performed at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the US Department of Energy ( DOE) Office of Science. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the US Department of Energy under contract DE-AC52-06NA25396. Y Luo acknowledges a Director's Postdoctoral Fellowship supported through the Los Alamos ADRD program. NR 24 TC 10 Z9 10 U1 2 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD JAN 21 PY 2015 VL 27 IS 2 AR 025601 DI 10.1088/0953-8984/27/2/025601 PG 9 WC Physics, Condensed Matter SC Physics GA AX2TP UT WOS:000346797700011 PM 25501402 ER PT J AU Martinez, HP Pawelczak, I Glenn, AM Carman, ML Zaitseva, N Payne, S AF Martinez, H. Paul Pawelczak, Iwona Glenn, Andrew M. Carman, M. Leslie Zaitseva, Natalia Payne, Stephen TI Pulse shape discrimination in non-aromatic plastics SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Pulse shape discrimination; Plastics; Scintillators; Aromatic; Non-aromatic ID ORGANIC SCINTILLATORS AB Recently it has been demonstrated that plastic scintillators have the ability to distinguish neutrons from gamma rays by way of pulse shape discrimination (PSD). This discovery has lead to new materials and new capabilities. Here we report our work with the effects of aromatic, non-aromatic, and mixed aromatic/non-aromatic matrices have on the performance of PSD plastic scintillators. (C) 2014 Elsevier B.V. All rights reserved C1 [Martinez, H. Paul; Pawelczak, Iwona; Glenn, Andrew M.; Carman, M. Leslie; Zaitseva, Natalia; Payne, Stephen] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Martinez, HP (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave L 188, Livermore, CA 94550 USA. FU U.S. DOE, NNSA, Office of Defense Nuclear Nonproliferation, Office of Nonproliferation Research and Development [NA-22]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was supported by the U.S. DOE, NNSA, Office of Defense Nuclear Nonproliferation, Office of Nonproliferation Research and Development (NA-22) and performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. LLNL-JRNL-654062. NR 14 TC 3 Z9 3 U1 4 U2 18 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JAN 21 PY 2015 VL 771 BP 28 EP 31 DI 10.1016/j.nima.2014.10.023 PG 4 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AX0KQ UT WOS:000346641800005 ER PT J AU Dazeley, S Asghari, A Bernstein, A Bowden, NS Mozin, V AF Dazeley, S. Asghari, A. Bernstein, A. Bowden, N. S. Mozin, V. TI A water-based neutron detector as a well multiplicity counter SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Water Cherenkov; Neutron detector; Multiplicity well counter; Spontaneous fission; Spent fuel; Gadolinium ID DOPED WATER AB We report the performance characteristics of a water based neutron detecting multiplicity counter for the non-destructive assay of fissile sources. This technique could replace or supplement existing He-3-based multiplicity counters. The counter is a 1.02 m(3) Lank containing pure deionized water doped with 0.5% GdCl3 It has highly reflective walls and eight 10-in. PMTs mounted at the top. An unshielded source well of 19 cm diameter, mounted at the top and center, extends 73 cm down into the detector. The counter was evaluated using low intensity Cf-252 and 6 Co sources, and a fast pulsing LED to simulate higher intensity backgrounds. At low gamma ray intensities (similar to 200 kBq or less) we report an absolute neutron detection efficiency of 28% and a 6 C0 rejection/suppression factor of similar to 10(8) to 1. For sources with high gamma ray intensities, the neutron efficiency was 22% + 1% up to a GuCo equivalent activity of 4 MBq. The detector background event rate, primarily due to muons and other cosmogenic particles, was found to be stable over a period of almost three months. The minimum detectable neutron source intensity above background was 3.1 n/s, assuming a one-hour data acquisition. 2014 Elsevier By. All rights reserved. C1 [Dazeley, S.; Bernstein, A.; Bowden, N. S.; Mozin, V.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Asghari, A.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. RP Dazeley, S (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave,L-211, Livermore, CA 94550 USA. EM dazeley2@llnl.gov FU US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; DOE [NA-22] FX We would like to thank Darrell Carter for his expert technical help with both the detector design and construction and John Steele for programming the trigger logic in the FPGA. This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344, release number LLNL-JRNL-654196. The authors wish to thank the DOE NA-22 for their support of this project. NR 18 TC 1 Z9 1 U1 0 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JAN 21 PY 2015 VL 771 BP 32 EP 38 DI 10.1016/j.nima.2014.10.028 PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AX0KQ UT WOS:000346641800006 ER PT J AU Foxe, M Hagmann, C Jovanovic, I Bernstein, A Kazkaz, K Mozin, V Pereverzev, SV Sangiorgio, S Sorensen, P AF Foxe, M. Hagmann, C. Jovanovic, I. Bernstein, A. Kazkaz, K. Mozin, V. Pereverzev, S. V. Sangiorgio, S. Sorensen, P. TI Low-energy (< 10 keV) electron ionization and recombination model for a liquid argon detector SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Liquid argon; Electron transport; Ionization track; Electron recombination ID ION RECOMBINATION; SIMULATION; TRANSPORT; XENON; THERMALIZATION; DRIFT AB Detailed understanding of the ionization process in noble liquid detectors is important for their use in applications such as the search for dark matter and coherent elastic neutrino nucleus scattering. The response of noble liquid detectors to low energy ionization events is poorly understood at this time. We describe a new simulation tool which predicts the ionization yield from electronic energy deposits (E < 10 keV) in liquid Ar, including the dependence of the yield on the applied electric drift field. The ionization signal produced in a liquid argon detector from Ar-37 beta decay and Fe-55 X-rays has been calculated using the new model. Published by Elsevier B.V. C1 [Foxe, M.; Jovanovic, I.] Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16802 USA. [Foxe, M.; Hagmann, C.; Bernstein, A.; Kazkaz, K.; Mozin, V.; Pereverzev, S. V.; Sangiorgio, S.; Sorensen, P.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Foxe, M.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Foxe, M (reprint author), Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16802 USA. EM michael.Foxe@pnnl.gov FU U.S. Department of Energy by the Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Nuclear Forensics Graduate Fellowship Program; U.S. Department of Homeland Security, Domestic Nuclear Detection Office; U.S. Department of Defense, Defense Threat Reduction Agency [PNNL-SA-100217] FX This work was performed tinder the auspices of the U.S. Department of Energy by the Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. A portion of M. Foxes research was performed under the Nuclear Forensics Graduate Fellowship Program, which is sponsored by the U.S. Department of Homeland Security, Domestic Nuclear Detection Office and the U.S. Department of Defense, Defense Threat Reduction Agency PNNL-SA-100217. NR 31 TC 4 Z9 4 U1 2 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JAN 21 PY 2015 VL 771 BP 88 EP 92 DI 10.1016/j.nima.2014.10.055 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AX0KQ UT WOS:000346641800013 ER PT J AU Classen, T Bernstein, A Bowden, NS Cabrera-Palmer, B Ho, A Jonkmans, G Kogler, L Reyna, D Sur, B AF Classen, T. Bernstein, A. Bowden, N. S. Cabrera-Palmer, B. Ho, A. Jonkmans, G. Kogler, L. Reyna, D. Sur, B. TI Development of an advanced antineutrino detector for reactor monitoring SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Nuclear reactor safeguards; Antineutrino detection AB Here we present the development of a compact antineutrino detector for the purpose of nuclear reactor monitoring, improving upon a previously successful design. This paper will describe the design improvements of the detector which increases the antineutrino detection efficiency threefold over the previous effort. There are two main design improvements over previous generations of detectors for nuclear reactor monitoring: dual-ended optical readout and single volume detection mass. The dual-ended optical readout eliminates the need for fiducialization and increases the uniformity of the detector's optical response. The containment of the detection mass in a single active volume provides more target mass per detector footprint, a key design criteria for operating within a nuclear power plant. This technology could allow for real-time monitoring of the evolution of a nuclear reactor core, independent of reactor operator declarations of fuel inventories, and may be of interest to the safeguards community. (C) 2014 Elsevier B.V. All rights reserved, C1 [Classen, T.; Bernstein, A.; Bowden, N. S.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Cabrera-Palmer, B.; Kogler, L.; Reyna, D.] Sandia Livermore Natl Labs, Livermore, CA 94550 USA. [Ho, A.; Jonkmans, G.; Sur, B.] Atom Energy Canada Ltd, Chalk River Nucl Labs, Chalk River, ON K0J 1J0, Canada. RP Classen, T (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM classen2@llnl.gov FU U.S. Department of Energy Office of Defense Nuclear Nonproliferation Research and Development; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC5-07NA27344, LLNL-JRNL-655279]; U.S. Department of Energy National Nuclear Security Administration [DE-AC04-94AL85000, SAND2014-151090] FX This work was supported by the U.S. Department of Energy Office of Defense Nuclear Nonproliferation Research and Development. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC5-07NA27344, LLNL-JRNL-655279.; Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy National Nuclear Security Administration under contract DE-AC04-94AL85000, SAND2014-151090. NR 10 TC 2 Z9 3 U1 0 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JAN 21 PY 2015 VL 771 BP 139 EP 146 DI 10.1016/j.nima.2014.10.022 PG 8 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA AX0KQ UT WOS:000346641800022 ER PT J AU Gao, XY Zhi, XY Li, HW Zhou, Y Lapidus, A Han, J Haynes, M Lobos, E Huntemann, M Pati, A Ivanova, NN Mavromatis, K Tindall, BJ Markowitz, V Woyke, T Klenk, HP Kyrpides, NC Li, WJ AF Gao, Xiao-Yang Zhi, Xiao-Yang Li, Hong-Wei Zhou, Yu Lapidus, Alla Han, James Haynes, Matthew Lobos, Elizabeth Huntemann, Marcel Pati, Amrita Ivanova, Natalia N. Mavromatis, Konstantinos Tindall, Brian J. Markowitz, Victor Woyke, Tanja Klenk, Hans-Peter Kyrpides, Nikos C. Li, Wen-Jun TI Draft genome sequence of Halomonas lutea strain YIM 91125(T) (DSM 23508(T)) isolated from the alkaline Lake Ebinur in Northwest China SO STANDARDS IN GENOMIC SCIENCES LA English DT Article DE Halomonas lutea; Aerobic; Gram-negative; Chemoorganotrophic; Moderately halophilic; Lake Ebinur ID STANDARD OPERATING PROCEDURE; SP-NOV.; MAXIMUM-LIKELIHOOD; MICROBIAL GENOMES; SOLAR SALTERN; BACTERIUM; PHYLOGENY; DATABASE; ARCHAEA; ENCYCLOPEDIA AB Species of the genus Halomonas are halophilic and their flexible adaption to changes of salinity and temperature brings considerable potential biotechnology applications, such as degradation of organic pollutants and enzyme production. The type strain Halomonas lutea YIM 91125T was isolated from a hypersaline lake in China. The genome of strain YIM 91125T becomes the twelfth species sequenced in Halomonas, and the thirteenth species sequenced in Halomonadaceae. We described the features of H. lutea YIM 91125T, together with the high quality draft genome sequence and annotation of its type strain. The 4,533,090 bp long genome of strain YIM 91125T with its 4,284 protein-coding and 84 RNA genes is a part of Genomic Encyclopedia of Type Strains, Phase I: the one thousand microbial genomes (KMG-I) project. From the viewpoint of comparative genomics, H. lutea has a larger genome size and more specific genes, which indicated acquisition of function bringing better adaption to its environment. DDH analysis demonstrated that H. lutea is a distinctive species, and halophilic features and nitrogen metabolism related genes were discovered in its genome. C1 [Gao, Xiao-Yang; Li, Wen-Jun] Chinese Acad Sci, Xinjiang Inst Ecol & Geog, Key Lab Biogeog & Bioresource Arid Land, Urumqi, Peoples R China. [Zhi, Xiao-Yang; Li, Hong-Wei; Li, Wen-Jun] Yunnan Univ, Key Lab Microbial Divers Southwest China, Minist Educ, Kunming, Peoples R China. [Zhi, Xiao-Yang; Li, Hong-Wei; Li, Wen-Jun] Yunnan Univ, Lab Conservat & Utilizat Bioresources, Yunnan Inst Microbiol, Kunming, Peoples R China. [Lapidus, Alla] St Petersburg State Univ, Theodosius Dobzhansky Ctr Genome Bionformat, St Petersburg 199034, Russia. [Lapidus, Alla] St Petersburg Acad Univ, Algorithm Biol Lab, St Petersburg, Russia. [Han, James; Haynes, Matthew; Lobos, Elizabeth; Huntemann, Marcel; Pati, Amrita; Ivanova, Natalia N.; Mavromatis, Konstantinos; Woyke, Tanja; Kyrpides, Nikos C.] DOE Joint Genome Inst, Walnut Creek, CA USA. [Markowitz, Victor] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Data Management & Technol Ctr, Berkeley, CA 94720 USA. [Tindall, Brian J.; Klenk, Hans-Peter] Leibniz Inst DSMZ German Collect Microorganisms &, Braunschweig, Germany. [Kyrpides, Nikos C.] King Abdulaziz Univ, Dept Biol Sci, Jeddah 21413, Saudi Arabia. [Li, Hong-Wei] Kunming Med Univ, Hosp Qujing City 1, Qujing Affiliated Hosp, Qujing, Peoples R China. [Zhou, Yu] Zhejiang Acad Agr Sci, State Key Lab Breeding Base Zhejiang Sustainable, Inst Qual & Standard Agroprod, Hangzhou, Zhejiang, Peoples R China. [Gao, Xiao-Yang] Univ Chinese Acad Sci, Beijing, Peoples R China. [Klenk, Hans-Peter] Newcastle Univ, Sch Biol, Newcastle Upon Tyne NE1 7RU, Tyne & Wear, England. RP Li, WJ (reprint author), Chinese Acad Sci, Xinjiang Inst Ecol & Geog, Key Lab Biogeog & Bioresource Arid Land, Urumqi, Peoples R China. EM liwenjun@ms.xjb.ac.cn RI Kyrpides, Nikos/A-6305-2014; Fac Sci, KAU, Biol Sci Dept/L-4228-2013; Lapidus, Alla/I-4348-2013; OI Kyrpides, Nikos/0000-0002-6131-0462; Lapidus, Alla/0000-0003-0427-8731; Ivanova, Natalia/0000-0002-5802-9485 FU US Department of Energy's Office of Science, Biological and Environmental Research Program; University of California, Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Russian Ministry of Science Mega-grant [11.G34.31.0068]; Chinese Academy of Sciences; Livermore National Laboratory [DE-AC52-07NA27344] FX Susanne Schneider is gratefully acknowledged the assistance for growing H. lutea cultures. We also thank Evelyne-Marie Brambilla for DNA extraction and quality control (both at the DSMZ). This work was performed under the auspices of the US Department of Energy's Office of Science, Biological and Environmental Research Program, and by the University of California, Lawrence Berkeley National Laboratory under Contract No. DE-AC02-05CH11231, Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. A. L. was supported in part by Russian Ministry of Science Mega-grant no. 11.G34.31.0068 (Dr. Stephen J O'Brien Principal Investigator). W.-J. Li was supported by 'Hundred Talents Program' of the Chinese Academy of Sciences. NR 49 TC 0 Z9 0 U1 0 U2 11 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD JAN 20 PY 2015 VL 10 AR 1 DI 10.1186/1944-3277-10-1 PG 9 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA CV2YO UT WOS:000364125400001 PM 25678942 ER PT J AU Aartsen, MG Ackermann, M Adams, J Aguilar, JA Ahlers, M Ahrens, M Altmann, D Anderson, T Arguelles, C Arlen, TC Auffenberg, J Bai, X Barwick, SW Baum, V Beatty, JJ Tjus, JB Becker, KH BenZvi, S Berghaus, P Berley, D Bernardini, E Bernhard, A Besson, DZ Binder, G Bindig, D Bissok, M Blaufuss, E Blumenthal, J Boersma, DJ Bohm, C Bos, F Bose, D Boser, S Botner, O Brayeur, L Bretz, HP Brown, AM Casey, J Casier, M Chirkin, D Christov, A Christy, B Clark, K Classen, L Clevermann, F Coenders, S Cowen, DF Silva, AHC Danninger, M Daughhetee, J Davis, JC Day, M de Andre, JPAM De Clercq, C De Ridder, S Desiati, P de Vries, KD de With, M DeYoung, T Diaz-Velez, JC Dunkman, M Eagan, R Eberhardt, B Eichmann, B Eisch, J Euler, S Evenson, PA Fadiran, O Fazely, AR Fedynitch, A Feintzeig, J Felde, J Feusels, T Filimonov, K Finley, C Fischer-Wasels, T Flis, S Franckowiak, A Frantzen, K Fuchs, T Gaisser, TK Gallagher, J Gerhardt, L Gier, D Gladstone, L Glusenkamp, T Goldschmidt, A Golup, G Gonzalez, JG Goodman, JA Gora, D Grandmont, DT Grant, D Gretskov, P Groh, JC Gross, A Ha, C Haack, C Ismail, AH Hallen, P Hallgren, A Halzen, F Hanson, K Hebecker, D Heereman, D Heinen, D Helbing, K Hellauer, R Hellwig, D Hickford, S Hill, GC Hoffman, KD Hoffmann, R Homeier, A Hoshina, K Huang, F Huelsnitz, W Hulth, PO Hultqvist, K Hussain, S Ishihara, A Jacobi, E Jacobsen, J Jagielski, K Japaridze, GS Jero, K Jlelati, O Jurkovic, M Kaminsky, B Kappes, A Karg, T Karle, A Kauer, M Kelley, JL Kheirandish, A Kiryluk, J Klas, J Klein, SR Kohne, JH Kohnen, G Kolanoski, H Koob, A Kopke, L Kopper, C Kopper, S Koskinen, DJ Kowalski, M Kriesten, A Krings, K Kroll, G Kroll, M Kunnen, J Kurahashi, N Kuwabara, T Labare, M Larsen, DT Larson, MJ Lesiak-Bzdak, M Leuermann, M Leute, J Lunemann, J Macias, O Madsen, J Maggi, G Maruyama, R Mase, K Matis, HS McNally, F Meagher, K Medici, M Meli, A Meures, T Miarecki, S Middell, E Middlemas, E Milke, N Miller, J Mohrmann, L Montaruli, T Morse, R Nahnhauer, R Naumann, U Niederhausen, H Nowicki, SC Nygren, DR Obertacke, A Odrowski, S Olivas, A Omairat, A O'Murchadha, A Palczewski, T Paul, L Penek, O Pepper, JA de los Heros, CP Pfendner, C Pieloth, D Pinat, E Posselt, J Price, PB Przybylski, GT Putz, J Quinnan, M Radel, L Rameez, M Rawlins, K Redl, P Rees, I Reimann, R Resconi, E Rhode, W Richman, M Riedel, B Robertson, S Rodrigues, JP Rongen, M Rott, C Ruhe, T Ruzybayev, B Ryckbosch, D Saba, SM Sander, HG Sandroos, J Santander, M Sarkar, S Schatto, K Scheriau, F Schmidt, T Schmitz, M Schoenen, S Schoneberg, S Schnowald, A Schukraft, A Schulte, L Schulz, O Seckel, D Sestayo, Y Seunarine, S Shanidze, R Sheremata, C Smith, MWE Soldin, D Spiczak, GM Spiering, C Stamatikos, M Stanev, T Stanisha, NA Stasik, A Stezelberger, T Stokstad, RG Stossl, A Strahler, EA Strom, R Strotjohann, NL Sullivan, GW Taavola, H Taboada, I Tamburro, A Tepe, A Ter-Antonyan, S Terliuk, A Tesic, G Tilav, S Toale, PA Tobin, MN Tosi, D Tselengidou, M Unger, E Usner, M Vallecorsa, S Van Eijndhoven, N Vandenbroucke, J Van Santen, J Vehring, M Voge, M Vraeghe, M Walck, C Wallraff, M Weaver, C Wellons, M Wendt, C Westerhoff, S Whelan, BJ Whitehorn, N Wichary, C Wiebe, K Wiebusch, CH Williams, DR Wissing, H Wolf, M Wood, TR Woschnagg, K Xu, DL Xu, XW Yanez, JP Yodh, G Yoshida, S Zarzhitsky, P Ziemann, J Zierke, S Zoll, M AF Aartsen, M. G. Ackermann, M. Adams, J. Aguilar, J. A. Ahlers, M. Ahrens, M. Altmann, D. Anderson, T. Arguelles, C. Arlen, T. C. Auffenberg, J. Bai, X. Barwick, S. W. Baum, V. Beatty, J. J. Tjus, J. Becker Becker, K. -H. BenZvi, S. Berghaus, P. Berley, D. Bernardini, E. Bernhard, A. Besson, D. Z. Binder, G. Bindig, D. Bissok, M. Blaufuss, E. Blumenthal, J. Boersma, D. J. Bohm, C. Bos, F. Bose, D. Boeser, S. Botner, O. Brayeur, L. Bretz, H. -P. Brown, A. M. Casey, J. Casier, M. Chirkin, D. Christov, A. Christy, B. Clark, K. Classen, L. Clevermann, F. Coenders, S. Cowen, D. F. Silva, A. H. Cruz Danninger, M. Daughhetee, J. Davis, J. C. Day, M. de Andre, J. P. A. M. De Clercq, C. De Ridder, S. Desiati, P. de Vries, K. D. de With, M. DeYoung, T. Diaz-Velez, J. C. Dunkman, M. Eagan, R. Eberhardt, B. Eichmann, B. Eisch, J. Euler, S. Evenson, P. A. Fadiran, O. Fazely, A. R. Fedynitch, A. Feintzeig, J. Felde, J. Feusels, T. Filimonov, K. Finley, C. Fischer-Wasels, T. Flis, S. Franckowiak, A. Frantzen, K. Fuchs, T. Gaisser, T. K. Gallagher, J. Gerhardt, L. Gier, D. Gladstone, L. Gluesenkamp, T. Goldschmidt, A. Golup, G. Gonzalez, J. G. Goodman, J. A. Gora, D. Grandmont, D. T. Grant, D. Gretskov, P. Groh, J. C. Gross, A. Ha, C. Haack, C. Ismail, A. Haj Hallen, P. Hallgren, A. Halzen, F. Hanson, K. Hebecker, D. Heereman, D. Heinen, D. Helbing, K. Hellauer, R. Hellwig, D. Hickford, S. Hill, G. C. Hoffman, K. D. Hoffmann, R. Homeier, A. Hoshina, K. Huang, F. Huelsnitz, W. Hulth, P. O. Hultqvist, K. Hussain, S. Ishihara, A. Jacobi, E. Jacobsen, J. Jagielski, K. Japaridze, G. S. Jero, K. Jlelati, O. Jurkovic, M. Kaminsky, B. Kappes, A. Karg, T. Karle, A. Kauer, M. Kelley, J. L. Kheirandish, A. Kiryluk, J. Klaes, J. Klein, S. R. Koehne, J. -H. Kohnen, G. Kolanoski, H. Koob, A. Koepke, L. Kopper, C. Kopper, S. Koskinen, D. J. Kowalski, M. Kriesten, A. Krings, K. Kroll, G. Kroll, M. Kunnen, J. Kurahashi, N. Kuwabara, T. Labare, M. Larsen, D. T. Larson, M. J. Lesiak-Bzdak, M. Leuermann, M. 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Sheremata, C. Smith, M. W. E. Soldin, D. Spiczak, G. M. Spiering, C. Stamatikos, M. Stanev, T. Stanisha, N. A. Stasik, A. Stezelberger, T. Stokstad, R. G. Stoessl, A. Strahler, E. A. Stroem, R. Strotjohann, N. L. Sullivan, G. W. Taavola, H. Taboada, I. Tamburro, A. Tepe, A. Ter-Antonyan, S. Terliuk, A. Tesic, G. Tilav, S. Toale, P. A. Tobin, M. N. Tosi, D. Tselengidou, M. Unger, E. Usner, M. Vallecorsa, S. van Eijndhoven, N. Vandenbroucke, J. van Santen, J. Vehring, M. Voge, M. Vraeghe, M. Walck, C. Wallraff, M. Weaver, Ch. Wellons, M. Wendt, C. Westerhoff, S. Whelan, B. J. Whitehorn, N. Wichary, C. Wiebe, K. Wiebusch, C. H. Williams, D. R. Wissing, H. Wolf, M. Wood, T. R. Woschnagg, K. Xu, D. L. Xu, X. W. Yanez, J. P. Yodh, G. Yoshida, S. Zarzhitsky, P. Ziemann, J. Zierke, S. Zoll, M. CA IceCube Collaboration TI Multipole analysis of IceCube data to search for dark matter accumulated in the Galactic halo SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID COSMIC-RAYS; ANISOTROPY; CONSTRAINTS; PERFORMANCE; PARTICLES; ENERGIES; DESIGN; SYSTEM; LIMITS; MODEL AB Dark matter which is bound in the Galactic halo might self-annihilate and produce a flux of stable final state particles, e. g. high energy neutrinos. These neutrinos can be detected with IceCube, a cubic-kilometer sized Cherenkov detector. Given IceCube's large field of view, a characteristic anisotropy of the additional neutrino flux is expected. In this paper we describe a multipole method to search for such a large-scale anisotropy in IceCube data. This method uses the expansion coefficients of a multipole expansion of neutrino arrival directions and incorporates signal-specific weights for each expansion coefficient. We apply the technique to a high-purity muon neutrino sample from the Northern Hemisphere. The final result is compatible with the null-hypothesis. As no signal was observed, we present limits on the self-annihilation cross-section averaged over the relative velocity distribution down to 1.9x10(-23) cm(3) s(-1) for a dark matter particle mass of 700-1,000 GeV and direct annihilation into nu(nu) over bar. The resulting exclusion limits come close to exclusion limits from gamma-ray experiments, that focus on the outer Galactic halo, for high dark matter masses of a few TeV and hard annihilation channels. C1 [Auffenberg, J.; Bissok, M.; Blumenthal, J.; Gier, D.; Gretskov, P.; Haack, C.; Hallen, P.; Heinen, D.; Hellwig, D.; Jagielski, K.; Koob, A.; Kriesten, A.; Krings, K.; Leuermann, M.; Paul, L.; Penek, Oe.; Puetz, J.; Raedel, L.; Reimann, R.; Rongen, M.; Schoenen, S.; Schukraft, A.; Vehring, M.; Wallraff, M.; Wichary, C.; Wiebusch, C. 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EM reimann@physik.rwth-aachen.de RI Maruyama, Reina/A-1064-2013; Koskinen, David/G-3236-2014; Aguilar Sanchez, Juan Antonio/H-4467-2015; Tjus, Julia/G-8145-2012; Sarkar, Subir/G-5978-2011; Beatty, James/D-9310-2011; Wiebusch, Christopher/G-6490-2012; Taavola, Henric/B-4497-2011 OI Maruyama, Reina/0000-0003-2794-512X; Koskinen, David/0000-0002-0514-5917; Aguilar Sanchez, Juan Antonio/0000-0003-2252-9514; Schukraft, Anne/0000-0002-9112-5479; Larsen, Dag Toppe/0000-0002-9898-2174; Groh, John/0000-0001-9880-3634; Sarkar, Subir/0000-0002-3542-858X; Beatty, James/0000-0003-0481-4952; Wiebusch, Christopher/0000-0002-6418-3008; Rott, Carsten/0000-0002-6958-6033; Ter-Antonyan, Samvel/0000-0002-5788-1369; Taavola, Henric/0000-0002-2604-2810 FU US National Science Foundation-Office of Polar Programs; US National Science Foundation-Physics Division; University of Wisconsin Alumni Research Foundation; Grid Laboratory of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin-Madison; Open Science Grid (OSG) grid infrastructure; US Department of Energy; National Energy Research Scientific Computing Center, the Louisiana Optical Network Initiative (LONI); Natural Sciences and Engineering Research Council of Canada; West-Grid and Compute/Calcul Canada; Swedish Research Council; Swedish Polar Research Secretariat; Swedish National Infrastructure for Computing (SNIC); Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF); Deutsche Forschungsgemeinschaft (DFG); Helmholtz Alliance for Astroparticle Physics (HAP); Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO); FWO Odysseus programme; Flanders Institute to encourage scientific and technological research in industry (IWT), Belgian Federal Science Policy Office (Belspo); University of Oxford, UK; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); Swiss National Science Foundation (SNSF), Switzerland; National Research Foundation of Korea (NRF); Danish National Research Foundation, Denmark (DNRF) FX We acknowledge the support from the following agencies: US National Science Foundation-Office of Polar Programs, US National Science Foundation-Physics Division, University of Wisconsin Alumni Research Foundation, the Grid Laboratory of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin-Madison, the Open Science Grid (OSG) grid infrastructure; US Department of Energy, and National Energy Research Scientific Computing Center, the Louisiana Optical Network Initiative (LONI) grid computing resources; Natural Sciences and Engineering Research Council of Canada, West-Grid and Compute/Calcul Canada; Swedish Research Council, Swedish Polar Research Secretariat, Swedish National Infrastructure for Computing (SNIC), and Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF), Deutsche Forschungsgemeinschaft (DFG), Helmholtz Alliance for Astroparticle Physics (HAP), Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO), FWO Odysseus programme, Flanders Institute to encourage scientific and technological research in industry (IWT), Belgian Federal Science Policy Office (Belspo); University of Oxford, UK; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); the Swiss National Science Foundation (SNSF), Switzerland; National Research Foundation of Korea (NRF); Danish National Research Foundation, Denmark (DNRF) NR 54 TC 10 Z9 10 U1 0 U2 6 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. 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Medvedeva, T. Mooney, M. Olsen, J. Piroue, P. Quan, X. Saka, H. Stickland, D. Tully, C. Werner, J. S. Zenz, S. C. Zuranski, A. Brownson, E. Mendez, H. Vargas, J. E. Ramirez Barnes, V. E. Benedetti, D. Bolla, G. Bortoletto, D. De Mattia, M. Hu, Z. Jha, M. K. Jones, M. Jung, K. Kress, M. Leonardo, N. Pegna, D. Lopes Maroussov, V. Merkel, P. Miller, D. H. Neumeister, N. Radburn-Smith, B. C. Shi, X. Shipsey, I. Silvers, D. Svyatkovskiy, A. Wang, F. Xie, W. Xu, L. Yoo, H. D. Zablocki, J. Zheng, Y. Parashar, N. Stupak, J. Adair, A. Akgun, B. Ecklund, K. M. Geurts, F. J. M. Li, W. Michlin, B. Padley, B. P. Redjimi, R. Roberts, J. Zabel, J. Betchart, B. Bodek, A. Covarelli, R. De Barbaro, P. Demina, R. Eshaq, Y. Ferbel, T. Garcia-Bellido, A. Goldenzweig, P. Han, J. Harel, A. Khukhunaishvili, A. Petrillo, G. Vishnevskiy, D. Ciesielski, R. Demortier, L. Goulianos, K. Lungu, G. Mesropian, C. Arora, S. Barker, A. Chou, J. P. Contreras-Campana, C. Contreras-Campana, E. Duggan, D. Ferencek, D. Gershtein, Y. Gray, R. Halkiadakis, E. Hidas, D. Kaplan, S. Lath, A. Panwalkar, S. Park, M. Patel, R. Salur, S. Schnetzer, S. Somalwar, S. Stone, R. Thomas, S. Thomassen, P. Walker, M. Rose, K. Spanier, S. York, A. Bouhali, O. Hernandez, A. Castaneda Eusebi, R. Flanagan, W. Gilmore, J. Kamon, T. Khotilovich, V. Krutelyov, V. Montalvo, R. Osipenkov, I. Pakhotin, Y. Perloff, A. Rose, A. Safonov, A. Sakuma, T. Suarez, I. Tatarinov, A. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kovitanggoon, K. Kunori, S. Lee, S. W. Libeiro, T. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Johns, W. Maguire, C. Mao, Y. Melo, A. Sharma, M. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Arenton, M. W. Boutle, S. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Wood, J. Clarke, C. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Sturdy, J. Belknap, D. A. Carlsmith, D. Cepeda, M. Dasu, S. Dodd, L. Duric, S. Friis, E. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Lanaro, A. Lazaridis, C. Levine, A. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Sarangi, T. Savin, A. Smith, W. H. Vuosalo, C. Woods, N. CA CMS Collaboration TI Search for long-lived neutral particles decaying to quark-antiquark pairs in proton-proton collisions at root s=8 TeV SO PHYSICAL REVIEW D LA English DT Article ID DISPLACED VERTICES AB A search is performed for long-lived massive neutral particles decaying to quark-antiquark pairs. The experimental signature is a distinctive topology of a pair of jets, originating at a secondary vertex. Events were collected with the CMS detector at the CERN LHC in proton-proton collisions at a center-of-mass energy of 8 TeV. The data analyzed correspond to an integrated luminosity of 18.5 fb(-1). No significant excess is observed above standard model expectations. Upper limits at 95% confidence level are set on the production cross section of a heavy neutral scalar particle, H, in the mass range of 200 to 1000 GeV, decaying promptly into a pair of long-lived neutral X particles in the mass range of 50 to 350 GeV, each in turn decaying into a quark-antiquark pair. For X with mean proper decay lengths of 0.4 to 200 cm, the upper limits are typically 0.5-200 fb. The results are also interpreted in the context of an R-parity-violating supersymmetric model with long-lived neutralinos decaying into a quark-antiquark pair and a muon. For pair production of squarks that promptly decay to neutralinos with mean proper decay lengths of 2-40 cm, the upper limits on the cross section are typically 0.5-3 fb. The above limits are the most stringent on these channels to date. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. 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R.; Walsh, R.; Wissing, C.] Deutsch Elekt Synchrotron, Hamburg, Germany. [Martin, M. Aldaya; Blobel, V.; Vignali, M. Centis; Draeger, A. R.; Erfle, J.; Garutti, E.; Goebel, K.; Goerner, M.; Haller, J.; Hoffmann, M.; Hoeing, R. S.; Kirschenmann, H.; Klanner, R.; Kogler, R.; Lange, J.; Lapsien, T.; Lenz, T.; Marchesini, I.; Ott, J.; Peiffer, T.; Pietsch, N.; Poehlsen, J.; Poehlsen, T.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Seidel, M.; Sola, V.; Stadie, H.; Steinbrueck, G.; Troendle, D.; Usai, E.; Vanelderen, L.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Frensch, F.; Giffels, M.; Hartmann, F.; Hauth, T.; Husemann, U.; Katkov, I.; Kornmayer, A.; Kuznetsova, E.; Pardo, P. Lobelle; Mozer, M. U.; Mueller, Th.; Nuernberg, A.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Roecker, S.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Wolf, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Ochesanu, S.; Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.; Aslanoglou, X.] Univ Athens, Athens, Greece. [Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, H-4012 Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, M.; Mittal, M.; Nishu, N.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Sharma, V.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Jain, Sa.; Jain, Sh.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Kailas, S.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Mumbai 400085, Maharashtra, India. [Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res, Mumbai 400005, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Verwilligen, P.; Zito, G.] INFN Sez Bari, Politecn Bari, Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Nuzzo, S.; Pompili, A.; Singh, G.; Venditti, R.] Univ Bari, Politecn Bari, Bari, Italy. [Creanza, D.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.; Radogna, R.] Politecn Bari, Bari, Italy. [Aleksandrov, A.; Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] INFN Sez Bologna, Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] INFN Sez Catania, CSFNSM, Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, CSFNSM, Catania, Italy. [Giordano, F.] CSFNSM, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] INFN Sez Firenze, Florence, Italy. [Civinini, C.; D'Alessandro, R.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] INFN Lab Nazl Frascati, Frascati, Italy. [Ferro, F.; Lo Vetere, M.; Robutti, E.; Tosi, S.] INFN Sez Genova, Genoa, Italy. [Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] INFN Sez Milano Bicocca, Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] INFN Sez Napoli, Naples, Italy. [Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Dosselli, U.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Gozzelino, A.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pegoraro, M.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Triossi, A.; Zotto, P.; Zucchetta, A.] INFN Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Dall'Osso, M.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.] Univ Padua, Padua, Italy. Univ Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Salvini, P.; Vitulo, P.] INFN Sez Pavia, Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] INFN Sez Perugia, Perugia, Italy. [Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] INFN Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Grassi, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Soffi, L.; Traczyk, P.] INFN Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Univ Roma, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Ortona, G.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] INFN Sez Torino, Turin, Italy. [Amapane, N.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Finco, L.; Migliore, E.; Monaco, V.; Ortona, G.; Pacher, L.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Argiro, S.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara Torino, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.; Zanetti, A.] INFN Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Diblen, S. Salva; Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, T. J.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Kim, J. Y.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, I. C.; Park, S.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Aleksandrov, A.; Choi, Y.; Choi, Y. K.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Komaragiri, J. R.; Ali, M. A. B. Md] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Wolszczak, W.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Hassan, Q.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Shah, M. A.; Shoaib, M.; Bargassa, P.; Da Cruz E Silva, C. Beirao; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Savina, M.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Zhokin, A.; Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Milosevic, J.; Rekovic, V.; Maestre, J. Alcaraz] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Milosevic, J.; Rekovic, V.; Maestre, J. Alcaraz] Vinca Inst Nucl Sci, Belgrade, Serbia. [Battilana, C.; Calvo, E.; Cerrada, M.; Llatas, M. Chamizo; Colino, N.; De la Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernndez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] CIEMAT, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, IFCA, E-39005 Santander, Spain. [Aleksandrov, A.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Dobson, M.; Dordevic, M.; Dorney, B.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Loureno, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Marrouche, J.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Musella, P.; Orsini, L.; Pape, L.; Perez, E.; Perrozzi, L.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Pimia, M.; Piparo, D.; Plagge, M.; Racz, A.; Rolandi, G.; Rovere, M.; Sakulin, H.; Schafer, C.; Schwick, C.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Treille, D.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Wardle, N.; Whri, H. K.; Wollny, H.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Hits, D.; Lustermann, W.; Mangano, B.; Marini, A. C.; Del Arbol, P. Martinez Ruiz; Meister, D.; Mohr, N.; Naegeli, C.; Nessi-Tedaldi, F.; Pandolfi, F.; Pauss, F.; Peruzzi, M.; Quittnat, M.; Rebane, L.; Rossini, M.; Starodumov, A.; Takahashi, M.; Theofilatos, K.; Wallny, R.; Weber, H. A.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Mejias, B. Millan; Ngadiuba, J.; Robmann, P.; Ronga, F. J.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli, Taiwan. [Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Kao, K. Y.; Lei, Y. J.; Liu, Y. F.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Tzeng, Y. M.; Wilken, R.] NTU, Taipei, Taiwan. [Asavapibhop, B.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Gamsizkan, H.; Karapinar, G.; Ocalan, K.; Sekmen, S.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Guelmez, E.; Isildak, B.; Kaya, M.; Kaya, O.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yuecel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Phys & Technol Inst, Natl Sci Ctr, UA-310108 Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.; Cheng, T.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Dunne, P.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Hall, G.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Mathias, B.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Lawson, P.; Richardson, C.; Rohlf, J.; Sperka, D.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Miceli, T.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Rikova, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Liu, H.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Negrete, M. Olmedo; Shrinivas, A.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Evans, D.; Holzner, A.; Kelley, R.; Klein, D.; Lebourgeois, M.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Welke, C.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Aleksandrov, A.; Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Incandela, J.; Justus, C.; Mccoll, N.; Richman, J.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Skinnari, L.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.; Winn, D.] Cornell Univ, Ithaca, NY USA. [Abdullin, S.] Fairfield Univ, Fairfield, CT 06430 USA. [Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kreis, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Sharma, S.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Yang, F.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Carver, M.; Cheng, T.; Curry, D.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Field, R. D.; Fisher, M.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Turner, P.; Varelas, N.] UIC, Chicago, IL USA. [Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Haytmyradov, M.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Gray, J.; Iii, R. P. Kenny; Malek, M.; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Skhirtladze, N.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Belloni, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Pearson, T.; Planer, M.; Ruchti, R.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hebda, P.; Hunt, A.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Barnes, V. E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Hu, Z.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, IN USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; De Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Khukhunaishvili, A.; Petrillo, G.; Vishnevskiy, D.] Univ Rochester, Rochester, NY USA. [Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Kaplan, S.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Salur, S.; Schnetzer, S.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Hernandez, A. Castaneda; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Krutelyov, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Rose, A.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kovitanggoon, K.; Kunori, S.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Dodd, L.; Duric, S.; Friis, E.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Lazaridis, C.; Levine, A.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. H.; Vuosalo, C.; Woods, N.] Univ Wisconsin, Madison, WI USA. [Fabjan, C.; Fruhwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. Suez Univ, Suez, Egypt. [Elgammal, S.] British Univ Egypt, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Radi, A.] Ain Shams Univ, Cairo, Egypt. [Radi, A.] Sultan Qaboos Univ, Muscat, Oman. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Bergholz, M.; Lohmann, W.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Vesztergombi, G.] Eotvos Lorand Univ, Budapest, Hungary. [Bhowmik, S.; Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Sharif Univ Technol, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.; Squillacioti, P.] Univ Siena, I-53100 Siena, Italy. [Moon, C. S.; Mermerkaya, H.] CNRS, IN2P3, Paris, France. [Savoy-Navarro, A.] Purdue Univ, W Lafayette, IN 47907 USA. [Heredia-de La Cruz, I.] Univ Michoacana, Morelia, Michoacan, Mexico. [Matveev, V.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Dubinin, M.] CALTECH, Pasadena, CA 91125 USA. [Adzic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. Ist Nazl Fis Nucl, Scuola Normale & Sez, Pisa, Italy. Univ Athens, Athens, Greece. Adiyaman Univ, Adiyaman, Turkey. Cag Univ, Mersin, Turkey. Mersin Univ, Mersin, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Bahtiyar, H.; Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Newbold, D. M.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. Erzincan Univ, Erzincan, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. [Kamon, T.] Kyungpook Natl Univ, Taegu, South Korea. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Paulini, Manfred/N-7794-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Menasce, Dario Livio/A-2168-2016; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Rolandi, Luigi (Gigi)/E-8563-2013; Sguazzoni, Giacomo/J-4620-2015; Ligabue, Franco/F-3432-2014; Calvo Alamillo, Enrique/L-1203-2014; Flix, Josep/G-5414-2012; Cerrada, Marcos/J-6934-2014; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Della Ricca, Giuseppe/B-6826-2013; Chinellato, Jose Augusto/I-7972-2012; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Kirakosyan, Martin/N-2701-2015; Tinoco Mendes, Andre David/D-4314-2011; Seixas, Joao/F-5441-2013; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; Matorras, Francisco/I-4983-2015; TUVE', Cristina/P-3933-2015; Dudko, Lev/D-7127-2012; KIM, Tae Jeong/P-7848-2015; Paganoni, Marco/A-4235-2016; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Trocsanyi, Zoltan/A-5598-2009; Cavallo, Nicola/F-8913-2012; candelise, vieri/H-2195-2015; Montanari, Alessandro/J-2420-2012; Hernandez Calama, Jose Maria/H-9127-2015; ciocci, maria agnese /I-2153-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Benussi, Luigi/O-9684-2014; Lo Vetere, Maurizio/J-5049-2012; Ragazzi, Stefano/D-2463-2009; Grandi, Claudio/B-5654-2015; Manganote, Edmilson/K-8251-2013; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Calderon, Alicia/K-3658-2014; VARDARLI, Fuat Ilkehan/B-6360-2013; Lokhtin, Igor/D-7004-2012; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Petrushanko, Sergey/D-6880-2012; Wulz, Claudia-Elisabeth/H-5657-2011 OI Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Androsov, Konstantin/0000-0003-2694-6542; Fiorendi, Sara/0000-0003-3273-9419; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Heath, Helen/0000-0001-6576-9740; Giubilato, Piero/0000-0003-4358-5355; Gallinaro, Michele/0000-0003-1261-2277; Tabarelli de Fatis, Tommaso/0000-0001-6262-4685; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Levchenko, Petr/0000-0003-4913-0538; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Gerosa, Raffaele/0000-0001-8359-3734; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Sogut, Kenan/0000-0002-9682-2855; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Sguazzoni, Giacomo/0000-0002-0791-3350; da Cruz e silva, Cristovao/0000-0002-1231-3819; Casarsa, Massimo/0000-0002-1353-8964; Ligabue, Franco/0000-0002-1549-7107; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Calvo Alamillo, Enrique/0000-0002-1100-2963; Flix, Josep/0000-0003-2688-8047; Cerrada, Marcos/0000-0003-0112-1691; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Della Ricca, Giuseppe/0000-0003-2831-6982; Chinellato, Jose Augusto/0000-0002-3240-6270; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Tinoco Mendes, Andre David/0000-0001-5854-7699; Seixas, Joao/0000-0002-7531-0842; Rovelli, Tiziano/0000-0002-9746-4842; Matorras, Francisco/0000-0003-4295-5668; TUVE', Cristina/0000-0003-0739-3153; Dudko, Lev/0000-0002-4462-3192; KIM, Tae Jeong/0000-0001-8336-2434; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Trocsanyi, Zoltan/0000-0002-2129-1279; Montanari, Alessandro/0000-0003-2748-6373; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Benussi, Luigi/0000-0002-2363-8889; Lo Vetere, Maurizio/0000-0002-6520-4480; Ragazzi, Stefano/0000-0001-8219-2074; Grandi, Claudio/0000-0001-5998-3070; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812 FU BMWFW; FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq; CAPES; FAPERJ; FAPESP (Brazil) FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/ IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP and NRF (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (USA). Individuals have received support from the MarieCurie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie doorWetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF; and the National Priorities Research Program by Qatar National Research Fund. NR 38 TC 15 Z9 15 U1 8 U2 59 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JAN 20 PY 2015 VL 91 IS 1 DI 10.1103/PhysRevD.91.012007 PG 21 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AZ6KO UT WOS:000348329000001 ER PT J AU Koh, CY Schaff, UY Piccini, ME Stanker, LH Cheng, LW Ravichandran, E Singh, BR Sommer, GJ Singh, AK AF Koh, Chung-Yan Schaff, Ulrich Y. Piccini, Matthew E. Stanker, Larry H. Cheng, Luisa W. Ravichandran, Easwaran Singh, Bal-Ram Sommer, Greg J. Singh, Anup K. TI Centrifugal Microfluidic Platform for Ultrasensitive Detection of Botulinum Toxin SO ANALYTICAL CHEMISTRY LA English DT Article ID SINGLE-DOMAIN ANTIBODIES; CLOSTRIDIUM-BOTULINUM; QUANTITATIVE DETECTION; BIOLOGICAL SAMPLES; ORAL TOXICITIES; A NEUROTOXIN; ASSAY; FOOD; PCR; CONFIRMATION AB We present an innovative centrifugal microfluidic immunoassay platform (SpinDx) to address the urgent biodefense and public health need for ultrasensitive point-of-care/incident detection of botulinum toxin. The simple, sample-to-answer centrifugal microfluidic immunoassay approach is based on binding of toxins to antibody-laden capture particles followed by sedimentation of the particles through a density-media in a microfluidic disk and quantification by laser-induced fluorescence. A blind, head-to-head comparison study of SpinDx versus the gold-standard mouse bioassay demonstrates 100-fold improvement in sensitivity (limit of detection = 0.09 pg/mL), while achieving total sample-to-answer time of <30 min with 2-mu L required volume of the unprocessed sample. We further demonstrate quantification of botulinum toxin in both exogeneous (human blood and serum spiked with toxins) and endogeneous (serum from mice intoxicated via oral, intranasal, and intravenous routes) samples. SpinDx can analyze, without any sample preparation, multiple sample types including whole blood, serum, and food. It is readily expandable to additional analytes as the assay reagents (i.e., the capture beads and detection antibodies) are disconnected from the disk architecture and the reader, facilitating rapid development of new assays. SpinDx can also serve as a general-purpose immunoassay platform applicable to diagnosis of other conditions and diseases. C1 [Koh, Chung-Yan; Schaff, Ulrich Y.; Piccini, Matthew E.; Sommer, Greg J.; Singh, Anup K.] Sandia Natl Labs, Livermore, CA 94551 USA. [Stanker, Larry H.; Cheng, Luisa W.] USDA ARS, Western Reg Res Ctr, Foodborne Contaminants Res Unit, Albany, CA 94710 USA. [Ravichandran, Easwaran; Singh, Bal-Ram] Univ Massachusetts Dartmouth, N Dartmouth, MA 02747 USA. RP Koh, CY (reprint author), Sandia Natl Labs, 7011 East Ave, Livermore, CA 94551 USA. EM ckoh@sandia.gov; aksingh@sandia.gov RI Ravichandran, Easwaran/N-7239-2016 OI Ravichandran, Easwaran/0000-0003-1613-0339 FU National Institute of Allergies and Infectious Disease (NIAID) [U01A1075441, R01AI098853]; United States Department of Agriculture, Agricultural Research Service, National Program project [NP108]; CRIS [5325-42000-043-00D]; National Institute of Allergy and Infectious Diseases Service [U54 AI065359]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000 - SAND2014-20313J] FX This work was funded by the National Institute of Allergies and Infectious Disease (NIAID) Grants U01A1075441 and R01AI098853. L.W.C. and L.H.S. were funded by the United States Department of Agriculture, Agricultural Research Service, National Program project NP108, CRIS 5325-42000-043-00D and the National Institute of Allergy and Infectious Diseases Service Grant U54 AI065359. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000 - SAND2014-20313J. NR 49 TC 10 Z9 10 U1 12 U2 49 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD JAN 20 PY 2015 VL 87 IS 2 BP 922 EP 928 DI 10.1021/ac504054u PG 7 WC Chemistry, Analytical SC Chemistry GA AZ6LX UT WOS:000348332300015 PM 25521812 ER PT J AU Shi, TJ Gao, YQ Gaffrey, MJ Nicora, CD Fillmore, TL Chrisler, WB Gritsenko, MA Wu, CC He, JT Bloodsworth, KJ Zhao, R Camp, DG Liu, T Rodland, KD Smith, RD Wiley, HS Qian, WJ AF Shi, Tujin Gao, Yuqian Gaffrey, Matthew J. Nicora, Carrie D. Fillmore, Thomas L. Chrisler, William B. Gritsenko, Marina A. Wu, Chaochao He, Jintang Bloodsworth, Kent J. Zhao, Rui Camp, David G., II Liu, Tao Rodland, Karin D. Smith, Richard D. Wiley, H. Steven Qian, Wei-Jun TI Sensitive Targeted Quantification of ERK Phosphorylation Dynamics and Stoichiometry in Human Cells without Affinity Enrichment SO ANALYTICAL CHEMISTRY LA English DT Article ID EPIDERMAL-GROWTH-FACTOR; ACTIVATED PROTEIN-KINASE; MASS-SPECTROMETRY; FACTOR RECEPTOR; MAP KINASE; QUANTITATIVE PROTEOMICS; DUAL PHOSPHORYLATION; SIGNALING NETWORKS; ANTIBODY-FREE; SITES AB Targeted mass spectrometry is a promising technology for site-specific quantification of posttranslational modifications. However, a major constraint is the limited sensitivity for quantifying low-abundance PTMs, requiring the use of affinity reagents for enrichment. Herein, we demonstrate the direct site-specific quantification of ERK phosphorylation isoforms (pT, pY, pTpY) and their relative stoichiometry using a sensitive targeted MS approach termed high-pressure, high-resolution separations with intelligent selection, and multiplexing (PRISM). PRISM provides effective enrichment of target peptides into a given fraction from complex mixture, followed by selected reaction monitoring quantification. Direct quantification of ERK phosphorylation in human mammary epithelial cells (HMEC) was demonstrated from as little as 25 mu g tryptic peptides from whole cell lysates. Compared to immobilized metal-ion affinity chromatography, PRISM provided similar to 10-fold higher signal intensities, presumably due to the better peptide recovery of PRISM. This approach was applied to quantify ERK phosphorylation dynamics in HMEC treated by different doses of epidermal growth factor at both the peak activation (10 min) and steady state (2 h). The maximal ERK activation was observed with 0.3 and 3 ng/mL doses for 10 min and 2 h time points, respectively. The doseresponse profiles of individual phosphorylated isoforms showed that singly phosphorylated pT-ERK never increases significantly, while the increase of pY-ERK paralleled that of pTpY-ERK. This data supports for a processive, rather than distributed model of ERK phosphorylation. The PRISM-SRM quantification of protein phosphorylation illustrates the potential for simultaneous quantification of multiple PTMs. C1 [Shi, Tujin; Gao, Yuqian; Gaffrey, Matthew J.; Nicora, Carrie D.; Chrisler, William B.; Gritsenko, Marina A.; Wu, Chaochao; He, Jintang; Bloodsworth, Kent J.; Camp, David G., II; Liu, Tao; Rodland, Karin D.; Smith, Richard D.; Qian, Wei-Jun] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99354 USA. [Fillmore, Thomas L.; Zhao, Rui; Wiley, H. Steven] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA. RP Wiley, HS (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA. EM steven.wiley@pnnl.gov; weijun.qian@pnnl.gov RI Smith, Richard/J-3664-2012; OI Smith, Richard/0000-0002-2381-2349; Wiley, Steven/0000-0003-0232-6867 FU NIH [DP2OD006668, P41GM103493, U24-CA-16001901]; DOE [DE-AC05-76RL0 1830] FX Portions of the research were supported by NIH Grants DP2OD006668, P41GM103493, and U24-CA-16001901. The experimental work described herein was performed in the Environmental Molecular Sciences Laboratory, Pacific Northwest National Laboratory, a national scientific user facility sponsored by the DOE under Contract DE-AC05-76RL0 1830. NR 44 TC 6 Z9 6 U1 5 U2 22 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD JAN 20 PY 2015 VL 87 IS 2 BP 1103 EP 1110 DI 10.1021/ac503797x PG 8 WC Chemistry, Analytical SC Chemistry GA AZ6LX UT WOS:000348332300039 PM 25517423 ER PT J AU Adamski, CJ Cardenas, AM Brown, NG Horton, LB Sankaran, B Prasad, BVV Gilbert, HF Palzkill, T AF Adamski, Carolyn J. Cardenas, Ana Maria Brown, Nicholas G. Horton, Lori B. Sankaran, Banumathi Prasad, B. V. Venkataram Gilbert, Hiram F. Palzkill, Timothy TI Molecular Basis for the Catalytic Specificity of the CTX-M Extended-Spectrum beta-Lactamases SO BIOCHEMISTRY LA English DT Article ID ANTIBIOTIC-RESISTANCE; ANGSTROM RESOLUTION; CRYSTAL-STRUCTURE; M ENZYMES; HYDROLYSIS; INTERFACE; STABILITY; EVOLUTION; EXPANSION; INSIGHTS AB Extended-spectrum beta-lactamases (ESBLs) pose a threat to public health because of their ability to confer resistance to extended-spectrum cephalosporins such as cefotaxime. The CTX-M beta-lactamases are the most widespread ESBL enzymes among antibiotic resistant bacteria. Many of the active site residues are conserved between the CTX-M family and non-ESBL beta-lactamases such as TEM-1, but the residues Ser237 and Arg276 are specific to the CTX-M family, suggesting that they may help to define the increased specificity for cefotaxime hydrolysis. To test this hypothesis, site-directed mutagenesis of these positions was performed in the CTX-M-14 beta-lactamase. Substitutions of Ser237 and Arg276 with their TEM-1 counterparts, Ala237 and Asn276, had a modest effect on cefotaxime hydrolysis, as did removal of the Arg276 side chain in an R276A mutant. The S237A:R276N and S237A:R276A double mutants, however, exhibited 29- and 14-fold losses in catalytic efficiency for cefotaxime hydrolysis, respectively, while the catalytic efficiency for benzylpenicillin hydrolysis was unchanged. Therefore, together, the Ser237 and Arg276 residues are important contributors to the cefotaximase substrate profile of the enzyme. High-resolution crystal structures of the CTX-M-14 S70G, S70G:S237A, and S70G:S237A:R276A variants alone and in complex with cefotaxime show that residues Ser237 and Arg276 in the wild-type enzyme promote the expansion of the active site to accommodate cefotaxime and favor a conformation of cefotaxime that allows optimal contacts between the enzyme and substrate. The conservation of these residues, linked to their effects on structure and catalysis, imply that their coevolution is an important specificity determinant in the CTX-M family. C1 [Adamski, Carolyn J.; Brown, Nicholas G.; Prasad, B. V. Venkataram; Gilbert, Hiram F.; Palzkill, Timothy] Baylor Coll Med, Verna & Marrs McLean Dept Biochem & Mol Biol, Houston, TX 77030 USA. [Cardenas, Ana Maria; Horton, Lori B.; Prasad, B. V. Venkataram; Palzkill, Timothy] Baylor Coll Med, Dept Mol Virol & Microbiol, Houston, TX 77030 USA. [Palzkill, Timothy] Baylor Coll Med, Dept Pharmacol, Houston, TX 77030 USA. [Sankaran, Banumathi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley Ctr Struct Biol, Berkeley, CA 94720 USA. RP Palzkill, T (reprint author), Baylor Coll Med, Verna & Marrs McLean Dept Biochem & Mol Biol, One Baylor Plaza, Houston, TX 77030 USA. EM timothyp@bcm.tmc.edu FU Houston Area Molecular Biophysics Training Program (NIGMS) of the Gulf Coast Consortia [T32 GM008280]; Keck Center of Biomedical Discovery Training Program of the Gulf Coast Consortia (NIH) [1 R90 DA023418-03]; Keck Center of Pharmacoinformatics Training Program of the Gulf Coast Consortia (NIH) [T90 DK070109-05]; NIH [AI32956]; Robert Welch Foundation [Q1279]; Berkeley Center for Structural Biology; National Institutes of Health, National Institute of General Medical Sciences; Howard Hughes Medical Institute; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by a training fellowship from the Houston Area Molecular Biophysics Training Program (NIGMS grant no. T32 GM008280) of the Gulf Coast Consortia to C.J.A., a training fellowship from the Keck Center of Biomedical Discovery Training Program of the Gulf Coast Consortia (NIH grant no. 1 R90 DA023418-03) to A.M.C., and a training fellowship from the Keck Center of Pharmacoinformatics Training Program of the Gulf Coast Consortia (NIH grant no. T90 DK070109-05) to N.G.B. This work was supported by NIH grant no. AI32956 to T.P. B.V.V.P. acknowledges support from Robert Welch Foundation (Q1279). This work was supported by The Berkeley Center for Structural Biology, supported in part by the National Institutes of Health, National Institute of General Medical Sciences, and the Howard Hughes Medical Institute. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. NR 31 TC 6 Z9 6 U1 0 U2 7 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD JAN 20 PY 2015 VL 54 IS 2 BP 447 EP 457 DI 10.1021/bi501195g PG 11 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA AZ6MH UT WOS:000348333300033 PM 25489790 ER PT J AU Korte, HL Saini, A Trotter, VV Butland, GP Arkin, AP Wall, JD AF Korte, Hannah L. Saini, Avneesh Trotter, Valentine V. Butland, Gareth P. Arkin, Adam P. Wall, Judy D. TI Independence of Nitrate and Nitrite Inhibition of Desulfovibrio vulgaris Hildenborough and Use of Nitrite as a Substrate for Growth SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID SULFATE-REDUCING BACTERIA; SULFIDE-OXIDIZING BACTERIA; GENE-EXPRESSION ANALYSIS; ELECTRON FLOW; OIL-FIELD; REDUCTASE; BINDING; DEHYDROGENASE; BIOREACTOR; INJECTION AB Sulfate-reducing microbes, such as Desulfovibrio vulgaris Hildenborough, cause souring of petroleum reservoirs through produced sulfide and precipitate heavy metals, either as sulfides or by alteration of the metal reduction state. Thus, inhibitors of these microbes, including nitrate and nitrite ions, are studied in order to limit their impact. Nitrite is a potent inhibitor of sulfate reducers, and it has been suggested that nitrate does not inhibit these microbes directly but by reduction to nitrite, which serves as the ultimate inhibitor. Here we provide evidence that nitrate inhibition of D. vulgaris can be independent of nitrite production. We also show that D. vulgaris can use nitrite as a nitrogen source or terminal electron acceptor for growth. Moreover, we report that use of nitrite as a terminal electron acceptor requires nitrite reductase (nrfA) as a D. vulgaris nrfA mutant cannot respire nitrite but remains capable of utilizing nitrite as a nitrogen source. These results illuminate previously uncharacterized metabolic abilities of D. vulgaris that may allow niche expansion in low-sulfate environments. Understanding these abilities may lead to better control of sulfate-reducing bacteria in industrial settings and more accurate prediction of their interactions in the environment. C1 [Korte, Hannah L.; Wall, Judy D.] Univ Missouri, Dept Biochem, Columbia, MO 65211 USA. [Korte, Hannah L.; Saini, Avneesh; Trotter, Valentine V.; Butland, Gareth P.; Arkin, Adam P.; Wall, Judy D.] Ecosyst & Networks Integrated Genes & Mol Assembl, Berkeley, CA 94720 USA. [Saini, Avneesh; Trotter, Valentine V.; Butland, Gareth P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Arkin, Adam P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Wall, JD (reprint author), Univ Missouri, Dept Biochem, Columbia, MO 65211 USA. EM wallj@missouri.edu RI Arkin, Adam/A-6751-2008; OI Arkin, Adam/0000-0002-4999-2931; Trotter, Valentine/0000-0002-1784-9487 FU U.S. Department of Energy, Office of Science, Office of Biological & Environmental Research [DE-AC02-05CH11231] FX This material by ENIGMA - Ecosystems and Networks Integrated with Genes and Molecular Assemblies (http://enigma.lbl.gov), a Scientific Focus Area Program at Lawrence Berkeley National Laboratory is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Biological & Environmental Research under contract number DE-AC02-05CH11231. We thank Paul D. Adams, LBNL SFA Laboratory Research Manager for ENIGMA, for his leadership and guidance. NR 45 TC 4 Z9 4 U1 3 U2 31 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JAN 20 PY 2015 VL 49 IS 2 BP 924 EP 931 DI 10.1021/es504484m PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AZ6LY UT WOS:000348332400029 PM 25534748 ER PT J AU Azzolina, NA Small, MJ Nakles, DV Glazewski, KA Peck, WD Gorecki, CD Bromhal, GS Dilmore, RM AF Azzolina, Nicholas A. Small, Mitchell J. Nakles, David V. Glazewski, Kyle A. Peck, Wesley D. Gorecki, Charles D. Bromhal, Grant S. Dilmore, Robert M. TI Quantifying the Benefit of Wellbore Leakage Potential Estimates for Prioritizing Long-Term MVA Well Sampling at a CO2 Storage Site SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID SYSTEM; BRINE AB This work uses probabilistic methods to simulate a hypothetical geologic CO2 storage site in a depleted oil and gas field, where the large number of legacy wells would make it cost-prohibitive to sample all wells for all measurements as part of the postinjection site care. Deep well leakage potential scores were assigned to the wells using a random subsample of 100 wells from a detailed study of 826 legacy wells that penetrate the basal Cambrian formation on the U.S. side of the U.S./Canadian border. Analytical solutions and Monte Carlo simulations were used to quantify the statistical power of selecting a leaking well. Power curves were developed as a function of (1) the number of leaking wells within the Area of Review; (2) the sampling design (random or judgmental, choosing first the wells with the highest deep leakage potential scores); (3) the number of wells included in the monitoring sampling plan; and (4) the relationship between a well's leakage potential score and its relative probability of leakage. Cases where the deep well leakage potential scores are fully or partially informative of the relative leakage probability are compared to a noninformative base case in which leakage is equiprobable across all wells in the Area of Review. The results show that accurate prior knowledge about the probability of well leakage adds measurable value to the ability to detect a leaking well during the monitoring program, and that the loss in detection ability due to imperfect knowledge of the leakage probability can be quantified. This work underscores the importance of a data-driven, risk-based monitoring program that incorporates uncertainty quantification into long-term monitoring sampling plans at geologic CO2 storage sites. C1 [Azzolina, Nicholas A.; Small, Mitchell J.; Nakles, David V.] Carnegie Mellon Univ, Dept Civil & Environm Engn, Pittsburgh, PA 15213 USA. [Glazewski, Kyle A.; Peck, Wesley D.; Gorecki, Charles D.] Univ N Dakota, Grand Forks, ND 58202 USA. [Bromhal, Grant S.; Dilmore, Robert M.] US Dept Energy Morgantown, Natl Energy Technol Lab, Morgantown, WV 26507 USA. RP Azzolina, NA (reprint author), Carnegie Mellon Univ, Dept Civil & Environm Engn, Pittsburgh, PA 15213 USA. EM nick.azzolina@gmail.com FU U.S. Department of Energy National Energy Technology Laboratory FX This study was funded by the U.S. Department of Energy National Energy Technology Laboratory. NR 27 TC 2 Z9 2 U1 1 U2 3 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JAN 20 PY 2015 VL 49 IS 2 BP 1215 EP 1224 DI 10.1021/es503742n PG 10 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA AZ6LY UT WOS:000348332400063 PM 25551254 ER PT J AU Myers, TL Cannon, BD Brauer, CS Hansen, SM Crowther, BG AF Myers, Tanya L. Cannon, Bret D. Brauer, Carolyn S. Hansen, Stewart M. Crowther, Blake G. TI Proton and gamma irradiation of Fabry-Perot quantum cascade lasers for space qualification SO APPLIED OPTICS LA English DT Article ID TEMPERATURE OPERATION; ROOM-TEMPERATURE; DOT LASERS; RADIATION; DIODES; DEGRADATION; DAMAGE AB Fabry-Perot quantum cascade lasers (QCLs) were characterized following irradiation by high-energy (64 MeV) protons and Cobalt-60 gamma rays. Seven QCLs were exposed to total accumulated radiation doses that varied from 20 to 46.3 krad(Si), which are typical exposure levels for electronic components in a space environment. The QCLs did not show any measurable changes in threshold current or slope efficiency suggesting the suitability of QCLs for use in space-based missions. (C) 2015 Optical Society of America C1 [Myers, Tanya L.; Cannon, Bret D.; Brauer, Carolyn S.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Hansen, Stewart M.] Space Dynam Lab, Logan, UT 84322 USA. [Crowther, Blake G.] Utah State Univ, Dept Elect & Comp Engn, Logan, UT 84322 USA. RP Myers, TL (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM tanya.myers@pnnl.gov FU U.S. Department of Energy Office of Defense Nuclear Nonproliferation Research and Development; U.S. DOE [DE-AC05-76RLO1830] FX The authors wish to thank Greg Carter and Bryan Broocks for assistance with the Cobalt-60 irradiation as well as the staff at Crocker Nuclear Laboratory at the University of California at Davis for their assistance with proton testing. We also thank the Space Dynamics Laboratory at Utah State University and the Lunar and Planetary Laboratory at the University of Arizona for allowing us to test the QCLs during their scheduled proton beam time. In addition, we thank John Bruno from Thorlabs for providing additional design details for the QCLs. The research described in this paper was supported in part by the U.S. Department of Energy Office of Defense Nuclear Nonproliferation Research and Development. PNNL is operated by Battelle for the U.S. DOE under Contract DE-AC05-76RLO1830. NR 21 TC 0 Z9 0 U1 4 U2 14 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1559-128X EI 2155-3165 J9 APPL OPTICS JI Appl. Optics PD JAN 20 PY 2015 VL 54 IS 3 BP 527 EP 534 DI 10.1364/AO.54.000527 PG 8 WC Optics SC Optics GA AZ6SI UT WOS:000348349500025 ER PT J AU Aliu, E Archer, A Aune, T Barnacka, A Behera, B Beilicke, M Benbow, W Berger, K Bird, R Buckley, JH Bugaev, V Byrum, K Cardenzana, JV Cerruti, M Chen, X Ciupik, L Connolly, MP Cui, W Dickinson, HJ Dumm, J Eisch, JD Errando, M Falcone, A Federici, S Feng, Q Finley, JP Fortin, P Fortson, L Furniss, A Galante, N Gillanders, GH Griffin, S Griffiths, ST Grube, J Gyuk, G Hakansson, N Hanna, D Holder, J Hughes, G Humensky, TB Johnson, CA Kaaret, P Kar, P Kertzman, M Khassen, Y Kieda, D Krawczynski, H Krennrich, F Kumar, S Lang, MJ Madhavan, A McArthur, S McCann, A Meagher, K Millis, J Moriarty, P Nieto, D de Bhroithe, AO Ong, RA Orr, M Otte, AN Park, N Perkins, JS Pohl, M Popkow, A Prokoph, H Pueschel, E Quinn, J Ragan, K Rajotte, J Reyes, LC Reynolds, PT Richards, GT Roache, E Sembroski, GH Shahinyan, K Staszak, D Telezhinsky, I Tucci, JV Tyler, J Varlotta, A Vassiliev, VV Wakely, SP Weinstein, A Welsing, R Wilhelm, A Williams, DA Zitzer, B AF Aliu, E. Archer, A. Aune, T. Barnacka, A. Behera, B. Beilicke, M. Benbow, W. Berger, K. Bird, R. Buckley, J. H. Bugaev, V. Byrum, K. Cardenzana, J. V. Cerruti, M. Chen, X. Ciupik, L. Connolly, M. P. Cui, W. Dickinson, H. J. Dumm, J. Eisch, J. D. Errando, M. Falcone, A. Federici, S. Feng, Q. Finley, J. P. Fortin, P. Fortson, L. Furniss, A. Galante, N. Gillanders, G. H. Griffin, S. Griffiths, S. T. Grube, J. Gyuk, G. Hakansson, N. Hanna, D. Holder, J. Hughes, G. Humensky, T. B. Johnson, C. A. Kaaret, P. Kar, P. Kertzman, M. Khassen, Y. Kieda, D. Krawczynski, H. Krennrich, F. Kumar, S. Lang, M. J. Madhavan, A. McArthur, S. McCann, A. Meagher, K. Millis, J. Moriarty, P. Nieto, D. de Bhroithe, A. O'Faolain Ong, R. A. Orr, M. Otte, A. N. Park, N. Perkins, J. S. Pohl, M. Popkow, A. Prokoph, H. Pueschel, E. Quinn, J. Ragan, K. Rajotte, J. Reyes, L. C. Reynolds, P. T. Richards, G. T. Roache, E. Sembroski, G. H. Shahinyan, K. Staszak, D. Telezhinsky, I. Tucci, J. V. Tyler, J. Varlotta, A. Vassiliev, V. V. Wakely, S. P. Weinstein, A. Welsing, R. Wilhelm, A. Williams, D. A. Zitzer, B. TI VERITAS OBSERVATIONS OF THE BL LAC OBJECT PG 1553+113 SO ASTROPHYSICAL JOURNAL LA English DT Article DE BL Lacertae objects: general ID EXTRAGALACTIC BACKGROUND LIGHT; LACERTAE OBJECTS; GAMMA-RAYS; OPTICAL SPECTROSCOPY; BLAZARS; TELESCOPE; RADIATION; SPECTRA; PG-1553+113; MODEL AB We present results from VERITAS observations of the BL Lac object PG 1553+113 spanning the years 2010, 2011, and 2012. The time-averaged spectrum, measured between 160 and 560 GeV, is well described by a power law with a spectral index of 4.33 +/- 0.09. The time-averaged integral flux above 200 GeV measured for this period was (1.69 +/- 0.06) x 10(-11) photons cm(-2) s(-1), corresponding to 6.9% of the Crab Nebula flux. We also present the combined gamma-ray spectrum from the Fermi Large Area Telescope and VERITAS covering an energy range from 100 MeV to 560 GeV. The data are well fit by a power law with an exponential cutoff at 101.9 +/- 3.2 GeV. The origin of the cutoff could be intrinsic to PG 1553+113 or be due to the gamma-ray opacity of our universe through pair production off the extragalactic background light (EBL). Given lower limits to the redshift of z > 0.395 based on optical/UV observations of PG 1553+113, the cutoff would be dominated by EBL absorption. Conversely, the small statistical uncertainties of the VERITAS energy spectrum have allowed us to provide a robust upper limit on the redshift of PG 1553+113 of z <= 0.62. A strongly elevated mean flux of (2.50 +/- 0.14) x10(-11) photons cm(-2) s(-1) (10.3% of the Crab Nebula flux) was observed during 2012, with the daily flux reaching as high as (4.44 +/- 0.71) x10(-11) photons cm(-2) s(-1) (18.3% of the Crab Nebula flux) on MJD 56048. The light curve measured during the 2012 observing season is marginally inconsistent with a steady flux, giving a chi(2) probability for a steady flux of 0.03%. C1 [Aliu, E.; Errando, M.] Columbia Univ Barnard Coll, Dept Phys & Astron, New York, NY 10027 USA. [Archer, A.; Beilicke, M.; Buckley, J. H.; Bugaev, V.; Krawczynski, H.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Aune, T.; Ong, R. A.; Popkow, A.; Vassiliev, V. V.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Barnacka, A.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Behera, B.; Chen, X.; Federici, S.; Hughes, G.; de Bhroithe, A. O'Faolain; Pohl, M.; Prokoph, H.; Telezhinsky, I.; Welsing, R.; Wilhelm, A.] DESY, D-15738 Zeuthen, Germany. [Benbow, W.; Cerruti, M.; Fortin, P.; Galante, N.; Roache, E.] Harvard Smithsonian Ctr Astrophys, Fred Lawrence Whipple Observ, Amado, AZ 85645 USA. [Berger, K.; Holder, J.; Kumar, S.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [Berger, K.; Holder, J.; Kumar, S.] Univ Delaware, Bartol Res Inst, Newark, DE 19716 USA. [Bird, R.; Khassen, Y.; Pueschel, E.; Quinn, J.] Univ Coll Dublin, Sch Phys, Dublin 4, Ireland. [Byrum, K.; Zitzer, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Cardenzana, J. V.; Dickinson, H. J.; Eisch, J. D.; Krennrich, F.; Madhavan, A.; Orr, M.; Weinstein, A.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Chen, X.; Federici, S.; Hakansson, N.; Pohl, M.; Telezhinsky, I.; Wilhelm, A.] Univ Potsdam, Inst Phys & Astron, D-14476 Potsdam, Germany. [Ciupik, L.; Grube, J.; Gyuk, G.] Adler Planetarium & Astron Museum, Dept Astron, Chicago, IL 60605 USA. [Connolly, M. P.; Gillanders, G. H.; Lang, M. J.; Moriarty, P.] Natl Univ Ireland Univ Coll Galway, Sch Phys, Galway, Ireland. [Cui, W.; Feng, Q.; Finley, J. P.; Sembroski, G. H.; Tucci, J. V.; Varlotta, A.] Purdue Univ, Dept Phys & Astron, W Lafayette, IN 47907 USA. [Dumm, J.; Fortson, L.; Shahinyan, K.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Falcone, A.] Penn State Univ, Dept Astron & Astrophys, Davey Lab 525, University Pk, PA 16802 USA. [Furniss, A.; Johnson, C. A.; Williams, D. A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Furniss, A.; Johnson, C. A.; Williams, D. A.] Univ Calif Santa Cruz, Dept Phys, Santa Cruz, CA 95064 USA. [Griffin, S.; Hanna, D.; Ragan, K.; Rajotte, J.; Staszak, D.; Tyler, J.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Griffiths, S. T.; Kaaret, P.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Humensky, T. B.; Nieto, D.] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Kar, P.; Kieda, D.] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. [Kertzman, M.] Depauw Univ, Dept Phys & Astron, Greencastle, IN 46135 USA. [McArthur, S.; Park, N.; Wakely, S. P.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [McCann, A.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Meagher, K.; Otte, A. N.; Richards, G. T.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Meagher, K.; Otte, A. N.; Richards, G. T.] Georgia Inst Technol, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Millis, J.] Anderson Univ, Dept Phys, Anderson, IN 46012 USA. [Moriarty, P.] Galway Mayo Inst Technol, Dept Life & Phys Sci, Galway, Ireland. [Perkins, J. S.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Reyes, L. C.] Calif Polytech State Univ San Luis Obispo, Dept Phys, San Luis Obispo, CA 94307 USA. [Reynolds, P. T.] Cork Inst Technol, Dept Appl Phys & Instrumentat, Cork, Ireland. RP Aliu, E (reprint author), Columbia Univ Barnard Coll, Dept Phys & Astron, New York, NY 10027 USA. RI Khassen, Yerbol/I-3806-2015; Nieto, Daniel/J-7250-2015; OI Khassen, Yerbol/0000-0002-7296-3100; Nieto, Daniel/0000-0003-3343-0755; Pueschel, Elisa/0000-0002-0529-1973; Cui, Wei/0000-0002-6324-5772; Bird, Ralph/0000-0002-4596-8563 FU U.S. Department of Energy Office of Science; U.S. National Science Foundation; Smithsonian Institution; NSERC in Canada; Science Foundation Ireland [SFI 10/RFP/AST2748]; STFC in the U.K. FX The VERITAS Collaboration is grateful to Trevor Weekes for his seminal contributions and leadership in the field of VHE gamma-ray astrophysics, which made this study possible. This research is supported by grants from the U.S. Department of Energy Office of Science, the U.S. National Science Foundation and the Smithsonian Institution, by NSERC in Canada, by Science Foundation Ireland (SFI 10/RFP/AST2748) and by STFC in the U.K. We acknowledge the excellent work of the technical support staff at the Fred Lawrence Whipple Observatory and at the collaborating institutions in the construction and operation of the instrument. NR 37 TC 7 Z9 7 U1 1 U2 10 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JAN 20 PY 2015 VL 799 IS 1 AR 7 DI 10.1088/0004-637X/799/1/7 PG 9 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AZ4SY UT WOS:000348214500007 ER PT J AU Chatzopoulos, E van Rossum, DR Craig, WJ Whalen, DJ Smidt, J Wiggins, B AF Chatzopoulos, E. van Rossum, Daniel R. Craig, Wheeler J. Whalen, Daniel J. Smidt, Joseph Wiggins, Brandon TI EMISSION FROM PAIR-INSTABILITY SUPERNOVAE WITH ROTATION SO ASTROPHYSICAL JOURNAL LA English DT Article DE radiative transfer; stars: massive; stars: rotation; supernovae: general; supernovae: individual (pair-instability) ID POPULATION III PROTOSTARS; STELLAR ASTROPHYSICS MESA; GAMMA-RAY BURSTS; M-CIRCLE-DOT; SUPERLUMINOUS SUPERNOVAE; 1ST STARS; MASSIVE STARS; LIGHT-CURVE; LUMINOUS SUPERNOVAE; RADIATIVE-TRANSFER AB Pair-instability supernovae (PISNe) have been suggested as candidates for some superluminous supernovae, such as SN 2007bi, and as one of the dominant types of explosion occurring in the early universe from massive, zero-metallicity Population III stars. The progenitors of such events can be rapidly rotating, therefore exhibiting different evolutionary properties due to the effects of rotationally induced mixing and mass-loss. Proper identification of such events requires rigorous radiation hydrodynamics and radiative transfer calculations that capture not only the behavior of the light curve but also the spectral evolution of these events. We present radiation hydrodynamics and radiation transport calculations for 90-300M(circle dot) rotating PISNe covering both the shock breakout and late light curve phases. We also investigate cases of different initial metallicity and rotation rate to determine the impact of these parameters on the detailed spectral characteristics of these events. In agreement with recent results on non-rotating PISNe, we find that for a range of progenitor masses and rotation rates these events have intrinsically red colors in contradiction with observations of superluminous supernovae. The spectroscopic properties of rotating PISNe are similar to those of non-rotating events with stripped hydrogen and helium envelopes. We find that the progenitor metallicity and rotation rate properties are erased after the explosion and cannot be identified in the resulting model spectra. It is the combined effects of pre-supernova mass-loss and the basic properties of the supernova ejecta such as mass, temperature, and velocity that have the most direct impact in the model spectra of PISNe. C1 [Chatzopoulos, E.; van Rossum, Daniel R.] Univ Chicago, Dept Astron & Astrophys, Flash Ctr Computat Sci, Chicago, IL 60637 USA. [Craig, Wheeler J.] Univ Texas Austin, Dept Astron, Austin, TX 78712 USA. [Whalen, Daniel J.] Heidelberg Univ, Zentrum Astron, Inst Theoret Astrophys, D-69120 Heidelberg, Germany. [Smidt, Joseph; Wiggins, Brandon] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Wiggins, Brandon] Brigham Young Univ, Dept Phys & Astron, Provo, UT 84602 USA. RP Chatzopoulos, E (reprint author), Univ Chicago, Dept Astron & Astrophys, Flash Ctr Computat Sci, 5640 S Ellis Ave, Chicago, IL 60637 USA. EM manolis@flash.uchicago.edu FU STScI [AR 12820, 13276]; National Science Foundation [AST-0909132, PHY-0822648]; Enrico Fermi Institute via the Enrico Fermi Fellowship FX We thank Wesley Even, Sean M. Couch, Donald Q. Lamb, Ryan Chornock, Ken Chen, Alexandra Kozyreva, and Ragnhild Lunnan for useful discussions and comments. This work was supported in part by the STScI grants AR 12820 and 13276 and the National Science Foundation under grants AST-0909132 and PHY-0822648 for the Physics Frontier Center "Joint Institute for Nuclear Astrophysics" (JINA). E.C. thanks the Enrico Fermi Institute for its support via the Enrico Fermi Fellowship. NR 81 TC 9 Z9 9 U1 0 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JAN 20 PY 2015 VL 799 IS 1 AR 18 DI 10.1088/0004-637X/799/1/18 PG 14 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AZ4SY UT WOS:000348214500017 ER PT J AU Funsten, HO Bzowski, M Cai, DM Dayeh, M DeMajistre, R Frisch, PC Heerikhuisen, J Higdon, DM Janzen, P Larsen, BA Livadiotis, G McComas, DJ Mobius, E Reese, CS Roelof, EC Reisenfeld, DB Schwadron, NA Zirnstein, EJ AF Funsten, H. O. Bzowski, M. Cai, D. M. Dayeh, M. DeMajistre, R. Frisch, P. C. Heerikhuisen, J. Higdon, D. M. Janzen, P. Larsen, B. A. Livadiotis, G. McComas, D. J. Moebius, E. Reese, C. S. Roelof, E. C. Reisenfeld, D. B. Schwadron, N. A. Zirnstein, E. J. TI SYMMETRY OF THE IBEX RIBBON OF ENHANCED ENERGETIC NEUTRAL ATOM (ENA) FLUX SO ASTROPHYSICAL JOURNAL LA English DT Article DE ISM: atoms; ISM: kinematics and dynamics; ISM: magnetic fields; ISM: structure; Sun: heliosphere ID INTERSTELLAR-BOUNDARY-EXPLORER; 1ST 5 YEARS; SOLAR-WIND; OUTER HELIOSPHERE; SPECTRAL PROPERTIES; INNER HELIOSHEATH; LO OBSERVATIONS; MODEL; HELIOPAUSE; IONS AB The circular ribbon of enhanced energetic neutral atom (ENA) emission observed by the Interstellar Boundary Explorer (IBEX) mission remains a critical signature for understanding the interaction between the heliosphere and the interstellar medium. We study the symmetry of the ribbon flux and find strong, spectrally dependent reflection symmetry throughout the energy range 0.7-4.3 keV. The distribution of ENA flux around the ribbon is predominantly unimodal at 0.7 and 1.1 keV, distinctly bimodal at 2.7 and 4.3 keV, and a mixture of both at 1.7 keV. The bimodal flux distribution consists of partially opposing bilateral flux lobes, located at highest and lowest heliographic latitude extents of the ribbon. The vector between the ribbon center and heliospheric nose (which defines the so-called BV plane) appears to play an organizing role in the spectral dependence of the symmetry axis locations as well as asymmetric contributions to the ribbon flux. The symmetry planes at 2.7 and 4.3 keV, derived by projecting the symmetry axes to a great circle in the sky, are equivalent to tilting the heliographic equatorial plane to the ribbon center, suggesting a global heliospheric ordering. The presence and energy dependence of symmetric unilateral and bilateral flux distributions suggest strong spectral filtration from processes encountered by an ion along its journey from the source plasma to its eventual detection at IBEX. C1 [Funsten, H. O.; Cai, D. M.; Higdon, D. M.; Larsen, B. A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Bzowski, M.] Polish Acad Sci, Space Res Ctr, PL-00716 Warsaw, Poland. [Dayeh, M.; Livadiotis, G.; McComas, D. J.; Zirnstein, E. J.] Southwest Res Inst, San Antonio, TX 78228 USA. [DeMajistre, R.; Roelof, E. C.] Johns Hopkins Univ, Appl Phys Lab, Laurel, MD 20723 USA. [Frisch, P. C.] Univ Chicago, Chicago, IL 60637 USA. [Heerikhuisen, J.; Zirnstein, E. J.] Univ Alabama, Huntsville, AL 35899 USA. [Janzen, P.; Reisenfeld, D. B.] Univ Montana, Missoula, MT 59812 USA. [McComas, D. J.] Univ Texas San Antonio, San Antonio, TX 78249 USA. [Moebius, E.; Schwadron, N. A.] Univ New Hampshire, Durham, NH 03824 USA. [Reese, C. S.] Brigham Young Univ, Provo, UT 84602 USA. RP Funsten, HO (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM hfunsten@lanl.gov; bzowski@cbk.waw.pl; maldayeh@swri.org; Bob.DeMajistre@jhuapl.edu; frisch@oddjob.uchicago.edu; jacob.heerikhuisen@uah.edu; paul.janzen@umontana.edu; eberhard.moebius@unh.edu; reese@stat.byu.edu RI Larsen, Brian/A-7822-2011; Reisenfeld, Daniel/F-7614-2015; OI Larsen, Brian/0000-0003-4515-0208; Funsten, Herbert/0000-0002-6817-1039; Moebius, Eberhard/0000-0002-2745-6978; Heerikhuisen, Jacob/0000-0001-7867-3633 FU NASA as a part of the Explorer Program; US Department of Energy; Polish National Science Center [2012-06-M-ST9-00455] FX We gratefully acknowledge all of the contributions made by the entire IBEX team who have been and continue to make this mission a tremendous success. IBEX and this work were funded by NASA as a part of the Explorer Program. Work at Los Alamos National Laboratory was performed under the auspices of the US Department of Energy. M.B. was supported by Polish National Science Center grant 2012-06-M-ST9-00455. NR 59 TC 6 Z9 6 U1 1 U2 10 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JAN 20 PY 2015 VL 799 IS 1 AR 68 DI 10.1088/0004-637X/799/1/68 PG 17 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AZ4SY UT WOS:000348214500066 ER PT J AU Leggett, SK Morley, CV Marley, MS Saumon, D AF Leggett, S. K. Morley, Caroline V. Marley, M. S. Saumon, D. TI NEAR-INFRARED PHOTOMETRY OF Y DWARFS: LOW AMMONIA ABUNDANCE AND THE ONSET OF WATER CLOUDS SO ASTROPHYSICAL JOURNAL LA English DT Article DE brown dwarfs; stars: atmospheres ID HUBBLE-SPACE-TELESCOPE; COOLEST BROWN DWARFS; SURVEY-EXPLORER WISE; DIGITAL SKY SURVEY; T-DWARFS; MULTIOBJECT SPECTROGRAPH; L/T TRANSITION; STANDARD STARS; LOW-MASS; DISCOVERY AB We present new near-infrared photometry for seven late-type T dwarfs and nine Y-type dwarfs, and lower limit magnitudes for a tenth Y dwarf, obtained at Gemini Observatory. We also present a reanalysis of H-band imaging data from the Keck Observatory Archive, for an 11th Y dwarf. These data are combined with earlier MKO-system photometry, Spitzer and WISE mid-infrared photometry, and available trigonometric parallaxes, to create a sample of late-type brown dwarfs that includes 10 T9-T9.5 dwarfs or dwarf systems, and 16 Y dwarfs. We compare the data to our models, which include updated H-2 and NH3 opacity, as well as low-temperature condensate clouds. The models qualitatively reproduce the trends seen in the observed colors; however, there are discrepancies of around a factor of two in flux for the Y0-Y1 dwarfs, with T-eff approximate to 350-400 K. At T-eff similar to 400 K, the problems could be addressed by significantly reducing the NH3 absorption, for example by halving the abundance of NH3 possibly by vertical mixing. At T-eff similar to 350 K, the discrepancy may be resolved by incorporating thick water clouds. The onset of these clouds might occur over a narrow range in T-eff, as indicated by the observed small change in 5 mu m flux over a large change in J -W2 color. Of the known Y dwarfs, the reddest in J-W2 are WISEP J182831.08 + 265037.8 and WISE J085510.83-071442.5. We interpret the former as a pair of identical 300-350 K dwarfs, and the latter as a 250 K dwarf. If these objects are similar to 3 Gyr old, their masses are similar to 10 and similar to 5 Jupiter-masses, respectively. C1 [Leggett, S. K.] Gemini Observ, Northern Operat Ctr, Hilo, HI 96720 USA. [Morley, Caroline V.] Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 95064 USA. [Marley, M. S.] NASA, Ames Res Ctr, Moffett Field, CA 94035 USA. [Saumon, D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Leggett, SK (reprint author), Gemini Observ, Northern Operat Ctr, 670 N Aohoku Pl, Hilo, HI 96720 USA. EM sleggett@gemini.edu OI Marley, Mark/0000-0002-5251-2943; Leggett, Sandy/0000-0002-3681-2989 FU NASA [NNH12AT89I]; Gemini Observatory; National Aeronautics and Space Administration FX D.S. is supported by NASA Origins NNH12AT89I. Based on observations obtained at the Gemini Observatory, which is operated by the Association of Universities for Research in Astronomy, Inc., under a cooperative agreement with the NSF on behalf of the Gemini partnership: the National Science Foundation (United States), the Science and Technology Facilities Council (United Kingdom), the National Research Council (Canada), CONICYT (Chile), the Australian Research Council (Australia), Ministerio da Ciencia, Tecnologia e Inovacao (Brazil) and Ministerio de Ciencia, Tecnologia e Innovacion Productiva (Argentina). S.K.L.'s research is supported by Gemini Observatory. This publication makes use of data products from the Wide-field Infrared Survey Explorer, which is a joint project of the University of California, Los Angeles, and the Jet Propulsion Laboratory/California Institute of Technology, funded by the National Aeronautics and Space Administration. This research has made use of the NASA/IPAC Infrared Science Archive, which is operated by the Jet Propulsion Laboratory, California Institute of Technology, under contract with the National Aeronautics and Space Administration. This research has made use of the Keck Observatory Archive (KOA), which is operated by the W. M. Keck Observatory and the NASA Exoplanet Science Institute (NExScI), under contract with the National Aeronautics and Space Administration. NR 69 TC 13 Z9 13 U1 1 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JAN 20 PY 2015 VL 799 IS 1 AR 37 DI 10.1088/0004-637X/799/1/37 PG 16 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AZ4SY UT WOS:000348214500036 ER PT J AU White, CJ Kasliwal, MM Nugent, PE Gal-Yam, A Howell, DA Sullivan, M Goobar, A Piro, AL Bloom, JS Kulkarni, SR Laher, RR Masci, F Ofek, EO Surace, J Ben-Ami, S Cao, Y Cenko, SB Hook, IM Jonsson, J Matheson, T Sternberg, A Quimby, RM Yaron, O AF White, Christopher J. Kasliwal, Mansi M. Nugent, Peter E. Gal-Yam, Avishay Howell, D. Andrew Sullivan, Mark Goobar, Ariel Piro, Anthony L. Bloom, Joshua S. Kulkarni, Shrinivas R. Laher, Russ R. Masci, Frank Ofek, Eran O. Surace, Jason Ben-Ami, Sagi Cao, Yi Cenko, S. Bradley Hook, Isobel M. Jonsson, Jakob Matheson, Thomas Sternberg, Assaf Quimby, Robert M. Yaron, Ofer TI SLOW-SPEED SUPERNOVAE FROM THE PALOMAR TRANSIENT FACTORY: TWO CHANNELS SO ASTROPHYSICAL JOURNAL LA English DT Article DE supernovae: general; supernovae: individual (iPTF 13an, PTF 09ego, PTF 09eiy, PTF 09eoi, PTF 10xk, PTF 10bvr, PTF 10ujn, PTF 10acdh, PTF 11hyh; SN 2002cx, SN 2002es); surveys; techniques: spectroscopic ID MASS WHITE-DWARFS; IA SUPERNOVAE; LIGHT CURVES; DETONATION SUPERNOVAE; LOW-LUMINOSITY; II SUPERNOVAE; REDSHIFT DATA; LOW-VELOCITY; SN 2008HA; GALAXIES AB Since the discovery of the unusual prototype SN 2002cx, the eponymous class of Type I (hydrogen-poor) supernovae with low ejecta speeds has grown to include approximately two dozen members identified from several heterogeneous surveys, in some cases ambiguously. Here we present the results of a systematic study of 1077 Type I supernovae discovered by the Palomar Transient Factory, leading to nine new members of this peculiar class. Moreover, we find there are two distinct subclasses based on their spectroscopic, photometric, and host galaxy properties: "SN 2002cx-like" supernovae tend to be in later-type or more irregular hosts, have more varied and generally dimmer luminosities, have longer rise times, and lack a Ti II trough when compared to "SN 2002es-like" supernovae. None of our objects show helium, and we counter a previous claim of two such events. We also find that the occurrence rate of these transients relative to Type Ia supernovae is 5.6(-3.8)(+22) % (90% confidence), lower compared to earlier estimates. Combining our objects with the literature sample, we propose that these subclasses have two distinct physical origins. C1 [White, Christopher J.] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA. [Kasliwal, Mansi M.; Piro, Anthony L.] Carnegie Inst Sci, Pasadena, CA 91101 USA. [Nugent, Peter E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Cosmol Ctr, Berkeley, CA 94720 USA. [Nugent, Peter E.; Bloom, Joshua S.] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Gal-Yam, Avishay; Ofek, Eran O.; Ben-Ami, Sagi; Yaron, Ofer] Weizmann Inst Sci, Benoziyo Ctr Astrophys, IL-76100 Rehovot, Israel. [Howell, D. Andrew] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Howell, D. Andrew] Las Cumbres Observ Global Telescope Network Inc, Goleta, CA 93117 USA. [Sullivan, Mark] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. [Goobar, Ariel] Stockholm Univ, AlbaNova, Dept Phys, Oskar Klein Ctr, SE-10691 Stockholm, Sweden. [Piro, Anthony L.] CALTECH, Pasadena, CA 91125 USA. [Kulkarni, Shrinivas R.; Cao, Yi] CALTECH, Cahill Ctr Astrophys, Pasadena, CA 91125 USA. [Laher, Russ R.; Masci, Frank; Surace, Jason] CALTECH, Spitzer Sci Ctr, Pasadena, CA 91125 USA. [Cenko, S. Bradley] NASA, Goddard Space Flight Ctr, Astrophys Sci Div, Greenbelt, MD 20771 USA. [Cenko, S. Bradley] Univ Maryland, Joint Space Sci Inst, College Pk, MD 20742 USA. [Hook, Isobel M.] Univ Oxford, Dept Phys Astrophys, Oxford OX1 3RH, England. [Hook, Isobel M.] INAF Osservatorio Astron Roma, I-00040 Monte Porzio Catone, RM, Italy. [Jonsson, Jakob] Savantic AB, SE-11863 Stockholm, Sweden. [Matheson, Thomas] Natl Opt Astron Observ, Tucson, AZ 85719 USA. [Sternberg, Assaf] Tech Univ Munich, Excellence Cluster Universe, D-85748 Garching, Germany. [Sternberg, Assaf] Max Planck Inst Astrophys, D-85748 Garching, Germany. [Quimby, Robert M.] Univ Tokyo, Kavli IPMU, Kashiwa, Chiba 2778583, Japan. [Quimby, Robert M.] San Diego State Univ, Dept Astron, San Diego, CA 92182 USA. RP White, CJ (reprint author), Princeton Univ, Dept Astrophys Sci, 4 Ivy Lane, Princeton, NJ 08544 USA. OI Sullivan, Mark/0000-0001-9053-4820 FU Hubble Fellowship; Carnegie-Princeton Fellowship; EU/FP7 via ERC [307260]; ISF; Minerva grant; Weizmann-UK grant; "Quantum Universe" I-Core Program of the Planning and Budgeting Committee; Israel Science Foundation; Kimmel Award; NSF [AST-1205732, PHY-1068881, PHY-1151197]; Sherman Fairchild Foundation; Willner Family Leadership Institute, Ilan Gluzman (Secaucus, NJ); Israeli Ministry of Science; Israel Science Foundation, Minerva, Weizmann-UK; I-CORE Program of the Planning and Budgeting Committee FX C. J. W. began this research as part of the summer student exchange program between Princeton and Carnegie. M. M. K. acknowledges generous support from the Hubble Fellowship and Carnegie-Princeton Fellowship. A. G.-Y. acknowledges support by the EU/FP7 via ERC grant 307260; ISF, Minerva, and Weizmann-UK grants; as well as the "Quantum Universe" I-Core Program of the Planning and Budgeting Committee and the Israel Science Foundation and the Kimmel Award. A. L. P. is supported through NSF grants AST-1205732, PHY-1068881, and PHY-1151197, as well as the Sherman Fairchild Foundation. E. O. O. is incumbent on the Arye Dissentshik career development chair and is grateful for support by grants from the Willner Family Leadership Institute, Ilan Gluzman (Secaucus, NJ), the Israeli Ministry of Science, the Israel Science Foundation, Minerva, Weizmann-UK, and the I-CORE Program of the Planning and Budgeting Committee and the Israel Science Foundation. NR 85 TC 17 Z9 17 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JAN 20 PY 2015 VL 799 IS 1 AR 52 DI 10.1088/0004-637X/799/1/52 PG 21 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AZ4SY UT WOS:000348214500050 ER PT J AU Bud'ko, SL AF Bud'ko, Sergey L. TI Superconductivity in K- and Na-doped BaFe2As2: What can we learn from heat capacity and pressure dependence of T-c SO MODERN PHYSICS LETTERS B LA English DT Article DE Iron pnictide superconductors; pressure; heat capacity ID HIGH-TEMPERATURE SUPERCONDUCTIVITY; IRON-BASED SUPERCONDUCTOR; UNCONVENTIONAL SUPERCONDUCTIVITY; METAL; STATE; IMPURITIES; CHEMISTRY; ANOMALIES; BEHAVIOR; KFE2AS2 AB A brief overview of changes in the superconducting transition temperature under pressure and evolution of specific heat capacity jump at T-c for two related families of iron-based superconductors, Ba1-xKxFe2As2 (0.2 <= x <= 1.0) and Ba1-xNaxFe2As2 (0.2 <= x <= 0.9) will be given. For Ba1-xKxFe2As2 the specific heat capacity jump at T-c measured over the whole extent of the superconducting dome shows clear deviation from the empirical, Delta C-p(T-c) proportional to T-c(3), scaling (known as the BNC scaling) for x > 0.7. At the same concentrations range apparent equivalence of effects of pressure and K-substitution on T-c fails. These observations suggests a significant change of the superconducting state for x > 0.7. In contrast, the data for the large portion of Ba1-xNaxFe2As2 (0.2 <= x <= 0.9) series follow the BNC scaling. However, the pressure dependence of T-c (measured up to similar to 12 kbar) have clear nonlinearities for Na concentration in 0.2-0.25 region, that may be consistent with T-c crossing the phase boundaries of the emergent, narrow, antiferromagnetic/tetragonal phase. Results will be discussed in context other studies of these two related families of iron-based superconductors. C1 [Bud'ko, Sergey L.] Iowa State Univ Sci & Technol, Ames Lab, US DOE, Ames, IA 50011 USA. [Bud'ko, Sergey L.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Bud'ko, SL (reprint author), Iowa State Univ Sci & Technol, Ames Lab, US DOE, Ames, IA 50011 USA. EM budko@iastate.edu FU US Department of Energy, Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-07CH11358] FX Work at the Ames Laboratory was supported by the US Department of Energy, Basic Energy Sciences, Division of Materials Sciences and Engineering under contract No. DE-AC02-07CH11358. Fruitful collaboration with Paul C. Canfield, members of the Novel Materials and Ground States research group (Ames Laboratory and Iowa State University) and of the Mercouri G. Kanatzidis research group (Northwestern University and Argonne National Laboratory) is greatly appreciated. A desire to "caress the detail, the divine detail" a contributed to the motivation for this work. NR 103 TC 1 Z9 1 U1 7 U2 37 PU WORLD SCIENTIFIC PUBL CO PTE LTD PI SINGAPORE PA 5 TOH TUCK LINK, SINGAPORE 596224, SINGAPORE SN 0217-9849 EI 1793-6640 J9 MOD PHYS LETT B JI Mod. Phys. Lett. B PD JAN 20 PY 2015 VL 29 IS 2 AR 1430019 DI 10.1142/S0217984914300191 PG 18 WC Physics, Applied; Physics, Condensed Matter; Physics, Mathematical SC Physics GA CA4XO UT WOS:000348910900001 ER PT J AU Haxton, DJ McCurdy, CW AF Haxton, Daniel J. McCurdy, C. William TI Two methods for restricted configuration spaces within the multiconfiguration time-dependent Hartree-Fock method SO PHYSICAL REVIEW A LA English DT Article ID MCTDH METHOD; WAVE-PACKET; PROPAGATING WAVEPACKETS; VARIATIONAL-PRINCIPLES; MOLECULAR-DYNAMICS; ROTATED HARTREE; EFFICIENT; HAMILTONIANS; OPERATORS; FRAMEWORK AB The multiconfiguration time-dependent Hartree-Fock (MCTDHF) method has shown promise in calculating electronic dynamics in molecules driven by strong and high-energy lasers. It must incorporate restricted configuration spaces (meaning that a particular combination of Slater determinants is used, instead of full configuration interaction) to be applied to big systems. Two different Ansatze are used to determine the essential term in the equations. The first Ansatz is the Lagrangian variational principle. The explicit, complete MCTDHF equations of motion, satisfying that principle, for arbitrary configuration spaces, are given. The property that a restricted configuration list must satisfy in order for the Lagrangian and McLachlan variational principles to give different results is identified. The second Ansatz keeps the density matrix block diagonal among equivalent orbitals, in a generalization of the method of Worth [J. Chem. Phys. 112, 8322 (2000)]. The methods perform well in calculating the dynamics of Be and BC2+ subject to ultrafast, ultrastrong lasers in severely truncated Hilbert spaces, although they exhibit differing degrees of numerical stability as implemented. C1 [Haxton, Daniel J.; McCurdy, C. William] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [McCurdy, C. William] Univ Calif Davis, Dept Chem, Davis, CA 95616 USA. RP Haxton, DJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. FU U.S. Department of Energy [DESC0007182]; U.S. Department of Energy Early Career research program; U.S. Department of Energy Office of Basic Energy Sciences, Division of Chemical Sciences [DE-AC02-05CH11231] FX We are indebted to H. Miyagi for correspondence and in particular for providing a corrected derivation of Eq. (53), and furthermore thank S. Kvaal, L. Madsen, and T. Sato for their comments on the manuscript. We thank T. N. Rescigno for continued guidance on the numerical aspects of the project. Computational resources were provided by the National Energy Research Scientific Computing (NERSC) center. Work at the University of California Davis was supported by U.S. Department of Energy Grant No. DESC0007182. D.J.H. acknowledges support through the U.S. Department of Energy Early Career research program. Work at the Lawrence Berkeley National Laboratory was supported by the U.S. Department of Energy Office of Basic Energy Sciences, Division of Chemical Sciences Contract No. DE-AC02-05CH11231. NR 64 TC 10 Z9 10 U1 2 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD JAN 20 PY 2015 VL 91 IS 1 AR 012509 DI 10.1103/PhysRevA.91.012509 PG 15 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA AZ6JH UT WOS:000348325700007 ER PT J AU Makrides, C Hazra, J Pradhan, GB Petrov, A Kendrick, BK Gonzalez-Lezana, T Balakrishnan, N Kotochigova, S AF Makrides, C. Hazra, J. Pradhan, G. B. Petrov, A. Kendrick, B. K. Gonzalez-Lezana, T. Balakrishnan, N. Kotochigova, S. TI Ultracold chemistry with alkali-metal-rare-earth molecules SO PHYSICAL REVIEW A LA English DT Article ID QUANTUM REACTIVE SCATTERING; POTENTIAL-ENERGY SURFACES; GENERAL-ORDER COLLISIONS; LOG-DERIVATIVE METHOD; CHEMICAL-REACTIONS; INSERTION REACTIONS; BEAM EXPERIMENTS; DYNAMICS; ATOM; TEMPERATURES AB A first principles study of the dynamics of Li-6(S-2) + (LiYb)-Li-6-Yb-174((2)Sigma(+)) -> Li-6(2)((1)Sigma(+)) + Yb-174(S-1) reaction is presented at cold and ultracold temperatures. The computations involve determination and analytic fitting of a three-dimensional potential energy surface for the Li2Yb system and quantum dynamics calculations of varying complexities, ranging from exact quantum dynamics within the close-coupling scheme, to statistical quantum treatment, and universal models. It is demonstrated that the two simplified methods yield zero-temperature limiting reaction rate coefficients in reasonable agreement with the full close-coupling calculations. The effect of the three-body term in the interaction potential is explored by comparing quantum dynamics results from a pairwise potential that neglects the three-body term to that derived from the full interaction potential. Inclusion of the three-body term in the close-coupling calculations was found to reduce the limiting rate coefficients by a factor of two. The reaction exoergicity populates vibrational levels as high as v = 19 of the Li-6(2) molecule in the limit of zero collision energy. Product vibrational distributions from the close-coupling calculations reveal sensitivity to inclusion of three-body forces in the interaction potential. Overall, the results indicate that a simplified model based on the long-range potential is able to yield reliable values of the total reaction rate coefficient in the ultracold limit but a more rigorous approach based on statistical quantum or quantum close-coupling methods is desirable when product rovibrational distribution is required. C1 [Makrides, C.; Petrov, A.; Kotochigova, S.] Temple Univ, Dept Phys, Philadelphia, PA 19122 USA. [Hazra, J.; Pradhan, G. B.; Balakrishnan, N.] Univ Nevada, Dept Chem, Las Vegas, NV 89154 USA. [Kendrick, B. K.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Gonzalez-Lezana, T.] IFF CSIC, Inst Fis Fundamental, E-28006 Madrid, Spain. RP Kotochigova, S (reprint author), Temple Univ, Dept Phys, Philadelphia, PA 19122 USA. EM skotoch@temple.edu RI Petrov, Alexander/I-7865-2013 OI Petrov, Alexander/0000-0003-1342-3160 FU Army Research Office, MURI [W911NF-12-1-0476]; National Science Foundation [PHY-1308573, PHY-1205838]; Spanish MICINN [FIS2011-29596-C02-01]; US Department of Energy of the Laboratory Directed Research and Development Program at Los Alamos National Laboratory [20140309ER]; National Security Administration of the US Department of Energy [DE-AC52-06NA25396] FX The Temple University and University of Nevada Las Vegas teams acknowledge support from the Army Research Office, MURI Grant No. W911NF-12-1-0476, and the National Science Foundation, Grants No. PHY-1308573 (S.K.) and No. PHY-1205838 (N.B.). T.G.L. acknowledges support from Project No. FIS2011-29596-C02-01 of the Spanish MICINN. B.K.K. acknowledges that part of this work was done under the auspices of the US Department of Energy under Project No. 20140309ER of the Laboratory Directed Research and Development Program at Los Alamos National Laboratory. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Security Administration of the US Department of Energy under Contract No. DE-AC52-06NA25396. NR 74 TC 7 Z9 7 U1 1 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD JAN 20 PY 2015 VL 91 IS 1 AR 012708 DI 10.1103/PhysRevA.91.012708 PG 12 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA AZ6JH UT WOS:000348325700009 ER PT J AU Shi, HL Parker, D Du, MH Singh, DJ AF Shi, Hongliang Parker, David Du, Mao-Hua Singh, David J. TI Connecting Thermoelectric Performance and Topological-Insulator Behavior: Bi2Te3 and Bi2Te2Se from First Principles SO PHYSICAL REVIEW APPLIED LA English DT Article ID CRYSTAL STRUCTURE; BISMUTH SELENIDE; SOLID SOLUTIONS; BAND-STRUCTURE; DIFFRACTION; DEFECTS; ALLOYS; SYSTEM; TE; SN AB Thermoelectric performance is of interest for numerous applications such as waste-heat recovery and solid-state energy conversion and will be seen to be closely connected to topological-insulator behavior. In this context, we here report first-principles transport and defect calculations for Bi2Te2Se in relation to Bi2Te3. The two compounds are found to contain remarkably different electronic structures in spite of being isostructural and isoelectronic. We discuss these results in terms of the topological-insulator characteristics of these compounds. C1 [Shi, Hongliang; Parker, David; Du, Mao-Hua; Singh, David J.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Shi, HL (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RI Shi, Hongliang/A-7568-2010; Du, Mao-Hua/B-2108-2010 OI Shi, Hongliang/0000-0003-0713-4688; Du, Mao-Hua/0000-0001-8796-167X FU U.S. Department of Energy, Basic Energy Sciences, Materials Science and Engineering Division; DOE S3TEC Energy Frontier Research Center FX This work is sponsored by the U.S. Department of Energy, Basic Energy Sciences, Materials Science and Engineering Division (H.S. and M.H.D.) and the DOE S3TEC Energy Frontier Research Center (D.P. and D.J.S.). NR 35 TC 30 Z9 30 U1 13 U2 65 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2331-7019 J9 PHYS REV APPL JI Phys. Rev. Appl. PD JAN 20 PY 2015 VL 3 IS 1 AR 014004 DI 10.1103/PhysRevApplied.3.014004 PG 10 WC Physics, Applied SC Physics GA AZ6LM UT WOS:000348331300002 ER PT J AU Tong, S Park, WI Choi, YY Stan, L Hong, S Roelofs, A AF Tong, Sheng Park, Woon Ik Choi, Yoon-Young Stan, Liliana Hong, Seungbum Roelofs, Andreas TI Mechanical Removal and Rescreening of Local Screening Charges at Ferroelectric Surfaces SO PHYSICAL REVIEW APPLIED LA English DT Article ID OXIDE SURFACES; THIN-FILMS; MICROSCOPY; POLARIZATION; SOLIDS AB We report the kinetics of screening charge removal and rescreening on periodically poled lithium niobate using charge-gradient microscopy and electrostatic force microscopy (EFM). A minimum pressure needs to be applied to initiate mechanical screening charge removal, and increasing the pressure leads to further removal of charge until a threshold is reached when all screening charges are removed. We fit all rescreening EFM contrast curves under various pressures into a universal exponential decay. The findings imply that we can control the screening degree of ferroelectric surfaces by mechanical means without affecting the polarization underneath. C1 [Tong, Sheng; Stan, Liliana; Roelofs, Andreas] Argonne Natl Lab, Nanosci & Technol Div, Lemont, IL 60439 USA. [Park, Woon Ik; Choi, Yoon-Young; Hong, Seungbum] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. RP Hong, S (reprint author), Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. EM hong@anl.gov; aroelofs@anl.gov RI Hong, Seungbum/B-7708-2009; Tong, Sheng/A-2129-2011; Roelofs, Andreas/H-1742-2011 OI Hong, Seungbum/0000-0002-2667-1983; Tong, Sheng/0000-0003-0355-7368; Roelofs, Andreas/0000-0003-4141-3082 FU U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division; Center for Nanoscale Materials; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work is supported by the U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division and by the Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facilities under Contract No. DE-AC02-06CH11357. EFM, PFM, and CGM work is performed at Materials Science Division, and SEM and PZT thin film deposition work is performed at Center for Nanoscale Materials. NR 27 TC 5 Z9 5 U1 5 U2 35 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2331-7019 J9 PHYS REV APPL JI Phys. Rev. Appl. PD JAN 20 PY 2015 VL 3 IS 1 AR 014003 DI 10.1103/PhysRevApplied.3.014003 PG 6 WC Physics, Applied SC Physics GA AZ6LM UT WOS:000348331300001 ER PT J AU Clerouin, J Robert, G Arnault, P Ticknor, C Kress, JD Collins, LA AF Clerouin, Jean Robert, Gregory Arnault, Philippe Ticknor, Christopher Kress, Joel D. Collins, Lee A. TI Evidence for out-of-equilibrium states in warm dense matter probed by x-ray Thomson scattering SO PHYSICAL REVIEW E LA English DT Article ID PLASMA; ENERGY AB A recent and unexpected discrepancy between ab initio simulations and the interpretation of a laser shock experiment on aluminum, probed by x-ray Thomson scattering (XRTS), is addressed. The ion-ion structure factor deduced from the XRTS elastic peak (ion feature) is only compatible with a strongly coupled out-of-equilibrium state. Orbital free molecular dynamics simulations with ions colder than the electrons are employed to interpret the experiment. The relevance of decoupled temperatures for ions and electrons is discussed. The possibility that it mimics a transient, or metastable, out-of-equilibrium state after melting is also suggested. C1 [Clerouin, Jean; Robert, Gregory; Arnault, Philippe] CEA, DAM, DIF, F-91297 Arpajon, France. [Ticknor, Christopher; Kress, Joel D.; Collins, Lee A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Clerouin, J (reprint author), CEA, DAM, DIF, F-91297 Arpajon, France. EM jean.clerouin@cea.fr RI Clerouin, jean/D-8528-2015; Ticknor, Christopher/B-8651-2014; OI Clerouin, jean/0000-0003-2144-2759; Ticknor, Christopher/0000-0001-9972-4524 FU Advanced Simulation and Computing Program (ASC); science campaigns 1 and 4; LANS, LLC for the NNSA of the U.S. DOE [DE-AC52-06NA25396]; CEA/DAM [P184]; NNSA/DP [P184] FX T. Ma and C. Starrett are warmly acknowledged for providing their data. We also thank F. Lambert for his essential contribution on the OFMD code. Some of the authors (C.T., J.D.K., and L.A.C.) gratefully acknowledge support from the Advanced Simulation and Computing Program (ASC) and science campaigns 1 and 4. Los Alamos National Laboratory is operated by LANS, LLC for the NNSA of the U.S. DOE under Contract No. DE-AC52-06NA25396. This work was performed under the auspices of an agreement P184 between CEA/DAM and NNSA/DP on cooperation on fundamental science. NR 29 TC 16 Z9 16 U1 1 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD JAN 20 PY 2015 VL 91 IS 1 AR 011101 DI 10.1103/PhysRevE.91.011101 PG 5 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA AZ6LF UT WOS:000348330600001 PM 25679563 ER PT J AU Starrett, CE Daligault, J Saumon, D AF Starrett, C. E. Daligault, J. Saumon, D. TI Pseudoatom molecular dynamics SO PHYSICAL REVIEW E LA English DT Article ID DENSE MATTER; PLASMAS; METALS; ATOM AB An approach to simulating warm and hot dense matter that combines density-functional-theory-based calculations of the electronic structure to classical molecular dynamics simulations with pair interaction potentials is presented. The method, which we call pseudoatom molecular dynamics, can be applied to single-component or multicomponent plasmas. It gives equation of state and self-diffusion coefficients with an accuracy comparable to orbital-free molecular dynamics simulations but is computationally much more efficient. C1 [Starrett, C. E.; Daligault, J.; Saumon, D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Starrett, CE (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM starrett@lanl.gov FU United States Department of Energy [DE-AC5206NA25396]; LDRD [20130244ER] FX This work was performed under the auspices of the United States Department of Energy under Contract DE-AC5206NA25396 and LDRD Grant No. 20130244ER. NR 32 TC 14 Z9 14 U1 0 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD JAN 20 PY 2015 VL 91 IS 1 AR 013104 DI 10.1103/PhysRevE.91.013104 PG 5 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA AZ6LF UT WOS:000348330600017 PM 25679720 ER PT J AU Jiao, L Chen, Y Kohama, Y Graf, D Bauer, ED Singleton, J Zhu, JX Weng, ZF Pang, GM Shang, T Zhang, JL Lee, HO Park, T Jaime, M Thompson, JD Steglich, F Si, QM Yuan, HQ AF Jiao, Lin Chen, Ye Kohama, Yoshimitsu Graf, David Bauer, E. D. Singleton, John Zhu, Jian-Xin Weng, Zongfa Pang, Guiming Shang, Tian Zhang, Jinglei Lee, Han-Oh Park, Tuson Jaime, Marcelo Thompson, J. D. Steglich, Frank Si, Qimiao Yuan, H. Q. TI Fermi surface reconstruction and multiple quantum phase transitions in the antiferromagnet CeRhIn5 SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE heavy fermion; quantum phase transitions; superconductivity; Fermi surface reconstruction; localized-itinerant transition ID CRITICAL-POINT; HEAVY; METALS; SUPERCONDUCTIVITY; CRITICALITY; PRESSURE AB Conventional, thermally driven continuous phase transitions are described by universal critical behavior that is independent of the specific microscopic details of a material. However, many current studies focus on materials that exhibit quantum-driven continuous phase transitions (quantum critical points, or QCPs) at absolute zero temperature. The classification of such QCPs and the question of whether they show universal behavior remain open issues. Here we report measurements of heat capacity and de Haas-van Alphen (dHvA) oscillations at low temperatures across a field-induced anti-ferromagnetic QCP (B-c0 approximate to 50 T) in the heavy-fermion metal CeRhIn5. A sharp, magnetic-field-induced change in Fermi surface is detected both in the dHvA effect and Hall resistivity at B-0* approximate to 30 T, well inside the antiferromagnetic phase. Comparisons with band-structure calculations and properties of isostructural CeCoIn5 suggest that the Fermi-surface change at B-0* is associated with a localized-to-itinerant transition of the Ce-4f electrons in CeRhIn5. Taken in conjunction with pressure experiments, our results demonstrate that at least two distinct classes of QCP are observable in CeRhIn5, a significant step toward the derivation of a universal phase diagram for QCPs. C1 [Jiao, Lin; Chen, Ye; Weng, Zongfa; Pang, Guiming; Shang, Tian; Zhang, Jinglei; Lee, Han-Oh; Steglich, Frank; Yuan, H. Q.] Zhejiang Univ, Ctr Correlated Matter, Hangzhou 310058, Zhejiang, Peoples R China. [Jiao, Lin; Chen, Ye; Weng, Zongfa; Pang, Guiming; Shang, Tian; Zhang, Jinglei; Lee, Han-Oh; Steglich, Frank; Yuan, H. Q.] Zhejiang Univ, Dept Phys, Hangzhou 310058, Zhejiang, Peoples R China. [Kohama, Yoshimitsu; Bauer, E. D.; Singleton, John; Zhu, Jian-Xin; Jaime, Marcelo; Thompson, J. D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Graf, David] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. [Park, Tuson] Sungkyunkwan Univ, Dept Phys, Suwon 440746, South Korea. [Steglich, Frank] Max Planck Inst Chem Phys Solids, D-01187 Dresden, Germany. [Si, Qimiao] Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. [Yuan, H. Q.] Nanjing Univ, Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Jiangsu, Peoples R China. RP Si, QM (reprint author), Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. EM qmsi@rice.edu; hqyuan@zju.edu.cn RI Jaime, Marcelo/F-3791-2015; OI Jaime, Marcelo/0000-0001-5360-5220; Bauer, Eric/0000-0003-0017-1937 FU National Basic Research Program of China (973 Program) [2011CBA00103, 2009CB929104]; Natural Science Foundation of China [11174245, 10934005]; Fundamental Research Funds for the Central Universities; Zhejiang Provincial Natural Science Foundation of China; Department of Energy (DOE); DOE/Office of Science Project Complex Electronic Materials; National Science Foundation (NSF); State of Florida; DOE Basic Energy Sciences Program Science; National Research Foundation [220-2011-1-C00014]; German Research Foundation Research Unit 960 Quantum Phase Transitions; NSF [DMR-1309531]; Robert A. Welch Foundation [C-1411] FX We thank S. Kirchner and R. Daou for valuable discussion. Work at Zhejiang University was supported by National Basic Research Program of China (973 Program) Grants 2011CBA00103 and 2009CB929104, Natural Science Foundation of China Grants 11174245 and 10934005, the Fundamental Research Funds for the Central Universities, and Zhejiang Provincial Natural Science Foundation of China. Work at Los Alamos National Laboratory was performed under the auspices of the Department of Energy (DOE) and was supported by the DOE/Office of Science Project Complex Electronic Materials. Work at the National High Magnetic Field Laboratory is also supported by the National Science Foundation (NSF), the State of Florida, and the DOE Basic Energy Sciences Program Science in 100 T.T.P. acknowledges support from National Research Foundation Grant 220-2011-1-C00014. Work at Dresden was partially supported by the German Research Foundation Research Unit 960 Quantum Phase Transitions. Work at Rice University was supported, in part, by NSF Grant DMR-1309531 and Robert A. Welch Foundation Grant C-1411. NR 30 TC 15 Z9 15 U1 8 U2 74 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JAN 20 PY 2015 VL 112 IS 3 BP 673 EP 678 DI 10.1073/pnas.1413932112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AZ2BY UT WOS:000348040700028 PM 25561536 ER PT J AU Guzman, GI Utrilla, J Nurk, S Brunk, E Monk, JM Ebrahim, A Palsson, BO Feist, AM AF Guzman, Gabriela I. Utrilla, Jose Nurk, Sergey Brunk, Elizabeth Monk, Jonathan M. Ebrahim, Ali Palsson, Bernhard O. Feist, Adam M. TI Model-driven discovery of underground metabolic functions in Escherichia coli SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE underground metabolism; substrate promiscuity; systems biology; isozyme discovery; genome-scale modeling ID STRUCTURE PREDICTION; ADAPTIVE EVOLUTION; GENOME ANNOTATION; PROTEIN-STRUCTURE; SCALE; AMINOTRANSFERASE; RECONSTRUCTIONS; BIOSYNTHESIS; SPECIFICITY; ASPARTATE AB Enzyme promiscuity toward substrates has been discussed in evolutionary terms as providing the flexibility to adapt to novel environments. In the present work, we describe an approach toward exploring such enzyme promiscuity in the space of a metabolic network. This approach leverages genome-scale models, which have been widely used for predicting growth phenotypes in various environments or following a genetic perturbation; however, these predictions occasionally fail. Failed predictions of gene essentiality offer an opportunity for targeting biological discovery, suggesting the presence of unknown underground pathways stemming from enzymatic cross-reactivity. We demonstrate a workflow that couples constraint-based modeling and bioinformatic tools with KO strain analysis and adaptive laboratory evolution for the purpose of predicting promiscuity at the genome scale. Three cases of genes that are incorrectly predicted as essential in Escherichia coli-aspC, argD, and gltA-are examined, and isozyme functions are uncovered for each to a different extent. Seven isozyme functions based on genetic and transcriptional evidence are suggested between the genes aspC and tyrB, argD and astC, gabT and puuE, and gltA and prpC. This study demonstrates how a targeted model-driven approach to discovery can systematically fill knowledge gaps, characterize underground metabolism, and elucidate regulatory mechanisms of adaptation in response to gene KO perturbations. C1 [Guzman, Gabriela I.; Utrilla, Jose; Ebrahim, Ali; Palsson, Bernhard O.; Feist, Adam M.] Univ Calif San Diego, Dept Bioengn, La Jolla, CA 92093 USA. [Monk, Jonathan M.] Univ Calif San Diego, Dept NanoEngn, La Jolla, CA 92093 USA. [Palsson, Bernhard O.] Univ Calif San Diego, Dept Pediat, La Jolla, CA 92093 USA. [Nurk, Sergey] Russian Acad Sci, St Petersburg Acad Univ, Algorithm Biol Lab, St Petersburg 196140, Russia. [Brunk, Elizabeth] Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, Emeryville, CA 94608 USA. [Palsson, Bernhard O.; Feist, Adam M.] Tech Univ Denmark, Novo Nordisk Fdn Ctr Biosustainabil, DK-2800 Lyngby, Denmark. RP Feist, AM (reprint author), Univ Calif San Diego, Dept Bioengn, La Jolla, CA 92093 USA. EM afeist@ucsd.edu RI Utrilla , Jose/A-3610-2013; OI Ebrahim, Ali/0000-0002-4009-2128 FU Novo Nordisk Foundation; NIH Grants/National Institute of General Medical Sciences Grant [1R01GM057089] FX We thank Zachary King for helpful discussions and insight, Richard Szubin for assistance with strain resequencing, and Daniel Zielinski for inspiration. This work was partially supported by the Novo Nordisk Foundation and NIH Grants/National Institute of General Medical Sciences Grant 1R01GM057089. NR 40 TC 16 Z9 16 U1 0 U2 16 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JAN 20 PY 2015 VL 112 IS 3 BP 929 EP 934 DI 10.1073/pnas.1414218112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AZ2BY UT WOS:000348040700071 PM 25564669 ER PT J AU Miller, JM Tomsick, JA Bachetti, M Wilkins, D Boggs, SE Christensen, FE Craig, WW Fabian, AC Grefenstette, BW Hailey, CJ Harrison, FA Kara, E King, AL Stern, DK Zhang, WW AF Miller, J. M. Tomsick, J. A. Bachetti, M. Wilkins, D. Boggs, S. E. Christensen, F. E. Craig, W. W. Fabian, A. C. Grefenstette, B. W. Hailey, C. J. Harrison, F. A. Kara, E. King, A. L. Stern, D. K. Zhang, W. W. TI NEW CONSTRAINTS ON THE BLACK HOLE LOW/HARD STATE INNER ACCRETION FLOW WITH NuSTAR SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE accretion, accretion disks; black hole physics ID X-RAY REFLECTION; ACTIVE GALACTIC NUCLEI; GRS 1739-278; DISK WIND; SPIN; MASS; SPECTRA; MODELS; JETS; SPECTROSCOPY AB We report on an observation of the Galactic black hole candidate GRS 1739-278 during its 2014 outburst, obtained with NuSTAR. The source was captured at the peak of a rising "low/hard" state, at a flux of similar to 0.3 Crab. A broad, skewed iron line and disk reflection spectrum are revealed. Fits to the sensitive NuSTAR spectra with a number of relativistically blurred disk reflection models yield strong geometrical constraints on the disk and hard X-ray "corona." Two models that explicitly assume a "lamp post" corona find its base to have a vertical height above the black hole of h = 5(-2)(+7) GM/c(2) and h = 18 +/- 4GM/c(2) (90% confidence errors); models that do not assume a "lamp post" return emissivity profiles that are broadly consistent with coronae of this size. Given that X-ray microlensing studies of quasars and reverberation lags in Seyferts find similarly compact coronae, observations may now signal that compact coronae are fundamental across the black hole mass scale. All of the models fit to GRS 1739-278 find that the accretion disk extends very close to the black hole-the least stringent constraint is r(in) = 5(-4)(+3) GM/c2. Only two of the models deliver meaningful spin constraints, but a = 0.8 +/- 0.2 is consistent with all of the fits. Overall, the data provide especially compelling evidence of an association between compact hard X-ray coronae and the base of relativistic radio jets in black holes. C1 [Miller, J. M.; King, A. L.] Univ Michigan, Dept Astron, Ann Arbor, MI 48109 USA. [Tomsick, J. A.; Boggs, S. E.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Bachetti, M.] Univ Toulouse, UPS OMP, IRAP, F-31100 Toulouse, France. [Bachetti, M.] CNRS, Intitut Rech Astrophys & Planetol, F-31028 Toulouse 4, France. [Wilkins, D.] St Marys Univ, Dept Phys & Astron, Halifax, NS B3H 3C3, Canada. [Christensen, F. E.] Danish Tech Univ, DK-2800 Lyngby, Denmark. [Craig, W. W.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Craig, W. W.; Hailey, C. J.] Columbia Univ, New York, NY 10027 USA. [Fabian, A. C.; Kara, E.] Univ Cambridge, Inst Astron, Cambridge CB3 OHA, England. [Grefenstette, B. W.; Harrison, F. A.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Stern, D. K.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Zhang, W. W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Miller, JM (reprint author), Univ Michigan, Dept Astron, 500 Church St, Ann Arbor, MI 48109 USA. EM jonmm@umich.edu RI Boggs, Steven/E-4170-2015; OI Boggs, Steven/0000-0001-9567-4224; Bachetti, Matteo/0000-0002-4576-9337 FU NASA [NNG08FD60C] FX J.M.M. thanks Javier Garcia and Thomas Dauser for helpful conversations. This work was supported under NASA Contract No. NNG08FD60C, and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by NASA. NR 39 TC 18 Z9 18 U1 0 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD JAN 20 PY 2015 VL 799 IS 1 AR L6 DI 10.1088/2041-8205/799/1/L6 PG 6 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA AZ3RD UT WOS:000348143500006 ER PT J AU Gerencser, L Boros, B Derrien, V Hanson, DK Wraight, CA Sebban, P Maroti, P AF Gerencser, Laszlo Boros, Bogata Derrien, Valerie Hanson, Deborah K. Wraight, Colin A. Sebban, Pierre Maroti, Peter TI Stigmatellin Probes the Electrostatic Potential in the Q(B) Site of the Photosynthetic Reaction Center SO BIOPHYSICAL JOURNAL LA English DT Article ID BACTERIAL REACTION CENTERS; ACCEPTOR QUINONE COMPLEX; INDUCED H+ BINDING; RHODOBACTER-SPHAEROIDES; PROTON-TRANSFER; RHODOPSEUDOMONAS-VIRIDIS; CONFORMATIONAL-CHANGES; SECONDARY QUINONE; FREE-ENERGY; PROTEIN AB The electrostatic potential in the secondary quinone (Q(B)) binding site of the reaction center (RC) of the photosynthetic bacterium Rhodobacter sphaeroides determines the rate and free energy change (driving force) of electron transfer to Q(B). It is controlled by the ionization states of residues in a strongly interacting cluster around the Q(B) site. Reduction of the Q(B) induces change of the ionization states of residues and binding of protons from the bulk. Stigmatellin, an inhibitor of the mitochondrial and photosynthetic respiratory chain, has been proven to be a unique voltage probe of the Q(B) binding pocket. It binds to the Q(B) site with high affinity, and the pK value of its phenolic group monitors the local electrostatic potential with high sensitivity. Investigations with different types of detergent as a model system of isolated RC revealed that the pK of stigmatellin was controlled overwhelmingly by electrostatic and slightly by hydrophobic interactions. Measurements showed a high pK value (>11) of stigmatellin in the Q(B) pocket of the dark-state wild-type RC, indicating substantial negative potential. When the local electrostatics of the Q(B) site was modulated by a single mutation, L213Asp -> Ala, or double mutations, L213Asp-L212Glu -> Ala-Ala (AA), the pK of stigmatellin dropped to 7.5 and 7.4, respectively, which corresponds to a >210 mV increase in the electrostatic potential relative to the wild-type RC. This significant pK drop (Delta pK > 3.5) decreased dramatically to (Delta pK > 0.75) in the RC of the compensatory mutant (AA+M44Asn -> AA+M44Asp). Our results indicate that the L213Asp is the most important actor in the control of the electrostatic potential in the Q(B) site of the dark-state wild-type RC, in good accordance with conclusions of former studies using theoretical calculations or light-induced charge recombination assay. C1 [Gerencser, Laszlo; Boros, Bogata; Maroti, Peter] Univ Szeged, Dept Biophys, Szeged, Hungary. [Derrien, Valerie; Sebban, Pierre] Univ Paris 11, Chim Phys Lab, Orsay, France. [Hanson, Deborah K.] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA. [Wraight, Colin A.] Univ Illinois, Dept Biochem, Urbana, IL 61801 USA. [Wraight, Colin A.] Univ Illinois, Ctr Biophys & Computat Biol, Urbana, IL 61801 USA. [Gerencser, Laszlo] Vrije Univ Amsterdam, Dept Phys & Astron, Amsterdam, Netherlands. RP Gerencser, L (reprint author), Univ Szeged, Dept Biophys, Szeged, Hungary. EM l.gerencser@vu.nl; pmaroti@sol.cc.u-szeged.hu FU Tarsadalmi Megujulas Operativ Program grants [TAMOP 4.2.2.A-11/1KONV-2012-0060, TAMOP 4.2.2. B]; COST European Cooperation in Sciences and Technology grant [CM1306]; FOM [126] FX This study has been supported by Tarsadalmi Megujulas Operativ Program grants TAMOP 4.2.2.A-11/1KONV-2012-0060, TAMOP 4.2.2. B, and COST European Cooperation in Sciences and Technology grant CM1306. L.G. is grateful to the FOM (No. 126) for financial support. NR 68 TC 1 Z9 1 U1 1 U2 16 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD JAN 20 PY 2015 VL 108 IS 2 BP 379 EP 394 DI 10.1016/j.bpj.2014.11.3463 PG 16 WC Biophysics SC Biophysics GA AZ4MN UT WOS:000348195700018 PM 25606686 ER PT J AU Troy, TP Tayebjee, MJY Nauta, K Kable, SH Schmidt, TW AF Troy, Tyler P. Tayebjee, Murad J. Y. Nauta, Klaas Kable, Scott H. Schmidt, Timothy W. TI Atmospheric oxidation intermediates: Laser spectroscopy of resonance-stabilized radicals from p-cymene SO CHEMICAL PHYSICS LETTERS LA English DT Article ID SUBSTITUTED BENZYL RADICALS; H-ATOM ABSTRACTION; EXCITATION-SPECTRA; GAS-PHASE; OH; DENSITY; THERMOCHEMISTRY; FLUORESCENCE; MODEL AB Several resonance-stabilized radicals are observed as products of an electrical discharge containing p-cymene, a biogenic monoterpene that contributes to secondary organic aerosols after atmospheric oxidation. Three radicals are identified by resonant 2-color 2-photon ionization mass spectrometry, corresponding to loss of a methyl group or hydrogen atom from the parent p-cymene structure. The radicals are found to absorb in the spectral region consistent with a benzylic chromophore. The spectrum observed on m/z 119 is assigned to alpha,4-dimethylbenzyl radical, and those on m/z 133 to the alpha,alpha,4-trimethylbenzyl and p-isopropylbenzyl radicals, the latter two being intermediates in the atmospheric oxidation of p-cymene. (C) 2014 Elsevier B.V. All rights reserved. C1 [Troy, Tyler P.; Nauta, Klaas; Kable, Scott H.; Schmidt, Timothy W.] Univ Sydney, Sch Chem, Sydney, NSW 2006, Australia. [Tayebjee, Murad J. Y.] Univ New S Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia. [Nauta, Klaas; Kable, Scott H.; Schmidt, Timothy W.] Univ New S Wales, Sch Chem, Sydney, NSW 2052, Australia. [Troy, Tyler P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Schmidt, TW (reprint author), Univ Sydney, Sch Chem, Sydney, NSW 2006, Australia. EM timothy.schmidt@unsw.edu.au RI Schmidt, Timothy/C-2506-2012; OI Schmidt, Timothy/0000-0002-7073-9578; Tayebjee, Murad/0000-0001-5639-027X FU Australian Research Councils [DP120102559]; Australian Renewable Energy Agency FX This research was supported under Australian Research Councils Discovery Projects funding scheme (DP120102559). MJYT thanks the Australian Renewable Energy Agency for a postdoctoral fellowship. TPT acknowledges receipt of an Australian Postgraduate Award. NR 45 TC 7 Z9 7 U1 2 U2 17 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2614 EI 1873-4448 J9 CHEM PHYS LETT JI Chem. Phys. Lett. PD JAN 20 PY 2015 VL 620 BP 129 EP 133 DI 10.1016/j.cplett.2014.12.007 PG 5 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AY5LX UT WOS:000347614700025 ER PT J AU Chen, JS Wang, JKK Carr, SV Vogel, SC Gourdon, O Dai, PC Morosan, E AF Chen, Justin S. Wang, Jiakui K. Carr, Scott V. Vogel, Sven C. Gourdon, Olivier Dai, Pengcheng Morosan, E. TI Chemical tuning of electrical transport in Ti1-xPtxSe2-y SO PHYSICAL REVIEW B LA English DT Article ID TISE2; SUPERCONDUCTIVITY; MONOLAYER; CRYSTAL; METALS; FILMS; MOS2 AB The structural and transport properties of polycrystalline Ti1-xPtxSe2-y (x <= 0.13, y <= 0.2) are studied, revealing highly tunable electrical properties, spanning nearly ten orders of magnitude in scaled resistivity. Using x-ray and neutron diffraction, Pt is found to dope on the Ti site. In the absence of Pt doping (for x = 0), Se deficiency (y > 0) increases the metallic character of TiSe2, while a large increase of the low-temperature resistivity is favored by a lack of Se deficiency (y = 0) and increasing amounts of doped Pt (x > 0). The chemical tuning of the resistivity in Ti1-xPtxSe2-y with Se deficiency and Pt doping results in a metal-to-insulator transition. Simultaneous Pt doping and Se deficiency (x, y > 0) confirms the competition between the two opposing trends in electrical transport, with the main outcome being the suppression of the charge density wave transition below 2 K for y = 2x = 0.18. Band structure calculations on a subset of Ti1-xPtxSe2-y compositions are in line with the experimental observations. C1 [Chen, Justin S.; Wang, Jiakui K.; Carr, Scott V.; Dai, Pengcheng; Morosan, E.] Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. [Vogel, Sven C.; Gourdon, Olivier] Los Alamos Natl Lab, Los Alamos Neutron Sci Ctr, Los Alamos, NM 87545 USA. RP Chen, JS (reprint author), Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. RI Dai, Pengcheng /C-9171-2012; OI Dai, Pengcheng /0000-0002-6088-3170; Vogel, Sven C./0000-0003-2049-0361 FU DOD PECASE; U.S. DOE, BES [DE-SC0012311]; Robert A. Welch Foundation [C-1839]; U.S. Department of Energy's Office of Basic Energy Sciences; DOE [DEAC52-06NA25396] FX E.M. and J.S.C. acknowledge support from the DOD PECASE. The neutron scattering work at Rice was supported by the U.S. DOE, BES, Contract No. DE-SC0012311 (P.D.). Part of the work is supported by the Robert A. Welch Foundation Grant No. C-1839 ( P.D.). This work has benefited from Lujan Neutron Scattering Center at LANSCE, which is funded by the U.S. Department of Energy's Office of Basic Energy Sciences. Los Alamos National Laboratory is operated by Los Alamos National Security LLC under DOE Contract No. DEAC52-06NA25396. NR 44 TC 2 Z9 2 U1 2 U2 31 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 20 PY 2015 VL 91 IS 4 AR 045125 DI 10.1103/PhysRevB.91.045125 PG 7 WC Physics, Condensed Matter SC Physics GA AZ6KG UT WOS:000348328200008 ER PT J AU Schleife, A Kanai, Y Correa, AA AF Schleife, Andre Kanai, Yosuke Correa, Alfredo A. TI Accurate atomistic first-principles calculations of electronic stopping SO PHYSICAL REVIEW B LA English DT Article ID DENSITY-FUNCTIONAL THEORY; DISPLACEMENT CASCADES; SLOW IONS; POWER; SIMULATION; SYSTEMS; GAS; SEMICONDUCTORS; APPROXIMATION; SCATTERING AB We show that atomistic first-principles calculations based on real-time propagation within time-dependent density functional theory are capable of accurately describing electronic stopping of light projectile atoms in metal hosts over a wide range of projectile velocities. In particular, we employ a plane-wave pseudopotential scheme to solve time-dependent Kohn-Sham equations for representative systems of H and He projectiles in crystalline aluminum. This approach to simulate nonadiabatic electron-ion interaction provides an accurate framework that allows for quantitative comparison with experiment without introducing ad hoc parameters such as effective charges, or assumptions about the dielectric function. Our work clearly shows that this atomistic first-principles description of electronic stopping is able to disentangle contributions due to tightly bound semicore electrons and geometric aspects of the stopping geometry (channeling versus off-channeling) in a wide range of projectile velocities. C1 [Schleife, Andre; Kanai, Yosuke; Correa, Alfredo A.] Lawrence Livermore Natl Lab, Quantum Simulat Grp, Livermore, CA 94550 USA. [Kanai, Yosuke] Univ N Carolina, Dept Chem, Chapel Hill, NC 27599 USA. RP Schleife, A (reprint author), Lawrence Livermore Natl Lab, Quantum Simulat Grp, Livermore, CA 94550 USA. EM schleife@illinois.edu; ykanai@unc.edu; correaa@llnl.gov RI Kanai, Yosuke/B-5554-2016 FU Physical and Life Sciences Directorate at Lawrence Livermore National Laboratory; U.S. Department of Energy at Lawrence Livermore National Laboratory [DE-AC52-07A27344] FX We acknowledge fruitful discussions with E. Draeger, Y. Miyamoto, and A. Arnau. A.S. was supported through the Physical and Life Sciences Directorate at Lawrence Livermore National Laboratory. Computing support for this work came from the Lawrence Livermore National Laboratory Institutional Computing Grand Challenge program. Part of this work was performed under the auspices of the U.S. Department of Energy at Lawrence Livermore National Laboratory under Contract DE-AC52-07A27344. NR 56 TC 11 Z9 11 U1 7 U2 30 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 20 PY 2015 VL 91 IS 1 AR 014306 DI 10.1103/PhysRevB.91.014306 PG 9 WC Physics, Condensed Matter SC Physics GA AZ6JM UT WOS:000348326200002 ER PT J AU Yeh, PC Jin, WC Zaki, N Zhang, DT Liou, JT Sadowski, JT Al-Mahboob, A Dadap, JI Herman, IP Sutter, P Osgood, RM AF Yeh, Po-Chun Jin, Wencan Zaki, Nader Zhang, Datong Liou, Jonathan T. Sadowski, Jerzy T. Al-Mahboob, Abdullah Dadap, Jerry I. Herman, Irving P. Sutter, Peter Osgood, Richard M., Jr. TI Layer-dependent electronic structure of an atomically heavy two-dimensional dichalcogenide SO PHYSICAL REVIEW B LA English DT Article ID TRANSITION-METAL DICHALCOGENIDES; FIELD-EFFECT TRANSISTORS; TUNGSTEN DISELENIDE; BAND-GAP; SINGLE-CRYSTALS; MONOLAYER MOS2; WSE2; PHOTOEMISSION; SEMICONDUCTOR; SPECTROSCOPY AB We report angle-resolved photoemission spectroscopic measurements of the evolution of the thickness-dependent electronic band structure of the atomically heavy two-dimensional layered dichalcogenide, tungsten diselenide (WSe2). Our data, taken on mechanically exfoliated WSe2 single crystals, provide direct evidence for shifting of the valence-band maximum from (Gamma) over bar (multilayer WSe2) to (K) over bar (single-layer WSe2). Further, our measurements also set a lower bound on the energy of the direct band gap and provide direct measurement of the hole effective mass. C1 [Yeh, Po-Chun; Liou, Jonathan T.; Osgood, Richard M., Jr.] Columbia Univ, Dept Elect Engn, New York, NY 10027 USA. [Jin, Wencan; Zaki, Nader; Zhang, Datong; Dadap, Jerry I.; Herman, Irving P.; Osgood, Richard M., Jr.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. [Sadowski, Jerzy T.; Al-Mahboob, Abdullah; Sutter, Peter] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Yeh, PC (reprint author), Columbia Univ, Dept Elect Engn, New York, NY 10027 USA. OI Sadowski, Jerzy/0000-0002-4365-7796 FU Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-FG 02-04-ER-46157]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]; U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences [DE-SC0001085]; Empire State Development's Division of Science, Technology and Innovation (NYSTAR); New York State Energy Research Development Authority (NYSERDA) FX The beamline measurements and analyses and the sample mounting were supported by the Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award Contract No. DE-FG 02-04-ER-46157 and were carried out in part at the Center for Functional Nanomaterials and National Synchrotron Light Source, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. The sample preparation and optical characterization (by D.Z., J.T.L., and I.P.H.) was supported as part of the Center for Re-Defining Photovoltaic Efficiency through Molecular Scale Control, an Energy Frontier Research Center funded by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences under Award No. DE-SC0001085. The EFRC work is also supported by a matching grant from the Empire State Development's Division of Science, Technology and Innovation (NYSTAR) as well as by the New York State Energy Research Development Authority (NYSERDA). NR 47 TC 17 Z9 17 U1 6 U2 63 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 20 PY 2015 VL 91 IS 4 AR 041407 DI 10.1103/PhysRevB.91.041407 PG 6 WC Physics, Condensed Matter SC Physics GA AZ6KG UT WOS:000348328200004 ER PT J AU Yue, M Wang, XY AF Yue, Meng Wang, Xiaoyu TI Assessing Cloud Transient Impacts of Solar and Battery Energy Systems on Grid Inertial Responses SO ELECTRIC POWER COMPONENTS AND SYSTEMS LA English DT Article DE PV; inertial response; grid-connected inverter; battery energy storage system; photovoltaic; cloud transient; solar generation ID LEAD-ACID-BATTERIES; DYNAMICAL MODELS AB To assess the dynamic impact of intermittency of rapidly increasing solar photovoltaic generation on the grid, this article presents the modeling and integration of the components that need to be considered, including the solar photovoltaic plant, battery energy storage system, grid-tied interface, and associated control systems. The complexity and accuracy of these models are suitable for evaluating the transient impact on bulk power systems. Of particular interest is the grid inertial response in such situations as different penetration levels of solar generation and fast cloud transient induced solar generation decrease coupled with outages that recurrently occur in the grid, e.g., a generator trip. The impact of such events on the grid frequency responses is investigated using a simplified simulation approach to account for the locational or spatial irradiance variation patterns and cloud movements. Responsive battery energy storage systems are recognized as an effective means to improve the inertial response. C1 [Yue, Meng; Wang, Xiaoyu] Brookhaven Natl Lab, Sustainable Energy Technol Dept, Upton, NY 11973 USA. RP Yue, M (reprint author), Brookhaven Natl Lab, Sustainable Energy Technol Dept, Upton, NY 11973 USA. EM yuemeng@bnl.gov NR 32 TC 1 Z9 1 U1 1 U2 9 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 1532-5008 EI 1532-5016 J9 ELECTR POW COMPO SYS JI Electr. Power Compon. Syst. PD JAN 20 PY 2015 VL 43 IS 2 BP 200 EP 211 DI 10.1080/15325008.2014.975387 PG 12 WC Engineering, Electrical & Electronic SC Engineering GA AX6QQ UT WOS:000347046900008 ER PT J AU Onen, A Cheng, DL Broadwater, RP Scirbona, C Cocks, G Hamilton, S Wang, XY Roark, J AF Onen, Ahmet Cheng, Danling Broadwater, Robert P. Scirbona, Charlie Cocks, George Hamilton, Stephanie Wang, Xiaoyu Roark, Jeffrey TI Economic Evaluation of Distribution System Smart Grid Investments SO ELECTRIC POWER COMPONENTS AND SYSTEMS LA English DT Article DE Monte Carlo simulation; phase balancing; coordinated control; Smart grid investments; capacitor design ID RELIABILITY ASSESSMENT; COORDINATED CONTROL; STORMS AB This article investigates the economic benefits of smart grid automation investments. A system consisting of 7 substations and 14 feeders is used in the evaluation. Here benefits that can be quantified in terms of dollar savings are considered, termed "hard dollar" benefits. Smart grid investment evaluations to be considered include investments in improved efficiency, more cost effective use of existing system capacity with automated switches, and coordinated control of capacitor banks and voltage regulators. These smart grid evaluations are sequentially ordered, resulting in a series of incremental hard dollar benefits. Hard dollar benefits come from improved efficiency, delaying large capital equipment investments, shortened storm restoration times, and reduced customer energy use. Analyses used in the evaluation involve hourly power flow analysis over multiple years and Monte Carlo simulations of switching operations during storms using a reconfiguration for a restoration algorithm. The economic analysis uses the time-varying value of the locational marginal price. Algorithms used include reconfiguration for restoration involving either manual or automated switches and coordinated control involving two modes of control. Field validations of phase balancing and capacitor design results are presented. The evaluation shows that investments in automation can improve performance while simultaneously lowering costs. C1 [Onen, Ahmet; Broadwater, Robert P.] Virginia Polytech Inst & State Univ, Dept Elect & Comp Engn, Blacksburg, VA 24061 USA. [Cheng, Danling] Elect Distribut Design Inc, Blacksburg, VA USA. [Scirbona, Charlie; Cocks, George] Orange & Rockland Utilities Inc, Spring Valley, NY USA. [Hamilton, Stephanie] Brookhaven Natl Lab, Upton, NY 11973 USA. [Wang, Xiaoyu] Brookhaven Natl Lab, Sustainable Energy Technol Dept, Upton, NY 11973 USA. [Roark, Jeffrey] Elect Power Res Inst, Palo Alto, CA USA. RP Onen, A (reprint author), Abdullah Gul Univ, Dept Elect & Elect Engn, Kayseri, Turkey. EM ahmet.onen@agu.edu.tr RI Onen, Ahmet/N-6632-2014; OI Onen, Ahmet/0000-0001-7086-5112 FU Electrical Distribution Design, Inc.; Orange & Rockland Utilities; Brookhaven National Laboratory FX The authors would like to thank Electrical Distribution Design, Inc., Orange & Rockland Utilities, and Brookhaven National Laboratory for providing data, funding, and technical assistance. NR 19 TC 3 Z9 3 U1 1 U2 12 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 1532-5008 EI 1532-5016 J9 ELECTR POW COMPO SYS JI Electr. Power Compon. Syst. PD JAN 20 PY 2015 VL 43 IS 2 BP 224 EP 233 DI 10.1080/15325008.2014.975873 PG 10 WC Engineering, Electrical & Electronic SC Engineering GA AX6QQ UT WOS:000347046900010 ER PT J AU Bishara, F Zupan, J AF Bishara, Fady Zupan, Jure TI Continuous flavor symmetries and the stability of asymmetric dark matter SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Beyond Standard Model; Cosmology of Theories beyond the SM ID FERMION-NUMBER VIOLATION; SUPERSYMMETRY; BARYOGENESIS; PHENOMENOLOGY; CONSTRAINTS; BARYON; MODELS; MASSES; PUZZLE; DECAY AB Generically, the asymmetric interactions in asymmetric dark matter (ADM) models could lead to decaying DM. We show that, for ADM that carries nonzero baryon number, the continuous flavor symmetries that generate the flavor structure in the quark sector also imply a looser lower bound on the mass scale of the asymmetric mediators between the dark and visible sectors. The mediators for B = 2 ADM that can produce a signal in the future indirect dark matter searches can thus also be searched for at the LHC. For two examples of the mediator models, with either the MFV or Froggatt-Nielsen flavor breaking pattern, we derive the FCNC constraints and discuss the search strategies at the LHC. C1 [Bishara, Fady] Univ Cincinnati, Dept Phys, Cincinnati, OH 45221 USA. [Bishara, Fady; Zupan, Jure] Dept Theoret Phys, Fermilab, Batavia, IL 60510 USA. RP Bishara, F (reprint author), Univ Cincinnati, Dept Phys, Cincinnati, OH 45221 USA. EM bisharfy@mail.uc.edu; zupanje@ucmail.uc.edu FU U.S. National Science Foundation under CAREER [PHY-1151392]; Fermilab Fellowship in Theoretical Physics; Fermi Research Alliance, LLC [DE-AC02-07CH11359]; United States Department of Energy; NSF [1066293]; KITP; National Science Foundation [NSF PHY11-25915] FX J.Z. and F.B. are supported by the U.S. National Science Foundation under CAREER Grant PHY-1151392. F.B. is supported by the Fermilab Fellowship in Theoretical Physics. Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. J.Z. is grateful to the Mainz Institute for Theoretical Physics (MITP) for its hospitality and its partial support during the completion of this work. J.Z. thanks the Aspen Center for Physics, supported by the NSF Grant # 1066293, and the KITP, supported in part by the National Science Foundation under Grant No. NSF PHY11-25915, for their warm hospitality. F.B. thanks Prateek Agrawal, Roni Harnik, and Felix Yu for helpful discussions. Some of the cross-sections were computed using MadGraph5 [85] using a model file generated by FeynRules 2.0 [86]. NR 91 TC 2 Z9 2 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN 19 PY 2015 IS 1 AR 089 DI 10.1007/JHEP01(2015)089 PG 34 WC Physics, Particles & Fields SC Physics GA CB4PX UT WOS:000349611400001 ER PT J AU Wang, WS Ye, YF Feng, J Chi, MF Guo, JH Yin, YD AF Wang, Wenshou Ye, Yifan Feng, Ji Chi, Miaofang Guo, Jinghua Yin, Yadong TI Enhanced Photoreversible Color Switching of Redox Dyes Catalyzed by Barium-Doped TiO2 Nanocrystals SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE doping; nanocrystals; oxygen vacancies; photocatalysis; titania ID ALKALINE-EARTH METAL; OXYGEN VACANCY; PHOTOCATALYSTS; MODULATION; SURFACE; LIGHT AB Colloidal barium-doped TiO2 nanocrystals have been developed that enable the highly reversible light-responsive color switching of redox dyes with excellent cycling performance and high switching rates. Oxygen vacancies resulting from the Ba doping serve as effective sacrificial electron donors (SEDs) to scavenge the holes photogenerated in TiO2 nanocrystals under UV irradiation and subsequently promote the reduction of methylene blue to its colorless leuco form. Effective color switching can therefore be realized without relying on external SEDs, thus greatly increasing the number of switching cycles. Badoping can also accelerate the recoloration under visible-light irradiation by shifting the absorption edge of TiO2 nanocrystals to a shorter wavelength. Such a system can be further casted into a solid film to produce a rewritable paper on which letters and patters can be repeatedly printed using UV light and then erased by heating; this process can be repeated for many cycles and does not require additional inks. C1 [Wang, Wenshou; Feng, Ji; Yin, Yadong] Univ Calif Riverside, Dept Chem, Riverside, CA 92521 USA. [Ye, Yifan] Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230029, Peoples R China. [Ye, Yifan; Guo, Jinghua] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Chi, Miaofang] Oak Ridge Natl Lab, Div Mat Sci, Oak Ridge, TN 37830 USA. RP Yin, YD (reprint author), Univ Calif Riverside, Dept Chem, Riverside, CA 92521 USA. EM yadong.yin@ucr.edu RI Wang, Wenshou/C-5579-2015; Yin, Yadong/D-5987-2011; Chi, Miaofang/Q-2489-2015 OI Wang, Wenshou/0000-0001-7313-4403; Yin, Yadong/0000-0003-0218-3042; Chi, Miaofang/0000-0003-0764-1567 FU U.S. Department of Energy [DE-FG02-09ER16096]; U.S. National Science Foundation under Major Research Instrumentation Program [DMR-0958796]; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; National Basic Research Program of China [2013CB834605]; National Natural Science Foundation of China [U1232102] FX We are grateful for financial support from the U.S. Department of Energy (DE-FG02-09ER16096). The XPS facility was acquired with funds from the U.S. National Science Foundation under the Major Research Instrumentation Program (DMR-0958796). The work performed on BL8.0.1 and 10.3.2 at the Advanced Light Source was supported by the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy (DE-AC02-05CH11231). Y. Ye gratefully acknowledges the supervision of Dr. Junfa Zhu at the University of Science and Technology of China, and financial support from the National Basic Research Program of China (2013CB834605) and the National Natural Science Foundation of China (U1232102). We would also like to thank Dr. Josep Roque-Rosell for assistance with XAS measurements. NR 26 TC 4 Z9 4 U1 15 U2 105 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD JAN 19 PY 2015 VL 54 IS 4 BP 1321 EP 1326 DI 10.1002/anie.201410408 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA AZ7BI UT WOS:000348372900048 PM 25598166 ER PT J AU Hadimani, RL Silva, JHB Pereira, AM Schlagel, DL Lograsso, TA Ren, Y Zhang, XY Jiles, DC Araujo, JP AF Hadimani, Ravi L. Silva, Joao H. B. Pereira, Andre M. Schlagel, Devo L. Lograsso, Thomas A. Ren, Yang Zhang, Xiaoyi Jiles, David C. Araujo, Joao P. TI Gd-5(Si,Ge)(4) thin film displaying large magnetocaloric and strain effects due to magnetostructural transition SO APPLIED PHYSICS LETTERS LA English DT Article ID FIELD-INDUCED STRAINS; MAGNETIC REFRIGERATION; ALLOYS; MAGNETOSTRICTION AB Magnetic refrigeration based on the magnetocaloric effect is one of the best alternatives to compete with vapor-compression technology. Despite being already in its technology transfer stage, there is still room for optimization, namely, on the magnetic responses of the magnetocaloric material. In parallel, the demand for different magnetostrictive materials has been greatly enhanced due to the wide and innovative range of technologies that emerged in the last years (from structural evaluation to straintronics fields). In particular, the Gd-5(SixGe1-x)(4) compounds are a family of well-known alloys that present both giant magnetocaloric and colossal magnetostriction effects. Despite their remarkable properties, very few reports have been dedicated to the nanostructuring of these materials: here, we report a similar to 800 nm Gd5Si2.7Ge1.3 thin film. The magnetic and structural investigation revealed that the film undergoes a first order magnetostructural transition and as a consequence exhibits large magnetocaloric effect (-Delta S-mMAX similar to 8.83 J kg(-1) K-1, Delta H = 5T) and giant thermal expansion (12000 p.p.m). The thin film presents a broader magnetic response in comparison with the bulk compound, which results in a beneficial magnetic hysteresis reduction. The Delta S-mMAX exhibited by the Gd-5(Si,Ge)(4) thin film makes it a promising candidate for micro/nano magnetic refrigeration area. (C) 2015 AIP Publishing LLC. C1 [Hadimani, Ravi L.; Jiles, David C.] Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA. [Hadimani, Ravi L.; Schlagel, Devo L.; Lograsso, Thomas A.; Jiles, David C.] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. [Silva, Joao H. B.; Araujo, Joao P.] Univ Porto, Fac Ciencias, Dept Fis & Astron, IFIMUP, P-4169007 Oporto, Portugal. [Silva, Joao H. B.; Araujo, Joao P.] Univ Porto, Fac Ciencias, Dept Fis & Astron, IN Inst Nanosci & Nanotechnol, P-4169007 Oporto, Portugal. [Pereira, Andre M.] Univ London Imperial Coll Sci Technol & Med, Blackett Lab, London SW7 2AZ, England. [Lograsso, Thomas A.] Ames Lab, Div Engn & Mat Sci, Ames, IA 50011 USA. [Ren, Yang; Zhang, Xiaoyi] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Araujo, JP (reprint author), Univ Porto, Fac Ciencias, Dept Fis & Astron, IFIMUP, Rua Campo Alegre 687, P-4169007 Oporto, Portugal. EM jearaujo@fc.up.pt RI Esteves de Araujo, Joao Pedro/D-4389-2011; Pereira, Andre/B-4648-2008; OI Esteves de Araujo, Joao Pedro/0000-0002-1646-7727; Pereira, Andre/0000-0002-8587-262X; Hadimani, Ravi/0000-0001-5939-556X; Lograsso, Thomas/0000-0002-8441-5320 FU FCT [SFRH/BD/88440/2012, PTDC/CTMNAN/115125/2009]; project EPSRC [EP/G060940/1]; DOE-Basic Energy Sciences [DE-AC02-07CH11358]; Barbara and James Palmer Endowment at the Department of Electrical and Computer Engineering of Iowa State University FX We would like to acknowledge V. K. Pecharsky for the useful discussions. J. H. B. Silva thanks FCT for the grant SFRH/BD/88440/2012 and the project PTDC/CTMNAN/115125/2009. A.M.P. acknowledges the project EPSRC EP/G060940/1 for the financial support. The work performed at the Ames Laboratory was supported by the DOE-Basic Energy Sciences under Contract No. DE-AC02-07CH11358 and Barbara and James Palmer Endowment at the Department of Electrical and Computer Engineering of Iowa State University. NR 69 TC 7 Z9 7 U1 4 U2 50 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 19 PY 2015 VL 106 IS 3 AR 032402 DI 10.1063/1.4906056 PG 5 WC Physics, Applied SC Physics GA AZ7EF UT WOS:000348381000040 ER PT J AU Kamaraju, N Pan, W Ekenberg, U Gvozdic, DM Boubanga-Tombet, S Upadhya, PC Reno, J Taylor, AJ Prasankumar, RP AF Kamaraju, N. Pan, W. Ekenberg, U. Gvozdic, D. M. Boubanga-Tombet, S. Upadhya, P. C. Reno, J. Taylor, A. J. Prasankumar, R. P. TI Terahertz magneto-optical spectroscopy of a two-dimensional hole gas SO APPLIED PHYSICS LETTERS LA English DT Article ID CYCLOTRON-RESONANCE; ELECTRON-GAS; HETEROSTRUCTURES; LINEWIDTH AB Two-dimensional hole gases (2DHGs) have attracted recent attention for their unique quantum physics and potential applications in areas including spintronics and quantum computing. However, their properties remain relatively unexplored, motivating the use of different techniques to study them. We used terahertz magneto-optical spectroscopy to investigate the cyclotron resonance frequency in a high mobility 2DHG, revealing a nonlinear dependence on the applied magnetic field. This is shown to be due to the complex non-parabolic valence band structure of the 2DHG, as verified by multiband Landau level calculations. We also find that impurity scattering dominates cyclotron resonance decay in the 2DHG, in contrast with the dominance of superradiant damping in two-dimensional electron gases. Our results shed light on the properties of 2DHGs, motivating further studies of these unique 2D nanosystems. (C) 2015 AIP Publishing LLC. C1 [Kamaraju, N.; Boubanga-Tombet, S.; Upadhya, P. C.; Taylor, A. J.; Prasankumar, R. P.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Pan, W.; Reno, J.] Sandia Natl Labs, Albuquerque, NM 87123 USA. [Ekenberg, U.] Semiconsultants, SE-18773 Taby, Sweden. [Gvozdic, D. M.] Univ Belgrade, Sch Elect Engn, Belgrade 11120, Serbia. [Boubanga-Tombet, S.] Tohoku Univ, Elect Commun Res Inst, Aoba Ku, Sendai, Miyagi 980, Japan. [Upadhya, P. C.] Indian Space Res Org, Lab Electroopt Syst, Bangalore 560058, Karnataka, India. RP Kamaraju, N (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol, POB 1663, Los Alamos, NM 87545 USA. EM nkamaraju@lanl.gov; rpprasan@lanl.gov RI Boubanga Tombet, Stephane/E-9985-2015 FU Department of Energy, Office of Basic Energy Sciences, Division of Material Sciences; U.S. Department of Energy [DE-AC52-06NA25396] FX This work was performed under the auspices of the Department of Energy, Office of Basic Energy Sciences, Division of Material Sciences. The THz magneto-optical measurements were performed at the Center for Integrated Nanotechnologies. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security administration of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. NR 31 TC 4 Z9 4 U1 2 U2 19 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 19 PY 2015 VL 106 IS 3 AR 031902 DI 10.1063/1.4906282 PG 4 WC Physics, Applied SC Physics GA AZ7EF UT WOS:000348381000025 ER PT J AU Selvamanickam, V Gharahcheshmeh, MH Xu, A Galstyan, E Delgado, L Cantoni, C AF Selvamanickam, V. Gharahcheshmeh, M. Heydari Xu, A. Galstyan, E. Delgado, L. Cantoni, C. TI High critical currents in heavily doped (Gd,Y)Ba2Cu3Ox superconductor tapes SO APPLIED PHYSICS LETTERS LA English DT Article ID YBCO-COATED CONDUCTORS; FILMS AB REBa2Cu3Ox ((REBCO), RE = rare earth) superconductor tapes with moderate levels of dopants have been optimized for high critical current density in low magnetic fields at 77 K, but they do not exhibit exemplary performance in conditions of interest for practical applications, i.e., temperatures less than 50K and fields of 2-30 T. Heavy doping of REBCO tapes has been avoided by researchers thus far due to deterioration in properties. Here, we report achievement of critical current densities (J(c)) above 20 MA/cm(2) at 30 K, 3 T in heavily doped (25 mol.% Zr-added) (Gd,Y)Ba2Cu3Ox superconductor tapes, which is more than three times higher than the J(c) typically obtained in moderately doped tapes. Pinning force levels above 1000 GN/m(3) have also been attained at 20 K. A composition map of lift factor in J(c) (ratio of J(c) at 30 K, 3 T to the J(c) at 77 K, 0 T) has been developed which reveals the optimum film composition to obtain lift factors above six, which is thrice the typical value. A highly c-axis aligned BaZrO3 (BZO) nanocolumn defect density of nearly 7 x 10(11) cm(-2) as well as 2-3 nm sized particles rich in Cu and Zr have been found in the high J(c) films. (C) 2015 AIP Publishing LLC. C1 [Selvamanickam, V.; Gharahcheshmeh, M. Heydari; Xu, A.; Galstyan, E.; Delgado, L.] Univ Houston, Dept Mech Engn, Houston, TX 77204 USA. [Selvamanickam, V.; Gharahcheshmeh, M. Heydari; Xu, A.; Galstyan, E.; Delgado, L.] Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. [Cantoni, C.] Oak Ridge Natl Lab, Oak Ridge, TN 37381 USA. RP Selvamanickam, V (reprint author), Univ Houston, Dept Mech Engn, 4800 Calhoun Rd, Houston, TX 77204 USA. EM selva@uh.edu RI Xu, Aixia/M-3514-2014 FU Advanced Research Projects Agency-Energy (ARPA-E) Award [DE-AR0000196]; Office of Naval Research Award [N00014-14-1-0182]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division FX The work at the University of Houston was supported by the Advanced Research Projects Agency-Energy (ARPA-E) Award No. DE-AR0000196 and the Office of Naval Research Award No. N00014-14-1-0182. C. Cantoni acknowledges support by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 29 TC 30 Z9 30 U1 3 U2 53 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 19 PY 2015 VL 106 IS 3 AR 032601 DI 10.1063/1.4906205 PG 5 WC Physics, Applied SC Physics GA AZ7EF UT WOS:000348381000052 ER PT J AU Shen, X Ahmadi-Majlan, K Ngai, JH Wu, D Su, D AF Shen, Xuan Ahmadi-Majlan, K. Ngai, Joseph H. Wu, Di Su, Dong TI Interfacial structure in epitaxial perovskite oxides on (001) Ge crystal SO APPLIED PHYSICS LETTERS LA English DT Article ID BATIO3 THIN-FILMS; 2-STEP GROWTH TECHNIQUE; MISFIT DISLOCATIONS; DIELECTRIC-PROPERTIES; SRTIO3; STRAIN; FERROELECTRICITY; RELAXATION; BOUNDARIES; EVOLUTION AB We investigated the interfacial structure of hetero-epitaxial SrZr0.68Ti0.32O3 thin film deposited on (001) Ge single crystal via transmission electron microscopy (TEM). The results from high-resolution scanning TEM and electron energy-loss spectroscopy show an atomically abrupt interface without secondary phase. We found misfit dislocations with Burgers vector of 1/2a < 111 > and threading dislocations with Burgers vector of a < 100 >. Furthermore, we observed the coupling between dislocation half-loop and anti-phase boundary induced by the lattice terrace of Ge along < 100 > direction and their decoupling after annealing. We proposed models based on half-loop theory to interpret the coupling and the dislocation reactions. (C) 2015 AIP Publishing LLC. C1 [Shen, Xuan; Wu, Di] Nanjing Univ, Coll Engn & Appl Sci, Collaborat Innovat Ctr Adv Mat, Natl Lab Solid State Microstruct, Nanjing 210093, Jiangsu, Peoples R China. [Shen, Xuan; Wu, Di] Nanjing Univ, Coll Engn & Appl Sci, Collaborat Innovat Ctr Adv Mat, Dept Mat Sci & Engn, Nanjing 210093, Jiangsu, Peoples R China. [Shen, Xuan; Su, Dong] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Ahmadi-Majlan, K.; Ngai, Joseph H.] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA. RP Su, D (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. EM dsu@bnl.gov RI Wu, Di/B-1147-2008; Su, Dong/A-8233-2013 OI Wu, Di/0000-0003-3619-1411; Su, Dong/0000-0002-1921-6683 FU U.S. Department of Energy, Office of Basic Energy Sciences [DEAC02-98CH10886]; China Scholarship Council; Brookhaven National Laboratory; University of Texas at Arlington; National Key Basic Research Program of China [2015CB921203] FX Electron microscopy studies were performed at the Center for Functional Nanomaterials, Brookhaven National Laboratory supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DEAC02-98CH10886. X.S. is grateful for the financial support of the China Scholarship Council and Brookhaven National Laboratory for his exchange program. K.A.-M. and J.H.N. acknowledge the support of The University of Texas at Arlington. D.W. thanks National Key Basic Research Program of China (2015CB921203) for support. We thank Dr. Woodhead for the proof reading. NR 36 TC 2 Z9 2 U1 2 U2 36 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 19 PY 2015 VL 106 IS 3 AR 032903 DI 10.1063/1.4906430 PG 5 WC Physics, Applied SC Physics GA AZ7EF UT WOS:000348381000056 ER PT J AU Si, WD Zhang, C Shi, XY Ozaki, T Jaroszynski, J Li, Q AF Si, Weidong Zhang, Cheng Shi, Xiaoya Ozaki, Toshinori Jaroszynski, Jan Li, Qiang TI Grain boundary junctions of FeSe0.5Te0.5 thin films on SrTiO3 bi-crystal substrates SO APPLIED PHYSICS LETTERS LA English DT Article ID HIGH MAGNETIC-FIELDS; T-C SUPERCONDUCTORS AB degrees Grain boundary junctions were fabricated in the epitaxial FeSe0.5Te0.5 thin films on [001] tilt SrTiO3 bi-crystal substrates with a CeO2 buffer layer. Critical current densities across the junctions with different mis-orientation angles of 4 degrees, 7 degrees, 15 degrees, and 24 degrees were measured at magnetic fields up to 30 T. It was found that the 4 degrees and 7 degrees junctions carry critical current densities comparable to that of the intra-grain film while those of the 15 degrees and 24 degrees junctions were suppressed drastically. A critical mis-orientation angle of around 9 degrees was identified that separates the strong coupling region from the weak link region. We found that the critical current densities across the grain boundary with a 24 degrees mis-orientation angle are modulated by the magnetic field, indicating a Josephson Effect. This junction is estimated to be in the intermediate-size regime with an effective transverse junction width L similar to 2.6-2.8 mu m and a Josephson penetration depth lambda(J) similar to 1.2 mu m. (C) 2015 AIP Publishing LLC. C1 [Si, Weidong; Zhang, Cheng; Shi, Xiaoya; Ozaki, Toshinori; Li, Qiang] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Jaroszynski, Jan] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. RP Li, Q (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. EM qiangli@bnl.gov RI Zhang, Cheng/R-6593-2016 OI Zhang, Cheng/0000-0001-6531-4703 FU U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Science and Engineering [DE-AC0298CH10886]; National Science Foundation [DMR-0654118]; State of Florida; U.S. Department of Energy FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Science and Engineering, under Contract No. DE-AC0298CH10886. A portion of this work was performed at the NHMFL, which was supported by National Science Foundation Cooperative Agreement No. DMR-0654118, the State of Florida, and the U.S. Department of Energy. NR 24 TC 0 Z9 0 U1 1 U2 24 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JAN 19 PY 2015 VL 106 IS 3 AR 032602 DI 10.1063/1.4906429 PG 4 WC Physics, Applied SC Physics GA AZ7EF UT WOS:000348381000053 ER PT J AU Collins, L Jesse, S Kilpatrick, JI Tselev, A Okatan, MB Kalinin, SV Rodriguez, BJ AF Collins, Liam Jesse, Stephen Kilpatrick, Jason I. Tselev, Alexander Okatan, M. Baris Kalinin, Sergei V. Rodriguez, Brian J. TI Kelvin probe force microscopy in liquid using electrochemical force microscopy SO Beilstein Journal of Nanotechnology LA English DT Article DE diffuse charge dynamics; double layer charging; electrochemical force microscopy; electrochemistry; Kelvin probe force microscopy ID NANOSCALE; SURFACE; INTERFACES; DYNAMICS; WATER AB Conventional closed loop-Kelvin probe force microscopy (KPFM) has emerged as a powerful technique for probing electric and transport phenomena at the solid-gas interface. The extension of KPFM capabilities to probe electrostatic and electrochemical phenomena at the solid-liquid interface is of interest for a broad range of applications from energy storage to biological systems. However, the operation of KPFM implicitly relies on the presence of a linear lossless dielectric in the probe-sample gap, a condition which is violated for ionically-active liquids (e.g., when diffuse charge dynamics are present). Here, electrostatic and electrochemical measurements are demonstrated in ionically-active (polar isopropanol, milli-Q water and aqueous NaCl) and ionically-inactive (non-polar decane) liquids by electrochemical force microscopy (EcFM), a multidimensional (i.e., bias-and time-resolved) spectroscopy method. In the absence of mobile charges (ambient and non-polar liquids), KPFM and EcFM are both feasible, yielding comparable contact potential difference (CPD) values. In ionically-active liquids, KPFM is not possible and EcFM can be used to measure the dynamic CPD and a rich spectrum of information pertaining to charge screening, ion diffusion, and electrochemical processes (e.g., Faradaic reactions). EcFM measurements conducted in isopropanol and milli-Q water over Au and highly ordered pyrolytic graphite electrodes demonstrate both sample-and solvent-dependent features. Finally, the feasibility of using EcFM as a local force-based mapping technique of material-dependent electrostatic and electrochemical response is investigated. The resultant high dimensional dataset is visualized using a purely statistical approach that does not require a priori physical models, allowing for qualitative mapping of electrostatic and electrochemical material properties at the solid-liquid interface. C1 [Collins, Liam; Rodriguez, Brian J.] Univ Coll Dublin, Sch Phys, Dublin 4, Ireland. [Collins, Liam; Kilpatrick, Jason I.; Rodriguez, Brian J.] Univ Coll Dublin, Conway Inst Biomol & Biomed Res, Dublin 4, Ireland. [Jesse, Stephen; Tselev, Alexander; Okatan, M. Baris; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Kalinin, Sergei V.] Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA. RP Rodriguez, BJ (reprint author), Univ Coll Dublin, Sch Phys, Dublin 4, Ireland. EM Brian.Rodriguez@ucd.ie RI Tselev, Alexander/L-8579-2015; Collins, Liam/A-3833-2016; Kalinin, Sergei/I-9096-2012; Jesse, Stephen/D-3975-2016; Okatan, M. Baris/E-1913-2016; OI Tselev, Alexander/0000-0002-0098-6696; Collins, Liam/0000-0003-4946-9195; Kalinin, Sergei/0000-0001-5354-6152; Jesse, Stephen/0000-0002-1168-8483; Okatan, M. Baris/0000-0002-9421-7846; Kilpatrick, Jason/0000-0002-8675-4262 FU UCD Research [R11335, SF938]; NANOREMEDIES under the Programme for Research in Third Level Institutions Cycle 5; European Regional Development Fund; Office of Basic Energy Sciences, U.S. Department of Energy [CNMS2012-036, CNMS2013-339] FX This publication has emanated from research conducted with the financial support of UCD Research (R11335 and SF938) and NANOREMEDIES, which is funded under the Programme for Research in Third Level Institutions Cycle 5 and co-funded by the European Regional Development Fund. This research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (CNMS2012-036 and CNMS2013-339). NR 61 TC 6 Z9 6 U1 9 U2 51 PU BEILSTEIN-INSTITUT PI FRANKFURT AM MAIN PA TRAKEHNER STRASSE 7-9, FRANKFURT AM MAIN, 60487, GERMANY SN 2190-4286 J9 BEILSTEIN J NANOTECH JI Beilstein J. Nanotechnol. PD JAN 19 PY 2015 VL 6 BP 201 EP 214 DI 10.3762/bjnano.6.19 PG 14 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA CA5HS UT WOS:000348940100001 PM 25671164 ER PT J AU Bauer, M Cohen, T Hill, R Solon, MP AF Bauer, Martin Cohen, Timothy Hill, Richard J. Solon, Mikhail P. TI Soft collinear effective theory for heavy WIMP annihilation SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Beyond Standard Model; Cosmology of Theories beyond the SM; Resummation; Effective field theories ID MINIMAL DARK-MATTER; STANDARD MODEL; BREAKING; SUPERSYMMETRY; SCATTERING; OPERATORS; SYMMETRY AB In a large class of models for Weakly Interacting Massive Particles (WIMPs), the WIMP mass M lies far above the weak scale m (W) . This work identifies universal Sudakov-type logarithms similar to alpha log(2)(2 M/m (W) ) that spoil the naive convergence of perturbation theory for annihilation processes. An effective field theory (EFT) framework is presented, allowing the systematic resummation of these logarithms. Another impact of the large separation of scales is that a long-distance wavefunction distortion from electroweak boson exchange leads to observable modifications of the cross section. Careful accounting of momentum regions in the EFT allows the rigorous disentanglement of this so-called Sommerfeld enhancement from the short-distance hard annihilation process. The WIMP is described as a heavy-particle field, while the electroweak gauge bosons are treated as soft and collinear fields. Hard matching coefficients are computed at renormalization scale mu similar to 2 M , then evolved down to mu similar to m (W) , where electroweak symmetry breaking is incorporated and the matching onto the relevant quantum mechanical Hamiltonian is performed. The example of an SU(2) (W) triplet scalar dark matter candidate annihilating to line photons is used for concreteness, allowing the numerical exploration of the impact of next-to-leading order corrections and log resummation. For M similar or equal to 3 TeV, the resummed Sommerfeld enhanced cross section is reduced by a factor of similar to 3 with respect to the treelevel fixed order result. C1 [Bauer, Martin; Hill, Richard J.; Solon, Mikhail P.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Bauer, Martin; Hill, Richard J.; Solon, Mikhail P.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Bauer, Martin] Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. [Cohen, Timothy] Princeton Univ, Dept Phys, Princeton, NJ 08544 USA. [Cohen, Timothy] Inst Adv Study, Sch Nat Sci, Princeton, NJ 08540 USA. [Cohen, Timothy] Univ Oregon, Inst Theoret Sci, Eugene, OR 97403 USA. [Cohen, Timothy] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Solon, Mikhail P.] Univ Calif Berkeley, Berkeley Ctr Theoret Phys, Dept Phys, Berkeley, CA 94270 USA. [Solon, Mikhail P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94270 USA. RP Bauer, M (reprint author), Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. EM m.bauer@thphys.uni-heidelberg.de; tcohen@uoregon.edu; richardhill@uchicago.edu; mpsolon@berkeley.edu RI Hill, Richard/C-8820-2017 OI Hill, Richard/0000-0003-1982-589X FU Alexander von Humboldt Foundation; DoE [DE-AC02-76SF00515, DE-FG02-13ER41958]; LHC Theory Initiative Postdoctoral Fellowship under the National Science Foundation [PHY-0969510]; National Science Foundation [NSF PHY11-25915]; U. S. Department of Energy [DE-AC02-05CH11231] FX We thank Thomas Becher, Matthew Dolan, Matthias Neubert, Michael Peskin, Jon Walsh, Hua-Xing Zhu for insightful discussions. In particular, we are grateful to Mariangela Lisanti, Aaron Pierce, and Tracy Slatyer for permission to use the Sommerfeld enhancement code developed for [41]. MB is supported by the Alexander von Humboldt Foundation. MB thanks SLAC, where some of this research was performed, for support and hospitality. TC is supported by DoE contract number DE-AC02-76SF00515 and by an LHC Theory Initiative Postdoctoral Fellowship, under the National Science Foundation grant PHY-0969510. TC thanks the KITP in Santa Barbara where some of this research was performed and for the support from the National Science Foundation under Grant No. NSF PHY11-25915. TC also thanks the MITP in Mainz where additional work was performed. RH is supported by the DOE Grant No. DE-FG02-13ER41958. TC and RH thank the Aspen Center for Physics where this work was initiated for the support under NSF Grant No. NSF PHY10-66293. MS acknowledges support from a Bloomenthal Fellowship at the University of Chicago and from the Office of Science, Office of High Energy Physics, of the U. S. Department of Energy under contract DE-AC02-05CH11231. NR 97 TC 17 Z9 17 U1 1 U2 7 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN 19 PY 2015 IS 1 AR 099 DI 10.1007/JHEP01(2015)099 PG 44 WC Physics, Particles & Fields SC Physics GA AZ6PT UT WOS:000348342000001 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Ochesanu, S Rougny, R Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Daci, N Heracleous, N Keaveney, J Lowette, S Maes, M Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Dobur, D Favart, L Gay, A Grebenyuk, A Leonard, A Mohammadi, A Pernie, L Randle-conde, A Reis, T Seva, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Zenoni, F Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Crucy, S Dildick, S Fagot, A Garcia, G Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Salva Diblen, S Sigamani, M Strobbe, N Thyssen, F Tytgat, M Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Nuttens, C Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, G Alda, WL Alves, GA Brito, L Martins, MC Martins, TD Molina, J Mora Herrera, C Pol, ME Rebello Teles, P Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santaolalla, J Santoro, A Sznajder, A Tonelli Manganote, E Pereira, AV Bernardes, C Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Novaes, SF Padula, SS Aleksandrov, A Genchev, V Hadjiiska, R Iaydjiev, P Marinov, A Piperov, S Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, C Plestina, R Romeo, F Tao, J Wang, Z Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, S Wang, D Xu, Z Zou, W Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Bodlak, M Finger, M Finger, M Assran, Y Elgammal, S Kamel, AE Radi, A Kadastik, M Murumaa, M Raidal, M Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, M Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Talvitie, J Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, J Favaro, C Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Rander, J Rosowsky, A Titov, M Baffioni, S Beaudette, F Busson, P Chapon, E Charlot, C Dahms, T Dalchenko, M Dobrzynski, L Filipovic, N Florent, A de Cassagnac, RG Mastrolorenzo, L Mine, P Naranjo, I Nguyen, M Ochando, C Ortona, G Paganini, P Regnard, S Salerno, R Sauvan, JB Sirois, Y Veelken, C Yilmaz, Y Zabi, A Agram, JL Andrea, J Aubin, A Bloch, D Brom, JM Chabert, E Collard, C Conte, E Fontaine, JC Gele, D Goerlach, U Goetzmann, C Bihan, AC Skovpen, K Van Hove, P Gadrat, S Beauceron, S Beaupere, N Bernet, C Boudoul, G Bouvier, E Brochet, S Montoya, CAC Chasserat, J Chierici, R Contardo, D Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Perries, S Alvarez, JDR Sabes, D Sgandurra, L Sordini, V Vander Donckt, M Verdier, P Viret, S Xiao, H Rurua, L Autermann, C Beranek, S Bontenackels, M Edelhoff, M Feld, L Heister, A Klein, K Lipinski, M Ostapchuk, A Preuten, M Raupach, F Sammet, J Schael, S Schulte, JF Weber, H Wittmer, B Zhukov, V Ata, M Brodski, M Dietz-Laursonn, E Duchardt, D Erdmann, M Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Millet, P Olschewski, M Padeken, K Papacz, P Reithler, H Schmitz, SA Sonnenschein, L Teyssier, D Thuer, S Weber, M Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Ahmad, WH Hoehle, F Kargoll, B Kress, T Kuessel, Y Kunsken, A Lingemann, J Nowack, A Nugent, IM Pooth, O Stahl, A Martin, MA Asin, I Bartosik, N Behr, J Behrens, U Bell, AJ Bethani, A Borras, K Burgmeier, A Cakir, A Calligaris, L Campbell, A Choudhury, S Costanza, F Pardos, CD Dolinska, G Dooling, S Dorland, T Eckerlin, G Eckstein, D Eichhorn, T Flucke, G Garcia, JG Geiser, A Gunnellini, P Hauk, J Hempel, M Jung, H Kalogeropoulos, A Kasemann, M Katsas, P Kieseler, J Kleinwort, C Korol, I Krucker, D Lange, W Leonard, J Lipka, K Lobanov, A Lohmann, W Lutz, B Mankel, R Marfin, I Melzer-Pellmann, IA Meyer, AB Mittag, G Mnich, J Mussgiller, A Naumann-Emme, S Nayak, A Ntomari, E Perrey, H Pitzl, D Placakyte, R Raspereza, A Cipriano, PMR Roland, B Ron, E Sahin, MO Salfeld-Nebgen, J Saxena, P Schoerner-Sadenius, T Schroder, M Seitz, C Spannagel, S Trevino, ADRV Walsh, R Wissing, C Blobel, V Vignali, MC Draeger, AR Erfle, J Garutti, E Goebel, K Gorner, M Haller, J Hoffmann, M Hoeing, RS Junkes, A Kirschenmann, H Klanner, R Kogler, R Lange, J Lapsien, T Lenz, T Marchesini, I Ott, J Peiffer, T Perieanu, A Pietsch, N Poehlsen, J Poehlsen, T Rathjens, D Sander, C Schettler, H Schleper, P Schlieckau, E Schmidt, A Seidel, M Sola, V Stadie, H Steinbruck, G Troendle, D Usai, E Vanelderen, L Vanhoefer, A Barth, C Baus, C Berger, J Boser, C Butz, E Chwalek, T De Boer, W Descroix, A Dierlamm, A Feindt, M Frensch, F Giffels, M Gilbert, A Hartmann, F Hauth, T Husemann, U Katkov, I Kornmayer, A Lobelle Pardo, P Mozer, M Muller, T Muller, T Nurnberg, A Quast, G Rabbertz, K Rocker, S Simonis, H Stober, FM Ulrich, R Wagner-Kuhr, J Wayand, S Weiler, T Wolf, R Anagnostou, G Daskalakis, G Geralis, T Giakoumopoulou, VA Kyriakis, A Loukas, D Markou, A Markou, C Psallidas, A Topsis-Giotis, I Agapitos, A Kesisoglou, S Panagiotou, A Saoulidou, N Stiliaris, E Aslanoglou, X Evangelou, I Flouris, G Foudas, C Kokkas, P Manthos, N Papadopoulos, I Paradas, E Strologas, J Bencze, G Hajdu, C Hidas, P Horvath, D Sikler, F Veszpremi, V Vesztergombi, G Zsigmond, AJ Beni, N Czellar, S Karancsi, J Molnar, J Palinkas, J Szillasi, Z Makovec, A Raics, P Trocsanyi, ZL Ujvari, B Swain, SK Beri, SB Bhatnagar, V Gupta, R Bhawandeep, U Kalsi, AK Kaur, M Kumar, R Mittal, M Nishu, N Singh, JB Kumar, A Kumar, A Ahuja, S Bhardwaj, A Choudhary, BC Kumar, A Malhotra, S Naimuddin, M Ranjan, K Sharma, V Banerjee, S Bhattacharya, S Chatterjee, K Dutta, S Gomber, B Jain, S Jain, S Khurana, R Modak, A Mukherjee, S Roy, D Sarkar, S Sharan, M Abdulsalam, A Dutta, D Kumar, V Mohanty, AK Pant, LM Shukla, P Topkar, A Aziz, T Banerjee, S Bhowmik, S Chatterjee, R Dewanjee, R Dugad, S Ganguly, S Ghosh, S Guchait, M Gurtu, A Kole, G Kumar, S Maity, M Majumder, G Mazumdar, K Mohanty, GB Parida, B Sudhakar, K Wickramage, N Bakhshiansohi, H Behnamian, H Etesami, S Fahim, A Goldouzian, R Khakzad, M Najafabadi, MM Naseri, M Mehdiabadi, SP Hosseinabadi, FR Safarzadeh, B Zeinali, M Felcini, M Grunewald, M Abbrescia, M Calabria, C Chhibra, S Colaleo, A Creanza, D De Filippis, N De Palma, M Fiore, L Iaselli, G Maggi, G Maggi, M My, S Nuzzo, S Pompili, A Pugliese, G Radogna, R Selvaggi, G Sharma, A Silvestris, L Venditti, R Verwilligen, P Abbiendi, G Benvenuti, AC Bonacorsi, D Braibant-Giacomelli, S Brigliadori, L Campanini, R Capiluppi, P Castro, A Cavallo, FR Codispoti, G Cuffiani, M Dallavalle, GM Fabbri, F Fanfani, A Fasanella, D Giacomelli, P Grandi, 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Taylor, D. Vuosalo, C. Woods, N. TI Search for disappearing tracks in proton-proton collisions at root s=8 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering; Supersymmetry; Exotics ID PARTICLES; LEVEL AB A search is presented for long-lived charged particles that decay within the CMS detector and produce the signature of a disappearing track. Disappearing tracks are identified as those with little or no associated calorimeter energy deposits and with missing hits in the outer layers of the tracker. The search uses proton-proton collision data recorded at root s = 8 TeV that corresponds to an integrated luminosity of 19.5 fb(-1). The results of the search are interpreted in the context of the anomaly-mediated supersymmetry breaking (AMSB) model. The number of observed events is in agreement with the background expectation, and limits are set on the cross section of direct electroweak chargino production in terms of the chargino mass and mean proper lifetime. At 95% confidence level, AMSB models with a chargino mass less than 260 GeV, corresponding to a mean proper lifetime of 0.2 ns, are excluded. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hartl, C.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Kiesenhofer, W.; Knuenz, V.; Krammer, M.; Kraetschmer, I.; Liko, D.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, H.; Schoefbeck, R.; Strauss, J.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] Inst Hochenergiephys OeAW, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. 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[Ata, M.; Brodski, M.; Dietz-Laursonn, E.; Duchardt, D.; Erdmann, M.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Millet, P.; Olschewski, M.; Padeken, K.; Papacz, P.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Teyssier, D.; Thueer, S.; Weber, M.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Kuensken, A.; Nowack, A.; Nugent, I. M.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B 3, Aachen, Germany. [Martin, M. Aldaya; Asin, I.; Bartosik, N.; Behr, J.; Behrens, U.; Bell, A. J.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. Diez; Dolinska, G.; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Garcia, J. 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S.; Junkes, A.; Kirschenmann, H.; Klanner, R.; Kogler, R.; Lange, J.; Lapsien, T.; Lenz, T.; Marchesini, I.; Ott, J.; Peiffer, T.; Perieanu, A.; Pietsch, N.; Poehlsen, J.; Poehlsen, T.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Seidel, M.; Sola, V.; Stadie, H.; Steinbrueck, G.; Troendle, D.; Usai, E.; Vanelderen, L.; Vanhoefer, A.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Frensch, F.; Giffels, M.; Gilbert, A.; Hartmann, F.; Hauth, T.; Husemann, U.; Katkov, I.; Kornmayer, A.; Lobelle Pardo, P.; Mozer, M. U.; Mueller, T.; Mueller, Th.; Nuernberg, A.; Quast, G.; Rabbertz, K.; Roecker, S.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Wolf, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, Inst Nucl & Particle Phys, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, M.; Kumar, R.; Mittal, M.; Nishu, N.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Sharma, V.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Jain, Sa.; Jain, Sh.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Kumar, V.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Mumbai 400085, Maharashtra, India. [Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res, Bombay 400005, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Selvaggi, G.; Sharma, A.; Silvestris, L.; Venditti, R.; Verwilligen, P.] INFN Sezione Bari, Bari, Italy. [Abbrescia, M.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T. .; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T. .; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Giordano, F.] CSFNSM, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gallo, E.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Ferretti, R.; Ferro, F.; Lo Vetere, M.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Ferretti, R.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Dinardo, M. 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[Bisello, D.; Branca, A.; Carlin, R.; Dall'Osso, M.; Galanti, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.] Univ Trento, Trento, Italy. [Gabusi, M.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Aleksandrov, A.; Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Longo, E.; Margaroli, F.; Micheli, F.; Organtini, G.; Rahatlou, S.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Biino, C.; Cartiglia, N.; Demaria, N.; Mariotti, C.; Maselli, S.; Musich, M.; Pastrone, N.; Pelliccioni, M.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Degano, A.; Migliore, E.; Monaco, V.; Pacher, L.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Torino, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Dept Chem, Chunchon 200701, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, T. J.; Ryu, M. S.] Chonbuk Natl Univ, Jeonju, South Korea. [Kim, J. Y.; Moon, D. H.; Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, I. C.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Komaragiri, J. R.; Ali, M. A. B. Md] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] Centro Investigac & Estudios Avanzados IPN, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autnoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beiro Da Cruz E Silva, C.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] State Atom Energy Commiss, Inst Theoret & Expt Phys, Moscow, Russia. [Andreev, V.; Kirakosyan, M.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Zhukov, V.; Belyaev, A.; Boos, E.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; F. de Trocniz, J.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, Santander, Spain. [Rabady, D.; Pernie, L.; Genchev, V.; Boudoul, G.; Contardo, D.; Lingemann, J.; Hartmann, F.; Kornmayer, A.; Mohanty, A. K.; Radogna, R.; Silvestris, L.; Giordano, F.; Gennai, S.; Gerosa, R.; Lucchini, M. T.; Marzocchi, B.; Di Guida, S.; Meola, S.; Paolucci, P.; Ciangottini, D.; Spiezia, A.; Donato, S.; Palla, F.; Micheli, F.; Traczyk, P.; Casasso, S.; Finco, L.; Candelise, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Magini, N.; Malgeri, L.; Mannelli, M.; Marrouche, J.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Orsini, L.; Pape, L.; Perez, E.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pimia, M.; Piparo, D.; Plagge, M.; Racz, A.; Rovere, M.; Sakulin, H.; Schafer, C.; Schwick, C.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Tsirou, A.; Wardle, N.; Wohri, H. K.; Wollny, H.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Buchmann, M. A.; Casal, B.; Chanon, N.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Hits, D.; Hoss, J.; Lustermann, W.; Mangano, B.; Marini, A. C.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Mohr, N.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pauss, F.; Perrozzi, L.; Peruzzi, M.; Quittnat, M.; Rebane, L.; Rossini, M.; Starodumov, A.; Takahashi, M.; Theofilatos, K.; Wallny, R.; Weber, H. A.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Canelli, M. F.; Chiochia, V.; De Cosa, A.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Mejias, B. Millan; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Chang, P.; Chang, Y. H.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Liu, Y. F.; Lu, R. -S.; Petrakou, E.; Tzeng, Y. M.; Wilken, R.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Ozdemir, K.; Polatoz, A.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Sekmen, S.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle East Tech Univ, Ankara, Turkey. [Guelmez, E.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Phys & Technol Inst, Ctr Nat Sci, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-storey, S. Seif; Senkin, S.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Bell, K. W.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Dauncey, P.; Davies, G.; Della Negra, M.; Dunne, P.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Mathias, B.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Imperial Coll, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.; Wu, Z.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Lawson, P.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Rikova, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Tu, Y.; Vartak, A.; Welke, C.; Wurthwein, F.; Yagil, A.] Univ Calif San Diego, San Diego, CA 92103 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Incandela, J.; Justus, C.; Mccoll, N.; Richman, J.; Stuart, D.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Krohn, M.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Skinnari, L.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Grunendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kreis, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Sharma, S.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Yang, F.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carver, M.; Curry, D.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Field, R. D.; Fisher, M.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Snowball, M.; Sperka, D.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Clarida, W.; Dilsiz, K.; Haytmyradov, M.; Merlo, J. -P.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Penzo, A.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Gray, J.; Kenny, R. P. I. I. I.; Majumder, D.; Malek, M.; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Chakaberia, I.; Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Skhirtladze, N.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Belloni, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD USA. [Apyan, A.; Barbieri, R.; Busza, W.; Cali, I. A.; Chan, M.; Matteo, L. Di; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Nourbakhsh, S.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, University, MS 38677 USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Ratnikov, F.; Snow, G. R.; Zvada, M.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Coll Buffalo, Buffalo, NY USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Lynch, S.; Marinelli, N.; Musienko, Y.; Pearson, T.; Planer, M.; Ruchti, R.; Smith, G.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Pirou, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ USA. [Brownson, E.; Malik, S.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Barnes, V. E.; Benedetti, D.; Bortoletto, D.; De Mattia, M.; Gutay, L.; Hu, Z.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Zablocki, J.] Purdue Univ, W Lafayette, IN USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Hindrichs, O.; Khukhunaishvili, A.; Korjenevski, S.; Petrillo, G.; Vishnevskiy, D.] Univ Rochester, Rochester, NY 14627 USA. [Ciesielski, R.; Demortier, L.; Goulianos, K.; Mesropian, C.] Rockefeller Univ, New York, NY USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Kaplan, S.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] State Univ New Jersey, Rutgers, Piscataway, NJ USA. [Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Hernandez, A. Castaneda; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Krutelyov, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Rose, A.; Safonov, A.; Suarez, I.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kovitanggoon, K.; Kunori, S.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Dodd, L.; Duric, S.; Friis, E.; Hall-Wilton, R.; Herndon, M.; Herv, A.; Klabbers, P.; Lanaro, A.; Lazaridis, C.; Levine, A.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. H.; Taylor, D.; Vuosalo, C.; Woods, N.] Univ Wisconsin, Madison, WI USA. [Fruehwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C. -E.] Vienna Univ Technol, Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, Brazil. [Assran, Y.] Suez Univ, Suez, Egypt. [Elgammal, S.] British Univ Egypt, Cairo, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. Ain Shams Univ, Cairo, Egypt. [Radi, A.] Sultan Qaboos Univ, Muscat, Oman. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ, Haute Alsace, Mulhouse, France. [Hempel, M.; Lohmann, W.; Marfin, I.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Bhowmik, S.; Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islam Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.; Squillacioti, P.] Univ Studi Siena, Siena, Italy. [Moon, C. S.] Ctr Natl Rech Scientif CNRS IN2P3, Paris, France. [Kim, V.] St Petersburg State Polytechn Univ, St Petersburg, Russia. [Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ quot Moscow Engn Phys Inst quo, Moscow, Russia. [Adzic, P.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Colafranceschi, S.] Univ Roma, FacoltA Ingn, Rome, Italy. [Rolandi, G.] Scuola Normale Sezione dellINFN, Pisa, Italy. [Nageli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Amsler, C.; Bakirci, M. N.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Gamsizkan, H.] Anadolu Univ, Eskisehir, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Ocalan, K.] Necmettin Erbakan Univ, Konya, Turkey. [Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, T.] Yildiz Tech Univ, Istanbul, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Bilki, B.] Argonne Natl Lab, Argonne, IL USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Bouhali, O.] Texas A&M Univ, College Stn, TX 77843 USA. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Sznajder, Andre/L-1621-2016; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Konecki, Marcin/G-4164-2015; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Cerrada, Marcos/J-6934-2014; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Della Ricca, Giuseppe/B-6826-2013; Chinellato, Jose Augusto/I-7972-2012; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Seixas, Joao/F-5441-2013; Vilela Pereira, Antonio/L-4142-2016; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; Matorras, Francisco/I-4983-2015; TUVE', Cristina/P-3933-2015; Dudko, Lev/D-7127-2012; KIM, Tae Jeong/P-7848-2015; Paganoni, Marco/A-4235-2016; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Calvo Alamillo, Enrique/L-1203-2014; Flix, Josep/G-5414-2012; candelise, vieri/H-2195-2015; Montanari, Alessandro/J-2420-2012; Hernandez Calama, Jose Maria/H-9127-2015; ciocci, maria agnese /I-2153-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Benussi, Luigi/O-9684-2014; Lo Vetere, Maurizio/J-5049-2012; Ragazzi, Stefano/D-2463-2009; Grandi, Claudio/B-5654-2015; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; D'Alessandro, Raffaello/F-5897-2015; Lokhtin, Igor/D-7004-2012; Wulz, Claudia-Elisabeth/H-5657-2011; Petrushanko, Sergey/D-6880-2012; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Cavallo, Nicola/F-8913-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Calderon, Alicia/K-3658-2014; VARDARLI, Fuat Ilkehan/B-6360-2013; Sen, Sercan/C-6473-2014; Paulini, Manfred/N-7794-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; OI Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Konecki, Marcin/0000-0001-9482-4841; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Cerrada, Marcos/0000-0003-0112-1691; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Della Ricca, Giuseppe/0000-0003-2831-6982; Chinellato, Jose Augusto/0000-0002-3240-6270; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Matorras, Francisco/0000-0003-4295-5668; TUVE', Cristina/0000-0003-0739-3153; Dudko, Lev/0000-0002-4462-3192; KIM, Tae Jeong/0000-0001-8336-2434; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Calvo Alamillo, Enrique/0000-0002-1100-2963; Flix, Josep/0000-0003-2688-8047; Montanari, Alessandro/0000-0003-2748-6373; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Benussi, Luigi/0000-0002-2363-8889; Lo Vetere, Maurizio/0000-0002-6520-4480; Ragazzi, Stefano/0000-0001-8219-2074; Grandi, Claudio/0000-0001-5998-3070; Rovelli, Tiziano/0000-0002-9746-4842; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Sen, Sercan/0000-0001-7325-1087; Paulini, Manfred/0000-0002-6714-5787; Heath, Helen/0000-0001-6576-9740 FU BMWFW (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COL-CIENCIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia); ERC IUT (Estonia); ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Republic of Korea); WCU (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (U.S.A.); NSF (U.S.A.); Marie-Curie program; European Research Council; EPLANET (European Union); Leventis Foundation; A.P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS program of Foundation for Polish Science; European Union, Regional Development Fund; Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR project (Italy) [20108T4XTM]; Thalis program; Aristeia program; EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COL-CIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT, and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE, and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR, and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (U.S.A.). Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A.P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF; and the National Priorities Research Program by Qatar National Research Fund.; Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; and the National Priorities Research Program by Qatar National Research Fund. NR 43 TC 9 Z9 9 U1 11 U2 64 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN 19 PY 2015 IS 1 AR 096 DI 10.1007/JHEP01(2015)096 PG 43 WC Physics, Particles & Fields SC Physics GA AZ6PS UT WOS:000348341900001 ER PT J AU Kasakov, S Zhao, C Barath, E Chase, ZA Fulton, JL Camaioni, DM Vjunov, A Shi, H Lercher, JA AF Kasakov, Stanislav Zhao, Chen Barath, Eszter Chase, Zizwe A. Fulton, John L. Camaioni, Donald M. Vjunov, Aleksei Shi, Hui Lercher, Johannes A. TI Glucose- and Cellulose-Derived Ni/C-SO3H Catalysts for Liquid Phase Phenol Hydrodeoxygenation SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE carbon support; IR spectroscopy; nanoparticles; phenol hydrodeoxygenation; X-ray absorption spectroscopy ID NICKEL NANOPARTICLES; AMORPHOUS-CARBON; NI NANOPARTICLES; METAL CATALYSTS; AQUEOUS-PHASE; ACID CATALYST; SO3H GROUPS; SOLID ACID; NI/HZSM-5; OIL AB Sulfonated carbons were explored as functionalized supports for Ni nanoparticles to hydrodeoxygenate (HDO) phenol. Both hexadecane and water were used as solvents. The dual-functional Ni catalysts supported on sulfonated carbon (Ni/C-SO3H) showed high rates for phenol hydrodeoxygenation in liquid hexadecane, but not in water. Glucose and cellulose were precursors to the carbon supports. Changes in the carbons resulting from sulfonation of the carbons resulted in variations of carbon sheet structures, morphologies and the surface concentrations of acid sites. While the C-SO3H supports were active for cyclohexanol dehydration in hexadecane and water, Ni/C-SO3H only catalysed the reduction of phenol to cyclohexanol in water. The state of 3-5 nm grafted Ni particles was analysed by in situ X-ray absorption spectroscopy. The results show that the metallic Ni was rapidly formed in situ without detectable leaching to the aqueous phase, suggesting that just the acid functions on Ni/C-SO3H are inhibited in the presence of water. Using in situ IR spectroscopy, it was shown that even in hexadecane, phenol HDO is limited by the dehydration step. Thus, phenol HDO catalysis was further improved by physically admixing C-SO3H with the Ni/C-SO3H catalyst to balance the two catalytic functions. The minimum addition of 7 wt% C-SO3H to the most active of the Ni/C-SO3H catalysts enabled nearly quantitative conversion of phenol and the highest selectivity (90%) towards cyclohexane in 6 h, at temperatures as low as 473 K, suggesting that the proximity to Ni limits the acid properties of the support. C1 [Kasakov, Stanislav; Zhao, Chen; Barath, Eszter; Lercher, Johannes A.] Tech Univ Munich, Dept Chem, D-85747 Garching, Germany. [Kasakov, Stanislav; Zhao, Chen; Barath, Eszter; Lercher, Johannes A.] Tech Univ Munich, Catalysis Res Ctr, D-85747 Garching, Germany. [Chase, Zizwe A.] Washington State Univ, Sch Chem & Biol Engn, Pullman, WA 99364 USA. [Fulton, John L.; Camaioni, Donald M.; Vjunov, Aleksei; Shi, Hui; Lercher, Johannes A.] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. RP Lercher, JA (reprint author), Tech Univ Munich, Dept Chem, D-85747 Garching, Germany. EM johannes.lercher@ch.tum.de RI Shi, Hui/J-7083-2014 FU US Department of Energy (DOE), Office of Basic Energy Sciences (BES), Division of Chemical Sciences, Geosciences and Biosciences; DOE [DE-AC05-76L01830, DE-AC02-06CH11357]; DOE/BES; Canadian Light Source; University of Washington; Advanced Photon Source FX This work was supported by the US Department of Energy (DOE), Office of Basic Energy Sciences (BES), Division of Chemical Sciences, Geosciences and Biosciences. Pacific Northwest National Laboratory is a multiprogram national laboratory operated for DOE by Battelle through Contract DE-AC05-76L01830. PNC/XSD facilities at the Advanced Photon Source, and research at these facilities, are supported by DOE/BES, the Canadian Light Source and its funding partners, the University of Washington, and the Advanced Photon Source. Use of the Advanced Photon Source, an Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory, was supported by the DOE under Contract No. DE-AC02-06CH11357. NR 49 TC 2 Z9 2 U1 7 U2 74 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD JAN 19 PY 2015 VL 21 IS 4 BP 1567 EP 1577 DI 10.1002/chem.201405242 PG 11 WC Chemistry, Multidisciplinary SC Chemistry GA AY9AI UT WOS:000347841500026 PM 25431188 ER PT J AU Mielke, SL Garrett, BC Fleming, DG Truhlar, DG AF Mielke, Steven L. Garrett, Bruce C. Fleming, Donald G. Truhlar, Donald G. TI Zero-point energy, tunnelling, and vibrational adiabaticity in the Mu + H-2 reaction SO MOLECULAR PHYSICS LA English DT Article DE vibrational adiabaticity; density of reactive states; cumulative reaction probability; Born-Oppenheimer diagonal correction; vibrational coupling; quantum mechanical reactive scattering; transition state; kinetic isotope effects; zero-point energy; tunnelling ID TRANSITION-STATE THEORY; CUMULATIVE REACTION PROBABILITIES; THERMAL RATE CONSTANTS; QUASICLASSICAL TRAJECTORY CALCULATIONS; POLYMER MOLECULAR-DYNAMICS; ATOM TRANSFER-REACTIONS; AB-INITIO CALCULATION; CHEMICAL-REACTIONS; REACTIVE SCATTERING; REACTION-RATES AB Isotopic substitution of muonium for hydrogen provides an unparalleled opportunity to deepen our understanding of quantum mass effects on chemical reactions. A recent topical review in this journal of the thermal and vibrationally state-selected reaction of Mu with H-2 raises a number of issues that are addressed here. We show that some earlier quantum mechanical calculations of the Mu + H-2 reaction, which are highlighted in this review, and which have been used to benchmark approximate methods, are in error by as much as 19% in the low-temperature limit. We demonstrate that an approximate treatment of the Born-Oppenheimer diagonal correction that was used in some recent studies is not valid for treating the vibrationally state-selected reaction. We also discuss why vibrationally adiabatic potentials that neglect bend zero-point energy are not a useful analytical tool for understanding reaction rates, and why vibrationally non-adiabatic transitions cannot be understood by considering tunnelling through vibrationally adiabatic potentials. Finally, we present calculations on a hierarchical family of potential energy surfaces to assess the sensitivity of rate constants to the quality of the potential surface. C1 [Mielke, Steven L.; Truhlar, Donald G.] Univ Minnesota, Dept Chem, Chem Theory Ctr, Minneapolis, MN 55455 USA. [Mielke, Steven L.; Truhlar, Donald G.] Univ Minnesota, Inst Supercomp, Minneapolis, MN 55455 USA. [Garrett, Bruce C.] Pacific NW Natl Lab, Phys Sci Div, Richland, WA 99352 USA. [Fleming, Donald G.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Fleming, Donald G.] Univ British Columbia, Dept Chem, Vancouver, BC, Canada. RP Mielke, SL (reprint author), Univ Minnesota, Dept Chem, Chem Theory Ctr, 207 Pleasant St SE, Minneapolis, MN 55455 USA. EM slmielke@umn.edu RI Truhlar, Donald/G-7076-2015 OI Truhlar, Donald/0000-0002-7742-7294 FU US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-FG02-86ER13579, DE-AC05-76RL01830] FX The US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences supported work at the University of Minnesota [grant number DE-FG02-86ER13579] and Pacific Northwest National Laboratory (PNNL) [contract number DE-AC05-76RL01830]. PNNL is a multiprogram national laboratory operated for DOE by Battelle Memorial Institute. NR 79 TC 9 Z9 9 U1 1 U2 38 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 0026-8976 EI 1362-3028 J9 MOL PHYS JI Mol. Phys. PD JAN 17 PY 2015 VL 113 IS 2 BP 160 EP 175 DI 10.1080/00268976.2014.951416 PG 16 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AW6DC UT WOS:000346358600005 ER PT J AU Kleidon, A Kravitz, B Renner, M AF Kleidon, Axel Kravitz, Ben Renner, Maik TI The hydrological sensitivity to global warming and solar geoengineering derived from thermodynamic constraints SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE hydrologic cycle; climate change; geoengineering; thermodynamics ID CLIMATE-CHANGE; ENTROPY PRODUCTION; SURFACE-ENERGY; HEAT-TRANSPORT; CYCLE; BALANCE; SYSTEM; EARTH AB We derive analytic expressions of the response of the hydrological cycle to surface warming from the surface energy balance in which turbulent heat fluxes are constrained by the thermodynamic limit of maximum power. For a given steady state temperature change, this approach predicts the transient and steady state response of surface energy partitioning and the hydrologic cycle. We show that the predicted hydrological sensitivities to greenhouse warming and solar geoengineering are comparable to the results from climate model simulations of the Geoengineering Model Intercomparison Project. Although not all effects can be explained, our approach nevertheless predicts the general trend as well as the magnitude of the changes in the global-scale hydrological cycle surprisingly well. This implies that much of the global-scale changes in the hydrologic cycle can be robustly predicted by the response of the thermodynamically constrained surface energy balance to altered radiative forcing. C1 [Kleidon, Axel; Renner, Maik] Max Planck Inst Biogeochem, Biospher Theory & Modelling Grp, D-07745 Jena, Germany. [Kravitz, Ben] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. RP Kleidon, A (reprint author), Max Planck Inst Biogeochem, Biospher Theory & Modelling Grp, D-07745 Jena, Germany. EM akleidon@bgc-jena.mpg.de RI Kleidon, Axel/O-7843-2014; OI Kleidon, Axel/0000-0002-3798-0730; Renner, Maik/0000-0002-2992-8414; Kravitz, Ben/0000-0001-6318-1150 FU Fund for Innovative Climate and Energy Research (FICER); U.S. Department of Energy [DE-AC05-76RL01830] FX We thank two anonymous reviewers for their helpful comments. Ben Kravitz is supported by the Fund for Innovative Climate and Energy Research (FICER). The Pacific Northwest National Laboratory is operated for the U.S. Department of Energy by Battelle Memorial Institute under contract DE-AC05-76RL01830. We thank all participants of the Geoengineering Model Intercomparison Project and their model development teams, CLIVAR/WCRP Working Group on Coupled Modeling for endorsing GeoMIP, and the scientists managing the Earth System Grid data nodes who have assisted with making GeoMIP output available. NR 23 TC 12 Z9 12 U1 1 U2 18 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JAN 16 PY 2015 VL 42 IS 1 BP 138 EP 144 DI 10.1002/2014GL062589 PG 7 WC Geosciences, Multidisciplinary SC Geology GA CA6PE UT WOS:000349036500019 ER PT J AU Couture, A Casten, RF Cakirli, RB AF Couture, A. Casten, R. F. Cakirli, R. B. TI Extended tests of an SU(3) partial dynamical symmetry SO PHYSICAL REVIEW C LA English DT Article AB Background: A recent survey of well-deformed rare earth nuclei showed that B(E2) values from the gamma band to the ground band could be explained rather well by a parameter-free description in terms of a partial dynamical symmetry (PDS). Purpose: Our purpose here is to extend this study to deformed and transitional nuclei in the actinide and A similar to 100 regions to determine if the success of the PDS description is general in medium-and heavy-mass nuclei and to investigate further where it breaks down. Method: As with the previous study we study the empirical relative B(E2: gamma to ground) values in comparison to a pure rotor (Alaga) model and to the SU(3) PDS. Results: The data for the actinides, albeit sparser than in the rare-earth region, are reasonably well accounted for by the PDS but with systematic discrepancies. For the Mo isotopes, the PDS improves on the Alaga rules but largely fails to account for the data. Conclusions: As in the rare earths, the parameter-free PDS gives improved predictions compared to the Alaga rules for the actinides. The differences between the PDS predictions and the data are shown to point directly to specific mixing effects. In the Mo isotopes, their transitional character is directly seen in the large deviations of the B(E2) values from the PDS in the direction of the selection rules of the vibrator. C1 [Couture, A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Casten, R. F.] Yale Univ, Wright Nucl Struct Lab, New Haven, CT 06520 USA. [Cakirli, R. B.] Istanbul Univ, Dept Phys, TR-34134 Istanbul, Turkey. RP Couture, A (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM acouture@lanl.gov FU US Department of Energy, Office of Science, Office of Nuclear Physics [DE-FG02-91ER40609, DE-AC52-06NA25396]; Max Planck Partner group FX We are grateful to Klaus Blaum, Ami Leviatan, and Norbert Pietrella for useful discussions. This material is based on work supported by the US Department of Energy, Office of Science, Office of Nuclear Physics, under Award Number DE-FG02-91ER40609 and contract number DE-AC52-06NA25396. R.B.C. acknowledges support by the Max Planck Partner group. NR 14 TC 2 Z9 2 U1 1 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JAN 16 PY 2015 VL 91 IS 1 AR 014312 DI 10.1103/PhysRevC.91.014312 PG 5 WC Physics, Nuclear SC Physics GA CA1NC UT WOS:000348678200002 ER PT J AU Marrochio, H Noronha, J Denicol, GS Luzum, M Jeon, S Gale, C AF Marrochio, Hugo Noronha, Jorge Denicol, Gabriel S. Luzum, Matthew Jeon, Sangyong Gale, Charles TI Solutions of conformal Israel-Stewart relativistic viscous fluid dynamics SO PHYSICAL REVIEW C LA English DT Article ID HEAVY-ION COLLISIONS; QUARK-GLUON PLASMA; HYDRODYNAMICS; VISCOSITY; SYSTEMS; SCHEME; MATTER; FLOW AB We use symmetry arguments developed by Gubser to construct the first radially expanding explicit solutions of the Israel-Stewart formulation of hydrodynamics. Along with a general semi-analytical solution, an exact analytical solution is given which is valid in the cold plasma limit where viscous effects from shear viscosity and the relaxation time coefficient are important. The radially expanding solutions presented in this paper can be used as nontrivial checks of numerical algorithms employed in hydrodynamic simulations of the quark-gluon plasma formed in ultrarelativistic heavy ion collisions. We show this explicitly by comparing such analytic and semianalytic solutions with the corresponding numerical solutions obtained using the MUSIC viscous hydrodynamics simulation code. C1 [Marrochio, Hugo; Noronha, Jorge] Univ Sao Paulo, Inst Fis, BR-05315970 Sao Paulo, Brazil. [Denicol, Gabriel S.; Luzum, Matthew; Jeon, Sangyong; Gale, Charles] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Luzum, Matthew] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. RP Marrochio, H (reprint author), Univ Sao Paulo, Inst Fis, CP 66318, BR-05315970 Sao Paulo, Brazil. RI Luzum, Matthew/C-4986-2015; Noronha, Jorge/E-5783-2013; Silveira Denicol, Gabriel/L-5048-2016; Noronha, Jorge/M-8800-2014 OI Luzum, Matthew/0000-0002-0367-7055; FU Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Natural Sciences and Engineering Research Council of Canada FX The authors acknowledge many useful exchanges with B. Schenke, and are grateful to I. Kozlov, J.-F. Paquet, D. H. Rischke, J.-B. Rose, and G. Vujanovic for discussions. This work was funded in part by Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP), in part by Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), and in part by the Natural Sciences and Engineering Research Council of Canada. G.S.D. acknowledges the support of a Banting fellowship provided by the Natural Sciences and Engineering Research Council of Canada. NR 42 TC 18 Z9 18 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. 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CA Collaboration, A TI Measurements of Higgs boson production and couplings in the four-lepton channel in pp collisions at center-of-mass energies of 7 and 8 TeV with the ATLAS detector SO PHYSICAL REVIEW D LA English DT Article ID HADRON COLLIDERS; QCD CORRECTIONS; PARTON DISTRIBUTIONS; STANDARD MODEL; CROSS-SECTIONS; NNLO QCD; LHC; DECAYS; TAUOLA; TOOL AB The final ATLAS Run 1 measurements of Higgs boson production and couplings in the decay channel H -> ZZ* -> l(+)l(-)l(+)l'(-), where l, l' = e or mu, are presented. These measurements were performed using pp collision data corresponding to integrated luminosities of 4.5 and 20.3 fb(-1) at center-of-mass energies of 7 and 8 TeV, respectively, recorded with the ATLAS detector at the LHC. The H -> ZZ* -> 4l signal is observed with a significance of 8.1 standard deviations, with an expectation of 6.2 standard deviations, at m(H) = 125.36 GeV, the combined ATLAS measurement of the Higgs boson mass from the H -> gamma gamma and H -> ZZ* -> 4l channels. The production rate relative to the Standard Model expectation, the signal strength, is measured in four different production categories in the H -> ZZ* -> 4l channel. The measured signal strength, at this mass, and with all categories combined, is 1.44(-0.33)(+0.40). The signal strength for Higgs boson production in gluon fusion or in association with (tt) over bar or (bb) over bar pairs is found to be 1.7(-0.4)(+0.5), while the signal strength for vector-boson fusion combined with WH/ZH associated production is found to be 0.3(-0.9)(+1.6). C1 [Jackson, P.; Lee, L.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. 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L.; Caforio, D.; De Castro, S.; Di Sipio, R.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Hageboeck, S.; Hellmich, D.; Hillert, S.; Huegging, F.; Janssen, J.; Khoriauli, G.; Koevesarki, P.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lehmacher, M.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Loddenkoetter, T.; Mergelmeyer, S.; Mijovic, L.; Mueller, K.; Nanava, G.; Nattermann, T.; Obermann, T.; Pohl, D.; Sarrazin, B.; Schaepe, S.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Stillings, J. A.; Tannoury, N.; Therhaag, J.; Uchida, K.; Uhlenbrock, M.; Vogel, A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Fitzgerald, E. A.; Gozpinar, S.; Sciolla, G.; Venturini, A.; Zambito, S.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Amaral Coutinho, Y.; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE, EE, IF, BR-21945 Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Univ Fed Juiz de Fora, Juiz de Fora, Brazil. Univ Fed Sao Joao del Rei, Sao Joao del Rei, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Klimentov, A.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Okawa, H.; Oliveira Damazio, D.; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Schovancova, J.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dita, P.; Dita, S.; Ducu, O. A.; Jinaru, A.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Nat Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Departamento Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; Marchand, J. F.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Battistin, M.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Franchino, S.; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jakobsen, S.; Jansen, H.; Jungst, R. M.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Martin, B.; Marzin, A.; Messina, A.; Meyer, J.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Savu, D. O.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. 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Y.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Shandong, Peoples R China. [Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Clermont Univ, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] IN2P3, CNRS, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Guo, J.; Hu, D.; Hughes, E. W.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Wulf, E.] Columbia Univ, Nevis Lab, New York, NY 10027 USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; Rotonda, L. La; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Collegato Cosenza, Lab Nazl Frascati, Milan, Italy. [Capua, M.; Crosetti, G.; Rotonda, L. La; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. 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S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Grahn, K. -J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Prokofiev, K.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dao, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Madar, R.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ronzani, M.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Albert Ludwigs Univ, Fak Mathemat & Phys, Freiburg, Germany. [Alexandre, G.; Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nektarijevic, S.; Nikolics, K.; Picazio, A.; Pohl, M.; Rosbach, K.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; O'Shea, V.; Oropeza Barrera, C.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Denis, R. D. St.; Stewart, G. A.; Thompson, A. S.; Wright, M.] Univ Glasgow, SUPA, Glasgow, Lanark, Scotland. [Bierwagen, K.; Bindi, M.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Keil, M.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J. -Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Ippolito, V.; Kessoku, K.; Mateos, D. Lopez; Mercurio, K. 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Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Topilin, N. D.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Graduate Sch Sci, Kobe, Hyogo, Japan. [Ishino, M.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Allison, L. J.; Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Readioff, N. P.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Dept Phys, Ljubljana 61000, Slovenia. [Alpigiani, C.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Schreyer, M.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Kempster, J. J.; Kersten, S.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Cooper, B. D.; Davison, A. R.; Davison, P.; Falla, R. J.; Gregersen, K.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Sircar, A.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Ezhilov, A.; Fiedler, F.; Torregrosa, E. Fullana; Goeringer, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Borri, M.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Chen, L.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Chen, L.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Brau, B.; Colon, G.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Mantifel, R.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Victoria, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Harper, D.; Hu, X.; Levin, D.; Liu, L.; Long, J. D.; Lu, N.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Panikashvili, N.; Qian, J.; Schwarz, T. A.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Meroni, C.; Perini, L.; Pizio, C.; Resconi, S.; Simoniello, R.; Tartarelli, G. 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Z.; Wittkowski, J.] Univ Munich, Fak Phys, D-81377 Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Weigell, P.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartmento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Konig, A. C.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. 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M.; Talyshev, A. A.; Tikhonov, Yu. A.] RAS, Budker Inst Nucl Phys, SB, Novosibirsk, Russia. [Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Tannenwald, B. B.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Braun, H. M.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fabbri, L.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Braun, H. M.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fabbri, L.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Gjelsten, B. K.; Gramstad, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Behr, K.; Boddy, C. R.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Livermore, S. S. A.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Meyer, C.; Ospanov, R.; Saxon, J.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Wemans, A. Do Valle; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Marques, C. N.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Silva, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Portugal. [Wemans, A. Do Valle] Univ Nova Lisboa, Dept Fis, Caparica, Portugal. [Wemans, A. Do Valle] Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Bohm, J.; Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Stanescu, C.; Taccini, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Taccini, C.; Trovatelli, M.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl lEnergie Sci Techn Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, Lphea Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Grabas, H. M. X.; Guyot, C.; Hanna, R.; Hassani, S.; Kozanecki, W.; Lanon, E.; Laporte, J. F.; Maiani, C.; Mal, P.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J. -P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay Commissariat lEnergie Atom & Energies, DSM, IRFU, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Suruliz, K.; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; O'Neil, D. C.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nef, P. D.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Carrillo-Montoya, G. D.; Hamity, G. N.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bessidskaia, O.; Bohm, C.; Clement, C.; Cribbs, W. A.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Aloisio, A.; Annovi, A.; Asman, B.; Bendtz, K.; Bertoli, G.; Bessidskaia, O.; Clement, C.; Cribbs, W. A.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Sjoelin, J.; Strandberg, S.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Urban, S. Cabrera; Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Rosenthal, O.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Iliadis, D.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Ren, Z. L.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Kordas, K.; Kouskoura, V.; Leisos, A.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Sidiropoulou, O.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Internat Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Brelier, B.; Chau, C. C.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Ramos, J. A. Manjarres; Palacino, G.; Qureshi, A.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Pinamonti, M.; Quayle, W. B.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Quayle, W. B.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. 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[Pinamonti, M.; Shi, L.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tikhomirov, V. O.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Toth, J.] Inst Nucl & Particle Phys, Wigner Res Ctr Phys, Budapest, Hungary. [Vickey, T.] Univ Oxford, Dept Phys, Oxford, England. [Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Xu, L.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. 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Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; De, Kaushik/N-1953-2013; Carquin, Edson/G-5221-2015; Mir, Lluisa-Maria/G-7212-2015; Riu, Imma/L-7385-2014; Cavalli-Sforza, Matteo/H-7102-2015; Marti-Garcia, Salvador/F-3085-2011; Vos, Marcel/G-8123-2015; Della Pietra, Massimo/J-5008-2012; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Grancagnolo, Sergio/J-3957-2015; Doyle, Anthony/C-5889-2009; spagnolo, stefania/A-6359-2012; Villaplana Perez, Miguel/B-2717-2015; Bosman, Martine/J-9917-2014; Boyko, Igor/J-3659-2013; Smirnova, Oxana/A-4401-2013; Livan, Michele/D-7531-2012; Villa, Mauro/C-9883-2009; Mitsou, Vasiliki/D-1967-2009; White, Ryan/E-2979-2015; Joergensen, Morten/E-6847-2015; Brooks, William/C-8636-2013; Di Domenico, Antonio/G-6301-2011; Connell, Simon/F-2962-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Snesarev, Andrey/H-5090-2013; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; BESSON, NATHALIE/L-6250-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; Staroba, Pavel/G-8850-2014; Goncalo, Ricardo/M-3153-2016 OI Belanger-Champagne, Camille/0000-0003-2368-2617; Veneziano, Stefano/0000-0002-2598-2659; Vazquez Schroeder, Tamara/0000-0002-9780-099X; Chen, Chunhui /0000-0003-1589-9955; Price, Darren/0000-0003-2750-9977; Filthaut, Frank/0000-0003-3338-2247; Terzo, Stefano/0000-0003-3388-3906; Smirnov, Sergei/0000-0002-6778-073X; Arratia, Miguel/0000-0001-6877-3315; Della Volpe, Domenico/0000-0001-8530-7447; Hays, Chris/0000-0003-2371-9723; Farrington, Sinead/0000-0001-5350-9271; Robson, Aidan/0000-0002-1659-8284; Weber, Michele/0000-0002-2770-9031; Wang, Kuhan/0000-0002-6151-0034; Grohsjean, Alexander/0000-0003-0748-8494; Irles, Adrian/0000-0001-5668-151X; La Rosa, Alessandro/0000-0001-6291-2142; Beck, Hans Peter/0000-0001-7212-1096; Prokofiev, Kirill/0000-0002-2177-6401; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; la rotonda, laura/0000-0002-6780-5829; Coccaro, Andrea/0000-0003-2368-4559; Galhardo, Bruno/0000-0003-0641-301X; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Wemans, Andre/0000-0002-9669-9500; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Perrino, Roberto/0000-0002-5764-7337; SULIN, VLADIMIR/0000-0003-3943-2495; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Tikhomirov, Vladimir/0000-0002-9634-0581; Warburton, Andreas/0000-0002-2298-7315; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; De, Kaushik/0000-0002-5647-4489; Carquin, Edson/0000-0002-7863-1166; Mir, Lluisa-Maria/0000-0002-4276-715X; Riu, Imma/0000-0002-3742-4582; Vos, Marcel/0000-0001-8474-5357; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Grancagnolo, Sergio/0000-0001-8490-8304; Doyle, Anthony/0000-0001-6322-6195; spagnolo, stefania/0000-0001-7482-6348; Villaplana Perez, Miguel/0000-0002-0048-4602; Bosman, Martine/0000-0002-7290-643X; Boyko, Igor/0000-0002-3355-4662; Smirnova, Oxana/0000-0003-2517-531X; Livan, Michele/0000-0002-5877-0062; Villa, Mauro/0000-0002-9181-8048; Mitsou, Vasiliki/0000-0002-1533-8886; White, Ryan/0000-0003-3589-5900; Joergensen, Morten/0000-0002-6790-9361; Brooks, William/0000-0001-6161-3570; Di Domenico, Antonio/0000-0001-8078-2759; Connell, Simon/0000-0001-6000-7245; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Goncalo, Ricardo/0000-0002-3826-3442 FU ANPCyT, Argentina FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3- CNRS, CEA- DSM/ IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, I- CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/ IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/ NRF, South Africa; MINECO, Spain; SRC andWallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier- 1 facilities at TRIUMF ( Canada), NDGF ( Denmark, Norway, Sweden), CC- IN2P3 ( France), KIT/ GridKA ( Germany), INFN- CNAF ( Italy), NL- T1 ( Netherlands), PIC ( Spain), ASGC ( Taiwan), RAL ( UK) and BNL ( USA) and in the Tier- 2 facilities worldwide. NR 104 TC 39 Z9 39 U1 21 U2 109 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JAN 16 PY 2015 VL 91 IS 1 AR 012006 DI 10.1103/PhysRevD.91.012006 PG 47 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CA1NH UT WOS:000348678700001 ER PT J AU Huang, P Wagner, CEM AF Huang, Peisi Wagner, Carlos E. M. TI CMS kinematic edge from sbottoms SO PHYSICAL REVIEW D LA English DT Article ID ANOMALOUS MAGNETIC-MOMENT; STANDARD MODEL; DARK-MATTER; MUON; SEARCH; SUPERSYMMETRY; LHC; SUPERGRAVITY; PARTICLE; PHYSICS AB We present two scenarios in the Minimal Supersymmetric Extension of the Standard Model (MSSM) that can lead to an explanation of the excess in the invariant mass distribution of two opposite charged, same flavor leptons, and the corresponding edge at an energy of about 78 GeV, recently reported by the CMS Collaboration. In both scenarios, sbottoms are pair produced, and decay to neutralinos and a b-jet. The heavier neutralinos further decay to a pair of leptons and the lightest neutralino through on-shell sleptons or off-shell neutral gauge bosons. These scenarios are consistent with the current limits on the sbottoms, neutralinos, and sleptons. Assuming that the lightest neutralino is stable we discuss the predicted relic density as well as the implications for darkmatter direct detection. We show that consistency between the predicted and the measured value of the muon anomalous magnetic moment may be obtained in both scenarios. Finally, we define the signatures of these models that may be tested at the 13 TeV run of the LHC. C1 [Huang, Peisi; Wagner, Carlos E. M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Wagner, Carlos E. M.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Huang, Peisi; Wagner, Carlos E. M.] Argonne Natl Lab, HEP Div, Argonne, IL 60439 USA. RP Huang, P (reprint author), Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. OI Huang, Peisi/0000-0003-3360-2641 FU U.S. Department of Energy [DE-FG0213ER41958, DE-AC0206CH11357, DE-FG02-04ER41286] FX We would like to thank N. Craig, C. Hill, B. Hooberman, G. Landsberg, A. Paramonov, L. T. Wang and D. Whiteson for useful discussions. We would also like to thank the Aspen Center for Physics, where this work was started and part of this work has been done. Work is supported by the U.S. Department of Energy under Contract No. DE-FG0213ER41958. Work at ANL is supported in part by the U.S. Department of Energy under Contract No. DE-AC0206CH11357. P. H. is partially supported by U.S. Department of Energy Grant No. DE-FG02-04ER41286. NR 47 TC 8 Z9 8 U1 1 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JAN 16 PY 2015 VL 91 IS 1 AR 015014 DI 10.1103/PhysRevD.91.015014 PG 8 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CA1NH UT WOS:000348678700005 ER PT J AU Kim, KW Smith, CA Daily, MD Cort, JR Davin, LB Lewis, NG AF Kim, Kye-Won Smith, Clyde A. Daily, Michael D. Cort, John R. Davin, Laurence B. Lewis, Norman G. TI Trimeric Structure of (+)-Pinoresinol-forming Dirigent Protein at 1.95 angstrom Resolution with Three Isolated Active Sites SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article ID DISEASE-RESISTANCE RESPONSE; ALLENE OXIDE CYCLASE; SECONDARY; MODEL; ARABIDOPSIS; SPECIFICITY; EXPRESSION; INSIGHTS; PEA AB Control over phenoxy radical-radical coupling reactions in vivo in vascular plants was enigmatic until our discovery of dirigent proteins (DPs, from the Latin dirigere, to guide or align). The first three-dimensional structure of a DP ((+)-pinoresinol-forming DP, 1.95 angstrom resolution, rhombohedral space group H32)) is reported herein. It has a tightly packed trimeric structure with an eight-stranded beta-barrel topology for each DP monomer. Each putative substrate binding and orientation coupling site is located on the trimer surface but too far apart for intermolecular coupling between sites. It is proposed that each site enables stereoselective coupling (using either two coniferyl alcohol radicals or a radical and a monolignol). Interestingly, there are six differentially conserved residues in DPs affording either the (+)- or (-)-antipodes in the vicinity of the putative binding site and region known to control stereoselectivity. DPs are involved in lignan biosynthesis, whereas dirigent domains/sites have been implicated in lignin deposition. C1 [Kim, Kye-Won; Davin, Laurence B.; Lewis, Norman G.] Washington State Univ, Inst Biol Chem, Pullman, WA 99164 USA. [Smith, Clyde A.] Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Daily, Michael D.; Cort, John R.] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99354 USA. RP Lewis, NG (reprint author), Washington State Univ, Inst Biol Chem, Pullman, WA 99164 USA. EM lewisn@wsu.edu FU U.S. Dept. of Energy, Office of Science, Basic Energy Sciences (BES) [DE-AC02-76SF00515]; DOE Office of Biological and Environmental Research (BER); National Institutes of Health, National Institute of General Medical Sciences [P41GM103393]; Dept. of Energy's BER FX We thank Marlisa Burton, Terri Lincoln, Mia Ryckman, and Paul Ziegler for assistance in DP purification. Use of the Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, is supported by the U.S. Dept. of Energy, Office of Science, Basic Energy Sciences (BES), under Contract No. DE-AC02-76SF00515. The SSRL Structural Molecular Biology Program is supported by the DOE Office of Biological and Environmental Research (BER), and by the National Institutes of Health, National Institute of General Medical Sciences (including P41GM103393). A portion of the work was performed in the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the Dept. of Energy's BER and located at Pacific Northwest National Laboratory (PNNL), Richland, WA. NR 40 TC 7 Z9 7 U1 5 U2 19 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD JAN 16 PY 2015 VL 290 IS 3 BP 1308 EP 1318 DI 10.1074/jbc.M114.611780 PG 11 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA AZ2IB UT WOS:000348056400002 PM 25411250 ER PT J AU Gaudet, R Roux, B Minor, DL AF Gaudet, Rachelle Roux, Benoit Minor, Daniel L., Jr. TI Insights into the molecular foundations of electrical excitation SO JOURNAL OF MOLECULAR BIOLOGY LA English DT Editorial Material C1 [Gaudet, Rachelle] Harvard Univ, Dept Mol & Cellular Biol, Cambridge, MA 02138 USA. [Roux, Benoit] Univ Chicago, Gordon Ctr Integrat Sci, Dept Biochem & Mol Biol, Dept Chem, Chicago, IL 60637 USA. [Minor, Daniel L., Jr.] Univ Calif San Francisco, Calif Inst Quantitat Biomed Res, Cardiovasc Res Inst, Dept Biochem & Biophys, San Francisco, CA 93858 USA. [Minor, Daniel L., Jr.] Univ Calif San Francisco, Calif Inst Quantitat Biomed Res, Dept Cellular & Mol Pharmacol, San Francisco, CA 93858 USA. [Minor, Daniel L., Jr.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Minor, DL (reprint author), Univ Calif San Francisco, Calif Inst Quantitat Biomed Res, Cardiovasc Res Inst, Dept Biochem & Biophys, San Francisco, CA 93858 USA. EM daniel.minor@ucsf.edu OI Gaudet, Rachelle/0000-0002-9177-054X FU NHLBI NIH HHS [R01 HL080050]; NIDCD NIH HHS [R01 DC007664]; NIMH NIH HHS [R01 MH093603] NR 18 TC 0 Z9 0 U1 1 U2 6 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0022-2836 EI 1089-8638 J9 J MOL BIOL JI J. Mol. Biol. PD JAN 16 PY 2015 VL 427 IS 1 SI SI BP 1 EP 2 PG 2 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA AZ8TB UT WOS:000348486300001 PM 25542854 ER PT J AU Payandeh, J Minor, DL AF Payandeh, Jian Minor, Daniel L., Jr. TI Bacterial Voltage-Gated Sodium Channels (BacNa(V)s) from the Soil, Sea, and Salt Lakes Enlighten Molecular Mechanisms of Electrical Signaling and Pharmacology in the Brain and Heart SO JOURNAL OF MOLECULAR BIOLOGY LA English DT Review DE voltage-gated sodium channel; structural biology; channel gating; ion permeation; channel pharmacology ID X-RAY-STRUCTURE; C-TERMINAL DOMAIN; SOLUTION NMR STRUCTURE; DEPENDENT K+ CHANNEL; EF-HAND DOMAIN; ION-CHANNEL; CRYSTAL-STRUCTURE; POTASSIUM CHANNEL; NA+ CHANNEL; SELECTIVITY FILTER AB Voltage-gated sodium channels (Na(V)s) provide the initial electrical signal that drives action potential generation in many excitable cells of the brain, heart, and nervous system. For more than 60 years, functional studies of Nays have occupied a central place in physiological and biophysical investigation of the molecular basis of excitability. Recently, structural studies of members of a large family of bacterial voltage-gated sodium channels (BacNa(V)s) prevalent in soil, marine, and salt lake environments that bear many of the core features of eukaryotic Nays have reframed ideas for voltage-gated channel function, ion selectivity, and pharmacology. Here, we analyze the recent advances, unanswered questions, and potential of BacNa(V)s as templates for drug development efforts. (C) 2014 The Authors. Published by Elsevier Ltd. C1 [Payandeh, Jian] Genentech Inc, Dept Biol Struct, San Francisco, CA 94080 USA. [Minor, Daniel L., Jr.] Univ Calif San Francisco, Calif Inst Quantitat Biomed Res, Dept Biochem & Biophys, Cardiovasc Res Inst, San Francisco, CA 93858 USA. [Minor, Daniel L., Jr.] Univ Calif San Francisco, Calif Inst Quantitat Biomed Res, Dept Cellular & Mol Pharmacol, San Francisco, CA 93858 USA. [Minor, Daniel L., Jr.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Payandeh, J (reprint author), Univ Calif San Francisco, Calif Inst Quantitat Biomed Res, Dept Biochem & Biophys, Cardiovasc Res Inst, San Francisco, CA 93858 USA. EM payandeh.jian@gene.com; daniel.minor@ucsf.edu FU National Institutes of Health [R01-HL080050, R01-DC007664, U54-GM094625] FX We thank M. Grabe for help with the conservation analysis; C. Arrigoni and F. Findeisen for help with the alignments and figures; B. Liebeskind and H. Zakon for figure assistance; and C. Arrigoni, F. Findeisen, and M. Grabe for comments on the manuscript. This work was supported by National Institutes of Health R01-HL080050, R01-DC007664, and U54-GM094625 grants to D.L.M. NR 199 TC 21 Z9 22 U1 2 U2 23 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0022-2836 EI 1089-8638 J9 J MOL BIOL JI J. Mol. Biol. PD JAN 16 PY 2015 VL 427 IS 1 SI SI BP 3 EP 30 DI 10.1016/j.jmb.2014.08.010 PG 28 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA AZ8TB UT WOS:000348486300002 PM 25158094 ER PT J AU Ryan, SD Mityushev, V Vinokur, VM Berlyand, L AF Ryan, S. D. Mityushev, V. Vinokur, V. M. Berlyand, L. TI Rayleigh approximation to ground state of the Bose and Coulomb glasses SO SCIENTIFIC REPORTS LA English DT Article ID DOMAINS; PHASE AB Glasses are rigid systems in which competing interactions prevent simultaneous minimization of local energies. This leads to frustration and highly degenerate ground states the nature and properties of which are still far from being thoroughly understood. We report an analytical approach based on the method of functional equations that allows us to construct the Rayleigh approximation to the ground state of a two-dimensional (2D) random Coulomb system with logarithmic interactions. We realize a model for 2D Coulomb glass as a cylindrical type II superconductor containing randomly located columnar defects (CD) which trap superconducting vortices induced by applied magnetic field. Our findings break ground for analytical studies of glassy systems, marking an important step towards understanding their properties. C1 [Ryan, S. D.; Berlyand, L.] Penn State Univ, Dept Math, University Pk, PA 16802 USA. [Mityushev, V.] Pedag Univ, Dept Comp Sci & Comp Methods, PL-30084 Krakow, Poland. [Vinokur, V. M.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Vinokur, VM (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM vinokour@anl.gov FU NSF [DMS-1106666, DMS-1405769]; U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division FX The authors would like to thank W. Nawalaniec for the algorithm used to study the transition from periodic to random hole locations in the numerical simulations. Work of L.B. was supported by the NSF grants DMS-1106666 and DMS-1405769, work of V.V. was supported by the U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division, and work of S.R. and V.M. was partially supported by the NSF grant DMS-1106666. NR 30 TC 1 Z9 1 U1 2 U2 5 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 16 PY 2015 VL 5 AR 7821 DI 10.1038/srep07821 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AY9YN UT WOS:000347903800002 PM 25592417 ER PT J AU Meng, XB AF Meng, Xiangbo TI Towards high-energy and durable lithiumion batteries via atomic layer deposition: elegantly atomic-scale material design and surface modification SO NANOTECHNOLOGY LA English DT Article ID ION BATTERIES; CATHODE MATERIALS; THIN-FILMS; PERFORMANCE; OXIDE; LI4TI5O12; BEHAVIOR; NITRIDE; SULFIDE; EPITAXY AB Targeted at fueling future transportation and sustaining smart grids, lithium-ion batteries (LIBs) are undergoing intensive investigation for improved durability and energy density. Atomic layer deposition (ALD), enabling uniform and conformal nanofilms, has recently made possible many new advances for superior LIBs. The progress was summarized by Liu and Sun in their latest review [1], offering many insightful views, covering the design of nanostructured battery components (i.e., electrodes and solid electrolytes), and nanoscale modification of electrode/electrolyte interfaces. This work well informs peers of interesting research conducted and it will also further help boost the applications of ALD in next-generation LIBs and other advanced battery technologies. C1 Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. RP Meng, XB (reprint author), Argonne Natl Lab, Div Energy Syst, 9700 S Cass Ave, Argonne, IL 60439 USA. EM xmeng@anl.gov OI Meng, Xiangbo/0000-0002-4631-7260 FU Center for Electrical Energy Storage: Tailored Interfaces, an Energy Frontier Research Center - US Department of Energy, Office of Science, and Office of Basic Energy Sciences FX X Meng appreciates the funding support of the Center for Electrical Energy Storage: Tailored Interfaces, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, and Office of Basic Energy Sciences. X Meng is grateful to Dr Jeffrey W Elam at Argonne for many constructive comments. NR 31 TC 2 Z9 2 U1 7 U2 70 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD JAN 16 PY 2015 VL 26 IS 2 AR 020501 DI 10.1088/0957-4484/26/2/020501 PG 4 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA AX5YC UT WOS:000346999500001 PM 25514439 ER PT J AU Lenhardt, JM Kim, SH Worsley, MA Leif, RN Campbell, PG Baumann, TF Satcher, JH AF Lenhardt, Jeremy M. Kim, Sung Ho Worsley, Marcus A. Leif, Roald N. Campbell, Patrick G. Baumann, Theodore F. Satcher, Joseph H., Jr. TI ROMP crosslinkers for the preparation of aliphatic aerogels SO JOURNAL OF NON-CRYSTALLINE SOLIDS LA English DT Article DE Ring opening metathesis polymerization; Aliphatic aerogel; Romp crosslinker ID AREA CARBON AEROGELS; ORGANIC AEROGELS; SILICA AEROGEL; DENSITY; DICYCLOPENTADIENE; POLYMERIZATION; CONDUCTIVITY; MORPHOLOGY; INSULATION; MONOLITHS AB Ring opening metathesis polymerization (ROMP) using Grubbs second generation catalyst generates aliphatic gels from norbornene based crosslinkable monomers with a functionality of 2 or 3. Supercritical drying of these gels (CO2) leads to the formation of aerogels with densities as low as 4 mg mL(-1). The microstructure was analyzed by SEM, and pore analyses by nitrogen adsorption. The use of crosslinkable monomers allows the straightforward synthesis of aerogels consisting of only carbon and hydrogen with C:H ratios up to ca. CH1.58 with a finer microstructure than that of DCPD. (C) 2014 Elsevier BM. All rights reserved. C1 [Lenhardt, Jeremy M.; Kim, Sung Ho; Worsley, Marcus A.; Leif, Roald N.; Campbell, Patrick G.; Baumann, Theodore F.; Satcher, Joseph H., Jr.] Lawrence Livermore Natl Lab, Div Mat Sci, Livermore, CA 94550 USA. [Satcher, Joseph H., Jr.] Lawrence Livermore Natl Lab, Nanoscale Synth & Characterizat Lab, Livermore, CA 94550 USA. RP Lenhardt, JM (reprint author), Lawrence Livermore Natl Lab, Div Mat Sci, 7000 East Ave, Livermore, CA 94550 USA. EM lenhardt2@llnl.gov OI Campbell, Patrick/0000-0003-0167-4624; Worsley, Marcus/0000-0002-8012-7727 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344, LLNL-JRNL-655922] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. IM release LLNL-JRNL-655922. NR 27 TC 3 Z9 3 U1 2 U2 14 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3093 EI 1873-4812 J9 J NON-CRYST SOLIDS JI J. Non-Cryst. Solids PD JAN 15 PY 2015 VL 408 BP 98 EP 101 DI 10.1016/j.jnoncrysol.2014.10.019 PG 4 WC Materials Science, Ceramics; Materials Science, Multidisciplinary SC Materials Science GA CJ2SY UT WOS:000355336000016 ER PT J AU Kerisit, S Pierce, EM Ryan, JV AF Kerisit, Sebastien Pierce, Eric M. Ryan, Joseph V. TI Monte Carlo simulations of coupled diffusion and surface reactions during the aqueous corrosion of borosilicate glasses SO JOURNAL OF NON-CRYSTALLINE SOLIDS LA English DT Article DE Monte Carlo; Borosilicate glasses; Diffusion; Alteration layer; Kinetics ID NUCLEAR-WASTE GLASSES; GRAAL MODEL; DISSOLUTION; KINETICS; WATER; TERM; MECHANISMS; MORPHOLOGY; LAYERS; STATE AB Borosilicate nuclear waste glasses develop complex altered layers as a result of coupled processes such as hydrolysis of network species, condensation of Si species, and diffusion. However, diffusion has often been overlooked in Monte Carlo models of the aqueous corrosion of borosilicate glasses. Therefore, three different models for dissolved Si diffusion in the altered layer were implemented in a Monte Carlo model and evaluated for glasses in the compositional range (75 - x) mol% SiO2 (12.5 + x/2) mol% B2O3 and (12.5 + x/2) mol% Na2O, where 0 <= x <= 20%, and corroded in static conditions at a surface-area-to-volume ratio of 1000 m(-1). The three models considered instantaneous homogenization (M1), linear concentration gradients (M2), and concentration profiles determined by solving Fick's 2nd law using a finite difference method (M3). Model M3 revealed that concentration profiles in the altered layer are not linear and show changes in shape and magnitude as corrosion progresses, unlike those assumed in model M2. Furthermore, model M3 showed that, for borosilicate glasses with a high forward dissolution rate compared to the diffusion rate, the gradual polymerization and densification of the altered layer is significantly delayed compared to models M1 and M2. Models M1 and M2 were found to be appropriate models only for glasses with high release rates such as simple borosilicate glasses with low ZrO2 content. (C) 2014 Elsevier B.V. All rights reserved. C1 [Kerisit, Sebastien] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. [Pierce, Eric M.] Oak Ridge Natl Lab, Energy & Environm Sci Directorate, Oak Ridge, TN 37831 USA. [Ryan, Joseph V.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. RP Kerisit, S (reprint author), Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. EM sebastien.kerisit@pnnl.gov RI Pierce, Eric/G-1615-2011 OI Pierce, Eric/0000-0002-4951-1931 FU Office of Nuclear Energy (Fuel Cycle Research and Development); Office of Environmental Management (Tank Waste Management) of the U.S. Department of Energy (DOE) [EM-21]; Office of Science's Office of Biological and Environmental Research (OBER); DOE by Battelle Memorial Institute [DE-AC05-76RL01830]; DOE [DE-AC05-00OR22725] FX This work was funded by the Office of Nuclear Energy (Fuel Cycle Research and Development) and the Office of Environmental Management (Tank Waste Management, EM-21) of the U.S. Department of Energy (DOE). Some computer simulations were performed as part of a DOE Office of Science-supported Science Theme User Proposal at the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL) Molecular Science Computing (MSC) facilities. The EMSL is a national scientific user facility sponsored by the Office of Science's Office of Biological and Environmental Research (OBER) and located at Pacific Northwest National Laboratory (PNNL). PNNL is operated for the DOE by Battelle Memorial Institute under Contract DE-AC05-76RL01830. Oak Ridge National Laboratory (ORNL) is managed by UT-Battelle LLC for the DOE under contract DE-AC05-00OR22725. NR 41 TC 1 Z9 1 U1 4 U2 21 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3093 EI 1873-4812 J9 J NON-CRYST SOLIDS JI J. Non-Cryst. Solids PD JAN 15 PY 2015 VL 408 BP 142 EP 149 DI 10.1016/j.jnoncrysol.2014.07.020 PG 8 WC Materials Science, Ceramics; Materials Science, Multidisciplinary SC Materials Science GA CJ2SY UT WOS:000355336000022 ER PT J AU Prelovsek, S Lang, CB Leskovec, L Mohler, D AF Prelovsek, Sasa Lang, C. B. Leskovec, Luka Mohler, Daniel TI Study of the Z(c)(+) channel using lattice QCD SO PHYSICAL REVIEW D LA English DT Article ID QUANTUM-FIELD THEORIES; VOLUME DEPENDENCE; SCATTERING MATRIX; ENERGY-SPECTRUM; GAUGE-THEORY; STATES AB Recently experimentalists have discovered several charged charmoniumlike hadrons Z(c)(+) with unconventional quark content (c) over barc (d) over baru. We perform a search for Z(c)(+) with mass below 4.2 GeV in the channel I-G (J(PC)) = 1(+)(1(+-)) using lattice QCD. The major challenge is presented by the two-meson states J/psi pi, psi(2S)pi, psi(1D)pi, D (D) over bar (*), D*(D) over bar*, eta(c)rho that are inevitably present in this channel. The spectrum of eigenstates is extracted using a number of meson-meson and diquark-antidiquark interpolating fields. For our pion mass of 266 MeV we find all the expected two-meson states but no additional candidate for Z(c)(+) below 4.2 GeV. Possible reasons for not seeing an additional eigenstate related to Z(c)(+) are discussed. We also illustrate how a simulation incorporating interpolators with a structure resembling low-lying two-meson states seems to render a Z(c)(+) candidate, which is however not robust after further two-meson states around 4.2 GeV are implemented. C1 [Prelovsek, Sasa] Univ Ljubljana, Dept Phys, Ljubljana 1000, Slovenia. [Prelovsek, Sasa; Leskovec, Luka] Jozef Stefan Inst, Ljubljana 1000, Slovenia. [Lang, C. B.] Graz Univ, Inst Phys, A-8010 Graz, Austria. [Mohler, Daniel] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Prelovsek, S (reprint author), Univ Ljubljana, Dept Phys, Jadranska 19, Ljubljana 1000, Slovenia. EM sasa.prelovsek@ijs.si; christian.lang@uni-graz.at; luka.leskovec@ijs.si; dmohler@fnal.gov OI leskovec, luka/0000-0002-8926-527X; Mohler, Daniel/0000-0003-1852-9562 FU Slovenian Research Agency ARRS Project [N1-0020]; Austrian Science Fund FWF Project [I1313-N27]; DFG [SFB/TRR55]; United States Department of Energy [De-AC02-07CH11359] FX We thank Anna Hasenfratz for providing the gauge configurations. S. P. thanks Changzheng Yuan and Anze Zupanc for discussion, D. M. is grateful for discussions with Jim Simone, and C. B. L. is grateful for discussion with M. Padmanath. The computations were done on the clusters at the Theoretical Physics department of Jozef Stefan Institute, at the University of Graz, NAWI Graz, and TRIUMF. We acknowledge the support by the Slovenian Research Agency ARRS Project No. N1-0020, by the Austrian Science Fund FWF Project No. I1313-N27, and by DFG Project No. SFB/TRR55. Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. De-AC02-07CH11359 with the United States Department of Energy. NR 42 TC 27 Z9 27 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JAN 15 PY 2015 VL 91 IS 1 AR 014504 DI 10.1103/PhysRevD.91.014504 PG 10 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CE6MH UT WOS:000351950100003 ER PT J AU Kim, H Tanatar, MA Flint, R Petrovic, C Hu, R White, BD Lum, IK Maple, MB Prozorov, R AF Kim, Hyunsoo Tanatar, M. A. Flint, R. Petrovic, C. Hu, Rongwei White, B. D. Lum, I. K. Maple, M. B. Prozorov, R. TI Nodal to Nodeless Superconducting Energy-Gap Structure Change Concomitant with Fermi-Surface Reconstruction in the Heavy-Fermion Compound CeCoIn5 SO PHYSICAL REVIEW LETTERS LA English DT Article ID QUANTUM CRITICAL-POINT; PENETRATION DEPTH; UNCONVENTIONAL SUPERCONDUCTIVITY; CE1-XYBXCOIN5; DENSITY; FIELD AB The London penetration depth lambda(T) wasmeasured in single crystals of Ce1-xRxCoIn5, R = La, Nd, and Yb down to T-min approximate to 50 mK (T-c/T-min similar to 50) using a tunnel-diode resonator. In the cleanest samples Delta lambda(T) is best described by the power law Delta lambda(T) proportional to T-n, with n similar to 1, consistent with the existence of line nodes in the superconducting gap. Substitutions of Ce with La, Nd, and Yb lead to similar monotonic suppressions of T-c; however, the effects on Delta lambda(T) differ. While La and Nd substitution leads to an increase in the exponent n and saturation at n similar to 2, as expected for a dirty nodal superconductor, Yb substitution leads to n > 3, suggesting a change from nodal to nodeless superconductivity. This superconducting gap structure change happens in the same doping range where changes of the Fermi-surface topology were reported, implying that the nodal structure and Fermi-surface topology are closely linked. C1 [Kim, Hyunsoo; Tanatar, M. A.; Flint, R.; Prozorov, R.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Petrovic, C.; Hu, Rongwei] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [White, B. D.; Lum, I. K.; Maple, M. B.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. RP Prozorov, R (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA. EM prozorov@ameslab.gov RI Petrovic, Cedomir/A-8789-2009; Flint, Rebecca/J-3628-2014 OI Petrovic, Cedomir/0000-0001-6063-1881; FU U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; U.S. DOE by Iowa State University [DE-AC02-07CH11358]; U.S. Department of Energy by Brookhaven Science Associates [DE-Ac02-98CH10886]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-FG02-04-ER46105]; AFOSR-MURI [FA9550-09-1-0603] FX We thank P. Coleman and O. Erten for stimulating discussions and sharing their theoretical work prior to publication. The work in Ames was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. Ames Laboratory is operated for the U.S. DOE by Iowa State University under Contract No. DE-AC02-07CH11358. Part of the work was carried out at the Brookhaven National Laboratory, which is operated for the U.S. Department of Energy by Brookhaven Science Associates (No. DE-Ac02-98CH10886). Research at UCSD was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Grant No. DE-FG02-04-ER46105. H. K. acknowledges support from AFOSR-MURI Grant No. FA9550-09-1-0603. NR 55 TC 12 Z9 12 U1 4 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 15 PY 2015 VL 114 IS 2 AR 027003 DI 10.1103/PhysRevLett.114.027003 PG 5 WC Physics, Multidisciplinary SC Physics GA CE6OB UT WOS:000351956500005 PM 25635560 ER PT J AU Meisel, Z George, S Ahn, S Browne, J Bazin, D Brown, BA Carpino, JF Chung, H Cyburt, RH Estrade, A Famiano, M Gade, A Langer, C Matos, M Mittig, W Montes, F Morrissey, DJ Pereira, J Schatz, H Schatz, J Scott, M Shapira, D Smith, K Stevens, J Tan, W Tarasov, O Towers, S Wimmer, K Winkelbauer, JR Yurkon, J Zegers, RGT AF Meisel, Z. George, S. Ahn, S. Browne, J. Bazin, D. Brown, B. A. Carpino, J. F. Chung, H. Cyburt, R. H. Estrade, A. Famiano, M. Gade, A. Langer, C. Matos, M. Mittig, W. Montes, F. Morrissey, D. J. Pereira, J. Schatz, H. Schatz, J. Scott, M. Shapira, D. Smith, K. Stevens, J. Tan, W. Tarasov, O. Towers, S. Wimmer, K. Winkelbauer, J. R. Yurkon, J. Zegers, R. G. T. TI Mass Measurements Demonstrate a Strong N=28 Shell Gap in Argon SO PHYSICAL REVIEW LETTERS LA English DT Article ID NUCLEAR; STABILITY; ISOTOPES; CLOSURE AB We present results from recent time-of-flight nuclear mass measurements at the National Superconducting Cyclotron Laboratory at Michigan State University. We report the first mass measurements of Ar-48 and Ar-49 and find atomic mass excesses of -22.28(31) MeV and -17.8(1.1) MeV, respectively. These masses provide strong evidence for the closed shell nature of neutron number N = 28 in argon, which is therefore the lowest even-Z element exhibiting the N = 28 closed shell. The resulting trend in binding-energy differences, which probes the strength of the N = 28 shell, compares favorably with shell-model calculations in the sd-pf shell using SDPF-U and SDPF-MU Hamiltonians. C1 [Meisel, Z.; George, S.; Ahn, S.; Browne, J.; Bazin, D.; Brown, B. A.; Cyburt, R. H.; Gade, A.; Langer, C.; Mittig, W.; Montes, F.; Morrissey, D. J.; Pereira, J.; Schatz, H.; Schatz, J.; Scott, M.; Stevens, J.; Tarasov, O.; Wimmer, K.; Winkelbauer, J. R.; Yurkon, J.; Zegers, R. G. T.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Meisel, Z.; Browne, J.; Brown, B. A.; Gade, A.; Mittig, W.; Schatz, H.; Scott, M.; Stevens, J.; Winkelbauer, J. R.; Zegers, R. G. T.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Meisel, Z.; George, S.; Ahn, S.; Browne, J.; Cyburt, R. H.; Langer, C.; Montes, F.; Pereira, J.; Schatz, H.; Smith, K.; Stevens, J.; Zegers, R. G. T.] Michigan State Univ, Joint Inst Nucl Astrophys, E Lansing, MI 48824 USA. [George, S.] Max Planck Inst Kernphys, D-69117 Heidelberg, Germany. [Carpino, J. F.; Chung, H.; Famiano, M.; Towers, S.] Western Michigan Univ, Dept Phys, Kalamazoo, MI 49008 USA. [Estrade, A.] Univ Edinburgh, Sch Phys & Astron, Edinburgh EH8 9YL, Midlothian, Scotland. [Matos, M.] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. [Morrissey, D. J.] Michigan State Univ, Dept Chem, E Lansing, MI 48824 USA. [Shapira, D.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Smith, K.; Tan, W.] Univ Notre Dame, Dept Phys, South Bend, IN 46556 USA. RP Meisel, Z (reprint author), Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. EM meisel@nscl.msu.edu RI Gade, Alexandra/A-6850-2008; Zegers, Remco/A-6847-2008; Tan, Wanpeng/A-4687-2008; Langer, Christoph/L-3422-2016 OI Gade, Alexandra/0000-0001-8825-0976; Tan, Wanpeng/0000-0002-5930-1823; FU National Science Foundation [PHY-0822648, PHY-1102511, PHY-1404442, PHY-1430152]; DFG [GE2183/1-1, GE2183/2-1] FX This project is based upon work supported by the National Science Foundation under Grants No. PHY-0822648, No. PHY-1102511, No. PHY-1404442, and No. PHY-1430152. S. G. acknowledges support from the DFG under Contracts No. GE2183/1-1 and No. GE2183/2-1. NR 40 TC 11 Z9 11 U1 0 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JAN 15 PY 2015 VL 114 IS 2 AR 022501 DI 10.1103/PhysRevLett.114.022501 PG 4 WC Physics, Multidisciplinary SC Physics GA CE6OB UT WOS:000351956500001 PM 25635542 ER PT J AU Lim, J Fabbris, G Haskel, D Schilling, JS AF Lim, J. Fabbris, G. Haskel, D. Schilling, J. S. TI Magnetic ordering at anomalously high temperatures in Dy at extreme pressures SO PHYSICAL REVIEW B LA English DT Article ID RARE-EARTH DIALUMINIDES; S-F EXCHANGE; KONDO-LATTICE; TRANSITION-TEMPERATURES; NONMAGNETIC TRANSITION; RHODIUM BORIDES; CERH3B2; METALS; GPA; SUPERCONDUCTIVITY AB In an attempt to destabilize the magnetic state of the heavy lanthanide Dy, extreme pressures were applied in an electrical resistivity measurement to 157 GPa over the temperature range 1.3-295 K. The magnetic ordering temperature T-o and spin-disorder resistance R-sd of Dy, as well as the superconducting pair-breaking effect Delta T-c in Y(1 at.% Dy), are found to track each other in a highly nonmonotonic fashion as a function of pressure. Above 73 GPa, the critical pressure for a 6% volume collapse in Dy, all three quantities increase sharply (dT(o)/dP similar or equal to 5.3 K/GPa), T-o appearing to rise above ambient temperature for P > 107 GPa. In contrast, To and Delta T-c for Gd and Y(0.5 at.% Gd), respectively, show no such sharp increase with pressure (dT(o)/dP similar or equal to 0.73K/GPa). Taken together, these results suggest that extreme pressure transports Dy into an unconventional magnetic state with an anomalously high magnetic ordering temperature. C1 [Lim, J.; Fabbris, G.; Schilling, J. S.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Fabbris, G.; Haskel, D.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Lim, J (reprint author), Washington Univ, Dept Phys, St Louis, MO 63130 USA. EM jss@wuphys.wustl.edu RI Fabbris, Gilberto/F-3244-2011 OI Fabbris, Gilberto/0000-0001-8278-4985 FU National Science Foundation (NSF) [DMR-1104742]; Carnegie/DOE Alliance Center (CDAC) through NNSA/DOE Grant [DE-FC52-08NA28554]; US Department of Energy, Office of Science [DE-AC02-06CH11357] FX The authors would like to thank T. Matsuoka and K. Shimizu for sharing information on their high-pressure electrical resistivity techniques used in this study. Thanks are due A. Gangopadhyay both for his critical reading of the manuscript and help in preparing the Y(Dy) alloy. This work was supported by the National Science Foundation (NSF) through Grant No. DMR-1104742 and by the Carnegie/DOE Alliance Center (CDAC) through NNSA/DOE Grant No. DE-FC52-08NA28554. Work at Argonne National Laboratory is supported by the US Department of Energy, Office of Science, under Contract No. DE-AC02-06CH11357. NR 54 TC 2 Z9 2 U1 6 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 15 PY 2015 VL 91 IS 4 AR 045116 DI 10.1103/PhysRevB.91.045116 PG 8 WC Physics, Condensed Matter SC Physics GA CE3YS UT WOS:000351766600003 ER PT J AU Tai, YY Wang, CCJ Graf, MJ Zhu, JX Ting, CS AF Tai, Yuan-Yen Wang, C. -C. Joseph Graf, Matthias J. Zhu, Jian-Xin Ting, C. S. TI Emergent topological mirror insulator in t(2g)-orbital systems SO PHYSICAL REVIEW B LA English DT Article ID PHASE; STATES; MODEL AB Motivated by the itinerant band structure of high-T-c iron pnictides, which exhibit four Dirac cones in the bulk, we demonstrate the prospect of pnictides with transition elements to be topological insulators in two dimensions. In this report, we explore interaction-induced topological phases, in contrast to the spin-orbit-coupling interaction, as the crucial mechanism for tuning Dirac metals into Z(2)-topological insulators protected by time reversal and mirror symmetries. We find spontaneous orbital currents generated through nearest-neighbor interorbital Coulomb interaction in the t(2g) manifold of the d orbitals. When spin degrees of freedom are incorporated, spontaneous orbital currents lead to two stable topological phases of the ground state. The first topological insulator is an anomalous orbital Hall phase, characterized by an even Chern number, while the second topological insulator is realized by protected mirror symmetries with a Z(2) index. C1 [Tai, Yuan-Yen; Ting, C. S.] Univ Houston, Texas Ctr Superconduct, Houston, TX 77004 USA. [Tai, Yuan-Yen; Ting, C. S.] Univ Houston, Dept Phys, Houston, TX 77004 USA. [Tai, Yuan-Yen; Wang, C. -C. Joseph; Graf, Matthias J.; Zhu, Jian-Xin] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Wang, C. -C. Joseph] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Zhu, Jian-Xin] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. RP Tai, YY (reprint author), Univ Houston, Texas Ctr Superconduct, Houston, TX 77004 USA. FU Robert A. Welch Foundation [E-1146]; AFOSR [FA9550-09-1-0656]; U.S. DOE [DE-AC52-06NA25396]; Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering; Center for Integrated Nanotechnologies, a DOE BES user facility FX We acknowledge Fan Zhang, J. Ren, G.-W. Chern, and Tanmoy Das for sharing their views on topological insulators. The work at Houston was supported in part by the Robert A. Welch Foundation under Grant No. E-1146 and AFOSR under Grant No. FA9550-09-1-0656. The work at Los Alamos was supported by the U.S. DOE Contract No. DE-AC52-06NA25396 through the LDRD program (Y.-Y.T., C.-C.J.W.), the Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering (M.J.G.). This work was supported in part by the Center for Integrated Nanotechnologies, a DOE BES user facility (J.-X. Z.). NR 41 TC 1 Z9 1 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JAN 15 PY 2015 VL 91 IS 4 AR 041111 DI 10.1103/PhysRevB.91.041111 PG 5 WC Physics, Condensed Matter SC Physics GA CE3YS UT WOS:000351766600001 ER PT J AU Sokolov, A Zhou, S Lavrentovich, OD Aranson, IS AF Sokolov, Andrey Zhou, Shuang Lavrentovich, Oleg D. Aranson, Igor S. TI Individual behavior and pairwise interactions between microswimmers in anisotropic liquid SO PHYSICAL REVIEW E LA English DT Article ID MOTILE BACTERIA; CRYSTALS AB A motile bacterium swims by generating flow in its surrounding liquid. Anisotropy of the suspending liquid significantly modifies the swimming dynamics and corresponding flow signatures of an individual bacterium and impacts collective behavior. We study the interactions between swimming bacteria in an anisotropic environment exemplified by lyotropic chromonic liquid crystal. Our analysis reveals a significant localization of the bacteria-induced flow along a line coaxial with the bacterial body, which is due to strong viscosity anisotropy of the liquid crystal. Despite the fact that the average viscosity of the liquid crystal is two to three orders of magnitude higher than the viscosity of pure water, the speed of bacteria in the liquid crystal is of the same order of magnitude as in water. We show that bacteria can transport a cargo (a fluorescent particle) along a predetermined trajectory defined by the direction of molecular orientation of the liquid crystal. We demonstrate that while the hydrodynamic interaction between flagella of two close-by bacteria is negligible, the observed convergence of the swimming speeds as well as flagella waves' phase velocities may occur due to viscoelastic interaction between the bacterial bodies. C1 [Sokolov, Andrey; Aranson, Igor S.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Zhou, Shuang; Lavrentovich, Oleg D.] Kent State Univ, Inst Liquid Crystal, Kent, OH 44242 USA. [Zhou, Shuang; Lavrentovich, Oleg D.] Kent State Univ, Chem Phys Interdisciplinary Program, Kent, OH 44242 USA. RP Sokolov, A (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM aronson@anl.gov FU U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Science and Engineering Division; U.S. National Science Foundation [DMR-1104850, DMS-1434185] FX A.S. and I.S.A. were supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Science and Engineering Division. S.Z. and O.D.L. were supported by the U.S. National Science Foundation Grants No. DMR-1104850 (Polscope analysis) and No. DMS-1434185 (reconstruction of flow patterns and estimates of elastic interactions). NR 33 TC 7 Z9 7 U1 2 U2 34 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD JAN 15 PY 2015 VL 91 IS 1 AR 013009 DI 10.1103/PhysRevE.91.013009 PG 6 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA CE6NX UT WOS:000351956100006 PM 25679710 ER PT J AU Marjuki, H Mishin, VP Chesnokov, AP Jones, J De La Cruz, JA Sleeman, K Tamura, D Nguyen, HT Wu, HS Chang, FY Liu, MT Fry, AM Cox, NJ Villanueva, JM Davis, CT Gubareva, LV AF Marjuki, Henju Mishin, Vasiliy P. Chesnokov, Anton P. Jones, Joyce De La Cruz, Juan A. Sleeman, Katrina Tamura, Daisuke Nguyen, Ha T. Wu, Ho-Sheng Chang, Feng-Yee Liu, Ming-Tsan Fry, Alicia M. Cox, Nancy J. Villanueva, Julie M. Davis, Charles T. Gubareva, Larisa V. TI Characterization of Drug-Resistant Influenza A(H7N9) Variants Isolated From an Oseltamivir-Treated Patient in Taiwan SO JOURNAL OF INFECTIOUS DISEASES LA English DT Article DE influenza virus; H7N9; oseltamivir; peramivir; R292K; E119V; I222K; I222R; mice; ferrets ID NEURAMINIDASE INHIBITOR RESISTANCE; A H7N9 VIRUS; A(H1N1) VIRUSES; R292K MUTATION; ACTIVE-SITE; FERRETS; VIRULENCE; FITNESS; TRANSMISSIBILITY; SENSITIVITY AB Background. Patients contracting influenza A(H7N9) infection often developed severe disease causing respiratory failure. Neuraminidase (NA) inhibitors (NAIs) are the primary option for treatment, but information on drug-resistance markers for influenza A(H7N9) is limited. Methods. Four NA variants of A/Taiwan/1/2013(H7N9) virus containing a single substitution (NA-E119V, NA-I222K, NA-I222R, or NA-R292K) recovered from an oseltamivir-treated patient were tested for NAI susceptibility in vitro; their replicative fitness was evaluated in cell culture, mice, and ferrets. Results. NA-R292K led to highly reduced inhibition by oseltamivir and peramivir, while NA-E119V, NA-I222K, and NA-I222R caused reduced inhibition by oseltamivir. Mice infected with any virus showed severe clinical signs with high mortality rates. NA-I222K virus was the most virulent in mice, whereas virus lacking NA change (NA-WT) and NA-R292K virus seemed the least virulent. Sequence analysis suggests that PB2-S714N increased virulence of NA-I222K virus in mice; NS1-K126R, alone or in combination with PB2-V227M, produced contrasting effects in NA-WT and NA-R292K viruses. In ferrets, all viruses replicated to high titers in the upper respiratory tract but produced only mild illness. NA-R292K virus, showed reduced replicative fitness in this animal model. Conclusions. Our data highlight challenges in assessment of the replicative fitness of H7N9 NA variants that emerged in NAI-treated patients. C1 [Marjuki, Henju; Mishin, Vasiliy P.; Chesnokov, Anton P.; Jones, Joyce; De La Cruz, Juan A.; Sleeman, Katrina; Tamura, Daisuke; Nguyen, Ha T.; Fry, Alicia M.; Cox, Nancy J.; Villanueva, Julie M.; Davis, Charles T.; Gubareva, Larisa V.] Ctr Dis Control & Prevent, Influenza Div, Natl Ctr Immunizat & Resp Dis, Atlanta, GA 30333 USA. [Chesnokov, Anton P.; De La Cruz, Juan A.; Nguyen, Ha T.] Battelle Mem Inst, Atlanta, GA USA. [Tamura, Daisuke] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. [Wu, Ho-Sheng; Chang, Feng-Yee; Liu, Ming-Tsan] Taiwan Ctr Dis Control, Taipei, Taiwan. RP Gubareva, LV (reprint author), Ctr Dis Control & Prevent, Influenza Div, Natl Ctr Immunizat & Resp Dis, 1600 Clifton Rd MS G16, Atlanta, GA 30333 USA. EM lgubareva@cdc.gov FU Centers for Disease Control and Prevention (CDC) Influenza Division; Biomedical Advanced Research and Development Authority; CDC FX This work was supported by the Centers for Disease Control and Prevention (CDC) Influenza Division and by an interagency agreement between Biomedical Advanced Research and Development Authority and the CDC. NR 46 TC 22 Z9 22 U1 1 U2 7 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 0022-1899 EI 1537-6613 J9 J INFECT DIS JI J. Infect. Dis. PD JAN 15 PY 2015 VL 211 IS 2 BP 249 EP 257 DI 10.1093/infdis/jiu447 PG 9 WC Immunology; Infectious Diseases; Microbiology SC Immunology; Infectious Diseases; Microbiology GA CC3CC UT WOS:000350221000012 PM 25124927 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adye, T Aefsky, S Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmad, A Ahmadov, F Aielli, G Kesson, TPA Akimoto, G Akimov, AV Alam, MA Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Ammosov, VV Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, TH Arfaoui, S Arguin, JF Argyropoulos, S Arik, E Arik, M Armbruster, AJ Arnaez, O Arnal, V Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ask, S Sman, B Asquith, L Assamagan, K Astalos, R Astbury, A Atkinson, M Atlay, NB Auerbach, B Auge, E Augsten, K Aurousseau, M Avolio, G Azuelos, G Azuma, Y Baak, MA Bacci, C Bach, AM Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, S Balek, P Balli, F Banas, E Banerjee, S Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Barber, T Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Bartsch, V Bassalat, A Basye, A Bates, RL Batkova, L Batley, JR Battistin, M Bauer, F Bawa, HS Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, K Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belloni, A Beloborodova, OL Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Berglund, E Beringer, J Bernard, C Bernat, P Bernhard, R Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertolucci, F Besana, MI Besjes, GJ Bessidskaia, O Besson, N Bethke, S Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biesiada, J Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Bittner, B Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blazek, T Bloch, I Blocker, C Blocki, J Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Boddy, CR Boehler, M Boek, J Boek, TT Boelaert, N Bogaerts, JA Bogdanchikov, AG Bogouch, A Bohm, C Bohm, J Boisvert, V Bold, T Boldea, V Boldyrev, AS Bolnet, NM Bomben, M Bona, M Boonekamp, M Bordoni, S Borer, C Borisov, A Borissov, G Borri, M Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boterenbrood, H Bouchami, J Boudreau, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutouil, S Boveia, A Boyd, J Boyko, IR Bozovic-Jelisavcic, I Bracinik, J Branchini, P Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brelier, B Brendlinger, K Brenner, R Bressler, S Bristow, TM Britton, D Brochu, FM Brock, I Brock, R Broggi, F Bromberg, C Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, G Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Brunet, S Bruni, A Brunia, G Bruschi, M Bryngemark, L Buanes, T Buat, Q Bucci, F Buchholz, P Buckingham, RM Buckley, AG Buda, SI Budagov, IA Budick, B Buehrer, F Bugge, L Bugge, MK Bulekov, O Bundock, AC Bunse, M Burckhart, H Burdin, S Burgess, T Burghgrave, B Burke, S Burmeister, I Busato, E Buscher, V Bussey, P Buszello, CP Butler, B Butler, JM Butt, AI Buttar, CM Butterworth, JM Buttinger, W Buzatu, A Byszewski, M Urban, SC Caforio, D Cakir, O Calafiura, P Calderini, G Calfayan, P Calkins, R Caloba, LP Caloi, R Calvet, D Calvet, S Toro, RC Camarri, P Cameron, D Caminada, LM Armadans, RC Campana, S Campanelli, M Canale, V Canelli, F Canepa, A Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Cardarelli, R Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, AA Carter, JR Carvalho, J Casadei, D Casado, MP Caso, C Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Cattani, G Caughron, S Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, B Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chan, K Chang, P Chapleau, B Chapman, JD Charfeddine, D Charlton, DG Chavda, V Barajas, CAC Cheatham, S Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, GS Chen, X Chen, Y Cheng, Y Cheplakov, A El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiefari, G Childers, JT Chilingarov, A Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Chouridou, S Chow, BKB Christidi, IA Chromek-Burckhart, D Chu, ML Chudoba, J Ciapetti, G Ciftci, AK Ciftci, R Cinca, D Cindro, V Ciocio, A Cirilli, M Cirkovic, P Citron, ZH Citterio, M Ciubancan, M Clark, A Clark, PJ Clarke, RN Cleland, W Clemens, JC Clement, B Clement, C Coadou, 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CA ATLAS Collaboration TI Jet energy measurement and its systematic uncertainty in proton-proton collisions at root s=7 TeV with the ATLAS detector SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID HEAVY-ION COLLISIONS; BARREL CALORIMETER; TRANSVERSE FLOW; CROSS-SECTIONS; BEAM TESTS; PHOTOPRODUCTION; SIMULATION; HERA; FRAGMENTATION; GENERATORS AB The jet energy scale (JES) and its systematic uncertainty are determined for jetsmeasured with the ATLAS detector using proton-proton collision data with a centre-of-mass energy of root s = 7 TeV corresponding to an integrated luminosity of 4.7 fb(-1). Jets are reconstructed from energy deposits forming topological clusters of calorimeter cells using the anti-kt algorithmwith distance parameters R = 0.4 or R = 0.6, and are calibrated using MC simulations. A residual JES correction is applied to account for differences between data and MC simulations. This correction and its systematic uncertainty are estimated using a combination of in situ techniques exploiting the transverse momentum balance between a jet and a reference object such as a photon or a Z boson, for 20 <= p(T)(jet) < 1000 GeV and pseudorapidities vertical bar eta vertical bar < 4.5. The effect of multiple proton-proton interactions is corrected for, and an uncertainty is evaluated using in situ techniques. The smallest JES uncertainty of less than 1% is found in the central calorimeter region (vertical bar eta vertical bar| < 1.2) for jets with 55 = p(T)(jet) < 500 GeV. For central jets at lower p(T), the uncertainty is about 3%. A consistent JES estimate is found using measurements of the calorimeter response of single hadrons in proton-proton collisions and test-beam data, which also provide the estimate for p(T)(jet) > 1 TeV. The calibration of forward jets is derived from dijet p(T) balance measurements. 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A.; Petersen, J.; Pomm, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Salzburger, A.; Savu, D. O.; Scanlon, T.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stewart, G. A.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Canelli, F.; Cheng, Y.; Fiascaris, M.; Gardner, R. W.; Jen-La Plante, I.; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Tuggle, J. M.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Cottin, G.; Diaz, M. A.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Shana, L. Y.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Xu, C.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing 210008, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Qingdao, Shandong, Peoples R China. [Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] IN2P3, CNRS, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Dodd, J.; Guo, J.; Hu, D.; Hughes, E. W.; Nikiforou, N.; Parsons, J. A.; Perepelitsa, D. V.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Willis, W.; Wulf, E.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Boelaert, N.; Dam, M.; Hoffmann, M. Dano; Galster, G.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Loevschall-Jensen, A. E.; Mackeprang, R.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, I-00044 Frascati, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Haleem, M.; Izen, J. M.; Lou, X.; Namasivayam, H.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Katzy, J.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Peschke, R.; Peters, R. F. Y.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Katzy, J.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Peschke, R.; Peters, R. F. Y.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Bunse, M.; Burmeister, I.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Reisinger, I.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Ciftci, R.; Czodrowski, P.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Seifert, F.; Socher, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Finelli, K. D.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Aurousseau, M.; Bhimji, W.; Bristow, T. M.; Debenedetti, C.; Edwards, N. C.; Walls, F. M. Garay; Harrington, R. D.; Korn, A.; Martin, V. J.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Aad, G.; Amoroso, S.; Barber, T.; Bernhard, R.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Jenni, P.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Madar, R.; Mahboubi, K.; Mohr, W.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Clark, P. J.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Latour, B. Martin dit; Mermod, P.; Herrera, C. Mora; Muenstermann, D.; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Caso, C.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Evangelakou, D.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Knue, A.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Meyer, J.; Morel, J.; Nackenhorst, O.; Nadal, J.; Pashapour, S.; Peters, R. F. Y.; Quadt, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Univ Grenoble 1, Lab Phys Subat & Cosmol, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] IN2P3, CNRS, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Jeanty, L.; Mateos, D. Lopez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Brandt, O.; Davygora, Y.; Dietzsch, T. A.; Dunforda, M.; Hanke, P.; Hofmann, J. I.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Lendermann, V.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulona, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kugel, A.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Evans, H.; Gagnon, P.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Whittington, D.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Olariu, A.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Karpov, S. N.; Kazarinov, M. Y.; Kharchenko, D.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Pallin, D.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Inamaru, Y.; King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Kurumida, R.; Matsushita, T.; Ochi, A.; Shimizu, S.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sasao, N.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Catmore, J. R.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; Edwards, C. A.; George, S.; Gibson, S. M.; Alo, R. Gon; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, P.] Royal Holloway Univ London, Dept Phys, London, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dobson, E.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Nash, M.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Tripiana, M. F.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Tripiana, M. F.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Tripiana, M. F.; Vannucci, F.] IN2P3, CNRS, Paris, France. [Kesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Buescher, V.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.; Wielers, M.] Lund Univ, Fys Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Arnaez, O.; Blum, W.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Fiedler, F.; Goeringer, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Neusiedl, A.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Forti, A.; Howarth, J.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Price, D.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Chen, L.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Chen, L.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] IN2P3, CNRS, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Mantifel, R.; Robertson, S. H.; Schram, M.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.] Univ Melbourne, Sch Phys, Parkville, Vic 3052, Australia. [Armbruster, A. J.; Chelstowska, M. A.; Cirilli, M.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, L.; Long, J. D.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Panikashvili, N.; Qian, J.; Scheirich, D.; Searcy, J.; Thun, R. P.; Walch, S.; Wilson, A.; Wu, Y.; Xu, L.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Ge, P.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Stelzer, H. J.; Ta, D.; Tollefson, K.; True, P.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alessandria, F.; Alimonti, G.; Andreazza, A.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Coelli, S.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Volpini, G.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Sci Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Asbah, N.; Azuelos, G.; Bouchami, J.; Dallaire, F.; Davies, M.; Gauthier, L.; Giunta, M.; Leroy, C.; Martin, J. P.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu; Tikhomirov, V. O.; Timoshenko, S.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Biebel, O.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; de Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Galea, C.; Heller, C.; Hertenberger, R.; Legger, F.; Lorenz, J.; Mann, A.; Meineck, C.; Nunnemann, T.; Oakes, L. B.; Rauscher, F.; Reznicek, P.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Schmitt, C.; Vladoiu, D.; Walker, R.; Will, J. Z.; Wittkowski, J.; Zibell, A.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bittner, B.; Bronner, J.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Giovannini, P.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Stern, S.; Stonjek, S.; Terzo, S.; Vanadia, M.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Sekhniaidzea, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Dao, V.; De Groot, N.; Filthaut, F.; Klok, P. F.; Konig, A. C.; Salvucci, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Garcia, J. A. Benitez; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Koutsman, A.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Meoni, E.; Mussche, I.; Oussoren, K. P.; Palacino, G.; Pani, P.; Codina, E. Perez; Salek, D.; Valencic, N.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Garcia, J. A. Benitez; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Koutsman, A.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Meoni, E.; Mussche, I.; Oussoren, K. P.; Palacino, G.; Pani, P.; Codina, E. Perez; Salek, D.; Valencic, N.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Burghgrave, B.; Calkins, R.; Chakraborty, D.; Cole, S.; de Lima, J. G. Rocha; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Beloborodova, O. L.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Budick, B.; Cranmer, K.; Haas, A.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.] NYU, Dept Phys, New York, NY 10003 USA. [Annovi, A.; Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. 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De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J-F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Auge, E.; Bassalat, A.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J-F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] IN2P3, CNRS, Orsay, France. [Endo, M.; Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Behr, K.; Boddy, C. R.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Larner, A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Degenhardt, J.; Desch, K.; Fratina, S.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Reece, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; VanBerg, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Donati, S.; Dotti, A.; Giannetti, P.; Roda, C.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Donati, S.; Dotti, A.; Giannetti, P.; Roda, C.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Savinov, V.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Do Valle Wemans, A.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Marques, C. N.; Oliveira, M.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Cincias, P-1699 Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Oliveira, M.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Do Valle Wemans, A.] Univ Granada, CAFPE, Granada, Spain. [Do Valle Wemans, A.] Univ Nova Lisboa, Dept Fis, Caparica, Portugal. [Do Valle Wemans, A.] Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Bohm, J.; Chudoba, J.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Dos Santos, D. Roda; Ruzicka, P.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Torregrosa, E. Fullana; Kodys, P.; Leitner, R.; Novakova, J.; Pleskot, V.; Rybar, M.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; Mattravers, C.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Nash, M.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Di Domenico, A.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Sidotia, A.; Camillocci, E. Solfaroli; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Di Domenico, A.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Marchese, F.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescua, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Grabas, H. M. X.; Guyot, C.; Hassani, S.; Kozanecki, W.; On, E. Lan; Laporte, J. F.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Mijovic, L.; Hong, V. Nguyen Thi; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.; Xu, C.] CEA Saclay Commissariat Energie Atom & Energies A, DSM IRFU Inst Rech Lois Fondamentales Univers, Gif Sur Yvette, France. [Grillo, A. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Keller, J. S.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; De Bruin, P. H. Sales; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Trottier-McDonald, M.; van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Hansson, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Batkova, L.; Blazek, T.; Federic, P.; Stavinaa, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Seman, M.; Strizenecb, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Castaneda-Miranda, E.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Carrillo-Montoya, G. D.; Huang, Y.; Leney, K. J. C.; Garcia, B. R. Mellado; Quayle, W. B.; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Sman, B.; Bendtz, K.; Bessidskaia, O.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Sman, B.; Bendtz, K.; Bessidskaia, O.; Clement, C.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Arfaoui, S.; Chen, K.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Arfaoui, S.; Chen, K.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; Cerri, A.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Rose, A.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Brelier, B.; Farooque, T.; Fatholahzadeh, B.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Losty, M. J.; Oakham, F. G.; Oram, C. J.; Savard, P.; Schouten, D.; Seustera, R.; Stelzer-Chiltona, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Bustos, A. C. Florez; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Napier, A.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Mendoza Navas, L.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Farrell, S.; Gerbaudo, D.; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Sez Trieste, Grp Collegato Udine, Trieste, Italy. [Acharya, B. S.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Garcia, E. Oliver; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Snchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Garcia, E. Oliver; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Snchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Garcia, E. Oliver; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Snchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Garcia, E. Oliver; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Snchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, CNM, IMB, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Garcia, E. Oliver; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Snchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Astbury, A.; Baker, O. K.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; Courneyea, L.; David, C.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R.; Marino, C. P.; Martyniuk, A. C.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Kimura, N.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Schaarschmidt, J.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw; Chen, X.; DosAnjos, A.; Castillo, L. R. Flores; Hard, A. S.; Jared, R. C.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Redelbach, A.; Schreyer, M.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Barisonzi, M.; Becker, K.; Beermann, T. A.; Boek, J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Hirschbuehl, D.; Kalinin, S.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Mechtel, M.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Sturm, P.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Adelman, J.; Bedikian, S.; Almenar, C. Cuenca; Cummings, J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London WC2R 2LS, England. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O. L.; Maximov, D. A.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Demirkoz, B.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gkialas, I.; Papageorgiou, K.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece. [Grinstein, S.; Juste Rozas, A.; Martinez, M.] ICREA, Barcelona, Spain. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. RI Tartarelli, Giuseppe Francesco/A-5629-2016; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Zaitsev, Alexandre/B-8989-2017; Martinez, Mario /I-3549-2015; Gabrielli, Alessandro/H-4931-2012; Peleganchuk, Sergey/J-6722-2014; Monzani, Simone/D-6328-2017; Garcia, Jose /H-6339-2015; Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014; Capua, Marcella/A-8549-2015; Demirkoz, Bilge/C-8179-2014; Mashinistov, Ruslan/M-8356-2015; Fullana Torregrosa, Esteban/A-7305-2016; Buttar, Craig/D-3706-2011; Smirnova, Oxana/A-4401-2013; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Wemans, Andre/A-6738-2012; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; Ciubancan, Liviu Mihai/L-2412-2015; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; De, Kaushik/N-1953-2013; Carvalho, Joao/M-4060-2013; Riu, Imma/L-7385-2014; Cabrera Urban, Susana/H-1376-2015; Cavalli-Sforza, Matteo/H-7102-2015; Marti-Garcia, Salvador/F-3085-2011; Della Pietra, Massimo/J-5008-2012; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Grancagnolo, Sergio/J-3957-2015; Doyle, Anthony/C-5889-2009; spagnolo, stefania/A-6359-2012; Tassi, Enrico/K-3958-2015; Ferrando, James/A-9192-2012; Livan, Michele/D-7531-2012; Moraes, Arthur/F-6478-2010; Villa, Mauro/C-9883-2009; Mir, Lluisa-Maria/G-7212-2015; White, Ryan/E-2979-2015; Brooks, William/C-8636-2013; Di Domenico, Antonio/G-6301-2011; Bosman, Martine/J-9917-2014; Joergensen, Morten/E-6847-2015; Boyko, Igor/J-3659-2013; Mitsou, Vasiliki/D-1967-2009; Carquin, Edson/G-5221-2015; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Canelli, Florencia/O-9693-2016; Staroba, Pavel/G-8850-2014; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Mindur, Bartosz/A-2253-2017; Fabbri, Laura/H-3442-2012; Gutierrez, Phillip/C-1161-2011; Gerbaudo, Davide/J-4536-2012; Solodkov, Alexander/B-8623-2017; Perrino, Roberto/B-4633-2010; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Snesarev, Andrey/H-5090-2013; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; Solfaroli Camillocci, Elena/J-1596-2012; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016 OI Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Coccaro, Andrea/0000-0003-2368-4559; Zaitsev, Alexandre/0000-0002-4961-8368; Gabrielli, Alessandro/0000-0001-5346-7841; Peleganchuk, Sergey/0000-0003-0907-7592; Monzani, Simone/0000-0002-0479-2207; Grancagnolo, Francesco/0000-0002-9367-3380; Korol, Aleksandr/0000-0001-8448-218X; Giordani, Mario/0000-0002-0792-6039; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Mashinistov, Ruslan/0000-0001-7925-4676; Fullana Torregrosa, Esteban/0000-0003-3082-621X; Smirnova, Oxana/0000-0003-2517-531X; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Wemans, Andre/0000-0002-9669-9500; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Camarri, Paolo/0000-0002-5732-5645; Tikhomirov, Vladimir/0000-0002-9634-0581; Warburton, Andreas/0000-0002-2298-7315; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; De, Kaushik/0000-0002-5647-4489; Carvalho, Joao/0000-0002-3015-7821; Riu, Imma/0000-0002-3742-4582; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Grancagnolo, Sergio/0000-0001-8490-8304; Doyle, Anthony/0000-0001-6322-6195; spagnolo, stefania/0000-0001-7482-6348; Ferrando, James/0000-0002-1007-7816; Livan, Michele/0000-0002-5877-0062; Moraes, Arthur/0000-0002-5157-5686; Villa, Mauro/0000-0002-9181-8048; Mir, Lluisa-Maria/0000-0002-4276-715X; White, Ryan/0000-0003-3589-5900; Brooks, William/0000-0001-6161-3570; Di Domenico, Antonio/0000-0001-8078-2759; Bosman, Martine/0000-0002-7290-643X; Joergensen, Morten/0000-0002-6790-9361; Boyko, Igor/0000-0002-3355-4662; Mitsou, Vasiliki/0000-0002-1533-8886; Carquin, Edson/0000-0002-7863-1166; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Canelli, Florencia/0000-0001-6361-2117; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Perrino, Roberto/0000-0002-5764-7337; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Mora Herrera, Maria Clemencia/0000-0003-3915-3170 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET; ERC; NSRF; European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; ICORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT , Japan; JSPS, Japan; CNRST, Morocco; FOM , Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern, Switzerland; Cantons of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, ICORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSFand Cantons of Bern andGeneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier 1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 100 TC 6 Z9 6 U1 11 U2 86 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JAN 15 PY 2015 VL 75 IS 1 AR 17 DI 10.1140/epjc/s10052-014-3190-y PG 101 WC Physics, Particles & Fields SC Physics GA CA6AY UT WOS:000348991900001 ER PT J AU Lopez, CA Bellesia, G Redondo, A Langan, P Chundawat, SPS Dale, BE Marrink, SJ Gnanakaran, S AF Lopez, Cesar A. Bellesia, Giovanni Redondo, Antonio Langan, Paul Chundawat, Shishir P. S. Dale, Bruce E. Marrink, Siewert J. Gnanakaran, S. TI MARTINI Coarse-Grained Model for Crystalline Cellulose Microfibers SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID X-RAY; LIGNOCELLULOSIC BIOMASS; NATIVE CELLULOSE; ELASTIC-MODULUS; FORCE-FIELD; I-BETA; INTERCONVERSION; TRANSFORMATION; SPECTROSCOPY; PRETREATMENT AB Commercial-scale biofuel production requires a deep understanding of the structure and dynamics of its principal target: cellulose. However, an accurate description and modeling of this carbohydrate structure at the mesoscale remains elusive, particularly because of its overwhelming length scale and configurational complexity. We have derived a set of MARTINI coarse-grained force field parameters for the simulation of crystalline cellulose fibers. The model is adapted to reproduce different physicochemical and mechanical properties of native cellulose I beta. The model is able not only to handle a transition from cellulose I beta to another cellulose allomorph, cellulose IIII, but also to capture the physical response to temperature and mechanical bending of longer cellulose nanofibers. By developing the MARTINI model of a solid cellulose crystalline fiber from the building blocks of a soluble cellobiose coarse-grained model, we have provided a systematic way to build MARTINI models for other crystalline biopolymers. C1 [Lopez, Cesar A.; Redondo, Antonio; Gnanakaran, S.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Bellesia, Giovanni] Univ Calif Santa Barbara, Dept Comp Sci, Santa Barbara, CA 93106 USA. [Langan, Paul] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Chundawat, Shishir P. S.] DOE Great Lakes Bioenergy Res Ctr, E Lansing, MI 48824 USA. [Chundawat, Shishir P. S.; Dale, Bruce E.] Michigan State Univ, GLBRC, Biomass Convers Res Lab, Dept Chem Engn & Mat Sci, Lansing, MI 48824 USA. [Marrink, Siewert J.] Univ Groningen, Groningen Biomol Sci & Biotechnol Inst, NL-9747 AG Groningen, Netherlands. [Marrink, Siewert J.] Univ Groningen, Zernike Inst Adv Mat, NL-9747 AG Groningen, Netherlands. RP Gnanakaran, S (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM gnana@lanl.gov RI Langan, Paul/N-5237-2015; Marrink, Siewert /G-3706-2014; OI Langan, Paul/0000-0002-0247-3122; Chundawat, Shishir/0000-0003-3677-6735; Gnanakaran, S/0000-0002-9368-3044; Lopez Bautista, Cesar/0000-0003-4684-3364 FU National Advanced Biofuels Consortium (NABC); Center for Nonlinear Studies; Laboratory Directed Research and Development (LDRD) Program at Los Alamos National Laboratory (LANL); DOE Great Lakes Bioenergy Research Center (DOE BER Office of Science) [DE-FC02-07ER64494] FX This work was supported by the National Advanced Biofuels Consortium (NABC), the Center for Nonlinear Studies, and the Laboratory Directed Research and Development (LDRD) Program at Los Alamos National Laboratory (LANL). S.P.S.C. and B.E.D. acknowledge support from the DOE Great Lakes Bioenergy Research Center (DOE BER Office of Science DE-FC02-07ER64494). We thank Jennifer Macke for editing the manuscript. NR 45 TC 9 Z9 9 U1 5 U2 30 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JAN 15 PY 2015 VL 119 IS 2 BP 465 EP 473 DI 10.1021/jp5105938 PG 9 WC Chemistry, Physical SC Chemistry GA AZ2XX UT WOS:000348093700008 PM 25417548 ER PT J AU Chialvo, AA Vlcek, L AF Chialvo, Ariel A. Vlcek, Lukas TI NO3- Coordination in Aqueous Solutions by N-15/N-14 and O-18/O-nat Isotopic Substitution: What Can We Learn from Molecular Simulation? SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID X-RAY-DIFFRACTION; ION-SOLVENT INTERACTIONS; CALCIUM NITRATE SOLUTIONS; RAMAN-SPECTROSCOPY; NEUTRON-DIFFRACTION; HYDRATION STRUCTURE; SYMMETRY-BREAKING; CONCENTRATION-DEPENDENCE; INFRARED-SPECTROSCOPY; ELECTROLYTE SOLUTIONS AB We explore the deconvolution of waternitrate correlations by the first-order difference approach involving neutron diffraction of heavy- and null-aqueous solutions of KNO3 under N-14/N-15 and O-nat(N)/O-18(N) substitutions to achieve a full characterization of the first water coordination around the nitrate ion. For that purpose we performed isobaricisothermal simulations of 3.5 m KNO3 aqueous solutions at ambient conditions to generate the relevant radial distribution functions required in the analysis (a) to identify the individual partial contributions to the total neutron-weighted distribution function, (b) to isolate and assess the contribution of NO3-.....K+ pair formation, (c) to test the accuracy of the neutron diffraction with isotope substitution based coordination calculations and X-ray diffraction based assumptions, and (d) to describe the water coordination around both the nitrogen and oxygen sites of the nitrate ion. C1 [Chialvo, Ariel A.; Vlcek, Lukas] Oak Ridge Natl Lab, Div Chem Sci, Geochem & Interfacial Sci Grp, Oak Ridge, TN 37831 USA. [Vlcek, Lukas] Oak Ridge Natl Lab, Joint Inst Computat Sci, Oak Ridge, TN 37831 USA. RP Chialvo, AA (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Geochem & Interfacial Sci Grp, Oak Ridge, TN 37831 USA. EM chialvoaa@ornl.gov RI Vlcek, Lukas/N-7090-2013; OI Vlcek, Lukas/0000-0003-4782-7702; Chialvo, Ariel/0000-0002-6091-4563 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division FX This work was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. NR 100 TC 6 Z9 6 U1 5 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JAN 15 PY 2015 VL 119 IS 2 BP 519 EP 531 DI 10.1021/jp510355u PG 13 WC Chemistry, Physical SC Chemistry GA AZ2XX UT WOS:000348093700015 PM 25514621 ER PT J AU Cosmidis, J Benzerara, K Nassif, N Tyliszczak, T Bourdelle, F AF Cosmidis, Julie Benzerara, Karim Nassif, Nadine Tyliszczak, Tolek Bourdelle, Franck TI Characterization of Ca-phosphate biological materials by scanning transmission X-ray microscopy (STXM) at the Ca L-2,L-3-, P L-2,L-3- and C K-edges SO ACTA BIOMATERIALIA LA English DT Article DE X-ray microscopy; Ca-phosphates; Polyphosphate; Nanoscale; XANES spectroscopy ID TRANSIENT PRECURSOR STRATEGY; CALCIUM-DEFICIENT APATITE; STRUCTURAL-CHARACTERIZATION; CARBONATED HYDROXYAPATITE; INORGANIC POLYPHOSPHATE; OCTACALCIUM PHOSPHATE; XANES SPECTROSCOPY; DISSOLUTION RATES; MARINE-SEDIMENTS; BONE APATITE AB Several naturally occurring biological materials, including bones and teeth, pathological calcifications, microbial mineral deposits formed in marine phosphogenesis areas, as well as bin-inspired cements used for bone and tooth repair are composed of Ca-phosphates. These materials are usually identified and characterized using bulk-scale analytical tools such as X-ray diffraction, Fourier transform infrared spectroscopy or nuclear magnetic resonance. However, there is a need for imaging techniques that provide information on the spatial distribution and chemical composition of the Ca-phosphate phases at the micrometer- and nanometer scales. Such analyses provide insightful indications on how the materials may have formed, e.g. through transient precursor phases that eventually remain spatially separated from the mature phase. Here, we present scanning transmission X-ray microscopy (STXM) analyses of Ca-phosphate reference compounds, showing the feasibility of fingerprinting Ca-phosphate-based materials. We calibrate methods to determine important parameters of Ca-phosphate phases, such as their Ca/P ratio and carbonate content at the similar to 25 nm scale, using X-ray absorption near-edge spectra at the C K-, Ca L-2,L-3- and P L-2,L-3-edges. As an illustrative case study, we also perform STXM analyses on hydroxyapatite precipitates formed in a dense fibrillar collagen matrix. This study paves the way for future research on Ca-phosphate biomineralization processes down to the scale of a few tens of nanometers. (C) 2014 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Cosmidis, Julie; Benzerara, Karim] Univ Paris 06, Univ Paris 04, Inst Mineral Phys Mat & Cosmochim, CNRS UMR 7590,MNHN,IRD UMR 206, F-75252 Paris 05, France. [Nassif, Nadine] Univ Paris 06, Lab Chim Mat Condensee LMCM, CNRS UMR 7574, Coll France, F-75231 Paris 05, France. [Tyliszczak, Tolek] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Bourdelle, Franck] Univ Lille 1, Lab Genie Civil & Geoenvironm LGCgE, F-59655 Villeneuve Dascq, France. RP Benzerara, K (reprint author), Univ Paris 06, Univ Paris 04, Inst Mineral Phys Mat & Cosmochim, CNRS UMR 7590,MNHN,IRD UMR 206, F-75252 Paris 05, France. EM karim.benzerara@impmc.upmc.fr RI IMPMC, Geobio/F-8819-2016; Benzerara, Karim/J-1532-2016 OI Benzerara, Karim/0000-0002-0553-0137 FU Simone and Cino Del Duca Fundation; European Research Council under the European Community [307110 - ERC CALCYAN]; Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences and Materials Sciences Division, U.S. Department of Energy, at the Lawrence Berkeley National Laboratory; NSERC; CIHR; NRC; University of Saskatchewan FX We thank Florence Babonneau, Yan Wang, Stanislas Von Euw, Christian Bonhomme and Frederique Pourpoint (College de France and UPMC, Paris), for providing some of the reference Ca-phosphates used in this study. Haohao Yi and Etienne Balan (IMPMC, Paris) are also thanked for providing compounds and analyses. We gratefully acknowledge support from the Simone and Cino Del Duca Fundation for funding J.C.'s salary. Part of the research leading to these results received funding from the European Research Council under the European Community's Seventh Framework Programme (FP7/2007-2013 Grant Agreement no.307110 - ERC CALCYAN). Advanced Light Source (ALS) Molecular Environmental Science beamline 11.0.2 is supported by the Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences and Materials Sciences Division, U.S. Department of Energy, at the Lawrence Berkeley National Laboratory. Beamline 10ID-1 at the CLS is supported by the NSERC, the CIHR, the NRC and the University of Saskatchewan. We thank Chithra Karunakaran and Jian Wang for their support of the STXM at the CLS. The authors are indebted to Hannah Miller (University of Colorado) for proofreading this article. NR 88 TC 10 Z9 10 U1 8 U2 60 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1742-7061 EI 1878-7568 J9 ACTA BIOMATER JI Acta Biomater. PD JAN 15 PY 2015 VL 12 BP 260 EP 269 DI 10.1016/j.actbio.2014.10.003 PG 10 WC Engineering, Biomedical; Materials Science, Biomaterials SC Engineering; Materials Science GA CA1QF UT WOS:000348686100027 PM 25305511 ER PT J AU Liezers, M Farmer, OT Dion, MP Thomas, ML Eiden, GC AF Liezers, M. Farmer, O. T., III Dion, M. P. Thomas, M. L. Eiden, G. C. TI The production of ultra-high purity single isotopes or tailored isotope mixtures by ICP-MS SO INTERNATIONAL JOURNAL OF MASS SPECTROMETRY LA English DT Article DE Isotope enrichment; ICP-MS; Ion implantation; Isotope dilution; Laser ablation ID PLASMA-MASS-SPECTROMETRY; ENERGY; SEPARATION; PLUTONIUM AB We report the development and testing of a collector arrangement for quadrupole inductively coupled plasma mass spectrometry (ICP-MS) that for the first time has been used to isolate small quantities of highly enriched (>99.99%) single isotopes, with deposition rates >10 ng h(-1). The collector assembly replaces the standard instrument detector allowing for implantation with simultaneous monitoring of the incident ion current. Even under zero bias implant conditions, low energy (<10 eV) ion, collection efficiency was observed to be very high 99%. Eu-151 ion currents of 0.1-0.5 nA were collected on a simple, planar foil without resorting to any type of cup configuration. Recovery of the enriched isotope from such foils is much simpler than from a more complex cup configuration. High rejection of adjacent mass isotopes was demonstrated by selectively implanting Er-167, then using laser ablation ICP-MS imaging to confirm the absence of any co-implanted Er-166 or Er-168. The important analytical possibilities of this new approach to isotope ratio measurement, tracer purification, and radiation measurements are discussed. (C) 2014 Elsevier B.V. All rights reserved. C1 [Liezers, M.; Farmer, O. T., III; Dion, M. P.; Thomas, M. L.; Eiden, G. C.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Liezers, M (reprint author), Pacific NW Natl Lab, POB 999, Richland, WA 99352 USA. EM martin.liezers@pnnl.gov OI Dion, Michael/0000-0002-3030-0050 NR 21 TC 5 Z9 5 U1 2 U2 8 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1387-3806 EI 1873-2798 J9 INT J MASS SPECTROM JI Int. J. Mass Spectrom. PD JAN 15 PY 2015 VL 376 BP 58 EP 64 DI 10.1016/j.ijms.2014.11.004 PG 7 WC Physics, Atomic, Molecular & Chemical; Spectroscopy SC Physics; Spectroscopy GA CA4NC UT WOS:000348880200012 ER PT J AU Li, ZS Potapenko, DV Rim, KT Flytzani-Stephanopoulos, M Flynn, GW Osgood, RM Wen, XD Batista, ER AF Li, Zhisheng Potapenko, Denis V. Rim, Kwang Taeg Flytzani-Stephanopoulos, Maria Flynn, George W. Osgood, Richard M. Wen, Xiao-Dong Batista, Enrique R. TI Reactions of Deuterated Methanol (CD3OD) on Fe3O4(111) SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SCANNING-TUNNELING-MICROSCOPY; AUGMENTED-WAVE METHOD; OXIDE SURFACES; EPITAXIAL FE3O4(111); HYDROGEN-PRODUCTION; WATER-ADSORPTION; FUEL-CELL; CCL4; CHEMISTRY; FEO(111) AB We report an experimental and theoretical investigation of the decomposition (partial oxidation) of deuterated methanol (CD3OD) on a single-crystal Fe3O4(111) surface. The crystal surface contains majority areas of a Fe-terminated Fe3O4(111) surface as well as smaller regions of O-terminated FeO(111) or biphase surface reconstruction. Our investigation uses a combination of scanning tunneling microscopy, temperature-programmed desorption, and density functional theory calculations to examine the surface reactions and adsorbates as a function of coverage. Our studies show that the reaction of methanol on this ironoxide surface is highly sensitive to atomic-level surface reconstructions. C1 [Li, Zhisheng; Potapenko, Denis V.; Osgood, Richard M.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. [Rim, Kwang Taeg; Flynn, George W.] Columbia Univ, Dept Chem, New York, NY 10027 USA. [Rim, Kwang Taeg; Flynn, George W.] Columbia Univ, Nanoscale Sci & Engn Ctr, New York, NY 10027 USA. [Flytzani-Stephanopoulos, Maria] Tufts Univ, Dept Chem & Biol Engn, Medford, MA 02155 USA. [Wen, Xiao-Dong] Chinese Acad Sci, Inst Coal Chem, State Key Lab Coal Convers, Taiyuan 030001, Shanxi, Peoples R China. [Wen, Xiao-Dong] Synfuels China, Beijing 100195, Peoples R China. [Wen, Xiao-Dong; Batista, Enrique R.] Los Alamos Natl Lab, Theoret Div, Los Alamos, NM 87545 USA. RP Osgood, RM (reprint author), Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. EM osgood@columbia.edu FU U.S. Department of Energy [DE-FG02-90ER14104, DE-FG02-05ER15730, DE-FG02-88ER13937]; EFRC [DE-SC0001085]; New York State Office of Science, Technology, and Academic Research (NYSTAR); National Science Foundation [CHE-07-01483, CHE-10-12058, DMR-1206768]; LDRD program at LANL; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC5206NA25396] FX We are indebted to Professor Jonathan Owen for stimulating discussions about iron-oxide chemistry and surface structure. This work was funded by the U.S. Department of Energy under Grant nos. DE-FG02-90ER14104 (R.M.O.), DE-FG02-05ER15730 (M.F.-S. and G.W.F.), DE-FG02-88ER13937 (G.W.F), and EFRC Award DE-SC0001085 (G.W.F.). We acknowledge financial support from the New York State Office of Science, Technology, and Academic Research (NYSTAR). Equipment and material support was provided by the National Science Foundation under grants CHE-07-01483, CHE-10-12058 (G.W.F.), and DMR-1206768 (R.M.O.). Work at Los Alamos National Laboratory (E.R.B., X.-D.W.) was supported by LDRD program at LANL. Some of the calculations were performed on the Chinook and Cascade computing systems at the Environmental Molecular Sciences Laboratory (EMSL) at PNNL. The Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-AC5206NA25396. NR 35 TC 1 Z9 1 U1 5 U2 23 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 15 PY 2015 VL 119 IS 2 BP 1113 EP 1120 DI 10.1021/jp510821g PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AZ2YA UT WOS:000348094000028 ER PT J AU Kim, B Kay, BD Dohnalek, Z Kim, YK AF Kim, Boseong Kay, Bruce D. Dohnalek, Zdenek Kim, Yu Kwon TI Ammonia Formation from NO Reaction with Surface Hydroxyls on Rutile TiO2(110)-1 x 1 SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SELECTIVE CATALYTIC-REDUCTION; OXYGEN VACANCIES; NITRIC-OXIDE; DISSOCIATIVE ADSORPTION; TIO2 SURFACES; WATER; CHEMISTRY; NH3; CHEMISORPTION; TITANIA AB The reaction of NO with the hydroxylated rutile TiO2(110)-1 x 1 surface (h-TiO2) was investigated as a function of NO coverage using temperature-programmed desorption. Our results show that NO reaction with h-TiO2 leads to formation of NH3, which is observed to desorb at similar to 400 K. Interestingly, the amount of NH3 produced depends nonlinearly on the dose of NO. The yield increases up to a saturation value of similar to 1.3 x 10 (13) NH3/cm(2) at a NO dose of 5 x 10(-13) NO/cm(2), but subsequently decreases at higher NO doses. Preadsorbed H2O is found to have a negligible effect on the NH3 desorption yield. Additionally, no NH3 is formed in the absence of surface hydroxyls (HObs) upon coadsorption of NO and (HO)-O-2 on a stoichiometric TiO2(110) (s-TiO2(110)). On the basis of these observations, we conclude that nitrogen from NO has a strong preference to react with HObs on the bridge-bonded oxygen rows (but not with H2O) to form NH3. The absolute NH3 yield is limited by competing reactions of HOb species with titanium-bound oxygen adatoms to form H2O. Our results provide new mechanistic insight about the interactions of NO with hydroxyl groups on TiO2(110). C1 [Kim, Boseong; Kim, Yu Kwon] Ajou Univ, Dept Energy Syst Res, Suwon 443749, South Korea. [Kim, Boseong; Kim, Yu Kwon] Ajou Univ, Dept Chem, Suwon 443749, South Korea. [Kay, Bruce D.; Dohnalek, Zdenek] Pacific NW Natl Lab, Chem & Mat Sci Div, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. RP Kim, YK (reprint author), Ajou Univ, Dept Energy Syst Res, Suwon 443749, South Korea. EM yukwonkim@ajou.ac.kr FU U.S. Department of Energy Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences; Department of Energy's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory (PNNL); U.S. DOE by Battelle Memorial Institute [DE-AC06-76RLO 1830]; National Research Foundation of Korea (NRF) - Ministry of Education, Science and Technology [NRF-2012R1A1A2007641] FX Part of this work was supported by the U.S. Department of Energy Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences, and performed at EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory (PNNL). PNNL is operated for the U.S. DOE by Battelle Memorial Institute under Contract No. DE-AC06-76RLO 1830. Y.K.K. acknowledges financial support from the Basic Science Research Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Education, Science and Technology (NRF-2012R1A1A2007641). NR 48 TC 1 Z9 1 U1 2 U2 30 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JAN 15 PY 2015 VL 119 IS 2 BP 1130 EP 1135 DI 10.1021/jp5109619 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA AZ2YA UT WOS:000348094000030 ER PT J AU Al-Qaradawi, I Abdel-Moati, M Al-Yafei, MAA Al-Ansari, E Al-Maslamani, I Holm, E Al-Shaikh, I Mauring, A Pinto, PV Abdulmalik, D Amir, A Miller, M Yigiterhan, O Persson, B AF Al-Qaradawi, Ilham Abdel-Moati, Mohamed Al-Yafei, Mohsin Al-Ansi Al-Ansari, Ebrahim Al-Maslamani, Ibrahim Holm, Elis Al-Shaikh, Ismail Mauring, Alexander Pinto, Primal V. Abdulmalik, Dana Amir, Amina Miller, Mark Yigiterhan, Oguz Persson, Bertil TI Radioactivity levels in the marine environment along the Exclusive Economic Zone (EEZ) of Qatar SO MARINE POLLUTION BULLETIN LA English DT Article DE Caesium-137; Radium-226; Uranium-238; Marine environment; Food-web representatives; EEZ of Qatar ID SPATIAL-DISTRIBUTION; HONG-KONG; CS-137; RADIONUCLIDES; SEDIMENTS; SEAWATER; PACIFIC; WATERS; TH-232; KUWAIT AB A study on (137)cs, K-40, Ra-226, Ra-228, and U-238 was carried out along the EEZ of Qatar. Results serve as the first ever baseline data. The level of Cs-132 (mean value 1.6 +/- 0.4 Bq m(-3)) in water filters was found to be in the same order of magnitude as reported by others in worldwide marine radioactivity studies. Results are also in agreement with values reported from other Gulf regions. The computed values of sediment-water distribution coefficients K-d, are lower than the values given by IAEA. Measurements were carried out for bottom sediments, biota samples like fish, oyster, sponge, seashell, mangrove, crab, shrimp, starfish, dugong and algae. The 'concentration factors' reported for biota samples are below the levels published by IAEA and cause no significant impact on human health for seafood consumers in Qatar. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Al-Qaradawi, Ilham; Pinto, Primal V.; Abdulmalik, Dana] Qatar Univ, Dept Phys, Doha, Qatar. [Abdel-Moati, Mohamed] Minist Environm, Doha, Qatar. [Al-Yafei, Mohsin Al-Ansi; Al-Ansari, Ebrahim; Al-Maslamani, Ibrahim; Al-Shaikh, Ismail; Yigiterhan, Oguz] Qatar Univ, Ctr Environm Studies, Doha, Qatar. [Holm, Elis; Mauring, Alexander] Norwegian Radiat Protect Author, Osteras, Norway. [Amir, Amina] Albayan Educ Complex, Doha, Qatar. [Miller, Mark] Sandia Natl Labs, Albuquerque, NM USA. [Persson, Bertil] Lund Univ, Dept Med Radiat Phys, S-22100 Lund, Sweden. RP Al-Qaradawi, I (reprint author), Qatar Univ, Dept Phys, Doha, Qatar. EM ilham@qu.edu.qa FU Qatar National Research Fund (QNRF), National Priorities Research Program (NPRP) project [NPRP 09-889-1-134] FX The authors would like to thank Qatar National Research Fund (QNRF) for funding this project as part of the National Priorities Research Program (NPRP) project number: NPRP 09-889-1-134. Thanks are due to Environmental Studies Centre of Qatar University for providing the Research Vessel used for the collection of samples and the Central Laboratory at Qatar University, for the ICPMS measurements. We would like to acknowledge the Wadsworth Center, New York and the Norwegian Radiation Protection Authority (NRPA) for their measurement of some of the samples for quality assurance. NR 30 TC 3 Z9 3 U1 6 U2 20 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0025-326X EI 1879-3363 J9 MAR POLLUT BULL JI Mar. Pollut. Bull. PD JAN 15 PY 2015 VL 90 IS 1-2 BP 323 EP 329 DI 10.1016/j.marpolbul.2014.10.021 PG 7 WC Environmental Sciences; Marine & Freshwater Biology SC Environmental Sciences & Ecology; Marine & Freshwater Biology GA CA5QX UT WOS:000348964000050 PM 25480154 ER PT J AU Chiang, JCH Fung, IY Wu, CH Cai, YH Edman, JP Liu, YW Day, JA Bhattacharya, T Mondal, Y Labrousse, CA AF Chiang, John C. H. Fung, Inez Y. Wu, Chi-Hua Cai, Yanjun Edman, Jacob P. Liu, Yuwei Day, Jesse A. Bhattacharya, Tripti Mondal, Yugarshi Labrousse, Clothilde A. TI Role of seasonal transitions and westerly jets in East Asian paleoclimate SO QUATERNARY SCIENCE REVIEWS LA English DT Article DE Paleoclimate; East Asian monsoon; Westerlies ID SUMMER MONSOON; TIBETAN PLATEAU; NORTH-ATLANTIC; MERIDIONAL TELECONNECTION; INTERANNUAL VARIABILITY; MODERN PRECIPITATION; MILLENNIAL-SCALE; ORBITAL-SCALE; PART I; CLIMATE AB The summer rainfall climate of East Asia underwent large and abrupt changes during past climates, in response to precessional forcing, glacial interglacial cycles as well as abrupt changes to the North Atlantic during the Last Glacial. However, current interpretations of said changes are typically formulated in terms of modulation of summer monsoon intensity, and do not account for the known complexity in the seasonal evolution of East Asian rainfall, which exhibits sharp transition from the Spring regime to the Meiyu, and then again from the Meiyu to the Summer regime. We explore the interpretation that East Asian rainfall climate undergoes a modulation of its seasonality during said paleoclimate changes. Following previous suggestions we focus on role of the westerly jet over Asia, namely that its latitude relative to Tibet is critical in determining the stepwise transitions in East Asian rainfall seasons. In support of this linkage, we show from observational data that the interannual co-variation of June (July August) rainfall and upper tropospheric zonal winds show properties consistent with an altered timing of the transition to the Meiyu (Summer), and with more northwardshifted westerlies for earlier transitions. We similarly suggest that East Asian paleoclimate changes resulted from an altered timing in the northward evolution of the jet and hence the seasonal transitions, in particular the transition of the jet from south of the Plateau to the north that determines the seasonal transition from Spring rains to the Meiyu. In an extreme scenario which we speculate the climate system tended towards during stadial (cold) phases of D/O stadials and periods of low Northern Hemisphere summer insolation the jet does not jump north of the Plateau, essentially keeping East Asia in prolonged Spring conditions. We argue that this hypothesis provides a viable explanation for a key paleoproxy signature of D/O stadials over East Asia, namely the heavier mean delta O-18 of precipitation as recorded in speleothem records. The southward jet position prevents the low-level monsoonal flow which is isotopically light from penetrating into the interior of East Asia; as such, precipitation there will be heavier, consistent with speleothem records. This hypothesis can also explain other key evidences of East Asian paleoclimate changes, in particular the occurrence of dusty conditions during North Atlantic stadials, and the southward migration of the Holocene optimal rainfall. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Chiang, John C. H.; Liu, Yuwei; Bhattacharya, Tripti; Mondal, Yugarshi; Labrousse, Clothilde A.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Chiang, John C. H.; Wu, Chi-Hua] Acad Sinica, Res Ctr Environm Changes, Taipei 115, Taiwan. [Wu, Chi-Hua; Edman, Jacob P.; Day, Jesse A.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Cai, Yanjun] Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian, Peoples R China. [Cai, Yanjun] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Chiang, JCH (reprint author), Univ Calif Berkeley, 547 McCone Hall, Berkeley, CA 94720 USA. EM jch_chiang@berkeley.edu RI Cai, Yanjun/A-9462-2010; Wu, Chi-Hua/K-5130-2016; Day, Jesse/N-7805-2014; OI Wu, Chi-Hua/0000-0001-9692-1418; Day, Jesse/0000-0003-1621-0742; Bhattacharya, Tripti/0000-0002-5528-3760 FU NSF [AGS-1405479, EAR-0909195] FX This work started from a graduate seminar on the East Asian paleomonsoon taught at UC Berkeley by JC and IF in the Spring of 2013. We acknowledge support from NSF grants AGS-1405479 (to JC) and EAR-0909195 (to IF); JC also acknowledges support from a Visiting Associate Professorship at Academia Sinica during Spring 2014, funded by the Consortium for Climate Change Study under the auspices of the Ministry of Science and Technology (MOST), Taiwan. CHW was also supported by MOST under grant 100-2119-M-001-029-MY5. Reinhard Schiemann kindly provided the jet occurrence data used in Fig. 7. We thank Zhisheng An, David Battisti, Huang-Hsiung Hsu, Shang-Ping Xie, Wenwen Kong and Kristina Lofman for valuable discussions. JC thanks the proprietors and staff of Fortunate Coffee for their hospitality during the writing of the manuscript. NR 64 TC 20 Z9 21 U1 5 U2 34 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0277-3791 J9 QUATERNARY SCI REV JI Quat. Sci. Rev. PD JAN 15 PY 2015 VL 108 BP 111 EP 129 DI 10.1016/j.quascirev.2014.11.009 PG 19 WC Geography, Physical; Geosciences, Multidisciplinary SC Physical Geography; Geology GA CA5PJ UT WOS:000348960000008 ER PT J AU Cheng, L Assary, RS Qu, XH Jain, A Ong, SP Rajput, NN Persson, K Curtiss, LA AF Cheng, Lei Assary, Rajeev S. Qu, Xiaohui Jain, Anubhav Ong, Shyue Ping Rajput, Nay Nidhi Persson, Kristin Curtiss, Larry A. TI Accelerating Electrolyte Discovery for Energy Storage with High-Throughput Screening SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID ORGANIC PHOTOVOLTAICS; SURFACE-CHEMISTRY; QUANTUM-CHEMISTRY; BATTERY; DECOMPOSITION; DESIGN; POTENTIALS; ENERGETICS; SOLVENTS; SALTS AB Computational screening techniques have been found to be an effective alternative to the trial and error of experimentation for discovery of new materials. With increased interest in development of advanced electrical energy storage systems, it is essential to find new electrolytes that function effectively. This Perspective reviews various methods for screening electrolytes and then describes a hierarchical computational scheme to screen multiple properties of advanced electrical energy storage electrolytes using high-throughput quantum chemical calculations. The approach effectively down-selects a large pool of candidates based on successive property evaluation. As an example, results of screening are presented for redox potentials, solvation energies, and structural changes of similar to 1400 organic molecules for nonaqueous redox flow batteries. Importantly, on the basis of high-throughput screening, in silico design of suitable candidate molecules for synthesis and electrochemical testing can be achieved. We anticipate that the computational approach described in this Perspective coupled with experimentation will have a significant role to play in the discovery of materials for future energy needs. C1 [Cheng, Lei; Assary, Rajeev S.; Curtiss, Larry A.] Argonne Natl Lab, Mat Sci Div, Argonne, IL 60439 USA. [Qu, Xiaohui; Jain, Anubhav; Rajput, Nay Nidhi; Persson, Kristin] Lawrence Berkeley Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Ong, Shyue Ping] Univ Calif San Diego, Dept NanoEngn, La Jolla, CA 92093 USA. RP Persson, K (reprint author), Lawrence Berkeley Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM kapersson@lbl.gov; curtiss@anl.gov RI Ong, Shyue Ping/D-7573-2014; Surendran Assary, Rajeev/E-6833-2012 OI Ong, Shyue Ping/0000-0001-5726-2587; Surendran Assary, Rajeev/0000-0002-9571-3307 FU U.S. Department of Energy, Basic Energy Science, Joint Center for Energy Storage Research [DE-AC02-06CH11357]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Materials Project (BES DOE) [EDCBEE] FX Support for this work came from the U.S. Department of Energy, Basic Energy Science, Joint Center for Energy Storage Research under Contract No. DE-AC02-06CH11357. The calculations were performed using the computational resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The Materials Project (BES DOE Grant No. EDCBEE) is gratefully acknowledged for infrastructure and software support. NR 35 TC 48 Z9 48 U1 18 U2 95 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JAN 15 PY 2015 VL 6 IS 2 BP 283 EP 291 DI 10.1021/jz502319n PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA AZ2XS UT WOS:000348093300005 PM 26263464 ER PT J AU Park, JS Kang, JG Yang, JH Metzger, W Wei, SH AF Park, Ji-Sang Kang, Joongoo Yang, Ji-Hui Metzger, Wyatt Wei, Su-Huai TI Stability and electronic structure of the low-Sigma grain boundaries in CdTe: a density functional study SO NEW JOURNAL OF PHYSICS LA English DT Article DE grain bondaries; II-VI semiconductors; impurity and defect levels in semiconductors; radiation effects in semiconductors ID SOLAR-CELLS; PERFORMANCE; FILMS; SI AB Using first-principles density functional calculations, we investigate the relative stability and electronic structure of the grain boundaries (GBs) in zinc-blende CdTe. Among the low-Sigma-value symmetric tilt Sigma 3 (111), Sigma 3 (112), Sigma 5 (120), and Sigma 5 (130) GBs, we show that the Sigma 3 (111) GB is always the most stable due to the absence of dangling bonds and wrong bonds. The Sigma 5 (120) GBs, however, are shown to be more stable than the Sigma 3 (112) GBs, even though the former has a higher Sigma value, and the latter is often used as a model system to study GB effects in zinc-blende semiconductors. Moreover, we find that although containing wrong bonds, the Sigma 5 (120) GBs are electrically benign due to the short wrong bond lengths, and thus are not as harmful as the Sigma 3 (112) GBs also having wrong bonds but with longer bond lengths. C1 [Park, Ji-Sang; Yang, Ji-Hui; Metzger, Wyatt; Wei, Su-Huai] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Kang, Joongoo] DGIST, Dept Emerging Mat Sci, Taegu 711873, South Korea. RP Park, JS (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM Suhuai.Wei@nrel.gov RI Park, Ji-Sang/F-9944-2010 OI Park, Ji-Sang/0000-0002-1374-8793 FU U.S. Department of Energy, EERE [DE-AC36-08GO28308]; DGIST MIREBraiN Program FX The work at NREL was supported by the U.S. Department of Energy, EERE, under contract no. DE-AC36-08GO28308. The work at DGIST was supported by the DGIST MIREBraiN Program. NR 37 TC 10 Z9 10 U1 1 U2 27 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD JAN 15 PY 2015 VL 17 AR 013027 DI 10.1088/1367-2630/17/1/013027 PG 7 WC Physics, Multidisciplinary SC Physics GA CA2TB UT WOS:000348759300012 ER PT J AU Huang, SY Gao, YF An, K Zheng, LL Wu, W Teng, ZK Liaw, PK AF Huang, Shenyan Gao, Yanfei An, Ke Zheng, Lili Wu, Wei Teng, Zhenke Liaw, Peter K. TI Deformation mechanisms in a precipitation-strengthened ferritic superalloy revealed by in situ neutron diffraction studies at elevated temperatures SO ACTA MATERIALIA LA English DT Article DE Neutron diffraction; Ferritic superalloy; High-temperature deformation behavior ID GRAIN-BOUNDARY DIFFUSION; RECOVERABLE CREEP DEFORMATION; NI-CR ALLOYS; PLASTIC-DEFORMATION; ELASTIC-CONSTANTS; SINGLE-CRYSTALS; ALPHA-IRON; FE; MICROSTRUCTURE; POLYCRYSTALS AB The ferritic superalloy Fe-10Ni-6.5Al-10Cr-3.4Mo strengthened by ordered (Ni,Fe)Al B2-type precipitates is a candidate material for ultra-supercritical steam turbine applications above 923 K. Despite earlier success in improving its room-temperature ductility, the creep resistance of this material at high temperatures needs to be further improved, which requires a fundamental understanding of the high-temperature deformation mechanisms at the scales of individual phases and grains. In situ neutron diffraction has been utilized to investigate the lattice strain evolution and the microscopic load-sharing mechanisms during tensile deformation of this ferritic superalloy at elevated temperatures. Finite-element simulations based on the crystal plasticity theory are employed and compared with the experimental results, both qualitatively and quantitatively. Based on these interphase and intergranular load-partitioning studies, it is found that the deformation mechanisms change from dislocation slip to those related to dislocation climb, diffusional flow and possibly grain boundary sliding, below and above 873 K, respectively. Insights into microstructural design for enhancing creep resistance are also discussed. (C) 2014 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Huang, Shenyan; Gao, Yanfei; Zheng, Lili; Wu, Wei; Teng, Zhenke; Liaw, Peter K.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Gao, Yanfei] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [An, Ke] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. RP Gao, YF (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. EM ygao7@utk.edu; pliaw@utk.edu RI Gao, Yanfei/F-9034-2010; An, Ke/G-5226-2011; OI Gao, Yanfei/0000-0003-2082-857X; An, Ke/0000-0002-6093-429X; Wu, Wei/0000-0002-8596-9253 FU U.S. Department of Energy (DOE), Office of Fossil Energy [DE-FG26-09NT0008089, DE-FE0005868]; National Science Foundation [CMMI 0800168]; Center for Defect Physics, an Energy Frontier Research Center - DOE Office of Science, Basic Energy Sciences; Scientific User Facilities Division of the DOE Office of Science, Basic Energy Sciences FX This work was supported by the U.S. Department of Energy (DOE), Office of Fossil Energy, under Grants DE-FG26-09NT0008089 and DE-FE0005868, with Vito Cedro and Richard Dunst as program managers, respectively (S.Y.H., W.W., Z.K.T. and P.K.L.), by the National Science Foundation CMMI 0800168 (L.L.Z.), and by the Center for Defect Physics, an Energy Frontier Research Center funded by the DOE Office of Science, Basic Energy Sciences (Y.F.G.). A portion of this research at the Spallation Neutron Source, Oak Ridge National Laboratory, was sponsored by the Scientific User Facilities Division of the DOE Office of Science, Basic Energy Sciences. The authors thank Ms. Rebecca Mills, Mr. Harley Skorpenske and Mr. Michael Rawlings for their experimental assistance. NR 39 TC 12 Z9 12 U1 4 U2 41 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD JAN 15 PY 2015 VL 83 BP 137 EP 148 DI 10.1016/j.actamat.2014.09.053 PG 12 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA AY5AL UT WOS:000347585800014 ER PT J AU Henze, GP Pavlak, GS Florita, AR Dodier, RH Hirsch, AI AF Henze, Gregor P. Pavlak, Gregory S. Florita, Anthony R. Dodier, Robert H. Hirsch, Adam I. TI An energy signal tool for decision support in building energy systems SO APPLIED ENERGY LA English DT Article DE Decision support; Operational building energy modeling; Bayesian updating ID VERIFICATION; UNCERTAINTY; MANAGEMENT AB A prototype energy signal tool is demonstrated for operational whole-building and system-level energy use evaluation. The purpose of the tool is to give a summary of building energy use which allows a building operator to quickly distinguish normal and abnormal energy use. Toward that end, energy use status is displayed as a traffic light, which is a visual metaphor for energy use which is substantially different from expected (red and yellow lights) or more or less the same as expected (green light). Which light to display for a given energy end-use is determined by comparing expected energy use to actual energy use. As expected energy use is necessarily uncertain, we cannot choose the appropriate light with certainty. Instead the energy signal tool chooses the light by minimizing the expected cost of displaying the wrong light. The expected energy use is represented by a probability distribution. Energy use is modeled by a low-order lumped parameter model. Uncertainty in energy use is quantified by a Monte Carlo exploration of the influence of model parameters on energy use. Distributions over model parameters are updated over time via Bayes' theorem. The simulation study is devised to assess whole building energy signal accuracy in the presence of uncertainty and faults at the submetered level, which may lead to tradeoffs at the whole building level not detectable without submetering. Published by Elsevier Ltd. C1 [Henze, Gregor P.; Pavlak, Gregory S.; Florita, Anthony R.] Univ Colorado, Dept Civil Environm & Architectural Engn, Boulder, CO 80309 USA. [Henze, Gregor P.; Hirsch, Adam I.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Henze, GP (reprint author), Univ Colorado, Dept Civil Environm & Architectural Engn, Boulder, CO 80309 USA. EM gregor.henze@colorado.edu RI Henze, Gregor/C-5505-2015; Pavlak, Gregory/M-9907-2015 OI Henze, Gregor/0000-0002-4084-9709; Pavlak, Gregory/0000-0003-4734-0750 NR 59 TC 4 Z9 4 U1 2 U2 10 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD JAN 15 PY 2015 VL 138 BP 51 EP 70 DI 10.1016/j.apenergy.2014.10.029 PG 20 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA AY4ZF UT WOS:000347582700006 ER PT J AU Wang, Q Zhang, CY Ding, Y Xydis, G Wang, JH Ostergaard, J AF Wang, Qi Zhang, Chunyu Ding, Yi Xydis, George Wang, Jianhui Ostergaard, Jacob TI Review of real-time electricity markets for integrating Distributed Energy Resources and Demand Response SO APPLIED ENERGY LA English DT Article DE Distributed Energy Resource; Demand Response; Real-time electricity market; Renewable energy; Smart grid ID STRATEGIES; IMPACTS; SYSTEM AB The high penetration of both Distributed Energy Resources (DER) and Demand Response (DR) in modern power systems requires a sequence of advanced strategies and technologies for maintaining system reliability and flexibility. Real-time electricity markets (RTM) are the non-discriminatory transaction platforms for providing necessary balancing services, where the market clearing (nodal or zonal prices depending on markets) is very close to real time operations of power systems. One of the primary functions of RTMs in modem power systems is establishing an efficient and effective mechanism for small DER and DR to participate in balancing market transactions, while handling their meteorological or intermittent characteristics, facilitating asset utilization, and stimulating their active responses. Consequently, RTMs are dedicated to maintaining the flexibility and reliability of power systems. This paper reviews advanced typical RTMs respectively in the North America, Australia and Europe, focusing on their market architectures and incentive policies for integrating DER and DR in electricity markets. In this paper, RTMs are classified into three groups: Group I applies nodal prices implemented by optimal power flow, which clears energy prices every 5 min. Group II applies zonal prices, with the time resolution of 5-min. Group III is a general balancing market, which clears zonal prices intro-hourly. The various successful advanced RTM experiences have been summarized and discussed, which provides a technical overview of the present RTMs integrating DER and DR. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Wang, Qi; Zhang, Chunyu; Ding, Yi; Ostergaard, Jacob] Tech Univ Denmark, Dept Elect Engn, DK-2800 Lyngby, Denmark. [Xydis, George] Ctr Res & Technol Hellas, Inst Res & Technol Thessaly, Volos, Greece. [Wang, Jianhui] Argonne Natl Lab, Decis & Informat Sci Div, Argonne, IL 60439 USA. [Ding, Yi] Zhejiang Univ, Coll Elect Engn, Hangzhou 310003, Zhejiang, Peoples R China. RP Ding, Y (reprint author), Tech Univ Denmark, Elektrovej, DK-2800 Lyngby, Denmark. EM qiwa@elektro.dtu.dk; chzh@elektro.dtu.dk; yding@elektro.dtu.dk; gxydis@mail.ireteth.certh.gr; jianhui.wang@anl.gov; joe@elektro.dtu.dk FU iPower FX The authors would like to acknowledge the iPower for funding this research and Dr. Peter Meibom, the Danish Energy analysis manager and Honorary Professor at the Department of Management Engineering, Technical University of Denmark, for the grant given of constructive comments and suggestions. NR 82 TC 33 Z9 33 U1 4 U2 33 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD JAN 15 PY 2015 VL 138 BP 695 EP 706 DI 10.1016/j.apenergy.2014.10.048 PG 12 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA AY4ZF UT WOS:000347582700061 ER PT J AU Ahn, TH Chai, JJ Pan, CL AF Ahn, Tae-Hyuk Chai, Juanjuan Pan, Chongle TI Sigma: Strain-level inference of genomes from metagenomic analysis for biosurveillance SO BIOINFORMATICS LA English DT Article; Proceedings Paper CT 14th Annual Bioinformatics Open Source Conference (BOSC) CY JUL 19-20, 2013 CL Special Interest Grp, Berlin, GERMANY SP Open Bioinformat Fdn HO Special Interest Grp ID HUMAN MICROBIOME; SEQUENCES AB Motivation: Metagenomic sequencing of clinical samples provides a promising technique for direct pathogen detection and characterization in biosurveillance. Taxonomic analysis at the strain level can be used to resolve serotypes of a pathogen in biosurveillance. Sigma was developed for strain-level identification and quantification of pathogens using their reference genomes based on metagenomic analysis. Results: Sigma provides not only accurate strain-level inferences, but also three unique capabilities: (i) Sigma quantifies the statistical uncertainty of its inferences, which includes hypothesis testing of identified genomes and confidence interval estimation of their relative abundances; (ii) Sigma enables strain variant calling by assigning metagenomic reads to their most likely reference genomes; and (iii) Sigma supports parallel computing for fast analysis of large datasets. The algorithm performance was evaluated using simulated mock communities and fecal samples with spike-in pathogen strains. C1 [Ahn, Tae-Hyuk; Chai, Juanjuan; Pan, Chongle] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. EM panc@ornl.gov FU Laboratory Directed Research and Development (LDRD) - Oak Ridge National Laboratory [DE-AC05-00OR22725]; Office of Advanced Scientific Computing Research; Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725] FX The authors would like to thank Richard Stouder, Loren Hauser, and Robert Cottingham for their support and assistance. This work was supported by Laboratory Directed Research and Development (LDRD) funding from Oak Ridge National Laboratory. The contribution of J.C. was sponsored by the Office of Advanced Scientific Computing Research. This research used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. NR 27 TC 11 Z9 11 U1 2 U2 12 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 1367-4803 EI 1460-2059 J9 BIOINFORMATICS JI Bioinformatics PD JAN 15 PY 2015 VL 31 IS 2 BP 170 EP 177 DI 10.1093/bioinformatics/btu641 PG 8 WC Biochemical Research Methods; Biotechnology & Applied Microbiology; Computer Science, Interdisciplinary Applications; Mathematical & Computational Biology; Statistics & Probability SC Biochemistry & Molecular Biology; Biotechnology & Applied Microbiology; Computer Science; Mathematical & Computational Biology; Mathematics GA AY8WU UT WOS:000347832300004 PM 25266224 ER PT J AU Harris, NL Cock, PJA Chapman, BA Goecks, J Hotz, HR Lapp, H AF Harris, Nomi L. Cock, Peter J. A. Chapman, Brad A. Goecks, Jeremy Hotz, Hans-Rudolf Lapp, Hilmar TI The Bioinformatics Open Source Conference (BOSC) 2013 SO BIOINFORMATICS LA English DT Editorial Material C1 [Harris, Nomi L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Cock, Peter J. A.] James Hutton Inst, Dundee DD2 5DA, Scotland. [Chapman, Brad A.] Harvard Univ, Sch Publ Hlth, Bioinformat Core, Boston, MA 02115 USA. [Goecks, Jeremy] George Washington Univ, Computat Biol Inst, Washington, DC 20052 USA. [Hotz, Hans-Rudolf] Friedrich Miescher Inst Biomed Res, Bioinformat Dept, CH-4058 Basel, Switzerland. [Lapp, Hilmar] Natl Evolutionary Synth Ctr NESCent, Durham, NC 27705 USA. RP Harris, NL (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, MS 972R525, Berkeley, CA 94720 USA. OI Cock, Peter/0000-0001-9513-9993 FU NHGRI NIH HHS [HG005133, HG005542, HG006620, R21 HG005133, RC2 HG005542, U41 HG006620] NR 3 TC 1 Z9 1 U1 1 U2 2 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 1367-4803 EI 1460-2059 J9 BIOINFORMATICS JI Bioinformatics PD JAN 15 PY 2015 VL 31 IS 2 BP 299 EP 300 DI 10.1093/bioinformatics/btu413 PG 2 WC Biochemical Research Methods; Biotechnology & Applied Microbiology; Computer Science, Interdisciplinary Applications; Mathematical & Computational Biology; Statistics & Probability SC Biochemistry & Molecular Biology; Biotechnology & Applied Microbiology; Computer Science; Mathematical & Computational Biology; Mathematics GA AY8WU UT WOS:000347832300032 PM 25024288 ER PT J AU Neppl, S Ernstorfer, R Cavalieri, AL Lemell, C Wachter, G Magerl, E Bothschafter, EM Jobst, M Hofstetter, M Kleineberg, U Barth, JV Menzel, D Burgdorfer, J Feulner, P Krausz, F Kienberger, R AF Neppl, S. Ernstorfer, R. Cavalieri, A. L. Lemell, C. Wachter, G. Magerl, E. Bothschafter, E. M. Jobst, M. Hofstetter, M. Kleineberg, U. Barth, J. V. Menzel, D. Burgdoerfer, J. Feulner, P. Krausz, F. Kienberger, R. TI Direct observation of electron propagation and dielectric screening on the atomic length scale SO NATURE LA English DT Article ID METAL-SURFACES; PHOTOEMISSION; SPECTROSCOPY AB The propagation and transport of electrons in crystals is a fundamental process pertaining to the functioning of most electronic devices. Microscopic theories describe this phenomenon as being based on the motion of Bloch wave packets(1). These wave packets are superpositions of individual Bloch states with the group velocity determined by the dispersion of the electronic band structure near the central wavevector in momentum space1. This concept has been verified experimentally in artificial superlattices by the observation of Bloch oscillations(2)-periodic oscillations of electrons in real and momentum space. Here we present a direct observation of electron wave packet motion in a real-space and real-time experiment, on length and time scales shorter than the Bloch oscillation amplitude and period. We show that attosecond metrology(3) (1 as=10(-18) seconds) now enables quantitative insight into weakly disturbed electron wave packet propagation on the atomic length scale without being hampered by scattering effects, which inevitably occur over macroscopic propagation length scales. Weuse sub-femtosecond(less than 10(-15) seconds) extreme-ultraviolet light pulses(3) to launch photoelectron wave packets inside a tungsten crystal that is covered by magnesium films of varied, well-defined thicknesses of a few angstroms(4). Probing the moment of arrival of the wave packets at the surface with attosecond precision reveals free-electron-like, ballistic propagation behaviour inside the magnesium adlayer-constituting the semi-classical limit of Bloch wave packet motion. Real-time access to electron transport through atomic layers and interfaces promises unprecedented insight into phenomena that may enable the scaling of electronic and photonic circuits to atomic dimensions. In addition, this experiment allows us to determine the penetration depth of electrical fields at optical frequencies at solid interfaces on the atomic scale. C1 [Neppl, S.; Jobst, M.; Barth, J. V.; Menzel, D.; Feulner, P.; Kienberger, R.] Tech Univ Munich, Dept Phys, D-85747 Garching, Germany. [Neppl, S.; Magerl, E.; Jobst, M.; Hofstetter, M.; Kleineberg, U.; Krausz, F.; Kienberger, R.] Max Planck Inst Quantum Opt, D-85748 Garching, Germany. [Ernstorfer, R.; Menzel, D.] Max Planck Gesell, Fritz Haber Inst, D-14195 Berlin, Germany. [Cavalieri, A. L.] Max Planck Inst Struct & Dynam Matter, D-22761 Hamburg, Germany. [Cavalieri, A. L.] Univ Hamburg, Fak Math Informat & Nat Wissensch, D-22761 Hamburg, Germany. [Cavalieri, A. L.] Ctr Free Electron Laser Sci CFEL, D-22761 Hamburg, Germany. [Lemell, C.; Wachter, G.; Burgdoerfer, J.] Vienna Univ Technol, Inst Theoret Phys, A-1040 Vienna, Austria. [Bothschafter, E. M.; Hofstetter, M.; Kleineberg, U.; Krausz, F.] Univ Munich, Fak Phys, D-85748 Garching, Germany. [Burgdoerfer, J.] Hungarian Acad Sci ATOMKI, Inst Nucl Res, H-4001 Debrecen, Hungary. RP Neppl, S (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM sneppl@lbl.gov; reinhard.kienberger@tum.de RI BARTH, Johannes/E-4060-2013; Lemell, Christoph/B-5147-2009; Bothschafter, Elisabeth/D-4021-2016; Ernstorfer, Ralph/D-1590-2009; OI BARTH, Johannes/0000-0002-6270-2150; Lemell, Christoph/0000-0003-2560-4495; Ernstorfer, Ralph/0000-0001-6665-3520; Menzel, Dietrich/0000-0002-7188-8532 FU Munich-Centre for Advanced Photonics; FWF special research programs [SFB-041, SFB-049, P21141-N16]; International Max Planck Research School for Advanced Photon Science (IMPRS-APS); ERC; Helmholtz Zentrum Berlin FX This research was supported by the Munich-Centre for Advanced Photonics. C.L., G.W. and J.B. acknowledge support by the FWF special research programs SFB-041 (ViCoM) and SFB-049 (NextLite) and project P21141-N16. G.W. is supported by the International Max Planck Research School for Advanced Photon Science (IMPRS-APS). R.K. acknowledges an ERC Starting Grant Calculations have been performed on the Vienna Scientific Cluster. S.N. and P.F. thank the Helmholtz Zentrum Berlin for support. We thank P. Echenique, E. E. Krasovskii, A. Kazansky and A. D. Sanchez-Portal for discussions. NR 30 TC 47 Z9 47 U1 16 U2 120 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD JAN 15 PY 2015 VL 517 IS 7534 BP 342 EP 346 DI 10.1038/nature14094 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AY8NK UT WOS:000347810300040 PM 25592539 ER PT J AU Plata, G Henry, CS Vitkup, D AF Plata, German Henry, Christopher S. Vitkup, Dennis TI Long-term phenotypic evolution of bacteria SO NATURE LA English DT Article ID GENETIC INTERACTION NETWORKS; SCALE METABOLIC RECONSTRUCTIONS; GENERATION; CONSERVATION; STRAINS; MODELS AB For many decades comparative analyses of protein sequences and structures have been used to investigate fundamental principles of molecular evolution(1,2). In contrast, relatively little is known about the long-term evolution of species' phenotypic and genetic properties. This represents an important gap in our understanding of evolution, as exactly these proprieties play key roles in natural selection and adaptation to diverse environments. Here we perform a comparative analysis of bacterial growth and gene deletion phenotypes using hundreds of genome-scale metabolic models. Overall, bacterial phenotypic evolution can be described by a two-stage process with a rapid initial phenotypic diversification followed by a slow long-term exponential divergence. The observed average divergence trend, with approximately similar fractions of phenotypic properties changing per unit time, continues for billions of years. We experimentally confirm the predicted divergence trend using the phenotypic profiles of 40 diverse bacterial species across more than 60 growth conditions. Our analysis suggests that, at long evolutionary distances, gene essentiality is significantly more conserved than the ability to utilize different nutrients, while synthetic lethality is significantly less conserved. We also find that although a rapid phenotypic evolution is sometimes observed within the same species, a transition from high to low phenotypic similarity occurs primarily at the genus level. C1 [Plata, German; Vitkup, Dennis] Columbia Univ, Dept Syst Biol, Ctr Computat Biol & Bioinformat, New York, NY 10032 USA. [Plata, German] Columbia Univ, Integrated Program Cellular Mol Struct & Genet St, New York, NY 10032 USA. [Henry, Christopher S.] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. [Vitkup, Dennis] Columbia Univ, Dept Biomed Informat, New York, NY 10032 USA. RP Vitkup, D (reprint author), Columbia Univ, Dept Syst Biol, Ctr Computat Biol & Bioinformat, New York, NY 10032 USA. EM dv2121@columbia.edu OI Plata, German/0000-0002-6470-7748 FU National Institute of General Medical Sciences [GM079759, U54CA121852]; Department of Energy, as part of the SB Knowledgebase [DE-AC02-06CH11357] FX We thank B. Bochner and Biolog for providing the experimental phenotypic growth data. We also thank members of the Vitkup laboratory for discussions. This work was supported in part by the National Institute of General Medical Sciences GM079759 grant to D.V. and the U54CA121852 grant to Columbia University. The work by C.S.H. was supported by the Department of Energy contract DE-AC02-06CH11357, as part of the SB Knowledgebase. NR 30 TC 15 Z9 15 U1 2 U2 36 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD JAN 15 PY 2015 VL 517 IS 7534 BP 369 EP U498 DI 10.1038/nature13827 PG 16 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AY8NK UT WOS:000347810300046 PM 25363780 ER PT J AU Li, LZ Bayn, I Lu, M Nam, CY Schroder, T Stein, A Harris, NC Englund, D AF Li, Luozhou Bayn, Igal Lu, Ming Nam, Chang-Yong Schroeder, Tim Stein, Aaron Harris, Nicholas C. Englund, Dirk TI Nanofabrication on unconventional substrates using transferred hard masks SO SCIENTIFIC REPORTS LA English DT Article ID ELECTRON-BEAM LITHOGRAPHY; SINGLE-CRYSTAL DIAMOND; PHOTONIC-CRYSTAL; SOFT LITHOGRAPHY; GAN NANOWIRES; FABRICATION; RESOLUTION; RESIST; SCATTERING; CIRCUITS AB A major challenge in nanofabrication is to pattern unconventional substrates that cannot be processed for a variety of reasons, such as incompatibility with spin coating, electron beam lithography, optical lithography, or wet chemical steps. Here, we present a versatile nanofabrication method based on re-usable silicon membrane hard masks, patterned using standard lithography and mature silicon processing technology. These masks, transferred precisely onto targeted regions, can be in the millimetre scale. They allow for fabrication on a wide range of substrates, including rough, soft, and non-conductive materials, enabling feature linewidths down to 10 nm. Plasma etching, lift-off, and ion implantation are realized without the need for scanning electron/ion beam processing, UV exposure, or wet etching on target substrates. C1 [Li, Luozhou; Bayn, Igal; Schroeder, Tim; Harris, Nicholas C.; Englund, Dirk] MIT, Dept Elect Engn & Comp Sci, Cambridge, MA 02139 USA. [Lu, Ming; Nam, Chang-Yong; Stein, Aaron] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Li, LZ (reprint author), MIT, Dept Elect Engn & Comp Sci, Cambridge, MA 02139 USA. EM luozhou@mit.edu; englund@mit.edu RI Schroder, Tim/M-8624-2014; OI Schroder, Tim/0000-0001-9017-0254; Stein, Aaron/0000-0003-4424-5416 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]; Alexander von Humboldt Foundation FX Research was carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. The authors thank M. Liu, F. Camino and F. Najafi for their invaluable assistance, and M. Cotlet for training us on optical measurements. T. Schroder was supported by the Alexander von Humboldt Foundation. NR 56 TC 8 Z9 9 U1 2 U2 50 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 15 PY 2015 VL 5 AR 7802 DI 10.1038/srep07802 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AY9WP UT WOS:000347898700002 PM 25588550 ER PT J AU Sun, C Zheng, S Wei, CC Wu, Y Shao, L Yang, Y Hartwig, KT Maloy, SA Zinkle, SJ Allen, TR Wang, H Zhang, X AF Sun, C. Zheng, S. Wei, C. C. Wu, Y. Shao, L. Yang, Y. Hartwig, K. T. Maloy, S. A. Zinkle, S. J. Allen, T. R. Wang, H. Zhang, X. TI Superior radiation-resistant nanoengineered austenitic 304L stainless steel for applications in extreme radiation environments SO SCIENTIFIC REPORTS LA English DT Article ID HEAVY-ION IRRADIATION; IN-SITU; MICROSTRUCTURAL EVOLUTION; STRUCTURAL-MATERIALS; GRAIN-BOUNDARIES; NEUTRON; METALS; DAMAGE; ALLOYS; REACTORS AB Nuclear energy provides more than 10% of electrical power internationally, and the increasing engagement of nuclear energy is essential to meet the rapid worldwide increase in energy demand. A paramount challenge in the development of advanced nuclear reactors is the discovery of advanced structural materials that can endure extreme environments, such as severe neutron irradiation damage at high temperatures. It has been known for decades that high dose radiation can introduce significant void swelling accompanied by precipitation in austenitic stainless steel (SS). Here we report, however, that through nanoengineering, ultra-fine grained (UFG) 304L SS with an average grain size of similar to 100 nm, can withstand Fe ion irradiation at 500 degrees C to 80 displacements-per-atom (dpa) with moderate grain coarsening. Compared to coarse grained (CG) counterparts, swelling resistance of UFG SS is improved by nearly an order of magnitude and swelling rate is reduced by a factor of 5. M23C6 precipitates, abundant in irradiated CG SS, are largely absent in UFG SS. This study provides a nanoengineering approach to design and discover radiation tolerant metallic materials for applications in extreme radiation environments. C1 [Sun, C.; Hartwig, K. T.; Zhang, X.] Texas A&M Univ, Dept Mat Sci & Engn, College Stn, TX 77843 USA. [Sun, C.; Zheng, S.; Maloy, S. A.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Wei, C. C.; Shao, L.] Texas A&M Univ, Dept Nucl Engn, College Stn, TX 77843 USA. [Wu, Y.; Yang, Y.] Univ Florida, Dept Mat Sci & Engn, Nucl Engn Program, Gainesville, FL 32611 USA. [Zinkle, S. J.] Univ Tennessee, Dept Nucl Engn, Knoxville, TN 37996 USA. [Allen, T. R.] Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA. [Wang, H.] Texas A&M Univ, Dept Elect & Comp Engn, College Stn, TX 77843 USA. [Zhang, X.] Texas A&M Univ, Dept Mech Engn, College Stn, TX 77843 USA. RP Zhang, X (reprint author), Texas A&M Univ, Dept Mat Sci & Engn, College Stn, TX 77843 USA. EM zhangx@tamu.edu RI Maloy, Stuart/A-8672-2009; OI Maloy, Stuart/0000-0001-8037-1319; Allen, Todd/0000-0002-2372-7259; Zinkle, Steven/0000-0003-2890-6915 FU NSF-DMR-Metallic Materials and Nanostructures Program [1304101]; DOE-NEUP [DE-AC07-05ID14517-00088120]; LANL LDRD program [20130118DR] FX We acknowledge financial support by NSF-DMR-Metallic Materials and Nanostructures Program under grant no. 1304101. Dr. C. Sun was supported by DOE-NEUP under contract no. DE-AC07-05ID14517-00088120 and currently by LANL LDRD program # 20130118DR. We also acknowledge the access to the DOE - Center for Integrated Nanotechnologies (CINT) at Los Alamos and Sandia National Laboratories. Access to the microscopy and imaging center (MIC) at Texas A&M University is also acknowledged. NR 52 TC 12 Z9 12 U1 11 U2 59 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 15 PY 2015 VL 5 AR 7801 DI 10.1038/srep07801 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AY9WP UT WOS:000347898700001 PM 25588326 ER PT J AU Wang, ZY Zhang, RJ Wang, SY Lu, M Chen, X Zheng, YX Chen, LY Ye, Z Wang, CZ Ho, KM AF Wang, Z. Y. Zhang, R. J. Wang, S. Y. Lu, M. Chen, X. Zheng, Y. X. Chen, L. Y. Ye, Z. Wang, C. Z. Ho, K. M. TI Broadband optical absorption by tunable Mie resonances in silicon nanocone arrays SO SCIENTIFIC REPORTS LA English DT Article ID NANOPILLAR ARRAYS; LIGHT-SCATTERING; MATRIX-METHOD; NANOSTRUCTURES; RESONATORS; SIMULATION; SURFACE; DESIGN AB Nanostructure arrays such as nanowire, nanopillar, and nanocone arrays have been proposed to be promising antireflection structures for photovoltaic applications due to their great light trapping ability. In this paper, the optical properties of Si nanopillar and nanocone arrays in visible and infrared region were studied by both theoretical calculations and experiments. The results show that the Mie resonance can be continuously tuned across a wide range of wavelength by varying the diameter of the nanopillars. However, Si nanopillar array with uniform diameter exhibits only discrete resonance mode, thus can't achieve a high broadband absorption. On the other hand, the Mie resonance wavelength in a Si nanocone array can vary continuously as the diameters of the cross sections increase from the apex to the base. Therefore Si nanocone arrays can strongly interact with the incident light in the broadband spectrum and the absorbance by Si nanocone arrays is higher than 95% over the wavelength from 300 to 2000 nm. In addition to the Mie resonance, the broadband optical absorption of Si nanocone arrays is also affected by Wood-Rayleigh anomaly effect and metal impurities introduced in the fabrication process. C1 [Wang, Z. Y.; Zhang, R. J.; Wang, S. Y.; Lu, M.; Zheng, Y. X.; Chen, L. Y.] Fudan Univ, Shanghai Engn Res Ctr Ultra Precis Opt Mfg, Shanghai 200433, Peoples R China. [Wang, Z. Y.; Zhang, R. J.; Wang, S. Y.; Lu, M.; Zheng, Y. X.; Chen, L. Y.] Fudan Univ, Dept Opt Sci & Engn, Shanghai 200433, Peoples R China. [Wang, S. Y.] Key Lab Informat Sci Electromagnet Waves MoE, Shanghai 200433, Peoples R China. [Wang, S. Y.; Ye, Z.; Wang, C. Z.; Ho, K. M.] Iowa State Univ, US Dept Energy, Ames Lab, Ames, IA 50011 USA. [Wang, S. Y.; Ye, Z.; Wang, C. Z.; Ho, K. M.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Chen, X.] Chinese Acad Sci, Shanghai Inst Tech Phys, Natl Lab Infrared Phys, Shanghai 200083, Peoples R China. RP Zhang, RJ (reprint author), Fudan Univ, Shanghai Engn Res Ctr Ultra Precis Opt Mfg, Shanghai 200433, Peoples R China. EM rjzhang@fudan.edu.cn; songyouwang@fudan.edu.cn RI Zhang, Rong-jun/B-1436-2012; Wang, Songyou/H-4529-2011; Wang, Zi Yi/D-6456-2015; OI Wang, Songyou/0000-0002-4249-3427; Zheng, Yu-Xiang/0000-0002-9116-4849 FU National Basic Research Program of China [2010CB933703, 2012CB934303]; Natural Science Foundation of China [11174058, 11374055, 61275160, 61427815]; National Science and Technology Major Project of China [2011ZX02109-004]; Fudan High-end computing center; US Department of Energy, Basic Energy Sciences; National Energy Research Scientific Computing Centre (NERSC) in Berkeley, CA [DE-AC02-07CH11358]; Division of Materials Science and Engineering FX Thanks to the insightful discussions with T.N. Zhang, Y. Zhang, X. C. Song and Y. Qiu. The work at Fudan university was supported by National Basic Research Program of China (No. 2010CB933703 and 2012CB934303), Natural Science Foundation of China (Grant No. 11174058, 11374055, 61275160 and 61427815), the No. 2 National Science and Technology Major Project of China (No. 2011ZX02109-004), and the Fudan High-end computing center. Work at Ames Laboratory was supported by the US Department of Energy, Basic Energy Sciences, and Division of Materials Science and Engineering, including a grant of computer time at the National Energy Research Scientific Computing Centre (NERSC) in Berkeley, CA under Contract No. DE-AC02-07CH11358. NR 34 TC 32 Z9 32 U1 17 U2 125 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JAN 15 PY 2015 VL 5 AR 7810 DI 10.1038/srep07810 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA AY9WR UT WOS:000347898900004 PM 25589290 ER PT J AU Vanderhoof, MK Williams, CA AF Vanderhoof, Melanie K. Williams, Christopher A. TI Persistence of MODIS evapotranspiration impacts from mountain pine beetle outbreaks in lodgepole pine forests, south-central Rocky Mountains SO AGRICULTURAL AND FOREST METEOROLOGY LA English DT Article DE Evapotranspiration; Water cycle; Bark beetles; Mountain pine beetles; Disturbance; MODIS ID SUB-ALPINE FOREST; ENERGY-EXCHANGE; WATER YIELD; STAND AGE; LEAF-AREA; VEGETATION; ALGORITHM; COLORADO; CARBON; SCALE AB The current extent and high severity (percent tree mortality) of mountain pine beetle outbreaks across western North America has been attributed to regional climate change, specifically warmer summer and winter temperatures and drier summers. This study paired multiple mountain pine beetle outbreak location datasets, both current and historical, with Moderate Resolution Imaging Spectroradiometer (MODIS) and Global Modeling and Assimilation Office (GMAO) Modern Era Retrospective-Analysis for Research and Applications (MERRA) products in order to quantify the full seasonal evapotranspiration impact of outbreak events for decades after outbreak (0 to 60 years). Following mountain pine beetle outbreaks in lodgepole pine (Pinus contorta) stands in the Colorado Rockies we observed an 18.7 +/- 1.4% (p < 0.01) reduction in the rate of summer evapotranspiration at 14 to 20 years since outbreak. We also observed a 21.6 +/- 2.2% (p < 0.01) increase in the rate of summer evapotranspiration, relative to non-attacked stands, in intermediate-aged stands 30 to 40 years since outbreak. Changes to growing season evapotranspiration correlated positively with changes in stand density, stand leaf area index (LAI) and the fraction of absorbed photosynthetically active radiation (fPAR), while high incoming solar radiation during the summer months acted to amplify changes to evapotranspiration even given relatively minor changes to summer WAR and LAI due to the rapid regeneration of understory vegetation. Lodgepole pine mortality from mountain pine beetle outbreaks showed lasting effects on stand-scale evapotranspiration which could have important implications for regional water resources. (C) 2014 Elsevier B.V. All rights reserved. C1 [Vanderhoof, Melanie K.; Williams, Christopher A.] Clark Univ, Grad Sch Geog, Worcester, MA 01610 USA. RP Vanderhoof, MK (reprint author), US EPA, ORISE, Off Res & Dev, Natl Ctr Environm Assessment, 1200 Penn Ave,NW 8623-P, Washington, DC 20460 USA. EM vanderhoof.melanie@epa.gov FU NASA Headquarters under the NASA Earth and Space Science Fellowship Program [12-Earth12R-59, 13-Earth13R-8]; Science of Terra and Aqua program [NASA ROSES09, NNX11AG53G]; National Science Foundation [1262691] FX This work was supported by NASA Headquarters under the NASA Earth and Space Science Fellowship Program (Grant no. 12-Earth12R-59 and 13-Earth13R-8). Additional financial support was received from the NASA ROSES09 Science of Terra and Aqua program (Grant no. NNX11AG53G) as well as the National Science Foundation (Grant no. 1262691). We thank Rocky Mountain National Park for their field support and Marcus Pasay for his assistance with field work. We also thank Dominik Kulakowski and Dan Jarvis for providing the dendroecological plot data, Brian Howell and Justin Backsen of the USFS Region 2, for their assistance with the historical ADS surveys, and the anonymous reviewers for the valuable comments. NR 79 TC 4 Z9 4 U1 0 U2 30 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-1923 EI 1873-2240 J9 AGR FOREST METEOROL JI Agric. For. Meteorol. PD JAN 15 PY 2015 VL 200 BP 78 EP 91 DI 10.1016/j.agrformet.2014.09.015 PG 14 WC Agronomy; Forestry; Meteorology & Atmospheric Sciences SC Agriculture; Forestry; Meteorology & Atmospheric Sciences GA AY4ZB UT WOS:000347582300008 ER PT J AU Fan, ZS Neff, JC Hanan, NP AF Fan, Zhaosheng Neff, Jason C. Hanan, Niall P. TI Modeling pulsed soil respiration in an African savanna ecosystem SO AGRICULTURAL AND FOREST METEOROLOGY LA English DT Article DE DOC; Birch effect; Microbial; Precipitation; Drying; Wetting ID DISSOLVED ORGANIC-CARBON; CONSTRAINED EVOLUTIONARY OPTIMIZATION; OAK-GRASS SAVANNA; RAIN PULSES; WATER; CO2; FLUXES; GROWTH; DECOMPOSITION; CALIFORNIA AB Savannas cover 60% of the African continent and play an important role in the global carbon (C) emissions from fire and land use. To better characterize the biophysical controls over soil respiration in these settings, half-hourly observations of volumetric soil-water content, temperature, and the concentration of carbon dioxide (CO2) at different soil depths were continually measured from 2005 to 2007 under trees ("sub-canopy") and between trees ("inter-canopy") in a savanna vegetation near Skukuza, Kruger National Park, South Africa. The measured soil climate and CO2 concentration data were assimilated into a process-based model that estimates the CO2 production and flux with coupled dynamics of dissolved organic C (DOC) and microbial biomass C. Our results show that temporal and spatial variations in CO2 flux were strongly influenced by precipitation and vegetation cover, with two times greater CO2 flux in the subcanopy plots (similar to 2421 g CO2 m(-2) yr(-1)) than in the inter-canopy plots (similar to 1290 g CO2 m(-2) yr(-1)). Precipitation influenced soil respiration by changing soil temperature and moisture; however, our modeling analysis suggests that the pulsed response of soil respiration to precipitation events (known as "Birch effect") is a key control on soil fluxes at this site. At this site, "Birch effect" contributed to approximately 50% and 65% of heterotrophic respiration or 20% and 39% of soil respiration in the sub-canopy and inter-canopy plots, respectively. These results suggest that pulsed response of respiration to precipitation events is an important component of the C cycle of savannas and should be considered in both measurement and modeling studies of carbon exchange in similar ecosystems. (C) 2014 Elsevier B.V. All rights reserved. C1 [Fan, Zhaosheng] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA. [Neff, Jason C.] Univ Colorado, Dept Geol Sci, Boulder, CO 80302 USA. [Hanan, Niall P.] S Dakota State Univ, Geog Informat Sci Ctr Excellence, Brookings, SD 57007 USA. RP Fan, ZS (reprint author), Argonne Natl Lab, Biosci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM zfan@anl.gov OI Hanan, Niall/0000-0002-9130-5306 FU NASA [NNX08AI77G, NNG04GE24G]; National Institute for Climate Change Research, U.S. Department of Energy [MPC 35UT-01]; U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, Climate and Environmental Science Division [DE-AC02-06CH11357] FX This research is based upon the work supported by (1) the NASA (award #: NNX08AI77G and NNG04GE24G), (2) the National Institute for Climate Change Research, U.S. Department of Energy (award #: MPC 35UT-01), and (3) the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, Climate and Environmental Science Division under contract DE-AC02-06CH11357. NR 64 TC 3 Z9 3 U1 3 U2 63 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-1923 EI 1873-2240 J9 AGR FOREST METEOROL JI Agric. For. Meteorol. PD JAN 15 PY 2015 VL 200 BP 282 EP 292 DI 10.1016/j.agrformet.2014.10.009 PG 11 WC Agronomy; Forestry; Meteorology & Atmospheric Sciences SC Agriculture; Forestry; Meteorology & Atmospheric Sciences GA AY4ZB UT WOS:000347582300027 ER PT J AU Ma, ZY Jiang, JC Shi, W Zhang, WG Mi, CC AF Ma, Zeyu Jiang, Jiuchun Shi, Wei Zhang, Weige Mi, Chunting Chris TI Investigation of path dependence in commercial lithium-ion cells for pure electric bus applications: Aging mechanism identification SO JOURNAL OF POWER SOURCES LA English DT Article DE Lithium-ion battery; Path dependence; Thermal aging; Degradation mechanisms; Incremental capacity analysis; Differential voltage analysis ID DIFFERENTIAL VOLTAGE ANALYSES; COMPOSITE POSITIVE ELECTRODE; BATTERY MANAGEMENT-SYSTEMS; JAHN-TELLER DISTORTION; PARAMETER-ESTIMATION; CHARGE ESTIMATOR; POLYMER BATTERY; ADAPTIVE STATE; VEHICLES; TEMPERATURE AB There is a growing need to provide more realistic and accurate State of Health estimations for batteries in electric vehicles. Thus, it is necessary to research various lithium-ion cell aging processes, including cell degradation and related path dependence. This paper focuses on quantitative analyses of cell aging path dependence in a repeatable laboratory setting, considering the influence of duty cycles, depth of discharge (DOD), and the frequency and severity of the thermal cycle, as reflected in pure electric buses operated in Beijing. Incremental capacity analysis (ICA) and differential voltage analysis (DVA) are applied to infer cell degradation mechanisms and quantify the attributions to capacity fade. It was observed that the cells experienced a higher rate of aging at 80% DOD and an accelerated aging at 40 degrees C in the thermal cycling, as a result of possible loss of active material (LAM) in both electrodes, in addition to the loss of lithium inventory (LLI) and inhibited kinetics. The slight capacity fade from low-temperature extremes likely caused by LLI due to lithium plating, whereas the noticeable fade after the high-temperature excursion was likely caused by LAM and hindrance to kinetics. These results may lead to improved battery management in EV applications. (C) 2014 Elsevier B.V. All rights reserved. C1 [Ma, Zeyu; Jiang, Jiuchun; Shi, Wei; Zhang, Weige] Beijing Jiaotong Univ, Sch Elect Engn, Natl Act Distribut Network Technol Res Ctr, Beijing 100044, Peoples R China. [Ma, Zeyu; Zhang, Weige; Mi, Chunting Chris] Univ Michigan, Dept Elect & Comp Engn, DOE GATE Ctr Elect Drive Transportat, Dearborn, MI 48128 USA. RP Mi, CC (reprint author), Univ Michigan, Dept Elect & Comp Engn, DOE GATE Ctr Elect Drive Transportat, 4901 Evergreen Rd, Dearborn, MI 48128 USA. EM mazeyuhb@gmail.com; chrismi@umich.edu RI 姜, 久春/B-8896-2015; Shi, Wei/G-8193-2012; OI 姜, 久春/0000-0003-4682-9191; Mi, Chris/0000-0002-5471-8953 FU National High Technology Research and Development Program of China [2011AA05A108, 2011AA11A246]; National Natural Science Foundation of China [51277010] FX This work was supported by the National High Technology Research and Development Program of China (No. 2011AA05A108 and No. 2011AA11A246), and the National Natural Science Foundation of China (No. 51277010). NR 33 TC 14 Z9 15 U1 12 U2 75 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD JAN 15 PY 2015 VL 274 BP 29 EP 40 DI 10.1016/j.jpowsour.2014.10.006 PG 12 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA AY0DT UT WOS:000347268700005 ER PT J AU Zhang, LL Duan, S Yang, XL Liang, G Huan, YH Cao, XZ Yang, J Li, M Croft, MC Lewis, C AF Zhang, Lu-Lu Duan, Song Yang, Xue-Lin Liang, Gan Huan, Yun-Hui Cao, Xing-Zhong Yang, Jing Li, Ming Croft, Mark C. Lewis, Cale TI Insight into cobalt-doping in Li2FeSiO4 cathode material for lithium-ion battery SO JOURNAL OF POWER SOURCES LA English DT Article DE Lithium ion battery; Cathode; Lithium iron silicate; Cobalt-doping ID ELECTROCHEMICAL PERFORMANCE; POSITIVE-ELECTRODE; HIGH-CAPACITY; COMPOSITE; CARBON; MN; FE; STABILITY; LI2COSIO4; CATALYST AB This study presents the preparation and electrochemical performance of cobalt-doped Li2FeSiO4/C (Codoped LFS/C) composite by using a solid-state reaction assisted with refluxing process. The Co-doped LFS/C composite delivers a higher discharge capacity of 142.5 mAh g(-1) at 3.0 C even after 100 cycles compared with pristine LFS/C. A clear feature of cobalt-doping in Li2FeSiO4 has been specified by X-ray powder diffraction, X-ray photoelectron spectroscopy coupled with Ar-ion sputtering, X-ray absorption spectroscopy, and positron annihilation lifetime spectroscopy. It is confirmed that Co has been successfully doped into the lattice of LFS, and Co-doping does not change the monoclinic structure of LFS and the oxidation state of Fe. Positron annihilation lifetime spectroscopy analysis further demonstrates that Co-doping increases the defect concentration and the electronic conductivity of LFS. The results clarify the nature of cobalt-doping in LFS and are helpful for understanding the enhancement mechanism of the electrochemical performance of LFS and other cathode materials. (C) 2014 Elsevier B.V. All rights reserved. C1 [Zhang, Lu-Lu; Duan, Song; Yang, Xue-Lin; Li, Ming] China Three Gorges Univ, Coll Mat & Chem Engn, Hubei Prov Collaborat Innovat Ctr New Energy Micr, Yichang 443002, Hubei, Peoples R China. [Zhang, Lu-Lu] Chinese Acad Sci, Shanghai Inst Ceram, CAS Key Lab Mat Energy Convers, Shanghai 200050, Peoples R China. [Liang, Gan; Lewis, Cale] Sam Houston State Univ, Dept Phys, Huntsville, TX 77341 USA. [Huan, Yun-Hui] Huazhong Univ Sci & Technol, Sch Mat Sci & Engn, State Key Lab Mat Proc & Die & Mould Technol, Wuhan 430074, Hubei, Peoples R China. [Cao, Xing-Zhong; Yang, Jing] Chinese Acad Sci, Inst High Energy Phys, Key Lab Nucl Anal Tech, Beijing 100049, Peoples R China. [Croft, Mark C.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Croft, Mark C.] Brookhaven Natl Lab, NSLS, Upton, NY 11973 USA. RP Yang, XL (reprint author), China Three Gorges Univ, Coll Mat & Chem Engn, Hubei Prov Collaborat Innovat Ctr New Energy Micr, 8 Daxue Rd, Yichang 443002, Hubei, Peoples R China. EM xlyang@ctgu.edu.cn FU National Science Foundation of China [51302153, 51272128]; Key Project of Hubei Provincial Department of Education [D20131303]; Opening Project of CAS Key Laboratory of Materials for Energy Conversion [CKEM131404]; Scientific Fund of China Three Gorges University [KJ2012B043]; Pew Foundation of Master Dissertation of China Three Gorges University [2013PY024]; Faculty Research Grant (FRG) from Sam Houston State University FX This work was supported by the National Science Foundation of China (51302153, 51272128); the Key Project of Hubei Provincial Department of Education (D20131303); the Opening Project of CAS Key Laboratory of Materials for Energy Conversion (CKEM131404); the Scientific Fund of China Three Gorges University (KJ2012B043); the Pew Foundation of Master Dissertation of China Three Gorges University (2013PY024); and the Faculty Research Grant (FRG) from Sam Houston State University. Moreover, the authors are grateful to Dr. Jianlin Li at Three Gorges University for his kind support to our research. NR 49 TC 14 Z9 14 U1 11 U2 83 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD JAN 15 PY 2015 VL 274 BP 194 EP 202 DI 10.1016/j.jpowsour.2014.10.048 PG 9 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA AY0DT UT WOS:000347268700025 ER PT J AU Wang, DP Belharouak, I Ortega, LH Zhang, XF Xu, R Zhou, DH Zhou, GW Amine, K AF Wang, Dapeng Belharouak, Ilias Ortega, Luis H. Zhang, Xiaofeng Xu, Rui Zhou, Dehua Zhou, Guangwen Amine, Khalil TI Synthesis of high capacity cathodes for lithium-ion batteries by morphology-tailored hydroxide co-precipitation SO JOURNAL OF POWER SOURCES LA English DT Article DE Lithium batteries; Hydroxide co-precipitation; Ammonia; Cathode; Continuously stirred tank reactor CSTR ID NICKEL MANGANESE OXIDES; ELECTROCHEMICAL PROPERTIES; ELECTRODES; PRECIPITATION; OPTIMIZATION; AMMONIA; GROWTH; CO AB Nickel manganese hydroxide co-precipitation inside a continuous stirred tank reactor was studied with sodium hydroxide and ammonium hydroxide as the precipitation agents. The ammonium hydroxide concentration had an effect on the primary and secondary particle evolution. The two-step precipitation mechanism proposed earlier was experimentally confirmed. In cell tests, Li- and Mn-rich composite cathode materials based on the hydroxide precursors demonstrated good electrochemical performance in terms of cycle life over a wide range of lithium content. (C) 2014 Elsevier B.V. All rights reserved. C1 [Wang, Dapeng; Belharouak, Ilias; Ortega, Luis H.; Zhang, Xiaofeng; Xu, Rui; Zhou, Dehua; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Belharouak, Ilias] Qatar Fdn, Qatar Environm & Energy Res Inst, Doha, Qatar. [Wang, Dapeng; Zhou, Guangwen] SUNY Binghamton, Binghamton, NY 13902 USA. RP Amine, K (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM belharouak@anl.gov; amine@gmail.com OI Belharouak, Ilias/0000-0002-3985-0278; Ortega, Luis/0000-0003-4917-3167 FU U.S. Department of Energy; Freedom CAR; Vehicle Technologies Office; U.S. Department of Energy Office of Science Laboratory [DE-AC02-06CH11357] FX This research was funded by the U.S. Department of Energy, Freedom CAR, and Vehicle Technologies Office. The electron microscopy was accomplished at the Electron Microscopy Center for Materials Research at Argonne National Laboratory, a U.S. Department of Energy Office of Science Laboratory operated under Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC. NR 34 TC 4 Z9 4 U1 0 U2 72 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD JAN 15 PY 2015 VL 274 BP 451 EP 457 DI 10.1016/j.jpowsour.2014.10.016 PG 7 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA AY0DT UT WOS:000347268700054 ER PT J AU Wang, Q Zheng, D McKinnon, ME Yang, XQ Qu, DY AF Wang, Qiang Zheng, Dong McKinnon, Meaghan E. Yang, Xiao-Qing Qu, Deyang TI Kinetic investigation of catalytic disproportionation of superoxide ions in the non-aqueous electrolyte used in Li-air batteries SO JOURNAL OF POWER SOURCES LA English DT Article DE Superoxide disproportionation; Lewis acid catalyst; Li-air battery; Reaction rate constant ID REDUCTION AB Superoxide reacts with carbonate solvents in Li-air batteries. Tris(pentafluorophenyl)borane is found to catalyze a more rapid superoxide (O-2(-)) disproportionation reaction than the reaction between superoxide and propylene carbonate (PC). With this catalysis, the negative impact of the reaction between the electrolyte and O-2(-) produced by the O-2 reduction can be minimized. A simple kinetic study using ESR spectroscopy was reported to determine reaction orders and rate constants for the reaction between PC and superoxide, and the disproportionation of superoxide catalyzed by Tris(pentafluorophenyl)borane and Li ions. The reactions are found to be first order and the rate constants are 0.033 S-1 M-(1,) 0.020 s(-1) M-1 and 0.67 s(-1) M-1 for reactions with PC, Li ion and Tris(pentafluorophenyl)borane, respectively. (C) 2014 Elsevier B.V. All rights reserved. C1 [Wang, Qiang; Zheng, Dong; McKinnon, Meaghan E.; Qu, Deyang] Univ Massachusetts, Dept Chem, Boston, MA 02125 USA. [Yang, Xiao-Qing] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Qu, DY (reprint author), Univ Massachusetts, Dept Chem, 100 Morrissey Blvd, Boston, MA 02125 USA. EM deyang.qu@umb.edu RI Zheng, Dong/J-9975-2015 OI Zheng, Dong/0000-0002-5824-3270 FU Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, under the program of Vehicle Technology Program [DEAC02-98CH10886] FX The authors from UMB are indebted to the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, under the program of Vehicle Technology Program, under Contract Number DEAC02-98CH10886. NR 14 TC 6 Z9 6 U1 3 U2 45 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD JAN 15 PY 2015 VL 274 BP 1005 EP 1008 DI 10.1016/j.jpowsour.2014.10.155 PG 4 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA AY0DT UT WOS:000347268700121 ER PT J AU Khurana, S LaBarbera, M Fedkin, MV Lvov, SN Abernathy, H Gerdes, K AF Khurana, Sanchit LaBarbera, Mark Fedkin, Mark V. Lvov, Serguei N. Abernathy, Harry Gerdes, Kirk TI Performance evaluation of a liquid tin anode solid oxide fuel cell operating under hydrogen, argon and coal SO JOURNAL OF POWER SOURCES LA English DT Article DE Solid oxide fuel cell; Liquid Metal Anode; Electrochemical Impedance Spectroscopy; Equivalent circuit modeling; Warburg impedance; Metal-air battery ID REFERENCE ELECTRODE PLACEMENT; ELECTROCHEMICAL IMPEDANCE; COMPOSITE CATHODES; DIRECT OXIDATION; DIFFUSION; SPECTROSCOPY; SOFC; POLARIZATION; INTERFACE; OIL AB A liquid tin anode solid oxide fuel cell is constructed and investigated under different operating conditions. Electrochemical Impedance Spectroscopy (EIS) is used to reflect the effect of fuel feed as the EIS spectra changes significantly on switching the fuel from argon to hydrogen. A cathode symmetric cell is used to separate the impedance from the two electrodes, and the results indicate that a major contribution to the charge-transfer and mass-transfer impedance arises from the anode. The OCP of 0.841 V for the cell operating under argon as a metal-air battery indicates the formation of a SnO2 layer at the electrolyte/anode interface. The increase in the OCP to 1.1 V for the hydrogen fueled cell shows that H-2 reduces the SnO2 film effectively. The effective diffusion coefficients are calculated using the Warburg element in the equivalent circuit model for the experimental EIS data, and the values of 1.9 10(-3) cm(2) s(-1) at 700 degrees C, 2.3 10(-3) cm(2) s(-1) at 800 degrees C and 3.5 10(-3) cm(2) s(-1) at 900 degrees C indicate the system was influenced by diffusion of hydrogen in the system. Further, the performance degradation over time is attributed to the irreversible conversion of Sn to SnO2 resulting from galvanic polarization. (C) 2014 Elsevier B.V. All rights reserved. C1 [Khurana, Sanchit; LaBarbera, Mark; Fedkin, Mark V.; Lvov, Serguei N.] Penn State Univ, Earth & Mineral Sci Energy Inst, University Pk, PA 16802 USA. [Khurana, Sanchit; LaBarbera, Mark; Lvov, Serguei N.] Penn State Univ, Dept Energy & Mineral Engn, University Pk, PA 16802 USA. [Lvov, Serguei N.] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Abernathy, Harry; Gerdes, Kirk] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. RP Lvov, SN (reprint author), Penn State Univ, Dept Energy & Mineral Engn, University Pk, PA 16802 USA. EM lvov@psu.edu FU National Energy Technology Laboratory (NEIL); RES [DE-FE0004000] FX The authors gratefully acknowledge the financial support of this work by National Energy Technology Laboratory (NEIL). As part of the National Energy Technology Laboratory's Regional University Alliance (NETL-RUA), a collaborative initiative of the NETL, this technical effort was performed under the RES contract DE-FE0004000. NR 47 TC 9 Z9 9 U1 1 U2 38 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD JAN 15 PY 2015 VL 274 BP 1049 EP 1054 DI 10.1016/j.jpowsour.2014.10.138 PG 6 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA AY0DT UT WOS:000347268700127 ER PT J AU Zhao, HN Fedkin, MV Dilmore, RM Lvov, SN AF Zhao, Haining Fedkin, Mark V. Dilmore, Robert M. Lvov, Serguei N. TI Carbon dioxide solubility in aqueous solutions of sodium chloride at geological conditions: Experimental results at 323.15, 373.15, and 423.15 K and 150 bar and modeling up to 573.15 K and 2000 bar SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID VAPOR-LIQUID-EQUILIBRIA; PHASE-EQUILIBRIA; HIGH-PRESSURE; HIGH-TEMPERATURES; CO2 SOLUBILITY; WATER-SYSTEM; PLUS WATER; THERMODYNAMIC PROPERTIES; MUTUAL SOLUBILITIES; HENRYS CONSTANTS AB A new experimental system was designed to measure the solubility of CO2 at pressures and temperatures (150 bar, 323.15-423.15 K) relevant to geologic CO2 sequestration. At 150 bar, new CO2 solubility data in the aqueous phase were obtained at 323.15, 373.15, and 423.15 K from 0 to 6 mol kg(-1) NaCl(aq) for the CO2-NaCl-H2O system. A gamma - phi (activity coefficient - fugacity coefficient) type thermodynamic model is presented for the calculation of both the solubility of CO2 in the aqueous phase and the solubility of H2O in the CO2-rich phase for the CO2-NaCl-H2O system. Validation of the model calculations against literature data and other models (MZLL2013, AD2010, SP2010, DS2006, and OLI) show that the proposed model is capable of predicting the solubility of CO2 in the aqueous phase for the CO2-H2O and CO2-NaCl-H2O systems with a high degree of accuracy (AAD <3.9%) at temperatures from 273.15 to 573.15 K and pressures up to 2000 bar. A comparison of modeling results with experimental values revealed a pressure-bounded "transition zone" in which the CO2 solubility decreases to a minimum then increases as the temperature increases. CO2 solubility is not a monotonic function of temperature in the transition zone but outside of that transition zone, the CO2 solubility is decrease or increase monotonically in response to increased temperature. A link of web-based CO2 solubility computational tool can be provided by sending a message to Haining Zhao at hzz5047@gmail.com. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Zhao, Haining; Lvov, Serguei N.] Penn State Univ, John & Willie Leone Family Dept Energy & Mineral, University Pk, PA 16802 USA. [Zhao, Haining; Fedkin, Mark V.; Lvov, Serguei N.] Penn State Univ, EMS Energy Inst, Electrochem Technol Program, University Pk, PA 16802 USA. [Zhao, Haining] Penn State Univ, EMS Energy Inst, Petr & Nat Gas Engn Program, University Pk, PA 16802 USA. [Lvov, Serguei N.] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Dilmore, Robert M.] Natl Energy Technol Lab, US Dept Energy, Pittsburgh, PA 15236 USA. RP Lvov, SN (reprint author), Penn State Univ, John & Willie Leone Family Dept Energy & Mineral, University Pk, PA 16802 USA. EM lvov@psu.edu OI Zhao, Haining/0000-0002-8703-0637 FU U.S. Department of Energy, National Energy Technology Laboratory and the Energy Institute of College of Earth and Mineral Sciences at the Pennsylvania State University FX This work was supported by the U.S. Department of Energy, National Energy Technology Laboratory and the Energy Institute of College of Earth and Mineral Sciences at the Pennsylvania State University. We particularly thank Dr. Alfonso Mucci for reading the manuscript and providing many useful recommendations. We thank Dr. Nicolas Spycher, Dr. Nikolay N. Akinfiev, Dr. Larryn W. Diamond and one anonymous reviewer for carefully reading the manuscript and providing many constructive suggestions, which greatly improved the quality of the manuscript. We also thank Dr. Nikolay N. Akinfiev and Dr. Nicolas Spycher for suggestions and access to their computer codes. Thanks to OLI System Inc. for providing us the powerful OLI Studio 9.0.6 software package, and we also thank Dr. Andre Anderko for reading the manuscript and making very useful suggestions. Finally, we thank Mr. Derek Hall for useful discussions and reading the manuscript. NR 79 TC 9 Z9 9 U1 1 U2 20 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD JAN 15 PY 2015 VL 149 BP 165 EP 189 DI 10.1016/j.gca.2014.11.004 PG 25 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA AX2AC UT WOS:000346744500012 ER PT J AU Foroozani, N Lim, J Fabbris, G Rosa, PFS Fisk, Z Schilling, JS AF Foroozani, N. Lim, J. Fabbris, G. Rosa, P. F. S. Fisk, Z. Schilling, J. S. TI Suppression of dense Kondo state in CeB6 under pressure SO PHYSICA B-CONDENSED MATTER LA English DT Article DE Dense Kondo lattice; Extreme pressure; Fermi liquid; Electrical resistivity; Synchrotron x-ray diffraction ID RARE-EARTH HEXABORIDES; INSULATOR SMB6; SYSTEM; CERIUM; TEMPERATURE; EXCITATIONS; SCATTERING; CRYSTALS; STRAIN; GPA AB To investigate whether the dense Kondo compound CeB6 might evolve into a topological insulator under sufficient pressure, four-point electrical resistivity measurements have been carried out over the temperature range 1.3 K-295 K in a diamond anvil cell to 122 GPa. The temperature T-max of the resistivity maximum initially increases slowly with pressure but disappears between 12 and 20 GPa. The marked changes observed under pressure suggest that a valence and/or structural transition may have occurred. Synchrotron x-ray diffraction measurements, however, fail to detect any change in crystal structure to 85 GPa. Although a transition into an insulating phase is not observed, this dense Kondo system is completely suppressed at 43 GPa, leaving behind what appears to be a conventional Fermi liquid metal. (C) 2014 Elsevier B.V. All rights reserved. C1 [Foroozani, N.; Lim, J.; Fabbris, G.; Schilling, J. S.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Fabbris, G.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Rosa, P. F. S.; Fisk, Z.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. RP Schilling, JS (reprint author), Washington Univ, Dept Phys, CB 1105,One Brookings Dr, St Louis, MO 63130 USA. EM jss@wuphys.wustl.edu RI Fabbris, Gilberto/F-3244-2011 OI Fabbris, Gilberto/0000-0001-8278-4985 FU National Science Foundation (NSF) [DMR-1104742]; Carnegie/DOE Alliance Center (CDAC) through NNSA/DOE Grant [DE-FC52-08NA28554]; U.S. Department of Energy, Office of Science [DE-AC02-06CH11357] FX The authors would like to express gratitude to T. Matsuoka and K. Shimizu for sharing information on their high-pressure electrical resistivity techniques used in this study. Thanks are due A. Gangopadhyay for his critical reading of the manuscript. This work was supported by the National Science Foundation (NSF) through Grant No. DMR-1104742 and by the Carnegie/DOE Alliance Center (CDAC) through NNSA/DOE Grant No. DE-FC52-08NA28554. Work at Argonne National Laboratory is supported by the U.S. Department of Energy, Office of Science, under contract No, DE-AC02-06CH11357. NR 39 TC 5 Z9 5 U1 3 U2 26 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0921-4526 EI 1873-2135 J9 PHYSICA B JI Physica B PD JAN 15 PY 2015 VL 457 BP 12 EP 16 DI 10.1016/j.physb.2014.10.001 PG 5 WC Physics, Condensed Matter SC Physics GA AX3ND UT WOS:000346845200003 ER PT J AU Fu, J Wu, JZ Custelcean, R Jiang, DE AF Fu, Jia Wu, Jianzhong Custelcean, Radu Jiang, De-en TI Nitrogen-doped porous aromatic frameworks for enhanced CO2 adsorption SO JOURNAL OF COLLOID AND INTERFACE SCIENCE LA English DT Article DE CO2 capture; Porous material; Material design; Nitrogen-doping; Molecular simulation ID CARBON-DIOXIDE CAPTURE; METAL-ORGANIC FRAMEWORKS; POLYMER NETWORKS; CATALYZED SYNTHESIS; MOLECULAR-DYNAMICS; FORCE-FIELD; GAS-UPTAKE; AB-INITIO; SEPARATION; SIMULATIONS AB Recently synthesized porous aromatic frameworks (PAFs) exhibit extremely high surface areas and exceptional thermal and hydrothermal stabilities. Using computer-aided design, we propose new PAFs, designated as NPAFs, by introducing nitrogen-containing groups to the biphenyl unit and predict their CO2 adsorption capacities with grand canonical Monte Carlo (GCMC) simulations. Among various NPAFs considered, one with imidazole groups shows the highest adsorption capacity for CO2 (11.5 wt% at 1 bar and 298 K), in comparison with 5 wt% for the parent PAF (PAF-1) at the same condition. At higher pressures (around 10 bar), however, another NPAF with pyridinic N groups performs much better than the rest due to its greater pore volume in addition to the N functionality. This study suggests that adding N functionality to the organic linkers is a promising way to increase CO2 adsorption capacity of PAFs at ambient condition. (C) 2014 Elsevier Inc. All rights reserved. C1 [Fu, Jia; Wu, Jianzhong] Univ Calif Riverside, Dept Chem & Environm Engn, Riverside, CA 92521 USA. [Custelcean, Radu] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Jiang, De-en] Univ Calif Riverside, Dept Chem, Riverside, CA 92521 USA. RP Jiang, DE (reprint author), Univ Calif Riverside, Dept Chem, Riverside, CA 92521 USA. EM djiang@ucr.edu RI Custelcean, Radu/C-1037-2009; Jiang, De-en/D-9529-2011; OI Custelcean, Radu/0000-0002-0727-7972; Jiang, De-en/0000-0001-5167-0731; Wu, Jianzhong/0000-0002-4582-5941 FU Laboratory Directed Research and Development Program at Oak Ridge National Laboratory; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was sponsored by the Laboratory Directed Research and Development Program at Oak Ridge National Laboratory, managed by UT-Battelle, LLC for the U.S. Department of Energy and used resources of the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the U.S. Department of Energy under Contract DE-AC02-05CH11231. NR 34 TC 8 Z9 8 U1 7 U2 135 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9797 EI 1095-7103 J9 J COLLOID INTERF SCI JI J. Colloid Interface Sci. PD JAN 15 PY 2015 VL 438 BP 191 EP 195 DI 10.1016/j.jcis.2014.09.079 PG 5 WC Chemistry, Physical SC Chemistry GA AX1EZ UT WOS:000346692100024 PM 25454441 ER PT J AU Walter, MD Sofield, CD Andersen, RA AF Walter, Marc D. Sofield, Chadwick D. Andersen, Richard A. TI Spin equilibria and thermodynamic constants for (C5H4R)(2)Mn, R = H or Me, in solid solutions of diamagnetic diluents SO JOURNAL OF ORGANOMETALLIC CHEMISTRY LA English DT Article DE Manganocene; Magnetic susceptibility data; Spin equilibrium; Thermodynamics ID PHASE ELECTRON-DIFFRACTION; OPEN-SHELL METALLOCENES; PHOTOELECTRON-SPECTRA; MOLECULAR-STRUCTURE; SERIES METALLOCENES; METAL-COMPLEXES; MANGANOCENE; CYCLOPENTADIENYL AB The solid state structure of (C5H4Me)(2)Mn is determined and its solid state magnetism investigated. (C5H4Me)(2)Mn is a chain polymer, as is the parent (C5H5)(2)Mn (Bunder W.; Weiss, E. Z. Naturforsch. 1978, 33b, 1237), and they exhibit very similar solid state magnetic susceptibilities that are modeled as an antiferromagnetically-coupled linear Heisenberg-chain of high-spin Mn(II) centers (S = 5/2) (Konig, E.; Desai, V. P.; Kanellakopulos, B.; Klenze, R. Chem. Phys. 1980, 54, 109). Doping of these manganocenes into diamagnetic hosts such as (C5H4Me)(2)Fe and (C5H5)(2)Fe, respectively, stabilizes the low-spin configuration (S = 1/2) relative to the high-spin configuration (S = 5/2). At higher temperatures the solid solutions of these manganocenes show spin-crossover behavior modeled by a Boltzmann distribution of spins to give Delta H-0 approximate to 1.7 kcal mol(-1) and Delta S-0 approximate to 5 cal (mol K)(-1) for the LS (sic) HS equilibria. (C) 2014 Elsevier B.V. All rights reserved. C1 [Walter, Marc D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Chem, Berkeley, CA 94720 USA. [Walter, Marc D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Walter, Marc D.; Sofield, Chadwick D.; Andersen, Richard A.] TU Braunschweig, Inst Anorgan & Analyt Chem, D-38106 Braunschweig, Germany. RP Walter, MD (reprint author), TU Braunschweig, Inst Anorgan & Analyt Chem, Hagenring 30, D-38106 Braunschweig, Germany. EM mwalter@tu-bs.de; raandersen@lbl.gov RI Walter, Marc/E-4479-2012 FU Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Office of Basic Energy Sciences (OBES) of the U.S. Department of Energy [DE-AC02-05CH11231]; German Academic Exchange Service (DAAD) FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences (OBES), of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We thank Fred Hollander (at CHEXRAY, the U.C. Berkeley X-ray diffraction facility) for assistance with the crystallography, the German Academic Exchange Service (DAAD) for a fellowship (M.D.W.), and Martin Head-Gordon for discussions. NR 42 TC 3 Z9 3 U1 0 U2 4 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0022-328X EI 1872-8561 J9 J ORGANOMET CHEM JI J. Organomet. Chem. PD JAN 15 PY 2015 VL 776 BP 17 EP 22 DI 10.1016/j.jorganchem.2014.10.032 PG 6 WC Chemistry, Inorganic & Nuclear; Chemistry, Organic SC Chemistry GA AX0IS UT WOS:000346636800003 ER PT J AU Biagioni, DJ Beylkin, D Beylkin, G AF Biagioni, David J. Beylkin, Daniel Beylkin, Gregory TI Randomized interpolative decomposition of separated representations SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Canonical tensor decomposition; Interpolative decomposition; Alternating least squares algorithm; Randomized projection; Self-guiding tensor iteration ID LOW-RANK APPROXIMATION; RANDOM PROJECTIONS; EFFICIENT ALGORITHMS; LARGE MATRICES; ORDER TENSORS; DIMENSIONS; OPERATORS AB We introduce an algorithm to compute tensor interpolative decomposition(dubbed CTDID) for the reduction of the separation rank of Canonical Tensor Decompositions (CTDs). Tensor ID selects, for a user-defined accuracy epsilon, a near optimal subset of terms of a CTD to represent the remaining terms via a linear combination of the selected terms. CTD-ID can be used as an alternative to or in combination with the Alternating Least Squares (ALS) algorithm. We present examples of its use within a convergent iteration to compute inverse operators in high dimensions. We also briefly discuss the spectral norm as a computational alternative to the Frobenius norm in estimating approximation errors of tensor ID. We reduce the problem of finding tensor IDs to that of constructing interpolative decompositions of certain matrices. These matrices are generated via randomized projection of the terms of the given tensor. We provide cost estimates and several examples of the new approach to the reduction of separation rank. (C) 2014 Elsevier Inc. All rights reserved. C1 [Biagioni, David J.] Natl Renewable Energy Lab, Computat Sci Ctr, Golden, CO 80401 USA. [Beylkin, Daniel] Yale Univ, Program Appl Math, New Haven, CT 06511 USA. [Beylkin, Gregory] Univ Colorado, Dept Appl Math, Boulder, CO 80309 USA. RP Beylkin, G (reprint author), Univ Colorado, Dept Appl Math, 526 UCB, Boulder, CO 80309 USA. RI Beylkin, Gregory/G-6653-2011 FU NREL [UGA-0-41026-08]; NSF [DMS-1228359, DMS-1009951]; DoD AFOSR NDSEG Fellowship [FA9550-11-C-0028]; DOE/ORNL [4000038129] FX D.J. Biagioni was partially supported by NREL grant UGA-0-41026-08 and NSF grant DMS-1228359. D. Beylkin received support under FA9550-11-C-0028 by the DoD AFOSR NDSEG Fellowship. G. Beylkin was partially supported by NSF grants DMS-1009951, DMS-1228359 and DOE/ORNL grant 4000038129. NR 62 TC 3 Z9 3 U1 2 U2 12 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JAN 15 PY 2015 VL 281 BP 116 EP 134 DI 10.1016/j.jcp.2014.10.009 PG 19 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AW7FE UT WOS:000346429300007 ER PT J AU He, Y Sun, YJ Liu, J Qin, H AF He, Yang Sun, Yajuan Liu, Jian Qin, Hong TI Volume-preserving algorithms for charged particle dynamics SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Lorentz force equation; Splitting method; Volume-preserving integrator; Boris algorithm; Conservative quantities ID GUIDING CENTER MOTION; SYSTEMS; FORMULATION; INTEGRATORS; SCHEMES AB The paper reports the development of volume-preserving algorithms using the splitting technique for charged particle motion under the Lorentz force. The source-free nature of the Lorentz vector field has been investigated. Based on the volume-preserving property of the dynamics, a class of numerical methods for advancing charged particles in a general electromagnetic field has been constructed by splitting the classical evolution operator. This new class of numerical methods, which includes the Boris algorithm as a special case, conserves phase space volume, and globally bounds the numerical errors of energy, momentum, and other adiabatic invariants up to the order of the method over a very long simulation time. These algorithms can be computed explicitly, and thus are effective for the long-term simulation of the multi-scale dynamics of plasmas. (C) 2014 Elsevier Inc. All rights reserved. C1 [Sun, Yajuan] Chinese Acad Sci, Acad Math & Syst Sci, LSEC, Beijing 100190, Peoples R China. [He, Yang; Liu, Jian; Qin, Hong] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China. [He, Yang; Liu, Jian; Qin, Hong] Univ Sci & Technol China, Collaborat Innovat Ctr Adv Fus Energy & Plasma Sc, Hefei 230026, Anhui, Peoples R China. [Qin, Hong] Princeton Univ, Plasma Phys Lab, Princeton, NJ 08543 USA. RP Sun, YJ (reprint author), Chinese Acad Sci, Acad Math & Syst Sci, LSEC, POB 2719, Beijing 100190, Peoples R China. EM sunyj@lsec.cc.ac.cn OI Liu, Jian/0000-0001-7484-401X FU National Natural Science Foundation of China [11271357, 11075162, 11261140328]; CSC; CAS Program for Interdisciplinary Collaboration Team; Foundation for Innovative Research Groups of the NNSFC [11321061]; National Basic Research Program of China [2010CB832702]; ITER-China Program [2014GB124005] FX This research was supported by the National Natural Science Foundation of China (11271357, 11075162, 11261140328), by CSC, the CAS Program for Interdisciplinary Collaboration Team, the Foundation for Innovative Research Groups of the NNSFC (11321061), the National Basic Research Program of China (2010CB832702) and the ITER-China Program (2014GB124005). NR 27 TC 21 Z9 21 U1 2 U2 17 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JAN 15 PY 2015 VL 281 BP 135 EP 147 DI 10.1016/j.jcp.2014.10.032 PG 13 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AW7FE UT WOS:000346429300008 ER PT J AU Safta, C Sargsyan, K Debusschere, B Najm, HN AF Safta, Cosmin Sargsyan, Khachik Debusschere, Bert Najm, Habib N. TI Hybrid discrete/continuum algorithms for stochastic reaction networks SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Chemical Master Equation; Fokker-Planck equation; Finite volume; Flux splitting; Hybrid discrete-continuum models ID CHEMICAL MASTER EQUATION; SIMULATION; SYSTEMS; KINETICS AB Direct solutions of the Chemical Master Equation (CME) governing Stochastic Reaction Networks (SRNs) are generally prohibitively expensive due to excessive numbers of possible discrete states in such systems. To enhance computational efficiency we develop a hybrid approach where the evolution of states with low molecule counts is treated with the discrete CME model while that of states with large molecule counts is modeled by the continuum Fokker-Planck equation. The Fokker-Planck equation is discretized using a 2nd order finite volume approach with appropriate treatment of flux components. The numerical construction at the interface between the discrete and continuum regions implements the transfer of probability reaction by reaction according to the stoichiometry of the system. The performance of this novel hybrid approach is explored for a two-species circadian model with computational efficiency gains of about one order of magnitude. Published by Elsevier Inc. C1 [Safta, Cosmin; Sargsyan, Khachik; Debusschere, Bert; Najm, Habib N.] Sandia Natl Labs, Livermore, CA 94551 USA. RP Safta, C (reprint author), Sandia Natl Labs, Livermore, CA 94551 USA. EM csafta@sandia.gov; ksargsy@sandia.gov; bjdebus@sandia.gov; hnnajm@sandia.gov OI Debusschere, Bert/0000-0001-7253-7059 FU U.S. Department of Energy Office of Science through the Applied Mathematics program in the Office of Advanced Scientific Computing Research (ASCR) [07-012783]; Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the U.S. Department of Energy Office of Science through the Applied Mathematics program in the Office of Advanced Scientific Computing Research (ASCR) under contract 07-012783 with Sandia National Laboratories. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract No. DE-AC04-94AL85000. NR 46 TC 3 Z9 3 U1 0 U2 6 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JAN 15 PY 2015 VL 281 BP 177 EP 198 DI 10.1016/j.jcp.2014.10.026 PG 22 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AW7FE UT WOS:000346429300010 ER PT J AU Morgan, NR Waltz, JI Burton, DE Charest, MR Canfield, TR Wohlbier, JG AF Morgan, Nathaniel R. Waltz, Jacob I. Burton, Donald E. Charest, Marc R. Canfield, Thomas R. Wohlbier, John G. TI A Godunov-like point-centered essentially Lagrangian hydrodynamic approach SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Lagrangian; Hydrodynamics; Point-centered; Godunov; Finite-element ID ARTIFICIAL VISCOSITY; UNSTRUCTURED GRIDS; SHOCK HYDRODYNAMICS; RIEMANN SOLVER; DYNAMICS; SCHEME; CONSERVATION; SYSTEMS; ENERGY; ERRORS AB We present an essentially Lagrangian hydrodynamic scheme suitable for modeling complex compressible flows on tetrahedron meshes. The scheme reduces to a purely Lagrangian approach when the flow is linear or if the mesh size is equal to zero; as a result, we use the term essentially Lagrangian for the proposed approach. The motivation for developing a hydrodynamic method for tetrahedron meshes is because tetrahedron meshes have some advantages over other mesh topologies. Notable advantages include reduced complexity in generating conformal meshes, reduced complexity in mesh reconnection, and preserving tetrahedron cells with automatic mesh refinement. A challenge, however, is tetrahedron meshes do not correctly deform with a lower order (i. e. piecewise constant) staggered-grid hydrodynamic scheme (SGH) or with a cell-centered hydrodynamic (CCH) scheme. The SGH and CCH approaches calculate the strain via the tetrahedron, which can cause artificial stiffness on large deformation problems. To resolve the stiffness problem, we adopt the point-centered hydrodynamic approach (PCH) and calculate the evolution of the flow via an integration path around the node. The PCH approach stores the conserved variables (mass, momentum, and total energy) at the node. The evolution equations for momentum and total energy are discretized using an edge-based finite element (FE) approach with linear basis functions. A multidirectional Riemann-like problem is introduced at the center of the tetrahedron to account for discontinuities in the flow such as a shock. Conservation is enforced at each tetrahedron center. The multidimensional Riemann-like problem used here is based on Lagrangian CCH work [8,19,37,38,44] and recent Lagrangian SGH work [33-35,39,45]. In addition, an approximate 1D Riemann problem is solved on each face of the nodal control volume to advect mass, momentum, and total energy. The 1D Riemann problem produces fluxes [18] that remove a volume error in the PCH discretization. A 2-stage Runge-Kutta method is used to evolve the solution in time. The details of the new hydrodynamic scheme are discussed; likewise, results from numerical test problems are presented. (C) 2014 The Authors. Published by Elsevier Inc. C1 [Morgan, Nathaniel R.; Waltz, Jacob I.; Burton, Donald E.; Charest, Marc R.] Los Alamos Natl Lab, X Computat Phys Div, Los Alamos, NM 87544 USA. [Canfield, Thomas R.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM USA. [Wohlbier, John G.] Los Alamos Natl Lab, Comp Computat & Stat Sci Div, Los Alamos, NM USA. RP Morgan, NR (reprint author), Los Alamos Natl Lab, X Computat Phys Div, POB 1663, Los Alamos, NM 87544 USA. EM nmorgan@lanl.gov FU NNSA through the Laboratory Directed Research and Development program at Los Alamos National Laboratory FX We would like to thank L. Dean Risinger for developing data structures for unstructured tetrahedron meshes. We also gratefully acknowledge the support of the NNSA through the Laboratory Directed Research and Development program at Los Alamos National Laboratory. The Los Alamos unlimited release number is LA-UR-14-20465. NR 66 TC 3 Z9 3 U1 0 U2 7 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JAN 15 PY 2015 VL 281 BP 614 EP 652 DI 10.1016/j.jcp.2014.10.048 PG 39 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AW7FE UT WOS:000346429300031 ER PT J AU Birrell, J Wilkening, J Rafelski, J AF Birrell, Jeremiah Wilkening, Jon Rafelski, Johann TI Boltzmann equation solver adapted to emergent chemical non-equilibrium SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Relativistic Boltzmann equation; Chemical non-equilibrium; Orthogonal polynomial spectral method ID QUARK-GLUON PLASMA; NEUTRINOS; FLUCTUATIONS; SPECTRA; SHARE AB We present a novel method to solve the spatially homogeneous and isotropic relativistic Boltzmann equation. We employ a basis set of orthogonal polynomials dynamically adapted to allow for emergence of chemical non-equilibrium. Two time dependent parameters characterize the set of orthogonal polynomials, the effective temperature T(t) and phase space occupation factor gamma(t). In this first paper we address (effectively) massless fermions and derive dynamical equations for T(t) and gamma(t) such that the zeroth order term of the basis alone captures the particle number density and energy density of each particle distribution. We validate our method and illustrate the reduced computational cost and the ability to easily represent final state chemical non-equilibrium by studying a model problem that is motivated by the physics of the neutrino freeze-out processes in the early Universe, where the essential physical characteristics include reheating from another disappearing particle component (e(+/-)-annihilation). (C) 2014 Elsevier Inc. All rights reserved. C1 [Birrell, Jeremiah] Univ Arizona, Program Appl Math, Tucson, AZ 85721 USA. [Birrell, Jeremiah; Rafelski, Johann] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Wilkening, Jon] Univ Calif Berkeley, Dept Math, Berkeley, CA 94721 USA. [Wilkening, Jon] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94721 USA. RP Birrell, J (reprint author), Univ Arizona, Program Appl Math, Tucson, AZ 85721 USA. EM jeremey.birrell@gmail.com FU DoD, Air Force Office of Scientific Research, National Defense Science and Engineering Graduate (NDSEG) Fellowship [32 CFR 168a]; US Department of Energy, Office of Science, Applied Scientific Computing Research [DE-AC02-05CH11231]; National Science Foundation [DMS-0955078]; U.S. Department of Energy [DE-FG02-04ER41318] FX J.B. would like to acknowledge Government support under and awarded by DoD, Air Force Office of Scientific Research, National Defense Science and Engineering Graduate (NDSEG) Fellowship, 32 CFR 168a. J.W. was supported in part by the US Department of Energy, Office of Science, Applied Scientific Computing Research, under award number DE-AC02-05CH11231, and by the National Science Foundation under award number DMS-0955078. J.R. was supported by a grant from the U.S. Department of Energy, DE-FG02-04ER41318. NR 26 TC 2 Z9 2 U1 0 U2 3 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JAN 15 PY 2015 VL 281 BP 896 EP 916 DI 10.1016/j.jcp.2014.10.056 PG 21 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AW7FE UT WOS:000346429300044 ER PT J AU Dai, WW Scannapieco, AJ AF Dai, William W. Scannapieco, Anthony J. TI Second-order accurate interface- and discontinuity-aware diffusion solvers in two and three dimensions SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Radiation; Diffusion; Mixing; Interface; Implicit ID NONEQUILIBRIUM RADIATION DIFFUSION; FINITE-DIFFERENCE METHODS; ADAPTIVE MESH REFINEMENT; NEWTON-KRYLOV METHOD; NUMERICAL SIMULATIONS; EQUATIONS; HYDRODYNAMICS; DISCRETIZATION; COEFFICIENTS; CONDUCTION AB A numerical scheme is developed for two- and three-dimensional time-dependent diffusion equations in numerical simulations involving mixed cells. The focus of the development is on the formulations for both transient and steady states, the property for large time steps, second-order accuracy in both space and time, the correct treatment of the discontinuity in material properties, and the handling of mixed cells. For a mixed cell, interfaces between materials are reconstructed within the cell so that each of resulting sub-cells contains only one material and the material properties of each sub-cell are known. Diffusion equations are solved on the resulting polyhedral mesh even if the original mesh is structured. The discontinuity of material properties between different materials is correctly treated based on governing physics principles. The treatment is exact for arbitrarily strong discontinuity. The formulae for effective diffusion coefficients across interfaces between materials are derived for general polyhedral meshes. The scheme is general in two and three dimensions. Since the scheme to be developed in this paper is intended for multi-physics code with adaptive mesh refinement (AMR), we present the scheme on mesh generated from AMR. The correctness and features of the scheme are demonstrated for transient problems and steady states in one-, two-, and three-dimensional simulations for heat conduction and radiation heat transfer. The test problems involve dramatically different materials. (C) 2014 Elsevier Inc. All rights reserved. C1 [Dai, William W.; Scannapieco, Anthony J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Dai, WW (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM dai@lanl.gov FU United States Department of Energy ASC program FX This research and development are funded by the United States Department of Energy ASC program. The authors are grateful to Frederick L. Cochran and Chong Chang for discussions about this work. NR 37 TC 1 Z9 1 U1 3 U2 8 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JAN 15 PY 2015 VL 281 BP 982 EP 1002 DI 10.1016/j.jcp.2014.10.040 PG 21 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA AW7FE UT WOS:000346429300048 ER PT J AU Deng, YX Helms, BA Rolandi, M AF Deng, Yingxin Helms, Brett A. Rolandi, Marco TI Synthesis of Pyridine Chitosan and its Protonic Conductivity SO JOURNAL OF POLYMER SCIENCE PART A-POLYMER CHEMISTRY LA English DT Article DE biopolymers; chitosan; polysaccharides ID MECHANICAL-PROPERTIES; CHITIN; NETWORKS C1 [Deng, Yingxin; Rolandi, Marco] Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USA. [Helms, Brett A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Rolandi, M (reprint author), Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USA. EM rolandi@uw.edu RI Foundry, Molecular/G-9968-2014; OI Deng, Yingxin/0000-0003-4091-6462; Helms, Brett/0000-0003-3925-4174 FU National Science Foundation CAREER Award [DMR 1150630]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by a National Science Foundation CAREER Award (DMR 1150630). Polymer synthesis and characterization was carried out as part of a User Project at the Molecular Foundry, which is supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 18 TC 4 Z9 5 U1 1 U2 18 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0887-624X EI 1099-0518 J9 J POLYM SCI POL CHEM JI J. Polym. Sci. Pol. Chem. PD JAN 15 PY 2015 VL 53 IS 2 SI SI BP 211 EP 214 DI 10.1002/pola.27430 PG 4 WC Polymer Science SC Polymer Science GA AW2YA UT WOS:000346151300011 ER PT J AU Chahal, HS Chahal, DS McBride, PM Helms, BA AF Chahal, Harvind S. Chahal, Dev S. McBride, Patrick M. Helms, Brett A. TI Synthetic Control Over the Dynamics of Mesoscaled Cargo Release From Colloidal Polymer Vectors Inside Live Cells SO JOURNAL OF POLYMER SCIENCE PART A-POLYMER CHEMISTRY LA English DT Article DE biological applications of polymers; controlled release; core-shell polymer colloids; endosome disruption; proton sponge; stimuli-sensitive polymers ID FREE EMULSION POLYMERIZATION; MESOPOROUS SILICA NANOPARTICLES; PH-RESPONSIVE MICROGELS; QUANTUM DOTS; CYTOSOLIC DELIVERY; LATEX-PARTICLES; DRUG-DELIVERY; IN-VITRO; LUMINESCENT NANOCRYSTALS; ENDOTHELIAL-CELLS AB Directed delivery of mesoscaled cargofor example, nanocrystals, proteins, or nucleic acidsto cells using polymer vectors impacts numerous biomedical fields. We introduce here the concept of dynamic complementarity as a simple, yet powerful approach to control the rate of mesoscaled cargo dissociation from colloidal polymer vectors once inside the cytosol. By tuning the degree of electrostatic reciprocity between the polymer vector and its cargo, it is possible to both deliver and release large cargo in live cells in a controllable manner over both long and short periods, pointing to a highly modular materials platform with molecularly tailored properties suited to task. (c) 2014 Wiley Periodicals, Inc. J. Polym. Sci., Part A: Polym. Chem. 2015, 53, 256-264 C1 [Chahal, Harvind S.; Chahal, Dev S.; McBride, Patrick M.; Helms, Brett A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Helms, BA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, One Cyclotron Rd, Berkeley, CA 94720 USA. EM bahelms@lbl.gov RI Foundry, Molecular/G-9968-2014; OI Helms, Brett/0000-0003-3925-4174 FU Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Science Undergraduate Laboratory Internship (SULI) program FX The authors thank Cheryl Goldbeck for assistance with flow cytometry, Georgeta Masson for SEM, Andrea Bayles for confocal fluorescence microscopy as well as Alice Thwin and Kurt Thorn for helpful discussions. Microscope access was generously provided by the Nikon Imaging Center at UCSF. All other work was performed at the Molecular Foundry and supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. P.M.M. was supported in part by the U.S. Department of Energy, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Science Undergraduate Laboratory Internship (SULI) program. These materials are available for collaborative research through the Molecular Foundry's User Program (foundry.lbl.gov). NR 58 TC 0 Z9 0 U1 1 U2 22 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0887-624X EI 1099-0518 J9 J POLYM SCI POL CHEM JI J. Polym. Sci. Pol. Chem. PD JAN 15 PY 2015 VL 53 IS 2 SI SI BP 256 EP 264 DI 10.1002/pola.27312 PG 9 WC Polymer Science SC Polymer Science GA AW2YA UT WOS:000346151300017 ER PT J AU Dowling, NM Johnson, SC Gleason, CE Jagust, WJ AF Dowling, N. Maritza Johnson, Sterling C. Gleason, Carey E. Jagust, William J. CA Alzheimers Dis Neuroimaging Initia TI The mediational effects of FDG hypometabolism on the association between cerebrospinal fluid biomarkers and neurocognitive function SO NEUROIMAGE LA English DT Article DE CSF biomarkers; Beta amyloid; FDG-PET; Tau; Alzheimer's disease; Longitudinal mediation; Parallel process latent growth; Structural equation modeling ID MILD COGNITIVE IMPAIRMENT; POSITRON-EMISSION-TOMOGRAPHY; PRECLINICAL ALZHEIMERS-DISEASE; BRAIN GLUCOSE-METABOLISM; MINI-MENTAL-STATE; APOLIPOPROTEIN-E; CSF BIOMARKERS; MEASUREMENT INVARIANCE; AMYLOID BURDEN; GENETIC RISK AB Positive cerebrospinal fluid (CSF) biomarkers of tau and amyloid beta42 suggest possible active underlying Alzheimer's disease (AD) including neurometabolic dysfunction and neurodegeneration leading to eventual cognitive decline. But the temporal relationship between CSF, imagingmarkers of neural function, and cognition has not been described. Using a statistical mediation model, we examined relationships between cerebrospinal fluid (CSF) analytes (hyperphosphorylated tau (p-Tau(181p)), beta-amyloid peptides 1-42 (A beta(1-42)), total tau (t-Tau), and their ratios); change in cognitive function; and change in [18F] fluorodeoxyglucose (FDG) uptake using positron emission tomography (PET). We hypothesized that a) abnormal CSF protein values at baseline, result in cognitive declines by decreasing neuronal glucose metabolism across time, and b) the role of altered glucose metabolism in the assumed causal chain varies by brain region and the nature of CSF protein alteration. Data from 412 individuals participating in Alzheimer's Disease Neuroimaging (ADNI) cohort studies were included in analyses. At baseline, individuals were cognitively normal (N = 82), or impaired: 241 with mild cognitive impairment, and 89 with Alzheimer's disease. A parallel-process latent growth curve model was used to test mediational effects of changes in regional FDG-PET uptake over time in relation to baseline CSF biomarkers and changes in cognition, measured with the 13-item Alzheimer Disease's Assessment Scale-cognitive subscale (ADAS-Cog). Findings suggested a causal sequence of events; specifically, FDG hypometabolism acted as a mediator between antecedent CSF biomarker alterations and subsequent cognitive impairment. Higher baseline concentrations of t-Tau, and p-Tau181p were more predictive of decline in cerebral glucose metabolism than lower baseline concentrations of A beta(1-42). FDG-PET changes appeared to mediate t-Tau or t-Tau/A beta(1-42)-associated cognitive change across all brain regions examined. Significant direct effects of alterations in A beta(1-42) levels on hypometabolism were observed in a single brain region: middle/inferior temporal gyrus. Results support a temporal framework model in which reduced CSF amyloid-related biomarkers occur earlier in the pathogenic pathway, ultimately leading to detrimental cognitive effects. Also consistent with this temporal framework model, baseline markers of neurofibrillary degeneration predicted changes in brain glucose metabolism in turn causing longitudinal cognitive changes, suggesting that tau-related burden precedes neurometabolic dysfunction. While intriguing, the hypothesized mediational relationships require further validation. Published by Elsevier Inc. C1 [Dowling, N. Maritza] Univ Wisconsin, Dept Biostat & Med Informat, Madison, WI 53792 USA. [Dowling, N. Maritza; Johnson, Sterling C.; Gleason, Carey E.] Univ Wisconsin, Alzheimers Dis Res Ctr, Madison, WI 53792 USA. [Johnson, Sterling C.; Gleason, Carey E.] William S Middleton Mem Vet Adm Med Ctr, Geriatr Res Educ & Clin Ctr, Madison, WI USA. [Jagust, William J.] Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA. [Jagust, William J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. RP Dowling, NM (reprint author), Univ Wisconsin, Sch Med & Publ Hlth, Dept Biostat & Med Informat, Madison, WI 53792 USA. EM nmdowlin@biostat.wisc.edu RI Kowall, Neil/G-6364-2012; OI Kowall, Neil/0000-0002-6624-0213; Preda, Adrian /0000-0003-3373-2438 FU Alzheimer's Disease Neuroimaging Initiative (ADNI) (National Institutes of Health) [U01 AG024904]; DOD ADNI (Department of Defense) [W81XWH-12-2-0012]; National Institute on Aging; National Institute of Biomedical Imaging and Bioengineering; Alzheimer's Association; Alzheimer's Drug Discovery Foundation; Araclon Biotech; BioClinica, Inc.; Biogen Idec Inc.; Bristol-Myers Squibb Company; Eisai Inc.; Elan Pharmaceuticals, Inc.; Eli Lilly and Company; EuroImmun; F. Hoffmann-La Roche Ltd and its affiliated company Genentech, Inc.; Fujirebio; GE Healthcare; IXICO Ltd.; Janssen Alzheimer Immunotherapy Research & Development, LLC.; Johnson & Johnson Pharmaceutical Research & Development LLC.; Medpace, Inc.; Merck Co., Inc.; Meso Scale Diagnostics, LLC.; NeuroRx Research; Neurotrack Technologies; Novartis Pharmaceuticals Corporation; Pfizer Inc.; Piramal Imaging; Servier; Synarc Inc.; Takeda Pharmaceutical Company; Canadian Institutes of Health Research; Alzheimer's Association [NIRG-12-242799]; National Institutes of Health [NIH-AG021155] FX Data collection and sharing for this project were funded by the Alzheimer's Disease Neuroimaging Initiative (ADNI) (National Institutes of Health Grant U01 AG024904) and DOD ADNI (Department of Defense award number W81XWH-12-2-0012). ADNI is funded by the National Institute on Aging, the National Institute of Biomedical Imaging and Bioengineering, and through generous contributions from the following: Alzheimer's Association; Alzheimer's Drug Discovery Foundation; Araclon Biotech; BioClinica, Inc.; Biogen Idec Inc.; Bristol-Myers Squibb Company; Eisai Inc.; Elan Pharmaceuticals, Inc.; Eli Lilly and Company; EuroImmun; F. Hoffmann-La Roche Ltd and its affiliated company Genentech, Inc.; Fujirebio; GE Healthcare;; IXICO Ltd.; Janssen Alzheimer Immunotherapy Research & Development, LLC.; Johnson & Johnson Pharmaceutical Research & Development LLC.; Medpace, Inc.; Merck & Co., Inc.; Meso Scale Diagnostics, LLC.; NeuroRx Research; Neurotrack Technologies; Novartis Pharmaceuticals Corporation; Pfizer Inc.; Piramal Imaging; Servier; Synarc Inc.; and Takeda Pharmaceutical Company. The Canadian Institutes of Health Research is providing funds to support ADNI clinical sites in Canada. Private sector contributions are facilitated by the Foundation for the National Institutes of Health (www.fnih.org). The grantee organization is the Northern California Institute for Research and Education, and the study is coordinated by the Alzheimer's Disease Cooperative Study at the University of California, San Diego. ADNI data are disseminated by the Laboratory for Neuro Imaging at the University of Southern California.; This research also was partially supported by a grant from the Alzheimer's Association (NIRG-12-242799, Dowling) and the National Institutes of Health (NIH-AG021155, Johnson). NR 81 TC 7 Z9 8 U1 4 U2 28 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 1053-8119 EI 1095-9572 J9 NEUROIMAGE JI Neuroimage PD JAN 15 PY 2015 VL 105 BP 357 EP 368 DI 10.1016/j.neuroimage.2014.10.050 PG 12 WC Neurosciences; Neuroimaging; Radiology, Nuclear Medicine & Medical Imaging SC Neurosciences & Neurology; Radiology, Nuclear Medicine & Medical Imaging GA AW1LG UT WOS:000346050300034 PM 25450107 ER PT J AU Sileghem, L Wallner, T Verhelst, S AF Sileghem, L. Wallner, T. Verhelst, S. TI A quasi-dimensional model for SI engines fueled with gasoline-alcohol blends: Knock modeling SO FUEL LA English DT Article DE Alcohol fuel; Spark ignition engine; Thermodynamic; Modeling; Knock ID AUTOIGNITION; IGNITION; METHANOL; COMBUSTION; MIXTURES AB As knock is one of the main factors limiting the efficiency of spark-ignition engines, the introduction of alcohol blends could help to mitigate knock concerns due to the elevated knock resistance of these blends. A model that can accurately predict their autoignition behavior would be of great value to engine designers. The current work aims to develop such a model for alcohol-gasoline blends. First, a mixing rule for the autoignition delay time of alcohol-gasoline blends is proposed. Subsequently, this mixing rule is used together with an autoignition delay time correlation of gasoline and an autoignition delay time correlation of methanol in a knock integral model that is implemented in a two-zone engine code. The predictive performance of the resulting model is validated through comparison against experimental measurements on a CFR engine for a range of gasoline-methanol blends. The knock limited spark advance, the knock intensity, the knock onset crank angle and the value of the knock integral at the experimental knock onset have been simulated and compared to the experimental values derived from in-cylinder pressure measurements. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Sileghem, L.; Verhelst, S.] Univ Ghent, Dept Flow Heat & Combust Mech, B-9000 Ghent, Belgium. [Wallner, T.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Sileghem, L (reprint author), Univ Ghent, Dept Flow Heat & Combust Mech, Sint Pietersnieuwstr 41, B-9000 Ghent, Belgium. EM Louis.Sileghem@UGent.be FU Research Foundation - Flanders [FWO11/ASP/056] FX L. Sileghem gratefully acknowledges a Ph. D. fellowship of the Research Foundation - Flanders (FWO11/ASP/056). The authors would like to thank BioMCN for providing the bio-methanol used in this study. NR 34 TC 4 Z9 4 U1 1 U2 20 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0016-2361 EI 1873-7153 J9 FUEL JI Fuel PD JAN 15 PY 2015 VL 140 BP 217 EP 226 DI 10.1016/j.fuel.2014.09.091 PG 10 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA AU2IA UT WOS:000345438400026 ER PT J AU Liu, S Gao, MC Liaw, PK Zhang, Y AF Liu, S. Gao, M. C. Liaw, P. K. Zhang, Y. TI Microstructures and mechanical properties of AlxCrFeNiTi0.25 alloys SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE Al-Cr-Fe-Ni-Ti; High entropy alloy; Microstructure; Mechanical property; CALPHAD calculation ID HIGH-ENTROPY ALLOY; THERMAL-STABILITY; BEHAVIOR; TEMPERATURE; PERFORMANCE; KINETICS AB Aiming to lower the cost and improve mechanical properties of AlCoCrFeNiTix high-entropy alloys that were studied previously, the present research investigated the effect of removing Co and lowering Ti contents at various Al contents, namely AlxCrFeNiTi0.25. The microstructures were investigated using optical microscopy, scanning electron microscopy, energy disperse spectroscopy, X-ray diffraction and transmission electron microscopy. Compression tests were conducted at room temperature. The present study showed that with increasing Al contents, the phase structures of the alloys changed from FCC + BCC to double BCC as the main phases. Among the alloys studied, all of them exhibit distinguished work hardening. Especially the Al0.5CrFeNiTi0.25 alloy has the highest fracture strength and plastic-strain limit of 3.47 GPa and 40%, respectively with a yield strength of 1.88 GPa. The observed microstructure is analyzed using CALPHAD calculations. (C) 2014 Elsevier B.V. All rights reserved. C1 [Liu, S.; Zhang, Y.] Univ Sci & Technol Beijing, State Key Lab Adv Met & Mat, Beijing 100083, Peoples R China. [Gao, M. C.] Natl Energy Technol Lab, Albany, OR 97321 USA. [Gao, M. C.] URS Corp, Albany, OR 97321 USA. [Liaw, P. K.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Zhang, Y (reprint author), Univ Sci & Technol Beijing, State Key Lab Adv Met & Mat, Beijing 100083, Peoples R China. EM drzhangy@ustb.edu.cn RI ZHANG, Yong/B-7928-2009 OI ZHANG, Yong/0000-0002-6355-9923 FU Natural Science Foundation (NSF) of China [NSFC51210105006]; Innovative Processing and Technologies Program of the National Energy Technology Laboratory's (NETL) Strategic Center for Coal under the RES contract [DE-FE-0004000]; US National Science Foundation [DMR-0909037, CMMI-0900271, CMMI-1100080]; Department of Energy (DOE), office of Nuclear Energy's Nuclear Energy University Program (NEUP) [00119262]; DOE, Office of Fossil Energy, National Energy Technology Laboratory [DE-FE-0008855, DE-FE-0011194]; Army Research Office [W911NF-13-1-0438] FX This research is supported by the Natural Science Foundation (NSF) of China, Granted No. NSFC51210105006. M.C.G. acknowledges the support of the Innovative Processing and Technologies Program of the National Energy Technology Laboratory's (NETL) Strategic Center for Coal under the RES contract DE-FE-0004000. We very much appreciate the financial support from the US National Science Foundation (DMR-0909037, CMMI-0900271, and CMMI-1100080), the Department of Energy (DOE), office of Nuclear Energy's Nuclear Energy University Program (NEUP) 00119262, the DOE, Office of Fossil Energy, National Energy Technology Laboratory (DE-FE-0008855 and DE-FE-0011194), and the Army Research Office (W911NF-13-1-0438) with C. Huber, C.V. Cooper, A. Ardell, E. Taleff, V. Cedro, R.O. Jensen, L.Tan, S. Lesica, S. Markovich, and S.N. Mathaudhu as contact monitors. NR 35 TC 15 Z9 16 U1 10 U2 70 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 EI 1873-4669 J9 J ALLOY COMPD JI J. Alloy. Compd. PD JAN 15 PY 2015 VL 619 BP 610 EP 615 DI 10.1016/j.jallcom.2014.09.073 PG 6 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA AS7IB UT WOS:000344429000090 ER PT J AU Raju, SV Oni, AA Godwal, BK Yan, J Drozd, V Srinivasan, S LeBeau, JM Rajan, K Saxena, SK AF Raju, S. V. Oni, A. A. Godwal, B. K. Yan, J. Drozd, V. Srinivasan, S. LeBeau, J. M. Rajan, K. Saxena, S. K. TI Effect of B and Cr on elastic strength and crystal structure of Ni3Al alloys under high pressure SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE Superalloys; High pressure; X-ray diffraction; Nano-indentation; Elastic properties ID NICKEL-BASED SUPERALLOYS; TEMPERATURE; INDENTATION; MODULUS; 1ST-PRINCIPLES; CHEMISTRY; CONSTANTS; HARDNESS; PHASE; NI AB Samples of Ni3Al, Ni3Al:B and Ni-Al-Cr super alloys were prepared by directional solidification method and their effect of alloying with ternary elements on the mechanical properties was investigated. In-situ X-ray diffraction studies were carried out on undoped Ni3Al, Ni3Al:B with boron 500 ppm and Ni-Al-Cr with 7.5 at.% of chromium super alloys at high pressure using diamond anvil cell. The results indicate that micro-alloying with B forms gamma'-phase (L1(2) structure), similar to the pure Ni Al-3, while Ni-Al-Cr alloy consists of gamma' precipitates in a matrix of gamma-phase (Ni-FCC structure). The crystal structure of all three alloys was stable up to 20 GPa. Micro alloying with boron increases bulk modulus of Ni3Al by 8% whereas alloying with chromium has the opposite effect decreasing the modulus by 11% when compared to undoped alloy. Further, the elastic modulus and hardness of Ni3Al, Ni3Al:B and Ni-Al-Cr alloys were determined using the nano-indentation technique, in combination with compressibility data which enabled the estimation of shear modulus and Poisson's ratio of these alloys. (C) 2014 Elsevier B.V. All rights reserved. C1 [Raju, S. V.; Drozd, V.; Saxena, S. K.] Florida Int Univ, Dept Mech Engn, CeSMEC, Miami, FL 33172 USA. [Oni, A. A.; LeBeau, J. M.] N Carolina State Univ, Dept Mat Sci & Engn, Raleigh, NC 27695 USA. [Godwal, B. K.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Yan, J.] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94730 USA. [Yan, J.] Univ Calif Santa Cruz, Dept Earth & Planetary Sci, Santa Cruz, CA 95064 USA. [Srinivasan, S.; Rajan, K.] Iowa State Univ, Dept Mat Sci & Engn, Iowa City, IA USA. RP Raju, SV (reprint author), Florida Int Univ, Dept Mech Engn, CeSMEC, Miami, FL 33172 USA. EM sraju@fiu.edu RI Drozd, Vadym/B-2518-2009 FU Air Force Office of Scientific Research [FA9550-12-1-0456]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors acknowledge support from the Air Force Office of Scientific Research (Grant No. FA9550-12-1-0456). The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Author SVR thanks Prof. Agarwal, Dept of Mechanical Engg. for useful discussions and help with nano-indentation measurements at the AMERI facility. NR 43 TC 7 Z9 7 U1 2 U2 38 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 EI 1873-4669 J9 J ALLOY COMPD JI J. Alloy. Compd. PD JAN 15 PY 2015 VL 619 BP 616 EP 620 DI 10.1016/j.jallcom.2014.09.012 PG 5 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA AS7IB UT WOS:000344429000091 ER PT J AU Halldorsson, S Lucumi, E Gomez-Sjoberg, R Fleming, RMT AF Halldorsson, Skarphedinn Lucumi, Edinson Gomez-Sjoeberg, Rafael Fleming, Ronan M. T. TI Advantages and challenges of microfluidic cell culture in polydimethylsiloxane devices SO BIOSENSORS & BIOELECTRONICS LA English DT Article DE Microfluidic; Cell culture; Polydimethylsiloxane ID ON-A-CHIP; NEURAL STEM-CELLS; IN-VITRO; OXYGEN LEVELS; QUANTITATIVE-ANALYSIS; SURFACE MODIFICATION; ENDOTHELIAL-CELLS; MASS-SPECTROMETRY; ANALYSIS SYSTEMS; MAMMALIAN-CELLS AB Culture of cells using various microfluidic devices is becoming more common within experimental cell biology. At the same time, a technological radiation of microfluidic cell culture device designs is currently in progress. Ultimately, the utility of microfluidic cell culture will be determined by its capacity to permit new insights into cellular function. Especially insights that would otherwise be difficult or impossible to obtain with macroscopic cell culture in traditional polystyrene dishes, flasks or well-plates. Many decades of heuristic optimization have gone into perfecting conventional cell culture devices and protocols. In comparison, even for the most commonly used microfluidic cell culture devices, such as those fabricated from polydimethylsiloxane (PDMS), collective understanding of the differences in cellular behavior between microfluidic and macroscopic culture is still developing. Moving in vitro culture from macroscopic culture to PDMS based devices can come with unforeseen challenges. Changes in device material, surface coating, cell number per unit surface area or per unit media volume may all affect the outcome of otherwise standard protocols. In this review, we outline some of the advantages and challenges that may accompany a transition from macroscopic to microfluidic cell culture. We focus on decisive factors that distinguish macroscopic from microfluidic cell culture to encourage a reconsideration of how macroscopic cell culture principles might apply to microfluidic cell culture. (C) 2014 The Authors. Published by Elsevier B.V. C1 [Halldorsson, Skarphedinn] Univ Iceland, Ctr Syst Biol, Reykjavik, Iceland. [Halldorsson, Skarphedinn] Univ Iceland, Biomed Ctr, Reykjavik, Iceland. [Gomez-Sjoeberg, Rafael] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Engn, Berkeley, CA 94720 USA. [Lucumi, Edinson; Fleming, Ronan M. T.] Univ Luxembourg, Luxembourg Ctr Syst Biomed, Esch Sur Alzette, Luxembourg. RP Fleming, RMT (reprint author), Univ Luxembourg, Luxembourg Ctr Syst Biomed, 7 Ave Hauts Fourneaux, Esch Sur Alzette, Luxembourg. EM ronan.mt.fleming@gmail.com FU National Research Fund, Luxembourg [6728678]; Icelandic Center for Research, START postdoctoral grant [130816-051] FX This work was supported in part by the National Research Fund, Luxembourg, Award #6728678 and Icelandic Center for Research, START postdoctoral grant no. 130816-051. NR 126 TC 70 Z9 71 U1 49 U2 276 PU ELSEVIER ADVANCED TECHNOLOGY PI OXFORD PA OXFORD FULFILLMENT CENTRE THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0956-5663 EI 1873-4235 J9 BIOSENS BIOELECTRON JI Biosens. Bioelectron. PD JAN 15 PY 2015 VL 63 BP 218 EP 231 DI 10.1016/j.bios.2014.07.029 PG 14 WC Biophysics; Biotechnology & Applied Microbiology; Chemistry, Analytical; Electrochemistry; Nanoscience & Nanotechnology SC Biophysics; Biotechnology & Applied Microbiology; Chemistry; Electrochemistry; Science & Technology - Other Topics GA AR1HT UT WOS:000343337000032 PM 25105943 ER PT J AU Wang, CH Poudel, L Taylor, AE Lawrence, JM Christianson, AD Chang, S Rodriguez-Rivera, JA Lynn, JW Podlesnyak, AA Ehlers, G Baumbach, RE Bauer, ED Gofryk, K Ronning, F McClellan, KJ Thompson, JD AF Wang, C. H. Poudel, L. Taylor, A. E. Lawrence, J. M. Christianson, A. D. Chang, S. Rodriguez-Rivera, J. A. Lynn, J. W. Podlesnyak, A. A. Ehlers, G. Baumbach, R. E. Bauer, E. D. Gofryk, K. Ronning, F. McClellan, K. J. Thompson, J. D. TI Quantum critical fluctuations in the heavy fermion compound Ce(Ni0.935Pd0.065)(2)Ge-2 SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE antiferromagnetic quantum critical point; non-Fermi liquid; Kondo disorder; heavy fermion; correlation length; correlation time ID LIQUID BEHAVIOR; MAGNETIC INSTABILITY; CENI2GE2; TEMPERATURES; ELECTRON; DISORDER; SYSTEMS; ALLOYS AB Electric resistivity, specific heat, magnetic susceptibility, and inelastic neutron scattering experiments were performed on a single crystal of the heavy fermion compound Ce(Ni0.935Pd0.065)(2)Ge-2 in order to study the spin fluctuations near an antiferromagnetic (AF) quantum critical point (QCP). The resistivity and the specific heat coefficient for T <= 1 K exhibit the power law behavior expected for a 3D itinerant AF QCP (rho(T) similar to T-3/2 and gamma(T) similar to gamma 0 - bT(1/2)). However, for 2 <= T <= 10 K, the susceptibility and specific heat vary as logT and the resistivity varies linearly with temperature. Furthermore, despite the fact that the resistivity and specific heat exhibit the non-Fermi liquid behavior expected at a QCP, the correlation length, correlation time, and staggered susceptibility of the spin fluctuations remain finite at low temperature. We suggest that these deviations from the divergent behavior expected for a QCP may result from alloy disorder. C1 [Wang, C. H.; Poudel, L.; Taylor, A. E.; Christianson, A. D.; Podlesnyak, A. A.; Ehlers, G.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Wang, C. H.; Lawrence, J. M.] Univ Calif Irvine, Irvine, CA 92697 USA. [Poudel, L.; Christianson, A. D.] Univ Tennessee, Knoxville, TN 37996 USA. [Chang, S.; Rodriguez-Rivera, J. A.; Lynn, J. W.] Natl Inst Stand & Technol, Gaithersburg, MD 20899 USA. [Rodriguez-Rivera, J. A.] Univ Maryland, College Pk, MD 20742 USA. [Baumbach, R. E.; Bauer, E. D.; Gofryk, K.; Ronning, F.; McClellan, K. J.; Thompson, J. D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Baumbach, R. E.] Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. [Gofryk, K.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Wang, CH (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RI Taylor, Alice/I-5616-2012; Instrument, CNCS/B-4599-2012; Ehlers, Georg/B-5412-2008; christianson, andrew/A-3277-2016; Podlesnyak, Andrey/A-5593-2013; Rodriguez-Rivera, Jose/A-4872-2013; OI Taylor, Alice/0000-0002-3036-3019; Ehlers, Georg/0000-0003-3513-508X; christianson, andrew/0000-0003-3369-5884; Podlesnyak, Andrey/0000-0001-9366-6319; Rodriguez-Rivera, Jose/0000-0002-8633-8314; Gofryk, Krzysztof/0000-0002-8681-6857; Ronning, Filip/0000-0002-2679-7957; Bauer, Eric/0000-0003-0017-1937 FU Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; Scientific User Facilities Division Office of Basic Energy Sciences, DOE; US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-FG02-03ER46036]; National Science Foundation [DMR-0944772] FX We thank C Stock for his assistance in the measurement at NIST, Min-Nan Ou for assistance at SNS, and C Batista for helpful conversations. Research at ORNL was sponsored by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, and was supported by the Scientific User Facilities Division Office of Basic Energy Sciences, DOE. Work at UC Irvine and Los Alamos National Laboratory was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; the work at UC-Irvine was funded under Award DE-FG02-03ER46036. This work utilized facilities supported in part by the National Science Foundation under Agreement No. DMR-0944772. NR 21 TC 2 Z9 2 U1 1 U2 16 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD JAN 14 PY 2015 VL 27 IS 1 AR 015602 DI 10.1088/0953-8984/27/1/015602 PG 7 WC Physics, Condensed Matter SC Physics GA CE6EO UT WOS:000351929600009 PM 25469766 ER PT J AU Wang, Q Cao, Y Wan, XG Denlinger, JD Qi, TF Korneta, OB Cao, G Dessau, DS AF Wang, Q. Cao, Y. Wan, X. G. Denlinger, J. D. Qi, T. F. Korneta, O. B. Cao, G. Dessau, D. S. TI Experimental electronic structure of the metallic pyrochlore iridate Bi2Ir2O7 SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE angle-resolved photoemission spectroscopy; electronic structure; pyrochlore iridate AB Angle-resolved photoemission measurements have been performed on Bi2Ir2O7 single crystals, a metallic end-member of the family of pyrochlore iridates. The density of states, the Fermi surface, and the near-Fermi-level band dispersion in the plane perpendicular to the (1, 1, 1) direction were all measured and found to be in rough overall agreement with our LDA + SOC density functional calculations. Assuming that this same calculation approach will extend to other members of the pyrochlore iridates, the overall agreement we found increases the possibility that some of the novel predicted phases such as quantum spin-ice or Weyl Fermion states will exist in this family of compounds. C1 [Wang, Q.; Cao, Y.; Dessau, D. S.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Wang, Q.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Cao, Y.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Wan, X. G.] Nanjing Univ, Natl Lab Solid State Microstruct, Nanjing 210093, Jiangsu, Peoples R China. [Wan, X. G.] Nanjing Univ, Dept Phys, Nanjing 210093, Jiangsu, Peoples R China. [Denlinger, J. D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Qi, T. F.; Korneta, O. B.; Cao, G.] Univ Kentucky, Dept Phys & Astron, Ctr Adv Mat, Lexington, KY 40506 USA. RP Wang, Q (reprint author), Univ Colorado, Dept Phys, Boulder, CO 80309 USA. EM dessau@colorado.edu OI Cao, Yue/0000-0002-3989-158X FU Department of Energy [DE-FG02-03ER46066]; NSF [DMR-0856234, DMR-1265162]; US Department of Energy; [EPS-0814194] FX This work was supported by the Department of Energy under grant DE-FG02-03ER46066 to the University of Colorado and grants NSF DMR-0856234, NSF DMR-1265162, and EPS-0814194 to the University of Kentucky. This work is also based in part upon research conducted at the Advanced Light Source, which is funded by the US Department of Energy. NR 22 TC 3 Z9 3 U1 15 U2 63 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD JAN 14 PY 2015 VL 27 IS 1 AR 015502 DI 10.1088/0953-8984/27/1/015502 PG 5 WC Physics, Condensed Matter SC Physics GA CE6EO UT WOS:000351929600005 PM 25469557 ER PT J AU Aad, G Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Andersb, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Auerbach, B Augsten, K Aurousseau, M Avolio, G Axen, B Azuelos, G Azuma, Y Baak, MA Baas, AE Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Balek, P Balli, F Banas, E Banerjee, S Bannoura, AAE Bansal, V Bansil, HS Barak, L Baranov, SP Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R 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M Cavasinni, V Ceradini, F Cerio, BC Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chang, P Chapleau, B Chapman, JD Charfeddine, D Charlton, DG Chau, CC Barajas, CAC Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, S Chen, X Chen, Y Chen, Y Cheng, HC Cheng, Y Cheplakov, A El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiefari, G Childers, JT Chilingarov, A Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Chouridou, S Chow, BKB Chromek-Burckhart, D Chu, ML Chudoba, J Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Ciftci, R Cinca, D Cindro, V Ciocio, A Citron, ZH Citterio, M Ciubancan, M Clark, A Clark, PJ Clarke, RN Cleland, W Clemens, JC Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Cogan, JG Cole, B Cole, S Colijn, AP Collot, J Colombo, T Compostella, G Muino, PC Coniavitis, E Connell, SH 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CA ATLAS Collaboration TI Search for the b(b)over-bar decay of the Standard Model Higgs boson in associated (W/Z)H production with the ATLAS detector SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID PARTON DISTRIBUTIONS; MONTE-CARLO; MASSLESS PARTICLES; BROKEN SYMMETRIES; HADRON COLLIDERS; LHC; TEVATRON AB A search for the b (b) over bar decay of the Standard Model Higgs boson is performed with the ATLAS experiment using the full dataset recorded at the LHC in Run 1. The integrated luminosities used are 4.7 and 20.3 fb(-1) from pp collisions at root s = 7 and 8 TeV, respectively. The processes considered are associated (WIZ)H production, where W -> e nu/mu nu, Z -> ee/mu mu, and Z -> nu nu. The observed (expected) deviation from the backgroundonly hypothesis corresponds to a significance of 1.4 (2.6) standard deviations and the ratio of the measured signal yield to the Standard Model expectation is found to be mu = 0.52 +/- 0.32 (stat.) +/- 0.24 (syst.) for a Higgs boson mass of 125.36 GeV. The analysis procedure is validated by a measurement of the yield of (W/Z)Z production with Z -> b (b) over bar in the same final states as for the Higgs boson search, from which the ratio of the observed signal yield to the Standard Model expectation is found to be 0.74 +/- 0.09 (stat.) +/- 0.14 (syst.). C1 [Jackson, P.; Lee, L.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Gingrich, D. M.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Ciftci, R.; Yildiz, H. Duran] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Yilmaz, M.] Gazi Univ, Dept Phys, Ankara, Turkey. [Kuday, S.] Istanbul Aydin Univ, Istanbul, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. [Barnovska, Z.; Berger, N.; Delmastro, M.; Di Ciaccio, L.; Elles, S.; Goy, C.; Hryn'ova, T.; Jezequel, S.; Keoshkerian, H.; Koletsou, I.; Lafaye, R.; Leveque, J.; Lombardo, V. P.; Massol, N.; Przysiezniak, H.; Sauvage, G.; Sauvan, E.; Schwoerer, M.; Simard, O.; Todorov, T.; Wingerter-Seez, I.] CNRS, IN2P3, LAPP, Annecy Le Vieux, France. [Barnovska, Z.; Berger, N.; Delmastro, M.; Di Ciaccio, L.; Elles, S.; Goy, C.; Hryn'ova, T.; Jezequel, S.; Keoshkerian, H.; Koletsou, I.; Lafaye, R.; Leveque, J.; Lombardo, V. P.; Massol, N.; Przysiezniak, H.; Sauvage, G.; Sauvan, E.; Schwoerer, M.; Simard, O.; Todorov, T.; Wingerter-Seez, I.] Univ Savoie, Annecy Le Vieux, France. [Asquith, L.; Auerbach, B.; Blair, R. E.; Chekanov, S.; Childers, J. T.; Feng, E. J.; Goshaw, A. T.; LeCompte, T.; Love, J.; Malon, D.; Nguyen, D. H.; Nodulman, L.; Paramonov, A.; Price, L. E.; Proudfoot, J.; Stanek, R. W.; van Gemmeren, P.; Vaniachine, A.; Yoshida, R.; Zhang, J.] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Cheu, E.; Johns, K. A.; Kaushik, V.; Lampen, C. L.; Lampl, W.; Lei, X.; Leone, R.; Loch, P.; Nayyar, R.; O'grady, F.; Rutherfoord, J. P.; Shupe, M. A.; Varnes, E. W.; Veatch, J.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Brandt, A.; Cote, D.; Darmora, S.; De, K.; Farbin, A.; Griffiths, J.; Hadavand, H. K.; Heelan, L.; Kim, H. Y.; Maeno, M.; Ozturk, N.; Pravahan, R.; Sosebee, M.; Spurlock, B.; Stradling, A. R.; Usai, G.; Vartapetian, A.; White, A.; Yu, J.] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA. [Angelidakis, S.; Antonaki, A.; Chouridou, S.; Fassouliotis, D.; Giokaris, N.; Ioannou, P.; Iordanidou, K.; Kourkoumelis, C.; Manousakis-Katsikakis, A.; Tsirintanis, N.] Univ Athens, Dept Phys, Athens, Greece. [Alexopoulos, T.; Byszewski, M.; Dris, M.; Gazis, E. N.; Iakovidis, G.; Karakostas, K.; Karastathis, N.; Leontsinis, S.; Maltezos, S.; Ntekas, K.; Panagiotopoulou, E.; Papadopoulou, Th. D.; Tsipolitis, G.; Vlachos, S.] Natl Tech Univ Athens, Dept Phys, Zografos, Greece. [Abdinov, O.; Khalil-zada, F.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Anjos, N.; Asbah, N.; Bosman, M.; Armadans, R. Caminal; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fracchia, S.; Giangiobbe, V.; Parra, G. Gonzalez; Grinstein, S.; Huang, Y.; Rozas, A. Juste; Korolkov, I.; Le Menedeu, E.; Paz, I. Lopez; Martinez, M.; Mir, L. M.; Berlingen, J. Montejo; Pages, A. Pacheco; Aranda, C. Padilla; Bueso, X. Portell; Riu, I.; Rubbo, F.; Sorin, V.; Succurro, A.; Tripiana, M. F.; Tsiskaridze, S.] Univ Autonoma Barcelona, Inst Fis DAltes Energies, E-08193 Barcelona, Spain. [Anjos, N.; Asbah, N.; Bosman, M.; Armadans, R. Caminal; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fracchia, S.; Giangiobbe, V.; Parra, G. Gonzalez; Grinstein, S.; Huang, Y.; Rozas, A. Juste; Korolkov, I.; Le Menedeu, E.; Paz, I. Lopez; Martinez, M.; Mir, L. M.; Berlingen, J. Montejo; Pages, A. Pacheco; Aranda, C. Padilla; Bueso, X. Portell; Riu, I.; Rubbo, F.; Sorin, V.; Succurro, A.; Tripiana, M. F.; Tsiskaridze, S.] Univ Autonoma Barcelona, Dept Fis, E-08193 Barcelona, Spain. [Agatonovic-Jovin, T.; Bozic, I.; Dimitrievska, A.; Krstic, J.; Marjanovic, M.; Popovic, D. S.; Sijacki, Dj.; Simic, Lj.; Milosavljevic, M. Vranjes] Univ Belgrade, Inst Phys, Belgrade, Serbia. [Mamuzic, J.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Buanes, T.; Dale, O.; Eigen, G.; Kastanas, A.; Liebig, W.; Lipniacka, A.; dit Latour, B. Martin; Rosendahl, P. L.; Sandaker, H.; Sjursen, T. B.; Smestad, L.; Stugu, B.; Ugland, M.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Axen, B.; Barnett, R. M.; Beringer, J.; Biesiada, J.; Brandt, G.; Brosamer, J.; Calafiura, P.; Caminada, L. M.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Dube, S.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Holmes, T. R.; Hurwitz, M.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Pollard, C. S.; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Virzi, J.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Axen, B.; Barnett, R. M.; Beringer, J.; Biesiada, J.; Brandt, G.; Brosamer, J.; Calafiura, P.; Caminada, L. M.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Dube, S.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Holmes, T. R.; Hurwitz, M.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Pollard, C. S.; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Virzi, J.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Herrberg-Schubert, R.; Hristova, I.; Kind, O.; Kolanoski, H.; Lacker, H.; Lohse, T.; Loscutoff, P.; Nikiforov, A.; Rehnisch, L.; Rieck, P.; Schulz, H.; Stamm, S.; Wendland, D.; zur Nedden, M.] Humboldt Univ, Dept Phys, D-10099 Berlin, Germany. [Agustoni, M.; Beck, H. P.; Cervelli, A.; Ereditato, A.; Gallo, V.; Haug, S.; Kruker, T.; Marti, L. F.; Meloni, F.; Schneider, B.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fdn Phys, Bern, Switzerland. [Agustoni, M.; Beck, H. P.; Cervelli, A.; Ereditato, A.; Gallo, V.; Haug, S.; Kruker, T.; Marti, L. F.; Meloni, F.; Schneider, B.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allbrooke, B. M. M.; Bella, L. Aperio; Bansil, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Giuliani, C.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Jakobs, K.; Kopp, A. K.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Palmer, J. D.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingulc, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Alberghi, G. L.; Bellagamba, L.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Caforio, D.; Corradi, M.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Ist Nazl Fis Nucl, Sez Bologna, Bologna, Italy. [Alberghi, G. L.; Caforio, D.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Hageboeck, S.; Hellmich, D.; Hillert, S.; Huegging, F.; Janssen, J.; Khoriauli, G.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Loddenkoetter, T.; Mergelmeyer, S.; Mijovic, L.; Mueller, K.; Nanava, G.; Nattermann, T.; Obermann, T.; Pohl, D.; Sarrazin, B.; Schaepe, S.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Stillings, J. A.; Tannoury, N.; Therhaag, J.; Uchida, K.; Uhlenbrock, M.; Vogel, A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Fitzgerald, E. A.; Gozpinar, S.; Sciolla, G.; Venturini, A.; Zambito, S.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE, EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; de Andrade Filho, L. Manhaes] Fed Univ Juiz De Fora UFJF, Juiz De Fora, Brazil. [Do Vale, M. A. B.] Fed Univ Sao Joao Del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. 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West Univ Timisoara, Timisoara, Romania. [Garzon, G. Otero y; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cottin, G.; Dyndal, M.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; Marchand, J. F.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Battistin, M.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Uhrssen, M. D.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Franchino, S.; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hajduk, Z.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jakobsen, S.; Jansen, H.; Jungst, R. M.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Martin, B.; Marzin, A.; Messina, A.; Meyer, J.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Savu, D. O.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Cheng, Y.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Guido, E.; Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei Shi, Anhui, Peoples R China. [Chen, S.; Li, Y.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Shandong, Peoples R China. [Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Liao, H.; Pallin, D.; Podlyski, F.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Liao, H.; Pallin, D.; Podlyski, F.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Liao, H.; Pallin, D.; Podlyski, F.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Guo, J.; Hu, D.; Hughes, E. W.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Wulf, E.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Coll Cosenza, Lab Nazl Frascati, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Gornicki, E.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. 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Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Bessner, M.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys IV, D-44221 Dortmund, Germany. [Anger, P.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Kajomovitz, E.; Kotwal, A.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Prokofiev, K.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Uscher, D. B.; Coniavitis, E.; Consorti, V.; Dao, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Herten, G.; Javurek, T.; Jenni, P.; Kiss, F.; Oneke, K. K.; Kruse, M. C.; Kuehn, S.; Lai, S.; Landgraf, U.; Madar, R.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ronzani, M.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fak Mathemat & Phys, D-79106 Freiburg, Germany. [Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Miucci, A.; Muenstermann, D.; Nektarijevic, S.; Nikolics, K.; Picazio, A.; Pohl, M.; Rosbach, K.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Univ Genoa, Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartmento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; O'Shea, V.; Barrera, C. Oropeza; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; Denis, R. D. St.; Stewart, G. A.; Thompson, A. S.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Bindi, M.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Keil, M.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Dietzsch, T. A.; Djuvsland, J. I.; Dunford, M.; Hanke, P.; Jongmanns, J.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Andersb, C. F.; Giulini, M.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, Inst Informat Technol, ZITI, Mannheim, Germany. [Nagasaka, Y.] Fac Appl Informat Sci, Hiroshima Inst Technol, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, NT, Peoples R China. Univ Hong Kong, Dept Phys, Hong Kong, Peoples R China. Hong Kong Univ Sci & Technol, Kowloon, Hong Kong, Peoples R China. [Brunet, S.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Morange, N.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Pluth, D.; Prell, S.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Soloshenko, A.; Topilin, N. D.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, C.; Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Jana, D. K.; Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Univ Salento, Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Readioff, N. P.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Sevan, B. P. Ker .; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Sevan, B. P. Ker .; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bona, M.; Bret, M. Cano; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Cooper, B. D.; Davison, A. R.; Davison, P.; Falla, R. J.; Gregersen, K.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Greenwood, Z. D.; Sawyer, L.; Sircar, A.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barlow, N.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Blum, W.; Uscher, V. B.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Goeringer, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Ulsing, T. A. H.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Barnes, S. L.; Borri, M.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Thompson, R. J.; Tomlinson, L.; Ughetto, M.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Gao, J.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Mantifel, R.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Jennens, D.; Kubota, T.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Dubbert, J.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Harper, D.; Hu, X.; Levin, D.; Liu, L.; Long, J. D.; Lu, N.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Panikashvili, N.; Qian, J.; Schwarz, T. A.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Cost, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Univ Milan, Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Consonni, S. M.; Fanti, M.; Perini, L.; Pizio, C.; Ragusa, F.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Carminati, L.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Romaniouk, A.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Tsiareshka, P. V.; Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Heller, C.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Merola, L.; Moser, H. G.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst Phys, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Patricelli, S.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Univ Naples Federico II, Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Di Donato, C.; Giordano, R.; Patricelli, S.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Koenig, A. C.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Burghgrave, B.; Calkins, R.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Tannenwald, B. B.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Behr, K.; Boddy, C. R.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Univ Pavia, Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Meyer, C.; Ospanov, R.; Saxon, J.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Univ Pisa, Ist Nazl Fis Nucl, Sez Pisa, I-56100 Pisa, Italy. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Mueller, J.; Prieur, D.; Sapp, K.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Wemans, A. Do Valle; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Marques, C. N.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao Fis Expt Particulas LIP, Lisbon, Portugal. [Dos Santos, S. P. Amor; Amorim, A.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, P-1699 Lisbon, Portugal. [Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.; Pina, J.] Univ Granada, Dept Fis Teor Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.; Pina, J.] Univ Granada, CAFPE, Granada, Spain. [Wemans, A. Do Valle] Univ Nova Lisboa, Dept Fis, P-1200 Lisbon, Portugal. [Wemans, A. Do Valle] Univ Nova Lisboa, CEFITEC, Fac Ciencias Tecnol, P-1200 Lisbon, Portugal. [Bohm, J.; Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Particle Phys Dept, Rutherford Appleton Lab, Didcot, Oxon, England. [Tanaka, S.] Ritsumeikan Univ, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Stanescu, C.; Taccini, C.; Trovatelli, M.] Univ Rome Tre, Ist Nazl Fis Nucl, Sez Roma Tre, I-00146 Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Taccini, C.; Trovatelli, M.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Techn Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA, Fac Sci Semlalia, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mal, P.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay, DSM IRFU Inst Rech Lois Fondamentales Univ, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Suruliz, K.; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; O'Neil, D. C.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nef, P. D.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Connell, S. H.; Lee, C. A.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Carrillo-Montoya, G. D.; Castaneda-Miranda, E.; Hamity, G. N.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bessidskaia, O.; Bohm, C.; Clement, C.; Cribbs, W. A.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.] Univ Stockholm, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bessidskaia, O.; Clement, C.; Cribbs, W. A.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Sjoelin, J.; Strandberg, S.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [AbouZeid, O. S.; Bartsch, V.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Guicheney, C.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Ren, Z. L.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei 115, Taiwan. [Abreu, H.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Alexandre, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Leisos, A.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Sidiropoulou, O.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Etzion, E.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [Brelier, B.; Chau, C. C.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Fortin, D.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Ramos, J. A. Manjarres; Palacino, G.; Qureshi, A.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Quayle, W. B.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Coll Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Brazzale, S. F.; Quayle, W. B.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Cobal, M.; Giordani, M. P.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Buszello, C. P.; Corso-Radu, A.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Pinamonti, M.; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Pinamonti, M.; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Fis Atom Mol Nucl, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Pinamonti, M.; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Pinamonti, M.; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. 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A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Kimura, N.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Redelbach, A.; Schreyer, M.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Barisonzi, M.; Becker, K.; Beermann, T. A.; Boek, T. T.; Braun, H. 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Shmeleva, Alevtina/M-6199-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; De, Kaushik/N-1953-2013; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Riu, Imma/L-7385-2014; Cavalli-Sforza, Matteo/H-7102-2015; Marti-Garcia, Salvador/F-3085-2011; Della Pietra, Massimo/J-5008-2012; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Grancagnolo, Sergio/J-3957-2015; Doyle, Anthony/C-5889-2009; spagnolo, stefania/A-6359-2012; Tassi, Enrico/K-3958-2015; Ciubancan, Liviu Mihai/L-2412-2015; Zhukov, Konstantin/M-6027-2015; Mir, Lluisa-Maria/G-7212-2015; Livan, Michele/D-7531-2012; Villa, Mauro/C-9883-2009; White, Ryan/E-2979-2015; Brooks, William/C-8636-2013; Di Domenico, Antonio/G-6301-2011; Connell, Simon/F-2962-2015; Bosman, Martine/J-9917-2014; Joergensen, Morten/E-6847-2015; Boyko, Igor/J-3659-2013; Mitsou, Vasiliki/D-1967-2009; Carquin, Edson/G-5221-2015 OI Fabbri, Laura/0000-0002-4002-8353; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Olshevskiy, Alexander/0000-0002-8902-1793; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Smirnova, Oxana/0000-0003-2517-531X; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Wemans, Andre/0000-0002-9669-9500; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Perrino, Roberto/0000-0002-5764-7337; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Tikhomirov, Vladimir/0000-0002-9634-0581; Warburton, Andreas/0000-0002-2298-7315; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; De, Kaushik/0000-0002-5647-4489; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Riu, Imma/0000-0002-3742-4582; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Grancagnolo, Sergio/0000-0001-8490-8304; Doyle, Anthony/0000-0001-6322-6195; spagnolo, stefania/0000-0001-7482-6348; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Mir, Lluisa-Maria/0000-0002-4276-715X; Livan, Michele/0000-0002-5877-0062; Villa, Mauro/0000-0002-9181-8048; White, Ryan/0000-0003-3589-5900; Brooks, William/0000-0001-6161-3570; Di Domenico, Antonio/0000-0001-8078-2759; Connell, Simon/0000-0001-6000-7245; Bosman, Martine/0000-0002-7290-643X; Joergensen, Morten/0000-0002-6790-9361; Boyko, Igor/0000-0002-3355-4662; Mitsou, Vasiliki/0000-0002-1533-8886; Carquin, Edson/0000-0002-7863-1166 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 100 TC 25 Z9 25 U1 9 U2 79 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN 14 PY 2015 IS 1 AR 069 DI 10.1007/JHEP01(2015)069 PG 89 WC Physics, Particles & Fields SC Physics GA CB4PN UT WOS:000349610300002 ER PT J AU Wang, HL Bai, Y Chen, S Luo, XY Wu, C Wu, F Lu, J Amine, K AF Wang, Huali Bai, Ying Chen, Shi Luo, Xiangyi Wu, Chuan Wu, Feng Lu, Jun Amine, Khalil TI Binder-Free V2O5 Cathode for Greener Rechargeable Aluminum Battery SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE aluminum battery; binder-free; V2O5 cathode; ionic liquid electrolyte; PTFE binder; PVDF binder ID SODIUM-ION BATTERIES; ENERGY-STORAGE; SECONDARY BATTERIES; KEY MATERIALS; DIRECT GROWTH; HIGH-CAPACITY; ANODE; MAGNESIUM; ARRAYS; ELECTROCHEMISTRY AB This letter reports on the investigation of a binder-free cathode material to be used in rechargeable aluminum batteries. This cathode is synthesized by directly depositing V2O5 on a Ni foam current collector. Rechargeable aluminum coin cells fabricated using the as-synthesized binder-free cathode delivered an initial discharge capacity of 239 mAh/g, which is much higher than that of batteries fabricated using a cathode composed of V2O5 nanowires and binder. An obvious discharge voltage plateau appeared at 0.6 V in the discharge curves of the Ni-V2O5 cathode, which is slightly higher than that of the V2O5 nanowire cathodes with common binders. This improvement is attributed to reduced electrochemical polarization. C1 [Wang, Huali; Bai, Ying; Chen, Shi; Wu, Chuan; Wu, Feng] Beijing Inst Technol, Sch Chem Engn & Environm, Beijing Key Lab Environm Sci & Engn, Beijing 100081, Peoples R China. [Luo, Xiangyi; Lu, Jun; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA. RP Bai, Y (reprint author), Beijing Inst Technol, Sch Chem Engn & Environm, Beijing Key Lab Environm Sci & Engn, Beijing 100081, Peoples R China. EM membrane@bit.edu.cn; junlu@anl.gov; amine@anl.gov RI wu, chuan/A-1447-2009; Luo, Xiangyi/K-6058-2015 OI Luo, Xiangyi/0000-0002-4817-1461 FU National 973 project of China [2015CB251100]; Program for New Century Excellent Talents in University [NCET-13-0033]; U.S. Department of Energy [DE-AC0206CH11357]; Vehicle Technologies Office, Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy (EERE) FX The present work was supported by the National 973 project of China (2015CB251100), and the Program for New Century Excellent Talents in University (Grant NCET-13-0033). This work was also supported by the U.S. Department of Energy under Contract DE-AC0206CH11357 with the main support provided by the Vehicle Technologies Office, Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy (EERE). The authors especially thank US-China Electric Vehicle and Battery Technology program between Argonne National Laboratory and Beijing Institute of Technology. NR 23 TC 25 Z9 25 U1 19 U2 235 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JAN 14 PY 2015 VL 7 IS 1 BP 80 EP 84 DI 10.1021/am508001h PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA AZ2TM UT WOS:000348085200011 PM 25521045 ER PT J AU Zhao, H Yuca, N Zheng, ZY Fu, YB Battaglia, VS Abdelbast, G Zaghib, K Liu, G AF Zhao, Hui Yuca, Neslihan Zheng, Ziyan Fu, Yanbao Battaglia, Vincent S. Abdelbast, Guerfi Zaghib, Karim Liu, Gao TI High Capacity and High Density Functional Conductive Polymer and SiO Anode for High-Energy Lithium-Ion Batteries SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE calendering; conductive polymer binder; lithium-ion battery; silicon monoxide ID SENSITIZED SOLAR-CELL; SILICA NANOPARTICLES; NEGATIVE ELECTRODE; HYBRID FILMS; DESIGN; BINDER; LI; PERFORMANCE; SIMULATION; LIMN2O4 AB High capacity and high density functional conductive polymer binder/SiO electrodes are fabricated and calendered to various porosities. The effect of calendering is investigated in the reduction of thickness and porosity, as well as the increase of density. SiO particle size remains unchanged after calendering. When compressed to an appropriate density, an improved cycling performance and increased energy density are shown compared to the uncalendered electrode and overcalendered electrode. The calendered electrode has a high-density of similar to 1.2 g/cm(3). A high loading electrode with an areal capacity of similar to 3.5 mAh/cm(2) at a C/10 rate is achieved using functional conductive polymer binder and simple and effective calendering method. C1 [Zhao, Hui; Zheng, Ziyan; Fu, Yanbao; Battaglia, Vincent S.; Liu, Gao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Yuca, Neslihan] Istanbul Tech Univ, Energy Inst, TR-34469 Istanbul, Turkey. [Zheng, Ziyan] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Abdelbast, Guerfi; Zaghib, Karim] Inst Rech Elect Hydroquebec IREQ, Montreal, PQ H2Z 1A4, Canada. RP Liu, G (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM gliu@lbl.gov RI Fu, Yanbao/F-9583-2011 OI Fu, Yanbao/0000-0001-7752-680X FU Energy Efficiency, Vehicle Technologies Office of the U.S. Department of Energy (U.S. DOE) under the Batteries for Advanced Transportation Technologies (BATT) Program - U.S. Department of Energy [DE-AC02-05 CH11231]; Scientific and Technological Research Council of Turkey (TUBITAK) in Ankara, Turkey FX This work was funded by the Assistant Secretary for Energy Efficiency, Vehicle Technologies Office of the U.S. Department of Energy (U.S. DOE) under the Batteries for Advanced Transportation Technologies (BATT) Program, which is supported by the U.S. Department of Energy under Contract # DE-AC02-05 CH11231. Neslihan Yuca thanks for the funding provided by The Scientific and Technological Research Council of Turkey (TUBITAK) in Ankara, Turkey. NR 33 TC 18 Z9 18 U1 16 U2 179 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JAN 14 PY 2015 VL 7 IS 1 BP 862 EP 866 DI 10.1021/am507376f PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA AZ2TM UT WOS:000348085200102 PM 25496355 ER PT J AU Chen, G Zakharov, LN Bowden, ME Karkamkar, AJ Whittemore, SM Garner, EB Mikulas, TC Dixon, DA Autrey, T Liu, SY AF Chen, Gang Zakharov, Lev N. Bowden, Mark E. Karkamkar, Abhijeet J. Whittemore, Sean M. Garner, Edward B., III Mikulas, Tanya C. Dixon, David A. Autrey, Tom Liu, Shih-Yuan TI Bis-BN Cyclohexane: A Remarkably Kinetically Stable Chemical Hydrogen Storage Material SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID AMMONIA-BORANE; THERMAL-DECOMPOSITION; BORON; VEHICLES; DENSITY; ENERGY; DEHYDROGENATION; CATALYSIS; PROGRESS AB A critical component for the successful development of fuel cell applications is hydrogen storage. For back-up power applications, where long storage periods under extreme temperatures are expected, the thermal stability of the storage material is particularly important. Here, we describe the development of an unusually kinetically stable chemical hydrogen storage material with a H-2 storage capacity of 4.7 wt%. The compound, which is the first reported parental BN isostere of cyclohexane featuring two BN units, is thermally stable up to 150 degrees C both in solution and as a neat material. Yet, it can be activated to rapidly desorb H-2 at room temperature in the presence of a catalyst without releasing other detectable volatile contaminants. We also disclose the isolation and characterization of two cage compounds with S-4 symmetry from the H-2 desorption reactions. C1 [Chen, Gang; Liu, Shih-Yuan] Boston Coll, Dept Chem, Chestnut Hill, MA 02467 USA. [Chen, Gang; Zakharov, Lev N.; Liu, Shih-Yuan] Univ Oregon, Dept Chem & Biochem, Eugene, OR 97403 USA. [Bowden, Mark E.; Karkamkar, Abhijeet J.; Whittemore, Sean M.; Autrey, Tom] Pacific NW Natl Lab, Richland, WA 99353 USA. [Garner, Edward B., III; Mikulas, Tanya C.; Dixon, David A.] Univ Alabama, Dept Chem, Tuscaloosa, AL 35487 USA. RP Liu, SY (reprint author), Boston Coll, Dept Chem, Chestnut Hill, MA 02467 USA. EM shihyuan.liu@bc.edu RI Liu, Shih-Yuan/J-7813-2012 OI Liu, Shih-Yuan/0000-0003-3148-9147 FU U.S. Department of Energy [DE-EE-0005658]; NSF [CHE-0923589]; University of Alabama FX S.-Y.L, T.A., and D.A.D. thank the U.S. Department of Energy (DE-EE-0005658) for financial support. Pacific Northwest National Laboratory is operated by Battelle. Funding for the University of Oregon Chemistry Research and Instrumentation Services has been furnished in part by the NSF (CHE-0923589). D.A.D. thanks the Robert Ramsay Chair Fund of The University of Alabama for support. G.C. thanks Dr. Senmiao Xu and Gabriel J. Lovinger for helpful discussions. NR 46 TC 17 Z9 17 U1 3 U2 61 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 14 PY 2015 VL 137 IS 1 BP 134 EP 137 DI 10.1021/ja511766p PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA AZ8RY UT WOS:000348483500034 PM 25494531 ER PT J AU Lassalle-Kaiser, B Merki, D Vrubel, H Gul, S Yachandra, VK Hu, XL Yano, J AF Lassalle-Kaiser, Benedikt Merki, Daniel Vrubel, Heron Gul, Sheraz Yachandra, Vittal K. Hu, Xile Yano, Junko TI Evidence from in Situ X-ray Absorption Spectroscopy for the Involvement of Terminal Disulfide in the Reduction of Protons by an Amorphous Molybdenum Sulfide Electrocatalyst SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID HYDROGEN EVOLUTION REACTION; INCOMPLETE CUBANE-TYPE; ACTIVE EDGE SITES; CATALYST; MOS2; EXAFS; NANOPARTICLES; ENERGY; WATER; GENERATION AB The reduction of protons into dihydrogen is important because of its potential use in a wide range of energy applications. The preparation of efficient and cheap catalysts for this reaction is one of the issues that need to be tackled to allow the widespread use of hydrogen as an energy carrier. In this paper, we report the study of an amorphous molybdenum sulfide (MoSx) proton reducing electrocatalyst under functional conditions, using in situ X-ray absorption spectroscopy. We probed the local and electronic structures of both the molybdenum and sulfur elements for the as prepared material as well as the precatalytic and catalytic states. The as prepared material is very similar to MoS3 and remains unmodified under functional conditions (pH = 2 aqueous HNO3) in the precatalytic state (+0.3 V vs RHE). In its catalytic state (-0.3 V vs RHE), the film is reduced to an amorphous form of MoS2 and shows spectroscopic features that indicate the presence of terminal disulfide units. These units are formed concomitantly with the release of hydrogen, and we suggest that the rate-limiting step of the HER is the reduction and protonation of these disulfide units. These results show the implication of terminal disulfide chemical motifs into HER driven by transition-metal sulfides and provide insight into their reaction mechanism. C1 [Lassalle-Kaiser, Benedikt; Gul, Sheraz; Yachandra, Vittal K.; Yano, Junko] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Lassalle-Kaiser, Benedikt] Synchrotron SOLEIL, F-91191 Gif Sur Yvette, France. [Merki, Daniel; Vrubel, Heron; Hu, Xile] Ecole Polytech Fed Lausanne, Inst Chem Sci & Engn, Lab Inorgan Synth & Catalysis, EPFL ISIC LSCI, CH-1015 Lausanne, Switzerland. RP Lassalle-Kaiser, B (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. EM benedikt.lassalle@synchrotron-soleil.fr; xile.hu@epfl.ch; jyano@lbl.gov RI hu, xile/A-7687-2010; Vrubel, Heron/E-9081-2016 OI hu, xile/0000-0001-8335-1196; FU DOE Office of Biological and Environmental Research; NIH [P41GM103393]; Office of Science, Office of Basic Energy Sciences (OBES), Division of Chemical Sciences, Geosciences, and Biosciences of the Department of Energy (DOE) [DE-AC02-05CH11231]; European Research Council [257096] FX Dr. Delphine Vantelon of the LUCIA beamline at SOLEIL is greatly acknowledged for the collection of S K-edge and Mo L-edge spectra on reference samples. XAS data collection was carried out at the Stanford Synchrotron Radiation Lightsource (SSRL) beamlines 4-3, operated by Stanford University for the U.S. DOE Office of Science and supported by the DOE Office of Biological and Environmental Research and by the NIH (including P41GM103393). XAS work was funded by the Director, Office of Science, Office of Basic Energy Sciences (OBES), Division of Chemical Sciences, Geosciences, and Biosciences of the Department of Energy (DOE) under contract DE-AC02-05CH11231 (J.Y. and V.K.Y). The work at EPFL is supported by a starting grant from the European Research Council (no. 257096). NR 40 TC 41 Z9 41 U1 25 U2 148 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 14 PY 2015 VL 137 IS 1 BP 314 EP 321 DI 10.1021/ja510328m PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA AZ8RY UT WOS:000348483500059 PM 25427231 ER PT J AU Manna, K Eedugurala, N Sadow, AD AF Manna, Kuntal Eedugurala, Naresh Sadow, Aaron D. TI Zirconium-Catalyzed Desymmetrization of Aminodialkenes and Aminodialkynes through Enantioselective Hydroamination SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID CARBON QUATERNARY STEREOCENTERS; ASYMMETRIC HYDROAMINATION; C-N; CONSTRUCTION; CYCLIZATION; COMPLEXES; TRANSFORMATIONS; BICYCLIZATION; AMINOALKENES; SC(III) AB The catalytic addition of alkenes and amines (hydroamination) typically provides alpha- or beta-amino stereocenters directly through C-N or C-H bond formation. Alternatively, desymmetrization reactions of symmetrical aminodialkenes or aminodialkynes provide access to stereogenic centers with the position controlled by the substrates structure. In the present study of an enantioselective zirconium-catalyzed hydroamination, stereocenters resulting from C-N bond formation and desymmetrization of a prochiral quaternary center are independently controlled by the catalyst and reaction conditions. Using a single catalyst, the method provides selective access to either diastereomer of optically enriched five-, six-, and seven-membered cyclic amines from aminodialkenes and enantioselective synthesis of five-, six-, and seven-membered cyclic imines from aminodialkynes. Experiments on hydroamination of aminodialkenes testing the effects of the catalyst:substrate ratio, the absolute concentration of the catalyst, and the absolute initial concentration of the primary amine substrate show that the latter parameter strongly influences the stereoselectivity of the desymmetrization process, whereas the absolute configuration of the a-amino stereocenter generated by C-N bond formation is not affected by these parameters. Interestingly, isotopic substitution (H2NR vs D2NR) of the substrate enhances the stereoselectivity of the enantioselective and diastereoselective processes in aminodialkene cyclization and the peripheral stereocenter in aminodialkyne desymmetrization/cyclization. C1 [Sadow, Aaron D.] US DOE, Ames Lab, Ames, IA 50011 USA. Iowa State Univ, Dept Chem, Ames, IA 50011 USA. RP Sadow, AD (reprint author), US DOE, Ames Lab, 1605 Gilman Hall, Ames, IA 50011 USA. EM sadow@iastate.edu FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences through the Ames Laboratory [DE-AC02-07CH11358] FX This research was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences through the Ames Laboratory (contract no. DE-AC02-07CH11358). Prof. M. Jeffries-EL is thanked for generous access to an HPLC. NR 37 TC 12 Z9 12 U1 1 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 14 PY 2015 VL 137 IS 1 BP 425 EP 435 DI 10.1021/ja511250m PG 11 WC Chemistry, Multidisciplinary SC Chemistry GA AZ8RY UT WOS:000348483500072 PM 25560913 ER PT J AU Schimpf, AM Lounis, SD Runnerstrom, EL Milliron, DJ Gamelin, DR AF Schimpf, Alina M. Lounis, Sebastien D. Runnerstrom, Evan L. Milliron, Delia J. Gamelin, Daniel R. TI Redox Chemistries and Plasmon Energies of Photodoped In2O3 and Sn-Doped In2O3 (ITO) Nanocrystals SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID COLLOIDAL SEMICONDUCTOR NANOCRYSTALS; TUNABLE INFRARED-ABSORPTION; METAL-OXIDE NANOCRYSTALS; ZNO QUANTUM DOTS; OPTICAL-PROPERTIES; ZINC-OXIDE; CDSE NANOCRYSTALS; SIZE DEPENDENCE; EXTRA ELECTRONS; RESONANCES AB Plasmonic doped semiconductor nanocrystals promise exciting opportunities for new technologies, but basic features of the relationships between their structures, compositions, electronic structures, and optical properties remain poorly understood. Here, we report a quantitative assessment of the impact of composition on the energies of localized surface plasmon resonances (LSPRs) in colloidal tin-doped indium oxide (Sn:In2O3, or ITO) nanocrystals. Using a combination of aliovalent doping and photodoping, the effects of added electrons and impurity ions on the energies of LSPRs in colloidal In2O3 and ITO nanocrystals have been evaluated. Photodoping allows electron densities to be tuned post-synthetically in ITO nanocrystals, independent of their Sn content. Because electrons added photochemically are easily titrated, photodoping also allows independent quantitative determination of the dependence of the LSPR energy on nanocrystal composition and changes in electron density. The data show that ITO LSPR energies are affected by both electron and Sn concentrations, with composition yielding a broader plasmon tuning range than achievable by tuning carrier densities alone. Aspects of the photodoping energetics, as well as magneto-optical properties of these ITO LSPRs, are also discussed. C1 [Schimpf, Alina M.; Gamelin, Daniel R.] Univ Washington, Dept Chem, Seattle, WA 98195 USA. [Lounis, Sebastien D.] Univ Calif Berkeley, Grad Grp Appl Sci & Technol, Berkeley, CA 94720 USA. [Runnerstrom, Evan L.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Lounis, Sebastien D.; Runnerstrom, Evan L.; Milliron, Delia J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Runnerstrom, Evan L.; Milliron, Delia J.] Univ Texas Austin, McKetta Dept Chem Engn, Austin, TX 78712 USA. RP Milliron, DJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. EM milliron@che.utexas.edu; gamelin@chem.washington.edu RI Milliron, Delia/D-6002-2012; Foundry, Molecular/G-9968-2014 FU U.S. National Science Foundation [CHE-1151726, DGE-1256082]; U.S. Department of Energy (ARPA-E); Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; Welch Foundation [F-1848]; University of Washington Clean Energy Institute FX The authors thank Gerard M. Carroll for valuable discussions. This research was supported by the U.S. National Science Foundation (CHE-1151726 to D.R.G. and Graduate Research Fellowship DGE-1256082 to A.M.S.) and by the U.S. Department of Energy (ARPA-E to D.J.M.). Some of this research was carried out at the Molecular Foundry, Lawrence Berkeley National Laboratory, a user facility supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. D.J.M. acknowledges support of the Welch Foundation (F-1848). The authors gratefully acknowledge additional support from the University of Washington Clean Energy Institute. NR 59 TC 22 Z9 22 U1 19 U2 85 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JAN 14 PY 2015 VL 137 IS 1 BP 518 EP 524 DI 10.1021/ja5116953 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA AZ8RY UT WOS:000348483500083 PM 25490191 ER PT J AU Casali, N Vignati, M Beeman, JW Bellini, F Cardani, L Dafinei, I Di Domizio, S Ferroni, F Gironi, L Nagorny, S Orio, F Pattavina, L Pessina, G Piperno, G Pirro, S Rusconi, C Schaffner, K Tomei, C AF Casali, N. Vignati, M. Beeman, J. W. Bellini, F. Cardani, L. Dafinei, I. Di Domizio, S. Ferroni, F. Gironi, L. Nagorny, S. Orio, F. Pattavina, L. Pessina, G. Piperno, G. Pirro, S. Rusconi, C. Schaeffner, K. Tomei, C. TI TeO2 bolometers with Cherenkov signal tagging: towards next-generation neutrinoless double-beta decay experiments SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID LIGHT DETECTORS; CRYSTAL; SEARCHES; CUORE; GE AB CUORE, an array of 988 TeO2 bolometers, is about to be one of the most sensitive experiments searching for neutrinoless double-beta decay. Its sensitivity could be further improved by removing the background from a radioactivity. A few years ago it was pointed out that the signal from beta s can be tagged by detecting the emitted Cherenkov light, which is not produced by alpha s. In this paper we confirm this possibility. For the first time we measured the Cherenkov light emitted by a CUORE crystal, and found it to be 100 eV at the Q-value of the decay. To completely reject the alpha background, we compute that one needs light detectors with baseline noise below 20 eV RMS, a value which is 3-4 times smaller than the average noise of the bolometric light detectors we are using. We point out that an improved light detector technology must be developed to obtain TeO2 bolometric experiments able to probe the inverted hierarchy of neutrino masses. C1 [Casali, N.; Pattavina, L.; Pirro, S.; Schaeffner, K.] Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, I-67010 Assergi, AQ, Italy. [Casali, N.] Univ Aquila, Dipartimento Sci Fis & Chim, I-67100 Coppito, AQ, Italy. [Vignati, M.; Bellini, F.; Cardani, L.; Ferroni, F.; Piperno, G.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Vignati, M.; Bellini, F.; Cardani, L.; Dafinei, I.; Ferroni, F.; Orio, F.; Piperno, G.; Tomei, C.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Beeman, J. W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Di Domizio, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Di Domizio, S.] Univ Genoa, Dipartimento Fis, I-16146 Genoa, Italy. [Gironi, L.; Pessina, G.; Rusconi, C.] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20126 Milan, Italy. [Gironi, L.] Univ Milano Bicocca, Dipartimento Fis, I-20126 Milan, Italy. [Nagorny, S.] Ist Nazl Fis Nucl, Gran Sasso Sci Inst, I-67100 Laquila, Italy. RP Casali, N (reprint author), Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, I-67010 Assergi, AQ, Italy. EM marco.vignati@roma1.infn.it RI Di Domizio, Sergio/L-6378-2014; Bellini, Fabio/D-1055-2009; Vignati, Marco/H-1684-2013; Gironi, Luca/P-2860-2016; Pattavina, Luca/I-7498-2015; Casali, Nicola/C-9475-2017 OI Di Domizio, Sergio/0000-0003-2863-5895; Bellini, Fabio/0000-0002-2936-660X; Vignati, Marco/0000-0002-8945-1128; Gironi, Luca/0000-0003-2019-0967; Pattavina, Luca/0000-0003-4192-849X; Casali, Nicola/0000-0003-3669-8247 FU European Research Council under contract LUCIFER [247115]; Italian Ministry of Research [2010ZXAZK9] FX The authors thank the CUORE collaboration for providing the TeO2 crystal. This work was supported by the European Research Council (FP7/2007-2013) under contract LUCIFER no. 247115 and by the Italian Ministry of Research under the PRIN 2010-2011 contract no. 2010ZXAZK9. NR 25 TC 17 Z9 17 U1 1 U2 8 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JAN 14 PY 2015 VL 75 IS 1 AR UNSP 12 DI 10.1140/epjc/s10052-014-3225-4 PG 5 WC Physics, Particles & Fields SC Physics GA CA6AV UT WOS:000348991600010 ER PT J AU Lee, S Alexoff, DL Shea, C Kim, D Schueller, M Fowler, JS Qu, WC AF Lee, Sojeong Alexoff, David L. Shea, Colleen Kim, Dohyun Schueller, Michael Fowler, Joanna S. Qu, Wenchao TI Tetraethylene glycol promoted two-step, one-pot rapid synthesis of indole-3[1-C-11]acetic acid SO TETRAHEDRON LETTERS LA English DT Article DE Carbon-11 labeled indole-3-acetic acid; Nucleophilic [C-11]cyanation; Tetraethylene glycol; Two-step one-pot ID GROWTH; CARBON; RADIOSYNTHESIS; BIOSYNTHESIS; JASMONATE; C-11 AB An operationally friendly, two-step, one-pot process has been developed for the rapid synthesis of carbon-11 labeled indole-3-acetic acid ([C-11]IAA or [C-11]auxin). By replacing an aprotic polar solvent with tetraethylene glycol, nucleophilic [C-11]cyanation and alkaline hydrolysis reactions were performed consecutively in a single pot without a time-consuming intermediate purification step. The entire production time for this updated procedure is 55 mm, which dramatically simplifies the entire synthesis and reduces the starting radioactivity required for a whole plant imaging study. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Lee, Sojeong; Alexoff, David L.; Shea, Colleen; Kim, Dohyun; Schueller, Michael; Fowler, Joanna S.; Qu, Wenchao] Brookhaven Natl Lab, Biol Environm & Climate Sci Dept, Upton, NY 11973 USA. [Lee, Sojeong] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. RP Qu, WC (reprint author), Brookhaven Natl Lab, Biol Environm & Climate Sci Dept, Upton, NY 11973 USA. EM wqu@bnl.gov FU U. S. Department of Energy, Office of Biological and Environmental Research within the Office of Science [DE-AC02-98CH10886] FX This manuscript has been co-authored by employees of Brookhaven Science Associates, LLC under Contract DE-AC02-98CH10886 with the U. S. Department of Energy, Office of Biological and Environmental Research within the Office of Science. We thank David Schlyer and Richard Ferrieri for advice and encouragement. NR 16 TC 2 Z9 2 U1 1 U2 4 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0040-4039 J9 TETRAHEDRON LETT JI Tetrahedron Lett. PD JAN 14 PY 2015 VL 56 IS 3 BP 517 EP 520 DI 10.1016/j.tetlet.2014.12.014 PG 4 WC Chemistry, Organic SC Chemistry GA AZ2ST UT WOS:000348083400008 ER PT J AU Deng, SHM Kong, XY Wang, XB AF Deng, S. H. M. Kong, Xiang-Yu Wang, Xue-Bin TI Probing the early stages of salt nucleation-Experimental and theoretical investigations of sodium/potassium thiocyanate cluster anions SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID SODIUM-CHLORIDE CLUSTERS; PHOTOELECTRON-SPECTROSCOPY; EXCESS ELECTRONS; CRYSTALLIZATION PROCESSES; CRYSTAL-GROWTH; DENSITY; PHOTODETACHMENT; SUPERHALOGENS; LOCALIZATION; IONIZATION AB Due to the fast solvent evaporation in electrospray ionization (ESI), the concentration of initially dilute electrolyte solutions rapidly increases to afford the formation of supersaturated droplets and generation of various pristine anhydrous salt clusters in the gas phase. The size, composition, and charge distributions of these clusters, in principle, witness the nucleation evolution in solutions. Herein, we report a microscopic study on the initial stage of nucleation and crystallization of sodium/potassium thiocyanate salt solutions simulated in the ESI process. Singly charged M-x(SCN)(x+1)(-), doubly charged M-y(SCN)(y+2)(2-) (M = Na, K), and triply charged K-z(SCN)(z+3)(3-) anion clusters (x, y, and z stand for the number of alkali atoms in the singly, doubly, and triply charged clusters, respectively) were produced via electrospray of the corresponding salt solutions and were characterized by negative ion photoelectron spectroscopy (NIPES). The vertical detachment energies (VDEs) of these sodium/potassium thiocyanate cluster anions were obtained, and theoretical calculations were carried out for the sodium thiocyanate clusters in assisting spectral identification. The measured VDEs of singly charged anions Mx(SCN)(x+1)(-) (M = Na and K) demonstrate that they are superhalogen anions. The existence of doubly charged anions M-y(SCN)(y+2)(2-) (y = 2x, x >= 4 and 3 for M = Na and K, respectively) and triply charged anions K-z(SCN)(z+3)(3-) (z = 3x, x >= 6) was initially discovered from the photoelectron spectra for those singly charged anions of M-x(SCN)(x+1)(-) with the same mass-to-charge ratio (m/z), and later independently confirmed by the observation of their distinct mass spectral distributions and by taking their NIPE spectra for those pure multiply charged anions with their m/z different from the singly charged species. For large clusters, multiply charged clusters were found to become preferred, but at higher temperatures, those multiply charged clusters were suppressed. The series of anion clusters investigated here range from molecular-like M-1(SCN)(2)(-) to nano-sized K-22(SCN)(25)(3-), providing a vivid molecular-level growth pattern reflecting the initial salt nucleation process. (C) 2015 AIP Publishing LLC. C1 [Deng, S. H. M.; Kong, Xiang-Yu; Wang, Xue-Bin] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP Wang, XB (reprint author), Pacific NW Natl Lab, Div Phys Sci, 902 Battelle Blvd,POB 999,MS K8-88, Richland, WA 99352 USA. EM xuebin.wang@pnnl.gov FU U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences; DOE's Office of Biological and Environmental Research FX This work was supported by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences (X.B.W.), and performed using EMSL, a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory, which is a multiprogram national laboratory operated for DOE by Battelle. The theoretical calculations were conducted on the ScGrid and Deepcomp7000 of the Supercomputing Center, Computer Network Information Center of the Chinese Academy of Sciences. NR 46 TC 1 Z9 1 U1 4 U2 25 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JAN 14 PY 2015 VL 142 IS 2 AR 024313 DI 10.1063/1.4905266 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AZ3LS UT WOS:000348129700030 PM 25591359 ER PT J AU Small, DW Sundstrom, EJ Head-Gordon, M AF Small, David W. Sundstrom, Eric J. Head-Gordon, Martin TI Restricted Hartree Fock using complex-valued orbitals: A long-known but neglected tool in electronic structure theory SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID DENSITY-FUNCTIONAL THEORY; COUPLED-CLUSTER THEORY; CONFIGURATION-INTERACTION METHOD; INTRINSIC REACTION COORDINATE; MATRIX RENORMALIZATION-GROUP; QUADRUPLY EXCITED CLUSTERS; INNER-PROJECTION TECHNIQUE; TRANSITION-METAL COMPOUNDS; GEMINAL MODEL CHEMISTRY; AB-INITIO CALCULATION AB Restricted Hartree Fock using complex-valued orbitals (cRHF) is studied. We introduce an orbital pairing theorem, with which we obtain a concise connection between cRHF and real-valued RHF, and use it to uncover the close relationship between cRHF, unrestricted Hartree Fock, and generalized valence bond perfect pairing. This enables an intuition for cRHF, contrasting with the generally unintuitive nature of complex orbitals. We also describe an efficient computer implementation of cRHF and its corresponding stability analysis. By applying cRHF to the Be + H-2 insertion reaction, a Woodward-Hoffmann violating reaction, and a symmetry-driven conical intersection, we demonstrate in genuine molecular systems that cRHF is capable of removing certain potential energy surface singularities that plague real-valued RHF and related methods. This complements earlier work that showed this capability in a model system. We also describe how cRHF is the preferred RHF method for certain radicaloid systems like singlet oxygen and antiaromatic molecules. For singlet O-2, we show that standard methods fail even at the equilibrium geometry. An implication of this work is that, regardless of their individual efficacies, cRHF solutions to the HF equations are fairly commonplace. (C) 2015 AIP Publishing LLC. C1 [Small, David W.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Small, DW (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. M.H.-G. is a part-owner of Q-CHEM, Inc. NR 200 TC 6 Z9 6 U1 6 U2 38 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JAN 14 PY 2015 VL 142 IS 2 AR 024104 DI 10.1063/1.4905120 PG 18 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA AZ3LS UT WOS:000348129700006 PM 25591335 ER EF