FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Lu, WC Wang, CZ Zhao, LZ Qin, W Ho, KM AF Lu, Wen-Cai Wang, C. Z. Zhao, Li-Zhen Qin, Wei Ho, K. M. TI Three-center tight-binding potential model for C and Si SO PHYSICAL REVIEW B LA English DT Article ID INITIO MOLECULAR-DYNAMICS; DENSITY-FUNCTIONAL THEORY; TOTAL-ENERGY CALCULATIONS; ELECTRON-SPIN-RESONANCE; WAVE BASIS-SET; CARBON; SILICON; C-6; SIMULATIONS; GERMANIUM AB A tight-binding potential model which goes beyond the Slater-Koster two-center approximation and includes explicit three-center and crystal field expressions is presented. Using carbon and silicon as examples, we show that various bulk structures, surface reconstructions, and the structures of clusters and liquids of C and Si can be well described by the present three-center tight-binding model. These results demonstrate that three-center interaction and crystal field effect are very important for improving the transferability of tight-binding models in describing the structures and properties of materials over a broad range of bonding configurations. C1 [Lu, Wen-Cai; Zhao, Li-Zhen; Qin, Wei] Qingdao Univ, Coll Phys, Qingdao 266071, Shandong, Peoples R China. [Lu, Wen-Cai; Zhao, Li-Zhen; Qin, Wei] Qingdao Univ, Lab Fiber Mat & Modern Text, Growing Base State Key Lab, Qingdao 266071, Shandong, Peoples R China. [Wang, C. Z.; Ho, K. M.] Iowa State Univ, Ames Lab US DOE, Ames, IA 50011 USA. [Wang, C. Z.; Ho, K. M.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Lu, WC (reprint author), Qingdao Univ, Coll Phys, Qingdao 266071, Shandong, Peoples R China. EM wencailu@jlu.edu.cn; wangcz@ameslab.gov FU US Department of Energy [DE-AC02-07CH11358]; Director for Energy Research, Office of Basic Energy Sciences, Division of Material Science and Engineering; National Natural Science Foundation of China [21273122, 21203105]; China Postdoctoral Science Foundation [2014M561885] FX Ames Laboratory is operated for the US Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. Work at Ames Laboratory was supported by the Director for Energy Research, Office of Basic Energy Sciences, Division of Material Science and Engineering including a grant for computer time at the National Energy Research Scientific Computing Center (NERSC) in Berkeley, CA. This work is also supported by the National Natural Science Foundation of China (Grant No. 21273122). L.Z. acknowledges the support by the National Natural Science Foundation of China (Grant No. 21203105) and W.Q. acknowledges the support by the China Postdoctoral Science Foundation (Grant No. 2014M561885). NR 45 TC 5 Z9 5 U1 2 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 29 PY 2015 VL 92 IS 3 AR 035206 DI 10.1103/PhysRevB.92.035206 PG 9 WC Physics, Condensed Matter SC Physics GA CO0LT UT WOS:000358843700003 ER PT J AU Vikram, V Chang, C Jain, B Bacon, D Amara, A Becker, MR Bernstein, G Bonnett, C Bridle, S Brout, D Busha, M Frieman, J Gaztanaga, E Hartley, W Jarvis, M Kacprzak, T Kovacs, A Lahav, O Leistedt, B Lin, H Melchior, P Peiris, H Rozo, E Rykoff, E Sanchez, C Sheldon, E Troxel, MA Wechsler, R Zuntz, J Abbott, T Abdalla, FB Armstrong, R Banerji, M Bauer, AH Benoit-Levy, A Bertin, E Brooks, D Buckley-Geer, E Burke, DL Capozzi, D Rosell, AC Kind, MC Castander, FJ Crocce, M Cunha, CE D'Andrea, CB da Costa, LN Depoy, DL Desai, S Diehl, HT Dietrich, JP Estrada, J Evrard, AE Neto, AF Fernandez, E Flaugher, B Fosalba, P Gerdes, D Gruen, D Gruendl, RA Honscheid, K James, D Kent, S Kuehn, K Kuropatkin, N Li, TS Maia, MAG Makler, M March, M Marshall, J Martini, P Merritt, KW Miller, CJ Miquel, R Neilsen, E Nichol, RC Nord, B Ogando, R Plazas, AA Romer, AK Roodman, A Sanchez, E Scarpine, V Sevilla, I Smith, RC Soares-Santos, M Sobreira, F Suchyta, E Swanson, MEC Tarle, G Thaler, J Thomas, D Walker, AR Weller, J AF Vikram, V. Chang, C. Jain, B. Bacon, D. Amara, A. Becker, M. R. Bernstein, G. Bonnett, C. Bridle, S. Brout, D. Busha, M. Frieman, J. Gaztanaga, E. Hartley, W. Jarvis, M. Kacprzak, T. Kovacs, A. Lahav, O. Leistedt, B. Lin, H. Melchior, P. Peiris, H. Rozo, E. Rykoff, E. Sanchez, C. Sheldon, E. Troxel, M. A. Wechsler, R. Zuntz, J. Abbott, T. Abdalla, F. B. Armstrong, R. Banerji, M. Bauer, A. H. Benoit-Levy, A. Bertin, E. Brooks, D. Buckley-Geer, E. Burke, D. L. Capozzi, D. Carnero Rosell, A. Kind, M. Carrasco Castander, F. J. Crocce, M. Cunha, C. E. D'Andrea, C. B. da Costa, L. N. Depoy, D. L. Desai, S. Diehl, H. T. Dietrich, J. P. Estrada, J. Evrard, A. E. Fausti Neto, A. Fernandez, E. Flaugher, B. Fosalba, P. Gerdes, D. Gruen, D. Gruendl, R. A. Honscheid, K. James, D. Kent, S. Kuehn, K. Kuropatkin, N. Li, T. S. Maia, M. A. G. Makler, M. March, M. Marshall, J. Martini, P. Merritt, K. W. Miller, C. J. Miquel, R. Neilsen, E. Nichol, R. C. Nord, B. Ogando, R. Plazas, A. A. Romer, A. K. Roodman, A. Sanchez, E. Scarpine, V. Sevilla, I. Smith, R. C. Soares-Santos, M. Sobreira, F. Suchyta, E. Swanson, M. E. C. Tarle, G. Thaler, J. Thomas, D. Walker, A. R. Weller, J. TI Wide-field lensing mass maps from Dark Energy Survey science verification data: Methodology and detailed analysis SO PHYSICAL REVIEW D LA English DT Article ID MAXIMUM-LIKELIHOOD; SHEAR MEASUREMENT; GALAXY DISTRIBUTIONS; PEAK STATISTICS; CLUSTER SURVEYS; DATA RELEASE; NOISE BIAS; SDSS-III; WEAK; CONSTRAINTS AB Weak gravitational lensing allows one to reconstruct the spatial distribution of the projected mass density across the sky. These "mass maps" provide a powerful tool for studying cosmology as they probe both luminous and dark matter. In this paper, we present a weak lensing mass map reconstructed from shear measurements in a 139 deg(2) area from the Dark Energy Survey (DES) science verification data. We compare the distribution of mass with that of the foreground distribution of galaxies and clusters. The overdensities in the reconstructed map correlate well with the distribution of optically detected clusters. We demonstrate that candidate superclusters and voids along the line of sight can be identified, exploiting the tight scatter of the cluster photometric redshifts. We cross-correlate the mass map with a foreground magnitude-limited galaxy sample from the same data. Our measurement gives results consistent with mock catalogs from N-body simulations that include the primary sources of statistical uncertainties in the galaxy, lensing, and photo-z catalogs. The statistical significance of the cross-correlation is at the 6.8 sigma level with 20 arcminute smoothing. We find that the contribution of systematics to the lensing mass maps is generally within measurement uncertainties. In this work, we analyze less than 3% of the final area that will be mapped by the DES; the tools and analysis techniques developed in this paper can be applied to forthcoming larger data sets from the survey. C1 [Vikram, V.] Argonne Natl Lab, Lemont, IL 60439 USA. [Vikram, V.; Jain, B.; Bernstein, G.; Brout, D.; Jarvis, M.; Armstrong, R.; March, M.] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. [Chang, C.; Amara, A.; Hartley, W.; Kacprzak, T.] Swiss Fed Inst Technol, Dept Phys, CH-8093 Zurich, Switzerland. [Bacon, D.; Capozzi, D.; D'Andrea, C. B.; Nichol, R. C.; Thomas, D.] Univ Portsmouth, Inst Cosmol & Gravitat, Portsmouth PO1 3FX, Hants, England. [Becker, M. R.; Busha, M.; Wechsler, R.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Becker, M. R.; Busha, M.; Rykoff, E.; Wechsler, R.; Burke, D. L.; Roodman, A.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, Stanford, CA 94305 USA. [Bonnett, C.; Kovacs, A.; Sanchez, C.; Fernandez, E.; Miquel, R.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Bridle, S.; Troxel, M. A.; Zuntz, J.] Univ Manchester, Sch Phys & Astron, Jodrell Bank Ctr Astrophys, Manchester M13 9PL, Lancs, England. [Frieman, J.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Frieman, J.; Lin, H.; Buckley-Geer, E.; Diehl, H. T.; Estrada, J.; Flaugher, B.; Kent, S.; Kuropatkin, N.; Merritt, K. W.; Neilsen, E.; Nord, B.; Scarpine, V.; Soares-Santos, M.; Sobreira, F.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Gaztanaga, E.; Bauer, A. H.; Castander, F. J.; Crocce, M.; Fosalba, P.] IEEC CSIC, Fac Ciencies, Inst Ciencies Espai, Barcelona 08193, Spain. [Lahav, O.; Leistedt, B.; Peiris, H.; Abdalla, F. B.; Benoit-Levy, A.; Brooks, D.] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Melchior, P.; Martini, P.; Suchyta, E.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Melchior, P.; Martini, P.; Suchyta, E.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Rozo, E.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Rykoff, E.; Wechsler, R.; Burke, D. L.; Roodman, A.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Sheldon, E.; Plazas, A. A.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Abbott, T.; James, D.; Smith, R. C.; Walker, A. R.] Natl Opt Astron Observ, Cerro Tololo Inter Amer Observ, La Serena, Chile. [Banerji, M.] Univ Cambridge, Inst Astron, Cambridge CB3 0HA, England. [Banerji, M.] Univ Cambridge, Kavli Inst Cosmol, Cambridge CB3 0HA, England. [Bertin, E.] Univ Paris 06, Inst Astrophys Paris, F-75014 Paris, France. [Bertin, E.] CNRS UMR7095, F-75014 Paris, France. [Carnero Rosell, A.; da Costa, L. N.; Fausti Neto, A.; Maia, M. A. G.; Ogando, R.; Sobreira, F.] Lab Interinst E Astron LIneA, BR-20921400 Rio De Janeiro, RJ, Brazil. [Carnero Rosell, A.; da Costa, L. N.; Maia, M. A. G.; Ogando, R.] Observ Nacl, BR-20921400 Rio De Janeiro, RJ, Brazil. [Kind, M. Carrasco; Gruendl, R. A.; Honscheid, K.; Sevilla, I.; Thaler, J.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kind, M. Carrasco; Gruendl, R. A.; Honscheid, K.; Swanson, M. E. C.] Univ Illinois, Natl Ctr Supercomp Applicat, Urbana, IL 61801 USA. [Cunha, C. E.] Robert Bosch LLC, Palo Alto, CA 94304 USA. [Depoy, D. L.; Li, T. S.; Marshall, J.] Texas A&M Univ, George P & Cynthia Woods Mitchell Inst Fundamenta, College Stn, TX 77843 USA. [Depoy, D. L.; Li, T. S.; Marshall, J.] Texas A&M Univ, Dept Phys & Astron, College Stn, TX 77843 USA. [Desai, S.; Dietrich, J. P.; Tarle, G.; Weller, J.] Univ Munich, Dept Phys, D-81679 Munich, Germany. [Dietrich, J. P.; Weller, J.] Excellence Cluster Universe, D-85748 Garching, Germany. [Evrard, A. E.; Gerdes, D.; Miller, C. J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Gruen, D.; Weller, J.] Max Planck Inst Extraterr Phys, D-85748 Garching, Germany. [Gruen, D.] Univ Observ Munich, D-81679 Munich, Germany. [Kuehn, K.] Australian Astron Observ, N Ryde, NSW 2113, Australia. [Makler, M.] Ctr Brasileiro Pesquisas Fis, ICRA, BR-22290180 Rio De Janeiro, RJ, Brazil. [Miller, C. J.] Univ Michigan, Dept Astron, Ann Arbor, MI 48109 USA. [Miquel, R.] Inst Catalana Recerca & Estudis Avancats, E-08010 Barcelona, Spain. [Plazas, A. A.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Romer, A. K.] Univ Sussex, Dept Phys & Astron, Brighton BN1 9QH, E Sussex, England. [Sanchez, E.; Sevilla, I.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid 28040, Spain. [Thomas, D.] South East Phys Network, SEPnet, Southampton SO17 1BJ, Hants, England. RP Chang, C (reprint author), Swiss Fed Inst Technol, Dept Phys, Wolfgang Pauli Str 16, CH-8093 Zurich, Switzerland. EM chihway.chang@phys.ethz.ch RI Ogando, Ricardo/A-1747-2010; Makler, Martin/G-2639-2012; Sanchez, Eusebio/H-5228-2015; Fosalba Vela, Pablo/I-5515-2016; Sobreira, Flavia/F-4168-2015; Fernandez, Enrique/L-5387-2014; Gaztanaga, Enrique/L-4894-2014; OI Suchyta, Eric/0000-0002-7047-9358; Ogando, Ricardo/0000-0003-2120-1154; Dietrich, Jorg/0000-0002-8134-9591; Makler, Martin/0000-0003-2206-2651; Weller, Jochen/0000-0002-8282-2010; Carrasco Kind, Matias/0000-0002-4802-3194; Sanchez, Eusebio/0000-0002-9646-8198; Sobreira, Flavia/0000-0002-7822-0658; Fernandez, Enrique/0000-0002-6405-9488; Gaztanaga, Enrique/0000-0001-9632-0815; Becker, Matthew/0000-0001-7774-2246; Banerji, Manda/0000-0002-0639-5141; Abdalla, Filipe/0000-0003-2063-4345 FU Swiss National Science Foundation [200021-149442, 200021-143906]; European Research Council [240672]; Deutsche Forschungsgemeinschaft (DFG) [SFB-Transregio 33]; DFG cluster of excellence "Origin and Structure of the Universe"; CAPES [3171-13-2]; European Research Council Advanced Grant [FP7/291329]; U.S. Department of Energy; U.S. National Science Foundation; Ministry of Science and Education of Spain; Science and Technology Facilities Council of the United Kingdom; Higher Education Funding Council for England; National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign; Kavli Institute of Cosmological Physics at the University of Chicago; Center for Cosmology and Astro-Particle Physics at the Ohio State University; Mitchell Institute for Fundamental Physics and Astronomy at Texas AM University; Financiadora de Estudos e Projetos; Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico; Ministerio da Ciencia e Tecnologia; Deutsche Forschungsgemeinschaft; National Science Foundation [AST-1138766]; MINECO [AYA2012-39559, ESP2013-48274, FPA2013-47986]; Centro de Excelencia Severo Ochoa [SEV-2012-0234]; European Union; Argonne National Laboratory; University of California at Santa Cruz; University of Cambridge; Centro de Investigaciones Energeticas; Medioambientales y Tecnologicas-Madrid; University of Chicago; University College London; DES-Brazil Consortium; Eidgenossische Technische Hochschule (ETH) Zurich; Fermi National Accelerator Laboratory; University of Edinburgh; University of Illinois at Urbana-Champaign; Institut de Ciencies de l'Espai (IEEC/CSIC); Institut de Fisica d'Altes Energies; Lawrence Berkeley National Laboratory; Ludwig-Maximilians Universitat; associated Excellence Cluster Universe; University of Michigan; National Optical Astronomy Observatory; University of Nottingham; Ohio State University; University of Pennsylvania; University of Portsmouth; SLAC National Accelerator Laboratory; Stanford University; University of Sussex; Texas AM University FX We are grateful for the extraordinary contributions of our CTIO colleagues and the DECam Construction, Commissioning and science verification teams in achieving the excellent instrument and telescope conditions that have made this work possible. The success of this project also relies critically on the expertise and dedication of the DES Data Management group. We thank Jake VanderPlas, Andy Connolly, Phil Marshall, Ludo van Waerbeke, and Rafal Szepietowski for discussions and collaborative work on mass mapping methodology. C. C and A. A. are supported by the Swiss National Science Foundation Grants No. 200021-149442 and No. 200021-143906. S. B. and J. Z. acknowledge support from European Research Council Starting Grant No. 240672. D. G. was supported by SFB-Transregio 33 "The Dark Universe" by the Deutsche Forschungsgemeinschaft (DFG) and the DFG cluster of excellence "Origin and Structure of the Universe." F. S. acknowledges financial support provided by CAPES under Contract No. 3171-13-2. O. L. acknowledges support from a European Research Council Advanced Grant No. FP7/291329. Funding for the DES Projects has been provided by the U.S. Department of Energy, the U.S. National Science Foundation, the Ministry of Science and Education of Spain, the Science and Technology Facilities Council of the United Kingdom, the Higher Education Funding Council for England, the National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign, the Kavli Institute of Cosmological Physics at the University of Chicago, the Center for Cosmology and Astro-Particle Physics at the Ohio State University, the Mitchell Institute for Fundamental Physics and Astronomy at Texas A&M University, Financiadora de Estudos e Projetos, Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro, Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and the Ministerio da Ciencia e Tecnologia, the Deutsche Forschungsgemeinschaft and the collaborating institutions in the Dark Energy Survey. The DES data management system is supported by the National Science Foundation under Grant No. AST-1138766. The DES participants from Spanish institutions are partially supported by MINECO under Grants No. AYA2012-39559, No. ESP2013-48274, No. FPA2013-47986, and Centro de Excelencia Severo Ochoa No. SEV-2012-0234, some of which include ERDF funds from the European Union. The collaborating institutions are Argonne National Laboratory, the University of California at Santa Cruz, the University of Cambridge, Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas-Madrid, the University of Chicago, University College London, the DES-Brazil Consortium, the Eidgenossische Technische Hochschule (ETH) Zurich, Fermi National Accelerator Laboratory, the University of Edinburgh, the University of Illinois at Urbana-Champaign, the Institut de Ciencies de l'Espai (IEEC/CSIC), the Institut de Fisica d'Altes Energies, Lawrence Berkeley National Laboratory, the Ludwig-Maximilians Universitat and the associated Excellence Cluster Universe, the University of Michigan, the National Optical Astronomy Observatory, the University of Nottingham, The Ohio State University, the University of Pennsylvania, the University of Portsmouth, SLAC National Accelerator Laboratory, Stanford University, the University of Sussex, and Texas A&M University. This paper has gone through internal review by the DES Collaboration. NR 93 TC 23 Z9 23 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JUL 29 PY 2015 VL 92 IS 2 AR 022006 DI 10.1103/PhysRevD.92.022006 PG 22 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CO0OZ UT WOS:000358853000001 ER PT J AU Chang, C Vikram, V Jain, B Bacon, D Amara, A Becker, MR Bernstein, G Bonnett, C Bridle, S Brout, D Busha, M Frieman, J Gaztanaga, E Hartley, W Jarvis, M Kacprzak, T Kovacs, A Lahav, O Lin, H Melchior, P Peiris, H Rozo, E Rykoff, E Sanchez, C Sheldon, E Troxel, MA Wechsler, R Zuntz, J Abbott, T Abdalla, FB Allam, S Annis, J Bauer, AH Benoit-Levy, A Brooks, D Buckley-Geer, E Burke, DL Capozzi, D Rosell, AC Kind, MC Castander, FJ Crocce, M D'Andrea, CB Desai, S Diehl, HT Dietrich, JP Doel, P Eifler, TF Evrard, AE Neto, AF Flaugher, B Fosalba, P Gruen, D Gruendl, RA Gutierrez, G Honscheid, K James, D Kent, S Kuehn, K Kuropatkin, N Maia, MAG March, M Martini, P Merritt, KW Miller, CJ Miquel, R Neilsen, E Nichol, RC Ogando, R Plazas, AA Romer, AK Roodman, A Sako, M Sanchez, E Sevilla, I Smith, RC Soares-Santos, M Sobreira, F Suchyta, E Tarle, G Thaler, J Thomas, D Tucker, D Walker, AR AF Chang, C. Vikram, V. Jain, B. Bacon, D. Amara, A. Becker, M. R. Bernstein, G. Bonnett, C. Bridle, S. Brout, D. Busha, M. Frieman, J. Gaztanaga, E. Hartley, W. Jarvis, M. Kacprzak, T. Kovacs, A. Lahav, O. Lin, H. Melchior, P. Peiris, H. Rozo, E. Rykoff, E. Sanchez, C. Sheldon, E. Troxel, M. A. Wechsler, R. Zuntz, J. Abbott, T. Abdalla, F. B. Allam, S. Annis, J. Bauer, A. H. Benoit-Levy, A. Brooks, D. Buckley-Geer, E. Burke, D. L. Capozzi, D. Carnero Rosell, A. Kind, M. Carrasco Castander, F. J. Crocce, M. D'Andrea, C. B. Desai, S. Diehl, H. T. Dietrich, J. P. Doel, P. Eifler, T. F. Evrard, A. E. Fausti Neto, A. Flaugher, B. Fosalba, P. Gruen, D. Gruendl, R. A. Gutierrez, G. Honscheid, K. James, D. Kent, S. Kuehn, K. Kuropatkin, N. Maia, M. A. G. March, M. Martini, P. Merritt, K. W. Miller, C. J. Miquel, R. Neilsen, E. Nichol, R. C. Ogando, R. Plazas, A. A. Romer, A. K. Roodman, A. Sako, M. Sanchez, E. Sevilla, I. Smith, R. C. Soares-Santos, M. Sobreira, F. Suchyta, E. Tarle, G. Thaler, J. Thomas, D. Tucker, D. Walker, A. R. TI Wide-Field Lensing Mass Maps from Dark Energy Survey Science Verification Data SO PHYSICAL REVIEW LETTERS LA English DT Article ID SHEAR MEASUREMENT; DATA RELEASE; MATTER; CONSTRAINTS; CFHTLENS; SIMULATIONS; SEXTRACTOR; STATISTICS; COSMOLOGY; REDSHIFTS AB We present a mass map reconstructed from weak gravitational lensing shear measurements over 139 deg(2) from the Dark Energy Survey science verification data. The mass map probes both luminous and dark matter, thus providing a tool for studying cosmology. We find good agreement between the mass map and the distribution of massive galaxy clusters identified using a red-sequence cluster finder. Potential candidates for superclusters and voids are identified using these maps. We measure the cross-correlation between the mass map and a magnitude-limited foreground galaxy sample and find a detection at the 6.8 sigma level with 20 arc min smoothing. These measurements are consistent with simulated galaxy catalogs based on N-body simulations from a cold dark matter model with a cosmological constant. This suggests low systematics uncertainties in the map. We summarize our key findings in this Letter; the detailed methodology and tests for systematics are presented in a companion paper. C1 [Chang, C.; Amara, A.; Hartley, W.; Kacprzak, T.] ETH, Dept Phys, CH-8093 Zurich, Switzerland. [Vikram, V.] Argonne Natl Lab, Lemont, IL 60439 USA. [Vikram, V.; Jain, B.; Bernstein, G.; Brout, D.; Jarvis, M.; Eifler, T. F.; March, M.; Sako, M.] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. [Bacon, D.; Capozzi, D.; D'Andrea, C. B.; Nichol, R. C.; Thomas, D.] Univ Portsmouth, Inst Cosmol & Gravitat, Portsmouth PO1 3FX, Hants, England. [Becker, M. R.; Busha, M.; Wechsler, R.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Becker, M. R.; Busha, M.; Rykoff, E.; Wechsler, R.; Burke, D. L.; Roodman, A.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, Stanford, CA 94305 USA. [Bonnett, C.; Kovacs, A.; Sanchez, C.; Miquel, R.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Bellaterra, Barcelona, Spain. [Bridle, S.; Troxel, M. A.; Zuntz, J.] Univ Manchester, Sch Phys & Astron, Jodrell Bank Ctr Astrophys, Manchester M13 9PL, Lancs, England. [Frieman, J.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Frieman, J.; Lin, H.; Allam, S.; Annis, J.; Buckley-Geer, E.; Diehl, H. T.; Flaugher, B.; Gutierrez, G.; Kent, S.; Kuropatkin, N.; Merritt, K. W.; Neilsen, E.; Soares-Santos, M.; Sobreira, F.; Tucker, D.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Gaztanaga, E.; Bauer, A. H.; Castander, F. J.; Crocce, M.; Fosalba, P.] CSIC, IEEC, Fac Ciencies, Inst Ciencies Espai, Bellaterra 08193, Barcelona, Spain. [Lahav, O.; Peiris, H.; Abdalla, F. B.; Benoit-Levy, A.; Brooks, D.; Doel, P.] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Melchior, P.; Martini, P.; Suchyta, E.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Melchior, P.; Martini, P.; Suchyta, E.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Rozo, E.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Rykoff, E.; Wechsler, R.; Burke, D. L.; Roodman, A.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Sheldon, E.; Plazas, A. A.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Abbott, T.; James, D.; Smith, R. C.; Walker, A. R.] Natl Opt Astron Observ, Cerro Tololo Interamer Observ, La Serena, Chile. [Carnero Rosell, A.; Fausti Neto, A.; Maia, M. A. G.; Ogando, R.; Sobreira, F.] Lab Interinst E Astron LIneA, BR-20921400 Rio De Janeiro, RJ, Brazil. [Carnero Rosell, A.; Maia, M. A. G.; Ogando, R.] Observat Nacl, BR-20921400 Rio De Janeiro, RJ, Brazil. [Kind, M. Carrasco; Gruendl, R. A.; Honscheid, K.; Sevilla, I.; Thaler, J.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kind, M. Carrasco; Gruendl, R. A.; Honscheid, K.] Univ Illinois, Natl Ctr Supercomp Applicat, Urbana, IL 61801 USA. [Desai, S.; Dietrich, J. P.; Tarle, G.] Univ Munich, Dept Phys, D-81679 Munich, Germany. [Dietrich, J. P.] Excellence Cluster Univ, D-85748 Garching, Germany. [Eifler, T. F.; Plazas, A. A.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Evrard, A. E.; Miller, C. J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Gruen, D.] Max Planck Inst Extraterr Phys, D-85748 Garching, Germany. [Gruen, D.] Univ Observ Munich, D-81679 Munich, Germany. [Kuehn, K.] Australian Astron Observ, N Ryde, NSW 2113, Australia. [Miller, C. J.] Univ Michigan, Dept Astron, Ann Arbor, MI 48109 USA. [Miquel, R.] Inst Catalana Recerca & Estudis Avancats, E-08010 Barcelona, Spain. [Romer, A. K.] Univ Sussex, Dept Phys & Astron, Brighton BN1 9QH, E Sussex, England. [Sanchez, E.; Sevilla, I.] Ctr Invest Energet Medioambient & Tecnol CIEMAT, Madrid 28040, Spain. [Thomas, D.] SEPnet, South East Phys Network, Southampton SO17 1BJ, Hants, England. RP Chang, C (reprint author), ETH, Dept Phys, Wolfgang Pauli Str 16, CH-8093 Zurich, Switzerland. EM chihway.chang@phys.ethz.ch RI Ogando, Ricardo/A-1747-2010; Sanchez, Eusebio/H-5228-2015; Fosalba Vela, Pablo/I-5515-2016; Gaztanaga, Enrique/L-4894-2014; OI Ogando, Ricardo/0000-0003-2120-1154; Tucker, Douglas/0000-0001-7211-5729; Sanchez, Eusebio/0000-0002-9646-8198; Gaztanaga, Enrique/0000-0001-9632-0815; Becker, Matthew/0000-0001-7774-2246; Suchyta, Eric/0000-0002-7047-9358; Dietrich, Jorg/0000-0002-8134-9591; Carrasco Kind, Matias/0000-0002-4802-3194; Abdalla, Filipe/0000-0003-2063-4345; Sobreira, Flavia/0000-0002-7822-0658 FU Swiss National Science Foundation [200021-149442, 200021-143906]; European Research Council Starting Grant [240672]; SFB-Transregio 33 "The Dark Universe", Deutsche Forschungsgemeinschaft (DFG); DFG cluster of excellence "Origin and Structure of the Universe"; CAPES [3171-13-2]; European Research Council Advanced Grant [FP7/291329]; U. S. Department of Energy; U. S. National Science Foundation; Ministry of Science and Education of Spain; Science and Technology Facilities Council of the United Kingdom; Higher Education Funding Council for England; National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign; Kavli Institute of Cosmological Physics at the University of Chicago; Center for Cosmology and Astro-Particle Physics at the Ohio State University; Mitchell Institute for Fundamental Physics and Astronomy at Texas AM University; Financiadora de Estudos e Projetos; Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico; Ministerio da Ciencia e Tecnologia; Deutsche Forschungsgemeinschaft; Collaborating Institutions in the Dark Energy Survey; National Science Foundation [AST-1138766]; MINECO [AYA2012-39559, ESP2013-48274, FPA2013-47986]; Centro de Excelencia Severo Ochoa [SEV-2012-0234]; European Union; Argonne National Laboratory; University of California at Santa Cruz; University of Cambridge; Centro de Investigaciones Energeticas; Medioambientales y Tecnologicas-Madrid; University of Chicago; University College London; DES-Brazil Consortium; Eidgenossische Technische Hochschule (ETH) Zurich; fermi National Accelerator Laboratory; University of Edinburgh; University of Illinois at Urbana-Champaign; Institut de Ciencies de l'Espai (IEEC/CSIC); Institut de Fisica d'Altes Energies; Lawrence Berkeley National Laboratory; Ludwig-Maximilians Universitat; associated Excellence Cluster Universe; University of Michigan; National Optical Astronomy Observatory; University of Nottingham; Ohio State University; University of Pennsylvania; University of Portsmouth; SLAC National Accelerator Laboratory; Stanford University; University of Sussex; Texas AM University FX We are grateful for the extraordinary contributions of our CTIO colleagues and the DECam Construction, Commissioning and Science Verification teams in achieving the excellent instrument and telescope conditions that have made this work possible. The success of this project also relies critically on the expertise and dedication of the DES Data Management group. We thank Jake VanderPlas, Andy Connolly, Phil Marshall, Ludo van Waerbeke, and Rafal Szepietowski for discussions and collaborative work on mass mapping methodology. C. C. and A. A. are supported by the Swiss National Science Foundation Grants No. 200021-149442 and No. 200021-143906. S. B. and J. Z. acknowledge support from a European Research Council Starting Grant No. 240672. D. G. was supported by SFB-Transregio 33 "The Dark Universe" by the Deutsche Forschungsgemeinschaft (DFG) and the DFG cluster of excellence "Origin and Structure of the Universe". F. S. acknowledges financial support provided by CAPES under Contract No. 3171-13-2. O. L. acknowledges support from a European Research Council Advanced Grant No. FP7/291329. Funding for the DES Projects has been provided by the U. S. Department of Energy, the U. S. National Science Foundation, the Ministry of Science and Education of Spain, the Science and Technology Facilities Council of the United Kingdom, the Higher Education Funding Council for England, the National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign, the Kavli Institute of Cosmological Physics at the University of Chicago, the Center for Cosmology and Astro-Particle Physics at the Ohio State University, the Mitchell Institute for Fundamental Physics and Astronomy at Texas A&M University, Financiadora de Estudos e Projetos, Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro, Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and the Ministerio da Ciencia e Tecnologia, the Deutsche Forschungsgemeinschaft, and the Collaborating Institutions in the Dark Energy Survey. The DES data management system is supported by the National Science Foundation under Grant No. AST-1138766. The DES participants from Spanish institutions are partially supported by MINECO under Grants No. AYA2012-39559, No. ESP2013-48274, No. FPA2013-47986, and Centro de Excelencia Severo Ochoa SEV-2012-0234, some of which include ERDF funds from the European Union. The Collaborating Institutions are Argonne National Laboratory, University of California at Santa Cruz, University of Cambridge, Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas-Madrid, University of Chicago, University College London, DES-Brazil Consortium, Eidgenossische Technische Hochschule (ETH) Zurich, fermi National Accelerator Laboratory, University of Edinburgh, University of Illinois at Urbana-Champaign, Institut de Ciencies de l'Espai (IEEC/CSIC), Institut de Fisica d'Altes Energies, Lawrence Berkeley National Laboratory, Ludwig-Maximilians Universitat and the associated Excellence Cluster Universe, University of Michigan, National Optical Astronomy Observatory, University of Nottingham, Ohio State University, University of Pennsylvania, University of Portsmouth, SLAC National Accelerator Laboratory, Stanford University, University of Sussex, and Texas A&M University. This paper has gone through internal review by the DES collaboration. NR 57 TC 18 Z9 18 U1 0 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 29 PY 2015 VL 115 IS 5 AR 051301 DI 10.1103/PhysRevLett.115.051301 PG 8 WC Physics, Multidisciplinary SC Physics GA CO0SO UT WOS:000358862800002 PM 26274409 ER PT J AU Hoffmann, KQ McGovern, M Chiu, CC de Pablo, JJ AF Hoffmann, Kyle Quynn McGovern, Michael Chiu, Chi-cheng de Pablo, Juan J. TI Secondary Structure of Rat and Human Amylin across Force Fields SO PLOS ONE LA English DT Article ID ISLET AMYLOID POLYPEPTIDE; PROTEIN-FOLDING SIMULATIONS; MOLECULAR-DYNAMICS SIMULATIONS; ALPHA-HELICAL STATES; PARTICLE MESH EWALD; DIABETES-MELLITUS; FIBRIL FORMATION; BETA-SHEET; MEMBRANE ENVIRONMENT; NMR-SPECTROSCOPY AB The aggregation of human amylin has been strongly implicated in the progression of Type II diabetes. This 37-residue peptide forms a variety of secondary structures, including random coils, alpha-helices, and beta-hairpins. The balance between these structures depends on the chemical environment, making amylin an ideal candidate to examine inherent biases in force fields. Rat amylin differs from human amylin by only 6 residues; however, it does not form fibrils. Therefore it provides a useful complement to human amylin in studies of the key events along the aggregation pathway. In this work, the free energy of rat and human amylin was determined as a function of alpha-helix and beta-hairpin content for the Gromos96 53a6, OPLS-AA/L, CHARMM22/CMAP, CHARMM22*, Amberff99sb*-ILDN, and Amberff03w force fields using advanced sampling techniques, specifically bias exchange metadynamics. This work represents a first systematic attempt to evaluate the conformations and the corresponding free energy of a large, clinically relevant disordered peptide in solution across force fields. The NMR chemical shifts of rIAPP were calculated for each of the force fields using their respective free energy maps, allowing us to quantitatively assess their predictions. We show that the predicted distribution of secondary structures is sensitive to the choice of force-field: Gromos53a6 is biased towards beta-hairpins, while CHARMM22/CMAP predicts structures that are overly alpha-helical. OPLS-AA/L favors disordered structures. Amberff99sb*-ILDN, AmberFF03w and CHARMM22* provide the balance between secondary structures that is most consistent with available experimental data. In contrast to previous reports, our findings suggest that the equilibrium conformations of human and rat amylin are remarkably similar, but that subtle differences arise in transient alpha-helical and beta-strand containing structures that the human peptide can more readily adopt. We hypothesize that these transient states enable dynamic pathways that facilitate the formation of aggregates and, eventually, amyloid fibrils. C1 [Hoffmann, Kyle Quynn; McGovern, Michael; de Pablo, Juan J.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. [Chiu, Chi-cheng] Natl Cheng Kung Univ, Dept Chem Engn, Tainan 70101, Taiwan. [de Pablo, Juan J.] Argonne Natl Lab, Argonne, IL 60439 USA. RP de Pablo, JJ (reprint author), Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. EM depablo@uchicago.edu FU National Science Foundation, Division of Engineering, Chemical, Bioengineering, Environmental and Thermal Systems [CBET 1264021] FX This work is supported by the National Science Foundation, Division of Engineering, Chemical, Bioengineering, Environmental and Thermal Systems, CBET 1264021. The funder had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 116 TC 5 Z9 5 U1 5 U2 29 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JUL 29 PY 2015 VL 10 IS 7 AR e0134091 DI 10.1371/journal.pone.0134091 PG 24 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO0JM UT WOS:000358836800102 PM 26221949 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amako, K Coutinho, 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CA ATLAS Collaboration TI Search for the Standard Model Higgs boson produced in association with top quarks and decaying into in collisions at with the ATLAS detector SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID PARTON DISTRIBUTIONS; MASSLESS PARTICLES; BROKEN SYMMETRIES; HADRON COLLIDERS; MONTE-CARLO; LHC; PAIR; NLO; PROGRAM; LEPTONS AB A search for the Standard Model Higgs boson produced in association with a top-quark pair, , is presented. The analysis uses 20.3 fb(-1) of pp collision data at , collected with the ATLAS detector at the Large Hadron Collider during 2012. The search is designed for the decay mode and uses events containing one or two electrons or muons. In order to improve the sensitivity of the search, events are categorised according to their jet and b-tagged jet multiplicities. A neural network is used to discriminate between signal and background events, the latter being dominated by +jets production. In the single-lepton channel, variables calculated using a matrix element method are included as inputs to the neural network to improve discrimination of the irreducible background. No significant excess of events above the background expectation is found and an observed (expected) limit of 3.4 (2.2) times the Standard Model cross section is obtained at 95 % confidence level. The ratio of the measured signal cross section to the Standard Model expectation is found to be assuming a Higgs boson mass of 125 Gev. C1 [Jackson, P.; Lee, L.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Yildiz, H. 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A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allbrooke, B. M. M.; Bella, L. Aperio; Bansil, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Owen, R. E.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Alberghi, G. L.; Bellagamba, L.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Corradi, M.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Alberghi, G. L.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Cioara, I. A.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Hageboeck, S.; Hansen, M. C.; Hellmich, D.; Hohn, D.; Huegging, F.; Janssen, J.; Khoriauli, G.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mergelmeyer, S.; Mijovic, L.; Mueller, K.; Nanava, G.; Obermann, T.; Pohl, D.; Ricken, O.; Sarrazin, B.; Schaepe, S.; Schopf, E.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Seema, P.; Stillings, J. A.; Tannoury, N.; Therhaag, J.; Uhlenbrock, M.; Velz, T.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Zimmermann, R.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Fitzgerald, E. A.; Sciolla, G.; Venturini, A.; Zambito, S.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Amaral Coutinho, Y.; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE, EE, IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Fed Univ Juiz de Fora UFJF, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Navarro, J. L. La Rosa; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Iengo, P.; Jaekel, M. R.; Jakobsen, S.; Jenni, P.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.; ATLAS Collaboration] CERN, CH-1211 Geneva 23, Switzerland. [Alison, J.; Anderson, K. J.; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.; Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan 250100, Shandong, Peoples R China. [Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. 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[Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, I-00044 Frascati, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Bessner, M.; Bloch, I.; Britzger, D.; Deterre, C.; Eckardt, C.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hengler, C.; Hiller, K. H.; Howarth, J.; Katzy, J.; Keller, J. S.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Moenig, K.; Petit, E.; Rubinskiy, I.; Sedov, G.; South, D.; Tackmann, K.; Wang, J.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.; Wasicki, C.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dao, V.; Di Simone, A.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Warsinsky, M.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Picazio, A.; Ristic, B.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bindi, M.; Blumenschein, U.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Keil, M.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, Lab Phys Subatom & Cosmol, CNRS, IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimares; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Keyes, R. A.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R. W.; Jussel, P.; Kneringer, E.; Lukas, W.; Usanova, A.] Univ Innsbruck, Inst Astro & Teilchenphys, A-6020 Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, S.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kukhtin, V.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Allport, P. P.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr; Savage, G.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Pilkington, A. D.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fys Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Mochizuki, K.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, E-28049 Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Hulsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Poettgen, R.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA USA. [Belanger-Champagne, C.; Chapleau, B.; Chuinard, A. J.; Corriveau, F.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Hu, X.; Levin, D.; Long, J. D.; Lu, N.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Xu, L.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Moser, H. G.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Konig, A. C.; Nektarijevic, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen, Inst Math Astrophys & Particle Phys, Nikhef, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Adelman, J.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Hariri, F.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Nellist, C.; Poggioli, L.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Zerwas, D.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS IN2P3, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pachal, K.; Pickering, M. A.; Ryder, N. C.; Sawyer, C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Lipeles, E.; Machado Miguens, J.; Meyer, C.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. Univ Nova Lisboa, Dep Fis, Caparica, Portugal. Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Di Ciaccio, A.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Stanescu, C.; Taccini, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Taccini, C.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Fac Sci Ain Chock, Reseau Univ Phys Hautes Energies, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Techn Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hann, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph; Schwemling, Ph; Schwindling, J.] CEA Saclay Commissariat Energie Atom & Energie Al, DSM IRFU Inst Rech Lois Fondamentales Univers, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; O'Neil, D. C.; Stelzer, B.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Mount, R.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.; Meehan, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Govender, N.; Lee, C. A.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hamity, G. N.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Hsu, P. J.; Jamin, D. O.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Munwes, Y.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Ilic, N.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Jovicevic, J.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Perez Codina, E.; Savard, P.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Cardarelli, R.; Corso-Radu, A.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Sez Trieste, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Neubauer, M. S.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Piqueras, D. Alvarez; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Piqueras, D. Alvarez; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Piqueras, D. Alvarez; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Piqueras, D. Alvarez; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Piqueras, D. Alvarez; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; Henkelmann, S.; King, S. 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B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Kuger, F.; Neumann, M.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Beermann, T. A.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Ctr Calcul Inst Natl Phys Nucl & Phys Particules, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London WC2R 2LS, England. [Anisenkov, A. V.; Bobrovnikov, V. S.; Buzykaev, R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Bawa, H. S.; Gao, Y. S.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beck, H. P.] Univ Fribourg, Dept Phys, CH-1700 Fribourg, Switzerland. [Castro, N. F.] Univ Porto, Fac Ciencias, Dept Fis & Astron, P-4100 Oporto, Portugal. [Chelkov, G. A.] Tomsk State Univ, Tomsk 634050, Russia. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] Inst Particle Phys, Victoria, BC, Canada. [Davies, E.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Grinstein, S.; Juste Rozas, A.; Martinez, M.] ICREA, Barcelona, Spain. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Khubua, J.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Li, B.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] State Univ, Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; Staroba, Pavel/G-8850-2014; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Boldyrev, Alexey/M-9684-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Brooks, William/C-8636-2013; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; De, Kaushik/N-1953-2013; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Mitsou, Vasiliki/D-1967-2009; Zhukov, Konstantin/M-6027-2015; Shmeleva, Alevtina/M-6199-2015; Gavrilenko, Igor/M-8260-2015; Veneziano, Stefano/J-1610-2012; Livan, Michele/D-7531-2012; spagnolo, stefania/A-6359-2012; Di Domenico, Antonio/G-6301-2011; Negrini, Matteo/C-8906-2014; Tassi, Enrico/K-3958-2015; Boyko, Igor/J-3659-2013; Ciubancan, Liviu Mihai/L-2412-2015; White, Ryan/E-2979-2015; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Martinez, Mario /I-3549-2015; Peleganchuk, Sergey/J-6722-2014; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Garcia, Jose /H-6339-2015; Smirnova, Oxana/A-4401-2013; Doyle, Anthony/C-5889-2009; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Pacheco Pages, Andres/C-5353-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Snesarev, Andrey/H-5090-2013 OI Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Tikhomirov, Vladimir/0000-0002-9634-0581; Warburton, Andreas/0000-0002-2298-7315; Brooks, William/0000-0001-6161-3570; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; De, Kaushik/0000-0002-5647-4489; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Mitsou, Vasiliki/0000-0002-1533-8886; Veneziano, Stefano/0000-0002-2598-2659; Livan, Michele/0000-0002-5877-0062; spagnolo, stefania/0000-0001-7482-6348; Di Domenico, Antonio/0000-0001-8078-2759; Negrini, Matteo/0000-0003-0101-6963; Boyko, Igor/0000-0002-3355-4662; Ciubancan, Liviu Mihai/0000-0003-1837-2841; White, Ryan/0000-0003-3589-5900; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Smirnova, Oxana/0000-0003-2517-531X; Doyle, Anthony/0000-0001-6322-6195; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Pacheco Pages, Andres/0000-0001-8210-1734; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; FU ANPCyT, Argentina; Yer-PhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; RGC, Hong Kong SAR, China; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We honour the memory of our colleague Richard St. Denis, who was a driving force of the work described here for a long time and died shortly before its completion. We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; Yer-PhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; RGC, Hong Kong SAR, China; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 116 TC 14 Z9 14 U1 14 U2 73 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JUL 29 PY 2015 VL 75 IS 7 AR 349 DI 10.1140/epjc/s10052-015-3543-1 PG 50 WC Physics, Particles & Fields SC Physics GA CN7IB UT WOS:000358606700001 ER PT J AU Campbell, BJ Rosenkranz, S Kang, HJ Stokes, HT Chupas, PJ Komiya, S Ando, Y Li, SL Dai, PC AF Campbell, B. J. Rosenkranz, S. Kang, H. J. Stokes, H. T. Chupas, P. J. Komiya, S. Ando, Y. Li, Shiliang Dai, Pengcheng TI Long-range two-dimensional superstructure in the superconducting electron-doped cuprate Pr0.88LaCe0.12CuO4 SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTOR; T-C; DIFFRACTION PATTERN; NEUTRON-DIFFRACTION; SINGLE-CRYSTAL; X-RAY; PHASE; YBA2CU3O6.35; TRANSITION; SYMMETRY AB Utilizing single-crystal synchrotron x-ray scattering, we observe distorted CuO2 planes in the electron-doped superconductor Pr1-xLaCexCuO4+delta, x = 0.12. Resolution-limited rods of scattering are indicative of a long-range two-dimensional 2 root 2 x 2 root 2 superstructure in the a-b plane, adhering to planar space-group symmetry p4gm, which is subject to stacking disorder perpendicular to the planes. This superstructure is present only in annealed, superconducting samples, but not in the as-grown, nonsuperconducting samples. These long-range distortions of the CuO2 planes, which are generally considered to be detrimental to superconductivity, have avoided detection to date due to the challenges of observing and interpreting subtle diffuse-scattering features. C1 [Campbell, B. J.; Stokes, H. T.] Brigham Young Univ, Dept Phys & Astron, Provo, UT 84602 USA. [Rosenkranz, S.; Chupas, P. J.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Kang, H. J.] Clemson Univ, Dept Phys & Astron, Clemson, SC 29634 USA. [Chupas, P. J.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Komiya, S.] Cent Res Inst Elect Power Ind, Yokosuka, Kanagawa 2400196, Japan. [Ando, Y.] Osaka Univ, Inst Sci & Ind Res, Ibaraki, Osaka 5670047, Japan. [Li, Shiliang] Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Li, Shiliang] Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China. [Dai, Pengcheng] Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. RP Campbell, BJ (reprint author), Brigham Young Univ, Dept Phys & Astron, Provo, UT 84602 USA. EM branton_campbell@byu.edu; srosenkranz@anl.gov RI Rosenkranz, Stephan/E-4672-2011; Dai, Pengcheng /C-9171-2012; Ando, Yoichi/B-8163-2013 OI Rosenkranz, Stephan/0000-0002-5659-0383; Dai, Pengcheng /0000-0002-6088-3170; Ando, Yoichi/0000-0002-3553-3355 FU U.S. NSF [DMR-0756568]; Research Corporation for Science Advancement; U.S. DOE BES [DE-SC0012311]; Robert A. Welch Foundation [C-1839]; Materials Science and Engineering Division, Basic Energy Sciences, Office of Science, U.S. DOE; DOE Office of Science [DE-AC02-06CH11357]; Japan Society for the Promotion of Science FX Synchrotron x-ray work was supported in part by the U.S. NSF, Grant No. DMR-0756568, and an award from Research Corporation for Science Advancement. PLCCO single-crystal growth at Rice and x-ray diffraction was supported by the U.S. DOE BES under Contract No. DE-SC0012311. Part of the materials work at Rice University is supported by the Robert A. Welch Foundation Grant No. C-1839. Work at Argonne (S.R., P.J.C.) was supported by the Materials Science and Engineering Division, Basic Energy Sciences, Office of Science, U.S. DOE. This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. Crystal growth performed in Japan was supported by a Grant-in-Aid for Science provided by the Japan Society for the Promotion of Science. NR 35 TC 1 Z9 1 U1 1 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUL 29 PY 2015 VL 92 IS 1 AR 014118 DI 10.1103/PhysRevB.92.014118 PG 7 WC Physics, Condensed Matter SC Physics GA CO0LA UT WOS:000358841400002 ER PT J AU Cook, AM Matern, S Hickey, C Aczel, AA Paramekanti, A AF Cook, A. M. Matern, S. Hickey, C. Aczel, A. A. Paramekanti, A. TI Spin-orbit coupled j(eff)=1/2 iridium moments on the geometrically frustrated fcc lattice SO PHYSICAL REVIEW B LA English DT Article ID HEISENBERG-ANTIFERROMAGNET; MAGNETIC-STRUCTURES; QUANTUM; TRANSITION; EXCHANGE AB Motivated by experiments on the double perovskites La2ZnIrO6 and La2MgIrO6, we study the magnetism of spin-orbit coupled j(eff) = 1/2 iridium moments on the three-dimensional, geometrically frustrated, face-centered cubic lattice. The symmetry-allowed nearest-neighbor interaction includes Heisenberg, Kitaev, and symmetric off-diagonal exchange. A Luttinger-Tisza analysis shows a rich variety of orders, including collinear A-type antiferromagnetism, stripe order with moments along the {111} direction, and incommensurate noncoplanar spirals, and we use Monte Carlo simulations to determine their magnetic ordering temperatures. We argue that existing thermodynamic data on these iridates underscores the presence of a dominant Kitaev exchange, and also suggest a resolution to the puzzle of why La2ZnIrO6, but not La2MgIrO6, exhibits "weak" ferromagnetism. C1 [Cook, A. M.; Hickey, C.; Paramekanti, A.] Univ Toronto, Dept Phys, Toronto, ON M5S 1A7, Canada. [Matern, S.] Univ Cologne, Inst Theoret Phys, D-50937 Cologne, Germany. [Aczel, A. A.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Paramekanti, A.] Canadian Inst Adv Res, Toronto, ON M5G 1Z8, Canada. RP Cook, AM (reprint author), Univ Toronto, Dept Phys, 60 St George St, Toronto, ON M5S 1A7, Canada. RI Aczel, Adam/A-6247-2016 OI Aczel, Adam/0000-0003-1964-1943 FU NSERC of Canada; Bonn-Cologne Graduate School of Physics and Astronomy; Scientific User Facilities Division of the US Department of Energy, Office of Basic Energy Sciences FX We thank G. Chen, J. P. Clancy, B. D. Gaulin, G. Jackeli, J. E. Greedan, Y. B. Kim, Y. J. Kim, and S. Trebst for useful discussions. We acknowledge support from NSERC of Canada (A.M.C., C.H., A.P.), the Bonn-Cologne Graduate School of Physics and Astronomy (S.M.), and the Scientific User Facilities Division of the US Department of Energy, Office of Basic Energy Sciences (A.A.A.). NR 64 TC 8 Z9 8 U1 3 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUL 29 PY 2015 VL 92 IS 2 AR 020417 DI 10.1103/PhysRevB.92.020417 PG 6 WC Physics, Condensed Matter SC Physics GA CO0LH UT WOS:000358842300001 ER PT J AU Harmand, M Ravasio, A Mazevet, S Bouchet, J Denoeud, A Dorchies, F Feng, Y Fourment, C Galtier, E Gaudin, J Guyot, F Kodama, R Koenig, M Lee, HJ Miyanishi, K Morard, G Musella, R Nagler, B Nakatsutsumi, M Ozaki, N Recoules, V Toleikis, S Vinci, T Zastrau, U Zhu, D Benuzzi-Mounaix, A AF Harmand, M. Ravasio, A. Mazevet, S. Bouchet, J. Denoeud, A. Dorchies, F. Feng, Y. Fourment, C. Galtier, E. Gaudin, J. Guyot, F. Kodama, R. Koenig, M. Lee, H. J. Miyanishi, K. Morard, G. Musella, R. Nagler, B. Nakatsutsumi, M. Ozaki, N. Recoules, V. Toleikis, S. Vinci, T. Zastrau, U. Zhu, D. Benuzzi-Mounaix, A. TI X-ray absorption spectroscopy of iron at multimegabar pressures in laser shock experiments SO PHYSICAL REVIEW B LA English DT Article ID EARTHS INNER-CORE; MELTING CURVE; TEMPERATURES AB Taking advantage of the new opportunities provided by x-ray free electron laser (FEL) sources when coupled to a long laser pulse as available at the Linear Coherent Light Source (LCLS), we have performed x-ray absorption near-edge spectroscopy (XANES) of laser shock compressed iron up to 420 GPa (+/- 50) and 10 800 K (+/- 1390). Visible diagnostics coupled with hydrodynamic simulations were used to infer the thermodynamical conditions along the Hugoniot and the release adiabat. A modification of the pre-edge feature at 7.12 keV in the XANES spectra is observed above pressures of 260 GPa along the Hugoniot. Comparing with ab initio calculations and with previous laser-heated diamond cell data, we propose that such changes in the XANES pre-edge could be a signature of molten iron. This interpretation then suggests that iron is molten at pressures and temperatures higher than 260 GPa (+/- 29) and 5680 K (+/- 700) along the principal Fe Hugoniot. C1 [Harmand, M.; Ravasio, A.; Denoeud, A.; Koenig, M.; Vinci, T.; Benuzzi-Mounaix, A.] UPMC, CEA, CNRS, LULI,Ecole Polytech, Palaiseau, France. [Harmand, M.; Guyot, F.; Morard, G.] UPMC, CNRS, IMPMC, MNHN,IRD, Paris, France. [Mazevet, S.; Musella, R.; Benuzzi-Mounaix, A.] Univ Paris Diderot, CNRS, Observ Paris, LUTH, Meudon, France. [Bouchet, J.; Recoules, V.] CEA, DAM, DIF, Arpajon, France. [Dorchies, F.; Fourment, C.; Gaudin, J.] Univ Bordeaux, CNRS, CEA, CELIA, Talence, France. [Feng, Y.; Galtier, E.; Lee, H. J.; Nagler, B.; Zastrau, U.; Zhu, D.] SLAC, LCLS, Stanford, CA USA. [Kodama, R.; Miyanishi, K.; Ozaki, N.] Osaka Univ, Grad Sch Engn, Osaka, Japan. [Nakatsutsumi, M.] European XFEL GmbH, D-22671 Hamburg, Germany. [Toleikis, S.] DESY, FLASH, Hamburg, Germany. [Zastrau, U.] Univ Jena, Inst Opt & Quantum Elect, D-07745 Jena, Germany. RP Harmand, M (reprint author), UPMC, CEA, CNRS, LULI,Ecole Polytech, Palaiseau, France. EM marion.harmand@impmc.upmc.fr RI GUYOT, Francois/C-3824-2016; IMPMC, Geobio/F-8819-2016; harmand, marion/Q-1248-2016; Kodama, Ryosuke/G-2627-2016 OI GUYOT, Francois/0000-0003-4622-2218; harmand, marion/0000-0003-0713-5824; FU French Agence Nationale de la Recherche (ANR); ANR IRONFEL; Planetlab; DOE Office of Science, Fusion Energy Science [SF00515]; LCLS, a National User Facility FX We acknowledge R. Torchio, P. Mounaix, D. Antonangeli, and D. Cabaret for helpful discussions. We thank our reviewers and the editor who helped to considerably improve the manuscript. This work is supported by the French Agence Nationale de la Recherche (ANR) with the ANR IRONFEL and Planetlab. This work was performed at the Matter at Extreme Conditions (MEC) instrument of LCLS, supported by the DOE Office of Science, Fusion Energy Science under Contract No. SF00515. This work was also supported by LCLS, a National User Facility operated by Stanford University on behalf of the US Department of Energy, Office of Basic Energy Sciences. NR 36 TC 10 Z9 10 U1 11 U2 40 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 29 PY 2015 VL 92 IS 2 AR 024108 DI 10.1103/PhysRevB.92.024108 PG 7 WC Physics, Condensed Matter SC Physics GA CO0LH UT WOS:000358842300003 ER PT J AU Lobo, RPSM Buhot, J Measson, MA Aoki, D Lapertot, G Lejay, P Homes, CC AF Lobo, R. P. S. M. Buhot, J. Measson, M. A. Aoki, D. Lapertot, G. Lejay, P. Homes, C. C. TI Optical conductivity of URu2Si2 in the Kondo liquid and hidden-order phases SO PHYSICAL REVIEW B LA English DT Article ID POINT-CONTACT SPECTROSCOPY; FERMION SYSTEM URU2SI2; SYMMETRY-BREAKING; SUPERCONDUCTOR URU2SI2; INFRARED PROPERTIES; LATTICE; TRANSITIONS; SURFACE; STATE; RESISTIVITY AB We measured the polarized optical conductivity of URu2Si2 from room temperature down to 5 K, covering the Kondo state, the coherent Kondo liquid regime, and the hidden-order phase. The normal state is characterized by an anisotropic behavior between the ab plane and c-axis responses. The ab-plane optical conductivity is strongly influenced by the formation of the coherent Kondo liquid: a sharp Drude peak develops and a hybridization gap at 12 meV leads to a spectral weight transfer to mid-infrared energies. The c-axis conductivity has a different behavior: the Drude peak already exists at 300 K and no particular anomaly or gap signature appears in the coherent Kondo liquid regime. When entering the hidden-order state, both polarizations see a dramatic decrease in the Drude spectral weight and scattering rate, compatible with a loss of about 50% of the carriers at the Fermi level. At the same time a density-wave-like gap appears along both polarizations at about 6.5 meV at 5 K. This gap closes respecting a mean-field thermal evolution in the ab plane. Along the c-axis it remains roughly constant and it "fills up" rather than closing. C1 [Lobo, R. P. S. M.] Univ Paris 06, ESPCI ParisTech, PSL Res Univ, Sorbonne Univ,CNRS,LPEM, F-75231 Paris 5, France. [Buhot, J.; Measson, M. A.] Univ Paris Diderot, UMR CNRS 7162, Lab Mat & Phenomenes Quant, F-75205 Paris 13, France. [Aoki, D.; Lapertot, G.] Univ Grenoble Alpes, INAC SPSMS, F-38000 Grenoble, France. [Aoki, D.; Lapertot, G.] CEA, INAC SX, F-38000 Grenoble, France. [Lejay, P.] CNRS, Inst Neel, F-38042 Grenoble, France. [Lejay, P.] Univ Grenoble Alpes, F-38042 Grenoble, France. [Homes, C. C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Lobo, RPSM (reprint author), Univ Paris 06, ESPCI ParisTech, PSL Res Univ, Sorbonne Univ,CNRS,LPEM, 10 Rue Vauquelin, F-75231 Paris 5, France. EM lobo@espci.fr RI Measson, Marie-aude/E-6388-2015; Aoki, Dai/K-3673-2012; OI Measson, Marie-aude/0000-0002-6495-7376; Aoki, Dai/0000-0003-2334-8360; Lobo, Ricardo/0000-0003-2355-6856 FU Office of Science, U.S. Department of Energy [DE-SC0012704]; French Agence Nationale de la Recherche (ANR PRINCESS); Labex SEAM [ANR-11-IDEX-0005-02] FX We thank D. B. Tanner, T. Timusk, G. Kotliar, A. Millis, and C. Pepin for fruitful discussions. Work at Brookhaven National Laboratory was supported by the Office of Science, U.S. Department of Energy, under Contract No. DE-SC0012704. The work in Universite Paris Diderot was supported by the French Agence Nationale de la Recherche (ANR PRINCESS) and the Labex SEAM (Grant No. ANR-11-IDEX-0005-02). NR 61 TC 3 Z9 3 U1 7 U2 24 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 29 PY 2015 VL 92 IS 4 AR 045129 DI 10.1103/PhysRevB.92.045129 PG 9 WC Physics, Condensed Matter SC Physics GA CO0MM UT WOS:000358845700005 ER PT J AU Tobin, JG Yu, SW Qiao, R Yang, WL Booth, CH Shuh, DK Duffin, AM Sokaras, D Nordlund, D Weng, TC AF Tobin, J. G. Yu, S. -W. Qiao, R. Yang, W. L. Booth, C. H. Shuh, D. K. Duffin, A. M. Sokaras, D. Nordlund, D. Weng, T. -C. TI Covalency in oxidized uranium SO PHYSICAL REVIEW B LA English DT Article ID X-RAY-ABSORPTION; PLUTONIUM INTERMETALLICS; EMISSION SPECTROSCOPY; 5F ORBITALS; OXIDES AB Using x-ray emission spectroscopy and absorption spectroscopy, it has been possible to directly access the states in the unoccupied conduction bands that are involved with 5f and 6d covalency in oxidized uranium. By varying the oxidizing agent, the degree of 5f covalency can be manipulated and monitored, clearly and irrevocably establishing the importance of 5f covalency in the electronic structure of the key nuclear fuel, uranium dioxide. C1 [Tobin, J. G.; Yu, S. -W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Qiao, R.; Yang, W. L.; Booth, C. H.; Shuh, D. K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Duffin, A. M.] Pacific NW Natl Lab, Washington, DC 99354 USA. [Sokaras, D.; Nordlund, D.; Weng, T. -C.] Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. RP Tobin, JG (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM Tobin1@LLNL.Gov RI Qiao, Ruimin/E-9023-2013; Yang, Wanli/D-7183-2011; Tobin, James/O-6953-2015; Nordlund, Dennis/A-8902-2008 OI Yang, Wanli/0000-0003-0666-8063; Nordlund, Dennis/0000-0001-9524-6908 FU U.S. Department of Energy, National Nuclear Security Administration [DE-AC52-07NA27344]; Director of the Office of Science, Office of Basic Energy Sciences (OBES), Division of Chemical Sciences, Geosciences, and Biosciences (CSGB), Heavy Element Chemistry (HEC) Program of the U.S. Department of Energy [DE-AC02-05CH11231]; Director of the Office of Science, OBES of the U.S. Department of Energy at LBNL [DE-AC02-05CH11231] FX Lawrence Livermore National Laboratory (LLNL) is operated by Lawrence Livermore National Security, LLC, for the U.S. Department of Energy, National Nuclear Security Administration, under Contract DE-AC52-07NA27344. Work at Lawrence Berkeley National Laboratory (LBNL) (C.H.B., D.K.S.) was supported by the Director of the Office of Science, Office of Basic Energy Sciences (OBES), Division of Chemical Sciences, Geosciences, and Biosciences (CSGB), Heavy Element Chemistry (HEC) Program of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The ALS is supported by the Director of the Office of Science, OBES of the U.S. Department of Energy at LBNL under Contract No. DE-AC02-05CH11231. The Stanford Synchrotron Radiation Lightsource is a national user facility operated by Stanford University on behalf of the DOE, Office of Basic Energy Sciences. The UF4 sample was originally prepared at Oak Ridge National Laboratory and provided to LLNL by J. S. Morrell of Y12 [9]. J.G.T. wishes to thank (1) Glenn Fox and the PRT Program at LLNL for support during his sabbatical at LBNL; (2) D.K.S. for his hosting of the sabbatical at GTSC/LBNL; and (3) C.H.B. for the opportunity to learn new hard x-ray skills and collect data in the middle of the night again. NR 27 TC 2 Z9 2 U1 2 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUL 29 PY 2015 VL 92 IS 4 AR 045130 DI 10.1103/PhysRevB.92.045130 PG 5 WC Physics, Condensed Matter SC Physics GA CO0MM UT WOS:000358845700006 ER PT J AU Walker, CL Krticka, M Baramsai, B Becvar, F Bredeweg, TA Chyzh, A Haight, RC Jandel, M Kroll, J Mitchell, GE O'Donnell, JM Rundberg, RS Ullmann, JL Valenta, S Wilhelmy, JB AF Walker, C. L. Krticka, M. Baramsai, B. Becvar, F. Bredeweg, T. A. Chyzh, A. Haight, R. C. Jandel, M. Kroll, J. Mitchell, G. E. O'Donnell, J. M. Rundberg, R. S. Ullmann, J. L. Valenta, S. Wilhelmy, J. B. TI Measurement of the Mo-97(n,gamma) reaction with the DANCE gamma calorimeter array SO PHYSICAL REVIEW C LA English DT Article ID STRENGTH FUNCTIONS; NEUTRON-CAPTURE; CROSS-SECTIONS; RESONANCE; ISOTOPES; DETECTOR; LIBRARY; SCIENCE; NUCLEI AB Spectra of. rays following the Mo-97(n,gamma) reaction were measured as a function of incident neutron energy with the DANCE (Detector for Advanced Neutron Capture Experiments) array of 160 BaF2 scintillation detectors at the Los Alamos Neutron Science Center using an enriched Mo-97 target. These spectra were used for the assignment of spins of the Mo-97 resonances up to neutron energy E-n = 1.7 keV, as well as in the study of photon strength functions (PSFs) in Mo-98. Analysis of the spectra with the nuclear statistical model showed that they can be well reproduced with the same PSF models which well described the gamma decay following slow neutron capture in Mo-95. On the other hand, the spectra are inconsistent with PSFs describing some other experimental data in Mo-98. C1 [Walker, C. L.; Baramsai, B.; Chyzh, A.; Mitchell, G. E.] N Carolina State Univ, Raleigh, NC 27695 USA. [Walker, C. L.; Baramsai, B.; Chyzh, A.; Mitchell, G. E.] Triangle Univ Nucl Lab, Durham, NC 27708 USA. [Walker, C. L.; Baramsai, B.; Bredeweg, T. A.; Haight, R. C.; Jandel, M.; O'Donnell, J. M.; Rundberg, R. S.; Ullmann, J. L.; Wilhelmy, J. B.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Krticka, M.; Becvar, F.; Kroll, J.; Valenta, S.] Charles Univ Prague, Fac Math & Phys, CZ-18000 Prague 8, Czech Republic. RP Krticka, M (reprint author), Charles Univ Prague, Fac Math & Phys, V Holesovickach 2, CZ-18000 Prague 8, Czech Republic. EM krticka@ipnp.troja.mff.cuni.cz FU U.S. Department of Energy [DE-NA0001784, DE-FG02-97-ER41042]; U.S. Department of Energy at Los Alamos National Laboratory - Los Alamos National Security, LLC [DE-AC52-06NA25396]; LLNL [DE-AC52-07NA27344]; Czech Science Foundation [13-07117S] FX This work was supported in part by the U.S. Department of Energy Grants No. DE-NA0001784 and No. DE-FG02-97-ER41042. This work benefited from the use of the LANSCE accelerator and was performed under the auspices of the U.S. Department of Energy at Los Alamos National Laboratory by Los Alamos National Security, LLC under Contract No. DE-AC52-06NA25396 and LLNL Contract No. DE-AC52-07NA27344. It was also supported by Grant No. 13-07117S of the Czech Science Foundation. NR 48 TC 2 Z9 2 U1 3 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JUL 29 PY 2015 VL 92 IS 1 AR 014324 DI 10.1103/PhysRevC.92.014324 PG 14 WC Physics, Nuclear SC Physics GA CO0NB UT WOS:000358847400001 ER PT J AU Cai, H Scott, E Kholghi, A Andreadi, C Rufini, A Karmokar, A Britton, RG Horner-Glister, E Greaves, P Jawad, D James, M Howells, L Ognibene, T Malfatti, M Goldring, C Kitteringham, N Walsh, J Viskaduraki, M West, K Miller, A Hemingway, D Steward, WP Gescher, AJ Brown, K AF Cai, Hong Scott, Edwina Kholghi, Abeer Andreadi, Catherine Rufini, Alessandro Karmokar, Ankur Britton, Robert G. Horner-Glister, Emma Greaves, Peter Jawad, Dhafer James, Mark Howells, Lynne Ognibene, Ted Malfatti, Michael Goldring, Christopher Kitteringham, Neil Walsh, Joanne Viskaduraki, Maria West, Kevin Miller, Andrew Hemingway, David Steward, William P. Gescher, Andreas J. Brown, Karen TI Cancer chemoprevention: Evidence of a nonlinear dose response for the protective effects of resveratrol in humans and mice SO SCIENCE TRANSLATIONAL MEDICINE LA English DT Article ID FAMILIAL ADENOMATOUS POLYPOSIS; ACCELERATOR MASS-SPECTROMETRY; ACTIVATED PROTEIN-KINASE; APC(MIN/+) MICE; PROSTATE-CANCER; BETA-CAROTENE; DIABETES-MELLITUS; COLORECTAL-CANCER; AGENT RESVERATROL; GLUCOSE-TOLERANCE AB Resveratrol is widely promoted as a potential cancer chemopreventive agent, but a lack of information on the optimal dose prohibits rationally designed trials to assess efficacy. To challenge the assumption that "more is better," we compared the pharmacokinetics and activity of a dietary dose with an intake 200 times higher. The dose-response relationship for concentrations generated and the metabolite profile of [C-14]-resveratrol in colorectal tissue of cancer patients helped us to define clinically achievable levels. In Apc(Min) mice (a model of colorectal carcinogenesis) that received a high-fat diet, the low resveratrol dose suppressed intestinal adenoma development more potently than did the higher dose. Efficacy correlated with activation of adenosine monophosphate-activated protein kinase (AMPK) and increased expression of the senescence marker p21. Nonlinear dose responses were observed for AMPK and mechanistic target of rapamycin (mTOR) signaling in mouse adenoma cells, culminating in autophagy and senescence. In human colorectal tissues exposed to low dietary concentrations of resveratrol ex vivo, we measured enhanced AMPK phosphorylation and autophagy. The expression of the cytoprotective NAD(P) H dehydrogenase, quinone 1 (NQO1) enzyme was also increased in tissues from cancer patients participating in our [C-14]-resveratrol trial. These findings warrant a revision of developmental strategies for diet-derived agents designed to achieve cancer chemoprevention. C1 [Cai, Hong; Scott, Edwina; Kholghi, Abeer; Andreadi, Catherine; Rufini, Alessandro; Karmokar, Ankur; Britton, Robert G.; Horner-Glister, Emma; Greaves, Peter; Jawad, Dhafer; James, Mark; Howells, Lynne; Steward, William P.; Gescher, Andreas J.; Brown, Karen] Univ Leicester, Dept Canc Studies, Canc Chemoprevent Grp, Leicester LE2 7LX, Leics, England. [Ognibene, Ted; Malfatti, Michael] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Goldring, Christopher; Kitteringham, Neil; Walsh, Joanne] Univ Liverpool, Dept Pharmacol & Therapeut, MRC, Ctr Drug Safety Sci, Liverpool L69 3GE, Merseyside, England. [Viskaduraki, Maria] Univ Leicester, Bioinformat & Biostat Support Hub, Leicester LE1 9HN, Leics, England. [West, Kevin; Miller, Andrew; Hemingway, David] Univ Hosp Leicester NHS Trust, Leicester LE1 5WW, Leics, England. RP Brown, K (reprint author), Univ Leicester, Dept Canc Studies, Canc Chemoprevent Grp, Leicester LE2 7LX, Leics, England. EM kb20@le.ac.uk FU Cancer Research UK [C325/A13101]; Libyan government through Benghazi University; NIH National Centre for Research Resources, Biomedical Technology Program [P41RR13461] FX This work was supported by Cancer Research UK (C325/A13101) with assistance from the Leicester Experimental Cancer Medicine Centre (C325/A15575, Cancer Research UK/UK Department of Health). A. Kholghi was funded by a studentship from the Libyan government through Benghazi University. AMS analysis was performed at the Research Resource for Biomedical AMS Laboratory, operated at LLNL, and supported by the NIH National Centre for Research Resources, Biomedical Technology Program grant #P41RR13461. NR 63 TC 20 Z9 20 U1 15 U2 35 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 1946-6234 EI 1946-6242 J9 SCI TRANSL MED JI Sci. Transl. Med. PD JUL 29 PY 2015 VL 7 IS 298 AR 298ra117 DI 10.1126/scitranslmed.aaa7619 PG 12 WC Cell Biology; Medicine, Research & Experimental SC Cell Biology; Research & Experimental Medicine GA CN9AZ UT WOS:000358739300003 PM 26223300 ER PT J AU Blum, LW Halford, A Millan, R Bonnell, JW Goldstein, J Usanova, M Engebretson, M Ohnsted, M Reeves, G Singer, H Clilverd, M Li, X AF Blum, L. W. Halford, A. Millan, R. Bonnell, J. W. Goldstein, J. Usanova, M. Engebretson, M. Ohnsted, M. Reeves, G. Singer, H. Clilverd, M. Li, X. TI Observations of coincident EMIC wave activity and duskside energetic electron precipitation on 18-19 January 2013 SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE EMIC waves; electron precipitation; radiation belts ID ION-CYCLOTRON WAVES; PITCH-ANGLE SCATTERING; RELATIVISTIC ELECTRON; RADIATION BELT; GEOMAGNETIC STORMS; PLASMAPAUSE; SIMULATION; SATELLITES; SAMPEX AB Electromagnetic ion cyclotron (EMIC) waves have been suggested to be a cause of radiation belt electron loss to the atmosphere. Here simultaneous, magnetically conjugate measurements are presented of EMIC wave activity, measured at geosynchronous orbit and on the ground, and energetic electron precipitation, seen by the Balloon Array for Radiation belt Relativistic Electron Losses (BARREL) campaign, on two consecutive days in January 2013. Multiple bursts of precipitation were observed on the duskside of the magnetosphere at the end of 18 January and again late on 19 January, concurrent with particle injections, substorm activity, and enhanced magnetospheric convection. The structure, timing, and spatial extent of the waves are compared to those of the precipitation during both days to determine when and where EMIC waves cause radiation belt electron precipitation. The conjugate measurements presented here provide observational support of the theoretical picture of duskside interaction of EMIC waves and MeV electrons leading to radiation belt loss. C1 [Blum, L. W.; Bonnell, J. W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Halford, A.; Millan, R.] Dartmouth Coll, Dept Phys & Astron, Hanover, NH 03755 USA. [Goldstein, J.] Southwest Res Inst, San Antonio, TX USA. [Usanova, M.; Li, X.] Lab Atmospher & Space Phys, Boulder, CO USA. [Engebretson, M.; Ohnsted, M.] Augsburg Coll, Dept Phys, Minneapolis, MN USA. [Reeves, G.] Los Alamos Natl Lab, Los Alamos, NM USA. [Singer, H.] NOAA, Space Weather Predict Ctr, Boulder, CO USA. [Clilverd, M.] British Antarctic Survey, Cambridge CB3 0ET, England. RP Blum, LW (reprint author), Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. EM lwblum@ssl.berkeley.edu OI Blum, Lauren/0000-0002-4797-5476; Reeves, Geoffrey/0000-0002-7985-8098; Halford, Alexa/0000-0002-5383-4602 FU JHU/APL [922613]; BARREL [NNX08AM58G]; NASA [NNX15AF56G]; NSF [PLR-1341493]; Natural Environmental Research Council under Antarctic Funding Initiative [AFI/11/22]; International Space Science Institute International Teams program; Canadian Space Agency FX This work was supported in part by the JHU/APL contract 922613 (RBSP-EFW). The Dartmouth portion of this work was supported by the BARREL grant NNX08AM58G. X. Li acknowledges NASA grant NNX15AF56G. Work at Augsburg College and provision of search coil data from Halley, Antarctica, were supported by NSF grant PLR-1341493. Test particle simulations (JG) were supported by the NASA Van Allen Probes mission's RBSP-ECT project. M.A.C. has received funding from the Natural Environmental Research Council under the Antarctic Funding Initiative (AFI/11/22). This work was also supported by the International Space Science Institute International Teams program. The authors thank I.R. Mann, D.K. Milling, and the rest of the CARISMA team for data, which can be accessed at www.carisma.ca.CARISMA is operated by the University of Alberta and funded by the Canadian Space Agency. Halley spectrograms can be accessed at space. augsburg.edu/searchcoil/browsehalley-graphs.html. The OMNI data were obtained from the GSFC/SPDF OMNIWeb interface at http://omniweb.gsfc.nasa.gov, which are derived from ACE and Wind solar wind plasma and magnetic field observations. BARREL measurements can be found at http://cdaweb.gsfc.nasa.gov/ and GOES at http://satdat.ngdc.noaa.gov/sem/goes/.LANL SOPA data were provided by G.Reeves (reeves@lanl.gov) and are available upon request. NR 50 TC 13 Z9 13 U1 0 U2 4 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JUL 28 PY 2015 VL 42 IS 14 BP 5727 EP 5735 DI 10.1002/2015GL065245 PG 9 WC Geosciences, Multidisciplinary SC Geology GA CO7CU UT WOS:000359316100007 ER PT J AU Fan, JW Rosenfeld, D Yang, Y Zhao, C Leung, LR Li, ZQ AF Fan, Jiwen Rosenfeld, Daniel Yang, Yan Zhao, Chun Leung, L. Ruby Li, Zhanqing TI Substantial contribution of anthropogenic air pollution to catastrophic floods in Southwest China SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE flood; pollution; aerosol impacts; extreme weather; black carbon ID DEEP CONVECTIVE CLOUDS; URBAN AEROSOL IMPACTS; ASIAN SUMMER MONSOON; CARBONACEOUS AEROSOL; ABSORBING AEROSOLS; PRECIPITATION; CLIMATE; MICROPHYSICS; SUPPRESSION; EMISSIONS AB Extreme weather events have become more frequent and are likely linked to increases in greenhouse gases and aerosols, which alter the Earth's radiative balance and cloud processes. On 8-9 July 2013, a catastrophic flood devastated the mountainous area to the northwest of the Sichuan Basin. Atmospheric simulations at a convection-permitting scale with aerosols and chemistry included show that heavy air pollution trapped in the basin significantly enhances the rainfall intensity over the mountainous areas through aerosol-enhanced conditional instability. That is, aerosols suppress convection by absorbing solar radiation and increasing atmospheric stability in the basin during daytime. This allows excess moist air to be transported to the mountainous areas and orographically lifted, generating strong convection and extremely heavy precipitation at night. We show that reducing pollution in the Sichuan Basin can effectively mitigate floods. It is suggested that coupling aerosol with meteorology can be crucial to improve weather forecast in polluted regions. C1 [Fan, Jiwen; Yang, Yan; Zhao, Chun; Leung, L. Ruby] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Rosenfeld, Daniel] Hebrew Univ Jerusalem, Inst Earth Sci, IL-91904 Jerusalem, Israel. [Yang, Yan] Chinese Acad Meteorol Sci, Beijing, Peoples R China. [Li, Zhanqing] Univ Maryland, Dept Atmospher & Ocean Sci, College Pk, MD 20742 USA. [Li, Zhanqing] Univ Maryland, ESSIC, College Pk, MD 20742 USA. [Li, Zhanqing] Beijing Normal Univ, State Key Lab Earth Surface Proc & Resource Ecol, Beijing 100875, Peoples R China. [Li, Zhanqing] Beijing Normal Univ, Joint Ctr Global Change Studies, Beijing 100875, Peoples R China. RP Fan, JW (reprint author), Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. EM Jiwen.Fan@pnnl.gov RI Zhao, Chun/A-2581-2012; Rosenfeld, Daniel/F-6077-2016; Fan, Jiwen/E-9138-2011; Li, Zhanqing/F-4424-2010 OI Zhao, Chun/0000-0003-4693-7213; Rosenfeld, Daniel/0000-0002-0784-7656; Li, Zhanqing/0000-0001-6737-382X FU U.S. Department of Energy (DOE) Office of Science Biological and Environmental Research as part of the Regional and Global Climate Modeling program (RGCM); Ministry of Science and Technology [2013CB955804]; DOE by Battelle Memorial Institute [DE-AC06-76RLO1830] FX This study was supported by the U.S. Department of Energy (DOE) Office of Science Biological and Environmental Research as part of the Regional and Global Climate Modeling program (RGCM), and the Ministry of Science and Technology (2013CB955804). The Pacific Northwest National Laboratory (PNNL) is operated for the DOE by Battelle Memorial Institute under contract DE-AC06-76RLO1830. The model simulations were performed using PNNL Institutional Computing. The model and observational data can be obtained by contacting Jiwen.Fan@pnnl.gov. NR 52 TC 16 Z9 16 U1 7 U2 32 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JUL 28 PY 2015 VL 42 IS 14 BP 6066 EP 6075 DI 10.1002/2015GL064479 PG 10 WC Geosciences, Multidisciplinary SC Geology GA CO7CU UT WOS:000359316100048 ER PT J AU Qin, LY Reger, AS Guo, E Yang, MP Zwart, P Casteel, DE Kim, C AF Qin, Liying Reger, Albert S. Guo, Elaine Yang, Matthew P. Zwart, Peter Casteel, Darren E. Kim, Choel TI Structures of cGMP-Dependent Protein Kinase (PKG) I alpha Leucine Zippers Reveal an Interchain Disulfide Bond Important for Dimer Stability SO BIOCHEMISTRY LA English DT Article ID OXIDANT-INDUCED ACTIVATION; LIGHT-CHAIN PHOSPHATASE; MOLECULAR DETAILS; CRYSTAL-STRUCTURE; BLOOD-PRESSURE; TFII-I; BETA; IRAG; BINDING; AUTOPHOSPHORYLATION AB cGMP-dependent protein kinase (PKG) I alpha is a central regulator of smooth muscle tone and vasorelaxation. The N-terminal leucine zipper (LZ) domain dimerizes and targets PKG la by interacting with G-kinase-anchoring proteins. The PKG Ia LZ contains C42 that is known to form a disulfide bond upon oxidation and to activate PKG Ia. To understand the molecular details of the PKG Ia LZ and C42-C42' disulfide bond, we determined crystal structures of the PKG Ia wild-type.(WT) LZ and C42L LZ. Our data demonstrate that the C42-C42' disulfide bond drathatically stabilizes PKG Ia and that the C42L mutant mimics the oxidized WT LZ structurally. C1 [Qin, Liying; Kim, Choel] Baylor Coll Med, Verna & Marrs McLean Dept Biochem & Mol Biol, Houston, TX 77030 USA. [Reger, Albert S.; Kim, Choel] Baylor Coll Med, Dept Pharmacol, Houston, TX 77030 USA. [Guo, Elaine] Rice Univ, Dept Chem, Houston, TX 77005 USA. [Yang, Matthew P.] Rice Univ, Dept Biochem, Houston, TX 77005 USA. [Zwart, Peter] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Casteel, Darren E.] Univ Calif San Diego, Dept Med, La Jolla, CA 92093 USA. RP Kim, C (reprint author), Baylor Coll Med, Verna & Marrs McLean Dept Biochem & Mol Biol, Houston, TX 77030 USA. EM ckim@bcm.edu FU National Institutes of Health [R01 GM090161] FX This work was funded by National Institutes of Health Grant R01 GM090161. NR 40 TC 1 Z9 1 U1 0 U2 1 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD JUL 28 PY 2015 VL 54 IS 29 BP 4419 EP 4422 DI 10.1021/acs.biochem.5b00572 PG 4 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CO0EE UT WOS:000358822100003 PM 26132214 ER PT J AU Lu, JL Elam, JW AF Lu, Junling Elam, Jeffrey W. TI Low Temperature ABC-Type Ru Atomic Layer Deposition through Consecutive Dissociative Chemisorption, Combustion, and Reduction Steps SO CHEMISTRY OF MATERIALS LA English DT Article ID RUTHENIUM THIN-FILMS; NOBLE-METALS; DEHYDROGENATION REACTIONS; REACTION-MECHANISM; GROWTH; OZONE; DIELECTRICS; PRECURSORS; ELECTRODES; CAPACITORS AB Thermal atomic layer deposition (ALD) of noble metals is frequently performed using Molecular oxygen as the nonmetal precursor to effect combustion-type chemistry at relatively high temperatures of 300 degrees C Bis-(ethylcyclopentadienyl)ruthenium (Ru(EtCp)2) is one of the commonly used metal precursors for Ru ALD. Using Ru(EtCp)(2) and oxygen as reactants, Ru ALD was achieved at near 300 degrees C. Here, we demonstrate that Ru ALD can proceed at as low as 150 degrees C by using successive exposures to oxygen and hydrogen as the coreactants. In situ quartz crystal microbalance (QCM) and quadrupole mass spectroscopy (QMS) measurements both suggest that this ABC-type ALD occurs through dissociative chemisorption, combustion, and reduction for the Ru(EtCp)(2)(,) oxygen, and hydrogen steps, respectively, in a similar manner to processes using ozone and hydrogen as coreactants reported previously. Moreover, we believe this molecular O-2 and H-2 based ABC-type ALD could be exploited for the ALD of other noble metals to decrease the deposition temperature and reduce Oxygen impurities: C1 [Lu, Junling; Elam, Jeffrey W.] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. RP Elam, JW (reprint author), Argonne Natl Lab, Div Energy Syst, 9700 S Cass Ave, Argonne, IL 60439 USA. EM jelam@anl.gov FU Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX This material is based upon work supported as part of the Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. NR 39 TC 3 Z9 3 U1 6 U2 31 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUL 28 PY 2015 VL 27 IS 14 BP 4950 EP 4956 DI 10.1021/acs.chemmater.5b00818 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CO0EN UT WOS:000358823000009 ER PT J AU Li, W Corradini, D Body, M Legein, C Salanne, M Ma, JW Chapman, KW Chupas, PJ Rollett, AL Julien, C Zhagib, K Duttine, M Demourgues, A Groult, H Dambournet, D AF Li, Wei Corradini, Dario Body, Monique Legein, Christophe Salanne, Mathieu Ma, Jiwei Chapman, Karena W. Chupas, Peter J. Rollett, Anne-Laure Julien, Christian Zhagib, Karim Duttine, Mathieu Demourgues, Alain Groult, Henri Dambournet, Damien TI High Substitution Rate in TiO2 Anatase Nanoparticles with Cationic Vacancies for Fast Lithium Storage SO CHEMISTRY OF MATERIALS LA English DT Article ID SPACE GAUSSIAN PSEUDOPOTENTIALS; PHOTOCATALYSIS; NANOMATERIALS; NANOSCALE; DETECTOR; LIXTIO2; OXIDES; WATER AB Doping is generally used to tune and enhance the properties of metal oxides. However, their chemical composition cannot be readily modified beyond low dopant amounts without disrupting the crystalline atomic structure. In the case of anatase TiO2, we introduce a new solution-based chemical route allowing the composition to be significantly modified, substituting the divalent O2- anions by monovalent F- and OH- anions resulting in the formation of cationic Ti4+ vacancies (square) whose concentration can be controlled by the reaction temperature. The resulting polyanionic anatase has the general composition Ti1-x-y square x+yO2-4(x+y)F4x(OH)(4y), reaching vacancy concentrations of up to 22%, i.e., Ti-0.78 square 0.22O1.12F0.4(OH)(0.48). Solid-state F-19 NMR spectroscopy reveals that fluoride ions can accommodate up to three different environments, depending on Ti and vacancies (i.e. Ti-3-F, Ti-2 square(1)-F, and Ti-1 square(2)-F), with a preferential location close to vacancies. DFT calculations further confirm the fluoride/vacancy ordering. When its characteristics were evaluated as an electrode for reversible Li-ion storage, the material shows a modified lithium reaction mechanism, which has been rationalized by the occurrence of cationic vacancies acting as additional lithium hosting sites within the anatase framework. Finally, the material shows a fast discharging/charging behavior, compared to TiO2, highlighting the benefits of the structural modifications and paving the way for the design of advanced electrode materials, based on a defect mediated mechanism. C1 [Li, Wei; Corradini, Dario; Salanne, Mathieu; Ma, Jiwei; Rollett, Anne-Laure; Julien, Christian; Duttine, Mathieu; Groult, Henri; Dambournet, Damien] Univ Paris 06, Univ Sorbonne, UMR PHENIX 8234, F-75005 Paris, France. [Li, Wei; Corradini, Dario; Salanne, Mathieu; Ma, Jiwei; Rollett, Anne-Laure; Julien, Christian; Duttine, Mathieu; Groult, Henri; Dambournet, Damien] CNRS, UMR PHENLX 8234, F-75005 Paris, France. [Body, Monique; Legein, Christophe] Univ Maine, LUNAM Univ, CNRS, UMR 6283,IMMM, F-72085 Le Mans 9, France. [Chapman, Karena W.; Chupas, Peter J.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Zhagib, Karim] Inst Rech Hydro Quebec, Energy Storage & Convers, Varennes, PQ J3X 1S1, Canada. [Duttine, Mathieu; Demourgues, Alain] Univ Bordeaux, CNRS, ICMCB, UPR 9048, F-33600 Pessac, France. [Salanne, Mathieu] CNRS, FR 3459, Reseau Stockage Electrochim Energie RS2E, F-80039 Amiens, France. RP Dambournet, D (reprint author), Univ Paris 06, Univ Sorbonne, UMR PHENIX 8234, F-75005 Paris, France. EM damien.dambournet@upmc.fr RI Legein, Christophe/B-3553-2008; Salanne, Mathieu /F-4029-2014; Body, Monique/C-4720-2013 OI Legein, Christophe/0000-0001-7426-8817; Salanne, Mathieu /0000-0002-1753-491X; Body, Monique/0000-0002-5895-3731 FU European Union under REA [321879]; Hydro-Quebec; UPMC; U.S. DOE [DE-AC02-06CH11357] FX The research leading to these results has received funding from the People Programme (Marie Curie Actions) of the European Union's Seventh Framework Programme (No. FP7/2007-2013), under REA Grant Agreement No. [321879] (FLUOSYNES). We also thank Hydro-Quebec and UPMC for support. C. Labrugere and S. Casale are acknowledged for XPS and HRTEM measurements. The work done at the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 41 TC 7 Z9 8 U1 7 U2 44 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUL 28 PY 2015 VL 27 IS 14 BP 5014 EP 5019 DI 10.1021/acs.chemmater.5b01407 PG 6 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CO0EN UT WOS:000358823000016 ER PT J AU Uberuaga, BP Pilania, G AF Uberuaga, Bias Pedro Pilania, Ghanshyam TI Effect of Cation Ordering on Oxygen Vacancy Diffusion Pathways in Double Perovskites SO CHEMISTRY OF MATERIALS LA English DT Article ID MICROWAVE DIELECTRIC-PROPERTIES; A-SITE; MOLECULAR-DYNAMICS; SOLID-SOLUTIONS; FUEL-CELLS; OXIDE; SYSTEM; CHEMISTRY; CONDUCTIVITY; MECHANISMS AB Perovskite structured oxides (ABO(3)) are attractive for a number of technological applications, including as superionics because of the high oxygen conductivities they exhibit. Double perovskites (AA'BB'O-6) provide even more flexibility for tailoring properties: Using accelerated molecular dynamics, we examine the role of cation ordering on oxygen vacancy mobility in one model double perovskite SrLaTiAlO6. We find that the mobility of the vacancy is very sensitive to the cation ordering, with a migration energy that vanes from 0.6 to 2.7 eV. In the extreme cases, the mobility is both higher and lower than either of the two end member single perovskites. Further, the nature of oxygen vacancy diffusion, whether one-dimensional, two-dimensional, or three-dimensional, also varies with cation ordering. We correlate the dependence of oxygen mobility on cation structure to: the distribution of Ti4+ cations, which provide unfavorable environments for the positively charged oxygen vacancy. Our results demonstrate the potential of using tailored double perovskite structures to precisely control the behavior of oxygen vacancies in these materials. C1 [Uberuaga, Bias Pedro; Pilania, Ghanshyam] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. RP Uberuaga, BP (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. EM blas@lanl.gov OI Pilania, Ghanshyam/0000-0003-4460-1572 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; National Nuclear Security Administration of the U.S. DOE [DE-AC52-06NA25396]; LANL LDRD program FX This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. DOE under contract DE-AC52-06NA25396. G.P. acknowledges support from the LANL LDRD program. NR 55 TC 7 Z9 7 U1 13 U2 57 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUL 28 PY 2015 VL 27 IS 14 BP 5020 EP 5026 DI 10.1021/acs.chemmater.5b01474 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CO0EN UT WOS:000358823000017 ER PT J AU Yan, JH Liu, XB Yao, M Wang, XF Wafle, TK Li, BY AF Yan, Jianhua Liu, Xingbo Yao, Meng Wang, Xianfeng Wafle, Trina K. Li, Bingyun TI Long-Life, High-Efficiency Lithium-Sulfur Battery from a Nanoassembled Cathode SO CHEMISTRY OF MATERIALS LA English DT Article ID LIQUID ELECTROLYTE; ENERGY-STORAGE; ION BATTERIES; CYCLE LIFE; PERFORMANCE; NANOTUBES; MECHANISM; CAPACITY AB Lithium-sulfur (Li-S) batteries suffer from major problems including poor cycle performance and low efficiency, mainly due to the high solubility of intermediate polysulfides and their side-reactions with the Li-anode. Here, we report the development of advanced, multilayered, sulfur cathodes composed of alternately arranged, negatively charged S-carbon nanotube layers and positively charged S-polyaniline layers that effectively immobilize polysulfides and reduce polysulfide migration onto the Li-anode. The use of a layer-by-layer nanoassembly technique leads to a binder-free, three-dimensional porous cathode via electrostatic attraction and enables the fabrication of Li-S cells with remarkably improved performance including a long cycle life exceeding 600 cycles and a high Coulombic efficiency of 97.5% at the 1 C rate. Moreover, these Li-S cells have presented a high-rate response up to 2.5 C with high sulfur utilization (a reversible capacity of 1100 mAhg(-1), 900 mAhg(-1), 700 mAhg(-1), and 450 mAhg(-1) of sulfur at 0.3, 0.6, 1, and 2.5 C rates, respectively). The results provide important progress toward the understanding of the role of multilayered cathodes and the realization of high-efficiency and long-term service life for Li-S batteries. C1 [Yan, Jianhua; Wang, Xianfeng; Li, Bingyun] W Virginia Univ, Biomat Bioengn & Nanotechnol Lab, Morgantown, WV 26506 USA. [Yan, Jianhua; Liu, Xingbo; Yao, Meng] W Virginia Univ, Dept Mech & Aerosp Engn, Morgantown, WV 26506 USA. [Wafle, Trina K.] W Virginia Univ, Natl Res Ctr Coal & Energy, Morgantown, WV 26506 USA. [Li, Bingyun] Reg Univ Alliance NETL RUA, Natl Energy Technol Lab, Morgantown, WV 26506 USA. RP Li, BY (reprint author), W Virginia Univ, Biomat Bioengn & Nanotechnol Lab, Morgantown, WV 26506 USA. EM bili@hsc.wvu.edu FU Research Challenge Grant of the West Virginia Higher Education Policy Commission Division of Science and Research; West Virginia Higher Education Policy Commission Division of Science and Research FX This work was funded by a Research Challenge Grant of the West Virginia Higher Education Policy Commission Division of Science and Research. The authors acknowledge use of the West Virginia University (WVU) Shared Research Facilities and financial support from West Virginia Higher Education Policy Commission Division of Science and Research. We appreciate the assistance of Weiqiang Ding, Ph.D., in collecting XPS, XRD, and FTIR data and Marcela Redigolo, Ph.D., in collecting SEM and EDS figures. We thank Jie Xiao, Ph.D., for discussions. NR 45 TC 12 Z9 12 U1 10 U2 95 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUL 28 PY 2015 VL 27 IS 14 BP 5080 EP 5087 DI 10.1021/acs.chemmater.5b01780 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CO0EN UT WOS:000358823000025 ER PT J AU Bhatt, MP Thelen, JL Balsara, NP AF Bhatt, Mahesh P. Thelen, Jacob L. Balsara, Nitash P. TI Effect of Copolymer Composition on Electronic Conductivity of Electrochemically Oxidized Poly(3-hexylthiophene)-b-poly(ethylene oxide) Block Copolymers SO CHEMISTRY OF MATERIALS LA English DT Article ID LIGHT-EMITTING-DIODES; THIN-FILM TRANSISTORS; LITHIUM BATTERY ELECTRODES; FIELD-EFFECT TRANSISTORS; BY-LAYER ELECTRODES; HYBRID SOLAR-CELLS; CONJUGATED POLYMERS; MOLECULAR-WEIGHT; PHOTOVOLTAIC APPLICATIONS; CHARGE-TRANSPORT AB This is a study of the effect of copolymer composition on the electronic conductivity of poly(3-hexylthiophene)-b-poly(ethylene oxide) (P3HT-b-PEO) block copolymers. A wide variety of P3HT-b-PEO block copolymers with P3HT volume fraction ranging from 0.28 to 0.86 were synthesized. Lithium bis(trifluoromethanesulfonyl) imide (LiTFSI) salt was added to the P3HT-b-PEO copolymers to enable electrochemical oxidation. Three terminal electrochemical cells were used to oxidize the P3HT microphase; the two outer electrodes were used to oxidize P3HT, while a nickel mesh located within the P3HT-b-PEO enabled measurement of electronic conductivity by ac impedance. Symmetric block copolymers with P3HT volume fractions in the vicinity of 0.5 exhibited the highest electronic conductivity in the oxidized state. The symmetric copolymers also exhibited the highest crystallinity. The intrinsic conductivity of oxidized P3HT microphases increases exponentially with increasing crystallinity. C1 [Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Bhatt, Mahesh P.; Thelen, Jacob L.; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Bhatt, Mahesh P.; Thelen, Jacob L.; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, JCESR, Berkeley, CA 94720 USA. [Bhatt, Mahesh P.; Thelen, Jacob L.; Balsara, Nitash P.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. RP Balsara, NP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM nbalsara@berkeley.edu FU Joint Center for Energy Storage Research, an Energy Innovation Hub - U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES); DOE, Office of Science, BES; Office of Vehicle Technologies of the U.S. Department of Energy under the Batteries for Advanced Transportation Technologies (BATT) Program [DE-AC02-05CH11231]; DOE, Office of Science, BES [DE-AC02-11231] FX This work was primarily supported as part of the Joint Center for Energy Storage Research, an Energy Innovation Hub funded by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES). X-ray scattering research at the Advanced Light Source was supported by DOE, Office of Science, BES. The electrochemical testing equipment was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy under Contract DE-AC02-05CH11231 under the Batteries for Advanced Transportation Technologies (BATT) Program. Work at the Molecular Foundry, Lawrence Berkeley National Laboratory was supported by DOE, Office of Science, BES under Contract DE-AC02-11231. NR 64 TC 3 Z9 3 U1 9 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUL 28 PY 2015 VL 27 IS 14 BP 5141 EP 5148 DI 10.1021/acs.chemmater.5b02085 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CO0EN UT WOS:000358823000033 ER PT J AU Babakiray, S Johnson, TA Borisov, P Holcomb, MB Lederman, D Marcus, MA Tarafder, K AF Babakiray, Sercan Johnson, Trent A. Borisov, Pavel Holcomb, Mikel B. Lederman, David Marcus, Matthew A. Tarafder, Kartick TI Structural properties of Bi2-xMnxSe3 thin films grown via molecular beam epitaxy SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID RAY PHOTOELECTRON-SPECTRA; TOPOLOGICAL INSULATORS; BI2SE3; SPECTROSCOPY; REFINEMENT; PARAMETERS; MANGANESE; CRYSTAL; SURFACE; PHASE AB The effects of Mn doping on the structural properties of the topological insulator Bi2Se3 in thin film form were studied in samples grown via molecular beam epitaxy. Extended x-ray absorption fine structure measurements, supported by density functional theory calculations, indicate that preferential incorporation occurs substitutionally in Bi sites across the entire film volume. This finding is consistent with x-ray diffraction measurements which show that the out of plane lattice constant expands while the in plane lattice constant contracts as the Mn concentration is increased. X-ray photoelectron spectroscopy indicates that the Mn valency is 2+ and that the Mn bonding is similar to that in MnSe. The expansion along the out of plane direction is most likely due to weakening of the Van der Waals interactions between adjacent Se planes. Transport measurements are consistent with this Mn 2+ substitution of Bi sites if additional structural defects induced by this substitution are taken into account. (C) 2015 AIP Publishing LLC. C1 [Babakiray, Sercan; Johnson, Trent A.; Borisov, Pavel; Holcomb, Mikel B.; Lederman, David] W Virginia Univ, Dept Phys & Astron, Morgantown, WV 26506 USA. [Marcus, Matthew A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Tarafder, Kartick] Dept Phys, Secunderabad 500078, Andhra Pradesh, India. RP Lederman, D (reprint author), W Virginia Univ, Dept Phys & Astron, Morgantown, WV 26506 USA. EM david.lederman@mail.wvu.edu RI Borisov, Pavel/A-6218-2015 OI Borisov, Pavel/0000-0003-1464-6999 FU West Virginia Higher Education Policy Commission; WVU Shared Research Facilities; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank F. Bridges for help with the interpretation of the EXAFS data and Y. Glinka and T. Stanescu for useful discussions regarding the transport data. This work was supported at WVU by a Research Challenge Grant from the West Virginia Higher Education Policy Commission and by the WVU Shared Research Facilities. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 48 TC 1 Z9 1 U1 5 U2 32 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 28 PY 2015 VL 118 IS 4 AR 045302 DI 10.1063/1.4927171 PG 7 WC Physics, Applied SC Physics GA CO1PR UT WOS:000358928000060 ER PT J AU Diwakar, PK Harilal, SS Phillips, MC Hassanein, A AF Diwakar, P. K. Harilal, S. S. Phillips, M. C. Hassanein, A. TI Characterization of ultrafast laser-ablation plasma plumes at various Ar ambient pressures SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID INDUCED BREAKDOWN SPECTROSCOPY; OPTICAL-EMISSION; NANOPARTICLE GENERATION; EXPANSION DYNAMICS; HIGH-VACUUM; GAS; NANOSECOND; EFFICIENCY; INTENSITY; METALS AB Recently, we reported morphological changes in ultrafast laser ablation plumes in varying ambient pressures [Diwakar et al., J. Appl. Phys. 116, 133301 (2014)]. In this paper, we report the emission features of fs laser ablated brass plasma plumes at various Ar background pressure levels ranging from vacuum to atmospheric conditions and correlated to changes in plume morphology. Spatially resolved wavelength dispersed images of the plume were recorded for characterizing the spectral features at various pressure levels and also used for obtaining spatial distribution of Cu I and Zn I species in the plume, signal-to-noise ratios, and fundamental parameters of the plasma, specifically temperature and density. The spatial evolution of plasma temperature and density showed significant changes at various ambient pressure levels; these results were correlated to morphological changes seen in the plume images. Optical time-of-flight profiles were used to study time evolution of various species in the plume and indicated oscillations of ablation plumes at intermediate pressure levels. Possible mechanisms for observed changes in plume shape, optical emission intensity, and dual peak structures in time-of-flight profiles are discussed. (C) 2015 AIP Publishing LLC. C1 [Diwakar, P. K.; Hassanein, A.] Purdue Univ, Sch Nucl Engn, Ctr Mat Extreme Environm, W Lafayette, IN 47907 USA. [Harilal, S. S.; Phillips, M. C.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Diwakar, PK (reprint author), Purdue Univ, Sch Nucl Engn, Ctr Mat Extreme Environm, W Lafayette, IN 47907 USA. RI Harilal, Sivanandan/B-5438-2014 OI Harilal, Sivanandan/0000-0003-2266-7976 FU DOE/NNSA Office of Nonproliferation and Verification Research and Development [NA-22]; U.S. National Science Foundation, PIRE project; U.S. Department of Energy [DE-AC05-76RL01830] FX This work was supported partly by the DOE/NNSA Office of Nonproliferation and Verification Research and Development (NA-22) and U.S. National Science Foundation, PIRE project. Pacific Northwest National Laboratory is a multi-program national laboratory operated by Battelle for the U.S. Department of Energy under Contract No. DE-AC05-76RL01830. NR 49 TC 2 Z9 2 U1 3 U2 27 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 28 PY 2015 VL 118 IS 4 AR 043305 DI 10.1063/1.4927625 PG 9 WC Physics, Applied SC Physics GA CO1PR UT WOS:000358928000015 ER PT J AU Hartig, KC Colgan, J Kilcrease, DP Barefield, J Jovanovic, I AF Hartig, K. C. Colgan, J. Kilcrease, D. P. Barefield, J. E., II Jovanovic, I. TI Laser-induced breakdown spectroscopy using mid-infrared femtosecond pulses SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID COPPER-BASED-ALLOYS; INDUCED PLASMA; WAVELENGTH DEPENDENCE; ELEMENTAL ANALYSIS; STEEL SAMPLES; LIBS; TEMPERATURE; SPECTRA AB We report on a laser-induced breakdown spectroscopy (LIBS) experiment driven by mid-infrared (2.05-mu m) fs pulses, in which time-resolved emission spectra of copper were studied. Ab-initio modeling is consistent with the results of new fs measurements at 2.05 mu m and traditional 800-nm fs-LIBS. Ablation by mid-infrared fs pulses results in a plasma with a lower plasma density and temperature compared to fs-LIBS performed at shorter laser wavelength. LIBS driven by mid-infrared fs pulses results in a signal-to-background ratio similar to 50% greater and a signal-to-noise ratio similar to 40% lower than fs-LIBS at near-infrared laser wavelength. (C) 2015 AIP Publishing LLC. C1 [Hartig, K. C.; Jovanovic, I.] Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16802 USA. [Hartig, K. C.; Barefield, J. E., II] Los Alamos Natl Lab, Chem Diagnost & Engn, Los Alamos, NM 87545 USA. [Colgan, J.; Kilcrease, D. P.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Hartig, KC (reprint author), Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16802 USA. EM ijovanovic@psu.edu OI Barefield, James/0000-0001-8674-6214; Kilcrease, David/0000-0002-2319-5934 FU U.S. Department of Homeland Security [2012.05 DN-130-NF0001]; National Nuclear Security Administration; G.T. Seaborg Institute, Chemistry Division, Theoretical Division; Laboratory Directed Research and Development Program at Los Alamos National Lab FX This material was supported by the U.S. Department of Homeland Security under Grant Award No. 2012.05 DN-130-NF0001 and the National Nuclear Security Administration. Additional support was provided by the G.T. Seaborg Institute, Chemistry Division, Theoretical Division, and the Laboratory Directed Research and Development Program at Los Alamos National Lab. We would also like to acknowledge Annie Hopkins and Scott Wandel for their assistance with the experimental setup, and we thank the anonymous referees for helpful suggestions. NR 41 TC 2 Z9 2 U1 1 U2 14 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 28 PY 2015 VL 118 IS 4 AR 043107 DI 10.1063/1.4927624 PG 6 WC Physics, Applied SC Physics GA CO1PR UT WOS:000358928000008 ER PT J AU Kanevce, A Kuciauskas, D Levi, DH Motz, AMA Johnston, SW AF Kanevce, Ana Kuciauskas, Darius Levi, Dean H. Motz, Alyssa M. Allende Johnston, Steven W. TI Two dimensional numerical simulations of carrier dynamics during time-resolved photoluminescence decays in two-photon microscopy measurements in semiconductors SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID DIFFUSION-LENGTH; SOLAR-CELLS; LIFETIME; CDTE; GAAS; RECOMBINATION; SILICON AB We use two-dimensional numerical simulations to analyze high spatial resolution time-resolved spectroscopy data. This analysis is applied to two-photon excitation time-resolved photoluminescence (2PE-TRPL) but is broadly applicable to all microscopic time-resolved techniques. By solving time-dependent drift-diffusion equations, we gain insight into carrier dynamics and transport characteristics. Accurate understanding of measurement results establishes the limits and potential of the measurement and enhances its value as a characterization method. Diffusion of carriers outside of the collection volume can have a significant impact on the measured decay but can also provide an estimate of carrier mobility as well as lifetime. In addition to material parameters, the experimental conditions, such as spot size and injection level, can impact the measurement results. Although small spot size provides better resolution, it also increases the impact of diffusion on the decay; if the spot size is much smaller than the diffusion length, it impacts the entire decay. By reproducing experimental 2PE-TRPL decays, the simulations determine the bulk carrier lifetime from the data. The analysis is applied to single-crystal and heteroepitaxial CdTe, material important for solar cells, but it is also applicable to other semiconductors where carrier diffusion from the excitation volume could affect experimental measurements. C1 [Kanevce, Ana; Kuciauskas, Darius; Levi, Dean H.; Motz, Alyssa M. Allende; Johnston, Steven W.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Motz, Alyssa M. Allende] Colorado Sch Mines, Golden, CO 80401 USA. RP Kanevce, A (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. OI Kuciauskas, Darius/0000-0001-8091-5718 FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory FX This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. NR 29 TC 4 Z9 4 U1 3 U2 18 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 28 PY 2015 VL 118 IS 4 AR 045709 DI 10.1063/1.4927299 PG 7 WC Physics, Applied SC Physics GA CO1PR UT WOS:000358928000076 ER PT J AU Li, YH Xia, Q Guo, SK Ma, ZQ Gao, YB Gong, XG Wei, SH AF Li, Yong-Hua Xia, Qin Guo, Shu-Kuan Ma, Zhong-Quan Gao, Yu-Bo Gong, Xin-Gao Wei, Su-Huai TI O-O bonding stabilized zinc vacancy as origin of p-type doping on Sigma 7 ZnO grain boundary SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID AUGMENTED-WAVE METHOD; ENERGY; SEMICONDUCTORS; EPITAXY; PLANE; OXIDE AB Using density functional theory calculations, we investigate different defects on ZnO Sigma 7 (12 (3) over bar0) grain boundary. We find that on this low energy grain boundary, the formation energy of V-Zn and O-i are drastically reduced by the formation of O-O bonds and V-Zn has lower formation energy than O-i. Interaction of defects on grain boundary can form new defect bands, and the calculated impurity band maximum is only 0.1 eV below V-Zn unoccupied levels. Therefore, we believe that the p-type layers observed in experiments near the Z(nO) grain boundaries can be attributed to V-Zn. (C) 2015 AIP Publishing LLC. C1 [Li, Yong-Hua; Xia, Qin; Guo, Shu-Kuan; Ma, Zhong-Quan; Gao, Yu-Bo] Shanghai Univ, Dept Phys, SHU Solar Energy R&D Lab, Shanghai 200444, Peoples R China. [Gong, Xin-Gao] Fudan Univ, Minist Educ, Key Lab Computat Phys Sci, State Key Lab Surface Phys, Shanghai 200433, Peoples R China. [Gong, Xin-Gao] Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China. [Wei, Su-Huai] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Li, YH (reprint author), Shanghai Univ, Dept Phys, SHU Solar Energy R&D Lab, Shanghai 200444, Peoples R China. EM lyhua@shu.edu.cn RI gong, xingao/D-6532-2011 FU Natural Science Foundation of China [11004128, 61274067]; U.S. Department of Energy [DE-AC36-08GO28308] FX The work at Shanghai University was supported by the Natural Science Foundation of China (Grant Nos. 11004128 and 61274067). Computing resources was provided by the High Performance Computing Center of Shanghai University. The Work at NREL was supported by the U.S. Department of Energy under Contract No. DE-AC36-08GO28308. NR 44 TC 1 Z9 1 U1 3 U2 17 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 28 PY 2015 VL 118 IS 4 AR 045708 DI 10.1063/1.4927295 PG 5 WC Physics, Applied SC Physics GA CO1PR UT WOS:000358928000075 ER PT J AU Martinello, M Checchin, M Grassellino, A Crawford, AC Melnychuk, O Romanenko, A Sergatskov, DA AF Martinello, M. Checchin, M. Grassellino, A. Crawford, A. C. Melnychuk, O. Romanenko, A. Sergatskov, D. A. TI Magnetic flux studies in horizontally cooled elliptical superconducting cavities SO JOURNAL OF APPLIED PHYSICS LA English DT Article AB Previous studies on magnetic flux expulsion as a function of cooldown procedures for elliptical superconducting radio frequency (SRF) niobium cavities showed that when the cavity beam axis is placed parallel to the helium cooling flow and sufficiently large thermal gradients are achieved, all magnetic flux could be expelled and very low residual resistance could be achieved. In this paper, we investigate flux trapping for the case of resonators positioned perpendicularly to the helium cooling flow, which is more representative of how SRF cavities are cooled in accelerators and for different directions of the applied magnetic field surrounding the resonator. We show that different field components have a different impact on the surface resistance, and several parameters have to be considered to fully understand the flux dynamics. A newly discovered phenomenon of concentration of flux lines at the cavity top leading to temperature rise at the cavity equator is presented. (C) 2015 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported License. C1 [Martinello, M.; Checchin, M.; Grassellino, A.; Crawford, A. C.; Melnychuk, O.; Romanenko, A.; Sergatskov, D. A.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Martinello, M.; Checchin, M.] IIT, Dept Phys, Chicago, IL 60616 USA. RP Martinello, M (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM mmartine@fnal.gov; annag@fnal.gov OI Melnychuk, Oleksandr/0000-0002-2089-8685; Crawford, Anthony C./0000-0003-4867-0495 FU U.S. Department of Energy, Offices of High Energy Physics and Basic Energy Science, via the LCLS-II High Q Program; United States Department of Energy [DE-AC02-07CH11359] FX This work was supported by the U.S. Department of Energy, Offices of High Energy Physics and Basic Energy Science, via the LCLS-II High Q Program. Authors would like to acknowledge technical assistance of A. Rowe, M. Merio, B. Golden, J. Rife, A. Diaz, D. Burk, B. Squires, G. Kirschbaum, D. Marks, and R. Ward for cavity preparation, testing, and for cryogenics support. We acknowledge for fruitful discussions and support of the experiment by M. Ross, R. Stanek, and H. Padamsee. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. NR 11 TC 6 Z9 6 U1 2 U2 2 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 28 PY 2015 VL 118 IS 4 AR 044505 DI 10.1063/1.4927519 PG 6 WC Physics, Applied SC Physics GA CO1PR UT WOS:000358928000042 ER PT J AU Armas-Perez, JC Londono-Hurtado, A Guzman, O Hernandez-Ortiz, JP de Pablo, JJ AF Armas-Perez, Julio C. Londono-Hurtado, Alejandro Guzman, Orlando Hernandez-Ortiz, Juan P. de Pablo, Juan J. TI Theoretically informed Monte Carlo simulation of liquid crystals by sampling of alignment-tensor fields SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID DROPLETS; NANOPARTICLES; TRANSITIONS; PARTICLE; ENERGY; CELLS; CONFIGURATIONS; INSTABILITY; INTERFACES; THICKNESS AB A theoretically informed coarse-grained Monte Carlo method is proposed for studying liquid crystals. The free energy functional of the system is described in the framework of the Landau-de Gennes formalism. The alignment field and its gradients are approximated by finite differences, and the free energy is minimized through a stochastic sampling technique. The validity of the proposed method is established by comparing the results of the proposed approach to those of traditional free energy minimization techniques. Its usefulness is illustrated in the context of three systems, namely, a nematic liquid crystal confined in a slit channel, a nematic liquid crystal droplet, and a chiral liquid crystal in the bulk. It is found that for systems that exhibit multiple metastable morphologies, the proposed Monte Carlo method is generally able to identify lower free energy states that are often missed by traditional approaches. Importantly, the Monte Carlo method identifies such states from random initial configurations, thereby obviating the need for educated initial guesses that can be difficult to formulate. (C) 2015 AIP Publishing LLC. C1 [Armas-Perez, Julio C.; Londono-Hurtado, Alejandro; Hernandez-Ortiz, Juan P.; de Pablo, Juan J.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. [Guzman, Orlando] Univ Autonoma Metropolitana, Dept Fis, Iztapalapa 09340, DF, Mexico. [Hernandez-Ortiz, Juan P.] Univ Nacl Colombia, Dept Mat & Minerales, Sede Medellin, Medellin, Colombia. [de Pablo, Juan J.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Armas-Perez, JC (reprint author), Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. EM depablo@uchicago.edu OI Hernandez-Ortiz, Juan/0000-0003-0404-9947 FU Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division, Biomaterials Program [DE-SC0004025]; Argonne National Laboratory; CONACYT [186166, 203840]; Universidad Nacional de Colombia; COLCIENCIAS [110-165-843-748]; [DE-AC02-06CH11357] FX The authors acknowledge support from the Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division, Biomaterials Program under Grant No. DE-SC0004025. Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. An award of computer time was provided by the Innovative and Novel Computational Impact on Theory and Experiment (INCITE) program of the Argonne Leadership Computing Facility at Argonne National Laboratory. Additional development work was performed using the Argonne Laboratory Resource Computing Center (LCRC) and The University of Chicago Midway cluster. J.C.A.-P. is thankful to CONACYT for Postdoctoral Fellowships Nos. 186166 and 203840. J.P.H.-O. is grateful to funding provided by the Universidad Nacional de Colombia Ph.D. grant and COLCIENCIAS under the Contract No. 110-165-843-748, "Patrimonio Autonomo Fondo Nacional de Financiamiento para la Ciencia, Tecnologia y la Innovacion Francisco Jose de Caldas." NR 68 TC 4 Z9 4 U1 5 U2 19 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUL 28 PY 2015 VL 143 IS 4 AR 044107 DI 10.1063/1.4926790 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CO1QC UT WOS:000358929100013 PM 26233107 ER PT J AU Johnson, PM Sears, TJ AF Johnson, Philip M. Sears, Trevor J. TI Photo-assisted intersystem crossing: The predominant triplet formation mechanism in some isolated polycyclic aromatic molecules excited with pulsed lasers SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID MULTIPHOTON IONIZATION SPECTROSCOPY; GROUND CATIONIC STATE; PHOTOELECTRON-SPECTROSCOPY; VACUUM-ULTRAVIOLET; RADIATIONLESS TRANSITIONS; ULTRAFAST DYNAMICS; SUPERSONIC BEAM; BENZENE; NAPHTHALENE; ABSORPTION AB Naphthalene, anthracene, and phenanthrene are shown to have very long-lived triplet lifetimes when the isolated molecules are excited with nanosecond pulsed lasers resonant with the lowest singlet state. For naphthalene, triplet state populations are created only during the laser pulse, excluding the possibility of normal intersystem crossing at the one photon level, and all molecules have triplet lifetimes greater than hundreds of microseconds, similar to the behavior previously reported for phenylacetylene. Although containing 7-12 thousand cm(-1) of vibrational energy, the triplet molecules have ionization thresholds appropriate to vibrationless T1 states. The laser power dependences (slopes of log-log power plots) of the excited singlet and triplet populations are about 0.7 for naphthalene and about 0.5 for anthracene. Kinetic modeling of the power dependences successfully reproduces the experimental results and suggests that the triplet formation mechanism involves an enhanced spin orbit coupling caused by sigma character in states at the 2-photon level. Symmetry adapted cluster-configuration interaction calculations produced excited state absorption spectra to provide guidance for estimating kinetic rates and the sigma character present in higher electronic states. It is concluded that higher excited state populations are significant when larger molecules are excited with pulsed lasers and need to be taken into account whenever discussing the molecular photodynamics (C) 2015 AIP Publishing LLC. C1 [Johnson, Philip M.; Sears, Trevor J.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Sears, Trevor J.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Johnson, PM (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. EM Philip.johnson@stonybrook.edu RI Sears, Trevor/B-5990-2013 OI Sears, Trevor/0000-0002-5559-0154 FU U.S. Department of Energy [DE-AC02-98CH10886, DE-SC00012704]; U.S. Department of Energy by its Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences FX We gratefully valuable discussions with Professor Thomas Weinacht concerning the dynamics of molecular excited states. T.J.S. is supported at Brookhaven National Laboratory under Contract Nos. DE-AC02-98CH10886 and DE-SC00012704 with the U.S. Department of Energy and supported by its Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences. NR 60 TC 0 Z9 0 U1 5 U2 19 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUL 28 PY 2015 VL 143 IS 4 AR 044305 DI 10.1063/1.4926925 PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CO1QC UT WOS:000358929100033 PM 26233127 ER PT J AU Tkachenko, AV Maslov, S AF Tkachenko, Alexei V. Maslov, Sergei TI Spontaneous emergence of autocatalytic information-coding polymers SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID RNA WORLD; ORIGIN; MODEL; REPLICATION; LIFE; SETS AB Self-replicating systems based on information-coding polymers are of crucial importance in biology. They also recently emerged as a paradigm in material design on nano-and micro-scales. We present a general theoretical and numerical analysis of the problem of spontaneous emergence of autocatalysis for heteropolymers capable of template-assisted ligation driven by cyclic changes in the environment. Our central result is the existence of the first order transition between the regime dominated by free monomers and that with a self-sustaining population of sufficiently long chains. We provide a simple, mathematically tractable model supported by numerical simulations, which predicts the distribution of chain lengths and the onset of autocatalysis in terms of the overall monomer concentration and two fundamental rate constants. Another key result of our study is the emergence of the kinetically limited optimal overlap length between a template and each of its two substrates. The template-assisted ligation allows for heritable transmission of the information encoded in chain sequences thus opening up the possibility of long-term memory and evolvability in such systems. (C) 2015 AIP Publishing LLC. C1 [Tkachenko, Alexei V.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Maslov, Sergei] Brookhaven Natl Lab, Biol Environm & Climate Sci Dept, Upton, NY 11973 USA. [Maslov, Sergei] Univ Illinois, Dept Bioengn, Urbana, IL 61801 USA. RP Tkachenko, AV (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. EM oleksiyt@bnl.gov; ssmaslov@gmail.com RI Tkachenko, Alexei/I-9040-2012; OI Tkachenko, Alexei/0000-0003-1291-243X; Maslov, Sergei/0000-0002-3701-492X FU Center for Functional Nanomaterials, U.S. DOE Office of Science User Facility, at Brookhaven National Laboratory [DE-SC0012704]; U.S. Department of Energy, Office of Biological Research [PM-031] FX This research used resources of the Center for Functional Nanomaterials, which is a U.S. DOE Office of Science User Facility, at Brookhaven National Laboratory under Contract No. DE-SC0012704. Work at Biosciences Department was supported by U.S. Department of Energy, Office of Biological Research, Grant No. PM-031. We would like to thank Professor Mark Lukin, Stony Brook University for valuable discussions. NR 18 TC 1 Z9 1 U1 0 U2 8 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUL 28 PY 2015 VL 143 IS 4 AR 045102 DI 10.1063/1.4922545 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CO1QC UT WOS:000358929100071 PM 26233165 ER PT J AU Whitmer, JK Fluitt, AM Antony, L Qin, J McGovern, M de Pablo, JJ AF Whitmer, Jonathan K. Fluitt, Aaron M. Antony, Lucas Qin, Jian McGovern, Michael de Pablo, Juan J. TI Sculpting bespoke mountains: Determining free energies with basis expansions SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID DENSITY-OF-STATES; MONTE-CARLO METHOD; MOLECULAR-DYNAMICS; LIQUID-CRYSTAL; MEAN FORCE; SIMULATION; ALGORITHM; METADYNAMICS; EFFICIENT; EQUALITY AB The intriguing behavior of a wide variety of physical systems, ranging from amorphous solids or glasses to proteins, is a direct manifestation of underlying free energy landscapes riddled with local minima separated by large barriers. Exploring such landscapes has arguably become one of statistical physics's great challenges. A new method is proposed here for uniform sampling of rugged free energy surfaces. The method, which relies on special Green's functions to approximate the Dirac delta function, improves significantly on existing simulation techniques by providing a boundary-agnostic approach that is capable of mapping complex features in multidimensional free energy surfaces. The usefulness of the proposed approach is established in the context of a simple model glass former and model proteins, demonstrating improved convergence and accuracy over existing methods. (C) 2015 AIP Publishing LLC. C1 [Whitmer, Jonathan K.] Univ Notre Dame Lac, Dept Chem & Biomol Engn, Notre Dame, IN 46556 USA. [Fluitt, Aaron M.; Antony, Lucas; Qin, Jian; McGovern, Michael; de Pablo, Juan J.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. [Qin, Jian; de Pablo, Juan J.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Whitmer, JK (reprint author), Univ Notre Dame Lac, Dept Chem & Biomol Engn, Notre Dame, IN 46556 USA. OI Antony, Lucas/0000-0003-1933-6500 FU Department of Energy, Basic Energy Sciences, Materials Research Division; University of Notre Dame; National Science Foundation [DGE-0718123]; University of Chicago Research Computing Center; Office of Science of the U.S. Department of Energy [DE-AC02-06CH11357] FX This work is supported by the Department of Energy, Basic Energy Sciences, Materials Research Division. J.K.W. acknowledges support from startup funds at the University of Notre Dame. A.M.F. acknowledges support from the National Science Foundation through Grant No. DGE-0718123. We gratefully acknowledge the computing resources provided on "Fusion," a 320-node computing cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory. We acknowledge the University of Chicago Research Computing Center for use of the Midway cluster and support of this work. An award of computer time was provided by the Innovative and Novel Computational Impact on Theory and Experiment (INCITE) program of the Argonne Leadership Computing Facility at Argonne National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-06CH11357. NR 52 TC 4 Z9 4 U1 3 U2 16 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUL 28 PY 2015 VL 143 IS 4 AR 044101 DI 10.1063/1.4927147 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CO1QC UT WOS:000358929100007 PM 26233101 ER PT J AU Han, LL Xin, HLL Kulinich, SA Yang, LJ Du, XW AF Han, Li-Li Xin, Huolin L. Kulinich, Sergei A. Yang, Li-Jun Du, Xi-Wen TI Hierarchical, Ultrathin Single-Crystal Nanowires of CdS Conveniently Produced in Laser-Induced Thermal Field SO LANGMUIR LA English DT Article ID ORIENTED ATTACHMENT; BRANCHED NANOWIRES; HIGH-QUALITY; GROWTH; HETEROSTRUCTURES; NANOPARTICLES; NANOSTRUCTURES; TRANSFORMATION; PERFORMANCE; GENERATION AB Hierarchical nanowires (HNWs) exhibit unique properties and have wide applications, while often suffering from imperfect structute. Herein, we rep oft a facile strategy toward ultrathin CdS HNWs with monocrystal structure, where a continuous-wave (CW) Nd:YAG laser is,employed to irradiate an oleic acid (OA) solution containing precursors and a light absorber. The high heating rate and large temperature gradient generated by the CW laser lead to the rapid formation of tiny zinc-blende CdS nanocrystals which then line-up into nano:wires with the help of OA molecules. Nett, the nanowires experience a phase transformation from zinc-blende to wurtzite structure, and the transformation-induced stress creates terrates on their surface, which promotes the growth of side branches and eventually results in monocrystal HNWs with an ultrathin diameter of 24 nm. The one-step synthesis of HNWs is conducted in air and completes in just 40 s, thus being very simple and rapid: The prepared CdS HNWs display photocatalytic performance superior to their: nanoparticle counterparts, thus showing promise for catalytic applications in the future. C1 [Han, Li-Li; Yang, Li-Jun; Du, Xi-Wen] Tianjin Univ, Sch Mat Sci & Engn, Tianjin 300072, Peoples R China. [Han, Li-Li; Xin, Huolin L.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Kulinich, Sergei A.] Tokai Univ, Inst Innovat Sci & Technol, Hiratsuka, Kanagawa 2591292, Japan. [Kulinich, Sergei A.] Aston Univ, Aston Inst Photon Technol, Birmingham B4 7ET, W Midlands, England. RP Kulinich, SA (reprint author), Tokai Univ, Inst Innovat Sci & Technol, 4-1-1 Kitakaname, Hiratsuka, Kanagawa 2591292, Japan. EM s_kulinich@yahoo.com; xwdu@tju.edu.cn RI Kulinich, Sergei/B-1887-2008; Xin, Huolin/E-2747-2010; Du, Xi-Wen/A-7347-2011 OI Kulinich, Sergei/0000-0002-1365-9221; Xin, Huolin/0000-0002-6521-868X; FU National Basic Research Program of China [2014CB931703]; Natural Science Foundation of China [51171127, 51102176, 51271129]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0012704] FX This work was supported by the National Basic Research Program of China (2014CB931703) and the Natural Science Foundation of China (Nos. 51171127, 51102176, and 51271129). Research carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory was supported by the U.S. Department of Energy, Office of Basic Energy Sciences under contract no. DE-SC0012704. NR 35 TC 0 Z9 0 U1 5 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD JUL 28 PY 2015 VL 31 IS 29 BP 8162 EP 8167 DI 10.1021/acs.langmuir.5b01923 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CO0EG UT WOS:000358822300030 PM 26154589 ER PT J AU Messinger, RJ Marks, TG Gleiman, SS Milstein, F Chmelka, BF AF Messinger, R. J. Marks, T. G. Gleiman, S. S. Milstein, F. Chmelka, B. F. TI Molecular Origins of Macroscopic Mechanical Properties of Elastomeric Organosiloxane Foams SO MACROMOLECULES LA English DT Article ID NUCLEAR-MAGNETIC-RESONANCE; FILLED SILICONE ELASTOMER; PROTON NMR RELAXATION; MULTIPLE-QUANTUM NMR; NETWORK STRUCTURE; SI-29 NMR; RUBBER; POLYMERS; DYNAMICS; H-1-NMR AB Molecular compositions, structures, interaction, polymer chain dynamics, and Micron-scale cell structures of elastomeric organosiloxane foams have been analyzed and correlated with their macroscopic mechanical properties. Open-cell organosiloxane foams were synthesized within a narrow range of relative densities (+/- 5% relative uncertainty) and with similar micron-scale pore structures, as determined from quantitative analyses of micro-X-ray computed tomography. (MXCT) images. Network cross-linking densities, polymer molecular weights; organic side-chain moieties, and inorganic filler contents were varied systematically, resulting in materials with significantly different mechanical properties. Solid-state single-pulse H-1 and Si-29 magic-angle-spinning (MAS), two-dimensional (2D) Si-29{H-1} hetereonuclear correlation (HETCOR), and transverse H-1 relaxation (T-2) nuclear magnetic resonance (NMR) spectroscopy measurements establish significant differences in molecular and polymer network characteristics that are correlated with the bulk mechanical properties of the organosiloxane foams. These Characteristics include differing extents of polymer cross-linking, concentrations of phenyl side-chain groups, mass fractions of low- to high-molecular-weight cross-linking chains, and polymer chain dynamics. The mechanical properties of the organosiloxane foams are accounted for by the differences in the molecular compositions, structures, and polymer chain dynamics of the foam frameworks, independent of cell microstructures. C1 [Messinger, R. J.; Chmelka, B. F.] Univ Calif Santa Barbara, Dept Chem Engn, Santa Barbara, CA 93106 USA. [Marks, T. G.; Milstein, F.] Univ Calif Santa Barbara, Dept Mech Engn, Santa Barbara, CA 93106 USA. [Gleiman, S. S.] Los Alamos Natl Lab, Inst Multiscale Mat Studies, Los Alamos, NM 87544 USA. RP Chmelka, BF (reprint author), Univ Calif Santa Barbara, Dept Chem Engn, Santa Barbara, CA 93106 USA. EM bradc@engineering.ucsb.edu RI Messinger, Robert/M-2471-2015 OI Messinger, Robert/0000-0002-5537-3870 FU U.S. Department of Energy through the Institute of Multiscale Materials Studies at Los Alamos National Laboratory; U.S. National Science Foundation (NSF) [CHE-0924654]; Warren and Katharine Schlinger Foundation; NSF MRSEC [DMR 1121053] FX The authors thank Dr. Brian Patterson, Dr. Michael Janicke, and Dr. Jerry Hu for assistance with the MXCT, solution-state NMR, and variable-temperature solid-state NMR measurements, respectively, and Prof. Moshe Gottlieb for helpful discussions that initiated these investigations. This work was supported by the U.S. Department of Energy through the Institute of Multiscale Materials Studies at Los Alamos National Laboratory and the U.S. National Science Foundation (NSF) under Grant CHE-0924654. R.J.M. acknowledges the Warren and Katharine Schlinger Foundation for a doctoral fellowship. Solid-state NMR measurements were conducted using the Material Research Laboratory Central Facilities at UCSB, which are supported by the NSF MRSEC Program under Award DMR 1121053. NR 58 TC 4 Z9 4 U1 8 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD JUL 28 PY 2015 VL 48 IS 14 BP 4835 EP 4849 DI 10.1021/acs.macromol.5b00532 PG 15 WC Polymer Science SC Polymer Science GA CO0EQ UT WOS:000358823300008 ER PT J AU Wang, DR Wujcik, KH Teran, AA Balsara, NP AF Wang, Dunyang Rita Wujcik, Kevin H. Teran, Alexander A. Balsara, Nitash P. TI Conductivity of Block Copolymer Electrolytes Containing Lithium Polysulfides SO MACROMOLECULES LA English DT Article ID LI-S BATTERIES; MOLECULAR-WEIGHT; SULFUR BATTERY; POLY(ETHYLENE OXIDE); POLYMER ELECTROLYTES; IONIC-CONDUCTIVITY; SALT; BEHAVIOR; CATHODE; PERFORMANCE AB Lithium-sulfur batteries are attractive due to their high theoretical specific energy, but the dissolution of lithium polysulfide intermediate species formed during discharge results in capacity fade and limited cycle life. In this study we present the first measurements of ionic conductivity of the polysulfides in a nanostructured block copolyrner. The morphology, thermal properties, and the conductivities of polystyrene-b-poly(ethylene oxide) (SEO) containing lithium polysulfides, Li2Sx (x = 4, 8), were studied using small-angle X-ray scattering (SAXS), differential scanning calorimetry (DSC), and ac impedance spectroscopy. We also measured conductivities of mixtures of poly(ethylene oxide) (PEO) and Li2Sx. X-ray absorption spectroscopy was used to confirm the nature of dissolved polysulfides. SAXS measurements on SEO/Li2Sx mixtures indicated that all samples had a lamellar morphology. DSC measurements indicated that SEO/Li2S8 interactions were more favorable than SEO/Li2S4 interactions. The effect of nanostructure on transport of Li2Sx was quantified by calculating a normalized conductivity, which is proportional to the ratio of the conductivity of SEO/Li2Sx to that of the PEO/Li2Sx. The normalized conductivities of both polysulfides peaked at intermediate concentrations. The efficacy of block copolymer electrolytes in Li-S batteries was evaluated by comparing ionic conductivities of polymer electrolytes containing Li2Sx with those containing lithium bis(trifluoromethanesulfonyl)imide (LiTFSI), a common salt used in PEO-based battery electrolytes. The transport of Li2Sx species in SEO is suppressed by factors ranging from 0.4 to 0.04 relative to LiTFSI, depending on x and salt concentration. To our knowledge, this study represents the first systematic investigation of the effect of molecular structure of polymer electrolytes on polysulfide migration. C1 [Wang, Dunyang Rita] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Wujcik, Kevin H.; Teran, Alexander A.; Balsara, Nitash P.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Wujcik, Kevin H.; Teran, Alexander A.; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Wang, Dunyang Rita; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. RP Balsara, NP (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. EM nbalsara@berkeley.edu FU Office of Science, Office of Basic Energy Science, U.S. Department of Energy under the Soft Matter Electron Microscopy Program [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Science, U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515] FX This work was supported by the Office of Science, Office of Basic Energy Science, U.S. Department of Energy, under Contract DE-AC02-05CH11231 under the Soft Matter Electron Microscopy Program. SAXS measurements were carried out at the Advanced Light Source (Lawrence Berkeley National Lab), beamline 7.3.3, supported by the Office of Science, Office of Basic Energy Science, U.S. Department of Energy, under Contract DE-AC02-05CH11231. XAS experiments were carried out at the Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-76SF00515. Elemental analysis is supported by the Microanalytical Laboratory of UC Berkeley, College of Chemistry. The authors gratefully acknowledge Tod Pascal and David Prendergast for providing the simulation results in Figure 1, Elena Kreimer for her assistance in elemental analysis, and Chenhui Zhu of the Advanced Light Source for his help with the X-ray scattering experiments. NR 49 TC 3 Z9 3 U1 12 U2 70 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD JUL 28 PY 2015 VL 48 IS 14 BP 4863 EP 4873 DI 10.1021/acs.macromol.5b00928 PG 11 WC Polymer Science SC Polymer Science GA CO0EQ UT WOS:000358823300010 ER PT J AU Cao, Z Carrillo, JMY Sheiko, SS Dobrynin, AV AF Cao, Zhen Carrillo, Jan-Michael Y. Sheiko, Sergei S. Dobrynin, Andrey V. TI Computer Simulations of Bottle Brushes: From Melts to Soft Networks SO MACROMOLECULES LA English DT Article ID PERSISTENCE LENGTH; NONLINEAR ELASTICITY; LYOTROPIC BEHAVIOR; MOLECULAR-DYNAMICS; NEUTRON-SCATTERING; POLYMER NETWORKS; POLYELECTROLYTES; MACROMOLECULES; CONFORMATION; ELASTOMERS AB Using a combination of Molecular dynamics simulations and analytical calculations, we study dens bottle-brush systems in a melt and network State. Analysis. of our simulation results shows That bottle-brush macromolecules in melt behave as ideal chains with effective Kuhn length b(K). Simulations show that the bottle-brush-induced bending rigidity is due to an entropy decrease caused by redistribution of the side chains upon backbone bending The Kuhn length of the bottle:brushes increases with increasing the side-chain degree of polymerization n(sc) as b(K) proportional to n(sc)(0.46). This model of bottle brush macromolecules is extended to describe mechanical properties of bottle brush networks in linear and nonlinear deformation regimes. In the linear deformation regime, the network shear modulus scales with the degree of polymerization of the side chains as G(0) proportional to (n(sc) + 1)(-1) as long as the ratio of the Kuhn length, b(K), to the size of the fully extended bottle-brush backbone between cross-links, R-max, is smaller than unity, b(K)/R-max << 1. Bottle-brush networks With b(K)/R-max proportional to 1 demonstrate behavior similar to that of networks Of semiflexible chains with G(0) proportional to n(sc)(-0.5). In the nonlinear network deformation regime, the deformation-dependent shear modulus is a universal function of the first strain invariant I-1 and bottle-brush backbone deformation ratio beta describing stretching ability of the bottle-brush backbone between cross-links. C1 [Cao, Zhen; Dobrynin, Andrey V.] Univ Connecticut, Polymer Program, Storrs, CT 06269 USA. [Cao, Zhen; Dobrynin, Andrey V.] Univ Connecticut, Inst Mat Sci, Storrs, CT 06269 USA. [Carrillo, Jan-Michael Y.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Carrillo, Jan-Michael Y.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Sheiko, Sergei S.] Univ N Carolina, Dept Chem, Chapel Hill, NC 27599 USA. RP Dobrynin, AV (reprint author), Univ Connecticut, Polymer Program, Storrs, CT 06269 USA. EM avd@ims.uconn.edu RI Carrillo, Jan-Michael/K-7170-2013; OI Carrillo, Jan-Michael/0000-0001-8774-697X; Dobrynin, Andrey/0000-0002-6484-7409 FU National Science Foundation [DMR-1409710, DMR-1407645, DMR-1436201]; United States Department of Energy [DE-AC04-94AL85000]; Office of Advanced Scientific Computing Research, U.S. Department of Energy; [DE-AC52-06NA25396]; [De-AC05-00OR22725] FX The authors are grateful to the National Science Foundation for the financial support under Grants DMR-1409710, DMR-1407645, and DMR-1436201. This work was performed at the U.S. Department of Energy, Center for Integrated Nano-technologies, at Los Alamos National Laboratory (Contract DE-AC52-06NA25396) and Sandia National Laboratories. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy under Contract DE-AC04-94AL85000. J.-M.Y.C's contribution was sponsored by the Office of Advanced Scientific Computing Research, U.S. Department of Energy, and performed at the Oak Ridge National Laboratory, which is managed by UT-Battelle, LLC, under Contract De-AC05-00OR22725. NR 46 TC 5 Z9 5 U1 4 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD JUL 28 PY 2015 VL 48 IS 14 BP 5006 EP 5015 DI 10.1021/acs.macromol.5b00682 PG 10 WC Polymer Science SC Polymer Science GA CO0EQ UT WOS:000358823300026 ER PT J AU Forlani, G Bertazzini, M Zarattini, M Funck, D Ruszkowski, M Nocek, B AF Forlani, Giuseppe Bertazzini, Michele Zarattini, Marco Funck, Dietmar Ruszkowski, Milosz Nocek, Boguslaw TI Functional properties and structural characterization of rice delta(1)-pyrroline-5-carboxylate reductase SO FRONTIERS IN PLANT SCIENCE LA English DT Article DE proline synthesis; P5C reductase; enzyme properties; substrate ambiguity; cation and anion effects; product inhibition; oligomeric structure ID ORNITHINE-DELTA-AMINOTRANSFERASE; PLANT P5C REDUCTASE; PYRROLINE-5-CARBOXYLATE REDUCTASE; PROLINE SYNTHESIS; HYPERSENSITIVE RESPONSE; STREPTOCOCCUS-PYOGENES; ARABIDOPSIS-THALIANA; CULTURED-CELLS; DEHYDROGENASE; STRESS AB The majority of plant species accumulate high intracellular levels of proline to cope with hyperosmotic stress conditions. Proline synthesis from glutamate is tightly regulated at both the transcriptional and the translational levels, yet little is known about the mechanisms for post-translational regulation of the enzymatic activities involved. The gene coding in rice (Oryza sativa L.) for delta(1)-pyrroline-5-carboxylate (P5C) reductase, the enzyme that catalyzes the second and final step in this pathway, was isolated and expressed in Escherichia coli. The structural and functional properties of the affinity-purified protein were characterized. As for most species, rice P5C reductase was able to use in vitro either NADH or NADPH as the electron donor. However, strikingly different effects of cations and anions were found depending on the pyridine nucleotide used, namely inhibition of NADH-dependent activity and stimulation of NADPH-dependent activity. Moreover, physiological concentrations of proline and NADP(+) were strongly inhibitory for the NADH-dependent reaction, whereas the NADPH-dependent activity was mildly affected. Our results suggest that only NADPH may be used in vivo and that stress-dependent variations in ion homeostasis and NADPH/NADP(+) ratio could modulate enzyme activity, being functional in promoting proline accumulation and potentially also adjusting NADPH consumption during the defense against hyperosmotic stress. The apparent molecular weight of the native protein observed in size exclusion chromatography indicated a high oligomerization state. We also report the first crystal structure of a plant P5C reductase at 3.40-angstrom resolution, showing a decameric quaternary assembly. Based on the structure, it was possible to identify dynamic structural differences among rice, human, and bacterial enzymes. C1 [Forlani, Giuseppe; Bertazzini, Michele; Zarattini, Marco] Univ Ferrara, Dept Life Sci & Biotechnol, Lab Plant Physiol & Biochem, I-44121 Ferrara, Italy. [Bertazzini, Michele; Funck, Dietmar] Univ Konstanz, Dept Biol, Plant Physiol & Biochem, Constance, Germany. [Ruszkowski, Milosz] NCI, Synchrotron Radiat Res Sect, Macromol Crystallog Lab, Argonne Natl Lab, Argonne, IL USA. [Nocek, Boguslaw] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA. RP Forlani, G (reprint author), Univ Ferrara, Dept Life Sci & Biotechnol, Lab Plant Physiol & Biochem, Via Luigi Borsari 46, I-44121 Ferrara, Italy. EM flg@unife.it RI Forlani, Giuseppe/B-7869-2009 OI Forlani, Giuseppe/0000-0003-2598-5718 FU AGER Foundation in the frame of the RISINNOVA project [2010-2369]; University of Konstanz; Intramural Research Program of the NCI, Center for Cancer Research; US Department of Energy, Office of Science, Office of Basic Energy Sciences [W-31-109-Eng-38]; DAAD (German Academic Exchange Service) fellowship FX This work was funded by AGER Foundation in the frame of the RISINNOVA project, grant # 2010-2369. Partial support from the University of Konstanz and the Intramural Research Program of the NCI, Center for Cancer Research, is also gratefully acknowledged. Diffraction data were collected at the SER-CAT beamline 22-ID at the Advanced Photon Source, Argonne National Laboratory. Use of the Advanced Photon Source was funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. W-31-109-Eng-38. MB was the recipient of a DAAD (German Academic Exchange Service) fellowship supporting a stage in DF's laboratory. NR 65 TC 3 Z9 3 U1 6 U2 15 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. PD JUL 28 PY 2015 VL 6 AR 565 DI 10.3389/fpls.2015.00565 PG 13 WC Plant Sciences SC Plant Sciences GA CN8VW UT WOS:000358724700001 PM 26284087 ER PT J AU Taufour, V Thimmaiah, S March, S Saunders, S Sun, KW Lamichhane, TN Kramer, MJ Bud'ko, SL Canfield, PC AF Taufour, Valentin Thimmaiah, Srinivasa March, Stephen Saunders, Scott Sun, Kewei Lamichhane, Tej Nath Kramer, Matthew J. Bud'ko, Sergey L. Canfield, Paul C. TI Structural and Ferromagnetic Properties of an Orthorhombic Phase of MnBi Stabilized with Rh Additions SO PHYSICAL REVIEW APPLIED LA English DT Article ID NEUTRON-DIFFRACTION; MAGNETIC-PROPERTIES; CRITICAL-POINT; TEMPERATURE PHASE; PERMANENT-MAGNETS; CRITICAL ISOTHERM; SINGLE-CRYSTALS; EQUATION; STATE; TRANSITIONS AB The article addresses the possibility of alloy elements in MnBi which may modify the thermodynamic stability of the NiAs-type structure without significantly degrading the magnetic properties. The addition of small amounts of Rh and Mn provides an improvement in the thermal stability with some degradation of the magnetic properties. The small amounts of Rh and Mn additions in MnBi stabilize an orthorhombic phase whose structural and magnetic properties are closely related to the ones of the previously reported hightemperature phase of MnBi (HT MnBi). To date, the properties of the HT MnBi, which is stable between 613 and 719 K, have not been studied in detail because of its transformation to the stable low-temperature MnBi (LT MnBi), making measurements near and below its Curie temperature difficult. The Rh-stabilized MnBi with chemical formula Mn1.0625-xRhxBi [x = 0.02(1)] adopts a new superstructure of the NiAs/Ni2In structure family. It is ferromagnetic below a Curie temperature of 416 K. The critical exponents of the ferromagnetic transition are not of the mean-field type but are closer to those associated with the Ising model in three dimensions. The magnetic anisotropy is uniaxial; the anisotropy energy is rather large, and it does not increase when raising the temperature, contrary to what happens in LT MnBi. The saturation magnetization is approximately 3 mu(B)/f.u. at low temperatures. While this exact composition may not be application ready, it does show that alloying is a viable route to modifying the stability of this class of rare-earth-free magnet alloys. C1 [Taufour, Valentin; March, Stephen; Saunders, Scott; Lamichhane, Tej Nath; Bud'ko, Sergey L.; Canfield, Paul C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Taufour, Valentin; Thimmaiah, Srinivasa; Sun, Kewei; Lamichhane, Tej Nath; Kramer, Matthew J.; Bud'ko, Sergey L.; Canfield, Paul C.] US DOE, Ames Lab, US DOE, Ames, IA 50011 USA. [Kramer, Matthew J.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. RP Taufour, V (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. EM taufour@ameslab.gov FU Critical Materials Institute, an Energy Innovation Hub - U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office; Office of Basic Energy Sciences, Materials Sciences Division, U.S. DOE; U.S. DOE's Advanced Research Projects Agency-Energy [11/CJ000/09/03]; DOE [DE-AC02-07CH11358] FX We thank G. J. Miller, A. Jesche, D. Finnemore, T. Kong, A. Bohmer, and W. E. Straszheim for useful discussions. The research was supported by the Critical Materials Institute, an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office. This work was also supported by the Office of Basic Energy Sciences, Materials Sciences Division, U.S. DOE. The microscopy was performed under funding from the U.S. DOE's Advanced Research Projects Agency-Energy under Contract No. 11/CJ000/09/03. This work was performed at the Ames Laboratory, operated for DOE by Iowa State University under Contract No. DE-AC02-07CH11358. NR 54 TC 4 Z9 4 U1 12 U2 39 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2331-7019 J9 PHYS REV APPL JI Phys. Rev. Appl. PD JUL 28 PY 2015 VL 4 IS 1 AR 014021 DI 10.1103/PhysRevApplied.4.014021 PG 9 WC Physics, Applied SC Physics GA CN7JK UT WOS:000358610300002 ER PT J AU Aguado-Puente, P Bristowe, NC Yin, B Shirasawa, R Ghosez, P Littlewood, PB Artacho, E AF Aguado-Puente, P. Bristowe, N. C. Yin, B. Shirasawa, R. Ghosez, Philippe Littlewood, P. B. Artacho, Emilio TI Model of two-dimensional electron gas formation at ferroelectric interfaces SO PHYSICAL REVIEW B LA English DT Article ID THIN-FILMS; LAALO3/SRTIO3 HETEROINTERFACE; OXIDE INTERFACES; STRAIN; POLARIZATION; CONDUCTIVITY; TRANSITION; BOUNDARY; POLARITY AB The formation of a two-dimensional electron gas at oxide interfaces as a consequence of polar discontinuities has generated an enormous amount of activity due to the variety of interesting effects it gives rise to. Here, we study under what circumstances similar processes can also take place underneath ferroelectric thin films. We use a simple Landau model to demonstrate that in the absence of extrinsic screening mechanisms, a monodomain phase can be stabilized in ferroelectric films by means of an electronic reconstruction. Unlike in the LaAlO3/SrTiO3 heterostructure, the emergence with thickness of the free charge at the interface is discontinuous. This prediction is confirmed by performing first-principles simulations of free-standing slabs of PbTiO3. The model is also used to predict the response of the system to an applied electric field, demonstrating that the two-dimensional electron gas can be switched on and off discontinuously and in a nonvolatile fashion. Furthermore, the reversal of the polarization can be used to switch between a two-dimensional electron gas and a two-dimensional hole gas, which should, in principle, have very different transport properties. We discuss the possible formation of polarization domains and how such configuration competes with the spontaneous accumulation of free charge at the interfaces. C1 [Aguado-Puente, P.; Artacho, Emilio] Donostia Int Phys Ctr, San Sebastian 20018, Spain. [Aguado-Puente, P.; Yin, B.; Artacho, Emilio] CIC Nanogune, San Sebastian 20018, Spain. [Bristowe, N. C.; Ghosez, Philippe] Univ Liege, Theoret Mat Phys, B-4000 Sart Tilman Par Liege, Belgium. [Bristowe, N. C.] Univ London Imperial Coll Sci Technol & Med, Dept Phys, London SW7 2AZ, England. [Yin, B.] Zhejiang Univ, Dept Engn Mech, Hangzhou 310027, Zhejiang, Peoples R China. [Shirasawa, R.] Univ Cambridge, Dept Earth Sci, Cambridge CB2 3EQ, England. [Littlewood, P. B.] Argonne Natl Lab, Phys Sci & Engn, Argonne, IL 60439 USA. [Littlewood, P. B.] Univ Chicago, James Frank Inst, Chicago, IL 60637 USA. [Artacho, Emilio] Univ Cambridge, Cavendish Lab, Theory Condensed Matter, Cambridge CB3 0HE, England. [Artacho, Emilio] Basque Fdn Sci Ikerbasque, Bilbao 48013, Spain. RP Aguado-Puente, P (reprint author), Donostia Int Phys Ctr, Paseo Manuel Lardizabal 4, San Sebastian 20018, Spain. EM p.aguado@nanogune.eu RI Aguado-Puente, Pablo/K-8991-2012; Bristowe, Nicholas/B-2230-2013; Yin, Binglun/M-5323-2015; Littlewood, Peter/B-7746-2008; Artacho, Emilio/G-2616-2015; Ghosez, Philippe/F-1954-2014; DONOSTIA INTERNATIONAL PHYSICS CTR., DIPC/C-3171-2014; nanoGUNE, CIC/A-2623-2015 OI Aguado-Puente, Pablo/0000-0001-6985-8038; Bristowe, Nicholas/0000-0003-1286-8440; Yin, Binglun/0000-0002-3384-4758; Artacho, Emilio/0000-0001-9357-1547; FU MINECO-Spain [FIS2012-37549-C05]; UK's EPSRC; ARC project TheMoTherm [10/15-03]; DOE-DES [DE-AC02-06CH11357]; Royal Commission for the Exhibition of 1851; Thomas Young Centre [TYC-101] FX We acknowledge computing resources of CAMGRID in Cambridge, DIPC in San Sebastian, and the Spanish Super-computer Network (RES). This work has been partly funded by MINECO-Spain (Grant No. FIS2012-37549-C05), UK's EPSRC, and the ARC project TheMoTherm (Grant No. 10/15-03). Work at Argonne was supported by DOE-DES under Contract No. DE-AC02-06CH11357. Ph.G. acknowledges a Research Professorship of the Francqui Foundation (Belgium), and N.C.B. a research fellowship from the Royal Commission for the Exhibition of 1851 and support from the Thomas Young Centre under grant TYC-101. NR 62 TC 4 Z9 4 U1 5 U2 54 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUL 28 PY 2015 VL 92 IS 3 AR 035438 DI 10.1103/PhysRevB.92.035438 PG 17 WC Physics, Condensed Matter SC Physics GA CN7GG UT WOS:000358601700005 ER PT J AU Ke, LQ van Schilfgaarde, M AF Ke, Liqin van Schilfgaarde, Mark TI Band-filling effect on magnetic anisotropy using a Green's function method SO PHYSICAL REVIEW B LA English DT Article ID SINGLE-MOLECULE MAGNETS; MAGNETOCRYSTALLINE ANISOTROPY; ELECTRONIC-STRUCTURE; METALS; FE; MONOLAYERS; ORIGIN; FILMS AB We use an analytical model to describe the magnetocrystalline anisotropy energy (MAE) in solids as a function of band filling. The MAE is evaluated in second-order perturbation theory, which makes it possible to decompose the MAE into a sum of transitions between occupied and unoccupied pairs. The model enables us to characterize the MAE as a sum of contributions from different, often competing terms. The nitridometalates Li-2[(Li1-xTx)N], with T = Mn, Fe, Co, Ni, provide a system where the model is very effective because atomiclike orbital characters are preserved and the decomposition is fairly clean. Model results are also compared against MAE evaluated directly from first-principles calculations for this system. Good qualitative agreement is found. C1 [Ke, Liqin] US DOE, Ames Lab, Ames, IA 50011 USA. [van Schilfgaarde, Mark] Kings Coll London, Dept Phys, London WC2R 2LS, England. RP Ke, LQ (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. EM liqinke@ameslab.gov FU US Department of Energy, Energy Efficiency and Renewable Energy, Vehicles Technology Office, Advanced Power Electronics and Electric Motors program [DE-AC02-07CH11358] FX We would like to thank A. Jesche, P. Canfield, V. Antropov, A. Chantis, B. Harmon, and D. Johnson for helpful discussions. Work at Ames Laboratory was supported by the US Department of Energy, Energy Efficiency and Renewable Energy, Vehicles Technology Office, Advanced Power Electronics and Electric Motors program, under Contract No. DE-AC02-07CH11358. NR 36 TC 5 Z9 5 U1 1 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUL 28 PY 2015 VL 92 IS 1 AR 014423 DI 10.1103/PhysRevB.92.014423 PG 9 WC Physics, Condensed Matter SC Physics GA CN7FM UT WOS:000358599600001 ER PT J AU Stone, MB Lumsden, MD Garlea, VO Grenier, B Ressouche, E Samulon, EC Fisher, IR AF Stone, M. B. Lumsden, M. D. Garlea, V. O. Grenier, B. Ressouche, E. Samulon, E. C. Fisher, I. R. TI Field-induced spin density wave and spiral phases in a layered antiferromagnet SO PHYSICAL REVIEW B LA English DT Article ID BOSE-EINSTEIN CONDENSATION; NEUTRON POWDER DIFFRACTION AB We determine the low-field ordered magnetic phases of the S = 1 dimerized antiferromagnet Ba3Mn2O8 using single-crystal neutron diffraction. We find that for magnetic fields between mu H-0 = 8.80 T and 10.56 T applied along the [1 (1) over bar0] direction the system exhibits spin density wave order with incommensurate wave vectors of type (eta,eta,epsilon). For mu H-0 > 10.56 T, the magnetic order changes to a spiral phase with incommensurate wave vectors only along the [hh0] direction. For both field-induced ordered phases, the magnetic moments are lying in the plane perpendicular to the field direction. The nature of these two transitions is fundamentally different: the low-field transition is a second-order transition to a spin density wave ground state, while the one at higher field, toward the spiral phase, is of first order. C1 [Stone, M. B.; Lumsden, M. D.; Garlea, V. O.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Grenier, B.; Ressouche, E.] CEA, INAC SPSMS, F-38000 Grenoble, France. [Grenier, B.; Ressouche, E.] Univ Grenoble Alpes, F-38000 Grenoble, France. [Samulon, E. C.; Fisher, I. R.] Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA. [Samulon, E. C.; Fisher, I. R.] Stanford Univ, Geballe Lab Adv Mat, Stanford, CA 94305 USA. RP Stone, MB (reprint author), Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RI Stone, Matthew/G-3275-2011; Garlea, Vasile/A-4994-2016; Lumsden, Mark/F-5366-2012 OI Stone, Matthew/0000-0001-7884-9715; Garlea, Vasile/0000-0002-5322-7271; Lumsden, Mark/0000-0002-5472-9660 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; National Science Foundation [DMR-0454672, DMR-1205165]; U.S. Department of Energy [DE-AC05-00OR22725] FX We acknowledge helpful discussions with C. Batista and Y. Kamiya. A portion of this research at ORNL's High Flux Isotope Reactor and Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. This work utilized facilities supported in part by the National Science Foundation under Agreement No. DMR-0454672. Work at Stanford was supported by the National Science Foundation, under Grant No. DMR-1205165. This manuscript has been authored by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 22 TC 0 Z9 0 U1 1 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUL 28 PY 2015 VL 92 IS 2 AR 020415 DI 10.1103/PhysRevB.92.020415 PG 5 WC Physics, Condensed Matter SC Physics GA CN7FX UT WOS:000358600700002 ER PT J AU Campbell, JM Miller, DJ Robens, T AF Campbell, John M. Miller, David J. Robens, Tania TI Next-to-leading order predictions for WW plus jet production SO PHYSICAL REVIEW D LA English DT Article ID ONE-LOOP AMPLITUDES; PP COLLISIONS; HADRON COLLIDERS; CROSS-SECTIONS; ROOT-S=7 TEV; HIGGS-BOSON; W+W; GAMMA; QCD; ZZ AB In this work we report on a next-to-leading order calculation of WW + jet production at hadron colliders, with subsequent leptonic decays of the W bosons included. The calculation of the one-loop contributions is performed using generalized unitarity methods in order to derive analytic expressions for the relevant amplitudes. These amplitudes have been implemented in the parton-level Monte Carlo generator MCFM, which we use to provide a complete next-to-leading order calculation. Predictions for total cross sections, as well as differential distributions for several key observables, are computed both for the LHC operating at 14 TeV as well as for a possible future 100 TeV proton-proton collider. C1 [Campbell, John M.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Miller, David J.] Univ Glasgow, Sch Phys & Astron, Glasgow G12 8QQ, Lanark, Scotland. [Robens, Tania] Tech Univ Dresden, IKTP, D-01069 Dresden, Germany. RP Campbell, JM (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. FU UK Science and Technology Facilities Council (STFC) [ST/L000446/1]; US DOE [DE-AC02-07CH11359] FX T. R. thanks Simon Badger, Ruth Britto, Fabrizio Caola, Pierpaolo Mastrolia, and Ciaran Williams for extremely useful discussions during this work, as well as the Fermilab theory group for their hospitality. D. J. M. is supported by the UK Science and Technology Facilities Council (STFC) under Grant No. ST/L000446/1. D. J. M. and T. R. also want to thank A. A. H. Graham for contributions during the early stages of this work. This research is supported by the US DOE under Contract No. DE-AC02-07CH11359. NR 66 TC 4 Z9 4 U1 5 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 28 PY 2015 VL 92 IS 1 AR 014033 DI 10.1103/PhysRevD.92.014033 PG 11 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CN7HN UT WOS:000358605200002 ER PT J AU Doppner, T Callahan, DA Hurricane, OA Hinkel, DE Ma, T Park, HS Hopkins, LFB Casey, DT Celliers, P Dewald, EL Dittrich, TR Haan, SW Kritcher, AL MacPhee, A Le Pape, S Pak, A Patel, PK Springer, PT Salmonson, JD Tommasini, R Benedetti, LR Bond, E Bradley, DK Caggiano, J Church, J Dixit, S Edgell, D Edwards, MJ Fittinghoff, DN Frenje, J Johnson, MG Grim, G Hatarik, R Havre, M Herrmann, H Izumi, N Khan, SF Kline, JL Knauer, J Kyrala, GA Landen, OL Merrill, FE Moody, J Moore, AS Nikroo, A Ralph, JE Remington, BA Robey, HF Sayre, D Schneider, M Streckert, H Town, R Turnbull, D Volegov, PL Wan, A Widmann, K Wilde, CH Yeamans, C AF Doeppner, T. Callahan, D. A. Hurricane, O. A. Hinkel, D. E. Ma, T. Park, H. -S. Hopkins, L. F. Berzak Casey, D. T. Celliers, P. Dewald, E. L. Dittrich, T. R. Haan, S. W. Kritcher, A. L. MacPhee, A. Le Pape, S. Pak, A. Patel, P. K. Springer, P. T. Salmonson, J. D. Tommasini, R. Benedetti, L. R. Bond, E. Bradley, D. K. Caggiano, J. Church, J. Dixit, S. Edgell, D. Edwards, M. J. Fittinghoff, D. N. Frenje, J. Johnson, M. Gatu Grim, G. Hatarik, R. Havre, M. Herrmann, H. Izumi, N. Khan, S. F. Kline, J. L. Knauer, J. Kyrala, G. A. Landen, O. L. Merrill, F. E. Moody, J. Moore, A. S. Nikroo, A. Ralph, J. E. Remington, B. A. Robey, H. F. Sayre, D. Schneider, M. Streckert, H. Town, R. Turnbull, D. Volegov, P. L. Wan, A. Widmann, K. Wilde, C. H. Yeamans, C. TI Demonstration of High Performance in Layered Deuterium-Tritium Capsule Implosions in Uranium Hohlraums at the National Ignition Facility SO PHYSICAL REVIEW LETTERS LA English DT Article AB We report on the first layered deuterium-tritium (DT) capsule implosions indirectly driven by a "high-foot" laser pulse that were fielded in depleted uranium hohlraums at the National Ignition Facility. Recently, high-foot implosions have demonstrated improved resistance to ablation-front Rayleigh-Taylor instability induced mixing of ablator material into the DT hot spot [Hurricane et al., Nature (London) 506, 343 (2014)]. Uranium hohlraums provide a higher albedo and thus an increased drive equivalent to an additional 25 TW laser power at the peak of the drive compared to standard gold hohlraums leading to higher implosion velocity. Additionally, we observe an improved hot-spot shape closer to round which indicates enhanced drive from the waist. In contrast to findings in the National Ignition Campaign, now all of our highest performing experiments have been done in uranium hohlraums and achieved total yields approaching 10(16) neutrons where more than 50% of the yield was due to additional heating of alpha particles stopping in the DT fuel. C1 [Doeppner, T.; Callahan, D. A.; Hurricane, O. A.; Hinkel, D. E.; Ma, T.; Park, H. -S.; Hopkins, L. F. Berzak; Casey, D. T.; Celliers, P.; Dewald, E. L.; Dittrich, T. R.; Haan, S. W.; Kritcher, A. L.; MacPhee, A.; Le Pape, S.; Pak, A.; Patel, P. K.; Springer, P. T.; Salmonson, J. D.; Tommasini, R.; Benedetti, L. R.; Bond, E.; Bradley, D. K.; Caggiano, J.; Church, J.; Dixit, S.; Edwards, M. J.; Fittinghoff, D. N.; Hatarik, R.; Izumi, N.; Khan, S. F.; Landen, O. L.; Moody, J.; Ralph, J. E.; Remington, B. A.; Robey, H. F.; Sayre, D.; Schneider, M.; Town, R.; Turnbull, D.; Wan, A.; Widmann, K.; Yeamans, C.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Edgell, D.; Knauer, J.] Univ Rochester, Laser Energet Lab, Rochester, NY 14623 USA. [Frenje, J.; Johnson, M. Gatu] MIT, Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA. [Grim, G.; Herrmann, H.; Kline, J. L.; Kyrala, G. A.; Merrill, F. E.; Volegov, P. L.; Wilde, C. H.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Havre, M.; Nikroo, A.; Streckert, H.] Gen Atom Co, San Diego, CA 92121 USA. [Moore, A. S.] Atom Weap Estab, Aldermaston RG7, England. RP Doppner, T (reprint author), Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94551 USA. RI IZUMI, Nobuhiko/J-8487-2016; Patel, Pravesh/E-1400-2011; Tommasini, Riccardo/A-8214-2009 OI IZUMI, Nobuhiko/0000-0003-1114-597X; Tommasini, Riccardo/0000-0002-1070-3565 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We would like to thank the entire NIF operations, cryogenics, diagnostics, and target teams for outstanding support. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 36 TC 18 Z9 18 U1 3 U2 26 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 28 PY 2015 VL 115 IS 5 AR 055001 DI 10.1103/PhysRevLett.115.055001 PG 5 WC Physics, Multidisciplinary SC Physics GA CN7JF UT WOS:000358609800010 PM 26274424 ER PT J AU Higginson, DP Vassura, L Gugiu, MM Antici, P Borghesi, M Brauckmann, S Diouf, C Green, A Palumbo, L Petrascu, H Sofia, S Stardubtsev, M Willi, O Kar, S Negoita, F Fuchs, J AF Higginson, D. P. Vassura, L. Gugiu, M. M. Antici, P. Borghesi, M. Brauckmann, S. Diouf, C. Green, A. Palumbo, L. Petrascu, H. Sofia, S. Stardubtsev, M. Willi, O. Kar, S. Negoita, F. Fuchs, J. TI Temporal Narrowing of Neutrons Produced by High-Intensity Short-Pulse Lasers SO PHYSICAL REVIEW LETTERS LA English DT Article ID ION-BEAMS; PROTON-BEAMS; FUSION; GENERATION; FACILITY; YIELDS AB The production of neutron beams having short temporal duration is studied using ultraintense laser pulses. Laser-accelerated protons are spectrally filtered using a laser-triggered microlens to produce a short duration neutron pulse via nuclear reactions induced in a converter material (LiF). This produces a similar to 3 ns duration neutron pulse with 10(4) n/MeV/sr/shot at 0.56 m from the laser-irradiated proton source. The large spatial separation between the neutron production and the proton source allows for shielding from the copious and undesirable radiation resulting from the laser-plasma interaction. This neutron pulse compares favorably to the duration of conventional accelerator sources and should scale up with, present and future, higher energy laser facilities to produce brighter and shorter neutron beams for ultrafast probing of dense materials. C1 [Higginson, D. P.; Vassura, L.; Diouf, C.; Sofia, S.; Fuchs, J.] Univ Paris 06, Ecole Polytech, CNRS CEA, Lab Utilisat Lasers Intenses,UMR 7605, F-91128 Palaiseau, France. [Vassura, L.; Antici, P.; Palumbo, L.] Univ Roma La Sapienza, Dipartimento SBAI, I-00161 Rome, Italy. [Gugiu, M. M.; Petrascu, H.; Negoita, F.] IFIN HH, Bucharest 077125, Romania. [Antici, P.] INRS EMT, Varennes, PQ, Canada. [Antici, P.] Ist Nazl Fis Nucl, I-00044 Frascati, Italy. [Borghesi, M.; Green, A.; Kar, S.] Queens Univ Belfast, Sch Math & Phys, Belfast BT7 1NN, Antrim, North Ireland. [Borghesi, M.] Acad Sci Czech Republic, Inst Phys, ELI Beamlines Project, Prague 18221, Czech Republic. [Brauckmann, S.; Willi, O.] Univ Dusseldorf, Inst Laser & Plasmaphys, D-40225 Dusseldorf, Germany. [Stardubtsev, M.; Fuchs, J.] Inst Appl Phys, Nizhnii Novgorod 603950, Russia. [Higginson, D. P.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Higginson, DP (reprint author), Univ Paris 06, Ecole Polytech, CNRS CEA, Lab Utilisat Lasers Intenses,UMR 7605, F-91128 Palaiseau, France. RI Fuchs, Julien/D-3450-2016; Kar, Satyabrata/E-5220-2010; Higginson, Drew/G-5942-2016 OI Fuchs, Julien/0000-0001-9765-0787; Higginson, Drew/0000-0002-7699-3788 FU Region Ile-de-France [E1127]; Laserlab-Europe [284464, 001528]; Agence Nationale de la Recherche [11-IDEX-0004-02]; DGA-MRIS scholarship; Romanian National Authority for Scientific Research, CNCS UEFISCDI [PN-II-ID-JRP-2011-1]; European Social Fund and the state budget of the Czech Republic [CZ.1.05/1.1.00/483/02.0061, CZ.1.07/2.3.00/ 20.0279]; Ministry of Education and Science of the Russian Federation [14.Z50.31.0007]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; LULI technical teams; DFG [GRK 1203]; EPSRC [EP/K022415/1, EP/J002550/1] FX We are grateful to Dr. K. Parsons and Dr. G. Hale for evaluating a newer 7Li(p, n)7 Be cross section that agrees better with previous experimental results. We acknowledge the support of the LULI technical teams. This work was supported by Grant No. E1127 from Region Ile-de-France. The research leading to these results has received funding from Laserlab-Europe (Grant Agreement No. 284464, Ec's seventh framework program) and Grant No. 001528. This work was partly done within the LABEX Plas@Par project and was supported by Grant No. 11-IDEX-0004-02 from Agence Nationale de la Recherche. L. V. was funded by a DGA-MRIS scholarship. H. P., M. M. G., and F. N. acknowledge support from the Romanian National Authority for Scientific Research, CNCS UEFISCDI, under Project No. PN-II-ID-JRP-2011-1. This work also partly supported by the DFG GRK 1203 program and by EPSRC Grants No. EP/K022415/1 and No. EP/J002550/1. M. B. acknowledges cofinancing by the European Social Fund and the state budget of the Czech Republic (Projects No. CZ.1.05/1.1.00/483/02.0061 and No. CZ.1.07/2.3.00/ 20.0279). This work was supported in part by the Ministry of Education and Science of the Russian Federation under Contract No. 14.Z50.31.0007. This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 44 TC 4 Z9 4 U1 5 U2 30 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 28 PY 2015 VL 115 IS 5 AR 054802 DI 10.1103/PhysRevLett.115.054802 PG 5 WC Physics, Multidisciplinary SC Physics GA CN7JF UT WOS:000358609800009 PM 26274423 ER PT J AU Pujari, BS Larson, P Antropov, VP Belashchenko, KD AF Pujari, B. S. Larson, P. Antropov, V. P. Belashchenko, K. D. TI Ab Initio Construction of Magnetic Phase Diagrams in Alloys: The Case of Fe1-xMnxPt SO PHYSICAL REVIEW LETTERS LA English DT Article ID ELECTRONIC-STRUCTURE; 1ST PRINCIPLES; SPIN DYNAMICS; TEMPERATURE; SYSTEMS; ORDER; MODEL AB A first-principles approach to the construction of concentration-temperature magnetic phase diagrams of metallic alloys is presented. The method employs self-consistent total energy calculations based on the coherent potential approximation for partially ordered and noncollinear magnetic states and is able to account for competing interactions and multiple magnetic phases. Application to the Fe1-xMnxPt "magnetic chameleon" system yields the sequence of magnetic phases at T = 0 and the c - T magnetic phase diagram in good agreement with experiment, and a new low-temperature phase is predicted at the Mn-rich end. The importance of non-Heisenberg interactions for the description of the magnetic phase diagram is demonstrated. C1 [Pujari, B. S.; Larson, P.; Belashchenko, K. D.] Univ Nebraska, Dept Phys & Astron, Lincoln, NE 68588 USA. [Pujari, B. S.; Larson, P.; Belashchenko, K. D.] Univ Nebraska, Nebraska Ctr Mat & Nanosci, Lincoln, NE 68588 USA. [Pujari, B. S.] Savitribai Phule Univ Pune, Ctr Modeling & Simulat, Pune 411007, Maharashtra, India. [Antropov, V. P.] Ames Lab, Ames, IA 50011 USA. RP Pujari, BS (reprint author), Univ Nebraska, Dept Phys & Astron, Lincoln, NE 68588 USA. RI Belashchenko, Kirill/A-9744-2008 OI Belashchenko, Kirill/0000-0002-8518-1490 FU National Science Foundation [DMR-1308751]; Nebraska MRSEC [DMR-0820521]; Critical Materials Institute; Energy Innovation Hub - U.S. DOE; Office of Basic Energy Science, Division of Materials Science and Engineering; U.S. DOE by Iowa State University [DE-AC02-07CH11358] FX The work at UNL was supported by the National Science Foundation through Grant No. DMR-1308751 and the Nebraska MRSEC (DMR-0820521) and was performed utilizing the Holland Computing Center of the University of Nebraska. Work at Ames Lab is supported in part by the Critical Materials Institute, an Energy Innovation Hub funded by the U.S. DOE and by the Office of Basic Energy Science, Division of Materials Science and Engineering. Ames Laboratory is operated for the U.S. DOE by Iowa State University under Contract No. DE-AC02-07CH11358. NR 31 TC 2 Z9 2 U1 2 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 28 PY 2015 VL 115 IS 5 AR 057203 DI 10.1103/PhysRevLett.115.057203 PG 5 WC Physics, Multidisciplinary SC Physics GA CN7JF UT WOS:000358609800016 PM 26274437 ER PT J AU Burke, CM Pande, V Khetan, A Viswanathan, V McCloskey, BD AF Burke, Colin M. Pande, Vikram Khetan, Abhishek Viswanathan, Venkatasubramanian McCloskey, Bryan D. TI Enhancing electrochemical intermediate solvation through electrolyte anion selection to increase nonaqueous Li-O-2 battery capacity SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE donor number; solubility; lithium nitrate; NMR; Li-air battery ID LI-AIR BATTERIES; NUCLEAR MAGNETIC-RESONANCE; DISCHARGE CAPACITY; DIMETHYL-SULFOXIDE; ACCEPTOR NUMBERS; IONIC SOLVATION; GUTMANN DONOR; SOLVENTS; OXYGEN; REDUCTION AB Among the "beyond Li-ion" battery chemistries, nonaqueous Li-O-2 batteries have the highest theoretical specific energy and, as a result, have attracted significant research attention over the past decade. A critical scientific challenge facing nonaqueous Li-O-2 batteries is the electronically insulating nature of the primary discharge product, lithium peroxide, which passivates the battery cathode as it is formed, leading to low ultimate cell capacities. Recently, strategies to enhance solubility to circumvent this issue have been reported, but rely upon electrolyte formulations that further decrease the overall electrochemical stability of the system, thereby deleteriously affecting battery rechargeability. In this study, we report that a significant enhancement (greater than fourfold) in Li-O-2 cell capacity is possible by appropriately selecting the salt anion in the electrolyte solution. Using Li-7 NMR and modeling, we confirm that this improvement is a result of enhanced Li+ stability in solution, which, in turn, induces solubility of the intermediate to Li2O2 formation. Using this strategy, the challenging task of identifying an electrolyte solvent that possesses the anticorrelated properties of high intermediate solubility and solvent stability is alleviated, potentially providing a pathway to develop an electrolyte that affords both high capacity and rechargeability. We believe the model and strategy presented here will be generally useful to enhance Coulombic efficiency in many electrochemical systems (e. g., Li-S batteries) where improving intermediate stability in solution could induce desired mechanisms of product formation. C1 [Burke, Colin M.; McCloskey, Bryan D.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Burke, Colin M.; McCloskey, Bryan D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Pande, Vikram; Viswanathan, Venkatasubramanian] Carnegie Mellon Univ, Dept Mech Engn, Pittsburgh, PA 15213 USA. [Khetan, Abhishek] Rhein Westfal TH Aachen, Inst Combust Technol, D-52056 Aachen, Germany. RP Viswanathan, V (reprint author), Carnegie Mellon Univ, Dept Mech Engn, Pittsburgh, PA 15213 USA. EM venkvis@cmu.edu; bmcclosk@berkeley.edu RI McCloskey, Bryan/A-6556-2015; OI McCloskey, Bryan/0000-0001-6599-2336; Viswanathan, Venkatasubramanian/0000-0003-1060-5495 FU Laboratory Directed Research and Development Program of LBNL under US Department of Energy [DE-AC02-05CH11231]; US DOE Vehicle Technologies Office [DE-0006869]; Deutsche Forschungsgemeinschaft FX The authors thank Alan Luntz, Dan Addison, Jeffrey Reimer, Hilda Buss, Jessica Nichols, and Christopher Dekmezian for helpful discussions and guidance on materials characterization. The work at University of California, Berkeley/Lawrence Berkeley National Laboratory (LBNL) was supported in part by previous work performed through the Laboratory Directed Research and Development Program of LBNL under US Department of Energy Contract DE-AC02-05CH11231. Support for C.M.B. was provided through the US DOE Vehicle Technologies Office under award DE-0006869. A.K. thankfully acknowledges the funding for his doctoral studies from the Deutsche Forschungsgemeinschaft. NR 40 TC 44 Z9 44 U1 11 U2 94 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUL 28 PY 2015 VL 112 IS 30 BP 9293 EP 9298 DI 10.1073/pnas.1505728112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CN7ZW UT WOS:000358656500055 PM 26170330 ER PT J AU Yu, XH Zhang, RF Weldon, D Vogel, SC Zhang, JZ Brown, DW Wang, Y Reiche, HM Wang, SM Du, SY Jin, CQ Zhao, YS AF Yu, Xiaohui Zhang, Ruifeng Weldon, David Vogel, Sven C. Zhang, Jianzhong Brown, Donald W. Wang, Yanbin Reiche, Helmut M. Wang, Shanmin Du, Shiyu Jin, Changqing Zhao, Yusheng TI High Pressure Phase-Transformation Induced Texture Evolution and Strengthening in Zirconium Metal: Experiment and Modeling SO SCIENTIFIC REPORTS LA English DT Article ID INITIO MOLECULAR-DYNAMICS; DEFORMATION-DIA; OMEGA-PHASE; TITANIUM; DIFFRACTION; TRANSITION; CRYSTALS; GPA; ZR AB We studied the phase-transition induced texture changes and strengthening mechanism for zirconium metal under quasi-hydrostatic compression and uni-axial deformation under confined high pressure using the deformation-DIA (D-DIA) apparatus. It is shown that the experimentally obtained texture for omega-phase Zr can be qualitatively described by combining a subset of orientation variants previously proposed in two different models. The determined flow stress for the high-pressure alpha-phase is 0.5-1.2 GPa, more than three times higher than that of the a-phase. Using first-principles calculations, we investigated the mechanical and electronic properties of the two Zr polymorphs. We find that the observed strengthening can be attributed to the relatively strong directional bonding in the omega phase, which significantly increases its shear plastic resistance over the alpha-phase Zr. The present findings provide an alternate route for Zr metal strengthening by high-pressure phase transformation. C1 [Yu, Xiaohui; Jin, Changqing; Zhao, Yusheng] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Yu, Xiaohui; Jin, Changqing; Zhao, Yusheng] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Yu, Xiaohui; Weldon, David; Vogel, Sven C.; Zhang, Jianzhong; Brown, Donald W.; Reiche, Helmut M.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Zhang, Ruifeng] Beihang Univ, Sch Mat Sci & Engn, Beijing 100191, Peoples R China. [Wang, Yanbin] Univ Chicago, Ctr Adv Radiat Sources, Chicago, IL 60469 USA. [Wang, Shanmin; Zhao, Yusheng] Univ Nevada, HiPSEC, Las Vegas, NV 89154 USA. [Wang, Shanmin; Zhao, Yusheng] Univ Nevada, Dept Phys & Astron, Las Vegas, NV 89154 USA. [Du, Shiyu] Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Div Funct Mat & Nanodevices, Ningbo 315201, Zhejiang, Peoples R China. [Jin, Changqing] Collaborat Innovat Ctr Quantum Matter, Beijing, Peoples R China. RP Zhang, RF (reprint author), Beihang Univ, Sch Mat Sci & Engn, Beijing 100191, Peoples R China. EM zrf@buaa.edu.cn; sven@lanl.gov; yusheng.zhao@unlv.edu OI Wang, Yanbin/0000-0001-5716-3183; Zhang, Jianzhong/0000-0001-5508-1782; Vogel, Sven C./0000-0003-2049-0361 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Science [W-31-109-Eng-38]; NSF [EAR-0968456, 1361276]; National Science Foundation - Earth Sciences [EAR-1128799]; Department of Energy- GeoSciences [DE-FG02-94ER14466]; DOE Office of Science [DE-AC02-06CH11357]; MOST; CAS; [DE-FC52-06NA27684] FX The authors would like to thank the U.S. Department of Energy, Office of Science, Office of Basic Energy Science, who supported our beam time under contract number W-31-109-Eng-38. The UNLV High Pressure Science and Engineering Center (HiPSEC) is a DOE NNSA Center of Excellence supported by Cooperative Agreement DE-FC52-06NA27684. The deformation experiments were performed at GeoSoilEnviroCARS (Sector 13), Advanced Photon Source (APS), Argonne National Laboratory, supported by NSF grants EAR-0968456 and 1361276. GeoSoilEnviroCARS is supported by the National Science Foundation - Earth Sciences (EAR-1128799) and Department of Energy- GeoSciences (DE-FG02-94ER14466). This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. The authors would like to thank to the Fundamental Research Funds for the Central Universities of Beihang University, National Natural Science Foundation of China (51471018 and 51402350), and National Thousand Young Talents Program of China. CQJ is supported by NSF, MOST & CAS through research projects. We would like to thank James H. Wilkerson for the effort on texture analysis. We would like to thank Norimasa Nishiyama for the assistance at APS. NR 31 TC 7 Z9 7 U1 6 U2 34 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUL 28 PY 2015 VL 5 AR 12552 DI 10.1038/srep12552 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CN6YB UT WOS:000358579300001 PM 26218405 ER PT J AU Arik, M Aune, S Barth, K Belov, A Brauninger, H Bremer, J Burwitz, V Cantatore, G Carmona, JM Cetin, SA Collar, JI Da Riva, E Dafni, T Davenport, M Dermenev, A Eleftheriadis, C Elias, N Fanourakis, G Ferrer-Ribas, E Galan, J Garcia, JA Gardikiotis, A Garza, JG Gazis, EN Geralis, T Georgiopoulou, E Giomataris, I Gninenko, S Marzoa, MG Hasinoff, MD Hoffmann, DHH Iguaz, FJ Irastorza, IG Jacoby, J Jakovcic, K Karuza, M Kavuk, M Krcmar, M Kuster, M Lakic, B Laurent, JM Liolios, A Ljubicic, A Luzon, G Neff, S Niinikoski, T Nordt, A Ortega, I Papaevangelou, T Pivovaroff, MJ Raffelt, G Rodriguez, A Rosu, M Ruz, J Savvidis, I Shilon, I Solanki, SK Stewart, L Tomas, A Vafeiadis, T Villar, J Vogel, JK Yildiz, SC Zioutas, K AF Arik, M. Aune, S. Barth, K. Belov, A. Braeuninger, H. Bremer, J. Burwitz, V. Cantatore, G. Carmona, J. M. Cetin, S. A. Collar, J. I. Da Riva, E. Dafni, T. Davenport, M. Dermenev, A. Eleftheriadis, C. Elias, N. Fanourakis, G. Ferrer-Ribas, E. Galan, J. Garcia, J. A. Gardikiotis, A. Garza, J. G. Gazis, E. N. Geralis, T. Georgiopoulou, E. Giomataris, I. Gninenko, S. Marzoa, M. Gomez Hasinoff, M. D. Hoffmann, D. H. H. Iguaz, F. J. Irastorza, I. G. Jacoby, J. Jakovcic, K. Karuza, M. Kavuk, M. Krcmar, M. Kuster, M. Lakic, B. Laurent, J. M. Liolios, A. Ljubicic, A. Luzon, G. Neff, S. Niinikoski, T. Nordt, A. Ortega, I. Papaevangelou, T. Pivovaroff, M. J. Raffelt, G. Rodriguez, A. Rosu, M. Ruz, J. Savvidis, I. Shilon, I. Solanki, S. K. Stewart, L. Tomas, A. Vafeiadis, T. Villar, J. Vogel, J. K. Yildiz, S. C. Zioutas, K. CA CAST Collaboration TI New solar axion search using the CERN Axion Solar Telescope with He-4 filling SO PHYSICAL REVIEW D LA English DT Article ID STRONG CP PROBLEM; COHERENT CONVERSION; CAST EXPERIMENT; MAGNETIC-FIELD; INVARIANCE; DETECTORS; PHOTONS AB The CERN Axion Solar Telescope (CAST) searches for a -> gamma conversion in the 9 T magnetic field of a refurbished LHC test magnet that can be directed toward the Sun. Two parallel magnet bores can be filled with helium of adjustable pressure to match the x-ray refractive mass m(gamma) to the axion search mass m(a). After the vacuum phase (2003-2004), which is optimal for m(a) less than or similar to 0.02 eV, we used He-4 in 2005-2007 to cover the mass range of 0.02-0.39 eV and He-3 in 2009-2011 to scan from 0.39 to 1.17 eV. After improving the detectors and shielding, we returned to He-4 in 2012 to investigate a narrow m(a) range around 0.2 eV ("candidate setting" of our earlier search) and 0.39-0.42 eV, the upper axion mass range reachable with He-4, to "cross the axion line" for the KSVZ model. We have improved the limit on the axion-photon coupling to g(a gamma) < 1.47 x 10(-10) GeV-1 (95% C.L.), depending on the pressure settings. Since 2013, we have returned to the vacuum and aim for a significant increase in sensitivity. C1 [Arik, M.; Cetin, S. A.; Kavuk, M.; Yildiz, S. C.] Dogus Univ, Istanbul, Turkey. [Aune, S.; Ferrer-Ribas, E.; Galan, J.; Giomataris, I.; Papaevangelou, T.] CEA Saclay, Ctr Etud Nucl Saclay, IRFU, F-91191 Gif Sur Yvette, France. [Barth, K.; Bremer, J.; Da Riva, E.; Davenport, M.; Elias, N.; Marzoa, M. Gomez; Laurent, J. M.; Niinikoski, T.; Ortega, I.; Shilon, I.; Stewart, L.; Vafeiadis, T.; Zioutas, K.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Belov, A.; Dermenev, A.; Gninenko, S.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Braeuninger, H.; Burwitz, V.; Kuster, M.; Nordt, A.] Max Planck Inst Extraterr Phys, D-85748 Garching, Germany. [Cantatore, G.; Karuza, M.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Cantatore, G.; Karuza, M.] Univ Trieste, Trieste, Italy. [Carmona, J. M.; Dafni, T.; Garcia, J. A.; Garza, J. G.; Iguaz, F. J.; Irastorza, I. G.; Luzon, G.; Ortega, I.; Rodriguez, A.; Shilon, I.; Tomas, A.; Villar, J.] Univ Zaragoza, Grp Invest Fis Nucl & Astroparticulas, Zaragoza, Spain. [Collar, J. I.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Collar, J. I.] Univ Chicago, KICP, Chicago, IL 60637 USA. [Eleftheriadis, C.; Liolios, A.; Savvidis, I.; Vafeiadis, T.] Aristotle Univ Thessaloniki, GR-54006 Thessaloniki, Greece. [Fanourakis, G.; Geralis, T.] Natl Ctr Sci Res Demokritos, Athens, Greece. [Gardikiotis, A.; Georgiopoulou, E.; Vafeiadis, T.; Zioutas, K.] Univ Patras, Dept Phys, GR-26110 Patras, Greece. [Gazis, E. N.] Natl Tech Univ Athens, Athens, Greece. [Hasinoff, M. D.] Univ British Columbia, Dept Phys & Astron, Vancouver, BC V5Z 1M9, Canada. [Hoffmann, D. H. H.; Kuster, M.; Neff, S.; Nordt, A.; Rosu, M.] Tech Univ Darmstadt, IKP, Darmstadt, Germany. [Jacoby, J.] Goethe Univ Frankfurt, Inst Angew Phys, Frankfurt, Germany. [Jakovcic, K.; Krcmar, M.; Lakic, B.; Ljubicic, A.] Rudjer Boskovic Inst, Zagreb, Croatia. [Karuza, M.] Univ Rijeka, Dept Phys, Rijeka 51000, Croatia. [Karuza, M.] Univ Rijeka, Ctr Micro & Nano Sci & Technol, Rijeka 51000, Croatia. [Pivovaroff, M. J.; Ruz, J.; Vogel, J. K.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Raffelt, G.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Solanki, S. K.] Max Planck Inst Sonnensyst Forsch, Gottingen, Germany. [Marzoa, M. Gomez] Ecole Polytech Fed Lausanne, Lab Transfert Chaleur & Masse, CH-1015 Lausanne, Switzerland. [Shilon, I.] Ben Gurion Univ Negev, Dept Phys, IL-84105 Beer Sheva, Israel. RP Garcia, JA (reprint author), Univ Zaragoza, Grp Invest Fis Nucl & Astroparticulas, Zaragoza, Spain. EM jagarpas@unizar.es RI Irastorza, Igor/B-2085-2012; Gracia Garza, Javier/F-5713-2016; Villar, Jose Angel/K-6630-2014; Galan, Javier/F-7986-2016; Papaevangelou, Thomas/G-2482-2016; Kuster, Markus/C-5742-2014; Iguaz Gutierrez, Francisco Jose/F-4117-2016 OI Irastorza, Igor/0000-0003-1163-1687; Gracia Garza, Javier/0000-0003-0800-1588; Villar, Jose Angel/0000-0003-0228-7589; Galan, Javier/0000-0001-7529-9834; Papaevangelou, Thomas/0000-0003-2829-9158; Iguaz Gutierrez, Francisco Jose/0000-0001-6327-9369 FU NSERC (Canada); MSES (Croatia); CEA (France); BMBF (Germany) [05 CC2EEA/9, 05 CC1RD1/0]; DFG (Germany) [HO 1400/7-1, EXC-153]; GSRT (Greece); NSRF: Heracleitus II (Russia); RFFR (Russia); Spanish Ministry of Economy and Competitiveness (MINECO) [FPA2008-03456, FPA2011-24058, EIC-CERN-2011-0006]; European Regional Development Fund (ERDF/FEDER); European Research Council (ERC) [ERC-2009-StG-240054]; Turkish Atomic Energy Authority (TAEK); National Science Foundation (USA) [0239812]; NASA [NAG5-10842]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We thank CERN for hosting CAST and for technical support to operate the magnet and cryogenics. We thank the CERN CFD team for their essential contribution to the CFD work. We acknowledge support from NSERC (Canada), MSES (Croatia), CEA (France), BMBF (Germany) under the Grants No. 05 CC2EEA/9 and No. 05 CC1RD1/0 and DFG (Germany) under Grants No. HO 1400/7-1 and No. EXC-153, GSRT (Greece), NSRF: Heracleitus II, RFFR (Russia), and the Spanish Ministry of Economy and Competitiveness (MINECO) under Grants No. FPA2008-03456, No. FPA2011-24058 and No. EIC-CERN-2011-0006. This work was partially funded by the European Regional Development Fund (ERDF/FEDER), the European Research Council (ERC) under Grant No. ERC-2009-StG-240054 (T-REX), Turkish Atomic Energy Authority (TAEK), National Science Foundation (USA) under Award No. 0239812 and NASA under the Grant No. NAG5-10842. Part of this work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 68 TC 8 Z9 8 U1 3 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 28 PY 2015 VL 92 IS 2 AR 021101 DI 10.1103/PhysRevD.92.021101 PG 6 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CN7HW UT WOS:000358606200001 ER PT J AU Atanasov, D Blaum, K Bosch, F Brandau, C Buhler, P Chen, XC Dillmann, I Faestermann, T Gao, BS Geissel, H Gernhauser, R Hagmann, S Izumikawa, T Hillenbrand, PM Kozhuharov, C Kurcewicz, J Litvinov, SA Litvinov, YA Ma, XW Munzenberg, G Najafi, MA Nolden, F Ohtsubo, T Ozawa, A Ozturk, FC Patyk, Z Reed, M Reifarth, R Sanjari, MS Schneider, D Steck, M Stohlker, T Sun, BH Suzaki, F Suzuki, T Trageser, C Tu, XL Uesaka, T Walker, P Wang, M Weick, H Winckler, N Woods, P Xu, HS Yamaguchi, T Yan, XL Zhang, YH AF Atanasov, Dinko Blaum, Klaus Bosch, Fritz Brandau, Carsten Buehler, Paul Chen, Xiangcheng Dillmann, Iris Faestermann, Thomas Gao, Bingshui Geissel, Hans Gernhaeuser, Roman Hagmann, Siegbert Izumikawa, Takuji Hillenbrand, Pierre-Michel Kozhuharov, Christophor Kurcewicz, Jan Litvinov, Sergey A. Litvinov, Yuri A. Ma, Xinwen Muenzenberg, Gottfried Najafi, Mohammad Ali Nolden, Fritz Ohtsubo, Takashi Ozawa, Akira Ozturk, Fatma Cagla Patyk, Zygmunt Reed, Matthew Reifarth, Rene Sanjari, Mohammad Shahab Schneider, Dieter Steck, Markus Stoehlker, Thomas Sun, Baohua Suzaki, Fumi Suzuki, Takeshi Trageser, Christian Tu, Xiaolin Uesaka, Tomohiro Walker, Philip Wang, Meng Weick, Helmut Winckler, Nicolas Woods, Philip Xu, Hushan Yamaguchi, Takayuki Yan, Xinliang Zhang, Yuhu CA FRS-ESR ILIMA SPARC TBWD Collaborations TI Between atomic and nuclear physics: radioactive decays of highly-charged ions SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article DE highly charged ions; radioactive decays; storage rings ID FRS-ESR FACILITY; STORED EXOTIC NUCLEI; ORBITAL ELECTRON-CAPTURE; ISOCHRONOUS MASS-SPECTROMETRY; EXPERIMENTAL STORAGE-RING; HALF-LIFE MEASUREMENTS; STATE BETA-DECAY; RESONANT SCHOTTKY PICKUP; RELATIVISTIC HEAVY-IONS; LARGE-SCALE MASS AB Highly charged radioactive ions can be stored for extended periods of time in storage rings which allows for precision measurements of their decay modes. The straightforward motivation for performing such studies is that fully ionised nuclei or few-electron ions can be viewed as clean quantum-mechanical systems, in which the interactions of the many electrons can be either excluded or treated precisely. Thus, the influence of the electron shell on the decay probability can be investigated. Another important motivation is stellar nucleosynthesis, which proceeds at high temperatures and the involved atoms are therefore highly ionised. Presented here is a compact review of the relevant experiments conducted at heavy-ion storage rings. Furthermore, we outline the perspectives for future experiments at new-generation storage-ring facilities. C1 [Atanasov, Dinko; Bosch, Fritz; Brandau, Carsten; Chen, Xiangcheng; Dillmann, Iris; Gao, Bingshui; Geissel, Hans; Hagmann, Siegbert; Hillenbrand, Pierre-Michel; Kozhuharov, Christophor; Litvinov, Sergey A.; Litvinov, Yuri A.; Muenzenberg, Gottfried; Najafi, Mohammad Ali; Nolden, Fritz; Ozturk, Fatma Cagla; Sanjari, Mohammad Shahab; Steck, Markus; Stoehlker, Thomas; Trageser, Christian; Tu, Xiaolin; Weick, Helmut; Winckler, Nicolas] GSI Helmholtzzentrum Schwerionenforsch, D-64291 Darmstadt, Germany. [Atanasov, Dinko; Blaum, Klaus; Gao, Bingshui; Litvinov, Yuri A.; Tu, Xiaolin; Winckler, Nicolas] Max Planck Inst Kernphys, D-69117 Heidelberg, Germany. [Blaum, Klaus; Litvinov, Yuri A.] Heidelberg Univ, Inst Phys, D-69120 Heidelberg, Germany. [Brandau, Carsten; Trageser, Christian] Univ Giessen, Inst Atom & Mol Phys, D-35392 Giessen, Germany. [Buehler, Paul] Stefan Meyer Inst Subatomare Phys, A-1090 Vienna, Austria. [Chen, Xiangcheng; Gao, Bingshui; Litvinov, Yuri A.; Ma, Xinwen; Tu, Xiaolin; Wang, Meng; Xu, Hushan; Yan, Xinliang; Zhang, Yuhu] Chinese Acad Sci, Inst Modern Phys, Lanzhou 730000, Peoples R China. [Dillmann, Iris; Geissel, Hans; Najafi, Mohammad Ali] Univ Giessen, Inst Phys 2, D-35392 Giessen, Germany. [Dillmann, Iris] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Faestermann, Thomas; Gernhaeuser, Roman; Najafi, Mohammad Ali] Tech Univ Munich, D-85748 Garching, Germany. [Gao, Bingshui] Univ Chinese Acad Sci, Beijing 100049, Peoples R China. [Hagmann, Siegbert; Reifarth, Rene] Goethe Univ Frankfurt, D-60438 Frankfurt, Germany. [Izumikawa, Takuji] Niigata Univ, Radioisotope Ctr, Niigata 9518510, Japan. [Kurcewicz, Jan] CERN, CH-1211 Geneva, Switzerland. [Ohtsubo, Takashi] Niigata Univ, Dept Phys, Niigata 9518510, Japan. [Ozawa, Akira] Univ Tsukuba, Inst Phys, Ibaraki 3058571, Japan. [Ozturk, Fatma Cagla] Istanbul Univ, Dept Phys, TR-34452 Istanbul, Turkey. [Patyk, Zygmunt] Natl Ctr Nucl Res, PL-00681 Warsaw, Poland. [Reed, Matthew] Australian Natl Univ, Dept Nucl Phys, RSPE, Canberra, ACT 2601, Australia. [Schneider, Dieter] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Stoehlker, Thomas] Helmholtz Inst Jena, D-07743 Jena, Germany. [Stoehlker, Thomas] Univ Jena, Inst Opt & Quantenelekt, D-07743 Jena, Germany. [Sun, Baohua] Beihang Univ, Sch Phys & Nucl Energy Engn, Beijing 100191, Peoples R China. [Suzaki, Fumi; Suzuki, Takeshi; Yamaguchi, Takayuki] Saitama Univ, Dept Phys, Saitama 3388570, Japan. [Uesaka, Tomohiro] RIKEN, Nishina Ctr Accelerator Based Sci, Wako, Saitama 3510198, Japan. [Walker, Philip] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England. [Woods, Philip] Univ Edinburgh, Sch Phys & Astron, Edinburgh EH9 3JZ, Midlothian, Scotland. RP Atanasov, D (reprint author), GSI Helmholtzzentrum Schwerionenforsch, D-64291 Darmstadt, Germany. EM y.litvinov@gsi.de RI Buehler, Paul/C-4851-2016; Sun, Baohua/C-6823-2009; OI Buehler, Paul/0000-0003-2049-1380; Sun, Baohua/0000-0001-9868-5711; Najafi, Mohammad Ali/0000-0002-2300-5301; Faestermann, Thomas/0000-0002-6603-8787 FU Helmholtz Alliance Program of the Helmholtz Association, 'Extremes of Density and Temperature: Cosmic Matter in the Laboratory' [HA216/EMMI]; Helmholtz Association [VH-NG 627]; HIC-for-FAIR through HGS-HIRE; DFG cluster of excellence 'Origin and Structure of the Universe' of the Technische Universitat Munchen; BMBF grant in the framework of the Internationale Zusammenarbeit in Bildung und Forschung [01DO12012]; BMBF [05P12RGFNJ-06GI7118, 06GI911I 70, 06GI7127/05P12R6FAN]; Japanese Ministry of Education, Science, Sport and Culture [A19204023, 25105506, 26287036]; External Cooperation Program of the Chinese Academy of Sciences [GJHZ1305]; 973 Program of China [2013CB834401]; National Natural Science Foundation of China [10925526, 11035007, U1232208, 11205205, 11235002]; Youth Innovation Promotion Association of the Chinese Academy of Sciences; Chinese Academy of Sciences [KJCX2-YW-N44]; joint Max Planck/CAS doctoral promotion program; UK STFC; Helmholtz/CAS Joint Research Group HCJRG [HCJRG-108] FX This work is in part supported by the Helmholtz/CAS Joint Research Group HCJRG (group no. HCJRG-108); the Helmholtz Alliance Program of the Helmholtz Association, contract no. HA216/EMMI 'Extremes of Density and Temperature: Cosmic Matter in the Laboratory'; the Helmholtz Association via the Young Investigators Project VH-NG 627; HIC-for-FAIR through HGS-HIRE; the DFG cluster of excellence 'Origin and Structure of the Universe' of the Technische Universitat Munchen; the BMBF grant in the framework of the Internationale Zusammenarbeit in Bildung und Forschung Projekt-Nr. 01DO12012; BMBF (contracts 05P12RGFNJ-06GI7118, 06GI911I 70 and 06GI7127/05P12R6FAN); the Japanese Ministry of Education, Science, Sport and Culture by Grant-In-Aid for Science Research under program nos. A19204023, 25105506, and 26287036; the External Cooperation Program of the Chinese Academy of Sciences grant no. GJHZ1305; the 973 Program of China (no. 2013CB834401); the National Natural Science Foundation of China through grant nos. 10925526, 11035007, U1232208, 11205205, 11235002; the Youth Innovation Promotion Association of the Chinese Academy of Sciences; the Chinese Academy of Sciences through grant no. KJCX2-YW-N44; the joint Max Planck/CAS doctoral promotion program; and by the UK STFC. NR 278 TC 4 Z9 4 U1 9 U2 35 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 EI 1361-6455 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD JUL 28 PY 2015 VL 48 IS 14 SI SI AR 144024 DI 10.1088/0953-4075/48/14/144024 PG 16 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CM2RN UT WOS:000357529800025 ER PT J AU Beiersdorfer, P AF Beiersdorfer, P. TI Highly charged ions in magnetic fusion plasmas: research opportunities and diagnostic necessities SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article DE highly charged ions; tokamaks; x-rays ID X-RAY SPECTROSCOPY; DIELECTRONIC SATELLITE SPECTRA; EXCITATION CROSS-SECTIONS; HIGH-TEMPERATURE PLASMAS; PRINCETON LARGE TORUS; HELIUM-LIKE NICKEL; COLLISIONAL IONIZATION EQUILIBRIUM; TRANSMISSION GRATING SPECTROMETER; HIGH-RESOLUTION MEASUREMENTS; DENSITY-SENSITIVE LINES AB Highly charged ions play a crucial role in magnetic fusion plasmas. These plasmas are excellent sources for producing highly charged ions and copious amounts of radiation for studying their atomic properties. These studies include calibration of density diagnostics, x-ray production by charge exchange, line identifications and accurate wavelength measurements, and benchmark data for ionization balance calculations. Studies of magnetic fusion plasmas also consume a large amount of atomic data, especially in order to develop new spectral diagnostics. Examples we give are the need for highly accurate wavelengths as references for measurements of bulk plasma motion, the need for accurate line excitation rates that encompass both electron-impact excitation and indirect line formation processes, for accurate position and resonance strength information of dielectronic recombination satellite lines that may broaden or shift diagnostic lines or that may provide electron temperature information, and the need for accurate ionization balance calculations. We show that the highly charged ions of several elements are of special current interest to magnetic fusion, notably highly charged ions of argon, iron, krypton, xenon, and foremost of tungsten. The electron temperatures thought to be achievable in the near future may produce W70+ ions and possibly ions with even higher charge states. This means that all but a few of the most highly charged ions are of potential interest as plasma diagnostics or are available for basic research. C1 Lawrence Livermore Natl Lab, Dept Phys, Livermore, CA 94550 USA. RP Beiersdorfer, P (reprint author), Lawrence Livermore Natl Lab, Dept Phys, Livermore, CA 94550 USA. EM beiersdorfer@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; DOE Office of Fusion Energy Sciences FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 and supported by the DOE Office of Fusion Energy Sciences. This work was carried out in part as a contribution to the International Atomic Energy Agency Coordinated Research Project 'Spectroscopic and Collisional Data for Tungsten from 1 eV to 20 keV.' NR 259 TC 9 Z9 9 U1 9 U2 32 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 EI 1361-6455 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD JUL 28 PY 2015 VL 48 IS 14 SI SI AR 144017 DI 10.1088/0953-4075/48/14/144017 PG 24 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CM2RN UT WOS:000357529800018 ER PT J AU Fontes, CJ Zhang, HL Jr, JA Clark, REH Kilcrease, DP Colgan, J Cunningham, RT Hakel, P Magee, NH Sherrill, ME AF Fontes, C. J. Zhang, H. L. Abdallah, J. Clark, R. E. H. Kilcrease, D. P. Colgan, J. Cunningham, R. T. Hakel, P. Magee, N. H. Sherrill, M. E. TI The Los Alamos suite of relativistic atomic physics codes SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article DE relativistic atomic physics; collisional-radiative modeling; generalized Breit; interaction ID ELECTRON-IMPACT IONIZATION; HIGHLY-CHARGED IONS; CROSS-SECTIONS; TRANSITION ARRAYS; WORKSHOP; SPECTRA; OPACITY; HYDROGENLIKE; EXCITATION; SCATTERING AB The Los Alamos suite of relativistic atomic physics codes is a robust, mature platform that has been used to model highly charged ions in a variety of ways. The suite includes capabilities for calculating data related to fundamental atomic structure, as well as the processes of photoexcitation, electron-impact excitation and ionization, photoionization and autoionization within a consistent framework. These data can be of a basic nature, such as cross sections and collision strengths, which are useful in making predictions that can be compared with experiments to test fundamental theories of highly charged ions, such as quantum electrodynamics. The suite can also be used to generate detailed models of energy levels and rate coefficients, and to apply them in the collisional-radiative modeling of plasmas over a wide range of conditions. Such modeling is useful, for example, in the interpretation of spectra generated by a variety of plasmas. In this work, we provide a brief overview of the capabilities within the Los Alamos relativistic suite along with some examples of its application to the modeling of highly charged ions. C1 [Fontes, C. J.; Zhang, H. L.; Abdallah, J.; Clark, R. E. H.; Kilcrease, D. P.; Colgan, J.; Cunningham, R. T.; Hakel, P.; Magee, N. H.; Sherrill, M. E.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Fontes, CJ (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM cjf@lanl.gov OI Hakel, Peter/0000-0002-7936-4231; Kilcrease, David/0000-0002-2319-5934 FU National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396] FX The authors wish to thank Yu Ralchenko and G Csanak for useful discussions. We would also like to thank SB Hansen for providing the gold experimental spectral data. This work was carried out under the auspices of the National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory and supported by contract no DE-AC52-06NA25396. NR 73 TC 24 Z9 24 U1 1 U2 10 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 EI 1361-6455 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD JUL 28 PY 2015 VL 48 IS 14 SI SI AR 144014 DI 10.1088/0953-4075/48/14/144014 PG 17 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CM2RN UT WOS:000357529800015 ER PT J AU Gumberidze, A Thorn, DB Fontes, CJ Najjari, B Zhang, HL Surzhykov, A Voitkiv, A Fritzsche, S Banas, D Beyer, H Chen, W DuBois, RD Geyer, S Grisenti, RE Hagmann, S Hegewald, M Hess, S Kozhuharov, C Martin, R Petridis, N Reuschl, R Simon, A Spillmann, U Trassinelli, M Trotsenko, S Weber, G Winters, DFA Winters, N Yu, D Stholker, T AF Gumberidze, A. Thorn, D. B. Fontes, C. J. Najjari, B. Zhang, H. L. Surzhykov, A. Voitkiv, A. Fritzsche, S. Banas, D. Beyer, H. Chen, W. DuBois, R. D. Geyer, S. Grisenti, R. E. Hagmann, S. Hegewald, M. Hess, S. Kozhuharov, C. Maertin, R. Petridis, N. Reuschl, R. Simon, A. Spillmann, U. Trassinelli, M. Trotsenko, S. Weber, G. Winters, D. F. A. Winters, N. Yu, D. Sthoelker, T. TI Ground-state excitation of heavy highly-charged ions SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article DE highly-charged ions; x-rays; storage rings; relativistic collisions; excitation; Breit interaction ID GENERALIZED BREIT INTERACTION; INTERMEDIATE VELOCITY RANGE; RADIATIVE ELECTRON-CAPTURE; BARE URANIUM IONS; CROSS-SECTIONS; DIELECTRONIC-RECOMBINATION; MAGNETIC SUBLEVELS; ATOM COLLISIONS; IMPACT; HE AB We have studied the excitation of H-like and He-like uranium (U91+ and U90+) in relativistic collisions with gaseous targets by observing the subsequent x-ray emission. The experiment was conducted at the ESR storage ring of the GSI accelerator facility in Darmstadt, Germany. The measurements were performed with a newly developed multi-phase target at different collision energies. This enabled us to explore the proton (nucleus) impact excitation as well as the electron impact excitation processes in the relativistic collisions. The large fine-structure splitting in uranium allowed us to unambiguously resolve excitation to different L-shell levels. Moreover, information about the population of different magnetic sublevels has been obtained via an angular differential study of the decay photons associated with the subsequent de-excitation process. The experimental results are compared with calculations performed within the relativistic framework including excitation mechanisms due to both protons (nucleus) and electrons. C1 [Gumberidze, A.; Beyer, H.; Chen, W.; Geyer, S.; Grisenti, R. E.; Hagmann, S.; Hegewald, M.; Hess, S.; Kozhuharov, C.; Petridis, N.; Reuschl, R.; Spillmann, U.; Winters, D. F. A.; Winters, N.; Sthoelker, T.] GSI Helmholtzzentrum Schwerionenforsch, D-64291 Darmstadt, Germany. [Thorn, D. B.] GSI Helmholtzzentrum Schwerionenforsch, ExtreMe Matter Inst EMMI, D-64291 Darmstadt, Germany. [Thorn, D. B.] GSI Helmholtzzentrum Schwerionenforsch, Div Res, D-64291 Darmstadt, Germany. [Thorn, D. B.] Frankfurt Inst Adv Studies, D-60438 Frankfurt, Germany. [Fontes, C. J.; Zhang, H. L.] Los Alamos Natl Lab, Computat Phys Div, Los Alamos, NM 87545 USA. [Najjari, B.] Inst Pluridisciplinaire Hubert Curien, Grp RaMsEs, F-67037 Strasbourg, France. [Surzhykov, A.; Fritzsche, S.; Beyer, H.; Maertin, R.; Trotsenko, S.; Weber, G.; Sthoelker, T.] Helmholtz Inst Jena, D-07743 Jena, Germany. [Voitkiv, A.] Univ Dusseldorf, Theoret Phys 1, D-40225 Dusseldorf, Germany. [Fritzsche, S.; Sthoelker, T.] Univ Jena, IOQ, D-07743 Jena, Germany. [Banas, D.] Jan Kochanowski Univ Humanities & Sci, Inst Phys, PL-25406 Kielce, Poland. [DuBois, R. D.] Missouri Univ Sci & Technol, Rolla, MO USA. [Geyer, S.; Grisenti, R. E.; Hagmann, S.; Hegewald, M.; Hess, S.] Goethe Univ Frankfurt, Inst Kernphys, D-60486 Frankfurt, Germany. [Simon, A.] Michigan State Univ, NSCL, E Lansing, MI 48223 USA. [Trassinelli, M.] CNRS, Inst NanoSci Paris, F-75005 Paris, France. [Trassinelli, M.] Univ Paris 06, Inst NanoSci Paris, Sorbonne Univ, F-75005 Paris, France. [Yu, D.] Inst Modern Phys, Lanzhou 730000, Peoples R China. RP Gumberidze, A (reprint author), GSI Helmholtzzentrum Schwerionenforsch, D-64291 Darmstadt, Germany. EM a.gumberidze@gsi.de RI Banas, Dariusz/F-5025-2011; Trassinelli, Martino/M-5326-2016 OI Banas, Dariusz/0000-0003-1566-5446; Trassinelli, Martino/0000-0003-4414-1801 FU Helmholtz Alliance Program of the Helmholtz Association [HA216/EMMI] FX This work was supported by the Helmholtz Alliance Program of the Helmholtz Association, contract HA216/EMMI 'Extremes of Density and Temperature: Cosmic Matter in the Laboratory'. NR 42 TC 0 Z9 0 U1 0 U2 25 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 EI 1361-6455 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD JUL 28 PY 2015 VL 48 IS 14 SI SI AR 144006 DI 10.1088/0953-4075/48/14/144006 PG 5 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CM2RN UT WOS:000357529800007 ER PT J AU Pindzola, MS Lee, TG Colgan, J AF Pindzola, M. S. Lee, T. G. Colgan, J. TI Energy differential cross sections for F9+-impact single and double ionization of He SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article DE atoms; ionization; differential ID COLLISIONS; HELIUM; ELECTRONS; ATOMS; IONS AB Time-dependent close-coupling methods are used to calculate energy differential cross sections for the single and double ionization of He by impact with F9+ ions at 4.0 MeV amu(-1). Single ionization energy differential cross sections using both a one active electron method and a two active electron method are compared with recent experimental results. Double ionization energy differential cross sections using a two active electron method are presented to guide future experiments. C1 [Pindzola, M. S.; Lee, T. G.] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. [Colgan, J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM USA. RP Pindzola, MS (reprint author), Auburn Univ, Dept Phys, Auburn, AL 36849 USA. EM tgl0002@auburn.edu FU US Department of Energy; US National Science Foundation FX We would like to thank D Misra of the Tata Institute of Fundamental Research for providing us with the low energy experimental data. This work was supported in part by grants from the US Department of Energy and the US National Science Foundation. Computational work was carried out at the National Energy Research Scientific Computing Center in Oakland, California. NR 10 TC 1 Z9 1 U1 0 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 EI 1361-6455 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD JUL 28 PY 2015 VL 48 IS 14 SI SI AR 144019 DI 10.1088/0953-4075/48/14/144019 PG 6 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CM2RN UT WOS:000357529800020 ER PT J AU Rice, JE Reinke, ML Ashbourn, JMA Gao, C Bitter, M Delgado-Aparicio, L Hill, K Howard, NT Hughes, JW Safronova, UI AF Rice, J. E. Reinke, M. L. Ashbourn, J. M. A. Gao, C. Bitter, M. Delgado-Aparicio, L. Hill, K. Howard, N. T. Hughes, J. W. Safronova, U. I. TI X-ray observations of medium Z H- and He-like ions with satellites from C-Mod tokamak plasmas SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article DE x-ray spectra; H-like ions; He-like ions; satellites ID CHARGED HELIUM-LIKE; HYDROGEN-LIKE IONS; ELECTRON-IMPACT EXCITATION; LASER-PRODUCED PLASMAS; LITHIUM-LIKE IONS; IMPURITY TRANSPORT; EXCITED-STATES; LINE EMISSION; TI-XXII; FE-XXV AB X-ray spectra of H- and He-like ions (and satellites) from argon, calcium and chlorine have been measured in Alcator C-Mod tokamak plasmas using a high wavelength resolution imaging x-ray spectrometer system. For H-like charge states, the Ly(alpha) doublet intensity ratio is found to be slightly greater than 1/2 due to interaction with the S-2(1/2) fine structure sub-level. Neighbouring satellites with spectator electrons occupying n = 2 through n = 7 have been modelled. The Ly(alpha) doublet ratio scalings with electron density and temperature are shown to be in good agreement with collisional-radiative modelling. For He-like ions, the n = 2 satellite intensities are in good agreement with calculations and can be used to determine the electron temperature. The high n Rydberg series has been resolved up to 1s(2)-1s14p, and satellites with spectator electrons up to the n = 12 level have been identified. C1 [Rice, J. E.; Gao, C.; Howard, N. T.; Hughes, J. W.] MIT, Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA. [Ashbourn, J. M. A.] Univ Oxford, Math Inst, Oxford, England. [Bitter, M.; Delgado-Aparicio, L.; Hill, K.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Safronova, U. I.] Univ Nevada, Reno, NV 89557 USA. RP Rice, JE (reprint author), MIT, Plasma Sci & Fus Ctr, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM rice@psfc.mit.edu FU DoE [DE-FC02-99ER54512] FX The authors would like to thank M Chilenski, K Fournier, M Gu, A Hubbard, A Ince-Cushman, B LaBombard, Y Podpaly, S Wolfe and the Alcator C-Mod operations and ICRF groups for expert running of the tokamak. Work at MIT was supported by DoE Contract No. DE-FC02-99ER54512 and in part by an appointment to the US DoE Fusion Energy Post-doctoral Research Program administered by ORISE. NR 84 TC 2 Z9 2 U1 0 U2 8 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 EI 1361-6455 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD JUL 28 PY 2015 VL 48 IS 14 SI SI AR 144013 DI 10.1088/0953-4075/48/14/144013 PG 8 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CM2RN UT WOS:000357529800014 ER PT J AU Schippers, S Borovik, A Buhr, T Hellhund, J Holste, K Kilcoyne, ALD Klumpp, S Martins, M Muller, A Ricz, S Fritzsche, S AF Schippers, S. Borovik, A., Jr. Buhr, T. Hellhund, J. Holste, K. Kilcoyne, A. L. D. Klumpp, S. Martins, M. Mueller, A. Ricz, S. Fritzsche, S. TI Stepwise contraction of the nf Rydberg shells in the 3d photoionization of multiply-charged xenon ions SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article DE photoionization of ions; synchrotron radiation; atomic structure ID 4F WAVE-FUNCTION; BA; XE; SEQUENCE; COLLAPSE; CS; PHOTOABSORPTION; SPECTRA AB Triple photoionization of Xe3+, Xe4+ and Xe5+ ions has been studied in the energy range 670-750 eV, including the 3d ionization threshold. The photon-ion merged-beam technique was used at a synchrotron light source to measure the absolute photoionization cross sections. These cross sections exhibit a progressively larger number of sharp resonances as the ion charge state is increased. This clearly visualizes the re-ordering of the epsilon f continuum into a regular series of (bound) Rydberg orbitals as the ionic core becomes more attractive. The energies and strengths of the resonances are extracted from the experimental data and are further analysed by relativistic atomic-structure calculations. C1 [Schippers, S.; Borovik, A., Jr.; Hellhund, J.; Holste, K.; Mueller, A.] Univ Giessen, Inst Atom & Mol Phys, D-35392 Giessen, Germany. [Buhr, T.] Phys Tech Bundesanstalt, D-38116 Braunschweig, Germany. [Kilcoyne, A. L. D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Klumpp, S.; Martins, M.] Univ Hamburg, Inst Expt Phys, D-22761 Hamburg, Germany. [Ricz, S.] Hungarian Acad Sci, Inst Nucl Res, H-4001 Debrecen, Hungary. [Fritzsche, S.] Helmholtz Inst Jena, D-07743 Jena, Germany. [Fritzsche, S.] Univ Jena, Inst Theoret Phys, D-07743 Jena, Germany. RP Schippers, S (reprint author), Univ Giessen, Inst Atom & Mol Phys, D-35392 Giessen, Germany. EM stefan.schippers@physik.uni-giessen.de RI Muller, Alfred/A-3548-2009; Kilcoyne, David/I-1465-2013; Schippers, Stefan/A-7786-2008; OI Muller, Alfred/0000-0002-0030-6929; Schippers, Stefan/0000-0002-6166-7138; Martins, Michael/0000-0002-1228-5029 FU German ministry for education and research (BMBF) within the 'Verbundforschung' funding scheme [05K10RG1, 05K10GUB] FX This research was carried out at the light source PETRA III at DESY, a member of the Helmholtz Association (HGF). We would like to thank L Glaser, F Scholz, J Seltmann, and J Viefhaus for assistance in using beamline P04. This research has been funded in part by the German ministry for education and research (BMBF) under contracts 05K10RG1 and 05K10GUB within the 'Verbundforschung' funding scheme. NR 32 TC 1 Z9 1 U1 0 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 EI 1361-6455 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD JUL 28 PY 2015 VL 48 IS 14 SI SI AR 144003 DI 10.1088/0953-4075/48/14/144003 PG 6 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CM2RN UT WOS:000357529800004 ER PT J AU Ngan, CY Wong, CH Choi, C Yoshinaga, Y Louie, K Jia, J Chen, C Bowen, B Cheng, HY Leonelli, L Kuo, R Baran, R Garcia-Cerdan, JG Pratap, A Wang, M Lim, J Tice, H Daum, C Xu, J Northen, T Visel, A Bristow, J Niyogi, KK Wei, CL AF Ngan, Chew Yee Wong, Chee-Hong Choi, Cindy Yoshinaga, Yuko Louie, Katherine Jia, Jing Chen, Cindy Bowen, Benjamin Cheng, Haoyu Leonelli, Lauriebeth Kuo, Rita Baran, Richard Garcia-Cerdan, Jose G. Pratap, Abhishek Wang, Mei Lim, Joanne Tice, Hope Daum, Chris Xu, Jian Northen, Trent Visel, Axel Bristow, James Niyogi, Krishna K. Wei, Chia-Lin TI Lineage-specific chromatin signatures reveal a regulator of lipid metabolism in microalgae SO NATURE PLANTS LA English DT Article ID CHLAMYDOMONAS-REINHARDTII; GENOME-WIDE; TRIACYLGLYCEROL ACCUMULATION; EPIGENETIC MODIFICATIONS; DEPRIVATION RESPONSES; BIODIESEL PRODUCTION; HISTONE METHYLATION; BIOFUEL PRODUCTION; PHOSPHORUS; ARABIDOPSIS AB Alga-derived lipids represent an attractive potential source of biofuels. However, lipid accumulation in algae is a stress response tightly coupled to growth arrest, thereby imposing a major limitation on productivity. To identify transcriptional regulators of lipid accumulation, we performed an integrative chromatin signature and transcriptomic analysis to decipher the regulation of lipid biosynthesis in the alga Chlamydomonas reinhardtii. Genome-wide histone modification profiling revealed remarkable differences in functional chromatin states between the algae and higher eukaryotes and uncovered regulatory components at the core of lipid accumulation pathways. We identified the transcription factor, PSR1, as a pivotal switch that triggers cytosolic lipid accumulation. Dissection of the PSR1-induced lipid profiles corroborates its role in coordinating multiple lipid-inducing stress responses. The comprehensive maps of functional chromatin signatures in a major clade of eukaryotic life and the discovery of a transcriptional regulator of algal lipid metabolism will facilitate targeted engineering strategies to mediate high lipid production in microalgae. C1 [Ngan, Chew Yee; Wong, Chee-Hong; Choi, Cindy; Yoshinaga, Yuko; Louie, Katherine; Chen, Cindy; Bowen, Benjamin; Cheng, Haoyu; Kuo, Rita; Pratap, Abhishek; Wang, Mei; Lim, Joanne; Tice, Hope; Daum, Chris; Northen, Trent; Visel, Axel; Bristow, James; Wei, Chia-Lin] US DOE, Joint Genorne Inst, Walnut Creek, CA 94598 USA. [Louie, Katherine; Bowen, Benjamin; Baran, Richard; Northen, Trent] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Jia, Jing; Xu, Jian] Chinese Acad Sci, Qingdao Inst BioEnergy & Bioproc Technol, Single Cell Ctr, CAS Key Lab Biofuels, Qingdao 266101, Shandong, Peoples R China. [Jia, Jing; Xu, Jian] Chinese Acad Sci, Qingdao Inst BioEnergy & Bioproc Technol, Shandong Key Lab Energy Genet, Qingdao 266101, Shandong, Peoples R China. [Leonelli, Lauriebeth; Garcia-Cerdan, Jose G.; Niyogi, Krishna K.] Univ Calif Berkeley, Howard Hughes Med Inst, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Visel, Axel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Genom Div, Berkeley, CA 94720 USA. [Visel, Axel] Univ Calif, Sch Nat Sci, Merced, CA 95343 USA. [Niyogi, Krishna K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Wei, CL (reprint author), US DOE, Joint Genorne Inst, Walnut Creek, CA 94598 USA. EM cwei@lbl.gov RI Visel, Axel/A-9398-2009; OI Visel, Axel/0000-0002-4130-7784; ngan, chew yee/0000-0001-6055-1072; Northen, Trent/0000-0001-8404-3259 FU Laboratory Directed Research and Development program at Lawrence Berkeley National Laboratory; Gordon and Betty Moore Foundation [GBMF3070]; Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX The authors thank S. Prochnik and P. Tran for their disc on and comments on the manuscript, I. Pennacchio for initiating effort in setting-up the C. reinhardtii culture, M. Kobayashi for technical advice on C reinhardtii culture, R. Acob Agbayani and J. Chow for execution of part of the experiments, S. Deshpande for coordinating sample processing and sequencing tracking. H.C. was supported by a grant from the Laboratory Directed Research and Development program at Lawrence Berkeley National Laboratory. K.K.N. is an investigator of the Howard Hughes Medical Institute and the Gordon and Betty Moore Foundation (through Grant GBMF3070). The work is conducted by the US Department of Energy Joint Genome Institute and supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 48 TC 8 Z9 8 U1 6 U2 15 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2055-026X EI 2055-0278 J9 NAT PLANTS JI Nat. Plants PD JUL 27 PY 2015 VL 1 IS 8 DI 10.1038/NPLANTS.2015.107 PG 11 WC Plant Sciences SC Plant Sciences GA CV6LC UT WOS:000364380700001 PM 27250540 ER PT J AU Anzai, C Hasselhuhn, A Hoschele, M Hoff, J Kilgore, W Steinhauser, M Ueda, T AF Anzai, Chihaya Hasselhuhn, Alexander Hoeschele, Maik Hoff, Jens Kilgore, William Steinhauser, Matthias Ueda, Takahiro TI Exact (NLO)-L-3 results for qq ' -> H plus X SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Higgs Physics; Effective field theories; QCD ID HIGGS-BOSON PRODUCTION; TO-LEADING ORDER; GLUON-FUSION; HARMONIC POLYLOGARITHMS; ANOMALOUS DIMENSIONS; VIRTUAL CORRECTIONS; FEYNMAN DIAGRAMS; HADRON COLLIDERS; CROSS-SECTIONS; MASS AB We compute the contribution to the total cross section for the inclusive production of a Standard Model Higgs boson induced by two quarks with different flavour in the initial state. Our calculation is exact in the Higgs boson mass and the partonic center-of-mass energy. We describe the reduction to master integrals, the construction of a canonical basis, and the solution of the corresponding differential equations. Our analytic result contains both Harmonic Polylogarithms and iterated integrals with additional letters in the alphabet. C1 [Anzai, Chihaya; Hasselhuhn, Alexander; Hoeschele, Maik; Steinhauser, Matthias] KIT, Inst Theoret Teilchenphys, D-76128 Karlsruhe, Germany. [Hoff, Jens] Deutsch Elektronen Synchrotron DESY, D-15738 Zeuthen, Germany. [Kilgore, William] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Ueda, Takahiro] Nikhef Theory Grp, NL-1098 XG Amsterdam, Netherlands. RP Anzai, C (reprint author), KIT, Inst Theoret Teilchenphys, Wolfgang Gaede Str 1, D-76128 Karlsruhe, Germany. EM chihaya.anzai@kit.edu; alexander.hasselhuhn@kit.edu; maik.hoeschele@kit.edu; jens.hoff@desy.de; kilgore@bnl.gov; matthias.steinhauser@kit.edu; tueda@nikhef.nl FU U.S. Department of Energy [DE-AC02-98CH10886]; European Commission [PITN-GA-2012-316704 (HIGGSTOOLS)]; BMBF [05H12VKE]; ERC Advanced Grant [320651 "HEPGAME"] FX We would like to thank Johannes Henn for many useful hints in connection to the construction of the canonical basis. The work of WBK is supported by the U.S. Department of Energy under Contract No. DE-AC02-98CH10886. Parts of this work were supported by the European Commission through contract PITN-GA-2012-316704 (HIGGSTOOLS), by BMBF through Grant No. 05H12VKE, and by the ERC Advanced Grant no. 320651 "HEPGAME". NR 93 TC 7 Z9 7 U1 0 U2 3 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JUL 27 PY 2015 IS 7 AR 140 DI 10.1007/JHEP07(2015)140 PG 26 WC Physics, Particles & Fields SC Physics GA CU4PV UT WOS:000363512900001 ER PT J AU Driben, R Yulin, AV Efimov, A AF Driben, R. Yulin, A. V. Efimov, A. TI Resonant radiation from oscillating higher order solitons SO OPTICS EXPRESS LA English DT Article ID PHOTONIC-CRYSTAL FIBERS; NONLINEAR PULSE-PROPAGATION; SELF-FREQUENCY SHIFT; OPTICAL-FIBERS; SUPERCONTINUUM GENERATION; CHERENKOV RADIATION; ADVANCED-STAGE; LINEAR WAVES; DISPERSION AB We present radiation mechanism exhibited by a higher order soliton. In a course of its evolution the higher-order soliton emits polychromatic radiation resulting in formation of multipeak frequency comb-like spectral band. The shape and spectral position of this band can be effectively controlled by the relative strength of the third order dispersion. An analytical description is corroborated by numerical simulations. It is shown that for longer pulses the described effect persists also under the action of higher order perturbations such as Raman and self-steepening. (C) 2015 Optical Society of America C1 [Driben, R.; Yulin, A. V.] ITMO Univ, Dept Nanophoton & Metamat, St Petersburg 197101, Russia. [Driben, R.] Univ Paderborn, Dept Phys, D-33098 Paderborn, Germany. [Yulin, A. V.] Univ Paderborn, CeOPP, D-33098 Paderborn, Germany. [Efimov, A.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol Mat Phys & Applica, Los Alamos, NM 87545 USA. RP Driben, R (reprint author), ITMO Univ, Dept Nanophoton & Metamat, 49 Kronverskii Ave, St Petersburg 197101, Russia. EM driben@mail.uni-paderborn.de RI Yulin, Alexey/B-6139-2015; OI Yulin, Alexey/0000-0002-2403-6564; Efimov, Anatoly/0000-0002-5559-4147 FU Russian Federation through ITMO Early Career Fellowship scheme [074-U01]; U.S. Department of Energy [DE-AC52-06NA25396] FX R.D. and A.V.Y gratefully acknowledges the support by the Russian Federation Grant 074-U01 through ITMO Early Career Fellowship scheme.; This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-AC52-06NA25396. NR 33 TC 4 Z9 4 U1 2 U2 7 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD JUL 27 PY 2015 VL 23 IS 15 BP 19112 EP 19117 DI 10.1364/OE.23.019112 PG 6 WC Optics SC Optics GA CR0TE UT WOS:000361035300054 PM 26367574 ER PT J AU Khanal, S Reno, JL Kumar, S AF Khanal, Sudeep Reno, John L. Kumar, Sushil TI 2.1 THz quantum-cascade laser operating up to 144 K based on a scattering-assisted injection design SO OPTICS EXPRESS LA English DT Article AB A 2.1 THz quantum cascade laser (QCL) based on a scattering-assisted injection and resonant-phonon depopulation design scheme is demonstrated. The QCL is based on a four-well period implemented in the GaAs/Al0.15Ga0.85As material system. The QCL operates up to a heat-sink temperature of 144 K in pulsed-mode, which is considerably higher than that achieved for previously reported THz QCLs operating around the frequency of 2 THz. At 46 K, the threshold current-density was measured as similar to 745 A/cm(2) with a peak-power output of similar to 10 mW. Electrically stable operation in a positive differential-resistance regime is achieved by a careful choice of design parameters. The results validate the robustness of scattering-assisted injection schemes for development of low-frequency (v < 2.5 THz) QCLs. (C) 2015 Optical Society of America C1 [Khanal, Sudeep; Kumar, Sushil] Lehigh Univ, Dept Elect Engn & Comp Sci, Bethlehem, PA 18015 USA. [Reno, John L.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. RP Khanal, S (reprint author), Lehigh Univ, Dept Elect Engn & Comp Sci, Bethlehem, PA 18015 USA. EM suk311@lehigh.edu FU United States National Science Foundation [ECCS 1128562, ECCS 1351142]; U.S. DOE's National Nuclear Security Administration [DE-AC04-94AL85000] FX This material is based upon work supported by the United States National Science Foundation under Grant Nos. ECCS 1128562 and ECCS 1351142. The work is also performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy (DOE), Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. DOE's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 21 TC 5 Z9 5 U1 3 U2 17 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD JUL 27 PY 2015 VL 23 IS 15 BP 19689 EP 19697 DI 10.1364/OE.23.019689 PG 9 WC Optics SC Optics GA CR0TE UT WOS:000361035300106 PM 26367626 ER PT J AU Grobner, J Reda, I Wacker, S Nyeki, S Behrens, K Gorman, J AF Groebner, Julian Reda, Ibrahim Wacker, Stefan Nyeki, Stephan Behrens, Klaus Gorman, J. TI Reply to comment by R. Philipona on "A new absolute reference for atmospheric longwave irradiance measurements with traceability to SI units" SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Editorial Material DE Atmospheric longwave radiation C1 [Groebner, Julian; Wacker, Stefan; Nyeki, Stephan] Physikal Meteorol Observatorium Davos World Radia, Davos, Switzerland. [Reda, Ibrahim] Natl Renewable Energy Lab, Golden, CO USA. [Behrens, Klaus] Deutsch Wetterdienst, Meteorol Observatorium Lindenberg Richard Assmann, Lindenberg, Germany. [Gorman, J.] Bur Meteorol, Melbourne, Vic, Australia. RP Grobner, J (reprint author), Physikal Meteorol Observatorium Davos World Radia, Davos, Switzerland. EM julian.groebner@pmodwrc.ch NR 4 TC 1 Z9 1 U1 0 U2 1 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD JUL 27 PY 2015 VL 120 IS 14 BP 6885 EP 6886 DI 10.1002/2015JD023345 PG 2 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA CP3TL UT WOS:000359804900011 ER PT J AU Zhang, Y Zhang, X Wang, K He, J Leung, LR Fan, JW Nenes, A AF Zhang, Yang Zhang, Xin Wang, Kai He, Jian Leung, L. Ruby Fan, Jiwen Nenes, Athanasios TI Incorporating an advanced aerosol activation parameterization into WRF-CAM5: Model evaluation and parameterization intercomparison SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE WRF-CAM5; CCN activation; aerosol indirect effects; model improvement and evaluation; East Asia ID COMMUNITY ATMOSPHERE MODEL; POLLUTION CONTROL POLICIES; GENERAL-CIRCULATION MODEL; CLOUD DROPLET FORMATION; AIR-QUALITY BENEFITS; PART I; CLIMATE MODELS; METEOROLOGICAL PREDICTIONS; SPECTRUM FORMATION; CUMULUS CLOUDS AB Aerosol activation into cloud droplets is an important process that governs aerosol indirect effects. The advanced treatment of aerosol activation by Fountoukis and Nenes (2005) and its recent updates, collectively called the FN series, have been incorporated into a newly developed regional coupled climate-air quality model based on the Weather Research and Forecasting model with the physics package of the Community Atmosphere Model version 5 (WRF-CAM5) to simulate aerosol-cloud interactions in both resolved and convective clouds. The model is applied to East Asia for two full years of 2005 and 2010. A comprehensive model evaluation is performed for model predictions of meteorological, radiative, and cloud variables, chemical concentrations, and column mass abundances against satellite data and surface observations from air quality monitoring sites across East Asia. The model performs overall well for major meteorological variables including near-surface temperature, specific humidity, wind speed, precipitation, cloud fraction, precipitable water, downward shortwave and longwave radiation, and column mass abundances of CO, SO2, NO2, HCHO, and O-3 in terms of both magnitudes and spatial distributions. Larger biases exist in the predictions of surface concentrations of CO and NOx at all sites and SO2, O-3, PM2.5, and PM10 concentrations at some sites, aerosol optical depth, cloud condensation nuclei over ocean, cloud droplet number concentration (CDNC), cloud liquid and ice water path, and cloud optical thickness. Compared with the default Abdul-Razzack Ghan (2000) parameterization, simulations with the FN series produce similar to 107-113% higher CDNC, with half of the difference attributable to the higher aerosol activation fraction by the FN series and the remaining half due to feedbacks in subsequent cloud microphysical processes. With the higher CDNC, the FN series are more skillful in simulating cloud water path, cloud optical thickness, downward shortwave radiation, shortwave cloud forcing, and precipitation. The model evaluation identifies several areas of improvements including emissions and their vertical allocation as well as model formulations such as aerosol formation, cloud droplet nucleation, and ice nucleation. C1 [Zhang, Yang; Zhang, Xin; Wang, Kai; He, Jian] N Carolina State Univ, Dept Marine Earth & Atmospher Sci, Raleigh, NC 27695 USA. [Zhang, Yang] Collaborat Innovat Ctr Reg Environm Qual, Beijing, Peoples R China. [Leung, L. Ruby; Fan, Jiwen] Pacific NW Natl Lab, Richland, WA 99352 USA. [Nenes, Athanasios] Georgia Inst Technol, Sch Earth & Atmospher Sci, Atlanta, GA 30332 USA. [Nenes, Athanasios] Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA. RP Zhang, Y (reprint author), N Carolina State Univ, Dept Marine Earth & Atmospher Sci, Box 8208, Raleigh, NC 27695 USA. EM yang_zhang@ncsu.edu RI Wang, Kai/D-4262-2013; Fan, Jiwen/E-9138-2011 OI Wang, Kai/0000-0002-2375-5989; FU U.S. Department of Energy, Office of Science Biological and Environmental Research as part of the Regional and Global Climate Modeling program [DE-SC0006695]; China National Basic Research Program [2010CB951803]; National Science Foundation [OCI-1053575]; National Energy Research Scientific Computing Center (NERSC); Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; DOE [DE-AC05-76RL01830] FX This work was sponsored by the U.S. Department of Energy, Office of Science Biological and Environmental Research as part of the Regional and Global Climate Modeling program (DE-SC0006695) and China National Basic Research Program (2010CB951803). Observational data in mainland China, Taiwan, Hong Kong, Japan, and South Korea, AERONET data, and satellite data were downloaded from their respective websites. Thanks are due to Ying Chen, a graduate student at NCSU for her help in performing the 2005 baseline simulation and downloading and processing observations over South Korea. This work used the Extreme Science and Engineering Discovery Environment (XSEDE) (KRAKEN and STAMPEDE), which is supported by the National Science Foundation grant number OCI-1053575, and the National Energy Research Scientific Computing Center (NERSC) (HOPPER), which is supported by the Office of Science of the U.S. Department of Energy under contract DE-AC02-05CH11231. The Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under contract DE-AC05-76RL01830. The data used to generate results presented in this paper will be available free of charge upon request; please contact Yang Zhang, yzhang9@ncsu.edu. NR 81 TC 8 Z9 8 U1 4 U2 24 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD JUL 27 PY 2015 VL 120 IS 14 BP 6952 EP 6979 DI 10.1002/2014JD023051 PG 28 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA CP3TL UT WOS:000359804900017 ER PT J AU Omitaomu, OA Singh, N Bhaduri, BL AF Omitaomu, Olufemi A. Singh, Nagendra Bhaduri, Budhendra L. TI Mapping suitability areas for concentrated solar power plants using remote sensing data SO JOURNAL OF APPLIED REMOTE SENSING LA English DT Article DE concentrated solar power; geographic information system; digital elevation model; power plant siting; solar radiation; solar power plant ID SATELLITE DATA; RADIATION MODEL; IRRADIANCE; CAPACITY; SURFACE; ENERGY AB The political push to increase power generation from renewable sources, such as solar energy, requires knowing the best places to site new solar power plants with respect to the applicable regulatory, operational, engineering, environmental, and socioeconomic criteria. Therefore, we present applications of remote sensing data for mapping suitable areas for concentrated solar power (CSP) plants. Our approach uses satellite data from National Aeronautical and Space Administration's Global Energy and Water Cycle Surface Radiation Budget project at a resolution of 1 deg for estimating global solar radiation for the study area. Then we develop a computational model built on a geographic information system (GIS) platform that divides the study area into a grid of cells and estimates the site suitability value for each cell by computing a list of metrics based on applicable site requirements using GIS data. The computed metrics include population density, solar energy potential, federal lands, and hazardous facilities. Overall, some 30 GIS datasets are used to compute eight metrics. The site suitability value for each cell is computed as an algebraic sum of all metrics for the cell with the assumption that all metrics have equal weight. Finally, we color each cell according to its suitability value. We present results for CSP that drives a stream turbine and parabolic mirror connected to a Stirling engine. (C) The Authors. Published by SPIE under a Creative Commons Attribution 3.0 Unported License. C1 [Omitaomu, Olufemi A.; Singh, Nagendra; Bhaduri, Budhendra L.] Oak Ridge Natl Lab, Geog Informat Sci & Technol Grp, Oak Ridge, TN 37831 USA. RP Omitaomu, OA (reprint author), Oak Ridge Natl Lab, Geog Informat Sci & Technol Grp, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM omitaomuoa@ornl.gov FU U.S. Department of Energy [DE-AC05-00OR22725] FX This manuscript is authored by employees of UT-Battelle, LLC, under contract DE-AC05-00OR22725 with the U.S. Department of Energy. Accordingly, the United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 41 TC 0 Z9 0 U1 8 U2 15 PU SPIE-SOC PHOTO-OPTICAL INSTRUMENTATION ENGINEERS PI BELLINGHAM PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98225 USA SN 1931-3195 J9 J APPL REMOTE SENS JI J. Appl. Remote Sens. PD JUL 27 PY 2015 VL 9 AR 097697 DI 10.1117/1.JRS.9.097697 PG 14 WC Environmental Sciences; Remote Sensing; Imaging Science & Photographic Technology SC Environmental Sciences & Ecology; Remote Sensing; Imaging Science & Photographic Technology GA CP3TP UT WOS:000359805300001 ER PT J AU Li, D Liu, T Zuo, XB Li, T Qiu, XY Evilevitch, A AF Li, Dong Liu, Ting Zuo, Xiaobing Li, Tao Qiu, Xiangyun Evilevitch, Alex TI Ionic switch controls the DNA state in phage lambda SO NUCLEIC ACIDS RESEARCH LA English DT Article ID DOUBLE-STRANDED DNA; ESCHERICHIA-COLI; IN-VITRO; BACTERIOPHAGE-LAMBDA; MAGNESIUM TRANSPORT; EJECTION FORCES; VIRUS; INFECTION; GENOME; PRESSURE AB We have recently found that DNA packaged in phage lambda undergoes a disordering transition triggered by temperature, which results in increased genome mobility. This solid-to-fluid like DNA transition markedly increases the number of infectious lambda particles facilitating infection. However, the structural transition strongly depends on temperature and ionic conditions in the surrounding medium. Using titration microcalorimetry combined with solution X-ray scattering, we mapped both energetic and structural changes associated with transition of the encapsidated lambda-DNA. Packaged DNA needs to reach a critical stress level in order for transition to occur. We varied the stress on DNA in the capsid by changing the temperature, packaged DNA length and ionic conditions. We found striking evidence that the intracapsid DNA transition is 'switched on' at the ionic conditions mimicking those in vivo and also at the physiologic temperature of infection at 37 degrees C. This ion regulated on-off switch of packaged DNA mobility in turn affects viral replication. These results suggest a remarkable adaptation of phage lambda to the environment of its host bacteria in the human gut. The metastable DNA state in the capsid provides a new paradigm for the physical evolution of viruses. C1 [Li, Dong; Liu, Ting; Evilevitch, Alex] Carnegie Mellon Univ, Dept Phys, Pittsburgh, PA 15213 USA. [Zuo, Xiaobing; Li, Tao] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Qiu, Xiangyun] George Washington Univ, Dept Phys, Washington, DC 20052 USA. [Evilevitch, Alex] Lund Univ, Dept Biochem & Struct Biol, SE-22100 Lund, Sweden. RP Evilevitch, A (reprint author), Carnegie Mellon Univ, Dept Phys, Pittsburgh, PA 15213 USA. EM alexe@cmu.edu RI Evilevitch, Alex/P-3103-2014; Li, Dong/D-9221-2015 OI Evilevitch, Alex/0000-0002-0245-9574; Li, Dong/0000-0002-5282-6918 FU Argonne National Laboratory for the US Department of Energy [DE-AC02-06CH11357]; Swedish Research Council VR [622-2008-726]; National Science Foundation [CHE-1152770] FX Argonne National Laboratory for the US Department of Energy [DE-AC02-06CH11357]; Swedish Research Council VR [622-2008-726 to A.E.]; National Science Foundation [CHE-1152770 to A.E.]. Funding for open access charge: Swedish Research Council VR [622-2008-726 to A.E.]; National Science Foundation [CHE-1152770 to A.E.]. NR 75 TC 3 Z9 3 U1 2 U2 12 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 EI 1362-4962 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD JUL 27 PY 2015 VL 43 IS 13 BP 6348 EP 6358 DI 10.1093/nar/gkv611 PG 11 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CP3JZ UT WOS:000359776500019 PM 26092697 ER PT J AU Ahmed, T Modine, NA Zhu, JX AF Ahmed, Towfiq Modine, N. A. Zhu, Jian-Xin TI Bonding between graphene and MoS2 monolayers without and with Li intercalation SO APPLIED PHYSICS LETTERS LA English DT Article ID LITHIUM ION BATTERIES; TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; ANODE; PSEUDOPOTENTIALS; PERFORMANCE; CAPACITY; METALS AB We performed density functional theory (DFT) calculations for a bi-layered heterostructure combining a graphene layer with a MoS2 layer with and without intercalated Li atoms. Our calculations demonstrate the importance of the van der Waals (vdW) interaction, which is crucial for forming stable bonding between the layers. Our DFT calculation correctly reproduces the linear dispersion, or Dirac cone, feature at the Fermi energy for the isolated graphene monolayer and the band gap for the MoS2 monolayer. For the combined graphene/MoS2 bi-layer, we observe interesting electronic structure and density of states (DOS) characteristics near the Fermi energy, showing both the gap like features of the MoS2 layer and in-gap states with linear dispersion contributed mostly by the graphene layer. Our calculated total DOS in this vdW heterostructure reveals that the graphene layer significantly contributes to pinning the Fermi energy at the center of the band gap of MoS2. We also find that intercalating Li ions in between the layers of the graphene/MoS2 heterostructure enhances the binding energy through orbital hybridizations between cations (Li adatoms) and anions (graphene and MoS2 monolayers). Moreover, we calculate the dielectric function of the Li intercalated graphene/MoS2 heterostructure, the imaginary component of which can be directly compared with experimental measurements of optical conductivity in order to validate our theoretical prediction. We observe sharp features in the imaginary component of the dielectric function, which shows the presence of a Drude peak in the optical conductivity, and therefore metallicity in the lithiated graphene/MoS2 heterostructure. (C) 2015 AIP Publishing LLC. C1 [Ahmed, Towfiq; Zhu, Jian-Xin] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Modine, N. A.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. [Zhu, Jian-Xin] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. RP Ahmed, T (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM atowfiq@lanl.gov; jxzhu@lanl.gov FU National Nuclear Security Administration of the U.S. DOE at Los Alamos National Laboratory [DE-AC52-06NA25396]; Sandia National Laboratories [DE-AC04-94AL85000]; U.S. DOE Office of Basics Energy Sciences; Center for Integrated Nanotechnologies-a U.S. DOE BES user facility FX We thank Jinkyoung Yoo and Enkeleda Dervishi for stimulating discussions. This work was carried out under the auspices of the National Nuclear Security Administration of the U.S. DOE at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396 and at Sandia National Laboratories under Contract No. DE-AC04-94AL85000. It was supported by the U.S. DOE Office of Basics Energy Sciences (T.A.) and was in part by the Center for Integrated Nanotechnologies-a U.S. DOE BES user facility (N.A.M. & J.-X.Z.). NR 30 TC 3 Z9 3 U1 20 U2 90 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUL 27 PY 2015 VL 107 IS 4 AR 043903 DI 10.1063/1.4927611 PG 5 WC Physics, Applied SC Physics GA CO1OF UT WOS:000358924200071 ER PT J AU Filippetto, D Qian, H Sannibale, F AF Filippetto, D. Qian, H. Sannibale, F. TI Cesium telluride cathodes for the next generation of high-average current high-brightness photoinjectors SO APPLIED PHYSICS LETTERS LA English DT Article ID GUN AB We report on the performances of a Cs2Te photocathode under extreme conditions of high peak time-dependent accelerating fields, continuous wave operations, and MHz pulse extraction with up to 0.3 mA average current. The measurements, performed in a normal conducting cavity, show extended lifetime and robustness, elucidate the main mechanisms for cathode degradation, and set the required system vacuum performance for compatibility with the operations of a high average power X-ray free electron laser user facility, opening the doors to the next generation of MHz-scale ultrafast scientific instruments. (C) 2015 AIP Publishing LLC. C1 [Filippetto, D.; Qian, H.; Sannibale, F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Filippetto, D (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, One Cyclotron Rd, Berkeley, CA 94720 USA. EM dfilippetto@lbl.gov OI Qian, Houjun/0000-0002-3213-0892 FU DOE [DE-AC02-05CH11231] FX The authors would like to thank M. Zolotorev for useful discussions, Russell Wells for the coordination of all mechanical activities that allowed us to perform the presented measurements, and to the personnel of INFN/LASA for providing the cathodes. The authors acknowledge support from DOE Grant No. DE-AC02-05CH11231. NR 20 TC 1 Z9 1 U1 2 U2 5 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUL 27 PY 2015 VL 107 IS 4 AR 042104 DI 10.1063/1.4927700 PG 5 WC Physics, Applied SC Physics GA CO1OF UT WOS:000358924200039 ER PT J AU Lee, J Trugman, SA Zhang, CL Talbayev, D Xu, XS Cheong, SW Yarotski, DA Taylor, AJ Prasankumar, RP AF Lee, J. Trugman, S. A. Zhang, C. L. Talbayev, D. Xu, X. S. Cheong, S. -W. Yarotski, D. A. Taylor, A. J. Prasankumar, R. P. TI The influence of charge and magnetic order on polaron and acoustic phonon dynamics in LuFe2O4 SO APPLIED PHYSICS LETTERS LA English DT Article ID MULTIFERROIC LUFE2O4; FLUCTUATIONS; GENERATION; SYSTEM AB Femtosecond optical pump-probe spectroscopy is used to reveal the influence of charge and magnetic order on polaron dynamics and coherent acoustic phonon oscillations in single crystals of charge-ordered, ferrimagnetic LuFe2O4. We experimentally observed the influence of magnetic order on polaron dynamics. We also observed a correlation between charge order and the amplitude of the acoustic phonon oscillations, due to photoinduced changes in the lattice constant that originate from the photoexcited electrons. This provides insight into the general behavior of coherent acoustic phonon oscillations in charge-ordered materials. (C) 2015 AIP Publishing LLC. C1 [Lee, J.; Trugman, S. A.; Yarotski, D. A.; Taylor, A. J.; Prasankumar, R. P.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Trugman, S. A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Zhang, C. L.; Cheong, S. -W.] Rutgers State Univ, Rutgers Ctr Emergent Mat, Piscataway, NJ 08854 USA. [Zhang, C. L.; Cheong, S. -W.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Talbayev, D.] Tulane Univ, Dept Phys & Engn Phys, New Orleans, LA 70118 USA. [Xu, X. S.] Univ Nebraska, Dept Phys & Astron, Nebraska Ctr Mat & Nanosci, Lincoln, NE 68588 USA. RP Lee, J (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol, POB 1663, Los Alamos, NM 87545 USA. EM kjindda@naver.com; rpprasan@lanl.gov RI Talbayev, Diyar/C-5525-2009; Yarotski, Dmitry/G-4568-2010; Xu, Xiaoshan/B-1255-2009 OI Talbayev, Diyar/0000-0003-3537-1656; Xu, Xiaoshan/0000-0002-4363-392X FU Laboratory Directed Research and Development program at LANL; National Nuclear Security administration of the U.S. Department of Energy [DE-AC52-06NA25396]; DOE [DE-FG02-07ER46382] FX We would like to thank Cristian Batista for helpful discussions. This work was performed at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences (BES) user facility and supported by the Laboratory Directed Research and Development program at LANL. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security administration of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. The work at Rutgers University was supported by the DOE under Grant No. DE-FG02-07ER46382. NR 37 TC 0 Z9 0 U1 7 U2 43 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUL 27 PY 2015 VL 107 IS 4 AR 042906 DI 10.1063/1.4927739 PG 5 WC Physics, Applied SC Physics GA CO1OF UT WOS:000358924200053 ER PT J AU Li, Z Foley, JJ Peng, S Sun, CJ Ren, Y Wiederrecht, GP Gray, SK Sun, YG AF Li, Zheng Foley, Jonathan J. Peng, Sheng Sun, Cheng-Jun Ren, Yang Wiederrecht, Gary P. Gray, Stephen K. Sun, Yugang TI Reversible Modulation of Surface Plasmons in Gold Nanoparticles Enabled by Surface Redox Chemistry SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE core-shell nanoparticles; gold nanocrystals; iron; surface plasmon resonance; surface redox chemistry ID ENHANCED RAMAN-SCATTERING; IRON-OXIDE NANOPARTICLES; METAL NANOPARTICLES; SIZE; OXIDATION; SPECTROSCOPY; HETERODIMERS; RESONANCE; DYNAMICS; FE AB Switchable surface redox chemistry is demonstrated in gold@iron/iron oxide core-shell nanoparticles with ambient oxidation and plasmon-mediated reduction to modulate the oxidation state of shell layers. The iron shell can be oxidized to iron oxide through ambient oxidation, leading to an enhancement and red-shift of the gold surface plasmon resonance (SPR). This enhanced gold SPR can drive reduction of the iron oxide shell under broadband illumination to reversibly blue-shift and significantly dampen gold SPR absorption. The observed phenomena provide a unique mechanism for controlling the plasmonic properties and surface chemistry of small metal nanoparticles. C1 [Li, Zheng; Foley, Jonathan J.; Peng, Sheng; Wiederrecht, Gary P.; Gray, Stephen K.; Sun, Yugang] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Sun, Cheng-Jun; Ren, Yang] Argonne Natl Lab, Xray Sci Div, Adv Photon Source, Argonne, IL 60439 USA. RP Wiederrecht, GP (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 South Cass Ave, Argonne, IL 60439 USA. EM wiederrecht@anl.gov; gray@anl.gov; ygsun@anl.gov RI Sun, Yugang /A-3683-2010; Li, Zheng/L-1355-2016 OI Sun, Yugang /0000-0001-6351-6977; Li, Zheng/0000-0001-5281-8101 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility [DE-AC02-06CH11357]; University of Washington; Advanced Photon Source; U.S. DOE [DE-AC02-06CH11357]; US Department of Energy-Basic Energy Sciences; Canadian Light Source FX This work was performed at the Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility under Contract no. DE-AC02-06CH11357. PNC/XSD facilities at the Advanced Photon Source, and research at these facilities, are supported by the US Department of Energy-Basic Energy Sciences, the Canadian Light Source and its funding partners, the University of Washington, and the Advanced Photon Source. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 35 TC 6 Z9 6 U1 10 U2 55 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD JUL 27 PY 2015 VL 54 IS 31 BP 8948 EP 8951 DI 10.1002/anie.201502012 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA CN5WC UT WOS:000358501500009 PM 26094976 ER PT J AU Hirai, K Yeom, B Chang, SH Chi, H Mansfield, JF Lee, B Lee, S Uher, C Kotov, NA AF Hirai, Kenji Yeom, Bongjun Chang, Shu-Hao Chi, Hang Mansfield, John F. Lee, Byeongdu Lee, Sungsik Uher, Ctirad Kotov, Nicholas A. TI Coordination Assembly of Discoid Nanoparticles SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE conductive materials; coordination bond; nanoparticles; supramolecular assemblies ID NANOCRYSTALS; SURFACE; DESIGN; CRYSTALLIZATION; SUPERLATTICES; ORGANIZATION; FRAMEWORKS; CRYSTALS; POLYMERS; LATTICE AB Supramolecular chemistry utilizes coordination bonds to assemble molecular building blocks into a variety of sophisticated constructs. However, traditional coordination assemblies are based on organic compounds that have limited ability to transport charge. Herein, we describe coordination assembly of anisotropic FeS2 pyrite nanoparticles (NPs) that can facilitate charge transport. Zn2+ ions form supramolecular complexes with carboxylate end-groups on NP surface, leading to multiparticle sheets with liquid-crystal-like organization. Conductivity and Hall carrier mobility of the p-type layered semiconductor films with Zn2+ coordination bridging exceed those known for coordination compounds, some by several orders of magnitude. The nanoscale porosity of the assembled sheets combined with fast hole transport leads to high electrocatalytic activity of the NP films. The coordination assembly of NPs embraces the versatility of several types of building blocks and opens a new design space for self-organized materials combining nanoscale and supramolecular structural motifs. C1 [Hirai, Kenji; Yeom, Bongjun; Chang, Shu-Hao; Kotov, Nicholas A.] Univ Michigan, Dept Chem Engn, Ann Arbor, MI 48109 USA. [Yeom, Bongjun] Myongji Univ, Dept Chem Engn, Gyeonggi Do 449728, South Korea. [Chi, Hang; Uher, Ctirad] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Mansfield, John F.] Univ Michigan, Elect Microbeam Anal Lab, Ann Arbor, MI 48109 USA. [Lee, Byeongdu; Lee, Sungsik] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Kotov, Nicholas A.] Univ Michigan, Dept Mat Sci & Engn, Dept Biomed Engn, Ann Arbor, MI 48109 USA. [Kotov, Nicholas A.] Univ Michigan, Biointerfaces Inst, Ann Arbor, MI 48109 USA. RP Uher, C (reprint author), Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. EM cuher@umich.edu; kotov@umich.edu RI Chi, Hang/F-1537-2011; Hirai, Kenji/D-9008-2017; OI Chi, Hang/0000-0002-1299-1150; Hirai, Kenji/0000-0003-3307-3970; Yeom, Bongjun/0000-0001-8914-0947; Kotov, Nicholas/0000-0002-6864-5804; Lee, Byeongdu/0000-0003-2514-8805 FU NSF [NSF 1463474, 1403777, 1411014, DMR-9871177]; Center for Photonic and Multiscale Nanomaterials (C-PHOM) - National Science Foundation (NSF) Materials Research Science and Engineering Center program [DMR 1120923]; US DOE FX K.H. is grateful to JSPS Postdoctoral Fellowships for Research Abroad. The key parts of this work were supported by the NSF project "Energy- and Cost-Efficient Manufacturing Employing Nanoparticles" (NSF 1463474 to N.A.K.). Partial support was also made by the Center for Photonic and Multiscale Nanomaterials (C-PHOM) funded by the National Science Foundation (NSF) Materials Research Science and Engineering Center program DMR 1120923 as well as NSF projects 1403777 and 1411014. We thank the University of Michigan's EMAL for its assistance with electron microscopy, and for the NSF grant DMR-9871177 for funding of the JEOL 2010F analytical electron microscope used in this work. We are also grateful to the X-ray MicroAnalysis Laboratory (XMAL) for assistance with the use of Bruker XRD instrument and the Department of Chemistry for assistance with the ICP-OES. Use of the Advanced Photon Source, an Office of Science User Facility operated for the US Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the US DOE. NR 35 TC 7 Z9 7 U1 4 U2 64 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD JUL 27 PY 2015 VL 54 IS 31 BP 8966 EP 8970 DI 10.1002/anie.201502057 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA CN5WC UT WOS:000358501500013 PM 26095101 ER PT J AU Datskos, P Cullen, DA Sharma, J AF Datskos, Panos Cullen, David A. Sharma, Jaswinder TI Step-by-Step Growth of Complex Oxide Microstructures SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE hierarchical structures; hybrids; oxides; silica; titanium oxide ID SILICA; SUPERHYDROPHOBICITY; NANOSTRUCTURES; NANOPARTICLES; SURFACES; DESIGN; SHAPE AB The synthesis of complex and hybrid oxide microstructures is of fundamental interest and practical applications. However, the design and synthesis of such structures is a challenging task. A solution-phase process to synthesize complex silica and silica-titania hybrid microstructures was developed by exploiting the emulsion-droplet-based step-by-step growth featuring shape control. The strategy is robust and can be extended to the preparation of complex hybrid structures consisting of two or more materials, with each having its own shape. C1 [Datskos, Panos; Sharma, Jaswinder] Oak Ridge Natl Lab, Nanosyst Separat & Mat Res Grp, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. [Cullen, David A.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Sharma, J (reprint author), Oak Ridge Natl Lab, Nanosyst Separat & Mat Res Grp, Energy & Transportat Sci Div, One Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM sharmajk@ornl.gov RI Cullen, David/A-2918-2015 OI Cullen, David/0000-0002-2593-7866 FU U.S. Department of Energy [DE-AC05-00OR22725]; Laboratory Director's Research and Development Program of the Oak Ridge National Laboratory; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX J.S. is a Research Staff at the Oak Ridge National Laboratory managed by UT-Battelle, LLC, for the U.S. Department of Energy under Contract DE-AC05-00OR22725. The work was supported by the Laboratory Director's Research and Development Program of the Oak Ridge National Laboratory. A portion of this research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 31 TC 9 Z9 9 U1 10 U2 41 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD JUL 27 PY 2015 VL 54 IS 31 BP 9011 EP 9015 DI 10.1002/anie.201503777 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA CN5WC UT WOS:000358501500023 PM 26095228 ER PT J AU Du, G Du, ZY Fang, DL Yang, H Zhong, RD Schneeloch, J Gu, GD Wen, HH AF Du, Guan Du, Zengyi Fang, Delong Yang, Huan Zhong, R. D. Schneeloch, J. Gu, G. D. Wen, Hai-Hu TI Fully gapped superconductivity in In-doped topological crystalline insulator Pb0.5Sn0.5Te SO PHYSICAL REVIEW B LA English DT Article ID TRANSITION; SNTE; )(0.84)IN0.16TE; INDIUM; STATES; FILMS AB Superconductors derived from topological insulators and topological crystalline insulators by chemical doping have long been considered to be candidates as topological superconductors. Pb0.5Sn0.5Te is a topological crystalline insulator with mirror symmetry protected surface states on (001)-, (011)-, and (111)-oriented surfaces. The superconductor (Pb0.5Sn0.5)(0.7)In0.3Te is produced by In doping in Pb0.5Sn0.5Te, and is thought to be a topological superconductor. Here we report scanning tunneling spectroscopy measurements of the superconducting state as well as the superconducting energy gap in (Pb0.5Sn0.5)(0.7)In0.3Te on a (001)-oriented surface. The spectrum can be well fitted by an anisotropic s-wave gap function of Delta(theta) = 0.72 + 0.18 cos 4 theta meV using Dynes model. The results show that the superconductor seems to be a fully gapped one without any in-gap states, in contradiction with the expectation of a topological superconductor. C1 [Du, Guan; Du, Zengyi; Fang, Delong; Yang, Huan; Wen, Hai-Hu] Nanjing Univ, Collaborat Innovat Ctr Adv Microstruct, Natl Lab Solid State Microstruct, Nanjing 210093, Jiangsu, Peoples R China. [Du, Guan; Du, Zengyi; Fang, Delong; Yang, Huan; Wen, Hai-Hu] Nanjing Univ, Collaborat Innovat Ctr Adv Microstruct, Dept Phys, Nanjing 210093, Jiangsu, Peoples R China. [Zhong, R. D.; Schneeloch, J.; Gu, G. D.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Du, G (reprint author), Nanjing Univ, Collaborat Innovat Ctr Adv Microstruct, Natl Lab Solid State Microstruct, Nanjing 210093, Jiangsu, Peoples R China. EM huanyang@nju.edu.cn; hhwen@nju.edu.cn RI Zhong, Ruidan/D-5296-2013 OI Zhong, Ruidan/0000-0003-1652-9454 FU Ministry of Science and Technology of China (973 projects) [2011CBA00102, 2012CB821403]; NSF of China; PAPD; Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, U.S. Department of Energy [DE-SC00112704]; Center for Emergent Superconductivity, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science FX We appreciate the useful discussions with Qianghua Wang and the help from Jianzhong Liu in using the Laue diffraction machine. This work was supported by the Ministry of Science and Technology of China (973 projects: 2011CBA00102, 2012CB821403), NSF of China and PAPD. Work at Brookhaven National Laboratory is supported by the Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, U.S. Department of Energy under Contract No. DE-SC00112704. R.Z. and J.S. are also supported as part of the Center for Emergent Superconductivity, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science. NR 48 TC 3 Z9 3 U1 3 U2 31 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUL 27 PY 2015 VL 92 IS 2 AR 020512 DI 10.1103/PhysRevB.92.020512 PG 5 WC Physics, Condensed Matter SC Physics GA CN7FT UT WOS:000358600300002 ER PT J AU Errandonea, D Boehler, R Ross, M AF Errandonea, D. Boehler, R. Ross, M. TI Comment on "Molybdenum sound velocity and shear modulus softening under shock compression" SO PHYSICAL REVIEW B LA English DT Editorial Material AB In this Comment we discuss recent results presented by Nguyen et al. on shock compressed molybdenum up to 438 GPa [Phys. Rev. B 89, 174109 (2014)]. The aim of Nguyen's article is to show that there is no phase transition near 210 GPa. We propose instead an interpretation of their data that this material shows the onset of partial melting along the Hugoniot at 240(20) GPa, which is evident from abrupt changes in the pressure dependence of the shear modulus. This interpretation may solve the significant controversy in the melting slopes derived from shock and static experiments. C1 [Errandonea, D.] Univ Valencia, ICMUV, Dept Fis Aplicada, MALTA Consolider Team, E-46100 Valencia, Spain. [Boehler, R.] Carnegie Inst Sci, Geophys Lab, Washington, DC 20015 USA. [Ross, M.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Errandonea, D (reprint author), Univ Valencia, ICMUV, Dept Fis Aplicada, MALTA Consolider Team, Edificio Invest ,C Dr Moliner 50, E-46100 Valencia, Spain. RI Boehler, Reinhard/L-3971-2016; Errandonea, Daniel/J-7695-2016 OI Boehler, Reinhard/0000-0003-0222-6997; Errandonea, Daniel/0000-0003-0189-4221 NR 12 TC 5 Z9 5 U1 2 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUL 27 PY 2015 VL 92 IS 2 AR 026101 DI 10.1103/PhysRevB.92.026101 PG 2 WC Physics, Condensed Matter SC Physics GA CN7FT UT WOS:000358600300007 ER PT J AU Kim, YK Koh, YY Kyung, WS Han, GR Lee, B Kim, KH Ok, JM Kim, JS Arita, M Shimada, K Namatame, H Taniguchi, M Mo, SK Kim, C AF Kim, Y. K. Koh, Y. Y. Kyung, W. S. Han, G. R. Lee, B. Kim, Kee Hoon Ok, J. M. Kim, Jun Sung Arita, M. Shimada, K. Namatame, H. Taniguchi, M. Mo, S. -K. Kim, C. TI Possible role of bonding angle and orbital mixing in iron pnictide superconductivity: Comparative electronic structure studies of LiFeAs and Sr2VO3FeAs SO PHYSICAL REVIEW B LA English DT Article AB A well-known universal feature among iron pnictide superconductors is the correlation between the As-Fe-As bonding angle and the superconducting transition temperature. However, the origin of such a correlation has not been clearly understood despite its potential importance in understanding the mechanism of superconductivity. Here, we present comparative electronic structure studies of LiFeAs and Sr2VO3FeAs, two representative systems without any dopant that can show bonding angle dependence of the electronic structure. Captured distinct features of the higher T-c compound Sr2VO3FeAs such as an unusual kz modulation and anomalous polarization dependence suggest that the difference between the two systems is in the interorbital coupling strength. This could be the essential element of the bonding angle dependence that allows an enhanced pairing instability and T-c. C1 [Kim, Y. K.; Koh, Y. Y.; Kyung, W. S.; Han, G. R.; Kim, C.] Yonsei Univ, Inst Phys & Appl Phys, Seoul 120749, South Korea. [Kim, Y. K.; Mo, S. -K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Lee, B.; Kim, Kee Hoon] Seoul Natl Univ, CeNSCMR, Dept Phys & Astron, Seoul 151747, South Korea. [Ok, J. M.; Kim, Jun Sung] Pohang Univ Sci & Technol, Dept Phys, Pohang 790784, South Korea. [Arita, M.; Shimada, K.; Namatame, H.; Taniguchi, M.] Hiroshima Univ, Hiroshima Synchrotron Radiat Ctr, Higashihiroshima, Hiroshima 7390046, Japan. RP Kim, YK (reprint author), Yonsei Univ, Inst Phys & Appl Phys, Seoul 120749, South Korea. EM changyoung@yonsei.ac.kr RI Mo, Sung-Kwan/F-3489-2013; Kim, Jun Sung/G-8861-2012; Shimada, Kenya/G-5080-2016; Kim, Yeong Kwan/L-8207-2016 OI Mo, Sung-Kwan/0000-0003-0711-8514; Kim, Jun Sung/0000-0002-1413-7265; Shimada, Kenya/0000-0002-1945-2352; FU National Research Foundation of Korea (NRF) [2010-0018092, 2006-08658]; National Creative Research Initiative through the NRF of Korea [2010-0018300]; NRF through the Mid Career Researcher Program [2012-013838]; NRF through Max Planck POSTECH/ KOREA Research Initiative Program [2011-0031558]; IBS [IBSR014-D1-2014-a02]; Office of Basic Energy Sciences, of the U.S. DOE [DE-AC02-05CH11231] FX This work was supported through (National Research Foundation of Korea (NRF) Grants No. 2010-0018092 and No. 2006-08658. The work at SNU was financially supported by the National Creative Research Initiative (2010-0018300) through the NRF of Korea. The work at POSTECH was supported by NRF through the Mid Career Researcher Program (Grant No. 2012-013838) and the Max Planck POSTECH/KOREA Research Initiative Program (No. 2011-0031558) and also by IBS (No. IBSR014-D1-2014-a02). The experiments at HiSOR were performed under the approval of HSRC (Proposals No. 11-A-11 and No. 12-A-23). The ALS is supported by the Office of Basic Energy Sciences, of the U.S. DOE under Contract No. DE-AC02-05CH11231. NR 24 TC 2 Z9 2 U1 2 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUL 27 PY 2015 VL 92 IS 4 AR 041116 DI 10.1103/PhysRevB.92.041116 PG 5 WC Physics, Condensed Matter SC Physics GA CN7GL UT WOS:000358602200002 ER PT J AU Nguyen, JH Akin, MC Chau, R Fratanduono, DE Ambrose, WP Fat'yanov, OV Asimow, PD Holmes, NC AF Nguyen, Jeffrey H. Akin, Minta C. Chau, Ricky Fratanduono, Dayne E. Ambrose, W. Patrick Fat'yanov, Oleg V. Asimow, Paul D. Holmes, Neil C. TI Reply to "Comment on 'Molybdenum sound velocity and shear modulus softening under shock compression' " SO PHYSICAL REVIEW B LA English DT Editorial Material AB We respond to the Comment by Errandonea et al. [Phys. Rev. B 92, 026101 (2015)] on their reinterpretation of our published data [Nguyen et al., Phys. Rev. B 89, 174109 (2014)]. In the original paper, we argued that there is no solid-solid phase transition along the Hugoniot at 2.1 Mbars. There is, however, a softening of the shear modulus starting at 2.6 Mbars. Errandonea et al. [Phys. Rev. B 92, 026101 (2015)] reinterpreted our data and concluded that there is a structural change near 2.3 Mbars on the Hugoniot. We will explore the differences and agreements in the two interpretations of our data. C1 [Nguyen, Jeffrey H.; Akin, Minta C.; Chau, Ricky; Fratanduono, Dayne E.; Ambrose, W. Patrick; Holmes, Neil C.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Fat'yanov, Oleg V.; Asimow, Paul D.] CALTECH, Pasadena, CA 91125 USA. RP Nguyen, JH (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. NR 12 TC 4 Z9 4 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUL 27 PY 2015 VL 92 IS 2 AR 026102 DI 10.1103/PhysRevB.92.026102 PG 2 WC Physics, Condensed Matter SC Physics GA CN7FT UT WOS:000358600300008 ER PT J AU Perez, EAC Papenbrock, T AF Perez, E. A. Coello Papenbrock, T. TI Effective theory for the nonrigid rotor in an electromagnetic field: Toward accurate and precise calculations of E2 transitions in deformed nuclei SO PHYSICAL REVIEW C LA English DT Article ID SPONTANEOUS SYMMETRY-BREAKING; DATA SHEETS; PHENOMENOLOGICAL LAGRANGIANS; COULOMB-EXCITATION; COLLECTIVE MODEL; LIGHT-NUCLEI; ER-168; STATES; BANDS; SCATTERING AB We present a model-independent approach to electric quadrupole transitions of deformed nuclei. Based on an effective theory for axially symmetric systems, the leading interactions with electromagnetic fields enter as minimal couplings to gauge potentials, while subleading corrections employ gauge-invariant nonminimal couplings. This approach yields transition operators that are consistent with the Hamiltonian, and the power counting of the effective theory provides us with theoretical uncertainty estimates. We successfully test the effective theory in homonuclear molecules that exhibit a large separation of scales. For ground-state band transitions of rotational nuclei, the effective theory describes data well within theoretical uncertainties at leading order. To probe the theory at subleading order, data with higher precision would be valuable. For transitional nuclei, next-to-leading-order calculations and the high-precision data are consistent within the theoretical uncertainty estimates. We also study the faint interband transitions within the effective theory and focus on the E2 transitions from the 0(2)(+) band ( the "beta band") to the ground-state band. Here the predictions from the effective theory are consistent with data for several nuclei, thereby proposing a solution to a long-standing challenge. C1 [Perez, E. A. Coello; Papenbrock, T.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Papenbrock, T.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. RP Perez, EAC (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. OI Papenbrock, Thomas/0000-0001-8733-2849 FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DEFG02-96ER40963, DE-AC05-00OR22725] FX We thank M. Allmond, M. Caprio, A. Ekstrom, C. Forssen, R. J. Furnstahl, H. Griesshammer, H.-W. Hammer, K. Jones, H. Krebs, and L. Platter for useful discussions. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics under Award No. DEFG02-96ER40963 (University of Tennessee) and under Contract No. DE-AC05-00OR22725 (Oak Ridge National Laboratory). NR 86 TC 7 Z9 7 U1 1 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JUL 27 PY 2015 VL 92 IS 1 AR 014323 DI 10.1103/PhysRevC.92.014323 PG 19 WC Physics, Nuclear SC Physics GA CN7HA UT WOS:000358603800002 ER PT J AU Lee, G Arrington, JR Hill, RJ AF Lee, Gabriel Arrington, John R. Hill, Richard J. TI Extraction of the proton radius from electron-proton scattering data SO PHYSICAL REVIEW D LA English DT Article ID ELECTROMAGNETIC FORM-FACTORS; RADIATIVE CORRECTIONS; POLARIZATION TRANSFER; MUONIC HYDROGEN; CROSS-SECTIONS; RATIO; (GEV/C)(2); PHYSICS AB We perform a new analysis of electron-proton scattering data to determine the proton electric and magnetic radii, enforcing model-independent constraints from form factor analyticity. A wide-ranging study of possible systematic effects is performed. An improved analysis is developed that rebins data taken at identical kinematic settings and avoids a scaling assumption of systematic errors with statistical errors. Employing standard models for radiative corrections, our improved analysis of the 2010 Mainz A1 Collaboration data yields a proton electric radius r(E) = 0.895(20) fm and magnetic radius r(M) = 0.776(38) fm. A similar analysis applied to world data (excluding Mainz data) implies r(E) = 0.916(24) fm and r(M) = 0.914(35) fm. The Mainz and world values of the charge radius are consistent, and a simple combination yields a value r(E) = 0.904(15) fm that is 4 sigma larger than the CREMA Collaboration muonic hydrogen determination. The Mainz and world values of the magnetic radius differ by 2.7 sigma, and a simple average yields r(M) = 0.851(26) fm. The circumstances under which published muonic hydrogen and electron scattering data could be reconciled are discussed, including a possible deficiency in the standard radiative correction model which requires further analysis. C1 [Lee, Gabriel; Hill, Richard J.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Lee, Gabriel; Hill, Richard J.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Lee, Gabriel] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Arrington, John R.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RP Lee, G (reprint author), Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. EM leeg@physics.technion.ac.il; johna@anl.gov; richardhill@uchicago.edu RI Hill, Richard/C-8820-2017 OI Hill, Richard/0000-0003-1982-589X FU NIST Precision Measurement Grant; U.S. Department of Energy, Office of Science, Office of High Energy Physics (DOE Grant) [DE-FG02-13ER41958]; Office of Nuclear Physics (DOE Grant) [DE-AC02-06CH11357]; ICORE Program of Planning and Budgeting Committee; ISF Grant [1937/12] FX We thank Z. Jiang for collaboration during the early stages of this work and G. Paz and I. Sick for discussions. Research was supported by a NIST Precision Measurement Grant, the U.S. Department of Energy, Office of Science, Office of High Energy Physics (DOE Grant No. DE-FG02-13ER41958), and Office of Nuclear Physics (DOE Grant No. DE-AC02-06CH11357). G. L. also acknowledges support by the ICORE Program of Planning and Budgeting Committee and by ISF Grant No. 1937/12. NR 97 TC 23 Z9 23 U1 2 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 27 PY 2015 VL 92 IS 1 AR 013013 DI 10.1103/PhysRevD.92.013013 PG 25 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CN7HJ UT WOS:000358604700002 ER PT J AU Martin, SP AF Martin, Stephen P. TI Z-boson pole mass at two-loop order in the pure (MS)over-bar scheme SO PHYSICAL REVIEW D LA English DT Article ID SELF-ENERGY DIAGRAMS; RENORMALIZATION-GROUP EQUATIONS; QUANTUM-FIELD THEORY; STANDARD-MODEL; MUON LIFETIME; RHO-PARAMETER; GAUGE BOSONS; TOP-QUARK; RADIATIVE-CORRECTIONS; NUMERICAL EVALUATION AB I obtain the complex pole squared mass of the Z boson at full two-loop order in the Standard Model in the pure (MS) over bar renormalization scheme. The input parameters are the running gauge couplings, the top-quark Yukawa coupling, the Higgs self-coupling, and the vacuum expectation value that minimizes the Landau gauge effective potential. The effects of nonzero Goldstone boson mass are resummed. Within a reasonable range of renormalization scale choices, the scale dependence of the computed pole mass is found to be comparable to the current experimental uncertainty, but the true theoretical error is likely somewhat larger. C1 [Martin, Stephen P.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Martin, Stephen P.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Martin, SP (reprint author), No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. FU National Science Foundation [PHY-1417028] FX This work was supported in part by the National Science Foundation Grant No. PHY-1417028. NR 67 TC 4 Z9 4 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 27 PY 2015 VL 92 IS 1 AR 014026 DI 10.1103/PhysRevD.92.014026 PG 9 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CN7HJ UT WOS:000358604700003 ER PT J AU Palacios, MA McLellan, R Beavers, CM Teat, SJ Weihe, H Piligkos, S Dalgarno, SJ Brechin, EK AF Palacios, Maria A. McLellan, Ross Beavers, Christine M. Teat, Simon J. Weihe, Hogni Piligkos, Stergios Dalgarno, Scott J. Brechin, Euan K. TI Facile Interchange of 3d and 4f Ions in Single-Molecule Magnets: Stepwise Assembly of [Mn-4], [Mn(3)Ln] and [Mn(2)Ln(2)] Cages within Calix[4]arene Scaffolds SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE calixarenes; clusters; coordination chemistry; magnetism; SMMs ID HIGH-FREQUENCY EPR; INELASTIC NEUTRON-SCATTERING; CLUSTERS; MANGANESE(III); COMPLEXES; INTERFERENCE; LANTHANIDE; RESONANCE; LN AB The central Mn-II ions in a series of calix[4] arenestabilised butterflies can be sequentially replaced with Ln(III) ions, maintaining the structural integrity of the molecule but transforming its magnetic properties. The replacement of Mn-II for Gd-III allows for the examination of the transferability of spin-Hamiltonian parameters within the family as well as permitting their reliable determination. The introduction of the 4f ions results in weaker intramolecular magnetic exchange, an increase in the number of low-lying excited states, and an increase in magnetisation relaxation, highlighting the importance of exchange over single-ion anisotropy for the observation of SMM behaviour in this family of complexes. The presence of the [TMII/III(TBC[4])(OH)(solvent)] metalloligand (TM = transition metal, TBC = p-tBu-calix[4]arene) suggests that magnetic calix[n]arene building blocks can be employed to encapsulate a range of different "guests" within structurally robust "hosts". C1 [Palacios, Maria A.; Brechin, Euan K.] Univ Edinburgh, EaStCHEM Sch Chem, Edinburgh EH9 3FJ, Midlothian, Scotland. [McLellan, Ross; Dalgarno, Scott J.] Heriot Watt Univ, Inst Chem Sci, Edinburgh EH14 4AS, Midlothian, Scotland. [Beavers, Christine M.; Teat, Simon J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Weihe, Hogni; Piligkos, Stergios] Univ Copenhagen, Dept Chem, DK-2100 Copenhagen, Denmark. RP Piligkos, S (reprint author), Univ Copenhagen, Dept Chem, Univ Pk 5, DK-2100 Copenhagen, Denmark. EM piligkos@kiku.dk; S.J.Dalgarno@hw.ac.uk; E.Brechin@ed.ac.uk RI Beavers, Christine/C-3539-2009; Weihe, Hogni/B-5770-2008; Piligkos, Stergios/C-7409-2013; Palacios Lopez, Maria Angeles /K-3903-2016; Dalgarno, Scott/A-7358-2010; OI Beavers, Christine/0000-0001-8653-5513; Weihe, Hogni/0000-0001-6194-1486; Piligkos, Stergios/0000-0002-4011-6476; Dalgarno, Scott/0000-0001-7831-012X; McLellan, Ross/0000-0001-9700-0258; Brechin, Euan/0000-0002-9365-370X FU EPSRC [EP/I03255X/1, EP/I031421/1]; Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231]; Danish Ministry of Science Innovation and Higher Education [10-081659] FX E.K.B. and S.J.D. acknowledge the financial support of the EPSRC (EP/I03255X/1&EP/I031421/1). The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under contract no DE-AC02-05CH11231. We thank the Danish Ministry of Science Innovation and Higher Education for a Sapere Aude Fellowship (10-081659). NR 45 TC 10 Z9 10 U1 7 U2 57 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD JUL 27 PY 2015 VL 21 IS 31 BP 11212 EP 11218 DI 10.1002/chem.201500001 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA CN1YG UT WOS:000358216200037 PM 26121216 ER PT J AU Tripp, HJ Sutton, G White, O Wortman, J Pati, A Mikhailova, N Ovchinnikova, G Payne, SH Kyrpides, NC Ivanova, N AF Tripp, H. James Sutton, Granger White, Owen Wortman, Jennifer Pati, Amrita Mikhailova, Natalia Ovchinnikova, Galina Payne, Samuel H. Kyrpides, Nikos C. Ivanova, Natalia TI Toward a standard in structural genome annotation for prokaryotes SO STANDARDS IN GENOMIC SCIENCES LA English DT Article ID MASS-SPECTROMETRY; PEPTIDE; IDENTIFICATION; PROTEOMICS AB Background: In an effort to identify the best practice for finding genes in prokaryotic genomes and propose it as a standard for automated annotation pipelines, 1,004,576 peptides were collected from various publicly available resources, and were used as a basis to evaluate various gene-calling methods. The peptides came from 45 bacterial replicons with an average GC content from 31 % to 74 %, biased toward higher GC content genomes. Automated, manual, and semi-manual methods were used to tally errors in three widely used gene calling methods, as evidenced by peptides mapped outside the boundaries of called genes. Results: We found that the consensus set of identical genes predicted by the three methods constitutes only about 70 % of the genes predicted by each individual method (with start and stop required to coincide). Peptide data was useful for evaluating some of the differences between gene callers, but not reliable enough to make the results conclusive, due to limitations inherent in any proteogenomic study. Conclusions: A single, unambiguous, unanimous best practice did not emerge from this analysis, since the available proteomics data were not adequate to provide an objective measurement of differences in the accuracy between these methods. However, as a result of this study, software, reference data, and procedures have been better matched among participants, representing a step toward a much-needed standard. In the absence of sufficient amount of exprimental data to achieve a universal standard, our recommendation is that any of these methods can be used by the community, as long as a single method is employed across all datasets to be compared. C1 [Tripp, H. James; Pati, Amrita; Mikhailova, Natalia; Ovchinnikova, Galina; Kyrpides, Nikos C.; Ivanova, Natalia] DOE Joint Genome Inst, Walnut Creek, CA USA. [Sutton, Granger] J Craig Venter Inst, Rockville, MD USA. [White, Owen] Univ Maryland, Sch Med, Inst Genome Sci, Baltimore, MD 21201 USA. [Wortman, Jennifer] Broad Inst, Cambridge, MA USA. [Payne, Samuel H.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Ivanova, N (reprint author), DOE Joint Genome Inst, Walnut Creek, CA USA. EM nnivanova@lbl.gov RI Kyrpides, Nikos/A-6305-2014; OI Kyrpides, Nikos/0000-0002-6131-0462; Payne, Samuel/0000-0002-8351-1994; Ivanova, Natalia/0000-0002-5802-9485 FU US Department of Energy's Office of Science, Biological and Environmental Research Program; University of California, Lawrence Berkeley National Laboratory [DE-AC02-05CH11231] FX The authors wish to thank Doug Hyatt of Oak Ridge National Laboratory for a detailed description of the algorithms employed by Prodigal as well as Mark Borodovsky (Georgia Tech) and Tatiana Tatusova (NCBI) for helpful comments and discussion. This work was performed under the auspices of the US Department of Energy's Office of Science, Biological and Environmental Research Program, and by the University of California, Lawrence Berkeley National Laboratory under contract No. DE-AC02-05CH11231. NR 17 TC 2 Z9 2 U1 1 U2 2 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD JUL 25 PY 2015 VL 10 AR 45 DI 10.1186/s40793-015-0034-9 PG 9 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DA7NK UT WOS:000367990800001 PM 26380633 ER PT J AU Yates, R Howieson, J De Meyer, SE Tian, R Seshadri, R Pati, A Woyke, T Markowitz, V Ivanova, N Kyrpides, N Loi, A Nutt, B Garau, G Sulas, L Reeve, W AF Yates, Ron Howieson, John De Meyer, Sofie E. Tian, Rui Seshadri, Rekha Pati, Amrita Woyke, Tanja Markowitz, Victor Ivanova, Natalia Kyrpides, Nikos Loi, Angelo Nutt, Brad Garau, Giovanni Sulas, Leonardo Reeve, Wayne TI High-quality permanent draft genome sequence of Rhizobium sullae strain WSM1592; a Hedysarum coronarium microsymbiont from Sassari, Italy SO STANDARDS IN GENOMIC SCIENCES LA English DT Article DE Root-nodule bacteria; Nitrogen fixation; Rhizobia; Alphaproteobacteria; GEBA-RNB ID NITROGEN-FIXATION; MICROBIAL GENOMES; SP-NOV; SYSTEM; LEGUMINOSARUM; BACTERIA; ACID AB Rhizobium sullae strain WSM1592 is an aerobic, Gram-negative, non-spore-forming rod that was isolated from an effective nitrogen (N-2) fixing root nodule formed on the short-lived perennial legume Hedysarum coronarium (also known as Sulla coronaria or Sulla). WSM1592 was isolated from a nodule recovered from H. coronarium roots located in Ottava, bordering Sassari, Sardinia in 1995. WSM1592 is highly effective at fixing nitrogen with H. coronarium, and is currently the commercial Sulla inoculant strain in Australia. Here we describe the features of R. sullae strain WSM1592, together with genome sequence information and its annotation. The 7,530,820 bp high-quality permanent draft genome is arranged into 118 scaffolds of 118 contigs containing 7.453 protein-coding genes and 73 RNA-only encoding genes. This rhizobial genome is sequenced as part of the DOE Joint Genome Institute 2010 Genomic Encyclopedia for Bacteria and Archaea-Root Nodule Bacteria (GEBA-RNB) project. C1 [Yates, Ron; Howieson, John; De Meyer, Sofie E.; Tian, Rui; Reeve, Wayne] Murdoch Univ, Ctr Rhizobium Studies, Murdoch, WA 6150, Australia. [Seshadri, Rekha; Pati, Amrita; Woyke, Tanja; Ivanova, Natalia; Kyrpides, Nikos] US DOE, Joint Genome Inst, Creek, CA USA. [Markowitz, Victor] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Data Management & Technol Ctr, Berkeley, CA 94720 USA. [Kyrpides, Nikos] King Abdulaziz Univ, Fac Sci, Dept Biol Sci, Jeddah, Saudi Arabia. [Garau, Giovanni] Univ Sassari, Dept Agr, Sardinia, Italy. [Sulas, Leonardo] CNR, Inst Anim Prod Syst Mediterranean Environm ISPAAM, Sassari, Italy. RP Reeve, W (reprint author), Murdoch Univ, Ctr Rhizobium Studies, Murdoch, WA 6150, Australia. EM W.Reeve@murdoch.edu.au RI Kyrpides, Nikos/A-6305-2014; Fac Sci, KAU, Biol Sci Dept/L-4228-2013; Faculty of, Sciences, KAU/E-7305-2017; OI Kyrpides, Nikos/0000-0002-6131-0462; Ivanova, Natalia/0000-0002-5802-9485; Garau, Giovanni/0000-0001-8292-8336 FU US Department of Energy's Office of Science, Biological and Environmental Research Program; University of California, Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Los Alamos National Laboratory [DE-AC02-06NA25396] FX This work was performed under the auspices of the US Department of Energy's Office of Science, Biological and Environmental Research Program, and by the University of California, Lawrence Berkeley National Laboratory under contract No. DE-AC02-05CH11231, Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344, and Los Alamos National Laboratory under contract No. DE-AC02-06NA25396. NR 37 TC 1 Z9 1 U1 0 U2 2 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD JUL 24 PY 2015 VL 10 AR 44 DI 10.1186/s40793-015-0020-2 PG 6 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DA7NI UT WOS:000367990600001 PM 26380632 ER PT J AU Kuznetsova, E Nocek, B Brown, G Makarova, KS Flick, R Wolf, YI Khusnutdinova, A Evdokimova, E Jin, K Tan, K Hanson, AD Hasnain, G Zallot, R de Crecy-Lagard, V Babu, M Savchenko, A Joachimiak, A Edwards, AM Koonin, EV Yakunin, AF AF Kuznetsova, Ekaterina Nocek, Boguslaw Brown, Greg Makarova, Kira S. Flick, Robert Wolf, Yuri I. Khusnutdinova, Anna Evdokimova, Elena Jin, Ke Tan, Kemin Hanson, Andrew D. Hasnain, Ghulam Zallot, Remi de Crecy-Lagard, Valerie Babu, Mohan Savchenko, Alexei Joachimiak, Andrzej Edwards, Aled M. Koonin, Eugene V. Yakunin, Alexander F. TI Functional Diversity of Haloacid Dehalogenase Superfamily Phosphatases from Saccharomyces cerevisiae BIOCHEMICAL, STRUCTURAL, AND EVOLUTIONARY INSIGHTS SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article ID ESCHERICHIA-COLI; PROTEIN PHOSPHATASE; BUDDING YEAST; GENE ENCODES; MITOCHONDRIAL PHOSPHATASE; SUBSTRATE SPECIFICITIES; PHOSPHORYLATION SITES; ALKALINE-PHOSPHATASE; THIAMIN BIOSYNTHESIS; ENZYME PROMISCUITY AB The haloacid dehalogenase (HAD)-like enzymes comprise a large superfamily of phosphohydrolases present in all organisms. The Saccharomyces cerevisiae genome encodes at least 19 soluble HADs, including 10 uncharacterized proteins. Here, we biochemically characterized 13 yeast phosphatases from the HAD superfamily, which includes both specific and promiscuous enzymes active against various phosphorylated metabolites and peptides with several HADs implicated in detoxification of phosphorylated compounds and pseudouridine. The crystal structures of four yeast HADs provided insight into their active sites, whereas the structure of the YKR070W dimer in complex with substrate revealed a composite substrate-binding site. Although the S. cerevisiae and Escherichia coli HADs share low sequence similarities, the comparison of their substrate profiles revealed seven phosphatases with common preferred substrates. The cluster of secondary substrates supporting significant activity of both S. cerevisiae and E. coli HADs includes 28 common metabolites that appear to represent the pool of potential activities for the evolution of novel HAD phosphatases. Evolution of novel substrate specificities of HAD phosphatases shows no strict correlation with sequence divergence. Thus, evolution of the HAD superfamily combines the conservation of the overall substrate pool and the substrate profiles of some enzymes with remarkable biochemical and structural flexibility of other superfamily members. C1 [Edwards, Aled M.] Univ Toronto, Struct Genom Consortium, Toronto, ON M5G 1L7, Canada. [Nocek, Boguslaw; Tan, Kemin; Joachimiak, Andrzej; Edwards, Aled M.] Argonne Natl Lab, Midwest Ctr Struct Genom & Struct Biol Ctr, Biosci Div, Argonne, IL 60439 USA. [Brown, Greg; Flick, Robert; Khusnutdinova, Anna; Evdokimova, Elena; Savchenko, Alexei; Yakunin, Alexander F.] Univ Toronto, Dept Chem Engn & Appl Chem, Toronto, ON M5S 3E5, Canada. [Makarova, Kira S.; Wolf, Yuri I.; Koonin, Eugene V.] Natl Lib Med, Natl Ctr Biotechnol Informat, NIH, Bethesda, MD 20894 USA. [Jin, Ke; Babu, Mohan] Univ Regina, Dept Biochem, Res & Innovat Ctr, Regina, SK S4S 0A2, Canada. [Hanson, Andrew D.; Hasnain, Ghulam; Zallot, Remi; de Crecy-Lagard, Valerie; Babu, Mohan] Univ Florida, Dept Hort Sci, Dept Microbiol & Cell Sci, Gainesville, FL 32611 USA. RP Yakunin, AF (reprint author), Univ Toronto, Dept Chem Engn & Appl Chem, 200 Coll St, Toronto, ON M5S 3E5, Canada. EM a.iakounine@utoronto.ca RI ZALLOT, Remi/D-3933-2014; Regan, Clinton/E-6250-2012; OI ZALLOT, Remi/0000-0002-7317-1578; Yakunin, Alexander/0000-0003-0813-6490 FU National Institutes of Health [GM094585]; Government of Canada through Genome Canada; Ontario Genomics Institute; Ontario Research Fund [2009-OGI-ABC-1405, ORF-GL2-01-004]; United States Department of Energy, Office of Biological and Environmental Research [DE-AC02-06CH11357]; U. S. National Science Foundation [IOS-1025398] FX This work was supported, in whole or in part, by National Institutes of Health Grant GM094585 (to A. J.). This work was also supported by the Government of Canada through Genome Canada, the Ontario Genomics Institute, and the Ontario Research Fund (Grants 2009-OGI-ABC-1405 and ORF-GL2-01-004 to A. F. Y.), by the United States Department of Energy, Office of Biological and Environmental Research, under Contract DE-AC02-06CH11357 (to A. J.), and by U. S. National Science Foundation Grant IOS-1025398 (to A. D. H.). The authors declare that they have no conflict of interest with the content of this article. NR 133 TC 8 Z9 8 U1 3 U2 20 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD JUL 24 PY 2015 VL 290 IS 30 BP 18678 EP 18698 DI 10.1074/jbc.M115.657916 PG 21 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CN5ZE UT WOS:000358512100037 PM 26071590 ER PT J AU Shanavas, KV Singh, DJ AF Shanavas, K. V. Singh, David J. TI Doping SrTiO3 supported FeSe by excess atoms and oxygen vacancies SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTIVITY; LAYER FESE/SRTIO3 FILMS; SINGLE-LAYER; PHASE-DIAGRAM; ORIGIN AB Photoemission studies of FeSe monolayer films on SrTiO3 substrate have shown electronic structures that deviate from pristine FeSe, consistent with heavy electron doping. With the help of first-principles calculations we studied the effect of excess Fe and Se atoms on the monolayer and oxygen vacancies in the substrate in order to understand the reported Fermi surface in this system. We find that both excess Fe and Se atoms prefer the same adsorption site above the bottom Se atoms on the monolayer. The adsorbed Fe is strongly magnetic and contributes electrons to the monolayer, while excess Se hybridizes with the monolayer Fe-d states and partially opens a gap just above the Fermi energy. We also find that the two-dimensional electron gas generated by the oxygen vacancies is partly transferred to the monolayer and can potentially suppress the hole pockets around the Gamma point. Thus, both O vacancies in the SrTiO3 substrate and excess Fe over the monolayer can provide high levels of electron doping. C1 [Shanavas, K. V.; Singh, David J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Shanavas, KV (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM kavungalvees@ornl.gov FU US Department of Energy, Basic Energy Sciences, Office of Science, Materials Sciences and Engineering Division FX This research was supported by the US Department of Energy, Basic Energy Sciences, Office of Science, Materials Sciences and Engineering Division. NR 34 TC 8 Z9 8 U1 4 U2 40 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 24 PY 2015 VL 92 IS 3 AR 035144 DI 10.1103/PhysRevB.92.035144 PG 6 WC Physics, Condensed Matter SC Physics GA CN4YN UT WOS:000358436600004 ER PT J AU Steinke, L Simonson, JW Yin, WG Smith, GJ Kistner-Morris, JJ Zellman, S Puri, A Aronson, MC AF Steinke, L. Simonson, J. W. Yin, W. -G. Smith, G. J. Kistner-Morris, J. J. Zellman, S. Puri, A. Aronson, M. C. TI CaMn2Al10: Itinerant Mn magnetism on the verge of magnetic order SO PHYSICAL REVIEW B LA English DT Article ID SPIN FLUCTUATIONS; ELECTRON FERROMAGNETISM; MANGANESE COMPOUNDS; PHASE-TRANSITIONS; CRYSTAL-GROWTH; QUANTUM; SUPERCONDUCTIVITY; ALLOYS; METALS; COEXISTENCE AB We report the discovery of CaMn2Al10, a metal with strong magnetic anisotropy and moderate electronic correlations. Magnetization measurements find a Curie-Weiss moment of 0.83 mu(B)/Mn, significantly reduced from the Hund's rule value, and the magnetic entropy obtained from specific heat measurements is correspondingly small, only approximate to 9% of R ln 2. These results imply that the Mn magnetism is highly itinerant, a conclusion supported by density functional theory calculations that find strong Mn-Al hybridization. Consistent with the layered nature of the crystal structure, the magnetic susceptibility chi is anisotropic below 20 K, with a maximum ratio of chi([010])/chi([001]) approximate to 3.5. A strong power-law divergence chi(T) similar to T-1.2 below 20 K implies incipient ferromagnetic order with a low Curie temperature T-C < 2 K. Our experiments indicate that CaMn2Al10 is a rare example of a system where the weak and itinerant Mn-based magnetism is poised on the verge of order. C1 [Steinke, L.; Yin, W. -G.; Aronson, M. C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Steinke, L.; Smith, G. J.; Kistner-Morris, J. J.; Zellman, S.; Puri, A.; Aronson, M. C.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Simonson, J. W.] Farmingdale State Coll, Dept Phys, Farmingdale, NY 11735 USA. RP Steinke, L (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. EM lsteinke@bnl.gov RI Yin, Weiguo/A-9671-2014 OI Yin, Weiguo/0000-0002-4965-5329 FU US Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH1886, DE-SC0012704] FX Work at Brookhaven National Laboratory was carried out under the auspices of US Department of Energy, Office of Basic Energy Sciences, Contract No. DE-AC02-98CH1886. Research carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, was supported by the US Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-SC0012704. NR 61 TC 1 Z9 1 U1 4 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 24 PY 2015 VL 92 IS 2 AR 020413 DI 10.1103/PhysRevB.92.020413 PG 5 WC Physics, Condensed Matter SC Physics GA CN4YK UT WOS:000358436300001 ER PT J AU Yuan, SJ Terzic, J Wang, JC Li, L Aswartham, S Song, WH Ye, F Cao, G AF Yuan, S. J. Terzic, J. Wang, J. C. Li, L. Aswartham, S. Song, W. H. Ye, F. Cao, G. TI Evolution of magnetism in single-crystal Ca2Ru1-xIrxO4 (0 <= x <= 0.65) SO PHYSICAL REVIEW B LA English DT Article ID METAL-INSULATOR-TRANSITION; WEAK FERROMAGNETISM; NONMETAL TRANSITION; GROUND-STATE; CA2RUO4; SR2IRO4; PHASE AB We report structural, magnetic, transport, and thermal properties of single-crystal Ca2Ru1-xIrxO4 (0 <= x <= 0.65). Ca2RuO4 is a structurally driven Mott insulator with a metal-insulator transition at T-MI = 357 K, which is well separated from antiferromagnetic order at T-N = 110 K. Substitution of a 5d element, Ir, for Ru enhances spin-orbit coupling and locking between the structural distortions and magnetic moment canting. Ir doping intensifies the distortion or rotation of Ru/IrO6 octahedra and induces weak ferromagnetic behavior along the c axis. In particular, Ir doping suppresses TN but concurrently causes an additional magnetic ordering T-N2 at a higher temperature up to 210 K for x = 0.65. The effect of Ir doping sharply contrasts with that of 3d-element doping such as Cr, Mn, and Fe, which suppresses TN and induces unusual negative volume thermal expansion. The stark difference between 3d- and 5d-element doping underlines a strong magnetoelastic coupling inherent in the Ir-rich oxides. C1 [Yuan, S. J.; Terzic, J.; Wang, J. C.; Li, L.; Aswartham, S.; Song, W. H.; Cao, G.] Univ Kentucky, Dept Phys & Astron, Ctr Adv Mat, Lexington, KY 40506 USA. [Wang, J. C.; Ye, F.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Wang, J. C.] Renmin Univ China, Dept Phys, Beijing 100872, Peoples R China. [Song, W. H.] Chinese Acad Sci, Inst Solid State Phys, Hefei 230031, Peoples R China. RP Yuan, SJ (reprint author), Univ Kentucky, Dept Phys & Astron, Ctr Adv Mat, Lexington, KY 40506 USA. EM shujuan.yuan@uky.edu; cao@uky.edu RI Ye, Feng/B-3210-2010; Li, Li/G-6406-2013 OI Ye, Feng/0000-0001-7477-4648; Li, Li/0000-0003-1683-8118 FU National Science Foundation [DMR-1265162]; China Scholarship Council FX This work was supported by the National Science Foundation via Grant No. DMR-1265162 and China Scholarship Council (J.C.W.). NR 35 TC 2 Z9 2 U1 11 U2 47 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUL 24 PY 2015 VL 92 IS 2 AR 024425 DI 10.1103/PhysRevB.92.024425 PG 5 WC Physics, Condensed Matter SC Physics GA CN4YK UT WOS:000358436300003 ER PT J AU Schuster, MD Quaglioni, S Johnson, CW Jurgenson, ED Navratil, P AF Schuster, Micah D. Quaglioni, Sofia Johnson, Calvin W. Jurgenson, Eric D. Navratil, Petr TI Operator evolution for ab initio electric dipole transitions of He-4 SO PHYSICAL REVIEW C LA English DT Article ID LORENTZ INTEGRAL TRANSFORM; EFFECTIVE-FIELD THEORY; RESPONSE FUNCTIONS; LIGHT-NUCLEI; FORCES; RADIUS; ATOMS; MODEL AB A goal of nuclear theory is to make quantitative predictions of low-energy nuclear observables starting from accurate microscopic internucleon forces. A major element of such an effort is applying unitary transformations to soften the nuclear Hamiltonian and hence accelerate the convergence of ab initio calculations as a function of the model space size. The consistent simultaneous transformation of external operators, however, has been overlooked in applications of the theory, particularly for nonscalar transitions. We study the evolution of the electric dipole operator in the framework of the similarity renormalization group method and apply the renormalized matrix elements to the calculation of the He-4 total photoabsorption cross section and electric dipole polarizability. All observables are calculated within the ab initio no-core shell model. We find that, although seemingly small, the effects of evolved operators on the photoabsorption cross section are comparable in magnitude to the correction produced by including the chiral three-nucleon force and cannot be neglected. C1 [Schuster, Micah D.; Johnson, Calvin W.] San Diego State Univ, San Diego, CA 92182 USA. [Quaglioni, Sofia; Jurgenson, Eric D.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Navratil, Petr] TRIUMF, Vancouver, BC V6T 2A3, Canada. RP Schuster, MD (reprint author), San Diego State Univ, 5500 Campanile Dr, San Diego, CA 92182 USA. EM mschuste@rohan.sdsu.edu; quaglioni1@llnl.gov; cjohnson@mail.sdsu.edu FU U.S. Department of Energy by the Lawrence Livermore National Laboratory (LLNL) [DE-AC52-07NA27344]; U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-FG02-96ER40985, DE-FC02-07ER41457]; Natural Sciences and Engineering Research Council of Canada (NSERC) [401945-2011]; Canadian National Research Council; [SCW1158] FX This work was performed in part under the auspices of the U.S. Department of Energy by the Lawrence Livermore National Laboratory (LLNL) under Contract No. DE-AC52-07NA27344. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Awards No. DE-FG02-96ER40985 and No. DE-FC02-07ER41457 as well as under Work Proposal No. SCW1158. Additional support came from the Natural Sciences and Engineering Research Council of Canada (NSERC) under Grant No. 401945-2011. TRIUMF receives funding via a contribution through the Canadian National Research Council. Computing support came from the LLNL institutional Computing Grand Challenge program. Additional resources came from the Computational Science Research Center and the Department of Physics at San Diego State University. NR 65 TC 3 Z9 3 U1 1 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JUL 24 PY 2015 VL 92 IS 1 AR 014320 DI 10.1103/PhysRevC.92.014320 PG 11 WC Physics, Nuclear SC Physics GA CN4YV UT WOS:000358437400002 ER PT J AU Bousso, R Katz, DM Zukowski, C AF Bousso, Raphael Katz, Dan Mainemer Zukowski, Claire TI Anthropic origin of the neutrino mass from cooling failure SO PHYSICAL REVIEW D LA English DT Article ID HOT DARK-MATTER; LYMAN-ALPHA SYSTEMS; COSMOLOGICAL CONSTANT; GALAXY FORMATION; INFLATIONARY UNIVERSE; MODELS; NEUTRALIZATION; CONDENSATION; EVOLUTION; CLUSTERS AB The sum of active neutrino masses is well constrained, 58 meV <= m(nu) less than or similar to 0.23 eV, but the origin of this scale is not well understood. Here we investigate the possibility that it arises by environmental selection in a large landscape of vacua. Earlier work noted the detrimental effects of neutrinos on large-scale structure. However, using Boltzmann codes to compute the smoothed density contrast on Mpc scales, we find that dark matter halos form abundantly for m(nu) greater than or similar to 10 eV. This finding rules out an anthropic origin of m(nu), unless a different catastrophic boundary can be identified. Here we argue that galaxy formation becomes inefficient for m(nu) greater than or similar to 10 eV. We show that in this regime, structure forms late and is dominated by cluster scales, as in a top-down scenario. This is catastrophic: baryonic gas will cool too slowly to form stars in an abundance comparable to our Universe. With this novel cooling boundary, we find that the anthropic prediction for m(nu) agrees at better than 2 sigma with current observational bounds. A degenerate hierarchy is mildly preferred. C1 [Bousso, Raphael; Katz, Dan Mainemer; Zukowski, Claire] Univ Calif Berkeley, Ctr Theoret Phys, Berkeley, CA 94720 USA. [Bousso, Raphael; Katz, Dan Mainemer; Zukowski, Claire] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Bousso, Raphael; Katz, Dan Mainemer; Zukowski, Claire] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Zukowski, Claire] Perimeter Inst Theoret Phys, Waterloo, ON N2L 2Y5, Canada. RP Bousso, R (reprint author), Univ Calif Berkeley, Ctr Theoret Phys, Berkeley, CA 94720 USA. FU Berkeley Center for Theoretical Physics; National Science Foundation [1214644, 1316783]; fqxi grant [RFP3-1323]; US Department of Energy [DE-AC02-05CH11231]; Government of Canada through Industry Canada; Province of Ontario through the Ministry of Research Innovation; NSF Graduate Fellowship FX We thank Niayesh Afshordi, Cora Dvorkin, Lawrence Hall, Wayne Hu, Julien Lesgourgues, Marilena Loverde, David J. E. Marsh, Hitoshi Murayama, Levon Pogosian, Joel Primack, Martin Rees, Uros Seljak, David Spergel, Alexander Vilenkin, and Martin White for very helpful discussions and correspondence. We are particularly grateful to Oliver Zahn for explaining how to use and adapt the CAMB software. This work was supported by the Berkeley Center for Theoretical Physics, by the National Science Foundation (Award No 1214644 and 1316783), by fqxi grant RFP3-1323, and by the US Department of Energy under Contract DE-AC02-05CH11231. Research at the Perimeter Institute is supported by the Government of Canada through Industry Canada and by the Province of Ontario through the Ministry of Research & Innovation. The work of C. Z. is supported by an NSF Graduate Fellowship. NR 91 TC 0 Z9 0 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JUL 24 PY 2015 VL 92 IS 2 AR 025037 DI 10.1103/PhysRevD.92.025037 PG 19 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CN4ZB UT WOS:000358438000005 ER PT J AU Hafiane, A Bielicki, JK Johansson, JO Genest, J AF Hafiane, Anouar Bielicki, John K. Johansson, Jan O. Genest, Jacques TI Novel Apo E-Derived ABCA1 Agonist Peptide (CS-6253) Promotes Reverse Cholesterol Transport and Induces Formation of pre beta-1 HDL In Vitro SO PLOS ONE LA English DT Article ID HIGH-DENSITY-LIPOPROTEIN; APOLIPOPROTEIN-A-I; SCAVENGER RECEPTOR BI; MIMETIC PEPTIDE; CELLULAR CHOLESTEROL; LIPID EFFLUX; AMPHIPATHIC PEPTIDES; BIDIRECTIONAL FLUX; HELICAL PEPTIDES; HUMAN PLASMA AB Apolipoprotein (apo) mimetic peptides replicate some aspects of HDL function. We have previously reported the effects of compound ATI-5261 on its ability to replicate many functions of native apo A-I in the process of HDL biogenesis. ATI-5261 induced muscle toxicity in wild type C57Bl/6 mice, increased CPK, ALT and AST and increase in triglyceride (Tg) levels. Aromatic phenylalanine residues on the non-polar face of ATI-5261, together with positively charged arginine residues at the lipid-water interface were responsible for these effects. This information was used to create a novel analog (CS-6253) that was non-toxic. We evaluated this peptide designed from the carboxyl terminus of apo E, in its ability to mimic apo A-I functionality. Our data shows that the lipidated particles generated by incubating cells overexpressing ABCA1 with lipid free CS-6253 enhances the rate of ABCA1 lipid efflux with high affinity interactions with native ABCA1 oligomeric forms and plasma membrane micro-domains. Interaction between ABCA1 and lipid free CS-6253 resulted in formation of nascent HDL-CS-6253 particles that are actively remodeled in plasma. Mature HDL-CS-6253 particles deliver cholesterol to liver cells via SR-BI in-vitro. CS-6253 significantly increases cholesterol efflux in murine macrophages and in human THP-1 macrophage-derived foam cells expressing ABCA1. Addition of CS-6253 to plasma dose-dependently displaced apo A-I from alpha-HDL particles and led to de novo formation of pre beta-1 HDL that stimulates ABCA1 dependent cholesterol efflux efficiently. When incubated with human plasma CS-6253 was also found to bind with HDL and LDL and promoted the transfer of cholesterol from HDL to LDL predominantly. Our data shows that CS-6253 mimics apo A-I in its ability to promote ABCA1-mediated formation of nascent HDL particles, and enhances formation of pre beta-1 HDL with increase in the cycling of apo A-I between the pre beta and alpha-HDL particles in-vitro. These mechanisms are potentially anti-atherogenic. C1 [Hafiane, Anouar; Genest, Jacques] McGill Univ, Cardiovasc Res Labs Lab, Res Inst, Ctr Hlth, Montreal, PQ H4A 3J1, Canada. [Bielicki, John K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Donner Lab, Berkeley, CA 94720 USA. [Johansson, Jan O.] Artery Therapeut, San Ramon, CA USA. RP Genest, J (reprint author), McGill Univ, Cardiovasc Res Labs Lab, Res Inst, Ctr Hlth, Montreal, PQ H4A 3J1, Canada. EM Jacques.genest@mcgill.ca FU Canadian Institutes of Health Research (CIHR) fund [MOP 15042]; Artery Therapeutics FX The study is funded by the Canadian Institutes of Health Research (CIHR) fund MOP 15042 (JG). Artery Therapeutics provided support in the form of salaries for authors JJ, but did not have any additional role in the study design, data collection and analysis, decision to publish, or preparation of the manuscript. The specific roles of these authors are articulated in the 'author contributions' section. NR 84 TC 7 Z9 7 U1 0 U2 7 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JUL 24 PY 2015 VL 10 IS 7 AR e0131997 DI 10.1371/journal.pone.0131997 PG 32 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CN7NT UT WOS:000358622000020 PM 26207756 ER PT J AU Kumar, MAS Peluso, M Chaudhary, P Dhawan, J Beheshti, A Manickam, K Thapar, U Pena, L Natarajan, M Hlatky, L Demple, B Naidu, M AF Kumar, M. A. Suresh Peluso, Michael Chaudhary, Pankaj Dhawan, Jasbeer Beheshti, Afshin Manickam, Krishnan Thapar, Upasna Pena, Louis Natarajan, Mohan Hlatky, Lynn Demple, Bruce Naidu, Mamta TI Fractionated Radiation Exposure of Rat Spinal Cords Leads to Latent Neuro-Inflammation in Brain, Cognitive Deficits, and Alterations in Apurinic Endonuclease 1 SO PLOS ONE LA English DT Article ID BASE EXCISION; APURINIC/APYRIMIDINIC ENDONUCLEASE-1; STEM/PROGENITOR CELLS; OBJECT RECOGNITION; CLUSTERED LESIONS; INDUCED APOPTOSIS; OXIDATIVE STRESS; PROGENITOR CELLS; STEM-CELLS; DNA-REPAIR AB Ionizing radiation causes degeneration of myelin, the insulating sheaths of neuronal axons, leading to neurological impairment. As radiation research on the central nervous system has predominantly focused on neurons, with few studies addressing the role of glial cells, we have focused our present research on identifying the latent effects of single/fractionated -low dose of low/high energy radiation on the role of base excision repair protein Apurinic Endonuclease-1, in the rat spinal cords oligodendrocyte progenitor cells' differentiation. Apurinic endonuclease-1 is predominantly upregulated in response to oxidative stress by low-energy radiation, and previous studies show significant induction of Apurinic Endonuclease-1 in neurons and astrocytes. Our studies show for the first time, that fractionation of protons cause latent damage to spinal cord architecture while fractionation of HZE (Si-28) induce increase in APE1 with single dose, which then decreased with fractionation. The oligodendrocyte progenitor cells differentiation was skewed with increase in immature oligodendrocytes and astrocytes, which likely cause the observed decrease in white matter, increased neuro-inflammation, together leading to the observed significant cognitive defects. C1 [Kumar, M. A. Suresh] Columbia Univ, Ctr Radiol Res, New York, NY 10032 USA. [Peluso, Michael; Beheshti, Afshin; Hlatky, Lynn; Naidu, Mamta] Tufts Univ, Sch Med, GeneSys Res Inst, Ctr Canc Syst Biol, Boston, MA 02111 USA. [Chaudhary, Pankaj] Queens Univ, Ctr Canc Res & Cell Biol, Belfast, Antrim, North Ireland. [Dhawan, Jasbeer] SUNY Stony Brook, Dept Psychol, Stony Brook, NY 11794 USA. [Manickam, Krishnan; Natarajan, Mohan] UTHSCSA, Dept Pathol, San Antonio, TX USA. [Thapar, Upasna; Demple, Bruce] SUNY Stony Brook, Dept Pharmacol Sci, Stony Brook, NY 11794 USA. [Pena, Louis] Brookhaven Natl Lab, Dept Biosci, Upton, NY 11973 USA. RP Naidu, M (reprint author), Tufts Univ, Sch Med, GeneSys Res Inst, Ctr Canc Syst Biol, Boston, MA 02111 USA. EM mamta@cancer-systems-biology.org OI Chaudhary, Pankaj/0000-0002-0381-3635; Beheshti, Afshin/0000-0003-4643-531X FU NASA [NNX11AO89G, NNAX13AD74G, NNX13AJ01G] FX NASA grants, NNX11AO89G and NNAX13AD74G to MN; NASA grant NNX13AJ01G to LH. NR 47 TC 1 Z9 1 U1 2 U2 2 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JUL 24 PY 2015 VL 10 IS 7 AR e0133016 DI 10.1371/journal.pone.0133016 PG 14 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CN7NT UT WOS:000358622000057 ER PT J AU Zhang, L Roling, LT Wang, X Vara, M Chi, MF Liu, JY Choi, SI Park, J Herron, JA Xie, ZX Mavrikakis, M Xia, YN AF Zhang, Lei Roling, Luke T. Wang, Xue Vara, Madeline Chi, Miaofang Liu, Jingyue Choi, Sang-Il Park, Jinho Herron, Jeffrey A. Xie, Zhaoxiong Mavrikakis, Manos Xia, Younan TI Platinum-based nanocages with subnanometer-thick walls and well-defined, controllable facets SO SCIENCE LA English DT Article ID FUEL-CELL ELECTROCATALYSTS; SHAPE-CONTROLLED SYNTHESIS; OXYGEN REDUCTION ACTIVITY; BY-LAYER DEPOSITION; NANOCRYSTALS; NANOFRAMES; DURABILITY; MONOLAYER; NANOCUBES; CATALYSTS AB A cost-effective catalyst should have a high dispersion of the active atoms, together with a controllable surface structure for the optimization of activity, selectivity, or both. We fabricated nanocages by depositing a few atomic layers of platinum (Pt) as conformal shells on palladium (Pd) nanocrystals with well-defined facets and then etching away the Pd templates. Density functional theory calculations suggest that the etching is initiated via a mechanism that involves the formation of vacancies through the removal of Pd atoms incorporated into the outermost layer during the deposition of Pt. With the use of Pd nanoscale cubes and octahedra as templates, we obtained Pt cubic and octahedral nanocages enclosed by {100} and {111} facets, respectively, which exhibited distinctive catalytic activities toward oxygen reduction. C1 [Zhang, Lei; Wang, Xue; Choi, Sang-Il; Xia, Younan] Georgia Inst Technol, Wallace H Coulter Dept Biomed Engn, Atlanta, GA 30332 USA. [Zhang, Lei; Wang, Xue; Choi, Sang-Il; Xia, Younan] Emory Univ, Atlanta, GA 30332 USA. [Zhang, Lei; Wang, Xue; Xie, Zhaoxiong] Xiamen Univ, State Key Lab Phys Chem Solid Surfaces, Collaborat Innovat Ctr Chem Energy Mat, Xiamen 361005, Fujian, Peoples R China. [Zhang, Lei; Wang, Xue; Xie, Zhaoxiong] Xiamen Univ, Dept Chem, Xiamen 361005, Fujian, Peoples R China. [Roling, Luke T.; Herron, Jeffrey A.; Mavrikakis, Manos] Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 53706 USA. [Vara, Madeline; Park, Jinho; Xia, Younan] Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA. [Chi, Miaofang] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Liu, Jingyue] Arizona State Univ, Dept Phys, Tempe, AZ 85287 USA. [Xia, Younan] Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA. RP Xia, YN (reprint author), Georgia Inst Technol, Wallace H Coulter Dept Biomed Engn, Atlanta, GA 30332 USA. EM younan.xia@bme.gatech.edu RI Xia, Younan/E-8499-2011; Xie, Zhaoxiong/G-3416-2010; Roling, Luke/B-8793-2015; Mavrikakis, Manos/D-5702-2012; Zhang, Lei/N-7527-2015; Chi, Miaofang/Q-2489-2015; Wang, Xue/D-4488-2012 OI Roling, Luke/0000-0001-9742-2573; Mavrikakis, Manos/0000-0002-5293-5356; Chi, Miaofang/0000-0003-0764-1567; Wang, Xue/0000-0002-6298-1858 FU Georgia Institute of Technology; China Scholarship Council; U.S. Department of Energy (DOE)-Basic Energy Sciences (BES), Office of Chemical Sciences [DE-FG02-05ER15731]; DOE Office of Biological and Environmental Research at the Pacific Northwest National Laboratory; DOE [DE-AC02-06CH11357, DE-AC02-05CH11231]; Oak Ridge National Laboratory's Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility FX The syntheses were supported by start-up funds from the Georgia Institute of Technology (to Y.X.). As jointly supervised PhD students from Xiamen University, L.Z. and X.W. were also partially supported by fellowships from the China Scholarship Council. The theoretical modeling work at University of Wisconsin-Madison was supported by the U.S. Department of Energy (DOE)-Basic Energy Sciences (BES), Office of Chemical Sciences, grant DE-FG02-05ER15731. Calculations were performed at supercomputing centers located at the Environmental Molecular Sciences Laboratory, which is sponsored by the DOE Office of Biological and Environmental Research at the Pacific Northwest National Laboratory; Center for Nanoscale Materials at Argonne National Laboratory, supported by DOE contract DE-AC02-06CH11357; and National Energy Research Scientific Computing Center, supported by DOE contract DE-AC02-05CH11231. Part of the electron microscopy work was performed through a user project supported by the Oak Ridge National Laboratory's Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. J.L. gratefully acknowledges the support by Arizona State University and the use of facilities in the John M. Cowley Center for High Resolution Electron Microscopy at Arizona State University. Data described can be found in the main figures and supplementary materials. The authors declare no conflict of interests. NR 27 TC 136 Z9 137 U1 128 U2 581 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JUL 24 PY 2015 VL 349 IS 6246 BP 412 EP 416 DI 10.1126/science.aab0801 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CN4DX UT WOS:000358381400039 PM 26206931 ER PT J AU Annapureddy, HVR Nune, SK Motkuri, RK McGrail, BP Dang, LEX AF Annapureddy, Harsha V. R. Nune, Satish K. Motkuri, Radha Kishan McGrail, B. Peter Dang, Liem X. TI A Combined Experimental and Computational Study on the Stability of Nanofluids Containing Metal Organic Frameworks SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID MOLECULAR-DYNAMICS; ADSORPTION; SIMULATION AB Computational studies on nanofluids composed of metal organic frameworks were performed using molecular modeling techniques. Grand Canonical Monte Carlo simulations were used to study the adsorption behavior of 1,1,1,3,3-pentafluoropropane (R-245fa) in a MIL-101 metal organic frameworks at various temperatures. To understand the stability of the nanofluid composed of MIL-101 particles, we performed molecular dynamics simulations to compute potentials of mean force between hypothetical MIL-101 fragments terminated with two different kinds of modulators in R-245fa and water. Our computed potentials of mean force results indicate that the metal organic frameworks particles tend to disperse better in water than in R-245fa. The reasons for this difference in dispersion were analyzed and are discussed in the paper. Our results agree with experimental results indicating that the potential models employed and modeling approaches provide good descriptions of molecular interactions and the reliabilities. C1 [Annapureddy, Harsha V. R.; Dang, Liem X.] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. [Nune, Satish K.; Motkuri, Radha Kishan; McGrail, B. Peter] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. RP Dang, LEX (reprint author), Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. RI Motkuri, Radha/F-1041-2014 OI Motkuri, Radha/0000-0002-2079-4798 FU U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; Office of Energy Efficiency and Renewable Energy, Geothermal Technologies Program FX This work was supported by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, and by the Office of Energy Efficiency and Renewable Energy, Geothermal Technologies Program. Pacific Northwest National Laboratory is a multiprogram national laboratory operated for DOE by Battelle. NR 28 TC 4 Z9 4 U1 2 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JUL 23 PY 2015 VL 119 IS 29 BP 8992 EP 8999 DI 10.1021/jp5079086 PG 8 WC Chemistry, Physical SC Chemistry GA CN7OM UT WOS:000358623900018 PM 25569021 ER PT J AU Kumar, R Knight, C Wick, CD Chen, B AF Kumar, Revati Knight, Chris Wick, Collin D. Chen, Bin TI Bringing Reactivity to the Aggregation-Volume-Bias Monte Carlo Based Simulation Framework: Water Nucleation Induced by a Reactive Proton SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID VALENCE-BOND MODEL; VAPOR-LIQUID NUCLEATION; HYDRATED EXCESS PROTON; HYDROPHOBIC INTERFACES; BIOMOLECULAR SYSTEMS; COMPUTER-SIMULATION; PHASE-EQUILIBRIA; AQUEOUS-SOLUTION; CRITICAL-POINT; TRANSPORT AB The development of the aggregation-volume-bias Monte Carlo based simulation technique has led to recent success in studying rare nucleation events, but thus far, this simulation method has been limited to nonreactive systems. This work presents the first application of this technique to study a reactive system of relevance to atmospheric chemistry, i.e., formation of water droplets in the presence of a reactive proton, by combining this approach with a multistate empirical valence bond (MSEVB) description of the excess proton (or the hydronium). It was shown that the ability for the hydronium to share its charge with adjacent water molecules changes dramatically with the cluster size, especially when clusters are small and the distribution of the charge is affected by the presence of an interface, emphasizing the need to use this more sophisticated MSEVB model for such a reactive system. In addition, the simulation results obtained from this system are compared to those with nonreactive hard-sphere ions of different sizes. Overall, the presence of a hydronium or ions appeared to dramatically change the free energy landscape of nucleation compared to the pure water system, leading to the formation of a stable precritical cluster. Although the free energy change due to the addition of the first few water molecules was shown to be very sensitive to the ionic details, the later portion of the free energy profile was found to be nearly independent of the nature of the ion. C1 [Kumar, Revati; Chen, Bin] Louisiana State Univ, Dept Chem, Baton Rouge, LA 70803 USA. [Kumar, Revati] Louisiana State Univ, Ctr Computat & Technol, Baton Rouge, LA 70803 USA. [Knight, Chris] Argonne Natl Lab, Leadership Comp Facil, Argonne, IL 60439 USA. [Wick, Collin D.] Louisiana Tech Univ, Coll Engn & Sci, Ruston, LA 71272 USA. RP Kumar, R (reprint author), Louisiana State Univ, Dept Chem, Baton Rouge, LA 70803 USA. EM revatik@lsu.edu; binchen@lsu.edu RI Kumar, Revati/E-7147-2014 OI Kumar, Revati/0000-0002-3272-8720 FU National Science Foundation [CHE-1052015, EPS-1003897]; (U.S.) Department of Energy (DOE) [DE-AC02-06CH11357]; Department of Chemistry; Center of Computation and Technology at Louisiana State University FX This work was supported by National Science Foundation (CHE-1052015 and EPS-1003897). C.K. acknowledges support by the (U.S.) Department of Energy (DOE) under Contract No. DE-AC02-06CH11357. R.K. acknowledges the Department of Chemistry and the Center of Computation and Technology at Louisiana State University for startup funds. Computer resources were provided by the Louisiana Optical Network Initiative (LONI), the Center for Computation and Technology, and the High Performance Computing at LSU. NR 47 TC 2 Z9 2 U1 1 U2 9 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JUL 23 PY 2015 VL 119 IS 29 BP 9068 EP 9075 DI 10.1021/jp508749x PG 8 WC Chemistry, Physical SC Chemistry GA CN7OM UT WOS:000358623900027 PM 25289603 ER PT J AU Chaudhari, MI Sabo, D Pratt, LR Rempe, SB AF Chaudhari, Mangesh I. Sabo, Dubravko Pratt, Lawrence R. Rempe, Susan B. TI Hydration of Kr(aq) in Dilute and Concentrated Solutions SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID QUASI-CHEMICAL THEORY; MOLECULAR-DYNAMICS METHOD; HYDROPHOBIC HYDRATION; WATER; KRYPTON; SIMULATIONS; MODELS; LIQUIDS; VOLUMES; IONS AB Molecular dynamics simulations of water with both multi-Kr and single Kr atomic solutes are carried out to implement quasi-chemical theory evaluation of the hydration free energy of Kr(aq). This approach obtains free energy differences reflecting Kr-Kr interactions at higher concentrations. Those differences are negative changes in hydration free energies with increasing concentrations at constant pressure. The changes are due to a slight reduction of packing contributions in the higher concentration case. The observed Kr-Kr distributions, analyzed with the extrapolation procedure of Kruger et al., yield a modestly attractive osmotic second virial coefficient, B-2 approximate to -60 cm(3)/mol. The thermodynamic analysis interconnecting these two approaches shows that they are closely consistent with each other, providing support for both approaches. C1 [Chaudhari, Mangesh I.] Sandia Natl Labs, Ctr Biol & Mat Sci, Albuquerque, NM 87123 USA. [Sabo, Dubravko] NYU, Dept Chem, New York, NY 10003 USA. [Pratt, Lawrence R.] Tulane Univ, Dept Chem & Biomol Engn, New Orleans, LA 70118 USA. [Rempe, Susan B.] Sandia Natl Labs, Ctr Biol & Mat Sci, Albuquerque, NM 87185 USA. RP Rempe, SB (reprint author), Sandia Natl Labs, Ctr Biol & Mat Sci, POB 5800, Albuquerque, NM 87185 USA. EM michaud@sandia.gov; dubravko.sabo@nyu.edu; lpratt@tulane.edu; slrempe@sandia.gov RI Pratt, Lawrence/H-7955-2012 OI Pratt, Lawrence/0000-0003-2351-7451 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL8500]; Sandia's LDRD program; Gulf of Mexico Research Initiative [12-05/GoMRI-002] FX We thank J. D. Weeks for telling us of ref 33. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL8500. The financial support of Sandia's LDRD program and the Gulf of Mexico Research Initiative (Consortium for Ocean Leadership Grant SA 12-05/GoMRI-002) is gratefully acknowledged. NR 34 TC 5 Z9 5 U1 0 U2 6 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JUL 23 PY 2015 VL 119 IS 29 BP 9098 EP 9102 DI 10.1021/jp508866h PG 5 WC Chemistry, Physical SC Chemistry GA CN7OM UT WOS:000358623900031 PM 25309975 ER PT J AU Gunawardana, KGSH Song, XY AF Gunawardana, K. G. S. H. Song, Xueyu TI Free Energy Calculations of Crystalline Hard Sphere Complexes Using Density Functional Theory SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID FUNDAMENTAL MEASURE-THEORY; WHITE BEAR VERSION; BINARY-MIXTURES; SUPERLATTICE FORMATION; LIQUID; FLUID; TRANSITION; SIMULATION; STABILITY; ENTROPY AB Recently developed fundamental measure density functional theory (FMT) is used to study binary hard sphere (HS) complexes in crystalline phases. By comparing the excess free energy, pressure, and phase diagram, we show that the fundamental measure functional yields good agreements to the available simulation results of AB, AB(2), and AB(13) crystals. Furthermore, we use this functional to study the HS models of five binary crystals, Cu5Zr(C15(b)), Cu51Zr14(beta), Cu10Zr7(phi), CuZr(B2), and CuZr2(C11(b)), which are observed in the Cu-Zr system. The FMT functional gives a well-behaved minimum for most of the hard sphere crystal complexes in the two-dimensional Gaussian parameter space, namely a crystalline phase. However, the current version of FMT functional (White Bear) fails to give a stable minimum for the structure Cu10Zr7(phi). We argue that the observed solid phases for the HS models of the Cu-Zr system are true thermodynamic stable phases and can be used as a reference system in perturbation calculations. C1 [Gunawardana, K. G. S. H.; Song, Xueyu] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Song, Xueyu] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. RP Song, XY (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA. EM xsong@iastate.edu FU Division of Materials Sciences and Engineering, Office of Basic Energy Sciences, U.S. Department of Energy [W-7405-ENG-82]; Iowa State University FX We are grateful to an anonymous referee for including the data of fcc crystal from the WBII functional that agree with the observation that there exists a secondary minimum at low alpha with high packing fractions (Figure 9). This research was sponsored by the Division of Materials Sciences and Engineering, Office of Basic Energy Sciences, U.S. Department of Energy, under Contract W-7405-ENG-82 with Iowa State University. NR 43 TC 1 Z9 1 U1 3 U2 6 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JUL 23 PY 2015 VL 119 IS 29 BP 9160 EP 9166 DI 10.1021/jp5090907 PG 7 WC Chemistry, Physical SC Chemistry GA CN7OM UT WOS:000358623900038 PM 25496266 ER PT J AU Shirota, H Matsuzaki, H Ramati, S Wishart, JF AF Shirota, Hideaki Matsuzaki, Hironori Ramati, Sharon Wishart, James F. TI Effects of Aromaticity in Cations and Their Functional Groups on the Low-Frequency Spectra and Physical Properties of Ionic Liquids SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article AB We have critically investigated the low-frequency spectra of six ionic liquids (ILs) consisting of systematically different cations having benzyl moieties or comparable-sized saturated cyclohexylmethyl groups, by means of femtosecond Raman-induced Kerr effect spectroscopy (fs-RIKES). The target ionic liquids are bis(trifluoromethylsulfonyl)amide ([NTf2](-)) salts of the 1-benzyl-3-methylimidazolium ([BzMIm](+)), 1-benzyl-1-methylpyrrolidinium ([BzMPyrr](+)), 1-benzylpyridinium ([BzPy](+)), 1-cyclohexylmethyl-3-methylimidazolium ([CHxmMIm](+)), 1-cyclohexylmethyl-1-methylpyrrolidinium ([CHxmMPyrr](+)), and 1-cyclohexylmethylpyridinium ([CHxmPy](+)) cations. The primary purpose of this study is to clarify the effects of charged and neutral aromatic moieties on the low-frequency spectrum and bulk properties such as liquid density, surface tension, shear viscosity, glass transition temperature, and melting point. We found that ILs with benzyl groups have larger surface tensions than those with the same cation bearing the cyclohexylmethyl group. The trend in the glass transition temperatures, comparing ILs having the same side group, is pyridinium > imidazolium > pyrrolidinium. The effects of a single aromatic moiety on the shear viscosity are inconclusive, although the viscosities of the ILs with aromatic moieties on both the cation and the benzyl group, i.e., [BzMIm][NTf2] and [BzPy][NTf2], are substantially lower than those of the other ILs at room temperature, as a consequence of their higher fragilities. In the low-frequency Kerr spectra in the frequency range of approximately 0.1 to 200 cm(-1) measured by fs-RIKES, the ILs possessing two aromatic groups show the largest relative intensity of the nuclear response to the electronic response. Both the charged and neutral aromatic rings show signals due to the ring libration; the neutral one appears at a lower frequency than the charged one. The relationship between the first moment of the broad low-frequency spectrum band and the bulk parameter consisting of the square root of the surface tension divided by the liquid density is obeyed by the cyclohexylmethyl derivatives whether the cation is aromatic or not, but not by the ILs with the neutral aromatic benzyl group. Quantum chemistry calculations have been also performed to understand the vibrational modes of the ionic species in the ILs. C1 [Shirota, Hideaki] Chiba Univ, Dept Nanomat Sci, Inage Ku, Chiba 2638522, Japan. [Shirota, Hideaki; Matsuzaki, Hironori] Chiba Univ, Dept Chem, Inage Ku, Chiba 2638522, Japan. [Ramati, Sharon; Wishart, James F.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Shirota, H (reprint author), Chiba Univ, Dept Nanomat Sci, Inage Ku, Chiba 2638522, Japan. EM shirota@faculty.chiba-u.jp; wishart@bnl.gov RI Wishart, James/L-6303-2013 OI Wishart, James/0000-0002-0488-7636 FU Tokyo Ohka Foundation for Promotion of Science and Technology; U.S. Department of Energy Office of Science, Division of Chemical Sciences, Geosciences and Biosciences [DE-AC02-98CH10886] FX Professor Richard M. Stratt (Brown University) is gratefully acknowledged, because the motivation of this study came up from discussion with him in a meeting (H.S.). J.F.W. and S.R. thank Ms. Nicole Zmich, Ms. Jasmine Hatcher, Dr. Tomasz Szreder, and Prof. Sharon Lall-Ramnarine for assistance with these studies and Dr. Huimin Luo for helpful discussions. The Tokyo Ohka Foundation for Promotion of Science and Technology supported the fs-RIKES, surface tension, and density measurements at Chiba University. The IL synthesis, viscometry, and thermal measurements at BNL were supported by the U.S. Department of Energy Office of Science, Division of Chemical Sciences, Geosciences and Biosciences under Contract No. DE-AC02-98CH10886. NR 0 TC 8 Z9 8 U1 1 U2 24 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JUL 23 PY 2015 VL 119 IS 29 BP 9173 EP 9187 DI 10.1021/jp509412z PG 15 WC Chemistry, Physical SC Chemistry GA CN7OM UT WOS:000358623900040 PM 25389916 ER PT J AU Chang, HJ Trease, NM Ilott, AJ Zeng, DL Du, LS Jerschow, A Grey, CP AF Chang, Hee Jung Trease, Nicole M. Ilott, Andrew J. Zeng, Dongli Du, Lin-Shu Jerschow, Alexej Grey, Clare P. TI Investigating Li Microstructure Formation on Li Anodes for Lithium Batteries by in Situ Li-6/Li-7 NMR and SEM SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SCANNING-ELECTRON-MICROSCOPY; ION BATTERIES; MAGNETIC-SUSCEPTIBILITY; LITHIUM/POLYMER CELLS; FIELD INHOMOGENEITY; BULK SUSCEPTIBILITY; CYCLING EFFICIENCY; STRUCTURAL-CHANGES; DENDRITIC GROWTH; MORPHOLOGY AB The growth of lithium microstructures during battery cycling has, to date, prohibited the use of Li metal anodes and raises serious safety concerns even in conventional lithium-ion rechargeable batteries, particularly if they are charged at high rates. The electrochemical conditions under which these Li microstructures grow have, therefore, been investigated by in situ nuclear magnetic resonance (NMR), scanning electron microscopy (SEM), and susceptibility calculations. Lithium metal symmetric bag cells containing LiPF6 in EC/DMC electrolytes were used. Distinct Li-7 NMR resonances were observed due to the Li metal bulk electrodes and microstructures, the changes in peak positions and intensities being monitored in situ during Li deposition. The changes in the NMR spectra, observed as a function of separator thickness and porosity (using Celgard and Whatmann glass microfiber membranes) and different applied pressures, were correlated with changes in the type of microstructure, by using SEM. Isotopically enriched Li-6 metal electrodes were used against natural abundance predominantly Li-7 metal counter electrodes to investigate radiofrequency (rf) field penetration into the Li anode and to confirm the assignment of the higher frequency peak to Li dendrites. The conclusions were supported by calculations performed to explore the effect of the different microstructures on peak position/broadening, the study showing that Li NMR spectroscopy can be used as a sensitive probe of both the amount and type of microstructure formation. C1 [Chang, Hee Jung; Trease, Nicole M.; Du, Lin-Shu; Grey, Clare P.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Ilott, Andrew J.; Jerschow, Alexej] NYU, Dept Chem, New York, NY 10003 USA. [Zeng, Dongli] Brookhaven Natl Lab, Dept Chem, Upton, NY 11793 USA. [Trease, Nicole M.; Grey, Clare P.] Univ Cambridge, Dept Chem, Cambridge CB2 1EW, England. RP Grey, CP (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. EM cpg27@cam.ac.uk FU North East Center for Chemical Energy Storage (NECCES); Energy Frontier Research Center; U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences [DE-SC0001294, DE-SC0012583]; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of FreedomCAR and Vehicle Technologies of the U.S. DOE [DE-AC03-765F00098, 6517749]; Lawrence Berkeley National Laboratory; New York State Energy Research Development Authority (NYSER-DA) FX We gratefuly thank Jim Quinn for helping with the SEM experiments and Adam Best, Baris Key, and Rangeet Bhattancharrya for helpful discussions. This work was supported as part of the North East Center for Chemical Energy Storage (NECCES), an Energy Frontier Research Center funded by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, under Awards DE-SC0001294 and DE-SC0012583 (N.M.T., A.J.I., and methodology), and by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of FreedomCAR and Vehicle Technologies of the U.S. DOE under Contract DE-AC03-765F00098 via Subcontract 6517749 with the Lawrence Berkeley National Laboratory (Li metal) and by the New York State Energy Research Development Authority (NYSER-DA) (H.J.C.). NR 47 TC 13 Z9 13 U1 11 U2 106 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 23 PY 2015 VL 119 IS 29 BP 16443 EP 16451 DI 10.1021/acs.jpcc.5b03396 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CN7ON UT WOS:000358624000005 ER PT J AU Yu, L Liu, Y Yang, F Evans, J Rodriguez, JA Liu, P AF Yu, Liang Liu, Yun Yang, Fan Evans, Jaime Rodriguez, Jose A. Liu, Ping TI CO Oxidation on Gold-Supported Iron Oxides: New Insights into Strong Oxide-Metal Interactions SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID INITIO MOLECULAR-DYNAMICS; LOW-TEMPERATURE OXIDATION; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; CATALYTIC-OXIDATION; ACTIVE GOLD; BASIS-SET; TITANIA; NANOPARTICLES; INTERFACE AB Very active FeOx-Au catalysts for CO oxidation are obtained after depositing nanoparticles of FeO, Fe3O4, and Fe2O3 on a Au(111) substrate. Neither FeO nor Fe2O3 is stable under the reaction conditions. Under an environment of CO/O-2, they undergo oxidation (FeO) or reduction (Fe2O3) to yield nanoparticles of Fe3O4 that are not formed in a bulk phase. Using a combined experimental and theoretical approach, we show a strong oxide-metal interaction (SOMI) between Fe3O4 nanostructures and Au(111), which gives the oxide special properties, allows the formation of an active phase, and provides a unique interface to facilitate a catalytic reaction. Our work highlights the important role that the SOMI can play in enhancing the catalytic performance of the oxide component in metal-oxide catalysts. C1 [Yu, Liang; Liu, Yun; Yang, Fan] Dalian Inst Chem Phys, iChEM Collaborat Innovat Ctr Chem Energy Mat, State Key Lab Catalysis, Dalian 116023, Peoples R China. [Evans, Jaime] Cent Univ Venezuela, Fac Ciencias, Caracas 1020A, Venezuela. [Rodriguez, Jose A.; Liu, Ping] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Rodriguez, JA (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM rodrigez@bnl.gov; pingliu3@bnl.gov RI YANG, FAN/J-2706-2012 OI YANG, FAN/0000-0002-1406-9717 FU US DOE, Office of BES [DE-SC0012704]; Office of Science of the U.S. DOE [DE-AC02-05CH11231]; NSFC [21303195, 21473191]; MOST [2013CB933100] FX Work carried at BNL was financed by the US DOE, Office of BES (Grant No. DE-SC0012704). Calculations were performed using computational resources at the Center for Functional Nanomaterials, a DOE user facility at Brookhaven National Laboratory, and at the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the U.S. DOE under Contract No. DE-AC02-05CH11231. INTEVEP and IDB financed the work done at the UCV. Work carried out at DICP was financed by NSFC (Grant No. 21303195, 21473191) and MOST (Grant No. 2013CB933100). We appreciate the valuable discussions with Prof. X. H. Bao. NR 49 TC 10 Z9 10 U1 12 U2 76 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 23 PY 2015 VL 119 IS 29 BP 16614 EP 16622 DI 10.1021/acs.jpcc.5b03315 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CN7ON UT WOS:000358624000024 ER PT J AU Li, X Hua, WJ Guo, JH Luo, Y AF Li, Xin Hua, Weijie Guo, Jinghua Luo, Yi TI Electronic Structure of Nitrogen-Doped Graphene in the Ground and Core-Excited States from First-Principles Simulations SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID X-RAY SPECTROSCOPY; TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; OXYGEN REDUCTION; HYDROGEN STORAGE; BORON; NITRIDE; APPROXIMATION; VACANCIES; SHIFTS AB We have calculated the N 1s near-edge X-ray absorption fine structure (NEXAFS) spectra of nitrogen-doped monolayer graphene (NG) using density functional theory (DFT) with the equivalent core hole approximation. The hexavacancy (6V) defect and its dependence on the nitrogen-doping concentration have been analyzed in detail via both N 1s -> pi* and N 1s -> sigma* transitions. The NEXAFS spectra are sensitive to the doping concentration of N in the pi* region: diluted doping weakens the main pi* peak and smears the oscillations in this region. The vacancy defect leads to a red-shift in both the pi and sigma spectra. A pyridinic nitrogen at the 6V defect center exhibits a sharp pi* peak at 398.4 eV, which agrees well with the experimental pre-edge structure at 398.6 eV. The sigma* peak is split in two, which can serve as the fingerprint to reveal the nature of the defect. A structural change from pyridinic to pyrrolic NG results in a distinctive difference in the spectral shape. The ground-state band structure has also been simulated at the DFT level with periodic boundary conditions. Similar profiles are found in the N 2p projected density of states above the Fermi level and in the N 1s NEXAFS spectra. C1 [Li, Xin; Hua, Weijie; Luo, Yi] KTH Royal Inst Technol, Sch Biotechnol, Dept Theoret Chem & Biol, S-10691 Stockholm, Sweden. [Li, Xin; Guo, Jinghua] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Hua, WJ (reprint author), KTH Royal Inst Technol, Sch Biotechnol, Dept Theoret Chem & Biol, S-10691 Stockholm, Sweden. EM hua@theochem.kth.se RI Hua, Weijie/F-3099-2010 OI Hua, Weijie/0000-0002-6706-651X FU Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX We acknowledge the support from Goran Gustafsson Foundation for Research in Natural Sciences and Medicine and the Swedish Research Council (VR). The work at the Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The Swedish National Infrastructure for Computing (SNIC) and the National Energy Research Scientific Computing Center (NERSC) are acknowledged for the computational resources. NR 54 TC 5 Z9 5 U1 12 U2 49 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 23 PY 2015 VL 119 IS 29 BP 16660 EP 16666 DI 10.1021/acs.jpcc.5b03981 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CN7ON UT WOS:000358624000029 ER PT J AU Ciemny, AA Dominik, W Ginter, T Grzywacz, R Janas, Z Kuich, M Mazzocchi, C Pfutzner, M Pomorski, M Zarzynski, F Bazin, D Baumann, T Bezbakh, A Crider, BP Cwiok, M Go, S Kaminski, G Kolos, K Korgul, A Kwan, E Liddick, S Miernik, K Paulauskas, SV Pereira, J Rykaczewski, K Sumithrarachchi, C Xiao, Y AF Ciemny, A. A. Dominik, W. Ginter, T. Grzywacz, R. Janas, Z. Kuich, M. Mazzocchi, C. Pfutzner, M. Pomorski, M. Zarzynski, F. Bazin, D. Baumann, T. Bezbakh, A. Crider, B. P. Cwiok, M. Go, S. Kaminski, G. Kolos, K. Korgul, A. Kwan, E. Liddick, S. Miernik, K. Paulauskas, S. V. Pereira, J. Rykaczewski, K. Sumithrarachchi, C. Xiao, Y. TI First observation of Ge-59 SO PHYSICAL REVIEW C LA English DT Article ID DECAY AB In an experiment at the A1900 spectrometer of the National Superconducting Cyclotron Laboratory at Michigan State University the new isotope Ge-59 was identified and the cross section for production of the most neutron-deficient Ge59-62 isotopes in the fragmentation of a Kr-78 beam at 150 MeV/nucleon measured. This experimental information is relevant for the hunt of new two-proton emitters in the region above the doubly-magic Ni-48. C1 [Ciemny, A. A.; Dominik, W.; Janas, Z.; Kuich, M.; Mazzocchi, C.; Pfutzner, M.; Pomorski, M.; Zarzynski, F.; Cwiok, M.; Korgul, A.; Miernik, K.] Warsaw Univ, Fac Phys, PL-02093 Warsaw, Poland. [Ginter, T.; Bazin, D.; Baumann, T.; Crider, B. P.; Kwan, E.; Liddick, S.; Paulauskas, S. V.; Pereira, J.; Sumithrarachchi, C.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Grzywacz, R.; Go, S.; Kolos, K.; Xiao, Y.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Grzywacz, R.; Rykaczewski, K.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Bezbakh, A.; Kaminski, G.] Joint Inst Nucl Res, Dubna 141980, Russia. [Kaminski, G.] Inst Nucl Phys PAN, PL-31342 Krakow, Poland. [Liddick, S.] Michigan State Univ, Dept Chem, E Lansing, MI 48824 USA. RP Mazzocchi, C (reprint author), Warsaw Univ, Fac Phys, PL-02093 Warsaw, Poland. EM chiara.mazzocchi@fuw.edu.pl FU Polish National Science Center [UMO-2011/01/B/ST2/01943]; US Department of Energy, Office of Science, Office of Nuclear Physics, under US DOE [DE-AC05-00OR22725 (ORNL), DE-FG02-96ER40983 (UTK)]; fund source National Nuclear Security Administration [DEFC03-03NA00143]; Stewardship Science Academic Alliance program through DOE [DE-FG52-08NA28552 (UTK)]; Polish Ministry of Science and Higher Education [0079/DIA/2014/43] FX We wish to acknowledge the National Superconducting Cyclotron Laboratory staff for assisting with the experiments and providing excellent quality radioactive beams. This work was supported by the Polish National Science Center under Contract No. UMO-2011/01/B/ST2/01943, by the US Department of Energy, Office of Science, Office of Nuclear Physics, under US DOE Grant Nos. DE-AC05-00OR22725 (ORNL) and DE-FG02-96ER40983 (UTK), by the fund source National Nuclear Security Administration Grant No. DEFC03-03NA00143, and under the Stewardship Science Academic Alliance program through DOE Cooperative Agreement No. DE-FG52-08NA28552 (UTK). A. A. Ciemny acknowledges support by the Polish Ministry of Science and Higher Education through Grant No. 0079/DIA/2014/43 ("Grant Diamentowy"). NR 14 TC 4 Z9 5 U1 2 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JUL 23 PY 2015 VL 92 IS 1 AR 014622 DI 10.1103/PhysRevC.92.014622 PG 4 WC Physics, Nuclear SC Physics GA CN4CI UT WOS:000358376100007 ER PT J AU Pfutzner, M Dominik, W Janas, Z Mazzocchi, C Pomorski, M Bezbakh, AA Borge, MJG Chrapkiewicz, K Chudoba, V Frederickx, R Kaminski, G Kowalska, M Krupko, S Kuich, M Kurcewicz, J Lis, AA Lund, MV Miernik, K Perkowski, J Raabe, R Randisi, G Riisager, K Sambi, S Tengblad, O Wenander, F AF Pfuetzner, M. Dominik, W. Janas, Z. Mazzocchi, C. Pomorski, M. Bezbakh, A. A. Borge, M. J. G. Chrapkiewicz, K. Chudoba, V. Frederickx, R. Kaminski, G. Kowalska, M. Krupko, S. Kuich, M. Kurcewicz, J. Lis, A. A. Lund, M. V. Miernik, K. Perkowski, J. Raabe, R. Randisi, G. Riisager, K. Sambi, S. Tengblad, O. Wenander, F. TI beta decay of He-6 into the alpha plus d continuum SO PHYSICAL REVIEW C LA English DT Article ID DELAYED DEUTERON EMISSION; MODEL AB The rare beta-decay channel of He-6 into the alpha + d continuum was investigated at the REX-ISOLDE facility. Bunches of postaccelerated He-6 ions were implanted into the optical time projection chamber (OTPC), where the decays with emission of charged particles were recorded. This novel technique allowed us to extend the low-energy end of the spectrum down to 150 keV in alpha + d center of mass, corresponding to a deuteron energy of 100 keV. The branching ratio for this process amounts to [2.78 +/- 0.07(stat) +/- 0.17(sys)] x 10(-6). The shape of the spectrum is found to be in a good agreement with a three-body model, while the total intensity is about 20% larger than the predicted one. C1 [Pfuetzner, M.; Dominik, W.; Janas, Z.; Mazzocchi, C.; Pomorski, M.; Chrapkiewicz, K.; Kuich, M.; Lis, A. A.; Miernik, K.] Univ Warsaw, Fac Phys, PL-02093 Warsaw, Poland. [Bezbakh, A. A.; Chudoba, V.; Kaminski, G.; Krupko, S.] Joint Inst Nucl Res, Dubna 141980, Moscow Region, Russia. [Borge, M. J. G.; Tengblad, O.] CSIC, Inst Estruct Mat, E-28006 Madrid, Spain. [Borge, M. J. G.; Kowalska, M.; Kurcewicz, J.; Wenander, F.] CERN, ISOLDE, CH-1211 Geneva 23, Switzerland. [Frederickx, R.; Raabe, R.; Randisi, G.; Sambi, S.] Katholieke Univ Leuven, Inst Kern & Stralingsfys, B-3001 Leuven, Belgium. [Kaminski, G.] Inst Nucl Phys PAN, PL-31342 Krakow, Poland. [Kuich, M.] Warsaw Univ Technol, Fac Phys, PL-00662 Warsaw, Poland. [Lund, M. V.; Riisager, K.] Aarhus Univ, Dept Phys & Astron, DK-8000 Aarhus C, Denmark. [Miernik, K.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Perkowski, J.] Univ Lodz, Fac Phys & Appl Comp Sci, PL-90236 Lodz, Poland. RP Pfutzner, M (reprint author), Univ Warsaw, Fac Phys, Pasteura 5, PL-02093 Warsaw, Poland. RI Tengblad, Olof/O-5852-2015 FU Polish National Science Center [UMO-2011/01/B/ST2/01943]; European Nuclear Science and Applications Research (ENSAR) [262010]; Research Foundation Flanders (FWO); BOF KU Leuven [GOA/2010/010]; Interuniversity Attraction Poles Programme [BriX network P7/12] FX We would like to thank the ISOLDE facility for providing the excellent beam. We are grateful to P. Descouvemont for providing us with the results of Ref. [15] in a tabular form. The work was partially supported by the Polish National Science Center under Contract No. UMO-2011/01/B/ST2/01943, by the European Nuclear Science and Applications Research (ENSAR) under Project No. 262010, by the Research Foundation Flanders (FWO), by GOA/2010/010 (BOF KU Leuven), and by the Interuniversity Attraction Poles Programme initiated by the Belgian Science Policy Office (BriX network P7/12). NR 21 TC 5 Z9 5 U1 2 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JUL 23 PY 2015 VL 92 IS 1 AR 014316 DI 10.1103/PhysRevC.92.014316 PG 7 WC Physics, Nuclear SC Physics GA CN4CI UT WOS:000358376100003 ER PT J AU Bailey, JA Bazavov, A Bernard, C Bouchard, CM DeTar, C Du, D El-Khadra, AX Foley, J Freeland, ED Gamiz, E Gottlieb, S Heller, UM Komijani, J Kronfeld, AS Laiho, J Levkova, L Liu, YZ Mackenzie, PB Meurice, Y Neil, E Qiu, SW Simone, JN Sugar, R Toussaint, D Van de Water, RS Zhou, R AF Bailey, Jon. A. Bazavov, A. Bernard, C. Bouchard, C. M. DeTar, C. Du, D. El-Khadra, A. X. Foley, J. Freeland, E. D. Gamiz, E. Gottlieb, Steven Heller, U. M. Komijani, J. Kronfeld, A. S. Laiho, J. Levkova, L. Liu, Yuzhi Mackenzie, P. B. Meurice, Y. Neil, E. Qiu, Si-Wei Simone, J. N. Sugar, R. Toussaint, D. Van de Water, R. S. Zhou, R. CA Fermilab Lattice Collaboration MILC Collaboration TI vertical bar V-ub vertical bar from B -> pi l nu decays and (2+1)-flavor lattice QCD SO PHYSICAL REVIEW D LA English DT Article ID YANG-MILLS THEORY; CHIRAL PERTURBATION-THEORY; GAUGE-THEORIES; FORM-FACTORS; HEAVY-QUARK; SYMMETRY; FERMIONS AB We present a lattice-QCD calculation of the B -> pi l nu semileptonic form factors and a new determination of the CKM matrix element vertical bar V-ub vertical bar. We use the MILC asqtad (2 + 1)-flavor lattice configurations at four lattice spacings and light-quark masses down to 1/20 of the physical strange-quark mass. We extrapolate the lattice form factors to the continuum using staggered chiral perturbation theory in the hard-pion and SU (2) limits. We employ a model-independent z parametrization to extrapolate our lattice form factors from large-recoil momentum to the full kinematic range. We introduce a new functional method to propagate information from the chiral-continuum extrapolation to the z expansion. We present our results together with a complete systematic error budget, including a covariance matrix to enable the combination of our form factors with other lattice-QCD and experimental results. To obtain vertical bar V-ub vertical bar, we simultaneously fit the experimental data for the B -> pi l nu differential decay rate obtained by the BABAR and Belle collaborations together with our lattice form-factor results. We find vertical bar V-ub vertical bar = (3.72 +/- 0.16) x 10(-3), where the error is from the combined fit to lattice plus experiments and includes all sources of uncertainty. Our form-factor results bring the QCD error on vertical bar V-ub vertical bar to the same level as the experimental error. We also provide results for the B -> pi l nu vector and scalar form factors obtained from the combined lattice and experiment fit, which are more precisely determined than from our lattice-QCD calculation alone. These results can be used in other phenomenological applications and to test other approaches to QCD. C1 [Bailey, Jon. A.] Seoul Natl Univ, Dept Phys & Astron, Seoul, South Korea. [Bazavov, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Bernard, C.; Komijani, J.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Bouchard, C. M.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Bouchard, C. M.] Coll William & Mary, Dept Phys, Williamsburg, VA 23185 USA. [DeTar, C.; Foley, J.; Levkova, L.; Qiu, Si-Wei] Univ Utah, Dept Phys & Astron, Salt Lake City, UT USA. [Du, D.; El-Khadra, A. X.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Du, D.; Laiho, J.] Syracuse Univ, Dept Phys, Syracuse, NY USA. [Freeland, E. D.] Sch Art Inst Chicago, Liberal Arts Dept, Chicago, IL USA. [Gamiz, E.] Univ Granada, CAFPE, Granada, Spain. [Gamiz, E.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Gottlieb, Steven] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Heller, U. M.] Amer Phys Soc, Ridge, NY USA. [Kronfeld, A. S.; Mackenzie, P. B.; Simone, J. N.; Van de Water, R. S.; Zhou, R.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Kronfeld, A. S.] Tech Univ Munich, Inst Adv Study, Garching, Germany. [Liu, Yuzhi; Neil, E.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Meurice, Y.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Neil, E.] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Sugar, R.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Toussaint, D.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. RP Du, D (reprint author), Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. EM dadu@syr.edu RI Gamiz, Elvira/E-8009-2016; Bouchard, Christopher/N-3723-2016 OI Gamiz, Elvira/0000-0001-5125-2687; Bouchard, Christopher/0000-0003-1639-7164 FU Office of Science of the United States Department of Energy; National Institute for Computational Science; Pittsburgh Supercomputer Center; San Diego Supercomputer Center; Texas Advanced Computing Center; National Science Foundation's Teragrid/XSEDE Program; U.S. Department of Energy [DE-FG02-91ER40628, DE-FC02-12ER41879, DE-SC0010120, DE-FG02-91ER40661, DE-FC02-06ER41443, DE-FG02-13ER42001, DE-FG02-13ER41976, DE-SC0010114, DE-AC02-98CH10886, DE-AC02-07CH11359]; National Science Foundation [PHY-1067881, PHY-10034278, PHY-1417805, PHY1212389, PHY-1316748]; URA Visiting Scholars' program; MINECO (Spain) [FPA2010-16696, FPA2006-05294]; Ramon y Cajal program; Junta de Andalucia (Spain) [FQM-101, FQM-6552]; European Commission [PCIG10-GA-2011-303781]; German Excellence Initiative; European Union Seventh Framework Programme [291763]; European Union's Marie Curie COFUND program; Basic Science Research Program of the National Research Foundation of Korea (NRF); Ministry of Education [2014027937]; Creative Research Initiatives Program of the NRF grant - Korean government (MEST) [2014001852] FX We thank Jochen Dingfelder for the helpful information about the experimental measurements and HFAG averaging procedure. D.D. thanks Peter Lepage for sharing his lsqfit code (github.com/gplepage/lsqfit), which is extensively used in the fitting procedures of the analysis. We also thank Heechang Na for valuable discussions. Computations for this work were carried out with resources provided by the USQCD Collaboration, the Argonne Leadership Computing Facility, the National Energy Research Scientific Computing Center, and the Los Alamos National Laboratory, which are funded by the Office of Science of the United States Department of Energy; and with resources provided by the National Institute for Computational Science, the Pittsburgh Supercomputer Center, the San Diego Supercomputer Center, and the Texas Advanced Computing Center, which are funded through the National Science Foundation's Teragrid/XSEDE Program. This work was supported in part by the U.S. Department of Energy under Grants No. DE-FG02-91ER40628 (C.B., J.K.), No. DE-FC02-12ER41879 (C.D., J.F., L.L.), No. DE-SC0010120 (S.G.), No. DE-FG02-91ER40661 (S.G., R.Z.), No. DE-FC02-06ER41443 (R.Z.), No. DE-FG02-13ER42001 (D.D., A.X.K.), No. DE-FG02-13ER41976 (D.T.), No. DE-SC0010114 (Y.M.); by the National Science Foundation under Grants No. PHY-1067881, No. PHY-10034278 (C.D., L.L., S.-W.Q.), No. PHY-1417805 (J.L., D.D.), No. PHY1212389 (R.Z.), No. PHY-1316748 (R.S.); by the URA Visiting Scholars' program (C.M.B., D.D., A.X.K., Y.L., Y.M.); by the MINECO (Spain) under Grants No. FPA2010-16696, No. FPA2006-05294, and the Ramon y Cajal program (E.G.); by the Junta de Andalucia (Spain) under Grants No. FQM-101 and No. FQM-6552 (E.G.); by the European Commission under Grant No. PCIG10-GA-2011-303781 (E.G.); by the German Excellence Initiative and the European Union Seventh Framework Programme under grant agreement No. 291763 as well as the European Union's Marie Curie COFUND program (A.S.K.); and by the Basic Science Research Program of the National Research Foundation of Korea (NRF) funded by the Ministry of Education (No. 2014027937) and the Creative Research Initiatives Program (No. 2014001852) of the NRF grant funded by the Korean government (MEST) (J.A.B.). This manuscript has been coauthored by an employee of Brookhaven Science Associates, LLC, under Contract No. DE-AC02-98CH10886 with the U.S. Department of Energy. Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. DE-AC02-07CH11359 with the U.S. Department of Energy. NR 76 TC 22 Z9 22 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JUL 23 PY 2015 VL 92 IS 1 AR 014024 DI 10.1103/PhysRevD.92.014024 PG 32 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CN4CO UT WOS:000358376900002 ER PT J AU Matvienko, D Kuzmin, A Eidelman, S Abdesselam, A Adachi, I Aihara, H Al Said, S Arinstein, K Asner, DM Aulchenko, V Aushev, T Ayad, R Babu, V Badhrees, I Bahinipati, S Bakich, AM Bansal, V Bhardwaj, V Bhuyan, B Biswal, J Bobrov, A Bondar, A Bonvicini, G Bozek, A Bracko, M Browder, TE Cervenkov, D Chen, A Cheon, BG Chilikin, K Chistov, R Cho, K Chobanova, V Choi, SK Choi, Y Cinabro, D Dalseno, J Dingfelder, J Dolezal, Z Drasal, Z Drutskoy, A Dutta, D Epifanov, D Farhat, H Fast, JE Ferber, T Fulsom, BG Gaur, V Gabyshev, N Garmash, A Getzkow, D Gillard, R Goh, YM Goldenzweig, P Golob, B Hara, T Hayasaka, K Hayashii, H He, XH Hou, WS Iijima, T Inguglia, G Ishikawa, A Itoh, R Iwasaki, Y Jaegle, I Joffe, D Joo, KK Julius, T Kawasaki, T Kim, DY Kim, JB Kim, JH Kim, KT Kim, MJ Kim, SH Kim, YJ Ko, BR Kodys, P Korpar, S Krokovny, P Kumar, R Lange, JS Lee, DH Li Gioi, L Libby, J Liventsev, D Miyabayashi, K Miyata, H Mizuk, R Mohanty, GB Moll, A Mussa, R Nakano, E Nakao, M Nanut, T Nayak, M Nisar, NK Nishida, S Ogawa, S Pakhlova, G Pal, B Park, CW Park, H Pedlar, TK Pesantez, L Pestotnik, R Petric, M Piilonen, LE Pulvermacher, C Ribezl, E Ritter, M Rostomyan, A Sakai, Y Sandilya, S Santelj, L Sanuki, T Schneider, O Schnell, G Schwanda, C Senyo, K Seon, O Sevior, ME Shapkin, M Shebalin, V Shen, CP Shibata, TA Shiu, JG Shwartz, B Sibidanov, A Simon, F Sohn, YS Sokolov, A Staric, M Steder, M Sumihama, M Sumisawa, K Tamponi, U Tanida, K Teramoto, Y Uchida, M Uehara, S Unno, Y Uno, S Urquijo, P Usov, Y Van Hulse, C Vanhoefer, P Varner, G Vinokurova, A Vorobyev, V Wagner, MN Wang, CH Wang, MZ Wang, P Watanabe, Y Williams, KM Won, E Yamamoto, H Yashchenko, S Yook, Y Zhang, ZP Zhilich, V Zhulanov, V Zupanc, A AF Matvienko, D. Kuzmin, A. Eidelman, S. Abdesselam, A. Adachi, I. Aihara, H. Al Said, S. Arinstein, K. Asner, D. M. Aulchenko, V. Aushev, T. Ayad, R. Babu, V. Badhrees, I. Bahinipati, S. Bakich, A. M. Bansal, V. Bhardwaj, V. Bhuyan, B. Biswal, J. Bobrov, A. Bondar, A. Bonvicini, G. Bozek, A. Bracko, M. Browder, T. E. Cervenkov, D. Chen, A. Cheon, B. G. Chilikin, K. Chistov, R. Cho, K. Chobanova, V. Choi, S. -K. Choi, Y. Cinabro, D. Dalseno, J. Dingfelder, J. Dolezal, Z. Drasal, Z. Drutskoy, A. Dutta, D. Epifanov, D. Farhat, H. Fast, J. E. Ferber, T. Fulsom, B. G. Gaur, V. Gabyshev, N. Garmash, A. Getzkow, D. Gillard, R. Goh, Y. M. Goldenzweig, P. Golob, B. Hara, T. Hayasaka, K. Hayashii, H. He, X. H. Hou, W. -S. Iijima, T. Inguglia, G. Ishikawa, A. Itoh, R. Iwasaki, Y. Jaegle, I. Joffe, D. Joo, K. K. Julius, T. Kawasaki, T. Kim, D. Y. Kim, J. B. Kim, J. H. Kim, K. T. Kim, M. J. Kim, S. H. Kim, Y. J. Ko, B. R. Kodys, P. Korpar, S. Krokovny, P. Kumar, R. Lange, J. S. Lee, D. H. Li Gioi, L. Libby, J. Liventsev, D. Miyabayashi, K. Miyata, H. Mizuk, R. Mohanty, G. B. Moll, A. Mussa, R. Nakano, E. Nakao, M. Nanut, T. Nayak, M. Nisar, N. K. Nishida, S. Ogawa, S. Pakhlova, G. Pal, B. Park, C. W. Park, H. Pedlar, T. K. Pesantez, L. Pestotnik, R. Petric, M. Piilonen, L. E. Pulvermacher, C. Ribezl, E. Ritter, M. Rostomyan, A. Sakai, Y. Sandilya, S. Santelj, L. Sanuki, T. Schneider, O. Schnell, G. Schwanda, C. Senyo, K. Seon, O. Sevior, M. E. Shapkin, M. Shebalin, V. Shen, C. P. Shibata, T. -A. Shiu, J. -G. Shwartz, B. Sibidanov, A. Simon, F. Sohn, Y. -S. Sokolov, A. Staric, M. Steder, M. Sumihama, M. Sumisawa, K. Tamponi, U. Tanida, K. Teramoto, Y. Uchida, M. Uehara, S. Unno, Y. Uno, S. Urquijo, P. Usov, Y. Van Hulse, C. Vanhoefer, P. Varner, G. Vinokurova, A. Vorobyev, V. Wagner, M. N. Wang, C. H. Wang, M. -Z. Wang, P. Watanabe, Y. Williams, K. M. Won, E. Yamamoto, H. Yashchenko, S. Yook, Y. Zhang, Z. P. Zhilich, V. Zhulanov, V. Zupanc, A. CA Belle Collaboration TI Study of D** production and light hadronic states in the (B)over-bar(0) -> D*(+)omega pi(-) decay SO PHYSICAL REVIEW D LA English DT Article ID EXCITED CHARMED MESONS; HEAVY-QUARK SYMMETRY AB We report on the first observations of (B) over bar (0) -> D-1 (2430)(0)omega, (B) over bar (0) -> D-1 (2420)(0)omega, and (B) over bar (0) -> D-2* (2460)(0)omega decays. The (B) over bar (0) -> D*(+) rho(1450)(-) decay is also observed. The branching fraction measurements are based on (771.6 +/- 10.6) x 10(6) B (B) over bar events collected at the Upsilon(4S) resonance with the Belle detector at the KEKB asymmetric-energy e(+)e(-) collider. The fractions of longitudinal polarization of the D** states as well as partial wave fractions of the D-1 (2430)(0) are obtained. We also set a 90% confidence level upper limit for the product of branching fractions of B((B) over bar (0) -> D*(+)b(1) (1235)(-)) x B(b(1) (1235)(-) -> omega pi(-)). The measurements show evidence of nontrivial final-state interaction phases for the rho-meson-like amplitudes. C1 [Schnell, G.; Van Hulse, C.] Univ Basque Country UPV EHU, Bilbao 48080, Spain. [Shen, C. P.] Beihang Univ, Beijing 100191, Peoples R China. [Dingfelder, J.; Pesantez, L.] Univ Bonn, D-53115 Bonn, Germany. [Matvienko, D.; Kuzmin, A.; Eidelman, S.; Arinstein, K.; Aulchenko, V.; Bobrov, A.; Bondar, A.; Gabyshev, N.; Garmash, A.; Krokovny, P.; Shebalin, V.; Shwartz, B.; Usov, Y.; Vinokurova, A.; Vorobyev, V.; Zhilich, V.; Zhulanov, V.] Budker Inst Nucl Phys SB RAS, Novosibirsk 630090, Russia. [Cervenkov, D.; Dolezal, Z.; Drasal, Z.; Kodys, P.] Charles Univ Prague, Fac Math & Phys, CR-12116 Prague, Czech Republic. [Joo, K. K.] Chonnam Natl Univ, Kwangju 660701, South Korea. [Pal, B.] Univ Cincinnati, Cincinnati, OH 45221 USA. [Ferber, T.; Inguglia, G.; Rostomyan, A.; Steder, M.; Yashchenko, S.] DESY, D-22607 Hamburg, Germany. [Getzkow, D.; Lange, J. S.; Wagner, M. N.] Univ Giessen, D-35392 Giessen, Germany. [Sumihama, M.] Gifu Univ, Gifu 5011193, Japan. [Adachi, I.; Hara, T.; Itoh, R.; Nakao, M.; Nishida, S.; Sakai, Y.; Sumisawa, K.; Uehara, S.; Uno, S.] SOKENDAI Grad Univ Adv Studies, Hayama 2400193, Japan. [Choi, S. -K.] Gyeongsang Natl Univ, Chinju 660701, South Korea. [Cheon, B. G.; Goh, Y. M.; Kim, S. H.; Unno, Y.] Hanyang Univ, Seoul 133791, South Korea. [Browder, T. E.; Jaegle, I.; Varner, G.] Univ Hawaii, Honolulu, HI 96822 USA. [Adachi, I.; Hara, T.; Itoh, R.; Iwasaki, Y.; Liventsev, D.; Nakao, M.; Nishida, S.; Sakai, Y.; Santelj, L.; Sumisawa, K.; Uehara, S.; Uno, S.] High Energy Accelerator Res Org KEK, Tsukuba, Ibaraki 3050801, Japan. [Schnell, G.] Basque Fdn Sci, IKERBASQUE, Bilbao 48013, Spain. [Bahinipati, S.] Indian Inst Technol, Bhubaneswar 751007, Satya Nagar, India. [Bhuyan, B.] Indian Inst Technol, Gauhati 781039, Assam, India. [Libby, J.; Nayak, M.] Indian Inst Technol Madras, Madras 600036, Tamil Nadu, India. [Wang, P.] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Schwanda, C.] Inst High Energy Phys, A-1050 Vienna, Austria. [Shapkin, M.; Sokolov, A.] Inst High Energy Phys, Protvino 142281, Russia. [Mussa, R.; Tamponi, U.] INFN Sez Torino, I-10125 Turin, Italy. [Aushev, T.; Chilikin, K.; Chistov, R.; Drutskoy, A.; Mizuk, R.; Pakhlova, G.] Inst Theoret & Expt Phys, Moscow 117218, Russia. [Biswal, J.; Bracko, M.; Golob, B.; Korpar, S.; Nanut, T.; Pestotnik, R.; Petric, M.; Ribezl, E.; Staric, M.; Zupanc, A.] J Stefan Inst, Ljubljana 1000, Slovenia. [Watanabe, Y.] Kanagawa Univ, Yokohama, Kanagawa 2218686, Japan. [Goldenzweig, P.; Pulvermacher, C.] Karlsruhe Inst Technol, Inst Expt Kernphys, D-76131 Karlsruhe, Germany. [Joffe, D.] Kennesaw State Univ, Kennesaw, GA 30144 USA. [Badhrees, I.] King Abdulaziz City Sci & Technol, Riyadh 11442, Saudi Arabia. [Al Said, S.] King Abdulaziz Univ, Dept Phys, Fac Sci, Jeddah 21589, Saudi Arabia. [Cho, K.; Kim, J. H.; Kim, Y. J.] Korea Inst Sci & Technol Informat, Taejon 305806, South Korea. [Kim, J. B.; Kim, K. T.; Ko, B. R.; Lee, D. H.; Won, E.] Korea Univ, Seoul 136713, South Korea. [Kim, M. J.; Park, H.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Schneider, O.] Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland. [Golob, B.] Univ Ljubljana, Fac Math & Phys, Ljubljana 1000, Slovenia. [Pedlar, T. K.] Luther Coll, Decorah, IA 52101 USA. [Bracko, M.; Korpar, S.] Univ Maribor, SLO-2000 Maribor, Slovenia. [Chobanova, V.; Dalseno, J.; Li Gioi, L.; Moll, A.; Ritter, M.; Simon, F.; Vanhoefer, P.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Julius, T.; Sevior, M. E.; Urquijo, P.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Drutskoy, A.; Mizuk, R.] Moscow Engn Phys Inst, Moscow 115409, Russia. [Aushev, T.; Pakhlova, G.] Moscow Inst Phys & Technol, Dolgoprudnyi 141700, Moscow Region, Russia. [Iijima, T.; Seon, O.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648602, Japan. [Hayasaka, K.; Iijima, T.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648602, Japan. [Hayashii, H.; Miyabayashi, K.] Nara Womens Univ, Nara 6308506, Japan. [Chen, A.] Natl Cent Univ, Chungli 32054, Taiwan. [Wang, C. H.] Natl United Univ, Miaoli 36003, Taiwan. [Hou, W. -S.; Shiu, J. -G.; Wang, M. -Z.] Natl Taiwan Univ, Dept Phys, Taipei 10617, Taiwan. [Bozek, A.] H Niewodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. [Kawasaki, T.; Miyata, H.] Niigata Univ, Niigata 9502181, Japan. [Matvienko, D.; Kuzmin, A.; Eidelman, S.; Arinstein, K.; Aulchenko, V.; Bobrov, A.; Bondar, A.; Gabyshev, N.; Garmash, A.; Krokovny, P.; Shebalin, V.; Shwartz, B.; Usov, Y.; Vinokurova, A.; Vorobyev, V.; Zhilich, V.; Zhulanov, V.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Nakano, E.; Teramoto, Y.] Osaka City Univ, Osaka 5588585, Japan. [Asner, D. M.; Bansal, V.; Fast, J. E.; Fulsom, B. G.] Pacific NW Natl Lab, Richland, WA 99352 USA. [He, X. H.] Peking Univ, Beijing 100871, Peoples R China. [Kumar, R.] Punjab Agr Univ, Ludhiana 141004, Punjab, India. [Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Tanida, K.] Seoul Natl Univ, Seoul 151742, South Korea. [Kim, D. Y.] Soongsil Univ, Seoul 156743, South Korea. [Bhardwaj, V.] Univ S Carolina, Columbia, SC 29208 USA. [Choi, Y.; Park, C. W.] Sungkyunkwan Univ, Suwon 440746, South Korea. [Bakich, A. M.; Sibidanov, A.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdesselam, A.; Al Said, S.; Ayad, R.; Badhrees, I.] Univ Tabuk, Fac Sci, Dept Phys, Tabuk 71451, Saudi Arabia. [Babu, V.; Dutta, D.; Gaur, V.; Mohanty, G. B.; Nisar, N. K.; Sandilya, S.] Tata Inst Fundamental Res, Bombay 400005, Maharashtra, India. [Dalseno, J.; Moll, A.; Simon, F.] Tech Univ Munich, Excellence Cluster Universe, D-85748 Garching, Germany. [Ogawa, S.] Toho Univ, Funabashi, Chiba 2748510, Japan. [Ishikawa, A.; Sanuki, T.; Yamamoto, H.] Tohoku Univ, Sendai, Miyagi 9808578, Japan. [Aihara, H.; Epifanov, D.] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Shibata, T. -A.; Uchida, M.] Tokyo Inst Technol, Tokyo 1528550, Japan. [Tamponi, U.] Univ Turin, I-10124 Turin, Italy. [Liventsev, D.; Piilonen, L. E.; Williams, K. M.] Virginia Polytech Inst & State Univ, CNP, Blacksburg, VA 24061 USA. [Bonvicini, G.; Cinabro, D.; Farhat, H.; Gillard, R.] Wayne State Univ, Detroit, MI 48202 USA. [Senyo, K.] Yamagata Univ, Yamagata 9908560, Japan. [Sohn, Y. -S.; Yook, Y.] Yonsei Univ, Seoul 120749, South Korea. RP Matvienko, D (reprint author), Univ Basque Country UPV EHU, Bilbao 48080, Spain. RI Aihara, Hiroaki/F-3854-2010; Pakhlova, Galina/C-5378-2014; Mizuk, Roman/B-3751-2014; Krokovny, Pavel/G-4421-2016; Chilikin, Kirill/B-4402-2014; EPFL, Physics/O-6514-2016; Chistov, Ruslan/B-4893-2014; Drutskoy, Alexey/C-8833-2016; Cervenkov, Daniel/D-2884-2017 OI Aihara, Hiroaki/0000-0002-1907-5964; Pakhlova, Galina/0000-0001-7518-3022; Krokovny, Pavel/0000-0002-1236-4667; Chilikin, Kirill/0000-0001-7620-2053; Chistov, Ruslan/0000-0003-1439-8390; Drutskoy, Alexey/0000-0003-4524-0422; Cervenkov, Daniel/0000-0002-1865-741X FU Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan; Japan Society for the Promotion of Science (JSPS); Tau-Lepton Physics Research Center of Nagoya University; Australian Research Council; Australian Department of Industry, Innovation, Science and Research; Austrian Science Fund [P 22742-N16, P 26794-N20]; National Natural Science Foundation of China [10575109, 10775142, 10875115, 11175187, 11475187]; Ministry of Education, Youth and Sports of the Czech Republic [LG14034]; Carl Zeiss Foundation; Deutsche Forschungsgemeinschaft; VolkswagenStiftung; Department of Science and Technology of India; Istituto Nazionale di Fisica Nucleare of Italy; National Research Foundation (NRF) of Korea [2011-0029457, 2012-0008143, 2012R1A1A2008330, 2013R1A1A3007772]; Basic Research Lab program under NRF [KRF-2011-0020333, KRF-2011-0021196]; Center for Korean J-PARC Users [NRF-2013K1A3A7A06056592]; Brain Korea 21-Plus program; Global Science Experimental Data Hub Center of the Korea Institute of Science and Technology Information; Polish Ministry of Science and Higher Education; National Science Center; Ministry of Education and Science of the Russian Federation; Russian Foundation for Basic Research; Slovenian Research Agency; Basque Foundation for Science (IKERBASQUE); Euskal Herriko Unibertsitatea (UPV/EHU) (Spain) [UFI 11/55]; Swiss National Science Foundation; National Science Council; Ministry of Education of Taiwan; U.S. Department of Energy; National Science Foundation; MEXT for Science Research in a Priority Area ("New Development of Flavor Physics"); JSPS for Creative Scientific Research ("Evolution of Tau-lepton Physics") FX We thank the KEKB group for the excellent operation of the accelerator; the KEK cryogenics group for the efficient operation of the solenoid; and the KEK computer group, the National Institute of Informatics, and the PNNL/EMSL computing group for valuable computing and SINET4 network support. We acknowledge support from the Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan, the Japan Society for the Promotion of Science (JSPS), and the Tau-Lepton Physics Research Center of Nagoya University; the Australian Research Council and the Australian Department of Industry, Innovation, Science and Research; Austrian Science Fund under Grants No. P 22742-N16 and No. P 26794-N20; the National Natural Science Foundation of China under Contracts No. 10575109, No. 10775142, No. 10875115, No. 11175187, and No. 11475187; the Ministry of Education, Youth and Sports of the Czech Republic under Contract No. LG14034; the Carl Zeiss Foundation, the Deutsche Forschungsgemeinschaft and the VolkswagenStiftung; the Department of Science and Technology of India; the Istituto Nazionale di Fisica Nucleare of Italy; National Research Foundation (NRF) of Korea Grants No. 2011-0029457, No. 2012-0008143, No. 2012R1A1A2008330, No. 2013R1A1A3007772; the Basic Research Lab program under NRF Grant No. KRF-2011-0020333, No. KRF-2011-0021196, Center for Korean J-PARC Users, No. NRF-2013K1A3A7A06056592; the Brain Korea 21-Plus program and the Global Science Experimental Data Hub Center of the Korea Institute of Science and Technology Information; the Polish Ministry of Science and Higher Education and the National Science Center; the Ministry of Education and Science of the Russian Federation and the Russian Foundation for Basic Research; the Slovenian Research Agency; the Basque Foundation for Science (IKERBASQUE) and the Euskal Herriko Unibertsitatea (UPV/EHU) under program UFI 11/55 (Spain); the Swiss National Science Foundation; the National Science Council and the Ministry of Education of Taiwan; and the U.S. Department of Energy and the National Science Foundation. This work is supported by a Grant-inAid from MEXT for Science Research in a Priority Area ("New Development of Flavor Physics") and from JSPS for Creative Scientific Research ("Evolution of Tau-lepton Physics"). NR 63 TC 2 Z9 2 U1 2 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 23 PY 2015 VL 92 IS 1 AR 012013 DI 10.1103/PhysRevD.92.012013 PG 28 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CN4CO UT WOS:000358376900001 ER PT J AU Mourigal, M Wu, S Stone, MB Neilson, JR Caron, JM McQueen, TM Broholm, CL AF Mourigal, M. Wu, Shan Stone, M. B. Neilson, J. R. Caron, J. M. McQueen, T. M. Broholm, C. L. TI Block Magnetic Excitations in the Orbitally Selective Mott Insulator BaFe2Se3 SO PHYSICAL REVIEW LETTERS LA English DT Article ID EXCHANGE INTERACTIONS; SPIN-WAVES; SUPERCONDUCTORS AB Iron pnictides and selenides display a variety of unusual magnetic phases originating from the interplay between electronic, orbital, and lattice degrees of freedom. Using powder inelastic neutron scattering on the two-leg ladder BaFe2Se3, we fully characterize the static and dynamic spin correlations associated with the Fe-4 block state, an exotic magnetic ground state observed in this low-dimensional magnet and in Rb0.89Fe1.58Se2. All the magnetic excitations of the Fe-4 block state predicted by an effective Heisenberg model with localized spins are observed below 300 meV and quantitatively reproduced. However, the data only account for 16(3)mu(2)(B) per Fe2+, approximatively 2/3 of the total spectral weight expected for localized S = 2 moments. Our results highlight how orbital degrees of freedom in iron-based magnets can conspire to stabilize an exotic magnetic state. C1 [Mourigal, M.; Wu, Shan; Neilson, J. R.; Caron, J. M.; McQueen, T. M.; Broholm, C. L.] Johns Hopkins Univ, Inst Quantum Matter, Baltimore, MD 21218 USA. [Mourigal, M.; Wu, Shan; Neilson, J. R.; Caron, J. M.; McQueen, T. M.; Broholm, C. L.] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Stone, M. B.; Broholm, C. L.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Neilson, J. R.; Caron, J. M.; McQueen, T. M.] Johns Hopkins Univ, Dept Chem, Baltimore, MD 21218 USA. [McQueen, T. M.; Broholm, C. L.] Johns Hopkins Univ, Dept Mat Sci & Engn, Baltimore, MD 21218 USA. RP Mourigal, M (reprint author), Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. EM mourigal@gatech.edu RI Stone, Matthew/G-3275-2011; Mourigal, Martin/F-4495-2010; BL18, ARCS/A-3000-2012; OI Stone, Matthew/0000-0001-7884-9715; Mourigal, Martin/0000-0003-2772-8440; Neilson, James/0000-0001-9282-5752 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Material Sciences and Engineering [DE-FG02-08ER46544]; U.S. Department of Energy, Office of Basic Energy Sciences, Scientific User Facilities Division FX The work at IQM was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Material Sciences and Engineering, under Grant No. DE-FG02-08ER46544. This research at Oak Ridge National Laboratory's Spallation Neutron Source was sponsored by the U.S. Department of Energy, Office of Basic Energy Sciences, Scientific User Facilities Division. We are grateful to D. Abernathy for support on ARCS and to S. Toth for making SPINW freely available. NR 39 TC 3 Z9 3 U1 7 U2 44 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 23 PY 2015 VL 115 IS 4 AR 047401 DI 10.1103/PhysRevLett.115.047401 PG 5 WC Physics, Multidisciplinary SC Physics GA CN4AC UT WOS:000358369200005 PM 26252707 ER PT J AU Temple, RC Mihai, AP Arena, DA Marrows, CH AF Temple, Rowan C. Mihai, Andrei P. Arena, Dario A. Marrows, Christopher H. TI Ensemble magnetic behavior of interacting CoFe nanoparticles SO FRONTIERS IN PHYSICS LA English DT Article DE magnetic nanoparticle; XMCD; orbital moment; dipole interactions; superparamagnetism; long range order ID RAY CIRCULAR-DICHROISM; FE NANOCLUSTERS; CLUSTERS; MOMENTS; IRON; ANISOTROPY; SIZE; SPIN AB Ferromagnetic nanoparticles in the 10-14 nm size range are examined for their size and interaction dependent magnetic properties. From X-ray magnetic circular dichroism the orbital-to-spin magnetic moment ratio is determined and found to decrease significantly with particle size. This is in accordance with previous complementary studies on smaller particles and highlights the difficulty of fitting to a simple core-shell model. Vibrating sample magnetometry experiments on samples with more than 1000 particles per square micron show a wide distribution of blocking temperatures from 50 to greater than 650 K. This is attributed to the dipole-dipole magnetic coupling forces between particles. The blocking temperatures show an unexpected negative correlation with increasing particle density. C1 [Temple, Rowan C.; Mihai, Andrei P.; Marrows, Christopher H.] Univ Leeds, Sch Phys & Astron, EC Stoner Bldg, Leeds LS2 9JT, W Yorkshire, England. [Arena, Dario A.] Brookhaven Natl Lab, Natl Synchrotron Light Source, Photon Sci, Upton, NY 11973 USA. RP Temple, RC (reprint author), Univ Leeds, Sch Phys & Astron, EC Stoner Bldg, Leeds LS2 9JT, W Yorkshire, England. EM r.c.temple@leeds.ac.uk FU EPSRC; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX The authors acknowledge financial support from the EPSRC Doctoral Training Grant. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. The authors would like to thank Dr. Mike Ward for assistance with the transmission electron microsope experiments. NR 40 TC 0 Z9 0 U1 0 U2 0 PU FRONTIERS RESEARCH FOUNDATION PI LAUSANNE PA EPFL SCIENCE PARK, BLDG D, LAUSANNE, 1015, SWITZERLAND SN 2296-424X J9 FRONT PHYS JI Front. Physics PD JUL 23 PY 2015 VL 3 AR 52 DI 10.3389/fphy.2015.00052 PG 7 WC Physics, Multidisciplinary SC Physics GA EB3LF UT WOS:000387265500001 ER PT J AU Li, Y Liou, MK Schreiber, WM Gibson, BF AF Li, Yi Liou, M. K. Schreiber, W. M. Gibson, B. F. TI Neutrino-pair bremsstrahlung from nucleon-nucleon scattering SO PHYSICAL REVIEW C LA English DT Article ID PROTON-PROTON BREMSSTRAHLUNG; PION-PRODUCTION THRESHOLD; SOFT-PHOTON THEOREM; LOW-ENERGY THEOREM; N COUPLINGS; STARS; EMISSIVITIES; PSEUDOSCALAR; COLLISIONS; EMISSION AB Background: Neutrino-pair bremsstrahlung processes from nucleon-nucleon scattering NN nu(nu) over bar (nn nu(nu) over bar, pp nu(nu) over bar, and np nu(nu) over bar) have recently attracted attention in studies of neutrino emission in neutron stars, because of the implications for the neutron star cooling. The calculated NN nu(nu) over bar emissivities within the neutron star environment are relatively insensitive to the two-nucleon dynamical model used in the calculations, but differ significantly from those obtained using an one-pion-exchange (OPE) model. Purpose: We investigate the free NN nu(nu) over bar cross sections using a realistic nucleon-nucleon scattering amplitude, comparing the relative sizes of the cross sections for the three processes nn nu(nu) over bar, pp nu(nu) over bar, and np nu(nu) over bar. Method: We employ a realistic one-boson-exchange (ROBE) model for NN scattering and combine those strong scattering amplitudes with the well-known nucleon weak interaction vertices to construct weak bremsstrahlung amplitudes. Using the resulting NN nu(nu) over bar amplitudes we investigate the relative importance of the vector (Gamma(mu)(V)), axial vector (Gamma(mu)(A)), and tensor (Gamma(mu)(T)) terms. The ROBE model bremsstrahlung amplitudes are also used as a two-nucleon dynamical model with which we calculate the cross sections d sigma/d omega for nn nu(nu) over bar, pp nu(nu) over bar, and np nu(nu) over bar. Results: The three free NN nu(nu) over bar cross sections d sigma/d omega are of similar order of magnitude. Each increases with increasing neutrino-pair energy omega. For the neutrino-pair energy of omega = 1MeV our nn nu(nu) over bar results are in quantitative agreement with those previously reported by Timmermans et al. [Phys. Rev. C65, 064007 (2002)], who used the leading-order term of the soft-neutrino-pair bremsstrahlung amplitude to calculate the cross sections. Differences between the nn nu(nu) over bar and pp nu(nu) over bar cross section are not discernible over the nucleon-nucleon incident energy region considered, due to the complete dominance of the axial vector component of the weak interaction nucleon vertex function Gamma(mu) as demonstrated analytically in Appendix A. The np nu(nu) over bar cross section is smaller than either the nn nu(nu) over bar or the pp nu(nu) over bar cross section for low to moderate values of omega; this characteristic only changes at larger neutrino-pair energies around omega similar to 50 MeV, which is above the low energy region characterized in Appendix B. Conclusions: The free NN nu(nu) over bar cross sections, calculated using a realistic nucleon-nucleon amplitude model, are new except for the nn nu(nu) over bar cross section at omega = 1MeV that was first reported by Timmermans et al., and at. = 0.5,1,2 MeV by Li et al. [Phys. Rev. C 80, 035505 (2009)]. The nn nu(nu) over bar and pp nu(nu) over bar cross sections are virtually identical in magnitude. All three NN nu(nu) over bar processes are dominated by the axial vector component of the vertex function Gamma(mu), with only slight deviations from this behavior being seen in the np nu(nu) over bar process at large neutrino-pair energies. C1 [Li, Yi] Guangxi Univ, Coll Phys & Technol, Nanning 530004, Guangxi, Peoples R China. [Liou, M. K.] CUNY Brooklyn Coll, Dept Phys, Brooklyn, NY 11210 USA. [Liou, M. K.] CUNY Brooklyn Coll, Inst Nucl Theory, Brooklyn, NY 11210 USA. [Schreiber, W. M.] CUNY Coll Staten Isl, Dept Phys, Staten Isl, NY 10314 USA. [Gibson, B. F.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Li, Y (reprint author), Guangxi Univ, Coll Phys & Technol, Nanning 530004, Guangxi, Peoples R China. FU Guangxi University; National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DEAC52-06NA25396]; CUNY Professional Staff Congress - Board of Higher Education Research Award Program FX Numerical results in this paper were performed on the supercomputer of the CUNY High Performance Computing Center situated at the College of Staten Island. The work of Y. Li was supported by a grant from Guangxi University, the work of M. K. Liou and W. M. Schreiber was supported in part by the CUNY Professional Staff Congress - Board of Higher Education Research Award Program, and the work of B. F. Gibson was carried out under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DEAC52-06NA25396. NR 36 TC 0 Z9 0 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JUL 22 PY 2015 VL 92 IS 1 AR 015504 DI 10.1103/PhysRevC.92.015504 PG 12 WC Physics, Nuclear SC Physics GA DO6MZ UT WOS:000377898900001 ER PT J AU Roux, S Hallam, SJ Woyke, T Sullivan, MB AF Roux, Simon Hallam, Steven J. Woyke, Tanja Sullivan, Matthew B. TI Viral dark matter and virus-host interactions resolved from publicly available microbial genomes SO ELIFE LA English DT Article ID SINGLE-CELL; PHAGE EVOLUTION; DNA VIRUSES; P1 PLASMID; HUMAN GUT; DIVERSITY; BACTERIOPHAGES; SYNECHOCOCCUS; PROPHAGES; BACTERIA AB The ecological importance of viruses is now widely recognized, yet our limited knowledge of viral sequence space and virus-host interactions precludes accurate prediction of their roles and impacts. In this study, we mined publicly available bacterial and archaeal genomic data sets to identify 12,498 high-confidence viral genomes linked to their microbial hosts. These data augment public data sets 10-fold, provide first viral sequences for 13 new bacterial phyla including ecologically abundant phyla, and help taxonomically identify 7-38% of 'unknown' sequence space in viromes. Genome-and network-based classification was largely consistent with accepted viral taxonomy and suggested that (i) 264 new viral genera were identified (doubling known genera) and (ii) cross-taxon genomic recombination is limited. Further analyses provided empirical data on extrachromosomal prophages and coinfection prevalences, as well as evaluation of in silico virus-host linkage predictions. Together these findings illustrate the value of mining viral signal from microbial genomes. C1 [Roux, Simon; Sullivan, Matthew B.] Univ Arizona, Dept Ecol & Evolutionary Biol, Tucson, AZ USA. [Hallam, Steven J.] Univ British Columbia, Dept Microbiol & Immunol, Vancouver, BC V5Z 1M9, Canada. [Hallam, Steven J.] Univ British Columbia, Grad Program Bioinformat, Vancouver, BC V5Z 1M9, Canada. [Woyke, Tanja] US DOE, Joint Genome Inst, Walnut Creek, CA USA. RP Sullivan, MB (reprint author), Ohio State Univ, Dept Microbiol, Columbus, OH 43210 USA. EM mbsulli@gmail.com FU Gordon and Betty Moore Foundation [3790]; Natural Sciences and Engineering Research Council of Canada (Conseil de Recherches en Sciences Naturelles et en Genie du Canada); Canada Foundation for Innovation (Fondation canadienne pour l'innovation); Canadian Institute for Advanced Research (L'Institut Canadien de Recherches Avancees); Tula Foundation; Ambrose Monell Foundation; G. Unger Vetlesen Foundation; U.S. Department of Energy (Department of Energy) [DE-AC02-05CH11231] FX Gordon and Betty Moore Foundation 3790 Matthew B Sullivan; Natural Sciences and Engineering Research Council of Canada (Conseil de Recherches en Sciences Naturelles et en Genie du Canada) Steven J Hallam; Canada Foundation for Innovation (Fondation canadienne pour l'innovation) Steven J Hallam; Canadian Institute for Advanced Research (L'Institut Canadien de Recherches Avancees) Steven J Hallam; Tula Foundation Steven J Hallam; Ambrose Monell Foundation Steven J Hallam; G. Unger Vetlesen Foundation Steven J Hallam; U.S. Department of Energy (Department of Energy) Joint Genome Institute (DE-AC02-05CH11231) Tanja Woyke NR 83 TC 26 Z9 26 U1 9 U2 14 PU ELIFE SCIENCES PUBLICATIONS LTD PI CAMBRIDGE PA SHERATON HOUSE, CASTLE PARK, CAMBRIDGE, CB3 0AX, ENGLAND SN 2050-084X J9 ELIFE JI eLife PD JUL 22 PY 2015 VL 4 AR e08490 DI 10.7554/eLife.08490 PG 20 WC Biology SC Life Sciences & Biomedicine - Other Topics GA DJ0HB UT WOS:000373882000001 ER PT J AU Webb, MA Jung, Y Pesko, DM Savoie, BM Yamamoto, U Coates, GW Balsara, NP Wang, ZG Miller, TF AF Webb, Michael A. Jung, Yukyung Pesko, Danielle M. Savoie, Brett M. Yamamoto, Umi Coates, Geoffrey W. Balsara, Nitash P. Wang, Zhen-Gang Miller, Thomas F., III TI Systematic Computational and Experimental Investigation of Lithium-Ion Transport Mechanisms in Polyester-Based Polymer Electrolytes SO ACS CENTRAL SCIENCE LA English DT Article ID UNITED-ATOM DESCRIPTION; POLYPHOSPHAZENE SOLID ELECTROLYTES; AMORPHOUS POLY(ETHYLENE OXIDE); ETHYLENE-OXIDE; MOLECULAR-DYNAMICS; TRANSFERABLE POTENTIALS; PHASE-EQUILIBRIA; POLYETHYLENE/POLY(ETHYLENE OXIDE); COMPLEX-FORMATION; PROPYLENE-OXIDE AB Understanding the mechanisms of lithium-ion transport in polymers is crucial for the design of polymer electrolytes. We combine modular synthesis, electrochemical characterization, and molecular simulation to investigate lithium-ion transport in a new family of polyester-based polymers and in poly(ethylene oxide) (PEO). Theoretical predictions of glass-transition temperatures and ionic conductivities in the polymers agree well with experimental measurements. Interestingly, both the experiments and simulations indicate that the ionic conductivity of PEO, relative to the polyesters, is far higher than would be expected from its relative glass-transition temperature. The simulations reveal that diffusion of the lithium cations in the polyesters proceeds via a different mechanism than in PEO, and analysis of the distribution of available cation solvation sites in the various polymers provides a novel and intuitive way to explain the experimentally observed ionic conductivities. This work provides a platform for the evaluation and prediction of ionic conductivities in polymer electrolyte materials. C1 [Webb, Michael A.; Savoie, Brett M.; Yamamoto, Umi; Wang, Zhen-Gang; Miller, Thomas F., III] CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA. [Jung, Yukyung; Coates, Geoffrey W.] Cornell Univ, Dept Chem & Chem Biol, Baker Lab, Ithaca, NY 14853 USA. [Pesko, Danielle M.; Balsara, Nitash P.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Miller, TF (reprint author), CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA. EM tfm@caltech.edu NR 58 TC 12 Z9 12 U1 12 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2374-7943 EI 2374-7951 J9 ACS CENTRAL SCI JI ACS Central Sci. PD JUL 22 PY 2015 VL 1 IS 4 BP 198 EP 205 DI 10.1021/acscentsci.5b00195 PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA CX8QI UT WOS:000365968300009 PM 27162971 ER PT J AU Coh, S Cohen, ML Louie, SG AF Coh, Sinisa Cohen, Marvin L. Louie, Steven G. TI Large electron-phonon interactions from FeSe phonons in a monolayer SO NEW JOURNAL OF PHYSICS LA English DT Article DE superconductivity; FeSe; phonons structure; nematic; monolayer; SrTiO3; electron-phonon coupling ID SINGLE-LAYER FESE; HIGH-TEMPERATURE SUPERCONDUCTIVITY; LATTICE VIBRATIONS; DENSITY; ORIGIN; STATES; FILMS AB We show that electron-phonon coupling can induce strong electron pairing in an FeSe monolayer on a SrTiO3 substrate (experimental indications for superconducting T-c are between 65 and 109 K). The role of the SrTiO3 substrate in increasing the coupling is two-fold. First, the interaction of the FeSe and TiO2 terminated face of SrTiO3 prevents the FeSe monolayer from undergoing a shear-type (orthorhombic, nematic) structural phase transition. Second, the substrate allows an anti-ferromagnetic ground state of FeSe which opens electron-phonon coupling channels within the monolayer that are prevented by symmetry in the non-magnetic phase. The spectral function for the electron-phonon coupling (alpha F-2) in our calculations agrees well with inelastic tunneling data. C1 [Coh, Sinisa] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Coh, S (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM sinisa@civet.berkeley.edu FU Theory Program at the Lawrence Berkeley National Lab through the Office of Basic Energy Sciences, US Department of Energy [DE-AC02-05CH11231]; National Science Foundation [DMR10-1006184]; Office of Science of the US Department of Energy FX This research was supported by the Theory Program at the Lawrence Berkeley National Lab through the Office of Basic Energy Sciences, US Department of Energy under Contract No. DE-AC02-05CH11231 which provided for the electron-phonon calculation; and by the National Science Foundation under Grant No. DMR10-1006184 which provided for the structural and magnetic study. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy. NR 45 TC 26 Z9 26 U1 6 U2 59 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD JUL 22 PY 2015 VL 17 AR 073027 DI 10.1088/1367-2630/17/7/073027 PG 6 WC Physics, Multidisciplinary SC Physics GA CO4MD UT WOS:000359134000003 ER PT J AU Li, C Li, YH Xing, YJ Zhang, ZL Zhang, XF Li, Z Shi, YT Ma, TL Ma, RZ Wang, KL Wei, JQ AF Li, Can Li, Yahui Xing, Yujin Zhang, Zelin Zhang, Xianfeng Li, Zhen Shi, Yantao Ma, Tingli Ma, Renzhi Wang, Kunlin Wei, Jinquan TI Perovskite Solar Cell Using a Two-Dimensional Titania Nanosheet Thin Film as the Compact Layer SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE perovskite solar cell; titania nanosheet; compact layer; electrophoretic deposition ID ORGANOLEAD HALIDE PEROVSKITE; ELECTROPHORETIC DEPOSITION; HYSTERESIS; CH3NH3PBI3; INTERFACE; LENGTHS; OXIDE AB The compact layer plays an important role in conducting electrons and blocking holes in perovskite solar cells (PSCs). Here, we use a two-dimensional titania nanosheet (TNS) thin film as the compact layer in CH3NH3PbI3 PSCs. TNS thin films with thicknesses ranging from 8 to 75 nm were prepared by an electrophoretic deposition method from a dilute TNS/tetrabutylammonium hydroxide solution. The TNS thin films contact the fluorine-doped tin oxide grains perfectly. Our results show that a 8-nm-thick TNS film is sufficient for acting as the compact layer. Currently, the PSC with a TNS compact layer has a high efficiency of 10.7% and relatively low hysteresis behavior. C1 [Li, Can; Li, Yahui; Zhang, Zelin; Wang, Kunlin; Wei, Jinquan] Tsinghua Univ, State Key Lab New Ceram & Fine Proc, Key Lab Adv Mat Proc Technol, Educ Minist, Beijing 100084, Peoples R China. [Li, Can; Li, Yahui; Zhang, Zelin; Wang, Kunlin; Wei, Jinquan] Tsinghua Univ, Sch Mat Sci & Engn, Beijing 100084, Peoples R China. [Xing, Yujin; Shi, Yantao; Ma, Tingli] Dalian Univ Technol, Sch Chem, State Key Lab Fine Chem, Dalian 116024, Peoples R China. [Zhang, Xianfeng] Natl Ctr Nanosci & Technol, Beijing 100190, Peoples R China. [Li, Zhen] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Ma, Renzhi] Natl Inst Mat, Tsukuba, Ibaraki 3050044, Japan. RP Wei, JQ (reprint author), Tsinghua Univ, State Key Lab New Ceram & Fine Proc, Key Lab Adv Mat Proc Technol, Educ Minist, Beijing 100084, Peoples R China. EM jqwei@tsinghua.edu.cn RI Wei, Jinquan/D-8925-2014; Li, Zhen/E-9341-2015 OI Wei, Jinquan/0000-0002-5827-2231; Li, Zhen/0000-0003-1177-2818 FU National Natural Science Foundation of China [51172122]; Tsinghua University Initiative Scientific Research Program [20111080939]; Shenzhen Jiawei Photovoltaic Lighting Co., Ltd. FX This work is financially supported by the National Natural Science Foundation of China (Grant 51172122), Tsinghua University Initiative Scientific Research Program (Grant 20111080939), and Shenzhen Jiawei Photovoltaic Lighting Co., Ltd. NR 23 TC 2 Z9 2 U1 17 U2 125 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JUL 22 PY 2015 VL 7 IS 28 BP 15117 EP 15122 DI 10.1021/acsami.5b01959 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CN6QC UT WOS:000358558300001 PM 26158908 ER PT J AU Ilyas, A Lavrik, NV Kim, HKW Aswath, PB Varanasi, VG AF Ilyas, Azhar Lavrik, Nickolay V. Kim, Harry K. W. Aswath, Pranesh B. Varanasi, Venu G. TI Enhanced Interfacial Adhesion and Osteogenesis for Rapid "Bone-like" Biomineralization by PECVD-Based Silicon Oxynitride Overlays SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE PECVD; qPCR; lithography; periosteal cells; gene expression; hydroxyapatite ID CHEMICAL-VAPOR-DEPOSITION; BIOACTIVE GLASS COATINGS; MECHANICAL-PROPERTIES; IN-VITRO; TITANIUM-DIOXIDE; XANES ANALYSIS; CELL-CULTURES; LIVING CELLS; PLASMA; FILMS AB Structurally unstable fracture sites require metal fixative devices, which have long healing times due to their lack of osteoinductivity. Bioactive glass coatings lack in interfacial bonding, delaminate, and have reduced bioactivity due to the high temperatures used for their fabrication. Here, we test the hypothesis that low-temperature PECVD amorphous silica can enhance adhesion to the underlying metal surface and that N incorporation enhances osteogenesis and rapid biomineralization. A model Ti/TiO2 SiOx interface was formed by first depositing Ti onto Si wafers, followed by surface patterning, thermal annealing to form TiO2, and depositing SiOx/Si(ON)(x) overlays. TEM micrographs Showed conformal SiOx layers on Ti/TiO2 overlays while XPS data revealed the formation of an elemental Ti-O-Si interface. Nanoscratch testing verified strong SiOx bonding with the underlying TiO2 layers. In vitro studies showed that the surface properties changed significantly to reveal the formation of hydroxycarbonate apatite within 6 h, and Si(ON)(x) surface chemistry induced osteogenic gene expression of human periosteal cells and led to a rapid "bone-like" biomineral formation within 4 weeks. XANES data revealed that the incorporation of N increased the surface HA bioactivity by increasing the carbonate to phosphate ratio. In conclusion, silicon oxynitride overlays on bone-implant systems enhance osteogenesis and biomineralization via surface nitrogen incorporation. C1 [Ilyas, Azhar; Varanasi, Venu G.] Texas A&M Univ, Baylor Coll Dent, Dept Biomed Sci, Dallas, TX 75246 USA. [Lavrik, Nickolay V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Kim, Harry K. W.] Univ Texas SW Med Ctr Dallas, Dept Orthopaed Surg, Dallas, TX 75390 USA. [Kim, Harry K. W.] Texas Scottish Rite Hosp Children, Ctr Excellence Hip Disorders, Dallas, TX 75219 USA. [Aswath, Pranesh B.] Univ Texas Arlington, Dept Mat Sci & Engn, Arlington, TX 76019 USA. RP Varanasi, VG (reprint author), Texas A&M Univ, Baylor Coll Dent, Dept Biomed Sci, 3302 Gaston Ave, Dallas, TX 75246 USA. EM varanasi@bcd.tamhsc.edu RI Lavrik, Nickolay/B-5268-2011 OI Lavrik, Nickolay/0000-0002-9543-5634 FU National Institutes of Health [1R03DE023872-01A1]; CNMS Grant [2010-080]; [24444100005]; [304-128170] FX The authors would like to thank Megen F. Velten for her valuable contributions to in vitro studies and analysis, Harry Meyer and Karren More for their help with nanofabricated surface characterization, and Vibhu Sharma for his assistance with nanoscratch testing. We also acknowledge the staff at the Center for Nanophase Material Science at the Oak Ridge National Laboratory and the Nanotechnology Research Center, University of Texas at Arlington, for their help and guidance on device fabrication and characterization. XANES experiments were conducted at the Canadian Light Source, Saskatoon, Canada, which is supported by NSERC, NRC, CIHR, and the University of Saskatchewan. The work was supported by a grant from National Institutes of Health (1R03DE023872-01A1) to V.G.V. and partially supported by Enhancement Grant (#24444100005, V.G.V., PI), Departmental Startup (#304-128170, V.G.V., PI), and CNMS Grant (#2010-080, V.G.V., PI). NR 51 TC 4 Z9 4 U1 6 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JUL 22 PY 2015 VL 7 IS 28 BP 15368 EP 15379 DI 10.1021/acsami.5b03319 PG 12 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CN6QC UT WOS:000358558300030 PM 26095187 ER PT J AU Kauffman, DR Thakkar, J Siva, R Matranga, C Ohodnicki, PR Zeng, CJ Jin, RC AF Kauffman, Douglas R. Thakkar, Jay Siva, Rajan Matranga, Christopher Ohodnicki, Paul R. Zeng, Chenjie Jin, Rongchao TI Efficient Electrochemical CO2 Conversion Powered by Renewable Energy SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE electrocatalysis; CO2 conversion; gold nanomaterials; renewable energy; catalysis; environmental ID CARBON-DIOXIDE; ELECTROCATALYTIC REDUCTION; AU NANOPARTICLES; SOLAR-CELL; SELECTIVE CONVERSION; CRYSTAL-STRUCTURE; PROTECTED AU-25; CATALYSTS; METHANOL; ELECTROREDUCTION AB The catalytic Conversion of CO2 into industrially relevant chemicals is one strategy for mitigating greenhouse gas emissions. Along these lines, electrochemical CO2 conversion technologies are attractive because they can operate with :high I:reaction rates at ambient conditions. However, electrochemical systems require electricity, and CO2 conversion processes must integrate with carbon-free, renewable-energy sources to be viable on larger scales. We utilize Au-25 nanoclusters as renewably powered CO2 conversion electrocatalysts with CO2 -> CO reaction rates between 400 and, 800 L of CO2 per gram of catalytic metal per hour and product selectivities between 80 and 95%. These performance metrics correspond to to conversion rates approaching 0.8-1.6 kg Of CO2 per gram of catalytic metal per hour. We also present data showing CO2 conversion rates and product selectivity strongly depend on catalyst loading. Optimized systems demonstrate stable operation and reaction turnover numbers (TONs) approaching 6 X 10(6) mol(CO2) mol(catalyst)(-1) during a multiday (36 h total hours) CO2 electrolysis experiment containing multiple start/stop cycles. TONs between 1 X 10(6) and 4 X 10(6) mol(CO2) mol(catalyst)(-1) were obtained when our system was powered by consumer-grade renewable-energy sources. Daytime. photovoltaic-powered CO2 conversion was demonstrated for 12 h and we mimicked low-light or nighttime operation for 24 h with a solar-rechargeable battery. This proof-of-principle study provides some of the initial performance data necessary for assessing the scalability and technical viability of electrochemical CO2 conversion technologies. Specifically, we show the following: (1) all electrochemical CO2 conversion systems will produce a net increase in CO2 emissions if they do not integrate with renewable-energy sources, (2) catalyst loading vs activity trends can be used to tune process rates and product distributions, and (3) state-of-the-art renewable-energy technologies are sufficient to power larger-scale, tonne per day CO2 conversion systems. C1 [Kauffman, Douglas R.; Thakkar, Jay; Siva, Rajan; Matranga, Christopher; Ohodnicki, Paul R.] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. [Zeng, Chenjie; Jin, Rongchao] Carnegie Mellon Univ, Dept Chem, Pittsburgh, PA 15213 USA. RP Kauffman, DR (reprint author), US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. EM Douglas.Kauffman@NETL.DOE.GOV FU AFOSR; agency of the United States Government FX R.J. acknowledges research support from AFOSR. This report was prepared as an account of work sponsored by an agency of the United States Government. Neither the United States Government nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. NR 55 TC 10 Z9 10 U1 19 U2 152 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JUL 22 PY 2015 VL 7 IS 28 BP 15626 EP 15632 DI 10.1021/acsami.5b04393 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CN6QC UT WOS:000358558300059 PM 26121278 ER PT J AU Jiang, JC Yaghi, OM AF Jiang, Juncong Yaghi, Omar M. TI Bronsted Acidity in Metal-Organic Frameworks SO CHEMICAL REVIEWS LA English DT Review ID TEMPERATURE-PROGRAMMED DESORPTION; HIGH PROTON CONDUCTIVITY; STATE NMR-SPECTROSCOPY; ONE-POT SYNTHESIS; SOLID-STATE; CATALYTIC-PROPERTIES; ALPHA-PINENE; PHOSPHOTUNGSTIC ACID; COORDINATION POLYMER; FUNCTIONAL-GROUPS C1 [Jiang, Juncong; Yaghi, Omar M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Chem, Div Mat Sci, Berkeley, CA 94720 USA. [Jiang, Juncong; Yaghi, Omar M.] Kavli Energy NanoSci Inst Berkeley, Berkeley, CA 94720 USA. [Yaghi, Omar M.] King Fahd Univ Petr & Minerals, Dhahran 34464, Saudi Arabia. RP Jiang, JC (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Chem, Div Mat Sci, Berkeley, CA 94720 USA. EM jcjiang@berkeley.edu; yaghi@berkeley.edu OI Yaghi, Omar/0000-0002-5611-3325 FU BASF SE (Ludwigshafen, Germany); U.S. Department of Defense, Defense Threat Reduction Agency Grant [HDTRA 1-12-1-0053]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Energy Frontier Research Center [DE-SC0001015] FX We gratefully acknowledge Prof. Y.-B. Zhang (ShanghaiTech University), Dr. H. Furukawa, and Mr. C. Diercks for their valuable input and proof-reading. Financial support for MOF research in the laboratories of O.M.Y. is provided by BASF SE (Ludwigshafen, Germany); U.S. Department of Defense, Defense Threat Reduction Agency Grant HDTRA 1-12-1-0053; and U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Energy Frontier Research Center grant DE-SC0001015. NR 251 TC 81 Z9 81 U1 55 U2 294 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0009-2665 EI 1520-6890 J9 CHEM REV JI Chem. Rev. PD JUL 22 PY 2015 VL 115 IS 14 BP 6966 EP 6997 DI 10.1021/acs.chemrev.5b00221 PG 32 WC Chemistry, Multidisciplinary SC Chemistry GA CN6PF UT WOS:000358556000006 PM 26088535 ER PT J AU Nafisi, M Stranne, M Fimognari, L Atwell, S Martens, HJ Pedas, PR Hansen, SF Nawrath, C Scheller, HV Kliebenstein, DJ Sakuragi, Y AF Nafisi, Majse Stranne, Maria Fimognari, Lorenzo Atwell, Susanna Martens, Helle J. Pedas, Pai R. Hansen, Sara F. Nawrath, Christiane Scheller, Henrik V. Kliebenstein, Daniel J. Sakuragi, Yumiko TI Acetylation of cell wall is required for structural integrity of the leaf surface and exerts a global impact on plant stress responses SO FRONTIERS IN PLANT SCIENCE LA English DT Article DE cell wall acetylation; trichomes; cuticles; epidermis; Bobytis cinerea; peroxidase; mRNA sequencing ID BOTRYTIS-CINEREA; O-ACETYLATION; ARABIDOPSIS-THALIANA; DISEASE RESISTANCE; DUF231 DOMAIN; CUTICLE; XYLOGLUCAN; XYLAN; PROTEINS; DEFENSE AB The epidermis on leaves protects plants from pathogen invasion and provides a waterproof barrier. It consists of a layer of cells that is surrounded by thick cell walls, which are partially impregnated by highly hydrophobic cuticular components. We show that the Arabidopsis T-DNA insertion mutants of REDUCED WALL ACE7YLATION 2 (rwa2), previously identified as having reduced O-acetylation of both pectins and hemicelluloses, exhibit pleiotrophic phenotype on the leaf surface. The cuticle layer appeared diffused and was significantly thicker and underneath cell wall layer was interspersed with electron-dense deposits. A large number of trichomes were collapsed and surface permeability of the leaves was enhanced in rwa2 as compared to the wild type. A massive reprogramming of the transcriptome was observed in rwa2 as compared to the wild type, including a coordinated up-regulation of genes involved in responses to abiotic stress, particularly detoxification of reactive oxygen species and defense against microbial pathogens (e.g., lipid transfer proteins, peroxidases). In accordance, peroxidase activities were found to be elevated in rwa2 as compared to the wild type. These results indicate that cell wall acetylation is essential for maintaining the structural integrity of leaf epidermis, and that reduction of cell wall acetylation leads to global stress responses in Arabidopsis. C1 [Nafisi, Majse; Stranne, Maria; Fimognari, Lorenzo; Hansen, Sara F.; Sakuragi, Yumiko] Copenhagen Plant Sci Ctr, Frederiksberg, Denmark. [Nafisi, Majse; Stranne, Maria; Fimognari, Lorenzo; Martens, Helle J.; Pedas, Pai R.; Hansen, Sara F.; Sakuragi, Yumiko] Univ Copenhagen, Dept Plant & Environm Sci, DK-1871 Frederiksberg, Denmark. [Atwell, Susanna; Kliebenstein, Daniel J.] Univ Calif Davis, Dept Plant Sci, Davis, CA 95616 USA. [Nawrath, Christiane] Univ Lausanne, Dept Plant Mol Biol, Lausanne, Switzerland. [Scheller, Henrik V.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Scheller, Henrik V.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Kliebenstein, Daniel J.] Danish Natl Res Fdn Ctr DynaMO, Frederiksberg, Denmark. RP Sakuragi, Y (reprint author), Univ Copenhagen, Dept Plant & Environm Sci, Fac Sci, Copenhagen Plant Sci Ctr, Thorvaldsensvej 40, DK-1871 Frederiksberg, Denmark. EM ysa@plen.ku.dk RI Atwell, Susanna/H-8630-2016; Scheller, Henrik/A-8106-2008; Pedas, Pai/G-3494-2014; OI Atwell, Susanna/0000-0001-8680-9721; Scheller, Henrik/0000-0002-6702-3560; Pedas, Pai/0000-0001-6733-7300; Sakuragi, Yumiko/0000-0002-9405-5197 FU Danish Advanced Technology Foundation [12-131834]; EU [317184]; Villum Foundation [VKR023371]; U.S. National Science foundation [1339125, 1021861]; USDA National Institute of Food and Agriculture [CA-D-PLS-7033-H]; Danish National Research Foundation [DNRF99]; U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE AC02-05CH11231] FX We acknowledge the Center for Advanced Bioimaging (CAB), Faculty of Science, University of Copenhagen for microscopy facilities and Catherine Skrzynski Nielsen and Piotr Binczycki for skilled preparation of the material for TEM. This work was supported by the Danish Advanced Technology Foundation [Biomass for the 21st century, grant number 001-2011-4]; the Danish Council for Strategic Research [Plant Power, grant number 12-131834]; EU FP7 People Programme Marie Curie Actions [PHOTO.COMM, grant number 317184]; The Villum Foundation [grant number VKR023371]; the U.S. National Science foundation [IOS grant numbers 1339125 and 1021861]; the USDA National Institute of Food and Agriculture [Hatch project number CA-D-PLS-7033-H]; the Danish National Research Foundation [DNRF99]; and the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [contract no.DE AC02-05CH11231]. NR 77 TC 0 Z9 0 U1 6 U2 18 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. PD JUL 22 PY 2015 VL 6 DI 10.3389/fpls.2015.00550 PG 13 WC Plant Sciences SC Plant Sciences GA CN8IP UT WOS:000358684000001 ER PT J AU Cloke, RR Marangoni, T Nguyen, GD Joshi, T Rizzo, DJ Bronner, C Cao, T Louie, SG Crommie, MF Fischer, FR AF Cloke, Ryan R. Marangoni, Tomas Nguyen, Giang D. Joshi, Trinity Rizzo, Daniel J. Bronner, Christopher Cao, Ting Louie, Steven. G. Crommie, Michael F. Fischer, Felix R. TI Site-Specific Substitutional Boron Doping of Semiconducting Armchair Graphene Nanoribbons SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID STRUCTURAL-CHARACTERIZATION; EDGE STATES; BAND-GAP; HETEROJUNCTIONS AB A fundamental requirement for the development of advanced electronic device architectures based on graphene nanoribbon (GNR) technology is the ability to modulate the band structure and charge carrier concentration by substituting specific carbon atoms in the hexagonal graphene lattice with p- or n-type dopant heteroatoms. Here we report the atomically precise introduction of group III dopant atoms into bottom-up fabricated semiconducting armchair GNRs (AGNRs). Trigonal-planar B atoms along the backbone of the GNR share an empty p-orbital with the extended pi-band for dopant functionality. Scanning tunneling microscopy (STM) topography reveals a characteristic modulation of the local density of states along the backbone of the GNR that is superimposable with the expected position and concentration of dopant B atoms. First-principles calculations support the experimental findings and provide additional insight into the band structure of B-doped 7-AGNRs. C1 [Cloke, Ryan R.; Marangoni, Tomas; Fischer, Felix R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Nguyen, Giang D.; Joshi, Trinity; Rizzo, Daniel J.; Bronner, Christopher; Cao, Ting; Louie, Steven. G.; Crommie, Michael F.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Louie, Steven. G.; Crommie, Michael F.; Fischer, Felix R.] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Crommie, Michael F.; Fischer, Felix R.] Univ Calif Berkeley, Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. [Crommie, Michael F.; Fischer, Felix R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Crommie, MF (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM crommie@berkeley.edu; ffischer@berkeley.edu RI Nguyen, Giang/R-1287-2016 OI Nguyen, Giang/0000-0003-4125-8203 FU U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES) [DE-SC0010409, DE-AC02-05CH11231]; Office of Naval Research BRC Program; National Science Foundation (NSF) [DMR-1206512, DMR10-1006184]; NIH [SRR023679A, S10-RR027172]; NSF Graduate Research Fellowship Program [DGE 1106400]; German National Academy of Sciences Leopoldina [LPDS 2014-09] FX Research supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), under award no. DE-SC0010409 (design, synthesis, and characterization of molecular building blocks) and Nanomachine Program award no. DE-AC02-05CH11231 (surface reaction characterization and STS image simulations), by the Office of Naval Research BRC Program (GNR characterization), by the National Science Foundation (NSF) award no. DMR-1206512 (image analysis), and DMR10-1006184 (basic theory and formalism). Berkeley NMR Facility is supported in part by NIH grant SRR023679A. X-ray Facility is supported in part by NIH Shared Instrumentation grant S10-RR027172, computational resources were provided by the NSF through XSEDE resources at the Texas Advanced Computing Center (TACC) at the University of Texas at Austin and NERSC at the Lawrence Berkeley National Laboratory. T.J. acknowledges support from NSF Graduate Research Fellowship Program under grant no. DGE 1106400. C.B. acknowledges support through the Fellowship Program of the German National Academy of Sciences Leopoldina under grant no. LPDS 2014-09. The authors acknowledge Dr. Antonio DiPasquale for assistance with X-ray analysis and Won-Woo Choi, Hsin-Zon Tsai, Arash A. Omrani, and Han Sae Jung for their technical assistance. NR 29 TC 28 Z9 28 U1 18 U2 89 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUL 22 PY 2015 VL 137 IS 28 BP 8872 EP 8875 DI 10.1021/jacs.5b02523 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA CN6PH UT WOS:000358556200002 PM 26153349 ER PT J AU Sanders, SN Kumarasamy, E Pun, AB Trinh, MT Choi, B Xia, JL Taffet, EJ Low, JZ Miller, JR Roy, X Zhu, XY Steigerwald, ML Sfeir, MY Campos, LM AF Sanders, Samuel N. Kumarasamy, Elango Pun, Andrew B. Trinh, M. Tuan Choi, Bonnie Xia, Jianlong Taffet, Elliot J. Low, Jonathan Z. Miller, John R. Roy, Xavier Zhu, X. -Y. Steigerwald, Michael L. Sfeir, Matthew Y. Campos, Luis M. TI Quantitative Intramolecular Singlet Fission in Bipentacenes SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID TRANSFER TICT STATES; EXCITON-FISSION; CRYSTALLINE TETRACENE; SOLAR-CELLS; PENTACENE; PHOTOVOLTAICS; FLUORESCENCE; EFFICIENCY; NANOPARTICLES; CONVERSION AB Singlet fission (SF) has the potential to significantly enhance the photocurrent in single-junction solar cells and thus raise the power conversion efficiency from the Shockley-Queisser limit of 33% to 44%. Until now, quantitative SF yield at room temperature has been observed only in crystalline solids or aggregates of oligoacenes. Here, we employ transient absorption spectroscopy, ultrafast photoluminescence spectroscopy, and triplet photosensitization to demonstrate intramolecular singlet fission (iSF) with triplet yields approaching 200% per absorbed photon in a series of bipentacenes. Crucially, in dilute solution of these systems, SF does not depend on intermolecular interactions. Instead, SF is an intrinsic property of the molecules, with both the fission rate and resulting triplet lifetime determined by the degree of electronic coupling between covalently linked pentacene molecules. We found that the triplet pair lifetime can be as short as 0.5 ns but can be extended up to 270 ns. C1 [Sanders, Samuel N.; Kumarasamy, Elango; Pun, Andrew B.; Trinh, M. Tuan; Choi, Bonnie; Xia, Jianlong; Taffet, Elliot J.; Low, Jonathan Z.; Roy, Xavier; Zhu, X. -Y.; Steigerwald, Michael L.; Campos, Luis M.] Columbia Univ, Dept Chem, New York, NY 10027 USA. [Miller, John R.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Sfeir, Matthew Y.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Steigerwald, ML (reprint author), Columbia Univ, Dept Chem, New York, NY 10027 USA. EM mls2064@columbia.edu; msfeir@bnl.gov; lcampos@columbia.edu RI Xia, Jianlong/I-9076-2012; OI Sfeir, Matthew/0000-0001-5619-5722; Sanders, Samuel/0000-0003-2702-8305; Pun, Andrew/0000-0002-3052-912X; Kumarasamy, Elango/0000-0002-7995-6894 FU NSF [DMR-1351293, DGE 11-44155, 1321405]; ACS Petroleum Research Fund; 3M Non-Tenured Faculty Award; Cottrell Scholar Award; A*STAR; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]; Air Force Office of Scientific Research [FA9550-14-1-0381] FX This work was funded by the NSF Career Award (DMR-1351293), ACS Petroleum Research Fund, 3M Non-Tenured Faculty Award, and Cottrell Scholar Award. S.N.S., A.B.P., and B.C. thank the NSF for GRFP (DGE 11-44155). X.Y.Z. acknowledges support by the NSF, Grant 1321405. J.Z.L. thanks A*STAR for funding. Research was carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, and in the Chemistry Department, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract DE-AC02-98CH10886, which also supports the LEAF Facility of the BNL Accelerator Center for Energy Research. SCXRD was performed in the Shared Materials Characterization Laboratory at Columbia University. X.R. thanks the Air Force Office of Scientific Research for support (AFOSR Award No. FA9550-14-1-0381). We are grateful to the Nuckolls lab for use of their computing cluster and UV-vis spectrophotometer. NR 42 TC 35 Z9 35 U1 19 U2 100 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUL 22 PY 2015 VL 137 IS 28 BP 8965 EP 8972 DI 10.1021/jacs.5b04986 PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA CN6PH UT WOS:000358556200022 PM 26102432 ER PT J AU Gilbert-Wilson, R Siebel, JF Adamska-Venkatesh, A Pham, CC Reijerse, E Wang, HX Cramer, SP Lubitz, W Rauchfuss, TB AF Gilbert-Wilson, Ryan Siebel, Judith F. Adamska-Venkatesh, Agnieszka Pham, Cindy C. Reijerse, Edward Wang, Hongxin Cramer, Stephen P. Lubitz, Wolfgang Rauchfuss, Thomas B. TI Spectroscopic Investigations of [FeFe] Hydrogenase Maturated with [Fe-57(2)(adt)(CN)(2)(CO)(4)](2-) SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID IRON-ONLY HYDROGENASE; RESONANCE VIBRATIONAL SPECTROSCOPY; ALGA CHLAMYDOMONAS-REINHARDTII; H-CLUSTER; ACTIVE-SITE; DESULFOVIBRIO-DESULFURICANS; CLOSTRIDIUM-PASTEURIANUM; ELECTRONIC-STRUCTURE; SULFUR CLUSTERS; ACTIVATION AB The preparation and spectroscopic characterization of a CO-inhibited [FeFe] hydrogenase with a selectively Fe-57-labeled binuclear subsite is described. The precursor [Fe-57(2)(adt)(CN)(2)(CO)(4)](2-) was synthesized from the Fe-57 metal, S-8, CO, (NEt4)CN, NH4Cl, and CH2O. (Et4N)(2)[Fe-57(2)(adt)(CN)(2)(CO)(4)] was then used for the maturation of the [FeFe] hydrogenase HydA1 from Chlamydomonas reinhardtii, to yield the enzyme selectively labeled at the [2Fe](H) subcluster. Complementary Fe-57 enrichment of the [4Fe-4S](H) cluster was realized by reconstitution with (FeCl3)-Fe-57 and Na2S. The H-ox-CO state of [2(57)Fe](H) and [4(57)Fe-4S](H) HydAl was characterized by Mossbauer, HYSCORE, ENDOR, and nuclear resonance vibrational spectroscopy. C1 [Gilbert-Wilson, Ryan; Rauchfuss, Thomas B.] Univ Illinois, Sch Chem Sci, Urbana, IL 61801 USA. [Siebel, Judith F.; Adamska-Venkatesh, Agnieszka; Reijerse, Edward; Lubitz, Wolfgang] Max Planck Inst Chem Energiekonvers, D-45470 Mulheim, Germany. [Pham, Cindy C.; Wang, Hongxin; Cramer, Stephen P.] Univ Calif Davis, Dept Chem, Davis, CA 95616 USA. [Wang, Hongxin; Cramer, Stephen P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Cramer, SP (reprint author), Univ Calif Davis, Dept Chem, Davis, CA 95616 USA. EM spjcramer@ucdavis.edu; wolfgang.lubitz@cec.mpg.de; rauchfuz@illinois.edu FU National Institutes of Health [GM061153, GM-65440]; Max-Planck Society; Deutsche Forschungsgemeinschaft [LU315/17-1]; US Department of Education [CFDA-84.200A] FX We thank Annika Gurowski and Agnes Stoer for their excellent technical assistance, Eckhard Bill and Bernd Mienert for their help with the Mossbauer spectroscopy, and Lars Lauterbach, Leland Gee, Yoshitaka Yoda and Kenji Tamasaku for their expertise in NRVS. This project was supported by the National Institutes of Health (GM061153, GM-65440), the Max-Planck Society, the Deutsche Forschungsgemeinschaft (DIP project LU315/17-1), and US Department of Education (CFDA-84.200A). The NRVS experiments were performed at SPRINGS BL09XU (JASRI proposed no.2014B1032) and BL19LXU (RIKEN proposal no 20140033). NR 55 TC 9 Z9 9 U1 7 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUL 22 PY 2015 VL 137 IS 28 BP 8998 EP 9005 DI 10.1021/jacs.5b03270 PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA CN6PH UT WOS:000358556200026 PM 26091969 ER PT J AU Campecino, JO Dudycz, LW Tumelty, D Berg, V Cabelli, DE Maroney, MJ AF Campecino, Julius O. Dudycz, Lech W. Tumelty, David Berg, Volker Cabelli, Diane E. Maroney, Michael J. TI A Semisynthetic Strategy Leads to Alteration of the Backbone Amidate Ligand in the NiSOD Active Site SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID NICKEL SUPEROXIDE-DISMUTASE; NATIVE CHEMICAL LIGATION; DESIGNED METALLOPROTEIN; OXIDATIVE CLEAVAGE; NITRILE HYDRATASE; PROTEIN; COMPLEXES; SULFUR; MECHANISM; DNA AB Computational investigations have implicated the amidate ligand in nickel, superoxide dismutase (NiSOD) in stabilizing Ni-centered redox catalysis and in preventing cysteine thiolate ligand oxidation. To test these predictions, we have used an experimental approach utilizing a semisynthetic scheme that employs native chemical ligation of a pentapeptide (HCDLP) to recombinant S. coelicolor NiSOD lacking these N-terminal residues, N Delta 5-NiSOD. Wild-type enzyme produced in this manner exhibits the characteristic spectral properties of recombinant WT-NiSOD and is as catalytically active. The semisynthetic scheme was also employed to construct a variant where, the amidate ligand was converted to a secondary amine, H1*-NiSOD, a novel strategy that retains a backbone N-donor atom. The H1*-NiSOD variant was found to have only similar to 1% of the catalytic activity of the recombinant wild-type enzyme, and had altered Spectroscopic properties. X-ray absorption spectroscopy reveals a four-coordinate planar site with N2S2-donor ligands, consistent with electronic absorption spectroscopic results indicating that the Ni center in H1*-NiSOD is mostly reduced in the as-isolated sample, as opposed to 50:50 Ni(II)/Ni(III) mixture that is typical for the recombinant wild-type enzyme. The EPR spectrum of as-isolated H1*-NiSOD accounts for similar to 11% of the Ni in the sample and is similar to WT-NiSOD, but more axial, with g(z) < g(x,y). N-14-hyperfine is observed on gz, confirming the addition of the apical histidine ligand in the Ni(III) complex. The altered electronic properties and implications for redox catalysis are discussed in light of prediction based on synthetic and computational models. C1 [Campecino, Julius O.; Berg, Volker; Maroney, Michael J.] Univ Massachusetts, Dept Chem, Amherst, MA 01003 USA. [Dudycz, Lech W.] Lex Co Res Lab, Shirley, MA 01464 USA. [Tumelty, David] New England Peptide, Gardner, MA 01440 USA. [Cabelli, Diane E.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Maroney, MJ (reprint author), Univ Massachusetts, Dept Chem, Amherst, MA 01003 USA. EM mmaroney@chem.umass.edu FU National Science Foundation [CHE-0809188]; Department of Energy, Office of Biological and Environmental Research; National Institutes of Health; US DOE Office of Science, Division of Chemical Sciences, Geosciences and Biosciences [DE-AC02-98CH10886] FX This work was supported by a grant from the National Science Foundation (CHE-0809188 to M.J.M.). Portions of this research were carried out at the Stanford Synchrotron Radiation Laboratory, a national user facility operated by Stanford University on behalf of the U.S. Department of Energy, Office of Basic Energy Sciences. The SSRL Structural Molecular Biology Program is supported by the Department of Energy, Office of Biological and Environmental Research, and by the National Institutes of Health. The kinetic studies conducted at Brookhaven National Laboratory were carried out at the Accelerator Center for Energy Research, which is supported by the US DOE Office of Science, Division of Chemical Sciences, Geosciences and Biosciences under Contract No. DE-AC02-98CH10886. We gratefully acknowledge the gift of Fmoc-S-o-nitrobenzyl cysteine from Dr. James J. Chambers and the design of the pelB WT-NiSOD plasmid by Carolyn Carr. The authors also acknowledge helpful discussions regarding NCL with Dr. Philip Dawson, and thank Dr. Michael Hendrich for providing his SpinCount EPR simulation software. NR 55 TC 2 Z9 2 U1 4 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUL 22 PY 2015 VL 137 IS 28 BP 9044 EP 9052 DI 10.1021/jacs.5b03629 PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA CN6PH UT WOS:000358556200031 PM 26135142 ER PT J AU Hrovat, DA Hou, GL Wang, XB Borden, WT AF Hrovat, David A. Hou, Gao-Lei Wang, Xue-Bin Borden, Weston Thatcher TI Negative Ion Photoelectron Spectroscopy Confirms the Prediction that 1,2,4,5-Tetraoxatetramethylenebenzene Has a Singlet Ground State SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID AB-INITIO CALCULATIONS; ELECTRON-AFFINITIES; BASIS-SETS; 1,2,4,5-TETRAMETHYLENEBENZENE; DIRADICALS; SPECTRUM; TRIPLET; TRIMETHYLENEMETHANE; MOLECULES; CHEMISTRY AB The negative ion photoelectron (NIPE) spectrum of 1,2,4,5-tetraoxatetramethylenebenzene radical anion (TOTMB center dot-) shows that, like the hydrocarbon, 1,2,4,5-tetramethylenebenzene (TMB), the TOTMB diradical has a singlet ground state and thus Violates Hund's rule. The NIPE spectrum of TOTMB center dot- gives a value of -Delta E-ST = 3.5 +/- 0.2 kcal/mol for the energy difference between the singlet and triplet states of TOTMB and a value of EA = 4.025 +/- 0.010 eV for the electron affinity of TOTMB. (10/10)CASPT2 calculations are successful in predicting the singlet-triplet energy difference in TOTMB almost exactly, giving a computed value of -Delta E-ST = 3.6 kcal/mol. The same type of calculations predict -Delta E-ST, = 6.1-6.3 kcal/mol in TMB. Thus, the calculated effect of the substitution of the four oxygens in TOTMB for the four methylene groups in TMB is very unusual, since the singlet state is selectively destabilized relative to the triplet state. The reason why TMB -> TOTMB is predicted to result in a decrease in the Size of -Delta E-ST is discussed. C1 [Hrovat, David A.; Borden, Weston Thatcher] Univ N Texas, Dept Chem, Denton, TX 76203 USA. [Hrovat, David A.; Borden, Weston Thatcher] Univ N Texas, Ctr Adv Sci Comp & Modeling, Denton, TX 76203 USA. [Hou, Gao-Lei; Wang, Xue-Bin] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP Wang, XB (reprint author), Pacific NW Natl Lab, Div Phys Sci, POB 999,MS K8-88, Richland, WA 99352 USA. EM xuebin.wang@pnnl.gov; borden@unt.edu FU National Science Foundation [CHE-0910527]; Robert A. Welch Foundation [B0027]; U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences; DOE's Office of Biological and Environmental Research FX The calculations at UNT were supported in part by Grant CHE-0910527 from the National Science Foundation and by Grant B0027 from the Robert A. Welch Foundation. The NIPES research at PNNL was supported by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences, and was performed at the EMSL, a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. NR 45 TC 5 Z9 5 U1 3 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUL 22 PY 2015 VL 137 IS 28 BP 9094 EP 9099 DI 10.1021/jacs.5b04416 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA CN6PH UT WOS:000358556200036 PM 26172391 ER PT J AU Dahlman, CJ Tan, YZ Marcus, MA Milliron, DJ AF Dahlman, Clayton J. Tan, Yizheng Marcus, Matthew A. Milliron, Delia J. TI Spectroelectrochemical Signatures of Capacitive Charging and Ion Insertion in Doped Anatase Titania Nanocrystals SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID TIO2 ANATASE; OPTICAL-PROPERTIES; LITHIUM-STORAGE; THIN-FILMS; PHOTOCATALYSIS; NANOPARTICLES; ELECTRODES; OXIDE; NANOMATERIALS; ACCUMULATION AB Solution-processed films of colloidal aliovalent niobium-doped anatase TiO2 nanocrystals exhibit modulation of optical transmittance in two Spectral regions near-infrared (NIR) and visible light as they undergo progressive and reversible charging in an electrochemical cell. The Nb-TiO2 nano crystal film supports a localized surface plasmon resonance in the NIR, which can be dynamically modulated via capacitive charging. When the nanocrystals are charged by insertion of lithium ions, inducing a well-known structural phase transition of the anatase lattice, strong modulation of visible transmittance is observed. Based on X-ray absorption near-edge spectroscopy, the conduction electrons localize only upon lithium ion insertion, thus rationalizing the two modes of optical switching observed in a single material. These multimodal electrochromic properties show promise for application in dynamic optical filters or smart windows. C1 [Dahlman, Clayton J.; Tan, Yizheng; Milliron, Delia J.] Univ Texas Austin, McKetta Dept Chem Engn, Austin, TX 78712 USA. [Tan, Yizheng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Marcus, Matthew A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Milliron, DJ (reprint author), Univ Texas Austin, McKetta Dept Chem Engn, 200 E Dean Keeton St, Austin, TX 78712 USA. EM milliron@che.utexas.edu RI Milliron, Delia/D-6002-2012; Foundry, Molecular/G-9968-2014; OI Dahlman, Clayton/0000-0002-4555-4846 FU U.S. Department of Energy (DOE) ARPA-E; Welch Foundation [F-1848]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; DOE [DE-AC02-76SF00515]; National Science Foundation [DGE 1106400] FX The authors thank Dr. Luca de Trizio for synthesis of Nb-TiO2 NCs used in preliminary studies and Dr. Guillermo Garcia for exploratory spectroelectrochemical measurements of Nb-TiO2 NCs. This research was supported by a U.S. Department of Energy (DOE) ARPA-E grant. D.J.M. acknowledges support of the Welch Foundation (F-1848). Some of this research was carried out at the Molecular Foundry, Lawrence Berkeley National Laboratory, a user facility supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. Use of SSRL, SLAC National Accelerator Laboratory, is supported by DOE under contract no. DE-AC02-76SF00515. C.J.D. was supported by a National Science Foundation Graduate Research Fellowship under grant no. DGE 1106400. NR 54 TC 12 Z9 12 U1 11 U2 78 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUL 22 PY 2015 VL 137 IS 28 BP 9160 EP 9166 DI 10.1021/jacs.5b04933 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA CN6PH UT WOS:000358556200044 PM 26154107 ER PT J AU Glazer, MPB Cho, J Almer, J Okasinski, J Braun, PV Dunand, DC AF Glazer, Matthew P. B. Cho, Jiung Almer, Jonathan Okasinski, John Braun, Paul V. Dunand, David C. TI In Operando Strain Measurement of Bicontinuous Silicon-Coated Nickel Inverse Opal Anodes for Li-Ion Batteries SO ADVANCED ENERGY MATERIALS LA English DT Article DE in operando; lithiation strain; microbatteries; silicon anodes; X-ray diffraction ID X-RAY-DIFFRACTION; IN-SITU XRD; LITHIUM-ION; AMORPHOUS-SILICON; THIN-FILMS; ELECTRODE MATERIALS; LITHIATION; STRESS; EVOLUTION; DELITHIATION AB Elastic strains are measured in operando in a nanostructured silicon-coated nickel inverse opal scaffold anode, using X-ray diffraction to study the Si (de)lithiation-induced Ni strains. The volume expansion upon lithiation of the Si in the anode is constrained by the surrounding Ni scaffold, causing mismatch stresses and strains in the Si and Ni phases during cycling. The Ni strains are measured in operando during (dis)charge cycles, using diffraction peak position and peak broadness to describe the distribution of strain in the Ni. During lithiation, compressive strains in the Ni first increase linearly with charge, after which a gradually decreasing strain rate is observed as the maximum lithiation state is approached; upon delithiation a similar process occurs. In-plane average compressive strains on the order of 990 +/- 40 epsilon are measured in the Ni scaffold during lithiation, corresponding to compressive stresses of 215 +/- 9 MPa. The decreasing strain rates and decreasing maximum and recovered strains suggest that plasticity in Ni and/or Si, as well as delamination between Ni and Si, may occur during cycling. Rate sensitivity in capacity is correlated with strain and a maximum Ni compressive stress of 230 +/- 40 MPa is measured at the maximum state of lithiation. C1 [Glazer, Matthew P. B.; Dunand, David C.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Cho, Jiung; Braun, Paul V.] Univ Illinois, Dept Mat Sci & Engn, Champaign, IL 61801 USA. [Cho, Jiung] Korea Basic Sci Inst, Gangneung Ctr, Kangnung 210702, South Korea. [Almer, Jonathan; Okasinski, John] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Dunand, DC (reprint author), Northwestern Univ, Dept Mat Sci & Engn, 2220 Campus Dr,Attent Room 2036, Evanston, IL 60208 USA. EM dunand@northwestern.edu RI Dunand, David/B-7515-2009 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357, DE-FG02-07ER46471]; U.S. DOE [DE-AC02-06CH11357] FX This research was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357 (electrochemical and X-ray characterization) and DE-FG02-07ER46471 (electrode fabrication). The authors thank Z. Liu, C. Hayner, and D. Snydacker (Northwestern University) for their helpful discussions and assistance during data collection and analysis, J. Wang (University of Illinois at Urbana-Champaign) for assistance throughout the project, and the staff of Sector 1 of the Advanced Photon Source (Argonne National Laboratory) for assistance in experiments and data acquisition. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 47 TC 7 Z9 7 U1 16 U2 103 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD JUL 22 PY 2015 VL 5 IS 14 AR 1500466 DI 10.1002/aenm.201500466 PG 10 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA CN4AG UT WOS:000358369700012 ER PT J AU Chung, D Verbeke, TJ Cross, KL Westpheling, J Elkins, JG AF Chung, Daehwan Verbeke, Tobin J. Cross, Karissa L. Westpheling, Janet Elkins, James G. TI Expression of a heat-stable NADPH-dependent alcohol dehydrogenase in Caldicellulosiruptor bescii results in furan aldehyde detoxification SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Thermophile; Pretreatment; Lignocellulose; Biofuel; Butanol dehydrogenase; Furfural; 5-hydroxymethylfurfural; Inhibitor; Genetic engineering; Caldicellulosiruptor bescii ID DILUTE-ACID PRETREATMENT; LIGNOCELLULOSIC BIOMASS CONVERSION; YELLOWSTONE-NATIONAL-PARK; SACCHAROMYCES-CEREVISIAE; HYDROGEN-PRODUCTION; PLANT BIOMASS; CELLULOLYTIC BACTERIUM; ENZYMATIC-HYDROLYSIS; ETHANOL-PRODUCTION; ESCHERICHIA-COLI AB Background: Compounds such as furfural and 5-hydroxymethylfurfural (5-HMF) are generated through the dehydration of xylose and glucose, respectively, during dilute-acid pretreatment of lignocellulosic biomass and are also potent microbial growth and fermentation inhibitors. The enzymatic reduction of these furan aldehydes to their corresponding, and less toxic, alcohols is an engineering approach that has been successfully implemented in both Saccharomyces cerevisiae and ethanologenic Escherichia coli, but has not yet been investigated in thermophiles relevant to biofuel production through consolidated bioprocessing (CBP). Developing CBP-relevant biocatalysts that are either naturally resistant to such inhibitors, or are amenable to engineered resistance, is therefore, an important component in making biofuels production from lignocellulosic biomass feasible. Results: A butanol dehydrogenase encoding gene from Thermoanaerobacter pseudethanolicus 39E (Teth39_1597), previously shown to have furfural and 5-HMF reducing capabilities, was cloned into a suicide plasmid, pDCW171 and transformed into a lactate dehydrogenase mutant of Caldicellulosiruptor bescii. Integration of the gene into the C. bescii chromosome was verified via PCR amplification and stable expression was observed up to 75 degrees C. Heterologous expression of the NADPH-dependent BdhA enzyme conferred increased resistance of the engineered strain to both furfural and 5-HMF relative to the wild-type and parental strains. Further, when challenged with 15 mM concentrations of either furan aldehyde, the ability to eliminate furfural or 5-HMF from the culture medium was significantly improved in the engineered strain. Conclusions: A genetically engineered strain of C. bescii (JWCB044) has been constructed that shows both an improved tolerance to furan aldehydes and an improved ability to eliminate furfural and 5-HMF from the culture medium. The work presented here represents the first example of engineering furan aldehyde resistance into a CBP-relevant thermophile and further validates C. bescii as being a genetically tractable microbe of importance for lignocellulosic biofuel production. C1 [Chung, Daehwan; Verbeke, Tobin J.; Cross, Karissa L.; Westpheling, Janet; Elkins, James G.] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA. [Chung, Daehwan; Westpheling, Janet] Univ Georgia, Dept Genet, Athens, GA 30602 USA. [Verbeke, Tobin J.; Cross, Karissa L.; Elkins, James G.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. RP Elkins, JG (reprint author), Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA. EM elkinsjg@ornl.gov RI Elkins, James/A-6199-2011 OI Elkins, James/0000-0002-8052-5688 FU U.S. Department of Energy, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Science Undergraduate Laboratory Internship (SULI) program; BioEnergy Science Center (BESC), U.S. Department of Energy Bioenergy Research Center - Office of Biological and Environmental Research in the DOE Office of Science, Oak Ridge National Laboratory; U.S. Department of Energy [DE-AC05-00OR22725] FX Karissa L. Cross was supported by the U.S. Department of Energy, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Science Undergraduate Laboratory Internship (SULI) program. This work was supported by the BioEnergy Science Center (BESC), which is a U.S. Department of Energy Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science, Oak Ridge National Laboratory. Oak Ridge National Laboratory is managed by UT-Battelle, LLC, for the U.S. Department of Energy under contract DE-AC05-00OR22725. This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 47 TC 4 Z9 4 U1 1 U2 20 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD JUL 22 PY 2015 VL 8 AR 102 DI 10.1186/s13068-015-0287-y PG 11 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA CN2TT UT WOS:000358275500001 PM 26203301 ER PT J AU Carrillo-Serrano, ME Bentz, W Cloet, IC Thomas, AW AF Carrillo-Serrano, Manuel E. Bentz, Wolfgang Cloet, Ian C. Thomas, Anthony W. TI rho meson form factors in a confining Nambu-Jona-Lasinio model SO PHYSICAL REVIEW C LA English DT Article ID QUARK-DIQUARK MODEL; EXTENDED NJL MODEL; DYNAMICAL MODEL; LIGHT; COVARIANT; SUPERCONDUCTIVITY; DISTRIBUTIONS; ANALOGY; LATTICE AB Elastic electromagnetic form factors for the rho(+) meson are calculated in a Nambu-Jona-Lasinio model which incorporates quark confinement through the use of the proper-time regularization scheme. A comparison is made with recent lattice QCD results and previous quark model calculations for static quantities and the Sachs form factors. The results are qualitatively in good agreement with the lattice QCD calculations, with the exception of the quadrupole moment and corresponding form factor, which may be related to a lack of spherical symmetry on the lattice. C1 [Carrillo-Serrano, Manuel E.; Thomas, Anthony W.] Univ Adelaide, CSSM, Adelaide, SA 5005, Australia. [Carrillo-Serrano, Manuel E.; Thomas, Anthony W.] Univ Adelaide, ARC Ctr Excellence Particle Phys Tera Scale, Dept Phys, Adelaide, SA 5005, Australia. [Bentz, Wolfgang] Tokai Univ, Sch Sci, Dept Phys, Hiratsuka, Kanagawa 2591292, Japan. [Cloet, Ian C.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RP Carrillo-Serrano, ME (reprint author), Univ Adelaide, CSSM, Adelaide, SA 5005, Australia. RI Thomas, Anthony/G-4194-2012 OI Thomas, Anthony/0000-0003-0026-499X FU Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357]; Australian Research Council through ARC Centre of Excellence in Particle Physics at the Terascale; ARC Australian Laureate Fellowship [FL0992247]; Japanese Ministry of Education, Sports, Science and Technology [25400270] FX This work was supported by the Department of Energy, Office of Nuclear Physics, Contract No. DE-AC02-06CH11357; the Australian Research Council through the ARC Centre of Excellence in Particle Physics at the Terascale and an ARC Australian Laureate Fellowship FL0992247 (AWT); and the Grant in Aid for Scientific Research (Kakenhi) of the Japanese Ministry of Education, Sports, Science and Technology, Project No. 25400270. NR 44 TC 4 Z9 4 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JUL 22 PY 2015 VL 92 IS 1 AR 015212 DI 10.1103/PhysRevC.92.015212 PG 8 WC Physics, Nuclear SC Physics GA CN4BV UT WOS:000358374600001 ER PT J AU Jimenez-Alba, A Yee, HU AF Jimenez-Alba, Amadeo Yee, Ho-Ung TI Second order transport coefficient from the chiral anomaly at weak coupling: Diagrammatic resummation SO PHYSICAL REVIEW D LA English DT Article ID QUARK-GLUON PLASMA; COLLISIONS; DYNAMICS; QCD AB We compute one of the second order transport coefficients arising from the chiral anomaly in a high-temperature weakly coupled regime of quark-gluon plasma. This transport coefficient is responsible for the CP-odd current that is proportional to the time derivative of the magnetic field, and can be considered as a first correction to the chiral magnetic conductivity at finite, small frequency. We observe that this transport coefficient has a nonanalytic dependence on the coupling as similar to 1/(g(4) log(1/g)) at the weak coupling regime, which necessitates a resummation of infinite ladder diagrams with leading pinch singularities to get a correct leading log result, a feature quite similar to what one finds in the computation of electric conductivity. We formulate and solve the relevant CP-odd Schwinger-Dyson equation in real-time perturbation theory that reduces to a coupled set of second order differential equations at leading log order. Our result for this second order transport coefficient indicates that chiral magnetic current has some resistance to the time change of the magnetic field; this shall be called the "chiral induction effect." We also discuss the case of color current induced by a color magnetic field. C1 [Jimenez-Alba, Amadeo] Univ Autonoma Madrid, Inst Fis Teor IFT UAM CSIC, Canto Blanco 28049, Spain. [Yee, Ho-Ung] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. [Yee, Ho-Ung] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. RP Jimenez-Alba, A (reprint author), Univ Autonoma Madrid, Inst Fis Teor IFT UAM CSIC, Canto Blanco 28049, Spain. EM amadeo.j@gmail.com; hyee@uic.edu FU FPU fellowship [AP2010-5686]; Plan Nacional de Altas Energias [FPA2009-07890]; Consolider Ingenio CPAN Grant [CSD200-00042]; Severo Ochoa Grant [SEV-2012-0249] FX A. J. would like to thank the Nuclear Theory Group at UIC for hospitality during his visit and Francisco Pena for useful comments. H. U. Y. thanks Sangyong Jeon, Dima Kharzeev, Kiminad Mamo, Rob Pisarski, Daisuke Satow, and Misha Stephanov for discussions. We thank Kristan Jensen for helpful correspondence on hydrostatic constraint analysis. A. J. has been supported by a FPU fellowship Grant No. AP2010-5686, Plan Nacional de Altas Energias Grant No. FPA2009-07890, Consolider Ingenio 2010 CPAN Grant No. CSD200-00042, and Severo Ochoa Grant No. SEV-2012-0249. NR 73 TC 4 Z9 4 U1 2 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 22 PY 2015 VL 92 IS 1 AR 014023 DI 10.1103/PhysRevD.92.014023 PG 30 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CN4CL UT WOS:000358376500001 ER PT J AU Lane, JMD AF Lane, J. Matthew D. TI Cooling rate and stress relaxation in silica melts and glasses via microsecond molecular dynamics SO PHYSICAL REVIEW E LA English DT Article ID AMORPHOUS SILICA; VITREOUS SILICA; TRANSITION; SIMULATION; POLYMERS; MECHANISMS; LIQUIDS AB We have conducted extremely long molecular dynamics simulations of glasses to microsecond times, which close the gap between experimental and atomistic simulation time scales by two to three orders of magnitude. Static, thermal, and structural properties of silica glass are reported for glass cooling rates down to 5 x 10(9) K/s and viscoelastic response in silica melts and glasses are studied over nine decades of time. We present results from relaxation of hydrostatic compressive stress in silica and show that time-temperature superposition holds in these systems for temperatures from 3500 to 1000 K. C1 Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Lane, JMD (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. FU Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The author would like to thank R. Chambers, R. Tandon, and M. Chandross at Sandia National Labs for useful discussions. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 35 TC 4 Z9 4 U1 0 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD JUL 22 PY 2015 VL 92 IS 1 AR 012320 DI 10.1103/PhysRevE.92.012320 PG 8 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA CN4CW UT WOS:000358377800007 PM 26274174 ER PT J AU Abazov, VM Abbott, B Acharya, BS Adams, M Adams, T Agnew, JP Alexeev, GD Alkhazov, G Alton, A Askew, A Atkins, S Augsten, K Avila, C Badaud, F Bagby, L Baldin, B Bandurin, DV Banerjee, S Barberis, E Baringer, P Bartlett, JF Bassler, U Bazterra, V Bean, A Begalli, M Bellantoni, L Beri, SB Bernardi, G Bernhard, R Bertram, I Besancon, M Beuselinck, R Bhat, PC Bhatia, S Bhatnagar, V Blazey, G Blessing, S Bloom, K Boehnlein, A Boline, D Boos, EE Borissov, G Borysova, M Brandt, A Brandt, O Brock, R Bross, A Brown, D Bu, XB Buehler, M Buescher, V Bunichev, V Burdin, S Buszello, CP Camacho-Perez, E Casey, BCK Castilla-Valdez, H Caughron, S Chakrabarti, S Chan, KM Chandra, A Chapon, E Chen, G Cho, SW Choi, S Choudhary, B Cihangir, S Claes, D Clutter, J Cooke, M Cooper, WE Corcoran, M Couderc, F Cousinou, MC Cutts, D Das, A Davies, G de Jong, SJ De la Cruz-Burelo, E Deliot, F Demina, R Denisov, D Denisov, SP Desai, S Deterre, C DeVaughan, K Diehl, HT Diesburg, M Ding, PF Dominguez, A Dubey, A Dudko, LV Duperrin, A Dutt, S Eads, M Edmunds, D Ellison, J Elvira, VD Enari, Y Evans, H Evdokimov, VN Faure, A Feng, L Ferbel, T Fiedler, F Filthaut, F Fisher, W Fisk, HE Fortner, M Fox, H Fuess, S Garbincius, PH Garcia-Bellido, A Garcia-Gonzalez, JA Gavrilov, V Geng, W Gerber, CE Gershtein, Y Ginther, G Gogota, O Golovanov, G Grannis, PD Greder, S Greenlee, H Grenier, G Gris, P Grivaz, JF Grohsjean, A Grunendahl, S Grunewald, MW Guillemin, T Gutierrez, G Gutierrez, P Haley, J Han, L Harder, K Harel, A Hauptman, JM Hays, J Head, T Hebbeker, T Hedin, D Hegab, H Heinson, AP Heintz, U Hensel, C Heredia-De La Cruz, I Herner, K Hesketh, G Hildreth, MD Hirosky, R Hoang, T Hobbs, JD Hoeneisen, B Hogan, J Hohlfeld, M Holzbauer, JL Howley, I Hubacek, Z Hynek, V Iashvili, I Ilchenko, Y Illingworth, R Ito, AS Jabeen, S Jaffre, M Jayasinghe, A Jeong, MS Jesik, R Jiang, P Johns, K Johnson, E Johnson, M Jonckheere, A Jonsson, P Joshi, J Jung, AW Juste, A Kajfasz, E Karmanov, D Katsanos, I Kaur, M Kehoe, R Kermiche, S Khalatyan, N Khanov, A Kharchilava, A Kharzheev, YN Kiselevich, I Kohli, JM Kozelov, AV Kraus, J Kumar, A Kupco, A Kurca, T Kuzmin, VA Lammers, S Lebrun, P Lee, HS Lee, SW Lee, WM Lei, X Lellouch, J Li, D Li, H Li, L Li, QZ Lim, JK Lincoln, D Linnemann, J Lipaev, VV Lipton, R Liu, H Liu, Y Lobodenko, A Lokajicek, M de Sa, RL Luna-Garcia, R Lyon, AL Maciel, AKA Madar, R Magana-Villalba, R Malik, S Malyshev, VL Mansour, J Martinez-Ortega, J McCarthy, R McGivern, CL Meijer, MM Melnitchouk, A Menezes, D Mercadante, PG Merkin, M Meyer, A Meyer, J Miconi, F Mondal, NK Mulhearn, M Nagy, E Narain, M Nayyar, R Neal, HA Negret, JP Neustroev, P Nguyen, HT Nunnemann, T Orduna, J Osman, N Osta, J Pal, A Parashar, N Parihar, V Park, SK Partridge, R Parua, N Patwa, A Penning, B Perfilov, M Peters, Y Petridis, K Petrillo, G Petroff, P Pleier, MA Podstavkov, VM Popov, AV Prewitt, M Price, D Prokopenko, N Qian, J Quadt, A Quinn, B Ratoff, PN Razumov, I Ripp-Baudot, I Rizatdinova, F Rominsky, M Ross, A Royon, C Rubinov, P Ruchti, R Sajot, G Sanchez-Hernandez, A Sanders, MP Santos, AS Savage, G Savitskyi, M Sawyer, L Scanlon, T Schamberger, RD Scheglov, Y Schellman, H Schwanenberger, C Schwienhorst, R Sekaric, J Severini, H Shabalina, E Shary, V Shaw, S Shchukin, AA Simak, V Skubic, P Slattery, P Smirnov, D Snow, GR Snow, J Snyder, S Soldner-Rembold, S Sonnenschein, L Soustruznik, K Stark, J Stoyanova, DA Strauss, M Suter, L Svoisky, P Titov, M Tokmenin, VV Tsai, YT Tsybychev, D Tuchming, B Tully, C Uvarov, L Uvarov, S Uzunyan, S Van Kooten, R van Leeuwen, WM Varelas, N Varnes, EW Vasilyev, IA Verkheev, AY Vertogradov, LS Verzocchi, M Vesterinen, M Vilanova, D Vokac, P Wahl, HD Wang, MHLS Warchol, J Watts, G Wayne, M Weichert, J Welty-Rieger, L Williams, MRJ Wilson, GW Wobisch, M Wood, DR Wyatt, TR Xie, Y Yamada, R Yang, S Yasuda, T Yatsunenko, YA Ye, W Ye, Z Yin, H Yip, K Youn, SW Yu, JM Zennamo, J Zhao, TG Zhou, B Zhu, J Zielinski, M Zieminska, D Zivkovic, L AF Abazov, V. M. Abbott, B. Acharya, B. S. Adams, M. Adams, T. Agnew, J. P. Alexeev, G. D. Alkhazov, G. Alton, A. Askew, A. Atkins, S. Augsten, K. Avila, C. Badaud, F. Bagby, L. Baldin, B. Bandurin, D. V. Banerjee, S. Barberis, E. Baringer, P. Bartlett, J. F. Bassler, U. Bazterra, V. Bean, A. Begalli, M. Bellantoni, L. Beri, S. B. Bernardi, G. Bernhard, R. Bertram, I. Besancon, M. Beuselinck, R. Bhat, P. C. Bhatia, S. Bhatnagar, V. Blazey, G. Blessing, S. Bloom, K. Boehnlein, A. Boline, D. Boos, E. E. Borissov, G. Borysova, M. Brandt, A. Brandt, O. Brock, R. Bross, A. Brown, D. Bu, X. B. Buehler, M. Buescher, V. Bunichev, V. Burdin, S. Buszello, C. P. Camacho-Perez, E. Casey, B. C. K. Castilla-Valdez, H. Caughron, S. Chakrabarti, S. Chan, K. M. Chandra, A. Chapon, E. Chen, G. Cho, S. W. Choi, S. Choudhary, B. Cihangir, S. Claes, D. Clutter, J. Cooke, M. Cooper, W. E. Corcoran, M. Couderc, F. Cousinou, M. -C. Cutts, D. Das, A. Davies, G. de Jong, S. J. De la Cruz-Burelo, E. Deliot, F. Demina, R. Denisov, D. Denisov, S. P. Desai, S. Deterre, C. DeVaughan, K. Diehl, H. T. Diesburg, M. Ding, P. F. Dominguez, A. Dubey, A. Dudko, L. V. Duperrin, A. Dutt, S. Eads, M. Edmunds, D. Ellison, J. Elvira, V. D. Enari, Y. Evans, H. Evdokimov, V. N. Faure, A. Feng, L. Ferbel, T. Fiedler, F. Filthaut, F. Fisher, W. Fisk, H. E. Fortner, M. Fox, H. Fuess, S. Garbincius, P. H. Garcia-Bellido, A. Garcia-Gonzalez, J. A. Gavrilov, V. Geng, W. Gerber, C. E. Gershtein, Y. Ginther, G. Gogota, O. Golovanov, G. Grannis, P. D. Greder, S. Greenlee, H. Grenier, G. Gris, Ph. Grivaz, J. -F. Grohsjean, A. Gruenendahl, S. Gruenewald, M. W. Guillemin, T. Gutierrez, G. Gutierrez, P. Haley, J. Han, L. Harder, K. Harel, A. Hauptman, J. M. Hays, J. Head, T. Hebbeker, T. Hedin, D. Hegab, H. Heinson, A. P. Heintz, U. Hensel, C. Heredia-De La Cruz, I. Herner, K. Hesketh, G. Hildreth, M. D. Hirosky, R. Hoang, T. Hobbs, J. D. Hoeneisen, B. Hogan, J. Hohlfeld, M. Holzbauer, J. L. Howley, I. Hubacek, Z. Hynek, V. Iashvili, I. Ilchenko, Y. Illingworth, R. Ito, A. S. Jabeen, S. Jaffre, M. Jayasinghe, A. Jeong, M. S. Jesik, R. Jiang, P. Johns, K. Johnson, E. Johnson, M. Jonckheere, A. Jonsson, P. Joshi, J. Jung, A. W. Juste, A. Kajfasz, E. Karmanov, D. Katsanos, I. Kaur, M. Kehoe, R. Kermiche, S. Khalatyan, N. Khanov, A. Kharchilava, A. Kharzheev, Y. N. Kiselevich, I. Kohli, J. M. Kozelov, A. V. Kraus, J. Kumar, A. Kupco, A. Kurca, T. Kuzmin, V. A. Lammers, S. Lebrun, P. Lee, H. S. Lee, S. W. Lee, W. M. Lei, X. Lellouch, J. Li, D. Li, H. Li, L. Li, Q. Z. Lim, J. K. Lincoln, D. Linnemann, J. Lipaev, V. V. Lipton, R. Liu, H. Liu, Y. Lobodenko, A. Lokajicek, M. de Sa, R. Lopes Luna-Garcia, R. Lyon, A. L. Maciel, A. K. A. Madar, R. Magana-Villalba, R. Malik, S. Malyshev, V. L. Mansour, J. Martinez-Ortega, J. McCarthy, R. McGivern, C. L. Meijer, M. M. Melnitchouk, A. Menezes, D. Mercadante, P. G. Merkin, M. Meyer, A. Meyer, J. Miconi, F. Mondal, N. K. Mulhearn, M. Nagy, E. Narain, M. Nayyar, R. Neal, H. A. Negret, J. P. Neustroev, P. Nguyen, H. T. Nunnemann, T. Orduna, J. Osman, N. Osta, J. Pal, A. Parashar, N. Parihar, V. Park, S. K. Partridge, R. Parua, N. Patwa, A. Penning, B. Perfilov, M. Peters, Y. Petridis, K. Petrillo, G. Petroff, P. Pleier, M. -A. Podstavkov, V. M. Popov, A. V. Prewitt, M. Price, D. Prokopenko, N. Qian, J. Quadt, A. Quinn, B. Ratoff, P. N. Razumov, I. Ripp-Baudot, I. Rizatdinova, F. Rominsky, M. Ross, A. Royon, C. Rubinov, P. Ruchti, R. Sajot, G. Sanchez-Hernandez, A. Sanders, M. P. Santos, A. S. Savage, G. Savitskyi, M. Sawyer, L. Scanlon, T. Schamberger, R. D. Scheglov, Y. Schellman, H. Schwanenberger, C. Schwienhorst, R. Sekaric, J. Severini, H. Shabalina, E. Shary, V. Shaw, S. Shchukin, A. A. Simak, V. Skubic, P. Slattery, P. Smirnov, D. Snow, G. R. Snow, J. Snyder, S. Soeldner-Rembold, S. Sonnenschein, L. Soustruznik, K. Stark, J. Stoyanova, D. A. Strauss, M. Suter, L. Svoisky, P. Titov, M. Tokmenin, V. V. Tsai, Y. -T. Tsybychev, D. Tuchming, B. Tully, C. Uvarov, L. Uvarov, S. Uzunyan, S. Van Kooten, R. van Leeuwen, W. M. Varelas, N. Varnes, E. W. Vasilyev, I. A. Verkheev, A. Y. Vertogradov, L. S. Verzocchi, M. Vesterinen, M. Vilanova, D. Vokac, P. Wahl, H. D. Wang, M. H. L. S. Warchol, J. Watts, G. Wayne, M. Weichert, J. Welty-Rieger, L. Williams, M. R. J. Wilson, G. W. Wobisch, M. Wood, D. R. Wyatt, T. R. Xie, Y. Yamada, R. Yang, S. Yasuda, T. Yatsunenko, Y. A. Ye, W. Ye, Z. Yin, H. Yip, K. Youn, S. W. Yu, J. M. Zennamo, J. Zhao, T. G. Zhou, B. Zhu, J. Zielinski, M. Zieminska, D. Zivkovic, L. CA D0 Collaboration TI Measurement of the Effective Weak Mixing Angle in p(p)over-bar -> Z/gamma* -> e(+)e(-) Events SO PHYSICAL REVIEW LETTERS LA English DT Article AB We present a measurement of the fundamental parameter of the standard model, the weak mixing angle sin(2)theta(l)(eff) which determines the relative strength of weak and electromagnetic interactions, in p (p) over bar -> Z/gamma* -> e(+)e(-) events at a center of mass energy of 1.96 TeV, using data corresponding to 9.7 fb(-1) of integrated luminosity collected by the D0 detector at the Fermilab Tevatron. The effective weak mixing angle is extracted from the forward-backward charge asymmetry as a function of the invariant mass around the Z boson pole. The measured value of sin(2)theta(l)(eff) = 0.23147 +/- 0.00047 is the most precise measurement from light quark interactions to date, with a precision close to the best LEP and SLD results. C1 [Hensel, C.; Maciel, A. K. A.; Santos, A. S.] Ctr Brasileiro Pesquisas Fis, ILAFEX, Rio De Janeiro, Brazil. [Begalli, M.] Univ Estado Rio de Janeiro, Rio De Janeiro, Brazil. [Mercadante, P. G.] Univ Fed ABC, Santo Andre, Brazil. [Han, L.; Jiang, P.; Liu, Y.; Yang, S.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Avila, C.; Negret, J. P.] Univ Los Andes, Bogota, Colombia. [Soustruznik, K.] Charles Univ Prague, Fac Math & Phys, Ctr Particle Phys, Prague, Czech Republic. [Augsten, K.; Hubacek, Z.; Hynek, V.; Simak, V.; Vokac, P.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Kupco, A.; Lokajicek, M.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Hoeneisen, B.] Univ San Francisco, Quito, Ecuador. [Badaud, F.; Gris, Ph.] Univ Clermont Ferrand, CNRS, IN2P3, LPC, Clermont, France. [Sajot, G.; Stark, J.] Univ Grenoble 1, CNRS, Inst Natl Polytech Grenoble, LPSC, Grenoble, France. 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G.] Univ Manchester, Manchester M13 9PL, Lancs, England. [Das, A.; Johns, K.; Lee, W. M.; Lei, X.; Nayyar, R.; Varnes, E. W.] Univ Arizona, Tucson, AZ 85721 USA. [Ellison, J.; Heinson, A. P.; Joshi, J.; Li, L.] Univ Calif Riverside, Riverside, CA 92521 USA. [Adams, T.; Askew, A.; Blessing, S.; Hoang, T.; Wahl, H. D.] Florida State Univ, Tallahassee, FL 32306 USA. [Bagby, L.; Baldin, B.; Bartlett, J. F.; Bellantoni, L.; Bhat, P. C.; Boehnlein, A.; Bross, A.; Bu, X. B.; Buehler, M.; Casey, B. C. K.; Cihangir, S.; Cooke, M.; Cooper, W. E.; Denisov, D.; Desai, S.; Diehl, H. T.; Diesburg, M.; Elvira, V. D.; Fisk, H. E.; Fuess, S.; Garbincius, P. H.; Ginther, G.; Greenlee, H.; Gruenendahl, S.; Herner, K.; Illingworth, R.; Ito, A. S.; Jabeen, S.; Johnson, M.; Jonckheere, A.; Jung, A. W.; Khalatyan, N.; Li, Q. Z.; Lincoln, D.; Lipton, R.; de Sa, R. Lopes; Lyon, A. L.; Melnitchouk, A.; Penning, B.; Podstavkov, V. M.; Rominsky, M.; Rubinov, P.; Savage, G.; Wang, M. H. L. S.; Xie, Y.; Yamada, R.; Yasuda, T.; Ye, Z.; Yin, H.; Youn, S. W.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Adams, M.; Bazterra, V.; Gerber, C. E.; Varelas, N.] Univ Illinois, Chicago, IL 60607 USA. [Blazey, G.; Eads, M.; Feng, L.; Fortner, M.; Hedin, D.; Menezes, D.; Uzunyan, S.] No Illinois Univ, De Kalb, IL 60115 USA. [Schellman, H.; Welty-Rieger, L.] Northwestern Univ, Evanston, IL 60208 USA. [Evans, H.; Lammers, S.; Parua, N.; Van Kooten, R.; Williams, M. R. J.; Zieminska, D.] Indiana Univ, Bloomington, IN 47405 USA. [Parashar, N.] Purdue Univ Calumet, Hammond, IN 46323 USA. [Chan, K. M.; Hildreth, M. D.; Osta, J.; Ruchti, R.; Smirnov, D.; Warchol, J.; Wayne, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Hauptman, J. M.; Lee, S. W.] Iowa State Univ, Ames, IA 50011 USA. [Baringer, P.; Bean, A.; Chen, G.; Clutter, J.; Sekaric, J.; Wilson, G. W.] Univ Kansas, Lawrence, KS 66045 USA. [Atkins, S.; Prokopenko, N.; Sawyer, L.; Wobisch, M.] Louisiana Tech Univ, Ruston, LA 71272 USA. [Barberis, E.; Wood, D. R.] Northeastern Univ, Boston, MA 02115 USA. [Alton, A.; Neal, H. A.; Qian, J.; Yu, J. M.; Zhou, B.; Zhu, J.] Univ Michigan, Ann Arbor, MI 48109 USA. [Brock, R.; Caughron, S.; Edmunds, D.; Fisher, W.; Geng, W.; Johnson, E.; Linnemann, J.; Schwienhorst, R.] Michigan State Univ, E Lansing, MI 48824 USA. [Bhatia, S.; Holzbauer, J. L.; Kraus, J.; Quinn, B.] Univ Mississippi, University, MS 38677 USA. [Bloom, K.; Claes, D.; DeVaughan, K.; Dominguez, A.; Katsanos, I.; Malik, S.; Snow, G. R.] Univ Nebraska, Lincoln, NE 68588 USA. [Gershtein, Y.] Rutgers State Univ, Piscataway, NJ 08855 USA. [Tully, C.] Princeton Univ, Princeton, NJ 08544 USA. [Iashvili, I.; Kharchilava, A.; Kumar, A.; Zennamo, J.] SUNY Buffalo, Buffalo, NY 14260 USA. [Demina, R.; Ferbel, T.; Garcia-Bellido, A.; Ginther, G.; Harel, A.; Petrillo, G.; Slattery, P.; Tsai, Y. -T.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Boline, D.; Chakrabarti, S.; Grannis, P. D.; Hobbs, J. D.; McCarthy, R.; Schamberger, R. D.; Tsybychev, D.; Ye, W.] SUNY Stony Brook, Stony Brook, NY 11794 USA. [Patwa, A.; Pleier, M. -A.; Snyder, S.; Yip, K.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Snow, J.] Langston Univ, Langston, OK 73050 USA. [Abbott, B.; Gutierrez, P.; Jayasinghe, A.; Severini, H.; Skubic, P.; Strauss, M.; Svoisky, P.] Univ Oklahoma, Norman, OK 73019 USA. [Haley, J.; Hegab, H.; Khanov, A.; Rizatdinova, F.] Oklahoma State Univ, Stillwater, OK 74078 USA. [Cutts, D.; Heintz, U.; Narain, M.; Parihar, V.; Partridge, R.] Brown Univ, Providence, RI 02912 USA. [Brandt, A.; Pal, A.] Univ Texas Arlington, Arlington, TX 76019 USA. [Ilchenko, Y.; Kehoe, R.; Liu, H.] So Methodist Univ, Dallas, TX 75275 USA. [Chandra, A.; Corcoran, M.; Hogan, J.; Orduna, J.; Prewitt, M.] Rice Univ, Houston, TX 77005 USA. [Bandurin, D. V.; Hirosky, R.; Li, H.; Mulhearn, M.; Nguyen, H. T.] Univ Virginia, Charlottesville, VA 22904 USA. [Watts, G.] Univ Washington, Seattle, WA 98195 USA. RP Abazov, VM (reprint author), Joint Nucl Res Inst, Dubna, Russia. RI Sharyy, Viatcheslav/F-9057-2014; Dudko, Lev/D-7127-2012; Merkin, Mikhail/D-6809-2012; Li, Liang/O-1107-2015; Gutierrez, Phillip/C-1161-2011 OI Sharyy, Viatcheslav/0000-0002-7161-2616; Dudko, Lev/0000-0002-4462-3192; Li, Liang/0000-0001-6411-6107; FU Department of Energy (United States of America); National Science Foundation (United States of America); Alternative Energies and Atomic Energy Commission (France); National Center for Scientific Research/National Institute of Nuclear and Particle Physics (France); Ministry of Education and Science of the Russian Federation (Russia); National Research Center Kurchatov Institute of the Russian Federation (Russia); Russian Foundation for Basic Research (Russia); National Council for the Development of Science and Technology (Brazil); Carlos Chagas Filho Foundation for the Support of Research in the State of Rio de Janeiro (Brazil); Department of Atomic Energy (India); Department of Science and Technology (India); Administrative Department of Science, Technology and Innovation (Colombia); National Council of Science and Technology (Mexico); National Research Foundation of Korea (Korea); Foundation for Fundamental Research on Matter (The Netherlands); Science and Technology Facilities Council (United Kingdom); Royal Society (United Kingdom); Ministry of Education, Youth and Sports (Czech Republic); Bundesministerium fur Bildung und Forschung (Federal Ministry of Education and Research) (Germany); Deutsche Forschungsgemeinschaft (German Research Foundation) (Germany); Science Foundation Ireland (Ireland); Swedish Research Council (Sweden); China Academy of Sciences (China); National Natural Science Foundation of China (China); Ministry of Education and Science of Ukraine (Ukraine) FX We thank the staffs at Fermilab and collaborating institutions, and acknowledge support from the Department of Energy and National Science Foundation (United States of America); Alternative Energies and Atomic Energy Commission and National Center for Scientific Research/National Institute of Nuclear and Particle Physics (France); Ministry of Education and Science of the Russian Federation, National Research Center Kurchatov Institute of the Russian Federation, and Russian Foundation for Basic Research (Russia); National Council for the Development of Science and Technology and Carlos Chagas Filho Foundation for the Support of Research in the State of Rio de Janeiro (Brazil); Department of Atomic Energy and Department of Science and Technology (India); Administrative Department of Science, Technology and Innovation (Colombia); National Council of Science and Technology (Mexico); National Research Foundation of Korea (Korea); Foundation for Fundamental Research on Matter (The Netherlands); Science and Technology Facilities Council and The Royal Society (United Kingdom); Ministry of Education, Youth and Sports (Czech Republic); Bundesministerium fur Bildung und Forschung (Federal Ministry of Education and Research) and Deutsche Forschungsgemeinschaft (German Research Foundation) (Germany); Science Foundation Ireland (Ireland); Swedish Research Council (Sweden); China Academy of Sciences and National Natural Science Foundation of China (China); and Ministry of Education and Science of Ukraine (Ukraine). We thank Dr. W. Sakumoto for his help in assuring that the CDF and D0 collaborations used a similar phenomenological framework for these measurements. NR 24 TC 9 Z9 9 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 22 PY 2015 VL 115 IS 4 AR 041801 DI 10.1103/PhysRevLett.115.041801 PG 8 WC Physics, Multidisciplinary SC Physics GA CN4AA UT WOS:000358369000002 PM 26252676 ER PT J AU Thoutam, LR Wang, YL Xiao, ZL Das, S Luican-Mayer, A Divan, R Crabtree, GW Kwok, WK AF Thoutam, L. R. Wang, Y. L. Xiao, Z. L. Das, S. Luican-Mayer, A. Divan, R. Crabtree, G. W. Kwok, W. K. TI Temperature-Dependent Three-Dimensional Anisotropy of the Magnetoresistance in WTe2 SO PHYSICAL REVIEW LETTERS LA English DT Article ID MAGNETIC-FIELD AZIMUTH; GIANT MAGNETORESISTANCE; SINGLE-CRYSTAL; GRAPHITE; SUPERCONDUCTORS; OSCILLATIONS; BISMUTH AB Extremely large magnetoresistance (XMR) was recently discovered in WTe2, triggering extensive research on this material regarding the XMR origin. Since WTe2 is a layered compound with metal layers sandwiched between adjacent insulating chalcogenide layers, this material has been considered to be electronically two-dimensional (2D). Here we report two new findings on WTe2 : (1) WTe2 is electronically 3D with a mass anisotropy as low as 2, as revealed by the 3D scaling behavior of the resistance R(H,theta) = R(epsilon H-theta) with epsilon(theta) = (cos(2)theta + gamma(-2)sin(2)theta)(1/2), theta being the magnetic field angle with respect to the c axis of the crystal and. being the mass anisotropy and (2) the mass anisotropy gamma varies with temperature and follows the magnetoresistance behavior of the Fermi liquid state. Our results not only provide a general scaling approach for the anisotropic magnetoresistance but also are crucial for correctly understanding the electronic properties of WTe2, including the origin of the remarkable "turn-on" behavior in the resistance versus temperature curve, which has been widely observed in many materials and assumed to be a metalinsulator transition. C1 [Thoutam, L. R.; Wang, Y. L.; Xiao, Z. L.; Crabtree, G. W.; Kwok, W. K.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Thoutam, L. R.; Xiao, Z. L.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Das, S.; Luican-Mayer, A.; Divan, R.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Crabtree, G. W.] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. [Crabtree, G. W.] Univ Illinois, Dept Elect, Chicago, IL 60607 USA. [Crabtree, G. W.] Univ Illinois, Dept Mech Engn, Chicago, IL 60607 USA. RP Thoutam, LR (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM ylwang@anl.gov; xiao@anl.gov OI Wang, Yong-Lei/0000-0003-0391-7757 FU DOE BES [DE-AC02-06CH11357]; Argonne's Center for Nanoscale Materials (CNM); NSF [DMR-1407175] FX This work was supported by DOE BES under Contract No. DE-AC02-06CH11357 which also funds Argonne's Center for Nanoscale Materials (CNM) and Electron Microscopy Center (EMC) where the nanopatterning and morphological analysis were performed. L. R. T. and Z. L. X. acknowledge NSF Grant No. DMR-1407175. NR 30 TC 24 Z9 24 U1 31 U2 136 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 22 PY 2015 VL 115 IS 4 AR 046602 DI 10.1103/PhysRevLett.115.046602 PG 5 WC Physics, Multidisciplinary SC Physics GA CN4AA UT WOS:000358369000012 PM 26252701 ER PT J AU Macridin, A Burov, A Stern, E Amundson, J Spentzouris, P AF Macridin, Alexandru Burov, Alexey Stern, Eric Amundson, James Spentzouris, Panagiotis TI Simulation of transverse modes with their intrinsic Landau damping for bunched beams in the presence of space charge SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article AB Transverse dipole modes in bunches with space charge are simulated using the SYNERGIA accelerator modeling package and analyzed with dynamic mode decomposition. The properties of the first three space charge modes, including their shape, damping rates, and tune shifts are described over the entire range of space charge strength. The intrinsic Landau damping predicted and estimated in 2009 by one of the authors is confirmed with a reasonable scaling factor of. similar or equal to 2.4. For the KV distribution, very good agreement with PATRIC simulations performed by Kornilov and Boine-Frankenheim is obtained. C1 [Macridin, Alexandru; Burov, Alexey; Stern, Eric; Amundson, James; Spentzouris, Panagiotis] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Macridin, A (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. FU U.S. Department of Energy [DE-AC02-07CH11359]; ComPASS project through the Scientic Discovery through Advanced Computing program in the DOE Office of High Energy Physics; DOE Office of Science User Facility [DE-AC02-06CH11357] FX This work was performed at Fermilab, operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the U.S. Department of Energy. SYNERGIA development is partially supported through the ComPASS project, funded through the Scientic Discovery through Advanced Computing program in the DOE Office of High Energy Physics. An award of computer time was provided by the Innovative and Novel Computational Impact on Theory and Experiment (INCITE) program. This research used resources of the Argonne Leadership Computing Facility, which is a DOE Office of Science User Facility supported under Contract No. DE-AC02-06CH11357. NR 22 TC 2 Z9 2 U1 1 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD JUL 22 PY 2015 VL 18 IS 7 AR 074401 DI 10.1103/PhysRevSTAB.18.074401 PG 10 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA CN4CZ UT WOS:000358378300003 ER PT J AU Lany, S AF Lany, Stephan TI Semiconducting transition metal oxides SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Review DE transition metal oxides; electronic structure calculation; band structure; polarons; defects ID DENSITY-FUNCTIONAL THEORY; NIO THIN-FILMS; ANATASE TIO2; ELECTRICAL-PROPERTIES; ELECTRONIC-STRUCTURE; MAGNETIC-PROPERTIES; SINGLE-CRYSTALS; HOLE TRANSPORT; EXACT EXCHANGE; SMALL-POLARON AB Open shell transition metal oxides are usually described as Mott or charge transfer insulators, which are often viewed as being disparate from semiconductors. Based on the premise that the presence of a correlated gap and semiconductivity are not mutually exclusive, this work reviews electronic structure calculations on the binary 3d oxides, so to distill trends and design principles for semiconducting transition metal oxides. This class of materials possesses the potential for discovery, design, and development of novel functional semiconducting compounds, e.g. for energy applications. In order to place the 3d orbitals and the sp bands into an integrated picture, band structure calculations should treat both contributions on the same footing and, at the same time, account fully for electron correlation in the 3d shell. Fundamentally, this is a rather daunting task for electronic structure calculations, but quasi-particle energy calculations in GW approximation offer a viable approach for band structure predictions in these materials. Compared to conventional semiconductors, the inherent multivalent nature of transition metal cations is more likely to cause undesirable localization of electron or hole carriers. Therefore, a quantitative prediction of the carrier self-trapping energy is essential for the assessing the semiconducting properties and to determine whether the transport mechanism is a band-like large-polaron conduction or a small-polaron hopping conduction. An overview is given for the binary 3d oxides on how the hybridization between the 3d crystal field symmetries with the O-p orbitals of the ligands affects the effective masses and the likelihood of electron and hole self-trapping, identifying those situations where small masses and band-like conduction are more likely to be expected. The review concludes with an illustration of the implications of the increased electronic complexity of transition metal cations on the defect physics and doping, using as an example the diversity of possible atomic and magnetic configurations of the O vacancy in TiO2, and the high levels of hole doping in Co2ZnO4 due to a self-doping mechanism that originates from the multivalence of Co. C1 Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Lany, S (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM stephan.lany@nrel.gov OI Lany, Stephan/0000-0002-8127-8885 FU US Department of Energy, Office of Science, Office of Basic Energy Sciences, as part of an Energy Frontier Research Center [DE-AC36-08GO28308] FX This work was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, as part of an Energy Frontier Research Center under contract No. DE-AC36-08GO28308 to NREL. SL thanks collaborators and colleagues for fruitful discussions and interactions on transition metal oxides, including E Arca, D S Ginley, T O Mason, A R Nagaraja, PF Ndione, T R Paudel, H Peng, J D Perkins, N H Perry, K R P Poeppelmeier, V Stevanovic, M F Toney, G Trimarchi, A Zakutayev, A Zunger. NR 130 TC 11 Z9 11 U1 34 U2 156 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD JUL 22 PY 2015 VL 27 IS 28 AR 283203 DI 10.1088/0953-8984/27/28/283203 PG 18 WC Physics, Condensed Matter SC Physics GA CM2GP UT WOS:000357498200003 PM 26126022 ER PT J AU Sprague, MA Satkauskas, I AF Sprague, Michael A. Satkauskas, Ignas TI Nesting an incompressible-flow code within a compressible-flow code: A two-dimensional study SO COMPUTERS & FLUIDS LA English DT Article DE Wind energy; Multi-scale; Model coupling; Computational fluid dynamics; Numerical weather prediction ID LARGE-EDDY SIMULATION; FORECASTING-MODEL; WEATHER RESEARCH; ONE-WAY AB We consider numerical algorithms appropriate for one- and two-way coupling between meso-scale and micro-scale fluid-dynamics codes for wind energy computing. At the meso-scale is a numerical weather-prediction code, which is typically based on the compressible-flow Euler equations. At the micro-scale, surrounding one or more wind turbines, is a computational fluid dynamics code, which is typically based on the incompressible-flow Navier-Stokes equations. When calculating short-duration flow around wind turbines, one-way coupling is sufficient, where the meso-scale computational model drives the micro-scale model. However, in long-duration simulations involving large wind farms, the influence of the wind farm on the meso-scale weather may no longer be insignificant and two-way coupling is warranted. In this study, we focus on a simple two-dimensional system, for which our goal is to devise one- and two-way coupling algorithms that can effectively transport a vortex propagating in laminar flow from one domain to the other. Two coupling schemes and their numerical implementation are described: partial-boundary coupling and projection coupling. In the former, the micro-scale-domain boundary is decomposed, based on the meso-scale solution, into sections corresponding to inflow and outflow. The micro-scale model has Dirichlet- and Neumann-type boundary conditions on these sections, respectively. In projection coupling, the meso-scale solution is projected onto the incompressible-flow solution space in the micro-scale domain, from which Dirichlet-type boundary conditions are derived. In these simulations, the uncoupled meso-scale solution is taken as the reference, and the best coupling method is that which produces solutions that deviate the least from the reference. In one-way coupling, under a simple two-dimensional laminar-flow test case, partial-boundary coupling was more effective than projection coupling. However, in two-way coupling, projection coupling was the best performer. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Sprague, Michael A.; Satkauskas, Ignas] Natl Renewable Energy Lab, Computat Sci Ctr, Golden, CO 80401 USA. [Satkauskas, Ignas] Univ Colorado, Dept Appl Math, Boulder, CO 80309 USA. RP Sprague, MA (reprint author), Natl Renewable Energy Lab, Computat Sci Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM Michael.A.Sprague@nrel.gov FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory [DE-AC36-08-GO28308]; Center for Research and Education in Wind (CREW); NREL Laboratory Directed Research and Development (LDRD) program FX The authors acknowledge useful discussions with Matt Churchfield, Julie Lundquist, Pat Moriarty, and John Michalakes, and feedback from the reviewers. This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. Funding was provided in part by a grant from the Center for Research and Education in Wind (CREW), and the NREL Laboratory Directed Research and Development (LDRD) program. NR 32 TC 0 Z9 0 U1 0 U2 0 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0045-7930 EI 1879-0747 J9 COMPUT FLUIDS JI Comput. Fluids PD JUL 22 PY 2015 VL 115 BP 75 EP 85 DI 10.1016/j.compfluid.2015.03.005 PG 11 WC Computer Science, Interdisciplinary Applications; Mechanics SC Computer Science; Mechanics GA CJ8SL UT WOS:000355773700007 ER PT J AU Simon, G Nadiga, BT AF Simon, Guillaume Nadiga, Balasubramanya T. TI Instability of a periodic flow in geostrophic and hydrostatic balance SO COMPUTERS & FLUIDS LA English DT Article DE Baroclinic instability; Quasi-geostrophic turbulence; Rotating flows; Stratified flows; Unbalanced instability ID KINETIC-ENERGY SPECTRA; SHEAR FLOWS; BAROCLINIC INSTABILITY; ATMOSPHERE; OCEAN; PREDICTABILITY; SIMULATIONS; DISSIPATION; TURBULENCE; MESOSCALE AB Instability of a flow in geostrophic and hydrostatic balance is investigated using numerical simulations of the fully nonlinear, rotating, stratified Boussinesq equations. Burger numbers less than one and small aspect ratio are considered. Although the model we consider has continuous stratification in the vertical, in terms of phenomenology, the large scale baroclinic instability we find is most closely related to that found in the classical setting of Eady 1949 [8]. Indeed, the growth rate and scale of the most unstable mode scale similarly. The advantage of the model we consider lies in being able to use it in studies of unbalanced processes. Preliminary experimentation suggests that there is a small scale instability at small values of Burger number. This instability is initiated in anticyclonic regions, is likely imbalanced, and likely leads to small scale dissipation. By considering two measures of balance one based on a wave-vortex decomposition and another based on the quasi-geostrophic omega equation we study the dependence of imbalance on Rossby number. We, however, find that kinetic energy spectra display slopes consistent with quasi-geostrophic turbulence, with no break in slope at high wavenumbers. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Simon, Guillaume; Nadiga, Balasubramanya T.] Los Alamos Natl Lab, Comp Computat & Stat Sci Div, Los Alamos, NM 87544 USA. RP Simon, G (reprint author), Los Alamos Natl Lab, Comp Computat & Stat Sci Div, Los Alamos, NM 87544 USA. EM gsimon@lanl.gov; balu@lanl.gov FU Laboratory Directed Research and Development (LDRD) program at Los Alamos National Laboratory [20110150ER] FX This research was supported by the Laboratory Directed Research and Development (LDRD) program at Los Alamos National Laboratory (Project No. 20110150ER). Computational resources were provided by Institutional Computing at the Los Alamos National Laboratory. NR 38 TC 0 Z9 0 U1 1 U2 7 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0045-7930 EI 1879-0747 J9 COMPUT FLUIDS JI Comput. Fluids PD JUL 22 PY 2015 VL 115 BP 173 EP 191 DI 10.1016/j.compfluid.2015.03.014 PG 19 WC Computer Science, Interdisciplinary Applications; Mechanics SC Computer Science; Mechanics GA CJ8SL UT WOS:000355773700014 ER PT J AU Bertram, E Klessen, RS Glover, SCO AF Bertram, Erik Klessen, Ralf S. Glover, Simon C. O. TI Structure analysis of simulated molecular clouds with the Delta-variance SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE ISM: clouds; ISM: molecules; galaxies: ISM ID PRINCIPAL COMPONENT ANALYSIS; SUPERSONIC ISOTHERMAL TURBULENCE; FULLY-DEVELOPED TURBULENCE; MODELING CO EMISSION; GALACTIC RING SURVEY; INTERSTELLAR TURBULENCE; STAR-FORMATION; VELOCITY CENTROIDS; POWER SPECTRUM; GRAVITATIONAL COLLAPSE AB We employ the Delta-variance analysis and study the turbulent gas dynamics of simulated molecular clouds (MCs). Our models account for a simplified treatment of time-dependent chemistry and the non-isothermal nature of the gas. We investigate simulations using three different initial mean number densities of n(0) = 30, 100 and 300 cm(-3) that span the range of values typical for MCs in the solar neighbourhood. Furthermore, we model the CO line emission in a post-processing step using a radiative transfer code. We evaluate Delta-variance spectra for centroid velocity (CV) maps as well as for integrated intensity and column density maps for various chemical components: the total, H-2 and (CO)-C-12 number density and the integrated intensity of both the (CO)-C-12 and (CO)-C-13 (J = 1 -> 0) lines. The spectral slopes of the Delta-variance computed on the CV maps for the total and H-2 number density are significantly steeper compared to the different CO tracers. We find slopes for the linewidth-size relation ranging from 0.4 to 0.7 for the total and H2 density models, while the slopes for the various CO tracers range from 0.2 to 0.4 and underestimate the values for the total and H-2 density by a factor of 1.5-3.0. We demonstrate that optical depth effects can significantly alter the Delta-variance spectra. Furthermore, we report a critical density threshold of similar to 100 cm(-3) at which the Delta-variance slopes of the various CO tracers change sign. We thus conclude that carbon monoxide traces the total cloud structure well only if the average cloud density lies above this limit. C1 [Bertram, Erik; Klessen, Ralf S.; Glover, Simon C. O.] Heidelberg Univ, Inst Theoret Astrophys, Zentrum Astron, D-69120 Heidelberg, Germany. [Klessen, Ralf S.] Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 95064 USA. [Klessen, Ralf S.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, SLAC, Menlo Pk, CA 94025 USA. RP Bertram, E (reprint author), Heidelberg Univ, Inst Theoret Astrophys, Zentrum Astron, Albert Ueberle Str 2, D-69120 Heidelberg, Germany. EM bertram@zah.uni-heidelberg.de FU Deutsche Forschungsgemeinschaft (DFG) [SFB 881]; SPP (priority program) 1573; Konrad-Adenauer-Stiftung (KAS) via their 'Promotionsforderung'; Teragrid [TG-MCA995024]; DFG via Emmy-Noether grant [BA 3706]; DFG via Frontier grant of Heidelberg University - German Excellence Initiative; Baden-Wurttemberg Foundation; European Research Council under the European Community [339177] FX We thank Volker Ossenkopf for informative discussions about the usage of the Delta-variance and for providing his IDL routines in order to compute the Delta-variance spectra. We also thank Lukas Konstandin for stimulating discussions about the theory of turbulence as well as the referee for a very constructive and detailed report, which helped to improve the paper. EB, SCOG and RSK acknowledge support from the Deutsche Forschungsgemeinschaft (DFG) via the SFB 881 (sub-projects B1, B2, B5 and B8) 'The Milky Way System', and the SPP (priority program) 1573, 'Physics of the ISM'. Furthermore, EB acknowledges financial support from the Konrad-Adenauer-Stiftung (KAS) via their 'Promotionsforderung'. Some of the simulations presented in this paper were performed using the Ranger cluster at the Texas Advanced Computing Center, using time allocated as part of Teragrid project TG-MCA995024. Additional simulations were performed on the kolob cluster at the University of Heidelberg, which is funded in part by the DFG via Emmy-Noether grant BA 3706, and via a Frontier grant of Heidelberg University, sponsored by the German Excellence Initiative as well as the Baden-Wurttemberg Foundation. RSK acknowledges support from the European Research Council under the European Community's Seventh Framework Programme (FP7/2007-2013) via the ERC Advanced Grant 'STARLIGHT: Formation of the First Stars' (project number 339177). NR 83 TC 2 Z9 2 U1 1 U2 2 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD JUL 21 PY 2015 VL 451 IS 1 BP 196 EP 209 DI 10.1093/mnras/stv948 PG 14 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CQ8AH UT WOS:000360827800016 ER PT J AU Baron, D Poznanski, D Watson, D Yao, YS Cox, NLJ Prochaska, JX AF Baron, Dalya Poznanski, Dovi Watson, Darach Yao, Yushu Cox, Nick L. J. Prochaska, J. Xavier TI Using Machine Learning to classify the diffuse interstellar bands SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE techniques: spectroscopic; surveys; dust, extinction; ISM: general; ISM: lines and bands; ISM: molecules ID HIGH-RESOLUTION PROFILES; MAGELLANIC CLOUDS; 6196 ANGSTROM; MOLECULES; FAMILIES; CARRIERS; MAPS; SPECTROSCOPY; SPECTRA; SODIUM AB Using over a million and a half extragalactic spectra from the Sloan Digital Sky Survey we study the correlations of the diffuse interstellar bands (DIBs) in the Milky Way. We measure the correlation between DIB strength and dust extinction for 142 DIBs using 24 stacked spectra in the reddening range E(B - V) < 0.2, many more lines than ever studied before. Most of the DIBs do not correlate with dust extinction. However, we find 10 weak and barely studied DIBs with correlations that are higher than 0.7 with dust extinction and confirm the high correlation of additional five strong DIBs. Furthermore, we find a pair of DIBs, 5925.9 and 5927.5 angstrom, which exhibits significant negative correlation with dust extinction, indicating that their carrier may be depleted on dust. We use Machine Learning algorithms to divide the DIBs to spectroscopic families based on 250 stacked spectra. By removing the dust dependence, we study how DIBs follow their local environment. We thus obtain six groups of weak DIBs, four of which are tightly associated with C-2 or CN absorption lines. C1 [Baron, Dalya; Poznanski, Dovi] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Watson, Darach] Univ Copenhagen, Niels Bohr Inst, Dark Cosmol Ctr, DK-2100 Copenhagen, Denmark. [Yao, Yushu] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Cox, Nick L. J.] Univ Toulouse, UPS OMP, IRAP, F-31028 Toulouse, France. [Cox, Nick L. J.] CNRS, IRAP, F-31028 Toulouse, France. [Prochaska, J. Xavier] Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 95064 USA. [Prochaska, J. Xavier] Univ Calif Santa Cruz, UCO Lick Observ, Santa Cruz, CA 95064 USA. RP Baron, D (reprint author), Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. EM dalyabaron@mail.tau.ac.il; dovi@tau.ac.il OI Watson, Darach/0000-0002-4465-8264 FU Alon fellowship for outstanding young researchers; Raymond and Beverly Sackler Chair for young scientists; Danish National Research Foundation; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Alfred P. Sloan Foundation; National Science Foundation; U.S. Department of Energy Office of Science; University of Arizona; Brazilian Participation Group; Brookhaven National Laboratory; Carnegie Mellon University; University of Florida; French Participation Group; German Participation Group; Harvard University; Instituto de Astrofisica de Canarias; Michigan State/Notre Dame/JINA Participation Group; Johns Hopkins University; Lawrence Berkeley National Laboratory; Max Planck Institute for Astrophysics; Max Planck Institute for Extraterrestrial Physics; New Mexico State University; New York University; Ohio State University; Pennsylvania State University; University of Portsmouth; Princeton University; Spanish Participation Group; University of Tokyo; University of Utah; Vanderbilt University; University of Virginia; University of Washington; Yale University FX DP acknowledges the support of the Alon fellowship for outstanding young researchers, and of the Raymond and Beverly Sackler Chair for young scientists. DB and DP thank the Dark Cosmology Center which is funded by the Danish National Research Foundation for hosting them while working on this topic.; The bulk of our computations was performed on the resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, using the open source scientific data base SciDB.2 The spectroscopic analysis was made using IPython (Perez & Granger 2007). We also used these Python packages: pyspeckit,3 healpy4 and astropy.5; This work made extensive use of SDSS-III6 data. Funding for SDSS-III has been provided by the Alfred P. Sloan Foundation, the Participating Institutions, the National Science Foundation, and the U.S. Department of Energy Office of Science. SDSS-III is managed by the Astrophysical Research Consortium for the Participating Institutions of the SDSS-III Collaboration including the University of Arizona, the Brazilian Participation Group, Brookhaven National Laboratory, Carnegie Mellon University, University of Florida, the French Participation Group, the German Participation Group, Harvard University, the Instituto de Astrofisica de Canarias, the Michigan State/Notre Dame/JINA Participation Group, Johns Hopkins University, Lawrence Berkeley National Laboratory, Max Planck Institute for Astrophysics, Max Planck Institute for Extraterrestrial Physics, New Mexico State University, New York University, Ohio State University, Pennsylvania State University, University of Portsmouth, Princeton University, the Spanish Participation Group, University of Tokyo, University of Utah, Vanderbilt University, University of Virginia, University of Washington and Yale University. NR 60 TC 3 Z9 3 U1 0 U2 2 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD JUL 21 PY 2015 VL 451 IS 1 BP 332 EP 352 DI 10.1093/mnras/stv977 PG 21 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CQ8AH UT WOS:000360827800028 ER PT J AU Allison, R Lindsay, SN Sherwin, BD de Bernardis, F Bond, JR Calabrese, E Devlin, MJ Dunkley, J Gallardo, P Henderson, S Hincks, AD Hlozek, R Jarvis, M Kosowsky, A Louis, T Madhavacheril, M McMahon, J Moodley, K Naess, S Newburgh, L Niemack, MD Page, LA Partridge, B Sehgal, N Spergel, DN Staggs, ST van Engelen, A Wollack, EJ AF Allison, Rupert Lindsay, Sam N. Sherwin, Blake D. de Bernardis, Francesco Bond, J. Richard Calabrese, Erminia Devlin, Mark J. Dunkley, Joanna Gallardo, Patricio Henderson, Shawn Hincks, Adam D. Hlozek, Renee Jarvis, Matt Kosowsky, Arthur Louis, Thibaut Madhavacheril, Mathew McMahon, Jeff Moodley, Kavilan Naess, Sigurd Newburgh, Laura Niemack, Michael D. Page, Lyman A. Partridge, Bruce Sehgal, Neelima Spergel, David N. Staggs, Suzanne T. van Engelen, Alexander Wollack, Edward J. TI The Atacama Cosmology Telescope: measuring radio galaxy bias through cross-correlation with lensing SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE large-scale structure of Universe-radio continuum: galaxies ID MICROWAVE BACKGROUND POLARIZATION; ACTIVE GALACTIC NUCLEI; LARGE-SCALE BIAS; VLA SKY SURVEY; K-Z RELATION; DARK-MATTER; 1ST SURVEY; LUMINOSITY FUNCTIONS; CONTINUUM SURVEYS; REDSHIFT CUTOFF AB We correlate the positions of radio galaxies in the FIRST survey with the cosmic microwave background lensing convergence estimated from the Atacama Cosmology Telescope over 470 deg(2) to determine the bias of these galaxies. We remove optically cross-matched sources below redshift z = 0.2 to preferentially select active galactic nuclei (AGN). We measure the angular cross-power spectrum C-t(kg) at 4.4 sigma significance in the multipole range 100 < 1 < 3000, corresponding to physical scales within approximate to 2-60 Mpc at an effective redshift z(eff) = 1.5. Modelling the AGN population with a redshift-dependent bias, the cross-spectrum is well fitted by the Planck best-fitting A cold dark matter cosmological model. Fixing the cosmology and assumed redshift distribution of sources, we fit for the overall bias model normalization, finding b(z(eff)) = 3.5 +/- 0.8 for the full galaxy sample and b(z(eff)) = 4.0 +/- 1.1(3.0 +/- 1.1) for sources brighter (fainter) than 2.5 mJy. This measurement characterizes the typical halo mass of radio-loud AGN: we find log (M-halo/M-circle dot) = 13.6(-0.4)(+0.3). C1 [Allison, Rupert; Lindsay, Sam N.; Calabrese, Erminia; Dunkley, Joanna; Jarvis, Matt; Louis, Thibaut; Naess, Sigurd] Univ Oxford, Subdept Astrophys, Oxford OX1 3RH, England. [Sherwin, Blake D.] Univ Calif Berkeley, Berkeley Ctr Cosmol Phys, LBL, Berkeley, CA 94720 USA. [Sherwin, Blake D.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [de Bernardis, Francesco; Gallardo, Patricio; Henderson, Shawn; Niemack, Michael D.] Cornell Univ, Dept Phys, Ithaca, NY 14853 USA. [Bond, J. Richard; van Engelen, Alexander] Univ Toronto, Canadian Inst Theoret Astrophys, Toronto, ON M5S 3H8, Canada. [Devlin, Mark J.] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. [Hincks, Adam D.] Univ British Columbia, Dept Phys & Astron, Vancouver, BC V6T 1Z4, Canada. [Hlozek, Renee; Spergel, David N.] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA. [Jarvis, Matt] Univ Western Cape, Dept Phys, ZA-7535 Bellville, South Africa. [Kosowsky, Arthur] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Madhavacheril, Mathew; Sehgal, Neelima] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [McMahon, Jeff] Univ Michigan, Dept Phys, Ann Arbor, MI 48103 USA. [Moodley, Kavilan] Univ KwaZulu Natal, Astrophys & Cosmol Res Unit, Sch Math Stat & Comp Sci, ZA-4041 Durban, South Africa. [Newburgh, Laura] Univ Toronto, Dunlap Inst Astron & Astrophys, Toronto, ON M5S 3H4, Canada. [Page, Lyman A.; Staggs, Suzanne T.] Princeton Univ, Joseph Henry Labs Phys, Princeton, NJ 08544 USA. [Partridge, Bruce] Haverford Coll, Dept Phys & Astron, Haverford, PA 19041 USA. [Wollack, Edward J.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Allison, R (reprint author), Univ Oxford, Subdept Astrophys, Denys Wilkinson Bldg, Oxford OX1 3RH, England. EM rupert.allison@astro.ox.ac.uk RI DE BERNARDIS, FLAVIA/C-9589-2016; Wollack, Edward/D-4467-2012 OI DE BERNARDIS, FLAVIA/0000-0001-9440-8629; Wollack, Edward/0000-0002-7567-4451 FU STFC PhD studentship; US National Science Foundation [AST-0408698, AST-0965625, PHY-0855887, PHY-1214379]; Princeton University; University of Pennsylvania; Cornell University; Canada Foundation for Innovation (CFI); Comision Nacional de Investigacion Cientifica y Tecnologica de Chile (CONICYT); CFI under Compute Canada; Government of Ontario; Ontario Research Fund; University of Toronto; NASA [NNX13AE56G, NNX14AB58G]; ERC [259505]; CONICYT [QUIMAL-120001, FONDECYT-1141113]; Misrahi research fund; Wilkinson research fund FX RA is supported by an STFC PhD studentship. This work was supported by the US National Science Foundation through awards AST-0408698 and AST-0965625 for the ACT project, as well as awards PHY-0855887 and PHY-1214379. Funding was also provided by Princeton University, the University of Pennsylvania, Cornell University and a Canada Foundation for Innovation (CFI) award to UBC. ACT operates in the Parque Astronomic Atacama in Northern Chile under the auspices of the Comision Nacional de Investigacion Cientifica y Tecnologica de Chile (CONICYT). Computations were performed on the GPC supercomputer at the SciNet HPC Consortium. SciNet is funded by the CFI under the auspices of Compute Canada, the Government of Ontario, the Ontario Research Fund 1/2 Research Excellence and the University of Toronto. The development of multichroic detectors and lenses was supported by NASA grants NNX13AE56G and NNX14AB58G. Funding from ERC grant 259505 supports SN, JD and TL. RD was supported by CONICYT grants QUIMAL-120001 and FONDECYT-1141113. We gratefully acknowledge support from the Misrahi and Wilkinson research funds. NR 84 TC 9 Z9 9 U1 0 U2 2 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD JUL 21 PY 2015 VL 451 IS 1 BP 849 EP 858 DI 10.1093/mnras/stv991 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CQ8AH UT WOS:000360827800064 ER PT J AU Zdziarski, AA Sikora, M Pjanka, P Tchekhovskoy, A AF Zdziarski, Andrzej A. Sikora, Marek Pjanka, Patryk Tchekhovskoy, Alexander TI Core shifts, magnetic fields and magnetization of extragalactic jets SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE acceleration of particles; magnetic fields; radiation mechanisms: non-thermal; ISM: jets and outflows; galaxies: jets; quasars: general ID ACTIVE GALACTIC NUCLEI; RELATIVISTIC JETS; BLACK-HOLES; X-RAY; LUMINOUS BLAZARS; KINETIC-ENERGY; RADIO-SOURCES; M87 JET; ACCRETION; TRANSITION AB We study the effect of radio-jet core shift, which is a dependence of the position of the jet radio core on the observational frequency. We derive a new method of measuring the jet magnetic field based on both the value of the shift and the observed radio flux, which complements the standard method that assumes equipartition. Using both methods, we re-analyse the blazar sample of Zamaninasab et al. We find that equipartition is satisfied only if the jet opening angle in the radio core region is close to the values found observationally, similar or equal to 0.1-0.2 divided by the bulk Lorentz factor, Gamma(j). Larger values, e.g. 1 /Gamma(i), would imply magnetic fields much above equipartition. A small jet opening angle implies in turn the magnetization parameter of << 1. We determine the jet magnetic flux taking into account this effect. We find that the transverse-averaged jet magnetic flux is fully compatible with the model of jet formation due to black hole (BH) spin-energy extraction and the accretion being a magnetically arrested disc (MAD). We calculate the jet average mass-flow rate corresponding to this model and find it consists of a substantial fraction of the mass accretion rate. This suggests the jet composition with a large fraction of baryons. We also calculate the average jet power, and find it moderately exceeds the accretion power, Mc(2), reflecting BH spin energy extraction. We find our results for radio galaxies at low Eddington ratios are compatible with MADs but require a low radiative efficiency, as predicted by standard accretion models. C1 [Zdziarski, Andrzej A.; Sikora, Marek; Pjanka, Patryk] Cent Astron M Kopernika, PL-00716 Warsaw, Poland. [Pjanka, Patryk] Uniwersytetu Warszawskiego, Obserwatorium Astron, PL-00478 Warsaw, Poland. [Tchekhovskoy, Alexander] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Tchekhovskoy, Alexander] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Tchekhovskoy, Alexander] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Zdziarski, AA (reprint author), Cent Astron M Kopernika, Bartycka 18, PL-00716 Warsaw, Poland. EM aaz@camk.edu.pl OI Pjanka, Patryk/0000-0003-3564-9689 FU Polish NCN grants [2012/04/M/ST9/00780, 2013/10/M/ST9/00729, DEC-2011/01/B/ST9/04845]; NASA - Chandra X-ray Centre [PF3-140115]; NASA [NAS8-03060] FX We thank Alexander Pushkarev for help with using the radio data for blazars, Tuomas Savolainen for his kind help with the parameters of the sample of the radio galaxies of 714, and Arieh Konigl for valuable comments on this work. This research has made use of data from the MOJAVE data base that is maintained by the MOJAVE team, and it has been supported in part by the Polish NCN grants 2012/04/M/ST9/00780, 2013/10/M/ST9/00729 and DEC-2011/01/B/ST9/04845. AT was supported by NASA through Einstein Postdoctoral Fellowship grant number PF3-140115 awarded by the Chandra X-ray Centre, which is operated by the Smithsonian Astrophysical Observatory for NASA under contract NAS8-03060. NR 42 TC 10 Z9 10 U1 0 U2 2 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD JUL 21 PY 2015 VL 451 IS 1 BP 927 EP 935 DI 10.1093/mnras/st986 PG 9 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CQ8AH UT WOS:000360827800071 ER PT J AU Bouchard, KE Ganguli, S Brainard, MS AF Bouchard, Kristofer E. Ganguli, Surya Brainard, Michael S. TI Role of the site of synaptic competition and the balance of learning forces for Hebbian encoding of probabilistic Markov sequences SO FRONTIERS IN COMPUTATIONAL NEUROSCIENCE LA English DT Article DE Hebbian plasticity; pre/post-synaptic; probability; sequences; birdsong ID TIMING-DEPENDENT PLASTICITY; LONG-TERM; SOMATOSENSORY CORTEX; SYNAPSES; NEURONS; RAT; POTENTIATION; HOMEOSTASIS; DEPRESSION; AMPLITUDE AB The majority of distinct sensory and motor events occur as temporally ordered sequences with rich probabilistic structure. Sequences can be characterized by the probability of transitioning from the current state to upcoming states (forward probability), as well as the probability of having transitioned to the current state from previous states (backward probability). Despite the prevalence of probabilistic sequencing of both sensory and motor events, the Hebbian mechanisms that mold synapses to reflect the statistics of experienced probabilistic sequences are not well understood. Here, we show through analytic calculations and numerical simulations that Hebbian plasticity (correlation, covariance, and STDP) with pre-synaptic competition can develop synaptic weights equal to the conditional forward transition probabilities present in the input sequence. In contrast, post-synaptic competition can develop synaptic weights proportional to the conditional backward probabilities of the same input sequence. We demonstrate that to stably reflect the conditional probability of a neuron's inputs and outputs, local Hebbian plasticity requires balance between competitive learning forces that promote synaptic differentiation and homogenizing learning forces that promote synaptic stabilization. The balance between these forces dictates a prior over the distribution of learned synaptic weights, strongly influencing both the rate at which structure emerges and the entropy of the final distribution of synaptic weights. Together, these results demonstrate a simple correspondence between the biophysical organization of neurons, the site of synaptic competition, and the temporal flow of information encoded in synaptic weights by Hebbian plasticity while highlighting the utility of balancing learning forces to accurately encode probability distributions, and prior expectations over such probability distributions. C1 [Bouchard, Kristofer E.] Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Bouchard, Kristofer E.] Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. [Ganguli, Surya] Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA. [Brainard, Michael S.] Univ Calif San Francisco, Dept Physiol, San Francisco, CA USA. [Brainard, Michael S.] Univ Calif San Francisco, Ctr Integrat Neurosci, San Francisco, CA 94143 USA. [Brainard, Michael S.] Howard Hughes Med Inst, Chevy Chase, MD USA. RP Bouchard, KE (reprint author), Lawrence Berkeley Natl Lab, Div Life Sci, 1 Cyclotron Rd,MS 977, Berkeley, CA 94720 USA. EM kristofer.bouchard@gmail.com FU NSF Graduate Research Fellowship FX We thank P. Sabes and J. Makin for helpful feedback on early versions of this manuscript. Circular network diagrams were provided by C. Swinehart, Samizdat Drafting Co. KB was funded by a NSF Graduate Research Fellowship, and a Lawrence Berkeley National Laboratory LDRD. SG would like to thank the Burroughs Wellcome, Sloan, Simons, McKnight, and James S. McDonnell Foundations. MB would like to thank NIH R01MH055987 and R01DC006636, and the Howard Hughes Medical Institute. NR 66 TC 1 Z9 1 U1 2 U2 11 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1662-5188 J9 FRONT COMPUT NEUROSC JI Front. Comput. Neurosci. PD JUL 21 PY 2015 VL 9 AR 92 DI 10.3389/fncom.2015.00092 PG 20 WC Mathematical & Computational Biology; Neurosciences SC Mathematical & Computational Biology; Neurosciences & Neurology GA CP8YA UT WOS:000360179700001 PM 26257637 ER PT J AU Pirrone, GF Vernon, BC Kent, MS Engen, JR AF Pirrone, Gregory F. Vernon, Briana C. Kent, Michael S. Engen, John R. TI Hydrogen Exchange Mass Spectrometry of Proteins at Langmuir Mono layers SO ANALYTICAL CHEMISTRY LA English DT Article ID NUCLEOTIDE EXCHANGE; CONFORMATIONAL DYNAMICS; NEUTRON REFLECTOMETRY; PHOSPHOLIPID-BILAYER; MEMBRANE-TRANSPORT; DRUG TARGETS; ARF FAMILY; HIV-1 NEF; MELITTIN; BINDING AB Hydrogen exchange (HX) mass spectrometry (MS) is valuable for providing conformational information for proteins/peptides that are very difficult to analyze with other methods such as peripheral membrane proteins and peptides that interact with membranes. We developed a new type of HX MS measurement that integrates Langmuir monolayers. A lipid monolayer was generated, a peptide or protein associated with it, and then the monolayer-associated peptide or protein was exposed to deuterium. The deuterated species was recovered from the monolayer, digested, and deuterium incorporation monitored by MS. Test peptides showed that deuterium recovery in an optimized protocol was equivalent to deuterium recovery in conventional solution HX MS. The reproducibility of the measurements was high, despite the requirement of generating a new monolayer for each deuterium labeling time. We validated that known conformational changes in the presence of a monolayer/membrane could be observed with the peptide melittin and the myristoylated protein Arf-1. Results in an accompanying paper show that the method can reveal details of conformational changes in a protein (HIV-1 Nef), which adopts a different conformation, depending on whether or not it is able to insert into the lipid layer. Overall, the HX MS Langmuir monolayer method provided new and meaningful conformational information for proteins that associate with lipid layers. The combination of HX MS results with neutron or X-ray reflection of the same proteins in Langmuir monolayers can be more informative than the isolated use of either method. C1 [Pirrone, Gregory F.; Engen, John R.] Northeastern Univ, Dept Chem & Chem Biol, Boston, MA 02115 USA. [Vernon, Briana C.; Kent, Michael S.] Sandia Natl Labs, Bioenergy & Def Technol, Albuquerque, NM 87185 USA. RP Engen, JR (reprint author), Northeastern Univ, Dept Chem & Chem Biol, 360 Huntington Ave, Boston, MA 02115 USA. EM j.engen@neu.edu FU NIH [GM086507, GM101135]; Waters Corporation; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX We gratefully acknowledge Mark Weir and Prof. Thomas E. Smithgall for cloning the Arf-1 gene into the pET-Deut vector. We also thank Prof. Thomas E. Wales for helpful discussion and critical insight with the manuscript. This work was supported by NIH Grant Nos. GM086507 and GM101135, and a research collaboration with the Waters Corporation. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration, under Contract No. DE-AC04-94AL85000. NR 55 TC 6 Z9 6 U1 3 U2 11 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD JUL 21 PY 2015 VL 87 IS 14 BP 7022 EP 7029 DI 10.1021/acs.analchem.5b01724 PG 8 WC Chemistry, Analytical SC Chemistry GA CN6PE UT WOS:000358555900008 PM 26134943 ER PT J AU Pirrone, GF Emert-Sedlak, LA Wales, TE Smithgall, TE Kent, MS Engen, JR AF Pirrone, Gregory F. Emert-Sedlak, Lori A. Wales, Thomas E. Smithgall, Thomas E. Kent, Michael S. Engen, John R. TI Membrane-Associated Conformation of HIV-1 Nef Investigated with Hydrogen Exchange Mass Spectrometry at a Langmuir Monolayer SO ANALYTICAL CHEMISTRY LA English DT Article ID CRYSTAL-STRUCTURE; DOWN-REGULATION; SH3 DOMAIN; PROTEIN; MYRISTOYLATION; ADSORPTION; NEUTRON; KINASE; DETERMINANT; CU(II)-IDA AB In the companion paper to this work, we described development of a new type of hydrogen exchange (HX) mass spectrometry (MS) measurement that integrates Langmuir monolayers. With Langmuir monolayers, the lipid packing density can be reproducibly controlled and changed as desired. Analysis of HX in proteins that may undergo conformational changes as a function of lipid packing (for example, conformational rearrangements after insertion into a lipid layer) are then possible. We previously used neutron reflection to characterize just such a conformational change in the myristoylated HIV-1 Nef protein (myrNef): at high lipid packing density, myrNef could not insert into the lipids and maintained a compact conformation adjacent to the monolayer, whereas at lower lipid packing density, myrNef was able to insert N-terminal arm residues, causing displacement of the core domain away from the monolayer. In order to locate where conformation may have been altered by lipid association, we applied the HX MS Langmuir monolayer method to myrNef associated with monolayers of packing densities identical to those used for the prior neutron reflection measurements. The results show that the N-terminal region and the C-terminal unstructured loop undergo conformational changes when associated with a low density lipid monolayer. The results are not consistent with the hypothesis of myrNef dimerization upon membrane association in the absence of other myrNef binding partners. The HX MS Langmuir monolayer method provides new and meaningful information for myrNef that helps explain necessary conformational changes required for function at the membrane. C1 [Pirrone, Gregory F.; Wales, Thomas E.; Engen, John R.] Northeastern Univ, Dept Chem & Chem Biol, Boston, MA 02115 USA. [Emert-Sedlak, Lori A.; Smithgall, Thomas E.] Univ Pittsburgh, Sch Med, Dept Microbiol & Mol Genet, Pittsburgh, PA 15219 USA. [Kent, Michael S.] Sandia Natl Labs, Bioenergy & Def Technol, Albuquerque, NM 87185 USA. RP Engen, JR (reprint author), Northeastern Univ, Dept Chem & Chem Biol, 360 Huntington Ave, Boston, MA 02115 USA. EM j.engen@neu.edu FU NIH [GM086507, GM101135, AI102724]; Waters Corporation; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94A185000] FX This work was supported by NIH Grant Nos. GM086507 and GM101135 (to J.R.E.) and AI102724 (to T.E.S.), and a research collaboration with the Waters Corporation. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration, under Contract No. DE-AC04-94A185000. NR 28 TC 2 Z9 2 U1 1 U2 8 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD JUL 21 PY 2015 VL 87 IS 14 BP 7030 EP 7035 DI 10.1021/acs.analchem.5b01725 PG 6 WC Chemistry, Analytical SC Chemistry GA CN6PE UT WOS:000358555900009 PM 26133569 ER PT J AU Zhang, LX Manard, BT Powell, BA Marcus, RK AF Zhang, Lynn X. Manard, Benjamin T. Powell, Brian A. Marcus, R. Kenneth TI Preliminary Assessment of Potential for Metal-Ligand Speciation in Aqueous Solution via the Liquid Sampling-Atmospheric Pressure Glow Discharge (LS-APGD) Ionization Source: Uranyl Acetate SO ANALYTICAL CHEMISTRY LA English DT Article ID PLASMA-MASS SPECTROMETRY; OPTICAL-EMISSION SOURCE; ELECTROSPRAY-IONIZATION; CARBOXYLATE COMPLEXES; OPERATING PARAMETERS; URANIUM; ION; WATER; METALLOMICS; SPECTRA AB The determination of metals, including the generation of metalligand speciation information, is essential across a myriad of biochemical, environmental, and industrial systems. Metal speciation is generally affected by the combination of some form of chromatographic separation (reflective of the metal-ligand chemistry) with element-specific detection for the quantification of the metal composing the chromatographic eluent. Thus, the identity of the metal-ligand is assigned by inference. Presented here, the liquid sampling-atmospheric pressure glow discharge (LS-APGD) is assessed as an ionization source for metal speciation, with the uranyl ion-acetate system used as a test system. Molecular mass spectra can be obtained from the same source by simple modification of the sustaining electrolyte solution. Specifically, chemical information pertaining to the degree of acetate complexation of uranyl ion (UO22+) is assessed as a function of pH in the spectral abundance of three metallic species: inorganic (nonligated) uranyl, UO2Ac(H2O)(n)(MeOH)(m)(+), and UO2Ac2(H2O)(n)(MeOH)(m)H+ (n = 1, 2, 3,...; m = 1, 2, 3,...). The product mass spectra are different from what are obtained from electrospray ionization sources that have been applied to this system. The resulting relationships between the speciation and pH values have been compared to calculated concentrations of the corresponding uranyl species: UO22+, UO2Ac+, UO2Ac2. The capacity for the LS-APGD to affect both atomic mass spectra and structurally significant spectra for organometallic complexes is a unique and potentially powerful combination. C1 [Zhang, Lynn X.; Marcus, R. Kenneth] Clemson Univ, Dept Chem, Clemson, SC 29634 USA. [Manard, Benjamin T.] Los Alamos Natl Lab, Chem Actinide Analyt Chem, Los Alamos, NM 87545 USA. [Powell, Brian A.] Clemson Univ, Dept Environm Engn & Earth Sci, Clemson, SC 29634 USA. RP Marcus, RK (reprint author), Clemson Univ, Dept Chem, Clemson, SC 29634 USA. EM marcusr@clemson.edu FU Defense Threat Reduction Agency [HDTRA1-14-1-0010] FX This work was supported by the Defense Threat Reduction Agency, Basic Research Award No. HDTRA1-14-1-0010, to Clemson University. NR 49 TC 5 Z9 5 U1 3 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD JUL 21 PY 2015 VL 87 IS 14 BP 7218 EP 7225 DI 10.1021/acs.analchem.5b01637 PG 8 WC Chemistry, Analytical SC Chemistry GA CN6PE UT WOS:000358555900033 PM 26134783 ER PT J AU Chen, TC Fillmore, TL Prost, SA Moore, RJ Ibrahim, YM Smith, RD AF Chen, Tsung-Chi Fillmore, Thomas L. Prost, Spencer A. Moore, Ronald J. Ibrahim, Yehia M. Smith, Richard D. TI Orthogonal Injection Ion Funnel Interface Providing Enhanced Performance for Selected Reaction Monitoring-Triple Quadrupole Mass Spectrometry SO ANALYTICAL CHEMISTRY LA English DT Article ID ATMOSPHERIC-PRESSURE; MULTICAPILLARY INLET; IONIZATION; TRANSMISSION; MS; NANOELECTROSPRAY AB The electrodynamic ion fining facilitates efficient focusing and transfer of charged particles in the higher-pressure regions (e.g., ion source interfaces) of mass spectrometers, thus providing increased sensitivity. An "off-axis" ion funnel design has been developed to reduce the source contamination and interferences from, e.g. ESI droplet residue and other poorly focused-neutral or charged particles with very high mass-to-charge ratios. In this study, a dual ion funnel interface consisting of an orthogonal higher pressure electrodynamic ion funnel (HPIF) and an ion funnel trap combined with a triple quadrupole mass spectrometer was 5 developed: and characterized. An orthogonal ion injection inlet and a repeller plate electrode was used to direct ions to ail ion funnel HPIF at a, pressure of 9-1,0 Torn Key factors for the HPIF performance-chatacterized included the effects of RF amplitude, the DC gradient, and operating pressure. Compared to the triple quadrupole Standard interface more than 4-fold improvement in the limit of detection for the direct quantitative MS analysis of low abundance peptides was observed. The sensitivity enhancement in liquid Chromatography selected reaction monitoring (LC-SRM) analyses of low abundance peptides spiked into a highly complex Mixture was also compared with that obtained using both a commercial S-lens interface and, an in-line dual-ion funnel interface: C1 [Chen, Tsung-Chi; Fillmore, Thomas L.; Prost, Spencer A.; Moore, Ronald J.; Ibrahim, Yehia M.; Smith, Richard D.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. RP Ibrahim, YM (reprint author), Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. EM yehia.ibrahim@pnnl.gov; rds@pnnl.gov RI Smith, Richard/J-3664-2012 OI Smith, Richard/0000-0002-2381-2349 FU NIH National Cancer Institute [1R33CA155252]; General Medical Sciences Proteomics Research Resource at Pacific Northwest National Laboratory (PNNL) [GM103493-12]; Laboratory Directed Research and Development Program at PNNL; Department of Energy Office of Biological and Environmental Research Genome Sciences Program under the Pan-omics program; DOE [DE-AC05-76RLO01830] FX The authors thank Dr. Tujin Shi, Dr. Ian Webb, Dr. Jonathan Cox, and Dr. Jia Guo for helpful discussions. The authors also thank Mr. Grant Fujimoto for the assistance for the data processing programming. Portions of this research were supported by the NIH National Cancer Institute (No. 1R33CA155252) and General Medical Sciences Proteomics Research Resource at Pacific Northwest National Laboratory (PNNL) (No. GM103493-12), the Laboratory Directed Research and Development Program at PNNL, and the Department of Energy Office of Biological and Environmental Research Genome Sciences Program under the Pan-omics program. All the experiments were performed in the Environmental Molecular Sciences Laboratory, a U.S. Department of Energy (DOE) national scientific user facility located at PNNL in Richland, WA. PNNL is a multiprogramming national laboratory operated by Battelle for the DOE, under Contract No. DE-AC05-76RLO01830. NR 23 TC 1 Z9 1 U1 10 U2 28 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD JUL 21 PY 2015 VL 87 IS 14 BP 7326 EP 7331 DI 10.1021/acs.analchem.5b01482 PG 6 WC Chemistry, Analytical SC Chemistry GA CN6PE UT WOS:000358555900047 PM 26107611 ER PT J AU Mascarenhas, R Thomas, PW Wu, CX Nocek, BP Hoang, QQ Liu, DL Fast, W AF Mascarenhas, Romila Thomas, Pei W. Wu, Chun-Xiang Nocek, Boguslaw P. Hoang, Quyen Q. Liu, Dali Fast, Walter TI Structural and Biochemical Characterization of AidC, a Quorum-Quenching Lactonase with Atypical Selectivity SO BIOCHEMISTRY LA English DT Article ID SIDEROPHORE BIOSYNTHETIC ENZYME; ACYL HOMOSERINE LACTONASE; BACILLUS-THURINGIENSIS; AMIDOHYDROLASE SUPERFAMILY; DIRECTED EVOLUTION; CRYSTAL-STRUCTURE; SPECIFICITY; AIIA; PROTEINS; PARAOXONASES AB Quorum-quenching catalysts are of interest for potential application as biuchemical tools for interrogating interbacterial cominunication pathways, as arttibiofonling agents, and as anti-infective agents in plants and animals. Herein, the structure and function of AidC, an N-acyl-Lhornoserine lactone (AHL) lactonase froth. Chryseobaoterium, is characterized. Steady-state kinetics show that zinc-supplemented AidC is the most efficient wild-type quorum-quenthing enzymes characterized to date,. with a k(cat)/K-M value cif approximately 2 X 10(6) M-1 s(-1) tor N-heptanoyl-L-homoserine lactone. The enzyme has stricter substrate selectivity and significantly lower K-M values (ca. 50 mu M for'preferred substrates) compared to those of typical AHL,lactonases (ca. >1 mM). X-ray crystal structures of AidC alone and with the product N-hexanoyl-L-homoSeritie, were determined at resolutions of 1.09 and 1.67 angstrom, respectively. Each structure displays as a dimer, and-climerie oligibmerization was also observed in solution by size-exclusion chromatography coupled with multiangle light scattering. The structures reveal two atypical features as, compared to previously characteriZed AHL lactonaseS: a "kinked" alpha-helix that forms part of a closed binding pocket, that provides affinity and enforces selectivity for Al-IL substrates and an active-site His substitution that is usually found, in a homologous family of phosphodiesterases. Implications for the catalytic mechanism of AHL lactonaseS are discussed. C1 [Thomas, Pei W.; Fast, Walter] Univ Texas Austin, Coll Pharm, Med Chem Div, Austin, TX 78712 USA. [Fast, Walter] Univ Texas Austin, Ctr Infect Dis, Austin, TX 78712 USA. [Mascarenhas, Romila; Liu, Dali] Loyola Univ, Dept Chem & Biochem, Chicago, IL 60660 USA. [Wu, Chun-Xiang; Hoang, Quyen Q.] Indiana Univ Sch Med, Dept Biochem & Mol Biol, Indianapolis, IN 46202 USA. [Nocek, Boguslaw P.] Argonne Natl Lab, Biosci Div, Struct Biol Ctr, Argonne, IL 60439 USA. RP Fast, W (reprint author), Univ Texas Austin, 107 W Dean Keeton St,Stop C0850,BME 6-202D, Austin, TX 78712 USA. EM dliu@luc.edu; walt.fast@austin.utexas.edu FU National Science Foundation [CHE-1308672]; Robert A. Welch Foundation [F-1572]; Loyola University Chicago; National Institutes of Health [GM111639]; U.S. Department of Energy, Office of Biological and Environmental Research [DE-AC02-06CH11357] FX This work was supported in part by National Science Foundation Grant CHE-1308672 (to W.F. and D.L.), the Robert A. Welch Foundation (Grant F-1572 to W.F.), Loyola University Chicago (to D.L.), and the National Institutes of Health (Grant GM111639 to Q.Q.H.). Results shown in this report are derived from work performed at Argonne National Laboratory, Structural Biology Center at the Advanced Photon Source. Argonne is operated by UChicago Argonne, LLC, for the U.S. Department of Energy, Office of Biological and Environmental Research, under Contract DE-AC02-06CH11357. NR 53 TC 3 Z9 3 U1 2 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD JUL 21 PY 2015 VL 54 IS 28 BP 4342 EP 4353 DI 10.1021/acs.biochem.5b00499 PG 12 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CN6OY UT WOS:000358555300008 PM 26115006 ER PT J AU Meier, PJ Cronin, KR Frost, EA Runge, TM Dale, BE Reinemann, DJ Detlor, J AF Meier, Paul J. Cronin, Keith R. Frost, Ethan A. Runge, Troy M. Dale, Bruce E. Reinemann, Douglas J. Detlor, Jennifer TI Potential for Electrified Vehicles to Contribute to US Petroleum and Climate Goals and Implications for Advanced Biofuels SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID LIFE-CYCLE ASSESSMENT; BENEFITS AB To examine the national fuel and emissions impacts from increasingly electrified light-duty transportation, we reconstructed the vehicle technology portfolios from two national vehicle studies. Using these vehicle portfolios, we normalized assumptions and examined sensitivity around the rates of electrified vehicle penetration, travel demand growth, and electricity decarbonization. We further examined the impact of substituting low-carbon advanced,cellulosic biofuels in place of petroleum. Twenty-seven scenarios were benchmarked against a 50% petroleum-reduction target and an 80% GHG-reduction target. We found that with high rates of electrification (40% of miles traveled) the petroleum-reduction benchmark could be satisfied, even with high travel demand growth. The same highly electrified scenarios, however, could not satisfy 80% GHG-reduction targets, even assuming 80% decarbonized electricity and no growth in travel demand. Regardless of precise consumer vehicle preferences, emissions are a function of the total reliance on electricity versus liquid fuels and the corresponding greenhouse gas intensities of both. We found that at a relatively high rate of electrification (40% of miles and 26% by fuel), an 80% GHG reduction could only be achieved with significant quantities of low-carbon liquid fuel in cases with low or moderate travel demand growth. C1 [Meier, Paul J.; Cronin, Keith R.; Frost, Ethan A.; Runge, Troy M.; Reinemann, Douglas J.; Detlor, Jennifer] Univ Wisconsin, Great Lakes Bioenergy Res Ctr, Madison, WI 53706 USA. [Meier, Paul J.; Cronin, Keith R.; Frost, Ethan A.; Runge, Troy M.; Reinemann, Douglas J.; Detlor, Jennifer] Univ Wisconsin, Wisconsin Energy Inst, Madison, WI 53706 USA. [Runge, Troy M.; Reinemann, Douglas J.] Univ Wisconsin, Dept Biol Syst Engn, Madison, WI 53706 USA. [Dale, Bruce E.] Michigan State Univ, Biomass Convers Res Lab, Dept Chem Engn & Mat Sci, Lansing, MI 48910 USA. [Dale, Bruce E.] Michigan State Univ, Great Lakes Bioenergy Res Ctr, Lansing, MI 48910 USA. RP Runge, TM (reprint author), Univ Wisconsin, Great Lakes Bioenergy Res Ctr, 1552 Univ Ave, Madison, WI 53706 USA. EM trunge@wisc.edu FU DOE Great Lakes Bioenergy Research Center - U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DEFC02-07ER64494]; Wisconsin Energy Institute at the University of Wisconsin-Madison FX This work was funded by DOE Great Lakes Bioenergy Research Center (www.greatlakesbioenergy.org) supported by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, through Cooperative Agreement DEFC02-07ER64494. Support was also provided by the Wisconsin Energy Institute at the University of Wisconsin-Madison. NR 37 TC 2 Z9 2 U1 4 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUL 21 PY 2015 VL 49 IS 14 BP 8277 EP 8286 DI 10.1021/acs.est.5b01691 PG 10 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CN6PY UT WOS:000358557900003 PM 26086692 ER PT J AU Frierdich, AJ Helgeson, M Liu, CS Wang, CM Rosso, KM Scherer, MM AF Frierdich, Andrew J. Helgeson, Maria Liu, Chengshuai Wang, Chongmin Rosso, Kevin M. Scherer, Michelle M. TI Iron Atom Exchange between Hematite and Aqueous Fe(II) SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID CRYSTALLINE IRON(III) OXIDES; FE ISOTOPE FRACTIONATION; MULTI-DIRECTION APPROACH; MICROBIAL REDUCTION; ELECTRON-TRANSFER; FE(II)-FE(III) ELECTRON; SURFACE CATALYSIS; WATER INTERFACE; FERROUS IRON; GOETHITE AB Aqueous Fe(II) has been shown to exchange with structural Fe(III) in goethite without any significant phase transformation. It remains unclear, however, whether aqueous Fe(II) undergoes similar exchange reactions with structural Fe(III) in hematite, a ubiquitous iron oxide mineral. Here, we use an enriched Fe-57 tracer to show that aqueous Fe(II) exchanges with structural Fe(III) in hematite at room temperature, and that the amount of exchange is influenced by particle size, pH, and Fe(II) concentration. Reaction of 80 nm-hematite (27 m(2) g(-1)) with aqueous Fe(II) at pH 7.0 for 30 days results in similar to 5% of its structural Fe(III) atoms exchanging with Fe(II) in solution, which equates to about one surface iron layer. Smaller, 50 nm-hematite particles (54 m(2) g(-1)) undergo about 25% exchange (similar to 3X surface iron) with aqueous Fe(II), demonstrating that structural Fe(III) in hematite is accessible to the fluid in the presence of Fe(II). The extent of exchange in hematite increases with pH up to 7.5 and then begins to decrease as the pH progresses to 8.0, likely due to surface site saturation by sorbed Fe(II). Similarly, when we vary the initial amount of added Fe(II), we observe decreasing amounts of exchange when aqueous Fe(II) is increased beyond surface saturation. This work shows that Fe(II) can catalyze iron atom exchange between bulk hematite and aqueous Fe(ll), despite hematite being the most thermodynamically stable iron oxide. C1 [Frierdich, Andrew J.; Helgeson, Maria; Scherer, Michelle M.] Univ Iowa, Dept Civil & Environm Engn, Iowa City, IA 52242 USA. [Frierdich, Andrew J.] Univ Wisconsin, Dept Geosci, Madison, WI 53706 USA. [Liu, Chengshuai] Guangdong Inst Ecoenvironm & Soil Sci, Guangzhou 510650, Guangdong, Peoples R China. [Wang, Chongmin; Rosso, Kevin M.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Scherer, MM (reprint author), Univ Iowa, Dept Civil & Environm Engn, Iowa City, IA 52242 USA. EM michelle-scherer@uiowa.edu RI Frierdich, Andrew/A-1596-2016 FU U.S. Department of Energy's (DOE) Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division through the Geosciences program at Pacific Northwest National Laboratory (PNNL); National Science Foundation (NSF) via an NSF Division of Earth Sciences Postdoctoral Fellowship [1347848]; Office of Biological and Environmental Research FX This research was supported by the U.S. Department of Energy's (DOE) Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division through the Geosciences program at Pacific Northwest National Laboratory (PNNL). Additional support was provided by the National Science Foundation (NSF) to A.J.F. via an NSF Division of Earth Sciences Postdoctoral Fellowship (Award No. 1347848). TEM analyses were performed using EMSL, a DOE Office of Science User Facility sponsored by the Office of Biological and Environmental Research and located at PNNL. NR 55 TC 8 Z9 9 U1 15 U2 74 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUL 21 PY 2015 VL 49 IS 14 BP 8479 EP 8486 DI 10.1021/acs.est.5b01276 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CN6PY UT WOS:000358557900025 PM 26069932 ER PT J AU Boone, EJ Laskin, A Laskin, J Wirth, C Shepson, PB Stirm, BH Pratt, KA AF Boone, Eric J. Laskin, Alexander Laskin, Julia Wirth, Christopher Shepson, Paul B. Stirm, Brian H. Pratt, Kerri A. TI Aqueous Processing of Atmospheric Organic Particles in Cloud Water Collected via Aircraft Sampling SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID IONIZATION-MASS-SPECTROMETRY; ISOPRENE-DERIVED ORGANOSULFATES; MOLECULAR CHARACTERIZATION; 2-METHYLGLYCERIC ACID; AEROSOL FORMATION; AMBIENT AEROSOL; UNITED-STATES; SOA FORMATION; PART 1; PHOTOOXIDATION AB Cloudwater and below-cloud atmospheric particle samples were collected onboard a research aircraft during the Southern Oxidant and Aerosol Study (SOAS) over a forested region of Alabama in June 2013. The organic molecular composition of the samples was studied to gain insights into the aqueous-phase processing of organic compounds within cloud droplets. High resolution mass spectrometry (HEMS) with nanospray desorption electrospray ionization (nano-DESI) and direct infusion electrospray ionization (ESI) were utilized to compare the organic composition of the particle and cloudwater samples, respectively. Isoprene and monoterpene-derived organosulfates and oligomers were identified in both the particles and cloudwater, showing the significant influence of biogenic volatile organic compound oxidation above the forested region. While the average O:C ratios of the organic compounds were similar between the atmospheric particle and doudwater samples, the chemical composition of these samples was quite different. Specifically, hydrolysis of organosulfates and formation of nitrogen-containing compounds were observed for the doudwater when compared to the atmospheric particle samples, demonstrating that cloud processing changes the composition of organic aerosol. C1 [Boone, Eric J.; Pratt, Kerri A.] Univ Michigan, Dept Chem, Ann Arbor, MI 48109 USA. [Laskin, Alexander] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA. [Laskin, Julia] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99354 USA. [Wirth, Christopher; Shepson, Paul B.] Purdue Univ, Dept Chem, W Lafayette, IN 47907 USA. [Shepson, Paul B.] Purdue Univ, Dept Earth Atmospher & Planetary Sci, W Lafayette, IN 47907 USA. [Shepson, Paul B.] Purdue Univ, Purdue Climate Change Res Ctr, W Lafayette, IN 47907 USA. [Stirm, Brian H.] Purdue Univ, Dept Aviat Technol, W Lafayette, IN 47907 USA. [Pratt, Kerri A.] Univ Michigan, Dept Earth & Environm Sci, Ann Arbor, MI 48109 USA. RP Pratt, KA (reprint author), Univ Michigan, Dept Chem, 930 North Univ Ave, Ann Arbor, MI 48109 USA. EM prattka@umich.edu RI Pratt, Kerri/F-8025-2010; Laskin, Alexander/I-2574-2012; Laskin, Julia/H-9974-2012 OI Pratt, Kerri/0000-0003-4707-2290; Laskin, Alexander/0000-0002-7836-8417; Laskin, Julia/0000-0002-4533-9644 FU NSF [AGS-1228496]; EPA [R835409]; Office of Biological and Environmental Research of the U.S Department of Energy (DOE); DOE by Battelle Memorial Institute [DE-AC06-76RL0 1830]; University of Michigan College of Literature, Science, and the Arts; Department of Chemistry FX Funding for SOAS sampling was provided by NSF (AGS-1228496) and EPA (R835409). High-resolution mass spectrometry analyses were performed at the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility located at the Pacific Northwest National Laboratory (PNNL) and sponsored by the Office of Biological and Environmental Research of the U.S Department of Energy (DOE). PNNL is operated for DOE by Battelle Memorial Institute under Contract No. DE-AC06-76RL0 1830. Travel funds to PNNL were provided by the University of Michigan College of Literature, Science, and the Arts and Department of Chemistry. NR 49 TC 6 Z9 6 U1 8 U2 70 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUL 21 PY 2015 VL 49 IS 14 BP 8523 EP 8530 DI 10.1021/acs.est.5b01639 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CN6PY UT WOS:000358557900030 PM 26068538 ER PT J AU Dixon, DR Schweiger, MJ Riley, BJ Pokorny, R Hrma, P AF Dixon, Derek R. Schweiger, Michael J. Riley, Brian J. Pokorny, Richard Hrma, Pavel TI Temperature Distribution within a Cold Cap during Nuclear Waste Vitrification SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID GLASS MELTING FURNACE; MELTER FEED; BATCH; DISSOLUTION; CONVERSION; SIMULATION; PARTICLES; DYNAMICS; QUARTZ; MODEL AB The kinetics of the feed-to-glass conversion affects the waste vitrification rate in an electric glass melter. The primary area of interest in this conversion process is the cold cap, a layer of reacting feed on top of the molten glass. The work presented here provides an experimental determination of the temperature distribution within the cold cap. Because direct measurement of the temperature field within the cold cap is impracticable, an indirect method was developed in which the textural features in a laboratory-made cold cap with a simulated high-level waste feed were mapped as a function of position using optical microscopy, scanning electron microscopy, energy dispersive spectroscopy, and X-ray diffraction. The temperature distribution within the cold cap was established by correlating microstructures of cold-cap regions with heat-treated feed samples of nearly identical structures at known temperatures. This temperature profile was compared with a mathematically simulated profile generated by a cold-cap model that has been developed to assess the rate of glass production in a melter. C1 [Dixon, Derek R.; Schweiger, Michael J.; Riley, Brian J.; Hrma, Pavel] Pacific NW Natl Lab, Richland, WA 99352 USA. [Pokorny, Richard] Univ Chem & Technol Prague, Dept Chem Engn, Tech 5, Prague 16628 6, Czech Republic. RP Dixon, DR (reprint author), Pacific NW Natl Lab, POB 999, Richland, WA 99352 USA. EM derek.dixon@pnnl.gov OI Riley, Brian/0000-0002-7745-6730 FU U.S. Department of Energy's (DOE) Waste Treatment and Immobilization Plant Federal Project Office; DOE by Battelle Memorial Institute [DE AC05 76RL0 1830]; Office of Biological and Environmental Research FX This work was supported by the U.S. Department of Energy's (DOE) Waste Treatment and Immobilization Plant Federal Project Office under the direction of Dr. Albert A. Kruger. Pacific Northwest National Laboratory (PNNL) is operated for the DOE by Battelle Memorial Institute under contract DE AC05 76RL0 1830. A portion of the research was performed at the Environmental Molecular Sciences Laboratory, a DOE Office of Science user facility sponsored by the Office of Biological and Environmental Research and located at PNNL. The authors would like to thank Shelley Carlson for mounting and polishing all specimens for SEM work, Mark Bowden for running micro-XRD on the cold-cap sample, and Dong-Sang Kim and Jaehun Chun for their help in discussions about this research. NR 30 TC 5 Z9 6 U1 2 U2 7 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUL 21 PY 2015 VL 49 IS 14 BP 8856 EP 8863 DI 10.1021/acs.est.5b00931 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CN6PY UT WOS:000358557900067 PM 26111202 ER PT J AU Preble, CV Dallmann, TR Kreisberg, NM Hering, SV Harley, RA Kirchstetter, TW AF Preble, Chelsea V. Dallmann, Timothy R. Kreisberg, Nathan M. Hering, Susanne V. Harley, Robert A. Kirchstetter, Thomas W. TI Effects of Particle Filters and Selective Catalytic Reduction on Heavy-Duty Diesel Drayage Truck Emissions at the Port of Oakland SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID ULTRAFINE PARTICLES; PARTICULATE MATTER; CALIFORNIA; EXPOSURE; VEHICLE; ENGINES; AFTERTREATMENT; REGENERATION; WATER; PM AB Effects of fleet modernization and use of diesel particle filters (DPF) and selective catalytic reduction (SCR) On heavy-duty diesel truck emissions were studied at the Port of Oakland in California. Nitrogen oxides (NOx), black carbon, (BC), particle number (PN), and size distributions were measured in the exhaust plumes of similar to 1400 drayage trucks. Average NOx, BC, and PN emission factors for newer engines (2010-2013 model years) equipped with both DPF and SCR were 69 +/- 15%; 92 +/- 32%, and 66 +/- 35% lower, respectively, than 2004-2006 engines Without these technologies. Intentional oxidation of NO to, NO2 for DPF regeneration increased tailpipe NO2 emissions, especially from older (1994-2006) engines with retrofit DPFs. Increased deployment of advanced controls has further skewed emission factor distributions; a small number of trucks emit a disproportionately large fraction of total BC and NOx. The fraction of DPP-equipped drayage trucks increased from 2 to 99% and the median engine age decreased from 11, to 6 years between 2009 and 2013. Over this period, fleet-average BC and NOx emission factors decreased by 76 +/- 22% and 53 +/- 8%, respectively. Emission changes occurred rapidly compared to what would have been observed due to natural (i.e., unforced) turnover of the Port truck fleet. These results provide a preview of more widespread emission changes expected Statewide and nationally in the coming years. C1 [Preble, Chelsea V.; Dallmann, Timothy R.; Harley, Robert A.; Kirchstetter, Thomas W.] Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA. [Kreisberg, Nathan M.; Hering, Susanne V.] Aerosol Dynam Inc, Berkeley, CA 94720 USA. [Kirchstetter, Thomas W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Harley, RA (reprint author), Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA. EM harley@ce.berkeley.edu RI Harley, Robert/C-9177-2016 OI Harley, Robert/0000-0002-0559-1917 FU California Air Resources Board (CARE) [09-340]; National Science Foundation Graduate Research Fellowship Program [1106400] FX This work was supported by the California Air Resources Board (CARE) under Contract No. 09-340 and by the National Science Foundation Graduate Research Fellowship Program under Grant No. 1106400. The statements and conclusions herein are those of the authors and do not necessarily reflect the views of the project sponsors. We thank the Bay Area Air Quality Management District for allowing us to use their mobile laboratory, TSI Inc. for loaning some CPCs, and CARE for use of their FMPS. We thank Mike Sutherland and Alicia Violet for providing truck and engine data from the Drayage Truck Registry, and Chandan Misra who served as project manager for this study. We also thank Steven DeMartini and Nick Tang for assistance with data analysis. NR 34 TC 7 Z9 7 U1 7 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUL 21 PY 2015 VL 49 IS 14 BP 8864 EP 8871 DI 10.1021/acs.est.5b01117 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CN6PY UT WOS:000358557900068 PM 26083075 ER PT J AU Austin, S Kontur, WS Ulbrich, A Oshlag, JZ Zhang, WP Higbee, A Zhang, YP Coon, JJ Hodge, DB Donohue, TJ Noguera, DR AF Austin, Samantha Kontur, Wayne S. Ulbrich, Arne Oshlag, J. Zachary Zhang, Weiping Higbee, Alan Zhang, Yaoping Coon, Joshua J. Hodge, David B. Donohue, Timothy J. Noguera, Daniel R. TI Metabolism of Multiple Aromatic Compounds in Corn Stover Hydrolysate by Rhodopseudomonas palustris SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID RHODOBACTER-SPHAEROIDES 2.4.1; P-COUMARATE DEGRADATION; SACCHAROMYCES-CEREVISIAE; ESCHERICHIA-COLI; ETHANOL-PRODUCTION; ACETIC-ACID; COENZYME-A; FERMENTATION; GROWTH; DETOXIFICATION AB Lignocellulosic biomass hydrolysates hold great potential as a feedstock for microbial biofuel production, due to their high concentration of fermentable Sugars. Present at lower concentrations are a Suite of aromatic compounds that can inhibit fermentation by biofuel-producing microbes. We have developed a microbial-mediated strategy for removing these aromatic compounds, using the purple notsulfur bacterium Rhodopseudomonas palustris, When grown photo-heterotrophically in an anaerobic environment, R. palustris removes most of the aromatics from ammonia fiber expansion (AFEX) treated corn stover hydrolysate (ACSH), while leaving the sugars mostly intact. We show that R. palustris can metabolize a host of aromatic stbstrates, in ACSH that have either been previously described as unable to support growth, such as methoxylated aromatics, and those that have not yet been tested, such as aromatic amides. Removing the aromatics from ACSH with R. palustris, allowed growth of a second microbe that could not grow in the untreated ACSH. By using defined mutants, we show that most of these aromatic compounds are metabolized by the benzoyl-CoA pathway. We also show that loss of enzymes in the benzoyl-CoA pathway prevents total degradation of the aromatics in the hydrolysate, and instead allows for biological transformation of this suite of aromatics into selected aromatic compounds potentially recoverable as an additional bioproduct C1 [Austin, Samantha; Oshlag, J. Zachary; Zhang, Weiping; Noguera, Daniel R.] Univ Wisconsin, Dept Civil & Environm Engn, Madison, WI 53706 USA. [Kontur, Wayne S.; Donohue, Timothy J.] Univ Wisconsin, Dept Bacteriol, Madison, WI 53706 USA. [Austin, Samantha; Kontur, Wayne S.; Oshlag, J. Zachary; Zhang, Weiping; Zhang, Yaoping; Coon, Joshua J.; Donohue, Timothy J.; Noguera, Daniel R.] Univ Wisconsin, DOE Great Lakes Bioenergy Res Ctr, Madison, WI 53706 USA. [Ulbrich, Arne; Higbee, Alan; Coon, Joshua J.] Univ Wisconsin, Dept Chem, Madison, WI 53706 USA. [Coon, Joshua J.] Univ Wisconsin, Dept Biomol Chem, Madison, WI 53706 USA. [Hodge, David B.] Michigan State Univ, Dept Chem Engn & Mat Sci, E Lansing, MI 48824 USA. [Hodge, David B.] Michigan State Univ, Dept Biosyst & Agr Engn, E Lansing, MI 48824 USA. RP Noguera, DR (reprint author), Univ Wisconsin, Dept Civil & Environm Engn, 1415 Engn Dr, Madison, WI 53706 USA. EM noguera@engr.wisc.edu FU US Department of Energy Great Lakes Bioenergy Research Center (DOE Office of Science) [BER DE-FC02-07ER64494]; NIGMS [T32 GM08349] FX We thank Jackie Bastyr-Cooper for assistance performing analytical tests, and facilities at MSU and UW for the production of corn stover hydrolysates. This work was funded by the US Department of Energy Great Lakes Bioenergy Research Center (DOE Office of Science BER DE-FC02-07ER64494). J. Zachary Oshlag was supported by a traineeship from the NIGMS Biotechnology Training grant (Grant T32 GM08349). We extend our thanks to Carrie S. Harwood for providing the R. palustris strains used in this study. NR 44 TC 1 Z9 1 U1 4 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUL 21 PY 2015 VL 49 IS 14 BP 8914 EP 8922 DI 10.1021/acs.est.5b02062 PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CN6PY UT WOS:000358557900074 PM 26121369 ER PT J AU Penton, CR Louis, DS Pham, A Cole, JR Wu, LY Luo, YQ Schuur, EAG Zhou, JZ Tiedje, JM AF Penton, Christopher R. Louis, Derek St. Pham, Amanda Cole, James R. Wu, Liyou Luo, Yiqi Schuur, E. A. G. Zhou, Jizhong Tiedje, James M. TI Denitrifying and diazotrophic community responses to artificial warming in permafrost and tallgrass prairie soils SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE nifH; nirK; nirS; nosZ; denitrification; climate change; permafrost; warming ID LENGTH-POLYMORPHISM ANALYSIS; LITTER DECOMPOSITION RATES; MICROBIAL COMMUNITIES; NITRITE REDUCTASE; ALASKAN TUNDRA; MARINE-SEDIMENTS; LIGNIN CONTROL; NIFH GENE; NITROGEN; ABUNDANCE AB Increasing temperatures have been shown to impact soil biogeochemical processes, although the corresponding changes to the underlying microbial functional communities are not well understood. Alterations in the nitrogen (N) cycling functional component are particularly important as N availability can affect microbial decomposition rates of soil organic matter and influence plant productivity. To assess changes in the microbial component responsible for these changes, the composition of the N-fixing (nifH), and denitrifying (nirS, nirK, nosZ) soil microbial communities was assessed by targeted pyrosequencing of functional genes involved in N cycling in two major biomes where the experimental effect of climate warming is under investigation, a tallgrass prairie in Oklahoma (OK) and the active layer above permafrost in Alaska (AK). Raw reads were processed for quality, translated with frameshift correction, and a total of 313,842 amino acid sequences were clustered and linked to a nearest neighbor using reference datasets. The number of OTUs recovered ranged from 231 (NifH) to 862 (NirK). The N functional microbial communities of the prairie, which had experienced a decade of experimental warming were the most affected with changes in the richness and/or overall structure of NifH, NirS, NirK and NosZ. In contrast, the AK permafrost communities, which had experienced only 1 year of warming, showed decreased richness and a structural change only with the nirK-harboring bacterial community. A highly divergent nirK-harboring bacterial community was identified in the permafrost soils, suggesting much novelty, while other N functional communities exhibited similar relatedness to the reference databases, regardless of site. Prairie and permafrost soils also harbored highly divergent communities due mostly to differing major populations. C1 [Penton, Christopher R.; Louis, Derek St.; Pham, Amanda; Cole, James R.; Tiedje, James M.] Michigan State Univ, Ctr Microbial Ecol, Dept Plant Soil & Microbial Sci, E Lansing, MI 48824 USA. [Penton, Christopher R.] Arizona State Univ, Coll Letters & Sci, Mesa, AZ 85212 USA. [Wu, Liyou; Zhou, Jizhong] Univ Oklahoma, Inst Environm Genom, Norman, OK 73019 USA. [Wu, Liyou; Luo, Yiqi; Zhou, Jizhong] Univ Oklahoma, Dept Microbiol & Plant Biol, Norman, OK 73019 USA. [Schuur, E. A. G.] No Arizona Univ, Ctr Ecosyst Sci & Soc, Dept Biol Sci, Flagstaff, AZ 86011 USA. [Zhou, Jizhong] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China. [Zhou, Jizhong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Penton, CR (reprint author), Arizona State Univ, Coll Letters & Sci, Arizona State Univ Polytech Campus,Mail Code 2780, Mesa, AZ 85212 USA. EM crpenton@asu.edu FU Department of Energy, Biological Systems Research on the Role of Microbial Communities in Carbon Cycling Program [DE-SC0004601]; U.S. Department of Energy Office of Science, Office of Biological and Environmental Sciences Division Terrestrial Ecosystem Sciences program [DE-SC0006982]; National Science Foundation CAREER program [0747195]; National Parks Inventory and Monitoring Program; National Science Foundation Bonanza Creek LTER program [1026415]; National Science Foundation Office of Polar Programs [1203777] FX This work is supported by the Department of Energy, Biological Systems Research on the Role of Microbial Communities in Carbon Cycling Program (DE-SC0004601). Samples were provided from field site activities supported in part by the following programs: U.S. Department of Energy Office of Science, Office of Biological and Environmental Sciences Division Terrestrial Ecosystem Sciences program, Award #DE-SC0006982; National Science Foundation CAREER program, Award #0747195; National Parks Inventory and Monitoring Program; National Science Foundation Bonanza Creek LTER program, Award #1026415; National Science Foundation Office of Polar Programs, Award #1203777. NR 59 TC 2 Z9 2 U1 13 U2 60 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD JUL 21 PY 2015 VL 6 AR 746 DI 10.3389/fmicb.2015.00746 PG 13 WC Microbiology SC Microbiology GA CN8UG UT WOS:000358719000001 PM 26284038 ER PT J AU Kumar, S Graves, CE Strachan, JP Kilcoyne, ALD Tyliszczak, T Nishi, Y Williams, RS AF Kumar, Suhas Graves, Catherine E. Strachan, John Paul Kilcoyne, A. L. David Tyliszczak, Tolek Nishi, Yoshio Williams, R. Stanley TI In-operando synchronous time-multiplexed O K-edge x-ray absorption spectromicroscopy of functioning tantalum oxide memristors SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID TRANSITION-METAL OXIDES; OXYGEN; IDENTIFICATION; SURFACES AB Memristors are receiving keen interest because of their potential varied applications and promising large-scale information storage capabilities. Tantalum oxide is a memristive material that has shown promise for high-performance nonvolatile computer memory. The microphysics has been elusive because of the small scale and subtle physical changes that accompany conductance switching. In this study, we probed the atomic composition, local chemistry, and electronic structure of functioning tantalum oxide memristors through spatially mapped O K-edge x-ray absorption. We developed a time-multiplexed spectromicroscopy technique to enhance the weak and possibly localized oxide modifications with spatial and spectral resolutions of < 30 nm and 70 meV, respectively. During the initial stages of conductance switching of a micrometer sized crosspoint device, the spectral changes were uniform within the spatial resolution of our technique. When the device was further driven with millions of high voltage-pulse cycles, we observed lateral motion and separation of similar to 100 nm-scale agglomerates of both oxygen interstitials and vacancies. We also demonstrate a unique capability of this technique by identifying the relaxation behavior in the material during electrical stimuli by identifying electric field driven changes with varying pulse widths. In addition, we show that changes to the material can be localized to a spatial region by modifying its topography or uniformity, as against spatially uniform changes observed here during memristive switching. The goal of this report is to introduce the capability of time-multiplexed x-ray spectromicroscopy in studying weak-signal transitions in inhomogeneous media through the example of the operation and temporal evolution of a memristor. (C) 2015 AIP Publishing LLC. C1 [Kumar, Suhas; Graves, Catherine E.; Strachan, John Paul; Williams, R. Stanley] Hewlett Packard Labs, Palo Alto, CA 94304 USA. [Kumar, Suhas; Nishi, Yoshio] Stanford Univ, Dept Elect Engn, Stanford, CA 94305 USA. [Kilcoyne, A. L. David; Tyliszczak, Tolek] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Strachan, JP (reprint author), Hewlett Packard Labs, 1501 Page Mill Rd, Palo Alto, CA 94304 USA. EM john-paul.strachan@hp.com RI Williams, R. Stanley/A-8281-2009; Kilcoyne, David/I-1465-2013; Kumar, Suhas/C-8061-2017; OI Williams, R. Stanley/0000-0003-0213-4259; Kumar, Suhas/0000-0002-6772-7250; Graves, Catherine/0000-0002-0907-583X FU Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231] FX X-ray measurements were performed at the Advanced Light Source at Lawrence Berkeley National Laboratory, CA, USA, at beamlines 5.3.2.2 and 11.0.2. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 33 TC 8 Z9 8 U1 5 U2 17 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 21 PY 2015 VL 118 IS 3 AR 034502 DI 10.1063/1.4926477 PG 7 WC Physics, Applied SC Physics GA CN4VT UT WOS:000358429200026 ER PT J AU Jacovella, U Holland, DMP Boye-Peronne, S Gans, B de Oliveira, N Joyeux, D Archer, LE Lucchese, RR Xu, H Pratt, ST AF Jacovella, U. Holland, D. M. P. Boye-Peronne, S. Gans, B. de Oliveira, N. Joyeux, D. Archer, L. E. Lucchese, R. R. Xu, H. Pratt, S. T. TI High-resolution vacuum-ultraviolet photoabsorption spectra of 1-butyne and 2-butyne SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID IONIZATION CROSS-SECTIONS; POLYATOMIC-MOLECULES; ELECTRONIC STATES; VUV ABSORPTION; RYDBERG SERIES; BASIS-SETS; PHOTOIONIZATION; PROPYNE; SPECTROSCOPY; THRESHOLD AB The absolute photoabsorption cross sections of 1- and 2-butyne have been recorded at high resolution by using the vacuum-ultraviolet Fourier-Transform spectrometer at the SOLEIL Synchrotron. Both spectra show more resolved structure than previously observed, especially in the case of 2-butyne. In this work, we assess the potential importance of Rydberg states with higher values of orbital angular momentum, l, than are typically observed in photoabsorption experiments from ground state molecules. We show how the character of the highest occupied molecular orbitals in 1- and 2-butyne suggests the potential importance of transitions to such high-l (l = 3 and 4) Rydberg states. Furthermore, we use theoretical calculations of the partial wave composition of the absorption cross section just above the ionization threshold and the principle of continuity of oscillator strength through an ionization threshold to support this conclusion. The new absolute photoabsorption cross sections are discussed in light of these arguments, and the results are consistent with the expectations. This type of argument should be valuable for assessing the potential importance of different Rydberg series when sufficiently accurate direct quantum chemical calculations are difficult, for example, in the n >= 5 manifolds of excited states of larger molecules. (C) 2015 AIP Publishing LLC. C1 [Jacovella, U.] ETH, Lab Phys Chem, CH-8093 Zurich, Switzerland. [Holland, D. M. P.] SERC, Daresbury Lab, STFC, Warrington WA4 4AD, Cheshire, England. [Boye-Peronne, S.; Gans, B.] CNRS, UMR 8214, Inst Sci Mol Orsay, F-91405 Orsay, France. [Boye-Peronne, S.; Gans, B.] Univ Paris 11, F-91405 Orsay, France. [de Oliveira, N.; Joyeux, D.; Archer, L. E.] Synchrotron Soleil, F-91192 Gif Sur Yvette, France. [Lucchese, R. R.] Texas A&M Univ, Dept Chem, College Stn, TX 77843 USA. [Xu, H.; Pratt, S. T.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Jacovella, U (reprint author), ETH, Lab Phys Chem, CH-8093 Zurich, Switzerland. FU Science and Technology Facilities Council, UK; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-AC02-06CH11357, DE-SC0012198]; Robert A. Welch Foundation [A-1020]; Texas A&M University Supercomputing Facility FX D.M.P.H. was supported by the Science and Technology Facilities Council, UK. This material is based on work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, respectively, under Contract Nos. DE-AC02-06CH11357 (for H.X. and S.T.P.) and DE-SC0012198 (for R.R.L.). R.R.L. also acknowledges the support of the Robert A. Welch Foundation under Grant No. A-1020. This work was supported by the Texas A&M University Supercomputing Facility. The work was performed on the DESIRS Beamline at SOLEIL under Proposal No. 20120675. We are grateful to Laurent Nahon of the DESIRS Beamline for his help and guidance and to the whole staff of SOLEIL for running the facility. NR 48 TC 3 Z9 3 U1 2 U2 20 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUL 21 PY 2015 VL 143 IS 3 AR 034304 DI 10.1063/1.4926541 PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN4VZ UT WOS:000358429800017 PM 26203024 ER PT J AU Nelson, WC Stegen, JC AF Nelson, William C. Stegen, James C. TI The reduced genomes of Parcubacteria (OD1) contain signatures of a symbiotic lifestyle SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE Parcubacteria; genomics; symbiosis; pan-genome; genome reconstruction; candidate phyla; groundwater; streamlining ID 16S RIBOSOMAL-RNA; CONSORTIUM CHLOROCHROMATIUM-AGGREGATUM; LEVEL STREPTOMYCIN RESISTANCE; CANDIDATE DIVISION OD1; ESCHERICHIA-COLI; MICROBIAL COMMUNITY; SUBSYSTEMS TECHNOLOGY; PROKARYOTIC SYMBIOSIS; UNCONFINED AQUIFER; PROTEIN FAMILIES AB Candidate phylum OD1 bacteria (also referred to as Parcubacteria) have been identified in a broad range of anoxic environments through community survey analysis. Although none of these species have been isolated in the laboratory, several genome sequences have been reconstructed from metagenomic sequence data and single-cell sequencing. The organisms have small (generally <1 Mb) genomes with severely reduced metabolic capabilities. We have reconstructed 8 partial to near-complete OD1 genomes from oxic groundwater samples, and compared them against existing genomic data. The conserved core gene set comprises 202 genes, or similar to 28% of the genomic complement. "Housekeeping" genes and genes for biosynthesis of peptidoglycan and Type IV pilus production are conserved. Gene sets for biosynthesis of cofactors, amino acids, nucleotides, and fatty acids are absent entirely or greatly reduced. The only aspects of energy metabolism conserved are the non-oxidative branch of the pentose-phosphate shunt and central glycolysis. These organisms also lack some activities conserved in almost all other known bacterial genomes, including signal recognition particle, pseudouridine synthase A, and FAD synthase. Pan-genome analysis indicates a broad genotypic diversity and perhaps a highly fluid gene complement, indicating historical adaptation to a wide range of growth environments and a high degree of specialization. The genomes were examined for signatures suggesting either a free-living, streamlined lifestyle, or a symbiotic lifestyle. The lack of biosynthetic capabilities and DNA repair, along with the presence of potential attachment and adhesion proteins suggest that the Parcubacteria are ectosymbionts or parasites of other organisms. The wide diversity of genes that potentially mediate cell-cell contact suggests a broad range of partner/prey organisms across the phylum. C1 [Nelson, William C.; Stegen, James C.] Pacific NW Natl Lab, Div Biol Sci, Microbiol, Richland, WA 99352 USA. RP Nelson, WC (reprint author), Pacific NW Natl Lab, Div Biol Sci, Microbiol, 902 Battelle Blvd,POB 999,MSIN J4 18, Richland, WA 99352 USA. EM william.nelson@pnnl.gov RI Nelson, William/E-9263-2016; Stegen, James/Q-3078-2016 OI Nelson, William/0000-0002-1873-3929; Stegen, James/0000-0001-9135-7424 FU US Department of Energy (DOE), Office of Biological and Environmental Research (BER), as part of Subsurface Biogeochemistry Research Program's Scientific Focus Area (SFA); Integrated Field-Scale Research Challenge (IFRC) at the Pacific Northwest National Laboratory (PNNL); Battelle [DE-AC06-76RLO 1830] FX The authors would like to thank Sarah Fansler and David Kennedy for sampling and sample preparation, and Allan Konopka, Jim Fredrickson, Margie Romine, and Mike Wilkins for their helpful discussions related to this work and manuscript. This research was supported by the US Department of Energy (DOE), Office of Biological and Environmental Research (BER), as part of Subsurface Biogeochemistry Research Program's Scientific Focus Area (SFA) and Integrated Field-Scale Research Challenge (IFRC) at the Pacific Northwest National Laboratory (PNNL). PNNL is operated for DOE by Battelle under contract DE-AC06-76RLO 1830. NR 74 TC 23 Z9 23 U1 7 U2 28 PU FRONTIERS RESEARCH FOUNDATION PI LAUSANNE PA PO BOX 110, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD JUL 21 PY 2015 VL 6 AR 713 DI 10.3389/fmicb.2015.00713 PG 14 WC Microbiology SC Microbiology GA CN8TU UT WOS:000358717500001 PM 26257709 ER PT J AU Jaiswal, A Podlesynak, A Ehlers, G Mills, R O'Keeffe, S Stevick, J Kempton, J Jelbert, G Dmowski, W Lokshin, K Egami, T Zhang, Y AF Jaiswal, Abhishek Podlesynak, Andrey Ehlers, Georg Mills, Rebecca O'Keeffe, Stephanie Stevick, Joseph Kempton, James Jelbert, Glenton Dmowski, Wojciech Lokshin, Konstantin Egami, Takeshi Zhang, Yang TI Coincidence of collective relaxation anomaly and specific heat peak in a bulk metallic glass-forming liquid SO PHYSICAL REVIEW B LA English DT Article ID MODE-COUPLING-THEORY; INTERMEDIATE SCATTERING FUNCTION; LENNARD-JONES MIXTURE; CU-ZR-AL; NEUTRON-SCATTERING; SUPERCOOLED LIQUIDS; PHASE-TRANSITION; BETA-RELAXATION; DYNAMICS; ALLOYS AB The study of relaxational behavior of multicomponent metallic liquids still holds the key to understanding and improving the glass-forming abilities of bulk metallic glasses. Herein, we report measurements of the collective relaxation times in a melted bulk metallic glass (LM601 Zr51Cu36Ni4Al9) in the kinetic regime (Q: 1.5-4.0 angstrom(-1)) using quasielastic neutron scattering. The results reveal an unusual slope change in the Angell plots of the collective relaxation time of this metallic liquid around 950 degrees C, beyond the melting point of the material. Specific heat capacity measurement also reveals the presence of a peak around the same temperature. The coincidence is rationalized using Adams-Gibbs theory, and motivates more careful experimental and computational studies of the metallic liquids in the future. C1 [Jaiswal, Abhishek; Zhang, Yang] Univ Illinois, Dept Nucl Plasma & Radiol Engn, Urbana, IL 61801 USA. [Podlesynak, Andrey; Ehlers, Georg; Mills, Rebecca] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [O'Keeffe, Stephanie; Stevick, Joseph; Kempton, James; Jelbert, Glenton] Liquidmetal Technol, Rancho Santa Margarita, CA 92688 USA. [Dmowski, Wojciech; Lokshin, Konstantin; Egami, Takeshi] Univ Tennessee, Dept Mat Sci & Engn, Dept Phys & Astron, Knoxville, TN 37996 USA. [Zhang, Yang] Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USA. RP Zhang, Y (reprint author), Univ Illinois, Dept Nucl Plasma & Radiol Engn, Urbana, IL 61801 USA. EM zhyang@illinois.edu RI Zhang, Yang/A-7975-2012; Instrument, CNCS/B-4599-2012; Ehlers, Georg/B-5412-2008; Podlesnyak, Andrey/A-5593-2013 OI Zhang, Yang/0000-0002-7339-8342; Ehlers, Georg/0000-0003-3513-508X; Podlesnyak, Andrey/0000-0001-9366-6319 FU NRC [NRC-HQ-12-G-38-0072]; UIUC Campus Research Board [RB14187]; U.S. Department of Energy, Office of Sciences, Basic Energy Sciences, Materials Science and Engineering Division; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy FX Y.Z. is supported by NRC faculty development Grant No. NRC-HQ-12-G-38-0072 and UIUC Campus Research Board Grant No. RB14187. Y.Z. and T.E. are supported by the U.S. Department of Energy, Office of Sciences, Basic Energy Sciences, Materials Science and Engineering Division. Part of the Research conducted at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. We thank Professor Brent Heuser and Peter Mouche at UIUC for their help with the DSC and TGA measurements using alumina cell, and Professor James F. Stubbins and Kuan-Che Lan for help with cutting the samples using diamond saw. NR 51 TC 1 Z9 1 U1 5 U2 28 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 21 PY 2015 VL 92 IS 2 AR 024202 DI 10.1103/PhysRevB.92.024202 PG 6 WC Physics, Condensed Matter SC Physics GA CN2MF UT WOS:000358254900003 ER PT J AU Perez-Morelo, DJ Osquiguil, E Kolton, AB Nieva, G Jung, IW Lopez, D Pastoriza, H AF Perez-Morelo, D. J. Osquiguil, E. Kolton, A. B. Nieva, G. Jung, I. W. Lopez, D. Pastoriza, H. TI Thermodynamic evidence for the Bose glass transition in twinned YBa2Cu3O7-delta crystals SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTORS; SINGLE-CRYSTALS; MAGNETIC-FIELDS; CASIMIR FORCE; LOCALIZATION; BOUNDARIES; VORTICES AB We used a micromechanical torsional oscillator to measure the magnetic response of a twinned YBa2Cu3O7-delta single crystal disk near the Bose glass transition. We observe an anomaly in the temperature dependence of the magnetization consistent with the appearance of a magnetic shielding perpendicular to the correlated pinning of the twin boundaries. This effect is related to the thermodynamic transition from the vortex liquid phase to a Bose glass state. C1 [Perez-Morelo, D. J.; Osquiguil, E.; Nieva, G.; Pastoriza, H.] Comis Nacl Energia Atom, Ctr Atom Bariloche, Lab Bajas Temp, San Carlos De Bariloche, Argentina. [Perez-Morelo, D. J.; Osquiguil, E.; Kolton, A. B.; Nieva, G.; Pastoriza, H.] Comis Nacl Energia Atom, Inst Balseiro, San Carlos De Bariloche, Argentina. [Kolton, A. B.] Comis Nacl Energia Atom, Ctr Atom Bariloche, Teoria Mat Condensada, San Carlos De Bariloche, Argentina. [Jung, I. W.; Lopez, D.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Perez-Morelo, DJ (reprint author), Comis Nacl Energia Atom, Ctr Atom Bariloche, Lab Bajas Temp, Av Bustillo 9500, San Carlos De Bariloche, Argentina. FU Consejo Nacional de Investigaciones Cientificas y Tecnicas (CONICET); PIP, CONICET [1122008010111001]; US Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility [DE-AC02-06CH11357] FX D.J.P.-M. is supported by a fellowship of Consejo Nacional de Investigaciones Cientificas y Tecnicas (CONICET). E.O. A.B.K., G.N., and H.P. are researchers of CONICET. This work was partially supported by PIP 1122008010111001, CONICET. This work was performed, in part, at the Center for Nanoscale Materials, a US Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility under Contract No. DE-AC02-06CH11357. We thank V. Bekeris for a careful reading of the manuscript and valuable suggestions. NR 19 TC 0 Z9 0 U1 1 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUL 21 PY 2015 VL 92 IS 2 AR 020510 DI 10.1103/PhysRevB.92.020510 PG 4 WC Physics, Condensed Matter SC Physics GA CN2MF UT WOS:000358254900002 ER PT J AU Griffioen, KA Arrington, J Christy, ME Ent, R Kalantarians, N Keppel, CE Kuhn, SE Melnitchouk, W Niculescu, G Niculescu, I Tkachenko, S Zhang, J AF Griffioen, K. A. Arrington, J. Christy, M. E. Ent, R. Kalantarians, N. Keppel, C. E. Kuhn, S. E. Melnitchouk, W. Niculescu, G. Niculescu, I. Tkachenko, S. Zhang, J. TI Measurement of the EMC effect in the deuteron SO PHYSICAL REVIEW C LA English DT Article ID NEUTRON STRUCTURE-FUNCTION; CROSS-SECTIONS; ELECTRON-SCATTERING; NUCLEAR-STRUCTURE; DEPENDENCE; TARGETS; PROTON; RATIOS AB We determined the structure function ratio R-EMC(d) = F-2(d)/(F-2(n) + F-2(p)) from recently published F-2(n)/F-2(d) data taken by the BONuS experiment using CLAS at Jefferson Lab. This ratio deviates from unity, with a slope dR(EMC)(d)/dx=-0.10 +/- 0.05 in the range of Bjorken x from 0.35 to 0.7, for invariant mass W > 1.4 GeV and Q(2) > 1GeV(2). The observed EMC effect for these kinematics is consistent with conventional nuclear physics models that include off-shell corrections, as well as with empirical analyses that find the EMC effect proportional to the probability of short-range nucleon-nucleon correlations C1 [Griffioen, K. A.] Coll William & Mary, Williamsburg, VA 23187 USA. [Arrington, J.] Argonne Natl Lab, Argonne, IL 60439 USA. [Christy, M. E.; Kalantarians, N.] Hampton Univ, Hampton, VA 23668 USA. [Ent, R.; Keppel, C. E.; Melnitchouk, W.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Kuhn, S. E.] Old Dominion Univ, Norfolk, VA 23529 USA. [Niculescu, G.; Niculescu, I.] James Madison Univ, Harrisonburg, VA 22807 USA. [Tkachenko, S.; Zhang, J.] Univ Virginia, Charlottesville, VA 22901 USA. RP Griffioen, KA (reprint author), Coll William & Mary, Williamsburg, VA 23187 USA. RI Zhang, Jixie/A-1461-2016 FU United States Department of Energy (DOE) [DE-AC05-06OR23177]; DOE, Office of Science, Office of Nuclear Physics [DE-FG02-96ER40960, DE-AC02-06CH11357, DE-FG02-97ER41025, DE-FG02-96ER41003]; National Science Foundation (NSF) [PHY-1307196]; NSF [PHY-1002644, PHY-1307415] FX We thank the staff of the Jefferson Lab accelerator and Hall B for their support on the BONuS experiment. This work was supported by the United States Department of Energy (DOE) Contract No. DE-AC05-06OR23177, under which Jefferson Science Associates, LLC operates Jefferson Lab. S.K., J.A., S.T., and K.G. acknowledge support from the DOE, Office of Science, Office of Nuclear Physics, under Grants No. DE-FG02-96ER40960, No. DE-AC02-06CH11357, No. DE-FG02-97ER41025, and No. DE-FG02-96ER41003, respectively. I.N. and G.N. acknowledge support from the National Science Foundation (NSF) under Grant No. PHY-1307196. M.E.C. acknowledges support from NSF Grants No. PHY-1002644 and No. PHY-1307415. NR 50 TC 2 Z9 2 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JUL 21 PY 2015 VL 92 IS 1 AR 015211 DI 10.1103/PhysRevC.92.015211 PG 5 WC Physics, Nuclear SC Physics GA CN2MT UT WOS:000358256300005 ER PT J AU Fan, Y Iwashita, T Egami, T AF Fan, Yue Iwashita, Takuya Egami, Takeshi TI Crossover from Localized to Cascade Relaxations in Metallic Glasses SO PHYSICAL REVIEW LETTERS LA English DT Article ID VISCOPLASTIC DEFORMATION; SUPERCOOLED LIQUIDS; AMORPHOUS SOLIDS; FLOW; TRANSITION; AVALANCHES; DYNAMICS; FRACTURE; ALLOYS AB Thermally activated deformation is investigated in two metallic glass systems with different cooling histories. By probing the atomic displacements and stress changes on the potential energy landscape, two deformation modes, a localized process and cascade process, have observed. The localized deformation involves fewer than 30 atoms and appears in both systems, and its size is invariant with cooling history. However, the cascade deformation is more frequently observed in the fast quenched system than in the slowly quenched system. The origin of the cascade process in the fast quenched system is attributed to the higher density of local minima on the underlying potential energy landscape. C1 [Fan, Yue; Egami, Takeshi] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Iwashita, Takuya; Egami, Takeshi] Univ Tennessee, Joint Inst Neutron Sci, Dept Phys & Astron, Knoxville, TN 37996 USA. [Egami, Takeshi] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Fan, Y (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM fany@ornl.gov RI FAN, YUE/H-1737-2011; Iwashita, Takuya/D-2724-2009 FU Eugene P. Wigner Fellowship; U.S. Department of Energy [DEA-C05-00OR22725]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division FX We thank J. R. Morris, J. S. Langer, S. Zinkle, B. D. Wirth, and Y. Q. Cheng for thoughtful discussions. Y. F. was supported by a Eugene P. Wigner Fellowship at the Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy under Contract No. DEA-C05-00OR22725. T. I. and T. E. were supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 53 TC 18 Z9 18 U1 13 U2 72 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 21 PY 2015 VL 115 IS 4 AR 045501 DI 10.1103/PhysRevLett.115.045501 PG 5 WC Physics, Multidisciplinary SC Physics GA CN2KX UT WOS:000358251000007 PM 26252694 ER PT J AU Posen, S Valles, N Liepe, M AF Posen, S. Valles, N. Liepe, M. TI Radio Frequency Magnetic Field Limits of Nb and Nb3Sn SO PHYSICAL REVIEW LETTERS LA English DT Article ID NIOBIUM SUPERCONDUCTING CAVITIES; LOW-TEMPERATURE BAKING AB Superconducting radio frequency (srf) cavities, essential components of many large particle accelerators, rely on the metastable flux-free state of superconducting materials. In this Letter, we present results of experiments measuring the magnetic field limits of two srf materials, Nb and Nb3Sn. Resonators made using these materials were probed using both high power rf pulses and dc magnetic fields. Nb, which is the current standard material for srf cavities in applications, was found to be limited by the superheating field H-sh when prepared using methods to avoid excessive rf dissipation at high fields. Nb3Sn, which is a promising alternative material that is still in the early stages of development for srf purposes, was found to be limited between the onset field of metastability H-c1 and H-sh. Analysis of the results shows that the limitation is consistent with nucleation of flux penetration at defects in the rf layer. C1 [Posen, S.; Valles, N.; Liepe, M.] Cornell Lab Accelerator Based Sci & Educ, Ithaca, NY 14853 USA. RP Posen, S (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM sep93@cornell.edu FU NSF [PHY-0841213, PHY-1416318]; DOE [ER41628]; Alfred P. Sloan Foundation FX Work supported by NSF Career Grant No. PHY-0841213, NSF Grant No. PHY-1416318, DOE Grant No. ER41628, and the Alfred P. Sloan Foundation. NR 42 TC 4 Z9 4 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 21 PY 2015 VL 115 IS 4 AR 047001 DI 10.1103/PhysRevLett.115.047001 PG 5 WC Physics, Multidisciplinary SC Physics GA CN2KX UT WOS:000358251000010 PM 26252705 ER PT J AU Muljadi, E Yu, YH AF Muljadi, Eduard Yu, Yi-Hsiang TI Review of Marine Hydrokinetic Power Generation and Power Plant SO ELECTRIC POWER COMPONENTS AND SYSTEMS LA English DT Article DE power electronics; ocean energy; tidal; renewable energy; wave; energy storage; variable generation; ocean current; marine hydrokinetic AB Marine hydrokinetic power generation is a relatively new type of renewable generation. Its predecessors, such as wind power generation, hydropower plant generation, geothermal generation, photovoltaic generation, and solar thermal generation, have gained a lot of attention because of their successful implementation. The successful integration of renewable generation into the electric power grid has energized the power system global communities to take the lessons learned, innovations, and market structure to focus on the large potential of marine hydrokinetic to also contribute to the pool of renewable energy generation. This article covers the broad spectrum of marine hydrokinetic generation. The state of the art of power take-off will be discussed. Types of electrical generators will be presented, and the options for implementation will also be presented. C1 [Muljadi, Eduard; Yu, Yi-Hsiang] Natl Renewable Energy Lab, Golden, CO USA. RP Muljadi, E (reprint author), 15013 Denver West Pkwy, Golden, CO 80401 USA. EM Eduard.muljadi@nrel.gov FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory FX This work was supported by the U.S. Department of Energy under contract no. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. NR 30 TC 0 Z9 0 U1 3 U2 29 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 1532-5008 EI 1532-5016 J9 ELECTR POW COMPO SYS JI Electr. Power Compon. Syst. PD JUL 21 PY 2015 VL 43 IS 12 SI SI BP 1422 EP 1433 DI 10.1080/15325008.2015.1030519 PG 12 WC Engineering, Electrical & Electronic SC Engineering GA CM6MG UT WOS:000357802100008 ER PT J AU Zhou, Q Zheng, JL Onishi, S Crommie, MF Zettl, AK AF Zhou, Qin Zheng, Jinglin Onishi, Seita Crommie, M. F. Zettl, Alex K. TI Graphene electrostatic microphone and ultrasonic radio SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE radio; ultrasonics; graphene; microphone; bat ID ECHOLOCATION CALLS; MIDDLE-EAR; BATS; FREQUENCIES; RESONATORS; EVOLUTION AB We present a graphene-based wideband microphone and a related ultrasonic radio that can be used for wireless communication. It is shown that graphene-based acoustic transmitters and receivers have a wide bandwidth, from the audible region (20 similar to 20 kHz) to the ultrasonic region (20 kHz to at least 0.5 MHz). Using the graphene-based components, we demonstrate efficient high-fidelity information transmission using an ultrasonic band centered at 0.3 MHz. The graphene-based microphone is also shown to be capable of directly receiving ultrasound signals generated by bats in the field, and the ultrasonic radio, coupled to electromagnetic (EM) radio, is shown to function as a high-accuracy rangefinder. The ultrasonic radio could serve as a useful addition to wireless communication technology where the propagation of EM waves is difficult. C1 [Zhou, Qin; Zheng, Jinglin; Onishi, Seita; Crommie, M. F.; Zettl, Alex K.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Zhou, Qin; Onishi, Seita; Crommie, M. F.; Zettl, Alex K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Zhou, Qin; Onishi, Seita; Crommie, M. F.; Zettl, Alex K.] Univ Calif Berkeley, Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. [Zhou, Qin; Onishi, Seita; Crommie, M. F.; Zettl, Alex K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Zettl, AK (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM azettl@berkeley.edu RI Zettl, Alex/O-4925-2016 OI Zettl, Alex/0000-0001-6330-136X FU Office of Energy Research, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, US Department of Energy [DE-AC02-05CH11231]; Office of Naval Research [N00014-09-1066]; National Science Foundation [EEC-083819] FX This work was supported in part by the Director, Office of Energy Research, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, US Department of Energy Contract DE-AC02-05CH11231, which provided for graphene growth and characterization; Office of Naval Research Grant N00014-09-1066, which provided for graphene transfer and electrode manufacture; and by National Science Foundation Grant EEC-083819, which provided for design, construction, and testing of the device. NR 26 TC 9 Z9 9 U1 4 U2 34 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUL 21 PY 2015 VL 112 IS 29 BP 8942 EP 8946 DI 10.1073/pnas.1505800112 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CN2BJ UT WOS:000358225100055 PM 26150483 ER PT J AU Zhang, YW Lucas, JM Song, P Beberwyck, B Fu, Q Xu, WL Alivisatos, AP AF Zhang, Yuwei Lucas, J. Matthew Song, Ping Beberwyck, Brandon Fu, Qiang Xu, Weilin Alivisatos, A. Paul TI Superresolution fluorescence mapping of single-nanoparticle catalysts reveals spatiotemporal variations in surface reactivity SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE single-molecule nanocatalysis; optical superresolution imaging; photocatalysis; surface restructuring ID MOLECULAR-DYNAMICS SIMULATION; CO OXIDATION; NANOCATALYSTS; NANOCRYSTALS; MICROSCOPY; SITES; TIME; HETEROGENEITIES; PHOTOCATALYSIS; SPECTROSCOPY AB For the practical application of nanocatalysts, it is desirable to understand the spatiotemporal fluctuations of nanocatalytic activity at the single-nanoparticle level. Here we use time-lapsed superresolution mapping of single-molecule catalysis events on individual nanoparticles to observe time-varying changes in the spatial distribution of catalysis events on Sb-doped TiO2 nanorods and Au triangle nanoplates. Compared with the active sites on well-defined surface facets, the defects of the nanoparticle catalysts possess higher intrinsic reactivity but lower stability. Corners and ends are more reactive but also less stable than flat surfaces. Averaged over time, the most stable sites dominate the total apparent activity of single nanocatalysts. However, the active sites with higher intrinsic activity but lower stability show activity at earlier time points before deactivating. Unexpectedly, some active sites are found to recover their activity ("self-healing") after deactivation, which is probably due to desorption of the adsorbate. Our superresolution measurement of different types of active catalytic sites, over both space and time, leads to a more comprehensive understanding of reactivity patterns and may enable the design of new and more productive heterogeneous catalysts. C1 [Zhang, Yuwei; Song, Ping; Fu, Qiang; Xu, Weilin] Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Elect Chem, Changchun 130022, Peoples R China. [Zhang, Yuwei; Song, Ping; Fu, Qiang; Xu, Weilin] Chinese Acad Sci, Changchun Inst Appl Chem, Jilin Prov Key Lab Low Carbon Chem Power, Changchun 130022, Peoples R China. [Lucas, J. Matthew] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. [Lucas, J. Matthew; Beberwyck, Brandon; Alivisatos, A. Paul] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Beberwyck, Brandon] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Alivisatos, A. Paul] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Alivisatos, A. Paul] Univ Calif Berkeley, Kavli Energy Nano Sci Inst, Berkeley, CA 94720 USA. RP Alivisatos, AP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM weilinxu@ciac.ac.cn; alivis@berkeley.edu RI Alivisatos , Paul /N-8863-2015 OI Alivisatos , Paul /0000-0001-6895-9048 FU National Basic Research Program of China (973 Program) [2012CB932800, 2014CB932700]; National Natural Science Foundation of China [21273220, 21303180, 201422307]; The Recruitment Program of Global Youth Experts" of China; Light-Material Interactions in Energy Conversion, an Energy Frontier Research Center - US Department of Energy (DOE) Office of Science [DE-SC0001293]; DOE Office of Science Graduate Fellowship Program (DOE SCGF) [DEAC05-06OR23100] FX Work was funded by the National Basic Research Program of China (973 Program, 2012CB932800 and 2014CB932700), National Natural Science Foundation of China (21273220, 21303180, and 201422307), and "The Recruitment Program of Global Youth Experts" of China. J.M.L. is supported as part of the Light-Material Interactions in Energy Conversion, an Energy Frontier Research Center funded by the US Department of Energy (DOE) Office of Science under Contract DE-SC0001293. B.B. was supported by a Fellowship from the DOE Office of Science Graduate Fellowship Program (DOE SCGF) under Contract DEAC05-06OR23100. NR 35 TC 7 Z9 7 U1 21 U2 65 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUL 21 PY 2015 VL 112 IS 29 BP 8959 EP 8964 DI 10.1073/pnas.1502005112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CN2BJ UT WOS:000358225100058 PM 26150516 ER PT J AU Dixit, PD Pang, TY Studier, FW Maslov, S AF Dixit, Purushottam D. Pang, Tin Yau Studier, F. William Maslov, Sergei TI Recombinant transfer in the basic genome of Escherichia coli SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE E. coli evolution; basic genome; core genome; recombinant transfer; generalized transduction ID GENE-TRANSFER; MOLECULAR EVOLUTION; RESTRICTION ENZYMES; POPULATION; STRAINS; SPECIATION; INNOVATION; MUTATION; BACTERIOPHAGES; TRANSFORMATION AB An approximation to the similar to 4-Mbp basic genome shared by 32 strains of Escherichia coli representing six evolutionary groups has been derived and analyzed computationally. A multiple alignment of the 32 complete genome sequences was filtered to remove mobile elements and identify the most reliable similar to 90% of the aligned length of each of the resulting 496 basic-genome pairs. Patterns of single base-pair mutations (SNPs) in aligned pairs distinguish clonally inherited regions from regions where either genome has acquired DNA fragments from diverged genomes by homologous recombination since their last common ancestor. Such recombinant transfer is pervasive across the basic genome, mostly between genomes in the same evolutionary group, and generates many unique mosaic patterns. The six least-diverged genome pairs have one or two recombinant transfers of length similar to 40-115 kbp (and few if any other transfers), each containing one or more gene clusters known to confer strong selective advantage in some environments. Moderately diverged genome pairs (0.4-1% SNPs) show mosaic patterns of interspersed clonal and recombinant regions of varying lengths throughout the basic genome, whereas more highly diverged pairs within an evolutionary group or pairs between evolutionary groups having >1.3% SNPs have few clonal matches longer than a few kilobase pairs. Many recombinant transfers appear to incorporate fragments of the entering DNA produced by restriction systems of the recipient cell. A simple computational model can closely fit the data. Most recombinant transfers seem likely to be due to generalized transduction by coevolving populations of phages, which could efficiently distribute variability throughout bacterial genomes. C1 [Dixit, Purushottam D.; Pang, Tin Yau; Studier, F. William; Maslov, Sergei] Brookhaven Natl Lab, Biol Environm & Climate Sci Dept, Upton, NY 11973 USA. RP Studier, FW (reprint author), Brookhaven Natl Lab, Biol Environm & Climate Sci Dept, Upton, NY 11973 USA. EM studier@bnl.gov; ssmaslov@gmail.com OI Maslov, Sergei/0000-0002-3701-492X FU Office of Biological and Environmental Research of the US Department of Energy [PM-031, ELS165]; Brookhaven National Laboratory FX This work was supported by Grants PM-031 and ELS165 from the Office of Biological and Environmental Research of the US Department of Energy and internal research funding from Brookhaven National Laboratory. NR 38 TC 14 Z9 14 U1 3 U2 20 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUL 21 PY 2015 VL 112 IS 29 BP 9070 EP 9075 DI 10.1073/pnas.1510839112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CN2BJ UT WOS:000358225100077 PM 26153419 ER PT J AU Hilbert, BJ Hayes, JA Stone, NP Duffy, CM Sankaran, B Kelch, BA AF Hilbert, Brendan J. Hayes, Janelle A. Stone, Nicholas P. Duffy, Caroline M. Sankaran, Banumathi Kelch, Brian A. TI Structure and mechanism of the ATPase that powers viral genome packaging SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE ASCE ATPase; thermophile; bacteriophage; translocase; motor protein ID DNA TRANSLOCATION; HEXAMERIC HELICASE; LARGE SUBUNIT; TERMINASE; BACTERIOPHAGE-T4; MACHINE; DOMAIN; MOTOR; SCATTERING; SYSTEM AB Many viruses package their genomes into procapsids using an ATPase machine that is among the most powerful known biological motors. However, how this motor couples ATP hydrolysis to DNA translocation is still unknown. Here, we introduce a model system with unique properties for studying motor structure and mechanism. We describe crystal structures of the packaging motor ATPase domain that exhibit nucleotide-dependent conformational changes involving a large rotation of an entire subdomain. We also identify the arginine finger residue that catalyzes ATP hydrolysis in a neighboring motor subunit, illustrating that previous models for motor structure need revision. Our findings allow us to derive a structural model for the motor ring, which we validate using small-angle X-ray scattering and comparisons with previously published data. We illustrate the model's predictive power by identifying the motor's DNA-binding and assembly motifs. Finally, we integrate our results to propose a mechanistic model for DNA translocation by this molecular machine. C1 [Hilbert, Brendan J.; Hayes, Janelle A.; Stone, Nicholas P.; Duffy, Caroline M.; Kelch, Brian A.] Univ Massachusetts, Sch Med, Dept Mol Pharmacol & Biochem, Worcester, MA 01605 USA. [Sankaran, Banumathi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley Ctr Struct Biol, Berkeley, CA 94720 USA. RP Kelch, BA (reprint author), Univ Massachusetts, Sch Med, Dept Mol Pharmacol & Biochem, Worcester, MA 01605 USA. EM brian.kelch@umassmed.edu FU Worcester Foundation; Pew Charitable Trusts FX We thank the Rhind, Rando, Schiffer, Royer, Ryder, and Bolon laboratories for discussions and use of instrumentation. We thank beamline scientists at ALS sector 5 (Lawrence Berkeley National Laboratory), APS 23-ID-B (Argonne National Laboratory), and NSLS X25 (Brookhaven National Laboratory) for technical support with X-ray diffraction data collection, and Z. Maben and Dr. J. Birtley for assistance with data collection of the ADP.BeF3 cocrystals. This work was initiated by a grant from the Worcester Foundation. B.A.K. is a Pew Scholar in the Biomedical Sciences, supported by the Pew Charitable Trusts. NR 60 TC 9 Z9 9 U1 3 U2 19 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUL 21 PY 2015 VL 112 IS 29 BP E3792 EP E3799 DI 10.1073/pnas.1506951112 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CN2BJ UT WOS:000358225100009 PM 26150523 ER PT J AU Zaitseva, N Glenn, A Carman, L Martinez, HP Hatarik, R Kapper, H Payne, S AF Zaitseva, Natalia Glenn, Andrew Carman, Leslie Martinez, H. Paul Hatarik, Robert Kapper, Helmut Payne, Stephen TI Scintillation properties of solution-grown trans-stilbene single crystals SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Trans-stilbene; Solution growth; Organic crystals; Organic scintillator; Pulse shape discrimination; Neutron detection ID PULSE-SHAPE DISCRIMINATION; ORGANIC SCINTILLATORS; FAST-NEUTRON; LIQUID SCINTILLATOR; RAPID GROWTH AB The scintillation properties of trans-stilbene crystals grown for the first time by application of the solution growth technique to the scale of 10 cm are reported. Measurements of the scintillation light output, pulse shape discrimination, and neutron detection efficiency were made with sets of crystals cut as 50 cm diameter cylinders of different lengths from 0.3 to 10 cm. Comparison to liquid scintillators and traditional melt-grown stilbene showed that at increasing sizes new solution-grown crystals exhibit better scintillation performance that makes them promising for use in large scale neutron detectors. Results are discussed in relation to structural imperfections attributed to different methods of growth. (C) 2015 Elsevier B.V. All rights reserved, C1 [Zaitseva, Natalia; Glenn, Andrew; Carman, Leslie; Martinez, H. Paul; Hatarik, Robert; Payne, Stephen] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Kapper, Helmut] Inst Kristallog & Mineral, D-52066 Aachen, Germany. RP Zaitseva, N (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94551 USA. EM zaitseva1@llnl.gov FU US Department of Energy - Lawrence Livermore National Laboratory [DE-AC5 07NA27344]; US Department of Homeland Security, Domestic Nuclear Detection Office (DNDO) [HSHQDC-09-X-00743] FX The work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC5 07NA27344. Financial support was provided by the US Department of Homeland Security, Domestic Nuclear Detection Office (DNDO), under competitively awarded IAA HSHQDC-09-X-00743. This support does not constitute an express or implied endorsement on the part of the Government. We also wish to thank Dr. Cheng Saw for performing X-ray diffraction analysis and Dr. Erik Brubaker for providing the anthracene crystals. NR 23 TC 12 Z9 12 U1 2 U2 13 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 21 PY 2015 VL 789 BP 8 EP 15 DI 10.1016/j.nima.2015.03.090 PG 8 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CI6LV UT WOS:000354871700002 ER PT J AU Aliaga, L Altinok, O Del Castillo, CA Bagby, L Bellantoni, L Bergan, WF Bodek, A Bradford, R Bravar, A Budd, H Butkevich, A Caicedo, DAM Cameiro, MF Christy, ME Chvojka, J da Motta, H Devan, J Diaz, GA Dytman, SA Eberly, B Felix, J Fields, L Fine, R Flight, R Gago, AM Gingu, C Golan, T Gomez, A Gran, R Harris, DA Higuera, A Howley, IJ Hurtado, K Kleykamp, J Kordosky, M Lanari, M Le, T Leister, AJ Lovlein, A Maher, E Mann, WA Marshall, CM McFarland, KS McGivern, CL McGowan, AM Messerly, B Miller, J Miller, V Mislivec, A Morfin, JG Mousseau, J Muhlbeier, T Naples, D Nelson, JK Norrick, A Ochoa, N O'Connor, CD Osmanov, B Osta, J Paoloner, V Patrick, CE Patrick, L Perdue, GN Lara, CEP Rakotondravohitra, L Ray, H Ren, L Rodrigues, PA Rubinov, P Rude, CR Ruterbories, D Schellman, H Schmitz, DW Salinas, CJS Tagg, N Tice, BG Urrutia, Z Valencia, E Walton, T Westerberg, A Wolcott, J Woodward, N Wospakrik, M Zavala, G Zhang, D Ziemer, BP AF Aliaga, L. Altinok, O. Del Castillo, C. Araujo Bagby, L. Bellantoni, L. Bergan, W. F. Bodek, A. Bradford, R. Bravar, A. Budd, H. Butkevich, A. Caicedo, D. A. Martinez Cameiro, M. F. Christy, M. E. Chvojka, J. da Motta, H. Devan, J. Diaz, G. A. Dytman, S. A. Eberly, B. Felix, J. Fields, L. Fine, R. Flight, R. Gago, A. M. Gingu, C. Golan, T. Gomez, A. Gran, R. Harris, D. A. Higuera, A. Howley, I. J. Hurtado, K. Kleykamp, J. Kordosky, M. Lanari, M. Le, T. Leister, A. J. Lovlein, A. Maher, E. Mann, W. A. Marshall, C. M. McFarland, K. S. McGivern, C. L. McGowan, A. M. Messerly, B. Miller, J. Miller, Vv. Mislivec, A. Morfin, J. G. Mousseau, J. Muhlbeier, T. Naples, D. Nelson, J. K. Norrick, A. Ochoa, N. O'Connor, C. D. Osmanov, B. Osta, J. Paoloner, V. Patrick, C. E. Patrick, L. Perdue, G. N. Lara, C. E. Perez Rakotondravohitra, L. Ray, H. Ren, L. Rodrigues, P. A. Rubinov, P. Rude, C. R. Ruterbories, D. Schellman, H. Schmitz, D. W. Salinas, C. J. Solano Tagg, N. Tice, B. G. Urrutia, Z. Valencia, E. Walton, T. Westerberg, A. Wolcott, J. Woodward, N. Wospakrik, M. Zavala, G. Zhang, D. Ziemer, B. P. TI MINERvA neutrino detector response measured with test beam data SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Hadron calorimetry; Electromagnetic calorimetry; Birks' law; Test beam ID CALIBRATION AB The MINERvA collaboration operated a scaled down replica of the solid scintillator tracking and sampling calorimeter regions of the MlNERvA detector in a hadron test beam at the Fermilab Test Beam Facility. This paper reports measurements with samples of protons, pions, and electrons from 0.35 to 2.0 GeV/c momentum. The calorimetric response to protons, pions, and electrons is obtained from these data. A measurement of the parameter in Birks' law and an estimate of the tracking efficiency are extracted from the proton sample. Overall the data are well described by a Geant4-based Monte Carlo simulation of the detector and particle interactions with agreements better than 4% for the calorimetric response, though some features of the data are not precisely modeled. These measurements are used to tune the MINERvA detector simulation and evaluate systematic uncertainties in support of the MINERvA neutrino cross-section measurement program. (C) 2015 Published by Elsevier B.V. C1 [Aliaga, L.; Bergan, W. F.; Devan, J.; Howley, I. J.; Kordosky, M.; Leister, A. J.; Nelson, J. K.; Norrick, A.; O'Connor, C. D.; Zhang, D.] Coll William & Mary, Dept Phys, Williamsburg, VA 23187 USA. [Del Castillo, C. Araujo; Diaz, G. A.; Gago, A. M.; Ochoa, N.; Lara, C. E. Perez] Pontificia Univ Catolic Peru, Dept Ciencias, Secc Fis, Lima, Peru. [Altinok, O.; Mann, W. A.] Tufts Univ, Dept Phys, Medford, MA 02155 USA. [Bagby, L.; Bellantoni, L.; Caicedo, D. A. Martinez; Gingu, C.; Golan, T.; Harris, D. A.; McFarland, K. S.; Morfin, J. G.; Osta, J.; Perdue, G. N.; Rakotondravohitra, L.; Rubinov, P.; Schmitz, D. W.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Bodek, A.; Bradford, R.; Budd, H.; Chvojka, J.; Diaz, G. A.; Fine, R.; Flight, R.; Golan, T.; Gomez, A.; Higuera, A.; Kleykamp, J.; Marshall, C. M.; McFarland, K. S.; McGowan, A. M.; Mislivec, A.; Perdue, G. N.; Rodrigues, P. A.; Ruterbories, D.; Wolcott, J.] Univ Rochester, Rochester, NY 14627 USA. [Bravar, A.; da Motta, H.] Univ Geneva, CH-1211 Geneva 4, Switzerland. [Butkevich, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Caicedo, D. A. Martinez; Cameiro, M. F.; Hurtado, K.; Muhlbeier, T.] Ctr Brasileiro Pesquisas Fis, BR-22290180 Urea, RJ, Brazil. [Christy, M. E.; Patrick, C. E.; Walton, T.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Dytman, S. A.; Eberly, B.; McGivern, C. L.; Messerly, B.; Naples, D.; Paoloner, V.; Ren, L.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Felix, J.; Higuera, A.; Valencia, E.; Zavala, G.] Univ Guanajuato, Guanajuato 36000, Guanajuato, Mexico. [Fields, L.; Patrick, L.; Schellman, H.] Northwestern Univ, Evanston, IL 60208 USA. [Gran, R.; Lanari, M.; Lovlein, A.; Miller, Vv.; Rude, C. R.; Westerberg, A.; Woodward, N.] Univ Minnesota, Dept Phys, Duluth, MN 55312 USA. [Hurtado, K.; Salinas, C. J. Solano] Univ Nacl Ingn, Lima, Peru. [Le, T.; Tice, B. G.] Rutgers State Univ, Piscataway, NJ 08854 USA. [Maher, E.] Massachusetts Coll Liberal Arts, North Adams, MA 01247 USA. [Miller, J.] Univ Tecn Feder Santa Maria, Dept Fis, Valparaiso, Chile. [Mousseau, J.; Osmanov, B.; Ray, H.; Wospakrik, M.] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. [Tagg, N.] Otterbein Univ, Dept Phys, Westerville, OH 43081 USA. [Ziemer, B. P.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. RP Gran, R (reprint author), Univ Minnesota, Dept Phys, Duluth, MN 55312 USA. OI Solano Salinas, Carlos Javier/0000-0001-7821-498X; /0000-0002-9584-2600; Hurtado Anampa, Kenyi/0000-0002-9779-3566; Schmitz, David/0000-0003-2165-7389 FU Fermi National Accelerator Laboratory under U.S. Department of Energy [DE-AC02-07CH11359]; United States National Science Foundation [PHY-0619727]; University of Rochester; NSF (USA); DOE (USA); CAPES (Brazil); CNPq (Brazil); CoNaCyT (Mexico); CONICYT (Chile); CONCYTEC (Peru); DGI-PUCP (Peru); IDI/IGI-UNI (Peru); Latin American Center for Physics (CLAF); Swiss National Science Foundation; RAS (Russia); Russian Ministry of Education and Science (Russia) FX This work was supported by the Fermi National Accelerator Laboratory under U.S. Department of Energy Contract no. DE-AC02-07CH11359 which included the MINERvA construction project. Construction of the test beam detector was granted by the United States National Science Foundation under Grant no, PHY-0619727 and by the University of Rochester. Support for participating scientists was provided by NSF and DOE (USA) by CAPES and CNPq (Brazil), by CoNaCyT (Mexico), by CONICYT (Chile), by CONCYTEC, DGI-PUCP and IDI/IGI-UNI (Peru), by Latin American Center for Physics (CLAF), by the Swiss National Science Foundation, and by RAS and the Russian Ministry of Education and Science (Russia). NR 26 TC 7 Z9 7 U1 0 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 21 PY 2015 VL 789 BP 28 EP 42 DI 10.1016/j.nima.2015.04.003 PG 15 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CI6LV UT WOS:000354871700004 ER PT J AU Guardincerri, E Bacon, J Borozdin, K Durham, JM Fabritius, J Hecht, A Milner, EC Miyadera, H Morris, CL Perry, J Poulson, D AF Guardincerri, Elena Bacon, Jeffrey Borozdin, Konstantin Durham, J. Matthew Fabritius, Joseph, II Hecht, Adam Milner, Edward C. Miyadera, Haruo Morris, Christopher L. Perry, John Poulson, Daniel TI Detecting special nuclear material using muon-induced neutron emission SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Muon tomography; Neutron tagged muons; Cosmic ray tracking; Muon tracking; Muon radiography; Muon imaging ID INDUCED FISSION AB The penetrating ability of cosmic ray muons makes them an attractive probe for imaging dense materials. Here, we describe experimental results from a new technique that uses neutrons generated by cosmic-ray muons to identify the presence of special nuclear material (SNM). Neutrons emitted from SNM are used to tag muon-induced fission events in actinides and laminography is used to form images of the stopping material. This technique allows the imaging of SNM-bearing objects tagged using muon tracking detectors located above or to the side of the objects, and may have potential applications in warhead verification scenarios. During the experiment described here we did not attempt to distinguish the type or grade of the SNM. Published by Elsevier B.V. C1 [Guardincerri, Elena; Bacon, Jeffrey; Borozdin, Konstantin; Durham, J. Matthew; Fabritius, Joseph, II; Miyadera, Haruo; Morris, Christopher L.; Perry, John; Poulson, Daniel] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Milner, Edward C.] So Methodist Univ, Dallas, TX 75205 USA. [Hecht, Adam; Perry, John] Univ New Mexico, Albuquerque, NM 87131 USA. RP Guardincerri, E (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. OI Durham, J. Matthew/0000-0002-5831-3398; Morris, Christopher/0000-0003-2141-0255; Perry, John/0000-0003-3639-5617 FU United States Department of State; Defense Threat Reduction Agency of the United States Department of Defense; U.S. Department of Energy [DE-AC52-06NA25396] FX This work was supported in part by the United States Department of State, and the Defense Threat Reduction Agency of the United States Department of Defense, but it does not necessarily reflect the views or position of the U.S. government on the issues discussed herein, Los Alamos National Laboratory is operated for the U.S. Department of Energy under Contract DE-AC52-06NA25396 NR 28 TC 2 Z9 2 U1 0 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 21 PY 2015 VL 789 BP 109 EP 113 DI 10.1016/j.nima.2015.03.070 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CI6LV UT WOS:000354871700012 ER PT J AU Aucott, TJ Bandstra, MS Negut, V Curtis, JC Meyer, RE Chiyers, DH Vetter, K AF Aucott, Timothy J. Bandstra, Mark S. Negut, Victor Curtis, Joseph C. Meyer, Ross E. Chiyers, Daniel H. Vetter, Kai TI Impact of detector efficiency and energy resolution on gamma-ray background rejection in mobile spectroscopy and imaging systems SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Background radiation; Gamma-ray detection; Gamma-ray spectroscopy; Gamma-ray imaging ID CODED-APERTURE; SENSITIVITY AB The presence of gamma-ray background significantly reduces detection sensitivity when searching for radioactive sources in the field, and the systematic variability in the background will limit the size and energy resolution of systems that can be used effectively. An extensive survey of the background was performed using both sodium iodide and high-purity germanium. By using a bivariate negative binomial model for the measured counts, these measurements can be resampled to simulate the performance of a detector array of arbitrary size and resolution. The response of the system as it moved past a stationary source was modeled for spectroscopic and coded aperture imaging algorithms and used for source injection into the background. The performance of both techniques is shown for various sizes and resolutions, as well as the relative performance for sodium iodide and germanium, It was found that at smaller detector sizes or better energy resolution, spectroscopy has higher detection sensitivity than imaging, while imaging is better suited to larger or poorer resolution detectors. (C) 2015 Elsevier B.V. All rights reserved C1 [Negut, Victor; Curtis, Joseph C.; Vetter, Kai] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Aucott, Timothy J.; Bandstra, Mark S.; Meyer, Ross E.; Chiyers, Daniel H.; Vetter, Kai] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. RP Aucott, TJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM Timothy.Aucott@SRS.gov FU U.S. Department of Homeland Security [2011-DN-077-ARI049-03]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the U.S. Department of Homeland Security under Grant Award 2011-DN-077-ARI049-03. The modeling and data curation were performed with the assistance of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract no. DE-AC02-05CH11231. This support does not constitute an express or implied endorsement on the part of the government. NR 15 TC 2 Z9 2 U1 1 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 21 PY 2015 VL 789 BP 128 EP 133 DI 10.1016/j.nima.2015.04.012 PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CI6LV UT WOS:000354871700014 ER PT J AU Oesch, PA Bouwens, RJ Illingworth, GD Franx, M Ammons, SM van Dokkum, PG Trenti, M Labbe, I AF Oesch, P. A. Bouwens, R. J. Illingworth, G. D. Franx, M. Ammons, S. M. van Dokkum, P. G. Trenti, M. Labbe, I. TI FIRST FRONTIER FIELD CONSTRAINTS ON THE COSMIC STAR FORMATION RATE DENSITY AT z similar to 10-THE IMPACT OF LENSING SHEAR ON COMPLETENESS OF HIGH-REDSHIFT GALAXY SAMPLES SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: evolution; galaxies: formation; galaxies: high-redshift; gravitational lensing: strong ID ULTRA-DEEP FIELD; LYMAN-BREAK GALAXIES; UV LUMINOSITY FUNCTIONS; FORMING GALAXIES; FAINT GALAXIES; CLUSTER A2744; ULTRAVIOLET LUMINOSITY; WFC3/IR OBSERVATIONS; FORMATION HISTORIES; MAGNIFICATION MAPS AB We search the complete Hubble Frontier Field data set of Abell 2744 and its parallel field for z similar to 10 sources to further refine the evolution of the cosmic star formation rate density (SFRD) between z similar to 8 and z similar to 10. We independently confirm two images of the recently discovered triply imaged z similar to 9.8 source by Zitrin et al. and set an upper limit for similar z similar to 10 galaxies with red colors of J(125)-H-160 > 1.2 in the parallel field of Abell 2744. We utilize extensive simulations to derive the effective selection volume of Lyman-break galaxies at z similar to 10, both in the lensed cluster field and in the adjacent parallel field. Particular care is taken to include position-dependent lensing shear to accurately account for the expected sizes and morphologies of highly magnified sources. We show that both source blending and shear reduce the completeness at a given observed magnitude in the cluster, particularly near the critical curves. These effects have a significant, but largely overlooked, impact on the detectability of high-redshift sources behind clusters, and substantially reduce the expected number of highly magnified sources. The detections and limits from both pointings result in an SFRD which is consistent within the uncertainties with previous estimates at z similar to 10 from blank fields. The combination of these new results with all other estimates is also consistent with a rapidly declining SFRD in the 170 Myr from z similar to 8 to z similar to 10 as predicted by cosmological simulations and dark-matter halo evolution in Lambda CDM. Once biases introduced by magnification-dependent completeness are accounted for, the full six cluster and parallel Frontier Field program will be an extremely powerful new data set to probe the evolution of the galaxy population at z > 8 before the advent of the James Webb Space Telescope. C1 [Oesch, P. A.] Yale Univ, Dept Phys, Yale Ctr Astron & Astrophys, New Haven, CT 06520 USA. [Bouwens, R. J.; Franx, M.; Labbe, I.] Leiden Univ, Leiden Observ, NL-2300 RA Leiden, Netherlands. [Illingworth, G. D.] Univ Calif Santa Cruz, UCO Lick Observ, Santa Cruz, CA 95064 USA. [Ammons, S. M.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [van Dokkum, P. G.] Yale Univ, Dept Astron, New Haven, CT 06520 USA. [Trenti, M.] Univ Cambridge, Inst Astron, Cambridge CB3 0HA, England. [Trenti, M.] Univ Cambridge, Kavli Inst Cosmol, Cambridge CB3 0HA, England. RP Oesch, PA (reprint author), Yale Univ, Dept Phys, Yale Ctr Astron & Astrophys, New Haven, CT 06520 USA. EM pascal.oesch@yale.edu OI Oesch, Pascal/0000-0001-5851-6649 FU NASA [NAG5-7697, HST-GO-11563.01, NAS 5-26555] FX We thank the anonymous referee for very helpful feedback and suggestions, which greatly improved this paper. This work was supported by NASA grant NAG5-7697 and NASA grant HST-GO-11563.01. We are grateful to the directors of STScI and SSC to execute the dedicated Frontier Field program. We thank Shy Genel and Mark Vogelsberger for providing and discussing the results of the Illustris simulation. This work utilizes gravitational lensing models produced by PIs Bradac, Ebeling, Merten & Zitrin, Sharon, and Williams funded as part of the HST Frontier Fields program conducted by STScI. STScI is operated by the Association of Universities for Research in Astronomy, Inc. under NASA contract NAS 5-26555. The lens models and data sets were obtained from the Mikulski Archive for Space Telescopes (MAST). NR 87 TC 26 Z9 26 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 20 PY 2015 VL 808 IS 1 AR 104 DI 10.1088/0004-637X/808/1/104 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO3MS UT WOS:000359062500104 ER PT J AU Parker, ML Tomsick, JA Miller, JM Yamaoka, K Lohfink, A Nowak, M Fabian, AC Alston, WN Boggs, SE Christensen, FE Craig, WW Furst, F Gandhi, P Grefenstette, BW Grinberg, V Hailey, CJ Harrison, FA Kara, E King, AL Stern, D Walton, DJ Wilms, J Zhang, WW AF Parker, M. L. Tomsick, J. A. Miller, J. M. Yamaoka, K. Lohfink, A. Nowak, M. Fabian, A. C. Alston, W. N. Boggs, S. E. Christensen, F. E. Craig, W. W. Fuerst, F. Gandhi, P. Grefenstette, B. W. Grinberg, V. Hailey, C. J. Harrison, F. A. Kara, E. King, A. L. Stern, D. Walton, D. J. Wilms, J. Zhang, W. W. TI NuSTAR AND SUZAKU OBSERVATIONS OF THE HARD STATE IN CYGNUS X-1: LOCATING THE INNER ACCRETION DISK SO ASTROPHYSICAL JOURNAL LA English DT Article DE accretion, accretion disks; black hole physics; X-rays: binaries; X-rays: individual (Cygnus X-1) ID X-RAY REFLECTION; ADVECTION-DOMINATED ACCRETION; SPECTROSCOPIC-TELESCOPE-ARRAY; BROAD-BAND SPECTRUM; BLACK-HOLE; LOW/HARD STATE; CYCLOTRON LINE; XMM-NEWTON; SOFT STATE; HDE 226868 AB We present simultaneous Nuclear Spectroscopic Telescope Array (NuSTAR) and Suzaku. observations of the X-ray binary Cygnus X-1 in the hard state. This is the first time this state has been observed in Cyg X-1 with NuSTAR, which enables us to study the reflection and broadband spectra in unprecedented detail. We confirm that the iron line cannot be fit with a combination of narrow lines and absorption features, instead requiring. a relativistically blurred profile in combination with a narrow line and absorption from the companion wind. We use the reflection models of Garcia et al. to simultaneously measure the black hole spin, disk inner radius, and coronal height in a self-consistent manner. Detailed fits to the iron line profile indicate a high level of relativistic blurring, indicative of reflection from the inner accretion disk. We find a high spin, a small inner disk radius, and a low source height. and rule out truncation to greater than three gravitational radii at the 3 sigma confidence level. In addition, we find that the line profile has not changed greatly in the switch from soft to hard states, and that the differences are consistent with changes in the underlying reflection spectrum rather than the relativistic blurring. We find that the blurring parameters are consistent when fitting either just the iron line or the entire broadband spectrum, which is well modeled with a Comptonized continuum plus reflection model. C1 [Parker, M. L.; Lohfink, A.; Fabian, A. C.; Alston, W. N.; Kara, E.] Inst Astron, Cambridge CB3 0HA, England. [Tomsick, J. A.; Boggs, S. E.; Craig, W. W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Miller, J. M.] Univ Michigan, Dept Astron, Ann Arbor, MI 48109 USA. [Yamaoka, K.] Nagoya Univ, Dept Particles & Astron, Solar Terr Environm Lab, Chikusa Ku, Nagoya, Aichi 4648601, Japan. [Nowak, M.; Grinberg, V.] MIT, Kavli Inst Astrophys, Cambridge, MA 02139 USA. [Christensen, F. E.] Danish Tech Univ, DK-2800 Lyngby, Denmark. [Craig, W. W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Fuerst, F.; Grefenstette, B. W.; Harrison, F. A.; Walton, D. J.] CALTECH, Pasadena, CA 91125 USA. [Gandhi, P.] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. [Hailey, C. J.] Columbia Univ, New York, NY 10027 USA. [King, A. L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Stern, D.; Walton, D. J.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Wilms, J.] Dr Karl Remeis Observ, D-96049 Bamberg, Germany. [Wilms, J.] Erlangen Ctr Astroparticle Phys, D-96049 Bamberg, Germany. [Zhang, W. W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Parker, ML (reprint author), Inst Astron, Madingley Rd, Cambridge CB3 0HA, England. RI Wilms, Joern/C-8116-2013; XRAY, SUZAKU/A-1808-2009; Boggs, Steven/E-4170-2015; OI Wilms, Joern/0000-0003-2065-5410; Boggs, Steven/0000-0001-9567-4224; Parker, Michael/0000-0002-8466-7317 FU Science and Technology Facilities Council (STFC); NASA ADAP grant [NNX13AE98G]; European Union Seventh Framework Programme (FP7), StrongGravity [312789]; Deutsches Zentrum fur Luft- und Raumfahrt grant [50 OR 1411]; National Aeronautics and Space Administration FX M.L.P. acknowledges financial support from the Science and Technology Facilities Council (STFC) and is grateful to Simon Gibbons for helpful discussions. J.A.T. acknowledges partial support from NASA ADAP grant NNX13AE98G. W.N.A., E.K., and A.C.F. acknowledge support from the European Union Seventh Framework Programme (FP7/2013-2017) under grant agreement no. 312789, StrongGravity. J.W. acknowledges support from Deutsches Zentrum fur Luft- und Raumfahrt grant 50 OR 1411. This work made use of data from the NuSTAR. mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. This research has made use of the NuSTAR. Data Analysis Software (NuSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). This research has made use of data obtained from the Suzaku. satellite, a collaborative mission between the space agencies of Japan (JAXA) and the USA (NASA). NR 81 TC 10 Z9 10 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 20 PY 2015 VL 808 IS 1 AR 9 DI 10.1088/0004-637X/808/1/9 PG 13 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO3MS UT WOS:000359062500009 ER PT J AU Simon, JD Drlica-Wagner, A Li, TS Nord, B Geha, M Bechtol, K Balbinot, E Buckley-Geer, E Lin, H Marshall, J Santiago, B Strigari, L Wang, M Wechsler, RH Yanny, B Abbott, T Bauer, AH Bernstein, GM Bertin, E Brooks, D Burke, DL Capozzi, D Rosell, AC Kind, MC D'Andrea, CB da Costa, LN DePoy, DL Desai, S Diehl, HT Dodelson, S Cunha, CE Estrada, J Evrard, AE Neto, AF Fernandez, E Finley, DA Flaugher, B Frieman, J Gaztanaga, E Gerdes, D Gruen, D Gruendl, RA Honscheid, K James, D Kent, S Kuehn, K Kuropatkin, N Lahav, O Maia, MAG March, M Martini, P Miller, CJ Miquel, R Ogando, R Romer, AK Roodman, A Rykoff, ES Sako, M Sanchez, E Schubnell, M Sevilla, I Smith, RC Soares-Santos, M Sobreira, F Suchyta, E Swanson, MEC Tarle, G Thaler, J Tucker, D Vikram, V Walker, AR Wester, W AF Simon, J. D. Drlica-Wagner, A. Li, T. S. Nord, B. Geha, M. Bechtol, K. Balbinot, E. Buckley-Geer, E. Lin, H. Marshall, J. Santiago, B. Strigari, L. Wang, M. Wechsler, R. H. Yanny, B. Abbott, T. Bauer, A. H. Bernstein, G. M. Bertin, E. Brooks, D. Burke, D. L. Capozzi, D. Carnero Rosell, A. Kind, M. Carrasco D'Andrea, C. B. da Costa, L. N. DePoy, D. L. Desai, S. Diehl, H. T. Dodelson, S. Cunha, C. E. Estrada, J. Evrard, A. E. Fausti Neto, A. Fernandez, E. Finley, D. A. Flaugher, B. Frieman, J. Gaztanaga, E. Gerdes, D. Gruen, D. Gruendl, R. A. Honscheid, K. James, D. Kent, S. Kuehn, K. Kuropatkin, N. Lahav, O. Maia, M. A. G. March, M. Martini, P. Miller, C. J. Miquel, R. Ogando, R. Romer, A. K. Roodman, A. Rykoff, E. S. Sako, M. Sanchez, E. Schubnell, M. Sevilla, I. Smith, R. C. Soares-Santos, M. Sobreira, F. Suchyta, E. Swanson, M. E. C. Tarle, G. Thaler, J. Tucker, D. Vikram, V. Walker, A. R. Wester, W. CA DES Collaboration TI STELLAR KINEMATICS AND METALLICITIES IN THE ULTRA-FAINT DWARF GALAXY RETICULUM II SO ASTROPHYSICAL JOURNAL LA English DT Article DE dark matter; galaxies: dwarf; galaxies: individual (Reticulum II); galaxies: stellar content; Local Group; stars: abundances ID MILKY-WAY SATELLITE; COMPLETE SPECTROSCOPIC SURVEY; SMALL-MAGELLANIC-CLOUD; DIGITAL SKY SURVEY; METAL-POOR STARS; SPHEROIDAL GALAXY; SEGUE 1; LOCAL GROUP; URSA-MAJOR; LUMINOSITY FUNCTION AB We present Magellan/M2FS, Very Large Telescope/GIRAFFE, and Gemini South/GMOS spectroscopy of the newly discovered Milky Way satellite Reticulum II. Based on the spectra of 25 Ret II member stars selected from Dark Energy Survey imaging, we measure a mean heliocentric velocity of 62.8 +/- 0.5 km s(-1) and a velocity dispersion of 3.3 +/- 0.7 km s(-1). The mass-to-light ratio of Ret II within its half-light radius is 470 +/- 210 M circle dot L circle dot, demonstrating that it is a strongly dark matter-dominated system. Despite its spatial proximity to the Magellanic Clouds, the radial velocity of Ret II differs from that of the LMC and SMC by 199 and 83 km s(-1), respectively, suggesting that it is not gravitationally bound to the Magellanic system. The likely member stars of Ret II span 1.3 dex in metallicity, with a dispersion of 0.28 +/- 0.09 dex, and we identify several extremely metal-poor stars with [Fe/H] < -3. In combination with its luminosity, size, and ellipticity, these results confirm that Ret II is an ultra-faint dwarf galaxy. With a mean metallicity of [Fe/H] = -2.65 +/- 0.07, Ret II matches Segue 1 as the most metal-poor galaxy known. Although Ret II is the third-closest dwarf galaxy to the Milky Way, the line-of-sight integral of the dark matter density squared is log(10)(J) 18 +/- 80.6 GeV-2 cm(-5) within 0 degrees.2, indicating that the predicted gamma-ray flux from dark matter annihilation in Ret II is lower than that of several other dwarf galaxies. C1 [Simon, J. D.] Carnegie Observ, Pasadena, CA 91101 USA. [Drlica-Wagner, A.; Nord, B.; Buckley-Geer, E.; Lin, H.; Yanny, B.; Diehl, H. T.; Dodelson, S.; Estrada, J.; Finley, D. A.; Flaugher, B.; Frieman, J.; Kent, S.; Kuropatkin, N.; Soares-Santos, M.; Sobreira, F.; Tucker, D.; Wester, W.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Li, T. S.; Marshall, J.; Strigari, L.; Wang, M.; DePoy, D. L.] Texas A&M Univ, George P & Cynthia Woods Mitchell Inst Fundamenta, College Stn, TX 77843 USA. [Li, T. S.; Marshall, J.; Strigari, L.; Wang, M.; DePoy, D. L.] Texas A&M Univ, Dept Phys & Astron, College Stn, TX 77843 USA. [Geha, M.] Yale Univ, Dept Astron, New Haven, CT 06520 USA. [Bechtol, K.; Dodelson, S.; Frieman, J.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Balbinot, E.] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England. [Balbinot, E.; Santiago, B.; Carnero Rosell, A.; da Costa, L. N.; Fausti Neto, A.; Maia, M. A. G.; Ogando, R.; Sobreira, F.] Lab Interinst E Astron LIneA, BR-20921400 Rio De Janeiro, RJ, Brazil. [Santiago, B.] Univ Fed Rio Grande do Sul, Inst Fis, BR-91501970 Porto Alegre, RS, Brazil. [Wechsler, R. H.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Wechsler, R. H.; Burke, D. L.; Cunha, C. E.; Roodman, A.; Rykoff, E. S.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, Stanford, CA 94305 USA. [Wechsler, R. H.; Burke, D. L.; Roodman, A.; Rykoff, E. S.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Abbott, T.; James, D.; Smith, R. C.; Walker, A. R.] Natl Opt Astron Observ, Cerro Tololo Inter Amer Observ, La Serena, Chile. [Bauer, A. H.; Gaztanaga, E.] CSIC, Inst Ciencies Espai, Fac Ciencies, IEEC, E-08193 Barcelona, Spain. [Bernstein, G. M.; Sako, M.] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. [Bertin, E.] Univ Paris 06, Sorbonne Univ, Inst Astrophys Paris, UMR 7095, F-75014 Paris, France. [Bertin, E.] Univ Paris 06, Inst Astrophys Paris, F-75014 Paris, France. [Bertin, E.] CNRS, UMR7095, F-75014 Paris, France. [Brooks, D.; Lahav, O.; March, M.] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Capozzi, D.; D'Andrea, C. B.] Univ Portsmouth, Inst Cosmol & Gravitat, Portsmouth PO1 3FX, Hants, England. [Carnero Rosell, A.; da Costa, L. N.; Maia, M. A. G.; Ogando, R.] Observ Nacl, BR-20921400 Rio De Janeiro, RJ, Brazil. [Kind, M. Carrasco; Gruendl, R. A.; Sevilla, I.] Univ Illinois, Dept Astron, Urbana, IL 61801 USA. [Kind, M. Carrasco; Gruendl, R. A.; Swanson, M. E. C.] Univ Illinois, Natl Ctr Supercomp Applicat, Urbana, IL 61801 USA. [Desai, S.] Univ Munich, Dept Phys, D-81679 Munich, Germany. [Evrard, A. E.; Gerdes, D.; Miller, C. J.; Schubnell, M.; Tarle, G.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Fernandez, E.; Miquel, R.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Gruen, D.] Max Planck Inst Extraterr Phys, D-85748 Garching, Germany. [Gruen, D.] Univ Observ Munich, D-81679 Munich, Germany. [Honscheid, K.; Martini, P.; Suchyta, E.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Honscheid, K.; Suchyta, E.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Kuehn, K.] Australian Astron Observ, N Ryde, NSW 2113, Australia. [Martini, P.] Ohio State Univ, Dept Astron, Columbus, OH 43210 USA. [Miller, C. J.] Univ Michigan, Dept Astron, Ann Arbor, MI 48109 USA. [Romer, A. K.] Univ Sussex, Dept Phys & Astron, Brighton BN1 9QH, E Sussex, England. [Sanchez, E.; Sevilla, I.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Thaler, J.] Univ Illinois, Dept Astron, Urbana, IL 61801 USA. [Vikram, V.] Argonne Natl Lab, Lemont, IL 60439 USA. RP Simon, JD (reprint author), Carnegie Observ, 813 Santa Barbara St, Pasadena, CA 91101 USA. RI Ogando, Ricardo/A-1747-2010; Sanchez, Eusebio/H-5228-2015; Sobreira, Flavia/F-4168-2015; Fernandez, Enrique/L-5387-2014; Gaztanaga, Enrique/L-4894-2014; Balbinot, Eduardo/E-8019-2015; OI Ogando, Ricardo/0000-0003-2120-1154; Sanchez, Eusebio/0000-0002-9646-8198; Sobreira, Flavia/0000-0002-7822-0658; Fernandez, Enrique/0000-0002-6405-9488; Gaztanaga, Enrique/0000-0001-9632-0815; Suchyta, Eric/0000-0002-7047-9358; Carrasco Kind, Matias/0000-0002-4802-3194; Balbinot, Eduardo/0000-0002-1322-3153; Strigari, Louis/0000-0001-5672-6079; Tucker, Douglas/0000-0001-7211-5729 FU National Science Foundation [AST-1108811, AST-1138766]; PAPDRJ; CAPES/FAPERJ; CAPES [3171-13-2]; NSF/MRI [AST-0923160]; NSF [AST-1312967, AST-1313045]; U.S. Department of Energy; U.S. National Science Foundation; Ministry of Science and Education of Spain; Science and Technology Facilities Council of the United Kingdom; Higher Education Funding Council for England; National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign; Kavli Institute of Cosmological Physics at the University of Chicago; Center for Cosmology and Astro-Particle Physics at the Ohio State University; Mitchell Institute for Fundamental Physics and Astronomy at Texas AM University; Deutsche Forschungsgemeinschaft; Financiadora de Estudos e Projetos; Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico; Ministerio da Ciencia, Tecnologia e Inovacao; Collaborating Institutions in the Dark Energy Survey; MINECO [AYA2012-39559, ES2P2013-48274, FPA2013-47986]; Centro de Excelencia Severo Ochoa [SEV-2012-0234]; European Union FX This publication is based upon work supported by the National Science Foundation under grant AST-1108811. We thank Dan Kelson for helpful conversations, Anna Frebel for providing the MIKE spectrum of HD 122563, and Becky Canning and Jimmy for helpful conversations on the reduction of VLT spectra. We also thank the anonymous referee for suggestions that improved the presentation of the paper. A.C.R. acknowledges financial support provided by the PAPDRJ. CAPES/FAPERJ Fellowship. F.S. acknowledges financial support provided by CAPES under contract No. 3171-13-2. This research has made use of NASA's Astrophysics Data System Bibliographic Services. M2FS was built through partial support via NSF/MRI grant AST-0923160 to Mario Mateo, Ian Thompson and Steven Shectman as co-PIs and its construction was assisted by Jeffrey Crane and John I. Bailey III. The M2FS observations used in this paper were carried out on our behalf by Mario Mateo and Matthew Walker, who were supported in part by NSF grants AST-1312967 (MM) and AST-1313045 (MW). Additional partial operational support of M2FS has been provided by the Department of Astronomy of the University of Michigan and by Carnegie Observatories. Funding for the DES Projects has been provided by the U.S. Department of Energy, the U.S. National Science Foundation, the Ministry of Science and Education of Spain, the Science and Technology Facilities Council of the United Kingdom, the Higher Education Funding Council for England, the National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign, the Kavli Institute of Cosmological Physics at the University of Chicago, the Center for Cosmology and Astro-Particle Physics at the Ohio State University, the Mitchell Institute for Fundamental Physics and Astronomy at Texas A&M University, Financiadora de Estudos e Projetos, Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro, Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and the Ministerio da Ciencia, Tecnologia e Inovacao, the Deutsche Forschungsgemeinschaft and the Collaborating Institutions in the Dark Energy Survey. The DES data management system is supported by the National Science Foundation under Grant Number AST-1138766. The DES participants from Spanish institutions are partially supported by MINECO under grants AYA2012-39559, ES2P2013-48274, FPA2013-47986, and Centro de Excelencia Severo Ochoa SEV-2012-0234, some of which include ERDF funds from the European Union. The Collaborating Institutions are Argonne National Laboratory, the University of California at Santa Cruz, the University of Cambridge, Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas-Madrid, the University of Chicago, University College London, the DES-Brazil Consortium, the University of Edinburgh, the Eidgenossische Technische Hochschule (ETH) Zurich, Fermi National Accelerator Laboratory, the University of Illinois at Urbana-Champaign, the Institut de Ciencies de l'Espai (IEEC/CSIC), the Institut de Fisica d'Altes Energies, Lawrence Berkeley National Laboratory, the Ludwig-Maximilians Universitat Munchen and the associated Excellence Cluster Universe, the University of Michigan, the National Optical Astronomy Observatory, the University of Nottingham, The Ohio State University, the University of Pennsylvania, the University of Portsmouth, SLAC National Accelerator Laboratory, Stanford University, the University of Sussex, and Texas A&M University. NR 82 TC 29 Z9 29 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 20 PY 2015 VL 808 IS 1 AR 95 DI 10.1088/0004-637X/808/1/95 PG 14 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO3MS UT WOS:000359062500095 ER PT J AU Tendulkar, SP Hascoet, R Yang, CW Kaspi, VM Beloborodov, AM An, HJ Bachetti, M Boggs, SE Christensen, FE Craig, WW Guiilot, S Hailey, CA Harrison, FA Stern, D Zhang, W AF Tendulkar, Shriharsh P. Hascoeet, Romain Yang, Chengwei Kaspi, Victoria M. Beloborodov, Andrei M. An, Hongjun Bachetti, Matteo Boggs, Steven E. Christensen, Finn E. Craig, William W. Guiilot, Sebastien Hailey, Charles A. Harrison, Fiona A. Stern, Daniel Zhang, William TI PHASE-RESOLVED NuSTAR AND SWIFT-XRT OBSERVATIONS OF MAGNETAR 4U 0142+61 SO ASTROPHYSICAL JOURNAL LA English DT Article DE pulsars: individual (4U 0142+61); stars: magnetars; stars: neutron ID X-RAY PULSARS; SOFT GAMMA-REPEATERS; HIGH-ENERGY CHARACTERISTICS; SOLAR-SYSTEM ABUNDANCES; NEUTRON-STARS; XMM-NEWTON; CHEMICAL-COMPOSITION; INTERSTELLAR-MEDIUM; CROSS-SECTIONS; 1E 1048.1-5937 AB We present temporal and spectral analysis of simultaneous 0.5-79 keV Swift-XRT and Nuclear Spectroscopic Telescope Array observations of the magnetar 4U 0142+61. The pulse profile changes significantly with photon energy between 3 and 35 keV. The pulse fraction increases with energy, reaching a value of approximate to 20%, similar to that observed in 1E 1841-045 and much lower than the approximate to 80% pulse fraction observed in 1E 2259+586. We do not detect the 55 ks phase modulation reported in previous Suzaku-HXD observations. The phase-averaged spectrum of 4U 0142+61 above 20 keV is dominated by a hard power law (PL) with a photon index Gamma(H) similar to 0.65, and the spectrum below 20 keV can be described by two blackbodies, a blackbody plus a soft PL, or by a Comptonized blackbody model. We study the full phase-resolved spectra using the e(+/-) outflow model of Beloborodov. Our results are consistent with the parameters of the active j-bundle derived from INTEGRAL data by Hascoet et al. We find that a significant degeneracy appears in the inferred parameters if the footprint of the j-bundle is allowed to be a thin ring instead of a polar cap. The degeneracy is reduced when the footprint is required to be the hot spot inferred from the soft X-ray data. C1 [Tendulkar, Shriharsh P.; Harrison, Fiona A.] CALTECH, Space Radiat Lab, Pasadena, CA 91125 USA. [Hascoeet, Romain; Beloborodov, Andrei M.; Hailey, Charles A.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Yang, Chengwei] Beijing Inst Technol, Beijing 100081, Peoples R China. [Yang, Chengwei; Kaspi, Victoria M.; Guiilot, Sebastien] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [An, Hongjun] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, Stanford, CA 94305 USA. [Bachetti, Matteo] Osservatorio Astron Cagliari, INAF, I-09047 Selargius, CA, Italy. [Boggs, Steven E.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Christensen, Finn E.; Craig, William W.] Tech Univ Denmark, Natl Space Inst, DTU Space, DK-2800 Lyngby, Denmark. [Craig, William W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Guiilot, Sebastien] Pontificia Univ Catolica Chile, Fac Fis, Inst Astrofis, Santiago 7820436, Chile. [Stern, Daniel] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Zhang, William] NASA, Goddard Space Flight Ctr, Astrophys Sci Div, Greenbelt, MD 20771 USA. RP Tendulkar, SP (reprint author), CALTECH, Space Radiat Lab, 1200 E Calif Blvd,MC 249-17, Pasadena, CA 91125 USA. EM spt@astro.caltech.edu RI XRAY, SUZAKU/A-1808-2009; Boggs, Steven/E-4170-2015; OI Boggs, Steven/0000-0001-9567-4224; Bachetti, Matteo/0000-0002-4576-9337; An, Hongjun/0000-0002-6389-9012; Tendulkar, Shriharsh/0000-0003-2548-2926 FU NASA [NNG08FD60C, NNX13AI34G]; National Aeronautics and Space Administration; NSERC Discovery Grant and Accelerator Supplement; FQRNT Centre de Recherche Astrophysique du Quebec; R. Howard Webster Foundation Fellowship from Canadian Institute for Advanced Research (CIFAR); Canada Research Chairs Program; Lorne Trottier Chair in Astrophysics and Cosmology FX This work was supported under NASA Contract No. NNG08FD60C, and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). V. M. K. acknowledges support from an NSERC Discovery Grant and Accelerator Supplement, the FQRNT Centre de Recherche Astrophysique du Quebec, an R. Howard Webster Foundation Fellowship from the Canadian Institute for Advanced Research (CIFAR), the Canada Research Chairs Program and the Lorne Trottier Chair in Astrophysics and Cosmology. A.M.B. acknowledges the support by NASA grant NNX13AI34G. NR 67 TC 5 Z9 5 U1 0 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 20 PY 2015 VL 808 IS 1 AR 32 DI 10.1088/0004-637X/808/1/32 PG 13 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO3MS UT WOS:000359062500032 ER PT J AU van Engelen, A Sherwin, BD Sehgal, N Addison, GE Allison, R Battaglia, N de Bernardis, F Bond, JR Calabrese, E Coughlin, K Crichton, D Datta, R Devlin, MJ Dunkley, J Dunner, R Gallardo, P Grace, E Gralla, M Hajian, A Hasselfield, M Henderson, S Hill, JC Hilton, M Hincks, AD Hlozek, R Huffenberger, KM Hughes, JP Koopman, B Kosowsky, A Louis, T Lungu, M Madhavacheril, M Maurin, L McMahon, J Moodley, K Munson, C Naess, S Nati, F Newburgh, L Niemack, MD Nolta, MR Page, LA Pappas, C Partridge, B Schmitt, BL Sievers, JL Simon, S Spergel, DN Staggs, ST Switzer, ER Ward, JT Wollack, EJ AF van Engelen, Alexander Sherwin, Blake D. Sehgal, Neelima Addison, Graeme E. Allison, Rupert Battaglia, Nick de Bernardis, Francesco Bond, J. Richard Calabrese, Erminia Coughlin, Kevin Crichton, Devin Datta, Rahul Devlin, Mark J. Dunkley, Joanna Duenner, Rolando Gallardo, Patricio Grace, Emily Gralla, Megan Hajian, Amir Hasselfield, Matthew Henderson, Shawn Hill, J. Colin Hilton, Matt Hincks, Adam D. Hlozek, Renee Huffenberger, Kevin M. Hughes, John P. Koopman, Brian Kosowsky, Arthur Louis, Thibaut Lungu, Marius Madhavacheril, Mathew Maurin, Loic McMahon, Jeff Moodley, Kavilan Munson, Charles Naess, Sigurd Nati, Federico Newburgh, Laura Niemack, Michael D. Nolta, Michael R. Page, Lyman A. Pappas, Christine Partridge, Bruce Schmitt, Benjamin L. Sievers, Jonathan L. Simon, Sara Spergel, David N. Staggs, Suzanne T. Switzer, Eric R. Ward, Jonathan T. Wollack, Edward J. TI THE ATACAMA COSMOLOGY TELESCOPE: LENSING OF CMB TEMPERATURE AND POLARIZATION DERIVED FROM COSMIC INFRARED BACKGROUND CROSS-CORRELATION SO ASTROPHYSICAL JOURNAL LA English DT Article DE cosmic background radiation; cosmology: observations; infrared: diffuse background; large-scale structure of universe ID SOUTH-POLE TELESCOPE; PROBE WMAP OBSERVATIONS; POWER SPECTRUM; DUST EMISSION; MICROWAVE; MAPS; GALAXIES; MASS; SKY; RECONSTRUCTION AB We present a measurement of the gravitational lensing of the Cosmic Microwave Background (CMB) temperature and polarization fields obtained by cross-correlating the reconstructed convergence signal from the first season of Atacama Cosmology Telescope Polarimeter data at 146 GHz with Cosmic Infrared Background (CIB) fluctuations measured using the Planck satellite. Using an effective overlap area of 92.7 square degrees, we detect gravitational lensing of the CMB polarization by large-scale structure at a statistical significance of 4.5 sigma. Combining both CMB temperature and polarization data gives a lensing detection at 9.1 sigma significance. A B-mode polarization lensing signal is present with a significance of 3.2 sigma. We also present the first measurement of CMB lensing-CIB correlation at small scales corresponding to l > 2000. Null tests and systematic checks show that our results are not significantly biased by astrophysical or instrumental systematic effects, including Galactic dust. Fitting our measurements to the best-fit lensing-CIB cross-power spectrum measured in Planck data, scaled by an amplitude A, gives A = 1.02(-0.08)(+0.12)(stat.) +/- 0.06(syst.), consistent with the Planck results. C1 [van Engelen, Alexander; Bond, J. Richard; Hajian, Amir; Nolta, Michael R.; Switzer, Eric R.] Univ Toronto, Canadian Inst Theoret Astrophys, Toronto, ON M5S 3H8, Canada. [van Engelen, Alexander; Sehgal, Neelima; Madhavacheril, Mathew] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Sherwin, Blake D.] Univ Calif Berkeley, LBL, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. [Sherwin, Blake D.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Addison, Graeme E.; Hasselfield, Matthew; Hincks, Adam D.] Univ British Columbia, Dept Phys & Astron, Vancouver, BC V6T 1Z4, Canada. [Allison, Rupert; Calabrese, Erminia; Dunkley, Joanna; Louis, Thibaut; Naess, Sigurd] Univ Oxford, Subdept Astrophys, Oxford OX1 3RH, England. [Battaglia, Nick] Carnegie Mellon Univ, McWilliams Ctr Cosmol, Dept Phys, Pittsburgh, PA 15213 USA. [de Bernardis, Francesco; Gallardo, Patricio; Henderson, Shawn; Koopman, Brian; Niemack, Michael D.] Cornell Univ, Dept Phys, Ithaca, NY 14853 USA. [Coughlin, Kevin; Datta, Rahul; McMahon, Jeff; Munson, Charles] Univ Michigan, Dept Phys, Ann Arbor, MI 48103 USA. [Crichton, Devin; Gralla, Megan] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Devlin, Mark J.; Lungu, Marius; Schmitt, Benjamin L.; Ward, Jonathan T.] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. [Duenner, Rolando; Maurin, Loic] Pontificia Univ Catolica Chile, Dept Astron & Astrofis, Santiago 22, Chile. [Grace, Emily; Page, Lyman A.; Pappas, Christine; Sievers, Jonathan L.; Simon, Sara; Staggs, Suzanne T.] Princeton Univ, Joseph Henry Labs Phys, Princeton, NJ 08544 USA. [Hasselfield, Matthew; Hlozek, Renee; Spergel, David N.] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA. [Hill, J. Colin] Columbia Univ, Dept Astron, New York, NY 10027 USA. [Hilton, Matt; Moodley, Kavilan] Univ KwaZulu Natal, Sch Math Stat & Comp Sci, Astrophys & Cosmol Res Unit, Durban 4041, South Africa. [Huffenberger, Kevin M.] Florida State Univ, Dept Phys, Tallahassee, FL 32306 USA. [Hughes, John P.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Kosowsky, Arthur] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Nati, Federico] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Newburgh, Laura] Univ Toronto, Dunlap Inst Astron & Astrophys, Toronto, ON M5S 3H4, Canada. [Partridge, Bruce] Haverford Coll, Dept Phys & Astron, Haverford, PA 19041 USA. [Sievers, Jonathan L.] Univ KwaZulu Natal, Sch Chem & Phys, Astrophys & Cosmol Res Unit, Durban 4041, South Africa. [Sievers, Jonathan L.] Univ KwaZulu Natal, Natl Inst Theoret Phys NITheP, Durban 4000, South Africa. [Switzer, Eric R.; Wollack, Edward J.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP van Engelen, A (reprint author), Univ Toronto, Canadian Inst Theoret Astrophys, Toronto, ON M5S 3H8, Canada. RI Nati, Federico/I-4469-2016; Wollack, Edward/D-4467-2012; OI Nati, Federico/0000-0002-8307-5088; Wollack, Edward/0000-0002-7567-4451; Madhavacheril, Mathew/0000-0001-6740-5350; Sievers, Jonathan/0000-0001-6903-5074; Huffenberger, Kevin/0000-0001-7109-0099 FU U.S. National Science Foundation [AST-0408698, AST-0965625, PHY-0855887, PHY-1214379]; Princeton University; University of Pennsylvania; Cornell University; University of Michigan; Canada Foundation for Innovation (CFI) award; NSF [AST-13122380]; Misrahi research fund; Oxford ERC grant [259505]; NASA [NNX13AE56G, NNX14AB58G]; CONICYT [QUIMAL-120001, FONDECYT-1141113]; Comision Nacional de Investigacion Cientifica y Tecnologica de Chile (CONICYT); Government of Ontario; Ontario Research Fund-Research Excellence; University of Toronto; Wilkinson research fund; Compute Canada FX We thank Duncan Hanson for discussion and clarification regarding Section 7. We additionally thank Olivier Dore, Gil Holder, Guilaine Lagache, and Marco Viero for useful correspondence. This work was supported by the U.S. National Science Foundation through awards AST-0408698 and AST-0965625 for the ACT project, as well as awards PHY-0855887 and PHY-1214379. Funding was also provided by Princeton University, the University of Pennsylvania, Cornell University, the University of Michigan, and a Canada Foundation for Innovation (CFI) award to U.B.C. A.K. is supported by NSF grant AST-13122380. We gratefully acknowledge support from the Misrahi and Wilkinson research funds. We acknowledge Oxford ERC grant 259505. The development of detectors and lenses was supported by NASA grants NNX13AE56G and NNX14AB58G. We also acknowledge support from CONICYT grants QUIMAL-120001 and FONDECYT-1141113. ACT operates in the Parque Astronomico Atacama in northern Chile under the auspices of the Comision Nacional de Investigacion Cientifica y Tecnologica de Chile (CONICYT). Computations were performed on the GPC supercomputer at the SciNet HPC Consortium. SciNet is funded by the CFI under the auspices of Compute Canada, the Government of Ontario, the Ontario Research Fund-Research Excellence; and the University of Toronto. NR 69 TC 24 Z9 24 U1 0 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 20 PY 2015 VL 808 IS 1 AR 7 DI 10.1088/0004-637X/808/1/7 PG 9 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO3MS UT WOS:000359062500007 ER PT J AU Wu, MY Hao, YF Lu, QM Huang, C Guo, F Wang, S AF Wu, Mingyu Hao, Yufei Lu, Quanming Huang, Can Guo, Fan Wang, Shui TI THE ROLE OF LARGE AMPLITUDE UPSTREAM LOW-FREQUENCY WAVES IN THE GENERATION OF SUPERTHERMAL IONS AT A QUASI-PARALLEL COLLISIONLESS SHOCK: CLUSTER OBSERVATIONS SO ASTROPHYSICAL JOURNAL LA English DT Article DE acceleration of particles; shock waves ID EJECTION-DRIVEN SHOCKS; EARTHS BOW SHOCK; PARTICLE-ACCELERATION; SIMULATIONS AB The superthermal ions at a quasi-parallel collisionless shock are considered to be generated during the reformation of the shock. Recently, hybrid simulations of a quasi-parallel shock have shown that during the reformation of a quasi-parallel shock the large-amplitude upstream low-frequency waves can trap the reflected ions at the shock front when they try to move upstream, and then these reflected ions can be accelerated several times to become superthermal ions. In this paper, with the Cluster observations of a quasi-parallel shock event, the relevance between the large-amplitude upstream low-frequency waves and the superthermal ions (about several keV) have been studied. The observations clearly show that the differential energy flux of superthermal ions in the upstream region is modulated by the upstream low-frequency waves, and the maxima of the differential energy flux are usually located between the peaks of these waves (including the shock front and the peak of the upstream wave just in front of the shock front). These superthermal ions are considered to originate from the reflected ions at the shock front, and the modulation is caused due to the trapping of the reflected ions between the upstream waves or the upstream waves and the shock front when these reflected ions try to travel upstream. It verifies the results from hybrid simulations, where the upstream waves play an important role in the generation of superthermal ions in a quasi-parallel shock. C1 [Wu, Mingyu; Hao, Yufei; Lu, Quanming; Huang, Can; Wang, Shui] Univ Sci & Technol China, Dept Geophys & Planetary Sci, CAS Key Lab Geospace Environm, Hefei 230026, Peoples R China. [Wu, Mingyu] Chinese Acad Sci, State Key Lab Space Weather, Beijing 100190, Peoples R China. [Wu, Mingyu; Lu, Quanming] Collaborat Innovat Ctr Astronaut Sci & Technol, Beijing, Peoples R China. [Guo, Fan] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Wu, MY (reprint author), Univ Sci & Technol China, Dept Geophys & Planetary Sci, CAS Key Lab Geospace Environm, Hefei 230026, Peoples R China. EM qmlu@ustc.edu.cn RI Guo, Fan/H-1723-2013; OI Guo, Fan/0000-0003-4315-3755 FU National Science Foundation of China [41331067, 41274144, 41174124, 41121003]; 973 Program [2013CBA01503, 2012CB825602]; Specialized Research Fund for State Key Laboratories; CAS Key Research Program [KZZD-EW-01-4]; China Postdoctoral Science Foundation [2014M550344] FX This work was supported by the National Science Foundation of China, grant Nos. 41331067, 41274144, 41174124, 41121003, 973 Program (2013CBA01503, 2012CB825602), the Specialized Research Fund for State Key Laboratories, and CAS Key Research Program KZZD-EW-01-4. M.W. was supported by the China Postdoctoral Science Foundation, grant No. 2014M550344. We thank the FGM, CIS, PEACE, and EFW instrument teams and ESA Cluster Active Archive. All the data of the Cluster Mission can be downloaded from the website of the Cluster Active Archive. NR 30 TC 1 Z9 1 U1 2 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 20 PY 2015 VL 808 IS 1 AR 2 DI 10.1088/0004-637X/808/1/2 PG 6 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO3MS UT WOS:000359062500002 ER PT J AU D'Aleo, A Moore, EG Xu, JD Daumann, LJ Raymond, KN AF D'Aleo, Anthony Moore, Evan G. Xu, Jide Daumann, Lena J. Raymond, Kenneth N. TI Optimization of the Sensitization Process and Stability of Octadentate Eu(III) 1,2-HOPO Complexes SO INORGANIC CHEMISTRY LA English DT Article ID LUMINESCENT LANTHANIDE COMPLEXES; MRI CONTRAST AGENTS; HIGHLY LUMINESCENT; EUROPIUM COMPLEXES; OPTICAL-ABSORPTION; WATER-MOLECULES; HIGH-RELAXIVITY; III COMPLEXES; LIGAND; DECORPORATION AB The synthesis of a series of octadentate ligands containing the 1-hydroxypyridin-2-one (1,2-HOPO) group in complex with europium(III) is reported. Within this series, the central bridge connecting two diethylenetriamine units linked to two 1,2-HOPO chromophores at the extremities (5-LIN-1,2-HOPO) is varied from a short ethylene chain (H(2,2)-1,2-HOPO) to a long pentaethylene oxide chain (H(17O5,2)-1,2-HOPO). The thermodynamic stability of the europium complexes has been studied and reveals these complexes may be effective for biological measurements. Extension of the central bridge results in exclusion of the inner-sphere water molecule observed for [Eu(H(2,2)-1,2-HOPO)](-) going from a nonacoordinated to an octacoordinated Eu(III) ion. With the longer chain length ligands, the complexes display increased luminescence properties in aqueous medium with an optimum of 20% luminescence quantum yield for the [Eu(H(17O5,2)-1,2-HOPO)](-) complex. The luminescence properties for [Eu(H(14O4,2)-1,2-HOPO)](-) and [Eu(H(17O5,2)-1,2-HOPO)](-) are better than that of the model bis-tetradentate [Eu(5LIN(Me)-1,2-HOPO)(2)](-) complex, suggesting a different geometry around the metal center despite the geometric freedom allowed by the longer central chain in the H(mOn,2) scaffold. These differences are also evidenced by examining the luminescence spectra at room temperature and at 77 K and by calculating the luminescence kinetic parameters of the europium complexes. C1 [Raymond, Kenneth N.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Raymond, KN (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM raymond@socrates.berkeley.edu FU NIH [HL69832]; Office of Science, Office of Basic Energy Sciences, and the Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL [DE-AC02-05CH11231]; Alexander von Humboldt Foundation FX Early portions of this work were partially supported by the NIH (Grant HL69832) and then subsequently supported by the Director, Office of Science, Office of Basic Energy Sciences, and the Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL under Contract No. DE-AC02-05CH11231. The authors thank Prof. Gilles Muller (San Jose State University) for the use of a low-temperature time-resolved luminescence spectrometer. L.J.D. is grateful for a postdoctoral fellowship of the Alexander von Humboldt Foundation. NR 51 TC 3 Z9 3 U1 10 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUL 20 PY 2015 VL 54 IS 14 BP 6807 EP 6820 DI 10.1021/acs.inorgchem.5b00748 PG 14 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CN6MQ UT WOS:000358549300018 PM 26151082 ER PT J AU Summerscales, OT Stull, JA Scott, BL Gordon, JC AF Summerscales, Owen T. Stull, Jamie A. Scott, Brian L. Gordon, John C. TI Syntheses and Reactivity Studies of Square-Planar Diamido-Pyridine Complexes Based on Earth-Abundant First-Row Transition Elements SO INORGANIC CHEMISTRY LA English DT Article ID ETHYLENE POLYMERIZATION CATALYSTS; ELECTRONIC-STRUCTURE; DIALKYL COMPLEXES; PORPHYRIN COMPLEXES; CRYSTAL-STRUCTURE; PINCER COMPLEXES; IRON DICHLORIDE; LIGANDS; BIS(IMINO)PYRIDINE; DEHYDROGENATION AB The new square-planar complexes M[NNN]-(pyridine) (M = Fe (1), Co(2); NNN = 2,6-bis(2,6-diisopropylphenylamidomethyl)pyridine) were synthesized and fully characterized to investigate small molecule activation on this platform and also associated ligand innocence. The equatorial pyridine solvent moiety could not be removed; a new bis-ligand species Co [NNN center dot H](2) (3) was synthesized in low yield while attempting to make the base-free derivative. Attempts to prepare the Ni analogue of 1 and 2 instead yielded crystals of a di-imino-pyridine complex Ni[PDI]Cl (4) (PDI = 2,6-bis(2,6-diisopropylphenyliminomethyppyridine), following loss of methylene backbone hydrogen atoms. Structural analysis indicates that the PDI ligand is a mono-anionic radical. This susceptibility of the ligand to oxidative dehydrogenation was also shown when the reaction of 2 with 2 equiv of trityl chloride yielded a new complex with an asymmetric imino amino pyridine ligand Co[NNN']Cl-2 (5) (NNN' = 2-(2,6-(diisopropylphenyliminomethyl)-6-(diisopropylphenylamidomethyl)-pyridine) in good yield. C1 [Summerscales, Owen T.; Gordon, John C.] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. [Stull, Jamie A.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. [Scott, Brian L.] Los Alamos Natl Lab, Mat & Phys Applicat Div, Los Alamos, NM 87545 USA. RP Summerscales, OT (reprint author), Los Alamos Natl Lab, Div Chem, POB 1663, Los Alamos, NM 87545 USA. EM osummerscales@lanl.gov; jgordon@lanl.gov RI Scott, Brian/D-8995-2017 OI Scott, Brian/0000-0003-0468-5396 FU Laboratory Directed Research and Development (LDRD); National Science Foundation CRIF:MU award of the Univ. of New Mexico [CHE04-43580]; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC5206NA25396] FX We would like to thank Laboratory Directed Research and Development (LDRD) for a Director's postdoctoral fellowship (O.T.S.). We are grateful for the use of the Bruker X-ray diffractometer purchased via the National Science Foundation CRIF:MU award to Prof. R. Kemp of the Univ. of New Mexico (CHE04-43580) and Dr. T. J. Boyle at Sandia National Laboratories for data collection. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under Contract No. DE-AC5206NA25396. NR 43 TC 0 Z9 0 U1 4 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUL 20 PY 2015 VL 54 IS 14 BP 6885 EP 6890 DI 10.1021/acs.inorgchem.5b00779 PG 6 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CN6MQ UT WOS:000358549300025 PM 26154893 ER PT J AU Lampland, NL Zhu, J Hovey, M Jana, B Ellern, A Sadow, AD AF Lampland, Nicole L. Zhu, Jing Hovey, Megan Jana, Barun Ellern, Arkady Sadow, Aaron D. TI Piano-Stool Lutetium Amido and Imido Compounds Supported by a Constrained Bis(oxazoline)cyclopentadienyl Ligand SO INORGANIC CHEMISTRY LA English DT Article ID C-H ACTIVATION; BOND ACTIVATION; INTRAMOLECULAR HYDROAMINATION; INTERMOLECULAR HYDROAMINATION; POLYMERIZATION CATALYSTS; BENZENE ACTIVATION; COMPLEXES; ZIRCONIUM; ALKYNES; MECHANISM AB {Bo(M)Cp(tet)}Lu(CH2Ph)(2) (1; Bo(M)Cp(tet) = MeC-(Ox(Me2))(2)C5Me4; Ox(Me2) = 4,4-dimethyl-2-oxazoline) was prepared in 95% yield from the reaction of Bo(M)C(p)(tet)H and Lu(CH2Ph)(3)THF3. Compound 1 reacts with 1 or 2 equiv of H2NCH2R (R = C6H5, 1-C10H7) to give the corresponding imido complexes [{Bo(M)Cp(tet)}LuNCH2R](2) (R = C6H5 (2a), 1-C10H7 (2b)) or amido complexes {Bo(M)C(p)(tet)}Lu(NHCH2R)(2) (R = C6H5 (3a), 1-C10H7 (3b)). Once isolated, the imido species are insoluble in nonprotic organic solvents. Crystallographic characterization reveals dimeric [{Bo(M)C(p)(tet)}-Lu(NCH2(1-C10H7)](2) in the solid state. The reaction of 1 and NH3B(C6F5)(3) affords crystallographically characterized {Bo(M)C(p)(tet)}Lu{NHB(C6F5)(2)}C6F5. This species is proposed to form via a transient lutetium imido, which undergoes C6F5 migration to the lutetium center. C1 [Sadow, Aaron D.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. RP Sadow, AD (reprint author), Iowa State Univ, Dept Chem, Ames, IA 50011 USA. EM sadow@iastate.edu FU National Science Foundation [CHE-0955635]; Office of Workforce Development for Teachers and Scientists through the Summer Undergraduate Laboratory Internship Program through the Ames Laboratory; U.S. Department of Energy [DE-AC02-07CH11358]; Iowa Energy Center FX The authors gratefully thank the National Science Foundation (CHE-0955635) for financial support. BoMCptetH was first prepared by M.H. and B.J.; M.H. was supported by the Office of Workforce Development for Teachers and Scientists through the Summer Undergraduate Laboratory Internship Program through the Ames Laboratory. The Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. B.J. was supported by a grant from the Iowa Energy Center. NR 66 TC 3 Z9 3 U1 6 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUL 20 PY 2015 VL 54 IS 14 BP 6938 EP 6946 DI 10.1021/acs.inorgchem.5b00927 PG 9 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CN6MQ UT WOS:000358549300031 PM 26110352 ER PT J AU Sanjeewa, LD McGuire, MA Garlea, VO Hu, LY Chumanov, G McMillen, CD Kolis, JW AF Sanjeewa, Liurukara D. McGuire, Michael A. Garlea, Vasile O. Hu, Longyu Chumanov, George McMillen, Colin D. Kolis, Joseph W. TI Hydrothermal Synthesis and Characterization of Novel Brackebuschite-Type Transition Metal Vanadates: Ba2M(VO4)(2)(OH), M = V3+, Mn3+, and Fe3+, with Interesting Jahn-Teller and Spin-Liquid Behavior SO INORGANIC CHEMISTRY LA English DT Article ID CRYSTAL-STRUCTURE; MAGNETIC-PROPERTIES; VANADIUM-OXIDES; CHEMISTRY; OCTAHEDRA; MINERALS; NAVGE2O6; LIVGE2O6; LATTICES AB A new series of transition metal vanadates, namely, Ba2M(VO4)(2)(OH) (M = V3+, Mn3+, and Fe3+), was synthesized as large single crystals hydrothermally in 5 M NaOH solution at 580 degrees C and 1 kbar. This new series of compounds is structurally reminiscent of the brackebuschite mineral type. The structure of Ba2V(VO4)(2)(OH) is monoclinic in space group P2(1)/m, a = 7.8783(2) angstrom, b = 6.1369(1) angstrom, c = 9.1836(2) angstrom, beta = 113.07(3)degrees, V = 408.51(2) angstrom(3). The other structures are similar and consist of one-dimensional trans edge-shared distorted octahedral chains running along the b-axis. The vanadate groups bridge across edges of their tetrahedra. Structural analysis of the Ba2Mn(VO4)(2)(OH) analogue yielded a new understanding of the Jahn-Teller effect in this structure type. Raman and infrared spectra were investigated to observe the fundamental vanadate and hydroxide vibrational modes. Single-crystal temperature-dependent magnetic studies on Ba2V(VO4)(2)(OH) reveal a broad feature over a wide temperature range with maximum at similar to 100 K indicating that an energy gap could exist between the antiferromagnetic singlet ground state and excited triplet states, making it potentially of interest for quantum magnetism studies. C1 [Sanjeewa, Liurukara D.; Hu, Longyu; Chumanov, George; McMillen, Colin D.; Kolis, Joseph W.] Clemson Univ, Dept Chem, Clemson, SC 29634 USA. [Sanjeewa, Liurukara D.; Hu, Longyu; Chumanov, George; McMillen, Colin D.; Kolis, Joseph W.] Clemson Univ, COMSET, Clemson, SC 29634 USA. [McGuire, Michael A.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Garlea, Vasile O.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP Kolis, JW (reprint author), Clemson Univ, Dept Chem, Clemson, SC 29634 USA. EM kjoseph@clemson.edu RI McGuire, Michael/B-5453-2009; Garlea, Vasile/A-4994-2016 OI McGuire, Michael/0000-0003-1762-9406; Garlea, Vasile/0000-0002-5322-7271 FU National Science Foundation [DMR-1410727]; Materials Sciences and Engineering Division and Scientific User Facilities Division FX This was work was supported by a grant from the National Science Foundation (DMR-1410727). Work at the Oak Ridge National Laboratory was sponsored by the Materials Sciences and Engineering Division and Scientific User Facilities Division. NR 51 TC 8 Z9 8 U1 3 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUL 20 PY 2015 VL 54 IS 14 BP 7014 EP 7020 DI 10.1021/acs.inorgchem.5b01037 PG 7 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CN6MQ UT WOS:000358549300040 PM 26154989 ER PT J AU Mashayak, SY Jochum, MN Koschke, K Aluru, NR Ruhle, V Junghans, C AF Mashayak, S. Y. Jochum, Mara N. Koschke, Konstantin Aluru, N. R. Ruehle, Victor Junghans, Christoph TI Relative Entropy and Optimization-Driven Coarse-Graining Methods in VOTCA SO PLOS ONE LA English DT Article ID MULTISCALE SIMULATION; MOLECULAR-DYNAMICS; BIOMOLECULAR SYSTEMS; SOFT MATTER; WATER; MODELS; POTENTIALS; PACKAGE; ALGORITHMS AB We discuss recent advances of the VOTCA package for systematic coarse-graining. Two methods have been implemented, namely the downhill simplex optimization and the relative entropy minimization. We illustrate the new methods by coarse-graining SPC/E bulk water and more complex water-methanol mixture systems. The CG potentials obtained from both methods are then evaluated by comparing the pair distributions from the coarse-grained to the reference atomistic simulations. In addition to the newly implemented methods, we have also added a parallel analysis framework to improve the computational efficiency of the coarse-graining process. C1 [Mashayak, S. Y.; Aluru, N. R.] Univ Illinois, Dept Mech Sci & Engn, Beckman Inst Adv Sci & Technol, Urbana, IL 61801 USA. [Jochum, Mara N.; Koschke, Konstantin] Max Planck Inst Polymer Res, D-55128 Mainz, Germany. [Ruehle, Victor] Univ Cambridge, Dept Chem, Cambridge CB2 1EW, England. [Junghans, Christoph] Los Alamos Natl Lab, Comp Computat & Stat Sci Div, Los Alamos, NM 87545 USA. RP Junghans, C (reprint author), Los Alamos Natl Lab, Comp Computat & Stat Sci Div, POB 1663, Los Alamos, NM 87545 USA. EM junghans@lanl.gov RI Aluru, N/A-4617-2014; Junghans, Christoph/G-4238-2010 OI Junghans, Christoph/0000-0003-0925-1458 FU NSF [480 1264282, 1420882]; AFOSR [11157642]; framework of the multiscale modeling initiative of theMax-Planck Society [SFB 625, M3]; National Science Foundation [NSF PHY11-25915]; LANL; Nestle Research Center; DFG Emmy Noether program [LA-UR-13-26878]; National Nuclear Security Administration of the U.S. DOE [DE-AC52- 06NA25396] FX SYM and NRA acknowledge financial support by the NSF under grant Nos. 480 1264282 and 1420882 and AFOSR under grant No. 11157642. CJ was financially supported by SFB 625 in the framework of the multiscale modeling initiative of the Max-Planck Society (M3). This research was supported in part by the National Science Foundation under grant number NSF PHY11-25915. CJ thanks LANL for a Director's fellowship and the MPG for hospitality in 2013 at MPI-P. K. Koschke acknowledges funding by the Nestle Research Center. MNJ acknowledges DFG Emmy Noether program for financial support. Assigned: LA-UR-13-26878. LANL is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. DOE under Contract DE-AC52- 06NA25396. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 52 TC 9 Z9 9 U1 0 U2 14 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JUL 20 PY 2015 VL 10 IS 7 AR e0131754 DI 10.1371/journal.pone.0131754 PG 20 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CN6LN UT WOS:000358546400016 PM 26192992 ER PT J AU Hultqvist, A Li, JV Kuciauskas, D Dippo, P Contreras, MA Levi, DH Bent, SF AF Hultqvist, Adam Li, Jian V. Kuciauskas, Darius Dippo, Patricia Contreras, Miguel A. Levi, Dean H. Bent, Stacey F. TI Reducing interface recombination for Cu(In,Ga)Se-2 by atomic layer deposited buffer layers SO APPLIED PHYSICS LETTERS LA English DT Article ID THIN-FILM PHOTOVOLTAICS; SOLAR-CELLS AB Partial CuInGaSe2 (CIGS) solar cell stacks with different atomic layer deposited buffer layers and pretreatments were analyzed by photoluminescence (PL) and capacitance voltage (CV) measurements to investigate the buffer layer/CIGS interface. Atomic layer deposited ZnS, ZnO, and SnOx buffer layers were compared with chemical bath deposited CdS buffer layers. Band bending, charge density, and interface state density were extracted from the CV measurement using an analysis technique new to CIGS. The surface recombination velocity calculated from the density of interface traps for a ZnS/CIGS stack shows a remarkably low value of 810 cm/s, approaching the range of single crystalline II-VI systems. Both the PL spectra and its lifetime depend on the buffer layer; thus, these measurements are not only sensitive to the absorber but also to the absorber/buffer layer system. Pretreatment of the CIGS prior to the buffer layer deposition plays a significant role on the electrical properties for the same buffer layer/CIGS stack, further illuminating the importance of good interface formation. Finally, ZnS is found to be the best performing buffer layer in this study, especially if the CIGS surface is pretreated with potassium cyanide. (C) 2015 AIP Publishing LLC. C1 [Hultqvist, Adam; Bent, Stacey F.] Stanford Univ, Dept Chem Engn, Stanford, CA 94305 USA. [Li, Jian V.; Kuciauskas, Darius; Dippo, Patricia; Contreras, Miguel A.; Levi, Dean H.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Hultqvist, A (reprint author), Stanford Univ, Dept Chem Engn, Stanford, CA 94305 USA. RI Li, Jian/B-1627-2016; OI Kuciauskas, Darius/0000-0001-8091-5718 FU Marcus and Amalia Wallenberg Foundation; National Renewable Energy Laboratory as a part of the Non-Proprietary Partnering Program [De-AC36-08-GO28308]; U.S. Department of Energy FX This study was conducted under the Center on Nanostructuring for Efficient Energy Conversion at Stanford University (A.H. and S.F.B.). The Marcus and Amalia Wallenberg Foundation are acknowledged for supporting through the Stig Hagstrom Stipend (A.H.). Finally, this work was supported by the National Renewable Energy Laboratory as a part of the Non-Proprietary Partnering Program under Contract No. De-AC36-08-GO28308 with the U.S. Department of Energy (J.V.L., D.K., P.D., M.A.C., and D.H.L.). NR 37 TC 6 Z9 6 U1 7 U2 40 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUL 20 PY 2015 VL 107 IS 3 AR 033906 DI 10.1063/1.4927096 PG 5 WC Physics, Applied SC Physics GA CN8FR UT WOS:000358675600070 ER PT J AU Mickel, PR Lohn, AJ Mamaluy, D Marinella, MJ AF Mickel, Patrick R. Lohn, Andrew J. Mamaluy, Denis Marinella, Matthew J. TI Power signatures and vacancy profile control in nanoscale memristive filaments SO APPLIED PHYSICS LETTERS LA English DT Article ID RESISTIVE SWITCHING MEMORY; DRIVEN ION MIGRATION; MECHANISMS; DEVICES AB We introduce a method for the controlled construction of oxygen vacancy profiles within the conducting filaments of TaOx resistive switching devices, with spatial resolutions approaching the sub-nanometer scale. We identify controllable power signatures in the resistive switching curves of memristive devices, and using analytical and numerical models demonstrate they are consistent with specific, designable radial vacancy profiles within the conducting filaments resulting from high-order hysteresis. The design of radial vacancy profiles is shown to address important technological challenges in memristive systems such as controlled state writing, half-select errors, and designed retention. (C) 2015 AIP Publishing LLC. C1 [Mickel, Patrick R.; Lohn, Andrew J.; Mamaluy, Denis; Marinella, Matthew J.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Mickel, PR (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM pmickel@gmail.com FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 24 TC 0 Z9 0 U1 5 U2 24 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUL 20 PY 2015 VL 107 IS 3 AR 033507 DI 10.1063/1.4927211 PG 5 WC Physics, Applied SC Physics GA CN8FR UT WOS:000358675600064 ER PT J AU Mihalcea, D Faillace, L Hartzell, J Panuganti, H Boucher, S Murokh, A Piot, P Thangaraj, JCT AF Mihalcea, D. Faillace, L. Hartzell, J. Panuganti, H. Boucher, S. Murokh, A. Piot, P. Thangaraj, J. C. T. TI Measurement of Ampere-class pulsed electron beams via field emission from carbon-nanotube cathodes in a radiofrequency gun SO APPLIED PHYSICS LETTERS LA English DT Article ID EMITTERS AB Pulsed field emission from cold carbon-nanotube cathodes placed in a radiofrequency resonant cavity was directly measured. The cathodes were located on the backplate of a conventional 1 + 1/2-cell resonant cavity operating at 1.3-GHz and resulted in the production of bunch train with maximum average current close to 0.7 Ampere. The measured Fowler-Nordheim characteristic, transverse emittance, and pulse duration are presented and, when possible, compared to numerical simulations. The implications of our results to the promise of high-average-current electron sources are briefly discussed. (C) 2015 AIP Publishing LLC. C1 [Mihalcea, D.; Panuganti, H.; Piot, P.] No Illinois Univ, Northern Illinois Ctr Accelerator & Detector Dev, De Kalb, IL 60115 USA. [Mihalcea, D.; Panuganti, H.; Piot, P.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Faillace, L.; Hartzell, J.; Boucher, S.; Murokh, A.] RadiaBeam Technol LLC, Santa Monica, CA 90404 USA. [Piot, P.; Thangaraj, J. C. T.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Mihalcea, D (reprint author), No Illinois Univ, Northern Illinois Ctr Accelerator & Detector Dev, De Kalb, IL 60115 USA. OI Panuganti, Harsha/0000-0002-9325-8021 FU U.S. Department of Energy (DOE) [DE-SC0004459]; Radiabeam Technologies, LLC.; DOE [DE-AC02-07CH11359] FX We are grateful to D. P. Grote and J.-L. Vay for their help with Warp, to B. Chase, P. Prieto, E. Lopez, J. Santucci, and R. Kellett for technical support and to E. Harms, S. Nagaitsev, and V. Shiltsev for support. This work was funded via U.S. Department of Energy (DOE) Contract DE-SC0004459 with Radiabeam Technologies, LLC. Fermilab is operated by the Fermi Research Alliance, LLC. for the DOE under Contract DE-AC02-07CH11359. NR 24 TC 1 Z9 1 U1 0 U2 6 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUL 20 PY 2015 VL 107 IS 3 AR 033502 DI 10.1063/1.4927052 PG 4 WC Physics, Applied SC Physics GA CN8FR UT WOS:000358675600059 ER PT J AU Mohlabeng, G Kong, K Li, J Para, A Yoo, J AF Mohlabeng, Gopolang Kong, Kyoungchul Li, Jin Para, Adam Yoo, Jonghee TI Dark matter directionality revisited with a high pressure xenon gas detector SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Dark Matter and Double Beta Decay ID NUCLEAR RECOIL AB An observation of the anisotropy of dark matter interactions in a direction-sensitive detector would provide decisive evidence for the discovery of galactic dark matter. Directional information would also provide a crucial input to understanding its distribution in the local Universe. Most of the existing directional dark matter detectors utilize particle tracking methods in a low-pressure gas time projection chamber. These low pressure detectors require excessively large volumes in order to be competitive in the search for physics beyond the current limit. In order to avoid these volume limitations, we consider a novel proposal, which exploits a columnar recombination effect in a high-pressure gas time projection chamber. The ratio of scintillation to ionization signals observed in the detector carries the angular information of the particle interactions. In this paper, we investigate the sensitivity of a future directional detector focused on the proposed high-pressure Xenon gas time projection chamber. We study the prospect of detecting an anisotropy in the dark matter velocity distribution. We find that tens of events are needed to exclude an isotropic distribution of dark matter interactions at 95% confidence level in the most optimistic case with head-to-tail information. However, one needs at least 10-20 times more events without head-to-tail information for light dark matter below similar to 50 GeV. For an intermediate mass range, we find it challenging to observe an anisotropy of the dark matter distribution. Our results also show that the directional information significantly improves precision measurements of dark matter mass and the elastic scattering cross section for a heavy dark matter. C1 [Mohlabeng, Gopolang; Kong, Kyoungchul] Univ Kansas, Dept Phys & Astron, Lawrence, KS 66045 USA. [Li, Jin] Inst for Basic Sci Korea, Ctr Underground Phys, Taejon 305811, South Korea. [Para, Adam; Yoo, Jonghee] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Mohlabeng, G (reprint author), Univ Kansas, Dept Phys & Astron, Lawrence, KS 66045 USA. EM gopolang.mohlabeng@ku.edu; kckong@ku.edu; jinlee@ibs.re.kr; para@fnal.gov; yoo@fnal.gov RI Yoo, Jonghee/K-8394-2016 FU National Research Foundation of South Africa [88614]; U.S. DOE [DE-FG02-12ER41809]; University of Kansas General Research Fund [2301566]; United States Department of Energy [DE-AC02-07CH11359] FX We thank D. Nygren for useful the discussion and comments, and Azriel Goldschmidt for pointing out an issue in our normalization. GM is partially supported by the National Research Foundation of South Africa under Grant No. 88614. GM and KK are supported partially by the U.S. DOE under Grant No. DE-FG02-12ER41809 and by the University of Kansas General Research Fund allocation 2301566. Fermi lab is operated by Fermi Research Alliance, LLC, under Contract DE-AC02-07CH11359 with the United States Department of Energy. NR 46 TC 3 Z9 3 U1 0 U2 1 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JUL 20 PY 2015 IS 7 AR 092 DI 10.1007/JHEP07(2015)092 PG 20 WC Physics, Particles & Fields SC Physics GA CN5DP UT WOS:000358450300001 ER PT J AU Fitzpatrick, AL Kachru, S Kaplan, J Raghu, S Torroba, G Wang, HJ AF Fitzpatrick, A. Liam Kachru, Shamit Kaplan, Jared Raghu, S. Torroba, Gonzalo Wang, Huajia TI Enhanced pairing of quantum critical metals near d=3+1 SO PHYSICAL REVIEW B LA English DT Article ID RENORMALIZATION-GROUP APPROACH; FERMI-LIQUID; DENSITY; WAVE; QCD AB We study the dynamics of a quantum critical boson coupled to a Fermi surface in intermediate energy regimes where the Landau damping of the boson can be parametrically controlled, either via large Fermi velocity or by large-N techniques. We develop a systematic approach to the BCS instability of such systems, including careful treatment of the enhanced log(2) and log(3) singularities which appear already at 1-loop. These singularities arise due to the exchange of a critical boson in the Cooper channel and are absent in Fermi liquid theory. We also treat possible instabilities to charge density wave (CDW) formation, and compare the scales Lambda(BCS) and Lambda(CDW) of the onset of the instabilities in different parametric regimes. We address the question of whether the dressing of the fermions into a non-Fermi liquid via interactions with the order parameter field can happen at energies > Lambda(BCS), Lambda(CDW). C1 [Fitzpatrick, A. Liam; Kachru, Shamit; Raghu, S.; Wang, Huajia] Stanford Univ, Stanford Inst Theoret Phys, Stanford, CA 94305 USA. [Fitzpatrick, A. Liam; Kachru, Shamit; Raghu, S.] SLAC, Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Kaplan, Jared] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Torroba, Gonzalo] Ctr Atom Bariloche, RA-8400 San Carlos De Bariloche, Rio Negro, Argentina. [Torroba, Gonzalo] Consejo Nacl Invest Cient & Tecn, San Carlos De Bariloche, Rio Negro, Argentina. RP Fitzpatrick, AL (reprint author), Stanford Univ, Stanford Inst Theoret Phys, Stanford, CA 94305 USA. FU National Science Foundation [PHY-0756174, PHY-1316665, 1066293]; DOE Office of Basic Energy Sciences [DE-AC02-76SF00515]; SLAC LDRD grant; John Templeton Foundation; Alfred P. Sloan Foundation; ERC Grant BSMOXFORD [228169]; CONICET; PIP Grant [11220110100752] FX We thank A. Chubukov, M. Mulligan, D. Son, and all the participants of the Stanford Non-Fermi Liquids Conference for interesting discussions about related subjects. S.K. is grateful to the Aspen Center for Physics and S.R. to the Kavli Institute for Theoretical Physics, UC Santa Barbara, for hospitality during the time this work was carried out. This work was supported in part by the National Science Foundation, Grants No. PHY-0756174 (S.K.) and No. PHY-1316665 (J.K.), DOE Office of Basic Energy Sciences, Contract No. DE-AC02-76SF00515 (S.K. and S.R.), a SLAC LDRD grant on "non-Fermi liquids" (A.L.F., S.R., and S.K.), the John Templeton Foundation (S.K. and S.R.), and the Alfred P. Sloan Foundation (J.K. and S.R.). This material is based on work supported in part by the National Science Foundation, Grants No. 1066293 and No. PHY-1316665. A.L.F. was partially supported by ERC Grant BSMOXFORD No. 228169. G.T. is supported by CONICET, and PIP Grant No. 11220110100752. NR 26 TC 3 Z9 3 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUL 20 PY 2015 VL 92 IS 4 AR 045118 DI 10.1103/PhysRevB.92.045118 PG 14 WC Physics, Condensed Matter SC Physics GA CN2LR UT WOS:000358253200004 ER PT J AU Brune, CR Caggiano, JA Sayre, DB Bacher, AD Hale, GM Paris, MW AF Brune, C. R. Caggiano, J. A. Sayre, D. B. Bacher, A. D. Hale, G. M. Paris, M. W. TI R-matrix description of particle energy spectra produced by low-energy H-3 + H-3 reactions SO PHYSICAL REVIEW C LA English DT Article ID 3 CHARGED-PARTICLES; NEUTRON SPECTRUM; SCATTERING; DECAY; T&T AB An R-matrix model for three-body final states is presented and applied to a recent measurement of the neutron energy spectrum from the H-3 + H-3 -> 2n + alpha reaction. The calculation includes the n alpha and nn interactions in the final state, angular momentum conservation, antisymmetrization, and the interference between different channels. A good fit to the measured spectrum is obtained, where clear evidence for the He-5 ground state is observed. The model is also used to predict the alpha-particle spectrum from H-3 + H-3 as well as particle spectra from He-3 + He-3. The R-matrix approach presented here is very general and can be adapted to a wide variety of problems with three-body final states. C1 [Brune, C. R.] Ohio Univ, Dept Phys & Astron, Edwards Accelerator Lab, Athens, OH 45701 USA. [Caggiano, J. A.; Sayre, D. B.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Bacher, A. D.] Indiana Univ, Cyclotron Facil IUCF, Bloomington, IN 47408 USA. [Hale, G. M.; Paris, M. W.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Brune, CR (reprint author), Ohio Univ, Dept Phys & Astron, Edwards Accelerator Lab, Athens, OH 45701 USA. FU U.S. Department of Energy [DE-FG02-88ER40387, DE-NA0001837, DE-AC52-06NA25396, DE-AC52-07NA27344]; Lawrence Livermore National Laboratory FX We thank Johan Frenje, Maria Gatu-Johnson, Dennis McNabb, Dieter Schneider, Ian Thompson, and Alex Zylstra for useful discussions. The work was supported in part by the U.S. Department of Energy, under Grants No. DE-FG02-88ER40387, No. DE-NA0001837, No. DE-AC52-06NA25396, and No. DE-AC52-07NA27344, and by Lawrence Livermore National Laboratory. NR 26 TC 7 Z9 7 U1 2 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JUL 20 PY 2015 VL 92 IS 1 AR 014003 DI 10.1103/PhysRevC.92.014003 PG 13 WC Physics, Nuclear SC Physics GA CN2MQ UT WOS:000358256000001 ER PT J AU Bar-Shalom, S Soni, A Wudka, J AF Bar-Shalom, Shaouly Soni, Amarjit Wudka, Jose TI Effective field theory analysis of Higgs naturalness SO PHYSICAL REVIEW D LA English DT Article ID ONE-COMPONENT MODEL; STANDARD-MODEL; VACUUM STABILITY; RENORMALIZATION GROUP; TRIVIALITY BOUNDS; SCALING LAWS; BOSON MASS; PHASE; LHC AB Assuming the presence of physics beyond the Standard Model (SM) with a characteristic scale M similar to O(10) TeV, we investigate the naturalness of the Higgs sector at scales below M using an effective field theory (EFT) approach. We obtain the complete set of higher-dimensional effective operators (at any dimension n >= 5) that give the leading one-loop EFT contributions to the Higgs mass with aWilsonian-like hard cutoff and discuss the (fine-) tuning between these terms and the SM one-loop contribution, which is required in order to alleviate the little hierarchy problem. We then show that this tuning can be translated into a condition for naturalness in the underlying new physics, a condition we denote by " EFT naturalness" and which we express as constraints on the corresponding higher-dimensional operator coefficients up to the scale of the effective action Lambda < M. We also determine the types of physics that can lead to EFT naturalness and discuss the current experimental constraints on the relevant operator coefficients. We show that these types of new physics are best probed in vector-boson and multiple-Higgs production. C1 [Bar-Shalom, Shaouly] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Soni, Amarjit] Brookhaven Natl Lab, Theory Grp, Upton, NY 11973 USA. [Wudka, Jose] Univ Calif Riverside, Dept Phys, Riverside, CA 92521 USA. RP Bar-Shalom, S (reprint author), Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. EM shaouly@physics.technion.ac.il; adlersoni@gmail.com; jose.wudka@ucr.edu FU U.S. Department of Energy [DE-AC02-98CH10886(BNL)]; UCR CoR grant FX `` We thank Michael Trott for making useful comments on the manuscript. The work of A. S. was supported in part by U.S. Department of Energy Contract No. DE-AC02-98CH10886(BNL) and J. W. is supported in part by a UCR CoR grant. NR 46 TC 2 Z9 2 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 20 PY 2015 VL 92 IS 1 AR 015018 DI 10.1103/PhysRevD.92.015018 PG 10 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CN2MW UT WOS:000358256700007 ER PT J AU Han, YL Wang, XL Yuan, CZ Shen, CP Wang, P Abdesselam, A Adachi, I Aihara, H Al Said, S Asner, DM Aushev, T Babu, V Badhrees, I Bansal, V Bhardwaj, V Biswal, J Bozek, A Bracko, M Chen, A Cheon, BG Chistov, R Cho, K Chobanova, V Choi, SK Cinabro, D Dalseno, J Danilov, M Dolezal, Z Drutskoy, A Dutta, D Eidelman, S Farhat, H Fast, JE Ferber, T Fulsom, BG Gaur, V Gabyshev, N Garmash, A Getzkow, D Gillard, R Glattauer, R Goh, YM Goldenzweig, P Golob, B Haba, J Hayasaka, K Hayashii, H He, XH Horiguchi, T Hou, WS Iijima, T Ishikawa, A Jaegle, I Joffe, D Joo, KK Kichimi, H Kim, DY Kim, JB Kim, JH Kim, KT Kim, SH Kim, YJ Kinoshita, K Ko, BR Kodys, P Krizan, P Krokovny, P Lewis, P Gioi, LL Libby, J Liventsev, D Lukin, P Masuda, M Matvienko, D Miyabayashi, K Miyata, H Mizuk, R Moll, A Moon, HK Mussa, R Nakano, E Nakao, M Nayak, M Nisar, NK Nishida, S Ogawa, S Okuno, S Ostrowicz, W Pakhlov, P Pakhlova, G Pal, B Park, H Pedlar, TK Pestotnik, R Petric, M Piilonen, LE Pulvermacher, C Ribezl, E Ritter, M Rostomyan, A Sahoo, H Sakai, Y Sandilya, S Santelj, L Sanuki, T Schneider, O Schnell, G Schwanda, C Senyo, K Sevior, ME Shapkin, M Shebalin, V Shibata, TA Shiu, JG Shwartz, B Simon, F Sohn, YS Sokolov, A Solovieva, E Stanic, S Steder, M Sumihama, M Tamponi, U Teramoto, Y Uchida, M Uehara, S Uglov, T Unno, Y Uno, S Usov, Y Van Hulse, C Vanhoefer, P Varner, G Vossen, A Wagner, MN Watanabe, Y Williams, KM Yashchenko, S Yook, Y Zhang, CC Zhang, ZP Zhilich, V Zhulanov, V Zupanc, A AF Han, Y. L. Wang, X. L. Yuan, C. Z. Shen, C. P. Wang, P. Abdesselam, A. Adachi, I. Aihara, H. Al Said, S. Asner, D. M. Aushev, T. Babu, V. Badhrees, I. Bansal, V. Bhardwaj, V. Biswal, J. Bozek, A. Bracko, M. Chen, A. Cheon, B. G. Chistov, R. Cho, K. Chobanova, V. Choi, S. -K. Cinabro, D. Dalseno, J. Danilov, M. Dolezal, Z. Drutskoy, A. Dutta, D. Eidelman, S. Farhat, H. Fast, J. E. Ferber, T. Fulsom, B. G. Gaur, V. Gabyshev, N. Garmash, A. Getzkow, D. Gillard, R. Glattauer, R. Goh, Y. M. Goldenzweig, P. Golob, B. Haba, J. Hayasaka, K. Hayashii, H. He, X. H. Horiguchi, T. Hou, W. -S. Iijima, T. Ishikawa, A. Jaegle, I. Joffe, D. Joo, K. K. Kichimi, H. Kim, D. Y. Kim, J. B. Kim, J. H. Kim, K. T. Kim, S. H. Kim, Y. J. Kinoshita, K. Ko, B. R. Kodys, P. Krizan, P. Krokovny, P. Lewis, P. Gioi, L. Li Libby, J. Liventsev, D. Lukin, P. Masuda, M. Matvienko, D. Miyabayashi, K. Miyata, H. Mizuk, R. Moll, A. Moon, H. K. Mussa, R. Nakano, E. Nakao, M. Nayak, M. Nisar, N. K. Nishida, S. Ogawa, S. Okuno, S. Ostrowicz, W. Pakhlov, P. Pakhlova, G. Pal, B. Park, H. Pedlar, T. K. Pestotnik, R. Petric, M. Piilonen, L. E. Pulvermacher, C. Ribezl, E. Ritter, M. Rostomyan, A. Sahoo, H. Sakai, Y. Sandilya, S. Santelj, L. Sanuki, T. Schneider, O. Schnell, G. Schwanda, C. Senyo, K. Sevior, M. E. Shapkin, M. Shebalin, V. Shibata, T. -A. Shiu, J. -G. Shwartz, B. Simon, F. Sohn, Y. -S. Sokolov, A. Solovieva, E. Stanic, S. Steder, M. Sumihama, M. Tamponi, U. Teramoto, Y. Uchida, M. Uehara, S. Uglov, T. Unno, Y. Uno, S. Usov, Y. Van Hulse, C. Vanhoefer, P. Varner, G. Vossen, A. Wagner, M. N. Watanabe, Y. Williams, K. M. Yashchenko, S. Yook, Y. Zhang, C. C. Zhang, Z. P. Zhilich, V. Zhulanov, V. Zupanc, A. CA Belle Collaboration TI Measurement of e(+)e(-) -> gamma chi(cJ) via initial state radiation at Belle SO PHYSICAL REVIEW D LA English DT Article ID CROSS-SECTION; ANNIHILATION; KEKB AB The process e(+)e(-) -> gamma chi(cJ) (J = 1, 2) is studied via initial state radiation using 980 fb(-1) of data at and around the Gamma(nS) (n = 1, 2, 3, 4, 5) resonances collected with the Belle detector at the KEKB asymmetricenergy e(+)e(-) collider. No significant signal is observed except from psi(2S) decays. Upper limits on the cross sections between root s = 3.80 and 5.56 GeV are determined at the 90% credibility level, which range from a few pb to a few tens of pb. We also set upper limits on the decay rate of the vector charmonium [psi(4040), psi(4160), and psi(4415)] and charmoniumlike [Y(4260), Y(4360), and Y(4660)] states to gamma chi(cJ). C1 [Schnell, G.; Van Hulse, C.] Univ Basque Country, UPV EHU, Bilbao 48080, Spain. [Shen, C. P.] Beihang Univ, Beijing 100191, Peoples R China. [Eidelman, S.; Gabyshev, N.; Garmash, A.; Krokovny, P.; Lukin, P.; Matvienko, D.; Shebalin, V.; Shwartz, B.; Usov, Y.; Zhilich, V.; Zhulanov, V.] RAS, Budker Inst Nucl Phys, SB, Novosibirsk 630090, Russia. [Dolezal, Z.; Kodys, P.] Charles Univ Prague, Fac Math & Phys, CR-12116 Prague, Czech Republic. [Joo, K. K.] Chonnam Natl Univ, Kwangju 660701, South Korea. [Kinoshita, K.; Pal, B.] Univ Cincinnati, Cincinnati, OH 45221 USA. [Ferber, T.; Rostomyan, A.; Steder, M.; Yashchenko, S.] Deutsches Elektronen Synchrotron, D-22607 Hamburg, Germany. [Getzkow, D.; Wagner, M. N.] Univ Giessen, D-35392 Giessen, Germany. [Sumihama, M.] Gifu Univ, Gifu 5011193, Japan. [Adachi, I.; Haba, J.; Nakao, M.; Nishida, S.; Sakai, Y.; Uehara, S.; Uno, S.] Grad Univ Adv Studies, SOKENDAI, Hayama, Kanagawa 2400193, Japan. [Choi, S. -K.] Gyeongsang Natl Univ, Chinju 660701, South Korea. [Cheon, B. G.; Goh, Y. M.; Kim, S. H.; Unno, Y.] Hanyang Univ, Seoul 133791, South Korea. [Jaegle, I.; Lewis, P.; Sahoo, H.; Varner, G.] Univ Hawaii, Honolulu, HI 96822 USA. [Adachi, I.; Haba, J.; Kichimi, H.; Liventsev, D.; Nakao, M.; Nishida, S.; Sakai, Y.; Santelj, L.; Uehara, S.; Uno, S.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki 3050801, Japan. [Schnell, G.] Ikerbasque, Basque Fdn Sci, Bilbao 48013, Spain. [Libby, J.; Nayak, M.] Indian Inst Technol, Madras 600036, Tamil Nadu, India. [Vossen, A.] Indiana Univ, Bloomington, IN 47408 USA. [Han, Y. L.; Yuan, C. Z.; Wang, P.; Zhang, C. C.] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Glattauer, R.; Schwanda, C.] Inst High Energy Phys, A-1050 Vienna, Austria. [Shapkin, M.; Sokolov, A.] Inst High Energy Phys, Protvino 142281, Russia. [Mussa, R.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Aushev, T.; Chistov, R.; Danilov, M.; Drutskoy, A.; Mizuk, R.; Pakhlov, P.; Pakhlova, G.; Solovieva, E.; Uglov, T.] Inst Theoret & Expt Phys, Moscow 117218, Russia. [Biswal, J.; Bracko, M.; Golob, B.; Krizan, P.; Pestotnik, R.; Petric, M.; Ribezl, E.; Zupanc, A.] Jozef Stefan Inst, Ljubljana 1000, Slovenia. [Watanabe, Y.] Kanagawa Univ, Yokohama, Kanagawa 2218686, Japan. [Goldenzweig, P.; Okuno, S.; Pulvermacher, C.] Karlsruhe Inst Technol, Inst Expt Kernphys, D-76131 Karlsruhe, Germany. [Joffe, D.] Kennesaw State Univ, Kennesaw, GA 30144 USA. [Badhrees, I.] King Abdulaziz City Sci & Technol, Riyadh 11442, Saudi Arabia. [Al Said, S.] King Abdulaziz Univ, Fac Sci, Dept Phys, Jeddah 21589, Saudi Arabia. [Cho, K.; Kim, J. H.; Kim, Y. J.] Korea Inst Sci & Technol Informat, Daejeon 305806, South Korea. [Kim, J. B.; Kim, K. T.; Ko, B. R.; Moon, H. K.] Korea Univ, Seoul 136713, South Korea. [Park, H.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Schneider, O.] Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland. [Golob, B.; Krizan, P.] Univ Ljubljana, Fac Math & Phys, Ljubljana 1000, Slovenia. [Pedlar, T. K.] Luther Coll, Decorah, IA 52101 USA. [Bracko, M.] Univ Maribor, SLO-2000 Maribor, Slovenia. [Chobanova, V.; Dalseno, J.; Gioi, L. Li; Moll, A.; Ritter, M.; Simon, F.; Vanhoefer, P.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Sevior, M. E.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Danilov, M.; Drutskoy, A.; Mizuk, R.; Pakhlov, P.] Moscow Phys Engn Inst, Moscow 115409, Russia. [Aushev, T.; Pakhlova, G.; Uglov, T.] Moscow Inst Phys & Technol, Dolgoprudnyi 141700, Moscow Region, Russia. [Iijima, T.] Nagoya Univ, Sch Sci, Nagoya, Aichi 4648602, Japan. [Hayasaka, K.; Iijima, T.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648602, Japan. [Hayashii, H.; Miyabayashi, K.] Nara Womens Univ, Nara 6308506, Japan. [Chen, A.] Natl Cent Univ, Chungli 32054, Taiwan. [Hou, W. -S.; Shiu, J. -G.] Natl Taiwan Univ, Dept Phys, Taipei 10617, Taiwan. [Bozek, A.; Ostrowicz, W.] H Niewodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. [Miyata, H.] Niigata Univ, Niigata 9502181, Japan. [Stanic, S.] Univ Nova Gorica, Nova Gorica 5000, Slovenia. [Eidelman, S.; Gabyshev, N.; Garmash, A.; Krokovny, P.; Lukin, P.; Matvienko, D.; Shebalin, V.; Shwartz, B.; Usov, Y.; Zhilich, V.; Zhulanov, V.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Nakano, E.; Teramoto, Y.] Osaka City Univ, Osaka 5588585, Japan. [Asner, D. M.; Bansal, V.; Fast, J. E.; Fulsom, B. G.] Pacific NW Natl Lab, Richland, WA 99352 USA. [He, X. H.] Peking Univ, Beijing 100871, Peoples R China. [Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Kim, D. Y.] Soongsil Univ, Seoul 156743, South Korea. [Bhardwaj, V.] Univ S Carolina, Columbia, SC 29208 USA. [Abdesselam, A.; Al Said, S.; Badhrees, I.] Univ Tabuk, Fac Sci, Dept Phys, Tabuk 71451, Saudi Arabia. [Babu, V.; Dutta, D.; Gaur, V.; Nisar, N. K.; Sandilya, S.] Tata Inst Fundamental Res, Mumbai 400005, Maharashtra, India. [Dalseno, J.; Moll, A.; Simon, F.] Tech Univ Munich, Excellence Cluster Universe, D-85748 Garching, Germany. [Ogawa, S.] Toho Univ, Funabashi, Chiba 2748510, Japan. [Horiguchi, T.; Ishikawa, A.; Sanuki, T.] Tohoku Univ, Sendai, Miyagi 9808578, Japan. [Masuda, M.] Univ Tokyo, Earthquake Res Inst, Tokyo 1130032, Japan. [Aihara, H.] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Shibata, T. -A.; Uchida, M.] Tokyo Inst Technol, Tokyo 1528550, Japan. [Tamponi, U.] Univ Turin, I-10124 Turin, Italy. [Wang, X. L.; Liventsev, D.; Piilonen, L. E.; Williams, K. M.] Virginia Polytech Inst & State Univ, CNP, Blacksburg, VA 24061 USA. [Cinabro, D.; Farhat, H.; Gillard, R.] Wayne State Univ, Detroit, MI 48202 USA. [Senyo, K.] Yamagata Univ, Yamagata 9908560, Japan. [Sohn, Y. -S.; Yook, Y.] Yonsei Univ, Seoul 120749, South Korea. RP Han, YL (reprint author), Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. RI Aihara, Hiroaki/F-3854-2010; Pakhlova, Galina/C-5378-2014; Pakhlov, Pavel/K-2158-2013; Uglov, Timofey/B-2406-2014; Danilov, Mikhail/C-5380-2014; Mizuk, Roman/B-3751-2014; Krokovny, Pavel/G-4421-2016; EPFL, Physics/O-6514-2016; Chistov, Ruslan/B-4893-2014; Drutskoy, Alexey/C-8833-2016; Solovieva, Elena/B-2449-2014; Faculty of, Sciences, KAU/E-7305-2017 OI Aihara, Hiroaki/0000-0002-1907-5964; Han, Yanliang/0000-0003-3769-8759; Pakhlova, Galina/0000-0001-7518-3022; Pakhlov, Pavel/0000-0001-7426-4824; Uglov, Timofey/0000-0002-4944-1830; Danilov, Mikhail/0000-0001-9227-5164; Krokovny, Pavel/0000-0002-1236-4667; Chistov, Ruslan/0000-0003-1439-8390; Drutskoy, Alexey/0000-0003-4524-0422; Solovieva, Elena/0000-0002-5735-4059; FU Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan; Japan Society for the Promotion of Science (JSPS); Tau-Lepton Physics Research Center of Nagoya University; Australian Research Council; Australian Department of Industry, Innovation, Science and Research; Austrian Science Fund [P 22742-N16, P 26794-N20]; National Natural Science Foundation of China [10575109, 10775142, 10875115, 11175187, 11475187]; Chinese Academy of Science Center for Excellence in Particle Physics; Ministry of Education, Youth, and Sports of the Czech Republic [LG14034]; Carl Zeiss Foundation; Deutsche Forschungsgemeinschaft; VolkswagenStiftung; Department of Science and Technology of India; Istituto Nazionale di Fisica Nucleare of Italy; National Research Foundation (NRF) of Korea [20110029457, 2012-0008143, 2012R1A1A2008330, 2013R1A1A3007772, 2014R1A2A2A01005286, 2014R1A2A2A01002734, 2014R1A1A2006456]; Basic Research Lab program under NRF [KRF-2011-0020333, KRF-2011-0021196]; Center for Korean J-PARC Users [NRF-2013K1A3A7A06056592]; Brain Korea 21-Plus program; Global Science Experimental Data Hub Center of the Korea Institute of Science and Technology Information; Polish Ministry of Science and Higher Education; National Science Center; Ministry of Education and Science of the Russian Federation; Russian Foundation for Basic Research; Slovenian Research Agency; Basque Foundation for Science (IKERBASQUE); Euskal Herriko Unibertsitatea (UPV/EHU) (Spain) [UFI 11/55]; Swiss National Science Foundation; National Science Council; Ministry of Education of Taiwan; U.S. Department of Energy; National Science Foundation; MEXT for Science Research in a Priority Area ("New Development of Flavor Physics"); JSPS for Creative Scientific Research ("Evolution of Tau-lepton Physics") FX We thank the KEKB group for the excellent operation of the accelerator; the KEK cryogenics group for the efficient operation of the solenoid; and the KEK computer group, the National Institute of Informatics, and the PNNL/EMSL computing group for valuable computing and SINET4 network support. We acknowledge support from the Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan, the Japan Society for the Promotion of Science (JSPS), and the Tau-Lepton Physics Research Center of Nagoya University; the Australian Research Council and the Australian Department of Industry, Innovation, Science and Research; Austrian Science Fund under Grants No. P 22742-N16 and No. P 26794-N20; the National Natural Science Foundation of China under Grants No. 10575109, No. 10775142, No. 10875115, No. 11175187, and No. 11475187; the Chinese Academy of Science Center for Excellence in Particle Physics; the Ministry of Education, Youth, and Sports of the Czech Republic under Grant No. LG14034; the Carl Zeiss Foundation, the Deutsche Forschungsgemeinschaft and the VolkswagenStiftung; the Department of Science and Technology of India; the Istituto Nazionale di Fisica Nucleare of Italy; National Research Foundation (NRF) of Korea Grants No. 20110029457, No. 2012-0008143, No. 2012R1A1A2008330, No. 2013R1A1A3007772, No. 2014R1A2A2A01005286, No. 2014R1A2A2A01002734, and No. 2014R1A1A2006456; the Basic Research Lab program under NRF Grants No. KRF-2011-0020333 and No. KRF-2011-0021196, Center for Korean J-PARC Users, Grant No. NRF-2013K1A3A7A06056592; the Brain Korea 21-Plus program and the Global Science Experimental Data Hub Center of the Korea Institute of Science and Technology Information; the Polish Ministry of Science and Higher Education and the National Science Center; the Ministry of Education and Science of the Russian Federation and the Russian Foundation for Basic Research; the Slovenian Research Agency; the Basque Foundation for Science (IKERBASQUE) and the Euskal Herriko Unibertsitatea (UPV/EHU) under Grant No. UFI 11/55 (Spain); the Swiss National Science Foundation; the National Science Council and the Ministry of Education of Taiwan; and the U.S. Department of Energy and the National Science Foundation. This work is supported by a Grant-in-Aid from MEXT for Science Research in a Priority Area ("New Development of Flavor Physics") and from JSPS for Creative Scientific Research ("Evolution of Tau-lepton Physics"). NR 26 TC 0 Z9 1 U1 3 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 20 PY 2015 VL 92 IS 1 AR 012011 DI 10.1103/PhysRevD.92.012011 PG 9 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CN2MW UT WOS:000358256700001 ER PT J AU Banci, L Brimble, MA Lee, H Najera, C Sessoli, R AF Banci, L. Brimble, M. A. Lee, H. Najera, C. Sessoli, R. TI IUPAC 2015 Distinguished Women in Chemistry or Chemical Engineering SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT News Item C1 [Banci, L.; Sessoli, R.] Univ Florence, I-50121 Florence, Italy. [Brimble, M. A.] Univ Auckland, Auckland 1, New Zealand. [Lee, H.] Korea Adv Inst Sci & Technol, Taejon, South Korea. [Lee, H.] CALTECH, Pasadena, CA 91125 USA. [Lee, H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Lee, H.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Najera, C.] Univ Alicante, Alicante, Spain. RP Banci, L (reprint author), Univ Florence, I-50121 Florence, Italy. NR 0 TC 0 Z9 0 U1 1 U2 32 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD JUL 20 PY 2015 VL 54 IS 30 BP 8593 EP 8593 DI 10.1002/anie.201505537 PG 1 WC Chemistry, Multidisciplinary SC Chemistry GA CM9TJ UT WOS:000358051600003 ER PT J AU Margulies, EA Wu, YL Gawel, P Miller, SA Shoer, LE Schaller, RD Diederich, F Wasielewski, MR AF Margulies, Eric A. Wu, Yi-Lin Gawel, Przemyslaw Miller, Stephen A. Shoer, Leah E. Schaller, Richard D. Diederich, Francois Wasielewski, Michael R. TI Sub-Picosecond Singlet Exciton Fission in Cyano-Substituted Diaryltetracenes SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE chromophores; photophysics; singlet fission; tetracene derivatives; time-resolved spectroscopy ID TRIPLET EXCITONS; TETRACENE CRYSTALS; ENERGY-TRANSFER; NANOCRYSTALS; MOLECULES; MECHANISM; FUSION AB Thin films of 5,11-dicyano-6,12-diphenyltetracene (TcCN) have been studied for their ability to undergo singlet exciton fission (SF). Functionalization of tetracene with cyano substituents yields a more stable chromophore with favorable energetics for exoergic SF (2E(T-1)-E(S-1)=-0.17eV), where S-1 and T-1 are singlet and triplet excitons, respectively. As a result of tuning the triplet-state energy, SF is faster in TcCN relative to the corresponding endoergic process in tetracene. SF proceeds with two time constants in the film samples (=0.8 +/- 0.2ps and =23 +/- 3ps), which is attributed to structural disorder within the film giving rise to one population with a favorable interchromophore geometry, which undergoes rapid SF, and a second population in which the initially formed singlet exciton must diffuse to a site at which this favorable geometry exists. A triplet yield analysis using transient absorption spectra indicates the formation of 1.6 +/- 0.3 triplets per initial excited state. C1 [Margulies, Eric A.; Wu, Yi-Lin; Miller, Stephen A.; Shoer, Leah E.; Wasielewski, Michael R.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Margulies, Eric A.; Wu, Yi-Lin; Miller, Stephen A.; Shoer, Leah E.; Wasielewski, Michael R.] Northwestern Univ, ANSER Ctr, Evanston, IL 60208 USA. [Schaller, Richard D.] Northwestern Univ, Dept Chem, Argonne, IL 60439 USA. [Schaller, Richard D.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Gawel, Przemyslaw; Diederich, Francois] Swiss Fed Inst Technol, Organ Chem Lab, CH-8093 Zurich, Switzerland. RP Diederich, F (reprint author), Swiss Fed Inst Technol, Organ Chem Lab, Vladimir Prelog Weg 3,HCI, CH-8093 Zurich, Switzerland. EM diederich@org.chem.ethz.ch; m-wasielewski@northwestern.edu OI Wu, Yi-Lin/0000-0003-0253-1625; Gawel, Przemyslaw/0000-0003-1555-376X FU Chemical Sciences, Geosciences, and Biosciences Division, Office of Basic Energy Sciences, U.S. Department of Energy (DOE) [DE-FG02-99ER14999]; Swiss National Science Foundation; ERC [246637]; Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility [DE-AC02-06CH11357]; National Science Foundation MRSEC program [DMR-1121262] FX This work was supported by the Chemical Sciences, Geosciences, and Biosciences Division, Office of Basic Energy Sciences, U.S. Department of Energy (DOE), under Grant No. DE-FG02-99ER14999 (M.R.W.), the Swiss National Science Foundation, and the ERC Advanced Grant No. 246637 ("OPTELOMAC"). This work was performed, in part, at the Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility under Contract No. DE-AC02-06CH11357. This work made use of the J. B. Cohen X-ray Diffraction Facility at the Materials Research Center of Northwestern University supported by the National Science Foundation MRSEC program (DMR-1121262). We thank Dr. Matthew Krzyaniak and Dr. Samuel Eaton for help with data analysis, acquiring time-resolved fluorescence data, and helpful discussions. NR 29 TC 8 Z9 8 U1 11 U2 59 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD JUL 20 PY 2015 VL 54 IS 30 BP 8679 EP 8683 DI 10.1002/anie.201501355 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA CM9TJ UT WOS:000358051600015 PM 26097009 ER PT J AU Wei, XL Xu, W Huang, JH Zhang, L Walter, E Lawrence , C Vijayakumar, M Henderson, WA Liu, TB Cosimbescu, L Li, B Sprenkle, V Wang, W AF Wei, Xiaoliang Xu, Wu Huang, Jinhua Zhang, Lu Walter, Eric Lawrence, Chad Vijayakumar, M. Henderson, Wesley A. Liu, Tianbiao Cosimbescu, Lelia Li, Bin Sprenkle, Vincent Wang, Wei TI Radical Compatibility with Nonaqueous Electrolytes and Its Impact on an All-Organic Redox Flow Battery SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE electrochemistry; electrolyte optimization; ESR spectroscopy; nonaqueous redox flow batteries; radicals ID RESEARCH-AND-DEVELOPMENT; ENERGY-STORAGE; PROGRESS; PERFORMANCE AB Nonaqueous redox flow batteries hold the promise of achieving higher energy density because of the broader voltage window than aqueous systems, but their current performance is limited by low redox material concentration, cell efficiency, cycling stability, and current density. We report a new nonaqueous all-organic flow battery based on high concentrations of redox materials, which shows significant, comprehensive improvement in flow battery performance. A mechanistic electron spin resonance study reveals that the choice of supporting electrolytes greatly affects the chemical stability of the charged radical species especially the negative side radical anion, which dominates the cycling stability of these flow cells. This finding not only increases our fundamental understanding of performance degradation in flow batteries using radical-based redox species, but also offers insights toward rational electrolyte optimization for improving the cycling stability of these flow batteries. C1 [Wei, Xiaoliang; Xu, Wu; Walter, Eric; Lawrence, Chad; Vijayakumar, M.; Henderson, Wesley A.; Liu, Tianbiao; Cosimbescu, Lelia; Li, Bin; Sprenkle, Vincent; Wang, Wei] Pacific NW Natl Lab, Richland, WA 99352 USA. [Huang, Jinhua; Zhang, Lu] Argonne Natl Lab, Argonne, IL 60439 USA. [Wei, Xiaoliang; Huang, Jinhua; Zhang, Lu; Wang, Wei] Joint Ctr Energy Storage Res, San Francisco, CA USA. RP Wei, XL (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99352 USA. EM Xiaoliang.Wei@pnnl.gov; Wei.Wang@pnnl.gov RI Wang, Wei/F-4196-2010; Liu, Tianbiao/A-3390-2011; Walter, Eric/P-9329-2016; OI Wang, Wei/0000-0002-5453-4695; Xu, Wu/0000-0002-2685-8684 FU U.S. Department of Energy's (DOE's) Office of Electricity Delivery and Energy Reliability (OE) [57558]; Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub - U.S. Department of Energy, Office of Science, Basic Energy Sciences; William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility - DOE's Office of Biological and Environmental Research [48374, 48293]; DOE [DE-AC05-76L01830] FX This research was financially supported by the U.S. Department of Energy's (DOE's) Office of Electricity Delivery and Energy Reliability (OE) under contract number 57558 (flow chemistry development and electrochemical tests); by the Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences (synthesis of DBMMB); and by the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research, under proposal numbers 48374 and 48293 (ESR measurements). PNNL is a multi-program national laboratory operated by Battelle for DOE under contract number DE-AC05-76L01830. NR 25 TC 40 Z9 40 U1 14 U2 110 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD JUL 20 PY 2015 VL 54 IS 30 BP 8684 EP 8687 DI 10.1002/anie.201501443 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA CM9TJ UT WOS:000358051600016 PM 25891480 ER PT J AU Parker, DSN Kaiser, RI Kostko, O Ahmed, M AF Parker, Dorian S. N. Kaiser, Ralf. I. Kostko, Oleg Ahmed, Musahid TI Selective Formation of Indene through the Reaction of Benzyl Radicals with Acetylene SO CHEMPHYSCHEM LA English DT Article DE combustion; gas-phase chemistry; mass spectrometry; polycyclic aromatic hydrocarbons; radicals ID POLYCYCLIC AROMATIC-HYDROCARBONS; PHENYL RADICALS; LOW-PRESSURE; AB-INITIO; FLAMES; PHOTOIONIZATION; PYROLYSIS; NAPHTHALENE; PATHWAYS; BENZENE AB The combustion of fossil fuels forms polycyclic aromatic hydrocarbons (PAHs) composed of five-and six-membered aromatic rings, such as indene (C9H8), which are carcinogenic, mutagenic, and deleterious to the environment. Indene, the simplest PAH with single five-and six-membered rings, has been predicted theoretically to be formed through the reaction of benzyl radicals with acetylene. Benzyl radicals are found in significant concentrations in combustion flames, owing to their highly stable aromatic and resonantly stabilized free-radical character. We provide compelling experimental evidence that indene is synthesized through the reaction of the benzyl radical (C7H7) with acetylene (C2H2) under combustion-like conditions at 600 K. The mechanism involves an initial addition step followed by cyclization and aromatization through atomic hydrogen loss. This reaction was found to form the indene isomer exclusively, which, in conjunction with the high concentrations of benzyl and acetylene in combustion environments, indicates that this pathway is the predominant route to synthesize the prototypical five-and six-membered PAH. C1 [Parker, Dorian S. N.; Kaiser, Ralf. I.] Univ Hawaii Manoa, Dept Chem, Honolulu, HI 96822 USA. [Kostko, Oleg; Ahmed, Musahid] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Kaiser, RI (reprint author), Univ Hawaii Manoa, Dept Chem, Honolulu, HI 96822 USA. EM ralfk@hawaii.edu; mahmed@lbl.gov RI Kostko, Oleg/B-3822-2009; Ahmed, Musahid/A-8733-2009 OI Kostko, Oleg/0000-0003-2068-4991; NR 31 TC 8 Z9 8 U1 3 U2 28 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1439-4235 EI 1439-7641 J9 CHEMPHYSCHEM JI ChemPhysChem PD JUL 20 PY 2015 VL 16 IS 10 BP 2091 EP 2093 DI 10.1002/cphc.201500313 PG 3 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CM8IU UT WOS:000357943900005 PM 25917234 ER PT J AU Parashar, V Durand, CP Hao, BY Amorim, RG Pandey, R Tiwari, B Zhang, DY Liu, Y Li, AP Yap, YK AF Parashar, Vyom Durand, Corentin P. Hao, Boyi Amorim, Rodrigo G. Pandey, Ravindra Tiwari, Bishnu Zhang, Dongyan Liu, Yang Li, An-Ping Yap, Yoke Khin TI Switching Behaviors of Graphene-Boron Nitride Nanotube Heterojunctions SO SCIENTIFIC REPORTS LA English DT Article ID BALLISTIC TRANSPORT; BILAYER GRAPHENE; ROOM-TEMPERATURE; ELECTRON-GAS; HETEROSTRUCTURES; GROWTH AB High electron mobility of graphene has enabled their application in high-frequency analogue devices but their gapless nature has hindered their use in digital switches. In contrast, the structural analogous, h-BN sheets and BN nanotubes (BNNTs) are wide band gap insulators. Here we show that the growth of electrically insulating BNNTs on graphene can enable the use of graphene as effective digital switches. These graphene-BNNT heterojunctions were characterized at room temperature by four-probe scanning tunneling microscopy (4-probe STM) under real-time monitoring of scanning electron microscopy (SEM). A switching ratio as high as 10(5) at a turn-on voltage as low as 0.5 V were recorded. Simulation by density functional theory (DFT) suggests that mismatch of the density of states (DOS) is responsible for these novel switching behaviors. C1 [Parashar, Vyom; Hao, Boyi; Amorim, Rodrigo G.; Pandey, Ravindra; Tiwari, Bishnu; Zhang, Dongyan; Yap, Yoke Khin] Michigan Technol Univ, Dept Phys, Houghton, MI 49931 USA. [Durand, Corentin P.; Li, An-Ping] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Liu, Yang] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. RP Yap, YK (reprint author), Michigan Technol Univ, Dept Phys, 1400 Townsend Dr, Houghton, MI 49931 USA. EM ykyap@mtu.edu RI Amorim, Rodrigo/N-4139-2016; Li, An-Ping/B-3191-2012 OI Amorim, Rodrigo/0000-0001-9611-8772; Li, An-Ping/0000-0003-4400-7493 FU U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division [DE-SC0012762]; US Army Research Laboratory, Weapons and Materials Directorate "Hybrid Nano and Nano-Bio Materials" Program; Center for Nanophase Materials Sciences [CNMS2012-083]; Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, the U.S. Department of Energy; Center for Integrated Nanotechnologies [U2011A1074]; U.S. Department of Energy, Office of Science by Los Alamos National Laboratory [DE-AC52-06NA25396]; Sandia National Laboratories [DE-AC04-94AL85000] FX This work is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division (Grant DE-SC0012762). The theoretical effort is supported by the US Army Research Laboratory, Weapons and Materials Directorate "Hybrid Nano and Nano-Bio Materials" Program. Part of the experimental work was conducted at the Center for Nanophase Materials Sciences (Project CNMS2012-083), which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, the U.S. Department of Energy. Part of this work was performed at the Center for Integrated Nanotechnologies (Project U2011A1074), an Office of Science User Facility operated for the U.S. Department of Energy, Office of Science by Los Alamos National Laboratory (Contract DE-AC52-06NA25396) and Sandia National Laboratories (Contract DE-AC04-94AL85000). NR 27 TC 4 Z9 4 U1 2 U2 70 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUL 20 PY 2015 VL 5 AR 12238 DI 10.1038/srep12238 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CN1AS UT WOS:000358148100003 PM 26192733 ER PT J AU Wang, JX Zhang, Y Capuano, CB Ayers, KE AF Wang, Jia X. Zhang, Yu Capuano, Christopher B. Ayers, Katherine E. TI Ultralow charge-transfer resistance with ultralow Pt loading for hydrogen evolution and oxidation using Ru@Pt core-shell nanocatalysts SO SCIENTIFIC REPORTS LA English DT Article ID HIGH-MASS TRANSPORT; WATER ELECTROLYSIS; ACIDIC MEDIA; ELECTROOXIDATION; ELECTRODES; CATALYSTS; NANOPARTICLES; PERFORMANCE; DEPOSITION; SURFACES AB We evaluated the activities of well-defined Ru@Pt core-shell nanocatalysts for hydrogen evolution and oxidation reactions (HER-HOR) using hanging strips of gas diffusion electrode (GDE) in solution cells. With gas transport limitation alleviated by micro-porous channels in the GDEs, the charge transfer resistances (CTRs) at the hydrogen reversible potential were conveniently determined from linear fit of ohmic-loss-corrected polarization curves. In 1 M HClO4 at 23 degrees C, a CTR as low as 0.04 Omega cm(-2) was obtained with only 20 mu g cm(-2) Pt and 11 mu g cm(-2) Ru using the carbon-supported Ru@Pt with 1:1 Ru: Pt atomic ratio. Derived from temperature-dependent CTRs, the activation barrier of the Ru@Pt catalyst for the HER-HOR in acids is 0.2 eV or 19 kJ mol(-1). Using the Ru@Pt catalyst with total metal loadings <50 mu g cm(-2) for the HER in proton-exchange-membrane water electrolyzers, we recorded uncompromised activity and durability compared to the baseline established with 3 mg cm(-2) Pt black. C1 [Wang, Jia X.; Zhang, Yu] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Capuano, Christopher B.; Ayers, Katherine E.] Proton OnSite, Wallingford, CT 06492 USA. RP Wang, JX (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM jia@bnl.gov; KAyers@protononsite.com RI Wang, Jia/B-6346-2011; OI Zhang, Yu/0000-0002-0814-2965; Ayers, Katherine/0000-0003-3246-1744 FU US Department of Energy, Division of Chemical Sciences, Geosciences and Biosciences Division [DE-AC02-98CH10886]; US Department of Energy, Office of Energy Efficiency and Renewable Energy [DE-FG02-12ER86531] FX This research was supported by the US Department of Energy, Division of Chemical Sciences, Geosciences and Biosciences Division under contract DE-AC02-98CH10886 and Office of Energy Efficiency and Renewable Energy under grant DE-FG02-12ER86531. NR 24 TC 6 Z9 6 U1 15 U2 77 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUL 20 PY 2015 VL 5 AR 12220 DI 10.1038/srep12220 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CN1AO UT WOS:000358147700001 PM 26191776 ER PT J AU Schijf, J Christenson, EA Potter, KJ AF Schijf, Johan Christenson, Emily A. Potter, Kailee J. TI Different binding modes of Cu and Pb vs. Cd, Ni, and Zn with the trihydroxamate siderophore desferrioxamine B at seawater ionic strength SO MARINE CHEMISTRY LA English DT Article DE desferrioxamine B; divalent metals; organic ligands; potentiometric titration; linear free-energy relations ID ENVIRONMENTALLY SIGNIFICANT METALS; NATURAL ORGANIC-LIGANDS; CENTRAL NORTH PACIFIC; COPPER COMPLEXING CAPACITY; SAN-FRANCISCO BAY; CHEMICAL SPECIATION; MARINE-PHYTOPLANKTON; MASS-SPECTROMETRY; SOUTHERN-OCEAN; COORDINATION CHEMISTRY AB The solution speciation in seawater of divalent trace metals (Cd, Cu, Ni, Pb, Zn) is dominated by strong, ostensibly metal-specific organic ligands that may play important roles in microbial metal acquisition and/or detoxification processes. We compare the effective stabilities of these metal-organic complexes to the stabilities of their complexes with a model siderophore, desferrioxamine B (DFOB). While metal-DFOB complexation has been studied in various dilute but often moderately coordinating media, for the purpose of this investigation we measured the stability constants in a non-coordinating background electrolyte at seawater ionic strength (0.7 M NaClO4). Potentiometric titrations of single metals (M) were performed in the presence of ligand (L) at different M:L molar ratios, whereupon the stability constants of multiple complexes were simultaneously determined by non-linear regression of the titration curves with FITEQL, using the optimal binding mode for each metal. Cadmium, Ni, and Zn, like trivalent Fe, sequentially form a bi-, tetra-, and hexadentate complex with DFOB as pH increases, consistent with their coordination number of 6 and regular octahedral geometry. Copper has a Jahn-Teller-distorted square-bipyramidal geometry whereas the geometry of Pb is cryptic, involving a range of bond lengths. Supported by a thermodynamic argument, our data suggest that this impedes binding of the third hydroxamate group and that the hexadentate Cu-DFOB and Pb-DFOB complex identified in earlier reports may instead be a deprotonated tetradentate complex. Absence of the hexadentate complex promotes the formation of a dinuclear (bidentate-tetradentate) complex, M2HL2+, albeit not for Pb in 0.7 M NaCl, evidently due to extensive complexation with chloride. Stabilities of the hexadentate Ni-DFOB, Zn-DFOB, and the tetradentate Pb-DFOB complex are nearly equal, yet about 2 orders of magnitude higher and 4 orders of magnitude lower than those of the hexadentate Cd-DFOB and tetradentate Cu-DFOB complex, respectively. Linear free-energy relations defined by the rare earth elements are able to predict stabilities of the Cd, Zn, and one of the Pb complexes, but underestimate those of the Ni and Cu complexes. The comparison with metal-specific organic ligands detected in seawater yields fair agreement for three of the five metals, implying that they could be siderophore-like. The Cd- and Ni-specific ligands are much stronger and may contain quite different functional groups. Calculations with MINEQL incorporating our new stability constants indicate that very high DFOB concentrations would be required to match the extent of metal-organic complexation observed in seawater, however DFOB may well represent a much broader class of structurally related-ligands. (C) 2015 Elsevier B.V. All rights reserved. C1 [Schijf, Johan; Christenson, Emily A.] Univ Maryland, Ctr Environm Sci, Chesapeake Biol Lab, Solomons, MD 20688 USA. [Potter, Kailee J.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Schijf, J (reprint author), Univ Maryland, Ctr Environm Sci, Chesapeake Biol Lab, POB 38, Solomons, MD 20688 USA. EM schijf@cbl.umces.edu RI Schijf, Johan/D-8259-2012 OI Schijf, Johan/0000-0001-9266-6982 FU NSF [OCE-0928450, OCE-0754609] FX Partial funding for this study was provided to J.S. by NSF (OCE-0928450). The REU project of K.J.P. was funded by NSF (OCE-0754609) and administered by the Maryland Sea Grant Program. Alison Zoll rendered the molecular structures in Fig. 2 with ChemDraw v.12.0. High school student Emily Carroll and REU student Lauren Hunker helped with method development in the early stages of this project. We are grateful for the thorough scrutiny and thoughtful comments of two anonymous reviewers and the mediation of a third reviewer. We also thank the organizers of the Special Issue for this opportunity and for their dedication. This is UMCES contribution #4951. NR 98 TC 4 Z9 4 U1 7 U2 38 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-4203 EI 1872-7581 J9 MAR CHEM JI Mar. Chem. PD JUL 20 PY 2015 VL 173 SI SI BP 40 EP 51 DI 10.1016/j.marchem.2015.02.014 PG 12 WC Chemistry, Multidisciplinary; Oceanography SC Chemistry; Oceanography GA CI8TO UT WOS:000355044800004 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, D Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ 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CA ATLAS Collaboration TI Search for invisible decays of the Higgs boson produced in association with a hadronically decaying vector boson in pp collisions at, root s=8 TeV with the ATLAS detector SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID MASSLESS PARTICLES; BROKEN SYMMETRIES; LHC AB A search for Higgs boson decays to invisible particles is performed using 20,3 of fb(-1) collision data at a centre-of-mass energy of 8 TeV recorded by the ArL As detector at the Large IHIadron Collider. The process considered is Higgs boson production in association with a vector boson (V = W or Z) that decays hadronically, resulting in events with two or more jets and large missing transverse momentum. No excess of candidates is observed in the data over the background expectation. The results are used to constrain V H production followed by H decaying to invisible particles for the Higgs boson mass range 115 < m(H) < 300 GeV. The 95 % confidence-level observed upper limit on sigma vH x BR(H -> inv.) varies from 1.6 pb at 115 GeV to 0.13 ph at 300 GeV. Assuming Standard Model production and including the gg -> H contribution as signal, the results also lead to an observed upper limit of 78 c/c at 95 % confidence level on the branching ratio of Higgs bosons decays to invisible particles at a mass of 125 GeV. C1 [Jackson, P.; Lee, L.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Yildiz, H. Duran] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Kuday, S.] Istanbul Aydin Univ, Istanbul, Turkey. 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A.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Hageboeck, S.; Hansen, M. C.; Hellmich, D.; Hohn, D.; Huegging, F.; Janssen, J.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mergelmeyer, S.; Mijovic, L.; Mueller, K.; Obermann, T.; Pohl, D.; Ricken, O.; Sarrazin, B.; Schaepe, S.; Schopf, E.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Seema, P.; Stillings, J. A.; Tannoury, N.; Therhaag, J.; Uhlenbrock, M.; Velz, T.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Fitzgerald, E. A.; Sciolla, G.; Venturini, A.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Amaral Coutinho, Y.; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Fiho, L.] Fed Univ Juiz de Fora UHF, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; La Rosa Navarro, J. L.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentovs, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, E.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Poychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciuhancan, M.; Constantinescu, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurera, J.; Olariu, A.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carters, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Boveia, A.; Catinaccio, A.; Cattai, A.; Dell'Acqua, A.; Di Girolamo, A.; Dudarev, A.; Hoecker, A.; Krasznahorkay, A.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y.; Krizka, K.; Li, H. L.; Merritt, E. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.; Wong, K. H. Yau] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kueshov, S.; Pezoa, R.; Prokoshin, E.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Hu, Q.; Jiang, Y.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhang, R.; Zhang, X.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.; Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Guo, J.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, E.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Calvet, D.; Pallin, D.; Santoni, C.; Simon, D.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, E.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidous, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Thompson, E. N.; Tuts, P. M.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, I. E.; Petersen, T. C.; Pingel, A.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Roonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, I-00044 Frascati, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Roonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Maecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lohodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lohodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Guischow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Arnold, H.; Betancourt, C.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Di Simone, A.; Giuliani, C.; Herten, G.; Kiss, F.; Kopp, A. K.; Ruehr, F.; Schillo, C.; Schmidt, E.; Sundermann, J. E.; Ungaro, E. C.; von Radziewski, H.; Weiser, C.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, R.; Miucci, A.; Muenstermann, D.; Paolozzi, L.; Picazio, A.; Ristic, B.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, E.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, E.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Denis, R. D. St.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schoremmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huths, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. R.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluges, E. -E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, NT, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Pok Fu Lam, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weiner, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R. W.; Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, I. V.; Demichev, M.; Dewhurst, A.; Gostkin, M. I.; Kazarinov, M. Y.; Khramov, E.; Ladygine, E.; Minashvili, I. A.; Mineev, M.; Plotnikova, E.; Potrap, I. N.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Yeletskikh, I.; Zhemchugov, A.] JINR Dubna, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, S.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Allport, P. P.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, R.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, R.; Krasny, M. W.; Lacour, D.; Laforges, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikoic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, E.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, R.; Krasny, M. W.; Lacour, D.; Laforges, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikoic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, E.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, R.; Krasny, M. W.; Lacour, D.; Laforges, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikoic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, E.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Poettgen, R.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Dewhurst, A.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Huhaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Tiese; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Huhaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Tiese; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantife, R.; Prince, S.; Roberisons, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Urquijo, P.; Vopi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Dewhurst, A.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Hu, X.; Levin, D.; Long, J. D.; Lu, N.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Wills, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrvnevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, I.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh; Soueid, R.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shineleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgosheins, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Dewhurst, A.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Moser, H. G.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. 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J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Konig, A. C.; Nektarijevic, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Kolleman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deij, P. C.; Van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vupen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Adelman, J.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, R.; Kazanin, V. E.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] RAS, Budker Inst Nucl Phys, SB, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishinukharnetov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, R.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, R.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. I.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Seifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. I.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Seifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. E.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Sawyer, C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Lipeles, E.; Machado Miguens, J.; Meyer, C.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedinin, O. L.; Gratchev, V.; Levehenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seiverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Calorio, D.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Sole, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, R.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Czech Tech Univ, Fac Math & Phys, CR-16635 Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Olovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Di Ciaccio, A.; Liberti, B.; Mazzaferro, L.; Salamon, A.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, E.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, E.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockaman, W. S.; Manning, R. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Kyriazopoulos, I.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikernatsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Mount, R.; Nef, R. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC, Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.; Meehan, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Govender, N.; Lee, C. A.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hamity, G. N.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Berg, O. Lund; Milstead, D. A.; Moa, I.; Molander, S.; Pani, R.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Berg, O. Lund; Milstead, D. A.; Moa, I.; Molander, S.; Pani, R.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys, Dept Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Hsu, P. J.; Jamin, D. O.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, E.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Munwes, Y.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakainura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakainura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Ilic, N.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Jovicevic, J.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, E.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Gerbaudo, I.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] Ist Nazl Fis Nucl, Grp Coll Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Neubauer, M. S.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, IMB CNM, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Swedish, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Kuger, E.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Beermann, T. A.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Guest, I.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London, England. [Anisenkov, A. V.; Bobrovnikov, V. S.; Buzykaev, R.; Kazanin, V. E.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Azuelos, G.; Gingrich, D. M.; Oakham, F. G.; Savard, P.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Bawa, H. S.; Gao, Y. S.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beck, H. P.] Univ Fribourg, Dept Phys, CH-1700 Fribourg, Switzerland. [Castro, N. F.] Univ Porto, Fac Ciencias, Dept Fis & Astron, P-4100 Oporto, Portugal. [Chelkov, G. A.] Tomsk State Univ, Tomsk 634050, Russia. [Chen, L.] Aix Marseille Univ, CPPM, Marseille, France. [Chen, L.] CNRS, IN2P3, Marseille, France. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. 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RI Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Boldyrev, Alexey/M-9684-2015; Livan, Michele/D-7531-2012; Tikhomirov, Vladimir/M-6194-2015; Di Domenico, Antonio/G-6301-2011; Boyko, Igor/J-3659-2013; Mitsou, Vasiliki/D-1967-2009; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Brooks, William/C-8636-2013; Korol, Aleksandr/A-6244-2014; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Petrucci, Fabrizio/G-8348-2012; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Martinez, Mario /I-3549-2015; Peleganchuk, Sergey/J-6722-2014; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Garcia, Jose /H-6339-2015; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Snesarev, Andrey/H-5090-2013; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; La Rosa Navarro, Jose Luis/K-4221-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Staroba, Pavel/G-8850-2014; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Carvalho, Joao/M-4060-2013; White, Ryan/E-2979-2015; Mashinistov, Ruslan/M-8356-2015; spagnolo, stefania/A-6359-2012; Buttar, Craig/D-3706-2011; Smirnova, Oxana/A-4401-2013; Doyle, Anthony/C-5889-2009; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; OI Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Livan, Michele/0000-0002-5877-0062; Tikhomirov, Vladimir/0000-0002-9634-0581; Di Domenico, Antonio/0000-0001-8078-2759; Boyko, Igor/0000-0002-3355-4662; Mitsou, Vasiliki/0000-0002-1533-8886; Warburton, Andreas/0000-0002-2298-7315; Brooks, William/0000-0001-6161-3570; Sannino, Mario/0000-0001-7700-8383; Korol, Aleksandr/0000-0001-8448-218X; Giordani, Mario/0000-0002-0792-6039; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Petrucci, Fabrizio/0000-0002-5278-2206; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Giorgi, Filippo Maria/0000-0003-1589-2163; Gauzzi, Paolo/0000-0003-4841-5822; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Goncalo, Ricardo/0000-0002-3826-3442; Carvalho, Joao/0000-0002-3015-7821; White, Ryan/0000-0003-3589-5900; Mashinistov, Ruslan/0000-0001-7925-4676; spagnolo, stefania/0000-0001-7482-6348; Smirnova, Oxana/0000-0003-2517-531X; Doyle, Anthony/0000-0001-6322-6195; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Coccaro, Andrea/0000-0003-2368-4559 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWTW, Austria; EWE, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNN, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET; ERC; NSRF; European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; IIGT, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; RGC, China; Hong Kong SAR, China; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Poland; MNE/IFA, Romania; MES of Russia; NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society and Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWTW and EWE, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNN and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, IIGT, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; RGC, Hong Kong SAR, China; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGE (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 52 TC 3 Z9 3 U1 12 U2 56 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JUL 18 PY 2015 VL 75 IS 7 AR 337 DI 10.1140/epjc/s10052-015-3551-1 PG 24 WC Physics, Particles & Fields SC Physics GA CS2NQ UT WOS:000361908400002 ER PT J AU Sharada, SM Stuck, D Sundstrom, EJ Bell, AT Head-Gordon, M AF Sharada, Shaama Mallikarjun Stueck, David Sundstrom, Eric J. Bell, Alexis T. Head-Gordon, Martin TI Wavefunction stability analysis without analytical electronic Hessians: application to orbital-optimised second-order Moller-Plesset theory and VV10-containing density functionals SO MOLECULAR PHYSICS LA English DT Article DE density functional theory; quantum chemistry; Brueckner orbitals; orbital optimisation; stability analysis ID HARTREE-FOCK EQUATIONS; CLUSTER DOUBLES MODEL; CORRELATION-ENERGY; UNRESTRICTED ORBITALS; MOLECULAR SYSTEMS; APPROXIMATION; POINTS; HYBRID; STATES; GAS AB Wavefunction stability analysis is commonly applied to converged self-consistent field (SCF) solutions to verify whether the electronic energy is a local minimum with respect to second-order variations in the orbitals. By iterative diagonalisation, the procedure calculates the lowest eigenvalue of the stability matrix or electronic Hessian. However, analytical expressions for the electronic Hessian are unavailable for most advanced post-Hartree-Fock (HF) wave function methods and even some Kohn-Sham (KS) density functionals. To address such cases, we formulate the Hessian-vector product within the iterative diagonalisation procedure as a finite difference of the electronic gradient with respect to orbital perturbations in the direction of the vector. As a model application, following the lowest eigenvalue of the orbital-optimised second-order Moller-Plesset perturbation theory (OOMP2) Hessian during H-2 dissociation reveals the surprising stability of the spin-restricted solution at all separations, with a second independent unrestricted solution. We show that a single stable solution can be recovered by using the regularised OOMP2 method (delta-OOMP2), which contains a level shift. Internal and external stability analyses are also performed for SCF solutions of a recently developed range-separated hybrid density functional, omega B97X-V, for which the analytical Hessian is not yet available due to the complexity of its long-range non-local VV10 correlation functional. C1 [Sharada, Shaama Mallikarjun; Bell, Alexis T.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Stueck, David; Sundstrom, Eric J.; Head-Gordon, Martin] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Stueck, David; Sundstrom, Eric J.; Bell, Alexis T.; Head-Gordon, Martin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Head-Gordon, M (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM mhg@cchem.berkeley.edu OI Bell, Alexis/0000-0002-5738-4645 FU Chevron Energy Technology Co.; Department of Energy Office of Science Graduate Fellowship Program (DOE SCGF); American Recovery and Reinvestment Act [DE-AC05- 06OR23100]; Office of Science, Office of Basic Energy Sciences, the US Department of Energy [DE-AC02-05CH11231] FX This research was supported by a grant from Chevron Energy Technology Co. and the Department of Energy Office of Science Graduate Fellowship Program (DOE SCGF). This study was made possible, in part, by the American Recovery and Reinvestment Act of 2009, administered by ORISE-ORAU [contract number DE-AC05- 06OR23100]; the Office of Science, Office of Basic Energy Sciences, the US Department of Energy [contract number DE-AC02-05CH11231]. NR 42 TC 3 Z9 3 U1 2 U2 12 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 0026-8976 EI 1362-3028 J9 MOL PHYS JI Mol. Phys. PD JUL 18 PY 2015 VL 113 IS 13-14 SI SI BP 1802 EP 1808 DI 10.1080/00268976.2015.1014442 PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CM8FJ UT WOS:000357933400031 ER PT J AU Zhang, M AF Zhang, Meng TI Structure and Function Relationship of Phospholipid Transfer Protein in Lipid Transfer Activity Revealed by Electron Microscopy SO CIRCULATION RESEARCH LA English DT Meeting Abstract CT American-Stroke-Association/American-Heart-Association Basic Cardiovascular Sciences Scientific Sessions - Pathways to Cardiovascular Therapeutics CY JUL 13-16, 2015 CL New Orleans, LA SP Amer Stroke Assoc, Amer Heart Assoc, Council Basic Cardiovascular Sci DE Phospholipid Transfer Protein; lipid transfer; Electron Microscopy C1 [Zhang, Meng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU LIPPINCOTT WILLIAMS & WILKINS PI PHILADELPHIA PA TWO COMMERCE SQ, 2001 MARKET ST, PHILADELPHIA, PA 19103 USA SN 0009-7330 EI 1524-4571 J9 CIRC RES JI Circ.Res. PD JUL 17 PY 2015 VL 117 SU 1 MA 127 PG 1 WC Cardiac & Cardiovascular Systems; Hematology; Peripheral Vascular Disease SC Cardiovascular System & Cardiology; Hematology GA DJ9SI UT WOS:000374552800120 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arika, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Auerbach, B Augsten, K Aurousseau, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Balek, P Balestri, T Balli, F Banas, E Banerjee, S Bannoura, AAE Bansil, HS Barak, L Baranov, SP Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Bassalat, 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Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehler, M Bogaerts, JA Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutouil, S Boveia, A Boyd, J Boyko, IR Bozic, I Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, K Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Bruschi, M Bryngemark, L Buanes, T Buat, Q Buchholz, P Buckley, AG Buda, SI Budagov, IA Buehrer, F Bugge, 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CA ATLAS Collaboration TI Constraints on the off-shell Higgs boson signal strength in the high-mass ZZ and WW final states with the ATLAS detector SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID PARTON DISTRIBUTIONS; HADRON COLLIDERS; LHC; SEARCH; PLUS AB Measurements of the ZZ and WW final states in the mass range above the 2m(Z) and 2m(W) thresholds provide a unique opportunity to measure the off-shell coupling strength of the Higgs boson. This paper presents constraints on the off-shell Higgs boson event yields normalised to the Standard Model prediction (signal strength) in the ZZ -> 4l, ZZ -> 2l2 nu and WW -> e nu mu nu final states. The result is based on pp collision data collected by the ATLAS experiment at the LHC, corresponding to an integrated luminosity of 20.3 fb(-1) at a collision energy of root s = 8 TeV. Using the CLs method, the observed 95 % confidence level (CL) upper limit on the off-shell signal strength is in the range 5.1-8.6, with an expected range of 6.7-11.0. In each case the range is determined by varying the unknown gg -> ZZ and gg -> WW background K-factor from higher-order quantum chromodynamics corrections between half and twice the value of the known signal K-factor. Assuming the relevant Higgs boson couplings are independent of the energy scale of the Higgs boson production, a combination with the on-shell measurements yields an observed (expected) 95 % CL upper limit on Gamma(H)/Gamma(SM)(H) in the range 4.5-7.5 (6.5-11.2) using the same variations of the background K-factor. Assuming that the unknown gg -> VV background K-factor is equal to the signal K-factor, this translates into an observed (expected) 95 % CL upper limit on the Higgs boson total width of 22.7 (33.0) MeV. C1 [Jackson, P.; Lee, L.; Soni, N.; White, M. 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[Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; Bruckman de Renstrom, P. A.; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Gossling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dao, V.; Di Simone, A.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Ancu, L. S.; Barone, G.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Picazio, A.; Ristic, B.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St. Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Arce, A. T. H.; Bindi, M.; Blumenschein, U.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Koletsou, I.; Lafaye, R.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lopez Mateos, D.; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Heidelberg, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Pok Fu Lam, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Krumnack, N.; Pluth, D.; Prell, S.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Cochran, J.; De Lorenzi, F.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Sumida, T.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, S.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] Natl Lab High Energy Phys, KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki 305, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Allport, P. P.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Price, J.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Dearnaley, W. J.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Lambourne, L.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Dearnaley, W. J.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Lambourne, L.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Kempster, J. J.; Lampen, C. L.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Aloisio, A.; Alonso, A.; Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS IN2P3, Paris, France. [Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Glasman, C.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Becker, M.; Bertella, C.; Caudron, J.; Ellinghaus, F.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Hohlfeld, M.; Karnevskiy, M.; Kleinknecht, K.; Kopke, L.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Sander, H. G.; Schaeffer, J.; Schmitt, C.; Schroeder, C.; Simioni, E.; Valderanis, C.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; TicseTorres, E.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; TicseTorres, E.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Hu, X.; Levin, D.; Long, J. D.; Lu, N.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Cavalli, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. 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P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Konig, A. C.; Nektarijevic, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; Van der Geer, R.; Van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; Van der Geer, R.; Van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, R.; Kazanin, V. F.; Kharlamov, G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] RAS, SB, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. 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L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Ideal, E.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS IN2P3, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pachal, K.; Pickering, M. A.; Ryder, N. C.; Sawyer, C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Muino, P. Conde; Escobar, C.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. 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[Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Phillips, P. W.; Sankey, D. P. C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Di Ciaccio, A.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Stanescu, C.; Taccini, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Taccini, C.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. 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B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Abreu, H.; Buat, Q.; Horton, A. J.; O'Neil, D. C.; Stelzer, B.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Mount, R.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. 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[Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Ilic, N.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Jovicevic, J.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Gerbaudo, D.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.] INFN, Grp Coll Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Neubauer, M. S.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Alvarez Piqueras, D.; Castillo Gimenez, V.; Costa, M. 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T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Alvarez Piqueras, D.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. 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RI Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Carvalho, Joao/M-4060-2013; Livan, Michele/D-7531-2012; Tikhomirov, Vladimir/M-6194-2015; Di Domenico, Antonio/G-6301-2011; Boyko, Igor/J-3659-2013; Mitsou, Vasiliki/D-1967-2009; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Brooks, William/C-8636-2013; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Snesarev, Andrey/H-5090-2013; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; Villa, Mauro/C-9883-2009; La Rosa Navarro, Jose Luis/K-4221-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; Staroba, Pavel/G-8850-2014; Goncalo, Ricardo/M-3153-2016; White, Ryan/E-2979-2015; Mashinistov, Ruslan/M-8356-2015; spagnolo, stefania/A-6359-2012; Buttar, Craig/D-3706-2011; Smirnova, Oxana/A-4401-2013; Doyle, Anthony/C-5889-2009; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Petrucci, Fabrizio/G-8348-2012; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Korol, Aleksandr/A-6244-2014; Capua, Marcella/A-8549-2015; Gavrilenko, Igor/M-8260-2015; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Martinez, Mario /I-3549-2015; Peleganchuk, Sergey/J-6722-2014; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Garcia, Jose /H-6339-2015 OI Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Carvalho, Joao/0000-0002-3015-7821; Livan, Michele/0000-0002-5877-0062; Tikhomirov, Vladimir/0000-0002-9634-0581; Di Domenico, Antonio/0000-0001-8078-2759; Boyko, Igor/0000-0002-3355-4662; Mitsou, Vasiliki/0000-0002-1533-8886; Warburton, Andreas/0000-0002-2298-7315; Brooks, William/0000-0001-6161-3570; Vykydal, Zdenek/0000-0003-2329-0672; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Villa, Mauro/0000-0002-9181-8048; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Goncalo, Ricardo/0000-0002-3826-3442; White, Ryan/0000-0003-3589-5900; Mashinistov, Ruslan/0000-0001-7925-4676; spagnolo, stefania/0000-0001-7482-6348; Smirnova, Oxana/0000-0003-2517-531X; Doyle, Anthony/0000-0001-6322-6195; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Belanger-Champagne, Camille/0000-0003-2368-2617; Prokofiev, Kirill/0000-0002-2177-6401; Veneziano, Stefano/0000-0002-2598-2659; Vazquez Schroeder, Tamara/0000-0002-9780-099X; Chen, Chunhui /0000-0003-1589-9955; Price, Darren/0000-0003-2750-9977; Terzo, Stefano/0000-0003-3388-3906; Smirnov, Sergei/0000-0002-6778-073X; Della Volpe, Domenico/0000-0001-8530-7447; Castro, Nuno/0000-0001-8491-4376; Farrington, Sinead/0000-0001-5350-9271; Robson, Aidan/0000-0002-1659-8284; Weber, Michele/0000-0002-2770-9031; Grohsjean, Alexander/0000-0003-0748-8494; Ochoa-Ricoux, Juan Pedro/0000-0001-7376-5555; Irles, Adrian/0000-0001-5668-151X; La Rosa, Alessandro/0000-0001-6291-2142; Beck, Hans Peter/0000-0001-7212-1096; Salamanna, Giuseppe/0000-0002-0861-0052; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Petrucci, Fabrizio/0000-0002-5278-2206; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Giorgi, Filippo Maria/0000-0003-1589-2163; Coccaro, Andrea/0000-0003-2368-4559; Cristinziani, Markus/0000-0003-3893-9171; Haas, Andrew/0000-0002-4832-0455; Galhardo, Bruno/0000-0003-0641-301X; Gaudiello, Andrea/0000-0001-7721-8217; Troncon, Clara/0000-0002-7997-8524; Vari, Riccardo/0000-0002-2814-1337; Gray, Heather/0000-0002-5293-4716; Dell'Asta, Lidia/0000-0002-9601-4225; Sannino, Mario/0000-0001-7700-8383; Korol, Aleksandr/0000-0001-8448-218X; Giordani, Mario/0000-0002-0792-6039; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; RGC, Hong Kong SAR, China; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We are very thankful to M. Bonvini, J. Campbell, S. Forte, F. Krauss, K. Melnikov, G. Passarino, and M. Spannowsky for their essential input in the estimation of uncertainties in the theoretical predictions for the signal and background processes and their interference. We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; RGC, Hong Kong SAR, China; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 66 TC 15 Z9 15 U1 16 U2 62 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JUL 17 PY 2015 VL 75 IS 7 AR 335 DI 10.1140/epjc/s10052-015-3542-2 PG 34 WC Physics, Particles & Fields SC Physics GA CS2NP UT WOS:000361908300011 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asmana, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Auerbach, B Augsten, K Aurousseaub, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Balek, P Balestri, T Balli, F Banas, E Banerjee, S Bannoura, AAE Bansil, HS Barak, L Baranov, SP Barberio, EL Barberis, D Barbero, M Barillaris, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, M Becker, S Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehler, M Bogaerts, JA Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boveia, A Boyd, J Boyko, IR Bozic, I Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, K Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Bruschi, M Bryngemark, L Buanes, T Buat, Q Buchholz, P Buckley, AG Buda, SI Budagov, IA Buehrer, F Bugge, L Bugge, MK Bulekov, O Burckhart, H Burdin, S Burghgrave, B Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Buszello, CP Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Buzykaev, R Urban, SC Caforio, D Cairo, VM Cakir, O Calafiura, P Calandri, A Calderini, G Calfayan, P Caloba, LP Calvet, D Calvet, S Toro, RC Camarda, S Camarri, P Cameron, D Caminada, LM Armadans, RC Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Cardarelli, R Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Caudron, J Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, BC Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chang, P Chapleau, B Chapman, JD Charlton, DG Chau, CC Barajas, CAC Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A Cheremushkina, E El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Childers, JT Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Choi, K Chouridou, S Chow, BKB Christodoulou, V Chromek-Burckhart, D Chu, ML Chudoba, J Chuinard, AJ Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Cinca, D Cindro, V Cioara, IA Ciocio, A Citron, ZH Ciubancan, M Clark, A Clark, BL Clark, PJ Clarke, RN Cleland, W Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Cogan, JG Cole Cole, S Colijn, AP Collot, J Colombo, T Compostella, G Muino, PC Coniavitis, E Connellb, SH Connelly, IA Consonni, SM Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cote, D Cottin, G Cowan, G Cox, BE Cranmer, K Cree, G Crepe-Renaudin, S Crescioli, F Cribbs, WA Ortuzar, MC Cristinziani, M Croft, V Crosetti, G Donszelmann, TC Cummings, J Curatolo, M Cuthbert, C Czirr, H Czodrowski, P D'Auria, S D'Onofrio, M De Sousa, MJDCS Da Via, C Dabrowski, W Dafinca, A Dai, T Dale, O Dallaire, F Dallapiccola, C Dam, M Dandoy, JR Dang, NP Daniells, AC Danninger, M Hoffmann, MD Dao, V Darbo, G Darmora, S Dassoulas, J Dattagupta, A Davey, W David, C Davidek, T Davies, E Davies, M Davison, P Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K De Asmundis, R De Castro, S De Cecco, S De Groot, N De Jong, P la Torre, H De Lorenzi, F De Nooij, L De Pedis, D De Salvo, A De Sanctis, U De Santo, A De Regie, JBDV Dearnaley, WJ Debbe, R Debenedetti, C Dedovich, DV Deigaard, I Del Peso, J Del Prete, T Delgove, D Deliot, F Delitzsch, CM Deliyergiyev, M Dell'Acqua, A Dell'Asta, L Dell'Orso, M Della Pietra, M della Volpe, D Delmastro, M Delsart, PA Deluca, C DeMarco, DA Demers, S Demichev, M Demilly, A Denisov, SP Derendarz, D Derkaoui, JE Derue, F Dervan, P Desch, K Deterre, C Deviveiros, PO Dewhurst, A Dhaliwal, S Di Ciaccio, A Di Ciaccio, L Di Domenico, A Di Donato, C Di Girolamo, A Di Girolamo, B Di Mattia, A Di Micco, B Di Nardo, R Di Simone, A Di Sipio, R Di Valentino, D Diaconu, C Diamond, M Dias, FA Diaz, MA Diehl, EB Dietrich, J Diglio, S Dimitrievska, A Dingfelder, J Dittus, F Djama, F Djobava, T Djuvsland, JI do Vale, MAB Dobos, D Dobre, M Doglioni, C Dohmae, T Dolejsi, J Dolezal, Z Dolgoshein, BA Donadelli, M Donati, S Dondero, P Donini, J Dopke, J Doria, A Dova, MT Doyle, AT Drechsler, E Dris, M Dubreuil, E Duchovni, E Duckeck, G Ducu, OA Duda, D Dudarev, A Duflot, L Duguid, L Duhrssen, M Dunford, M Yildiz, HD Duren, M Durglishvili, A Duschinger, D Dyndal, M Eckardt, C Ecker, KM Edgar, RC Edson, W Edwards, NC Ehrenfeld, W Eifert, T Eigen, G Einsweiler, K Ekelof, T El Kacimi, M Ellert, M Elles, S Ellinghaus, F Elliot, AA Ellis, N Elmsheuser, J Elsing, M Emeliyanov, D Enari, Y Endner, OC Endo, M Engelmann, R Erdmann, J Ereditato, A Ernis, G Ernst, J Ernst, M Errede, S Ertel, E Escalier, M Esch, H Escobar, C Esposito, B Etienvre, AI Etzion, E Evans, H Ezhilov, A Fabbri, L Facini, G Fakhrutdinov, RM Falciano, S Falla, RJ Faltova, J Fang, Y Fanti, M Farbin, A Farilla, A Farooque, T Farrell, S Farrington, SM Farthouat, P Fassi, F Fassnacht, P Fassouliotis, D Giannelli, MF Favareto, A Fayard, L Federic, P Fedin, OL Fedorko, W Feigl, S Feligioni, L Feng, C Feng, EJ Feng, H Fenyuk, AB Martinez, PF Perez, SF Ferrag, S Ferrando, J Ferrari, A Ferrari, P Ferrari, R De Lima, DEF Ferrer, A Ferrere, D Ferretti, C Parodi, AF Fiascaris, M Fiedler, F Filipcic, A Filipuzzi, M Filthaut, F Fincke-Keeler, M Finelli, KD Fiolhais, MCN Fiorini, L Firan, A Fischer, A Fischer, C Fischer, J Fisher, WC Fitzgerald, EA Flechl, M Fleck, I Fleischmann, P Fleischmann, S Fletcher, GT Fletcher, G Flick, T Floderus, A Castillo, LRF Flowerdew, MJ Formica, A Forti, A Fournier, D Fox, H Fracchia, S Francavilla, P Franchini, M Francis, D Franconi, L Franklin, M Fraternali, M Freeborn, D French, ST Friedrich, F Froidevaux, D Frost, JA Fukunaga, C Torregrosa, EF Fulsom, BG Fuster, J Gabaldon, C Gabizon, O Gabrielli, A Gabrielli, A Gadatsch, S Gadomski, S Gagliardi, G Gagnon, BP Galea, C Galhardo, B Gallas, EJ Gallop, BJ Gallus, P Galster, G Gan, KK Gao, J Gao, Y Gao, YS Walls, FMG Garberson, F Garcia, C Navarro, JEG Garcia-Sciveres, M Gardner, RW Garelli, N Garonne, V Gatti, C Gaudiello, A Gaudioa, G Gaur, B Gauthier, L Gauzzi, P Gavrilenko, IL Gay, C Gaycken, G Gazis, EN Ge, P Gecse, Z Gee, CNP Geerts, DAA Geich-Gimbel, C Geisler, MP Gemme, C Genest, MH Gentile, S George, M George, S Gerbaudo, D Gershon, A Ghazlane, H Giacobbe, B Giagu, S Giangiobbe, V Giannetti, P Gibbard, B Gibson, SM Gilchriese, M Gillam, TPS Gillberg, D Gilles, G Gingrich, DM Giokaris, N 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Nedden, M. zur Zurzolo, G. Zwalinski, L. TI Measurement of the top quark mass in the t(t)over-bar -> lepton plus jets and t(t)over-bar -> dilepton channels using root s=7 TeV ATLAS data SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID CARLO EVENT GENERATOR; PARTON DISTRIBUTIONS; HADRON COLLIDERS; STANDARD MODEL; LHC; PHYSICS AB The top quark mass was measured in the channels t (t) over bar -> lepton+jets and t (t) over bar -> dilepton (lepton = e, mu) based on ATLAS data recorded in 2011. The data were taken at the LHC with a proton-proton centre-of-mass energy of root s = 7 TeV and correspond to an integrated luminosity of 4.6 fb(-1). The t (t) over bar -> lepton+jets analysis uses a three-dimensional template technique which determines the top quark mass together with a global jet energy scale factor (JSF), and a relative b-to-light-jet energy scale factor (bJSF), where the terms b-jets and light-jets refer to jets originating from b-quarks and u,d,c, s-quarks or gluons, respectively. The analysis of the t (t) over bar -> dilepton channel exploits a one-dimensional template method using the m(lb) observable, defined as the average invariant mass of the two lepton+b-jet pairs in each event. The top quark mass is measured to be 172.33 +/- 0.75(stat + JSF + bJSF) +/- 1.02(syst) GeV, and 173.79 +/- 0.54(stat) +/- 1.30(syst) GeV in the t (t) over bar -> lepton+jets and t (t) over bar -> dilepton channels, respectively. The combination of the two results yields m(top) = 172.99 +/- 0.48(stat) +/- 0.78(syst) GeV, with a total uncertainty of 0.91 GeV. C1 [Jackson, P.; Lee, L.; Soni, N.; White, M. 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Montejo; Pages, A. Pacheco; Aranda, C. Padilla; Riu, I.; Sorin, V.; Succurro, A.; Tripiana, M. F.; Tsiskaridze, S.; Valery, L.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Anjos, N.; Bosman, M.; Armadans, R. Caminal; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fischer, C.; Fracchia, S.; Giangiobbe, V.; Parra, G. Gonzalez; Grinstein, S.; Rozas, A. Juste; Korolkov, I.; Lange, J. C.; Le Menedeu, E.; Paz, I. Lopez; Martinez, M.; Mir, L. M.; Berlingen, J. Montejo; Pages, A. Pacheco; Aranda, C. Padilla; Riu, I.; Sorin, V.; Succurro, A.; Tripiana, M. F.; Tsiskaridze, S.; Valery, L.] Univ Autonoma Barcelona, Dept Fis, E-08193 Barcelona, Spain. [Agatonovic-Jovin, T.; Bozic, I.; Dimitrievska, A.; Krstic, J.; Marjanovic, M.; Popovic, D. S.; Sijacki, Dj.; Simic, Lj.; Vranjes, N.; Milosavljevic, M. Vranjes; Zivkovic, L.] Univ Belgrade, Inst Phys, Belgrade, Serbia. [Buanes, T.; Dale, O.; Eigen, G.; Kastanas, A.; Lipniacka, A.; Maeland, S.; Latour, B. Martin dit; Parker, K. A.; Rosendahl, P. L.; Sandaker, H.; Sjursen, T. B.; Smestad, L.; Stugu, B.; Ugland, M.; Zalieckas, J.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Amadio, B. T.; Axen, B.; Barnett, R. M.; Beringer, J.; Brosamer, J.; Calafiura, P.; Caminada, L. M.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Schramm, S.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Amadio, B. T.; Axen, B.; Barnett, R. M.; Beringer, J.; Brosamer, J.; Calafiura, P.; Caminada, L. M.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Dietrich, J.; Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Herrberg-Schubert, R.; Hristova, I.; Kind, O. M.; Kolanoski, H.; Lacker, H.; Lohse, T.; Nikiforov, A.; Rehnisch, L.; Rieck, P.; Schulz, H.; Stamm, S.; Nedden, M. zur] Humboldt Univ, Dept Phys, D-10099 Berlin, Germany. [Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allbrooke, B. M. M.; Bella, L. Aperio; Bansil, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Owen, R. E.; Ozturk, N.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Bellagamba, L.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Corradi, M.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstrom, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstrom, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, I-40126 Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Cioara, I. A.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Hageboeck, S.; Hansen, M. C.; Hellmich, D.; Hohn, D.; Huegging, F.; Janssen, J.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mergelmeyer, S.; Mijovic, L.; Mueller, K.; Obermann, T.; Pohl, D.; Ricken, O.; Sarrazin, B.; Schaepe, S.; Schopf, E.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Seema, P.; Stillings, J. A.; Tannoury, N.; Therhaag, J.; Uhlenbrock, M.; Velz, T.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Fitzgerald, E. A.; Sciolla, G.; Venturini, A.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; de Andrade Filho, L. Manhaes] Fed Univ Juiz De Fora UFJF, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao Del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Navarro, J. L. La Rosa; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Popeneciu, G. A.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politeh Bucharest, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Garzon, G. Otero Y.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Corso-Radu, A.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Iengo, P.; Jaekel, M. R.; Jakobsen, S.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Shandong, Peoples R China. [Guo, J.; Lie, L.; Li, Y.; Yang, H.] Shanghai Jiao Tong Univ, Shanghai Key Lab Particle Phys & Cosmol, Dept Phys & Astron, Shanghai 200030, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Capua, M.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Capua, M.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Capua, M.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Thompson, E. N.; Tuts, P. M.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, I-00044 Frascati, Italy. [Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Liebig, W.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Corso-Radu, A.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Flechl, M.; Giuliani, C.; Herten, G.; Hetherly, J. W.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, j.; Guescini, F.; Iacobucci, G.; Katre, A.; LaRosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Picazio, A.; Ristic, B.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. 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S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, Lab Phys Subatom & Cosmol, CNRS IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Guimaraes da Costa, J. Barreiro; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Heidelberg, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Palacino, G.] Univ Hong Kong, Dept Phys, Pok Fu Lam, Hong Kong, Peoples R China. [Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, B. P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R. W.; Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, S.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat Fis, Lecce, Italy. [Affolder, A. A.; Allport, P. P.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, A.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, A.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Corso-Radu, A.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Pilkington, A. D.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; LeDortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; LeDortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; LeDortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Institutionen, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; la Torre, H. De; Del Peso, J.; Glasman, C.; Merin, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Hulsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Poettgen, R.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; LeGuirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; LeGuirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, A.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Hu, X.; Levin, D.; Long, J. D.; Lu, N.; Mckee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusaa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Carminati, L.; Consonni, S. M.; Corso-Radu, A.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusaa, F.; Shojaii, S.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, I-20133 Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, ag, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillaris, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Moser, H. G.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; Von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Conventi, F.; De Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Canale, V.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Konig, A. C.; Nektarijevic, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; De Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; De Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Corso-Radu, A.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Corso-Radu, A.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS IN2P3, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooke, M.; Cooper-Sarkar, A. M.; Corso-Radu, A.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Sawyer, C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudioa, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncaloa, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Gomes, A.; Jorge, P. M.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, P-1699 Lisbon, Portugal. [Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Castro, N. F.] Univ Nova Lisboa, Dept Fis, Fac Ciencias Tecnol, Caparica, Portugal. [Castro, N. F.] Univ Nova Lisboa, CEFITEC, Fac Ciencias Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr, Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Corso-Radu, A.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kunaa, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kunaa, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Hautes Energies Univ Hassan II, Reseau Univ Phys, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Corso-Radu, A.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Firmino Da Costa, J. Goncalves Pinto; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Ristic, B.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, DSM IRFU Inst Rech Lois Fondament Univers, Commissariat Energie Atom & Energies Alternat, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Corso-Radu, A.; Horton, A. J.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Corso-Radu, A.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moyse, E. J. W.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Corso-Radu, A.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnuclear Phys, Kosice 04353, Slovakia. [Hamilton, A.; Meehan, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseaub, M.; Castaneda-Miranda, E.; Connellb, S. H.; Govender, N.; Lee, C. A.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Corso-Radu, A.; Hamity, G. N.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asmana, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asmana, B.] Oskar Klein Ctr, S-10691 Stockholm, Sweden. [Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron & Chem, Stony Brook, NY 11794 USA. [Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Hsu, P. J.; Jamin, D. O.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; LoSterzo, F.; Mazini, R.; Ristic, B.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei 115, Taiwan. [Cheatham, S.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Corso-Radu, A.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Munwes, Y.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, S.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Abreu, H.; Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Abreu, H.; Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Ilic, N.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Garcia, J. A. Benitez; Canepa, A.; Chekulaev, S. V.; Jovicevic, J.; Koutsman, A.; Ramos, J. Manjarres; Oram, C. J.; Codina, E. Perez; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Taylor, W.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] INFN, Grp Collegato Udine, Sez Trieste, Udine, Italy. [Barisonzi, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim, Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Neubauer, M. S.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Swedish, S.] Univ British Columbia, Dept Phys, Vancouver, BC V5Z 1M9, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Julius Maximilians Univ, Fak Phys & Astron, Wurzburg, Germany. [Bannoura, A. A. E.; Beermann, T. A.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Mattig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich C Phys, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Ctr Calcul, Inst Natl Phys Nucl & Phys Particules IN2P3, Villeurbanne, France. [Abulaiti, Y.; Acharya, B. S.; Aguilar-Saavedra, J. A.; Aielli, G.; Akerstedt, H.; Alexa, C.; Aloisio, A.; Alviggi, M. G.; Coutinho, Y. Amaral; Dos Santos, S. P. Amor; Amorim, A.; Andreazza, A.; Andrei, V.; Annovi, A.; Antonov, A.; Anulli, F.; Araque, J. P.; Arik, M.; Asmana, B.; Baas, A. 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Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. EM atlas.publications@cern.ch RI Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Snesarev, Andrey/H-5090-2013; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; Villa, Mauro/C-9883-2009; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; Staroba, Pavel/G-8850-2014; Gavrilenko, Igor/M-8260-2015; Gauzzi, Paolo/D-2615-2009; White, Ryan/E-2979-2015; Mashinistov, Ruslan/M-8356-2015; spagnolo, stefania/A-6359-2012; Buttar, Craig/D-3706-2011; Smirnova, Oxana/A-4401-2013; Doyle, Anthony/C-5889-2009; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Martinez, Mario /I-3549-2015; Peleganchuk, Sergey/J-6722-2014; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Gladilin, Leonid/B-5226-2011; Carvalho, Joao/M-4060-2013; Livan, Michele/D-7531-2012; Tikhomirov, Vladimir/M-6194-2015; Di Domenico, Antonio/G-6301-2011; Boyko, Igor/J-3659-2013; Mitsou, Vasiliki/D-1967-2009; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Brooks, William/C-8636-2013; Gorelov, Igor/J-9010-2015 OI Vykydal, Zdenek/0000-0003-2329-0672; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Villa, Mauro/0000-0002-9181-8048; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Gauzzi, Paolo/0000-0003-4841-5822; White, Ryan/0000-0003-3589-5900; Mashinistov, Ruslan/0000-0001-7925-4676; spagnolo, stefania/0000-0001-7482-6348; Smirnova, Oxana/0000-0003-2517-531X; Doyle, Anthony/0000-0001-6322-6195; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Gladilin, Leonid/0000-0001-9422-8636; Carvalho, Joao/0000-0002-3015-7821; Livan, Michele/0000-0002-5877-0062; Tikhomirov, Vladimir/0000-0002-9634-0581; Di Domenico, Antonio/0000-0001-8078-2759; Boyko, Igor/0000-0002-3355-4662; Mitsou, Vasiliki/0000-0002-1533-8886; Warburton, Andreas/0000-0002-2298-7315; Brooks, William/0000-0001-6161-3570; Gorelov, Igor/0000-0001-5570-0133 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; RGC, Hong Kong SAR, China; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; RGC, Hong Kong SAR, China; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 79 TC 6 Z9 6 U1 8 U2 50 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JUL 17 PY 2015 VL 75 IS 7 AR 330 DI 10.1140/epjc/s10052-015-3544-0 PG 36 WC Physics, Particles & Fields SC Physics GA CS2NP UT WOS:000361908300006 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Ochesanu, S Rougny, R De Klundert, MV Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Daci, N Heracleous, N Keaveney, J Lowette, S Maes, M Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Dobur, D Favart, L Gay, APR Grebenyuk, A Leonard, A Mohammadi, A Pernie, L Randle-Conde, A Reis, T Seva, T Thomas, L Velde, CV Vanlaer, P Wang, J Zenoni, F Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Crucy, S Fagot, A Garcia, G Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Diblen, SS Sigamani, M Strobbe, N Thyssen, F Tytgat, M Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Nuttens, C Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alda, WL Alves, GA Brito, L Martins, MC Martins, TD Molina, J Herrera, CM Pol, ME Teles, PR Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santaolalla, J Santoro, A Sznajder, A Manganote, EJT Pereira, AV Bernardes, CA Dogra, S Tomei, TRFP 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Panwalkar, S. Park, M. Salur, S. Schnetzer, S. Sheffield, D. Somalwar, S. Stone, R. Thomas, S. Thomassen, P. Walker, M. Rose, K. Spanier, S. York, A. Bouhali, O. Hernandez, A. Castaneda Dildick, S. Eusebi, R. Flanagan, W. Gilmore, J. Kamon, T. Khotilovich, V. Krutelyov, V. Montalvo, R. Osipenkov, I. Pakhotin, Y. Patel, R. Perloff, A. Roe, J. Rose, A. Safonov, A. Suarez, I. Tatarinov, A. Ulmer, K. A. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kovitanggoon, K. Kunori, S. Lee, S. W. Libeiro, T. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Johns, W. Maguire, C. Mao, Y. Melo, A. Sharma, M. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Arenton, M. W. Boutle, S. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Wolfe, E. Wood, J. Clarke, C. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Sturdy, J. Belknap, D. A. Carlsmith, D. Cepeda, M. Dasu, S. Dodd, L. Duric, S. Friis, E. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Lanaro, A. Lazaridis, C. Levine, A. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Sarangi, T. Savin, A. Smith, W. H. Taylor, D. Vuosalo, C. Woods, N. CA CMS Collaboration TI Constraints on the pMSSM, AMSB model and on other models from the search for long-lived charged particles in proton-proton collisions at root s=8TeV SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID HIERARCHY AB Stringent limits are set on the long-lived lepton-like sector of the phenomenological minimal supersymmetric standard model (pMSSM) and the anomaly-mediated super-symmetry breaking (AMSB) model. The limits are derived from the results presented in a recent search for long-lived charged particles in proton-proton collisions, based on data collected by the CMS detector at a centre-of-mass energy of 8 TeV at the Large Hadron Collider. In the pMSSM parameter sub-space considered, 95.9% of the points predicting charginos with a lifetime of at least 10 ns are excluded. These constraints on the pMSSM are the first obtained at the LHC. Charginos with a lifetime greater than 100 ns and masses up to about 800 GeV in the AMSB model are also excluded. The method described can also be used to set constraints on other models. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hartl, C.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Kiesenhofer, W.; Knuenz, V.; Krammer, M.; Kraetschmer, I.; Liko, D.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, H.; Schoefbeck, R.; Strauss, J.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] Inst Hochenergiephys OeAW, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. 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B.; Mittag, G.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Nayak, A.; Ntomari, E.; Perrey, H.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Cipriano, P. M. Ribeiro; Roland, B.; Ron, E.; Sahin, M. O.; Salfeld-Nebgen, J.; Saxena, P.; Schoerner-Sadenius, T.; Schroeder, M.; Seitz, C.; Spannagel, S.; Trevino, A. D. R. Vargas; Walsh, R.; Wissing, C.] DESY, Hamburg, Germany. [Blobel, V.; Vignali, M. Centis; Draeger, A. R.; Erfle, J.; Garutti, E.; Goebel, K.; Goerner, M.; Haller, J.; Hoffmann, M.; Hoeing, R. S.; Junkes, A.; Kirschenmann, H.; Klanner, R.; Kogler, R.; Lapsien, T.; Lenz, T.; Marchesini, I.; Marconi, D.; Ott, J.; Peiffer, T.; Perieanu, A.; Pietsch, N.; Poehlsen, J.; Poehlsen, T.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Seidel, M.; Sola, V.; Stadie, H.; Steinbrueck, G.; Troendle, D.; Usai, E.; Vanelderen, L.; Vanhoefer, A.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Frensch, F.; Giffels, M.; Gilbert, A.; Hartmann, F.; Hauth, T.; Husemann, U.; Katkov, I.; Kornmayer, A.; Pardo, P. Lobelle; Mozer, M. U.; Mueller, T.; Mueller, Th.; Nuernberg, A.; Quast, G.; Rabbertz, K.; Roecker, S.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Wolf, R.] Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.; Tziaferi, E.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, M.; Kumar, R.; Mittal, M.; Nishu, N.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Sharma, V.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Jain, Sa.; Jain, Sh.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Mumbai 400085, Maharashtra, India. [Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res, Mumbai 400005, Maharashtra, India. [Sharma, S.] IISER, Pune, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Selvaggi, G.; Sharma, A.; Silvestris, L.; Venditti, R.; Verwilligen, P.] Ist Nazl Fis Nucl, Sez Baria, I-70126 Bari, Italy. [Abbrescia, M.; Calabria, C.; Chhibra, S. S.; Cristella, L.; De Palma, M.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Giordano, F.] CSFNSM, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Ferretti, R.; Ferro, F.; Lo Vetere, M.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Ferretti, R.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Carlin, R.; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Dosselli, U.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Passaseo, M.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Carlin, R.; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Longo, E.; Margaroli, F.; Micheli, F.; Organtini, G.; Rahatlou, S.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Finco, L.; Migliore, E.; Monaco, V.; Pacher, L.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Daegu, South Korea. [Kim, T. J.; Ryu, M. S.] Chonbuk Natl Univ, Jeonju, South Korea. [Kim, J. Y.; Moon, D. H.; Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, I. C.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania. [Komaragiri, J. R.; Ali, M. A. B. Md; Abdullah, W. A. T. Wan] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De la Cruz-Burelo, E.; Heredia-de la Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Golutvin, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Savina, M.; Shmatov, S.; Shulha, S.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, L.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De la Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, IFCA, E-39005 Santander, Spain. [Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Marrouche, J.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Orsini, L.; Pape, L.; Perez, E.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Rolandi, G.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Wollny, H.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Buchmann, M. A.; Casal, B.; Chanon, N.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Hits, D.; Hoss, J.; Lustermann, W.; Mangano, B.; Marini, A. C.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Mohr, N.; Musella, P.; Naegeli, C.; Nessi-Tedaldi, F.; Pandolfi, F.; Pauss, F.; Perrozzi, L.; Peruzzi, M.; Quittnat, M.; Rebane, L.; Rossini, M.; Starodumov, A.; Takahashi, M.; Theofilatos, K.; Wallny, R.; Weber, H. A.] ETH, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Taroni, S.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Chang, P.; Chang, Y. H.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tzeng, Y. M.; Wilken, R.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Gamsizkan, H.; Isildak, B.; Karapinar, G.; Ocalan, K.; Sekmen, S.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Albayrak, E. A.; Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-storey, S. Seif; Senkin, S.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Dauncey, P.; Davies, G.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Mathias, B.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Pastika, N.; Scarborough, T.; Wu, Z.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Lawson, P.; Richardson, C.; Rohlf, J.; John, J. St.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Laird, E.; Landsberg, G.; Narain, M.; Sagir, S.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Rikova, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Incandela, J.; Justus, C.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Krohn, M.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Skinnari, L.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kreis, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Yang, F.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carver, M.; Curry, D.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Field, R. D.; Fisher, M.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Snowball, M.; Sperka, D.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.] UIC, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Haytmyradov, M.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.; Xiao, M.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Gray, J.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Chakaberia, I.; Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Skhirtladze, N.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Belloni, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bierwagen, K.; Busza, W.; Cali, I. A.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Nourbakhsh, S.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Ratnikov, F.; Snow, G. R.; Zvada, M.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; Trocino, D.; Wang, R. J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northeastern Univ, Evanston, IL USA. [Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Lynch, S.; Marinelli, N.; Musienko, Y.; Pearson, T.; Planer, M.; Ruchti, R.; Smith, G.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Malik, S.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Barnes, V. E.; Benedetti, D.; Bortoletto, D.; De Mattia, M.; Gutay, L.; Hu, Z.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Miller, D. H.; Neumeister, N.; Primavera, F.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Zablocki, J.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Hindrichs, O.; Khukhunaishvili, A.; Korjenevski, S.; Petrillo, G.; Verzetti, M.; Vishnevskiy, D.] Univ Rochester, Rochester, NY 14627 USA. [Ciesielski, R.; Demortier, L.; Goulianos, K.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Kaplan, S.; Lath, A.; Panwalkar, S.; Park, M.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Hernandez, A. Castaneda; Dildick, S.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Krutelyov, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Patel, R.; Perloff, A.; Roe, J.; Rose, A.; Safonov, A.; Suarez, I.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kovitanggoon, K.; Kunori, S.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Wolfe, E.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Dodd, L.; Duric, S.; Friis, E.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Lazaridis, C.; Levine, A.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. H.; Taylor, D.; Vuosalo, C.; Woods, N.] Univ Wisconsin, Madison, WI 53706 USA. [Fruehwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Rabady, D.; Pernie, L.; Genchev, V.; Boudoul, G.; Contardo, D.; Lingemann, J.; Hartmann, F.; Kornmayer, A.; Radogna, R.; Silvestris, L.; Giordano, F.; Gennai, S.; Gerosa, R.; Lucchini, M. T.; Di Guida, S.; Meola, S.; Paolucci, P.; Spiezia, A.; Donato, S.; Palla, F.; Micheli, F.; Traczyk, P.; Finco, L.; Candelise, V.; Stickland, D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Beluffi, C.] Univ Haute Alsace Mulhouse, Univ Strasbourg, CNRS IN2P3, Inst Pluridisciplinaire Hubert Curien, Strasbourg, France. [Giammanco, A.] NICPB, Tallinn, Estonia. [Popov, A.; Zhukov, V.; Katkov, I.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, SP, Brazil. [Plestina, R.; Bernet, C.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, Palaiseau, France. [Finger, M., Jr.] Joint Inst Nucl Res, Dubna, Russia. [Assran, Y.] Suez Univ, Suez, Egypt. [Elgammal, S.; Radi, A.] British Univ Egypt, Cairo, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Radi, A.] Ain Shams Univ, Cairo, Egypt. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Bagaturia, I.] Ilia State Univ, Tbilisi, Rep of Georgia. [Hempel, M.; Karacheban, O.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Horvath, D.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Karancsi, J.] Univ Debrecen, Debrecen, Hungary. [Bhowmik, S.; Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Plasma Phys Res Ctr, Sci & Res Branch, Tehran, Iran. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.; Squillacioti, P.] Univ Siena, I-53100 Siena, Italy. [Moon, C. S.] CNRS, IN2P3, Paris, France. [Savoy-Navarro, A.] Purdue Univ, W Lafayette, IN 47907 USA. [Matveev, V.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, Moscow, Russia. [Azarkin, M.; Dremin, I.; Leonidov, A.] Moscow Engn Phys Inst, Moscow 115409, Russia. [Dubinin, M.] CALTECH, Pasadena, CA 91125 USA. Univ Belgrade, Fac Phys, Belgrade, Serbia. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Rolandi, G.] Ist Nazl Fis Nucl, Scuola Normale & Sez, Pisa, Italy. [Sphicas, P.] Univ Athens, Athens, Greece. [Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.; Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Kangal, E. E.] Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. [Gamsizkan, H.] Anadolu Univ, Eskisehir, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Ocalan, K.] Necmettin Erbakan Univ, Konya, Turkey. [Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, T.] Yildiz Tech Univ, Istanbul, Turkey. [Newbold, D. M.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Milenovic, P.] Univ Belgrade, Fac Phys, Vinca Inst Nucl Sci, Belgrade, Serbia. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. [Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. [CMS Collaboration] CERN, CH-1211 Geneva 23, Switzerland. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Sguazzoni, Giacomo/J-4620-2015; Ligabue, Franco/F-3432-2014; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Paulini, Manfred/N-7794-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; ciocci, maria agnese /I-2153-2015; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Chinellato, Jose Augusto/I-7972-2012; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Stahl, Achim/E-8846-2011; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Menasce, Dario/A-2168-2016; Paganoni, Marco/A-4235-2016; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Dogra, Sunil /B-5330-2013; Leonidov, Andrey/M-4440-2013; Calvo Alamillo, Enrique/L-1203-2014; Hernandez Calama, Jose Maria/H-9127-2015; Cerrada, Marcos/J-6934-2014; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Novaes, Sergio/D-3532-2012; Della Ricca, Giuseppe/B-6826-2013; Andreev, Vladimir/M-8665-2015; Lokhtin, Igor/D-7004-2012; Manganote, Edmilson/K-8251-2013; Gennai, Simone/P-2880-2015; TUVE', Cristina/P-3933-2015; Dudko, Lev/D-7127-2012; VARDARLI, Fuat Ilkehan/B-6360-2013; Vinogradov, Alexey/O-2375-2015; Petrushanko, Sergey/D-6880-2012; Cakir, Altan/P-1024-2015; Montanari, Alessandro/J-2420-2012; Matorras, Francisco/I-4983-2015; KIM, Tae Jeong/P-7848-2015 OI Gonzi, Sandro/0000-0003-4754-645X; Bilki, Burak/0000-0001-9515-3306; Sguazzoni, Giacomo/0000-0002-0791-3350; Casarsa, Massimo/0000-0002-1353-8964; Ligabue, Franco/0000-0002-1549-7107; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Ghezzi, Alessio/0000-0002-8184-7953; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Ciulli, Vitaliano/0000-0003-1947-3396; Androsov, Konstantin/0000-0003-2694-6542; Fiorendi, Sara/0000-0003-3273-9419; Martelli, Arabella/0000-0003-3530-2255; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Ogul, Hasan/0000-0002-5121-2893; ciocci, maria agnese /0000-0003-0002-5462; Di Matteo, Leonardo/0000-0001-6698-1735; Boccali, Tommaso/0000-0002-9930-9299; Gerosa, Raffaele/0000-0001-8359-3734; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Chinellato, Jose Augusto/0000-0002-3240-6270; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Stahl, Achim/0000-0002-8369-7506; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Menasce, Dario/0000-0002-9918-1686; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Calvo Alamillo, Enrique/0000-0002-1100-2963; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Cerrada, Marcos/0000-0003-0112-1691; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; TUVE', Cristina/0000-0003-0739-3153; Dudko, Lev/0000-0002-4462-3192; Montanari, Alessandro/0000-0003-2748-6373; Matorras, Francisco/0000-0003-4295-5668; KIM, Tae Jeong/0000-0001-8336-2434 FU BMWFW (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia); ERC IUT (Estonia); ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP (Republic of Korea); NRF (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (NewZealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie programme (European Union); European Research Council (European Union); EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS programme of Foundation for Polish Science; European Union, Regional Development Fund; Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR (Italy) [20108T4XTM]; Thalis programme; Aristeia programme; EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP and NRF (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (NewZealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (USA). Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS programme of Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; and the National Priorities Research Program by Qatar National Research Fund. NR 28 TC 1 Z9 1 U1 9 U2 35 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JUL 17 PY 2015 VL 75 IS 7 AR 325 DI 10.1140/epjc/s10052-015-3533-3 PG 29 WC Physics, Particles & Fields SC Physics GA CS2NP UT WOS:000361908300001 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S 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Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, M Becker, S Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Black, CW Black, JE Black, KM Blackburn, D 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H Burdin, S Burghgrave, B Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Buszello, CP Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Buzykaev, R Urban, SC Caforio, D Cairo, VM Cakir, O Calafiura, P Calandri, A Calderini, G Calfayan, P Caloba, LP Calvet, D Calvet, S Toro, RC Camarda, S Camarri, P Cameron, D Caminada, LM Armadans, RC Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Cardarelli, R Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Caudron, J Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, BC Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chang, P Chapleau, B Chapman, JD Charlton, DG Chau, CC Barajas, CAC Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A Cheremushkina, E El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Childers, JT Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Choi, K Chouridou, S Chow, BKB Christodoulou, V Chromek-Burckhart, D Chu, ML Chudoba, J Chuinard, AJ Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Cinca, D Cindro, V Cioara, IA Ciocio, A Citron, ZH Ciubancan, M Clark, A Clark, BL Clark, PJ Clarke, RN Cleland, W Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Cogan, JG Cole, B Cole, S Colijn, AP Collot, J Colombo, T Compostella, G Muino, PC Coniavitis, E Connell, SH Connelly, IA Consonni, SM Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cote, D Cottin, G Cowan, G Cox, BE Cranmer, K Cree, G Crepe-Renaudin, S Crescioli, F Cribbs, WA Ortuzar, MC Cristinziani, M Croft, V Crosetti, G Donszelmann, TC Cummings, J Curatolo, M Cuthbert, C Czirr, H Czodrowski, P D'Auria, S D'Onofrio, M De Sousa, MJDS Da Via, C Dabrowski, W Dafinca, A Dai, T Dale, O Dallaire, F Dallapiccola, C Dam, M Dandoy, JR Dang, NP Daniells, AC Danninger, M Hoffmann, MD Dao, V Darbo, G Darmora, S Dassoulas, J Dattagupta, A Davey, W David, C Davidek, T Davies, E Davies, M Davison, P Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Castro, S De Cecco, S De Groot, N de Jong, P De la Torre, H De Lorenzi, F De Nooij, L De Pedis, D De Salvo, A De Sanctis, U De Santo, A De Regie, JBD Dearnaley, WJ Debbe, R Debenedetti, C Dedovich, DV Deigaard, I Del Peso, J Del Prete, T Delgove, D Deliot, F Delitzsch, CM Deliyergiyev, M Dell'Acqua, A Dell'Asta, L Dell'Orso, M Della Pietra, 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CA ATLAS Collaboration TI Search for long-lived, weakly interacting particles that decay to displaced hadronic jets in proton-proton collisions at root s=8 TeV with the ATLAS detector SO PHYSICAL REVIEW D LA English DT Article ID SUPERSYMMETRY; HIGGS AB A search for the decay of neutral, weakly interacting, long-lived particles using data collected by the ATLAS detector at the LHC is presented. This analysis uses the full data set recorded in 2012: 20.3 fb(-1) of proton-proton collision data at root s = 8 TeV. The search employs techniques for reconstructing decay vertices of long-lived particles decaying to jets in the inner tracking detector and muon spectrometer. Signal events require at least two reconstructed vertices. No significant excess of events over the expected background is found, and limits as a function of proper lifetime are reported for the decay of the Higgs boson and other scalar bosons to long-lived particles and for Hidden Valley Z' and Stealth SUSY benchmark models. The first search results for displaced decays in Z' and Stealth SUSY models are presented. The upper bounds of the excluded proper lifetimes are the most stringent to date. C1 [Jackson, P.; Lee, L.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Yildiz, H. Duran] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Kuday, S.] Istanbul Aydin Univ, Istanbul, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. [Barnovska, Z.; Berger, N.; Delmastro, M.; Di Ciaccio, L.; Elles, S.; Hryn'ova, T.; Jezequel, S.; Koletsou, I.; Lafaye, R.; Leveque, J.; Massol, N.; Sauvage, G.; Sauvan, E.; Schwoerer, M.; Simard, O.; Todorov, T.; Wingerter-Seez, I.; Yatsenko, E.] CNRS, IN2P3, LAPP, Annecy Le Vieux, France. [Barnovska, Z.; Berger, N.; Delmastro, M.; Di Ciaccio, L.; Elles, S.; Hryn'ova, T.; Jezequel, S.; Koletsou, I.; Lafaye, R.; Leveque, J.; Massol, N.; Sauvage, G.; Sauvan, E.; Schwoerer, M.; Simard, O.; Todorov, T.; Wingerter-Seez, I.; Yatsenko, E.] Univ Savoie Mont Blanc, Annecy Le Vieux, France. [Auerbach, B.; Blair, R. E.; Chekanov, S.; Feng, E. J.; LeCompte, T.; Love, J.; Malon, D.; Nguyen, D. H.; Paramonov, A.; Price, L. E.; Proudfoot, J.; van Gemmeren, P.; Vaniachine, A.; Wang, R.; Yoshida, R.; Zhang, J.] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Cheu, E.; Johns, K. A.; Lampen, C. L.; Lampl, W.; Lei, X.; Leone, R.; Loch, P.; Nayyar, R.; O'grady, F.; Shupe, M. A.; Varnes, E. W.; Veatch, J.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Brandt, A.; Bullock, D.; Carrillo-Montoya, G. D.; Cote, D.; Darmora, S.; De, K.; Farbin, A.; Griffiths, J.; Hadavand, H. K.; Heelan, L.; Kim, H. Y.; Ozturk, N.; Schovancova, J.; Sosebee, M.; Stradling, A. R.; Usai, G.; Vartapetian, A.; White, A.; Yu, J.] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA. [Angelidakis, S.; Chouridou, S.; Fassouliotis, D.; Giokaris, N.; Ioannou, P.; Kourkoumelis, C.; Manousakis-Katsikakis, A.; Tsirintanis, N.] Univ Athens, Dept Phys, Athens, Greece. [Alexander, G.; Benekos, N.; Dris, M.; Gazis, E. N.; Karakostas, K.; Karastathis, N.; Leontsinis, S.; Maltezos, S.; Ntekas, K.; Panagiotopoulou, E.; Papadopoulou, Th. D.; Tsipolitis, G.; Vlachos, S.] Natl Tech Univ Athens, Dept Phys, GR-15773 Zografos, Greece. [Abdinov, O.; Ahmadov, F.; Huseynov, N.; Javadov, N.; Khalil-zada, F.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Anjos, N.; Bosman, M.; Caminal Armadans, R.; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fischer, C.; Fracchia, S.; Giangiobbe, V.; Gonzalez Parra, G.; Grinstein, S.; Juste Rozas, A.; Korolkov, I.; Lange, J. C.; Le Menedeu, E.; Lopez Paz, I.; Martinez, M.; Mir, L. M.; Montejo Berlingen, J.; Pacheco Pages, A.; Padilla Aranda, C.; Riu, I.; Sorin, V.; Succurro, A.; Tripiana, M. F.; Tsiskaridze, S.; Valery, L.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Anjos, N.; Bosman, M.; Caminal Armadans, R.; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fischer, C.; Fracchia, S.; Giangiobbe, V.; Gonzalez Parra, G.; Grinstein, S.; Juste Rozas, A.; Korolkov, I.; Lange, J. C.; Le Menedeu, E.; Lopez Paz, I.; Martinez, M.; Mir, L. M.; Montejo Berlingen, J.; Pacheco Pages, A.; Padilla Aranda, C.; Riu, I.; Sorin, V.; Succurro, A.; Tripiana, M. F.; Tsiskaridze, S.; Valery, L.] Univ Autonoma Barcelona, Dept Fis, E-08193 Barcelona, Spain. [Agatonovic-Jovin, T.; Bozic, I.; Dimitrievska, A.; Krstic, J.; Marjanovic, M.; Popovic, D. S.; Sijacki, Dj.; Simic, Lj.; Vranjes, N.; Milosavljevic, M. Vranjes; Zivkovic, L.] Univ Belgrade, Inst Phys, Belgrade, Serbia. [Buanes, T.; Dale, O.; Kastanas, A.; Liebig, W.; Lipniacka, A.; Maeland, S.; Latour, B. Martin Dit; Rosendahl, P. L.; Sandaker, H.; Sjursen, T. B.; Smestad, L.; Stugu, B.; Ugland, M.; Zalieckas, J.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Amadio, B. T.; Axen, B.; Barnett, R. M.; Beringer, J.; Brosamer, J.; Calafiura, P.; Caminada, L. M.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, L.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Amadio, B. T.; Axen, B.; Barnett, R. M.; Beringer, J.; Brosamer, J.; Calafiura, P.; Caminada, L. M.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, L.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Dietrich, J.; Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Herrberg-Schubert, R.; Hristova, I.; Kind, O. M.; Kolanoski, H.; Lacker, H.; Lohse, T.; Nikiforov, A.; Rehnisch, L.; Rieck, P.; Schulz, H.; Stamm, S.; zur Nedden, M.] Humboldt Univ, Dept Phys, Berlin, Germany. [Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allbrooke, B. M. M.; Bella, L. Aperio; Bansil, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Hawkes, C. M.; Head, S. J.; Hiller, K. H.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Owen, R. E.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Alberghi, G. L.; Bellagamba, L.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Corradi, M.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, Bologna, Italy. [Alberghi, G. L.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Cioara, I. A.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Hageboeck, S.; Hansen, M. C.; Hellmich, D.; Hohn, D.; Huegging, F.; Janssen, J.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mergelmeyer, S.; Mijovic, L.; Mueller, K.; Obermann, T.; Pohl, D.; Ricken, O.; Sarrazin, B.; Schaepe, S.; Schopf, E.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Seema, P.; Stillings, J. A.; Tannoury, N.; Therhaag, J.; Uhlenbrock, M.; Velz, T.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Fitzgerald, E. A.; Sciolla, G.; Venturini, A.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Fed Univ Juiz de Fora UFJF, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; La Rosa Navarro, J. L.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Gonzalez, B. Alvarez; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Iengo, P.; Jaekel, M. R.; Jakobsen, S.; Jenni, P.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Liu, B.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, DK-1168 Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, Frascati, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Ancu, L. S.; Barone, G.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nessi, M.; Paolozzi, L.; Picazio, A.; Ristic, B.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bindi, M.; Blumenschein, U.; Brandt, G.; Clement, C.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R. W.; Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Iowa City, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] Dubna Joint Nucl Res Inst, Dubna 141980, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, S.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Allport, P. P.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Teixeira Dias Castanheira, M.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Poettgen, R.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Hu, X.; Levin, D.; Long, J. D.; Lu, N.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Xu, L.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. 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A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzoloa, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Koenig, S.; Nektarijevic, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Gjelsten, B. K.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Sawyer, C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr, Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Aloisio, A.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwegler, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, DSM IRFU Inst Rech Lois Fondament Univers, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Torres, H.; van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Ilic, N.; Kagan, M.; Kocian, M.; Mount, R.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.; Meehan, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Govender, N.; Lee, C. A.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hamilton, A.; Hsu, C.; March, L.; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Munwes, Y.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Jovicevic, J.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] Ist Nazl Fis Nucl, Sez Trieste, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Neubauer, M. S.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. 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L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Beermann, T. A.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. 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[Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Khubua, J.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Pinamonti, M.] SISSA, Int Sch Adv Studies, I-34014 Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. 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RI Livan, Michele/D-7531-2012; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; spagnolo, stefania/A-6359-2012; Di Domenico, Antonio/G-6301-2011; Negrini, Matteo/C-8906-2014; Tassi, Enrico/K-3958-2015; Boyko, Igor/J-3659-2013; Ciubancan, Liviu Mihai/L-2412-2015; White, Ryan/E-2979-2015; Mitsou, Vasiliki/D-1967-2009; Zhukov, Konstantin/M-6027-2015; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Petrucci, Fabrizio/G-8348-2012; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Martinez, Mario /I-3549-2015; Peleganchuk, Sergey/J-6722-2014; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Garcia, Jose /H-6339-2015; Korol, Aleksandr/A-6244-2014; Kantserov, Vadim/M-9761-2015; BESSON, NATHALIE/L-6250-2015; La Rosa Navarro, Jose Luis/K-4221-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; Staroba, Pavel/G-8850-2014; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Buttar, Craig/D-3706-2011; Smirnova, Oxana/A-4401-2013; Doyle, Anthony/C-5889-2009; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Snesarev, Andrey/H-5090-2013; Veneziano, Stefano/J-1610-2012; Tikhomirov, Vladimir/M-6194-2015; Villa, Mauro/C-9883-2009; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Brooks, William/C-8636-2013; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; De, Kaushik/N-1953-2013; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015 OI Price, Darren/0000-0003-2750-9977; Belanger-Champagne, Camille/0000-0003-2368-2617; Livan, Michele/0000-0002-5877-0062; Camarri, Paolo/0000-0002-5732-5645; spagnolo, stefania/0000-0001-7482-6348; Di Domenico, Antonio/0000-0001-8078-2759; Negrini, Matteo/0000-0003-0101-6963; Boyko, Igor/0000-0002-3355-4662; Ciubancan, Liviu Mihai/0000-0003-1837-2841; White, Ryan/0000-0003-3589-5900; Mitsou, Vasiliki/0000-0002-1533-8886; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Petrucci, Fabrizio/0000-0002-5278-2206; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Giorgi, Filippo Maria/0000-0003-1589-2163; Coccaro, Andrea/0000-0003-2368-4559; Della Volpe, Domenico/0000-0001-8530-7447; Sotiropoulou, Calliope-Louisa/0000-0001-9851-1658; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Sannino, Mario/0000-0001-7700-8383; Korol, Aleksandr/0000-0001-8448-218X; Giordani, Mario/0000-0002-0792-6039; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Smirnova, Oxana/0000-0003-2517-531X; Doyle, Anthony/0000-0001-6322-6195; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Veneziano, Stefano/0000-0002-2598-2659; Tikhomirov, Vladimir/0000-0002-9634-0581; Villa, Mauro/0000-0002-9181-8048; Warburton, Andreas/0000-0002-2298-7315; Brooks, William/0000-0001-6161-3570; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; De, Kaushik/0000-0002-5647-4489; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; RGC, China; Hong Kong SAR, China; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia; NRC KI; Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; RGC, Hong Kong SAR, China; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 49 TC 2 Z9 2 U1 10 U2 57 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JUL 17 PY 2015 VL 92 IS 1 AR 012010 DI 10.1103/PhysRevD.92.012010 PG 28 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CM9MO UT WOS:000358032700004 ER PT J AU Davoudiasl, H Zhang, Y AF Davoudiasl, Hooman Zhang, Yue TI Baryon number violation via Majorana neutrinos in the early Universe, at the LHC, and deep underground SO PHYSICAL REVIEW D LA English DT Article ID BARYOGENESIS; MASS AB We propose and investigate a novel, minimal, and experimentally testable framework for baryogenesis, dubbed dexiogenesis, using baryon number violating effective interactions of right-handed Majorana neutrinos responsible for the seesaw mechanism. The distinct LHC signature of our framework is samesign top quark final states, possibly originating from displaced vertices. The region of parameters relevant for LHC phenomenology can also yield concomitant signals in nucleon decay experiments. We provide a simple ultraviolet origin for our effective operators, by adding a color-triplet scalar, which could ultimately arise from a grand unified theory. C1 [Davoudiasl, Hooman] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Zhang, Yue] CALTECH, Walter Burke Inst Theoret Phys, Pasadena, CA 91125 USA. RP Davoudiasl, H (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. EM hooman@bnl.gov; yuezhang@theory.caltech.edu FU United States Department of Energy [DE-SC0012704]; Gordon and Betty Moore Foundation [776]; DOE [DE-FG02-92ER40701]; DOE Early Career Award [DE-SC0010255] FX We would like to thank B. Dev, P. Meade, R. Mohapatra, and G. Senjanovic for discussions. We also thank B. Dev and R. Mohapatra for informing us of their forthcoming paper on related topics [40]. The work of H. D. is supported in part by the United States Department of Energy under Contract No. DE-SC0012704. The work of Y. Z. is supported by the Gordon and Betty Moore Foundation through Grant No. 776 to the Caltech Moore Center for Theoretical Cosmology and Physics, and by DOE Grant No. DE-FG02-92ER40701, and also by a DOE Early Career Award under Grant No. DE-SC0010255. Y. Z. thanks the BNL theory group for hospitality at the final stage of this paper. NR 42 TC 3 Z9 3 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JUL 17 PY 2015 VL 92 IS 1 AR 016005 DI 10.1103/PhysRevD.92.016005 PG 6 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CM9MO UT WOS:000358032700010 ER PT J AU Lu, QQ Liu, ZL Luo, Y Zhang, GH Huang, ZY Wang, HM Liu, C Miller, JT Lei, AW AF Lu, Qingquan Liu, Zhiliang Luo, Yi Zhang, Guanghui Huang, Zhiyuan Wang, Huamin Liu, Chao Miller, Jeffrey T. Lei, Aiwen TI Copper-/Cobalt-Catalyzed Highly Selective Radical Dioxygenation of Alkenes SO ORGANIC LETTERS LA English DT Article ID MOLECULAR-OXYGEN; METAL-FREE; AEROBIC DIOXYGENATION; N-HYDROXYPHTHALIMIDE; ORGANIC-SYNTHESIS; TERMINAL ALKYNES; HYDROXAMIC ACID; OXIDATION; OLEFINS; KETONES AB A highly selective radical dioxygenation of alkenes using hydroxamic acid and O-2 was developed, and copper/cobalt was used as the catalyst without assistance of any additional ligands or bases. Mechanistic investigation disclosed that copper salt and O-2 work in concert to activate hydroxamic acid, with Cu(I) and Cu(II) concurrently existing in this reaction. C1 [Lu, Qingquan; Liu, Zhiliang; Luo, Yi; Zhang, Guanghui; Huang, Zhiyuan; Wang, Huamin; Liu, Chao; Lei, Aiwen] Wuhan Univ, Inst Adv Studies IAS, Coll Chem & Mol Sci, Wuhan 430072, Hubei, Peoples R China. [Lei, Aiwen] Jiangxi Normal Univ, Natl Res Ctr Carbohydrate Synth, Nanchang 330022, Jiangxi, Peoples R China. [Miller, Jeffrey T.] Purdue Univ, Dept Chem Engn, W Lafayette, IN 47907 USA. [Liu, Chao; Miller, Jeffrey T.; Lei, Aiwen] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Lei, AW (reprint author), Wuhan Univ, Inst Adv Studies IAS, Coll Chem & Mol Sci, Wuhan 430072, Hubei, Peoples R China. EM aiwenlei@whu.edu.cn RI Zhang, Guanghui/C-4747-2008 OI Zhang, Guanghui/0000-0002-5854-6909 FU 973 Program [2012CB725302]; National Natural Science Foundation of China [21390400, 21025206, 21272180, 21302148]; Research Fund for the Doctoral Program of Higher Education of China [20120141130002]; Ministry of Science and Technology of China [2012YQ120060]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by the 973 Program (2012CB725302), the National Natural Science Foundation of China (21390400, 21025206, 21272180, and 21302148), the Research Fund for the Doctoral Program of Higher Education of China (20120141130002), and the Ministry of Science and Technology of China (2012YQ120060). The Program of Introducing Talents of Discipline to Universities of China (111 Program) is also acknowledged. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. MRCAT operations are supported by the Department of Energy and the MRCAT member institutions. NR 48 TC 19 Z9 19 U1 11 U2 94 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1523-7060 EI 1523-7052 J9 ORG LETT JI Org. Lett. PD JUL 17 PY 2015 VL 17 IS 14 BP 3402 EP 3405 DI 10.1021/acs.orglett.5b01223 PG 4 WC Chemistry, Organic SC Chemistry GA CN4JD UT WOS:000358395500007 PM 26125090 ER PT J AU Johnson, RE de Rond, T Lindsay, VNG Keasling, JD Sarpong, R AF Johnson, Rebecca E. de Rond, Tristan Lindsay, Vincent N. G. Keasling, Jay D. Sarpong, Richmond TI Synthesis of Cycloprodigiosin Identifies the Natural Isolate as a Scalemic Mixture SO ORGANIC LETTERS LA English DT Article ID PRODIGIOSIN; HYDROCHLORIDE; BIOSYNTHESIS; APOPTOSIS; PYRROLES AB The enantiomers of the natural product cycloprodigiosin were prepared using an expedient five-step synthetic sequence that takes advantage of a Schollkopf-Barton-Zard (SBZ) pyrrole annulation with a chiral isocyanoacetate and a nitrocyclohexene derivative. Using chiral HPLC and X-ray crystallographic analyses of the synthetically prepared Material and natural isolate (isolated from the marine bacterium Pseudoalteromonas rubra), naturally occurring cyclo-prodigiosin was determined to be a scalemic mixture occurring in an enantiomeric ratio of 83:17 (R)/(S) at C4'. C1 [Johnson, Rebecca E.; de Rond, Tristan; Lindsay, Vincent N. G.; Sarpong, Richmond] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Dept Bioengn, Berkeley, CA 94720 USA. [Keasling, Jay D.] Univ Calif Berkeley, Inst QB3, Berkeley, CA 94720 USA. [Keasling, Jay D.] Joint BioEnergy Inst, Emeryville, CA 94608 USA. [Keasling, Jay D.] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94270 USA. RP Sarpong, R (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM rsarpong@berkeley.edu FU NIGMS [NIGMS 086374]; FRQNT [B3]; National Science Foundation [1341894]; U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231]; NIH [S10-RR027172] FX We are grateful to the NIGMS for financial support (NIGMS 086374) and to FRQNT (B3) for a postdoctoral scholarship to V.N.G.L. This work is supported in part by the National Science Foundation (Grant No. 1341894). This work was part of the DOE Joint BioEnergy Institute (http://www.jbei.org), supported by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, through Contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the U.S. Department of Energy. We thank Dr. Antonio DiPasquale (UC Berkeley) for solving the crystal structure of (R)-2 center dot HCl and determining its absolute stereochemistry (Supported by NIH Shared Instrumentation Grant S10-RR027172). We acknowledge the CYLView program (developed by Prof. Claude Y. Legault, Dept. of Chemistry, Universite de Sherbrooke) for X-ray depictions. NR 28 TC 2 Z9 2 U1 2 U2 13 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1523-7060 EI 1523-7052 J9 ORG LETT JI Org. Lett. PD JUL 17 PY 2015 VL 17 IS 14 BP 3474 EP 3477 DI 10.1021/acs.orglett.5b01527 PG 4 WC Chemistry, Organic SC Chemistry GA CN4JD UT WOS:000358395500025 PM 26114660 ER PT J AU Wu, HF Qiao, Q Teng, P Hu, YG Antoniadis, D Zuo, XB Cai, JF AF Wu, Haifan Qiao, Qiao Teng, Peng Hu, Yaogang Antoniadis, Dimitrios Zuo, Xiaobing Cai, Jianfeng TI New Class of Heterogeneous Helical Peptidomimetics SO ORGANIC LETTERS LA English DT Article ID GAMMA-AAPEPTIDES; ALPHA/BETA-PEPTIDES; SECONDARY STRUCTURE; PEPTOID OLIGOMERS; BETA-PEPTIDES; SIDE-CHAINS; FOLDAMERS; DESIGN; BACKBONE; ACIDS AB A new class of unnatural heterogeneous foldamers is reported to contain alternative a-amino acid and sulfono-gamma-AA amino acid residues in a 1:1 repeat pattern. Two-dimensional NMR data show that two 1:1 alpha/sulfono-gamma-AA peptides with diverse side chains form analogous right-handed helical structures in solution. The effects of sequence length, side chain, N-capping, and temperature on folding. propensity were further investigated using circular dichroism and small-angle X-ray scattering. C1 [Wu, Haifan; Qiao, Qiao; Teng, Peng; Hu, Yaogang; Antoniadis, Dimitrios; Cai, Jianfeng] Univ S Florida, Dept Chem, Tampa, FL 33620 USA. [Zuo, Xiaobing] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Cai, JF (reprint author), Univ S Florida, Dept Chem, 4202 E Fowler Ave, Tampa, FL 33620 USA. EM jianfengcai@usf.edu RI Teng, Peng/K-1046-2015; Wu, Haifan/F-8818-2014; OI Wu, Haifan/0000-0002-2050-9950; Zuo, Xiaobing/0000-0002-0134-4804 FU NSF [1351265] FX This work is supported by NSF CAREER 1351265. We thank Prof. Mark McLaughlin (USF, Department of Chemistry) for useful discussions. NR 38 TC 7 Z9 7 U1 1 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1523-7060 EI 1523-7052 J9 ORG LETT JI Org. Lett. PD JUL 17 PY 2015 VL 17 IS 14 BP 3524 EP 3527 DI 10.1021/acs.orglett.5b01608 PG 4 WC Chemistry, Organic SC Chemistry GA CN4JD UT WOS:000358395500038 PM 26153619 ER PT J AU Jiang, WJ Upadhyaya, P Zhang, W Yu, GQ Jungfleisch, MB Fradin, FY Pearson, JE Tserkovnyak, Y Wang, KL Heinonen, O te Velthuis, SGE Hoffmann, A AF Jiang, Wanjun Upadhyaya, Pramey Zhang, Wei Yu, Guoqiang Jungfleisch, M. Benjamin Fradin, Frank Y. Pearson, John E. Tserkovnyak, Yaroslav Wang, Kang L. Heinonen, Olle te Velthuis, Suzanne G. E. Hoffmann, Axel TI Blowing magnetic skyrmion bubbles SO SCIENCE LA English DT Article ID DOMAIN-WALLS; SPIN-TORQUE; DYNAMICS; LATTICE; DRIVEN; FILMS AB The formation of soap bubbles from thin films is accompanied by topological transitions. Here we show how a magnetic topological structure, a skyrmion bubble, can be generated in a solid-state system in a similar manner. Using an inhomogeneous in-plane current in a system with broken inversion symmetry, we experimentally "blow" magnetic skyrmion bubbles from a geometrical constriction. The presence of a spatially divergent spin-orbit torque gives rise to instabilities of the magnetic domain structures that are reminiscent of Rayleigh-Plateau instabilities in fluid flows. We determine a phase diagram for skyrmion formation and reveal the efficient manipulation of these dynamically created skyrmions, including depinning and motion. The demonstrated current-driven transformation from stripe domains to magnetic skyrmion bubbles could lead to progress in skyrmion-based spintronics. C1 [Jiang, Wanjun; Zhang, Wei; Jungfleisch, M. Benjamin; Fradin, Frank Y.; Pearson, John E.; Heinonen, Olle; te Velthuis, Suzanne G. E.; Hoffmann, Axel] Argonne Natl Lab, Mat Sci Div, Lemont, IL 60439 USA. [Upadhyaya, Pramey; Yu, Guoqiang; Wang, Kang L.] Univ Calif Los Angeles, Dept Elect Engn, Device Res Lab, Los Angeles, CA 90095 USA. [Tserkovnyak, Yaroslav] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Heinonen, Olle] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [Heinonen, Olle] Northwestern Univ, Northwestern Argonne Inst Sci & Engn, Evanston, IL 60208 USA. [Heinonen, Olle] Univ Chicago, Computat Inst, Chicago, IL 60637 USA. RP Hoffmann, A (reprint author), Argonne Natl Lab, Mat Sci Div, Lemont, IL 60439 USA. EM hoffmann@anl.gov RI Yu, Guoqiang/F-1871-2013; Hoffmann, Axel/A-8152-2009; te Velthuis, Suzanne/I-6735-2013; Jungfleisch, Matthias Benjamin/G-1069-2015; Jiang, Wanjun/E-6994-2011; OI Yu, Guoqiang/0000-0002-7439-6920; Hoffmann, Axel/0000-0002-1808-2767; te Velthuis, Suzanne/0000-0002-1023-8384; Jungfleisch, Matthias Benjamin/0000-0001-8204-3677; Jiang, Wanjun/0000-0003-0918-3862; Heinonen, Olle/0000-0002-3618-6092 FU U.S. Department of Energy (DOE), Office of Science, Materials Science and Engineering Division; DOE, Office of Science, Basic Energy Sciences [DE-AC02-06CH11357]; NSF Nanosystems Engineering Research Center for Translational Applications of Nanoscale Multiferroic Systems FX Work carried out at Argonne National Laboratory was supported by the U.S. Department of Energy (DOE), Office of Science, Materials Science and Engineering Division. Lithography was carried out at the Center for Nanoscale Materials, an Office of Science user facility, which is supported by the DOE, Office of Science, Basic Energy Sciences, under contract no. DE-AC02-06CH11357. Work performed at the University of California, Los Angeles, was partially supported by the NSF Nanosystems Engineering Research Center for Translational Applications of Nanoscale Multiferroic Systems. We thank I. Martin and I. Aronson for insightful discussion. NR 47 TC 126 Z9 127 U1 55 U2 233 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JUL 17 PY 2015 VL 349 IS 6245 SI SI BP 283 EP 286 DI 10.1126/science.aaa1442 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CN1ZB UT WOS:000358218600045 PM 26067256 ER PT J AU Tan, BS Hsu, YT Zeng, B Hatnean, MC Harrison, N Zhu, Z Hartstein, M Kiourlappou, M Srivastava, A Johannes, MD Murphy, TP Park, JH Balicas, L Lonzarich, GG Balakrishnan, G Sebastian, SE AF Tan, B. S. Hsu, Y. -T. Zeng, B. Hatnean, M. Ciomaga Harrison, N. Zhu, Z. Hartstein, M. Kiourlappou, M. Srivastava, A. Johannes, M. D. Murphy, T. P. Park, J. -H. Balicas, L. Lonzarich, G. G. Balakrishnan, G. Sebastian, Suchitra E. TI Unconventional Fermi surface in an insulating state SO SCIENCE LA English DT Article ID INDUCED SUPERCONDUCTIVITY; QUANTUM CRITICALITY; KONDO INSULATORS; SMB6; GAP; EXCITATIONS; VALENCE; PRESSURE; CERHIN5; LIQUIDS AB Insulators occur in more than one guise; a recent finding was a class of topological insulators, which host a conducting surface juxtaposed with an insulating bulk. Here, we report the observation of an unusual insulating state with an electrically insulating bulk that simultaneously yields bulk quantum oscillations with characteristics of an unconventional Fermi liquid. We present quantum oscillation measurements of magnetic torque in high-purity single crystals of the Kondo insulator SmB6, which reveal quantum oscillation frequencies characteristic of a large three-dimensional conduction electron Fermi surface similar to the metallic rare earth hexaborides such as PrB6 and LaB6. The quantum oscillation amplitude strongly increases at low temperatures, appearing strikingly at variance with conventional metallic behavior. C1 [Tan, B. S.; Hsu, Y. -T.; Hartstein, M.; Kiourlappou, M.; Srivastava, A.; Lonzarich, G. G.; Sebastian, Suchitra E.] Univ Cambridge, Cavendish Lab, Cambridge CB3 OHE, England. [Zeng, B.; Murphy, T. P.; Park, J. -H.; Balicas, L.] Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. [Hatnean, M. Ciomaga; Balakrishnan, G.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Harrison, N.; Zhu, Z.] Los Alamos Natl Lab, Natl High Magnet Field Lab, Los Alamos, NM 87504 USA. [Johannes, M. D.] Naval Res Lab, Ctr Computat Mat Sci, Washington, DC 20375 USA. RP Sebastian, SE (reprint author), Univ Cambridge, Cavendish Lab, JJ Thomson Ave, Cambridge CB3 OHE, England. EM suchitra@phy.cam.ac.uk RI Balakrishnan, Geetha/P-5977-2016; OI Balakrishnan, Geetha/0000-0002-5890-1149; Harrison, Neil/0000-0001-5456-7756 FU Royal Society; Winton Programme for the Physics of Sustainability; European Research Council (ERC) under the European Union [337425]; U.S. Department of Energy (DOE)-Basic Energy Sciences (BES) [DE-SC0002613]; Engineering and Physical Sciences Research Council (EPSRC) [EP/L014963/1]; DOE Office of Science, BES-Materials Science and Engineering "Science of 100 Tesla" program; Office of Naval Research (ONR) through the Naval Research Laboratory's Basic Research Program; EPSRC [EP/K012894/1]; NSF [DMR-1157490]; state of Florida FX B.S.T., Y.-T.H., M.H., M.K., A.S., and S.E.S. acknowledge support from the Royal Society, the Winton Programme for the Physics of Sustainability, and the European Research Council (ERC) under the European Union's Seventh Framework Programme (grant FP/2007-2013)/ERC Grant Agreement 337425. B.Z. and L.B. acknowledge support from the U.S. Department of Energy (DOE)-Basic Energy Sciences (BES) through award DE-SC0002613. M.C.H. and G.B. acknowledge support from Engineering and Physical Sciences Research Council (EPSRC) grant EP/L014963/1. N.H. and Z.Z. acknowledge support from the DOE Office of Science, BES-Materials Science and Engineering "Science of 100 Tesla" program. M.D.J. acknowledges support for this project by the Office of Naval Research (ONR) through the Naval Research Laboratory's Basic Research Program. G.G.L. acknowledges support from EPSRC grant EP/K012894/1. A portion of this work was performed at the National High Magnetic Field Laboratory, which is supported by NSF Cooperative Agreement DMR-1157490 and the state of Florida. We acknowledge valuable inputs from G. Baskaran, D. Benkert, A. K. Cheetham, D. Chowdhury, P. Coleman, N. R. Cooper, M. P. M. Dean, O. Ertem, J. Flouquet, R. H. Friend, R. Golombok, C. Harris, S. A. Hartnoll, T. Kasuya, G. Khaliullin, E.-A. Kim, J. Knolle, P. A. Lee, P. B. Littlewood, C. Liu, K. Miyake, J. E. Moore, O. Petrenko, S. Sachdev, A. Shekhter, N. Shitsevalova, Q. Si, A. Thomson, S. Todadri, C. M. Varma, and J. Zaanen. We thank magnet laboratory personnel, including J. Billings, R. Carrier, E. S. Choi, B. L. Dalton, D. Freeman, L. J. Gordon, M. Hicks, C. H. Mielke, J. M. Petty, and J. N. Piotrowski, for their assistance. Data will be made available at the institutional data repository www.data.cam.ac.uk/data-repository. NR 49 TC 31 Z9 31 U1 15 U2 82 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JUL 17 PY 2015 VL 349 IS 6245 SI SI BP 287 EP 290 DI 10.1126/science.aaa7974 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CN1ZB UT WOS:000358218600046 PM 26138105 ER PT J AU Park, J Elmlund, H Ercius, P Yuk, JM Limmer, DT Chen, Q Kim, K Han, SH Weitz, DA Zettl, A Alivisatos, AP AF Park, Jungwon Elmlund, Hans Ercius, Peter Yuk, Jong Min Limmer, David T. Chen, Qian Kim, Kwanpyo Han, Sang Hoon Weitz, David A. Zettl, A. Alivisatos, A. Paul TI 3D structure of individual nanocrystals in solution by electron microscopy SO SCIENCE LA English DT Article ID GOLD NANOPARTICLES; ATOMIC-RESOLUTION; GROWTH; TOMOGRAPHY; CELL; CONTRAST AB Knowledge about the synthesis, growth mechanisms, and physical properties of colloidal nanoparticles has been limited by technical impediments. We introduce a method for determining three-dimensional (3D) structures of individual nanoparticles in solution. We combine a graphene liquid cell, high-resolution transmission electron microscopy, a direct electron detector, and an algorithm for single-particle 3D reconstruction originally developed for analysis of biological molecules. This method yielded two 3D structures of individual platinum nanocrystals at near-atomic resolution. Because our method derives the 3D structure from images of individual nanoparticles rotating freely in solution, it enables the analysis of heterogeneous populations of potentially unordered nanoparticles that are synthesized in solution, thereby providing a means to understand the structure and stability of defects at the nanoscale. C1 [Park, Jungwon; Chen, Qian; Alivisatos, A. Paul] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Park, Jungwon; Weitz, David A.] Harvard Univ, Dept Appl Phys, Cambridge, MA 02138 USA. [Park, Jungwon; Weitz, David A.] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. [Elmlund, Hans] Monash Univ, Sch Biomed Sci, Dept Biochem & Mol Biol, Clayton, Vic 3800, Australia. [Elmlund, Hans] ARC Ctr Excellence Adv Mol Imaging, Clayton, Vic 3800, Australia. [Ercius, Peter] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Yuk, Jong Min; Zettl, A.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Yuk, Jong Min; Chen, Qian; Zettl, A.; Alivisatos, A. Paul] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Yuk, Jong Min; Zettl, A.; Alivisatos, A. Paul] Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. [Limmer, David T.] Princeton Univ, Princeton Ctr Theoret Sci, Princeton, NJ 08540 USA. [Chen, Qian] Univ Calif Berkeley, Miller Inst Basic Res Sci, Berkeley, CA 93720 USA. [Kim, Kwanpyo] Ulsan Natl Inst Sci & Technol, Dept Phys, Ulsan 689798, South Korea. [Han, Sang Hoon] Amore Pacific Co, R&D Ctr, Yongin 446829, South Korea. RP Alivisatos, AP (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM alivis@berkeley.edu RI Zettl, Alex/O-4925-2016; Kim, Kwanpyo/D-9121-2011; Alivisatos , Paul /N-8863-2015; Yuk, Jong Min/I-8770-2016; Park, Jungwon/O-1153-2016 OI Zettl, Alex/0000-0001-6330-136X; Kim, Kwanpyo/0000-0001-8497-2330; Alivisatos , Paul /0000-0001-6895-9048; Yuk, Jong Min/0000-0002-4677-7363; Park, Jungwon/0000-0003-2927-4331 FU Physical Chemistry of Inorganic Nanostructures Program [KC3103]; Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy (DOE) [DE-AC02-05CH11231]; NSF [DMR-1310266, DMR-1206512]; Harvard Materials Research Science and Engineering Center [DMR-1420570]; Amore Pacific; Multimodal Australian Sciences Imaging and Visualization Environment; Monash University; DOE Office of Energy Research, Basic Energy Sciences, Materials Sciences and Engineering Division [DE-AC02-05CH11231]; Molecular Foundry; Office of Naval Research [N00014-12-1]; Defense Threat Reduction Agency [HDTRA1-13-1-0035]; Princeton Center for Theoretical Science; Miller Institute for Basic Research in Science at UC Berkeley; National Research Foundation of Korea - Ministry of Education [NRF-2014R1A1A2058178]; DOE [DE-AC02-05CH11231] FX Supported by the Physical Chemistry of Inorganic Nanostructures Program (KC3103), Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy (DOE) under contract DE-AC02-05CH11231 (J.P. and A.P.A.); NSF grant DMR-1310266, Harvard Materials Research Science and Engineering Center grant DMR-1420570, and Amore Pacific (J.P., S.H.H., and D.A.W.); the Multimodal Australian Sciences Imaging and Visualization Environment (www.massive.org.au) and funds from Monash University (H.E.); the DOE Office of Energy Research, Basic Energy Sciences, Materials Sciences and Engineering Division under contract DE-AC02-05CH11231 within the SP2-Bonded Materials Program and the Molecular Foundry (construction of GLC and TEM characterization), Office of Naval Research grant N00014-12-1 (graphene growth), NSF grant DMR-1206512 (graphene transfer methods development), and postdoctoral support from Defense Threat Reduction Agency grant HDTRA1-13-1-0035 (J.M.Y., K.K., and A.Z.); the Princeton Center for Theoretical Science (D.T.L.); a Miller fellowship from Miller Institute for Basic Research in Science at UC Berkeley (Q.C.); and the Basic Science Research Program through the National Research Foundation of Korea funded by Ministry of Education grant NRF-2014R1A1A2058178 (K.K.). Electron microscopy was performed at the Molecular Foundry supported by DOE contract DE-AC02-05CH11231. NR 28 TC 41 Z9 42 U1 33 U2 201 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JUL 17 PY 2015 VL 349 IS 6245 SI SI BP 290 EP 295 DI 10.1126/science.aab1343 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CN1ZB UT WOS:000358218600047 PM 26185247 ER PT J AU Shi, NN Tsai, CC Camino, F Bernard, GD Yu, NF Wehner, R AF Shi, Norman Nan Tsai, Cheng-Chia Camino, Fernando Bernard, Gary D. Yu, Nanfang Wehner, Ruediger TI Keeping cool: Enhanced optical reflection and radiative heat dissipation in Saharan silver ants SO SCIENCE LA English DT Article ID REFRACTIVE-INDEX; DESERT; FILMS AB Saharan silver ants, Cataglyphis bombycina, forage under extreme temperature conditions in the African desert. We show that the ants' conspicuous silvery appearance is created by a dense array of triangular hairs with two thermoregulatory effects. They enhance not only the reflectivity of the ant's body surface in the visible and near-infrared range of the spectrum, where solar radiation culminates, but also the emissivity of the ant in the mid-infrared. The latter effect enables the animals to efficiently dissipate heat back to the surroundings via blackbody radiation under full daylight conditions. This biological solution for a thermoregulatory problem may lead to the development of biomimetic coatings for passive radiative cooling of objects. C1 [Shi, Norman Nan; Tsai, Cheng-Chia; Yu, Nanfang] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. [Camino, Fernando] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Bernard, Gary D.] Univ Washington, Dept Elect Engn, Seattle, WA 98195 USA. [Wehner, Ruediger] Univ Zurich, Brain Res Inst, Zurich, Switzerland. RP Yu, NF (reprint author), Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. EM ny2214@columbia.edu; rwehner@zool.uzh.ch FU NSF [PHY-1411445, ECCS-1307948]; Air Force Office of Scientific Research, Multidisciplinary University Research Initiative program [FA9550-14-1-0389]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0012704] FX We acknowledge intriguing discussions with N. Pierce; help with experiments from Z. Li, M.-H. Kim, B. Patterson, and M. Y. Sfeir; and R. F. Foelix for kindly preparing and providing Fig. 1B. The work was supported by NSF (grants PHY-1411445 and ECCS-1307948) and the Air Force Office of Scientific Research, Multidisciplinary University Research Initiative program (grant FA9550-14-1-0389). Research was carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under contract no. DE-SC0012704. Data reported in this paper are archived at http://datadryad.org/resource/doi:10.5061/dryad.2bm50. Author contributions are as follows: R.W. and G.D.B. initiated the study, N.N.S., C.-C. Tsai, and N. Y. designed the study and conducted the analyses, and all authors contributed to developing the study and to drafting the manuscript. NR 17 TC 21 Z9 21 U1 32 U2 121 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JUL 17 PY 2015 VL 349 IS 6245 SI SI BP 298 EP 301 DI 10.1126/science.aab3564 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CN1ZB UT WOS:000358218600049 PM 26089358 ER PT J AU Li, H Wang, XG Liang, C Hao, ZQ Zhou, LS Ma, S Li, XB Yang, S Yao, F Jiang, Y AF Li, Hui Wang, Xugao Liang, Chao Hao, Zhanqing Zhou, Lisha Ma, Sam Li, Xiaobin Yang, Shan Yao, Fei Jiang, Yong TI Aboveground-belowground biodiversity linkages differ in early and late successional temperate forests SO SCIENTIFIC REPORTS LA English DT Article ID COMMUNITY STRUCTURE; PLANT DIVERSITY; RIBOSOMAL-RNA; TERRESTRIAL ECOSYSTEMS; MICROBIAL COMMUNITIES; SOIL MICROBES; PRODUCTIVITY; MECHANISMS; GRASSLANDS; FEEDBACKS AB Understanding ecological linkages between above-and below-ground biota is critical for deepening our knowledge on the maintenance and stability of ecosystem processes. Nevertheless, direct comparisons of plant-microbe diversity at the community level remain scarce due to the knowledge gap between microbial ecology and plant ecology. We compared the alpha-and beta-diversities of plant and soil bacterial communities in two temperate forests that represented early and late successional stages. We documented different patterns of aboveground-belowground diversity relationships in these forests. We observed no linkage between plant and bacterial alpha-diversity in the early successional forest, and even a negative correlation in the late successional forest, indicating that high bacterial beta-diversity is not always linked to high plant alpha-diversity. Beta-diversity coupling was only found at the late successional stage, while in the early successional forest, the bacterial beta-diversity was closely correlated with soil property distances. Additionally, we showed that the dominant competitive tree species in the late successional forest may play key roles in driving forest succession by shaping the soil bacterial community in the early successional stage. This study sheds new light on the potential aboveground-belowground linkage in natural ecosystems, which may help us understand the mechanisms that drive ecosystem succession. C1 [Li, Hui; Wang, Xugao; Liang, Chao; Hao, Zhanqing; Zhou, Lisha; Li, Xiaobin; Yang, Shan; Yao, Fei; Jiang, Yong] Chinese Acad Sci, Inst Appl Ecol, State Key Lab Forest & Soil Ecol, Shenyang 110164, Peoples R China. [Liang, Chao] Univ Wisconsin, Great Lakes Bioenergy Res Ctr, Madison, WI 53706 USA. [Ma, Sam] Chinese Acad Sci, Kunming Inst Zool, Computat Biol & Med Ecol Lab, State Key Lab Genet Resources & Evolut, Kunming 650223, Peoples R China. RP Jiang, Y (reprint author), Chinese Acad Sci, Inst Appl Ecol, State Key Lab Forest & Soil Ecol, Shenyang 110164, Peoples R China. EM jiangyong@iae.ac.cn RI Jiang, Yong/A-2263-2012; wang, xugao/B-1111-2015 OI Jiang, Yong/0000-0001-7518-5810; wang, xugao/0000-0003-1207-8852 FU Strategic Priority Research Program of the Chinese Academy of Sciences [XDB15010300]; National Basic Research Program of China [2011CB403204]; State Key Laboratory of Forest and Soil Ecology, Chinese Academy of Sciences [LFSE2013-14]; National Natural Science Foundation of China [41471218, 41371076] FX This work was supported by the Strategic Priority Research Program of the Chinese Academy of Sciences (XDB15010300), the National Basic Research Program of China (2011CB403204), the State Key Laboratory of Forest and Soil Ecology, Chinese Academy of Sciences (Grant No. LFSE2013-14) and the National Natural Science Foundation of China (41471218 and 41371076). We thank our field crew from the Changbai Mountain National Station of Forest Ecosystem Observation and Research for their help collecting the soil cores; Dr. Matthew Lee Settles and Dr. Suresh Iyer from Institute for Bioinformatics and Evolutionary Studies (IBEST), University of Idaho, USA for technical assistance with 454 pyrosequencing analysis; Dr. Dandan Ye from Kunming Institute of Zoology, Chinese Academy of Sciences for assistance with bioinformatics analysis; Dr. Ye Deng from Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences for helpful discussions. NR 35 TC 4 Z9 4 U1 28 U2 89 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUL 17 PY 2015 VL 5 AR 12234 DI 10.1038/srep12234 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CM9OW UT WOS:000358039400001 PM 26184121 ER PT J AU Mazur, A De Meyer, SE Tian, R Wielbo, J Zebracki, K Seshadri, R Reddy, TBK Markowitz, V Ivanova, NN Pati, A Woyke, T Kyrpides, NC Reeve, W AF Mazur, Andrzej De Meyer, Sofie E. Tian, Rui Wielbo, Jerzy Zebracki, Kamil Seshadri, Rekha Reddy, T. B. K. Markowitz, Victor Ivanova, Natalia N. Pati, Amrita Woyke, Tanja Kyrpides, Nikos C. Reeve, Wayne TI High-quality permanent draft genome sequence of Rhizobium leguminosarum bv. viciae strain GB30; an effective microsymbiont of Pisum sativum growing in Poland SO STANDARDS IN GENOMIC SCIENCES LA English DT Article DE Root-nodule bacteria; Nitrogen fixation; Rhizobia; Alphaproteobacteria; GEBA-RNB ID MICROBIAL GENOMES; SP-NOV; TRIFOLII; SYSTEM; REVISION; DATABASE; NODULES AB Rhizobium leguminosarum bv. viciae GB30 is an aerobic, motile, Gram-negative, non-spore-forming rod that can exist as a soil saprophyte or as a legume microsymbiont of Pisum sativum. GB30 was isolated in Poland from a nodule recovered from the roots of Pisum sativum growing at Janow. GB30 is also an effective microsymbiont of the annual forage legumes vetch and pea. Here we describe the features of R. leguminosarum bv. viciae strain GB30, together with sequence and annotation. The 7,468,464 bp high-quality permanent draft genome is arranged in 78 scaffolds of 78 contigs containing 7,227 protein-coding genes and 75 RNA-only encoding genes, and is part of the GEBA-RNB project proposal. C1 [Mazur, Andrzej; Wielbo, Jerzy; Zebracki, Kamil] Marie Curie Sklodowska Univ, Dept Genet & Microbiol, Lublin, Poland. [De Meyer, Sofie E.; Tian, Rui; Reeve, Wayne] Murdoch Univ, Ctr Rhizobium Studies, Murdoch, WA 6150, Australia. [Seshadri, Rekha; Reddy, T. B. K.; Ivanova, Natalia N.; Pati, Amrita; Woyke, Tanja; Kyrpides, Nikos C.] DOE Joint Genome Inst, Walnut Creek, CA USA. [Markowitz, Victor] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Data Management & Technol Ctr, Berkeley, CA 94720 USA. [Kyrpides, Nikos C.] King Abdulaziz Univ, Dept Biol Sci, Jeddah 21413, Saudi Arabia. RP Reeve, W (reprint author), Murdoch Univ, Ctr Rhizobium Studies, Murdoch, WA 6150, Australia. EM W.Reeve@murdoch.edu.au RI Kyrpides, Nikos/A-6305-2014; Fac Sci, KAU, Biol Sci Dept/L-4228-2013; OI Kyrpides, Nikos/0000-0002-6131-0462; Ivanova, Natalia/0000-0002-5802-9485 FU US Department of Energy's Office of Science, Biological and Environmental Research Program; University of California, Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Los Alamos National Laboratory [DE-AC02-06NA25396] FX This work was performed under the auspices of the US Department of Energy's Office of Science, Biological and Environmental Research Program, and by the University of California, Lawrence Berkeley National Laboratory under contract No. DE-AC02-05CH11231, Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344, and Los Alamos National Laboratory under contract No. DE-AC02-06NA25396. NR 45 TC 1 Z9 1 U1 1 U2 3 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD JUL 16 PY 2015 VL 10 AR 36 DI 10.1186/s40793-015-0029-6 PG 7 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DA7MT UT WOS:000367989100001 PM 26221417 ER PT J AU Zhao, WX Vaithiyalingam, S Filippo, JS Maranon, DG Jimenez-Sainz, J Fontenay, GV Kwon, Y Leung, SG Lu, L Jensen, RB Chazin, WJ Wiese, C Sung, P AF Zhao, Weixing Vaithiyalingam, Sivaraja Filippo, Joseph San Maranon, David G. Jimenez-Sainz, Judit Fontenay, Gerald V. Kwon, Youngho Leung, Stanley G. Lu, Lucy Jensen, Ryan B. Chazin, Walter J. Wiese, Claudia Sung, Patrick TI Promotion of BRCA2-Dependent Homologous Recombination by DSS1 via RPA Targeting and DNA Mimicry SO MOLECULAR CELL LA English DT Article ID SUSCEPTIBILITY GENE BRCA2; STRAND-BREAK REPAIR; RAD51 FILAMENT FORMATION; USTILAGO-MAYDIS; ARABIDOPSIS-THALIANA; FOOT MALFORMATION; MEDIATOR FUNCTION; GENOME STABILITY; DAMAGE RESPONSE; PROTEIN AB The tumor suppressor BRCA2 is thought to facilitate the handoff of ssDNA from replication protein A (RPA) to the RAD51 recombinase during DNA break and replication fork repair by homologous recombination. However, we find that RPA-RAD51 exchange requires the BRCA2 partner DSS1. Biochemical, structural, and in vivo analyses reveal that DSS1 allows the BRCA2-DSS1 complex to physically and functionally interact with RPA. Mechanistically, DSS1 acts as a DNA mimic to attenuate the affinity of RPA for ssDNA. A mutation in the solvent-exposed acidic domain of DSS1 compromises the efficacy of RPA-RAD51 exchange. Thus, by targeting RPA and mimicking DNA, DSS1 functions with BRCA2 in a two-component homologous recombination mediator complex in genome maintenance and tumor suppression. Our findings may provide a paradigm for understanding the roles of DSS1 in other biological processes. C1 [Zhao, Weixing; Filippo, Joseph San; Kwon, Youngho; Lu, Lucy; Sung, Patrick] Yale Univ, Dept Mol Biophys & Biochem, Sch Med, New Haven, CT 06520 USA. [Vaithiyalingam, Sivaraja; Chazin, Walter J.] Vanderbilt Univ, Dept Biochem, Nashville, TN 37232 USA. [Vaithiyalingam, Sivaraja; Chazin, Walter J.] Vanderbilt Univ, Dept Chem, Nashville, TN 37232 USA. [Vaithiyalingam, Sivaraja; Chazin, Walter J.] Vanderbilt Univ, Struct Biol Ctr, Nashville, TN 37232 USA. [Maranon, David G.; Wiese, Claudia] Colorado State Univ, Dept Environm & Radiol Hlth Sci, Ft Collins, CO 80523 USA. [Jimenez-Sainz, Judit; Jensen, Ryan B.] Yale Univ, Dept Therapeut Radiol, Sch Med, New Haven, CT 06520 USA. [Fontenay, Gerald V.; Leung, Stanley G.; Wiese, Claudia] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. RP Chazin, WJ (reprint author), Vanderbilt Univ, Dept Biochem, Nashville, TN 37232 USA. EM walter.chazin@vanderbilt.edu; patrick.sung@yale.edu FU US National Institutes of Health [ES015252, ES007061, CA168635, CA92584, ES021454, GM65484]; NSF [0922862]; NIH [S10 RR025677]; Vanderbilt University FX We thank Stephen Kowalczykowski for the phCMV1-BRCA2 vector and Alan Ashworth for the pEGFP-DSS1 vector. This work was supported by US National Institutes of Health grants ES015252, ES007061, CA168635, CA92584, ES021454, and GM65484. Access to facilities was supported by P30 ES00267 and P30 CA068485. NMR instrumentation was supported by grants from the NSF (0922862), NIH (S10 RR025677), and Vanderbilt University matching funds. NR 61 TC 13 Z9 13 U1 1 U2 17 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 1097-2765 EI 1097-4164 J9 MOL CELL JI Mol. Cell PD JUL 16 PY 2015 VL 59 IS 2 BP 176 EP 187 DI 10.1016/j.molcel.2015.05.032 PG 12 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA CT0AV UT WOS:000362457000007 PM 26145171 ER PT J AU Hamada, Y Grippo, MA AF Hamada, Yuki Grippo, Mark A. TI Remote-sensing application for facilitating land resource assessment and monitoring for utility-scale solar energy development (vol 9, 097694, 2015) SO JOURNAL OF APPLIED REMOTE SENSING LA English DT Correction C1 [Hamada, Yuki; Grippo, Mark A.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Hamada, Y (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. NR 1 TC 0 Z9 0 U1 1 U2 1 PU SPIE-SOC PHOTO-OPTICAL INSTRUMENTATION ENGINEERS PI BELLINGHAM PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98225 USA SN 1931-3195 J9 J APPL REMOTE SENS JI J. Appl. Remote Sens. PD JUL 16 PY 2015 VL 9 AR 099998 DI 10.1117/1.JRS.9.099998 PG 1 WC Environmental Sciences; Remote Sensing; Imaging Science & Photographic Technology SC Environmental Sciences & Ecology; Remote Sensing; Imaging Science & Photographic Technology GA CP3SJ UT WOS:000359801600001 ER PT J AU Klippenstein, SJ Pratt, ST AF Klippenstein, Stephen J. Pratt, Stephen T. TI A Tribute to Lawrence B. Harding, Joe V. Michael, and Albert F. Wagner for Their 100 Years of Combustion Kinetics Studies at Argonne SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Biographical-Item C1 [Klippenstein, Stephen J.; Pratt, Stephen T.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Klippenstein, SJ (reprint author), Argonne Natl Lab, Argonne, IL 60439 USA. NR 1 TC 0 Z9 0 U1 0 U2 0 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7075 EP + PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600002 ER PT J AU Klippenstein, SJ Pratt, ST AF Klippenstein, Stephen J. Pratt, Stephen T. TI A Tribute to Lawrence B. Harding, Joe V. Michael, and Albert F. Wagner for Their 100 Years of Combustion Kinetics Studies at Argonne SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Biographical-Item C1 [Klippenstein, Stephen J.; Pratt, Stephen T.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Klippenstein, SJ (reprint author), Argonne Natl Lab, Argonne, IL 60439 USA. OI Klippenstein, Stephen/0000-0001-6297-9187 NR 1 TC 0 Z9 0 U1 3 U2 3 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7075 EP + DI 10.1021/acs.jpca.5b01917 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600001 ER PT J AU Klippenstein, SJ Pratt, ST AF Klippenstein, Stephen J. Pratt, Stephen T. TI A Tribute to Lawrence B. Harding, Joe V. Michael, and Albert F. Wagner for Their 100 Years of Combustion Kinetics Studies at Argonne SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Biographical-Item C1 [Klippenstein, Stephen J.; Pratt, Stephen T.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Klippenstein, SJ (reprint author), Argonne Natl Lab, Argonne, IL 60439 USA. NR 1 TC 0 Z9 0 U1 1 U2 2 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7075 EP + PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600003 ER PT J AU Burke, MP Goldsmith, CF Klippenstein, SJ Welz, O Huang, HF Antonov, IO Savee, JD Osborn, DL Zador, J Taatjes, CA Shepsll, L AF Burke, Michael P. Goldsmith, C. Franklin Klippenstein, Stephen J. Welz, Oliver Huang, Haifeng Antonov, Ivan O. Savee, John D. Osborn, David L. Zador, Judit Taatjes, Craig A. Shepsll, Leonid TI Multiscale Informatics for Low-Temperature Propane Oxidation: Further Complexities in Studies of Complex Reactions SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID PHENOMENOLOGICAL RATE COEFFICIENTS; DETAILED KINETIC-MODEL; PLUS O-2 REACTIONS; MASTER-EQUATION; UNCERTAINTY QUANTIFICATION; ARRHENIUS PARAMETERS; SENSITIVITY-ANALYSIS; 2-STAGE IGNITION; PROPYL RADICALS; GAS-PHASE AB The present paper describes further development of the multiscale informatics approach to kinetic model formulation of Burke et al. (Burke, M. P.; Klippenstein, S. J.; Harding, L. B. Proc. Combust. Inst. 2013, 34, 547-555) that directly incorporates elementary kinetic theories as a means to provide reliable, physics-based extrapolation of kinetic models to unexplored conditions. Here, we extend and generalize the multiscale informatics strategy to treat systems of considerable complexity-involving multiwell reactions, potentially missing reactions, nonstatistical product branching ratios, and non-Boltzmann (i.e., nonthermal) reactant distributions. The methodology is demonstrated here for a subsystem of low-temperature propane oxidation, as a representative system for low-temperature fuel oxidation. A multiscale model is assembled and informed by a wide variety of targets that include ab initio calculations of molecular properties, rate constant measurements of isolated reactions, and complex systems measurements. Active model parameters are chosen to accommodate both "parametric" and "structural" uncertainties. Theoretical parameters (e.g., barrier heights) are included as active model parameters to account for parametric uncertainties in the theoretical treatment; experimental parameters (e.g., initial temperatures) are included to account for parametric uncertainties in the physical models of the experiments. RMG software is used to assess potential structural uncertainties due to missing reactions. Additionally, branching ratios among product channels are included as active model parameters to account for structural uncertainties related to difficulties in modeling sequences of multiple chemically activated steps. The approach is demonstrated here for interpreting time-resolved measurements of OH, HO2, n-propyl, i-propyl, propene, oxetane, and methyloxirane from photolysis-initiated low-temperature oxidation of propane at pressures from 4 to 60 Torr and temperatures from 300 to 700 K. In particular, the multiscale informed model provides a consistent quantitative explanation of both ab initio calculations and time-resolved species measurements. The present results show that interpretations of OH measurements are significantly more complicated than previously thought-in addition to barrier heights for key transition states considered previously, OH profiles also depend on additional theoretical parameters for R + O-2 reactions, secondary reactions, QOOH + O-2 reactions, and treatment of non-Boltzmann reaction sequences. Extraction of physically rigorous information from those measurements may require more sophisticated treatment of all of those model aspects, as well as additional experimental data under more conditions, to discriminate among possible interpretations and ensure model reliability. C1 [Burke, Michael P.] Columbia Univ, Dept Mech Engn, Dept Chem Engn, New York, NY 10027 USA. [Burke, Michael P.] Columbia Univ, Data Sci Inst, New York, NY 10027 USA. [Burke, Michael P.; Goldsmith, C. Franklin; Klippenstein, Stephen J.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Goldsmith, C. Franklin] Brown Univ, Sch Engn, Providence, RI 02912 USA. [Welz, Oliver; Huang, Haifeng; Antonov, Ivan O.; Savee, John D.; Osborn, David L.; Zador, Judit; Taatjes, Craig A.; Shepsll, Leonid] Sandia Natl Labs, Combust Res Facil, Livermore, CA USA. RP Burke, MP (reprint author), 500 West 120th St,228 Mudd Bldg,MC 4703, New York, NY 10027 USA. EM mpburke@columbia.edu RI Zador, Judit/A-7613-2008; OI Zador, Judit/0000-0002-9123-8238; Klippenstein, Stephen/0000-0001-6297-9187 FU Argonne National Lab; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, at Argonne, Argonne-Sandia Consortium on High-Pressure Combustion Chemistry [DE-AC02-06CH11357, 59044, 014544]; National Nuclear Security Administration [DE-AC04-94-AL85000] FX This work was supported by a Director's Postdoctoral Fellowship from Argonne National Lab and by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, under Contract No. DE-AC02-06CH11357 at Argonne as part of the Argonne-Sandia Consortium on High-Pressure Combustion Chemistry, (ANL FWP # 59044; SNL FWP # 014544). Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the National Nuclear Security Administration under contract DE-AC04-94-AL85000. NR 106 TC 5 Z9 5 U1 9 U2 49 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7095 EP 7115 DI 10.1021/acs.jpca.5b01003 PG 21 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600004 PM 25946172 ER PT J AU Welz, O Burke, MP Antonov, IO Goldsmith, CF Savee, JD Osborn, DL Taatjes, CA Klippenstein, SJ Sheps, L AF Welz, Oliver Burke, Michael P. Antonov, Ivan O. Goldsmith, C. Franklin Savee, John D. Osborn, David L. Taatjes, Craig A. Klippenstein, Stephen J. Sheps, Leonid TI New Insights into Low-Temperature Oxidation of Propane from Synchrotron Photoionization Mass Spectrometry and Multiscale Informatics Modeling SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID SLOWLY REACTING MIXTURES; PLUS O-2 REACTIONS; 480 DEGREES-C; COMBUSTION CHEMISTRY; N-BUTANE; AUTOIGNITION CHEMISTRY; PRODUCT FORMATION; PROPYL RADICALS; ALKYLPEROXY RADICALS; CHEMICAL-KINETICS AB Low-temperature propane oxidation was studied at P = 4 Torr and T = 530, 600, and 670 K by time-resolved multiplexed photoionization mass spectrometry (MPIMS), which probes the reactants, intermediates, and products with isomeric selectivity using tunable synchrotron vacuum UV ionizing radiation. The oxidation is initiated by pulsed laser photolysis of oxalyl chloride, (COCl)(2), at 248 nm, which rapidly generates a similar to 1:1 mixture of 1-propyl (n-propyl) and 2-propyl (i-propyl) radicals via the fast Cl + propane reaction. At all three temperatures, the major stable product species is propene, formed in the propyl + O-2 reactions by direct HO2 elimination from both n- and i-propyl peroxy radicals. The experimentally derived propene yields relative to the initial concentration of Cl atoms are (20 +/- 4)% at 530 K, (55 +/- 11)% at 600 K, and (86 +/- 17)% at 670 K at a reaction time of 20 ms. The lower yield of propene at low temperature reflects substantial formation of propyl peroxy radicals, which do not completely decompose on the experimental time scale. In addition, C3H6O isomers methyloxirane, oxetane, acetone, and propanal are detected as minor products. Our measured yields of oxetane and methyloxirane, which are coproducts of OH radicals, suggest a revision of the OH formation pathways in models of low-temperature propane oxidation. The experimental results are modeled and interpreted using a multiscale informatics approach, presented in detail in a separate publication (Burke, M. P.; Goldsmith, C. F.; Klippenstein, S. J.; Welz, O.; Huang H.; Antonov I. O.; Savee J. D.; Osborn D. L.; Zador, J.; Taatjes, C. A.; Sheps, L. Multiscale Informatics for Low-Temperature Propane Oxidation: Further Complexities in Studies of Complex Reactions. J. Phys. Chem A. 2015, DOI: 10.1021/acs.jpca.5b01003). The model predicts the time profiles and yields of the experimentally observed primary products well, and shows satisfactory agreement for products formed mostly via secondary radical-radical reactions. C1 [Welz, Oliver; Antonov, Ivan O.; Savee, John D.; Osborn, David L.; Taatjes, Craig A.; Sheps, Leonid] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. [Burke, Michael P.; Goldsmith, C. Franklin; Klippenstein, Stephen J.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60493 USA. [Burke, Michael P.] Columbia Univ, Dept Chem Engn, Dept Mech Engn, New York, NY 10027 USA. [Burke, Michael P.] Columbia Univ, Data Sci Inst, New York, NY 10027 USA. RP Welz, O (reprint author), Univ Duisburg Essen, Inst Combust & Gas Dynam, Duisburg, Germany. EM oliver.welz@uni-due.de; lsheps@sandia.gov OI Klippenstein, Stephen/0000-0001-6297-9187 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; National Nuclear Security Administration [DE-AC04-94AL85000]; Argonne National Lab; Office of Science, BES/DOE [DE-AC02-05CH11231]; [DE-AC02-06CH11357] FX We thank Mr. Howard Johnsen (Sandia) and the staff at the Chemical Dynamics Beamline at the ALS for excellent technical support of these experiments. This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences. The work at Argonne National Laboratory was supported under contract DE-AC02-06CH11357. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the National Nuclear Security Administration, under contract DE-AC04-94AL85000. The work of O.W., M.P.B., C.F.G., SJ.K., C.A.T., and L.S. was part of the Argonne-Sandia Consortium on High-Pressure Combustion Chemistry. M.P.B. and C.F.G. were also supported by Director's Postdoctoral Fellowships from Argonne National Lab. The Advanced Light Source is supported by the Director, Office of Science, BES/DOE, under contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the DOE. NR 60 TC 4 Z9 4 U1 12 U2 53 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7116 EP 7129 DI 10.1021/acs.jpca.5b01008 PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600005 PM 25860187 ER PT J AU Parker, DSN Kaiser, RI Troy, TP Kostko, O Ahmed, M Mebel, AM AF Parker, Dorian S. N. Kaiser, Ralf I. Troy, Tyler P. Kostko, Oleg Ahmed, Musahid Mebel, Alexander M. TI Toward the Oxidation of the Phenyl Radical and Prevention of PAH Formation in Combustion Systems SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID SINGLE-COLLISION CONDITIONS; POLYCYCLIC AROMATIC-HYDROCARBONS; MOLECULAR-OXYGEN O-2; VUV PHOTOIONIZATION; UNIMOLECULAR DECOMPOSITION; THERMAL-DECOMPOSITION; AB-INITIO; C6H5; MECHANISM; BENZENE AB The reaction of the phenyl radical (C6H5) with molecular oxygen (O-2) plays a central role in the degradation of poly- and monocyclic aromatic radicals in combustion systems which would otherwise react with fuel components to form polycyclic aromatic hydrocarbons (PAHs) and eventually soot. Despite intense theoretical and experimental scrutiny over half a century, the overall reaction channels have not all been experimentally identified. Tunable vacuum ultraviolet photoionization in conjunction with a combustion simulating chemical reactor uniquely provides the complete isomer specific product spectrum and branching ratios of this prototype reaction. In the reaction of phenyl radicals and molecular oxygen at 873 K and 1003 K, ortho-benzoquinone (o-C6H4O2), the phenoxy radical (C6H5O), and cyclopentadienyl radical (C5H5) were identified as primary products formed through emission of atomic hydrogen, atomic oxygen and carbon dioxide. Furan (C4H4O), acrolein (C3H4O), and ketene (C2H2O) were also identified as primary products formed through ring opening and fragmentation of the 7-membered ring 2-oxepinoxy radical. Secondary reaction products para-benzoquinone (p-C6H4O2), phenol (C6H5OH), cyclopentadiene (C5H6), 2,4-cyclopentadienone (C5H4O), vinylacetylene (C4H4), and acetylene (C2H2) were also identified. The pyranyl radical (C5H5O) was not detected; however, electronic structure calculations show that it is formed and isomerizes to 2,4-cyclopentadienone through atomic hydrogen emission. In combustion systems, barrierless phenyl-type radical oxidation reactions could even degrade more complex aromatic radicals. An understanding of these elementary processes is expected to lead to a better understanding toward the elimination of carcinogenic, mutagenic, and environmentally hazardous byproducts of combustion systems such as PAHs. C1 [Parker, Dorian S. N.; Kaiser, Ralf I.] Univ Hawaii Manoa, Dept Chem, Honolulu, HI 96822 USA. [Troy, Tyler P.; Kostko, Oleg; Ahmed, Musahid] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Mebel, Alexander M.] Florida Int Univ, Dept Chem & Biochem, Miami, FL 33199 USA. RP Kaiser, RI (reprint author), Univ Hawaii Manoa, Dept Chem, Honolulu, HI 96822 USA. EM ralfk@hawaii.edu; MAhmed@lbl.gov; mebela@fiu.edu RI Kostko, Oleg/B-3822-2009; Mebel, Alexander/A-5234-2009; Ahmed, Musahid/A-8733-2009 OI Kostko, Oleg/0000-0003-2068-4991; FU U.S. Department of Energy, Office of Science [DE-FG02-03ER15411, DE-FG02-04ER15570]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy through Chemical Sciences Division [DE-AC02-05CH11231] FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, DE-FG02-03ER15411 to the University of Hawaii and DE-FG02-04ER15570 to FIU. The authors MA., O.K, and T.P.T, and the Advanced Light Source are supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract DE-AC02-05CH11231, through the Chemical Sciences Division. A.M.M. would like to acknowledge the Instructional & Research Computing Center (IRCC, web: http://ircc.fiu.edu) at FIU for providing HPC computing resources that have contributed to the research results reported within this paper. NR 40 TC 8 Z9 8 U1 7 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7145 EP 7154 DI 10.1021/jp509170x PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600008 PM 25354358 ER PT J AU Ormond, TK Scheer, AM Nimlos, MR Robichaud, DJ Troy, TP Ahmed, M Daily, JW Nguyen, TL Stanton, JF Ellison, GB AF Ormond, Thomas K. Scheer, Adam M. Nimlos, Mark R. Robichaud, David J. Troy, Tyler P. Ahmed, Musahid Daily, John W. Nguyen, Thanh Lam Stanton, John F. Ellison, G. Barney TI Pyrolysis of Cyclopentadienone: Mechanistic Insights from a Direct Measurement of Product Branching Ratios SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID INFRARED-ABSORPTION SPECTRA; AB-INITIO THERMOCHEMISTRY; PHOTOELECTRON-SPECTROSCOPY; THERMAL-DECOMPOSITION; PHOTOIONIZATION MASS; FLOW REACTOR; RADICALS; OXIDATION; COMBUSTION; MOLECULES AB The thermal decomposition of cyclopentadienone (C5H4=O) has been studied in a flash pyrolysis continuous flow microreactor. Passing dilute samples of o-phenylene sulfite (C6H4O2SO) in He through the microreactor at elevated temperatures yields a relatively dean source of C5H4=O. The pyrolysis of C5H4=O was investigated over the temperature range 1000-2000 K. Below 1600 K, we have identified two decomposition channels: (1) C5H4=0 (+ M) --> CO + HC=C-CH=CH2 and (2) C5H4=O (+ M) --> CO + HC=CH + HC=CH. There is no evidence of radical or H atom chain reactions. To establish the thermochemistry for the pyrolysis of cyclopentadienone, ab initio electronic structure calculations (AE-CCSD(T)/aug-cc-pCVQZ//AE-CCSD(T)/cc-pVQZ and anharmonic FC-CCSD(T)/ANO1 ZPEs) were used to find Delta H-f(0)(C5H4=O) to be 16 +/- 1 kcal mol(-1) and Delta H-f(0)(CE2=CH-C=CH) to be 71 +/- 1 kcal mol(-1). The calculations predict the reaction enthalpies Delta H-rxn(0)(1) to be 28 +/- 1 kcal mol(-1) (Delta H-rxn(298)(1) is 30 +/- kcal mol(-1)) and Delta H-rxn(0)(2) to be 66 +/- 1 kcal mol(-1) (Delta H-rxn(298)(2) is 69 +/- 1 kcal mol(-1)). Following pyrolysis of C5H4=0, photoionization mass spectrometry was used to measure the relative concentrations of HCC-CHCH2 and HCCH. Reaction 1 dominates at low pyrolysis temperatures (1000-1400 K). At temperatures above 1400 K, reaction 2 becomes the dominant channel. We have used the product branching ratios Over the temperature range 1000-1600 K to extract the ratios of unimolecular rate coefficients for reactions 1 and 2. If Arrhenius expressions are used, the difference of activation energies for reactions 1 and 2, E-2 - E-1, is found to be 16 +/- 1 kcal mol(-1) and the ratio of the pre-exponential factors, A(2)/A(1) is 7.0 +/- 0.3. C1 [Ormond, Thomas K.; Nimlos, Mark R.; Robichaud, David J.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Ormond, Thomas K.; Ellison, G. Barney] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. [Scheer, Adam M.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. [Troy, Tyler P.; Ahmed, Musahid] Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Daily, John W.] Univ Colorado, Ctr Combust & Environm Res, Dept Mech Engn, Boulder, CO 80309 USA. [Nguyen, Thanh Lam; Stanton, John F.] Univ Texas Austin, Inst Theoret Chem, Dept Chem, Austin, TX 78712 USA. RP Ormond, TK (reprint author), Natl Renewable Energy Lab, 15013 Denever West Pkway, Golden, CO 80401 USA. RI Ahmed, Musahid/A-8733-2009 FU National Science Foundation [CHE-0848606, CHE-1112466]; Robert A. Welch Foundation [F-1283]; United States Department of Energy, Basic Energy Sciences [DE-FG02-07ER15884]; United States Department of Energy's Bioenergy Technology Office [DE-AC36-99GO10337]; Office of Energy Research, Office of Basic Energy Sciences, and Chemical Sciences Division of the U.S. Department of Energy [DE-AC02-05CH11231] FX We would like to acknowledge support from the National Science Foundation (CHE-0848606 and CHE-1112466) for J.W.D, J.F.S., and G.B.E. J.F.S. also acknowledges support from the Robert A. Welch Foundation (Grant F-1283) and the United States Department of Energy, Basic Energy Sciences (DE-FG02-07ER15884). M.R.N. is supported by United States Department of Energy's Bioenergy Technology Office under Contract No. DE-AC36-99GO10337. M.A, T.P.T., and M.RN. and the Advanced Light Source are supported by the Director, Office of Energy Research, Office of Basic Energy Sciences, and Chemical Sciences Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 61 TC 7 Z9 7 U1 4 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7222 EP 7234 DI 10.1021/jp511390f PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600016 PM 25608038 ER PT J AU Jasper, AW AF Jasper, Ahren W. TI Multidimensional Effects in Nonadiabatic Statistical Theories of Spin-Forbidden Kinetics: A Case Study of O-3 + CO -> CO2 SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID TRANSITION-STATE-THEORY; BORN-OPPENHEIMER TRAJECTORIES; ACTIVATED ELECTRON-TRANSFER; FAST DIELECTRIC-RELAXATION; POTENTIAL-ENERGY SURFACES; CURVE CROSSING PROBLEMS; REACTION-RATE CONSTANTS; PHASE-SPACE THEORY; MOLECULAR-DYNAMICS; MONTE-CARLO AB The appropriateness of treating crossing seams of electronic states of different spins as nonadiabatic transition states in statistical Calculations of spin-forbidden reaction rates is considered. We show that the spin-forbidden reaction coordinate, the nuclear coordinate perpendicular to the crossing seam, is coupled to the remaining nuclear degrees of freedom. This coupling gives rise to multidimensional effects that are not typically included in statistical treatments of spin-forbidden kinetics. Three qualitative categories of multidimensional effects may be identified: static multidimensional effects due to the geometry-dependence of the local shape of the crossing seam and of the spin-orbit coupling, dynamical multidimensional effects due to energy exchange with the reaction coordinate during the seam crossing, and nonlocal (history-dependent) multidimensional effects due to interference of the electronic variables at second, third, and later seam crossings. Nonlocal multidimensional effects are intimately related to electronic decoherence, where electronic dephasing acts to erase the history of the system. A semiclassical model based on short-time full-dimensional trajectories that includes all three multidimensional effects as well as a model for electronic decoherence is presented. The results of this multidimensional nonadiabatic statistical theory (MNST) for the O-3 + CO -> CO2 reaction are compared with the results of statistical theories employing one-dimensional (Landau-Zener and weak coupling) models for the transition probability and with those calculated previously using multistate trajectories. The MNST method is shown to accurately reproduce the multistate decay-of-mixing trajectory results, so long as consistent thresholds are used. The MNST approach has several advantages over multistate trajectory approaches and is more suitable in chemical kinetics calculations at low temperatures and for complex systems. The error in statistical calculations that neglect multidimensional effects is shown to be as large as a factor of 2 for this system, with static multidimensional effects identified as the largest source of error. C1 Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. RP Jasper, AW (reprint author), Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. EM ajasper@sandia.gov RI Jasper, Ahren/A-5292-2011 FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy; United States Department of Energy [DE-AC04-94-AL85000]; AITSTME project as part of the Predictive Theory and Modeling component of the Materials Genome Initiative FX The author thanks F. M. Haas for many helpful discussions regarding the combustion relevance of this reaction. This work was supported by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy under contract no. DE-AC04-94-AL85000. Software development was supported by the AITSTME project as part of the Predictive Theory and Modeling component of the Materials Genome Initiative. NR 72 TC 9 Z9 9 U1 3 U2 10 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7339 EP 7351 DI 10.1021/jp512942w PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600028 PM 25871914 ER PT J AU Moshammer, K Jasper, AW Popolan-Vaida, DM Lucassen, A Dievarti, P Selim, H Eskola, AJ Taatjes, CA Leone, SR Sarathy, SM Ju, YG Dagaut, P Kohse-Hoinghaus, K Hansen, N AF Moshammer, Kai Jasper, Ahren W. Popolan-Vaida, Denisia M. Lucassen, Arnas Dievarti, Pascal Selim, Hatem Eskola, Arkke J. Taatjes, Craig A. Leone, Stephen R. Sarathy, S. Mani Ju, Yiguang Dagaut, Philippe Kohse-Hoeinghaus, Katharina Hansen, Nils TI Detection and Identification of the Keto-Hydroperoxide (HOOCH2OCHO) and Other Intermediates during Low-Temperature Oxidation of Dimethyl Ether SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID PHOTOIONIZATION MASS-SPECTROMETRY; FUEL-RICH FLAMES; NORMAL-HEXADECANE AUTOXIDATION; LIQUID-PHASE AUTOXIDATION; DENSITY-FUNCTIONAL THEORY; JET-STIRRED REACTOR; ELEVATED-TEMPERATURES; COMBUSTION CHEMISTRY; BURNING VELOCITIES; PREMIXED FLAMES AB In this paper we report the detection and identification of the keto-hydroperoxide (hydroperoxymethyl formate, HPMF, HOOCH2OCHO) and other partially oxidized intermediate species arising from the low-temperature (540 K) oxidation of dimethyl ether (DME). These observations were made possible by coupling a jet-stirred reactor with molecular-beam sampling capabilities, operated near atmospheric pressure, to a reflectron time-of-flight mass spectrometer that employs single-photon ionization via tunable synchrotron-generated vacuumultraviolet radiation. On the basis of experimentally observed ionization thresholds and fragmentation appearance energies, interpreted with the aid of ab initio calculations, we have identified HPMF and its conceivable decomposition products HC(O)O(O)CH (formic acid anhydride), HC(O)OOH (performic acid), and HOC(O)OH (carbonic acid). Other intermediates that were detected and identified include HC(O)OCH3 (methyl formate), cycl-CH2-O-CH2-O- (1,3-dioxetane), CH3OOH (methyl hydroperoxide), HC(O)OH (formic acid), and H2O2 (hydrogen peroxide). We show that the theoretical characterization of multiple conformeric structures of some intermediates is required when interpreting the experimentally observed ionization thresholds, and a simple method is presented for estimating the importance of multiple conformers at the estimated temperature (similar to 100 K) of the present molecular beam. We also discuss possible formation pathways of the detected species: for example, supported by potential energy surface calculations, we show that performic acid may be a minor channel of the O-2 + CH2OCH2OOH reaction, resulting from the decomposition of the HOOCH2OCHOOH intermediate, which predominantly leads to the HPMF. C1 [Moshammer, Kai; Jasper, Ahren W.; Lucassen, Arnas; Eskola, Arkke J.; Taatjes, Craig A.; Hansen, Nils] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. [Moshammer, Kai; Kohse-Hoeinghaus, Katharina] Univ Bielefeld, Dept Chem, D-33615 Bielefeld, Germany. [Popolan-Vaida, Denisia M.; Leone, Stephen R.] Univ Calif Berkeley, Dept Chem & Phys, Berkeley, CA 94720 USA. [Popolan-Vaida, Denisia M.; Leone, Stephen R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Dievarti, Pascal; Ju, Yiguang] Princeton Univ, Dept Mech & Aerosp Engn, Princeton, NJ 08544 USA. [Selim, Hatem; Sarathy, S. Mani] King Abdullah Univ Sci & Technol, Clean Combust Res Ctr, Thuwal 239556900, Saudi Arabia. [Dagaut, Philippe] CNRS, INSIS, F-45071 Orleans 2, France. RP Hansen, N (reprint author), Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. EM nhansen@sandia.gov RI Dagaut, Philippe/C-1709-2008; Hansen, Nils/G-3572-2012; Kohse-Hoinghaus, Katharina/A-3867-2012; Sarathy, S. Mani/M-5639-2015; Lucassen, Arnas/G-3803-2013; Jasper, Ahren/A-5292-2011 OI Dagaut, Philippe/0000-0003-4825-3288; Sarathy, S. Mani/0000-0002-3975-6206; Lucassen, Arnas/0000-0003-2967-2030; FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; U.S. Department of Energy, Office of Basic Energy Sciences [DE-S C0001198]; Department of Energy Gas Phase Chemical Physics Program at Lawrence Berkeley National Laboratory [DEAC02-05CH11231]; Alexander von Humboldt Foundation; DFG [SFB 686, TP B3]; European Research Council under the European Community's Seventh Framework Programme/ERC [291049-2G-05afe]; King Abdullah University of Science and Technology; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DEACO2-05CH11231]; National Nuclear Security Administration [DE-AC04-94-AL85000] FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. The work was initiated by the Combustion Energy Frontier Research Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Basic Energy Sciences, under Award Number DE-S C0001198. D.M.P.V. and S.R.L. are supported by the Department of Energy Gas Phase Chemical Physics Program at Lawrence Berkeley National Laboratory, under contract DEAC02-05CH11231. D.M.P.V. is particularly grateful to the Alexander von Humboldt Foundation for a Feodor Lynen fellowship and she greatly acknowledges the technical support by James Breen, Erik Granlund, and William Thur during the designing process and the fabrication of the JSR system. KM. and K.K.H. are grateful for partial support by DFG within the large-scale research structure SFB 686, TP B3. P. Dagaut has received funding from the European Research Council under the European Community's Seventh Framework Programme (FP7/2007-2013)/ERC grant agreement No. 291049-2G-05afe. Researchers at the Clean Combustion Research Center acknowledge funding from King Abdullah University of Science and Technology. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DEACO2-05CH11231. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the National Nuclear Security Administration under contract DE-AC04-94-AL85000. NR 94 TC 17 Z9 17 U1 9 U2 73 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7361 EP 7374 DI 10.1021/acs.jpca5b00101 PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600030 PM 25695304 ER PT J AU Savee, JD Borkar, S Welz, O Sztaray, B Taatjes, CA Osborn, DL AF Savee, John D. Borkar, Sampada Welz, Oliver Sztaray, Balint Taatjes, Craig A. Osborn, David L. TI Multiplexed Photoionization Mass Spectrometry Investigation of the O(P-3) + Propyne Reaction SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID ELECTRON-IMPACT IONIZATION; SET MODEL CHEMISTRY; CROSS-SECTION; OXYGEN-ATOMS; COMBUSTION CHEMISTRY; CHEMICAL-DYNAMICS; BRANCHING RATIOS; LIGHT-SOURCE; GAS-PHASE; CHANNELS AB The reaction of O(P-3) + propyne (C3H4) was investigated at 298 K and 4 Torr using time-resolved multiplexed photoionization mass spectrometry and a synchrotron-generated tunable vacuum ultraviolet light source. The time-resolved mass spectra of the observed products suggest five major channels under our conditions: C2H3 + HCO, CH3 + HCCO, H + CH3CCO, C2H4 + CO, and C2H2 + H-2 + CO. The relative branching ratios for these channels were found to be 1.00, (0.35 +/- 0.11), (0.18 +/- 0.10), (0.73 +/- 0.27), and (1.31 +/- 0.62). In addition, we observed signals consistent with minor production of C3H3 + OH and H-2 + CH2CCO, although we cannot conclusively assign them as direct product channels from O(P-3) + propyne. The direct abstraction mechanism plays only a minor role (<= 1%), and we estimate that O(P-3) addition to the central carbon of propyne accounts for 10% of products, with addition to the terminal carbon accounting for the remaining 89%. The isotopologues observed in experiments using d(1)-propyne (CH3CCD) and analysis of product branching in light of previously computed stationary points on the singlet and triplet potential energy surfaces (PESs) relevant to O(P-3) + propyne suggest that, under our conditions, (84 +/- 14)% of the observed product channels from O(P-3) + propyne result from intersystem crossing from the initial triplet PES to the lower-lying singlet PES. C1 [Savee, John D.; Welz, Oliver; Taatjes, Craig A.; Osborn, David L.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. [Borkar, Sampada; Sztaray, Balint] Univ Pacific, Dept Chem, Stockton, CA 95211 USA. RP Osborn, DL (reprint author), Sandia Natl Labs, Combust Res Facil, Mail Stop 9055, Livermore, CA 94551 USA. EM dlosbor@sandia.gov FU U.S. Department of Energy Office of Science, Office of Basic Energy Sciences; National Nuclear Security Administration [DE-AC04-94-AL85000]; Office of Science, Office of Basic Energy Sciences, the U.S. Department of Energy at Lawrence Berkeley National Laboratory [DE-AC02-05CH11231] FX We thank Mr. Howard Johnsen and the staff of the Chemical Dynamics Beamline at the Advanced Light Source for technical support of these experiments. This material is based upon work supported by the U.S. Department of Energy Office of Science, Office of Basic Energy Sciences. Sandia is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the National Nuclear Security Administration under contract no. DE-AC04-94-AL85000. This research used resources of the Advanced Light Source, a DOE Office of Science User Facility, which is supported by the Director, Office of Science, Office of Basic Energy Sciences, the U.S. Department of Energy under contract no. DE-AC02-05CH11231 at Lawrence Berkeley National Laboratory. NR 74 TC 4 Z9 4 U1 5 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7388 EP 7403 DI 10.1021/acs.jpca.5b00491 PG 16 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600032 PM 25985181 ER PT J AU Forthomme, D Hause, ML Yu, HG Dagdigian, PJ Sears, TJ Hall, GE AF Forthomme, Damien Hause, Michael L. Yu, Hua-Gen Dagdigian, Paul J. Sears, Trevor J. Hall, Gregory E. TI Doppler-Resolved Kinetics of Saturation Recovery SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID ROTATIONAL ENERGY-TRANSFER; STATE-TO-STATE; INFRARED DOUBLE-RESONANCE; FREQUENCY-MODULATION SPECTROSCOPY; RATE CONSTANTS; VELOCITY DISTRIBUTION; SPEED DEPENDENCE; TIME EVOLUTION; CROSS-SECTION; COLLISIONS AB Frequency-modulated laser transient absorption has been used to monitor the ground-state rotational energy-transfer rates of CN radicals in a double-resonance, depletion recovery experiment. When a pulsed laser is used to burn a hole in the equilibrium ground-state population of one rotational state without velocity selection, the population recovery rate is found to depend strongly on the Doppler detuning of a narrow-band probe laser. Similar effects should be apparent for any relaxation rate process that competes effectively with velocity randomization. Alternative methods of extracting thermal rate constants in the presence of these non-thermal conditions are evaluated. Total recovery rate constants, analogous to total removal rate constants in an experiment preparing a single initial rotational level, are in good agreement with quantum scattering calculations, but are slower than previously reported experiments and show qualitatively different rotational state dependence between Ar and He collision partners. Quasi-classical trajectory studies confirm that the differing rotational state dependence is primarily a kinematic effect. C1 [Forthomme, Damien; Hause, Michael L.; Yu, Hua-Gen; Sears, Trevor J.; Hall, Gregory E.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Dagdigian, Paul J.] Johns Hopkins Univ, Dept Chem, Baltimore, MD 21218 USA. [Sears, Trevor J.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. RP Hall, GE (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM gehall@bnl.gov RI Yu, Hua-Gen/N-7339-2015; Sears, Trevor/B-5990-2013; Hall, Gregory/D-4883-2013 OI Sears, Trevor/0000-0002-5559-0154; Hall, Gregory/0000-0002-8534-9783 FU U.S. Department of Energy, Office of Science [DE-AC02-98CH10886, DE-SC0012704]; Division of Chemical Sciences, Geosciences, and Biosciences within the Office of Basic Energy Sciences; U.S. Department of Energy, Office of Science, Basic Energy Sciences [DESC0002323] FX This work was carried out at Brookhaven National Laboratory under Contracts No. DE-AC02-98CH10886 and DE-SC0012704 from the U.S. Department of Energy, Office of Science, and supported by its Division of Chemical Sciences, Geosciences, and Biosciences within the Office of Basic Energy Sciences. The theoretical portion of this work performed at JHU was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, under Award No. DESC0002323. We are grateful to George McBane and Millard Alexander for helpful discussions. NR 57 TC 0 Z9 0 U1 0 U2 7 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7439 EP 7450 DI 10.1021/acs.jpca.5b00628 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600036 PM 25815527 ER PT J AU Westbrook, CK Pitz, WJ Mehl, M Glaude, PA Herbinet, O Bax, S Battin-Leclerc, F Mathieu, O Petersen, EL Bugler, J Curran, HJ AF Westbrook, Charles K. Pitz, William J. Mehl, Marco Glaude, Pierre-Alexandre Herbinet, Olivier Bax, Sarah Battin-Leclerc, Frederique Mathieu, Olivier Petersen, Eric L. Bugler, John Curran, Henry J. TI Experimental and Kinetic Modeling Study of 2-Methyl-2-Butene: Allylic Hydrocarbon Kinetics SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID JET-STIRRED REACTOR; LOW-TEMPERATURE; SHOCK-TUBE; 1-HEXENE OXIDATION; CHEMICAL-KINETICS; BIODIESEL FUELS; DOUBLE-BOND; GAS-PHASE; COMBUSTION; IGNITION AB Two experimental studies have been carried out on the oxidation of 2-methyl-2-butene, one measuring ignition delay times behind reflected shock waves in a stainless steel shock tube, and the other measuring fuel, intermediate, and product species mole fractions in a jet-stirred reactor (JSR). The shock tube ignition experiments were carried out at three different pressures, approximately 1.7, 11.2, and 31 atm, and at each pressure, fuel-lean (phi = 0.5), stoichiometric (phi = 1.0), and fuel-rich (phi = 2.0) mixtures were examined, with each fuel/oxygen mixture diluted in 99% Ar, for initial postshock temperatures between 1330 and 1730 K. The JSR experiments were performed at nearly atmospheric pressure (800 Torr), with stoichiometric fuel/oxygen mixtures with 0.01 mole fraction of 2M2B fuel, a residence time in the reactor of 1.5 s, and mole fractions of 36 different chemical species were measured over a temperature range from 600 to 1150 K. These JSR experiments represent the first such study reporting detailed species measurements for an unsaturated, branched hydrocarbon fuel larger than iso-butene. A detailed chemical kinetic reaction mechanism was developed to study the important reaction pathways in these experiments, with particular attention on the role played by allylic C-H bonds and allylic pentenyl radicals. The results show that, at high temperatures, this olefinic fuel reacts rapidly, similar to related alkane fuels, but the pronounced thermal stability of the allylic pentenyl species inhibits low temperature reactivity, so 2M2B does not produce "cool flames" or negative temperature coefficient behavior. The connections between olefin hydrocarbon fuels, resulting allylic fuel radicals, the resulting lack of low-temperature reactivity, and the gasoline engine concept of octane sensitivity are discussed. C1 [Westbrook, Charles K.; Pitz, William J.; Mehl, Marco] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Glaude, Pierre-Alexandre; Herbinet, Olivier; Bax, Sarah; Battin-Leclerc, Frederique] Univ Lorraine, CNRS, Lab React & Genie Proc, Nancy, France. [Mathieu, Olivier; Petersen, Eric L.] Texas A&M Univ, Dept Mech Engn, College Stn, TX 77843 USA. [Bugler, John; Curran, Henry J.] Natl Univ Ireland, Sch Chem, Galway, Ireland. RP Westbrook, CK (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM westbrookck@earthlink.net RI Petersen, Eric/M-3609-2014; Mehl, Marco/A-8506-2009; OI Petersen, Eric/0000-0002-4572-5916; Mehl, Marco/0000-0002-2227-5035; Glaude, Pierre-Alexandre/0000-0001-9166-8388; Curran, Henry/0000-0002-5124-8562; herbinet, olivier/0000-0002-2155-098X FU U.S. Department of Energy, Office of Basic Energy Sciences, Vehicle Technologies Office; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; TEES Turbomachnery Laboratory; European Commission through the "Clean ICE" Advanced Research Grant of the European Research Council; Irish Research Council FX The authors thank Dr. Ellen Meeks of Reaction Design, who first suggested this study of 2-methyl 2-butene. The work at LLNL was supported by the U.S. Department of Energy, Office of Basic Energy Sciences (program manager, Wade Sisk), Vehicle Technologies Office (program manager Gurpreet Singh and Leo Breton) and was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. The efforts at Texas A&M University were supported, in part, by the TEES Turbomachnery Laboratory. The work at the Universite de Lorraine was supported by the European Commission through the "Clean ICE" Advanced Research Grant of the European Research Council. NUI Galway would like to acknowledge the support of the Irish Research Council in funding their portion of this work. NR 65 TC 14 Z9 14 U1 7 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7462 EP 7480 DI 10.1021/acs.jpca.5b00687 PG 19 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600038 PM 25822578 ER PT J AU Singh, RI Mebel, AM Frenldach, M AF Singh, Ravi I. Mebel, Alexander M. Frenldach, Michael TI Oxidation of Graphene-Edge Six- and Five-Member Rings by Molecular Oxygen SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID POLYCYCLIC AROMATIC-HYDROCARBONS; POTENTIAL-ENERGY SURFACE; MONTE-CARLO-SIMULATION; THERMAL-DECOMPOSITION; REACTION-MECHANISM; SOOT FORMATION; NAPHTHYL RADICALS; CARBON CLUSTERS; AIR-POLLUTION; LAYER GROWTH AB To gain qualitative and quantitative understanding Of oxidation processes of large polycyclic aromatics, soot particles, and graphene edges, a theoretical Study is reported for the pyrenyl-O-2 reaction system. First, possible reaction pathways and their energetics were investigated Using high-level ab initio calculations. The results were utilized in RRKM-master equation calculations of rate coefficients and relative product yields at temperatures and pressures relevant to combustion. Finally, the deduced oxidation mechanisms of six- and five-member rings and the computed rate coefficients were employed in kinetic Monte Carlo simulations of oxidation of a graphene "molecule" evolving inflame-like environments. Among the major findings from the latter simulations are the following: The oxidation system exhibits two basic pathways, thermal decomposition and regeneration of oxyradicals. Their competition is temperature-dependent, with the former dominating,at higher and the latter at lower temperatures. The overall oxidation of the graphene time-dependent, with the initial rates consistent with the known experimental data. substrate is computed to be C1 [Mebel, Alexander M.] Florida Int Univ, Dept Chem & Biochem, Miami, FL 33199 USA. [Singh, Ravi I.; Frenldach, Michael] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. [Frenldach, Michael] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Mebel, AM (reprint author), Florida Int Univ, Dept Chem & Biochem, Miami, FL 33199 USA. EM mebela@fiu.edu; frenklach@berkeley.edu RI Mebel, Alexander/A-5234-2009 FU Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Sciences of the U.S. Department of Energy [DE-FG02-04ER15570, DE-AC03-76F00098]; U.S. Army Corps of Engineers, Humphreys Engineering Center Support Activity [W912HQ-11-C-0035]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was funded by the Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Sciences of the U.S. Department of Energy (Grant DE-FG02-04ER15570 to Florida International University and Contract DE-AC03-76F00098 to Lawrence Berkeley National Laboratory) and by the U.S. Army Corps of Engineers, Humphreys Engineering Center Support Activity (Contract W912HQ-11-C-0035 to University of California at Berkeley). This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract DE-AC02-05CH11231. A.M.M. acknowledges the Instructional & Research Computing Center (IRCC, web: http://ircc.fiu.edu) at Florida International University for providing HPC computing resources that have contributed to the research results reported within this paper. NR 67 TC 8 Z9 8 U1 4 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7528 EP 7547 DI 10.1021/acs.jpca.5b00868 PG 20 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600042 PM 25894330 ER PT J AU Xu, H Pratt, ST AF Xu, Hong Pratt, S. T. TI Photodissociation of Methyl Iodide via Selected Vibrational Levels of the (B)over-tilde (E-2(3/2))6s Rydberg State SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID MAGNETIC CIRCULAR-DICHROISM; RESONANCE RAMAN-SCATTERING; PUMP-PROBE TECHNIQUE; B-STATE; PREDISSOCIATION DYNAMICS; MULTIPHOTON IONIZATION; 193.3 NM; ALKYL IODIDES; QUANTUM YIELD; CH3I AB We have determined the I P-2(3/2) and P-2(1/2) branching fractions following the photodissociation of methyl iodide (CH3I) via a number of vibronic bands associated with the (B) over tilde (E-2(3/2))6s Rydberg state at excitation wavelengths between 201.2 and 1927. nm. Vacuum ultraviolet light at 118.2 nm was used to ionize both the product iodine atoms and the methyl radical cofragments, and velocity map ion imaging was used to determine the product translational energy distribution's and angular distributions. The known relative photoionitation cross sections for (IP3/2)-P-2 and P-2(1/2) at 118.2 nm were used to determine the corresponding branching fractions. The results extend our earlier work at 193 nm by Xu et al. (J. Chem. Phys. 2013, 139, 214310), and complement the clogely related work of Gonzalez et al. (J. Chem. Phys. 2011, 135, 021102). We find that for most of the excited vibronic levels of the (B) over tilde state studied, the I P-2(3/2) branching ratio is small, but nonzero, and thatthis channel is associated with internally excited CH3 radicals. The results are discussed in relation to the recent theoretical results of Alekseyev et al. (J. Chem. Phys. 2011, 134, 044303). C1 [Xu, Hong; Pratt, S. T.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Pratt, ST (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM stpratt@anl.gov FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-AC02-06CH11357] FX This material is based on work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences under contract No. DE-AC02-06CH11357. NR 68 TC 1 Z9 1 U1 4 U2 9 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7548 EP 7558 DI 10.1021/acs.jpca.5b00860 PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600043 PM 25946320 ER PT J AU Fridlyand, A Godsborough, SS Brezinsky, K AF Fridlyand, Aleksandr Godsborough, S. Scott Brezinsky, Kenneth TI Chemical Kinetic Influences of Alkyl Chain Structure on the High Pressure and Temperature Oxidation of a Representative Unsaturated Biodiesel: Methyl Nonenoate SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID PULSE SHOCK-TUBE; DOUBLE-BOND; OXYGENATED FUELS; COMBUSTION; PYROLYSIS; AUTOIGNITION; HYDROCARBONS; SENSITIVITY; MECHANISMS; CHEMISTRY AB The high pressure and temperature oxidation of methyl trans-2-nonenoate, methyl trans-3-nonenoate, 1-octene, and trans-2-octene are investigated experimentally to probe the influence of the double bond position on the chemical kinetics of long esters and alkenes. Single pulse shock tube experiments are performed in the ranges p = 3.8-6.2 MPa and T = 850-1500 K, with an average reaction time of 2 ms. Gas chromatographic measurements indicate increased reactivity for trans-2-octene compared to 1-octene, whereas both methyl nonenoate isomers have reactivities similar to that of 1-octene. A difference in the yield of stable intermediates is observed for the octenes when compared to the methyl nonenoates. Chemical kinetic models are developed with the aid of the Reaction Mechanism Generator to interpret the experimental results. The models are created using two different base chemistry submodels to investigate the influence of the foundational chemistry (i.e., C0-C4), whereas Monte Carlo simulations are performed to examine the quality of agreement with the experimental results. Significant uncertainties are found in the chemistry of unsaturated esters with the double bonds located close to the ester groups. This work highlights the importance of the foundational chemistry in predictive chemical kinetics of biodiesel combustion at engine relevant conditions. C1 [Fridlyand, Aleksandr; Godsborough, S. Scott; Brezinsky, Kenneth] Univ Illinois, Dept Mech & Ind Engn, Chicago, IL 60607 USA. [Fridlyand, Aleksandr; Godsborough, S. Scott] Argonne Natl Lab, Div Energy Syst, Lemont, IL 60439 USA. RP Brezinsky, K (reprint author), Univ Illinois, Dept Mech & Ind Engn, 842 W Taylor St, Chicago, IL 60607 USA. EM kenbrez@uic.edu FU Office of Energy Efficiency and Renewable Energy, Office of Vehicle Technology [DE-AC02-06CH11357] FX The authors thank Dr. Stephen Garner, Dr. Tomasz Malewicki, and Miroslaw Liszka for their help with the experiments. The authors also thank Professor William H. Green and Shamel Merchant from the Massachusetts Institute of Technology for their guidance on using RMG. This manuscript has been created in part by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357, with funding provided by the Office of Energy Efficiency and Renewable Energy, Office of Vehicle Technology. NR 48 TC 3 Z9 3 U1 1 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7559 EP 7577 DI 10.1021/acs.jpca.5b00914 PG 19 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600044 PM 25710595 ER PT J AU Altinay, G Macdonald, RG AF Altinay, Gokhan Macdonald, R. Glen TI Determination of the Rate Constants for the NH2((XB1)-B-2) + NH2((XB1)-B-2) and NH2((XB1)-B-2) + H Recombination Reactions in N-2 as a Function of Temperature and Pressure SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID THERMAL UNIMOLECULAR REACTIONS; COLLISION RATE CONSTANTS; FALL-OFF RANGE; RECOMBINATION REACTION; PRESSURE-DEPENDENCE; TEMPERATURE; KINETICS; GAS; AMMONIA; ATOM AB The recombination rate constants for the reactions NH2 + NH2 -> N2H4 (reaction k(1b)) and NH2 + H -> NH3 (reaction k(2b)) with N-2 as a third-body have been measured as a function of temperature and pressure. The temperature range was from 292 to 533 K and the pressure range from a few Torr up to 300-400 Torr, well within the pressure falloff region. The NH2 radical was produced by 193 nm pulsed-laser photolysis of NH3 in a temperature controlled flow chamber. High-resolution time-resolved laser absorption spectroscopy was used to follow the temporal concentration profiles of both NH2 and NH3, simultaneously. The NH2 radical was monitored at 14800.65 cm(-1) using the (1)2(31) (0,7,0)(A) over tilde (2)A(1) (1)3(31) (0,0,0)(X) over tilde B-2(1) ro-vibronic transition, and NH3 monitored at 3336.39 cm(-1) on the (q)Q(3)(3)s (1,0,0,0) <- (0,0,0,0) ro-vibrational transition. The necessary collisional broadening parameters for each molecule were measured in separate experiments. The pressure and temperature dependence of k(1b) can be represented by the Troe parameters: k(0), the low-pressure three-body recombination rate constant, k(0)(T) = (1.14+/ 0.59) x 10(-19)T(-(3.41 +/- 0.28)) cm(6) molecule(-2) s(-1), and F-cent, the pressure broadening parameter, F-cent = 0.15+/ 0.12, independent of temperature. The data could not be fit by three-independent parameters, and the high-pressure limiting rate constant k(infinity)(T) = 9.33 x 10(-10)T(-0.414) e(33/T) cm(3) molecule(-1) s(-1) was taken from the high-quality theoretical calculations of Klippenstein et al. (J. Phys. Chem A 2009, 113, 10241). The pressure and temperature dependence of k(2b), can be represented by the Troe parameters: k(0)(T) = (9.95+/ 0.58) x 10(-26)T((-1.76 +/- 0.092)) cm(6) molecule(-2) s(-1), F-cent = 0.5+/ 0.2, k = 2.6 x 10(-10) cm(3) molecule(-1) s(-1). Again, the data could not be fit with three independent parameters, and k(2b) was chosen to be 2.6 X 10(-10) cm(3) molecule(-1) s(-1) and fixed in the analysis. C1 [Altinay, Gokhan; Macdonald, R. Glen] Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA. RP Macdonald, RG (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Lemont, IL 60439 USA. EM rgmacdonald@anl.gov FU U.S. Department of Energy, Office of Basic Energy Science, Division of Chemical Sciences, Geosciences, and Biosciences, US. Department of Energy [DE-AC02-06CH11357] FX This material is based upon work supported by the U.S. Department of Energy, Office of Basic Energy Science, Division of Chemical Sciences, Geosciences, and Biosciences, US. Department of Energy under Contract No. DE-AC02-06CH11357. NR 51 TC 1 Z9 1 U1 3 U2 7 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7593 EP 7610 DI 10.1021/acs.jpca.5b00917 PG 18 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600046 PM 25871301 ER PT J AU Takeshita, TY Lindquist, BK Dunning, TH AF Takeshita, Tyler Y. Lindquist, Beth K. Dunning, Thom H., Jr. TI Insights into the Electronic Structure of Ozone and Sulfur Dioxide from Generalized Valence Bond Theory: Bonding in O-3 and SO2 SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID CORRELATED MOLECULAR CALCULATIONS; GAUSSIAN-BASIS SETS; CONFIGURATION-INTERACTION CALCULATIONS; IMPROVED QUANTUM-THEORY; WAVE-FUNCTIONS; ATOMS ALUMINUM; SYSTEMS; MODELS; ARGON; SPIN AB There are many well-known differences in the physical and chemical properties of ozone (O-3) and sulfur dioxide (SO2). O-3 has longer and weaker bonds than O-2, whereas SO2 has shorter and stronger bonds than SO. The O-O-2 bond is dramatically weaker than the O-SO bond, and the singlet triplet gap in SO2 is more than double that in O-3. In addition, O-3 is a very reactive species, while SO2 is far less so. These disparities have been attributed to variations in the amount of diradical character in the two molecules. In this work, we use generalized valence bond (GVB) theory to characterize the electronic structure of ozone and sulfur dioxide, showing O-3 does indeed possess significant diradical character, whereas SO2 is effectively a closed shell molecule. The GVB results provide critical insights into the genesis of the observed difference in these two isoelectronic species. SO2 possesses a recoupled pair bond dyad in the a ''(pi) system, resulting in SO double bonds. The pi system of O-3, on the other hand, has a lone pair on the central oxygen atom plus a pair of electrons in orbitals on the terminal oxygen atoms that give rise to a relatively weak pi interaction. C1 [Takeshita, Tyler Y.; Lindquist, Beth K.; Dunning, Thom H., Jr.] Univ Illinois, Dept Chem, Urbana, IL 61801 USA. RP Dunning, TH (reprint author), Univ Washington, Northwest Inst Adv Comp, Pacific NW Natl Lab, 127 Sieg Hall, Seattle, WA 98195 USA. EM thdjr@uw.edu FU Distinguished Chair for Research Excellence in Chemistry; National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign; National Science Foundation FX This work was supported by the Distinguished Chair for Research Excellence in Chemistry and the National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign. One of the authors (B.A.L.) is the grateful recipient of a National Science Foundation Graduate Research Fellowship. NR 46 TC 9 Z9 9 U1 2 U2 10 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7683 EP 7694 DI 10.1021/acs.jpca.5b00998 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600052 PM 26068052 ER PT J AU Sivaramakrishnan, R Michael, JV Harding, LB Klippenstein, SJ AF Sivaramakrishnan, Raghu Michael, Joe V. Harding, Lawrence B. Klippenstein, Stephen J. TI Resolving Some Paradoxes in the Thermal Decomposition Mechanism of Acetaldehyde SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID TOTAL ATOMIZATION ENERGIES; SHOCK-TUBE; PYROLYSIS; RADICALS; MOLECULES; PHOTODISSOCIATION; OXIDATION; PATHWAYS; ETHANOL; ACETONE AB The mechanism for the thermal decomposition of acetaldehyde has been revisited with an analysis of literature kinetics experiments using theoretical kinetics. The present modeling study was motivated by recent observations, with very sensitive diagnostics, of some unexpected products in high temperature microtubular reactor experiments on the thermal decomposition of CH3CHO and its deuterated analogs, CH3CDO, CD3CHO, and CD3CDO. The observations of these products prompted the authors of these studies to suggest that the enol tautomer, CH2CHOH (vinyl alcohol), is a primary intermediate in the thermal decomposition of acetaldehyde. The present modeling efforts on acetaldehyde decomposition incorporate a master equation reanalysis Of the CH3CHO potential energy surface (PES). The lowest-energy process on this PES is an isomerization of CH3CHO to CH2CHOH. However, the subsequent product channels for CH2CHOH are substantially higher in energy, and the only unimolecular process that can be thermally accessed is a reisomerizatiorr to CH3CHO. The incorporation of these new theoretical kinetics predictions into models for selected literature experiments on CH3CHO thermal decomposition confirms out earlier experiment and theory-based conclusions that the dominant decomposition process in CH3CHO at high temperatures is CC bond fission with a minor contribution (similar to 10-20%) from the roaming mechanism to form CH4 and CO. The present modeling efforts also incorporate a master-equation analysis, of the H + CH2HOH potential energy surface. This bimolecular reaction is the primary mechanism for removal of CH2CHOH, which can accumulate to minor amounts at high temperatures, T > 1000 K, in most lab-scale experiments that use large initial concentrations of CH3CHO. Our modeling efforts indicate that the observation of ketene, water, and acetylene in the recent microtubular experiments are primarily due to bimolecular reactions of CH3CHO and CH2CHOH with H-atoms and have no bearing on the unimolecular decomposition mechanism of CH3CHO. The present simulations also indicate that experiments using these microtubular reactors when interpreted with the aid of high-level theoretical calculations and kinetics modeling can offer insights into the chemistry of elusive intermediates in the high-temperature pyrolysis of organic molecules. C1 [Sivaramakrishnan, Raghu; Michael, Joe V.; Harding, Lawrence B.; Klippenstein, Stephen J.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Sivaramakrishnan, R (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM raghu@anl.gov RI SIVARAMAKRISHNAN, RAGHU/C-3481-2008; OI SIVARAMAKRISHNAN, RAGHU/0000-0002-1867-1254; Klippenstein, Stephen/0000-0001-6297-9187 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-AC02-06CH11357] FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, under Contract DE-AC02-06CH11357. We thank Branko Ruscic (ANL) for aid in narrowing down the source of differences between the current thermochemistry and that found in the Burcat thermochemical database. R.S. is delighted to acknowledge the active mentorship by Larry Harding, Joe Michael, Al Wagner, and other colleagues in the Argonne Chemical Dynamics Group, who have served as role models for aspiring junior scientists (such as himself) in the field of chemical kinetics/dynamics. NR 46 TC 2 Z9 2 U1 7 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7724 EP 7733 DI 10.1021/acs.jpca.5b01032 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600056 PM 25793559 ER PT J AU Antonov, IO Kwok, J Zador, J Sheps, L AF Antonov, Ivan O. Kwok, Justin Zador, Judit Sheps, Leonid TI A Combined Experimental and Theoretical Study of the Reaction OH+2-Butene in the 400-800 K Temperature Range SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID RADICAL-MOLECULE REACTIONS; POTENTIAL-ENERGY SURFACE; TRANSITION-STATE THEORY; GAS-PHASE REACTIONS; ORGANIC-COMPOUNDS; COMBUSTION CHEMISTRY; OH RADICALS; N-BUTANOL; KINETICS; OXIDATION AB We report a combined experimental and theoretical study of the OH + cis-2-butene and OH + trans-2-butene reactions at combustion-relevant conditions: pressures of 1-20 bar and temperatures of 400-800 K. We probe the OH radical time histories by laser-induced fluorescence and analyze these experimental measurements with aid from time-dependent master-equation calculations. Importantly, our investigation covers a temperature range where experimental data on OH + alkene chemistry in general are lacking, and interpretation of such data is challenging due to the complexity of the competing reaction pathways. Guided by theory, we unravel this complex behavior and determine the temperature- and pressure-dependent rate coefficients for the three most important OH + 2-butene reaction channels at our conditions: H abstraction, OH addition to the double bond, and back-dissociation of the OH-butene adduct. C1 [Antonov, Ivan O.; Kwok, Justin; Zador, Judit; Sheps, Leonid] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. RP Sheps, L (reprint author), Sandia Natl Labs, Combust Res Facil, Mail Stop 9055, Livermore, CA 94551 USA. EM lsheps@sandia.gov RI Zador, Judit/A-7613-2008 OI Zador, Judit/0000-0002-9123-8238 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; National Nuclear Security Administration [DE-AC04-94AL85000] FX J.Z. thanks Prof. C. Franklin Goldsmith for providing the program to generate CHEMKIN-style Arrhenius fits to the calculated rate coefficients. This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the National Nuclear Security Administration, under contract DE-AC04-94AL85000. The work of L.S. and I.O.A. was part of the Argonne-Sandia Consortium on High-Pressure Combustion Chemistry. NR 50 TC 0 Z9 0 U1 10 U2 28 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7742 EP 7752 DI 10.1021/acs.jpca.5b01012 PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600058 PM 25860092 ER PT J AU Goldsmith, CF Harding, LB Georgievskii, Y Miller, JA Klippenstein, SJ AF Goldsmith, C. Franklin Harding, Lawrence B. Georgievskii, Yuri Miller, James A. Klippenstein, Stephen J. TI Temperature and Pressure-Dependent Rate Coefficients for the Reaction of Vinyl Radical with Molecular Oxygen SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID TRANSITION-STATE THEORY; AB-INITIO; C2H3+O-2 REACTION; MASTER EQUATION; KINETICS; O-2; ETHYLENE; THERMOCHEMISTRY; COMBUSTION; OXIDATION AB State-of-the-art calculations of the C2H3O2 potential energy surface are presented. A new method is described for computing the interaction potential for R + O-2 reactions. The method, which combines accurate determination of the quartet potential along the doublet minimum energy path with multireference calculations of the doublet/quartet splitting, decreases the uncertainty in the doublet potential and thence the rate constants by more than a factor of 2. The temperature and pressure-dependent rate coefficients are computed using variable reaction coordinate transition-state theory, variational transition-state theory, and conventional transition-state theory, as implemented in a new RRKM/ME code. The Main bimolecular product Channels are CH2O + HCO at lower temperatures and CH2CHO + O at higher temperatures. Above 10 atm, the collisional stabilization of CH2CHOO directly competes with these two product channels. CH2CHOO decomposes primarily to CH2O + HCO. The next two most significant bimolecular products are OCHCHO + H and (CHCHO)-C-3 + OH, and not C2H2 + HO2. C2H3 + O-2 will be predominantly chain branching above 1700 K. Uncertainty analysis is presented for the two most important transition states. The uncertainties in these two barrier heights result in a significant uncertainty in the temperature at which CH2CHO + O overtakes all other product channels. C1 [Goldsmith, C. Franklin; Harding, Lawrence B.; Georgievskii, Yuri; Miller, James A.; Klippenstein, Stephen J.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Goldsmith, C. Franklin] Brown Univ, Sch Engn, Providence, RI 02912 USA. RP Goldsmith, CF (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. OI Klippenstein, Stephen/0000-0001-6297-9187 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, Argonne-Sandia Consortium on High-Pressure Combustion Chemistry (FWP) [DE-AC02-06CH11357, 59044]; Brown University; Argonne Director's Post-doctoral Fellowship FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences under Contract No. DE-AC02-06CH11357 as part of the Argonne-Sandia Consortium on High-Pressure Combustion Chemistry (FWP # 59044). C.F.G. gratefully acknowledges financial support from the Argonne Director's Post-doctoral Fellowship and from Brown University. NR 56 TC 11 Z9 11 U1 5 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7766 EP 7779 DI 10.1021/acs.jpca.5b01088 PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600060 PM 25978112 ER PT J AU Klippenstein, SJ Miller, JA Jasper, AW AF Klippenstein, Stephen J. Miller, James A. Jasper, Ahren W. TI Kinetics of Propargyl Radical Dissociation SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID TRANSITION-STATE THEORY; CORRELATED MOLECULAR CALCULATIONS; GAUSSIAN-BASIS SETS; MASTER EQUATION; THERMAL-DECOMPOSITION; AB-INITIO; ALIPHATIC FUELS; RECOMBINATION REACTION; AROMATIC-COMPOUNDS; FORMATION PATHWAYS AB Due to the prominent role of the propargyl radical for hydrocarbon growth within combustion environments, it is important to understand the kinetics of its formation and loss. The ab initio transition state theory-based master equation method is used to obtain theoretical kinetic predictions for the temperature and pressure dependence of the thermal decomposition of propargyl, which may be its primary loss channel under some conditions. The potential energy surface for the decomposition of propargyl is first mapped at a high level of theory with a combination of coupled cluster and multireference perturbation calculations. Variational transition state theory is then used to predict the microcanonical rate coefficients, which are subsequently implemented within the multiple-well multiple-channel master equation. A variety of energy transfer parameters are considered, and the sensitivity of the thermal rate predictions to these parameters is explored. The predictions for the thermal decomposition rate coefficient are found to be in good agreement with the limited experimental data. Modified Arrhenius representations of the rate constants are reported for utility in combustion modeling. C1 [Klippenstein, Stephen J.; Miller, James A.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Jasper, Ahren W.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. RP Miller, JA (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM jim.miller1946@gmail.com RI Jasper, Ahren/A-5292-2011; OI Klippenstein, Stephen/0000-0001-6297-9187 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-AC02-06CH11357]; United States Department of Energy [DE-AC04-94-AL85000] FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences under Contract DE-AC02-06CH11357. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy under Contract DE-AC04-94-AL85000. NR 65 TC 7 Z9 7 U1 7 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7780 EP 7791 DI 10.1021/acs.jpca.5b01127 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600061 PM 25871530 ER PT J AU Ruscic, B AF Ruscic, Branko TI Active Thermochemical Tables: Sequential Bond Dissociation Enthalpies of Methane, Ethane, and Methanol and the Related Thermochemistry SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID SET MODEL CHEMISTRY; PHOTOELECTRON-PHOTOION COINCIDENCE; FIELD IONIZATION-PHOTOELECTRON; AB-INITIO THERMOCHEMISTRY; ACETYLENE-VINYLIDENE ISOMERIZATION; DENSITY-FUNCTIONAL GEOMETRIES; POTENTIAL-ENERGY SURFACE; ZERO-POINT ENERGIES; GAS-PHASE; CARBON-MONOXIDE AB Active Thermochemical Tables (ATcT) thermochemistry for the sequential bond dissociations of methane, ethane, and methanol systems were obtained by analyzing and solving a very large thermochemical network (TN). Values for all possible C-H, C-C, C-O, and O-H bond dissociation enthalpies at 298.15 K (BDE298) and bond dissociation energies at 0 K (D-0) are presented. The corresponding ATcT standard gas-phase enthalpies of formation of the resulting CHn, n = 4-0 species (methane, methyl, methylene, methylidyne, and carbon atom), C2Hn, n = 6-0 species (ethane, ethyl, ethylene, ethylidene, vinyl, ethylidyne, acetylene, vinylidene, ethynyl, and ethynylene), and COHn, n = 4-0 species (methanol, hydroxymethyl, methoxy, formaldehyde, hydroxymethylene, formyl, isoformyl, and carbon monoxide) are also presented. The ATcT thermochemistry of carbon dioxide, water, hydroxyl, and carbon, oxygen, and hydrogen atoms is also included, together with the sequential BDEs of CO2 and H2O. The provenances of the ATcT enthalpies of formation, which are quite distributed and involve a large number of relevant determinations, are analyzed by variance decomposition and discussed in terms of principal contributions. The underlying reasons for periodic appearances of remarkably low and/or unusually high BDEs, alternating along the dissociation sequences, are analyzed and quantitatively rationalized. The present ATcT results are the most accurate thermochemical values currently available for these species. C1 [Ruscic, Branko] Argonne Natl Lab, Chem Sci & Engn Div, Chicago, IL 60439 USA. [Ruscic, Branko] Univ Chicago, Computat Inst, Chicago, IL 60637 USA. RP Ruscic, B (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, Chicago, IL 60439 USA. EM ruscic@anl.gov RI Ruscic, Branko/A-8716-2008 OI Ruscic, Branko/0000-0002-4372-6990 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences [DE-AC02-06CH11357] FX This work was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences under Contract No. DE-AC02-06CH11357. NR 182 TC 17 Z9 17 U1 8 U2 46 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7810 EP 7837 DI 10.1021/acs.jpca.5b01346 PG 28 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600064 PM 25760799 ER PT J AU Annesley, CJ Randazzo, JB Klippenstein, SJ Harding, LB Jasper, AW Georgievskii, Y Ruscic, B Tranter, RS AF Annesley, Christopher J. Randazzo, John B. Klippenstein, Stephen J. Harding, Lawrence B. Jasper, Ahren W. Georgievskii, Yuri Ruscic, Branko Tranter, Robert S. TI Thermal Dissociation and Roaming Isomerization of Nitromethane: Experiment and Theory SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID ACTIVE THERMOCHEMICAL TABLES; POTENTIAL-ENERGY SURFACE; NITRO-NITRITE REARRANGEMENT; REFERENCE WAVE-FUNCTIONS; COUPLED-CLUSTER THEORY; REFLECTED SHOCK-TUBE; RATE CONSTANTS; AB-INITIO; UNIMOLECULAR REACTIONS; METHYL RADICALS AB The thermal decomposition of nitromethane provides a classic example of the competition between roaming mediated isomerization and simple bond fission. A recent theoretical analysis suggests that as the pressure is increased from 2 to 200 Torr the product distribution undergoes a sharp transition from roaming dominated to bond-fission dominated. Laser schlieren densitometry is used to explore the variation in the effect of roaming on the density gradients for CH3NO2 decomposition in a shock tube for pressures of 30, 60, and 120 Torr at temperatures ranging from 1200 to 1860 K. A complementary theoretical analysis provides a novel exploration of the effects of roaming on the thermal decomposition kinetics. The analysis focuses on the roaming dynamics in a reduced dimensional space consisting of the rigid-body motions of the CH3 and NO2 radicals. A high-level reduced-dimensionality potential energy surface is developed from fits to large-scale multireference ab initio calculations. Rigid body trajectory simulations coupled with master equation kinetics calculations provide high-level a priori predictions for the thermal branching between roaming and dissociation. A statistical model provides a qualitative/semiquantitative interpretation of the results. Modeling efforts explore the relation between the predicted roaming branching and the observed gradients. Overall, the experiments are found to be fairly consistent with the theoretically proposed branching ratio, but they are also consistent with a no-roaming scenario and the underlying reasons are discussed. The theoretical predictions are also compared with prior theoretical predictions, with a related statistical model, and with the extant experimental data for the decomposition of CH3NO2, and for the reaction of CH3 with NO2. C1 [Annesley, Christopher J.; Randazzo, John B.; Klippenstein, Stephen J.; Harding, Lawrence B.; Georgievskii, Yuri; Ruscic, Branko; Tranter, Robert S.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Jasper, Ahren W.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. RP Klippenstein, SJ (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM sjk@anl.gov; Tranter@anl.gov RI Jasper, Ahren/A-5292-2011; Ruscic, Branko/A-8716-2008; OI Ruscic, Branko/0000-0002-4372-6990; Klippenstein, Stephen/0000-0001-6297-9187 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; United States Department of Energy [DE-AC04-94-AL85000]; Army Research Office as part of their Molecular Structure and Dynamics program [W911NF1310251]; [DE-AC02-06CH11357] FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences. The work at Argonne was supported under Contract No. DE-AC02-06CH11357. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy under Contract No. DE-AC04-94-AL85000. Support for S.J.K. was provided by the Army Research Office under Grant W911NF1310251 as part of their Molecular Structure and Dynamics program. NR 95 TC 7 Z9 7 U1 5 U2 27 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7872 EP 7893 DI 10.1021/acs.jpca.5b01563 PG 22 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600068 PM 25886024 ER PT J AU Shepard, R Brozell, SR Gidofalvi, G AF Shepard, Ron Brozell, Scott R. Gidofalvi, Gergely TI The Representation and Parametrization of Orthogonal Matrices SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID CONVERGENCE ACCELERATION; POLAR DECOMPOSITION; ALGORITHMS; OPTIMIZATION; PERTURBATION; COMPUTATION; ROTATIONS; COMPLEXES; DYNAMICS; ORBITALS AB Four representations and parametrizations of,orthogonal matt-ices Q is an element of R-mxn in terms of the minimal niimber of essential paraineters {phi} are discussed: the exponential representation, the Householder reflector representation, the Givens rotation representation, and the rational Cayley transform representation. Both square n = m and rectangular fr < m situations are considered. Two separate kinds of parametrizations are considered one in which the individual columns of :Q are distinct; the Stiefel manifold, and the other in which only span(Q) is significant, the Grossmann manifold. The practical issues of numerical stability, continuity, and uniqueness are discussed. The computation of Qin terms of the essential parameters {01, and also the extraction of {phi} for a given Q are Considered for all of the parametrizations. The transformation of gradient arrays between the Qand {phi} variables is discussed for all representations. It is out hope that developers of new methods will benefit from this comparative presentation of an important but rarely analyzed subject. C1 [Shepard, Ron; Brozell, Scott R.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Gidofalvi, Gergely] Gonzaga Univ, Dept Chem & Biochem, Spokane, WA 99258 USA. RP Shepard, R (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM shepard@tcg.anl.gov FU Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, U.S. Department of Energy [DEAC02-06CH11357]; Research Corporation for Science Advancement; Howard Hughes Medical Institute through the Undergraduate Science Education Program FX This work was supported by the Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, U.S. Department of Energy, under Contract DEAC02-06CH11357. S.R.B. acknowledges the use of computational facilities at the Ohio Supercomputer Center. G.G. was supported by an award from the Research Corporation for Science Advancement and a grant to Gonzaga University from the Howard Hughes Medical Institute through the Undergraduate Science Education Program. R.S. thanks J.B.H. and M. Minkoff for comments during the preparation of this manuscript. We also thank the anonymous referees for their helpful suggestions and for bringing several relevant references to our attention. NR 84 TC 0 Z9 0 U1 3 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 16 PY 2015 VL 119 IS 28 BP 7924 EP 7939 DI 10.1021/acs.jpca.5b02015 PG 16 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CN3PA UT WOS:000358337600071 PM 25946418 ER PT J AU Birn, J Liu, YH Daughton, W Hesse, M Schindler, K AF Birn, Joachim Liu, Yi-Hsin Daughton, William Hesse, Michael Schindler, Karl TI Reconnection and interchange instability in the near magnetotail SO EARTH PLANETS AND SPACE LA English DT Article DE Reconnection; Interchange; Magnetotail dynamics; Substorms ID MAGNETIC RECONNECTION; PLASMA SHEET; FLOW; CLUSTER AB This paper provides insights into the possible coupling between reconnection and interchange/ballooning in the magnetotail related to substorms and flow bursts. The results presented are largely based on recent simulations of magnetotail dynamics, exploring onset and progression of reconnection. 2.5-dimensional particle-in-cell (PIC) simulations with different tail deformation demonstrate a clear boundary between stable and unstable cases depending on the amount of deformation, explored up to the real proton/electron mass ratio. The evolution prior to onset, as well as the evolution of stable cases, are governed by the conservation of integral flux tube entropy S as imposed in ideal MHD, maintaining a monotonic increase with distance downtail. This suggests that ballooning instability in the tail should not be expected prior to the onset of tearing and reconnection. 3-D MHD simulations confirm this conclusion, showing no indication of ballooning prior to reconnection, if the initial state is ballooning stable. The simulation also shows that, after imposing resistivity necessary to initiate reconnection, the reconnection rate and energy release initially remain slow. However, when S becomes reduced from plasmoid ejection and lobe reconnection, forming a negative slope in S as a function of distance from Earth, the reconnection rate and energy release increase drastically. The latter condition has been shown to be necessary for ballooning/interchange instability, and the cross-tail structures that develop subsequently in the MHD simulation are consistent with such modes. The simulations support a concept in which tail activity is initiated by tearing instability but significantly enhanced by the interaction with ballooning/interchange enabled by plasmoid loss and lobe reconnection. C1 [Birn, Joachim] Space Sci Inst, Boulder, CO 80301 USA. [Birn, Joachim] Los Alamos Natl Lab, Los Alamos, NM USA. [Liu, Yi-Hsin; Hesse, Michael] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Daughton, William] Los Alamos Natl Lab, Los Alamos, NM USA. [Schindler, Karl] Ruhr Univ Bochum, Bochum, Germany. RP Birn, J (reprint author), Space Sci Inst, Boulder, CO 80301 USA. EM jbirn@spacescience.org RI Daughton, William/L-9661-2013; NASA MMS, Science Team/J-5393-2013 OI NASA MMS, Science Team/0000-0002-9504-5214 FU NSF's GEM program; NASA's MMS/SMART Theory and Modeling program; Heliophysics Theory Program; NSF [OCI 07-25070]; state of Illinois.; SRT Program FX Part of this work was performed at Los Alamos under the auspices of the US Department of Energy, supported by the NSF's GEM and by NASA's MMS/SMART Theory and Modeling, SR&T and Heliophysics Theory Programs. The simulations were performed using resources from the Los Alamos Institutional Computing Program, with further resources from the Blue Waters sustained-petascale computing project, which is supported by the NSF (OCI 07-25070) and the state of Illinois. NR 24 TC 1 Z9 1 U1 1 U2 10 PU SPRINGER HEIDELBERG PI HEIDELBERG PA TIERGARTENSTRASSE 17, D-69121 HEIDELBERG, GERMANY SN 1880-5981 J9 EARTH PLANETS SPACE JI Earth Planets Space PD JUL 16 PY 2015 VL 67 AR 110 DI 10.1186/s40623-015-0282-3 PG 9 WC Geosciences, Multidisciplinary SC Geology GA CN6SO UT WOS:000358564700001 ER PT J AU Wing, S Fairfield, DH Johnson, JR Ohtani, SI AF Wing, Simon Fairfield, Donald H. Johnson, Jay R. Ohtani, Shin-I. TI On the field-aligned electric field in the polar cap SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE polar cap; polar rain; field-aligned electric field; parallel electric potential; electron acceleration; monoenergetic electron ID MAGNETIC-FIELD; HIGH-LATITUDES; PLASMA SHEET; LOW-ALTITUDE; PRECIPITATION; ARCS; CURRENTS; DAYSIDE; REGIONS; CUSP AB The Johns Hopkins University Applied Physics Laboratory open-field line particle precipitation model predicts downward field-aligned electric field to maintain charge quasi-neutrality. Previous studies confirmed the existence of such electric fields. However, the present study shows that upward field-aligned electric field can be found within upward field-aligned current (FAC) region. In the upward FAC region, upward electric field that accelerates electron downward is seen with the occurrence rates of 82%-96%. In contrast, the occurrence rates in the downward FAC regions are 3%-11%. Polar rain electrons located in the upward FAC region adjacent to closed field lines often show a ramping up of energy with increasing latitude before reaching a plateau. This plateau may be attributed to the magnetosheath electrons that progressively have higher antisunward velocity and lower density with increasing distance from the subsolar point before they asymptotically reach the solar wind values. C1 [Wing, Simon; Ohtani, Shin-I.] Johns Hopkins Univ, Appl Phys Lab, Laurel, MD 20723 USA. [Fairfield, Donald H.] NASA, Goddard Space Flight Ctr, Space Weather Lab, Greenbelt, MD 20771 USA. [Johnson, Jay R.] Princeton Univ, Plasma Phys Lab, Princeton, NJ USA. RP Wing, S (reprint author), Johns Hopkins Univ, Appl Phys Lab, Johns Hopkins Rd, Laurel, MD 20723 USA. EM simon.wing@jhuapl.edu RI Ohtani, Shinichi/E-3914-2016 OI Ohtani, Shinichi/0000-0002-9565-6840 FU NSF [AGS-1058456, ATM0902730, AGS-1203299]; NASA [NNX13AE12G, NNX15AJ01G, NNH11AR07I, NNX14AM27G, NNH14AY20I]; DOE [DE-AC02-09CH11466] FX The Air Force Research Laboratory has been helpful in the acquisition of DMSP SSJ4/SSJ5 and magnetometer data, as has the World Data Center in Boulder, Colorado. NASA OMNIWeb Plus (http://omniweb.gsfc.nasa.gov/) provides the solar wind data. All the derived data products in this paper are available upon request by e-mail (simon.wing@jhuapl.edu). Simon Wing acknowledges support from NSF grant AGS-1058456 and NASA grants (NNX13AE12G and NNX15AJ01G). Jay R. Johnson acknowledges support from NASA grants (NNH11AR07I, NNX14AM27G, and NNH14AY20I), NSF grants (ATM0902730 and AGS-1203299), and DOE contract DE-AC02-09CH11466. NR 32 TC 3 Z9 3 U1 2 U2 7 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JUL 16 PY 2015 VL 42 IS 13 BP 5090 EP 5099 DI 10.1002/2015GL064229 PG 10 WC Geosciences, Multidisciplinary SC Geology GA CN8LG UT WOS:000358691300002 ER PT J AU Kim, EH Johnson, JR Valeo, E Phillips, CK AF Kim, Eun-Hwa Johnson, Jay R. Valeo, Ernest Phillips, Cynthia K. TI Global modeling of ULF waves at Mercury SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE Mercury; field line resonance; mode conversion; ULF waves; ion-ion hybrid resonance ID FIELD LINE RESONANCES; MESSENGERS 1ST FLYBY; ION-CYCLOTRON WAVES; MAGNETIC-FIELD; MULTICOMPONENT PLASMA; MAGNETOSPHERE; CONVERSION; FREQUENCY; ENVIRONMENT; SIMULATION AB ULF waves in the ion cyclotron frequency range waves are regularly observed at Mercury's magnetosphere. Although previous statistical studies have shown that ULF waves are primarily compressional near the equator and transverse with linear polarization at higher latitude, the underlying reason for this distribution of wave polarization has not been understood. In order to address this key question, we have developed a two-dimensional, finite element code that solves the full wave equations in global magnetospheric geometry. Using this code, we show that (1) efficient mode conversion from the fast compressional waves to the ion-ion hybrid resonance occurs at Mercury consistent with previous calculations; (2) such mode-converted waves globally oscillate similar to field line resonance at Earth; and (3) compressional wave energy is primarily localized near the equator, while field-aligned transverse, linearly polarized waves generated by mode conversion at the ion-ion hybrid resonance radiate to higher latitude. Based on these wave solutions, we suggest that the strong transverse component of observed ULF waves at Mercury in high magnetic latitude can be explained as excitation of the field line resonant waves at the ion-ion hybrid resonance. C1 [Kim, Eun-Hwa; Johnson, Jay R.] Princeton Univ, Princeton Ctr Heliophys, Princeton, NJ 08544 USA. [Kim, Eun-Hwa; Johnson, Jay R.; Valeo, Ernest; Phillips, Cynthia K.] Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. RP Kim, EH (reprint author), Princeton Univ, Princeton Ctr Heliophys, Princeton, NJ 08544 USA. EM ehkim@pppl.gov FU NASA [NNH09AK63I, NNH11AQ46I, NNH11AR071, NNX14AM27G, NNH14AY20I, NNX13XAE12G, NNX15AJ01G]; NSF [AGS1203299]; DOE [DE-AC02-09CH11466] FX The work at Princeton University was supported by NASA grants (NNH09AK63I, NNH11AQ46I, NNH11AR071, NNX14AM27G, NNH14AY20I, NNX13XAE12G, and NNX15AJ01G), NSF grant AGS1203299, and DOE contract DE-AC02-09CH11466. The United States Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The numerical data used in the figures may be obtained by contacting the corresponding author. NR 48 TC 5 Z9 5 U1 0 U2 5 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JUL 16 PY 2015 VL 42 IS 13 BP 5147 EP 5154 DI 10.1002/2015GL064531 PG 8 WC Geosciences, Multidisciplinary SC Geology GA CN8LG UT WOS:000358691300009 ER PT J AU Kim, K Fee, D Yokoo, A Lees, JM AF Kim, Keehoon Fee, David Yokoo, Akihiko Lees, Jonathan M. TI Acoustic source inversion to estimate volume flux from volcanic explosions SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE infrasound; waveform inversion; volcanology; FDTD modeling ID SOURCE PARAMETERS; SAKURAJIMA VOLCANO; FINITE-DIFFERENCE; INFRASOUND; ERUPTION; PROPAGATION; TOPOGRAPHY; SIMULATION; EQUATIONS; DYNAMICS AB We present an acoustic waveform inversion technique for infrasound data to estimate volume fluxes from volcanic eruptions. Previous inversion techniques have been limited by the use of a 1-D Green's function in a free space or half space, which depends only on the source-receiver distance and neglects volcanic topography. Our method exploits full 3-D Green's functions computed by a numerical method that takes into account realistic topographic scattering. We apply this method to vulcanian eruptions at Sakurajima Volcano, Japan. Our inversion results produce excellent waveform fits to field observations and demonstrate that full 3-D Green's functions are necessary for accurate volume flux inversion. Conventional inversions without consideration of topographic propagation effects may lead to large errors in the source parameter estimate. The presented inversion technique will substantially improve the accuracy of eruption source parameter estimation (cf. mass eruption rate) during volcanic eruptions and provide critical constraints for volcanic eruption dynamics and ash dispersal forecasting for aviation safety. Application of this approach to chemical and nuclear explosions will also provide valuable source information (e.g., the amount of energy released) previously unavailable. C1 [Kim, Keehoon; Fee, David] Univ Alaska Fairbanks, Inst Geophys, Alaska Volcano Observ, Wilson Infrasound Observ, Fairbanks, AK 99775 USA. [Yokoo, Akihiko] Kyoto Univ, Inst Geothermal Sci, Kumamoto, Japan. [Lees, Jonathan M.] Univ N Carolina, Dept Geol Sci, Chapel Hill, NC USA. RP Kim, K (reprint author), Lawrence Livermore Natl Lab, Geophys Monitoring Program, Livermore, CA 94551 USA. EM kkim32@alaska.edu RI Kim, Keehoon/J-8279-2015 OI Kim, Keehoon/0000-0002-8635-0428 FU National Science Foundation EAR [1331084]; Geophysical Institute of the University of Alaska Fairbanks FX The authors thank Sakurajima Volcano Observatory for their invaluable help including logistical support with the field experiment. We are grateful to Matthew Haney for constructive and helpful discussions. This work was made possible with financial support from National Science Foundation EAR grant 1331084 and the Geophysical Institute of the University of Alaska Fairbanks. The authors also thank Bernard Chouet and an anonymous reviewer for their helpful comments. NR 36 TC 3 Z9 3 U1 1 U2 9 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JUL 16 PY 2015 VL 42 IS 13 BP 5243 EP 5249 DI 10.1002/2015GL064466 PG 7 WC Geosciences, Multidisciplinary SC Geology GA CN8LG UT WOS:000358691300021 ER PT J AU Jimenez-Martinez, J de Anna, P Tabuteau, H Turuban, R Le Borgne, T Meheust, Y AF Jimenez-Martinez, Joaquin de Anna, Pietro Tabuteau, Herve Turuban, Regis Le Borgne, Tanguy Meheust, Yves TI Pore-scale mechanisms for the enhancement of mixing in unsaturated porous media and implications for chemical reactions SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE unsaturated porous media; mixing; chemical reactions ID STEADY-STATE FLOW; STOCHASTIC-ANALYSIS; SOLUTE TRANSPORT; HYDRODYNAMIC DISPERSION; HETEROGENEOUS MEDIA; VELOCITY COVARIANCE; WATER SATURATION; SAND; FLUX; SOIL AB Porous media in which different fluid phases coexist are common in nature (e.g., vadose zone and gas-oil reservoirs). In partially saturated porous media, the intricate spatial distributions of the wetting and nonwetting phases causes their flow to be focused onto preferential paths. Using a novel 2-D experimental setup allowing pore-scale measurement of concentration fields in a controlled unsaturated flow, we highlight mechanisms by which mixing of an invading fluid with the resident fluid is significantly enhanced when decreasing saturation. The mean scalar dissipation rate is observed to decrease slowly in time, while under saturated conditions it decays rapidly. This slow decrease is due to sustained longitudinal solute fingering, which causes concentration gradients to remain predominantly transverse to the average flow. Consequently, the effective reactivity is found to be much larger than under saturated conditions. These results provide new insights into the role that multiphase flows play on mixing/reaction in porous media. C1 [Jimenez-Martinez, Joaquin; Turuban, Regis; Le Borgne, Tanguy; Meheust, Yves] Univ Rennes 1, CNRS, Geosci Rennes, UMR 6118, Rennes, France. [de Anna, Pietro] MIT, Dept Civil & Environm Engn, Cambridge, MA 02139 USA. [Tabuteau, Herve] Univ Rennes 1, CNRS, UMR 6251, IPR, Rennes, France. RP Jimenez-Martinez, J (reprint author), Los Alamos Natl Lab, Los Alamos, NM USA. EM jjimenez@lanl.gov; yves.meheust@univ-rennes1.fr RI Jimenez-Martinez, Joaquin/B-9680-2013; Tabuteau, Herve/B-2153-2010; OI Jimenez-Martinez, Joaquin/0000-0002-2063-6490; Tabuteau, Herve/0000-0001-7878-9361; Meheust, Yves/0000-0003-1284-3251 FU Rennes-Metropole through an A.I.S.; INSU/CNRS through the EC2CO program [AO2014-906387]; Interreg project CLIMAWAT, EU-RDF INTERREG IVA France (Channel)-England program FX J.J.-M. expresses his gratitude to Fondation Rennes 1. Y.M. acknowledges support from Rennes-Metropole through an A.I.S. grant from equipment. The authors gratefully acknowledge support from INSU/CNRS through the EC2CO program, under project AO2014-906387. The experimental work was also supported by the Interreg project CLIMAWAT, EU-RDF INTERREG IVA France (Channel)-England program. NR 52 TC 8 Z9 8 U1 6 U2 31 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JUL 16 PY 2015 VL 42 IS 13 BP 5316 EP 5324 DI 10.1002/2015GL064513 PG 9 WC Geosciences, Multidisciplinary SC Geology GA CN8LG UT WOS:000358691300030 ER PT J AU Bi, XY Gao, ZQ Liu, YG Liu, F Song, QT Huang, J Huang, HJ Mao, WK Liu, CX AF Bi, Xueyan Gao, Zhiqiu Liu, Yangang Liu, Feng Song, Qingtao Huang, Jian Huang, Huijun Mao, Weikang Liu, Chunxia TI Observed drag coefficients in high winds in the near offshore of the South China Sea SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE drag coefficient; high winds; South China Sea ID TROPICAL CYCLONES; MOMENTUM FLUX; PART II; QUALITY-CONTROL; BOUNDARY-LAYER; SURFACE-LAYER; EXCHANGE; HURRICANES; BEHAVIOR; PROGRESS AB This paper investigates the relationships between friction velocity, 10m drag coefficient, and 10m wind speed using data collected at two offshore observation towers (one over the sea and the other on an island) from seven typhoon episodes in the South China Sea from 2008 to 2014. The two towers were placed in areas with different water depths along a shore-normal line. The depth of water at the tower over the sea averages about 15m, and the depth of water near the island is about 10m. The observed maximum 10min average wind speed at a height of 10m is about 32ms(-1). Momentum fluxes derived from three methods (eddy covariance, inertial dissipation, and flux profile) are compared. The momentum fluxes derived from the flux profile method are larger (smaller) over the sea (on the island) than those from the other two methods. The relationship between the 10m drag coefficient and the 10m wind speed is examined by use of the data obtained by the eddy covariance method. The drag coefficient first decreases with increasing 10m wind speed when the wind speeds are 5-10ms(-1), then increases and reaches a peak value of 0.002 around a wind speed of 18ms(-1). The drag coefficient decreases with increasing 10m wind speed when 10m wind speeds are 18-27ms(-1). A comparison of the measurements from the two towers shows that the 10m drag coefficient from the tower in 10m water depth is about 40% larger than that from the tower in 15m water depth when the 10m wind speed is less than 10ms(-1). Above this, the difference in the 10m drag coefficients of the two towers disappears. C1 [Bi, Xueyan; Gao, Zhiqiu] Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing, Peoples R China. [Bi, Xueyan; Huang, Jian; Huang, Huijun; Mao, Weikang; Liu, Chunxia] China Meteorol Adm, Guangzhou Inst Trop & Marine Meteorol, Guangdong Prov Key Lab Reg Numer Weather Predict, Guangzhou, Guangdong, Peoples R China. [Bi, Xueyan; Liu, Yangang] Brookhaven Natl Lab, Upton, NY 11973 USA. [Liu, Feng] Univ Illinois Urban Champaign, Prairie Res Inst, Div Illinois State Water Survey, Climate & Atmospher Sci Sect, Champaign, IL USA. [Song, Qingtao] Natl Satellite Ocean Applicat Serv, Beijing, Peoples R China. [Song, Qingtao] SOA, Key Lab Space Ocean Remote Sensing & Applicat, Beijing, Peoples R China. RP Gao, ZQ (reprint author), Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing, Peoples R China. EM zgao@mail.iap.ac.cn RI Liu, Yangang/H-6154-2011 FU National Natural Science Foundation of China [40906023, 41205011, 41475061, 41175013, 41076012, 41276019]; National Program on Key Basic Research Project of China (973) [2011CB403501]; U.S. DOE ESM via the FASTER project; U.S. DOE ESM via ASR program FX This work was supported by the National Natural Science Foundation of China under grants 40906023, 41205011, 41475061, 41175013, 41076012, and 41276019 and the National Program on Key Basic Research Project of China (973) under grant 2011CB403501. This work is also supported by the U.S. DOE ESM via the FASTER project (http://www.bnl.gov/esm/) and ASR program. The authors are particularly grateful to D. Richter and two anonymous reviewers for their careful reviews and valuable comments, which led to substantial improvement of this manuscript. We thank all the crew members who took part in the campaigns and collected the valuable data. The authors would like to also thank Zhiqun Shi and Wenchao Chen of the Guangdong Climate Centre for their help with the data on the tower on Zhizai Island. We thank our colleague, Zhongkuo Zhao for a lot of useful discussion and help in data processing. The data and code (in MATLAB formats) used in this paper can be obtained from the first author. NR 52 TC 1 Z9 2 U1 2 U2 17 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD JUL 16 PY 2015 VL 120 IS 13 BP 6444 EP 6459 DI 10.1002/2015JD023172 PG 16 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA CN8MN UT WOS:000358695200009 ER PT J AU Chen, Q Fan, JW Hagos, S Gustafson, WI Berg, LK AF Chen, Qian Fan, Jiwen Hagos, Samson Gustafson, William I., Jr. Berg, Larry K. TI Roles of wind shear at different vertical levels: Cloud system organization and properties SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE wind shear; convection organization; deep convection; cloud properties ID LIVED SQUALL LINES; MESOSCALE CONVECTIVE SYSTEMS; PART I; MODEL; MICROPHYSICS; SENSITIVITY; PARAMETERIZATION; TRANSPORT; MOMENTUM; PRECIPITATION AB Understanding critical processes that contribute to the organization of mesoscale convective systems (MCSs) is important for accurate weather forecasts and climate predictions. In this study, we investigate the effects of wind shear at different vertical levels on the organization and properties of convective systems using the Weather Research and Forecasting model with spectral bin microphysics. Based on a control run for a MCS with weak wind shear (Ctrl), we find that increasing wind shear at the lower troposphere (L-shear) leads to a more organized quasi-line convective system. Strong wind shear in the middle troposphere (M-shear) tends to produce large vorticity and form a mesocyclone circulation and an isolated strong storm that leans toward supercellular structure. By increasing wind shear at the upper vertical levels only (U-shear), the organization of the convection is not changed much, but the convective intensity is weakened. Increasing wind shear in the middle troposphere for the selected case results in a significant drying, and the drying is more significant when conserving moisture advection at the lateral boundaries, contributing to the suppressed convective strength and precipitation relative to Ctrl. Precipitation in the L-shear and U-shear does not change much from Ctrl. Evident changes of cloud macrophysical and microphysical properties in the strong wind shear cases are mainly due to large changes in convective organization and water vapor. The insights obtained from this study help us better understand the major factors contributing to convective organization and precipitation. C1 [Chen, Qian] Nanjing Univ Informat Sci & Technol, Collaborat Innovat Ctr Forecast & Evaluat Meteoro, Key Lab Aerosol Cloud Precipitat, China Meteorol Adm, Nanjing, Jiangsu, Peoples R China. [Chen, Qian; Fan, Jiwen; Hagos, Samson; Gustafson, William I., Jr.; Berg, Larry K.] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. RP Fan, JW (reprint author), Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. EM jiwen.fan@pnnl.gov RI Gustafson, William/A-7732-2008; Berg, Larry/A-7468-2016; Fan, Jiwen/E-9138-2011 OI Gustafson, William/0000-0001-9927-1393; Berg, Larry/0000-0002-3362-9492; FU U.S. Department of Energy (DOE) Atmospheric System Research (ASR) Program; DOE [DE-AC06-76RLO1830]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH1123]; National Science Foundation of China [41405126]; National Basic Research Program of China [2014CB441403]; Public Meteorology Special Foundation of Ministry of Science and Technology of China [GYHY201306047]; Priority Academic Program Development (PAPD) of Jiangsu Higher Education Institution; Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration [KDW1301]; U.S. DOE FX This study was supported by the U.S. Department of Energy (DOE) Atmospheric System Research (ASR) Program. The Pacific Northwest National Laboratory (PNNL) is operated for the DOE by Battelle Memorial Institute under contract DE-AC06-76RLO1830. This research used PNNL Institutional Computing resources and also resources at the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under contract DE-AC02-05CH1123. Qian Chen also acknowledges support from the National Science Foundation of China (grant 41405126), the National Basic Research Program of China (grant 2014CB441403), the Public Meteorology Special Foundation of Ministry of Science and Technology of China (grant GYHY201306047), the Priority Academic Program Development (PAPD) of Jiangsu Higher Education Institution and Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration (grant KDW1301). Gustafson acknowledges support from a U.S. DOE Early Career grant. The authors are grateful for helpful discussion with Heng Xiao at PNNL. The simulation data can be obtained by contacting the corresponding author, Dr. Jiwen Fan (Jiwe.Fan@pnnl.gov). NR 64 TC 0 Z9 0 U1 3 U2 9 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD JUL 16 PY 2015 VL 120 IS 13 BP 6551 EP 6574 DI 10.1002/2015JD023253 PG 24 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA CN8MN UT WOS:000358695200016 ER PT J AU Muhlbauer, A Ackerman, TP Lawson, RP Xie, S Zhang, Y AF Muhlbauer, A. Ackerman, T. P. Lawson, R. P. Xie, S. Zhang, Y. TI Evaluation of cloud-resolving model simulations of midlatitude cirrus with ARM and A-train observations SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE cirrus; cloud resolving model simulations ID NUMERICAL WEATHER PREDICTION; HETEROGENEOUS ICE NUCLEATION; RADIATION DRY BIAS; EMPIRICAL PARAMETERIZATION; HUMIDITY MEASUREMENTS; AIRCRAFT MEASUREMENTS; PROFILING RADAR; ANVIL CIRRUS; PART II; SCALE AB Cirrus clouds are ubiquitous in the upper troposphere and still constitute one of the largest uncertainties in climate predictions. This paper evaluates cloud-resolving model (CRM) and cloud system-resolving model (CSRM) simulations of a midlatitude cirrus case with comprehensive observations collected under the auspices of the Atmospheric Radiation Measurements (ARM) program and with spaceborne observations from the National Aeronautics and Space Administration A-train satellites. The CRM simulations are driven with periodic boundary conditions and ARM forcing data, whereas the CSRM simulations are driven by the ERA-Interim product. Vertical profiles of temperature, relative humidity, and wind speeds are reasonably well simulated by the CSRM and CRM, but there are remaining biases in the temperature, wind speeds, and relative humidity, which can be mitigated through nudging the model simulations toward the observed radiosonde profiles. Simulated vertical velocities are underestimated in all simulations except in the CRM simulations with grid spacings of 500m or finer, which suggests that turbulent vertical air motions in cirrus clouds need to be parameterized in general circulation models and in CSRM simulations with horizontal grid spacings on the order of 1km. The simulated ice water content and ice number concentrations agree with the observations in the CSRM but are underestimated in the CRM simulations. The underestimation of ice number concentrations is consistent with the overestimation of radar reflectivity in the CRM simulations and suggests that the model produces too many large ice particles especially toward the cloud base. Simulated cloud profiles are rather insensitive to perturbations in the initial conditions or the dimensionality of the model domain, but the treatment of the forcing data has a considerable effect on the outcome of the model simulations. Despite considerable progress in observations and microphysical parameterizations, simulating the microphysical, macrophysical, and radiative properties of cirrus remains challenging. Comparing model simulations with observations from multiple instruments and observational platforms is important for revealing model deficiencies and for providing rigorous benchmarks. However, there still is considerable need for reducing observational uncertainties and providing better observations especially for relative humidity and for the size distribution and chemical composition of aerosols in the upper troposphere. C1 [Muhlbauer, A.; Ackerman, T. P.] Univ Washington, Joint Inst Study Atmosphere & Ocean, Seattle, WA 98195 USA. [Ackerman, T. P.] Univ Washington, Dept Atmospher Sci, Seattle, WA 98195 USA. [Lawson, R. P.] SPEC Inc, Boulder, CO USA. [Xie, S.; Zhang, Y.] Lawrence Livermore Natl Lab, Livermore, CA USA. RP Muhlbauer, A (reprint author), Univ Washington, Joint Inst Study Atmosphere & Ocean, Seattle, WA 98195 USA. EM andreasm@atmos.washington.edu RI Zhang, Yunyan/F-9783-2011 FU University of Washington eScience Institute; National Science Foundation (NSF) [1144017]; Joint Institute for the Study of the Atmosphere and Ocean (JISAO) under NOAA [NA10OAR4320148, 2320]; Department of Energy (DOE) Atmospheric Radiation Measurements (ARM) program; DOE [DE-AC52-07NA27344] FX The first author thanks Hugh Morrison (NCAR) for providing the double-moment cloud microphysics code. This work is facilitated through the use of advanced computational, storage, and networking infrastructures provided by the Hyak supercomputer system, supported in part by the University of Washington eScience Institute. Andreas Muhlbauer and Thomas Ackerman acknowledge funding received from the National Science Foundation (NSF) under grant 1144017. This publication is partially funded by the Joint Institute for the Study of the Atmosphere and Ocean (JISAO) under NOAA Cooperative Agreement NA10OAR4320148, Contribution 2320. Work at Lawrence Livermore National Laboratory (LLNL) was supported by the Department of Energy (DOE) Atmospheric Radiation Measurements (ARM) program and performed under the auspices of the DOE by LLNL under contract DE-AC52-07NA27344. We greatly appreciate the effort of the SPARTICUS science team (Jay Mace, Thomas Ackerman, Jennifer Comstock, Tim Garrett, Eric Jensen, Xiaohong Liu, Greg McFarquhar, and David Mitchell) who devoted much of their time to make the SPARTICUS field campaign possible. The ARM data used in this study are available from the data archive of the ARM Climate Research Facility website at http://www.arm.gov. CloudSat data are available through the CloudSat data processing center at http://www.cloudsat.cira.colostate.edu. ERA-Interim data are available through the NCAR/CISL Research Data Archive at http://rda.ucar.edu. CERES satellite data are available at http://ceres.larc.nasa.gov. MODIS imagery is available through the NASA Earth Observing System Data and Information System at https://earthdata.nasa.gov. NR 85 TC 5 Z9 5 U1 4 U2 24 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD JUL 16 PY 2015 VL 120 IS 13 BP 6597 EP 6618 DI 10.1002/2014JD022570 PG 22 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA CN8MN UT WOS:000358695200018 ER PT J AU Cui, YY Brioude, J McKeen, SA Angevine, WM Kim, SW Frost, GJ Ahmadov, R Peischl, J Bousserez, N Liu, Z Ryerson, TB Wofsy, SC Santoni, GW Kort, EA Fischer, ML Trainer, M AF Cui, Yu Yan Brioude, Jerome McKeen, Stuart A. Angevine, Wayne M. Kim, Si-Wan Frost, Gregory J. Ahmadov, Ravan Peischl, Jeff Bousserez, Nicolas Liu, Zhen Ryerson, Thomas B. Wofsy, Steve C. Santoni, Gregory W. Kort, Eric A. Fischer, Marc L. Trainer, Michael TI Top-down estimate of methane emissions in California using a mesoscale inverse modeling technique: The South Coast Air Basin SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE methane; emission inventory; inverse modeling; Los Angeles ID NATURAL-GAS INFRASTRUCTURE; LOS-ANGELES BASIN; ANTHROPOGENIC EMISSIONS; QUALITY; SIMULATIONS; UNCERTAINTY; CAMPAIGN; CALNEX; TEXAS; NOX AB Methane (CH4) is the primary component of natural gas and has a larger global warming potential than CO2. Recent top-down studies based on observations showed CH4 emissions in California's South Coast Air Basin (SoCAB) were greater than those expected from population-apportioned bottom-up state inventories. In this study, we quantify CH4 emissions with an advanced mesoscale inverse modeling system at a resolution of 8kmx8km, using aircraft measurements in the SoCAB during the 2010 Nexus of Air Quality and Climate Change campaign to constrain the inversion. To simulate atmospheric transport, we use the FLEXible PARTicle-Weather Research and Forecasting (FLEXPART-WRF) Lagrangian particle dispersion model driven by three configurations of the Weather Research and Forecasting (WRF) mesoscale model. We determine surface fluxes of CH4 using a Bayesian least squares method in a four-dimensional inversion. Simulated CH4 concentrations with the posterior emission inventory achieve much better correlations with the measurements (R-2=0.7) than using the prior inventory (U.S. Environmental Protection Agency's National Emission Inventory 2005, R-2=0.5). The emission estimates for CH4 in the posterior, 46.39.2 Mg CH4/h, are consistent with published observation-based estimates. Changes in the spatial distribution of CH4 emissions in the SoCAB between the prior and posterior inventories are discussed. Missing or underestimated emissions from dairies, the oil/gas system, and landfills in the SoCAB seem to explain the differences between the prior and posterior inventories. We estimate that dairies contributed 5.91.7 Mg CH4/h and the two sectors of oil and gas industries (production and downstream) and landfills together contributed 39.68.1 Mg CH4/h in the SoCAB. C1 [Cui, Yu Yan; Brioude, Jerome; McKeen, Stuart A.; Angevine, Wayne M.; Kim, Si-Wan; Frost, Gregory J.; Ahmadov, Ravan; Peischl, Jeff; Ryerson, Thomas B.; Trainer, Michael] NOAA, Div Chem Sci, Earth Syst Res Lab, Boulder, CO 80305 USA. [Cui, Yu Yan; Brioude, Jerome; McKeen, Stuart A.; Angevine, Wayne M.; Kim, Si-Wan; Frost, Gregory J.; Ahmadov, Ravan; Peischl, Jeff] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. [Brioude, Jerome] CNRS Meteo France Univ La Reunion, Lab Atmosphere & Cyclones, UMR8105, St Denis, Reunion. [Bousserez, Nicolas] Univ Colorado, Dept Mech Engn, Boulder, CO 80309 USA. [Liu, Zhen] Sandia Natl Labs, Livermore, CA USA. [Wofsy, Steve C.; Santoni, Gregory W.] Harvard Univ, Dept Earth & Planetary Sci, Cambridge, MA 02138 USA. [Kort, Eric A.] Univ Michigan, Dept Atmospher Ocean & Space Sci, Ann Arbor, MI 48109 USA. [Fischer, Marc L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Brioude, J (reprint author), NOAA, Div Chem Sci, Earth Syst Res Lab, Boulder, CO 80305 USA. EM jerome.brioude@noaa.gov RI Kort, Eric/F-9942-2012; Ahmadov, Ravan/F-2036-2011; Angevine, Wayne/H-9849-2013; Brioude, Jerome/E-4629-2011; Peischl, Jeff/E-7454-2010; Liu, Zhen/C-3027-2011; Kim, Si-Wan/I-3979-2013; Frost, Gregory/I-1958-2013; Manager, CSD Publications/B-2789-2015; Trainer, Michael/H-5168-2013 OI Kort, Eric/0000-0003-4940-7541; Ahmadov, Ravan/0000-0002-6996-7071; Angevine, Wayne/0000-0002-8021-7116; Peischl, Jeff/0000-0002-9320-7101; Kim, Si-Wan/0000-0002-7889-189X; FU National Research Council Research Associateship Award; NOAA's Atmospheric Chemistry, Carbon Cycle, and Climate Program; California Energy Commission Public Interest Environmental Research Program [DE-AC02-05CH11231]; Laboratory Directed Research and Development program at Sandia National Laboratories; United States Department of Energy's National Nuclear Security Administration [DEAC04-94AL85000] FX FLEXPART-WRF model is available at the official FLEXPART website (http://flexpart.eu). NOAA P-3 observation data are available and can be downloaded at http://www.esrl.noaa.gov/csd/projects/calnex. The posterior emission inventory is available online as supporting information in NetCDF format. The lognormal Bayesian inverse software was developed at CSD/NOAA and CIRES. The WRF initial/boundary data were provided by NOAA/NCEP and NCAR. U.S. EPA NEI 2005 provided the prior emission data. We thank the High Performance Computing Program for their support in running FLEXPART-WRF. We thank Sandia National Laboratories who supported NG production and distribution data. The lead author would like to thank in particular the generous support of a National Research Council Research Associateship Award. This work was supported in part by NOAA's Atmospheric Chemistry, Carbon Cycle, and Climate Program. M.L.F. acknowledges support from the California Energy Commission Public Interest Environmental Research Program to LBNL under contract no. DE-AC02-05CH11231. Z.L. was supported under the Laboratory Directed Research and Development program at Sandia National Laboratories. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under contract DEAC04-94AL85000. Our thanks are given to the three anonymous reviewers who helped to substantially improve the quality of this paper. NR 42 TC 3 Z9 3 U1 3 U2 34 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD JUL 16 PY 2015 VL 120 IS 13 BP 6698 EP 6711 DI 10.1002/2014JD023002 PG 14 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA CN8MN UT WOS:000358695200024 ER PT J AU Cova, F Ronnebro, ECE Choi, YJ Gennari, FC Larochette, PA AF Cova, Federico Roennebro, Ewa C. E. Choi, Young Joon Gennari, Fabiana C. Arneodo Larochette, Pierre TI New Insights into the Thermodynamic Behavior of 2LiBH(4)-MgH2 Composite for Hydrogen Storage SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID LIBH4; HYDRIDE; REVERSIBILITY; BOROHYDRIDES; KINETICS; SORPTION; MG AB The composite 2LiBH(4):MgH2 has been studied as a potential hydrogen storage material due to its high storage capacity. The present work is aimed at clarifying the thermodynamic behavior of the system, especially within the temperature region above 400 degrees C. Different reaction paths which have important implication for storage applications during hydrogen absorption and desorption at vadous temperatures were revealed. At temperatures over 413 degrees C, two different absorption pressure plateaus are observed. This indicates that two different reactions occur: Mg hydrogenation at higher pressures and the re-formation of LiBH4 from H-2, LiH, and MgB2 at lower pressures. On the other hand, at temperatures below 413 degrees C only one plateau is present in the system. During desorption, the double plateau can be observed at temperatures as low as 375 degrees C. This effect restricts the applicability of this composite as a hydrogen storage material. C1 [Cova, Federico; Gennari, Fabiana C.; Arneodo Larochette, Pierre] Consejo Nacl Invest Cient & Tecn, Inst Balseiro, UNCuyo, San Carlos De Bariloche, Rio Negro, Argentina. [Cova, Federico; Gennari, Fabiana C.; Arneodo Larochette, Pierre] CNEA, Ctr Atom Bariloche, San Carlos De Bariloche, Rio Negro, Argentina. [Roennebro, Ewa C. E.; Choi, Young Joon] Pacific NW Natl Lab, Richland, WA 99352 USA. [Choi, Young Joon] Globalfoundries, Malta, NY 12020 USA. RP Cova, F (reprint author), Consejo Nacl Invest Cient & Tecn, Inst Balseiro, UNCuyo, R8402AGP, San Carlos De Bariloche, Rio Negro, Argentina. EM covaf@cab.cnea.gov.ar FU CONICET (National Council of Scientific and Technological Research); CNEA (National Commission of Atomic Energy); ANPCyT (PICT) [1052]; Instituto Balseiro (University of Cuyo); DOE EERE Hydrogen Fuel Cell Technology Office (FCTO) FX This study has been partially supported by CONICET (National Council of Scientific and Technological Research), CNEA (National Commission of Atomic Energy), ANPCyT (PICT No. 1052), and Instituto Balseiro (University of Cuyo). Part of this work was funded by DOE EERE Hydrogen Fuel Cell Technology Office (FCTO). NR 20 TC 4 Z9 4 U1 4 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 16 PY 2015 VL 119 IS 28 BP 15816 EP 15822 DI 10.1021/acs.jpcc.5b02047 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CN3PB UT WOS:000358337700004 ER PT J AU Haldoupis, E Borycz, J Shi, HL Vogiatzis, KD Bai, P Queen, WL Gagliardi, L Siepmann, JI AF Haldoupis, Emmanuel Borycz, Joshua Shi, Huiliang Vogiatzis, Konstantinos D. Bai, Peng Queen, Wendy L. Gagliardi, Laura Siepmann, J. Ilja TI Ab Initio Derived Force Fields for Predicting CO2 Adsorption and Accessibility of Metal Sites in the Metal-Organic Frameworks M-MOF-74 (M = Mn, Co, Ni, Cu) SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID CRYSTALLINE POROUS MATERIALS; CARBON-DIOXIDE ADSORPTION; UNITED-ATOM DESCRIPTION; PHASE-EQUILIBRIA; TRANSFERABLE POTENTIALS; BASIS-SETS; CAPTURE; SIMULATIONS; HYDROGEN; DESIGN AB Metal-organic frameworks (MOFs) are versatile nanoporous materials that have gained significant interest as low heat capacity, high selectivity sorbents for CO2 capture applications. Large-scale atomistic simulations for identifying high-performance MOFs are possible, but are limited to systems for which existing molecular mechanics force fields describe the interactions between the guest and framework atoms with sufficient accuracy. However, standard force fields are not applicable to cases involving coordinatively unsaturated metal centers that can strongly bind specific sorbate molecules. It has been previously shown that improved force fields can be derived from quantum mechanical calculations. In this work, we derived force fields for an isostructural series of MOFs, M-MOF-74, where M = Mn, Co, Ni, and Cu, from first principles. Monte Carlo calculations in the Gibbs ensemble were used to calculate the CO2 adsorption isotherms in order to assess the quality of the derived force field parameters and to determine a generally applicable procedure for obtaining a reliable force field for a targeted MOF and adsorbate system. The computed CO2 adsorption isotherms for the different M-MOF-74 members agree with experimental measurements at low loading and show that Ni-MOF-74 possesses the highest affinity toward CO2 and Cu-MOF-74 the weakest. In addition, we explored the source of open metal site and pore inaccessibility in these materials and quantified its impact on adsorption, especially the discrepancies often observed between experiments and simulations at high loadings. C1 [Haldoupis, Emmanuel; Borycz, Joshua; Shi, Huiliang; Vogiatzis, Konstantinos D.; Bai, Peng; Gagliardi, Laura; Siepmann, J. Ilja] Univ Minnesota, Dept Chem, Minneapolis, MN 55455 USA. [Haldoupis, Emmanuel; Borycz, Joshua; Shi, Huiliang; Vogiatzis, Konstantinos D.; Bai, Peng; Gagliardi, Laura; Siepmann, J. Ilja] Univ Minnesota, Chem Theory Ctr, Minneapolis, MN 55455 USA. [Haldoupis, Emmanuel; Borycz, Joshua; Shi, Huiliang; Vogiatzis, Konstantinos D.; Bai, Peng; Gagliardi, Laura; Siepmann, J. Ilja] Univ Minnesota, Supercomp Inst, Minneapolis, MN 55455 USA. [Shi, Huiliang; Bai, Peng; Siepmann, J. Ilja] Univ Minnesota, Dept Chem Engn & Mat Sci, Minneapolis, MN 55455 USA. [Queen, Wendy L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Queen, Wendy L.] Ecole Polytech Fed Lausanne, Inst Sci & Ingn Chim, ISIC Valais, CH-1950 Sion, Switzerland. RP Gagliardi, L (reprint author), Univ Minnesota, Dept Chem, 207 Pleasant St SE, Minneapolis, MN 55455 USA. EM gagliard@umn.edu; siepmann@umn.edu RI Foundry, Molecular/G-9968-2014; Bai, Peng/L-8516-2013 OI Bai, Peng/0000-0002-6881-4663 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences [DE-FG02-12ER16362] FX This research was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences under Award DE-FG02-12ER16362. The Minnesota Supercomputing Institute provided part of the computational resources for this work. NR 72 TC 13 Z9 13 U1 25 U2 213 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 16 PY 2015 VL 119 IS 28 BP 16058 EP 16071 DI 10.1021/acs.jpcc.5b03700 PG 14 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CN3PB UT WOS:000358337700032 ER PT J AU McBriarty, ME Campbell, GP Drake, TL Elam, JW Stair, PC Ellis, DE Bedzyk, MJ AF McBriarty, Martin E. Campbell, Gavin P. Drake, Tasha L. Elam, Jeffrey W. Stair, Peter C. Ellis, Donald E. Bedzyk, Michael J. TI Atomic-Scale View of VOx-WOx Coreduction on the alpha-Al2O3 (0001) Surface SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SELECTIVE CATALYTIC-REDUCTION; INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; RAY STANDING-WAVE; OXIDE CATALYSTS; TUNGSTEN-OXIDE; LAYER DEPOSITION; BASIS-SET; V-W; OXIDATION AB The catalytic activity of oxide-supported vanadium oxide is improved by the presence of tungsten oxide for the selective catalytic reduction of nitric oxides. We propose a mechanism for V-W synergy through studies of the reduction oxidation behavior of near-monolayer VOx and WOx species grown by atomic layer deposition on the alpha-Al2O3 (0001) single crystal surface. In situ X-ray standing wave measurements reveal an overlayer of W6+ species that is correlated with the substrate lattice as well as a redox-reversible shift from uncorrelated V5+ to correlated V4+. X-ray photoelectron spectroscopy and electronic structure calculations show a partial reduction of W6+ in the presence of V4+, improving the Bronsted acidity in mixed V-W catalyst systems. This mechanism of V-W synergy suggests that control of W d-states might be used as a design parameter for Bronssted acid in multiconponent oxide catalysts. C1 [McBriarty, Martin E.; Campbell, Gavin P.; Bedzyk, Michael J.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Drake, Tasha L.; Stair, Peter C.; Ellis, Donald E.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Ellis, Donald E.; Bedzyk, Michael J.] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [Elam, Jeffrey W.] Argonne Natl Lab, Energy Syst Div, Lemont, IL 60439 USA. [Stair, Peter C.] Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA. RP Bedzyk, MJ (reprint author), Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. EM bedzyk@northwestern.edu RI Bedzyk, Michael/B-7503-2009; OI McBriarty, Martin/0000-0002-7802-3267 FU National Science Foundation Graduate Research Fellowships [DGE-0824162, DGE-1324585]; Institute for Catalysis in Energy Processes (U.S. Department of Energy (DOE)) [DE-FG0203ER15457]; Northwestern University MRSEC (NSF) [DMR-1121262]; Institute for Atom-efficient Chemical Transformations (IACT), Energy Frontier Research Center - U.S. DOE Office of Basic Energy Sciences; Initiative for Sustainability and Energy at Northwestern University; E. I. duPont de Nemours Co.; Northwestern University; The Dow Chemical Co.; State of Illinois through the Department of Commerce and the Board of Education (HECA); Northwestern University MRSEC; U.S. DOE [DE-AC0206CH11357]; NSEC [NSF EEC-0647560]; MRSEC; Keck Foundation; Illinois FX M.E.M. and T.L.D. were supported by National Science Foundation Graduate Research Fellowships under Grants DGE-0824162 and DGE-1324585, respectively. M.E.M., T.L.D., P.C.S., D.E.E., and M.J.B. were supported in part by the Institute for Catalysis in Energy Processes (U.S. Department of Energy (DOE) under Contract DE-FG0203ER15457). G.P.C. was supported by the Northwestern University MRSEC (NSF Award DMR-1121262). J.W.E. was supported by the Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center funded by the U.S. DOE Office of Basic Energy Sciences. Additional support was provided by the Initiative for Sustainability and Energy at Northwestern University. Synchrotron X-ray measurements were performed at the Argonne National Laboratory (ANL) Advanced Photon Source, Sector 33 and Sector 5 (DND-CAT), which is supported by E. I. duPont de Nemours & Co., Northwestern University, The Dow Chemical Co., the State of Illinois through the Department of Commerce and the Board of Education (HECA), and the Northwestern University MRSEC. ANL is supported by the U.S. DOE under Contract DE-AC0206CH11357. AFM and XPS were performed at the NIFTI and Keck-II facilities of NUANCE Center at Northwestern University, supported by NSEC (NSF EEC-0647560), MRSEC, the Keck Foundation, the State of Illinois, and Northwestern University. We are grateful to Dr. D.T. Keane and Dr. Z. Zhang for assistance at the APS and to Dr. John Ciraldo from Rubicon Technologies, Inc., for providing sapphire substrates. NR 54 TC 2 Z9 2 U1 1 U2 28 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 16 PY 2015 VL 119 IS 28 BP 16179 EP 16187 DI 10.1021/acs.jpcc.5b04802 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CN3PB UT WOS:000358337700044 ER PT J AU Zhang, X Mu, S Chastanet, G Daro, N Palamarciuc, T Rosa, P Letard, JF Liu, J Sterbinsky, GE Arena, DA Etrillard, C Kundys, B Doudin, B Dowben, PA AF Zhang, Xin Mu, Sai Chastanet, Guillaume Daro, Nathalie Palamarciuc, Tatiana Rosa, Patrick Letard, Jean-Francois Liu, Jing Sterbinsky, George E. Arena, Dario A. Etrillard, Celine Kundys, Bohdan Doudin, Bernard Dowben, Peter A. TI Complexities in the Molecular Spin Crossover Transition SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID RAY-ABSORPTION-SPECTROSCOPY; MAGNETIC-PROPERTIES; SINGLE MOLECULES; ELECTRONIC-STRUCTURE; FE(II) COMPLEXES; METAL TRANSITION; ULTRATHIN FILMS; LIGHT; STATE; PRESSURE AB Variable-temperature studies of the electronic structures of four different Fe(II) spin crossover molecules, [Fe(H2B(pz)(2))(2)(bipy)] (pz = pyrazol-1-yl, bipy = 2,2'-bipyridine), [Fe(H2B(pz)(2))(2)(phen)], [Fe(phen)(2)(NCS)(2)] (phen = 9,10-phenantroline), and [Fe(PM-AzA)(2)(NCS)(2)] (PM-AzA = 4-phenyldiazenyl-N-(pyridin-2-ylmethylene)aniline) by X-ray absorption spectroscopy (XAS), combined with electrical properties studies of the [Fe(PM-AzA)(2)(NCS)(2)] single crystal are presented. We show that both the XAS signature of the spin state of powdered samples and the dielectric permittivity of the [Fe(PM-AzA)(2)(NCS)(2)] single crystal change at significantly lower temperatures than the magnetometry, structure, and resistivity indicators of a spin crossover transition. The changes in electronic structure are in agreement with the expectations from density functional theory (DFT) results for the different molecular electronic structures associated with the high-spin and low-spin states. These findings suggest that the electronic structure phase ordering process does not simply follow the spin transition. C1 [Zhang, Xin; Mu, Sai; Dowben, Peter A.] Univ Nebraska, Dept Phys & Astron, Lincoln, NE 68588 USA. [Chastanet, Guillaume; Daro, Nathalie; Palamarciuc, Tatiana; Rosa, Patrick; Letard, Jean-Francois] Univ Bordeaux, CNRS, ICMCB, UPR 9048, F-33600 Pessac, France. [Liu, Jing] Northeastern Univ, Dept Chem Engn, Boston, MA 02115 USA. [Liu, Jing; Sterbinsky, George E.; Arena, Dario A.] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. [Etrillard, Celine; Kundys, Bohdan; Doudin, Bernard] Univ Strasbourg, IPCMS, F-67034 Strasbourg, France. [Etrillard, Celine; Kundys, Bohdan; Doudin, Bernard] Univ Strasbourg, Lab Nanostruct Interact Environm NIE, UMR CNRS UdS 7504, F-67034 Strasbourg, France. RP Dowben, PA (reprint author), Univ Nebraska, Dept Phys & Astron, Lincoln, NE 68588 USA. EM pdowben@unl.edu RI mu, sai/D-1166-2015; Zhang, Xin/J-5478-2015; Liu, Jing/E-7184-2016; Doudin, Bernard/I-4758-2016 OI mu, sai/0000-0002-2608-8958; Zhang, Xin/0000-0001-9232-427X; Doudin, Bernard/0000-0002-0657-4780 FU National Science Foundation through the Nebraska MRSEC [DMR-1420645]; Agence Nationale de la Recherche [MULTISELF 11-BS08-06, Labex NIE 11-LABX-0058_NIE, ANR-10-IDEX-0002-02]; International Center for Frontier Research in Chemistry (icFRC, Strasbourg); U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX We acknowledge a number of helpful discussions with Jia Chen (Columbia University) and Axel Enders (Nebraska). This research was supported by the National Science Foundation through the Nebraska MRSEC (DMR-1420645). Partial financial support of the Agence Nationale de la Recherche (MULTISELF 11-BS08-06, Labex NIE 11-LABX-0058_NIE within the Investissement d'Avenir program ANR-10-IDEX-0002-02) and the International Center for Frontier Research in Chemistry (icFRC, Strasbourg) is also gratefully acknowledged. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under contract no. DE-AC02-98CH10886. A critical reading of the manuscript by Dr. Samir F. Matar (CNRS) is acknowledged. NR 71 TC 3 Z9 3 U1 1 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 16 PY 2015 VL 119 IS 28 BP 16293 EP 16302 DI 10.1021/acs.jpcc.5b02220 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CN3PB UT WOS:000358337700057 ER PT J AU Korkola, JE Collisson, EA Heiser, L Oates, C Bayani, N Itani, S Esch, A Thompson, W Griffith, OL Wang, NJ Kuo, WL Cooper, B Billig, J Ziyad, S Hung, JL Jakkula, L Feiler, H Lu, YL Mills, GB Spellman, PT Tomlin, C Mukherjee, S Gray, JW AF Korkola, James E. Collisson, Eric A. Heiser, Laura Oates, Chris Bayani, Nora Itani, Sleiman Esch, Amanda Thompson, Wallace Griffith, Obi L. Wang, Nicholas J. Kuo, Wen-Lin Cooper, Brian Billig, Jessica Ziyad, Safiyyah Hung, Jenny L. Jakkula, Lakshmi Feiler, Heidi Lu, Yiling Mills, Gordon B. Spellman, Paul T. Tomlin, Claire Mukherjee, Sach Gray, Joe W. TI Decoupling of the PI3K Pathway via Mutation Necessitates Combinatorial Treatment in HER2+Breast Cancer SO PLOS ONE LA English DT Article ID METASTATIC BREAST-CANCER; KINASE INHIBITOR; CELL-LINES; TRASTUZUMAB; LAPATINIB; THERAPY; CHEMOTHERAPY; ACTIVATION; RESISTANCE; PIK3CA AB We report here on experimental and theoretical efforts to determine how best to combine drugs that inhibit HER2 and AKT in HER2+ breast cancers. We accomplished this by measuring cellular and molecular responses to lapatinib and the AKT inhibitors (AKT(i)) GSK690693 and GSK2141795 in a panel of 22 HER2+ breast cancer cell lines carrying wild type or mutant PIK3CA. We observed that combinations of lapatinib plus AKTi were synergistic in HER2(+)/PIK3CA(mut) cell lines but not in HER2(+)/PIK3CA(wt)cell lines. We measured changes in phospho-protein levels in 15 cell lines after treatment with lapatinib, AKT(i) or lapatinib + AKT(i) to shed light on the underlying signaling dynamics. This revealed that pS6RP levels were less well attenuated by lapatinib in HER2(+)/PIK3CA(mut)cells compared to HER2(+)/PIK3CA(wt)cells and that lapatinib + AKT(i) reduced p-S6RP levels to those achieved in HER2(+)/PIK3CA(wt) cells with lapatinib alone. We also found that that compensatory upregulation of p-HER3 and p-HER2 is blunted in PIK3CA(mut) cells following lapatinib + AKT(i)-treatment. Responses of HER2(+) SKBR3 cells transfected with lentiviruses carrying control or PIK3CAmut sequences were similar to those observed in HER2(+)/PIK3CA(mut) cell lines but not in HER2(+)/PIK3CA(wt)cell lines. We used a nonlinear ordinary differential equation model to support the idea that PIK3CA mutations act as downstream activators of AKT that blunt lapatinib inhibition of downstream AKT signaling and that the effects of PIK3CA mutations can be countered by combining lapatinib with an AKT(i). This combination does not confer substantial benefit beyond lapatinib in HER2(+)/PIK3CA(wt) cells. C1 [Korkola, James E.; Heiser, Laura; Esch, Amanda; Thompson, Wallace; Wang, Nicholas J.; Feiler, Heidi; Spellman, Paul T.; Gray, Joe W.] Oregon Hlth & Sci Univ, Dept Biomed Engn, Portland, OR 97239 USA. [Bayani, Nora; Griffith, Obi L.; Kuo, Wen-Lin; Cooper, Brian; Billig, Jessica; Ziyad, Safiyyah; Hung, Jenny L.; Jakkula, Lakshmi; Feiler, Heidi] Lawrence Berkeley Natl Labs, Div Life Sci, Berkeley, CA USA. [Collisson, Eric A.] Univ Calif San Francisco, Div Heme Onc, San Francisco, CA 94143 USA. [Oates, Chris; Mukherjee, Sach] Netherlands Canc Inst, Div Biochem, Amsterdam, Netherlands. [Oates, Chris] Univ Warwick, Ctr Complex Sci, Coventry CV4 7AL, W Midlands, England. [Itani, Sleiman; Tomlin, Claire] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. [Lu, Yiling; Mills, Gordon B.] Univ Texas Houston, MD Anderson Canc Ctr, Dept Syst Biol, Houston, TX 77030 USA. RP Gray, JW (reprint author), Oregon Hlth & Sci Univ, Dept Biomed Engn, Portland, OR 97239 USA. EM grayjo@ohsu.edu OI Griffith, Obi/0000-0002-0843-4271 FU National Institutes of Health, National Cancer Institute [U54 CA 112970, U24 CA 126477, U01 CA164720]; OHSU Knight Cancer Institute [5P30CA069533-16]; Susan G. Komen Foundation [SAC110012]; Prospect Creek Foundation FX This work was supported by the National Institutes of Health, National Cancer Institute grants U54 CA 112970, the U24 CA 126477, the U01 CA164720, by the OHSU Knight Cancer Institute 5P30CA069533-16, by the Susan G. Komen Foundation SAC110012 and by the Prospect Creek Foundation. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 36 TC 1 Z9 1 U1 0 U2 1 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JUL 16 PY 2015 VL 10 IS 7 AR e0133219 DI 10.1371/journal.pone.0133219 PG 19 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CN1RQ UT WOS:000358198200057 PM 26181325 ER PT J AU Bera, MK Luo, GM Schlossman, ML Soderholm, L Lee, S Antonio, MR AF Bera, Mrinal K. Luo, Guangming Schlossman, Mark L. Soderholm, L. Lee, Sungsik Antonio, Mark R. TI Erbium(III) Coordination at the Surface of an Aqueous Electrolyte SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID X-RAY-ABSORPTION; AIR-WATER-INTERFACE; EARTH BASIC NITRATES; FINE-STRUCTURE; CHLORIDE COMPLEXES; K-EDGE; AIR/WATER INTERFACE; CRYSTAL-STRUCTURES; ION HYDRATION; BROMIDE ION AB Grazing-incidence (GI) X-ray absorption spectroscopy (XAS) under conditions of total external reflection is used to explore the coordination environment of the trivalent erbium ion, Er3+, at an electrolytevapor interface. A parallel study of the bulk aqueous electrolyte (1 M ErCl3 in HCl at pH = 1.54) shows that theEr(3+) ions have a simple hydration shell with an average ErOH2 bond distance of 2.33(1) angstrom, consistent with previous descriptions of the aquated cation, [Er(OH2)(8)](3+). No other correlations are observed in the electrolyte EXAFS (extended X-ray absorption fine structure) data acquired at room temperature. In contrast, the coordination of the Er3+ ions at the electrolytehelium interface, as interrogated by use of electron-yield detection, reveal correlations beyond the ErOH2 hydration shell that are unexpectedly well-defined. Analyses show an environment that consists of a first coordination sphere of 67 O atoms at 2.36(1) angstrom and a second one of 3 Cl atoms at 2.89(2) angstrom, suggesting the formation of a neutral [(H2O)(67)ErCl3] entity at the surface of the electrolyte. The presence of a third, distant peak in the Fourier transform data is attributed to ErEr correlations (in possible combination with contributions from distant ErO and ErCl interactions). The best-Z and -integer fits reveal 3 Er atoms at 3.20(2) angstrom, confirming the near-surface-enrichment of Er3+ as revealed previously by use of X-ray reflectivity measurements (J. Phys. Chem. C 2013, 117, 19082). Here, the strong associations between the Er-aqua-chloro entities at the electrolytevapor interface are shown to be consistent with the formation of domains of polynuclear cluster motifs, such as would arise through hydrolysis reactions of the aquated Er3+ cations. The local structural results and the calculated surface coverage are of relevance to understand the myriad reactions involved in the hydrometallurgical process of solvent extraction (SX) for metal purification, which involves the transfer of a selected metal ion, like Er, across an interface from an aqueous electrolyte to an organic phase. C1 [Bera, Mrinal K.; Luo, Guangming; Soderholm, L.; Antonio, Mark R.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Lee, Sungsik] Argonne Natl Lab, Adv Photon Source Xray Sci Div, Argonne, IL 60439 USA. [Schlossman, Mark L.] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. RP Antonio, MR (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM mantonio@anl.gov OI Antonio, Mark/0000-0002-1208-4534 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences [DE-AC02-06CH11357] FX This work and the use of the Advanced Photon Source are supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences, under Contract DE-AC02-06CH11357. NR 105 TC 3 Z9 3 U1 2 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JUL 16 PY 2015 VL 119 IS 28 BP 8734 EP 8745 DI 10.1021/acs.jpcb.5b02958 PG 12 WC Chemistry, Physical SC Chemistry GA CN3PC UT WOS:000358337800009 PM 25974706 ER PT J AU Chaudhari, MI Soniat, ML Rempe, SB AF Chaudhari, Mangesh I. Soniat, Marielle Rempe, Susan B. TI Octa-Coordination and the Aqueous Ba2+ Ion SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID INITIO MOLECULAR-DYNAMICS; QUASI-CHEMICAL THEORY; DENSITY-FUNCTIONAL THEORY; GENERALIZED GRADIENT APPROXIMATION; X-RAY-DIFFRACTION; AB-INITIO; K+ CHANNEL; POTASSIUM CHANNEL; FREE-ENERGY; SELECTIVITY FILTER AB The hydration structure of Ba2+ ion is important for understanding blocking mechanisms in potassium ion channels. Here, we combine statistical mechanical theory, ab initio molecular dynamics simulations, and electronic structure methods to calculate the hydration free energy and local hydration structure of Ba2+(aq). The predicted hydration free energy (-304 +/- 1 kcal/mol) agrees with the experimental value (-303 kcal/mol) when a maximally occupied, unimodal inner solvation shell is treated. In the local environment defined by the first shell of hydrating waters, Ba2+ is directly and stably coordinated by eight (8) waters. Octa-coordination resembles the crystal structure of Ba2+ and K+ bound in potassium ion channels, but differs from the local hydration structure of K+(aq) determined earlier. C1 [Chaudhari, Mangesh I.; Rempe, Susan B.] Sandia Natl Labs, Ctr Biol & Engn Sci, Albuquerque, NM 87185 USA. [Soniat, Marielle] Univ New Orleans, Dept Chem, New Orleans, LA 70148 USA. RP Rempe, SB (reprint author), Sandia Natl Labs, Ctr Biol & Engn Sci, POB 5800, Albuquerque, NM 87185 USA. EM slrempe@sandia.gov FU U.S. Department of Energy's (DOE) National Nuclear Security Administration [DE-AC04-94AL85000]; Sandia's LDRD program; State of Louisiana Board of Regents; U.S. DOE's Office of Science [DE-AC52-06NA25396]; SNL FX We thank Lawrence R. Pratt, Sameer Varma, and Dubravko Sabo for helpful discussions. Sandia National Laboratories (SNL) is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's (DOE) National Nuclear Security Administration under contract DE-AC04-94AL85000. This work was supported by Sandia's LDRD program (M.I.C. and S.B.R.) and the State of Louisiana Board of Regents (M.S.), and performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. DOE's Office of Science by Los Alamos National Laboratory (Contract DE-AC52-06NA25396) and SNL. NR 96 TC 5 Z9 5 U1 3 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JUL 16 PY 2015 VL 119 IS 28 BP 8746 EP 8753 DI 10.1021/acs.jpcb.5b03050 PG 8 WC Chemistry, Physical SC Chemistry GA CN3PC UT WOS:000358337800010 PM 26085171 ER PT J AU Ludwig, J An, L Pattengale, B Kong, QY Zhang, XY Xi, PX Huang, JE AF Ludwig, John An, Li Pattengale, Brian Kong, Qingyu Zhang, Xiaoyi Xi, Pinxian Huang, Jier TI Ultrafast Hole Trapping and Relaxation Dynamics in p-Type CuS Nanodisks SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID QUANTUM DOTS; SULFIDE NANOCRYSTALS; CARRIER DYNAMICS; ELECTRON; DEGRADATION; EVOLUTION; WATER; CU2S AB CuS nanocrystals are potential materials for developing low-cost solar energy conversion devices. Understanding the underlying dynamics of photoinduced carriers in CuS nanocrystals is essential to improve their performance in these devices. In this work, we investigated the photoinduced hole dynamics in CuS nanodisks (NDs) using the combination of transient optical (OTA) and X-ray (XTA) absorption spectroscopy. OTA results show that the broad transient absorption in the visible region is attributed to the photoinduced hot and trapped holes. The hole trapping process occurs on a subpicosecond time scale, followed by carrier recombination (similar to 100 ps). The nature of the hole trapping sites, revealed by XTA, is characteristic of S or organic ligands on the surface of CuS NDs. These results not only suggest the possibility to control the hole dynamics by tuning the surface chemistry of CuS but also represent the first time observation of hole dynamics in semiconductor nanocrystals using XTA. C1 [Ludwig, John; Pattengale, Brian; Huang, Jier] Marquette Univ, Dept Chem, Milwaukee, WI 53201 USA. [An, Li; Xi, Pinxian] Lanzhou Univ, State Key Lab Appl Organ Chem, Key Lab Nonferrous Met Chem & Resources Utilizat, Lanzhou 730000, Gansu, Peoples R China. [An, Li; Xi, Pinxian] Lanzhou Univ, Res Ctr Biomed Nanotechnol, Lanzhou 730000, Gansu, Peoples R China. [Kong, Qingyu; Zhang, Xiaoyi] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60349 USA. RP Zhang, XY (reprint author), Argonne Natl Lab, Xray Sci Div, Argonne, IL 60349 USA. EM xyzhang@aps.anl.gov; xipx@lzu.edu.cn; jier.huang@marquette.edu FU Marquette University; China NSFC [21201092, Lzujbky-2014-m02]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Chemical, Biological and Geological Sciences Program, Basic Energy Science, Office of Science of the U.S. Department of Energy [DE-FG02-06ER06-13] FX This work was supported by the Marquette University new faculty startup fund and China NSFC: 21201092 and Lzujbky-2014-m02. Use of the Advanced Photon Source and the Center for Nanoscale Materials at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award No. DE-AC02-06CH11357. The femtosecond laser used in the XTA measurements was funded by a Midscale Instrumentation grant (DE-FG02-06ER06-13) from the Chemical, Biological and Geological Sciences Program, Basic Energy Science, Office of Science of the U.S. Department of Energy. NR 28 TC 10 Z9 10 U1 8 U2 53 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JUL 16 PY 2015 VL 6 IS 14 BP 2671 EP 2675 DI 10.1021/acs.jpclett.5b01078 PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CN3PU UT WOS:000358339600003 PM 26266846 ER PT J AU Penwell, SB Ginsberg, LDS Ginsberg, NS AF Penwell, Samuel B. Ginsberg, Lucas D. S. Ginsberg, Naomi S. TI Bringing Far-Field Subdiffraction Optical Imaging to Electronically Coupled Optoelectronic Molecular Materials Using Their Endogenous Chromophores SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID STIMULATED-EMISSION DEPLETION; EXCITON DIFFUSION LENGTH; POLYMER MEH-PPV; STED MICROSCOPY; QUANTUM DOTS; 2-PHOTON EXCITATION; SINGLE-WAVELENGTH; DIFFRACTION-LIMIT; GENE-EXPRESSION; ENERGY-TRANSFER AB We demonstrate that subdiffraction resolution can be achieved in fluorescence imaging of functional materials with densely packed, endogenous, electronically coupled chromophores by modifying stimulated emission depletion (STED) microscopy. This class of chromophores is not generally compatible with STED imaging due to strong two-photon absorption cross sections. Yet, we achieve 90 nm resolution and high contrast in images of clusters of conjugated polymer polyphenylenevinylene-derivative nanoparticles by modulating the excitation intensity in the material. This newfound capability has the potential to significantly broaden the range of fluorophores that can be employed in super-resolution fluorescence imaging. Moreover, solution-processed optoelectronics and photosynthetic or other naturally luminescent biomaterials exhibit complex energy and charge transport characteristics and luminescence variations in response to nanoscale heterogeneity in their complex, physical structures. Our discovery will furthermore transform the current understanding of these materials' structure function relationships that have until now made them notoriously challenging to characterize on their native, subdiffraction scales. C1 [Penwell, Samuel B.; Ginsberg, Lucas D. S.; Ginsberg, Naomi S.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Ginsberg, Naomi S.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Ginsberg, Naomi S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci, Berkeley, CA 94720 USA. [Ginsberg, Naomi S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. [Ginsberg, Naomi S.] Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. RP Ginsberg, NS (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM nsginsberg@berkeley.edu FU David and Lucile Packard Fellowship for Science and Engineering; Dow Chemical Company [244699]; Department of Energy [DE-AC05-060R23100] FX This work has been supported by a David and Lucile Packard Fellowship for Science and Engineering to N.S.G. and by The Dow Chemical Company under contract #244699. We thank A. Tosi and M. Buttafava of SPAD lab, Politecnico di Milano, for discussions and the generous trial of the fast-gated SPAD and N. Bertone and PicoQuant GmbH for providing a demo of the HydraHarp400 photon counting apparatus. We thank D. M. Neumark for the use of a grating stretcher. S.B.P. acknowledges a Department of Energy Graduate Research Fellowship (contract no. DE-AC05-060R23100) and N.S.G. acknowledges an Alfred P. Sloan Research Fellowship. NR 54 TC 2 Z9 2 U1 2 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JUL 16 PY 2015 VL 6 IS 14 BP 2767 EP 2772 DI 10.1021/acs.jpclett.5b01200 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CN3PU UT WOS:000358339600020 PM 26266861 ER PT J AU Aad, G Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaitia, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TP Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Auerbach, B Augsten, K Aurousseau, M Avolio, G Axen, B Azuelos, G Azuma, Y Baak, MA Baas, AE Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Balek, P Balli, F Banas, E Banerjee, S Bannoura, AAE Bansil, HS Barak, L Baranov, SP Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F Da Costa, JBG Bartoldus, R Barton, AE Bartos, P Bartsch, V Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Battistin, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Becot, C Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, K Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boddy, CR Boehler, M Boek, TT Bogaerts, JA Bogdanchikov, AG Bogouch, A Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boterenbrood, H Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutouil, S Boveia, A Boyd, J Boyko, IR Bozic, I Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brelier, B Brendlinger, K Brennan, AJ Brenner, R Bressler, S Bristow, K Bristow, TM Britton, D Brochu, FM Brock, I Brock, R Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Brunet, S Bruni, A Bruni, G Bruschi, M Bryngemark, L Buanes, T Buat, Q Bucci, F Buchholz, P Buckley, AG Buda, SI Budagov, IA Buehrer, F Bugge, L Bugge, MK Bulekov, O Bundock, AC Burckhart, H Burdin, S Burghgrave, B Burke, S Burmeister, I Busato, E Buescher, D Buescher, V Bussey, P Buszello, CP Butler, B Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Byszewski, M Urban, SC Caforio, D Cakir, O Calafiura, P Calandri, A Calderini, G Calfayan, P Caloba, LP Calvet, D Calvet, S Toro, RC Camarda, S Cameron, D Caminada, LM Armadans, RC Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Cardarelli, R Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Cattani, G Caudron, J Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, BC Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chang, P Chapleau, B Chapman, JD Charfeddine, D Charlton, DG Chau, CC Barajas, CAC Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A Cheremushkina, E El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiefari, G Childers, JT Chilingarov, A Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Chouridou, S Chow, BKB Chromek-Burckhart, D Chu, ML Chudoba, J Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Ciftci, R Cinca, D Cindro, V Ciocio, A Citron, ZH Citterio, M Ciubancan, M Clark, A Clark, PJ Clarke, RN Cleland, W Clemens, JC Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Cogan, JG Cole, B Cole, S Colijn, AP Collot, J Colombo, T Compostella, G Muino, PC Coniavitis, E Connell, SH Connelly, IA Consonni, SM Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cooper-Smith, NJ Copic, K Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cote, D Cottin, G Cowan, G Cox, BE Cranmer, K Cree, G Crepe-Renaudin, S Crescioli, F Cribbs, WA Ortuzar, MC Cristinziani, M Croft, V Crosettia, G Donszelmann, TC Cummings, J Curatolo, M Cuthbert, C Czirr, H Czodrowski, P D'Auria, S D'Onofrio, M De Sousaa, MJDCS Da Via, C Dabrowskia, W Dafinca, A Dai, T Dale, O Dallaire, F Dallapiccola, C Dam, M Daniells, AC Danninger, M Hoffmann, MD Dao, V Darboa, G Darmora, S Dassoulas, J Dattagupta, A Davey, W David, C Davidek, T Davies, E Davies, M Davignon, O Davison, AR Davison, P Davygoraa, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K De Asmundisa, R De Castroa, S De Cecco, S De Groot, N De Jong, P De la Torre, H De Lorenzi, F De Nooij, L De Pedisa, D De Salvoa, A De Sanctis, U De Santo, A De Regie, JBDV Dearnaley, WJ Debbe, R Debenedetti, C Dechenaux, B Dedovich, DV Deigaard, I Del Peso, J Del Prete, T Deliot, F Delitzsch, CM Deliyergiyev, M Dell'Acqua, A Dell'Asta, L Dell'Orso, M Della Pietra, M Della Volpe, D Delmastro, M Delsart, PA Deluca, C DeMarco, DA Demers, S Demichev, M Demilly, A Denisov, SP Derendarz, D DerkaouiD, JE Derue, F Dervan, P Desch, K Deterre, C Deviveiros, PO Dewhurst, A Dhaliwal, S Di Ciaccio, A Di Ciaccio, L Di Domenico, A Di DonatoA, C Di Girolamo, A Di Girolamo, B Di Mattia, A Di Micco, B Di Nardo, R Di Simone, A Sipio, R Di Valentino, D Dias, FA Diaza, MA Diehl, EB Dietrich, J Dietzsch, TA Diglio, S Dimitrievska, A Dingfelder, J Ditaa, P Ditaa, S Dittus, F Djama, F Djobava, T Djuvsland, JI Do Valec, MAB Dobos, D Doglioni, C Doherty, T Dohmae, T Dolejsi, J Dolezal, Z Dolgoshein, BA Donadelli, M Donati, S Dondero, P Donini, J Dopke, J Doria, A Dova, MT Doyle, AT Dris, M Dubbert, J Dube, S Dubreuil, E Duchovni, E Duckeck, G Ducua, OA Duda, D Dudarev, A Dudziak, F Duflot, L Duguid, L Duehrssen, M Dunford, M Yildiz, HD Dueren, M Durglishvili, A Duschinger, D Dwuznik, M Dyndal, M Edson, W Edwards, NC Ehrenfeld, W Eifert, T Eigen, G Einsweiler, K Ekelof, T El Kacimi, M Ellert, M Elles, S Ellinghaus, F Elliot, AA Ellis, N Elmsheuser, J Elsing, M Emeliyanov, D Enari, Y Endner, OC Endo, M Engelmann, R Erdmann, J Ereditato, A Eriksson, D Ernis, G Ernst, J Ernst, M Ernwein, J Errede, S Ertel, E Escalier, M Esch, H Escobar, C Esposito, B Etienvre, AI Etzion, E Evans, H Ezhilov, A Fabbri, L Facini, G Fakhrutdinov, RM Falciano, S Falla, RJ Faltova, J Fanga, Y Fanti, M Farbin, A Farilla, A Farooque, T Farrell, S Farrington, SM Farthouat, P Fassi, F Fassnacht, P Fassouliotis, D Favareto, A Fayard, L Federic, P Fedin, OL Fedorko, W Feigl, S Feligioni, L Fengd, C Feng, EJ Feng, H Fenyuk, AB Martinez, PF Perez, SF Ferrag, S Ferrando, J Ferrari, A Ferrari, P Ferrari, R de Lima, DEF Ferrer, A Ferrere, D Ferretti, C Parodi, AF Fiascaris, M Fiedler, F Filipcic, A Filipuzzi, M Filthaut, F Fincke-Keeler, M Finelli, KD Fiolhais, MCN Fiorini, L Firan, A Fischer, A Fischer, J Fisher, WC Fitzgerald, EA Flechl, M Fleck, I Fleischmann, P Fleischmann, S Fletcher, GT Fletcher, G Flick, T Floderus, A Castillo, LRF Flowerdew, MJ Formica, A Forti, A Fournier, D Fox, H Fracchia, S Francavilla, P Franchini, M Franchino, S Francis, D Franconi, L Franklin, M Fraternali, M French, ST Friedrich, C Friedrich, F Froidevaux, D Frost, JA Fukunaga, C Torregrosa, EF Fulsom, BG Fuster, J Gabaldon, C Gabizon, O Gabriellia, A Gabriellia, A Gadatsch, S Gadomski, S Gagliardia, G Gagnon, P Galea, C Galhardoa, B Gallas, EJ Gallop, BJ Gallus, P Galster, G Gan, KK Gaob, J Gao, YS Walls, FMG Garberson, F Garcia, C Navarro, JEG Garcia-Sciveres, M Gardner, RW Garelli, N Garonne, V Gatti, C Gaudio, G Gaur, B Gauthier, L Gauzzi, P Gavrilenko, IL Gay, C Gaycken, G Gazis, 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CA ATLAS Collaboration TI Observation and measurement of Higgs boson decays to WW* with the ATLAS detector SO PHYSICAL REVIEW D LA English DT Article ID HADRON COLLIDERS; STANDARD MODEL; PARTON DISTRIBUTIONS; MASSLESS PARTICLES; BROKEN SYMMETRIES; NNLO QCD; LHC; SEARCH; COLLISIONS; PROGRAM AB We report the observation of Higgs boson decays to WW* based on an excess over background of 6.1 standard deviations in the dilepton final state, where the Standard Model expectation is 5.8 standard deviations. Evidence for the vector-boson fusion (VBF) production process is obtained with a significance of 3.2 standard deviations. The results are obtained from a data sample corresponding to an integrated luminosity of 25 fb(-1) from root s = 7 and 8 TeV pp collisions recorded by the ATLAS detector at the LHC. For a Higgs boson mass of 125.36 GeV, the ratio of the measured value to the expected value of the total production cross section times branching fraction is 1.09(-0.15)(+0.16)(stat)(-0.14)(+0.17)(syst). The corresponding ratios for the gluon fusion and vector-boson fusion production mechanisms are 1.02 +/- 0.19(stat)(-0.18)(+0.22)(syst) and 1.27(-0.40)(+0.44)(stat)(-0.21)(+0.30)(syst), respectively. At root s = 8 TeV, the total production cross sections are measured to be sigma(gg -> H -> WW*) = 4.6 +/- 0.9(stat)(-0.7)(+0.8)(syst) pb and sigma(VBF H -> WW*) = 0.51(-0.15)(+0.17)(stat)(-0.08)(+0.13)(syst) pb. The fiducial cross section is determined for the gluon-fusion process in exclusive final states with zero or one associated jet. C1 [Jackson, P.; Lee, L.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. 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R.; Usai, G.; Vartapetian, A.; White, A.; Wingerter-Seez, I.; Yu, J.] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA. [Angelidakis, S.; Chouridou, S.; Fassouliotis, D.; Giokaris, N.; Ioannou, P.; Iordanidou, K.; Kourkoumelis, C.; Manousakis-Katsikakis, A.; Tsirintanis, N.] Univ Athens, Dept Phys, Athens, Greece. [Alexopoulos, T.; Byszewski, M.; Dris, M.; Gazis, E. N.; Iakovidis, G.; Karakostas, K.; Karastathis, N.; Leontsinis, S.; Maltezos, S.; Ntekas, K.; Panagiotopoulou, E.; Papadopoulou, Th. D.; Tsipolitis, G.; Vlachos, S.] Natl Tech Univ Athens, Dept Phys, Zografos, Greece. [Abdinov, O.; Khalil-Zada, F.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Anjos, N.; Bosman, M.; Armadans, R. Caminal; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fracchia, S.; Giangiobbe, V.; Parra, G. Gonzalez; Grinstein, S.; Rozas, A. Juste; Korolkov, I.; Le Menedeu, E.; Paz, I. Lopez; Martinez, M.; Mir, L. M.; Berlingen, J. Montejo; Pages, A. Pacheco; Aranda, C. Padilla; Riu, I.; Rubbo, F.; Sorin, V.; Succurro, A.; Tripiana, M. F.; Tsiskaridze, S.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Anjos, N.; Bosman, M.; Armadans, R. Caminal; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fracchia, S.; Giangiobbe, V.; Parra, G. Gonzalez; Grinstein, S.; Rozas, A. Juste; Korolkov, I.; Le Menedeu, E.; Paz, I. Lopez; Martinez, M.; Mir, L. M.; Berlingen, J. Montejo; Pages, A. Pacheco; Aranda, C. Padilla; Riu, I.; Rubbo, F.; Sorin, V.; Succurro, A.; Tripiana, M. F.; Tsiskaridze, S.] Univ Autonoma Barcelona, Dept Fis, E-08193 Barcelona, Spain. [Agatonovic-Jovin, T.; Bozic, I.; Dimitrievska, A.; Krstica, J.; Marjanovica, M.; Popovica, D. S.; Sijackia, Dj.; Simica, Lj.; Milosavljevica, M. Vranjes] Univ Belgrade, Inst Phys, Belgrade, Serbia. [Mamuzicb, J.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Buanes, T.; Dale, O.; Eigen, G.; Kastanas, A.; Liebig, W.; Lipniacka, A.; Latour, B. Martin Dit; Rosendahl, P. L.; Sandaker, H.; Sjursen, T. B.; Smestad, L.; Stugu, B.; Ugland, M.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Axen, B.; Barnett, R. M.; Beringer, J.; Brandt, G.; Brosamer, J.; Calafiura, P.; Caminada, L. M.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Dube, S.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Hurwitz, M.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Virzi, J.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Axen, B.; Barnett, R. M.; Beringer, J.; Brandt, G.; Brosamer, J.; Calafiura, P.; Caminada, L. M.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Dube, S.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Hurwitz, M.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Virzi, J.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Dietrich, J.; Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Herrberg-Schubert, R.; Hristova, I.; Kind, O.; Kolanoski, H.; Lacker, H.; Lohse, T.; Nikiforov, A.; Rehnisch, L.; Rieck, P.; Schulz, H.; Stamm, S.; Wendland, D.; Nedden, M. Zur] Humboldt Univ, Dept Phys, Berlin, Germany. [Agustoni, M.; Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Schneider, B.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Agustoni, M.; Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Schneider, B.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allbrooke, B. M. M.; Bella, L. Aperio; Bansil, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Palmer, J. D.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istina, S.; Ozcana, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Phys Engn, Gaziantep, Turkey. [Alberghi, G. L.; Bellagamba, L.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Caforio, D.; Corradi, M.; De Castroa, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Gabriellia, A.; Giacobbea, B.; Giorgia, F. M.; Grafstroma, P.; Manghia, F. Lasagni; Massaa, I.; Massaa, L.; Mengarellia, A.; Negrinia, M.; Polinia, A.; Rinaldia, L.; Romanoa, M.; Sbarraa, C.; Sbrizzia, A.; Semprini-Cesaria, N.; Spighia, R.; Tupputia, S. A.; Valentinettia, S.; Villaa, M.; Zoccolia, A.] INFN Sez Bologna, Bologna, Italy. [Alberghi, G. L.; Caforio, D.; De Castroa, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Gabriellia, A.; Grafstroma, P.; Manghia, F. Lasagni; Massaa, I.; Massaa, L.; Mengarellia, A.; Piccininia, M.; Romanoa, M.; Sbrizzia, A.; Tupputia, S. A.; Valentinettia, S.; Villaa, M.; Zoccolia, A.] Univ Bologna, Dipartmento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Hagebock, S.; Hellmich, D.; Huegging, F.; Janssen, J.; Khoriauli, G.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mergelmeyer, S.; Mijovic, L.; Mueller, K.; Nanava, G.; Nattermann, T.; Obermann, T.; Pohl, D.; Sarrazin, B.; Schaepe, S.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Seema, P.; Stillings, J. A.; Tannoury, N.; Therhaag, J.; Uhlenbrock, M.; Velz, T.; Vogel, A.; Von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Fitzgerald, E. A.; Sciolla, G.; Venturini, A.; Zambito, S.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchika, C.; Marroquima, F.; Nepomucenoa, A. A.; Seixasa, J. M.] Univ Fed Rio de Janeiro, COPPE, EE, IF, BR-21945 Rio De Janeiro, Brazil. [Cerqueira, A. S.; Filhob, L. Manhaes De Andrade] Univ Fed Juiz de Fora, Elect Circuits Dept, Juiz de Fora, Brazil. [Do Valec, M. A. B.] Univ Fed Sao Joao del Rei, Sao Joao del Rei, Brazil. [Donadelli, M.; Leited, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Schovancova, J.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Ditaa, P.; Ditaa, S.; Ducua, O. A.; Jinarua, A.; Maurera, J.; Olariua, A.; Pantea, D.; Rotarua, M.; Stoiceaa, G.; Tudorachea, A.; Tudorachea, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciub, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Garzon, G. Otero Y.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.; Yusuf, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; Marchand, J. F.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Psztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Battistin, M.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Fernandez Perez, S.; Franchino, S.; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jakobsen, S.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Martin, B.; Marzin, A.; Messina, A.; Meyer, J.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; Van der Ster, D.; Van Eldik, N.; Van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Cheng, Y.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Krizka, K.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Tompkins, L.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaza, M. A.; Vogela, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshovb, S.; Pezoab, R.; Prokoshinb, F.; Whiteb, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fanga, Y.; Jina, S.; Loua, X.; Lua, F.; Ouyanga, Q.; Rena, H.; Shana, L. Y.; Suna, X.; Wanga, J.; Xu, D.; Yaoa, L.; Zhua, H.; Zhuanga, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gaob, J.; Guanb, L.; Hanb, L.; Jiangb, Y.; Lib, B.; Liub, J. B.; Liub, K.; Liub, M.; Liub, Y.; Pengb, H.; Songb, H. Y.; Xu, L.; Zhang, R.; Zhao, Z.; Zhub, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Lic, Y.; Wangc, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Fengd, C.; Ge, P.; Mad, L. L.; Zhang, X.; Zhao, Y.; Zhud, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Lie, L.; Yange, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Podlyski, F.; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Podlyski, F.; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Podlyski, F.; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] IN2P3, CNRS, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Guo, J.; Hu, D.; Hughes, E. W.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosettia, G.; La Rotondaa, L.; Mastroberardinoa, A.; Policicchioa, A.; Salvatorea, D.; Scarfonea, V.; Schioppaa, M.; Susinnoa, G.; Tassia, E.] Ist Nazl Fis Nucl, Grp Coll Cosenza, Lab Nazl Frascati, Cosenza, Italy. [Capua, M.; Crosettia, G.; La Rotondaa, L.; Mastroberardinoa, A.; Policicchioa, A.; Salvatorea, D.; Scarfonea, V.; Schioppaa, M.; Susinnoa, G.; Tassia, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowskia, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bolda, I.; Kisielewskaa, D.; Kopernya, S.; Kowalskia, T. Z.; Mindura, B.; Przybyciena, M.; Zeml, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palkab, M.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Phys Dept, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Camarda, S.; Deterre, C.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Monig, K.; Morton, A.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Camarda, S.; Deterre, C.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Monig, K.; Morton, A.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Gossling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Wang, C.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dao, V.; Di Simone, A.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Madar, R.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ronzani, M.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; Von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; Della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nektarijevic, S.; Nikolics, K.; Picazio, A.; Pohl, M.; Rosbach, K.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darboa, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardia, G.; Gemmea, C.; Guidoa, E.; Morettinia, P.; Osculatia, B.; Parodia, F.; Passaggioa, S.; Rossia, L. P.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardia, G.; Guidoa, E.; Osculatia, B.; Parodia, F.; Schiavia, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelavaa, J.; Tskhadadzea, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubuab, J.; Mosidzeb, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Bindi, M.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Keil, M.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llcer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Phys Inst 2, D-37073 Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlanea, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Da Costa, J. Barreiro Guimaraes; Butler, B.; Catastini, P.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.; Della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygoraa, Y.; Dietzsch, T. A.; Djuvsland, J. I.; Dunford, M.; Hankea, P.; Jongmannsa, J.; Khomicha, A.; Klugea, E. -E.; Laiera, H.; Langa, V. S.; Meiera, K.; Muellera, F.; Poddara, S.; Scharfa, V.; Schultz-Coulona, H. -C.; Stamena, R.; Wesselsa, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulinib, M.; Kasieczkab, G.; Narayanb, R.; Schaetzelb, S.; Schmittb, S.; Schoeningb, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretzc, M.; Kugelc, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Prokofievc, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. Univ Innsbruck, Inst Astro & Teilchenphys, A-6020 Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Morange, N.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Topilin, N. D.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorinia, E.; Orlandoa, N.; Primaveraa, M.; Spagnoloa, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Gorinia, E.; Orlandoa, N.; Spagnoloa, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dassoulas, J.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Readioff, N. P.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Savage, G.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Cooper, B. D.; Davison, A. R.; Davison, P.; Falla, R. J.; Gregersen, K.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Pilkington, A. D.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Sircar, A.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS IN2P3, Paris, France. [Akesson, T. P.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fys Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Poettgen, R.; Rave, S.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Thompson, R. J.; Tomlinson, L.; Wang, K.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Hallewell, G. D.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Liu, J.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Hallewell, G. D.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Liu, J.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Fleischmann, P.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Jennens, D.; Kubota, T.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Goldfarb, S.; Hu, X.; Levin, D.; Liu, L.; Long, J. D.; Lu, N.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Panikashvili, N.; Qian, J.; Schwarz, T. A.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugnia, D.; Laria, T.; Mandellia, L.; Mazzaa, S. M.; Meronia, C.; Perinia, L.; Pizioa, C.; Ragusaa, F.; Resconia, S.; Shojaiia, S.; Simonielloa, R.; Tartarellia, G. F.; Troncona, C.; Turraa, R.; Pereza, M. Villaplana] INFN Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Mazzaa, S. M.; Perinia, L.; Pizioa, C.; Ragusaa, F.; Shojaiia, S.; Simonielloa, R.; Turraa, R.; Pereza, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.; Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] PN Lebedev Phys Inst, Acad Sci, Moscow 117924, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.; Zhang, D.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; Von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; De Asmundisa, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordanoa, R.; Iengoa, P.; Izzoa, V.; Merolaa, L.; Patricellia, S.; Perrellaa, S.; Rossia, E.; Sancheza, A.; Sekhniaidzea, G.; Zurzoloa, G.] INFN Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Di Donato, C.; Giordanoa, R.; Merolaa, L.; Patricellia, S.; Perrellaa, S.; Rossia, E.; Sancheza, A.; Zurzoloa, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Koenig, A. C.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; De Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; Van der Geer, R.; Van der Graaf, H.; Van der Leeuw, R.; Van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; De Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; Van der Geer, R.; Van der Graaf, H.; Van der Leeuw, R.; Van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Kharlamov, A.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Haley, J.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS IN2P3, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, K.; Boddy, C. R.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pachal, K.; Pickering, M. A.; Pinder, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livana, M.; Negria, A.; Poleselloa, G.; Rebuzzia, D. M.; Rimoldia, A.; Vercesia, V.] INFN Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livana, M.; Negria, A.; Rebuzzia, D. M.; Rimoldia, A.] Univ Pavia, Dipartimento Fis, Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Lester, C. M.; Lipeles, E.; Meyer, C.; Ospanov, R.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannettia, P.; Leonea, S.; Rodaa, C.; Scuria, F.; Volpia, G.; Whitea, S.] INFN Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannettia, P.; Leonea, S.; Rodaa, C.; Scuria, F.; Volpia, G.; Whitea, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Mueller, J.; Prieur, D.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousaa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Galhardoa, B.; Gomesab, A.; Goncaloa, R.; Jorgea, P. M.; Lopesa, L.; Miguensa, J. Machado; Maioab, A.; Maneiraa, J.; Onofrea, A.; Palma, A.; Pedroa, R.; Pinaab, J.; Pintoa, B.; Santosa, H.; Saraivaa, J. G.; Silvaa, J.; Delgadoa, A. Tavares; Velosoa, F.; Woltersa, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; De Sousaa, M. J. Da Cunha Sargedas; Gomesab, A.; Jorgea, P. M.; Miguensa, J. Machado; Maioab, A.; Maneiraa, J.; Palma, A.; Pedroa, R.; Pinaab, J.; Delgadoa, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardoa, B.; Velosoa, F.; Woltersa, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomesab, A.; Maioab, A.; Pinaab, J.; Saraivaa, J. G.; Silvaa, J.] Univ Lisbon, Ctr Fis Nucl, Lisbon, Portugal. [Onofrea, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Fac Ciencias & Tecnol, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Pedisa, D.; De Salvoa, A.; Di Domenico, A.; Falciano, S.; Gabriellia, A.; Gauzzi, P.; Gentilea, S.; Giagua, S.; Kunaa, M.; Lacavaa, F.; Lucia, C.; Luminaria, L.; Marzanoa, F.; Mirabellia, G.; Monzania, S.; Nisatia, A.; Pasqualuccia, E.; Petroloa, E.; Pontecorvoa, L.; Rescignoa, M.; Rosatia, S.; Tehrania, F. Safai; Sidotia, A.; Vanadiaa, M.; Varia, R.; Venezianoa, S.; Verduccia, M.; Zanello, L.] INFN Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabriellia, A.; Gauzzi, P.; Gentilea, S.; Giagua, S.; Kunaa, M.; Lacavaa, F.; Lucia, C.; Monzania, S.; Vanadiaa, M.; Verduccia, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossia, G. C.; Iuppaa, R.; Libertia, B.; Mazzaferroa, L.; Paolozzia, L.; Salamona, A.; Santonicoa, R.] INFN Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossia, G. C.; Iuppaa, R.; Mazzaferroa, L.; Paolozzia, L.; Santonicoa, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziania, E.; Iodicea, M.; Orestanoa, D.; Passeria, A.; Pastorea, F.; Petruccia, F.; Puddua, D.; Salamannaa, G.; Stanescua, C.; Taccinia, C.; Trovatellia, M.] INFN Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestanoa, D.; Pastorea, F.; Petruccia, F.; Puddua, D.; Salamannaa, G.; Taccinia, C.; Trovatellia, M.] Univ Roma Tre, Dipartimento Matemat Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Fassi, F.; Gouighria, M.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlaneb, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdamic, D.] Univ Cadi Ayyad, Fac Sci Semlalia, Lphea Marrakech, Morocco. [Boutouil, S.; DerkaouiD, J. E.; Ouchrifd, M.; Tayalatid, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; DerkaouiD, J. E.; Ouchrifd, M.; Tayalatid, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Haddade, N.; Idrissie, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mal, P.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nef, P. D.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Blazek, T.; Federic, P.; Plazaka, L.; Stavinaa, P.; Sykoraa, I.; Tokara, S.; Zenisa, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladivab, E.; Strizenecb, P.; Urbanb, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamiltona, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Leeb, C. A.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Carrillo-Montoya, G. D.; Hamity, G. N.; Hsu, C.; Marchc, L.; Garciac, B. R. Mellado; Ruanc, X.; Vickeyc, T.; Boeriuc, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaitia, Y.; Akerstedt, H.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Jon-Anda, K.; Khandanyana, H.; Kima, H.; Klimeka, P.; Lundberga, O.; Milsteada, D. A.; Moaa, T.; Molandera, S.; Petridisa, A.; Plucinskia, P.; Rossettia, V.; Shcherbakova, A.; Silversteina, S. B.; Sjolina, J.; Strandberga, S.; Tylmada, M.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaitia, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Gellerstedt, K.; Hellman, S.; Jon-Anda, K.; Khandanyana, H.; Kima, H.; Klimeka, P.; Lundberga, O.; Milsteada, D. A.; Moaa, T.; Molandera, S.; Petridisa, A.; Plucinskia, P.; Rossettia, V.; Shcherbakova, A.; Sjolina, J.; Strandberga, S.; Tylmada, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Asquith, L.; Bartsch, V.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Hsu, P. J.; Jamin, D. O.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Ren, Z. L.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Sidiropoulou, O.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Cooke, M.; Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Brelier, B.; Chau, C. C.; DeMarco, D. A.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Koutsmana, A.; Orama, C. J.; Codinaa, E. Perez; Schoutena, D.; Seustera, R.; Stelzer-Chiltona, O.; Tafirouta, R.; Triggera, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Benitez Garcia, J. A.; Ramosb, J. Manjarres; Palacinob, G.; Qureshib, A.; Taylorb, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Brazzale, S. F.; Cobal, M.; Giordania, M. P.; Miglioranzia, S.; Pinamontiac, M.; Quaylea, W. B.; Shawa, K.; Soualaha, R.] INFN Grp Coll Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Quaylea, W. B.; Shawa, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordania, M. P.; Miglioranzia, S.; Pinamontiac, M.; Soualaha, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; De la Hoz, S. Gonzalez; Jimenez, Y. Hernndez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torr; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] IFIC, Valencia, Spain. [Ferrer, A.; Fuster, J.; Garcia, C.; Higon-Rodriguez, E.; Quiles, A. Irles; Lacasta, C.; Garcia, E. Oliver; Adam, E. Romero; Ros, E.; Salt, J.; Pastor, E. Torr; Valero, A.; Gallego, E. Valladolid] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Urban, S. Cabrera; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Marti-Garcia, S.; Moles-Valls, R.; Garcia, E. Oliver; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Pastor, E. Torr; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; De la Hoz, S. Gonzalez; Jimenez, Y. Hernndez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torr; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, IMB, CNM, Valencia, Spain. [Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Marti-Garcia, S.; Moles-Valls, R.; Garcia, E. Oliver; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Pastor, E. Torr; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Siragusa, G.; Strohmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Barisonzi, M.; Beermann, T. A.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Tepel, F.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Baker, O. K.; Bedikian, S.; Cummings, J.; Demers, S.; Garberson, F.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] IN2P3, Ctr Calcul, Villeurbanne, France. Kings Coll London, Dept Phys, London WC2R 2LS, England. [Ahmadov, F.; Huseynov, N.; Javadov, N.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Anisenkov, A. V.; Bobrovnikov, V. S.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Azuelos, G.; Gingrich, D. M.; Oakham, F. G.; Savard, P.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beck, H. P.] Univ Fribourg, Dept Phys, CH-1700 Fribourg, Switzerland. [Chelkov, G. A.] Tomsk State Univ, Tomsk 634050, Russia. [Chen, L.] Aix Marseille Univ, CPPM, Marseille, France. [Chen, L.] CNRS IN2P3, Marseille, France. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Davies, E.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Barcelona, Spain. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelavaa, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Jenni, P.] CERN, CH-1211 Geneva 23, Switzerland. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Lib, B.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Lic, Y.] Univ Paris 11, LAL, Orsay, France. [Lic, Y.] CNRS IN2P3, Orsay, France. [Lin, S. C.] Acad Sinica, Acad Sinica Grid Comp, Inst Phys, Taipei 115, Taiwan. [Liub, K.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Liub, K.] Univ Paris Diderot, Paris, France. [Liub, K.] CNRS IN2P3, Paris, France. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Messina, A.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Pinamontiac, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tikhomirov, V. O.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Vickeyc, T.] Univ Oxford, Dept Phys, Oxford, England. [Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Xu, L.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Yusuf, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Korol, Aleksandr/A-6244-2014; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Petrucci, Fabrizio/G-8348-2012; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Martinez, Mario /I-3549-2015; Peleganchuk, Sergey/J-6722-2014; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Jones, Roger/H-5578-2011; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Snesarev, Andrey/H-5090-2013; Kantserov, Vadim/M-9761-2015; BESSON, NATHALIE/L-6250-2015; Ippolito, Valerio/L-1435-2016; KHODINOV, ALEKSANDR/D-6269-2015; Staroba, Pavel/G-8850-2014; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; De, Kaushik/N-1953-2013; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Smirnova, Oxana/A-4401-2013; Doyle, Anthony/C-5889-2009; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Brooks, William/C-8636-2013; Grancagnolo, Sergio/J-3957-2015; Di Domenico, Antonio/G-6301-2011; Boyko, Igor/J-3659-2013; Ciubancan, Liviu Mihai/L-2412-2015; Mitsou, Vasiliki/D-1967-2009; Zhukov, Konstantin/M-6027-2015; Shmeleva, Alevtina/M-6199-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013 OI La Rosa, Alessandro/0000-0001-6291-2142; Beck, Hans Peter/0000-0001-7212-1096; Prokofiev, Kirill/0000-0002-2177-6401; Vazquez Schroeder, Tamara/0000-0002-9780-099X; Chen, Chunhui /0000-0003-1589-9955; Terzo, Stefano/0000-0003-3388-3906; Smirnov, Sergei/0000-0002-6778-073X; Giorgi, Filippo Maria/0000-0003-1589-2163; Coccaro, Andrea/0000-0003-2368-4559; Cristinziani, Markus/0000-0003-3893-9171; Galhardo, Bruno/0000-0003-0641-301X; Castro, Nuno/0000-0001-8491-4376; Farrington, Sinead/0000-0001-5350-9271; Robson, Aidan/0000-0002-1659-8284; Weber, Michele/0000-0002-2770-9031; Grohsjean, Alexander/0000-0003-0748-8494; Irles, Adrian/0000-0001-5668-151X; Dell'Asta, Lidia/0000-0002-9601-4225; Korol, Aleksandr/0000-0001-8448-218X; Giordani, Mario/0000-0002-0792-6039; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Petrucci, Fabrizio/0000-0002-5278-2206; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Mindur, Bartosz/0000-0002-5511-2611; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Nisati, Aleandro/0000-0002-5080-2293; Troncon, Clara/0000-0002-7997-8524; Vari, Riccardo/0000-0002-2814-1337; Gray, Heather/0000-0002-5293-4716; Hays, Chris/0000-0003-2371-9723; Jones, Roger/0000-0002-6427-3513; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Kantserov, Vadim/0000-0001-8255-416X; Ippolito, Valerio/0000-0001-5126-1620; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Gauzzi, Paolo/0000-0003-4841-5822; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; De, Kaushik/0000-0002-5647-4489; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Smirnova, Oxana/0000-0003-2517-531X; Doyle, Anthony/0000-0001-6322-6195; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Brooks, William/0000-0001-6161-3570; Grancagnolo, Sergio/0000-0001-8490-8304; Di Domenico, Antonio/0000-0001-8078-2759; Boyko, Igor/0000-0002-3355-4662; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Mitsou, Vasiliki/0000-0002-1533-8886; Tikhomirov, Vladimir/0000-0002-9634-0581; Warburton, Andreas/0000-0002-2298-7315 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; GRICES, Portugal; FCT, Portugal; MERYS (MECTS), Romania; MES of Russia, Russian Federation; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 128 TC 16 Z9 16 U1 9 U2 65 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 16 PY 2015 VL 92 IS 1 AR 012006 DI 10.1103/PhysRevD.92.012006 PG 84 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CM9IN UT WOS:000358022200001 ER PT J AU Aad, G Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G 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CA ATLAS Collaboration TI Evidence of W gamma gamma Production in pp Collisions at root s=8 TeV and Limits on Anomalous Quartic Gauge Couplings with the ATLAS Detector SO PHYSICAL REVIEW LETTERS LA English DT Article ID CROSS-SECTION; BOSON COUPLINGS; CONSTRAINTS AB This Letter reports evidence of triple gauge boson production pp -> W(l nu)gamma gamma + X, which is accessible for the first time with the 8 TeV LHC data set. The fiducial cross section for this process is measured in a data sample corresponding to an integrated luminosity of 20.3 fb(-1), collected by the ATLAS detector in 2012. Events are selected using the W boson decay to e nu or mu nu as well as requiring two isolated photons. The measured cross section is used to set limits on anomalous quartic gauge couplings in the high diphoton mass region. C1 [Davies, E.; Jackson, P.; Lee, L.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. 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P.; Yusuff, I.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jakobsen, S.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y.; Krizka, K.; Li, H. L.; Melachrinos, C.; Merritt, F. S.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Shandong, Peoples R China. [Guo, J.; Li, L.; Wang, C.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Clermont Univ, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chen, L.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, Frascati, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dao, V.; Di Simone, A.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Camacho Toro, R.; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Picazio, A.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, High Energy Phys Inst, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bindi, M.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Keil, M.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R. W.; Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Allison, L. J.; Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Price, J.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr; Savage, G.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Pilkington, A. D.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Poettgen, R.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Liu, J.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Liu, J.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Hu, X.; Levin, D.; Liu, L.; Long, J. D.; Lu, N.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Consonni, S. M.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.; Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu; Smirnov, Y.; Soldatov, E. Yu; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Moser, H. G.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; Von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Iengo, P.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Koenig, A. C.; Nektarijevic, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; Van der Geer, R.; Van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef, Natl Inst Subat Phys, Amsterdam, Netherlands. [Adelman, J.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] Univ Illinois, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Kharlamov, A.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu A.] RAS, Budker Inst Nucl Phys, SB, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Haley, J.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pachal, K.; Pickering, M. A.; Ryder, N. C.; Sawyer, C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Lipeles, E.; Machado Miguens, J.; Meyer, C.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Fac Ciencias & Tecnol, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Aloisio, A.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Mirabelli, G.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Veneziano, S.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Stanescu, C.; Taccini, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Taccini, C.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA, Fac Sci Semlalia, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph; Schwemling, Ph; Schwindling, J.] CEA Saclay, IRFU, DSM, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; Horton, A. J.; O'Neil, D. C.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Mount, R.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.; Meehan, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Lee, C. A.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hamity, G. N.; March, L.; Garcia, B. R. Mellado; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Eriksson, D.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Hsu, P. J.; Jamin, D. O.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Yang, Y.; Zhang, L.] Acad Sinica, Inst Phys, Taipei 115, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Sotiropoulou, C. L.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Ilic, N.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Qureshi, A.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Swedish, S.] Univ British Columbia, Dept Phys, Vancouver, BC V5Z 1M9, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kwan, T.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Beermann, T. A.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] IN2P3, Ctr Calcul, Villeurbanne, France. Kings Coll London, Dept Phys, London, England. [Ahmadov, F.; Huseynov, N.; Javadov, N.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Anisenkov, A. V.; Bobrovnikov, V. S.; Kazanin, V. F.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. 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[Jenni, P.] CERN, Geneva, Switzerland. [Khubua, J.] GTU, Tbilisi, Rep of Georgia. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Li, B.] Acad Sinica, Inst Phys, Taipei 115, Taiwan. [Li, Y.] Univ Paris 11, LAL, Orsay, France. [Li, Y.] CNRS, IN2P3, Orsay, France. [Lin, S. C.] Acad Sinica, Acad Sinica Grid Comp, Inst Phys, Taipei 115, Taiwan. [Liu, K.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Liu, K.] Univ Paris Diderot, Paris, France. [Liu, K.] CNRS, IN2P3, Paris, France. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tikhomirov, V. O.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Inst Particle & Nucl Phys, Wigner Res Ctr Phys, Budapest, Hungary. [Vickey, T.] Univ Oxford, Dept Phys, Oxford, England. [Xu, L.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Grancagnolo, Sergio/J-3957-2015; White, Ryan/E-2979-2015; Mitsou, Vasiliki/D-1967-2009; Zhukov, Konstantin/M-6027-2015; Shmeleva, Alevtina/M-6199-2015; Doyle, Anthony/C-5889-2009; Livan, Michele/D-7531-2012; spagnolo, stefania/A-6359-2012; Di Domenico, Antonio/G-6301-2011; Negrini, Matteo/C-8906-2014; Tassi, Enrico/K-3958-2015; Boyko, Igor/J-3659-2013; Ciubancan, Liviu Mihai/L-2412-2015; Kantserov, Vadim/M-9761-2015; La Rosa Navarro, Jose Luis/K-4221-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Staroba, Pavel/G-8850-2014; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Gerbaudo, Davide/J-4536-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Martinez, Mario /I-3549-2015; Peleganchuk, Sergey/J-6722-2014; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Garcia, Jose /H-6339-2015; Korol, Aleksandr/A-6244-2014; Capua, Marcella/A-8549-2015; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Smirnova, Oxana/A-4401-2013; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Snesarev, Andrey/H-5090-2013; Gavrilenko, Igor/M-8260-2015; Veneziano, Stefano/J-1610-2012; Tikhomirov, Vladimir/M-6194-2015; Villa, Mauro/C-9883-2009; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Brooks, William/C-8636-2013; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; De, Kaushik/N-1953-2013; Carvalho, Joao/M-4060-2013; Tartarelli, Giuseppe Francesco/A-5629-2016; Petrucci, Fabrizio/G-8348-2012; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; OI Grancagnolo, Sergio/0000-0001-8490-8304; White, Ryan/0000-0003-3589-5900; Mitsou, Vasiliki/0000-0002-1533-8886; Doyle, Anthony/0000-0001-6322-6195; Livan, Michele/0000-0002-5877-0062; spagnolo, stefania/0000-0001-7482-6348; Di Domenico, Antonio/0000-0001-8078-2759; Negrini, Matteo/0000-0003-0101-6963; Boyko, Igor/0000-0002-3355-4662; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Korol, Aleksandr/0000-0001-8448-218X; Giordani, Mario/0000-0002-0792-6039; Capua, Marcella/0000-0002-2443-6525; Mashinistov, Ruslan/0000-0001-7925-4676; Smirnova, Oxana/0000-0003-2517-531X; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Veneziano, Stefano/0000-0002-2598-2659; Tikhomirov, Vladimir/0000-0002-9634-0581; Villa, Mauro/0000-0002-9181-8048; Warburton, Andreas/0000-0002-2298-7315; Brooks, William/0000-0001-6161-3570; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; De, Kaushik/0000-0002-5647-4489; Carvalho, Joao/0000-0002-3015-7821; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Petrucci, Fabrizio/0000-0002-5278-2206; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Giorgi, Filippo Maria/0000-0003-1589-2163; Coccaro, Andrea/0000-0003-2368-4559 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; RGC, China; Hong Kong SAR, China; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT , Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC, and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST, and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR, and VSC CR, Czech Republic; DNRF, DNSRC, and Lundbeck Foundation, Denmark; EPLANET, ERC, and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG, and AvH Foundation, Germany; GSRT and NSRF, Greece; RGC, Hong Kong SAR, China; ISF, MINERVA, GIF, I-CORE, and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF, and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society, and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK), and BNL (USA) and in the Tier-2 facilities worldwide. NR 59 TC 6 Z9 6 U1 10 U2 64 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 16 PY 2015 VL 115 IS 3 AR 031802 DI 10.1103/PhysRevLett.115.031802 PG 18 WC Physics, Multidisciplinary SC Physics GA CM9JO UT WOS:000358024900002 PM 26230784 ER PT J AU Narvaez, J Saremi, S Hong, JW Stengel, M Catalan, G AF Narvaez, Jackeline Saremi, Sahar Hong, Jiawang Stengel, Massimiliano Catalan, Gustau TI Large Flexoelectric Anisotropy in Paraelectric Barium Titanate SO PHYSICAL REVIEW LETTERS LA English DT Article ID POLARIZATION; SURFACE; BATIO3 AB The bending-induced polarization of barium titanate single crystals has been measured with an aim to elucidate the origin of the large difference between theoretically predicted and experimentally measured flexoelectricity in this material. The results indicate that part of the difference is due to polar regions (short-range order) that exist above T-C and up to T* approximate to 200-225 degrees C. Above T*, however, the flexovoltage coefficient still shows an unexpectedly large anisotropy for a cubic material, with (001)-oriented crystals displaying 10 times more flexoelectricity than (111)-oriented crystals. Theoretical analysis shows that this anisotropy cannot be a bulk property, and we therefore interpret it as indirect evidence for the theoretically predicted but experimentally elusive contribution of surface piezoelectricity to macroscopic bending-induced polarization. C1 [Narvaez, Jackeline; Saremi, Sahar; Catalan, Gustau] ICN2 Inst Catala Nanociencia & Nanotecnol, Bellaterra 08193, Barcelona, Spain. [Narvaez, Jackeline] CSIC, Bellaterra 08193, Barcelona, Spain. [Hong, Jiawang] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Stengel, Massimiliano] CSIC, Inst Ciencia Mat Barcelona ICMA, Bellaterra 08193, Barcelona, Spain. [Stengel, Massimiliano; Catalan, Gustau] ICREA, Barcelona 08010, Spain. RP Narvaez, J (reprint author), ICN2 Inst Catala Nanociencia & Nanotecnol, Campus UAB, Bellaterra 08193, Barcelona, Spain. EM jackeline.narvaez@cin2.es; gustau.catalan@cin2.es RI Catalan, Gustau/D-3233-2015; Stengel, Massimiliano/E-2934-2010; Hong, Jiawang/B-2864-2009 OI Catalan, Gustau/0000-0003-0214-4828; Stengel, Massimiliano/0000-0003-4175-3888; Hong, Jiawang/0000-0002-9915-8072 FU ERC Starting grant from the EU [ERC 308023]; Spanish MINECO [FIS2013-48668-C2-1-P, FIS2013-48668-C2-2-P]; Severo Ochoa Excellence Programme [SEV-2013-0295]; "Next Big Ideas" project at Oak Ridge National Laboratory FX This research has been funded by an ERC Starting grant from the EU (ERC 308023) and by National Plan Grants No. FIS2013-48668-C2-1-P and No. FIS2013-48668-C2-2-P from the Spanish MINECO. ICN2 acknowledges support by the Severo Ochoa Excellence Programme SEV-2013-0295. J. H acknowledges support from "Next Big Ideas" project at Oak Ridge National Laboratory. NR 37 TC 10 Z9 10 U1 7 U2 62 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 16 PY 2015 VL 115 IS 3 AR 037601 DI 10.1103/PhysRevLett.115.037601 PG 5 WC Physics, Multidisciplinary SC Physics GA CM9JO UT WOS:000358024900006 PM 26230825 ER PT J AU Chow, WW Straatsma, CJE Anderson, DZ AF Chow, Weng W. Straatsma, Cameron J. E. Anderson, Dana Z. TI Numerical model for atomtronic circuit analysis SO PHYSICAL REVIEW A LA English DT Article ID DYNAMICS AB A model for studying atomtronic devices and circuits based on finite-temperature Bose-condensed gases is presented. The approach involves numerically solving equations of motion for atomic populations and coherences, derived using the Bose-Hubbard Hamiltonian and the Heisenberg picture. The resulting cluster expansion is truncated at a level giving balance between physics rigor and numerical demand mitigation. This approach allows parametric studies involving time scales that cover both the rapid population dynamics relevant to nonequilibrium state evolution, as well as the much longer time durations typical for reaching steady-state device operation. The model is demonstrated by studying the evolution of a Bose-condensed gas in the presence of atom injection and extraction in a double-well potential. In this configuration phase locking between condensates in each well of the potential is readily observed, and its influence on the evolution of the system is studied. C1 [Chow, Weng W.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Straatsma, Cameron J. E.; Anderson, Dana Z.] Univ Colorado, JILA, Boulder, CO 80309 USA. [Straatsma, Cameron J. E.] Univ Colorado, Dept Elect Comp & Energy Engn, Boulder, CO 80309 USA. [Anderson, Dana Z.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Anderson, Dana Z.] NIST, Boulder, CO 80309 USA. RP Anderson, DZ (reprint author), Univ Colorado, JILA, Boulder, CO 80309 USA. EM dana@jila.colorado.edu FU Sandia LDRD program - U.S. Department of Energy [DE-AC04-94AL85000]; U.S. Air Force Office of Scientific Research [FA9550-14-1-0327]; U.S. National Science Foundation [PHY1125844]; Charles Stark Draper Laboratory [SC001-0000000759] FX This work is partially supported by the Sandia LDRD program, funded by the U.S. Department of Energy under Contract No. DE-AC04-94AL85000, and by the U.S. Air Force Office of Scientific Research under Contract No. FA9550-14-1-0327, the U.S. National Science Foundation under Contract No. PHY1125844, and the Charles Stark Draper Laboratory under Contract No. SC001-0000000759. NR 23 TC 2 Z9 2 U1 2 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD JUL 16 PY 2015 VL 92 IS 1 AR 013621 DI 10.1103/PhysRevA.92.013621 PG 8 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CM9HQ UT WOS:000358019200008 ER PT J AU Diallo, SO AF Diallo, S. O. TI Pore-size dependence and characteristics of water diffusion in slitlike micropores SO PHYSICAL REVIEW E LA English DT Article ID SINGLE-PARTICLE DYNAMICS; ACTIVATED CARBON-FIBERS; NEUTRON-SCATTERING; SUPERCOOLED WATER; HYDROPHILIC SURFACE; CONFINED SPACE; ADSORPTION; MOLECULES; NANOPORES; MOTIONS AB The temperature dependence of the dynamics of water inside microporous activated carbon fibers (ACF) is investigated by means of incoherent elastic and quasielastic neutron-scattering techniques. The aim is to evaluate the effect of increasing pore size on the water dynamics in these primarily hydrophobic slit-shaped channels. Using two different micropore sizes (similar to 12 and 18 angstrom, denoted, respectively, ACF-10 and ACF-20), a clear suppression of the mobility of the water molecules is observed as the pore gap or temperature decreases. This suppression is accompanied by a systematic dependence of the average translational diffusion coefficient D-r and relaxation time [tau(0)] of the restricted water on pore size and temperature. The observed D-r values are tested against a proposed scaling law, in which the translational diffusion coefficient D-r of water within a porous matrix was found to depend solely on two single parameters, a temperature-independent translational diffusion coefficient D-c associated with the water bound to the pore walls and the ratio theta of this strictly confined water to the total water inside the pore, yielding unique characteristic parameters for water transport in these carbon channels across the investigated temperature range. C1 Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. RP Diallo, SO (reprint author), Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. EM omardiallos@ornl.gov RI Diallo, Souleymane/B-3111-2016 OI Diallo, Souleymane/0000-0002-3369-8391 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX The author is thankful to R. Goyette, R. Mills, R. Moody, and M. Rucker at the Spallation Neutron Source (SNS), Oak Ridge National Laboratory (ORNL), for their excellent technical support during the measurements. He is also indebted to Eugene Mamontov for many stimulating scientific discussions over the last few years. He thanks both E. Mamontov and A. Kolesnikov for their critical reading of the manuscript. The author owes much gratitude to M. Sliwinska-Bartkowiak, A. A. Chialvo, L. Vleck, and J. S. Hayes for recent collaborations on the diffusion properties of water confined inside related nanoporous carbon materials, which have motivated the present work. The use of the MANTID software package [52] is gratefully acknowledged. This work at ORNL's SNS is sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 52 TC 7 Z9 7 U1 5 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD JUL 16 PY 2015 VL 92 IS 1 AR 012312 DI 10.1103/PhysRevE.92.012312 PG 10 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA CM9IY UT WOS:000358023300004 PM 26274167 ER PT J AU Lam, RK England, AH Smith, JW Rizzuto, AM Shih, O Prendergast, D Saykally, RJ AF Lam, Royce K. England, Alice H. Smith, Jacob W. Rizzuto, Anthony M. Shih, Orion Prendergast, David Saykally, Richard J. TI The hydration structure of dissolved carbon dioxide from X-ray absorption spectroscopy SO CHEMICAL PHYSICS LETTERS LA English DT Editorial Material ID INITIO MOLECULAR-DYNAMICS; AB-INITIO; AQUEOUS-SOLUTION; WATER-MOLECULES; ACID FORMATION; CO2; DEHYDRATION; BICARBONATE; SYSTEM; ION AB The dissolution of carbon dioxide in water and its subsequent hydrolysis reactions comprise one of the most central processes in all of science, yet it remains incompletely understood despite enormous effort. We report the detailed characterization of dissolved CO2 gas through the combination of X-ray spectroscopy and first principles theory. The molecule acts as a hydrophobe in water with an average hydrogen bond number of 0.56. The carbon atom interacts weakly with a single water at a distance of >2.67 angstrom and the carbonyl oxygens serve as weak hydrogen bond acceptors, thus locally enhancing the tetrahedral water hydrogen bonding structure. Published by Elsevier B.V. C1 [Lam, Royce K.; England, Alice H.; Smith, Jacob W.; Rizzuto, Anthony M.; Shih, Orion; Saykally, Richard J.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Lam, Royce K.; England, Alice H.; Smith, Jacob W.; Rizzuto, Anthony M.; Saykally, Richard J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Prendergast, David] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Saykally, RJ (reprint author), Univ Calif Berkeley, Dept Chem, D31 Hildebrand Hall, Berkeley, CA 94720 USA. EM saykally@berkeley.edu RI Foundry, Molecular/G-9968-2014; OI Lam, Royce/0000-0003-2878-038X NR 46 TC 4 Z9 4 U1 0 U2 33 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2614 EI 1873-4448 J9 CHEM PHYS LETT JI Chem. Phys. Lett. PD JUL 16 PY 2015 VL 633 BP 214 EP 217 DI 10.1016/j.cplett.2015.05.039 PG 4 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CM4LD UT WOS:000357655100037 ER PT J AU Gordon, SP Tseng, E Salamov, A Zhang, JW Meng, XD Zhao, ZY Kang, DW Underwood, J Grigoriev, IV Figueroa, M Schilling, JS Chen, F Wang, Z AF Gordon, Sean P. Tseng, Elizabeth Salamov, Asaf Zhang, Jiwei Meng, Xiandong Zhao, Zhiying Kang, Dongwan Underwood, Jason Grigoriev, Igor V. Figueroa, Melania Schilling, Jonathan S. Chen, Feng Wang, Zhong TI Widespread Polycistronic Transcripts in Fungi Revealed by Single-Molecule mRNA Sequencing SO PLOS ONE LA English DT Article ID POLY(A) SIGNALS; HUMAN GENOME; SEQ; EXPRESSION; GENES; INTERFERENCE; MECHANISMS; COMPLEXITY; GENERATION; PLATFORM AB Genes in prokaryotic genomes are often arranged into clusters and co-transcribed into polycistronic RNAs. Isolated examples of polycistronic RNAs were also reported in some higher eukaryotes but their presence was generally considered rare. Here we developed a long-read sequencing strategy to identify polycistronic transcripts in several mushroom forming fungal species including Plicaturopsis crispa, Phanerochaete chrysosporium, Trametes versicolor, and Gloeophyllum trabeum. We found genome-wide prevalence of polycistronic transcription in these Agaricomycetes, involving up to 8% of the transcribed genes. Unlike polycistronic mRNAs in prokaryotes, these co-transcribed genes are also independently transcribed. We show that polycistronic transcription may interfere with expression of the downstream tandem gene. Further comparative genomic analysis indicates that polycistronic transcription is conserved among a wide range of mushroom forming fungi. In summary, our study revealed, for the first time, the genome prevalence of polycistronic transcription in a phylogenetic range of higher fungi. Furthermore, we systematically show that our long-read sequencing approach and combined bioinformatics pipeline is a generic powerful tool for precise characterization of complex transcriptomes that enables identification of mRNA isoforms not recovered via short-read assembly. C1 [Gordon, Sean P.; Salamov, Asaf; Meng, Xiandong; Zhao, Zhiying; Kang, Dongwan; Grigoriev, Igor V.; Chen, Feng; Wang, Zhong] Joint Genome Inst, Dept Energy, Walnut Creek, CA 94598 USA. [Tseng, Elizabeth; Underwood, Jason] Pacific Biosci, Menlo Pk, CA USA. [Zhang, Jiwei; Schilling, Jonathan S.] Univ Minnesota, Dept Bioprod & Biosyst Engn, St Paul, MN 55108 USA. [Figueroa, Melania] Univ Minnesota, Dept Plant Pathol, St Paul, MN USA. [Wang, Zhong] Univ Calif, Sch Nat Sci, Merced, CA USA. RP Wang, Z (reprint author), Joint Genome Inst, Dept Energy, Walnut Creek, CA 94598 USA. EM zhongwang@lbl.gov FU Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Pacific Biosciences FX The work was conducted by the U.S. Department of Energy Joint Genome Institute and supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Pacific Biosciences provided support in the form of salaries for authors ET and JU, but did not have any additional role in the study design, data collection and analysis, decision to publish, or preparation of the manuscript. The specific roles of these authors are articulated in the 'author contributions' section. NR 43 TC 7 Z9 7 U1 0 U2 8 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JUL 15 PY 2015 VL 10 IS 7 AR e0132628 DI 10.1371/journal.pone.0132628 PG 15 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CN1RL UT WOS:000358197600134 PM 26177194 ER PT J AU Jiang, KZ Bu, LZ Wang, PT Guo, SJ Huang, XQ AF Jiang, Kezhu Bu, Lingzheng Wang, Pengtang Guo, Shaojun Huang, Xiaoqing TI Trimetallic PtSnRh Wavy Nanowires as Efficient Nanoelectrocatalysts for Alcohol Electrooxidation SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE platinum; tin; rhodium; wavy nanowires; alcohol electrooxidation ID OXYGEN REDUCTION REACTION; ETHANOL FUEL-CELLS; HIGH-INDEX FACETS; ELECTROCATALYTIC ACTIVITY; PLATINUM NANOCRYSTALS; METHANOL OXIDATION; CATALYSTS; ULTRATHIN; ATTACHMENT; NI AB The design and creation of efficient catalysts for alcohol oxidation reaction has attracted great research attention because alcohols are promising fuels for direct fuel cell reactions because of their high energy density, easy storage, and transportation. We herein report an efficient strategy that allows the preparation of ternary PtSnM (M = Co, Ni, and Rh) wavy nanowires (WNWs) with ultrathin diameter of only around 2 nm and tunable compositions in high yield. Detailed catalytic studies show that all the ternary WNWs exhibit high performance for ethanol oxidation reaction (EOR) and methanol oxidation reaction (MOR), and their performance shows interesting composition-dependent electrocatalytic activity with PtSnRh WNWs having the best activity for both EOR and MOR. The PtSnRh WNWs are also more stable than commercial Pt/C catalyst, as revealed by long-time chronoamperometric (CA) measurements. The present work highlights the use of multimetallic WNWs as highly active and durable nanocatalysts in enhancing alcohol electrooxidation, which will open a new way in tuning 1D multimetallic nanostructures for boosting other fuel cell reactions, various heterogeneous reactions, and beyond. C1 [Jiang, Kezhu; Bu, Lingzheng; Wang, Pengtang; Huang, Xiaoqing] Soochow Univ, Coll Chem Chem Engn & Mat Sci, Suzhou 215123, Jiangsu, Peoples R China. [Guo, Shaojun] Los Alamos Natl Lab, Phys Chem & Appl Spect, Los Alamos, NM 87545 USA. RP Guo, SJ (reprint author), Los Alamos Natl Lab, Phys Chem & Appl Spect, POB 1663, Los Alamos, NM 87545 USA. EM shaojun.guo.nano@gmail.com; hxq006@suda.edu.cn RI Guo, Shaojun/A-8449-2011 OI Guo, Shaojun/0000-0002-5941-414X FU Soochow University; Young Thousand Talented Program FX This work was financially supported by the start-up funding from Soochow University and Young Thousand Talented Program. NR 42 TC 10 Z9 10 U1 21 U2 72 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JUL 15 PY 2015 VL 7 IS 27 BP 15061 EP 15067 DI 10.1021/acsami.5b04391 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CN4JA UT WOS:000358395200063 PM 26098177 ER PT J AU Alcantar-Vazquez, B Herrera, PRD Gonzalez, AB Duan, YH Pfeiffer, H AF Alcantar-Vazquez, Brenda Herrera, Pablo R. Diaz Gonzalez, Alejandro Barrera Duan, Yuhua Pfeiffer, Heriberto TI Analysis of the CO2-H2O Chemisorption in Lithium Silicates at Low Temperatures (30-80 degrees C) SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID CO2 ABSORPTION PROPERTIES; LI4SIO4-BASED SORBENTS; OXOSILICATE LI8SIO6; CAPTURE PROPERTIES; KINETIC-ANALYSIS; SOYBEAN OIL; ORTHOSILICATE; ZIRCONATE; SORPTION; ABSORBENT AB Li8SiO6 and Li4SiO4 were synthesized by,a solid-state reaction. Then; dynamic and isothermal :thermogravimetric water vapor sorption experiments were performed using two carrier gases: N-2 and CO2. Initially, the Li8SiO6-H2O-(N-2 or CO2) systems were analyzed It was evidenced that Li8SiO6 can trap water physically and chemically, producing Li-OH superficial species When CO2 was used as the carrier gas, Li8SiO6 continued chemisorbing H2O but CO2 was trapped as well, forming Li2CO3 and Li4SiO4 as secondary phases. On the basis of these results, the Li4SiO4-H2O-CO2 system was also analyzed. The experimental results and different theoretical thermodynamic calculations confirmed that Li8SiO6, can chernisorb 2 moles of CO2 per mole of ceramic at a low temperature-range (30-80 degrees C). Finally, different CO2 chemisorption kinetic experiments were performed to analyze and quantify the trapped CO2. C1 [Alcantar-Vazquez, Brenda; Herrera, Pablo R. Diaz; Gonzalez, Alejandro Barrera; Pfeiffer, Heriberto] Univ Nacl Autonoma Mexico, Inst Invest Mat, Mexico City 04510, DF, Mexico. [Duan, Yuhua] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. RP Alcantar-Vazquez, B (reprint author), Univ Nacl Autonoma Mexico, Inst Invest Mat, Circuito Exterior S-N,Cd Univ, Mexico City 04510, DF, Mexico. EM bcecilia_19@iim.unam.mx FU Project SENER-CONACYT [150358]; Project PAPIIP-UNAM [IN-102313] FX This work was financially supported by the Projects SENER-CONACYT (Grant 150358) and PAPIIP-UNAM (Grant IN-102313). The authors thank Adriana Tejeda and Omar Novelo for technical help. NR 68 TC 3 Z9 3 U1 6 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD JUL 15 PY 2015 VL 54 IS 27 BP 6884 EP 6892 DI 10.1021/acs.iecr.5b01110 PG 9 WC Engineering, Chemical SC Engineering GA CN4IZ UT WOS:000358395100007 ER PT J AU Yu, MZ Miller, DC Biegler, LT AF Yu, Mingzhao Miller, David C. Biegler, Lorenz T. TI Dynamic Reduced Order Models for Simulating Bubbling Fluidized Bed Adsorbers SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID PROPER ORTHOGONAL DECOMPOSITION; CO2 CAPTURE; REDUCTION; OPTIMIZATION; REACTOR; SYSTEMS; PLANTS; PHASE AB Spatially distributed first-principles process models provide an accurate physical description of chemical processes, but lead to large-scale models whose numerical solution can be challenging and computationally expensive. Therefore, fast reduced order models are requited for model-based real-the applications, such as advanced process control and dynamic real-time optimization. In this papery-we focus on the model reduction Of a bubbling fluidized bed (BFB) adsorber, which is a key component of a postcombustion carbon capture System. From a temporal aspect, dynamic reduced models are generated using the nullspace projection and eigenvalue analysis method, with the basic idea of quasi-steady state approximation for the states with fast dynamics. From a spatial aspect, dynamic reduced models are developed using orthogonal collocation and proper orthogonal decomposition to reduce the size of the rigorous model. Finally, a computationally efficient and accurate dynamic reduced model is developed for the BFB adsorber by combining temporal and spatial model reduction techniques, Which is,suitable for an online optimization-based control strategy. C1 [Yu, Mingzhao; Biegler, Lorenz T.] Carnegie Mellon Univ, Dept Chem Engn, Pittsburgh, PA 15213 USA. [Miller, David C.] Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. RP Biegler, LT (reprint author), Carnegie Mellon Univ, Dept Chem Engn, Pittsburgh, PA 15213 USA. EM biegler@cmu.edu FU United States Government FX This article was prepared as an account of work sponsored by an agency of the United States Government. Neither the United States Government nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or, assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof. NR 41 TC 7 Z9 7 U1 3 U2 11 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD JUL 15 PY 2015 VL 54 IS 27 BP 6959 EP 6974 DI 10.1021/acs.iecr.5b01270 PG 16 WC Engineering, Chemical SC Engineering GA CN4IZ UT WOS:000358395100015 ER PT J AU Liu, C Yang, B Tyo, E Seifert, S DeBartolo, J von Issendorff, B Zapol, P Vajda, S Curtiss, LA AF Liu, Cong Yang, Bing Tyo, Eric Seifert, Soenke DeBartolo, Janae von Issendorff, Bernd Zapol, Peter Vajda, Stefan Curtiss, Larry A. TI Carbon Dioxide Conversion to Methanol over Size-Selected Cu-4 Clusters at Low Pressures SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID CO2 HYDROGENATION; ELECTROCATALYTIC CONVERSION; METAL-CLUSTERS; ACTIVE-SITE; CATALYSTS; REDUCTION; SELECTIVITY; EPOXIDATION; MORPHOLOGY; SURFACES AB The activation of CO2 and its hydrogenation to methanol are of much interest as a way to utilize captured CO2. Here, we investigate the use of size-selected Cu-4 clusters supported on Al2O3 thin films for CO2 reduction in the presence of hydrogen. The catalytic activity was measured under near-atmospheric reaction conditions with a low CO2 partial pressure, and the oxidation state of the clusters was investigated by in situ grazing incidence X-ray absorption spectroscopy. The results indicate that size-selected Cu-4 clusters are the most active low-pressure catalyst for catalytic CO2 conversion to CH3OH. Density functional theory calculations reveal that Cu-4 clusters have a low activation barrier for conversion of CO2 to CH3OH. This study suggests that small Cu clusters may be excellent and efficient catalysts for the recycling of released CO2. C1 [Liu, Cong; Yang, Bing; Tyo, Eric; Zapol, Peter; Vajda, Stefan; Curtiss, Larry A.] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. [Seifert, Soenke; DeBartolo, Janae] Argonne Natl Lab, Xray Sci Div, Lemont, IL 60439 USA. [Vajda, Stefan] Argonne Natl Lab, Nanosci & Technol Div, Lemont, IL 60439 USA. [von Issendorff, Bernd] Univ Freiburg, Phys Inst, D-79104 Freiburg, Germany. [Vajda, Stefan] Yale Univ, Dept Chem & Environm Engn, Sch Engn & Appl Sci, New Haven, CT 06520 USA. [Vajda, Stefan] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. RP Zapol, P (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Lemont, IL 60439 USA. EM zapol@anl.gov; vajda@anl.gov; curtiss@anl.gov RI Yang, Bing/A-3779-2010; von Issendorff, Bernd/B-1941-2015; OI Yang, Bing/0000-0001-9476-9934; von Issendorff, Bernd/0000-0002-4358-4494; Liu, Cong/0000-0002-2145-5034 FU U.S. Department of Energy, Office of Science, BES-Division of Materials Science and Engineering and BES-Scientific User Facilities [DE-AC02-06CH11357]; ANL FX This work was supported by the U.S. Department of Energy, Office of Science, BES-Division of Materials Science and Engineering and BES-Scientific User Facilities under Contract DE-AC02-06CH11357. We acknowledge the computing resources operated by the Laboratory Computing Resource Center (ANL) and the ANL Center for Nanoscale Materials. We also thank Dr. Alex Martinson (ANL) for ALD coating. We thank the support of the Director's Postdoctoral Fellowship from ANL to Dr. Cong Liu. NR 32 TC 26 Z9 26 U1 38 U2 233 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUL 15 PY 2015 VL 137 IS 27 BP 8676 EP 8679 DI 10.1021/jacs.5b03668 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA CN1NM UT WOS:000358186700006 PM 26115184 ER PT J AU Hedden, M Francis, N Haraldsen, JT Ahmed, T Constantin, C AF Hedden, Morgan Francis, Nick Haraldsen, Jason T. Ahmed, Towfiq Constantin, Costel TI Thermoelectric Properties of Nano-Meso-Micro beta-MnO2 Powders as a Function of Electrical Resistance SO NANOSCALE RESEARCH LETTERS LA English DT Article DE Thermoelectric properties; Transition metal oxides; Manganese oxide; Seebeck coefficient; Figure of merit; Particle size versus electrical resistance ID MANGANESE-DIOXIDE AB Particle sizes of manganese oxide (beta-MnO2) powders were modified by using a mortar and pestle ground method for period of times that varied between 15-60 min. Particle size versus ground time clearly shows the existence of a size-induced regime transition (i.e., regime I and II). Thermoelectric properties of beta-MnO2 powders as a function of electrical resistance in the range of R-P = 10 - 80 Omega were measured. Based on the data presented, we propose a model for the beta-MnO2 system in which nanometer-scale MnO2 crystallites bond together through weak van der Waals forces to form larger conglomerates that span in size from nanometer to micrometer scale. C1 [Hedden, Morgan; Francis, Nick; Haraldsen, Jason T.; Constantin, Costel] James Madison Univ, Dept Phys & Astron, Harrisonburg, VA 22807 USA. [Ahmed, Towfiq] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Constantin, C (reprint author), James Madison Univ, Dept Phys & Astron, 901 Carrier Dr, Harrisonburg, VA 22807 USA. EM constacx@jmu.edu FU Department of Physics and Astronomy at James Madison University; 4-VA Collaborative at James Madison University; Los Alamos National Laboratory; National Nuclear Security Administration of the US Department of Energy [DE-AC52-06NA25396] FX CC and JTH acknowledge support from the Department of Physics and Astronomy at James Madison University. CC acknowledges support by the 4-VA Collaborative at James Madison University. TA acknowledges support by Los Alamos National Laboratory, an affirmative action equal opportunity employer, operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the US Department of Energy under Contract DE-AC52-06NA25396. NR 19 TC 2 Z9 2 U1 7 U2 22 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1556-276X J9 NANOSCALE RES LETT JI Nanoscale Res. Lett. PD JUL 15 PY 2015 VL 10 AR 292 DI 10.1186/s11671-015-1000-6 PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA CN1YB UT WOS:000358215700001 PM 26168867 ER PT J AU Lee, S Zhang, WR Khatkhatay, F Jia, QX Wang, HY MacManus-Driscoll, JL AF Lee, Shinbuhm Zhang, Wenrui Khatkhatay, Fauzia Jia, Quanxi Wang, Haiyan MacManus-Driscoll, Judith L. TI Strain Tuning and Strong Enhancement of Ionic Conductivity in SrZrO3-RE2O3 (RE = Sm, Eu, Gd, Dy, and Er) Nanocomposite Films SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article ID OXIDE FUEL-CELLS; THIN-FILMS; FERROELECTRIC-FILMS; LOCAL CONDUCTION; ELECTROLYTES; INTERFACES; TUNABILITY; DIFFUSION AB Fast ion transport channels at interfaces in thin films have attracted great attention due to a range of potential applications for energy materials and devices, for, solid oxide fuel cells, sensors, and memories. Here, it is shown that in vertical nanocomposite heteroepitaxial films of SrZrO3-RE2O3 (RE = Sm, Eu, Gd, Dy, and Er) the ionic conductivity of the composite can be tuned and strongly enhanced using embedded, stiff, and vertical nanopillars of RE2O3. With increasing lattice constant of RE2O3 from Er2O3 to Sm2O3, it is found that the tensile strain in the SrZrO3 increases proportionately, and the ionic conductivity of the composite increases accordingly, by an order of magnitude. The results here conclusively show, for the first time, that strain in films can be effectively used to tune the ionic conductivity of the materials. C1 [Lee, Shinbuhm; MacManus-Driscoll, Judith L.] Univ Cambridge, Dept Mat Sci & Met, Cambridge CB3 0FS, England. [Zhang, Wenrui; Khatkhatay, Fauzia; Wang, Haiyan] Texas A&M Univ, Dept Elect & Comp Engn, College Stn, TX 77843 USA. [Jia, Quanxi] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. RP Lee, S (reprint author), Univ Cambridge, Dept Mat Sci & Met, 27 Charles Babbage Rd, Cambridge CB3 0FS, England. EM jld35@cam.ac.uk RI LEE, SHINBUHM/A-9494-2011; Zhang, Wenrui/D-1892-2015 OI LEE, SHINBUHM/0000-0002-4907-7362; Zhang, Wenrui/0000-0002-0223-1924 FU European Research Council (ERC) [ERC-2009-AdG-247276-NOVOX]; UK Engineering and Physical Sciences Research Council (EPSRC); U.S. National Science Foundation [DMR-1401266]; NNSA's Laboratory Directed Research and Development Program FX This work was supported by the European Research Council (ERC) (Advanced Investigator Grant No. ERC-2009-AdG-247276-NOVOX), the UK Engineering and Physical Sciences Research Council (EPSRC), and the U.S. National Science Foundation (Grant No. DMR-1401266). The work at Los Alamos was partially supported by the NNSA's Laboratory Directed Research and Development Program and was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. NR 30 TC 10 Z9 10 U1 12 U2 76 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD JUL 15 PY 2015 VL 25 IS 27 BP 4328 EP 4333 DI 10.1002/adfm.201404420 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CM9AG UT WOS:000357996600017 ER PT J AU Hruszkewycz, SO Holt, MV Allain, M Chamard, V Polvino, SM Murray, CE Fuoss, PH AF Hruszkewycz, S. O. Holt, M. V. Allain, M. Chamard, V. Polvino, S. M. Murray, C. E. Fuoss, P. H. TI Efficient modeling of Bragg coherent x-ray nanobeam diffraction SO OPTICS LETTERS LA English DT Article ID NANOSCALE; PTYCHOGRAPHY; MICROSCOPY AB X-ray Bragg diffraction experiments that utilize tightly focused coherent beams produce complicated Bragg diffraction patterns that depend on scattering geometry, characteristics of the sample, and properties of the x-ray focusing optic. Here, we use a Fourier-transform-based method of modeling the 2D intensity distribution of a Bragg peak and apply it to the case of thin films illuminated with a Fresnel zone plate in three different Bragg scattering geometries. The calculations agree well with experimental coherent diffraction patterns, demonstrating that nanodiffraction patterns can be modeled at nonsymmetric Bragg conditions with this approach-a capability critical for advancing nanofocused x-ray diffraction microscopy. (C) 2015 Optical Society of America C1 [Hruszkewycz, S. O.; Fuoss, P. H.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Holt, M. V.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Allain, M.; Chamard, V.] Aix Marseille Univ, CNRS, Inst Fresnel, Cent Marseille,UMR 7249, F-13013 Marseille, France. [Polvino, S. M.] Columbia Univ, Dept Appl Phys & Math, New York, NY 10027 USA. [Murray, C. E.] IBM Corp, TJ Watson Res Ctr, Yorktown Hts, NY 10598 USA. RP Hruszkewycz, SO (reprint author), Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. EM shrus@anl.gov RI Chamard, Virginie/B-3704-2016 OI Chamard, Virginie/0000-0002-6894-4169 FU Basic Energy Sciences, Office of Science, U.S. Department of Energy (BES); French National Research Agency (L' Agence Nationale de la Recherche) [ANR-11-BS10-0005] FX Basic Energy Sciences, Office of Science, U.S. Department of Energy (BES); French National Research Agency (L' Agence Nationale de la Recherche) (ANR-11-BS10-0005). NR 16 TC 5 Z9 5 U1 7 U2 31 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 0146-9592 EI 1539-4794 J9 OPT LETT JI Opt. Lett. PD JUL 15 PY 2015 VL 40 IS 14 BP 3241 EP 3244 DI 10.1364/OL.40.003241 PG 4 WC Optics SC Optics GA CM8PB UT WOS:000357963000006 PM 26176439 ER PT J AU Quesada, A Monti, M Krug, IP Rougemaille, N Nickel, F Gottlob, DM Doganay, H N'Diaye, AT Chen, G Serrano, A McCarty, KF Fernandez, JF Schneider, CM Schmid, AK de la Figuera, J AF Quesada, A. Monti, M. Krug, I. P. Rougemaille, N. Nickel, F. Gottlob, D. M. Doganay, H. N'Diaye, A. T. Chen, G. Serrano, A. McCarty, K. F. Fernandez, J. F. Schneider, C. M. Schmid, A. K. de la Figuera, J. TI Reversible temperature-driven domain transition in bistable Fe magnetic nanostrips grown on Ru(0001) SO PHYSICAL REVIEW B LA English DT Article ID ROOM-TEMPERATURE; W(110) AB High-aspect-ratio Fe nanostrips are studied with real-space micromagnetic imaging methods. We experimentally demonstrate reversible switching from essentially homogeneous single-domain states at room temperature to multidomain diamond states at elevated temperature. This temperature-dependent magnetic bistability can be understood and modeled by accounting for the temperature dependence of the magnetocrystalline, shape, and magnetoelastic anisotropies. These results show how the transition temperature between two magnetic domain states can be tailored by controlling epitaxial strain and particle geometry, which may generate new opportunities for magnetic memory and logic device design. C1 [Quesada, A.; Serrano, A.; Fernandez, J. F.] CSIC, Inst Ceram & Vidrio, E-28049 Madrid, Spain. [Monti, M.; de la Figuera, J.] CSIC, Inst Quim Fis Rocasolano, E-28006 Madrid, Spain. [Krug, I. P.; Nickel, F.; Gottlob, D. M.; Doganay, H.; Schneider, C. M.] Res Ctr Julich GmbH, Peter Grunberg Inst PGI6, JARA FIT, D-52425 Julich, Germany. [Krug, I. P.] Tech Univ Berlin, Inst Opt & Atom Phys, D-10632 Berlin, Germany. [Rougemaille, N.] CNRS, Inst NEEL, F-38042 Grenoble, France. [Rougemaille, N.] Univ Grenoble Alpes, Inst NEEL, F-38042 Grenoble, France. [N'Diaye, A. T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Chen, G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [McCarty, K. F.] Sandia Natl Labs, Livermore, CA 94550 USA. RP Quesada, A (reprint author), CSIC, Inst Ceram & Vidrio, Plaza Murillo 2, E-28049 Madrid, Spain. EM a.quesada@icv.csic.es RI Chen, Gong/H-3074-2015; Serrano, Aida /F-4696-2016; Fernandez, Jose/M-4402-2014; Schneider, Claus/H-7453-2012; Quesada, Adrian/L-6475-2014; OI Serrano, Aida /0000-0002-6162-0014; Fernandez, Jose/0000-0001-5894-9866; Schneider, Claus/0000-0002-3920-6255; Quesada, Adrian/0000-0002-6994-0514; Monti, Matteo/0000-0003-3595-4472 FU Spanish MINECO [MAT2012-38045-C04-01, MAT2013-48009-C4-1-P]; European Commission [310516]; Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division, of the U.S. Department of Energy [DE-AC02-05CH11231]; Spanish Ministerio de Economia y Competitividad FX The authors acknowledge financial support from the Spanish MINECO through Projects No. MAT2012-38045-C04-01 and No. MAT2013-48009-C4-1-P and from the European Commission through the project NANOPYME FP7-NMP-2012-SMALL-6 NANOPYME (No. 310516). Experiments performed at the Molecular Foundry, National Center for Electron Microscopy, Lawrence Berkeley National Laboratory, were supported by the Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. A.Q. and M.M. would like to acknowledge financial support from the Spanish Ministerio de Economia y Competitividad through the Juan de la Cierva program, and through a FPI contract. NR 38 TC 1 Z9 1 U1 2 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUL 15 PY 2015 VL 92 IS 2 AR 024416 DI 10.1103/PhysRevB.92.024416 PG 6 WC Physics, Condensed Matter SC Physics GA CM9HV UT WOS:000358019900006 ER PT J AU Vasseur, R AF Vasseur, Romain TI Logarithmic correlations in quantum Hall plateau transitions SO PHYSICAL REVIEW B LA English DT Article ID NONLINEAR SIGMA-MODELS; CONFORMAL FIELD-THEORIES; SPIN CHAINS; ANOMALOUS DIMENSIONS; POTTS-MODEL; CRITICAL EXPONENTS; MINIMAL MODELS; SUPERCONDUCTORS; LOCALIZATION; PERCOLATION AB The critical behavior of quantum Hall transitions in two-dimensional disordered electronic systems can be described by a class of complicated, nonunitary conformal field theories with logarithmic correlations. The nature and the physical origin of these logarithmic correlation functions remain, however, mysterious. Using the replica trick and the underlying symmetries of these quantum critical points, we show here how to construct nonperturbatively disorder-averaged observables in terms of Green's functions that scale logarithmically at criticality. In the case of the spin quantum Hall transition, which may occur in disordered superconductors with spin-rotation symmetry and broken time reversal invariance, we argue that our results are compatible with an alternative approach based on supersymmetry. The generalization to the integer quantum Hall plateau transition is also discussed. C1 [Vasseur, Romain] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Vasseur, Romain] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Vasseur, R (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. FU Quantum Materials program of LBNL FX I wish to thank J. Cardy for useful discussions that motivated this work and for helpful comments on the manuscript. I also thank J.L. Jacobsen and H. Saleur for collaborations on related matters and J.E. Moore, A. Nahum, A.C. Potter, and especially R. Bondesan for insightful discussions and comments on the manuscript. I am supported through the Quantum Materials program of LBNL. NR 67 TC 1 Z9 1 U1 2 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 15 PY 2015 VL 92 IS 1 AR 014205 DI 10.1103/PhysRevB.92.014205 PG 16 WC Physics, Condensed Matter SC Physics GA CM9HS UT WOS:000358019400001 ER PT J AU Solvignon, P Liyanage, N Chen, JP Choi, S Slifer, K Aniol, K Averett, T Boeglin, W Camsonne, A Cates, GD Chang, CC Chudakov, E Craver, B Cusanno, F Deur, A Dutta, D Ent, R Feuerbach, R Frullani, S Gao, H Garibaldi, F Gilman, R Glashausser, C Gorbenko, V Hansen, O Higinbotham, DW Ibrahim, H Jiang, X Jones, M Kelleher, A Kelly, J Keppel, C Kim, W Korsch, W Kramer, K Kumbartzki, G LeRose, JJ Lindgren, R Ma, B Margaziotis, DJ Markowitz, P McCormick, K Meziani, ZE Michaels, R Moffit, B Monaghan, P Camacho, CM Paschke, K Reitz, B Saha, A Shneor, R Singh, J Sulkosky, V Tobias, A Urciuoli, GM Wang, K Wijesooriya, K Wojtsekhowski, B Woo, S Yang, JC Zheng, X Zhu, L AF Solvignon, P. Liyanage, N. Chen, J. -P. Choi, Seonho Slifer, K. Aniol, K. Averett, T. Boeglin, W. Camsonne, A. Cates, G. D. Chang, C. C. Chudakov, E. Craver, B. Cusanno, F. Deur, A. Dutta, D. Ent, R. Feuerbach, R. Frullani, S. Gao, H. Garibaldi, F. Gilman, R. Glashausser, C. Gorbenko, V. Hansen, O. Higinbotham, D. W. Ibrahim, H. Jiang, X. Jones, M. Kelleher, A. Kelly, J. Keppel, C. Kim, W. Korsch, W. Kramer, K. Kumbartzki, G. LeRose, J. J. Lindgren, R. Ma, B. Margaziotis, D. J. Markowitz, P. McCormick, K. Meziani, Z. -E. Michaels, R. Moffit, B. Monaghan, P. Camacho, C. Munoz Paschke, K. Reitz, B. Saha, A. Shneor, R. Singh, J. Sulkosky, V. Tobias, A. Urciuoli, G. M. Wang, K. Wijesooriya, K. Wojtsekhowski, B. Woo, S. Yang, J. -C. Zheng, X. Zhu, L. CA Jefferson Lab E01-012 Collaboratio TI Moments of the neutron g(2) structure function at intermediate Q(2) SO PHYSICAL REVIEW C LA English DT Article ID DEEP-INELASTIC-SCATTERING; PRECISION-MEASUREMENT; SUM-RULES; TARGET; ASYMMETRIES AB We present new experimental results for the He-3 spin structure function g(2) in the resonance region atQ 2 values between 1.2 and 3.0 (GeV/c)(2). Spin dependent moments of the neutron were extracted. Our main result, the inelastic contribution to the neutron d(2) matrix element, was found to be small at < Q(2)> = 2.4 (GeV/c)(2) and in agreement with the lattice QCD calculation. The Burkhardt-Cottingham sum rule for He-3 and the neutron was tested with the measured data and using the Wandzura-Wilczek relation for the low x unmeasured region. C1 [Solvignon, P.; Slifer, K.; Ma, B.] Univ New Hampshire, Durham, NH 03824 USA. [Liyanage, N.; Cates, G. D.; Craver, B.; Lindgren, R.; Paschke, K.; Singh, J.; Tobias, A.; Wang, K.; Zheng, X.] Univ Virginia, Charlottesville, VA 22904 USA. [Chen, J. -P.; Camsonne, A.; Chudakov, E.; Deur, A.; Ent, R.; Feuerbach, R.; Hansen, O.; Higinbotham, D. W.; Jones, M.; Keppel, C.; LeRose, J. J.; Michaels, R.; Reitz, B.; Saha, A.; Wojtsekhowski, B.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Choi, Seonho] Seoul Natl Univ, Seoul 151747, South Korea. [Aniol, K.; Margaziotis, D. J.] Calif State Univ Los Angeles, Los Angeles, CA 90032 USA. [Averett, T.; Kelleher, A.; Kramer, K.; Moffit, B.; Sulkosky, V.] Coll William & Mary, Williamsburg, VA 23187 USA. [Boeglin, W.; Markowitz, P.] Florida Int Univ, Miami, FL 33199 USA. [Chang, C. C.; Kelly, J.] Univ Maryland, College Pk, MD 20742 USA. [Cusanno, F.; Frullani, S.; Garibaldi, F.] Ist Nazl Fis Nucl, Grp Collegato Sanita, Sez Roma, I-00161 Rome, Italy. [Dutta, D.; Gao, H.; Wijesooriya, K.] Duke Univ, Durham, NC 27708 USA. [Gilman, R.; Glashausser, C.; Jiang, X.; Kumbartzki, G.; McCormick, K.] Rutgers State Univ, Piscataway, NJ 08855 USA. [Gorbenko, V.] Kharkov Inst Phys & Technol, UA-61108 Kharkov, Ukraine. [Ibrahim, H.] Cairo Univ, Giza 12613, Egypt. [Kim, W.; Woo, S.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Korsch, W.] Univ Kentucky, Lexington, KY 40506 USA. [Ma, B.; Monaghan, P.; Zhu, L.] MIT, Cambridge, MA 02139 USA. [Meziani, Z. -E.] Temple Univ, Philadelphia, PA 19122 USA. [Camacho, C. Munoz] Univ Clermont Ferrand, F-63177 Clermont Ferrand, France. [Camacho, C. Munoz] CNRS IN2P3 LPC, F-63177 Clermont Ferrand, France. [Shneor, R.] Tel Aviv Univ, IL-69978 Tel Aviv, Israel. [Urciuoli, G. M.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Yang, J. -C.] Chungnam Natl Univ, Taejon 305764, South Korea. RP Solvignon, P (reprint author), Univ New Hampshire, Durham, NH 03824 USA. OI Singh, Jaideep/0000-0002-4810-4824 FU NSF; DOE [DE-AC05-060R23177] FX We would like to acknowledge the outstanding support from the Jefferson Lab Hall A technical staff. This work was supported by the NSF and DOE Contract No. DE-AC05-060R23177 under which JSA, LLC operates JLab. NR 33 TC 2 Z9 2 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JUL 15 PY 2015 VL 92 IS 1 AR 015208 DI 10.1103/PhysRevC.92.015208 PG 5 WC Physics, Nuclear SC Physics GA CM9II UT WOS:000358021500001 ER PT J AU Nelson, NJ Grinstein, FF AF Nelson, Nicholas J. Grinstein, Fernando F. TI Effects of initial condition spectral content on shock-driven turbulent mixing SO PHYSICAL REVIEW E LA English DT Article ID RICHTMYER-MESHKOV INSTABILITY; LARGE-EDDY SIMULATION; RAYLEIGH-TAYLOR; MODELS; PERTURBATION; CONVECTION; DYNAMICS; RESHOCK; GROWTH AB The mixing of materials due to the Richtmyer-Meshkov instability and the ensuing turbulent behavior is of intense interest in a variety of physical systems including inertial confinement fusion, combustion, and the final stages of stellar evolution. Extensive numerical and laboratory studies of shock-driven mixing have demonstrated the rich behavior associated with the onset of turbulence due to the shocks. Here we report on progress in understanding shock-driven mixing at interfaces between fluids of differing densities through three-dimensional (3D) numerical simulations using the RAGE code in the implicit large eddy simulation context. We consider a shock-tube configuration with a band of high density gas (SF6) embedded in low density gas (air). Shocks with a Mach number of 1.26 are passed through SF6 bands, resulting in transition to turbulence driven by the Richtmyer-Meshkov instability. The system is followed as a rarefaction wave and a reflected secondary shock from the back wall pass through the SF6 band. We apply a variety of initial perturbations to the interfaces between the two fluids in which the physical standard deviation, wave number range, and the spectral slope of the perturbations are held constant, but the number of modes initially present is varied. By thus decreasing the density of initial spectral modes of the interface, we find that we can achieve as much as 25% less total mixing at late times. This has potential direct implications for the treatment of initial conditions applied to material interfaces in both 3D and reduced dimensionality simulation models. C1 [Nelson, Nicholas J.; Grinstein, Fernando F.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Nelson, NJ (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM njnelson@lanl.gov OI Nelson, Nicholas/0000-0002-4967-5258 FU Nicholas C. Metropolis Post-Doctoral Fellowship, Advanced Simulation Capabilities Initiative at Los Alamos National Laboratory; U.S. Department of Energy, NNSA [DE-AC52-06NA25396] FX We thank Jon Reisner and Betrand Rollin for their helpful contributions to the formulation of this work and Ray Ristorcelli for suggesting improvements in our analysis. N.J.N. is supported by a Nicholas C. Metropolis Post-Doctoral Fellowship as part of the Advanced Simulation Capabilities Initiative at Los Alamos National Laboratory. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the U.S. Department of Energy, NNSA, under Contract No. DE-AC52-06NA25396. NR 49 TC 0 Z9 0 U1 1 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD JUL 15 PY 2015 VL 92 IS 1 AR 013014 DI 10.1103/PhysRevE.92.013014 PG 15 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA CM9IW UT WOS:000358023100008 PM 26274276 ER PT J AU Rai, DK Beaucage, G Ratkanthwar, K Beaucage, P Ramachandran, R Hadjichristidis, N AF Rai, Durgesh K. Beaucage, Gregory Ratkanthwar, Kedar Beaucage, Peter Ramachandran, Ramnath Hadjichristidis, Nikos TI Determination of the interaction parameter and topological scaling features of symmetric star polymers in dilute solution SO PHYSICAL REVIEW E LA English DT Article ID ANGLE NEUTRON-SCATTERING; SELF-ASSEMBLING BEHAVIOR; THERMODYNAMIC PROPERTIES; ANIONIC-POLYMERIZATION; SEMIDILUTE SOLUTIONS; SHAPED POLYMERS; DRUG-DELIVERY; POLYETHYLENE; DEPENDENCE; CONFORMATIONS AB Star polymers provide model architectures to understand the dynamic and rheological effects of chain confinement for a range of complex topological structures like branched polymers, colloids, and micelles. It is important to describe the structure of such macromolecular topologies using small-angle neutron and x-ray scattering to facilitate understanding of their structure-property relationships. Modeling of scattering from linear, Gaussian polymers, such as in the melt, has applied the random phase approximation using the Debye polymer scattering function. The Flory-Huggins interaction parameter can be obtained using neutron scattering by this method. Gaussian scaling no longer applies for more complicated chain topologies or when chains are in good solvents. For symmetric star polymers, chain scaling can differ from nu = 0.5 (d(f) = 2) due to excluded volume, steric interaction between arms, and enhanced density due to branching. Further, correlation between arms in a symmetric star leads to an interference term in the scattering function first described by Benoit for Gaussian chains. In this work, a scattering function is derived which accounts for interarm correlations in symmetric star polymers as well as the polymer-solvent interaction parameter for chains of arbitrary scaling dimension using a hybrid Unified scattering function. The approach is demonstrated for linear, four-arm and eight-arm polyisoprene stars in deuterated p-xylene. C1 [Rai, Durgesh K.] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. [Beaucage, Gregory] Univ Cincinnati, Mat Sci & Engn, Cincinnati, OH 45221 USA. [Ratkanthwar, Kedar; Hadjichristidis, Nikos] Univ Athens, Dept Chem, GR-15771 Athens, Greece. [Ratkanthwar, Kedar; Hadjichristidis, Nikos] KAUST, Catalysis Ctr, Div Phys Sci & Engn, Thuwal, Saudi Arabia. [Beaucage, Peter] Cornell Univ, Dept Mat Sci & Engn, Ithaca, NY 14853 USA. [Ramachandran, Ramnath] Procter & Gamble, Cincinnati, OH 45202 USA. RP Beaucage, G (reprint author), Univ Cincinnati, Mat Sci & Engn, Cincinnati, OH 45221 USA. EM beaucag@uc.edu OI Ratkanthwar, Kedar/0000-0002-6324-696X; Rai, Durgesh/0000-0001-7257-7210 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (USA) FX The research conducted at ORNL's High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (USA). We acknowledge the support of the National Institute of Standards and Technology (USA), U.S. Department of Commerce, in providing the neutron research facilities used in this work. NR 59 TC 1 Z9 1 U1 3 U2 29 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD JUL 15 PY 2015 VL 92 IS 1 AR 012602 DI 10.1103/PhysRevE.92.012602 PG 8 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA CM9IW UT WOS:000358023100005 PM 26274195 ER PT J AU LaRue, JL Katayama, T Lindenberg, A Fisher, AS Ostrom, H Nilsson, A Ogasawara, H AF LaRue, Jerry L. Katayama, Tetsuo Lindenberg, Aaron Fisher, Alan S. Ostrom, Henrik Nilsson, Anders Ogasawara, Hirohito TI THz-Pulse-Induced Selective Catalytic CO Oxidation on Ru SO PHYSICAL REVIEW LETTERS LA English DT Article ID RAY-EMISSION SPECTROSCOPY; CARBON-MONOXIDE; FT-IRAS; DESORPTION; RU(001); SURFACE; LASER; METALS; OXYGEN; ADSORPTION AB We demonstrate the use of intense, quasi-half-cycle THz pulses, with an associated electric field component comparable to intramolecular electric fields, to direct the reaction coordinate of a chemical reaction by stimulating the nuclear motions of the reactants. Using a strong electric field from a THz pulse generated via coherent transition radiation from an ultrashort electron bunch, we present evidence that CO oxidation on Ru(0001) is selectively induced, while not promoting the thermally induced CO desorption process. The reaction is initiated by the motion of the O atoms on the surface driven by the electric field component of the THz pulse, rather than thermal heating of the surface. C1 [LaRue, Jerry L.; Katayama, Tetsuo; Nilsson, Anders; Ogasawara, Hirohito] SLAC Natl Accelerator Lab, SUNCAT Ctr Interface Sci & Catalysis, Menlo Pk, CA 94025 USA. [Lindenberg, Aaron] SLAC Natl Accelerator Lab, Stanford PULSE Inst, Menlo Pk, CA 94025 USA. [Lindenberg, Aaron] SLAC Natl Accelerator Lab, SIMES Inst Mat & Energy Sci, Menlo Pk, CA 94025 USA. [Lindenberg, Aaron] Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA. [Fisher, Alan S.] SLAC Natl Accelerator Lab, Accelerator Directorate, Menlo Pk, CA 94025 USA. [Ostrom, Henrik; Nilsson, Anders] Stockholm Univ, AlbaNova Univ Ctr, Dept Phys, SE-10691 Stockholm, Sweden. [Ogasawara, Hirohito] SLAC Natl Accelerator Lab, SSRL, Menlo Pk, CA 94025 USA. RP Ogasawara, H (reprint author), SLAC Natl Accelerator Lab, SUNCAT Ctr Interface Sci & Catalysis, Menlo Pk, CA 94025 USA. EM hirohito@slac.stanford.edu RI Ogasawara, Hirohito/D-2105-2009 OI Ogasawara, Hirohito/0000-0001-5338-1079 FU U.S. Department of Energy, Basic Energy Science, through the SUNCAT Center for Interface Science and Catalysis; Swedish Research Council; U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division FX This work is supported by the U.S. Department of Energy, Basic Energy Science, through the SUNCAT Center for Interface Science and Catalysis and the Swedish Research Council. Portions of this research were carried out at the Linac Coherent Light Source, a Directorate of SLAC National Accelerator Laboratory and an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Stanford University. AML acknowledges support by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 32 TC 5 Z9 5 U1 3 U2 30 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 15 PY 2015 VL 115 IS 3 AR 036103 DI 10.1103/PhysRevLett.115.036103 PG 5 WC Physics, Multidisciplinary SC Physics GA CM9JK UT WOS:000358024500005 PM 26230806 ER PT J AU Lidral, AC Liu, H Bullard, SA Bonde, G Machida, J Visel, A Uribe, LMM Li, X Amendt, B Cornell, RA AF Lidral, Andrew C. Liu, Huan Bullard, Steven A. Bonde, Greg Machida, Junichiro Visel, Axel Uribe, Lina M. Moreno Li, Xiao Amendt, Brad Cornell, Robert A. TI A single nucleotide polymorphism associated with isolated cleft lip and palate, thyroid cancer and hypothyroidism alters the activity of an oral epithelium and thyroid enhancer near FOXE1 SO HUMAN MOLECULAR GENETICS LA English DT Article ID GENOME-WIDE ASSOCIATION; RECEPTOR NUCLEAR TRANSLOCATOR; MAJOR GENETIC DETERMINANT; CONGENITAL HYPOTHYROIDISM; REGULATORY SEQUENCES; ABERRANT METHYLATION; POLYALANINE TRACT; CELL CARCINOMA; NEURAL CREST; SERUM TSH AB Three common diseases, isolated cleft lip and cleft palate (CLP), hypothyroidism and thyroid cancer all map to the FOXE1 locus, but causative variants have yet to be identified. In patients with CLP, the frequency of coding mutations in FOXE1 fails to account for the risk attributable to this locus, suggesting that the common risk alleles reside in nearby regulatory elements. Using a combination of zebrafish and mouse transgenesis, we screened 15 conserved non-coding sequences for enhancer activity, identifying three that regulate expression in a tissue specific pattern consistent with endogenous foxe1 expression. These three, located -82.4, -67.7 and +22.6 kb from the FOXE1 start codon, are all active in the oral epithelium or branchial arches. The -67.7 and +22.6 kb elements are also active in the developing heart, and the -67.7 kb element uniquely directs expression in the developing thyroid. Within the -67.7 kb element is the SNP rs7850258 that is associated with all three diseases. Quantitative reporter assays in oral epithelial and thyroid cell lines show that the rs7850258 allele (G) associated with CLP and hypothyroidism has significantly greater enhancer activity than the allele associated with thyroid cancer (A). Moreover, consistent with predicted transcription factor binding differences, the -67.7 kb element containing rs7850258 allele G is significantly more responsive to both MYC and ARNT than allele A. By demonstrating that this common non-coding variant alters FOXE1 expression, we have identified at least in part the functional basis for the genetic risk of these seemingly disparate disorders. C1 [Lidral, Andrew C.; Uribe, Lina M. Moreno] Univ Iowa, Dept Orthodont, Iowa City, IA 52241 USA. [Liu, Huan] Univ Iowa, Dows Res Inst, Iowa City, IA 52241 USA. [Bullard, Steven A.] Univ Iowa, Dept Endocrinol, Iowa City, IA 52241 USA. [Bonde, Greg; Li, Xiao; Amendt, Brad; Cornell, Robert A.] Univ Iowa, Dept Anat, Iowa City, IA 52241 USA. [Liu, Huan] Wuhan Univ, Sch & Hosp Stomatol, Minist Educ, State Key Lab Breeding Base Basic Sci Stomatol Hu, Wuhan 430079, Peoples R China. [Liu, Huan] Wuhan Univ, Sch & Hosp Stomatol, Minist Educ, Key Lab Oral Biomed, Wuhan 430079, Peoples R China. [Machida, Junichiro] Toyota Mem Hosp, Dept Oral & Maxillofacial Surg, Toyota, Aichi, Japan. [Visel, Axel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Genom Div, Berkeley, CA 94720 USA. [Visel, Axel] Dept Energy Joint Genome Inst, Walnut Creek, CA USA. RP Lidral, AC (reprint author), Univ Iowa, Coll Dent, Dept Orthodont, Iowa City, IA 52241 USA. EM andrew-lidral@uiowa.edu RI Visel, Axel/A-9398-2009 OI Visel, Axel/0000-0002-4130-7784 FU NCATS NIH HHS [UL1 TR000442, 2 UL1 TR000442-06]; NIDCR NIH HHS [R01 DE014667, R01 DE023575, R01DE021071, U01 DE024427, U01DE020060] NR 85 TC 6 Z9 6 U1 3 U2 9 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0964-6906 EI 1460-2083 J9 HUM MOL GENET JI Hum. Mol. Genet. PD JUL 15 PY 2015 VL 24 IS 14 BP 3895 EP 3907 DI 10.1093/hmg/ddv047 PG 13 WC Biochemistry & Molecular Biology; Genetics & Heredity SC Biochemistry & Molecular Biology; Genetics & Heredity GA CM2PV UT WOS:000357524700001 PM 25652407 ER PT J AU Socolofsky, SA Adams, EE Boufadel, MC Aman, ZM Johansen, O Konkel, WJ Lindo, D Madsen, MN North, EW Paris, CB Rasmussen, D Reed, M Ronningen, P Sim, LH Uhrenholdt, T Anderson, KG Cooper, C Nedwed, TJ AF Socolofsky, Scott A. Adams, E. Eric Boufadel, Michel C. Aman, Zachary M. Johansen, Oistein Konkel, Wolfgang J. Lindo, David Madsen, Mads N. North, Elizabeth W. Paris, Claire B. Rasmussen, Dorte Reed, Mark Ronningen, Petter Sim, Lawrence H. Uhrenholdt, Thomas Anderson, Karl G. Cooper, Cortis Nedwed, Tim J. TI Intercomparison of oil spill prediction models for accidental blowout scenarios with and without subsea chemical dispersant injection SO MARINE POLLUTION BULLETIN LA English DT Article DE Subsea blowout; Droplet size distribution; Chemical dispersant; Model prediction; Multiphase plume; Lagrangian particle tracking ID DEEP-WATER OIL; MULTIPHASE PLUMES; GAS BLOWOUTS; SYNTHETIC DISPERSANTS; INTERFACIAL-TENSION; DROPLET BREAKUP; PART I; EVOLUTION; CIRCULATION; VISCOSITY AB We compare oil spill model predictions for a prototype subsea blowout with and without subsea injection of chemical dispersants in deep and shallow water, for high and low gas-oil ratio, and in weak to strong crossflows. Model results are compared for initial oil droplet size distribution, the nearfield plume, and the farfield Lagrangian particle tracking stage of hydrocarbon transport. For the conditions tested (a blowout with oil flow rate of 20,000 bbl/d, about 1/3 of the Deepwater Horizon), the models predict the volume median droplet diameter at the source to range from 03 to 6 mm without dispersant and 0.01 to 0.8 mm with dispersant. This reduced droplet size owing to reduced interfacial tension results in a one to two order of magnitude increase in the downstream displacement of the initial oil surfacing zone and may lead to a significant fraction of the spilled oil not reaching the sea surface. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Socolofsky, Scott A.] Texas A&M Univ, Zachry Dept Civil Engn, Div Coastal & Ocean Engn, College Stn, TX 77843 USA. [Adams, E. Eric] MIT, Dept Civil & Environm Engn, RM Parsons Lab, Cambridge, MA 02139 USA. [Boufadel, Michel C.] New Jersey Inst Technol, Dept Environm Engn, Ctr Nat Resources Dev & Protect, Newark, NJ 07102 USA. [Aman, Zachary M.] Univ Western Australia, Sch Mech & Chem Engn, Ctr Energy, Crawley, WA, Australia. [Johansen, Oistein; Reed, Mark; Ronningen, Petter] SINTEF Mat & Chem, Environm Technol, Trondheim, Norway. [Konkel, Wolfgang J.] ExxonMobil Biomed Sci Inc, Annandale, NJ 08801 USA. [Lindo, David; Paris, Claire B.] Rosenstiel Sch Marine & Atmospher Sci, Miami, FL 33140 USA. [Madsen, Mads N.; Rasmussen, Dorte; Uhrenholdt, Thomas] DHI Water & Environm, Horsholm, Denmark. [North, Elizabeth W.] Univ Maryland, Ctr Environm Sci, Horn Point Lab, Cambridge, MD 21613 USA. [Sim, Lawrence H.] US DOE, Natl Energy Technol Lab, Albany, OR 97321 USA. [Anderson, Karl G.] Shell Projects & Technol, Houston, TX 77252 USA. [Cooper, Cortis] Chevron Energy Technol Corp, San Ramon, CA 94583 USA. [Nedwed, Tim J.] Upstream Res Co, Spring, TX 77339 USA. RP Socolofsky, SA (reprint author), Texas A&M Univ, Zachry Dept Civil Engn, Div Coastal & Ocean Engn, 3136 TAMU, College Stn, TX 77843 USA. EM socolofs@tamu.edu; eeadams@mit.edu; boufadel@gmail.com; zachary.aman@uwa.edu.au; oeis-joh@online.no; wolfgang.j.konkel@exxonmobil.com; dlindo@rsmas.miami.edu; mm@dhigroup.com; enorth@umces.edu; cparis@rsmas.miami.edu; dor@dhigroup.com; Mark.Reed@sintef.no; Petter.Ronningen@sintef.no; Lawrence.Sim@contr.netl.doe.gov; thu@dhigroup.com; karl.g.anderson@shell.com; cortcooper@chevron.com; tim.j.nedwed@exxonmobil.com FU API Joint Industry Task Force D3 Subsurface Dispersant Injection team; BP/Gulf of Mexico Research Initiative through the Gulf Integrated Spill Response (GISR); Center for Integrated Modeling and Analysis of the Gulf Ecosystem (C-IMAGE) consortia FX The modeling runs summarized in the paper figures were conducted pro bono by each of the modeling teams. The model intercomparison workshop and the analysis of the model results was supported jointly by the API Joint Industry Task Force D3 Subsurface Dispersant Injection team and by the BP/Gulf of Mexico Research Initiative through the Gulf Integrated Spill Response (GISR) and Center for Integrated Modeling and Analysis of the Gulf Ecosystem (C-IMAGE) consortia. NR 38 TC 19 Z9 19 U1 3 U2 30 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0025-326X EI 1879-3363 J9 MAR POLLUT BULL JI Mar. Pollut. Bull. PD JUL 15 PY 2015 VL 96 IS 1-2 BP 110 EP 126 DI 10.1016/j.marpolbul.2015.05.039 PG 17 WC Environmental Sciences; Marine & Freshwater Biology SC Environmental Sciences & Ecology; Marine & Freshwater Biology GA CM0DP UT WOS:000357348900025 PM 26021288 ER PT J AU Miao, YB Mo, K Zhou, ZJ Liu, X Lan, KC Zhang, GM Miller, MK Powers, KA Mei, ZG Park, JS Almer, J Stubbins, JF AF Miao, Yinbin Mo, Kun Zhou, Zhangjian Liu, Xiang Lan, Kuan-Che Zhang, Guangming Miller, Michael K. Powers, Kathy A. Mei, Zhi-Gang Park, Jun-Sang Almer, Jonathan Stubbins, James F. TI On the microstructure and strengthening mechanism in oxide dispersion-strengthened 316 steel: A coordinated electron microscopy, atom probe tomography and in situ synchrotron tensile investigation SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Oxide dispersion-strengthened steel; Atom probe tomography; Scanning transmission electron microscopy; Synchrotron X-ray scattering ID SMALL-ANGLE SCATTERING; NANOSTRUCTURED FERRITIC ALLOY; AUSTENITIC STAINLESS-STEEL; X-RAY-DIFFRACTION; 9CR ODS STEEL; ALPHA' PRECIPITATION; MARTENSITIC STEELS; HIGH-TEMPERATURES; DEFORMATION; IRRADIATION AB An oxide dispersion-strengthened (ODS) 316 steel was developed to simultaneously provide the advantages of ODS steels in mechanical strength and radiation tolerance as well as the excellence of austenitic steels in creep performance and corrosion resistance. The precipitate phases within the austenite matrix were identified by the combined techniques of atom probe tomography (APT), scanning transmission electron microscopy equipped with electron dispersive X-ray spectroscopy (STEM-EDS), and synchrotron wide-angle and small-angle X-ray scattering (WAXS and SAXS). Coarse TiN, hexagonal YAlO3 and orthorhombic YAlO3 precipitates were found along with fine Y-Ti-O nanoparticles. In situ WAXS experiments were performed at room and elevated temperatures to examine the size effect on the load partitioning phenomenon for TiN, hexagonal YAlO3 and Y2Ti2O7 phases. In addition, the dislocation density evolution throughout the tensile tests was analyzed by the modified Williamson-Hall method and confirmed by transmission electron microscopy (TEM) observations, revealing the difference in plasticity at various temperatures. (C) 2015 Elsevier B.V. All rights reserved. C1 [Miao, Yinbin; Liu, Xiang; Lan, Kuan-Che; Zhang, Guangming; Stubbins, James F.] Univ Illinois, Dept Nucl Plasma & Radiol Engn, Urbana, IL 61801 USA. [Mo, Kun; Mei, Zhi-Gang] Argonne Natl Lab, Nucl Engn Div, Lemont, IL 60439 USA. [Zhou, Zhangjian; Zhang, Guangming] Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing 100083, Peoples R China. [Miller, Michael K.; Powers, Kathy A.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Park, Jun-Sang; Almer, Jonathan] Argonne Natl Lab, Adv Photon Source, Lemont, IL 60439 USA. RP Miao, YB (reprint author), 216 Talbot Lab,104 South Wright St, Urbana, IL 61801 USA. EM miao2@illinois.edu RI Liu, Xiang/D-2005-2017; OI Liu, Xiang/0000-0002-2634-1888; Miao, Yinbin/0000-0002-3128-4275 FU 973 DOE INL [120293]; U.S. Department of Energy (DOE) [DEFG02-07ER46453, DE-FG02-07ER46471]; Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. DOE; DOE Office of Science [DE-AC02-06CH11357] FX This work was supported by 973 DOE INL 120293. The TEM experiments were carried out in part at the Frederick Seitz Materials Research Laboratory Central Facilities, University of Illinois, which is partially supported by the U.S. Department of Energy (DOE) under Grants DEFG02-07ER46453 and DE-FG02-07ER46471. Atom probe tomography (APT) was conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. M.K.M. was sponsored by the Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. DOE. This research used sources of the Advanced Photon Source, a U.S. DOE Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract no. DE-AC02-06CH11357. NR 68 TC 12 Z9 13 U1 9 U2 39 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD JUL 15 PY 2015 VL 639 BP 585 EP 596 DI 10.1016/j.msea.2015.05.064 PG 12 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA CM2YV UT WOS:000357549200076 ER PT J AU Castelluccio, GM McDowell, DL AF Castelluccio, Gustavo M. McDowell, David L. TI Microstructure and mesh sensitivities of mesoscale surrogate driving force measures for transgranular fatigue cracks in polycrystals SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Fatigue; Microstructure; Crystal plasticity; Cyclic loading; Probability and statistics ID HIGH-CYCLE FATIGUE; CUBIC ELASTICITY; EARLY-STAGE; SLIP; SIMULATIONS; NUCLEATION; INITIATION; MAGNESIUM; SURFACE; GROWTH AB The number of cycles required to form and grow microstructurally small fatigue cracks in metals exhibits substantial variability, particularly for low applied strain amplitudes. This variability is commonly attributed to the heterogeneity of cyclic plastic deformation within the microstructure, and presents a challenge to minimum life design of fatigue resistant components. This paper analyzes sources of variability that contribute to the driving force of transgranular fatigue cracks within nucleant grains. We employ crystal plasticity finite element simulations that explicitly render the polycrystalline microstructure and Fatigue Indicator Parameters (FlPs) averaged over different volume sizes and shapes relative to the anticipated fatigue damage process zone. Volume averaging is necessary to both achieve description of a finite fatigue damage process zone and to regularize mesh dependence in simulations. Results from constant amplitude remote applied straining are characterized in terms of the extreme value distributions of volume averaged FlPs. Grain averaged FIP values effectively mitigate mesh sensitivity, but they smear out variability within grains. Volume averaging over bands that encompass critical transgranular slip planes appear to present the most attractive approach to mitigate mesh sensitivity while preserving variability within grains. Published by Elsevier B.V. C1 [Castelluccio, Gustavo M.; McDowell, David L.] Georgia Inst Technol, George W Woodruff Sch Mech Engn, Atlanta, GA 30332 USA. [McDowell, David L.] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA. RP Castelluccio, GM (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA. EM castellg@gatech.edu FU Integrated Systems Solutions, Inc. FX G.M. Castelluccio and D.L. McDowell are grateful for the support provided by Integrated Systems Solutions, Inc. (Technical Monitor: Dr. Nam Phan, NAVAIR). NR 36 TC 4 Z9 4 U1 0 U2 10 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD JUL 15 PY 2015 VL 639 BP 626 EP 639 DI 10.1016/j.msea.2015.05.048 PG 14 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA CM2YV UT WOS:000357549200080 ER PT J AU Shin, YM Lumpkin, AH Thurman-Keup, RM AF Shin, Y. M. Lumpkin, A. H. Thurman-Keup, R. M. TI TeV/m nano-accelerator: Investigation on feasibility of CNT-channeling acceleration at Fermilab SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 6th International Conference Channeling: Charged and Neutral Particles Channeling Phenomena CY OCT 05-10, 2014 CL Capri, ITALY DE TeV/m; Channel; CNT; ASTA; Fermilab ID CHARGED-PARTICLES; CRYSTALS AB The development of high gradient acceleration and tight phase-space control of high power beams is a key element for future lepton and hadron colliders since the increasing demands for higher energy and luminosity significantly raise costs of modern HEP facilities. Atomic channels in crystals are known to consist of 10-100 V/angstrom potential barriers capable of guiding and collimating a high energy beam providing continuously focused acceleration with exceptionally high gradients (TeV/m). However, channels in natural crystals are only angstrom-size and physically vulnerable to high energy interactions, which has prevented crystals from being applied to high power accelerators. Carbon-based nano-crystals such as carbon-nanotubes (CNTs) and graphenes have a large degree of dimensional flexibility and thermomechanical strength, which could be suitable for channeling acceleration of MW beams. Nano-channels of the synthetic crystals can accept a few orders of magnitude larger phase-space volume of channeled particles with much higher thermal tolerance than natural crystals. This paper presents the current status of CNT-channeling acceleration research at the Advanced Superconducting Test Accelerator (ASTA) in Fermilab. (C) 2015 Elsevier B.V. All rights reserved. C1 [Shin, Y. M.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Shin, Y. M.; Lumpkin, A. H.; Thurman-Keup, R. M.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Shin, YM (reprint author), No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. FU DOE [DEAC02-07CH11359] FX This work was supported by the DOE contract No. DEAC02-07CH11359 to the Fermi Research Alliance LLC. We thank Darren J. Crawford, and Daniel R. Broemmelsiek of Accelerator Division (AD) and Jayakar C. Thangaraj, Philippe R. G. Piot, and Vladimir D. Shiltsev of Accelerator Physics Center (APC) in Fermi National Accelerator Laboratory (FNAL) for the helpful discussion on the idea and the support for the experimental plan. NR 36 TC 1 Z9 1 U1 2 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD JUL 15 PY 2015 VL 355 BP 94 EP 100 DI 10.1016/j.nimb.2015.03.009 PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CL8RR UT WOS:000357242300021 ER PT J AU Ma, C Tschauner, O Beckett, JR Liu, Y Rossman, GR Zhuravlev, K Prakapenka, V Dera, P Taylor, LA AF Ma, Chi Tschauner, Oliver Beckett, John R. Liu, Yang Rossman, George R. Zhuravlev, Kirill Prakapenka, Vitali Dera, Przemyslaw Taylor, Lawrence A. TI Tissintite, (Ca, Na, square)AlSi2O6, a highly-defective, shock-induced, high-pressure clinopyroxene in the Tissint martian meteorite SO EARTH AND PLANETARY SCIENCE LETTERS LA English DT Article DE tissintite; (CaNa square)AlSi2O6; new high-pressure pyroxene; Ca-Eskola; Tissint martian shergottite; synchrotron diffraction ID CRYSTAL-STRUCTURE REFINEMENT; SUBSOLIDUS PHASE-RELATIONS; CA-ESKOLA COMPONENT; ECLOGITIC CLINOPYROXENE; LOWER-MANTLE; ORDINARY CHONDRITES; MIXING PROPERTIES; SYSTEM; JADEITE; PLAGIOCLASE AB Tissintite is a new vacancy-rich, high-pressure clinopyroxene, with a composition essentially equivalent to plagioclase. It was discovered in maskelynite (shocked plagioclase) and is commonly observed included within, or in contact with, shock-melt pockets in the Tissint meteorite, a depleted olivine-phyric shergottite fall from Mars. The simple composition of tissintite (An58-69) and its precursor plagioclase (An59-69) together with the limited occurrence, both spatially (only in maskelynite less than similar to 25 mu m of a shock melt pocket) and in terms of bulk composition, make tissintite a "goldilocks" phase. It formed during a shock event severe enough to allow nucleation and growth of vacancy-rich clinopyroxene from a melt of not too calcic and not too sodic plagioclase composition that was neither too hot nor too cold. With experimental calibration, these limitations on occurrence can be used to place strong constraints on the thermal history of a shock event. The kinetics for nucleation and growth of tissintite are probably slower for more-sodic plagioclase precursors, so tissintite is most likely to occur in depleted olivinephyric shergottites like Tissint and other highly shocked meteorites and lunar and terrestrial rocks that consistently contained calcic plagioclase precursors in the appropriate compositional range for a shock of given intensity. Tissintite, (Ca0.45Na0.31 square(0.24))(Al0.97Fe0.03Mg0.01)(Si1.80Al0,20)O-6, is a C2/c clinopyroxene, containing 42-60 mol% of the Ca-Eskola component, by far the highest known. The cell parameters are a = 9.21 (17) angstrom, b = 9.09 (4) angstrom, c = 5.20 (2) angstrom, beta = 109.6 (9)degrees, V = 410 (8) angstrom(3), Z = 4. The density is 3.32 g/cm(3) and we estimate a cell volume for the Ca-Eskola end-member pyroxene of 411 +/- 13 angstrom(3), which is consistent with a previous estimate and, therefore, supports the importance of this component in clinopyroxenes from ultra-high pressure metamorphic rocks from the Earth's upper mantle. At least in C2/c clinopyroxenes as sodic as tissintite, the a- and b-cell parameters as a function of vacancy concentration intersect at similar to 0.3 vacancies pfu, much lower than the Ca-Eskola end-member (0.5), an inversion of anisotropy suggesting an elastic instability that drives clinopyroxene toward a disordered trigonal structure closely related to that of wadeite; it may mark the boundary beyond which the breakdown of vacancy-rich clinopyroxene to a wadeite-structured phase + stishovite becomes stable, although this was not observed in Tissint (C) 2015 Elsevier B.V. All rights reserved, C1 [Ma, Chi; Beckett, John R.; Rossman, George R.] CALTECH, Div Geol & Planetary Sci, Pasadena, CA 91125 USA. [Tschauner, Oliver] Univ Nevada, High Pressure Sci & Engn Ctr, Las Vegas, NV 89154 USA. [Tschauner, Oliver] Univ Nevada, Dept Geosci, Las Vegas, NV 89154 USA. [Liu, Yang] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Zhuravlev, Kirill; Prakapenka, Vitali] Univ Chicago, Argonne Natl Lab, GSECARS, Argonne, IL 60439 USA. [Dera, Przemyslaw] Univ Hawaii Manoa, Sch Ocean & Earth Sci & Technol, Hawail Inst Geophys & Planetol, Honolulu, HI 96822 USA. [Taylor, Lawrence A.] Univ Tennessee, Planetcny Geosci Inst, Dept Earth & Planetary Sci, Knoxville, TN 37996 USA. RP Ma, C (reprint author), CALTECH, Div Geol & Planetary Sci, Pasadena, CA 91125 USA. EM chi@gps.caltech.edu OI Rossman, George/0000-0002-4571-6884 FU NSF [EAR-0318518, DMR-0080065] FX SEM, EBSD and EPMA analyses were carried out at the Caltech GPS Division Analytical Facility, which is supported, in part, by NSF Grants EAR-0318518 and DMR-0080065. Synchrotron diffraction was carried out at the 13-IDD beamline of the Advanced Photon Source and the 12.2.2 beamline of the Advanced Light Source. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-ACO2-06CH11357. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-ACO2-05CH11231. OT acknowledges the support from DOE Cooperative Agreement #DE-NA0001982. GRR acknowledges NSF EAR grant 322082. YL acknowledges support from Jet Propulsion Laboratory, which is managed by California Institute of Technology under a contract with NASA, and NASA grant NNN13D465T. LAT and JRB acknowledge NASA Cosmochemistry grants NNX11AG58G and NNX12AH63G, respectively. PD gratefully acknowledges support from NSF grants EAR 1344942 and 1440005. Formal reviews by A. El Goresy and an anonymous reviewer and additional comments by T. Kubo all led to significant improvements. NR 74 TC 9 Z9 9 U1 9 U2 21 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0012-821X EI 1385-013X J9 EARTH PLANET SC LETT JI Earth Planet. Sci. Lett. PD JUL 15 PY 2015 VL 422 BP 194 EP 205 DI 10.1016/j.epsl.2015.03.057 PG 12 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CJ2YN UT WOS:000355350700020 ER PT J AU Schaef, HT Loring, JS Glezakou, VA Miller, QRS Chen, J Owen, AT Lee, MS Ilton, ES Felmy, AR McGrail, BP Thompson, CJ AF Schaef, Herbert T. Loring, John S. Glezakou, Vassiliki-Alexandra Miller, Quin R. S. Chen, Jeffrey Owen, Antoinette T. Lee, Mal-Soon Ilton, Eugene S. Felmy, Andrew R. McGrail, B. Pete Thompson, Christopher J. TI Competitive sorption of CO2 and H2O in 2:1 layer phyllosilicates SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID X-RAY-DIFFRACTION; SOCIETY SOURCE CLAYS; SUPERCRITICAL CARBON-DIOXIDE; DENSITY-FUNCTIONAL THEORY; BASE-LINE; IN-SITU; HOMOIONIC MONTMORILLONITE; HYDRATION PROPERTIES; NA-MONTMORILLONITE; WATER-VAPOR AB Expandable clays such as montmorillonite have interlayer exchange sites whose hydration state can be systematically varied from near anhydrous to almost bulk-like water conditions. This phenomenon has new significance with the simultaneous implementation of geological sequestration and secondary utilization of CO2 to both mitigate climate warming and enhance extraction of methane from hydrated clay-rich formations. In this study, the partitioning of CO2 and H2O between Na-, Ca-, and Mg-exchanged montmorillonite and variably hydrated supercritical CO2 (scCO(2)) was investigated using in situ X-ray diffraction (HXRD), infrared (IR) spectroscopic titrations, and quartz crystal microbalance (QCM) measurements. Density functional theory calculations provided mechanistic insights. Structural volumetric changes were correlated to quantified changes in sorbed H2O and CO2 concentrations as a function of percent H2O saturation in scCO(2). Intercalation of CO2 is inhibited when the clay is fully collapsed (dehydrated interlayer), peaks sharply with the introduction of some H2O and partial expansion of the interlayer region, and then decreases systematically with further hydration of the clay. This behavior is discussed in the context of recent theoretical calculations of the montmorillonite H2O-CO2 system. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Schaef, Herbert T.; Loring, John S.; Glezakou, Vassiliki-Alexandra; Chen, Jeffrey; Lee, Mal-Soon; Ilton, Eugene S.; Felmy, Andrew R.] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. [Miller, Quin R. S.] Univ Wyoming, Dept Geol & Geophys, Laramie, WY 82071 USA. [Owen, Antoinette T.; McGrail, B. Pete; Thompson, Christopher J.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. RP Schaef, HT (reprint author), Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. EM todd.schaef@pnnl.gov; chris.thompson@pnnl.gov RI Lee, Mal-Soon/K-4161-2013 OI Lee, Mal-Soon/0000-0001-6851-177X FU U.S. Department of Energy Office of Fossil Energy Research and Office of Basic Energy Sciences, Geosciences Program; DOE by Battelle Memorial Institute [DE-AC06-76RLO-1830] FX This work was funded by the U.S. Department of Energy Office of Fossil Energy Research and Office of Basic Energy Sciences, Geosciences Program. Instrument development was conducted under the Carbon Sequestration Initiative, a Laboratory Directed Research and Development program at Pacific Northwest National Laboratory (PNNL). Part of this work was performed at EMSL, a national scientific user facility at PNNL that is managed by the DOE's office of Biological and Environmental Research. The authors acknowledge useful discussions with Dr. R. Rousseau. A portion of the simulations work was performed using PNNL's Institutional Computing (PIC) program, focused on Laboratory needs and DOE missions. PNNL is operated for DOE by Battelle Memorial Institute under Contract No. DE-AC06-76RLO-1830. NR 60 TC 18 Z9 18 U1 10 U2 74 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD JUL 15 PY 2015 VL 161 BP 248 EP 257 DI 10.1016/j.gca.2015.03.027 PG 10 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CJ0BR UT WOS:000355137900014 ER PT J AU Wang, YX Liu, B Li, QY Cartmell, S Ferrara, S Deng, ZQD Xiao, J AF Wang, Yuxing Liu, Bo Li, Qiuyan Cartmell, Samuel Ferrara, Seth Deng, Zhiqun Daniel Xiao, Jie TI Lithium and lithium ion batteries for applications in microelectronic devices: A review SO JOURNAL OF POWER SOURCES LA English DT Review DE Lithium microbattery; 3D design; Materials selection; Thin-film; Review ID SILVER VANADIUM-OXIDE; SOL-GEL METHOD; ELECTROLYTIC MANGANESE-DIOXIDE; PULSED-LASER DEPOSITION; LIMN2O4 THIN-FILMS; CRYSTALLINE POLYMER ELECTROLYTES; LI4TI5O12 ANODE MATERIAL; X-RAY-DIFFRACTION; ELECTROCHEMICAL PROPERTIES; CATHODE MATERIAL AB Batteries employing lithium chemistry have been intensively investigated because of their high energy attributes which may be deployed for vehicle electrification and large-scale energy storage applications. Another important direction of battery research for micro-electronics, however, is relatively less discussed in the field but growing fast in recent years. This paper reviews chemistry and electrochemistry in different microbatteries along with their cell designs to meet the goals of their various applications. The state-of-the-art knowledge and recent progress of microbatteries for emerging micro-electronic devices may shed light on the future development of microbatteries towards high energy density and flexible design. (C) 2015 Elsevier B.V. All rights reserved. C1 [Wang, Yuxing; Liu, Bo; Li, Qiuyan; Cartmell, Samuel; Ferrara, Seth; Xiao, Jie] Pacific NW Natl Lab, Energy & Environm Directorate, Electrochem Mat & Syst Grp, Richland, WA 99352 USA. [Deng, Zhiqun Daniel] Pacific NW Natl Lab, Energy & Environm Directorate, Hydrol Tech Grp, Richland, WA 99352 USA. RP Deng, ZQD (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, Hydrol Tech Grp, Richland, WA 99352 USA. EM Zhiqun.deng@pnnl.gov; Jie.Xiao@pnnl.gov RI Deng, Daniel/A-9536-2011; Wang, Yuxing/F-3195-2017 OI Deng, Daniel/0000-0002-8300-8766; Wang, Yuxing/0000-0002-7828-9399 FU U.S. Department of Energy Wind and Water Power Technologies Office; U.S. Army Corps of Engineers, Portland District; Laboratory Directed Research and Development (LDRD) Program at PNNL FX The study was funded by the U.S. Department of Energy Wind and Water Power Technologies Office and the U.S. Army Corps of Engineers, Portland District. JX and BL would like to thank the support from The Laboratory Directed Research and Development (LDRD) Program at PNNL for the work of solid state electrolyte. The study was conducted at Pacific Northwest National Laboratory, operated by Battelle for the U.S. Department of Energy. NR 210 TC 53 Z9 54 U1 78 U2 444 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD JUL 15 PY 2015 VL 286 BP 330 EP 345 DI 10.1016/j.jpowsour.2015.03.164 PG 16 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA CI8MW UT WOS:000355027400038 ER PT J AU Smith, RP Weller, TE Howard, CA Dean, MPM Rahnejat, KC Saxena, SS Ellerby, M AF Smith, Robert P. Weller, Thomas E. Howard, Christopher A. Dean, Mark P. M. Rahnejat, Kaveh C. Saxena, Siddharth S. Ellerby, Mark TI Superconductivity in graphite intercalation compounds SO PHYSICA C-SUPERCONDUCTIVITY AND ITS APPLICATIONS LA English DT Article DE Intercalation; Superconductivity; Graphite; Low-dimension ID MEDIATED SUPERCONDUCTIVITY; LITHIUM; METAL; GRAPHENE; SODIUM; STAGE; STATE; CAC6; C6CA; BAC6 AB The field of superconductivity in the class of materials known as graphite intercalation compounds has a history dating back to the 1960s (Dresselhaus and Dresselhaus, 1981; Enoki et al., 2003). This paper recontextualizes the field in light of the discovery of superconductivity in CaC6 and YbC6 in 2005. In what follows, we outline the crystal structure and electronic structure of these and related compounds. We go on to experiments addressing the superconducting energy gap, lattice dynamics, pressure dependence, and how these relate to theoretical studies. The bulk of the evidence strongly supports a BCS superconducting state. However, important questions remain regarding which electronic states and phonon modes are most important for superconductivity, and whether current theoretical techniques can fully describe the dependence of the superconducting transition temperature on pressure and chemical composition. (C) 2015 Elsevier B.V. All rights reserved. C1 [Smith, Robert P.; Saxena, Siddharth S.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Weller, Thomas E.; Howard, Christopher A.; Rahnejat, Kaveh C.; Ellerby, Mark] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Dean, Mark P. M.] Brookhaven Natl Lab, Dept Condensed Matter Phys & Mat Sci, Upton, NY 11973 USA. RP Ellerby, M (reprint author), UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. EM mark.ellerby@ucl.ac.uk RI Saxena, Siddharth/D-2025-2012; Dean, Mark/B-4541-2011; Smith, Robert/A-1286-2014 OI Saxena, Siddharth/0000-0002-6321-5629; Dean, Mark/0000-0001-5139-3543; Smith, Robert/0000-0002-6881-5690 FU EPSRC; Royal Society, University College London; Cavendish Laboratory-Cambridge; U.S. Department of Energy (DOE), Division of Materials Science [DE-SC0012704] FX We would like to acknowledge the EPSRC, the Royal Society, University College London and Cavendish Laboratory-Cambridge for their support and financial contributions. The work at Brookhaven National Laboratory was supported by the U.S. Department of Energy (DOE), Division of Materials Science, under Contract No. DE-SC0012704. NR 66 TC 6 Z9 6 U1 8 U2 50 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0921-4534 EI 1873-2143 J9 PHYSICA C JI Physica C PD JUL 15 PY 2015 VL 514 BP 50 EP 58 DI 10.1016/j.physc.2015.02.029 PG 9 WC Physics, Applied SC Physics GA CI2IC UT WOS:000354568600007 ER PT J AU Bud'ko, SL Canfield, PC AF Bud'ko, Sergey L. Canfield, Paul C. TI Superconductivity of magnesium diboride SO PHYSICA C-SUPERCONDUCTIVITY AND ITS APPLICATIONS LA English DT Article DE Magnesium diboride; Two-band superconductivity; Superconducting gap; BCS ID MGB2 THIN-FILMS; POINT-CONTACT SPECTROSCOPY; UPPER CRITICAL-FIELD; ALUMINUM-DOPED MGB2; TRANSITION-TEMPERATURE; 2-BAND SUPERCONDUCTOR; ANISOTROPY PARAMETERS; TRANSPORT-PROPERTIES; SINGLE-CRYSTALS; PRESSURE AB Over the past 14 years MgB2 has gone from a startling discovery to a promising, applied superconductor. In this article we present a brief overview of the synthesis and the basic superconducting properties of this remarkable compound. In particular, the effect of pressure, substitutions and neutron irradiation on superconducting properties are discussed. (C) 2015 Elsevier B.V. All rights reserved. C1 [Bud'ko, Sergey L.] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Bud'ko, SL (reprint author), Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. EM budko@ameslab.gov FU U.S. Department of Energy, Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-07CH11358] FX Work at the Ames Laboratory was supported by the U.S. Department of Energy, Basic Energy Sciences, Division of Materials Sciences and Engineering under Contract No. DE-AC02-07CH11358. NR 116 TC 4 Z9 4 U1 3 U2 74 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0921-4534 EI 1873-2143 J9 PHYSICA C JI Physica C PD JUL 15 PY 2015 VL 514 BP 142 EP 151 DI 10.1016/j.physc.2015.02.024 PG 10 WC Physics, Applied SC Physics GA CI2IC UT WOS:000354568600014 ER PT J AU Sarrao, JL Bauer, ED Mitchell, JN Tobash, PH Thompson, JD AF Sarrao, J. L. Bauer, E. D. Mitchell, J. N. Tobash, P. H. Thompson, J. D. TI Superconductivity in plutonium compounds SO PHYSICA C-SUPERCONDUCTIVITY AND ITS APPLICATIONS LA English DT Article DE Plutonium; Superconductivity; PuCoGa5 ID SINGLE-CRYSTAL GROWTH; PUCOGA5; SPIN; SPECTROSCOPY; TEMPERATURE; ACTINIDES; ELECTRONS; PURHGA5; PU AB Although the family of plutonium-based superconductors is relatively small, consisting of four compounds all of which crystallize in the tetragonal HoCoGa5 structure, these materials serve as an important bridge between the known Ce- and U-based heavy fermion superconductors and the high-temperature cuprate superconductors. Further, the partial localization of 5f electrons that characterizes the novel electronic properties of elemental plutonium appears to be central to the relatively high superconducting transition temperatures that are observed in PuCoGa5, PuRhGa5, PuCoIn5, and PuRhIn5. (C) 2015 Elsevier B.V. All rights reserved. C1 [Sarrao, J. L.; Bauer, E. D.; Mitchell, J. N.; Tobash, P. H.; Thompson, J. D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Sarrao, JL (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM sarrao@lanl.gov OI Mitchell, Jeremy/0000-0001-7109-3505; Bauer, Eric/0000-0003-0017-1937 FU Office of Basic Energy Sciences, Division of Materials Science and Engineering; Los Alamos National Laboratory Laboratory Directed Research and Development (LDRD) program; U.S. Department of Energy FX Work at Los Alamos National Laboratory was performed under the auspices of the U.S. Department of Energy and was supported by the Office of Basic Energy Sciences, Division of Materials Science and Engineering as well as the Los Alamos National Laboratory Laboratory Directed Research and Development (LDRD) program. NR 47 TC 2 Z9 2 U1 2 U2 21 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0921-4534 EI 1873-2143 J9 PHYSICA C JI Physica C PD JUL 15 PY 2015 VL 514 BP 184 EP 188 DI 10.1016/j.physc.2015.02.031 PG 5 WC Physics, Applied SC Physics GA CI2IC UT WOS:000354568600018 ER PT J AU White, BD Thompson, JD Maple, MB AF White, B. D. Thompson, J. D. Maple, M. B. TI Unconventional superconductivity in heavy-fermion compounds SO PHYSICA C-SUPERCONDUCTIVITY AND ITS APPLICATIONS LA English DT Article DE Unconventional superconductivity; Heavy-fermion behavior; Quantum critical point; Non-Fermi liquid behavior; Magnetic fluctuations; Kondo lattice ID PRESSURE-INDUCED SUPERCONDUCTIVITY; UPPER CRITICAL-FIELD; CRITICAL MAGNETIC-FIELD; QUANTUM CRITICAL-POINT; F-ELECTRON MATERIALS; HIGH-TEMPERATURE SUPERCONDUCTIVITY; KONDO-LATTICE; NEUTRON-SCATTERING; PHASE-DIAGRAM; HIDDEN ORDER AB Over the past 35 years, research on unconventional superconductivity in heavy-fermion systems has evolved from the surprising observations of unprecedented superconducting properties in compounds that convention dictated should not superconduct at all to performing explorations of rich phase spaces in which the delicate interplay between competing ground states appears to support emergent superconducting states. In this article, we review the current understanding of superconductivity in heavy-fermion compounds and identify a set of characteristics that is common to their unconventional superconducting states. These core properties are compared with those of other classes of unconventional superconductors such as the cuprates and iron-based superconductors. We conclude by speculating on the prospects for future research in this field and how new advances might contribute towards resolving the long-standing mystery of how unconventional superconductivity works. (C) 2015 Elsevier B.V. All rights reserved. C1 [White, B. D.; Maple, M. B.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [White, B. D.; Maple, M. B.] Univ Calif San Diego, Ctr Adv Nanosci, La Jolla, CA 92093 USA. [Thompson, J. D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Maple, MB (reprint author), Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. EM mbmaple@ucsd.edu FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-FG02-04-ER46105]; National Science Foundation [DMR-1206553]; National Nuclear Security Administration under the Stewardship Science Academic Alliance program, the U.S. Department of Energy [DE-NA0001841]; U.S. DOE Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; U.S. Department of Energy FX Work at the University of California, San Diego was performed with financial support from the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award Grant No. DE-FG02-04-ER46105, the National Science Foundation under Grant No. DMR-1206553, and the National Nuclear Security Administration under the Stewardship Science Academic Alliance program through the U.S. Department of Energy Grant No. DE-NA0001841. Work at Los Alamos was performed under the auspices of the U.S. Department of Energy and was supported by the U.S. DOE Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. NR 421 TC 10 Z9 10 U1 6 U2 71 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0921-4534 EI 1873-2143 J9 PHYSICA C JI Physica C PD JUL 15 PY 2015 VL 514 BP 246 EP 278 DI 10.1016/j.physc.2015.02.044 PG 33 WC Physics, Applied SC Physics GA CI2IC UT WOS:000354568600024 ER PT J AU Chu, CW Canfield, PC Dynes, RC Fisk, Z Batlogg, B Deutscher, G Geballe, TH Zhao, ZX Greene, RL Hosono, H Maple, MB AF Chu, C. W. Canfield, P. C. Dynes, R. C. Fisk, Z. Batlogg, B. Deutscher, G. Geballe, T. H. Zhao, Z. X. Greene, R. L. Hosono, H. Maple, M. B. TI Epilogue: Superconducting materials past, present and future SO PHYSICA C-SUPERCONDUCTIVITY AND ITS APPLICATIONS LA English DT Editorial Material DE Epilogue; Room temperature superconductivity; Perspectives AB Experimental contributors to the field of superconducting materials share their informal views on the subject. (C) 2015 Published by Elsevier B.V. C1 [Chu, C. W.] Univ Houston, Dept Phys, Houston, TX 77004 USA. [Chu, C. W.] Univ Calif San Diego, Texas Ctr Superconduct, La Jolla, CA 92093 USA. [Canfield, P. C.] US DOE, Ames Lab, Ames, IA 50011 USA. [Canfield, P. C.] Iowa State Univ Sci & Technol, Dept Phys & Astron, Ames, IA 50011 USA. [Dynes, R. C.; Maple, M. B.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Fisk, Z.] Univ Calif Irvine, Dept Phys, Irvine, CA 92697 USA. [Batlogg, B.] Swiss Fed Inst Technol, Lab F Festkorperphys, Zurich, Switzerland. [Deutscher, G.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Geballe, T. H.] Stanford Univ, Dept Appl Phys & Mat Sci, Stanford, CA 94305 USA. [Zhao, Z. X.] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Greene, R. L.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Hosono, H.] Tokyo Inst Technol, Mat & Struct Lab, Midori Ku, Yokohama, Kanagawa 2268503, Japan. RP Maple, MB (reprint author), Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. EM mbmaple@ucsd.edu RI Hosono, Hideo/J-3489-2013 OI Hosono, Hideo/0000-0001-9260-6728 NR 15 TC 1 Z9 1 U1 4 U2 44 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0921-4534 EI 1873-2143 J9 PHYSICA C JI Physica C PD JUL 15 PY 2015 VL 514 BP 437 EP 443 DI 10.1016/j.physc.2015.03.003 PG 7 WC Physics, Applied SC Physics GA CI2IC UT WOS:000354568600036 ER PT J AU Aranda, MM Rementeria, R Poplawsky, J Urones-Garrote, E Capdevila, C AF Aranda, M. M. Rementeria, R. Poplawsky, J. Urones-Garrote, E. Capdevila, C. TI The role of C and Mn at the austenite/pearlite reaction front during non-steady-state pearlite growth in a Fe-C-Mn steel SO SCRIPTA MATERIALIA LA English DT Article DE Divergent pearlite; Interface diffusion; Growth rate; Pearlitic steel ID EUTECTOID STEEL AB The role of C and Mn during the growth of pearlite under non-steady state conditions is analyzed by comparing phase compositions of austenite, ferrite and cementite (gamma+alpha+theta) through the use of transmission electron microscopy (TEM), energy dispersive X-ray spectroscopy (EDS), and atom probe tomography (APT) measurements across the austenite/pearlite interface. A local Mn enrichment and C depletion at the austenite/pearlite interface has been measured, which causes a change in the transformation driving force with time during divergent pearlite growth. (C) 2015 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Aranda, M. M.; Rementeria, R.; Capdevila, C.] CENIM CSIC, Mat Res Grp, Madrid 28040, Spain. [Poplawsky, J.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Urones-Garrote, E.] Univ Complutense Madrid, Fac Ciencias Quim, CNME, E-28040 Madrid, Spain. RP Aranda, MM (reprint author), CENIM CSIC, Mat Res Grp, Avda Gregorio Amo 8, Madrid 28040, Spain. RI Poplawsky, Jonathan/Q-2456-2015; OI Poplawsky, Jonathan/0000-0002-4272-7043; Rementeria, Rosalia/0000-0003-2364-7344 FU ORNL's Center for Nanophase Materials Sciences (CNMS), a U.S. Department of Energy, Office of Science User Facility; MINECO; FEDER [ENE2009-13766-C04-01, MAT2013-47460-C5-2-P] FX The authors acknowledge Acerinox for manufacturing the steel. This research was supported by ORNL's Center for Nanophase Materials Sciences (CNMS), which is a U.S. Department of Energy, Office of Science User Facility. Authors acknowledge financial support to MINECO and FEDER in the form of ENE2009-13766-C04-01 and MAT2013-47460-C5-2-P projects. NR 9 TC 4 Z9 4 U1 1 U2 22 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6462 J9 SCRIPTA MATER JI Scr. Mater. PD JUL 15 PY 2015 VL 104 BP 67 EP 70 DI 10.1016/j.scriptamat.2015.04.005 PG 4 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA CI8VZ UT WOS:000355051100018 ER PT J AU Choi, KS Zhu, ZH Sun, X De Moor, E Taylor, MD Speer, JG Matlock, DK AF Choi, Kyoo Sil Zhu, Zihua Sun, Xin De Moor, Emmanuel Taylor, Mark D. Speer, John G. Matlock, David K. TI Determination of carbon distributions in quenched and partitioned microstructures using nanoscale secondary ion mass spectroscopy SO SCRIPTA MATERIALIA LA English DT Article DE Nano-SIMS; EBSD; Carbon partitioning kinetics; Quenching and partitioning ID Q-AND-P; AUSTENITE; STEEL; MARTENSITE; BAINITE; TRANSFORMATION; ELEMENTS AB A multi-modal characterization technique, which combines nanoscale secondary ion mass spectroscopy (Nano-SIMS) with a spatial resolution of similar to 100 nm and electron back scatter diffraction (EBSD) to determine carbon distributions in austenite and martensite in a quenched and partitioned (Q&P) Fe-0.29C-2.95Mn-1.59Si steel is presented. Significant carbon enrichment of austenite was measured with decreased levels of carbon in martensite, supporting the carbon partitioning mechanism. Fresh untempered martensite could be identified, and different degrees of enrichment were observed for blocky and lath austenite. (C) 2015 Published by Elsevier Ltd. on behalf of Acta Materialia Inc. C1 [Choi, Kyoo Sil; Zhu, Zihua; Sun, Xin] Pacific NW Natl Lab, Richland, WA 99352 USA. [De Moor, Emmanuel; Taylor, Mark D.; Speer, John G.; Matlock, David K.] Colorado Sch Mines, Adv Steel Proc & Prod Res Ctr ASPPRC, Golden, CO 80401 USA. RP Choi, KS (reprint author), Pacific NW Natl Lab, POB 999, Richland, WA 99352 USA. EM kyoosil.choi@pnnl.gov RI de moor, emmanuel/E-9373-2012; Zhu, Zihua/K-7652-2012 OI de moor, emmanuel/0000-0001-6538-1121; FU US Department of Energy (DOE) [DE-AC05-76RL01830]; DOE's Vehicle Technologies Office under the Automotive Lightweight Materials Program; Office of Biological and Environmental Research; ASPPRC, an industry-university cooperative research center at the Colorado School of Mines FX PNNL is operated by the Battelle Memorial Institute for the US Department of Energy (DOE) under Contract No. DE-AC05-76RL01830. This work was funded by the DOE's Vehicle Technologies Office under the Automotive Lightweight Materials Program managed by Mr. William Joost. The Nano-SIMS experiment was performed in Environmental Molecular Sciences Laboratory, a DOE Office of Science User Facility sponsored by the Office of Biological and Environmental Research and located at PNNL. The support from the sponsors of the ASPPRC, an industry-university cooperative research center at the Colorado School of Mines, is also gratefully acknowledged. NR 24 TC 6 Z9 6 U1 2 U2 26 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6462 J9 SCRIPTA MATER JI Scr. Mater. PD JUL 15 PY 2015 VL 104 BP 79 EP 82 DI 10.1016/j.scriptamat.2015.03.027 PG 4 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA CI8VZ UT WOS:000355051100021 ER PT J AU Boncher, WL Lin, TC Cordes, NL Hehlen, MP AF Boncher, William L. Lin, Terri C. Cordes, Nikolaus L. Hehlen, Markus P. TI Sequestration of cerium(III) bromide into mesoporous silica SO MICROPOROUS AND MESOPOROUS MATERIALS LA English DT Article DE Cerium bromide; Scintillator; Mesoporous silica ID REFRACTIVE-INDEX; SCINTILLATORS AB A variety of surface-functionalized mesoporous silica monoliths were reacted with a cerium(III) bromide molecular complex and a successful scaffold for luminescent materials is demonstrated. The variation in structure of the materials is shown through infrared spectroscopy, and the luminescent properties illustrate the varying coordination environment of cerium(III) bromide. (C) 2015 Elsevier Inc. All rights reserved. C1 [Boncher, William L.; Lin, Terri C.; Cordes, Nikolaus L.; Hehlen, Markus P.] Los Alamos Natl Lab, Mat Sci & Technol, Polymers & Coatings, Los Alamos, NM 87545 USA. RP Boncher, WL (reprint author), Los Alamos Natl Lab, Mat Sci & Technol, Polymers & Coatings, Mailstop E549,POB 1663, Los Alamos, NM 87545 USA. EM boncher@lanl.gov OI Boncher, William/0000-0001-9155-5527; Cordes, Nikolaus/0000-0003-3367-5592 FU Department of Energy (DOE) Los Alamos National Laboratory (LANL) Laboratory Directed Research and Development (LDRD) program [20120246ER] FX This work is supported by the Department of Energy (DOE) Los Alamos National Laboratory (LANL) Laboratory Directed Research and Development (LDRD) program, 20120246ER. NR 31 TC 1 Z9 1 U1 0 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1387-1811 EI 1873-3093 J9 MICROPOR MESOPOR MAT JI Microporous Mesoporous Mat. PD JUL 15 PY 2015 VL 211 BP 158 EP 161 DI 10.1016/j.micromeso.2015.03.007 PG 4 WC Chemistry, Applied; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CH9EZ UT WOS:000354340100019 ER PT J AU Khadilkar, AB Rozelle, PL Pisupati, SV AF Khadilkar, Aditi B. Rozelle, Peter L. Pisupati, Sarma V. TI A study on initiation of ash agglomeration in fluidized bed gasification systems SO FUEL LA English DT Article DE Reducing; Mineral matter transformation; Particle; Ash; High rank coal; FactSage (TM) ID COAL ASH; BEHAVIOR; COMBUSTION AB Agglomeration in fluidized beds begins locally by the sticking of slag-liquid-covered particles. Analysis of the composite fuel is not adequate in predicting agglomeration problems. Separation of the high rank Pittsburgh seam coal into particle classes based on specific gravity (SG1: < 1.3 g/cm(3); SG2: 1.3-1.6 g/cm(3); SG3: 1.6-2.6 g/cm(3) and SG4: > 2.6 g/cm(3)) and particle size (PS1 through PS7) helped to identify important particle-level slag-liquid formation tendencies. Slag-liquid formation tendencies under fluidized bed operating temperatures were determined both computationally and experimentally. Particles rich in certain iron and calcium phases melt at very low temperatures that are well within fluidized bed operating conditions. The iron rich particle classes (SG3 and SG4) showed the presence of several phases containing iron in different oxidation states. The presence of these iron phases was not detected in the composite bulk fuel. The possibilities of equilibrium liquid phase formation in the presence of different ratios of these iron and calcium oxides to alumino-silicates were determined. Presence of hematite was found to delay slag-liquid formation. Each of the particle classes showed distinct slag-liquid formation tendencies that indicate initiation of agglomeration around SG3 and SG4 particles. The study revealed the importance of particle class-level differences in mineral matter composition for the prediction of agglomeration during fluidized bed gasification. A novel integrated ash agglomeration model that accounts for particle hydrodynamics as well as particle class level ash chemistry has been outlined to predict agglomeration kinetics. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Khadilkar, Aditi B.; Pisupati, Sarma V.] Penn State Univ, John & Willie Leone Family Dept Energy & Mineral, University Pk, PA 16802 USA. [Khadilkar, Aditi B.; Pisupati, Sarma V.] Penn State Univ, EMS Energy Inst, University Pk, PA 16802 USA. [Rozelle, Peter L.] US DOE, Off Fossil Energy, Washington, DC 20585 USA. [Khadilkar, Aditi B.; Pisupati, Sarma V.] Natl Energy Technol Lab, Morgantown, WV 26507 USA. RP Pisupati, SV (reprint author), Penn State Univ, John & Willie Leone Family Dept Energy & Mineral, University Pk, PA 16802 USA. EM sxp17@psu.edu FU National Energy Technology Laboratory (USDOE) under the RES contract [0004000] FX Financial support for this work was partially provided by National Energy Technology Laboratory (USDOE) under the RES contract 0004000. NR 31 TC 4 Z9 4 U1 1 U2 24 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0016-2361 EI 1873-7153 J9 FUEL JI Fuel PD JUL 15 PY 2015 VL 152 BP 48 EP 57 DI 10.1016/j.fuel.2015.01.039 PG 10 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA CG3VF UT WOS:000353207000007 ER PT J AU Bo, SH Grey, CP Khalifah, PG AF Bo, Shou-Hang Grey, Clare P. Khalifah, Peter G. TI Defect-Tolerant Diffusion Channels for Mg2+ Ions in Ribbon-Type Borates: Structural Insights into Potential Battery Cathodes MgVBO4 and MgxFe2-xB2O5 SO CHEMISTRY OF MATERIALS LA English DT Article ID RECHARGEABLE MAGNESIUM BATTERIES; HIGH-CAPACITY; LITHIUM BATTERIES; CRYSTAL-STRUCTURE; MG2B2O5 NANOWIRES; ELECTRODES; OLIVINES; VISUALIZATION; CONSTRAINTS; WARWICKITES AB The reversible room temperature intercalation of Mg2+ ions is difficult to achieve but may offer substantial advantages in the design of next-generation batteries if this electrochemical process can be successfully realized. Two types of quadruple ribbon-type transition metal borates (MgxFe2-xB2O5 and MgVBO4) with high theoretical capacities (186 and 360 mAh/g) have been synthesized and structurally characterized through the combined Rietveld refinement of synchrotron and time-of-flight neutron diffraction data. Neither MgVBO4 nor MgxFe2-xB2O5 can be chemically oxidized at room temperature, though Mg can be dynamically removed from the latter phase at elevated temperatures (approximately 200-500 degrees C). It is found that Mg diffusion in the MgxFe2-xB2O5 structure is more facile for the inner two octahedral sites than for the two outer octahedral sites in the ribbons, a result supported by both the refined site occupancies after Mg removal and bond valence sum difference map calculations of diffusion paths in the pristine material. Mg diffusion in this pyroborate MgxFe2-xB2O5 framework is also found to be tolerant to the presence of Mg/Fe disorder since Mg ions can diffuse through interstitial channels which bypass Fe-containing sites. C1 [Bo, Shou-Hang; Grey, Clare P.; Khalifah, Peter G.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Grey, Clare P.] Univ Cambridge, Dept Chem, Cambridge CB2 1EW, England. [Khalifah, Peter G.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Grey, CP (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. EM cpg27@cam.ac.uk; kpete@bnl.gov FU North East Center for Chemical Energy Storage (NECCES), an Energy Frontier Research Center - U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0012583]; Brookhaven National Laboratory [DEAC02-98CH10086]; U.S. Department of Energy; Office of Basic Energy Sciences, U.S. Department of Energy, at the Spallation Neutron Source, Oak Ridge National Laboratory [DEAC05-00OR22725]; UT Battelle; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX Research supported as part of the North East Center for Chemical Energy Storage (NECCES), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Basic Energy Sciences, under Award # DE-SC0012583, including matching support from NYSTAR-NYSERDA. This work was carried out in part at Brookhaven National Laboratory under Contract No. DEAC02-98CH10086 with the U.S. Department of Energy. Neutron diffraction studies were supported by the Office of Basic Energy Sciences, U.S. Department of Energy, at the Spallation Neutron Source, Oak Ridge National Laboratory under contract DEAC05-00OR22725 with UT Battelle. The POWGEN beamline staff, and in particular, Dr. P. Whitfield, are greatly acknowledged for their help in the neutron powder diffraction data collection and for stimulating discussions on TOP neutron diffraction. Use of the Advanced Photon Source (11-BM beamline) at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. We thank Dr. Sian Dutton and Mr. Hugh Glass for many helpful discussions concerning magnesium metal borate compounds. We also thank Dr. Kyung-Wan Nam for X-ray absorption spectroscopy measurement and Mr. Jue Liu for his assistance in the chemical oxidation experiments. NR 43 TC 9 Z9 9 U1 9 U2 68 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUL 14 PY 2015 VL 27 IS 13 BP 4630 EP 4639 DI 10.1021/acs.chemmater.5b01040 PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CN0LI UT WOS:000358104700016 ER PT J AU Ramasamy, K Kotula, PG Fidler, AF Brumbach, MT Pietryga, JM Ivanov, SA AF Ramasamy, Karthik Kotula, Paul G. Fidler, Andrew F. Brumbach, Michael T. Pietryga, Jeffrey M. Ivanov, Sergei A. TI SnxGe1-x Alloy Nanocrystals: A First Step toward Solution-Processed Group IV Photovoltaics SO CHEMISTRY OF MATERIALS LA English DT Article ID GERMANIUM NANOCRYSTALS; QUANTUM DOTS; SOLAR-CELLS; GAP MATERIALS; ENERGY-GAP; SN; SI AB Nontoxic, sustainable, and cost-effective, Group IV materials are attractive for a broad range of electronic and optoelectronic applications, although the indirect principal band gaps of silicon and germanium (Ge) present complications that impact device design and cost. Previous studies have shown that the band structures of these materials can be modified by the influence of quantum confinement in nanostructures or by alloying with tin (Sn) in metastable thin films; to date, neither method has produced a material with a direct band gap of appropriate energy for application in, for example, efficient solar photovoltaics. We have developed a facile colloidal method for the synthesis of size-controlled, homogeneous SnxGe1-x alloy nanocrystals (NCs) with remarkably high tin concentration (x up to 0.42). We demonstrate that NCs of the same size exhibit a pronounced, systematic red-shift in the optical band gap, and a significant increase in molar absorptivity, with increasing Sn-content, and a measurable photoluminescence was observed from NCs with high contents. The indications of at least partial direct-gap character in these NCs, combined with their broad tunability throughout the infrared, suggest their promise for use in solution-processed solar cells. C1 [Ramasamy, Karthik; Ivanov, Sergei A.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Fidler, Andrew F.; Pietryga, Jeffrey M.] Los Alamos Natl Lab, Ctr Adv Solar Photophys, Los Alamos, NM 87545 USA. [Kotula, Paul G.; Brumbach, Michael T.] Sandia Natl Labs, Mat Characterizat Dept, Albuquerque, NM 87185 USA. RP Ivanov, SA (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. EM ivanov@lanl.gov RI Kotula, Paul/A-7657-2011; Ivanov, Sergei/B-5505-2011 OI Kotula, Paul/0000-0002-7521-2759; FU Center for Advanced Solar Photophysics (CASP), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; LANL Director's Postdoctoral Fellowship; LANL LDRD; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396]; U.S. Department of Energy [DEAC04-94AL85000] FX J.M.P. acknowledges the support of the Center for Advanced Solar Photophysics (CASP), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. A.F.F. is supported by a LANL Director's Postdoctoral Fellowship. K.R. is supported by a LANL LDRD funding. This work was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE), Office of Science. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the U.S. Department of Energy under Contract No. DEAC04-94AL85000. NR 42 TC 8 Z9 8 U1 7 U2 41 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUL 14 PY 2015 VL 27 IS 13 BP 4640 EP 4649 DI 10.1021/acs.chemmater.5b01041 PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CN0LI UT WOS:000358104700017 ER PT J AU Kirkeminde, A Shen, J Gong, MG Cui, J Ren, SQ AF Kirkeminde, Alec Shen, Jian Gong, Maogang Cui, Jun Ren, Shenqiang TI Metal-Redox Synthesis of MnBi Hard Magnetic Nanoparticles SO CHEMISTRY OF MATERIALS LA English DT Article ID LOW-TEMPERATURE PHASE; ELECTRONIC-STRUCTURE AB High coercivity MnBi alloy is a promising candidate as earth abundant permanent magnet for energy-critical technologies. We report here a new metal-redox method to synthesize colloidal MnBi nanoparticles, exhibiting a saturation magnetization of 49 emu/g and coercivity of 15 kOe. It is shown that the magnetic properties of the MnBi nanoalloys can be readily modified by precursor stoichiometry, temperature ramp rate, and reaction temperature, making it a versatile scalable strategy for generation of MnBi. C1 [Kirkeminde, Alec; Ren, Shenqiang] Univ Kansas, Dept Chem, Lawrence, KS 66045 USA. [Shen, Jian; Gong, Maogang; Ren, Shenqiang] Temple Univ, Dept Mech Engn, Philadelphia, PA 19122 USA. [Cui, Jun] Pacific NW Natl Lab, Richland, WA USA. RP Gong, MG (reprint author), Temple Univ, Dept Mech Engn, Philadelphia, PA 19122 USA. EM gongmaogang207@163.com; shenqiang.ren@temple.edu RI Gong, Maogang/B-3588-2016 OI Gong, Maogang/0000-0002-2031-781X FU U.S. National Science Foundation (NSF) [NSF-DMR-1451326]; [NSF-CMMI-1332658] FX This work is funded by the U.S. National Science Foundation (NSF) under Award NSF-DMR-1451326 (CAREER, magnetically hard nanocrystals) and NSF-CMMI-1332658 (nano-manufacturing through metal-redox). NR 18 TC 8 Z9 8 U1 9 U2 51 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUL 14 PY 2015 VL 27 IS 13 BP 4677 EP 4681 DI 10.1021/acs.chemmater.5b01224 PG 5 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CN0LI UT WOS:000358104700021 ER PT J AU Kim, IS Borycz, J Platero-Prats, AE Tussupbayev, S Wang, TC Farha, OK Hupp, JT Gagliardi, L Chapman, KW Cramer, CJ Martinson, ABF AF Kim, In Soo Borycz, Joshua Platero-Prats, Ana E. Tussupbayev, Samat Wang, Timothy C. Farha, Omar K. Hupp, Joseph T. Gagliardi, Laura Chapman, Karena W. Cramer, Christopher J. Martinson, Alex B. F. TI Targeted Single-Site MOF Node Modification: Trivalent Metal Loading via Atomic Layer Deposition SO CHEMISTRY OF MATERIALS LA English DT Article ID ASSISTED LIGAND INCORPORATION; INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; ORGANIC FRAMEWORKS; CATALYSIS; FUNCTIONALIZATION; ADSORPTION; EFFICIENT; VANADIUM AB Postsynthetic functionalization of metal organic frameworks (MOFs) enables the controlled, high-density incorporation of new atoms on a crystallographically precise framework. Leveraging the broad palette of known atomic layer deposition (ALD) chemistries, ALD in MOFs (AIM) is one such targeted approach to construct diverse, highly functional, few-atom clusters. We here demonstrate the saturating reaction of trimethylindium (InMe3) with the node hydroxyls and ligated water of NU-1000, which takes place without significant loss of MOF crystallinity or internal surface area. We computationally identify the elementary steps by which trimethylated trivalent metal compounds (ALD precursors) react with this Zr-based MOP node to generate a uniform and well characterized new surface layer on the node itself, and we predict a final structure that is fully consistent with experimental X-ray pair distribution function (PDF) analysis. We further demonstrate tunable metal loading through controlled number density of the reactive handles (-OH and -OH2) achieved through node dehydration at elevated temperatures. C1 [Kim, In Soo; Hupp, Joseph T.; Martinson, Alex B. F.] Argonne Natl Lab, Adv Photon Source, Div Mat Sci, Argonne, IL 60439 USA. [Platero-Prats, Ana E.; Chapman, Karena W.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Borycz, Joshua; Tussupbayev, Samat; Gagliardi, Laura; Cramer, Christopher J.] Univ Minnesota, Dept Chem, Supercomp Inst, Minneapolis, MN 55455 USA. [Borycz, Joshua; Tussupbayev, Samat; Gagliardi, Laura; Cramer, Christopher J.] Univ Minnesota, Chem Theory Ctr, Minneapolis, MN 55455 USA. [Wang, Timothy C.; Farha, Omar K.; Hupp, Joseph T.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Farha, Omar K.] King Abdulaziz Univ, Fac Sci, Dept Chem, Jeddah, Saudi Arabia. RP Cramer, CJ (reprint author), Univ Minnesota, Dept Chem, Supercomp Inst, 207 Pleasant St SE, Minneapolis, MN 55455 USA. EM cramer@umn.edu; martinson@anl.gov RI Cramer, Christopher/B-6179-2011; Platero-Prats, Ana Eva/B-2870-2017; Faculty of, Sciences, KAU/E-7305-2017; OI Cramer, Christopher/0000-0001-5048-1859; Platero-Prats, Ana Eva/0000-0002-2248-2739; Tussupbayev, Samat/0000-0003-3470-1510; Martinson, Alex/0000-0003-3916-1672 FU Inorganometallic Catalysis Design Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0012702]; US DOE [DE-AC02-06CH11357] FX This work was supported as part of the Inorganometallic Catalysis Design Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award DE-SC0012702. Work done at Argonne made use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. DOE/Office of Science by Argonne National Laboratory, and was supported by the US DOE, Contract DE-AC02-06CH11357. We thank Dr. J. W. Elam and Dr. J. A. Libera for technical assistance and the use of their in situ FTIR system. We also thank Dr. L. M. Utschig-Johnson and Dr. S. R Soltau for the use of their ICP-OES system. Finally, we thank Prof. D. G. Truhlar and Dr. L. Fernandez for helpful discussions. NR 55 TC 22 Z9 22 U1 23 U2 95 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUL 14 PY 2015 VL 27 IS 13 BP 4772 EP 4778 DI 10.1021/acs.chemmater.5b01560 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CN0LI UT WOS:000358104700032 ER PT J AU Bielinski, AR Kazyak, E Schleputz, CM Jung, HJ Wood, KN Dasgupta, NP AF Bielinski, Ashley R. Kazyak, Eric Schlepuetz, Christian M. Jung, Hee Joon Wood, Kevin N. Dasgupta, Neil P. TI Hierarchical ZnO Nanowire Growth with Tunable Orientations on Versatile Substrates Using Atomic Layer Deposition Seeding SO CHEMISTRY OF MATERIALS LA English DT Article ID SENSITIZED SOLAR-CELLS; ZINC-OXIDE NANOWIRES; SEMICONDUCTOR NANOWIRES; LATTICE CONTRACTION; PATTERNED GROWTH; LOW-TEMPERATURE; ESHELBY TWIST; ARRAYS; NANOSTRUCTURES; NANORODS AB The ability to synthesize semiconductor nanowires with deterministic and tunable control of orientation and morphology on a wide range of substrates, while high precision and repeatability are maintained, is a challenge currently faced for the development of many nanoscale material systems. Here we show that atomic layer deposition (ALD) presents a reliable method of surface and interfacial modification to guide nanowire orientation on a variety of substrate materials and geometries, including high-aspect-ratio, three-dimensional templates. We demonstrate control of the orientation and geometric properties of hydrothermally grown single crystalline ZnO nanowires via the deposition of a ZnO seed layer by ALD. The crystallographic texture and roughness of the seed layer result in tunable preferred nanowire orientations and densities for identical hydrothermal growth conditions. The structural and chemical relationship between the ALD layers and nanowires was investigated with synchrotron X-ray diffraction, high-resolution transmission electron microscopy, and X-ray photoelectron spectroscopy to elucidate the underlying mechanisms of orientation and morphology control. The resulting control parameters were utilized to produce hierarchical nanostructures with tunable properties on a wide range of substrates, including vertical micropillars, paper fibers, porous polymer membranes, and biological substrates. This illustrates the power of AID for interfacial engineering of heterogeneous material systems at the nanoscale, to provide a highly controlled and scalable seeding method for bottom-up synthesis of integrated nanosystems. C1 [Bielinski, Ashley R.; Kazyak, Eric; Wood, Kevin N.; Dasgupta, Neil P.] Univ Michigan, Dept Mech Engn, Ann Arbor, MI 48109 USA. [Schlepuetz, Christian M.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Jung, Hee Joon] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. RP Dasgupta, NP (reprint author), Univ Michigan, Dept Mech Engn, Ann Arbor, MI 48109 USA. EM ndasgupt@umich.edu RI Schleputz, Christian/C-4696-2008 OI Schleputz, Christian/0000-0002-0485-2708 FU DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357]; National Science Foundation [DGE 1256260, DMR-0320740, DMR-0420785] FX This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. This material is based upon work supported by the National Science Foundation Graduate Research Fellow-ship under Grant No. (DGE 1256260). Any opinion, findings, and conclusions or recommendations expressed in this material are those of the authors(s) and do not necessarily reflect the views of the National Science Foundation. This research used resources of the University of Michigan Electron Microbeam Analysis Laboratory including instruments supported by National Science Foundation grants No. DMR-0320740 and No. DMR-0420785. The authors thank Prof. Jianping Fu for providing the Si micropost substrates. NR 61 TC 5 Z9 5 U1 7 U2 71 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUL 14 PY 2015 VL 27 IS 13 BP 4799 EP 4807 DI 10.1021/acs.chemmater.5b01624 PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CN0LI UT WOS:000358104700035 ER PT J AU Henderson, IM Quintana, HA Martinez, JA Paxton, WF AF Henderson, Ian M. Quintana, Hope A. Martinez, Julio A. Paxton, Walter F. TI Capable Cross-links: Polymersomes Reinforced with Catalytically Active Metal-Ligand Bonds SO CHEMISTRY OF MATERIALS LA English DT Article ID BIS-TERPYRIDINE COMPLEXES; TRANSITION-METALS; FUNCTIONALIZED POLYMERSOMES; REPLACEMENT REACTIONS; VESICLES; DELIVERY; 2,2',2''-TERPYRIDINE; ARCHITECTURES; COORDINATION; STABILITIES AB Polymersomes, hollow spherical nano-to-microscale polymer assemblies, have increasingly become important constructs in the development of biomimetic materials that expand the library of functional and robust analogs to lipid-based vesicles. As compared to liposomes, polymersomes possess superior physical properties and the nearly unlimited potential for synthetic fine-tuning. Herein we improve on the physical properties of these polymer vesicles by introducing platinum-based metal-ligand cross-links into the hydrophobic core, which gave the vesicles demonstrated resistance to destabilization by surfactants over un-cross-linked polymersomes. The formation of cross-links was capable of being selectively reversed by the addition of phosphines. In addition, the Pt(0) cross-links retained their catalytic activity for the hydrosilylation of alkenes. C1 [Henderson, Ian M.; Paxton, Walter F.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. [Quintana, Hope A.; Martinez, Julio A.] New Mexico State Univ, Dept Chem & Mat Engn, Las Cruces, NM 88003 USA. RP Paxton, WF (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol, POB 5800, Albuquerque, NM 87185 USA. EM wfpaxto@sandia.gov FU Laboratory Directed Research and Development program; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors thank Katie L. Jungjohann for her assistance with electron microscopy. This work was performed at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. Supported by the Laboratory Directed Research and Development program at Sandia National Laboratories, a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 47 TC 2 Z9 2 U1 3 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUL 14 PY 2015 VL 27 IS 13 BP 4808 EP 4813 DI 10.1021/acs.chemmater.5b01677 PG 6 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CN0LI UT WOS:000358104700036 ER PT J AU Wozny, S Yang, MJ Nardes, AM Mercado, CC Ferrere, S Reese, MO Zhou, WL Zhu, K AF Wozny, Sarah Yang, Mengjin Nardes, Alexandre M. Mercado, Candy C. Ferrere, Suzanne Reese, Matthew O. Zhou, Weilie Zhu, Kai TI Controlled Humidity Study on the Formation of Higher Efficiency Formamidinium Lead Triiodide-Based Solar Cells SO CHEMISTRY OF MATERIALS LA English DT Article ID PEROVSKITE; LIGHT; PERFORMANCE; TRIHALIDE; IODIDE; STATE AB We report on the effect of humidity on the structural, optical, and electrical properties of formamidinium lead halide perovskite (FAPbI(3); prepared by a solvent engineering method) and the device characteristics of planar FAPbI(3) solar cells. The relative humidity strongly affects the perovskite film morphology, which changes from a uniform, fully covered FAPbI(3) film at low relative humidity (e.g., similar to 2%) to an inhomogeneous film consisting of many voids (or pinholes) at high humidity (30%-40%). This morphological deterioration with increasing humidity is also accompanied by a reduction of the film crystallinity, decay of optical property, and shorter carrier lifetime. The device based on a planar FAPbI3 film shows the best conversion efficiency of 16.6% (with the stabilized output efficiency of 16.4%) at a low humidity (similar to 2%). Higher humidity leads to lower device performance, mainly due to the loss of open-circuit voltage and fill factor, which is consistent with the decrease in recombination resistance. C1 [Wozny, Sarah; Zhou, Weilie] Univ New Orleans, Adv Mat Res Inst, New Orleans, LA 70148 USA. [Yang, Mengjin; Nardes, Alexandre M.; Ferrere, Suzanne; Reese, Matthew O.; Zhu, Kai] Natl Renewable Energy Lab, Chem & Nanosci Ctr, Golden, CO 80401 USA. [Mercado, Candy C.] Univ Colorado, Renewable & Sustainable Energy Inst, Boulder, CO 80309 USA. RP Zhou, WL (reprint author), Univ New Orleans, Adv Mat Res Inst, 2000 Lakeshore Dr, New Orleans, LA 70148 USA. EM wzhou@uno.edu; Kai.Zhu@nrel.gov OI Yang, Mengjin/0000-0003-2019-4298 FU Louisiana Board of Regent [LEQSF (2008-11)-RD-B-10, LEQSF (2011-13)-RD-B-08]; U.S. Department of Energy [DE-AC36-08-GO28308]; U.S. Department of Energy (DOE) Sun Shot Initiative under the Next Generation Photovoltaics 3 program [DE-FOA-0000990] FX This study was supported by the Louisiana Board of Regent Contracts LEQSF (2008-11)-RD-B-10 and LEQSF (2011-13)-RD-B-08, and the work at the National Renewable Energy Laboratory was supported by the U.S. Department of Energy under Contract DE-AC36-08-GO28308. M.Y. and K.Z. acknowledge the support on the device preparation and characterization by the U.S. Department of Energy (DOE) Sun Shot Initiative under the Next Generation Photovoltaics 3 program (DE-FOA-0000990). We thank Helix) Moutinho for assistance with FESEM measurements, Jeffery Aguiar, and Shiva Adireddy for helpful discussions. NR 30 TC 41 Z9 42 U1 33 U2 174 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUL 14 PY 2015 VL 27 IS 13 BP 4814 EP 4820 DI 10.1021/acs.chemmater.5b01691 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CN0LI UT WOS:000358104700037 ER PT J AU Chandra, N Tracy, CJ Cho, JH Picraux, ST Hathwar, R Goodnick, SM AF Chandra, Nishant Tracy, Clarence J. Cho, Jeong-Hyun Picraux, S. T. Hathwar, Raghuraj Goodnick, Stephen M. TI Vertically grown Ge nanowire Schottky diodes on Si and Ge substrates SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID BARRIER DIODES; DEVICES AB The processing and performance of Schottky diodes formed from arrays of vertical Ge nanowires (NWs) grown on Ge and Si substrates are reported. The goal of this work is to investigate CMOS compatible processes for integrating NWs as components of vertically scaled integrated circuits, and elucidate transport in vertical Schottky NWs. Vertical phosphorus (P) doped Ge NWs were grown using vapor-liquid-solid epitaxy, and nickel (Ni)-Ge Schottky contacts were made to the tops of the NWs. Current-voltage (I-V) characteristics were measured for variable ranges of NW diameters and numbers of nanowires in the arrays, and the I-V characteristics were fit using modified thermionic emission theory to extract the barrier height and ideality factor. As grown NWs did not show rectifying behavior due to the presence of heavy P side-wall doping during growth, resulting in a tunnel contact. After sidewall etching using a dilute peroxide solution, rectifying behavior was obtained. Schottky barrier heights of 0.3-0.4V and ideality factors close to 2 were extracted using thermionic emission theory, although the model does not give an accurate fit across the whole bias range. Attempts to account for enhanced side-wall conduction due to non-uniform P doping profile during growth through a simple shunt resistance improve the fit, but are still insufficient to provide a good fit. Full three-dimensional numerical modeling using Silvaco Atlas indicates that at least part of this effect is due to the presence of fixed charge and acceptor like traps on the NW surface, which leads to effectively high ideality factors. (c) 2015 AIP Publishing LLC. C1 [Chandra, Nishant; Tracy, Clarence J.; Hathwar, Raghuraj; Goodnick, Stephen M.] Arizona State Univ, Sch Elect Comp & Energy Engn, Tempe, AZ 85287 USA. [Cho, Jeong-Hyun; Picraux, S. T.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. RP Cho, JH (reprint author), Univ Minnesota, Dept Elect & Comp Engn, St Paul, MN 55455 USA. EM jcho@umn.edu FU National Science Foundation through NSF [100133]; Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Science User Facility at Los Alamos National Laboratory [DE-AC52-06NA25396] FX The authors would like to acknowledge support for this work through the National Science Foundation through NSF Award No. 100133. This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Science User Facility at Los Alamos National Laboratory (Contract No. DE-AC52-06NA25396). NR 28 TC 1 Z9 1 U1 3 U2 18 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 14 PY 2015 VL 118 IS 2 AR 024301 DI 10.1063/1.4923407 PG 7 WC Physics, Applied SC Physics GA CM8OH UT WOS:000357961000023 ER PT J AU Jacobsen, MK Velisavljevic, N Sinogeikin, SV AF Jacobsen, M. K. Velisavljevic, N. Sinogeikin, S. V. TI Pressure-induced kinetics of the alpha to omega transition in zirconium SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID MEASURING GRUNEISEN-PARAMETER; ARAGONITE TRANSFORMATION; PHASE-TRANSFORMATIONS; BCC TRANSFORMATION; JUMP METHOD; TITANIUM; SIMULATIONS; TEMPERATURE; EQUATIONS; YTTERBIUM AB Diamond anvil cells (DAC) coupled with x-ray diffraction (XRD) measurements are one of the primary techniques for investigating structural stability of materials at high pressure-temperature (P-T) conditions. DAC-XRD has been predominantly used to resolve structural information at set P-T conditions and, consequently, provides P-T phase diagram information on a broad range of materials. With advances in large scale synchrotron x-ray facilities and corresponding x-ray diagnostic capabilities, it is now becoming possible to perform sub-second time resolved measurements on micron sized DAC samples. As a result, there is an opportunity to gain valuable information about the kinetics of structural phase transformations and extend our understanding of material behavior at high P-T conditions. Using DAC-XRD time resolved measurements, we have investigated the kinetics of the alpha to omega transformation in zirconium. We observe a clear time and pressure dependence in the martensitic alpha-omega transition as a function of pressure-jump, i. e., drive pressure. The resulting data are fit using available kinetics models, which can provide further insight into transformation mechanism that influence transformation kinetics. Our results help shed light on the discrepancies observed in previous measurements of the alpha-omega transition pressure in zirconium. (C) 2015 AIP Publishing LLC. C1 [Jacobsen, M. K.; Velisavljevic, N.] Los Alamos Natl Lab, Shock & Detonat Phys WX 9, Los Alamos, NM 87545 USA. [Sinogeikin, S. V.] Carnegie Inst Sci, Geophys Lab, HPCAT, Washington, DC 20015 USA. RP Velisavljevic, N (reprint author), Los Alamos Natl Lab, Shock & Detonat Phys WX 9, POB 1663, Los Alamos, NM 87545 USA. EM nenad@lanl.gov OI Jacobsen, Matthew/0000-0002-0326-2562 FU DOE-NNSA [DE-AC52-06NA25396, DE-NA0001974]; LANL Science Campaign 1; LANL Science Campaign 2; DOE-BES [DE-FG02-99ER45775, DE-AC02-06CH11357]; NSF; U.S. DOE [DE-AC02-06CH11357] FX Los Alamos National Laboratory (LANL) is operated by LANS, LLC, for the DOE-NNSA under Contract No. DE-AC52-06NA25396. The authors acknowledge funding support from LANL Science Campaigns 1 and 2. This work was performed at HPCAT (Sector 16), Advanced Photon Source (APS), Argonne National Laboratory. HPCAT operations are supported by DOE-NNSA under Award No. DE-NA0001974 and DOE-BES under Award No. DE-FG02-99ER45775, with partial instrumentation funding by NSF. APS is supported by DOE-BES, under Contract No. DE-AC02-06CH11357. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 48 TC 3 Z9 3 U1 6 U2 24 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 14 PY 2015 VL 118 IS 2 AR 025902 DI 10.1063/1.4926724 PG 9 WC Physics, Applied SC Physics GA CM8OH UT WOS:000357961000048 ER PT J AU Johnston, LT Biener, MM Ye, JC Baumann, TF Kucheyev, SO AF Johnston, L. T. Biener, M. M. Ye, J. C. Baumann, T. F. Kucheyev, S. O. TI Pore architecture of nanoporous gold and titania by hydrogen thermoporometry SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID POROUS VYCOR GLASS; ELECTRON-MICROSCOPY; SURFACE-AREA; ADSORPTION; SCATTERING; ISOTHERMS; EVOLUTION AB Nanoporous gold (NPG) and materials derived from it by templating have complex pore architecture that determines their technologically relevant physical properties. Here, we apply high-resolution hydrogen thermoporometry to study the pore structure of NPG and NPG-derived titania nanofoam (TNF). Results reveal complex multimodal pore size distributions for NPG and TNF. The freezing-melting hysteresis is pronounced, with freezing and melting scans having entirely different shapes. Experiments involving partial freeze-melt cycles reveal the lack of direct correlation between individual freezing and melting peaks, pointing to phenomena that are beyond the Gibbs-Thomson formalism. The depression of the average freezing temperature scales linearly with the ratio of the internal surface area (measured by gas sorption) and the total pore volume derived from the density of monoliths. Thermoporometry yields total pore volumes in good agreement with those derived from monolith densities for both NPG and TNF. (c) 2015 AIP Publishing LLC. C1 [Johnston, L. T.; Biener, M. M.; Ye, J. C.; Baumann, T. F.; Kucheyev, S. O.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Johnston, LT (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM kucheyev@llnl.gov FU U.S. DOE by LLNL [DE-AC52-07NA27344] FX We are grateful to A. V. Hamza, R. R. Miles, and B. J. Kozioziemski for valuable discussions and programmatic support of this work. This work was performed under the auspices of the U.S. DOE by LLNL under Contract No. DE-AC52-07NA27344. NR 30 TC 1 Z9 1 U1 3 U2 20 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 14 PY 2015 VL 118 IS 2 AR 025303 DI 10.1063/1.4926738 PG 7 WC Physics, Applied SC Physics GA CM8OH UT WOS:000357961000040 ER PT J AU Martin, JE van Swol, F AF Martin, James E. van Swol, Frank TI Driven assembly with multiaxial fields: Creating a soft mode in assemblies of anisometric induced dipoles SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID TRIAXIAL MAGNETIC-FIELDS; STRUCTURED COMPOSITES; BIAXIAL FIELD; SIMULATION; PARTICLES AB In this paper, we show that multiaxial fields can induce time-averaged, noncentrosymmetric interactions between particles having polarization anisotropy, yet the multiaxial field itself does not exert either a force or a torque on an isolated particle. These induced interactions lead to particle assemblies whose energy is strongly dependent on both the translational and orientational degrees of freedom of the system. The situation is similar to a collection of permanent dipoles, but the symmetry of the time-averaged interaction is quite distinct, and the scale of the system energy can be dynamically controlled by the magnitude of the applied multiaxial field. In this paper, the case of polarizable rods is considered in detail, and it is suggested that collections of rods embedded in spheres can be used to create a material with a dynamically tunable magnetic permeability or dielectric permittivity. We report on Monte Carlo simulations performed to investigate the behavior of assemblies of both multiaxial-field induced dipoles and permanent dipoles arranged onto two-dimensional lattices. The ground state of the induced dipoles is an orientational soft mode of aligned dipoles, whereas that of the permanent dipoles is a vortex state. (c) 2015 AIP Publishing LLC. C1 [Martin, James E.; van Swol, Frank] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Martin, JE (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Division of Materials Science, Office of Basic Energy Sciences, U.S. Department of Energy (DOE) FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. This work was supported by the Division of Materials Science, Office of Basic Energy Sciences, U.S. Department of Energy (DOE). NR 26 TC 0 Z9 0 U1 1 U2 11 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 14 PY 2015 VL 118 IS 2 AR 024904 DI 10.1063/1.4923301 PG 9 WC Physics, Applied SC Physics GA CM8OH UT WOS:000357961000035 ER PT J AU Moseley, J Metzger, WK Moutinho, HR Paudel, N Guthrey, HL Yan, YF Ahrenkiel, RK Al-Jassim, MM AF Moseley, John Metzger, Wyatt K. Moutinho, Helio R. Paudel, Naba Guthrey, Harvey L. Yan, Yanfa Ahrenkiel, Richard K. Al-Jassim, Mowafak M. TI Recombination by grain-boundary type in CdTe SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID ELECTRON BACKSCATTER DIFFRACTION; ORIENTATION IMAGING MICROSCOPY; POSITIONING TWIN BOUNDARIES; FILM SOLAR-CELLS; POLYCRYSTALLINE CDTE; THIN-FILMS; ENERGY; DEFECTS; METALS AB We conducted cathodoluminescence (CL) spectrum imaging and electron backscatter diffraction on the same microscopic areas of CdTe thin films to correlate grain-boundary (GB) recombination by GB "type." We examined misorientation-based GB types, including coincident site lattice (CSL) Sigma = 3, other-CSL (Sigma = 5-49), and general GBs (Sigma > 49), which make up similar to 47%-48%, similar to 6%-8%, and similar to 44%-47%, respectively, of the GB length at the film back surfaces. Statistically averaged CL total intensities were calculated for each GB type from sample sizes of >= 97 GBs per type and were compared to the average grain-interior CL intensity. We find that only similar to 16%-18% of Sigma = 3 GBs are active non-radiative recombination centers. In contrast, all other-CSL and general GBs are observed to be strong non-radiative centers and, interestingly, these GB types have about the same CL intensity. Both as-deposited and CdCl2-treated films were studied. The CdCl2 treatment reduces non-radiative recombination at both other-CSL and general GBs, but GBs are still recombination centers after the CdCl2 treatment. (C) 2015 AIP Publishing LLC. C1 [Moseley, John; Metzger, Wyatt K.; Moutinho, Helio R.; Guthrey, Harvey L.; Ahrenkiel, Richard K.; Al-Jassim, Mowafak M.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Moseley, John; Ahrenkiel, Richard K.] Colorado Sch Mines, Golden, CO 80401 USA. [Paudel, Naba; Yan, Yanfa] Univ Toledo, Dept Phys & Astron, Toledo, OH 43606 USA. RP Moseley, J (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM john.moseley@nrel.gov FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory FX This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. J. Moseley would like to thank Dr. N. Haegel for critical reviews of this manuscript. NR 48 TC 14 Z9 14 U1 3 U2 46 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 14 PY 2015 VL 118 IS 2 AR 025702 DI 10.1063/1.4926726 PG 9 WC Physics, Applied SC Physics GA CM8OH UT WOS:000357961000046 ER PT J AU Yang, JH Yin, WJ Park, JS Burst, J Metzger, WK Gessert, T Barnes, T Wei, SH AF Yang, Ji-Hui Yin, Wan-Jian Park, Ji-Sang Burst, James Metzger, Wyatt K. Gessert, Tim Barnes, Teresa Wei, Su-Huai TI Enhanced p-type dopability of P and As in CdTe using non-equilibrium thermal processing SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID MOLECULAR-BEAM EPITAXY; TOTAL-ENERGY CALCULATIONS; II-VI SEMICONDUCTORS; WAVE BASIS-SET; SOLAR-CELLS; SINGLE-CRYSTAL; EFFICIENCY; DIFFUSION; CDCL2; FILMS AB One of the main limiting factors in CdTe solar cells is its low p-type dopability and, consequently, low open-circuit voltage (V-OC). We have systematically studied P and As doping in CdTe with first-principles calculations in order to understand how to increase the hole density. We find that both P and As p-type doping are self-compensated by the formation of AX centers. More importantly, we find that although high-temperature growth is beneficial to obtain high hole density, rapid cooling is necessary to sustain the hole density and to lower the Fermi level close to the valence band maximum (VBM) at room temperature. Thermodynamic simulations suggest that by cooling CdTe from a high growth temperature to room temperature under Te-poor conditions and choosing an optimal dopant concentration of about 10(18) /cm(3), P and As doping can reach a hole density above 10(17) /cm(3) at room temperature and lower the Fermi level to within similar to 0.1 eV above the VBM. These results suggest a promising pathway to improve the V-OC and efficiency of CdTe solar cells. (c) 2015 AIP Publishing LLC. C1 [Yang, Ji-Hui; Yin, Wan-Jian; Park, Ji-Sang; Burst, James; Metzger, Wyatt K.; Gessert, Tim; Barnes, Teresa; Wei, Su-Huai] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Yang, JH (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM suhuai.wei@nrel.gov RI Yin, Wanjian/F-6738-2013; Park, Ji-Sang/F-9944-2010 OI Park, Ji-Sang/0000-0002-1374-8793 FU U.S. Department of Energy, EERE/SunShot program [DE-AC36-08GO28308] FX This work was funded by the U.S. Department of Energy, EERE/SunShot program, under Contract No. DE-AC36-08GO28308. The calculations are done on peregrine supercomputer and NERSC supercomputer. NR 48 TC 6 Z9 6 U1 4 U2 23 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 14 PY 2015 VL 118 IS 2 AR 025102 DI 10.1063/1.4926748 PG 6 WC Physics, Applied SC Physics GA CM8OH UT WOS:000357961000037 ER PT J AU King, SB Stephansen, AB Yokoi, Y Yandell, MA Kunin, A Takayanagi, T Neumark, DM AF King, Sarah B. Stephansen, Anne B. Yokoi, Yuki Yandell, Margaret A. Kunin, Alice Takayanagi, Toshiyuki Neumark, Daniel M. TI Electron accommodation dynamics in the DNA base thymine SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID NUCLEIC-ACID BASES; STRAND BREAKS; AB-INITIO; IONIZATION-POTENTIALS; EXCITED-STATES; NEGATIVE-IONS; ATTACHMENT; ENERGY; ANIONS; PHOTOELECTRON AB The dynamics of electron attachment to the DNA base thymine are investigated using femtosecond time-resolved photoelectron imaging of the gas phase iodide-thymine (I-T) complex. An ultraviolet pump pulse ejects an electron from the iodide and prepares an iodine-thymine temporary negative ion that is photodetached with a near-IR probe pulse. The resulting photoelectrons are analyzed with velocity-map imaging. At excitation energies ranging from -120 meV to + 90 meV with respect to the vertical detachment energy (VDE) of 4.05 eV for I-T, both the dipole-bound and valence-bound negative ions of thymine are observed. A slightly longer rise time for the valence-bound state than the dipole-bound state suggests that some of the dipole-bound anions convert to valence-bound species. No evidence is seen for a dipole-bound anion of thymine at higher excitation energies, in the range of 0.6 eV above the I-T VDE, which suggests that if the dipole-bound anion acts as a "doorway" to the valence-bound anion, it only does so at excitation energies near the VDE of the complex. (C) 2015 AIP Publishing LLC. C1 [King, Sarah B.; Yandell, Margaret A.; Kunin, Alice; Neumark, Daniel M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Stephansen, Anne B.] Univ Copenhagen, Dept Chem, DK-2100 Copenhagen O, Denmark. [Yokoi, Yuki; Takayanagi, Toshiyuki] Saitama Univ, Dept Chem, Sakura Ku, Saitama, Saitama 3388570, Japan. [Neumark, Daniel M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Neumark, DM (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM dneumark@berkeley.edu RI Takayanagi, Toshiyuki/F-1020-2012; Neumark, Daniel/B-9551-2009; OI Neumark, Daniel/0000-0002-3762-9473; Stephansen, Anne B./0000-0001-8730-002X; Kunin, Alice/0000-0002-3002-8317 FU National Science Foundation (NSF) [CHE-1011819]; Villum Foundation; NSF Graduate Research Fellowship; Ministry of Education, Culture, Sports, Science, and Technology of Japan [21550005] FX The work described in this paper was funded by the National Science Foundation (NSF) under Grant No. CHE-1011819. A.B.S. gratefully acknowledges support from The Villum Foundation. M.A.Y. gratefully acknowledges support from a NSF Graduate Research Fellowship. T.T. acknowledges support from the Ministry of Education, Culture, Sports, Science, and Technology of Japan (Grant No. 21550005). NR 56 TC 7 Z9 7 U1 5 U2 26 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUL 14 PY 2015 VL 143 IS 2 AR 024312 DI 10.1063/1.4923343 PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CM8OL UT WOS:000357961400029 PM 26178110 ER PT J AU Manzer, S Horn, PR Mardirossian, N Head-Gordon, M AF Manzer, Samuel Horn, Paul R. Mardirossian, Narbe Head-Gordon, Martin TI Fast, accurate evaluation of exact exchange: The occ-RI-K algorithm SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID DENSITY-FUNCTIONAL THEORY; HARTREE-FOCK EXCHANGE; AUXILIARY BASIS-SETS; LINEAR SCALING COMPUTATION; APPROXIMATE COULOMB POTENTIALS; BENCHMARK INTERACTION ENERGIES; CONSISTENT BASIS-SETS; ZETA-VALENCE QUALITY; GAUSSIAN-BASIS SETS; FITTING BASIS-SETS AB Construction of the exact exchange matrix, K, is typically the rate-determining step in hybrid density functional theory, and therefore, new approaches with increased efficiency are highly desirable. We present a framework with potential for greatly improved efficiency by computing a compressed exchange matrix that yields the exact exchange energy, gradient, and direct inversion of the iterative subspace (DIIS) error vector. The compressed exchange matrix is constructed with one index in the compact molecular orbital basis and the other index in the full atomic orbital basis. To illustrate the advantages, we present a practical algorithm that uses this framework in conjunction with the resolution of the identity (RI) approximation. We demonstrate that convergence using this method, referred to hereafter as occupied orbital RI-K (occ-RI-K), in combination with the DIIS algorithm is well-behaved, that the accuracy of computed energetics is excellent (identical to conventional RI-K), and that significant speedups can be obtained over existing integral-direct and RI-K methods. For a 4400 basis function C68H22 hydrogen-terminated graphene fragment, our algorithm yields a 14x speedup over the conventional algorithm and a speedup of 3.3x over RI-K. (C) 2015 AIP Publishing LLC. C1 [Manzer, Samuel] Univ Calif Berkeley, Dept Chem, Kenneth S Pitzer Ctr Theoret Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Manzer, S (reprint author), Univ Calif Berkeley, Dept Chem, Kenneth S Pitzer Ctr Theoret Chem, Berkeley, CA 94720 USA. EM mhg@cchem.berkeley.edu FU Scientific Discovery through Advanced Computing (SciDAC) program - U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research, and Basic Energy Sciences; NIH SBIR Grant [GM096678] FX Support for this work was provided through the Scientific Discovery through Advanced Computing (SciDAC) program funded by the U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research, and Basic Energy Sciences. We also acknowledge partial support of this work from Q-Chem, Inc. through NIH SBIR Grant No. GM096678. M.H.-G. is a part-owner of Q-Chem, Inc. NR 113 TC 8 Z9 8 U1 1 U2 18 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUL 14 PY 2015 VL 143 IS 2 AR 024113 DI 10.1063/1.4923369 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CM8OL UT WOS:000357961400015 PM 26178096 ER PT J AU Zaporozhets, IA Ivanov, VV Lyakh, DI Adamowicz, L AF Zaporozhets, Irina A. Ivanov, Vladimir V. Lyakh, Dmitry I. Adamowicz, Ludwik TI Discontinuities-free complete-active-space state-specific multi-reference coupled cluster theory for describing bond stretching and dissociation SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID SINGLE-REFERENCE FORMALISM; MANY-ELECTRON THEORY; EXCITED-STATES; PERTURBATION-THEORY; MOLECULAR SYSTEMS; WAVE-FUNCTIONS; CAS REFERENCE; N-2 MOLECULE; IMPLEMENTATION; MODEL AB The earlier proposed multi-reference state-specific coupled-cluster theory with the complete active space reference [CASCC; Lyakh et al., J. Chem. Phys. 122, 024108 (2005)] suffered from a problem of energy discontinuities when the formal reference state was changing in the calculation of the potential energy curve (PEC). A simple remedy to the discontinuity problem is found and is presented in this work. It involves using natural complete active space self-consistent field active orbitals in the complete active space coupled-cluster calculations. The approach gives smooth PECs for different types of dissociation problems, as illustrated in the calculations of the dissociation of the single bond in the hydrogen fluorine molecule and of the symmetric double-bond dissociation in the water molecule. (C) 2015 AIP Publishing LLC. C1 [Zaporozhets, Irina A.; Ivanov, Vladimir V.] Kharkov Natl Univ, Dept Chem, Kharkov, Ukraine. [Lyakh, Dmitry I.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Adamowicz, Ludwik] Univ Arizona, Dept Chem & Biochem, Tucson, AZ 85721 USA. RP Zaporozhets, IA (reprint author), Kharkov Natl Univ, Dept Chem, Kharkov, Ukraine. EM 1z-irina@rambler.ru; vivanov@karazin.ua; quant4me@gmail.com; ludwik@u.arizona.edu NR 53 TC 0 Z9 0 U1 2 U2 10 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUL 14 PY 2015 VL 143 IS 2 AR 024109 DI 10.1063/1.4926392 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CM8OL UT WOS:000357961400011 PM 26178092 ER PT J AU Buceta, D Tojo, C Vukmirovic, MB Deepak, FL Lopez-Quintela, MA AF Buceta, David Tojo, Concha Vukmirovic, Miomir B. Deepak, Francis Leonard Arturo Lopez-Quintela, M. TI Controlling Bimetallic Nanostructures by the Microemulsion Method with Subnanometer Resolution Using a Prediction Model SO LANGMUIR LA English DT Article ID NANOPARTICLES; METHANOL; ELECTROOXIDATION; SIZE AB We present a theoretical model to predict the atomic structure of Au/Pt nanoparticles synthesized in microemulsions. Excellent concordance with the experimental results shows that the structure of the nanoparticles can be controlled at subnanometer resolution simply by changing the reactant concentration. The results of this study not only offer a better understanding of the complex mechanisms governing reactions in microemulsions, but open up a simple new way to synthesize bimetallic nanoparticles with ad hoc controlled nanostructures. C1 [Buceta, David; Arturo Lopez-Quintela, M.] Univ Santiago de Compostela, Lab Magnetismo & Nanotecnol, E-15782 Santiago De Compostela, Spain. [Buceta, David; Vukmirovic, Miomir B.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Tojo, Concha] Univ Vigo, Dept Phys Chem, E-36310 Vigo, Spain. [Deepak, Francis Leonard] INL Int Iberian Nanotechnol Lab, P-4715330 Braga, Portugal. RP Lopez-Quintela, MA (reprint author), Univ Santiago de Compostela, Lab Magnetismo & Nanotecnol, E-15782 Santiago De Compostela, Spain. EM malopez.quintela@usc.es RI INL, Citations/K-3436-2015; Buceta, David/I-1337-2015 OI INL, Citations/0000-0002-3745-5100; Buceta, David/0000-0002-3297-6695 FU Ministerio de Ciencia e Innovacion, Spain [MAT2012-36754-C02-01]; Xunta de Galicia [GRC2013-044, REDES 2014/019]; Xunta de Galicia (FEDER Funds); Xunta de Galicia, Spain [POS-A/2013/018]; U.S. Department of Energy, Division of Chemical Science [DE-AC02-98CH10886] FX Works at University of Santiago de Compostela and University of Vigo were supported by Ministerio de Ciencia e Innovacion, Spain (MAT2012-36754-C02-01) and Xunta de Galicia (GRC2013-044, FEDER Funds, REDES 2014/019). D.B. thanks for the postdoc grant from Xunta de Galicia, Spain (POS-A/2013/018). Work at BNL was supported by the U.S. Department of Energy, Division of Chemical Science (Contract No. DE-AC02-98CH10886). We thank Dr. R. R. Adzic (BNL) for useful discussions. NR 22 TC 2 Z9 2 U1 1 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD JUL 14 PY 2015 VL 31 IS 27 BP 7435 EP 7439 DI 10.1021/acs.langmuir.5b01455 PG 5 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CN0LL UT WOS:000358105000001 PM 26035721 ER PT J AU Lee, JW Mani, A Templeton, JA AF Lee, Jonathan W. Mani, Ali Templeton, Jeremy A. TI Atomistic and Molecular Effects in Electric Double Layers at High Surface Charges SO LANGMUIR LA English DT Article ID DENSITY-FUNCTIONAL THEORY; FREE-ENERGY; MODEL; CAPACITANCE; SIMULATION; WATER AB The Poisson-Boltzmann theory for electrolytes near a charged surface is known to be invalid due to unaccounted physics associated with high ioh concentration regimes. To investigate this regime, fluids density functional theory (f-DFT) and molecular dynamics (MD) simulations were used to determine electric surface potential as a function of surface charge. Based on these detailed computations, for electrolytes with nonpolar solvent, the surface potential is shown to depend quadratically on the surface charge in the high charge limit. We demonstrate that modified Poisson-Boltzmann theories can model this limit if they are augmented with atomic packing densities provided by MD. However, when the solvent is a highly polar molecule, water in this case, an intermediate regime is identified in which a constant capacitance is realized. Simulation results demonstrate the mechanism underlying this regime, and for the salt water system studied here, it persists throughout the range of physically realistic surface charge densities so the potential's quadratic surface charge dependence is not obtained. C1 [Lee, Jonathan W.; Templeton, Jeremy A.] Sandia Natl Labs, Thermal Fluid Sci & Engn Dept, Livermore, CA 94550 USA. [Mani, Ali] Stanford Univ, Dept Mech Engn, Stanford, CA 94305 USA. RP Templeton, JA (reprint author), Sandia Natl Labs, Thermal Fluid Sci & Engn Dept, Livermore, CA 94550 USA. EM jatempl@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Laboratory Directed Research and Development (LDRD) program at Sandia National Laboratories; Advanced Scientific Computing (ASC) program at Sandia National Laboratories FX The authors would like to thank Amalie Frischknecht and Kranthi Mandadapu for helpful comments on a draft of this manuscript. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. Funding for this work was provided by the Laboratory Directed Research and Development (LDRD) and Advanced Scientific Computing (ASC) programs at Sandia National Laboratories, and its support is gratefully acknowledged. NR 25 TC 3 Z9 3 U1 2 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD JUL 14 PY 2015 VL 31 IS 27 BP 7496 EP 7502 DI 10.1021/acs.langmuir.5b00215 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CN0LL UT WOS:000358105000008 PM 26079793 ER PT J AU Loring, JS Chen, J Benezeth, P Qafoku, O Ilton, ES Washton, NM Thompson, CJ Martin, PF McGrail, BP Rosso, KM Felmy, AR Schaef, HT AF Loring, John S. Chen, Jeffrey Benezeth, Pascale Qafoku, Odeta Ilton, Eugene S. Washton, Nancy M. Thompson, Christopher J. Martin, Paul F. McGrail, B. Peter Rosso, Kevin M. Felmy, Andrew R. Schaef, Herbert T. TI Evidence for Carbonate Surface Complexation during Forsterite Carbonation in Wet Supercritical Carbon Dioxide SO LANGMUIR LA English DT Article ID MAGNESIUM-OXIDE; CO2 SEQUESTRATION; WATER; ADSORPTION; MINERALS; REACTIVITY; SPECTRA; NMR; MEDIA; FTIR AB Continental flood basalts are attractive formations for geologic sequestration of carbon dioxide because of their reactive divalent-cation containing silicates, such as forsterite (Mg2SiO4), suitable for long-term trapping of CO2 mineralized as metal carbonates. The goal of this study was to investigate at a molecular level the carbonation products formed during the reaction of forsterite with supercritical CO2 (scCO(2)) as a function of the concentration of H2O adsorbed to the forsterite surface. Experiments were performed at 50 degrees C and 90 bar using an in situ IR titration capability, and postreaction samples were examined by ex situ techniques, including scanning electron microscopy (SEM), X-ray photoelectron spectroscopy (XPS), focused ion beam transmission electron microscopy (FIB-TEM), thermal gravimetric analysis mass spectrometry (TGA-MS), and magic angle spinning nuclear magnetic resonance (MAS NMR). Carbonation products and reaction extents varied greatly with adsorbed H2O. We show for the first time evidence of Mg-carbonate surface complexation under wet scCO(2) conditions. Carbonate is found to be coordinated to Mg at the forsterite surface in a predominately bidentate fashion at adsorbed H2O concentrations below 27 mu mol/m(2). Above this concentration and up to 76 mu mol/m(2), monodentate coordinated complexes become dominant. Beyond a threshold adsorbed H2O concentration of 76 mu mol/m(2), crystalline carbonates continuously precipitate as magnesite, and the particles that form are hundreds of times larger than the estimated thicknesses of the adsorbed water films of about 7 to 15 angstrom. At an applied level, these results suggest that mineral carbonation in scCO(2) dominated fluids near the wellbore and adjacent to caprocks will be insignificant and limited to surface complexation, unless adsorbed H2O concentrations are high enough to promote crystalline carbonate formation. At a fundamental level, the surface complexes and their dependence on adsorbed H2O concentration give insights regarding forsterite dissolution processes and magnesite nucleation and growth. C1 [Loring, John S.; Chen, Jeffrey; Qafoku, Odeta; Ilton, Eugene S.; Washton, Nancy M.; Thompson, Christopher J.; Martin, Paul F.; McGrail, B. Peter; Rosso, Kevin M.; Felmy, Andrew R.; Schaef, Herbert T.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Benezeth, Pascale] CNRS, GET, UMR 5563, F-31400 Toulouse, France. RP Loring, JS (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM john.loring@pnnl.gov FU Geosciences Research Program in the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences; U.S. Department of Energy, Office of Fossil Energy; Pacific Northwest National Laboratory's Carbon Sequestration Initiative, a Laboratory Directed Research and Development Program; DOE's Office of Biological and Environmental Research; DOE by Battelle Memorial Institute [DE-AC06-76RLO-1830] FX We appreciate helpful discussions with James J. DeYoreo about our results, as well as the comments of three anonymous reviewers. We thank Libor Kovarik for performing the FIB-TEM analysis. This work was supported by (1) the Geosciences Research Program in the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences, and (2) the U.S. Department of Energy, Office of Fossil Energy. Development of the IR titration instrumentation for this research was funded through Pacific Northwest National Laboratory's Carbon Sequestration Initiative, a Laboratory Directed Research and Development Program. Several of the analyses were performed at EMSL, the Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research, and located at PNNL. PNNL is operated for DOE by Battelle Memorial Institute under Contract# DE-AC06-76RLO-1830. NR 50 TC 4 Z9 4 U1 11 U2 48 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD JUL 14 PY 2015 VL 31 IS 27 BP 7533 EP 7543 DI 10.1021/acs.langmuir.5b01052 PG 11 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CN0LL UT WOS:000358105000012 PM 26079871 ER PT J AU Tian, Z Hess, A Fellin, CR Nulwala, H Allcock, HR AF Tian, Zhicheng Hess, Andrew Fellin, Christopher R. Nulwala, Hunaid Allcock, Harry R. TI Phosphazene High Polymers and Models with Cyclic Aliphatic Side Groups: New Structure-Property Relationships SO MACROMOLECULES LA English DT Article ID POLYPHOSPHAZENE; METHACRYLATE); MEMBRANES; CHLORIDE AB Poly(dichlorophosphazene) is a versatile precursor material for accessing new polymeric materials via the introduction of various side groups by chlorine replacement reactions. Herein, methods are described for the synthesis of a new series of phosphazene single- and mixed-substituent high polymers containing cyclic aliphatic rings, -CnH2n-1, (where n = 4-8). These reactions were preceded by model reactions using small molecule cyclic trimeric phosphazenes. The new high polymers are amorphous, transparent, and film- and membrane-forming materials with a wide range of glass transition temperatures (-60 to +40 degrees C) depending on the side groups and cosubstituents. All are hydrophobic and resistant to hydrolytic breakdown. C1 [Tian, Zhicheng; Hess, Andrew; Fellin, Christopher R.; Allcock, Harry R.] Penn State Univ, Dept Chem, University Pk, PA 16802 USA. [Nulwala, Hunaid] Carnegie Mellon Univ, Dept Chem, Pittsburgh, PA 15213 USA. [Nulwala, Hunaid] Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. RP Allcock, HR (reprint author), Penn State Univ, Dept Chem, University Pk, PA 16802 USA. EM hral@psu.edu OI Nulwala, Hunaid/0000-0001-7481-3723 FU National Energy Technology Laboratory (NETL)/Department of Energy (DOE) [RES1000026] FX The authors thank for Dr. Hemant P. Yennawar for assistance with the wide-angle X-ray diffraction experiments. This work was made with support under Contract RES1000026 awarded by National Energy Technology Laboratory (NETL)/Department of Energy (DOE). NR 34 TC 6 Z9 7 U1 6 U2 31 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD JUL 14 PY 2015 VL 48 IS 13 BP 4301 EP 4311 DI 10.1021/acs.macromol.5b00946 PG 11 WC Polymer Science SC Polymer Science GA CN0LK UT WOS:000358104900007 ER PT J AU Fan, F Wang, YY Hong, T Heres, MF Saito, T Sokolov, AP AF Fan, Fei Wang, Yangyang Hong, Tao Heres, Maximilian F. Saito, Tomonori Sokolov, Alexei P. TI Ion Conduction in Polymerized Ionic Liquids with Different Pendant Groups SO MACROMOLECULES LA English DT Article ID DIELECTRIC-RELAXATION; PERCHLORATE COMPLEXES; VISCOELASTIC BEHAVIOR; MICROPHASE SEPARATION; POLY(IONIC LIQUID)S; AMORPHOUS MATERIALS; THERMAL-PROPERTIES; GLASS-TRANSITION; ELECTROLYTES; TRANSPORT AB Polymerized ionic liquids (PolyILs) are promising candidates for energy storage and electrochemical devices applications. Understanding their ionic transport mechanism is the key for designing highly conductive PolyILs. By using broadband dielectric spectroscopy (BDS), rheology, and differential scanning calorimetry (DSC), a systematic study has been carried out to provide a better understanding of the ionic transport mechanism in PolyILs with different pendant groups. The variation of pendant groups results in different dielectric, mechanical, and thermal properties of these PolyILs. The Walden plot analysis shows that the data points for all these PolyILs fall above the ideal Walden line, and the deviation from the ideal line increases upon approaching the glass transition temperature (T-g). The conductivity for these PolyILs at their T(g)s are much higher than the usually reported value similar to 10(-15) S/cm for polymer electrolytes, in which the ionic transport is closely coupled to the segmental dynamics. These results indicate a decoupling of ionic conductivity from the segmental relaxation in these materials. The degree of decoupling increases with the increase of the fragility of polymer segmental relaxation. We relate this observation to a decrease in polymer packing efficiency with an increase in fragility. C1 [Fan, Fei; Hong, Tao; Sokolov, Alexei P.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Wang, Yangyang] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Heres, Maximilian F.] Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA. [Saito, Tomonori; Sokolov, Alexei P.] Oak Ridge Natl Lab, Chem Sci Div, Oak Ridge, TN 37831 USA. RP Fan, F (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. EM ffan@vols.utk.edu RI Wang, Yangyang/A-5925-2010; Saito, Tomonori/M-1735-2016 OI Wang, Yangyang/0000-0001-7042-9804; Saito, Tomonori/0000-0002-4536-7530 FU NSF Polymer Program [DMR-1408811]; Division of Materials Science and Engineering, U.S. Department of Energy, Office of Basic Energy Sciences FX F.F. thanks the NSF Polymer Program (DMR-1408811) for funding. T.S. and A.P.S. acknowledge the financial support from the Division of Materials Science and Engineering, U.S. Department of Energy, Office of Basic Energy Sciences. NR 70 TC 15 Z9 15 U1 11 U2 69 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD JUL 14 PY 2015 VL 48 IS 13 BP 4461 EP 4470 DI 10.1021/acs.macromol.5b00257 PG 10 WC Polymer Science SC Polymer Science GA CN0LK UT WOS:000358104900025 ER PT J AU Majewski, PW Yager, KG AF Majewski, Pawel W. Yager, Kevin G. TI Block Copolymer Response to Photothermal Stress Fields SO MACROMOLECULES LA English DT Article ID SHEAR-INDUCED ALIGNMENT; THIN-FILMS; DIBLOCK COPOLYMERS; IONIC-CONDUCTIVITY; ELECTRIC-FIELDS; MAGNETIC-FIELDS; ORIENTATION; TRANSITION; PATTERNS; MICROSTRUCTURE AB Block copolymer materials can be aligned using shear forces; in order to fully exploit this phenomenon for controlling nanoscale order, the coupling between applied forces and molecular properties must be elucidated. We use a photothermal method to generate extreme and controllable thermal and stress fields in thin films of cylinder-forming block copolymers. By studying morphological ordering as a function of time, shear rate, polymer material, molecular weight, and film thickness, we elucidate the critical parameters with respect to efficient ordering. We find that ordering efficiency depends weakly on the block copolymer interaction parameter and strongly on the difference in mechanical response of the two phases. Morphologies can be aligned only when the inverse shear rate is smaller than the material's relaxation time. Overall, photothermal shear alignment provides an efficient means of ordering and aligning nanoscale morphologies over macroscopic areas, using a surprisingly short (subsecond) shear pulse. C1 [Majewski, Pawel W.; Yager, Kevin G.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Majewski, PW (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. EM pmajewski@bnl.gov; kyager@bnl.gov RI Yager, Kevin/F-9804-2011 OI Yager, Kevin/0000-0001-7745-2513 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0012704] FX Research was carried out at the Center for Functional Nanomaterials, and National Synchrotron Light Source, Brookhaven National Laboratory, which are supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract DE-SC0012704. NR 58 TC 6 Z9 6 U1 6 U2 27 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD JUL 14 PY 2015 VL 48 IS 13 BP 4591 EP 4598 DI 10.1021/acs.macromol.5b00955 PG 8 WC Polymer Science SC Polymer Science GA CN0LK UT WOS:000358104900038 ER PT J AU Hur, SM Onses, MS Ramirez-Hernandez, A Nealey, PF Rogers, JA de Pablo, JJ AF Hur, Su-Mi Onses, M. Serdar Ramirez-Hernandez, Abelardo Nealey, Paul F. Rogers, John A. de Pablo, Juan J. TI Interplay of Surface Energy and Bulk Thermodynamic Forces in Ordered Block Copolymer Droplets SO MACROMOLECULES LA English DT Article ID MONTE-CARLO SIMULATIONS; THIN-FILMS; DIBLOCK COPOLYMERS; WETTING BEHAVIOR; PARTICLES; NANODROPLETS; POLYMERS; MODEL; MELTS AB The wetting state of a simple liquid on a solid substrate, as summarized by Young's equation, is dictated by the interfacial energies of the different phases that coexist in the system. For simple fluids, rotational symmetry gives rise to symmetric droplets around the axis perpendicular to the substrate. This is not the case for nanostructured fluids, such as block copolymers, where the inherent thermodynamic ordering forces compete with surface tension. This competition is particularly important in nanoscale droplets, where the size of the droplets is a small multiple of the natural periodicity of the block copolymer in the bulk. In the nanoscale regime, droplet shape and internal structure arise from a subtle interplay between interfacial and bulk contributions to the free energy. In this work, we examine the consequences of surface polymer interaction energies on droplet morphology through a concerted simulation and experimental effort. When the block copolymer is deposited on a neutral substrate, we find noncircular arrangements with perpendicular domains. However, when a preferential substrate is used, the resulting morphology depends on droplet size. In large droplets, we observe bottle-cap-shaped structures with a ring of perpendicular domains along the perimeter, while small droplets exhibit stripes of perpendicular domains. C1 [Hur, Su-Mi; Ramirez-Hernandez, Abelardo; Nealey, Paul F.; de Pablo, Juan J.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Hur, Su-Mi; Ramirez-Hernandez, Abelardo; Nealey, Paul F.; de Pablo, Juan J.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. [Onses, M. Serdar; Rogers, John A.] Univ Illinois, Beckman Inst, Dept Mat Sci & Engn, Urbana, IL 61801 USA. [Onses, M. Serdar; Rogers, John A.] Univ Illinois, Frederick Seitz Mat Res Lab, Urbana, IL 61801 USA. [Onses, M. Serdar] Erciyes Univ, Dept Mat Sci & Engn, Nanotechnol Res Ctr ERNAM, TR-38039 Kayseri, Turkey. [Hur, Su-Mi] Chonnam Natl Univ, Sch Polymer Sci & Engn, Kwangju 500757, South Korea. RP Rogers, JA (reprint author), Univ Illinois, Beckman Inst, Dept Mat Sci & Engn, Urbana, IL 61801 USA. EM jrogers@illinois.edu; depablo@uchicago.edu RI Ramirez-Hernandez, Abelardo/A-1717-2011; Rogers, John /L-2798-2016 OI Ramirez-Hernandez, Abelardo/0000-0002-3569-5223; FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; Air Force Office of Scientific Research MURI [FA9550-12-1-0471] FX An award of computer time was provided by the INCITE program of the Argonne Leadership Computing Facility. We gratefully acknowledge the computing resources provided on Blues, high-performance computing cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory. S.M.H., A.R.H., P.F.N, and J.J.d.P. acknowledge support from U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. The experimental work was supported by the Air Force Office of Scientific Research MURI FA9550-12-1-0471. NR 44 TC 2 Z9 2 U1 5 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD JUL 14 PY 2015 VL 48 IS 13 BP 4717 EP 4723 DI 10.1021/acs.macromol.5b00630 PG 7 WC Polymer Science SC Polymer Science GA CN0LK UT WOS:000358104900049 ER PT J AU Lee, SR Wright, AF Modine, NA Battaile, CC Foiles, SM Thomas, JC Van der Ven, A AF Lee, S. R. Wright, A. F. Modine, N. A. Battaile, C. C. Foiles, S. M. Thomas, J. C. Van der Ven, A. TI First-principles survey of the structure, formation energies, and transition levels of As-interstitial defects in InGaAs SO PHYSICAL REVIEW B LA English DT Article ID POINT-DEFECTS; ELECTRON-GAS; PSEUDOPOTENTIALS; SEMICONDUCTORS; ALLOYS; SOLIDS; STRAIN AB While point defects in elemental (Si) and compound (GaAs, GaN, AlN) semiconductors have been extensively studied both experimentally and theoretically, only limited theoretical studies of these defects exist for technologically important binary (SixGe1-x) and pseudobinary (InxGa1-xAs, InxGa1-xN, AlxGa1-xN) semiconductor alloys. Here, we use density-functional theory and a recently developed bounds-analysis approach to survey the atomic structures, formation energies, and charge-state transition levels of the stable and metastable states of As interstitials in the pseudobinary alloy In0.5Ga0.5As. Our studies consider seven different candidate defect structures for the As interstitial, with calculations performed for selected defect charge states in the range q = -2 to + 3. In each case, the mean and standard deviations of the defect-formation energy are determined using statistical sampling methods that place the defect into a wide variety of differing local-alloy environments. When examined from the point of view of the mean formation energy of the defect, the stable configurations of the As interstitial in In0.5Ga0.5As are found to resemble previous findings for GaAs, with a C-1h-p001(III) interstitial structure in a q = + 1 charge state favored near midgap and below, and a C-2v-110(a) split-interstitial structure in a q = -1 charge state favored above midgap (the named point-group symmetries refer to the underlying symmetry that the alloy defect would possess if within GaAs). The statistical sampling reveals a strong dependence of the defect-formation energy on the local-alloy environment, with the standard deviation sigma of the formation energy approaching 0.21 eV for the most stable As-interstitial structures. Because the range of ground-state energies encountered by an As-interstitial defect when moving through the alloy is found to be quite large, approaching similar to 1.2 eV (+/- 3 sigma), defect-diffusion pathways in In0.5Ga0.5As will have spatial and temporal complexities not found in GaAs. C1 [Lee, S. R.; Wright, A. F.; Modine, N. A.; Battaile, C. C.; Foiles, S. M.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Thomas, J. C.; Van der Ven, A.] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. RP Lee, SR (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM srlee@sandia.gov OI Foiles, Stephen/0000-0002-1907-454X FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 47 TC 4 Z9 4 U1 8 U2 26 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUL 14 PY 2015 VL 92 IS 4 AR 045205 DI 10.1103/PhysRevB.92.045205 PG 14 WC Physics, Condensed Matter SC Physics GA CM7GA UT WOS:000357857500002 ER PT J AU Zhao, YX Allada, K Aniol, K Annand, JRM Averett, T Benmokhtar, F Bertozzi, W Bradshaw, PC Bosted, P Camsonne, A Canan, M Cates, GD Chen, C Chen, JP Chen, W Chirapatpimol, K Chudakov, E Cisbani, E Cornejo, JC Cusanno, F Dalton, M Deconinck, W de Jager, CW De Leo, R Deng, X Deur, A Ding, H Dolph, PAM Dutta, C Dutta, D El Fassi, L Frullani, S Gao, H Garibaldi, F Gaskell, D Gilad, S Gilman, R Glamazdin, O Golge, S Guo, L Hamilton, D Hansen, O Higinbotham, DW Holmstrom, T Huang, J Huang, M Ibrahim, HF Iodice, M Jiang, X Jin, G Jones, MK Katich, J Kelleher, A Kim, W Kolarkar, A Korsch, W LeRose, JJ Li, X Li, Y Lindgren, R Liyanage, N Long, E Lu, HJ Margaziotis, DJ Markowitz, P Marrone, S McNulty, D Meziani, ZE Michaels, R Moffit, B Camacho, CM Nanda, S Narayan, A Nelyubin, V Norum, B Oh, Y Osipenko, M Parno, D Peng, JC Phillips, SK Posik, M Puckett, AJR Qian, X Qiang, Y Rakhman, A Ransome, R Riordan, S Saha, A Sawatzky, B Schulte, E Shahinyan, A Shabestari, MH Sirca, S Stepanyan, S Subedi, R Sulkosky, V Tang, LG Tobias, WA Urciuoli, GM Vilardi, I Wang, K Wojtsekhowski, B Wang, Y Yan, X Yao, H Ye, Y Ye, Z Yuan, L Zhan, X Zhang, Y Zhang, YW Zhao, B Zheng, X Zhu, L Zhu, X Zong, X AF Zhao, Y. X. Allada, K. Aniol, K. Annand, J. R. M. Averett, T. Benmokhtar, F. Bertozzi, W. Bradshaw, P. C. Bosted, P. Camsonne, A. Canan, M. Cates, G. D. Chen, C. Chen, J. -P. Chen, W. Chirapatpimol, K. Chudakov, E. Cisbani, E. Cornejo, J. C. Cusanno, F. Dalton, M. Deconinck, W. de Jager, C. W. De Leo, R. Deng, X. Deur, A. Ding, H. Dolph, P. A. M. Dutta, C. Dutta, D. El Fassi, L. Frullani, S. Gao, H. Garibaldi, F. Gaskell, D. Gilad, S. Gilman, R. Glamazdin, O. Golge, S. Guo, L. Hamilton, D. Hansen, O. Higinbotham, D. W. Holmstrom, T. Huang, J. Huang, M. Ibrahim, H. F. Iodice, M. Jiang, X. Jin, G. Jones, M. K. Katich, J. Kelleher, A. Kim, W. Kolarkar, A. Korsch, W. LeRose, J. J. Li, X. Li, Y. Lindgren, R. Liyanage, N. Long, E. Lu, H. -J. Margaziotis, D. J. Markowitz, P. Marrone, S. McNulty, D. Meziani, Z. -E. Michaels, R. Moffit, B. Camacho, C. Munoz Nanda, S. Narayan, A. Nelyubin, V. Norum, B. Oh, Y. Osipenko, M. Parno, D. Peng, J. -C. Phillips, S. K. Posik, M. Puckett, A. J. R. Qian, X. Qiang, Y. Rakhman, A. Ransome, R. Riordan, S. Saha, A. Sawatzky, B. Schulte, E. Shahinyan, A. Shabestari, M. H. Sirca, S. Stepanyan, S. Subedi, R. Sulkosky, V. Tang, L. -G. Tobias, W. A. Urciuoli, G. M. Vilardi, I. Wang, K. Wojtsekhowski, B. Wang, Y. Yan, X. Yao, H. Ye, Y. Ye, Z. Yuan, L. Zhan, X. Zhang, Y. Zhang, Y. -W. Zhao, B. Zheng, X. Zhu, L. Zhu, X. Zong, X. CA Jefferson Lab Hall A Collaboration TI Double spin asymmetries of inclusive hadron electroproduction from a transversely polarized He-3 target SO PHYSICAL REVIEW C LA English DT Article AB We report the measurement of beam-target double spin asymmetries (A(LT)) in the inclusive production of identified hadrons, (e) over right arrow + 3He(up arrow) -> h + X, using a longitudinally polarized 5.9-GeV electron beam and a transversely polarized He-3 target. Hadrons (pi(+/-), K-+/-, and proton) were detected at 16 degrees with an average momentum < Ph > = 2.35 GeV/c and a transverse momentum (p(T)) coverage from 0.60 to 0.68 GeV/c. Asymmetries from the He-3 target were observed to be nonzero for pi(+/-) production when the target was polarized transversely in the horizontal plane. The pi(+) and pi(-) asymmetries have opposite signs, analogous to the behavior of A(LT) in semi-inclusive deep-inelastic scattering. C1 [Zhao, Y. X.; Lu, H. -J.; Yan, X.; Ye, Y.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Allada, K.; Bertozzi, W.; Deconinck, W.; Gilad, S.; Huang, J.; Moffit, B.; Puckett, A. J. R.; Sulkosky, V.; Zhan, X.] MIT, Cambridge, MA 02139 USA. [Allada, K.; Bosted, P.; Camsonne, A.; Chen, J. -P.; Chudakov, E.; de Jager, C. W.; Deur, A.; Gaskell, D.; Gilman, R.; Hansen, O.; Higinbotham, D. W.; Jones, M. K.; LeRose, J. J.; Michaels, R.; Moffit, B.; Nanda, S.; Qiang, Y.; Saha, A.; Sawatzky, B.; Sulkosky, V.; Wojtsekhowski, B.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Aniol, K.; Cornejo, J. C.; Margaziotis, D. J.] Calif State Univ Los Angeles, Los Angeles, CA 90032 USA. [Annand, J. R. M.; Hamilton, D.] Univ Glasgow, Glasgow G12 8QQ, Lanark, Scotland. [Averett, T.; Bradshaw, P. C.; Katich, J.; Kelleher, A.; Zhao, B.] Coll William & Mary, Williamsburg, VA 23187 USA. [Benmokhtar, F.; Parno, D.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Canan, M.; Golge, S.] Old Dominion Univ, Norfolk, VA 23529 USA. [Cates, G. D.; Chirapatpimol, K.; Dalton, M.; de Jager, C. W.; Deng, X.; Ding, H.; Dolph, P. A. M.; Jin, G.; Lindgren, R.; Liyanage, N.; Nelyubin, V.; Norum, B.; Riordan, S.; Shabestari, M. H.; Subedi, R.; Tobias, W. A.; Wang, K.; Zheng, X.] Univ Virginia, Charlottesville, VA 22904 USA. [Chen, C.; Tang, L. -G.; Ye, Z.; Yuan, L.; Zhu, L.] Hampton Univ, Hampton, VA 23187 USA. [Chen, W.; Gao, H.; Huang, M.; Qiang, Y.; Zhu, X.; Zong, X.] Duke Univ, Durham, NC 27708 USA. [Cisbani, E.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Cisbani, E.; Frullani, S.; Garibaldi, F.] Ist Super Sanita, I-00161 Rome, Italy. [Cusanno, F.; Frullani, S.; Garibaldi, F.; Urciuoli, G. M.] Ist Nazl Fis Nucl, Sez Roma, I-00161 Rome, Italy. [De Leo, R.; Marrone, S.; Vilardi, I.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [De Leo, R.; Marrone, S.; Vilardi, I.] Univ Bari, I-70126 Bari, Italy. [Dutta, C.; Kolarkar, A.; Korsch, W.] Univ Kentucky, Lexington, KY 40506 USA. [Dutta, D.; Narayan, A.] Mississippi State Univ, Mississippi State, MS 39762 USA. [El Fassi, L.; Gilman, R.; Jiang, X.; Ransome, R.; Schulte, E.] Rutgers State Univ, Piscataway, NJ 08855 USA. [Glamazdin, O.] Kharkov Phys & Technol Inst, UA-61108 Kharkov, Ukraine. [Guo, L.; Huang, J.; Jiang, X.; Puckett, A. J. R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Guo, L.; Markowitz, P.] Florida Int Univ, Miami, FL 33199 USA. [Holmstrom, T.] Longwood Univ, Farmville, VA 23909 USA. [Ibrahim, H. F.] Cairo Univ, Giza 12613, Egypt. [Iodice, M.] Ist Nazl Fis Nucl, Sez Roma Tre, I-00146 Rome, Italy. [Kim, W.; Stepanyan, S.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Li, X.; Li, Y.] China Inst Atom Energy, Beijing, Peoples R China. [Long, E.] Kent State Univ, Kent, OH 44242 USA. [McNulty, D.] Univ Massachusetts, Amherst, MA 01003 USA. [Meziani, Z. -E.; Posik, M.; Sawatzky, B.; Yao, H.] Temple Univ, Philadelphia, PA 19122 USA. [Camacho, C. Munoz] Univ Clermont Ferrand, IN2P3, F-63177 Aubiere, France. [Oh, Y.] Seoul Natl Univ, Seoul, South Korea. [Osipenko, M.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Peng, J. -C.; Wang, Y.; Zhu, L.] Univ Illinois, Urbana, IL 61801 USA. [Phillips, S. K.] Univ New Hampshire, Durham, NH 03824 USA. [Qian, X.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Rakhman, A.] Syracuse Univ, Syracuse, NY 13244 USA. [Shahinyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Sirca, S.] Univ Ljubljana, SI-1000 Ljubljana, Slovenia. [Zhang, Y.; Zhang, Y. -W.] Lanzhou Univ, Lanzhou 730000, Gansu, Peoples R China. RP Zhao, YX (reprint author), Univ Sci & Technol China, Hefei 230026, Peoples R China. EM yxzhao@jlab.org RI Rakhman, Adurahim/K-8146-2012; Cisbani, Evaristo/C-9249-2011; Dalton, Mark/B-5380-2016; Narayan, Amrendra/Q-3243-2016; Parno, Diana/B-7546-2017; Ye, Zhihong/E-6651-2017 OI Rakhman, Adurahim/0000-0002-9880-6074; Cisbani, Evaristo/0000-0002-6774-8473; Dalton, Mark/0000-0001-9204-7559; Narayan, Amrendra/0000-0003-3814-9559; Parno, Diana/0000-0002-9363-0401; Ye, Zhihong/0000-0002-1873-2344 FU US National Science Foundation; Department of Energy (DOE) [DE-AC05-06OR23177]; National Natural Science Foundation of China [11135002, 11120101004]; UK Science and Technology Facilities Council [57071/1, 50727/1] FX We acknowledge the outstanding support of the JLab Hall A staff and the Accelerator Division in accomplishing this experiment. This work was supported in part by the US National Science Foundation and by Department of Energy (DOE) Contract No. DE-AC05-06OR23177, under which the Jefferson Science Associates operates the Thomas Jefferson National Accelerator Facility. This work was also supported by the National Natural Science Foundation of China under Grants No. 11135002 and No. 11120101004 and the UK Science and Technology Facilities Council under Grants No. 57071/1 and No. 50727/1. NR 23 TC 5 Z9 5 U1 1 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JUL 14 PY 2015 VL 92 IS 1 AR 015207 DI 10.1103/PhysRevC.92.015207 PG 6 WC Physics, Nuclear SC Physics GA CM7GL UT WOS:000357858700007 ER PT J AU Ozaki, S Arai, T Hattori, K Itakura, K AF Ozaki, Sho Arai, Takashi Hattori, Koichi Itakura, Kazunori TI Euler-Heisenberg-Weiss action for QCD plus QED SO PHYSICAL REVIEW D LA English DT Article ID HEAVY-ION COLLISIONS; FINITE-TEMPERATURE; MAGNETIC-FIELD; GAUGE-THEORIES; QUANTUM ELECTRODYNAMICS; VACUUM POLARIZATION; CHIRAL-SYMMETRY; QUARK; CHROMODYNAMICS; FLUCTUATIONS AB We derive an analytic expression for one-loop effective action of QCD + QED at zero and finite temperatures by using the Schwinger proper time method. The result is a nonlinear effective action not only for electromagnetic and chromo-electromagnetic fields but also for the Polyakov loop, and thus reproduces the Euler-Heisenberg action in QED, QCD, and QED + QCD, and also the Weiss potential for the Polyakov loop at finite temperature. As applications of this "Euler-Heisenberg-Weiss" action in QCD + QED, we investigate quark pair productions induced by QCD + QED fields at zero temperature and the Polyakov loop in the presence of strong electromagnetic fields. Quark one-loop contribution to the effective potential of the Polyakov loop explicitly breaks the center symmetry, and is found to be enhanced by the magnetic field, which is consistent with the inverse magnetic catalysis observed in lattice QCD simulation. C1 [Ozaki, Sho; Arai, Takashi; Itakura, Kazunori] KEK, High Energy Accelerator Res Org, IPNS, Theory Ctr, Tsukuba, Ibaraki 3050801, Japan. [Hattori, Koichi] RIKEN BNL Res Ctr, Brookhaven Natl Lab, Upton, NY 11973 USA. [Hattori, Koichi] RIKEN, Theoret Res Div, Nishina Ctr, Wako, Saitama 3510198, Japan. [Itakura, Kazunori] Grad Univ Adv Studies SOKENDAI, Tsukuba, Ibaraki 3050801, Japan. RP Ozaki, S (reprint author), KEK, High Energy Accelerator Res Org, IPNS, Theory Ctr, Tsukuba, Ibaraki 3050801, Japan. EM sho@post.kek.jp; tarai@post.kek.jp; koichi.hattori@riken.jp; kazunori.itakura@kek.jp FU Center for the Promotion of Integrated Sciences (CPIS) of Sokendai; JSPS [25287066] FX This work was supported in part by the Center for the Promotion of Integrated Sciences (CPIS) of Sokendai. The research of K. H. is supported by JSPS Grant-in-Aid No. 25287066. NR 56 TC 3 Z9 3 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. 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CA ATLAS Collaboration TI Search for a Heavy Neutral Particle Decaying to e mu, e tau, or mu tau in pp Collisions at root s=8 TeV with the ATLAS Detector SO PHYSICAL REVIEW LETTERS LA English DT Article AB This Letter presents a search for a heavy neutral particle decaying into an opposite-sign different-flavor dilepton pair, e(+/-) mu(-/+), e(+/-) tau(-/+), or mu(+/-) tau(-/+) using 20.3 fb(-1) of pp collision data at root s = 8 TeV collected by the ATLAS detector at the LHC. The numbers of observed candidate events are compatible with the standard model expectations. Limits are set on the cross section of new phenomena in two scenarios: the production of (nu) over tilde (tau) in R-parity-violating supersymmetric models and the production of a lepton-flavor-violating Z' vector boson. C1 [Jackson, P.; Lee, L.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. 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S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Azuelos, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Gillberg, D.; Gingrich, D. M.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkins, A. D.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Iengo, P.; Jaekel, M. R.; Jakobsen, S.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oakham, F. G.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Savard, P.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, Bw.; Vetterli, M. C.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, S.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Peng, H.; Song, H. Y.; Xu, L.; Zhang, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.; Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Anger, P.; Chen, L.; Feng, C.; Ma, L. L.; Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Thompson, E. N.; Tuts, P. M.] CNRS, Clermont Ferrand, France. [Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Thompson, E. N.; Tuts, P. M.; Zhou, L.] Columbia Univ, Nevis Lab, New York, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Collegato Cosenza, Nazl Frascati Lab, Cosenza, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Phys Nucl, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, C.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Nazl Frascati Lab, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dao, V.; Di Simone, A.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Aloisio, A.; Ancu, L. S.; Barone, G.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Picazio, A.; Pinamonti, M.; Ristic, B.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, High Energy Phys Inst, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Denis, R. D. St.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bindi, M.; Blumenschein, U.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.] Univ Grenoble Alpes, Lab Phys Subatom & Cosmol, CNRS, IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokoshin, F.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R. W.; Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, J.; Henderson, R. C. W.; Hughes, E. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Price, J.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; George, M.; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grinstein, S.; Grossi, G. C.; Jana, D. K.; Juste Rozas, A.; Martinez, M.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjoermark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Poettgen, R.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Pilkington, A. D.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Conventi, F.; Della Pietra, M.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Conventi, F.; Della Pietra, M.; Diglio, S.; Djama, F.; Feligioni, L.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Hu, X.; Levin, D.; Long, J. D.; Lu, N.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Xu, L.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Villaplana Perez, M.] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Turra, R.; Villaplana Perez, M.] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.; Yacoob, S.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Conventi, F.; Della Pietra, M.; Di Donato, C.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Koenig, A. C.; Nektarijevic, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Beacham, J. B.; Daya-Ishmukhametova, R. K.; Gan, K. K.; Kagan, H.; Kass, R. D.; Looper, K. A.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Khanov, A.; Rizatdinova, F.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Aloisio, A.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lin, S. C.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simon, D.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. 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R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Lipeles, E.; Machado Miguens, J.; Meyer, C.; Stahlman, J.; Thomson, E.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dipartimento Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Fac Ciencias & Tecnol, Caparica, Portugal. Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Nemecek, S.; Sicho, P.; Staroba, P.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Fedin, O. L.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Di Ciaccio, A.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Stanescu, C.; Taccini, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Taccini, C.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Fac Sci Ain Chock, Reseau Univ Phys Hautes Energies, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Amerchich, Marrakesh, Morocco. [Boutouil, S.; Derkaoui, J. E.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, DSM IRFU Inst Rech Lois Fondamentales Univers, Commissariat Energie Atom & Energies Alternat, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; O'Neil, D. C.; Stelzer, B.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Mount, R.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.; Meehan, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Govender, N.; Lee, C. A.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hamity, G. N.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Eriksson, D.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Li, Y.; Limosani, A.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Aloisio, A.; Chu, M. L.; Hou, S.; Hsu, P. J.; Lin, S. C.; Liu, B.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Munwes, Y.; Oren, Y.; Silver, Y.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Ilic, N.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Venturi, N.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [Bawa, H. S.; Canepa, A.; Chekulaev, S. V.; Gao, Y. S.; Jovicevic, J.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Benitez Garcia, J. A.; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Benitez Garcia, J. A.; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Neubauer, M. S.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Perez, S. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, A.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Urban, J.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Swedish, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Beermann, T. A.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, S.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Tepel, F.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich C Phys, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Ahmadov, F.; Huseynov, N.; Javadov, N.] Kings Coll London, Dept Phys, London, England. [Azuelos, G.; Gingrich, D. M.; Oakham, F. G.; Savard, P.; Vetterli, M. C.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Beck, H. P.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Castro, N. F.] Univ Fribourg, Dept Phys, CH-1700 Fribourg, Switzerland. [Chelkov, G. A.] Univ Porto, Fac Ciencias, Dept Fis & Astron, P-4100 Oporto, Portugal. [Chen, L.] Tomsk State Univ, Tomsk 634050, Russia. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] Univ Napoli Parthenope, Naples, Italy. [Davies, E.] Inst Particle Phys, Waterloo, ON, Canada. [Greenwood, Z. D.; Sawyer, L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Hsu, P. J.] Inst Catalana Recerca & Estudis Avancats, Barcelona, Spain. [Ilchenko, Y.; Onyisi, P. U. E.] Natl Tsing Hua Univ, Dept Phys, Hsinchu, Taiwan. [Jejelava, J.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jenni, P.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Kono, T.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Konoplich, R.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Li, B.] Manhattan Coll, New York, NY USA. [Liu, B.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Nessi, M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Purohit, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Shi, L.; Soh, D. A.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Smirnova, L. N.; Turchikhin, S.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Tikhomirov, V. O.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Toth, J.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Xu, L.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Yusuff, I.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Smirnova, Oxana/A-4401-2013; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Vranjes Milosavljevic, Marija/F-9847-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Snesarev, Andrey/H-5090-2013; Gavrilenko, Igor/M-8260-2015; Veneziano, Stefano/J-1610-2012; Tikhomirov, Vladimir/M-6194-2015; Villa, Mauro/C-9883-2009; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Brooks, William/C-8636-2013; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; De, Kaushik/N-1953-2013; Carvalho, Joao/M-4060-2013; White, Ryan/E-2979-2015; Mitsou, Vasiliki/D-1967-2009; Zhukov, Konstantin/M-6027-2015; Shmeleva, Alevtina/M-6199-2015; Grancagnolo, Sergio/J-3957-2015; Doyle, Anthony/C-5889-2009; Livan, Michele/D-7531-2012; spagnolo, stefania/A-6359-2012; Di Domenico, Antonio/G-6301-2011; Negrini, Matteo/C-8906-2014; Tassi, Enrico/K-3958-2015; Boyko, Igor/J-3659-2013; Ciubancan, Liviu Mihai/L-2412-2015; Gerbaudo, Davide/J-4536-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Martinez, Mario /I-3549-2015; Peleganchuk, Sergey/J-6722-2014; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Garcia, Jose /H-6339-2015; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; Staroba, Pavel/G-8850-2014; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012 OI Mashinistov, Ruslan/0000-0001-7925-4676; Smirnova, Oxana/0000-0003-2517-531X; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Veneziano, Stefano/0000-0002-2598-2659; Tikhomirov, Vladimir/0000-0002-9634-0581; Villa, Mauro/0000-0002-9181-8048; Warburton, Andreas/0000-0002-2298-7315; Brooks, William/0000-0001-6161-3570; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; De, Kaushik/0000-0002-5647-4489; Carvalho, Joao/0000-0002-3015-7821; White, Ryan/0000-0003-3589-5900; Mitsou, Vasiliki/0000-0002-1533-8886; Grancagnolo, Sergio/0000-0001-8490-8304; Doyle, Anthony/0000-0001-6322-6195; Livan, Michele/0000-0002-5877-0062; spagnolo, stefania/0000-0001-7482-6348; Di Domenico, Antonio/0000-0001-8078-2759; Negrini, Matteo/0000-0003-0101-6963; Boyko, Igor/0000-0002-3355-4662; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; RGC, Hong Kong SAR, China; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; DOE, United States of America; NSF, United States of America; Leverhulme Trust, United Kingdom; Canton of Geneva, Switzerland FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; RGC, Hong Kong SAR, China; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 41 TC 8 Z9 8 U1 15 U2 70 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 14 PY 2015 VL 115 IS 3 AR 031801 DI 10.1103/PhysRevLett.115.031801 PG 18 WC Physics, Multidisciplinary SC Physics GA CM7IK UT WOS:000357864800006 ER PT J AU Ort, DR Merchant, SS Alric, J Barkan, A Blankenship, RE Bock, R Croce, R Hanson, MR Hibberd, JM Long, SP Moore, TA Moroney, J Niyogi, KK Parry, MAJ Peralta-Yahya, PP Prince, RC Redding, KE Spalding, MH van Wijk, KJ Vermaas, WFJ von Caemmerer, S Weber, APM Yeates, TO Yuan, JS Zhu, XG AF Ort, Donald R. Merchant, Sabeeha S. Alric, Jean Barkan, Alice Blankenship, Robert E. Bock, Ralph Croce, Roberta Hanson, Maureen R. Hibberd, Julian M. Long, Stephen P. Moore, Thomas A. Moroney, James Niyogi, Krishna K. Parry, Martin A. J. Peralta-Yahya, Pamela P. Prince, Roger C. Redding, Kevin E. Spalding, Martin H. van Wijk, Klaas J. Vermaas, Wim F. J. von Caemmerer, Susanne Weber, Andreas P. M. Yeates, Todd O. Yuan, Joshua S. Zhu, Xin Guang TI Redesigning photosynthesis to sustainably meet global food and bioenergy demand SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE light capture/conversion; carbon capture/conversion; smart canopy; enabling plant biotechnology tools; sustainable crop production ID CO2 DIFFUSION; PHOTORESPIRATORY BYPASSES; CANOPY PHOTOSYNTHESIS; C-4 PHOTOSYNTHESIS; SYSTEMS BIOLOGY; ANTENNA SIZE; EFFICIENCY; RUBISCO; PRODUCTIVITY; INCREASE AB The world's crop productivity is stagnating whereas population growth, rising affluence, and mandates for biofuels put increasing demands on agriculture. Meanwhile, demand for increasing cropland competes with equally crucial global sustainability and environmental protection needs. Addressing this looming agricultural crisis will be one of our greatest scientific challenges in the coming decades, and success will require substantial improvements at many levels. We assert that increasing the efficiency and productivity of photosynthesis in crop plants will be essential if this grand challenge is to be met. Here, we explore an array of prospective redesigns of plant systems at various scales, all aimed at increasing crop yields through improved photosynthetic efficiency and performance. Prospects range from straightforward alterations, already supported by preliminary evidence of feasibility, to substantial redesigns that are currently only conceptual, but that may be enabled by new developments in synthetic biology. Although some proposed redesigns are certain to face obstacles that will require alternate routes, the efforts should lead to new discoveries and technical advances with important impacts on the global problem of crop productivity and bioenergy production. C1 [Ort, Donald R.] Univ Illinois, USDA ARS, Global Change & Photosynth Res Unit, Urbana, IL 61801 USA. [Ort, Donald R.; Long, Stephen P.] Univ Illinois, Inst Genom Biol, Urbana, IL 61801 USA. [Ort, Donald R.; Long, Stephen P.] Univ Illinois, Dept Plant Biol, Urbana, IL 61801 USA. [Merchant, Sabeeha S.; Yeates, Todd O.] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. [Merchant, Sabeeha S.; Yeates, Todd O.] Univ Calif Los Angeles, Dept Energy, Inst Genom & Prote, Los Angeles, CA 90095 USA. [Alric, Jean] CNRS, Unite Mixte Rech Biol Vegetale & Microbiol Enviro, F-13115 St Paul Les Durance, France. [Barkan, Alice] Univ Oregon, Dept Biol, Eugene, OR 97403 USA. [Blankenship, Robert E.] Washington Univ, Dept Biol, St Louis, MO 63130 USA. [Blankenship, Robert E.] Washington Univ, Dept Chem, St Louis, MO 63130 USA. [Bock, Ralph] Max Planck Inst Mol Pflanzenphysiol, D-14476 Potsdam, Germany. [Croce, Roberta] Vrije Univ Amsterdam, Dept Phys & Astron, NL-1081 Amsterdam, Netherlands. [Hanson, Maureen R.] Cornell Univ, Dept Mol Biol & Genet, Ithaca, NY 14853 USA. [Hibberd, Julian M.] Univ Cambridge, Dept Plant Sci, Cambridge CB2 3EA, England. [Long, Stephen P.] Univ Illinois, Dept Crop Sci, Urbana, IL 61801 USA. [Moore, Thomas A.; Redding, Kevin E.] Arizona State Univ, Dept Chem & Biochem, Tempe, AZ 85287 USA. [Moore, Thomas A.; Redding, Kevin E.; Vermaas, Wim F. J.] Arizona State Univ, Ctr Bioenergy & Photosynth, Tempe, AZ 85287 USA. [Moroney, James] Louisiana State Univ, Dept Biol Sci, Baton Rouge, LA 70803 USA. [Niyogi, Krishna K.] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Niyogi, Krishna K.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Niyogi, Krishna K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Parry, Martin A. J.] Rothamsted Res, Harpenden AL5 2JQ, Herts, England. [Peralta-Yahya, Pamela P.] Georgia Inst Technol, Dept Chem & Biochem, Atlanta, GA 30332 USA. [Prince, Roger C.] ExxonMobil Biomed Sci, Annandale, NJ 08801 USA. [Spalding, Martin H.] Iowa State Univ, Dept Genet Dev & Cell Biol, Ames, IA 50011 USA. [van Wijk, Klaas J.] Cornell Univ, Dept Plant Biol, Ithaca, NY 14853 USA. [Vermaas, Wim F. J.] Arizona State Univ, Sch Life Sci, Tempe, AZ 85287 USA. [von Caemmerer, Susanne] Australian Natl Univ, Res Sch Biol, Canberra, ACT 2601, Australia. [Weber, Andreas P. M.] Univ Dusseldorf, Dept Plant Biochem, D-40225 Dusseldorf, Germany. [Weber, Andreas P. M.] Univ Dusseldorf, Cluster Excellence Plant Sci, D-40225 Dusseldorf, Germany. [Yuan, Joshua S.] Texas A&M Univ, Dept Plant Pathol & Microbiol, College Stn, TX 77843 USA. [Zhu, Xin Guang] Chinese Acad Sci, CAS Key Lab Computat Biol, CAS MPG Partner Inst Computat Biol, Shanghai Inst Biol Sci, Shanghai 200031, Peoples R China. RP Ort, DR (reprint author), Univ Illinois, USDA ARS, Global Change & Photosynth Res Unit, Urbana, IL 61801 USA. EM d-ort@illinois.edu RI Weber, Andreas/A-6250-2011; croce, roberta/N-4067-2014; von Caemmerer, Susanne/C-9317-2009; Alric, Jean/E-3538-2013; OI Weber, Andreas/0000-0003-0970-4672; croce, roberta/0000-0003-3469-834X; Alric, Jean/0000-0003-3574-2234; Hanson, Maureen/0000-0001-8141-3058; Parry, Martin/0000-0002-4477-672X; Yeates, Todd/0000-0001-5709-9839; Long, Stephen/0000-0002-8501-7164 FU Bill and Melinda Gates Foundation at the University of Illinois; Cold Spring Harbor Laboratory Corporate Sponsor Program FX We thank Haley Ahlers, who works on the Realizing Improved Photosynthetic Efficiency (RIPE) project funded by the Bill and Melinda Gates Foundation at the University of Illinois, for assistance with graphics. This paper was conceived at the workshop "Redesigning Photosynthesis-Identifying Opportunities and Novel Ideas" held at the Banbury Center, Cold Spring Harbor Laboratory, Cold Spring Harbor, NY, May 13-16, 2013. We thank the Cold Spring Harbor Laboratory Banbury Center for hosting and the Cold Spring Harbor Laboratory Corporate Sponsor Program for funding the workshop. NR 63 TC 59 Z9 63 U1 53 U2 179 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUL 14 PY 2015 VL 112 IS 28 BP 8529 EP 8536 DI 10.1073/pnas.1424031112 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CM7MU UT WOS:000357878700028 PM 26124102 ER PT J AU Kassner, ER Eyvazov, AB Pichler, B Munsie, TJS Dabkowska, HA Luke, GM Davis, JCS AF Kassner, Ethan R. Eyvazov, Azar B. Pichler, Benjamin Munsie, Timothy J. S. Dabkowska, Hanna A. Luke, Graeme M. Davis, J. C. Seamus TI Supercooled spin liquid state in the frustrated pyrochlore Dy2Ti2O7 SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE spin liquid; supercooled liquids; magnetic dynamics; periodic boundaries ID MAGNETIC MONOPOLES; ICE; DYNAMICS; ENTROPY AB A "supercooled" liquid develops when a fluid does not crystallize upon cooling below its ordering temperature. Instead, the microscopic relaxation times diverge so rapidly that, upon further cooling, equilibration eventually becomes impossible and glass formation occurs. Classic supercooled liquids exhibit specific identifiers including microscopic relaxation times diverging on a Vogel-Tammann-Fulcher (VTF) trajectory, a Havriliak-Negami (HN) form for the dielectric function epsilon(omega,T), and a general Kohlrausch-Williams-Watts (KWW) form for time-domain relaxation. Recently, the pyrochlore Dy2Ti2O7 has become of interest because its frustrated magnetic interactions may, in theory, lead to highly exotic magnetic fluids. However, its true magnetic state at low temperatures has proven very difficult to identify unambiguously. Here, we introduce high-precision, boundary-free magnetization transport techniques based upon toroidal geometries and gain an improved understanding of the time-and frequency-dependent magnetization dynamics of Dy2Ti2O7. We demonstrate a virtually universal HN form for the magnetic susceptibility chi(omega, T), a general KWW form for the real-time magnetic relaxation, and a divergence of the microscopic magnetic relaxation rates with the VTF trajectory. Low-temperature Dy2Ti2O7 therefore exhibits the characteristics of a supercooled magnetic liquid. One implication is that this translationally invariant lattice of strongly correlated spins may be evolving toward an unprecedented magnetic glass state, perhaps due to many-body localization of spin. C1 [Kassner, Ethan R.; Eyvazov, Azar B.; Pichler, Benjamin; Davis, J. C. Seamus] Cornell Univ, Dept Phys, Atom & Solid State Phys Lab, Ithaca, NY 14853 USA. [Pichler, Benjamin] Stanford Univ, Dept Phys, Palo Alto, CA 94301 USA. [Munsie, Timothy J. S.; Dabkowska, Hanna A.; Luke, Graeme M.] McMaster Univ, Brockhouse Inst Mat Res, Hamilton, ON L8S 4L8, Canada. [Munsie, Timothy J. S.; Luke, Graeme M.] McMaster Univ, Dept Phys, Hamilton, ON L8S 4M1, Canada. [Luke, Graeme M.] Canadian Inst Adv Res, Toronto, ON M5G 1Z8, Canada. [Davis, J. C. Seamus] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Davis, J. C. Seamus] Univ St Andrews, Sch Phys, St Andrews KY16 9SS, Fife, Scotland. [Davis, J. C. Seamus] Cornell Univ, Kavli Inst Cornell Nanoscale Sci, Ithaca, NY 14850 USA. RP Davis, JCS (reprint author), Cornell Univ, Dept Phys, Atom & Solid State Phys Lab, Ithaca, NY 14853 USA. EM jcseamusdavis@gmail.com RI Luke, Graeme/A-9094-2010 FU Gordon and Betty Moore Foundation's Emergent Phenomena in Quantum Systems Initiative [GBMF4544]; Engineering and Physical Sciences Research Council Programme Grant FX We are grateful to E. Fradkin, B. Gaulin, M. Gingras, S. Grigera, D. Hawthorn, R. Hill, E.-A. Kim, J. Kycia, M. J. Lawler, A. P. Mackenzie, R. Melko, and J. Sethna for very helpful discussions and communications. This research is funded by the Gordon and Betty Moore Foundation's Emergent Phenomena in Quantum Systems Initiative through Grant GBMF4544 and by the Engineering and Physical Sciences Research Council Programme Grant "Topological Protection and Non-Equilibrium States in Correlated Electron Systems." NR 44 TC 5 Z9 5 U1 2 U2 15 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUL 14 PY 2015 VL 112 IS 28 BP 8549 EP 8554 DI 10.1073/pnas.1511006112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CM7MU UT WOS:000357878700031 PM 26130810 ER PT J AU Willett, JW Herrou, J Briegel, A Rotskoff, G Crosson, S AF Willett, Jonathan W. Herrou, Julien Briegel, Ariane Rotskoff, Grant Crosson, Sean TI Structural asymmetry in a conserved signaling system that regulates division, replication, and virulence of an intracellular pathogen SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE Brucella abortus; two-component system; cell cycle; ChpT; CtrA ID GENERAL STRESS-RESPONSE; BACTERIAL-CELL-CYCLE; BRUCELLA-ABORTUS; HISTIDINE-KINASE; ALPHA-PROTEOBACTERIA; TRANSDUCTION PATHWAYS; ESCHERICHIA-COLI; TRANSCRIPTIONAL REGULATION; CAULOBACTER-CRESCENTUS; SINORHIZOBIUM-MELILOTI AB We have functionally and structurally defined an essential protein phosphorelay that regulates expression of genes required for growth, division, and intracellular survival of the global zoonotic pathogen Brucella abortus. Our study delineates phosphoryl transfer through this molecular pathway, which initiates from the sensor kinase CckA and proceeds through the ChpT phosphotransferase to two regulatory substrates: CtrA and CpdR. Genetic perturbation of this system results in defects in cell growth and division site selection, and a specific viability deficit inside human phagocytic cells. Thus, proper control of B. abortus division site polarity is necessary for survival in the intracellular niche. We further define the structural foundations of signaling from the central phosphotransferase, ChpT, to its response regulator substrate, CtrA, and provide evidence that there are at least two modes of interaction between ChpT and CtrA, only one of which is competent to catalyze phosphoryltransfer. The structure and dynamics of the active site on each side of the ChpT homodimer are distinct, supporting a model in which quaternary structure of the 2:2 ChpT-CtrA complex enforces an asymmetric mechanism of phosphoryl transfer between ChpT and CtrA. Our study provides mechanistic understanding, from the cellular to the atomic scale, of a conserved transcriptional regulatory system that controls the cellular and infection biology of B. abortus. More generally, our results provide insight into the structural basis of two-component signal transduction, which is broadly conserved in bacteria, plants, and fungi. C1 [Willett, Jonathan W.; Herrou, Julien; Rotskoff, Grant; Crosson, Sean] Univ Chicago, Dept Biochem & Mol Biol, Chicago, IL 60637 USA. [Willett, Jonathan W.; Herrou, Julien; Crosson, Sean] Univ Chicago, Argonne Natl Lab, Howard Taylor Ricketts Lab, Argonne, IL 60439 USA. [Briegel, Ariane] CALTECH, Div Biol & Biol Engn, Pasadena, CA 91125 USA. [Crosson, Sean] Univ Chicago, Comm Microbiol, Chicago, IL 60637 USA. RP Crosson, S (reprint author), Univ Chicago, Dept Biochem & Mol Biol, 920 E 58Th St, Chicago, IL 60637 USA. EM scrosson@uchicago.edu OI Willett, Jonathan/0000-0002-5467-4145; Rotskoff, Grant/0000-0002-7772-5179 FU federal funds from NIH-National Institute of Allergy and Infectious Diseases Grants [U19 AI107792, R01 AI107159]; NIH Ruth Kirschstein Postdoctoral Fellowship [F32 GM109661]; Michigan Economic Development Corporation; Michigan Technology Tri-Corridor Grant [085P1000817]; NIH Grant [P41 GM103622] FX We thank Aretha Fiebig and members of the S.C. laboratory for discussions and guidance during the preparation of this manuscript and Elena Solomaha and Ryan Duggan for technical assistance. This project has been funded in whole or in part with federal funds from NIH-National Institute of Allergy and Infectious Diseases Grants U19 AI107792 and R01 AI107159 (to S.C.). J.W.W. is supported by NIH Ruth Kirschstein Postdoctoral Fellowship F32 GM109661. Funding for LS-CAT Sector 21 was provided by the Michigan Economic Development Corporation and the Michigan Technology Tri-Corridor Grant 085P1000817. Small angle X-ray scattering at Advanced Photon Source-BioCAT is supported by NIH Grant P41 GM103622. NR 78 TC 8 Z9 12 U1 2 U2 14 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUL 14 PY 2015 VL 112 IS 28 BP E3709 EP E3718 DI 10.1073/pnas.1503118112 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CM7MU UT WOS:000357878700013 PM 26124143 ER PT J AU Chalupsky, J Bohacek, P Burian, T Hajkova V Hau-Riege, SP Heimann, PA Juha, L Messerschmidt, M Moeller, SP Nagler, B Rowen, M Schlotter, WF Swiggers, ML Turner, JJ Krzywinski, J AF Chalupsky, J. Bohacek, P. Burian, T. Hajkova, V. Hau-Riege, S. P. Heimann, P. A. Juha, L. Messerschmidt, M. Moeller, S. P. Nagler, B. Rowen, M. Schlotter, W. F. Swiggers, M. L. Turner, J. J. Krzywinski, J. TI Imprinting a Focused X-Ray Laser Beam to Measure Its Full Spatial Characteristics SO PHYSICAL REVIEW APPLIED LA English DT Article ID FREE-ELECTRON LASER; COHERENT-LIGHT SOURCE; MOLECULAR-SOLIDS; PHASE RETRIEVAL; PULSES; RADIATION; REGION AB The new generation of x-ray free-electron lasers opens up unique avenues for exploring matter under exotic and extreme conditions. Extensive spatial characterization of focused, typically (sub) micron-sized, laser beams is indispensable but, nevertheless, difficult to be accomplished due to excessive radiation intensities. Methods exist allowing indirect or semidirect focus characterization from a safe distance far from the focal point. Here we present a direct method of in-focus numerical phase recovery exploiting multishot desorption imprints in poly(methyl methacrylate). Shapes of the imprints serve as input data for the newly developed code PHARE (phase recovery), inspired by the iterative Gerchberg-Saxton algorithm. A procedure of dynamic input-output mixing guarantees that the algorithm always converges to a self-consistent paraxial Helmholtz equation solution, which is thereafter optimized for transverse spatial coherence. Very good agreement with single-shot ablation imprints in lead tungstate (PbWO4) is found. The experiment is carried out at the Linac Coherent Light Source with a focused beam monochromatized at 800 eV. The results of the coherence optimization indicate that the act of monochromatization may have an effect on otherwise very good transverse coherence of free-electron laser beams. C1 [Chalupsky, J.; Bohacek, P.; Burian, T.; Hajkova, V.; Juha, L.] Acad Sci Czech Republic, Inst Phys, Prague 18221, Czech Republic. [Hau-Riege, S. P.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Heimann, P. A.; Messerschmidt, M.; Moeller, S. P.; Nagler, B.; Rowen, M.; Schlotter, W. F.; Swiggers, M. L.; Turner, J. J.; Krzywinski, J.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. RP Chalupsky, J (reprint author), Acad Sci Czech Republic, Inst Phys, Slovance 2, Prague 18221, Czech Republic. EM chal@fzu.cz RI Messerschmidt, Marc/F-3796-2010 OI Messerschmidt, Marc/0000-0002-8641-3302 FU Czech Ministry of Education via Czech-U.S. scientific cooperation within KONTAKT [ME10046, LH14072]; Academy of Sciences of the Czech Republic; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]; LCLS; Stanford University through the Stanford Institute for Materials Energy Sciences (SIMES); Lawrence Berkeley National Laboratory (LBNL), University of Hamburg through the BMBF priority program [FSP 301]; Center for Free Electron Laser Science (CFEL); U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The Czech authors gratefully acknowledge funding from the Czech Ministry of Education via Grants No. ME10046 and No. LH14072 supporting the Czech-U.S. scientific cooperation within the funding scheme KONTAKT. J. C. thanks the Academy of Sciences of the Czech Republic for postdoctoral financial support. Use of the Linac Coherent Light Source (LCLS), SLAC National Accelerator Laboratory, is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515. The SXR Instrument is funded by a consortium whose membership includes the LCLS, Stanford University through the Stanford Institute for Materials Energy Sciences (SIMES), Lawrence Berkeley National Laboratory (LBNL), University of Hamburg through the BMBF priority program FSP 301, and the Center for Free Electron Laser Science (CFEL). Part of this work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 45 TC 2 Z9 2 U1 5 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2331-7019 J9 PHYS REV APPL JI Phys. Rev. Appl. PD JUL 14 PY 2015 VL 4 IS 1 AR 014004 DI 10.1103/PhysRevApplied.4.014004 PG 11 WC Physics, Applied SC Physics GA CM7IH UT WOS:000357864500001 ER PT J AU Cao, Y Ievlev, AV Morozovska, AN Chen, LQ Kalinin, SV Maksymovych, P AF Cao, Ye Ievlev, Anton V. Morozovska, Anna N. Chen, Long-Qing Kalinin, Sergei V. Maksymovych, Petro TI Intrinsic space charge layers and field enhancement in ferroelectric nanojunctions SO APPLIED PHYSICS LETTERS LA English DT Article ID THIN-FILMS; DOMAIN-STRUCTURES; CONDUCTIVITY; BIFEO3; POLARIZATION; OXIDES; DIODE; WALLS; MODEL AB Conducting characteristics of topological defects in ferroelectric materials, such as charged domain walls, engendered a broad interest on their scientific merit and the possibility of novel applications utilizing domain engineering. At the same time, the problem of electron transport in ferroelectrics still remains full of unanswered questions and becomes yet more relevant over the growing interest in ferroelectric semiconductors and new improper ferroelectric materials. We have employed self-consistent phase-field modeling to investigate the physical properties of a local metal-fen-oelectric (Pb(Zr0.2Ti0.8)O-3) junction in applied electric field. We revealed an up to 10-fold local enhancement of electric field realized by large polarization gradient and over-polarization effects due to inherent non-linear dielectric properties of Pb(Zr0.2Ti0.8)O-3. The effect is independent of bias polarity and maintains its strength prior, during and after ferroelectric switching. The observed field enhancement can be considered on similar grounds as increased doping level, giving rise to reduced switching bias and threshold voltages for charge injection, electrochemical and photoelectrochemical processes. (C) 2015 AIP Publishing LLC. C1 [Cao, Ye; Ievlev, Anton V.; Kalinin, Sergei V.; Maksymovych, Petro] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Morozovska, Anna N.] Natl Acad Sci Ukraine, Inst Phys, UA-03028 Kiev, Ukraine. [Chen, Long-Qing] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. RP Cao, Y (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RI Kalinin, Sergei/I-9096-2012; Maksymovych, Petro/C-3922-2016; Cao, Ye/L-1271-2016; Ievlev, Anton/H-3678-2012 OI Kalinin, Sergei/0000-0001-5354-6152; Maksymovych, Petro/0000-0003-0822-8459; Cao, Ye/0000-0002-7365-7447; Ievlev, Anton/0000-0003-3645-0508 FU Division of Materials Sciences and Engineering, Basic Energy Sciences, Department of Energy; Center for Nanophase Materials Sciences; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-FG02-07ER46417(Chen)]; U.S. Department of Energy [DE-AC0500OR22725] FX This research was sponsored by the Division of Materials Sciences and Engineering, Basic Energy Sciences, Department of Energy (Y.C., S.V.K., and P.M.). Research was conducted at the Center for Nanophase Materials Sciences, which also provided support (A.V.I.) and which is a DOE Office of Science User Facility. The phase-field simulation was performed in collaboration with Professor Long-Qing Chen at Penn State, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award No. DE-FG02-07ER46417(Chen). We thank Pu Yu and Ramamoorthy Ramesh for providing the PZT sample on which the I-V curves were recorded.14 This manuscript has been authored by UT-Battelle, LLC, under Contract No. DE-AC0500OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for the United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 40 TC 1 Z9 1 U1 7 U2 36 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUL 13 PY 2015 VL 107 IS 2 AR 022903 DI 10.1063/1.49263291 PG 5 WC Physics, Applied SC Physics GA CN6FS UT WOS:000358530300036 ER PT J AU Khromova, I Navarro-Cia, M Brener, I Reno, JL Ponomarev, A Mitrofanov, O AF Khromova, I. Navarro-Cia, M. Brener, I. Reno, J. L. Ponomarev, A. Mitrofanov, O. TI Dipolar resonances in conductive carbon micro-fibers probed by near-field terahertz spectroscopy SO APPLIED PHYSICS LETTERS LA English DT Article ID METAMATERIALS; FREQUENCIES; RESONATORS; GRAPHITE AB We observe dipole resonances in thin conductive carbon micro-fibers by detecting an enhanced electric field in the near-field of a single fiber at terahertz (THz) frequencies. Time-domain analysis of the electric field shows that each fiber sustains resonant current oscillations at the frequency defined by the fiber's length. Strong dependence of the observed resonance frequency and degree of field enhancement on the fibers' conductive properties enable direct non-contact probing of the THz conductivity in single carbon micro-fibers. We find the conductivity of the fibers to be within the range of 1-5 x 10(4) S/m. This approach is suitable for experimental characterization of individual doped semiconductor resonators for THz metamaterials and devices. (C) 2015 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution 3.0 Unported License. C1 [Khromova, I.; Navarro-Cia, M.; Mitrofanov, O.] UCL, Dept Elect & Elect Engn, London WC1E 7JE, England. [Khromova, I.] ITMO Univ, Int Res Ctr Nanophoton & Metamat, St Petersburg 199034, Russia. [Khromova, I.] Univ Publ Navarra, Dept Elect & Elect Engn, Navarra 31006, Spain. [Navarro-Cia, M.] Univ London Imperial Coll Sci Technol & Med, Dept Elect & Elect Engn, Opt & Semicond Devices Grp, London SW7 2BT, England. [Brener, I.; Reno, J. L.; Mitrofanov, O.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. [Brener, I.; Reno, J. L.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Ponomarev, A.] St Petersburg State Polytech Univ, St Petersburg 194064, Russia. RP Khromova, I (reprint author), UCL, Dept Elect & Elect Engn, Torrington Pl, London WC1E 7JE, England. RI Mitrofanov, Oleg/C-1938-2008; Khromova, Irina/C-7587-2011; Navarro-Cia, Miguel/L-4517-2013; OI Mitrofanov, Oleg/0000-0003-3510-2675; Khromova, Irina/0000-0002-9977-3411; Navarro-Cia, Miguel/0000-0003-0256-6465; Ponomarev, Andrey/0000-0003-2803-8281 FU Royal Society [UF130493]; RFBR [14-22-02064 ofi-m]; Imperial College London; Government of the Russian Federation [074-U01]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the Royal Society [Grant No. UF130493], RFBR [Project No. 14-22-02064 ofi-m] and Imperial College London [Junior Research Fellowship] and partially supported by the Government of the Russian Federation [Grant No. 074-U01]. This work was performed at UCL and, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. The authors thank FideNa (Spain) for the SEM images. NR 27 TC 10 Z9 10 U1 3 U2 21 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUL 13 PY 2015 VL 107 IS 2 AR 021102 DI 10.1063/1.4926628 PG 4 WC Physics, Applied SC Physics GA CN6FS UT WOS:000358530300002 ER PT J AU Landon, CD Wilke, RHT Brumbach, MT Brennecka, GL Blea-Kirby, M Ihlefeld, JF Marinella, MJ Beechem, TE AF Landon, Colin D. Wilke, Rudeger H. T. Brumbach, Michael T. Brennecka, Geoff L. Blea-Kirby, Mia Ihlefeld, Jon F. Marinella, Matthew J. Beechem, Thomas E. TI Thermal transport in tantalum oxide films for memristive applications SO APPLIED PHYSICS LETTERS LA English DT Article ID MODEL; CONDUCTIVITY; VOLTAGE; DEVICES; RRAM AB The thermal conductivity of amorphous TaOx memristive films having variable oxygen content is measured using time domain thermoreflectance. Thermal transport is described by a two-part model where the electrical contribution is quantified via the Wiedemann-Franz relation and the vibrational contribution by the minimum thermal conductivity limit for amorphous solids. The vibrational contribution remains constant near 0.9W/mK regardless of oxygen concentration, while the electrical contribution varies from 0 to 3.3 W/mK. Thus, the dominant thermal carrier in TaOx switches between vibrations and charge carriers and is controllable either by oxygen content during deposition, or dynamically by field-induced charge state migration. (C) 2015 AIP Publishing LLC. C1 [Landon, Colin D.; Wilke, Rudeger H. T.; Brumbach, Michael T.; Blea-Kirby, Mia; Ihlefeld, Jon F.; Marinella, Matthew J.; Beechem, Thomas E.] Sandia Natl Labs, Albuquerque, NM 87123 USA. [Brennecka, Geoff L.] Colorado Sch Mines, Golden, CO 80401 USA. RP Landon, CD (reprint author), Sandia Natl Labs, Albuquerque, NM 87123 USA. RI Brennecka, Geoff/J-9367-2012 OI Brennecka, Geoff/0000-0002-4476-7655 FU Sandia National Laboratories Laboratory Directed Research and Development Program; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors gratefully acknowledge financial support from Sandia National Laboratories Laboratory Directed Research and Development Program. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 32 TC 3 Z9 3 U1 3 U2 35 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUL 13 PY 2015 VL 107 IS 2 AR 023108 DI 10.1063/1.4926921 PG 4 WC Physics, Applied SC Physics GA CN6FS UT WOS:000358530300044 ER PT J AU Ren, XC Riley, JR Koleske, DD Lauhon, LJ AF Ren, Xiaochen Riley, James R. Koleske, Daniel D. Lauhon, Lincoln J. TI Correlated high-resolution x-ray diffraction, photoluminescence, and atom probe tomography analysis of continuous and discontinuous InxGa1-xN quantum wells SO APPLIED PHYSICS LETTERS LA English DT Article ID SPECIMEN PREPARATION; SURFACE SEGREGATION; HYDROGEN; GROWTH; SCATTERING; BARRIERS AB Atom probe tomography (APT) is used to characterize the influence of hydrogen dosing during GaN barrier growth on the indium distribution of InxGa1-xN quantum wells, and correlated micro-photoluminescence is used to measure changes in the emission spectrum and efficiency. Relative to the control growth. hydrogen dosing leads to a 50% increase in emission intensity arising from discontinuous quantum wells that are narrower, of lower indium content, and with more abrupt interfaces. Simulations of carrier distributions based on APT composition profiles indicate that the greater carrier confinement leads to an increased radiative recombination rate. Furthermore. APT analysis of quantum well profiles enables refinement of x-ray diffraction analysis for more accurate nondestructive measurements of composition. (C) 2015 AIP Publishing LLC. C1 [Ren, Xiaochen; Riley, James R.; Lauhon, Lincoln J.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60201 USA. [Koleske, Daniel D.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Lauhon, LJ (reprint author), Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60201 USA. EM lauhon@northwestern.edu RI Lauhon, Lincoln/B-7526-2009; REN, XIAOCHEN/G-3364-2012; OI REN, XIAOCHEN/0000-0001-5665-1038; Lauhon, Lincoln/0000-0001-6046-3304 FU Sandia's Solid-State Lighting Science Energy Frontier Research Center - U.S. Department of Energy, Office of Basic Energy Sciences; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; National Science Foundation's MRSEC program [DMR-1121262] FX The work was primarily supported by the Sandia's Solid-State Lighting Science Energy Frontier Research Center, funded by the U.S. Department of Energy, Office of Basic Energy Sciences. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. Atom-probe tomography was performed at the Northwestern University Center for Atom-Probe Tomography (NUCAPT). NUCAPT is a Shared Facility at the Materials Research Center of Northwestern University, supported by the National Science Foundation's MRSEC program (DMR-1121262). NR 36 TC 1 Z9 1 U1 4 U2 19 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUL 13 PY 2015 VL 107 IS 2 AR 022107 DI 10.1063/1.4926808 PG 5 WC Physics, Applied SC Physics GA CN6FS UT WOS:000358530300023 ER PT J AU Shao, T Qi, ZM Wang, YY Li, YY Yang, M Wang, Y Zhang, GB Liu, M AF Shao, Tao Qi, Zeming Wang, Yuyin Li, Yuanyuan Yang, Mei Wang, Yu Zhang, Guobin Liu, Miao TI Tunable metal-insulator transition in Nd1-xYxNiO3 (x=0.3, 0.4) perovskites thin film at near room temperature SO APPLIED PHYSICS LETTERS LA English DT Article ID RAY-ABSORPTION SPECTROSCOPY; RNIO3 PEROVSKITES; LOCAL-STRUCTURE AB Metal-insulator transition (MIT) occurs due to the charge disproportionation and lattice distortions in rare-earth nickelates. Existing studies revealed that the MIT behavior of rare-earth nickelates is fairly sensitive to external stress/pressure, suggesting a viable route for MIT strain engineering. Unlike applying extrinsic strain, the MIT can also be modulated by through rare-earth cation mixing, which can be viewed as intrinsic quantum stress. We choose Nd1-xYxNiO3 (x = 0.3, 0.4) perovskites thin films as a prototype system to exhibit the tunable sharp MIT at near room temperature. By adjusting Y concentration, the transition temperature of the thin films can be changed within the range of 340-360 K. X-ray diffraction, X-ray absorption tine structure (XAFS), and in situ infrared spectroscopy are employed to probe the structural and optical property variation affected by composition and temperature. The infrared transmission intensity decreases with temperature across the MIT, indicating a pronounced thermochromic effect. Meanwhile, the XAFS result exhibits that the crystal atomistic structure changes accompanying with the Y atoms incorporation and MIT phase transition. The heavily doped Y atoms result in the pre-edge peak descent and Ni-O bond elongation, suggesting an enhanced charge disproportionation effect and the weakening of hybridization between Ni-3d and O-2p orbits. (C) 2015 AIP Publishing LLC. C1 [Shao, Tao; Qi, Zeming; Wang, Yuyin; Li, Yuanyuan; Yang, Mei; Zhang, Guobin] Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230029, Anhui, Peoples R China. [Wang, Yu] Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai Synchrotron Radiat Facil, Shanghai 201204, Peoples R China. [Liu, Miao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Qi, ZM (reprint author), Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230029, Anhui, Peoples R China. EM zmqi@ustc.edu.cn RI Liu, Miao/N-9937-2013 OI Liu, Miao/0000-0002-1843-9519 FU National Natural Science Foundation of China [11275203, U1232128, U1232129]; National Key Scientific Instrument and Equipment Development Project [2011YQ130018]; Technological Development Grant of Hefei Science Center of CAS [2014TDG-HSC002]; Research foundation of Key Laboratory of Neutron Physics, China Academy of Engineering Physics [2013BB04] FX This work was supported by the National Natural Science Foundation of China (Nos. 11275203, U1232128, and U1232129), National Key Scientific Instrument and Equipment Development Project (2011YQ130018), Technological Development Grant of Hefei Science Center of CAS (2014TDG-HSC002), and Research foundation of Key Laboratory of Neutron Physics, China Academy of Engineering Physics Grant No. 2013BB04). NR 31 TC 0 Z9 0 U1 9 U2 31 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUL 13 PY 2015 VL 107 IS 2 AR 021904 DI 10.1063/1.49269171 PG 5 WC Physics, Applied SC Physics GA CN6FS UT WOS:000358530300012 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Ochesanu, S Rougny, R Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Daci, N Heracleous, N Keaveney, J Lowette, S Maes, M Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Dobur, D Favart, L Gay, APR Grebenyuk, A Leonard, A Mohammadi, A Pernie, L Randle-conde, A Reis, T Seva, T Thomas, L Velde, CV Vanlaer, P Wang, J Zenoni, F Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Crucy, S Dildick, S Fagot, A Garcia, G Mccartin, J Rios, AAO Ryckbosch, D Diblen, SS Sigamani, M Strobbe, N Thyssen, F Tytgat, M Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Nuttens, C Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alda, WL Alves, GA Brito, L Martins, MC Martins, TD Molina, J Herrera, CM Pol, ME Teles, PR Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santaolalla, J Santoro, A Sznajder, A Manganote, EJT Pereira, AV Bernardes, CA Dogra, S Tomei, TRFP Gregores, EM 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Ross, I. Sarangi, T. Savin, A. Smith, W. H. Taylor, D. Vuosalo, C. Woods, N. CA CMS Collaboration TI Constraints on the spin-parity and anomalous HVV couplings of the Higgs boson in proton collisions at 7 and 8 TeV SO PHYSICAL REVIEW D LA English DT Article ID ATLAS DETECTOR; MASSLESS PARTICLES; BROKEN SYMMETRIES; DENSITY-FUNCTION; CP-VIOLATION; FINAL-STATES; DECAYS; LHC; LEPTONS; SEARCH AB The study of the spin-parity and tensor structure of the interactions of the recently discovered Higgs boson is performed using the H -> ZZ, Z gamma*, gamma*gamma* -> 4l, H -> WW -> l(nu)l(nu), and H -> gamma gamma decay modes. The full data set recorded by the CMS experiment during the LHC run 1 is used, corresponding to an integrated luminosity of up to 5.1 fb(-1) at a center-of-mass energy of 7 TeV and up to 19.7 fb(-1) at 8 TeV. A wide range of spin-two models is excluded at a 99% confidence level or higher, or at a 99.87% confidence level for the minimal gravitylike couplings, regardless of whether assumptions are made on the production mechanism. Any mixed-parity spin-one state is excluded in the ZZ and WW modes at a greater than 99.999% confidence level. Under the hypothesis that the resonance is a spin-zero boson, the tensor structure of the interactions of the Higgs boson with two vector bosons ZZ, Z gamma, gamma gamma, and WW is investigated and limits on eleven anomalous contributions are set. Tighter constraints on anomalous HVV interactions are obtained by combining the HZZ and HWW measurements. All observations are consistent with the expectations for the standard model Higgs boson with the quantum numbers J(PC) = 0(++). C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. 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M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Longo, E.; Margaroli, F.; Micheli, F.; Organtini, G.; Rahatlou, S.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. 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H.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, I. C.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania. [Komaragiri, J. R.; Ali, M. A. B. Md] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Linares, E. Casimiro; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Pineda, A. Morelos] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Silva, C. Beirao Da Cruz E.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Iglesias, L. 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[Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Perfilov, M.; Petrushanko, S.; Savrin, V.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade 11001, Serbia. [Maestre, J. Alcaraz; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De la Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Pernie, L.; Genchev, V.; Boudoul, G.; Contardo, D.; Lingemann, J.; Hartmann, F.; Kornmayer, A.; Mohanty, A. K.; Radogna, R.; Sharma, A.; Silvestris, L.; Giordano, F.; Gennai, S.; Gerosa, R.; Lucchini, M. T.; Marzocchi, B.; Di Guida, S.; Meola, S.; Paolucci, P.; Ciangottini, D.; Spiezia, A.; Donato, S.; Palla, F.; Micheli, F.; Traczyk, P.; Casasso, S.; Finco, L.; Candelise, V.; Abbaneo, D.; Auffray, E.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Marrouche, J.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Orsini, L.; Pape, L.; Perez, E.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Rolandi, G.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Tsirou, A.; Veres, G. 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F.; Chiochia, V.; De Cosa, A.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Mejias, B. Millan; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Kao, K. Y.; Liu, Y. F.; Lu, R. -S.; Petrakou, E.; Tzeng, Y. M.; Wilken, R.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Dept Phys, Fac Sci, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Gamsizkan, H.; Isildak, B.; Karapinar, G.; Ocalan, K.; Sekmen, S.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Albayrak, E. A.; Guelmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Phys & Technol Inst, Natl Sci Ctr, UA-310108 Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-storey, S. Seif; Senkin, S.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Newbold, D. M.; Bell, K. W.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Dauncey, P.; Davies, G.; Della Negra, M.; Dunne, P.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Mathias, B.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Lawson, P.; Richardson, C.; Rohlf, J.; John, J. St.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Berry, E.; Christopher, G.; Cutts, D.; Demiragli, Z.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Rikova, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Simon, S.; Tadel, M.; Tu, Y.; Vartak, A.; Welke, C.; Wuerthwein, F.; Yagil, A.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. 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RI Benussi, Luigi/O-9684-2014; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Paulini, Manfred/N-7794-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ogul, Hasan/S-7951-2016; ciocci, maria agnese /I-2153-2015; Tinoco Mendes, Andre David/D-4314-2011; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Sznajder, Andre/L-1621-2016; Vilela Pereira, Antonio/L-4142-2016; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Hernandez Calama, Jose Maria/H-9127-2015; Cerrada, Marcos/J-6934-2014; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Novaes, Sergio/D-3532-2012; Della Ricca, Giuseppe/B-6826-2013; Chinellato, Jose Augusto/I-7972-2012; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Stahl, Achim/E-8846-2011; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Petrushanko, Sergey/D-6880-2012; Cakir, Altan/P-1024-2015; Montanari, Alessandro/J-2420-2012; Matorras, Francisco/I-4983-2015; Gennai, Simone/P-2880-2015; TUVE', Cristina/P-3933-2015; Dudko, Lev/D-7127-2012; KIM, Tae Jeong/P-7848-2015; Menasce, Dario/A-2168-2016; Paganoni, Marco/A-4235-2016; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Calvo Alamillo, Enrique/L-1203-2014; Vinogradov, Alexey/O-2375-2015; Ragazzi, Stefano/D-2463-2009; Lokhtin, Igor/D-7004-2012; Manganote, Edmilson/K-8251-2013; Fano, Livio/K-2460-2015; Grandi, Claudio/B-5654-2015; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; VARDARLI, Fuat Ilkehan/B-6360-2013; Hoorani, Hafeez/D-1791-2013; Dogra, Sunil /B-5330-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Kovac, Marko/D-5817-2017; OI Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Ogul, Hasan/0000-0002-5121-2893; ciocci, maria agnese /0000-0003-0002-5462; Tinoco Mendes, Andre David/0000-0001-5854-7699; Seixas, Joao/0000-0002-7531-0842; Sznajder, Andre/0000-0001-6998-1108; Vilela Pereira, Antonio/0000-0003-3177-4626; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Cerrada, Marcos/0000-0003-0112-1691; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; Chinellato, Jose Augusto/0000-0002-3240-6270; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Stahl, Achim/0000-0002-8369-7506; Gulmez, Erhan/0000-0002-6353-518X; Montanari, Alessandro/0000-0003-2748-6373; Matorras, Francisco/0000-0003-4295-5668; TUVE', Cristina/0000-0003-0739-3153; Dudko, Lev/0000-0002-4462-3192; KIM, Tae Jeong/0000-0001-8336-2434; Menasce, Dario/0000-0002-9918-1686; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Calvo Alamillo, Enrique/0000-0002-1100-2963; Ragazzi, Stefano/0000-0001-8219-2074; Fano, Livio/0000-0002-9007-629X; Grandi, Claudio/0000-0001-5998-3070; Rovelli, Tiziano/0000-0002-9746-4842; Gallinaro, Michele/0000-0003-1261-2277; Ulrich, Ralf/0000-0002-2535-402X; Reis, Thomas/0000-0003-3703-6624; Luukka, Panja/0000-0003-2340-4641; Jacob, Jeson/0000-0001-6895-5493; Martinez Ruiz del Arbol, Pablo/0000-0002-7737-5121; Androsov, Konstantin/0000-0003-2694-6542; ORTONA, Giacomo/0000-0001-8411-2971 FU Austrian Federal Ministry of Science, Research and Economy; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; Brazilian Funding Agency (CNPq); Brazilian Funding Agency (CAPES); Brazilian Funding Agency (FAPERJ); Brazilian Funding Agency (FAPESP); Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research, Estonia; Estonian Research Council, Estonia [IUT23-4, IUT23-6]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules/CNRS, France; Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; Bundesministerium fur Bildung und Forschung, Germany; Deutsche Forschungsgemeinschaft, Germany; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation, Hungary; National Innovation Office, Hungary; Department of Atomic Energy, India; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Ministry of Science, ICT and Future Planning, Republic of Korea; National Research Foundation (NRF), Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education (Malaysia); University of Malaya (Malaysia); Mexican Funding Agency (CINVESTAV); Mexican Funding Agency (CONACYT); Mexican Funding Agency (SEP); Mexican Funding Agency (UASLP-FAI); Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education, Poland; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Spain; Desarrollo e Innovacion and Programa Consolider-Ingenio, Spain; Swiss Funding Agency (ETH Board); Swiss Funding Agency (ETH Zurich); Swiss Funding Agency (PSI); Swiss Funding Agency (SNF); Swiss Funding Agency (UniZH); Swiss Funding Agency (Canton Zurich); Swiss Funding Agency (SER); Ministry of Science and Technology, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine, Ukraine; State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, UK; US Department of Energy; US National Science Foundation; Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS programme of Foundation for Polish Science from European Union; Regional Development Fund; Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR Project (Italy) [20108T4XTM]; EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund FX We thank Markus Schulze for optimizing the JHUGEN Monte Carlo simulation program for this analysis. We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses.; Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via IUT23-4 and IUT23-6 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules/CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Ministry of Science, ICT and Future Planning, and National Research Foundation (NRF), Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine, and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, UK; the US Department of Energy, and the US National Science Foundation. Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P.; Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS programme of Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR Project No. 20108T4XTM (Italy); the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; and the National Priorities Research Program by Qatar National Research Fund. NR 105 TC 30 Z9 30 U1 7 U2 53 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 13 PY 2015 VL 92 IS 1 AR 012004 DI 10.1103/PhysRevD.92.012004 PG 55 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CM7GQ UT WOS:000357859300001 ER PT J AU Gaire, B Haxton, DJ Sturm, FP Williams, J Gatton, A Bocharova, I Gehrken, N Schoffler, M Gassert, H Zeller, S Voigtsberger, J Jahnke, T Zohrabi, M Reedy, D Nook, C Landers, AL Belkacem, A Cocke, CL Ben-Itzhak, I Dorner, R Weber, T AF Gaire, B. Haxton, D. J. Sturm, F. P. Williams, J. Gatton, A. Bocharova, I. Gehrken, N. Schoeffler, M. Gassert, H. Zeller, S. Voigtsberger, J. Jahnke, T. Zohrabi, M. Reedy, D. Nook, C. Landers, A. L. Belkacem, A. Cocke, C. L. Ben-Itzhak, I. Doerner, R. Weber, Th. TI Auger decay and subsequent fragmentation pathways of ethylene following K-shell ionization SO PHYSICAL REVIEW A LA English DT Article ID DOUBLE PHOTOIONIZATION SPECTRA; VALENCE DOUBLE-IONIZATION; PHOTON DOUBLE-IONIZATION; ANGULAR-DISTRIBUTIONS; MOMENTUM SPECTROSCOPY; CROSS-SECTIONS; HELIUM ATOM; RECOIL-ION; MOLECULES; THRESHOLD AB The fragmentation pathways and dynamics of ethylene molecules after core ionization are explored using coincident measurements of the Auger electron and fragment ions by employing the cold target recoil-ion momentum spectroscopy method. The influence of several factors on the dynamics and kinematics of the dissociation is studied. These include propensity rules, ionization mechanisms, symmetry of the orbitals from which the Auger electrons originate, multiple scattering, conical intersections, interference, and possible core-hole localization for the double ionization of this polyatomic molecule. Energy correlation maps allow probing the multidimensional potential energy surfaces and, in combination with our multiconfiguration self-consistent field calculations, identifying the populated electronic states of the dissociating dication. The measured angular distributions of the Auger electrons in the molecular frame further support and augment these assignments. The deprotonation and molecular hydrogen ion elimination channels show a nearly isotropic Auger electron angular distribution with a small elongation along the direction perpendicular to the molecular axis. For the symmetric breakup the angular distributions show a clear influence of multiple scattering on the outgoing electrons. The lowest kinetic energy release feature of the symmetric breakup channel displays a fingerprint of entangled Auger and photoelectron motion in the angular emission pattern identifying this transition as an excellent candidate to probe core-hole localization at a conical intersection of a polyatomic molecule. C1 [Gaire, B.; Haxton, D. J.; Sturm, F. P.; Bocharova, I.; Gehrken, N.; Belkacem, A.; Weber, Th.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Haxton, D. J.] Lawrence Berkeley Natl Lab, Xray Sci Lab, Berkeley, CA 94720 USA. [Sturm, F. P.; Gehrken, N.; Schoeffler, M.; Gassert, H.; Zeller, S.; Voigtsberger, J.; Jahnke, T.; Doerner, R.] Goethe Univ Frankfurt, Inst Kernphys, D-60438 Frankfurt, Germany. [Williams, J.; Gatton, A.; Reedy, D.; Nook, C.; Landers, A. L.] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. [Zohrabi, M.; Cocke, C. L.; Ben-Itzhak, I.] Kansas State Univ, Dept Phys, JR Macdonald Lab, Manhattan, KS 66506 USA. RP Gaire, B (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RI Doerner, Reinhard/A-5340-2008; Schoeffler, Markus/B-6261-2008 OI Doerner, Reinhard/0000-0002-3728-4268; Schoeffler, Markus/0000-0001-9214-6848 FU Office of Science, Office of Basic Energy Sciences, the Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL [DE-AC02-05CH11231, DE-FG02-86ER13491]; Deutsche Akademische Austausch Dienst (DAAD); Deutsche Forschungs Gemeinschaft (DFG) FX This research used the Advance Light Source and resources of the National Energy Research Scientific Computing Center, DOE Offices of Science User Facilities supported by the Director, Office of Science, Office of Basic Energy Sciences, the Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL under Contract No. DE-AC02-05CH11231. We thank the staff of the Advanced Light Source, in particular beamline 11.0.2 scientists H. Bluhm and T. Tyliszczak for their outstanding support. JRML personnel were supported by Grant No. DE-FG02-86ER13491 from the same funding agency. We acknowledge the financial support of the Deutsche Akademische Austausch Dienst (DAAD) and the Deutsche Forschungs Gemeinschaft (DFG). NR 57 TC 2 Z9 2 U1 3 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD JUL 13 PY 2015 VL 92 IS 1 AR 013408 DI 10.1103/PhysRevA.92.013408 PG 13 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CM7EV UT WOS:000357854100011 ER PT J AU Greenman, L Koch, CP Whaley, KB AF Greenman, Loren Koch, Christiane P. Whaley, K. Birgitta TI Laser pulses for coherent xuv Raman excitation SO PHYSICAL REVIEW A LA English DT Article ID FEMTOSECOND SPECTROSCOPY; STATES; IONIZATION; MOLECULES; DYNAMICS AB We combine multichannel electronic structure theory with quantum optimal control to derive femtosecond-time-scale Raman pulse sequences that coherently populate a valence excited state. For a neon atom, Raman target populations of up to 13% are obtained. Superpositions of the ground and valence Raman states with a controllable relative phase are found to be reachable with up to 4.5% population and arbitrary phase control facilitated by the pump pulse carrier-envelope phase. Analysis of the optimized pulse structure reveals a sequential mechanism in which the valence excitation is reached via a fast (femtosecond) population transfer through an intermediate resonance state in the continuum rather than avoiding intermediate-state population with simultaneous or counterintuitive (stimulated Raman adiabatic passage) pulse sequences. Our results open a route to coupling valence excitations and core-hole excitations in molecules and aggregates that locally address specific atoms and represent an initial step towards realization of multidimensional spectroscopy in the xuv and x-ray regimes. C1 [Greenman, Loren; Whaley, K. Birgitta] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Greenman, Loren; Whaley, K. Birgitta] Univ Calif Berkeley, Kenneth S Pitzer Ctr Theoret Chem, Berkeley, CA 94720 USA. [Greenman, Loren; Whaley, K. Birgitta] Lawrence Berkeley Natl Lab, Chem Sci, Berkeley, CA 94720 USA. [Koch, Christiane P.] Univ Kassel, Theoret Phys, D-34132 Kassel, Germany. RP Whaley, KB (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM whaley@berkeley.edu RI Koch, Christiane/C-5948-2008 OI Koch, Christiane/0000-0001-6285-5766 FU NSF [CHE-1048789]; NSF international collaboration Grant [OISE-1158954]; State Hessen Initiative for the Development of Scientific and Economic Excellence (LOEWE) within focus project Electron Dynamic of Chiral Systems; DAAD FX The authors would like to thank Michael Goerz and Daniel Reich for assistance with the Krotov control code and Stefan Pabst and Robin Santra for help with the XCID TDCIS code. Additionally, we would like to acknowledge Xuan Li, Bill McCurdy, Dan Haxton, Giuseppe Sansone, Ali Belkacem, and Holger Mueller for helpful discussions. We acknowledge computational resources obtained under NSF Grant No. CHE-1048789 and travel assistance provided by NSF international collaboration Grant No. OISE-1158954 and the DAAD. C.P.K. is grateful for financial support from the State Hessen Initiative for the Development of Scientific and Economic Excellence (LOEWE) within the focus project Electron Dynamic of Chiral Systems. NR 35 TC 3 Z9 3 U1 2 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD JUL 13 PY 2015 VL 92 IS 1 AR 013407 DI 10.1103/PhysRevA.92.013407 PG 7 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CM7EV UT WOS:000357854100010 ER PT J AU Aczel, AA Li, L Garlea, VO Yan, JQ Weickert, F Zapf, VS Movshovich, R Jaime, M Baker, PJ Keppens, V Mandrus, D AF Aczel, A. A. Li, L. Garlea, V. O. Yan, J. -Q. Weickert, F. Zapf, V. S. Movshovich, R. Jaime, M. Baker, P. J. Keppens, V. Mandrus, D. TI Spin-liquid ground state in the frustrated J(1)-J(2) zigzag chain system BaTb2O4 SO PHYSICAL REVIEW B LA English DT Article ID ANTIFERROMAGNET; TB2MO2O7; DIFFRACTION; BALN(2)O(4); LANTHANIDE; RELAXATION; Y2MO2O7; ICE; LN AB We have investigated polycrystalline samples of the zigzag chain system BaTb2O4 with magnetic susceptibility, heat capacity, neutron powder diffraction, and muon spin relaxation (mu SR). No magnetic transitions are observed in the bulk measurements, while neutron diffraction reveals the presence of low-temperature, short-range, intrachain magnetic correlations between Tb3+ ions. mu SR indicates that these correlations are dynamic, as no signatures of static magnetism are detected by the technique down to 0.095 K. These combined findings provide strong evidence for a spin-liquid ground state in BaTb2O4. C1 [Aczel, A. A.; Garlea, V. O.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Li, L.; Yan, J. -Q.; Keppens, V.; Mandrus, D.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Yan, J. -Q.; Mandrus, D.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Weickert, F.; Zapf, V. S.; Movshovich, R.; Jaime, M.] Los Alamos Natl Lab, MPA CMMS, Los Alamos, NM 87545 USA. [Baker, P. J.] Rutherford Appleton Lab, STFC, ISIS Facil, Harwell Oxford OX11 0QX, Oxon, England. RP Aczel, AA (reprint author), Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. EM aczelaa@ornl.gov RI Baker, Peter/E-4216-2010; Garlea, Vasile/A-4994-2016; Aczel, Adam/A-6247-2016; Li , Ling /J-3322-2016; Jaime, Marcelo/F-3791-2015 OI Baker, Peter/0000-0002-2306-2648; Garlea, Vasile/0000-0002-5322-7271; Aczel, Adam/0000-0003-1964-1943; Li , Ling /0000-0002-2866-8323; Jaime, Marcelo/0000-0001-5360-5220 FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences; Scientific User Facilities Division; Materials Science and Engineering Division; NSF; U.S. DOE; State of Florida; U.S. Department of Energy [DE-AC05-00OR22725]; Department of Energy FX We acknowledge useful discussions with B. D. Gaulin, M. J. P. Gingras, J. A. M. Paddison, and J. R. Stewart. This research was supported by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences. A.A. A. and V.O.G. were supported by the Scientific User Facilities Division. J.-Q.Y. and D. M. were supported by the Materials Science and Engineering Division. The neutron experiments were performed at the High Flux Isotope Reactor, which is sponsored by the Scientific User Facilities Division. Work at NHMFL-LANL was supported by NSF, U.S. DOE, and the State of Florida. We thank the staff of ISIS, where the mu SR experiments were performed, for their hospitality. This manuscript has been authored by UT-Batelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The U.S. Government retains a nonexclusive, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for U.S. Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan. NR 46 TC 3 Z9 3 U1 1 U2 27 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUL 13 PY 2015 VL 92 IS 4 AR 041110 DI 10.1103/PhysRevB.92.041110 PG 5 WC Physics, Condensed Matter SC Physics GA CM7FR UT WOS:000357856400002 ER PT J AU Flaherty, FA Trelenberg, TW Li, JA Fatema, R Skofronick, JG Van Winkle, DH Safron, SA Boatner, LA AF Flaherty, F. A. Trelenberg, T. W. Li, J. A. Fatema, R. Skofronick, J. G. Van Winkle, D. H. Safron, S. A. Boatner, L. A. TI Polar catastrophe and the structure of KTa1-xNbxO3 surfaces: Results from elastic and inelastic helium atom scattering SO PHYSICAL REVIEW B LA English DT Article ID ELEVATED-TEMPERATURES; OXIDE INTERFACES; PEROVSKITES; TRANSITION; KTAO3 AB The structure and dynamics of cleaved (001) surfaces of potassium tantalates doped with niobium, KTa1-xNbxO3 (KTN), with x ranging from 0% to 30%, were measured by helium atom scattering (HAS). Through HAS time-of-flight (TOF) experiments, a dispersionless branch (Einstein phonon branch) with energy of 13-14 meV was observed across the surface Brillouin zone in all samples. When this observation is combined with the results from earlier experimental and theoretical studies on these materials, a consistent picture of the stable surface structure emerges: After cleaving the single-crystal sample, the surface should be composed of equal areas of KO and TaO2/NbO2 terraces. The data, however, suggest that K+ and O2- ions migrate from the bulk to the surface, forming a charged KO lattice that is neutralized primarily by additional K+ ions bridging pairs of surface oxygens. This structural and dynamic modification at the (001) surface of KTN appears due to its formally charged KO(-1) and TaO2/NbO2(+1) layers and avoids a "polar catastrophe." This behavior is contrasted with the (001) surface behavior of the fluoride perovskite KMnF3 with its electrically neutral KF and MnF2 layers. C1 [Flaherty, F. A.] Valdosta State Univ, Dept Phys, Valdosta, GA 31698 USA. [Trelenberg, T. W.; Li, J. A.; Fatema, R.; Skofronick, J. G.; Van Winkle, D. H.] Florida State Univ, Dept Phys, Tallahassee, FL 32306 USA. [Safron, S. A.] Florida State Univ, Dept Chem & Biochem, Tallahassee, FL 32306 USA. [Boatner, L. A.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Flaherty, FA (reprint author), Valdosta State Univ, Dept Phys, Valdosta, GA 31698 USA. EM flaherty@valdosta.edu; rip@phy.fsu.edu RI Boatner, Lynn/I-6428-2013 OI Boatner, Lynn/0000-0002-0235-7594 FU U.S. Department of Energy [DE-FG02-97ER45635]; U.S. Department of Energy, Basic Energy Sciences, Material Sciences and Engineering Division; Valdosta State University FX The authors wish to acknowledge the U.S. Department of Energy for partial support of this research through Grant No. DE-FG02-97ER45635. Research at the Oak Ridge National Laboratory for one author (L.A.B.) was sponsored by the U.S. Department of Energy, Basic Energy Sciences, Material Sciences and Engineering Division. Data analysis by one author (F.A.F.) was facilitated by a Faculty Research Seed Grant from Valdosta State University. The authors wish to thank Scott Baxter for rendering Fig. 4. NR 34 TC 0 Z9 0 U1 0 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUL 13 PY 2015 VL 92 IS 3 AR 035414 DI 10.1103/PhysRevB.92.035414 PG 5 WC Physics, Condensed Matter SC Physics GA CM7FP UT WOS:000357856100007 ER PT J AU Han, F Wan, XG Phelan, D Stoumpos, CC Sturza, M Malliakas, CD Li, QA Han, TH Zhao, QB Chung, DY Kanatzidis, MG AF Han, Fei Wan, Xiangang Phelan, Daniel Stoumpos, Constantinos C. Sturza, Mihai Malliakas, Christos D. Li, Qing'an Han, Tian-Heng Zhao, Qingbiao Chung, Duck Young Kanatzidis, Mercouri G. TI Antiferromagnetic Kondo lattice in the layered compound CePd1-xBi2 and comparison to the superconductor LaPd1-xBi2 SO PHYSICAL REVIEW B LA English DT Article ID ELECTRONIC-STRUCTURE; MAGNETIC-PROPERTIES; HEAT-CAPACITY; SYSTEMS; 1ST-PRINCIPLES; BEHAVIOR; FIELD; CEAL2 AB The layered compound CePd1-xBi2 with the tetragonal ZrCuSi2-type structure was obtained from excess Bi flux. Magnetic susceptibility data of CePd1-xBi2 show an antiferromagnetic ordering below 6 K and are anisotropic along the c axis and the ab plane. The anisotropy is attributed to crystal-electric-field (CEF) effects and a CEF model which is able to describe the susceptibility data is given. An enhanced Sommerfeld coefficient. of 0.191 J mol Ce-1 K-2 obtained from specific-heat measurement suggests a moderate Kondo effect in CePd1-xBi2. Other than the antiferromagnetic peak at 6 K, the resistivity curve shows a shoulder like behavior around 75 K which could be attributed to the interplay between Kondo and CEF effects. Magnetoresistance and Hall-effect measurements suggest that the interplay reconstructs the Fermi-surface topology of CePd1-xBi2 around 75 K. Electronic structure calculations reveal that the Pd vacancies are important to the magnetic structure and enhance the CEF effects which quench the orbital moment of Ce at low temperatures. C1 [Han, Fei; Phelan, Daniel; Stoumpos, Constantinos C.; Sturza, Mihai; Malliakas, Christos D.; Li, Qing'an; Han, Tian-Heng; Zhao, Qingbiao; Chung, Duck Young; Kanatzidis, Mercouri G.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Wan, Xiangang] Nanjing Univ, Collaborat Innovat Ctr Adv Microstruct, Sch Phys, Natl Lab Solid State Microstruct, Nanjing 210093, Jiangsu, Peoples R China. [Malliakas, Christos D.; Kanatzidis, Mercouri G.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Han, Tian-Heng] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA. [Han, Tian-Heng] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. RP Han, F (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM m-kanatzidis@northwestern.edu RI Han, Fei/N-2021-2013; OI Han, Fei/0000-0001-7782-2713; Stoumpos, Constantinos/0000-0001-8396-9578 FU US Department of Energy Office of Science Laboratory [DE-AC02-06CH11357]; NSF of China [11374137, 91122035, 11174124]; UChicago Argonne, LLC FX This work is supported by UChicago Argonne, LLC, operator of Argonne National Laboratory, a US Department of Energy Office of Science Laboratory operated under Contract No. DE-AC02-06CH11357. Work done at Nanjing University (by X.W.) is supported by the NSF of China (Grants No. 11374137, No. 91122035, and No. 11174124). NR 36 TC 3 Z9 3 U1 1 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUL 13 PY 2015 VL 92 IS 4 AR 045112 DI 10.1103/PhysRevB.92.045112 PG 8 WC Physics, Condensed Matter SC Physics GA CM7FR UT WOS:000357856400005 ER PT J AU Wang, M Valdivia, P Yi, M Chen, JX Zhang, WL Ewings, RA Perring, TG Zhao, Y Harriger, LW Lynn, JW Bourret-Courchesne, E Dai, PC Lee, DH Yao, DX Birgeneau, RJ AF Wang, Meng Valdivia, P. Yi, Ming Chen, J. X. Zhang, W. L. Ewings, R. A. Perring, T. G. Zhao, Yang Harriger, L. W. Lynn, J. W. Bourret-Courchesne, E. Dai, Pengcheng Lee, D. H. Yao, D. X. Birgeneau, R. J. TI Spin waves and spatially anisotropic exchange interactions in the S=2 stripe antiferromagnet Rb0.8Fe1.5S2 SO PHYSICAL REVIEW B LA English DT Article ID SUPERCONDUCTORS; MAGNETISM AB An inelastic neutron scattering study of the spin waves corresponding to the stripe antiferromagnetic order in insulating Rb0.8Fe1.5S2 throughout the Brillouin zone is reported. The spin wave spectra are well described by a Heisenberg Hamiltonian with anisotropic in-plane exchange interactions. Integrating the ordered moment and the spin fluctuations results in a total moment squared of 27.6 +/- 4.2 mu(2)(B)/Fe, consistent with S approximate to 2. Unlike XFe2As2 (X = Ca, Sr, and Ba), where the itinerant electrons have a significant contribution, our data suggest that this stripe antiferromagnetically ordered phase in Rb0.8Fe1.5S2 is a Mott-like insulator with fully localized 3d electrons and a high-spin ground state configuration. Nevertheless, the anisotropic exchange couplings appear to be universal in the stripe phase of Fe pnictides and chalcogenides. C1 [Wang, Meng; Valdivia, P.; Yi, Ming; Lee, D. H.; Birgeneau, R. J.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Chen, J. X.; Yao, D. X.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Zhang, W. L.] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Ewings, R. A.; Perring, T. G.] Rutherford Appleton Lab, STFC, ISIS Pulsed Muon & Neutron Source, Didcot OX11 0QX, Oxon, England. [Zhao, Yang; Harriger, L. W.; Lynn, J. W.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Zhao, Yang] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. [Bourret-Courchesne, E.; Lee, D. H.; Birgeneau, R. J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Sci Mat, Berkeley, CA 94720 USA. [Dai, Pengcheng] Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. [Birgeneau, R. J.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Wang, M (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM wangm@berkeley.edu RI Dai, Pengcheng /C-9171-2012; WANG, MENG/E-6595-2012 OI Dai, Pengcheng /0000-0002-6088-3170; WANG, MENG/0000-0002-8232-2331 FU Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC02-05CH11231]; Basic Energy Sciences U.S. DOE Grant [DE-AC03-76SF008]; U.S. DOE, BES [DE-SC0012311]; [NBRPC-2012CB821400]; [NSFC-11275279] FX We thank Qimiao Si, Yao Shen, and Jun Zhao for useful discussions. This work is supported by the Director, Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy, under Contract No. DE-AC02-05CH11231 and the office of Basic Energy Sciences U.S. DOE Grant No. DE-AC03-76SF008. We also acknowledge support from NBRPC-2012CB821400 and NSFC-11275279. Work at Rice is supported by the U.S. DOE, BES under Contract No. DE-SC0012311 (P.D.). NR 39 TC 7 Z9 7 U1 2 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUL 13 PY 2015 VL 92 IS 4 AR 041109 DI 10.1103/PhysRevB.92.041109 PG 5 WC Physics, Condensed Matter SC Physics GA CM7FR UT WOS:000357856400001 ER PT J AU Gomez-Ramos, M Moro, AM Gomez-Camacho, J Thompson, IJ AF Gomez-Ramos, M. Moro, A. M. Gomez-Camacho, J. Thompson, I. J. TI Transfer induced by core excitation within an extended distorted-wave Born approximation method SO PHYSICAL REVIEW C LA English DT Article ID ADIABATIC-APPROXIMATION; CHANNELS CALCULATIONS; DEUTERON-BREAKUP AB Background: Dynamic core-excitation effects have been found to be of importance in breakup reactions and may be of relevance when obtaining spectroscopic information from transfer reactions. Purpose: In this paper we extend the distorted-wave Born approximation (DWBA) formalism in order to allow for noncentral components in the core-core term appearing in the transition operator, which allows for dynamic core-excitation effects. Then we study these effects by applying the formalism to different (d, p) reactions. Methods: The expression of the nonlocal kernels required for the evaluation of the DWBA amplitudes has been extended so as to include noncentral parts in the core-core interaction. The DWBA scattering amplitude is then obtained by solving the corresponding inhomogeneous equation, with the new computed kernels, and the usual outgoing boundary conditions. A new DWBA code has been developed for this purpose. Results: For Be-10(d, p)Be-11, core-excitation effects are found to be almost negligible (<3%). The importance of this effect has been found to depend to a large extent on the excitation energy of the core. This has been confirmed in the Ne-30(d, p)Ne-31 case, for which the excitation energy of the first 2+ state is 0.8 MeV, and the effect of core excitation increases to approximate to 10%. Conclusions: We find dynamic core-excitation effects in transfer reactions to have small contributions to cross sections, in general. However, they should not be neglected, since they may modify the spectroscopic information obtained from these reactions and may become of importance in reactions with nuclei with a core with high deformation and low excitation energy. C1 [Gomez-Ramos, M.; Moro, A. M.; Gomez-Camacho, J.] Univ Seville, Fac Fis, Dept FAMN, E-41080 Seville, Spain. [Gomez-Camacho, J.] Ctr Nacl Aceleradores, E-41092 Seville, Spain. [Thompson, I. J.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Gomez-Ramos, M (reprint author), Univ Seville, Fac Fis, Dept FAMN, Apdo 1065, E-41080 Seville, Spain. EM mgomez40@us.es; moro@us.es; gomez@us.es; thompson97@llnl.gov RI Moro, Antonio/E-6538-2010 OI Moro, Antonio/0000-0002-0012-8894 FU Spanish Consolider-Ingenio Programme CPAN [CSD2007-00042]; Junta de Andalucia [FQM160, P07-FQM-02894]; Spanish Ministerio de Economia y Competitividad [FPA-2013-47327-C02-01-R]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Spanish Ministerio de Educacion, Cultura y Deporte; [FPA2009-07653] FX We are thankful to Professor Hermann Wolter for his suggestions and critical reading of the drafts for this paper. This work has been partially supported under grant FPA2009-07653, by the Spanish Consolider-Ingenio 2010 Programme CPAN (CSD2007-00042), by Junta de Andalucia (FQM160, P07-FQM-02894), and by Spanish Ministerio de Economia y Competitividad (FPA-2013-47327-C02-01-R) and under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. M.G.-R. acknowledges a research grant by the Spanish Ministerio de Educacion, Cultura y Deporte. NR 38 TC 3 Z9 3 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JUL 13 PY 2015 VL 92 IS 1 AR 014613 DI 10.1103/PhysRevC.92.014613 PG 11 WC Physics, Nuclear SC Physics GA CM7GJ UT WOS:000357858500002 ER PT J AU Monnai, A AF Monnai, Akihiko TI Effective distributions of quasiparticles for thermal photons SO PHYSICAL REVIEW C LA English DT Article ID QUARK-GLUON PLASMA; HEAVY-ION COLLISIONS; CENTRALITY DEPENDENCE; AZIMUTHAL ANISOTROPY; ROOT-S(NN)=2.76 TEV; NUCLEAR COLLISIONS; COLLECTIVE FLOW; ELLIPTIC FLOW; COLLABORATION; PERSPECTIVE AB It has been found in recent heavy-ion experiments that the second and the third flow harmonics of direct photons are larger than most theoretical predictions. In this study, I construct effective parton phase-space distributions with in-medium interaction using quasiparticle models so that they are consistent with a lattice QCD equation of state. Then I investigate their effects on thermal photons using a hydrodynamic model. Numerical results indicate that elliptic flow and transverse momentum spectra are modified by the corrections to Fermi-Dirac and Bose-Einstein distributions. C1 RIKEN BNL Res Ctr, Brookhaven Natl Lab, Upton, NY 11973 USA. RP Monnai, A (reprint author), RIKEN BNL Res Ctr, Brookhaven Natl Lab, Upton, NY 11973 USA. EM amonnai@riken.jp FU RIKEN Special Postdoctoral Researcher program FX The author would like to thank M. Asakawa, M. Kitazawa, K. Morita, A. Ohnishi, and B. Schenke for insightful comments. The work of A.M. is supported by RIKEN Special Postdoctoral Researcher program. Some of the results are calculated using RIKEN Integrated Cluster of Clusters (RICC). NR 59 TC 2 Z9 2 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JUL 13 PY 2015 VL 92 IS 1 AR 014905 DI 10.1103/PhysRevC.92.014905 PG 6 WC Physics, Nuclear SC Physics GA CM7GJ UT WOS:000357858500003 ER PT J AU Vasilyev, OA Klumov, BA Tkachenko, AV AF Vasilyev, Oleg A. Klumov, Boris A. Tkachenko, Alexei V. TI Chromatic patchy particles: Effects of specific interactions on liquid structure SO PHYSICAL REVIEW E LA English DT Article ID LENNARD-JONES SYSTEM; CRYSTALLIZATION; SIMULATIONS; NUCLEATION; CRYSTALS; GLASSES; PACKING; VALENCE; SPACE AB We study the structural and thermodynamic properties of patchy particle liquids, with a special focus on the role of "color," i.e., specific interactions between individual patches. A possible experimental realization of such "chromatic" interactions is by decorating the particle patches with single-stranded DNA linkers. The complementarity of the linkers can promote selective bond formation between predetermined pairs of patches. By using MD simulations, we compare the local connectivity, the bond orientation order, and other structural properties of the aggregates formed by the "colored" and "colorless" systems. The analysis is done for spherical particles with two different patch arrangements (tetrahedral and cubic). It is found that the aggregated (liquid) phase of the "colorless" patchy particles is better connected, denser and typically has stronger local order than the corresponding "colored" one. This, in turn, makes the colored liquid less stable thermodynamically. Specifically, we predict that in a typical case the chromatic interactions should increase the relative stability of the crystalline phase with respect to the disordered liquid, thus expanding its region in the phase diagram. C1 [Vasilyev, Oleg A.] Max Planck Inst Intelligente Syst, Stuttgart, Germany. [Vasilyev, Oleg A.] Univ Stuttgart, Inst Theoret Phys 4, D-70174 Stuttgart, Germany. [Klumov, Boris A.] Joint Inst High Temp, Moscow, Russia. [Klumov, Boris A.] RAS, LD Landau Theoret Phys Inst, Chernogolovka, Russia. [Tkachenko, Alexei V.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Vasilyev, OA (reprint author), Max Planck Inst Intelligente Syst, Heisenbergstr 3, Stuttgart, Germany. RI Tkachenko, Alexei/I-9040-2012 OI Tkachenko, Alexei/0000-0003-1291-243X FU European Research Council under FP7 IRSESMarie-Curie grants [PIRSES-GA-2010-269139, PIRSES-GA-2010-269181]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0012704]; Russian Science Foundation [14-12-01185, 14-50-00124] FX This study is supported by European Research Council under FP7 IRSESMarie-Curie grants PIRSES-GA-2010-269139 and PIRSES-GA-2010-269181. Research carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-SC0012704. Structural analysis was supported by the Russian Science Foundation, Project No. 14-12-01185. Numerical simulations were supported by the Russian Science Foundation, Project No. 14-50-00124. NR 35 TC 3 Z9 3 U1 4 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD JUL 13 PY 2015 VL 92 IS 1 AR 012308 DI 10.1103/PhysRevE.92.012308 PG 10 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA CM7HU UT WOS:000357863100005 PM 26274163 ER PT J AU Upton, MH Choi, Y Park, H Liu, J Meyers, D Chakhalian, J Middey, S Kim, JW Ryan, PJ AF Upton, M. H. Choi, Yongseong Park, Hyowon Liu, Jian Meyers, D. Chakhalian, J. Middey, S. Kim, Jong-Woo Ryan, Philip J. TI Novel Electronic Behavior Driving NdNiO3 Metal-Insulator Transition SO PHYSICAL REVIEW LETTERS LA English DT Article ID NEUTRON-DIFFRACTION; RARE-EARTH; THIN-FILMS; RNIO3 R; OXIDES; CHARGE; ND AB We present evidence that the metal-insulator transition (MIT) in a tensile-strained NdNiO3 (NNO) film is facilitated by a redistribution of electronic density and that it neither requires Ni charge disproportionation nor a symmetry change [U. Staub et al., Phys. Rev. Lett. 88, 126402 (2002); R. Jaramillo et al., Nat. Phys. 10, 304 (2014)]. Given that epitaxial tensile strain in thin NNO films induces preferential occupancy of the e(g) d(x2-y2) orbital we propose that the larger transfer integral of this orbital state with the O 2p orbital state mediates a redistribution of electronic density from the Ni atom. A decrease in the Ni d(x2-y2) orbital occupation is directly observed by resonant inelastic x-ray scattering below the MIT temperature. Furthermore, an increase in the Nd charge occupancy is measured by x-ray absorption at the Nd L-3 edge. Both spin-orbit coupling and crystal field effects combine to break the degeneracy of the Nd 5d states, shifting the energy of the Nd e(g) d(x2-y2) orbit towards the Fermi level, allowing the A site to become an active acceptor during the MIT. This work identifies the relocation of electrons from the Ni 3d to the Nd 5d orbitals across the MIT. We propose that the insulating gap opens between the Ni 3d and O 2p states, resulting from Ni 3d electron localization. The transition seems to be neither a purely Mott-Hubbard transition nor a simple charge transfer. C1 [Upton, M. H.; Choi, Yongseong; Kim, Jong-Woo; Ryan, Philip J.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Park, Hyowon] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. [Park, Hyowon] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Liu, Jian] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Liu, Jian] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Meyers, D.; Chakhalian, J.; Middey, S.] Univ Arkansas, Dept Phys, Fayetteville, AR 72701 USA. RP Upton, MH (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. EM mhupton@aps.anl.gov; pryan@aps.anl.gov RI Chakhalian, Jak/F-2274-2015; Middey, Srimanta/D-9580-2013; Liu, Jian/I-6746-2013 OI Middey, Srimanta/0000-0001-5893-0946; Liu, Jian/0000-0001-7962-2547 FU U.S. Department of Energy, Office of Science [DEAC02-06CH11357]; DOD-ARO [0402-17291]; UIC; ANL FX Work at the Advanced Photon Source is supported by the U.S. Department of Energy, Office of Science under Grant No. DEAC02-06CH11357. J.C., D.M. and S.M. were supported by DOD-ARO under the Grant No. 0402-17291. H. Park gratefully acknowledges the support of start-up funds from UIC and ANL. H. P. also acknowledges the computing resources provided on Blues, a high-performance computing cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory. NR 26 TC 7 Z9 7 U1 11 U2 79 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 13 PY 2015 VL 115 IS 3 AR 036401 DI 10.1103/PhysRevLett.115.036401 PG 5 WC Physics, Multidisciplinary SC Physics GA CM7II UT WOS:000357864600012 PM 26230808 ER PT J AU Misztal, PK Hewitt, CN Wildt, J Blande, JD Eller, ASD Fares, S Gentner, DR Gilman, JB Graus, M Greenberg, J Guenther, AB Hansel, A Harley, P Huang, M Jardine, K Karl, T Kaser, L Keutsch, FN Kiendler-Scharr, A Kleist, E Lerner, BM Li, T Mak, J Nolscher, AC Schnitzhofer, R Sinha, V Thornton, B Warneke, C Wegener, F Werner, C Williams, J Worton, DR Yassaa, N Goldstein, AH AF Misztal, P. K. Hewitt, C. N. Wildt, J. Blande, J. D. Eller, A. S. D. Fares, S. Gentner, D. R. Gilman, J. B. Graus, M. Greenberg, J. Guenther, A. B. Hansel, A. Harley, P. Huang, M. Jardine, K. Karl, T. Kaser, L. Keutsch, F. N. Kiendler-Scharr, A. Kleist, E. Lerner, B. M. Li, T. Mak, J. Noelscher, A. C. Schnitzhofer, R. Sinha, V. Thornton, B. Warneke, C. Wegener, F. Werner, C. Williams, J. Worton, D. R. Yassaa, N. Goldstein, A. H. TI Atmospheric benzenoid emissions from plants rival those from fossil fuels SO SCIENTIFIC REPORTS LA English DT Article ID VOLATILE ORGANIC-COMPOUNDS; BIOGENIC EMISSIONS; COMPOUND EMISSIONS; ACID BIOSYNTHESIS; SHIKIMATE PATHWAY; SALICYLIC-ACID; VOC EMISSIONS; AEROSOL; TOLUENE; DIVERSITY AB Despite the known biochemical production of a range of aromatic compounds by plants and the presence of benzenoids in floral scents, the emissions of only a few benzenoid compounds have been reported from the biosphere to the atmosphere. Here, using evidence from measurements at aircraft, ecosystem, tree, branch and leaf scales, with complementary isotopic labeling experiments, we show that vegetation (leaves, flowers, and phytoplankton) emits a wide variety of benzenoid compounds to the atmosphere at substantial rates. Controlled environment experiments show that plants are able to alter their metabolism to produce and release many benzenoids under stress conditions. The functions of these compounds remain unclear but may be related to chemical communication and protection against stress. We estimate the total global secondary organic aerosol potential from biogenic benzenoids to be similar to that from anthropogenic benzenoids (similar to 10 Tg y(-1)), pointing to the importance of these natural emissions in atmospheric physics and chemistry. C1 [Misztal, P. K.; Fares, S.; Worton, D. R.; Goldstein, A. H.] Univ Calif Berkeley, Environm Sci Policy & Management, Berkeley, CA 94720 USA. [Misztal, P. K.; Guenther, A. B.; Harley, P.; Huang, M.; Kaser, L.] Natl Ctr Atmospher Res, Div Atmospher Chem, Boulder, CO 80301 USA. [Hewitt, C. N.] Univ Lancaster, Lancaster Environm Ctr, Lancaster LA1 4YQ, England. [Wildt, J.; Kleist, E.] Forschungszentrum Julich, Inst IBG 2, Phytosphare, D-52425 Julich, Germany. [Blande, J. D.; Li, T.] Univ Eastern Finland, Dept Environm Sci, Kuopio 70211, Finland. [Eller, A. S. D.; Gilman, J. B.; Graus, M.; Lerner, B. M.; Warneke, C.] Univ Colorado, CIRES, Boulder, CO 80309 USA. [Eller, A. S. D.] Univ Colorado, Dept Ecol & Evolutionary Biol, Boulder, CO 80309 USA. [Fares, S.] Council Agr Res & Econ, Res Ctr Soil Plant Syst, Rome, Italy. [Gentner, D. R.] Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA. [Gentner, D. R.] Yale Univ, Chem & Environm Engn, New Haven, CT 06520 USA. [Gilman, J. B.; Graus, M.; Warneke, C.] ESRL NOAA, Div Chem Sci, Boulder, CO 80305 USA. [Guenther, A. B.] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Guenther, A. B.] Washington State Univ, Dept Civil & Environm Engn, Pullman, WA 99164 USA. [Hansel, A.; Kaser, L.; Schnitzhofer, R.] Univ Innsbruck, Inst Ion Phys & Appl Phys, A-6020 Innsbruck, Austria. [Harley, P.] Estonian Univ Life Sci, Dept Plant Physiol, Tartu, Estonia. [Jardine, K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Climate Sci Dept, Berkeley, CA 94720 USA. [Karl, T.] Univ Innsbruck, Inst Atmospher & Cryospher Sci, A-6020 Innsbruck, Austria. [Keutsch, F. N.] Univ Wisconsin, Dept Chem, Madison, WI 53706 USA. [Kiendler-Scharr, A.] Forschungszentrum Julich, Troposphare, Inst IEK 8, D-52425 Julich, Germany. [Mak, J.] SUNY Stony Brook, Sch Marine & Atmospher Sci, Stony Brook, NY 11794 USA. [Noelscher, A. C.; Williams, J.] Max Planck Inst Chem, D-55128 Mainz, Germany. [Sinha, V.] Indian Inst Sci Educ & Res Mohali, Dept Earth & Environm Sci, Mohali, India. [Thornton, B.] Univ No Colorado, Sch Biol Sci, Greeley, CO 80639 USA. [Wegener, F.; Werner, C.] Univ Bayreuth, AgroEcosyst Res, BAYCEER, D-95447 Bayreuth, Germany. [Worton, D. R.] Aerosol Dynam Inc, Berkeley, CA 94710 USA. [Yassaa, N.] Univ Sci & Technol Houari Boumediene, Fac Chem, Algiers, Algeria. [Yassaa, N.] CDER, Algiers, Algeria. RP Misztal, PK (reprint author), Univ Calif Berkeley, Environm Sci Policy & Management, Berkeley, CA 94720 USA. EM pkm@berkeley.edu RI Sinha, Vinayak/C-2309-2009; Karl, Thomas/D-1891-2009; Fares, Silvano/H-4322-2011; Graus, Martin/E-7546-2010; Gilman, Jessica/E-7751-2010; Jardine, Kolby/N-2802-2013; Manager, CSD Publications/B-2789-2015; Werner, Christiane/B-2948-2009; Kiendler-Scharr, Astrid/E-8439-2011; Worton, David/A-8374-2012; Hansel, Armin/F-3915-2010; Warneke, Carsten/E-7174-2010; Lerner, Brian/H-6556-2013 OI Misztal, Pawel K/0000-0003-1060-1750; Blande, James/0000-0001-6822-0649; Sinha, Vinayak/0000-0002-5508-0779; Karl, Thomas/0000-0003-2869-9426; Fares, Silvano/0000-0002-1990-0928; Graus, Martin/0000-0002-2025-9242; Gilman, Jessica/0000-0002-7899-9948; Jardine, Kolby/0000-0001-8491-9310; Werner, Christiane/0000-0002-7676-9057; Kiendler-Scharr, Astrid/0000-0003-3166-2253; Worton, David/0000-0002-6558-5586; Hansel, Armin/0000-0002-1062-2394; Lerner, Brian/0000-0001-8721-8165 FU Austrian Science Fund (FWF) [L518-N20]; DOC-fFORTE-fellowship of the Austrian Academy of Science; National Science Foundation FX We thank Gunner Schade (Texas A&M University, USA) and Neil Cape (Centre for Ecology & Hydrology, UK) for useful comments and discussions. The work at Manitou Forest was financially supported by the Austrian Science Fund (FWF) under the project number L518-N20. LK is a recipient of a DOC-fFORTE-fellowship of the Austrian Academy of Science. The National Center for Atmospheric Research is sponsored by the National Science Foundation operated by the University Corporation for Atmospheric Research. NR 42 TC 13 Z9 14 U1 6 U2 51 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUL 13 PY 2015 VL 5 AR 12064 DI 10.1038/srep12064 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CM7CQ UT WOS:000357848400001 PM 26165168 ER PT J AU Kochem, A O'Hagan, M Wiedner, ES van Gastel, M AF Kochem, Amelie O'Hagan, Molly Wiedner, Eric S. van Gastel, Maurice TI Combined Spectroscopic and Electrochemical Detection of a Ni-I center dot center dot center dot H-N Bonding Interaction with Relevance to Electrocatalytic H-2 Production SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE HYSCORE; electrochemistry; hydrogen; nickel; protonation ID ORDER REGULAR APPROXIMATION; HYDROGEN-PRODUCTION; PENDANT AMINES; MOLECULAR ELECTROCATALYSTS; NICKEL ELECTROCATALYST; HARTREE-FOCK; OXIDATION; CATALYST; COMPLEXES; WATER AB The [Ni((P2N2R')-N-R)(2)](2+) family of complexes are exceptionally active catalysts for proton reduction to H-2. In this manuscript, we explore the first protonation step of the proposed catalytic cycle by using a catalytically inactive Ni-I complex possessing a sterically demanding variation of the ligand. Due to the paramagnetic nature of the Ni-I oxidation state, the protonated Ni-I intermediate has been characterized through a combination of cyclic voltammetry, electron nuclear double resonance (ENDOR) spectroscopy, and hyperfine sublevel correlation (HYSCORE) spectroscopy. Both the electrochemical and spectroscopic studies indicate that the Ni-I complex is protonated at a pendant amine that is endo to Ni, which suggests the presence of an intramolecular Ni-I center dot center dot center dot HN bonding interaction. Using density functional theory, the hydrogen bond was found to involve three doubly-occupied, localized molecular orbitals: the 3d(xz), 3d(z2), and 3d(yz) orbitals of nickel. These studies provide the first direct experimental evidence for this critical catalytic intermediate, and implications for catalytic H-2 production are discussed. C1 [Kochem, Amelie; O'Hagan, Molly] Max Planck Inst Chem Energy Convers, D-45470 Mulheim An Der Ruhr, Germany. [Wiedner, Eric S.; van Gastel, Maurice] Pacific NW Natl Lab, Div Phys Sci, Ctr Mol Electrocatalysis, Richland, WA 99352 USA. RP Wiedner, ES (reprint author), Pacific NW Natl Lab, Div Phys Sci, Ctr Mol Electrocatalysis, POB 999,K2-57, Richland, WA 99352 USA. EM eswiedner@pnnl.gov; maurice.van-gastel@cec.mpg.de RI van Gastel, Maurice/G-8572-2012 OI van Gastel, Maurice/0000-0002-1547-6365 FU Max Planck Society; Center for Molecular Electrocatalysis, an Energy Frontier Research Center - US Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences FX The authors thank Prof. Mihail Atanasov and Dr. Dan DuBois for helpful discussions. We also thank Dr. Jonathan M. Darmon for designing the Frontispiece. Research was supported by the Max Planck Society (EPR, ENDOR, and HYSCORE spectroscopy, computational studies), and as part of the Center for Molecular Electrocatalysis, an Energy Frontier Research Center funded by the US Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (synthesis of Ni complexes, electrochemistry, NMR spectroscopy). Pacific Northwest National Laboratory is operated by Battelle for DOE. NR 64 TC 3 Z9 3 U1 0 U2 15 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD JUL 13 PY 2015 VL 21 IS 29 BP 10338 EP 10347 DI 10.1002/chem.201500954 PG 98 WC Chemistry, Multidisciplinary SC Chemistry GA CL9WE UT WOS:000357328200001 PM 26041715 ER PT J AU Zhou, M Yi, S Luk, TS Gan, QQ Fan, SH Yu, ZF AF Zhou, Ming Yi, Soongyu Luk, Ting Shan Gan, Qiaoqiang Fan, Shanhui Yu, Zongfu TI Analog of superradiant emission in thermal emitters SO PHYSICAL REVIEW B LA English DT Article ID COUPLED-MODE THEORY; PHOTONIC CRYSTALS; NANOSCALE; NANOSTRUCTURES; METAMATERIALS; CONVERSION; RADIATION; BAND AB When wave effects of thermal photons become significant, thermal emitters can exhibit intriguing coherent effects. Here, we show that the superradiant emission, which was originally found in quantum emitters, can be realized in resonant thermal emitters. Similar to the superradiance in quantum emitters, the in-phase oscillation of resonant emitters reduces the lifetime of thermal photons in the emitters. Unlike the atomic superradiance, one remarkable consequence of the thermal superradiance is the anomalous power scaling, where the emission power can scale inversely with the number of thermal emitters. More thermal emitters generate less power due to the coherent interference of thermal photons. C1 [Zhou, Ming; Yi, Soongyu; Yu, Zongfu] Univ Wisconsin, Dept Elect & Comp Engn, Madison, WI 53706 USA. [Luk, Ting Shan] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Gan, Qiaoqiang] SUNY Buffalo, Dept Elect Engn, Buffalo, NY 14260 USA. [Fan, Shanhui] Stanford Univ, Dept Elect Engn, Stanford, CA 94305 USA. [Fan, Shanhui] Stanford Univ, Ginzton Lab, Stanford, CA 94305 USA. RP Zhou, M (reprint author), Univ Wisconsin, Dept Elect & Comp Engn, 1415 Johnson Dr, Madison, WI 53706 USA. RI Fan, Shanhui/B-4659-2012 FU Office of Naval Research [N00014-14-1-0300]; Wisconsin Alumni Research Foundation; DOE "Light-Material Interactions in Energy Conversion" Energy Frontier Research Center [DE-SC0001293] FX The authors thank Linxiao Zhu for useful discussion. Support for this research was provided by the Office of Naval Research under Grant No. N00014-14-1-0300 and by the Wisconsin Alumni Research Foundation. S.F. is supported by the DOE "Light-Material Interactions in Energy Conversion" Energy Frontier Research Center under Grant No. DE-SC0001293. NR 44 TC 5 Z9 5 U1 3 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUL 13 PY 2015 VL 92 IS 2 AR 024302 DI 10.1103/PhysRevB.92.024302 PG 7 WC Physics, Condensed Matter SC Physics GA CM7FN UT WOS:000357855900007 ER PT J AU Kacher, J Mishra, RK Minor, AM AF Kacher, Josh Mishra, Raja K. Minor, Andrew M. TI Multiscale characterization of dislocation processes in Al 5754 SO PHILOSOPHICAL MAGAZINE LA English DT Article DE dislocation dynamics; aluminium alloys; mechanical behaviour; EBSD; in situ electron microscopy; dislocation interactions; electron microscopy; dislocation mechanics ID VOLTAGE ELECTRON-MICROSCOPY; STRAIN-RATE SENSITIVITY; LE-CHATELIER BANDS; SOLID-SOLUTIONS; MG ALLOYS; ALUMINUM; DEFORMATION AB Multiscale characterization was performed on an Al-Mg alloy, Al 5754 O-temper, including in situ mechanical deformation in both the scanning electron microscope and the transmission electron microscope. Scanning electron microscopy characterization showed corresponding inhomogeneity in the dislocation and Mg distribution, with higher levels of Mg correlating with elevated levels of dislocation density. At the nanoscale, in situ transmission electron microscopy straining experiments showed that dislocation propagation through the Al matrix is characterized by frequent interactions with obstacles smaller than the imaging resolution that resulted in the formation of dislocation debris in the form of dislocation loops. Post-mortem chemical characterization and comparison to dislocation loop behaviour in an Al-Cr alloy suggests that these obstacles are small Mg clusters. Previous theoretical work and indirect experimental evidence have suggested that these Mg nanoclusters are important factors contributing to strain instabilities in Al-Mg alloys. This study provides direct experimental characterization of the interaction of glissile dislocations with these nanoclusters and the stress needed for dislocations to overcome them. C1 [Kacher, Josh; Minor, Andrew M.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Kacher, Josh; Minor, Andrew M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA. [Mishra, Raja K.] Gen Motors Res & Dev, Warren, MI USA. RP Kacher, J (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. EM jkacher@berkeley.edu RI Foundry, Molecular/G-9968-2014 FU National Science Foundation; Division of Civil; Mechanical and Manufacturing Innovation [1235610] FX This work was supported by the National Science Foundation, Division of Civil, Mechanical and Manufacturing Innovation [GOALI Grant 1235610]. NR 22 TC 0 Z9 0 U1 4 U2 11 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 1478-6435 EI 1478-6443 J9 PHILOS MAG JI Philos. Mag. PD JUL 13 PY 2015 VL 95 IS 20 BP 2198 EP 2209 DI 10.1080/14786435.2015.1054914 PG 12 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering; Physics, Applied; Physics, Condensed Matter SC Materials Science; Metallurgy & Metallurgical Engineering; Physics GA CM1BW UT WOS:000357415800005 ER PT J AU White, M AF White, Martin TI Reconstruction within the Zeldovich approximation SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE gravitation; galaxies: haloes; galaxies: statistics; cosmological parameters; large-scale structure of Universe ID BARYON ACOUSTIC-OSCILLATIONS; GRAVITATIONAL-INSTABILITY; REDSHIFT-SPACE; PERTURBATION-THEORY; DATA RELEASE; GALAXIES; SCALE; DISTORTIONS; DISTANCE; MATTER AB The Zeldovich approximation, first-order Lagrangian perturbation theory, provides a good description of the clustering of matter and galaxies on large scales. The acoustic feature in the large-scale correlation function of galaxies imprinted by sound waves in the early Universe has been successfully used as a 'standard ruler' to constrain the expansion history of the Universe. The standard ruler can be improved if a process known as density field reconstruction is employed. In this paper, we develop the Zeldovich formalism to compute the correlation function of biased tracers in both real and redshift space using the simplest reconstruction algorithm with a Gaussian kernel and compare to N-body simulations. The model qualitatively describes the effects of reconstruction on the simulations, though its quantitative success depends upon how redshift-space distortions are handled in the reconstruction algorithm. C1 [White, Martin] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [White, Martin] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [White, Martin] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP White, M (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM mwhite@berkeley.edu RI White, Martin/I-3880-2015 OI White, Martin/0000-0001-9912-5070 NR 49 TC 14 Z9 14 U1 0 U2 0 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD JUL 11 PY 2015 VL 450 IS 4 BP 3822 EP 3828 DI 10.1093/mnras/stv842 PG 7 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CQ7YY UT WOS:000360824000033 ER PT J AU Chen, A Luo, J Wang, A Broadbent, C Zhong, J Dilmanian, FA Zafonte, F Zhong, Z AF Chen, A. Luo, J. Wang, A. Broadbent, C. Zhong, J. Dilmanian, F. A. Zafonte, F. Zhong, Z. TI Fat to muscle ratio measurements with dual energy x-ray absorbtiometry SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Dual energy x-ray absorptiometry; Obesity research; Fat-to-muscle ratio ID SYNCHROTRON-RADIATION; CORONARY-ANGIOGRAPHY AB Accurate measurement of the fat-to-muscle ratio in animal model is important for obesity research. An efficient way to measure the fat to muscle ratio in animal model using dual energy absorptiornetry is presented in this paper. A radioactive source exciting x-ray fluorescence from a target material is used to provide the two x-ray energies needed. The x-rays, after transmitting through the sample, are measured with an energy sensitive Ge detector. Phantoms and specimens were measured. The results showed that the method was sensitive to the Gat to muscle ratios with good linearity. A standard deviation of a few percent in the fat to muscle ratio could be observed with the x-ray dose of 0.001 mGy. (C) 2015 Elsevier B.V. All rights reserved. C1 [Chen, A.] Shenzhen Coll Int Educ, Shenzhen, Guangdong, Peoples R China. [Luo, J.] SUNY Buffalo, Dept Biomed Engn, Buffalo, NY 14260 USA. [Wang, A.] Carnegie Mellon Univ, Dept Comp Sci, Pittsburgh, PA 15213 USA. [Broadbent, C.] Columbia Univ, Sch Engn, New York, NY 10027 USA. [Zhong, J.] Dartmouth Coll, Dept English, Hanover, NH 03755 USA. [Dilmanian, F. A.] SUNY Stony Brook, Dept Radiat Oncol, Dept Neurol, Stony Brook, NY 11794 USA. [Dilmanian, F. A.] SUNY Stony Brook, Dept Radiol, Stony Brook, NY 11794 USA. [Zafonte, F.; Zhong, Z.] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. RP Zhong, Z (reprint author), Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Bldg 743, Upton, NY 11973 USA. FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]; Brookhaven National Laboratory LDRD [05-057] FX Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract number DE-AC02-98CH10886, the Brookhaven National Laboratory LDRD 05-057, We thank Steven Townsend, Lori Steigler, and Rick Greene (all from Brookhaven Lab) for their expert technical assistance in radiation protection and source management, Nancye Wright and Gretchen Cisco, both from Brookhaven Lab, for their administrative assistance. NR 7 TC 0 Z9 0 U1 0 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 11 PY 2015 VL 788 BP 24 EP 28 DI 10.1016/j.nima.2015.03.001 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CI6LM UT WOS:000354870700005 ER PT J AU Meierbachtol, K Tovesson, F Shields, D Arnold, C Blakeley, R Bredeweg, T Devlin, M Hecht, AA Heffern, LE Jorgenson, J Laptev, A Mader, D O'Donnell, JM Sierk, A White, M AF Meierbachtol, K. Tovesson, F. Shields, D. Arnold, C. Blakeley, R. Bredeweg, T. Devlin, M. Hecht, A. A. Heffern, L. E. Jorgenson, J. Laptev, A. Mader, D. O'Donnell, J. M. Sierk, A. White, M. TI The SPIDER fission fragment spectrometer for fission product yield measurements SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Spectrometer; Fission mass yields; 2E-2 nu method; Cf-252 ID TIME-OF-FLIGHT; FAN-TUTTE SPECTROMETER; URANIUM; RADIATION; ENERGY; VELOCITIES; MASS AB The SPectrometer for Ion DEtermination in fission Research (SPIDER) has been developed for measuring mass yield distributions of fission products from spontaneous and neutron-induced fission. The 2E-2v method of measuring the kinetic energy (E) and velocity (v) of both outgoing fission products has been utilized, with the goal of measuring the mass of the fission products with an average resolution of 1 atomic mass unit (amu). The SPIDER instrument, consisting of detector components for time-of-flight, trajectory, and energy measurements, has been assembled and tested using Th-229 and (CF)-C-252 radioactive decay sources. For commissioning, the fully assembled system measured fission products from spontaneous fission of Cf-252. Individual measurement resolutions were met for time-of-flight (250 ps FWHM), spacial resolution (2 mm FHWM), and energy (92 keV FWHM for 8.376 MeV). Mass yield results measured from Cf-252 spontaneous fission products are reported from an E-v measurement. (C) 2015 Elsevier B.V. All rights reserved. C1 [Meierbachtol, K.; Tovesson, F.; Shields, D.; Arnold, C.; Bredeweg, T.; Devlin, M.; Jorgenson, J.; Laptev, A.; O'Donnell, J. M.; Sierk, A.; White, M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Blakeley, R.; Hecht, A. A.; Heffern, L. E.; Mader, D.] Univ New Mexico, Albuquerque, NM 87131 USA. [Shields, D.] Colorado Sch Mines, Golden, CO 80401 USA. RP Meierbachtol, K (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RI Devlin, Matthew/B-5089-2013; Laptev, Alexander/D-4686-2009; OI Devlin, Matthew/0000-0002-6948-2154; Laptev, Alexander/0000-0002-9759-9907; White, Morgan/0000-0003-3876-421X FU US Department of Energy by Los Alamos Security, LLC [DE-AC52-06NA25396] FX This work benefited from the use of the LANSCE accelerator facility and was performed under the auspices of the US Department of Energy by Los Alamos Security, LLC under Contract DE-AC52-06NA25396. NR 27 TC 2 Z9 2 U1 0 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 11 PY 2015 VL 788 BP 59 EP 66 DI 10.1016/j.nima.2015.02.032 PG 8 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CI6LM UT WOS:000354870700011 ER PT J AU Martinik, T Henzl, V Grape, S Svard, SJ Jansson, P Swinhoe, MT Tobin, SJ AF Martinik, Tomas Henzl, Vladimir Grape, Sophie Svard, Staffan Jacobsson Jansson, Peter Swinhoe, Martyn T. Tobin, Stephen J. TI Simulation of differential die-away instrument's response to asymmetrically burned spent nuclear fuel SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Differential die-away; Spent nuclear fuel; Asymmetrical burn-up AB Previous simulation studies of Differential Die Away (DDA) instrument's response to active interrogation of spent nuclear fuel from a pressurized water reactor (PWR) yielded promising results in terms of its capability to accurately measure or estimate basic spent fuel assembly (SFA) characteristics, such as multiplication, initial enrichment (IE) and burn-up (BU) as well as the total plutonium content. These studies were however performed only for a subset of idealized SFAs with a symmetric BU with respect to its longitudinal axis. Therefore, to complement the previous results, additional simulations have been performed of the DDA instrument's response to interrogation of asymmetrically burned spent nuclear fuel in order to determine whether derailed assay of SFAs from all 4 sides will be necessary in real life applications or whether a cost and time saving single sided assay could be used to achieve results of similar qualify as previously reported in case of symmetrically burned SFAs. The results of this study suggest that DDA instrument response depends on the position of the individual neutron defectors and in fact can be split in two modes. The first mode, measured by the back defectors, is not significantly sensitive to the spatial distribution of fissile isotopes and neutron absorbers, but rather reflects the total amount of both contributors as in the cases or symmetrically burned SFAs. In contrary, the second mode, measured by the front detectors, yields certain sensitivity to the orientation of the asymmetrically burned SFA inside the assaying instrument. This study thus provides evidence that the DDA instrument can potentially be utilized as necessary in both ways, i.e. a quick determination of the average SFA characteristics in a single assay, as well as a more detailed characterization involving several DDA observables through assay of the SFA from all of its four sides that can possibly map the burn-up distribution and/or identify diversion or replacement of pins. (C) 2015 Elsevier B.V. All rights reserved. C1 [Martinik, Tomas; Grape, Sophie; Svard, Staffan Jacobsson; Jansson, Peter; Tobin, Stephen J.] Uppsala Univ, Dept Phys & Astron, SE-75120 Uppsala, Sweden. [Martinik, Tomas; Henzl, Vladimir; Swinhoe, Martyn T.; Tobin, Stephen J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Tobin, Stephen J.] Swedish Nucl Fuel & Waste Management Co, SE-10124 Stockholm, Sweden. RP Martinik, T (reprint author), Uppsala Univ, Dept Phys & Astron, Box 516 Sweden, SE-75120 Uppsala, Sweden. EM tomas.martinik@physics.uu.se FU Next Generation Safeguards Initiative (NGSI); Office of Nonproliferation and Arms Control (NPAC); National Nuclear Security Administration (NNSA); Uppsala University FX The authors would like to acknowledge the support of Next Generation Safeguards Initiative (NGSI), Office of Nonproliferation and Arms Control (NPAC), National Nuclear Security Administration (NNSA), and Uppsala University. NR 15 TC 1 Z9 1 U1 1 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 11 PY 2015 VL 788 BP 79 EP 85 DI 10.1016/j.nima.2015.02.058 PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CI6LM UT WOS:000354870700015 ER PT J AU Vahsen, SE Hedges, MT Jaegle, I Ross, SJ Seong, IS Thorpe, TN Yamaoka, J Kadyk, JA Garcia-Sciveres, M AF Vahsen, S. E. Hedges, M. T. Jaegle, I. Ross, S. J. Seong, I. S. Thorpe, T. N. Yamaoka, J. Kadyk, J. A. Garcia-Sciveres, M. TI 3-D tracking in a miniature time projection chamber SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE TPC; GEM; Pixel; Directional; Neutron; Dark matter ID DARK-MATTER DETECTOR; FAST-NEUTRON DETECTION; PIXEL CHIP; READOUT; DRIFT; TPC; GEM; SIMULATION; AMPLIFICATION; DIFFUSION AB The three-dimensional (3-D) detection of millimeter-scale ionization trails is of interest for detecting nuclear recoils in directional fast neutron detectors and in direction-sensitive searches for weakly interacting massive particles (WIMPs), which may constitute the Dark Matter of the universe. We report on performance characterization of a miniature gas target Time Projection Chamber (TPC) where the drift charge is avalanche-multiplied with Gas Electron Multipliers (GEMs) and detected with the ATLAS FE-I3 Pixel Application Specific Integrated Circuit (ASIC). We report on measurements of gain, gain resolution, point resolution, diffusion, angular resolution, and energy resolution with low-energy X-rays, cosmic rays, and alpha particles, using the gases Ar:CO2 (70:30) and He:CO2 (70:30) at atmospheric pressure. We discuss the implications for future, larger directional neutron and Dark Matter detectors. With an eye to designing and selecting components for these, we generalize our results into analytical expressions for detector performance whenever possible. We conclude by demonstrating the 3-D directional detection of a fast neutron source. (C) 2015 Elsevier B.V. All rights reserved. C1 [Vahsen, S. E.; Hedges, M. T.; Jaegle, I.; Ross, S. J.; Seong, I. S.; Thorpe, T. N.; Yamaoka, J.] Univ Hawaii, Honolulu, HI 96322 USA. [Kadyk, J. A.; Garcia-Sciveres, M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Vahsen, SE (reprint author), Univ Hawaii, 2505 Correa Rd, Honolulu, HI 96322 USA. EM sevahsen@hawaii.edu FU U.S. Department of Homeland Security [2011-DN-077-ARI050-03]; Office of High Energy Physics of the U.S. Department of Energy [DE-SC0007852, DE-AC02-05CH11231] FX We thank Marc Rosen for his assistance in designing the support structure and test vessel. We thank Blake Pollard and Kamaluoawaiku Beamer for performing electric field simulations. We thank Peter Lewis and Bret Polopolus-Meredith for assistance during the revision process. This work was supported in part by the U.S. Department of Homeland Security under award 2011-DN-077-ARI050-03 and in part by the Office of High Energy Physics of the U.S. Department of Energy under awards DE-SC0007852 and DE-AC02-05CH11231. NR 39 TC 5 Z9 5 U1 1 U2 7 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 11 PY 2015 VL 788 BP 95 EP 105 DI 10.1016/j.nima.2015.03.009 PG 11 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CI6LM UT WOS:000354870700017 ER PT J AU Rasco, BC Fijalkowska, A Karny, M Rykaczewski, KP Wolinska-Cichocka, M Grzywacz, R Goetz, KC AF Rasco, B. C. Fijalkowska, A. Karny, M. Rykaczewski, K. P. Wolinska-Cichocka, M. Grzywacz, R. Goetz, K. C. TI The nonlinear light output of NaI(Tl) detectors in the Modular Total Absorption Spectrometer SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Beta decay; Total absorption spectrometry; NaI(Tl); Simulation; MTAS ID GAMMA-RAY SPECTROMETER; BETA-DECAY; SIMULATION AB A new detector array, the Modular Total Absorption Spectrometer (MTAS), was commissioned at the Holifield Radioactive Ion Beam Facility (HRIBF) at Oak Ridge National Lab (ORNL). Total absorption gamma spectra measured with MTAS are expected to improve beta-feeding patterns and beta strength functions in fission products. MTAS is constructed out of hexagonal NaI(Tl) detectors with a unique central module surrounded by 18 identical crystals assembled in three rings. The total NaI(Tl) mass of MTAS is over 1000 kg. The response of the central and other 18 MTAS modules to gamma-radiation was simulated using the GEANT4 toolkit modified to analyze the nonlinear light output of NaI(Tl). A detailed description of the GEANT4 modifications made is discussed. Simulated energy resolution of MTAS modules is found to agree well with the measurements for single gamma transitions of 662 keV (Cs-137) with 8.2% full width half maximum (FWHM), 835 keV (Mn-54) with FWHM of 7.5% FWHM, and 1115 keV (Zn-65) with FWHM of 6.5%. Simulations of single and multiple gamma-rays from Co-66 are also discussed. (C) 2015 Elsevier B.V. All rights reserved. C1 [Rasco, B. C.] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. [Fijalkowska, A.; Karny, M.] Univ Warsaw, Fac Phys, PL-02093 Warsaw, Poland. [Rykaczewski, K. P.; Wolinska-Cichocka, M.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Wolinska-Cichocka, M.] Oak Ridge Associated Univ, Oak Ridge, TN 37831 USA. [Wolinska-Cichocka, M.] Univ Warsaw, Heavy Ion Lab, PL-02093 Warsaw, Poland. [Grzywacz, R.; Goetz, K. C.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37966 USA. RP Rasco, BC (reprint author), Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. EM crasco@lsu.edu FU US DOE [DE-FG02-96ER40978]; Office of Nuclear Physics FX This work was supported by the US DOE by Award no. DE-FG02-96ER40978, Office of Nuclear Physics. NR 28 TC 3 Z9 3 U1 0 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 11 PY 2015 VL 788 BP 137 EP 145 DI 10.1016/j.nima.2015.03.087 PG 9 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CI6LM UT WOS:000354870700023 ER PT J AU Xie, ZP Deibele, C Schulte, MJ Hu, YH AF Xie, Zaipeng Deibele, Craig Schulte, Michael J. Hu, Yu-Hen TI Transverse beam stability measurement and analysis for the SNS accumulator ring SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Beam stability; Diagnostics; Particle accelerators; Beam instrumentation AB A field programmable gate array (FPGA)-based transverse feedback damper system was implemented in the Spallation Neutron Source (SNS) accumulator ring with the intention to stabilize the electron-proton (e-p) instability in the frequency range of 1-300 MHz. The transverse feedback damper could also be used as a diagnostic tool by measuring the beam transfer function (BTF). An analysis of the BTF measurements provides the stability diagram for the production beam at SNS. This paper describes the Feedback damper system and its setup as the BTF diagnostic tool. Experimental BTF results are presented and beam stability is analyzed by use of the BTF measurements for the SNS accumulator ring. (C) 2015 The Authors. Published by Elsevier B.V. C1 [Xie, Zaipeng; Schulte, Michael J.; Hu, Yu-Hen] Univ Wisconsin, Madison, WI 53706 USA. [Deibele, Craig] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Deibele, C (reprint author), Univ Wisconsin, Madison, WI 53706 USA. EM deibele@ornl.gov OI Xie, Zaipeng/0000-0003-1637-1511 FU Research Accelerator Division, Office of Basic Energy Sciences, US Department of Energy FX The authors are grateful to Dr. Robert Hardin for setting up the BTF measurement and Dr. Viatcheslay Danilov for technical discussions, The authors would also like to sincerely thank A. Webster, C. Peters, J. Bryan and J. Diamond for their technical expertise. Research conducted at ORNL's Spallation Neutron Source was sponsored by the Research Accelerator Division, Office of Basic Energy Sciences, US Department of Energy. NR 19 TC 0 Z9 0 U1 1 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 11 PY 2015 VL 788 BP 161 EP 167 DI 10.1016/j.nima.2015.03.038 PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CI6LM UT WOS:000354870700026 ER PT J AU Henzlova, D Menlove, HO Marlow, JB AF Henzlova, D. Menlove, H. O. Marlow, J. B. TI Design and performance of A He-3-free coincidence counter based on parallel plate boron-lined proportional technology SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Boron-lined proportional counter; He-3 replacement; Coincidence counting AB Thermal neutron counters utilized and developed for deployment as non-destructive assay (NDA) instruments in the held of nuclear safeguards traditionally rely on He-3-based proportional counting systems. He-3-based proportional counters have provided core NDA detection capabilities for several decades and have proven to be extremely reliable with range of features highly desirable for nuclear Facility deployment. Facing the current depletion of He-3 gas supply and the continuing uncertainty of options for future resupply, a search for detection technologies that could provide feasible short-term alternative to He-3 gas was initiated worldwide. As part of this effort, Los Alamos National Laboratory (LANL) designed and built a He-3-free full scale thermal neutron coincidence counter based on boron-lined proportional technology. The boron-lined technology was selected in a comprehensive inter-comparison exercise based on its favorable performance against safeguards specific parameters. This paper provides an overview of the design and initial performance evaluation of the prototype High Level Neutron counter-Boron (HLNB). The initial results suggest that current HLNB design is capable to provide similar to 80% performance of a selected reference He-3-based coincidence counter (High Level Neutron Coincidence Counter, HLNCC). Similar samples are expected to be measurable in both systems, however, slightly longer measurement times may be anticipated for large samples in HLNB. The initial evaluation helped to identify potential for further performance improvements via additional tailoring of boron-layer thickness. (C) 2015 Elsevier B.V. All rights reserved. C1 [Henzlova, D.; Menlove, H. O.; Marlow, J. B.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Henzlova, D (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM henzlova@lanl.gov FU U.S. Department of Energy, National Nuclear Security Administration, through the Office of Nuclear Nonproliferation and International Security's Next Generation Safeguards Initiative (NGSI) FX This work was funded by the U.S. Department of Energy, National Nuclear Security Administration, through the Office of Nuclear Nonproliferation and International Security's Next Generation Safeguards Initiative (NGSI). NR 19 TC 0 Z9 0 U1 0 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 11 PY 2015 VL 788 BP 188 EP 193 DI 10.1016/j.nima.2015.02.050 PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CI6LM UT WOS:000354870700030 ER PT J AU Fomin, N Greene, GL Allen, RR Cianciolo, V Crawford, C Ito, TM Huffman, PR Iverson, EB Mahurin, R Snow, WM AF Fomin, N. Greene, G. L. Allen, R. R. Cianciolo, V. Crawford, C. Ito, T. M. Huffman, P. R. Iverson, E. B. Mahurin, R. Snow, W. M. TI Fundamental neutron physics beamline at the spallation neutron source at ORNL (vol 773, pg 45, 2015) SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Correction C1 [Fomin, N.; Greene, G. L.] Univ Tennessee, Knoxville, TN 37996 USA. [Greene, G. L.; Allen, R. R.; Cianciolo, V.; Huffman, P. R.; Iverson, E. B.] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Crawford, C.] Univ Kentucky, Lexington, KY USA. [Huffman, P. R.] N Carolina State Univ, Raleigh, NC 27695 USA. [Mahurin, R.] Middle Tennessee State Univ, Murfreesboro, TN 37130 USA. [Snow, W. M.] Indiana Univ, Bloomington, IN USA. [Snow, W. M.] Ctr Explorat Energy & Matter, Bloomington, IN USA. [Ito, T. M.] Los Alamos Natl Lab, Los Alamos, NM USA. [Mahurin, R.] Univ Manitoba, Winnipeg, MB, Canada. RP Fomin, N (reprint author), Univ Tennessee, Knoxville, TN 37996 USA. EM nfomin@utk.edu NR 1 TC 0 Z9 0 U1 1 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 11 PY 2015 VL 788 BP 203 EP 203 DI 10.1016/j.nima.2015.03.029 PG 1 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CI6LM UT WOS:000354870700032 ER PT J AU Ackermann, M Arcavi, I Baldini, L Ballet, J Barbiellini, G Bastieri, D Bellazzini, R Bissaldi, E Blandford, RD Bonino, R Bottacini, E Brandt, TJ Bregeon, J Bruel, P Buehler, R Buson, S Caliandro, GA Cameron, RA Caragiulo, M Caraveo, PA Cavazzuti, E Cecchi, C Charles, E Chekhtman, A Chiang, J Chiaro, G Ciprini, S Claus, R Cohen-Tanugi, J Cutini, S D'Ammando, F de Angelis, A de Palma, F Desiante, R Di Venere, L Drell, PS Favuzzi, C Fegan, SJ Franckowiak, A Funk, S Fusco, P Gal-Yam, A Gargano, F Gasparrini, D Giglietto, N Giordano, F Giroletti, M Glanzman, T Godfrey, G Grenier, IA Grove, JE Guiriec, S Harding, AK Hayashi, K Hewitt, JW Hill, AB Horan, D Jogler, T Johannesson, G Kocevski, D Kuss, M Larsson, S Lashner, J Latronico, L Li, J Li, L Longo, F Loparco, F Lovellette, MN Lubrano, P Malyshev, D Mayer, M Mazziotta, MN McEnery, JE Michelson, PF Mizuno, T Monzani, ME Morselli, A Murase, K Nugent, P Nuss, E Ofek, E Ohsugi, T Orienti, M Orlando, E Ormes, JF Paneque, D Pesce-Rollins, M Piron, F Pivato, G Raino, S Rando, R Razzano, M Reimer, A Reimer, O Schulz, A Sgro, C Siskind, EJ Spada, F Spandre, G Spinelli, P Suson, DJ Takahashi, H Thayer, JB Tibaldo, L Torres, DF Troja, E Vianello, G Werner, M Wood, KS Wood, M AF Ackermann, M. Arcavi, I. Baldini, L. Ballet, J. Barbiellini, G. Bastieri, D. Bellazzini, R. Bissaldi, E. Blandford, R. D. Bonino, R. Bottacini, E. Brandt, T. J. Bregeon, J. Bruel, P. Buehler, R. Buson, S. Caliandro, G. A. Cameron, R. A. Caragiulo, M. Caraveo, P. A. Cavazzuti, E. Cecchi, C. Charles, E. Chekhtman, A. Chiang, J. Chiaro, G. Ciprini, S. Claus, R. Cohen-Tanugi, J. Cutini, S. D'Ammando, F. de Angelis, A. de Palma, F. Desiante, R. Di Venere, L. Drell, P. S. Favuzzi, C. Fegan, S. J. Franckowiak, A. Funk, S. Fusco, P. Gal-Yam, A. Gargano, F. Gasparrini, D. Giglietto, N. Giordano, F. Giroletti, M. Glanzman, T. Godfrey, G. Grenier, I. A. Grove, J. E. Guiriec, S. Harding, A. K. Hayashi, K. Hewitt, J. W. Hill, A. B. Horan, D. Jogler, T. Johannesson, G. Kocevski, D. Kuss, M. Larsson, S. Lashner, J. Latronico, L. Li, J. Li, L. Longo, F. Loparco, F. Lovellette, M. N. Lubrano, P. Malyshev, D. Mayer, M. Mazziotta, M. N. McEnery, J. E. Michelson, P. F. Mizuno, T. Monzani, M. E. Morselli, A. Murase, K. Nugent, P. Nuss, E. Ofek, E. Ohsugi, T. Orienti, M. Orlando, E. Ormes, J. F. Paneque, D. Pesce-Rollins, M. Piron, F. Pivato, G. Raino, S. Rando, R. Razzano, M. Reimer, A. Reimer, O. Schulz, A. Sgro, C. Siskind, E. J. Spada, F. Spandre, G. Spinelli, P. Suson, D. J. Takahashi, H. Thayer, J. B. Tibaldo, L. Torres, D. F. Troja, E. Vianello, G. Werner, M. Wood, K. S. Wood, M. TI SEARCH FOR EARLY GAMMA-RAY PRODUCTION IN SUPERNOVAE LOCATED IN A DENSE CIRCUMSTELLAR MEDIUM WITH THE FERMI LAT SO ASTROPHYSICAL JOURNAL LA English DT Article DE cosmic rays; gamma rays: general; methods: data analysis; supernovae: general ID LARGE-AREA TELESCOPE; SHOCK BREAKOUT; SN 2010JL; CONFIDENCE-INTERVALS; EMISSION; EXPLOSIONS; WIND AB Supernovae (SNe) exploding in a dense circumstellar medium (CSM) are hypothesized to accelerate cosmic rays in collisionless shocks and emit GeV gamma-rays and TeV neutrinos on a timescale of several months. We perform the first systematic search for gamma-ray emission in Fermi Large Area Telescope data in the energy range from 100 MeV to 300 GeV from the ensemble of 147 SNe Type IIn exploding in a dense CSM. We search for a gamma-ray excess at each SNe location in a one-year time window. In order to enhance a possible weak signal, we simultaneously study the closest and optically brightest sources of our sample in a joint-likelihood analysis in three different time windows (1 year, 6 months, and 3 months). For the most promising source of the sample, SN 2010jl (PTF 10aaxf), we repeat the analysis with an extended time window lasting 4.5 years. We do not find a significant excess in gamma-rays for any individual source nor for the combined sources and provide model-independent flux upper limits for both cases. In addition, we derive limits on the gamma-ray luminosity and the ratio of gamma-ray-to-optical luminosity ratio as a function of the index of the proton injection spectrum assuming a generic gamma-ray production model. Furthermore, we present detailed flux predictions based on multi-wavelength observations and the corresponding flux upper limit at a 95% confidence level (CL) for the source SN 2010jl (PTF 10aaxf). C1 [Ackermann, M.; Buehler, R.; Mayer, M.; Schulz, A.] Deutsch Elektronen Synchrotron DESY, D-15738 Zeuthen, Germany. [Baldini, L.] Univ Pisa, I-56127 Pisa, Italy. [Baldini, L.] Ist Nazl Fis Nucl, Sez Pisa, I-56127 Pisa, Italy. [Ballet, J.; Grenier, I. A.] Univ Paris Diderot, CEA Saclay, CNRS, Lab AIM,CEA IRFU,Serv Astrophys, F-91191 Gif Sur Yvette, France. [Barbiellini, G.; Desiante, R.; Longo, F.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Barbiellini, G.; Longo, F.] Univ Trieste, Dipartimento Fis, I-34127 Trieste, Italy. [Bastieri, D.; Buson, S.; Rando, R.] Ist Nazl Fis Nucl, Sez Padova, I-35131 Padua, Italy. [Bastieri, D.; Buson, S.; Chiaro, G.; Rando, R.] Univ Padua, Dipartimento Fis & Astron G Galilei, I-35131 Padua, Italy. [Bellazzini, R.; Kuss, M.; Pesce-Rollins, M.; Pivato, G.; Razzano, M.; Sgro, C.; Spada, F.; Spandre, G.; Spinelli, P.] Ist Nazl Fis Nucl, Sez Pisa, I-56127 Pisa, Italy. [Bissaldi, E.; Caragiulo, M.; de Palma, F.; Favuzzi, C.; Fusco, P.; Gargano, F.; Giglietto, N.; Giordano, F.; Loparco, F.; Mazziotta, M. N.; Raino, S.; Spinelli, P.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Blandford, R. D.; Bottacini, E.; Caliandro, G. A.; Cameron, R. A.; Charles, E.; Chiang, J.; Claus, R.; Drell, P. S.; Franckowiak, A.; Funk, S.; Glanzman, T.; Godfrey, G.; Hill, A. B.; Jogler, T.; Malyshev, D.; Michelson, P. F.; Monzani, M. E.; Orlando, E.; Paneque, D.; Reimer, A.; Reimer, O.; Thayer, J. B.; Tibaldo, L.; Vianello, G.; Wood, M.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, Dept Phys, WW Hansen Expt Phys Lab, Stanford, CA 94305 USA. [Blandford, R. D.; Bottacini, E.; Caliandro, G. A.; Cameron, R. A.; Charles, E.; Chiang, J.; Claus, R.; Drell, P. S.; Franckowiak, A.; Funk, S.; Glanzman, T.; Godfrey, G.; Hill, A. B.; Jogler, T.; Malyshev, D.; Michelson, P. F.; Monzani, M. E.; Orlando, E.; Paneque, D.; Reimer, A.; Reimer, O.; Thayer, J. B.; Tibaldo, L.; Vianello, G.; Wood, M.] Stanford Univ, SLAC Natl Accelerator Lab, Stanford, CA 94305 USA. [Bonino, R.; Latronico, L.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Bonino, R.] Univ Turin, Dipartimento Fis Gen Amadeo Avogadro, I-10125 Turin, Italy. [Brandt, T. J.; Guiriec, S.; Harding, A. K.; Hewitt, J. W.; Kocevski, D.; McEnery, J. E.; Troja, E.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Bregeon, J.; Cohen-Tanugi, J.; Nuss, E.; Piron, F.] Univ Montpellier, IN2P3, CNRS, Lab Univers & Particules Montpellier, F-34059 Montpellier, France. [Bruel, P.; Fegan, S. J.; Horan, D.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Caliandro, G. A.] Consorzio Interuniv Fis Spaziale CIFS, I-10133 Turin, Italy. [Caraveo, P. A.] INAF Ist Astrofis Spaziale & Fis Cosm, I-20133 Milan, Italy. [Cavazzuti, E.; Ciprini, S.; Cutini, S.; Gasparrini, D.] Agenzia Spaziale Italiana ASI Sci Data Ctr, I-00133 Rome, Italy. [Cecchi, C.; Ciprini, S.; Cutini, S.; Gasparrini, D.; Lubrano, P.] Ist Nazl Fis Nucl, Sez Perugia, I-06123 Perugia, Italy. [Cecchi, C.; Lubrano, P.] Univ Perugia, Dipartimento Fis, I-06123 Perugia, Italy. [Chekhtman, A.] George Mason Univ, Coll Sci, Fairfax, VA 22030 USA. [Chekhtman, A.] Naval Res Lab, Washington, DC 20375 USA. [Ciprini, S.; Cutini, S.; Gasparrini, D.] Osserv Astron Roma, INAF, I-00040 Rome, Italy. [D'Ammando, F.; Giroletti, M.; Orienti, M.] Ist Radioastron, INAF, I-40129 Bologna, Italy. [D'Ammando, F.] Univ Bologna, Dipartimento Astron, I-40127 Bologna, Italy. [de Angelis, A.] Univ Udine, Dipartimento Fis, I-33100 Udine, Italy. [de Angelis, A.] Ist Nazl Fis Nucl, Grp Collegato Udine, Sez Trieste, I-33100 Udine, Italy. [de Palma, F.] Univ Telemat Pegaso, I-80132 Naples, Italy. [Desiante, R.] Univ Udine, I-33100 Udine, Italy. [Di Venere, L.; Favuzzi, C.; Fusco, P.; Giglietto, N.; Giordano, F.; Loparco, F.; Raino, S.; Spinelli, P.] Univ Bari, Dipartimento Fis M Merlin, I-70126 Bari, Italy. [Di Venere, L.; Favuzzi, C.; Fusco, P.; Giglietto, N.; Giordano, F.; Loparco, F.; Raino, S.; Spinelli, P.] Politecn Bari, I-70126 Bari, Italy. [Grove, J. E.; Lovellette, M. N.; Wood, K. S.] Naval Res Lab, Div Space Sci, Washington, DC 20375 USA. [Hayashi, K.] Japan Aerosp Explorat Agcy, Inst Space & Astronaut Sci, Chuo Ku, Sagamihara, Kanagawa 2525210, Japan. [Hewitt, J. W.] Univ Maryland Baltimore Cty, Dept Phys, Baltimore, MD 21250 USA. [Hewitt, J. W.] Univ Maryland Baltimore Cty, Ctr Space Sci & Technol, Baltimore, MD 21250 USA. [Hewitt, J. W.] Ctr Res & Explorat Space Sci & Technol CRESST, Greenbelt, MD 20771 USA. [Hill, A. B.] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. [Johannesson, G.] Univ Iceland, Inst Sci, IS-107 Reykjavik, Iceland. [Larsson, S.] Stockholm Univ, Dept Phys, AlbaNova, SE-10691 Stockholm, Sweden. [Larsson, S.; Li, L.] Oskar Klein Ctr Cosmoparticle Phys, AlbaNova, SE-10691 Stockholm, Sweden. [Larsson, S.] Stockholm Univ, Dept Astron, SE-10691 Stockholm, Sweden. [Lashner, J.] Wesleyan Univ, Middletown, CT 06459 USA. [Li, J.; Torres, D. F.] CSIC, Inst Space Sci, IEEC, E-08193 Barcelona, Spain. [Li, L.] KTH Royal Inst Technol, Dept Phys, AlbaNova, SE-10691 Stockholm, Sweden. [McEnery, J. E.; Troja, E.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [McEnery, J. E.; Troja, E.] Univ Maryland, Dept Astron, College Pk, MD 20742 USA. [Mizuno, T.; Ohsugi, T.] Hiroshima Univ, Hiroshima Astrophys Sci Ctr, Higashihiroshima, Hiroshima 7398526, Japan. [Morselli, A.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, I-00133 Rome, Italy. [Murase, K.] Inst Adv Study, Princeton, NJ 08540 USA. [Murase, K.] Penn State Univ, Dept Astron & Astrophys, Dept Phys, Ctr Particle & Gravitat Astrophys, University Pk, PA 16802 USA. [Nugent, P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Nugent, P.] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Ofek, E.] Weizmann Inst Sci, Benoziyo Ctr Astrophys, IL-76100 Rehovot, Israel. [Ormes, J. F.] Univ Denver, Dept Phys & Astron, Denver, CO 80208 USA. [Paneque, D.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Reimer, A.; Reimer, O.; Werner, M.] Leopold Franzens Univ Innsbruck, Inst Astro & Teilchenphys, A-6020 Innsbruck, Austria. [Reimer, A.; Reimer, O.; Werner, M.] Leopold Franzens Univ Innsbruck, Inst Theoret Phys, A-6020 Innsbruck, Austria. [Siskind, E. J.] NYCB Real Time Comp Inc, Lattingtown, NY 11560 USA. [Suson, D. J.] Purdue Univ Calumet, Dept Chem & Phys, Hammond, IN 46323 USA. [Takahashi, H.] Hiroshima Univ, Dept Phys Sci, Higashihiroshima, Hiroshima 7398526, Japan. [Torres, D. F.] Inst Catalana Recerca & Estudis Avancats ICREA, Barcelona, Spain. [Gal-Yam, A.; Guiriec, S.] Weizmann Inst Sci, Dept Particle Phys & Astrophys, IL-76100 Rehovot, Israel. [Arcavi, I.; Hill, A. B.] Las Cumbres Observ Global Telescope Network, Goleta, CA 93117 USA. [Arcavi, I.; Razzano, M.] Univ Calif Santa Barbara, Kavli Inst Theoret Phys, Santa Barbara, CA 93106 USA. RP Ackermann, M (reprint author), Deutsch Elektronen Synchrotron DESY, D-15738 Zeuthen, Germany. EM afrancko@slac.stanford.edu RI Morselli, Aldo/G-6769-2011; Sgro, Carmelo/K-3395-2016; Reimer, Olaf/A-3117-2013; Bissaldi, Elisabetta/K-7911-2016; Funk, Stefan/B-7629-2015; Johannesson, Gudlaugur/O-8741-2015; Torres, Diego/O-9422-2016; Orlando, E/R-5594-2016; Bonino, Raffaella/S-2367-2016; Loparco, Francesco/O-8847-2015; Mazziotta, Mario /O-8867-2015; Gargano, Fabio/O-8934-2015; giglietto, nicola/I-8951-2012; Di Venere, Leonardo/C-7619-2017 OI Gasparrini, Dario/0000-0002-5064-9495; Baldini, Luca/0000-0002-9785-7726; Murase, Kohta/0000-0002-5358-5642; Larsson, Stefan/0000-0003-0716-107X; Giordano, Francesco/0000-0002-8651-2394; Caraveo, Patrizia/0000-0003-2478-8018; Sgro', Carmelo/0000-0001-5676-6214; SPINELLI, Paolo/0000-0001-6688-8864; Hill, Adam/0000-0003-3470-4834; Pesce-Rollins, Melissa/0000-0003-1790-8018; orienti, monica/0000-0003-4470-7094; Giroletti, Marcello/0000-0002-8657-8852; Bonino, Raffaella/0000-0002-4264-1215; Morselli, Aldo/0000-0002-7704-9553; Reimer, Olaf/0000-0001-6953-1385; Bissaldi, Elisabetta/0000-0001-9935-8106; Funk, Stefan/0000-0002-2012-0080; Johannesson, Gudlaugur/0000-0003-1458-7036; Torres, Diego/0000-0002-1522-9065; Loparco, Francesco/0000-0002-1173-5673; Mazziotta, Mario /0000-0001-9325-4672; Gargano, Fabio/0000-0002-5055-6395; giglietto, nicola/0000-0002-9021-2888; Di Venere, Leonardo/0000-0003-0703-824X FU W.M. Keck Foundation; Willner Family Leadership Institute Ilan Gluzman (Secaucus NJ); Israeli Ministry of Science; Israel Science Foundation; Minerva; I-CORE Program of the Planning and Budgeting Committee; EU/FP7 via ERC grant [307260]; Quantum Universe I-Core program by the Israeli Committee for Planning and Budgeting; ISF; WIS-UK "Making Connections"; Kimmel award; ARCHES award FX The Fermi-LAT Collaboration acknowledges generous ongoing support from a number of agencies and institutes that have supported both the development and the operation of the LAT as well as scientific data analysis. These include the National Aeronautics and Space Administration and the Department of Energy in the United States, the Commissariat a l'Energie Atomique and the Centre National de la Recherche Scientifique/Institut National de Physique Nucleaire et de Physique des Particules in France, the Agenzia Spaziale Italiana and the Istituto Nazionale di Fisica Nucleare in Italy, the Ministry of Education, Culture, Sports, Science and Technology (MEXT), High Energy Accelerator Research Organization (KEK) and Japan Aerospace Exploration Agency (JAXA) in Japan, and the K.A. Wallenberg Foundation, the Swedish Research Council and the Swedish National Space Board in Sweden. Additional support for science analysis during the operations phase is gratefully acknowledged from the Istituto Nazionale di Astrofisica in Italy and the Centre National d'Etudes Spatiales in France. This paper is based on observations obtained with the Samuel Oschin Telescope as part of the Palomar Transient Factory project, a scientific collaboration between the California Institute of Technology, Columbia University, Las Cumbres Observatory, the Lawrence Berkeley National Laboratory, the National Energy Research Scientific Computing Center, the University of Oxford, and the Weizmann Institute of Science. Some of the data presented herein were obtained at the W.M. Keck Observatory, which is operated as a scientific partnership among the California Institute of Technology, the University of California, and NASA; the Observatory was made possible by the generous financial support of the W.M. Keck Foundation. We are grateful for excellent staff assistance at the Palomar, Lick, and Keck Observatories. E.O.O. is the incumbent of the Arye Dissentshik career development chair and is grateful for support by grants from the Willner Family Leadership Institute Ilan Gluzman (Secaucus NJ), the Israeli Ministry of Science, the Israel Science Foundation, Minerva and the I-CORE Program of the Planning and Budgeting Committee and The Israel Science Foundation. A.G.-Y. is supported by the EU/FP7 via ERC grant No. 307260, the Quantum Universe I-Core program by the Israeli Committee for Planning and Budgeting and the ISF, Minerva and ISF grants, WIS-UK "Making Connections", and Kimmel and ARCHES awards. NR 34 TC 4 Z9 4 U1 0 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 10 PY 2015 VL 807 IS 2 AR 169 DI 10.1088/0004-637X/807/2/169 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO2EB UT WOS:000358967000055 ER PT J AU Keisler, R Hoover, S Harrington, N Henning, JW Ade, PAR Aird, KA Austermann, JE Beall, JA Bender, AN Benson, BA Bleem, LE Carlstrom, JE Chang, CL Chiang, HC Cho, HM Citron, R Crawford, TM Crites, AT de Haan, T Dobbs, MA Everett, W Gallicchio, J Gao, J George, EM Gilbert, A Halverson, NW Hanson, D Hilton, GC Holder, GP Holzapfel, WL Hou, Z Hrubes, JD Huang, N Hubmayr, J Irwin, KD Knox, L Lee, AT Leitch, EM Li, D Luong-Van, D Marrone, DP McMahon, JJ Mehl, J Meyer, SS Mocanu, L Natoli, T Nibarger, JP Novosad, V Padin, S Pryke, C Reichardt, CL Ruhl, JE Saliwanchik, BR Sayre, JT Schaffer, KK Shirokoff, E Smecher, G Stark, AA Story, KT Tucker, C Vanderlinde, K Vieira, JD Wang, G Whitehorn, N Yefremenko, V Zahn, O AF Keisler, R. Hoover, S. Harrington, N. Henning, J. W. Ade, P. A. R. Aird, K. A. Austermann, J. E. Beall, J. A. Bender, A. N. Benson, B. A. Bleem, L. E. Carlstrom, J. E. Chang, C. L. Chiang, H. C. Cho, H-M. Citron, R. Crawford, T. M. Crites, A. T. de Haan, T. Dobbs, M. A. Everett, W. Gallicchio, J. Gao, J. George, E. M. Gilbert, A. Halverson, N. W. Hanson, D. Hilton, G. C. Holder, G. P. Holzapfel, W. L. Hou, Z. Hrubes, J. D. Huang, N. Hubmayr, J. Irwin, K. D. Knox, L. Lee, A. T. Leitch, E. M. Li, D. Luong-Van, D. Marrone, D. P. McMahon, J. J. Mehl, J. Meyer, S. S. Mocanu, L. Natoli, T. Nibarger, J. P. Novosad, V. Padin, S. Pryke, C. Reichardt, C. L. Ruhl, J. E. Saliwanchik, B. R. Sayre, J. T. Schaffer, K. K. Shirokoff, E. Smecher, G. Stark, A. A. Story, K. T. Tucker, C. Vanderlinde, K. Vieira, J. D. Wang, G. Whitehorn, N. Yefremenko, V. Zahn, O. TI MEASUREMENTS OF SUB-DEGREE B-MODE POLARIZATION IN THE COSMIC MICROWAVE BACKGROUND FROM 100 SQUARE DEGREES OF SPTPOL DATA SO ASTROPHYSICAL JOURNAL LA English DT Article DE cosmic background radiation; cosmology: observations ID SOUTH-POLE TELESCOPE; LARGE-SCALE STRUCTURE; CMB POLARIZATION; POWER SPECTRUM; ANISOTROPIES; TEMPERATURE; COMPUTATION; PARAMETERS; PHYSICS; RADIO AB We present a measurement of the B-mode polarization power spectrum (the BB spectrum) from 100 deg(2) of sky observed with SPTpol, a polarization-sensitive receiver currently installed on the South Pole Telescope. The observations used in this work were taken during 2012 and early 2013 and include data in spectral bands centered at 95 and 150 GHz. We report the BB spectrum in five bins in multipole space, spanning the range 300 <= l <= 2300, and for three spectral combinations: 95 GHz x 95 GHz, 95 GHz x 150 GHz, and 150 GHz x 150 GHz. We subtract small (<0.5 sigma in units of statistical uncertainty) biases from these spectra and account for the uncertainty in those biases. The resulting power spectra are inconsistent with zero power but consistent with predictions for the BB spectrum arising from the gravitational lensing of E-mode polarization. If we assume no other source of BB power besides lensed B modes, we determine a preference for lensed B modes of 4.9 sigma. After marginalizing over tensor power and foregrounds, namely, polarized emission from galactic dust and extragalactic sources, this significance is 4.3 sigma. Fitting for a single parameter, A(lens), that multiplies the predicted lensed B-mode spectrum, and marginalizing over tensor power and foregrounds, we find A(lens) = 1.08 +/- 0.26, indicating that our measured spectra are consistent with the signal expected from gravitational lensing. The data presented here provide the best measurement to date of the B-mode power spectrum on these angular scales. C1 [Keisler, R.; Irwin, K. D.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Keisler, R.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, Stanford, CA 94305 USA. [Hoover, S.; Henning, J. W.; Bender, A. N.; Benson, B. A.; Bleem, L. E.; Carlstrom, J. E.; Chang, C. L.; Citron, R.; Crawford, T. M.; Crites, A. T.; Gallicchio, J.; Hou, Z.; Leitch, E. M.; Mehl, J.; Meyer, S. S.; Mocanu, L.; Natoli, T.; Schaffer, K. K.; Shirokoff, E.; Story, K. T.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Hoover, S.; Bleem, L. E.; Carlstrom, J. E.; Natoli, T.; Story, K. T.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Harrington, N.; de Haan, T.; George, E. M.; Holzapfel, W. L.; Huang, N.; Lee, A. T.; Reichardt, C. L.; Whitehorn, N.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Henning, J. W.; Austermann, J. E.; Everett, W.; Halverson, N. W.] Univ Colorado, Dept Astrophys & Planetary Sci, Boulder, CO 80309 USA. [Ade, P. A. R.; Tucker, C.] Cardiff Univ, Sch Phys & Astron, Cardiff CF24 3AA, S Glam, Wales. [Aird, K. A.; Hrubes, J. D.; Luong-Van, D.] Univ Chicago, Chicago, IL 60637 USA. [Austermann, J. E.; Beall, J. A.; Gao, J.; Hilton, G. C.; Hubmayr, J.; Li, D.; Nibarger, J. P.] NIST, Quantum Devices Grp, Boulder, CO 80305 USA. [Bender, A. N.; Dobbs, M. A.; Gilbert, A.; Hanson, D.; Holder, G. P.; Smecher, G.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Bender, A. N.; Bleem, L. E.; Carlstrom, J. E.; Chang, C. L.; Mehl, J.; Wang, G.; Yefremenko, V.] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Benson, B. A.; Carlstrom, J. E.; Chang, C. L.; Crawford, T. M.; Crites, A. T.; Leitch, E. M.; Meyer, S. S.; Mocanu, L.; Shirokoff, E.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Benson, B. A.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Carlstrom, J. E.; Meyer, S. S.; Schaffer, K. K.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Chiang, H. C.] Univ KwaZulu Natal, Sch Math Stat & Comp Sci, Durban, South Africa. [Cho, H-M.; Li, D.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Crites, A. T.; Padin, S.] CALTECH, Pasadena, CA 91125 USA. [Dobbs, M. A.] Canadian Inst Adv Res, CIFAR Program Cosmol & Grav, Toronto, ON M5G 1Z8, Canada. [Halverson, N. W.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Knox, L.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Lee, A. T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Marrone, D. P.] Univ Arizona, Steward Observ, Tucson, AZ 85721 USA. [McMahon, J. J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Ruhl, J. E.; Saliwanchik, B. R.; Sayre, J. T.] Case Western Reserve Univ, Ctr Educ & Res Cosmol & Astrophys, Dept Phys, Cleveland, OH 44106 USA. [Novosad, V.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Pryke, C.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Reichardt, C. L.] Univ Melbourne, Sch Phys, Parkville, Vic 3010, Australia. [Schaffer, K. K.] Sch Art Inst Chicago, Liberal Arts Dept, Chicago, IL 60603 USA. [Smecher, G.] Three Speed Log Inc, Vancouver, BC V6A 2J8, Canada. [Stark, A. A.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Vanderlinde, K.] Univ Toronto, Dunlap Inst Astron & Astrophys, Toronto, ON M5S 3H4, Canada. [Vanderlinde, K.] Univ Toronto, Dept Astron Astrophys, Toronto, ON M5S 3H4, Canada. [Vieira, J. D.] Univ Illinois, Dept Astron, Urbana, IL 61801 USA. [Vieira, J. D.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Zahn, O.] Univ Calif Berkeley, Berkeley Ctr Cosmol Phys, Dept Phys, Berkeley, CA 94720 USA. [Zahn, O.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Keisler, R (reprint author), Stanford Univ, Dept Phys, 382 Via Pueblo Mall, Stanford, CA 94305 USA. EM rkeisler@stanford.edu RI Novosad, V /J-4843-2015; OI Tucker, Carole/0000-0002-1851-3918; CRAWFORD, THOMAS/0000-0001-9000-5013; Aird, Kenneth/0000-0003-1441-9518; Reichardt, Christian/0000-0003-2226-9169; Stark, Antony/0000-0002-2718-9996 FU National Science Foundation [PLR-1248097, AST-1402161]; NSF Physics Frontier Center [PHY-0114422]; Kavli Foundation; Gordon and Betty Moore Foundation through Grant GBMF [947]; Natural Sciences and Engineering Research Council of Canada; Canadian Institute for Advanced Research; Canada Research Chairs program; Fermi Research Alliance, LLC [De-AC02-07CH11359]; U.S. Department of Energy; NSF [AST-0956135]; UChicago Argonne, LLC, Operator of Argonne National Laboratory (Argonne); Argonne, a U.S. Department of Energy Office of Science Laboratory [DE-AC02-06CH11357]; Argonne Center for Nanoscale Materials; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX The South Pole Telescope program is supported by the National Science Foundation through grant PLR-1248097. Partial support is also provided by the NSF Physics Frontier Center grant PHY-0114422 to the Kavli Institute of Cosmological Physics at the University of Chicago, the Kavli Foundation, and the Gordon and Betty Moore Foundation through Grant GBMF#947 to the University of Chicago. The McGill authors acknowledge funding from the Natural Sciences and Engineering Research Council of Canada, Canadian Institute for Advanced Research, and Canada Research Chairs program. J.W.H. is supported by the National Science Foundation under Award No. AST-1402161. B.B. is supported by the Fermi Research Alliance, LLC, under Contract No. De-AC02-07CH11359 with the U.S. Department of Energy. The CU Boulder group acknowledges support from NSF AST-0956135. This work is also supported by the U.S. Department of Energy. Work at Argonne National Lab is supported by UChicago Argonne, LLC, Operator of Argonne National Laboratory (Argonne). Argonne, a U.S. Department of Energy Office of Science Laboratory, is operated under Contract No. DE-AC02-06CH11357. We also acknowledge support from the Argonne Center for Nanoscale Materials. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The data analysis pipeline uses the scientific python stack (Jones et al. 2001; Hunter 2007; van der Walt et al. 2011) and the HDF5 file format (The HDF Group 1997). NR 56 TC 33 Z9 33 U1 1 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 10 PY 2015 VL 807 IS 2 AR 151 DI 10.1088/0004-637X/807/2/151 PG 18 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO2EB UT WOS:000358967000037 ER PT J AU Tagliaferri, G Ghisellini, G Perri, M Hayashida, M Balokovic, M Covino, S Giommi, P Madejski, GM Puccetti, S Sbarrato, T Boggs, SE Chiang, J Christensen, FE Craig, WW Hailey, CJ Harrison, FA Stern, D Zhang, WW AF Tagliaferri, G. Ghisellini, G. Perri, M. Hayashida, M. Balokovic, M. Covino, S. Giommi, P. Madejski, G. M. Puccetti, S. Sbarrato, T. Boggs, S. E. Chiang, J. Christensen, F. E. Craig, W. W. Hailey, C. J. Harrison, F. A. Stern, D. Zhang, W. W. TI NuSTAR AND MULTIFREQUENCY STUDY OF THE TWO HIGH-REDSHIFT BLAZARS S5 0836+710 AND PKS 2149-306 SO ASTROPHYSICAL JOURNAL LA English DT Article DE BL Lacertae objects: individual (PKS 2149-306, S5 0836+710); galaxies: active; galaxies: jets; quasars: general; X-rays: general ID ACTIVE GALACTIC NUCLEI; LARGE-AREA TELESCOPE; RADIO-LOUD QUASARS; BLACK-HOLE; X-RAY; RELATIVISTIC JETS; SIMPLIFIED VIEW; DISTANT BLAZAR; SOURCE CATALOG; FERMI BLAZARS AB Powerful blazars are flat-spectrum radio quasars whose emission is dominated by a Compton component peaking between a few hundred keV and a few hundred MeV. We observed two bright blazars, PKS 2149-306 at redshift z = 2.345 and S5 0836+710 at z = 2.172, in the hard X-ray band with the Nuclear Spectroscopic Telescope Array satellite. Simultaneous soft-X-rays and UV-optical observations were performed with the Swift satellite, while near-infrared (near-IR) data were obtained with the Rapid Eye Mount telescope. To study their variability, we repeated these observations for both sources on a timescale of a few months. While no fast variability was detected during a single observation, both sources were variable in the X-ray band, up to 50%, between the two observations, with larger variability at higher energies. No variability was detected in the optical/NIR band. These data, together with Fermi-Large Area Telescope, Wide-field Infrared Survey Explorer, and other literature data, are then used to study the overall spectral energy distributions (SEDs) of these blazars. Although the jet nonthermal emission dominates the SED, it leaves the UV band unhidden, allowing us to detect the thermal emission of the disk. and to estimate the black hole mass. The nonthermal emission is well reproduced by a one-zone leptonic model by the synchrotron, self-Compton, and external Compton processes. Our data are better reproduced if we assume that the location of the dissipation region of the jet, R-diss, is in. between the torus and the broad-line region. The observed variability is explained by changing a minimum number of model parameters by a very small amount. C1 [Tagliaferri, G.; Ghisellini, G.; Covino, S.; Sbarrato, T.] INAF Osservatorio Astron Brera, I-23807 Merate, Italy. [Perri, M.; Giommi, P.; Puccetti, S.] ASI Sci Data Ctr, I-00133 Rome, Italy. [Perri, M.; Puccetti, S.] INAF Osservatorio Astron Roma, I-00040 Monte Porzio Catone, Italy. [Hayashida, M.] Univ Tokyo, Inst Cosm Ray Res, Kashiwa, Chiba 2778582, Japan. [Balokovic, M.; Harrison, F. A.] CALTECH, Cahill Ctr Astrophys, Pasadena, CA 91125 USA. [Madejski, G. M.; Chiang, J.] SLAC Natl Accelerator Lab, Kavli Inst Particle Astrophys & Cosmol, Menlo Pk, CA 94025 USA. [Sbarrato, T.] Univ Milano Bicocca, Dipartimento Fis G Occhialini, I-20126 Milan, Italy. [Boggs, S. E.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Christensen, F. E.; Craig, W. W.] Tech Univ Denmark, DTU Space Natl Space Inst, DK-2800 Lyngby, Denmark. [Craig, W. W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Hailey, C. J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Stern, D.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Zhang, W. W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Tagliaferri, G (reprint author), INAF Osservatorio Astron Brera, Via E Bianchi 46, I-23807 Merate, Italy. EM gianpiero.tagliaferri@brera.inaf.it RI Boggs, Steven/E-4170-2015; OI Puccetti, Simonetta/0000-0002-2734-7835; Sbarrato, Tullia/0000-0002-3069-9399; Covino, Stefano/0000-0001-9078-5507; Tagliaferri, Gianpiero/0000-0003-0121-0723; Boggs, Steven/0000-0001-9567-4224; giommi, paolo/0000-0002-2265-5003; Perri, Matteo/0000-0003-3613-4409; Ghisellini, Gabriele/0000-0002-0037-1974 FU ASI-INAF grant [I/037/12/0]; NASA [NNG08FD60C] FX We acknowledge financial support from the ASI-INAF grant I/037/12/0. This work was supported under NASA Contract No. NNG08FD60C and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by NASA. We thank the NuSTAR Operations, Software and Calibration teams for support with the execution and analysis of these observations. We also thank the Swift team for quickly approving and executing the requested ToO observations. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (Caltech, USA). The Fermi-LAT Collaboration acknowledges generous ongoing support from a number of agencies and institutes that have supported both the development and the operation of the LAT, as well as scientific data analysis. These include the National Aeronautics and Space Administration and the Department of Energy in the United States; the Commissariat a l'Energie Atomique and the Centre National de la Recherche Scientifique/Institut National de Physique Nucleaire et de Physique des Particules in France; the Agenzia Spaziale Italiana and the Istituto Nazionale di Fisica Nucleare in Italy; the Ministry of Education, Culture, Sports, Science and Technology (MEXT), High Energy Accelerator Research Organization (KEK), and Japan Aerospace Exploration Agency (JAXA) in Japan; and the K. A. Wallenberg Foundation, the Swedish Research Council, and the Swedish National Space Board in Sweden. Additional support for science analysis during the operations phase is gratefully acknowledged from the Istituto Nazionale di Astrofisica in Italy and the Centre National d'Etudes Spatiales in France. Part of this work is based on archival data, software, or online services provided by the ASI Data Center (ASDC). NR 72 TC 6 Z9 6 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 10 PY 2015 VL 807 IS 2 AR 167 DI 10.1088/0004-637X/807/2/167 PG 9 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CO2EB UT WOS:000358967000053 ER PT J AU Lentz, EJ Bruenn, SW Hix, WR Mezzacappa, A Messer, OEB Endeve, E Blondin, JM Harris, JA Marronetti, P Yakunin, KN AF Lentz, Eric J. Bruenn, Stephen W. Hix, W. Raphael Mezzacappa, Anthony Messer, O. E. Bronson Endeve, Eirik Blondin, John M. Harris, J. Austin Marronetti, Pedro Yakunin, Konstantin N. TI THREE-DIMENSIONAL CORE-COLLAPSE SUPERNOVA SIMULATED USING A 15 M-circle dot PROGENITOR SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE neutrinos; stars: evolution; stars: massive; supernovae: general ID NEUTRINO-HYDRODYNAMICS SIMULATIONS; 3 DIMENSIONS; DRIVEN SUPERNOVA; MASSIVE STARS; SASI ACTIVITY; EXPLOSIONS; SHOCK; NUCLEOSYNTHESIS; MECHANISMS; TRANSPORT AB We have performed ab initio neutrino radiation hydrodynamics simulations in three and two spatial dimensions (3D and 2D) of core-collapse supernovae from the same 15 M-circle dot progenitor through 440 ms after core bounce. Both 3D and 2D models achieve explosions; however, the onset of explosion (shock revival) is delayed by similar to 100 ms in 3D relative to the 2D counterpart and the growth of the diagnostic explosion energy is slower. This is consistent with previously reported 3D simulations utilizing iron-core progenitors with dense mantles. In the similar to 100 ms before the onset of explosion, diagnostics of neutrino heating and turbulent kinetic energy favor earlier explosion in 2D. During the delay, the angular scale of convective plumes reaching the shock surface grows and explosion in 3D is ultimately lead by a single, large-angle plume, giving the expanding shock a directional orientation not dissimilar from those imposed by axial symmetry in 2D simulations. We posit that shock revival and explosion in the 3D simulation may be delayed until sufficiently large plumes form, whereas such plumes form more rapidly in 2D, permitting earlier explosions. C1 [Lentz, Eric J.; Hix, W. Raphael; Mezzacappa, Anthony; Messer, O. E. Bronson; Endeve, Eirik; Harris, J. Austin; Yakunin, Konstantin N.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Lentz, Eric J.; Hix, W. Raphael; Messer, O. E. Bronson; Yakunin, Konstantin N.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Bruenn, Stephen W.] Florida Atlantic Univ, Dept Phys, Boca Raton, FL 33431 USA. [Mezzacappa, Anthony; Endeve, Eirik; Yakunin, Konstantin N.] Oak Ridge Natl Lab, Joint Inst Computat Sci, Oak Ridge, TN 37831 USA. [Messer, O. E. Bronson] Oak Ridge Natl Lab, Natl Ctr Computat Sci, Oak Ridge, TN 37831 USA. [Endeve, Eirik] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Blondin, John M.] N Carolina State Univ, Dept Phys, Raleigh, NC 27695 USA. [Marronetti, Pedro] Natl Sci Fdn, Div Phys, Arlington, VA 22207 USA. RP Lentz, EJ (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. EM elentz@utk.edu RI Lentz, Eric/M-7173-2015; Hix, William/E-7896-2011; Messer, Bronson/G-1848-2012; Mezzacappa, Anthony/B-3163-2017 OI Endeve, Eirik/0000-0003-1251-9507; Lentz, Eric/0000-0002-5231-0532; Hix, William/0000-0002-9481-9126; Messer, Bronson/0000-0002-5358-5415; Mezzacappa, Anthony/0000-0001-9816-9741 FU U.S. Department of Energy Offices of Nuclear Physics and Advanced Scientific Computing Research; NASA Astrophysics Theory Program [NNH11AQ72I]; National Science Foundation PetaApps Program [OCI-0749242, OCI-0749204,, OCI-0749248]; National Science Foundation through its employee IR/D program; Innovative and Novel Computational Impact on Theory and Experiment (INCITE) program at the Oak Ridge Leadership Computing Facility (OLCF); Innovative and Novel Computational Impact on Theory and Experiment (INCITE) program at the Argonne Leadership Computing Facility; DOE Office of Science User Facilities [DE-AC05-00OR22725, DE-AC02-06CH11357] FX This research was supported by the U.S. Department of Energy Offices of Nuclear Physics and Advanced Scientific Computing Research; the NASA Astrophysics Theory Program (grant NNH11AQ72I); and the National Science Foundation PetaApps Program (grants OCI-0749242, OCI-0749204, and OCI-0749248). P.M. is supported by the National Science Foundation through its employee IR/D program. The opinions and conclusions expressed herein are those of the authors and do not represent the National Science Foundation. This research was also supported by an award of computer time provided by the Innovative and Novel Computational Impact on Theory and Experiment (INCITE) program at the Oak Ridge Leadership Computing Facility (OLCF) and at the Argonne Leadership Computing Facility, which are DOE Office of Science User Facilities supported under contracts DE-AC05-00OR22725 and DE-AC02-06CH11357, respectively. Animation by Mike Matheson at OLCF. NR 38 TC 26 Z9 26 U1 1 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD JUL 10 PY 2015 VL 807 IS 2 AR L31 DI 10.1088/2041-8205/807/2/L31 PG 8 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CM8HC UT WOS:000357938600011 ER PT J AU Lupoi, JS Smith-Moritz, A Singh, S McQualter, R Scheller, HV Simmons, BA Henry, RJ AF Lupoi, Jason S. Smith-Moritz, Andreia Singh, Seema McQualter, Richard Scheller, Henrik V. Simmons, Blake A. Henry, Robert J. TI Localization of polyhydroxybutyrate in sugarcane using Fourier-transform infrared microspectroscopy and multivariate imaging SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Infrared imaging; Focal plane array; Polyhydroxybutyrate; Sugarcane; Multivariate imaging ID FT-IR MICROSPECTROSCOPY; CELL-WALL POLYSACCHARIDES; MARINE-ENVIRONMENT; SPECTROSCOPY; POLY(3-HYDROXYBUTYRATE); PYROLYSIS; CHEMICALS; POLYMERS; SPECTRA; BIOMASS AB Background: Slow-degrading, fossil fuel-derived plastics can have deleterious effects on the environment, especially marine ecosystems. The production of bio-based, biodegradable plastics from or in plants can assist in supplanting those manufactured using fossil fuels. Polyhydroxybutyrate (PHB) is one such biodegradable polyester that has been evaluated as a possible candidate for relinquishing the use of environmentally harmful plastics. Results: PHB, possessing similar properties to polyesters produced from non-renewable sources, has been previously engineered in sugarcane, thereby creating a high-value co-product in addition to the high biomass yield. This manuscript illustrates the coupling of a Fourier-transform infrared microspectrometer, equipped with a focal plane array (FPA) detector, with multivariate imaging to successfully identify and localize PHB aggregates. Principal component analysis imaging facilitated the mining of the abundant quantity of spectral data acquired using the FPA for distinct PHB vibrational modes. PHB was measured in the chloroplasts of mesophyll and bundle sheath cells, acquiescent with previously evaluated plant samples. Conclusion: This study demonstrates the power of IR microspectroscopy to rapidly image plant sections to provide a snapshot of the chemical composition of the cell. While PHB was localized in sugarcane, this method is readily transferable to other value-added co-products in different plants. C1 [Lupoi, Jason S.; Simmons, Blake A.; Henry, Robert J.] Univ Queensland, Queensland Alliance Agr & Food Innovat, St Lucia, Qld 4072, Australia. [Lupoi, Jason S.; Smith-Moritz, Andreia; Singh, Seema; Scheller, Henrik V.; Simmons, Blake A.] Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, Emeryville, CA 94608 USA. [Singh, Seema; Simmons, Blake A.] Sandia Natl Labs, Biol & Engn Sci Ctr, Livermore, CA 94551 USA. Univ Queensland, Australian Inst Bioengn & Nanotechnol, St Lucia, Qld 4072, Australia. Univ N Texas, Dept Biol Sci, Denton, TX 76203 USA. [Lupoi, Jason S.] Sage Analyt, Boulder, CO 80301 USA. RP Lupoi, JS (reprint author), Univ Queensland, Queensland Alliance Agr & Food Innovat, St Lucia, Qld 4072, Australia. EM jslupoi@lbl.gov RI Henry, Robert/B-5824-2008; Scheller, Henrik/A-8106-2008; OI Henry, Robert/0000-0002-4060-0292; Scheller, Henrik/0000-0002-6702-3560; McQualter, Richard/0000-0003-3703-1356 FU University of Queensland; Joint BioEnergy Institute; Office of Science, Office of Biological and Environmental Research of the US Department of Energy [DE-AC02-05CH11231] FX This manuscript was supported as part of collaboration between the University of Queensland and the Joint BioEnergy Institute. The work conducted by the Joint BioEnergy Institute was supported by the Office of Science, Office of Biological and Environmental Research of the US Department of Energy under contract no. DE-AC02-05CH11231. The authors would like to thank Steve Ruzin and Denise Schichnes, at the CNR Biological Imaging Facility at the University of California-Berkeley, for the assistance with and use of the Leica cryotome, and Shunlin Wang of Bruker Optics, Inc., Fremont, CA, for providing guidance related to the Bruker FTIR Tensor instrument. NR 46 TC 0 Z9 0 U1 5 U2 11 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD JUL 10 PY 2015 VL 8 AR 98 DI 10.1186/s13068-015-0279-y PG 9 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA CN0OZ UT WOS:000358114500001 PM 26199643 ER PT J AU Punjabi, V Perdrisat, CF Jones, MK Brash, EJ Carlson, CE AF Punjabi, V. Perdrisat, C. F. Jones, M. K. Brash, E. J. Carlson, C. E. TI The structure of the nucleon: Elastic electromagnetic form factors SO EUROPEAN PHYSICAL JOURNAL A LA English DT Review ID ELECTRON-PROTON SCATTERING; GENERALIZED PARTON DISTRIBUTIONS; CONSTITUENT-QUARK-MODEL; FUNDAMENTAL PHYSICAL CONSTANTS; CODATA RECOMMENDED VALUES; SQUARED 4-MOMENTUM TRANSFERS; HIGH MOMENTUM-TRANSFERS; POLARIZED ELECTRONS; DEUTERON SCATTERING; CROSS-SECTIONS AB Precise proton and neutron form factor measurements at Jefferson Lab, using spin observables, have recently made a significant contribution to the unraveling of the internal structure of the nucleon. Accurate experimental measurements of the nucleon form factors are a test-bed for understanding how the nucleon's static properties and dynamical behavior emerge from QCD, the theory of the strong interactions between quarks. There has been enormous theoretical progress, since the publication of the Jefferson Lab proton form factor ratio data, aiming at reevaluating the picture of the nucleon. We will review the experimental and theoretical developments in this field and discuss the outlook for the future. C1 [Punjabi, V.] Norfolk State Univ, Norfolk, VA 23504 USA. [Perdrisat, C. F.; Carlson, C. E.] Coll William & Mary, Williamsburg, VA 23187 USA. [Jones, M. K.; Brash, E. J.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Brash, E. J.] Christopher Newport Univ, Newport News, VA 23606 USA. RP Punjabi, V (reprint author), Norfolk State Univ, Norfolk, VA 23504 USA. EM punjabi@jlab.org FU U.S. Department of Energy [DE-FG02-89ER40525]; DOE [DE-AC05-06OR23177]; National Science Foundation (USA) [PHY-1208056, PHY-1205905, PHY-1066374] FX We would like to thank Dr. C. Ayerbe Gayoso for useful discussions and critical reading of the manuscript. This work was supported by U.S. Department of Energy grant DE-FG02-89ER40525 (VP) and by DOE contract DE-AC05-06OR23177, under which Jefferson Science Associates, LLC, operates the Thomas Jefferson National Accelerator Facility (MKJ), and by National Science Foundation (USA) grants PHY-1208056 (EJB), PHY-1205905 (CEC), and PHY-1066374 (CFP). NR 327 TC 11 Z9 12 U1 0 U2 5 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6001 EI 1434-601X J9 EUR PHYS J A JI Eur. Phys. J. A PD JUL 10 PY 2015 VL 51 IS 7 AR 79 DI 10.1140/epja/i2015-15079-x PG 44 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA CM6WQ UT WOS:000357832500001 ER PT J AU Adam, J Adamova, D Aggarwal, MM Rinella, GA Agnello, M Agrawal, N Ahammed, Z Ahn, SU Aimo, I Aiola, S Ajaz, M Akindinov, A Alam, SN Aleksandrov, D Alessandro, B Alexandre, D Molina, RA Alici, A Alkin, A Alme, J Alt, T Altinpinar, S Altsybeev, I Prado, CAG Andrei, C Andronic, A Anguelov, V Anielski, J Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshaser, H Arcelli, S Armesto, N Arnaldi, R Arsene, IC Arslandok, M Audurier, B Augustinus, A Averbeck, R Azmi, MD Bach, M Badala, A Baek, YW Bagnasco, S Bailhache, R Bala, R Baldisseri, A Pedrosa, FBD Baral, RC Barbano, AM Barbera, R Barile, F Barnafodi, GG Barnby, LS Barret, V Bartalini, P Barth, K Bartke, J Bartsch, E Basile, M Bastid, N Basu, S Bathen, B Batigne, G Camejo, AB Batyunya, B Batzing, PC Bearden, IG Beck, H Bedda, C Behera, NK Belikov, I Bellini, F 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CA ALICE Collaboration TI Inclusive, prompt and non-prompt J/psi production at mid-rapidity in Pb-Pb collisions at root S-NN=2.76 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID HEAVY-ION COLLISIONS; TRANSVERSE-MOMENTUM DEPENDENCE; PROTON-PROTON COLLISIONS; ENERGY-LOSS; ROOT-S=7 TEV; PP COLLISIONS; JET TOMOGRAPHY; AA COLLISIONS; MONTE-CARLO; QCD MATTER AB The transverse momentum (p(T)) dependence of the nuclear modification factor R-AA and the centrality dependence of the average transverse momentum for inclusive J/psi have been measured with ALICE for Pb-Pb collisions at root S-NN = 2.76TeV in the e(+)e(-) decay channel at mid-rapidity (vertical bar y vertical bar < 0.8). The is significantly smaller than the one observed for pp collisions at the same centre-of-mass energy. Consistently, an increase of RAA is observed towards low p(T). These observations might be indicative of a sizable contribution of charm quark coalescence to the J/psi production. Additionally, the fraction of non-prompt J/psi from beauty hadron decays, f(B), has been determined in the region 1.5 < p(T) < 10 GeV/c in three centrality intervals. No significant centrality dependence of fB is observed. Finally, the RAA of non-prompt J/psi is discussed and compared with model predictions. The nuclear modification in the region 4.5 < p(T) < 10 GeV/c is found to be stronger than predicted by most models. C1 [Takaki, J. D. Tapia] Univ Kansas, Lawrence, KS 66045 USA. [Grigoryan, A.; Gulkanyan, H.; Papikyan, V.] Yerevan Phys Inst, AI Alikhanyan Natl Sci Lab, Yerevan 375036, Armenia. [Bello Martinez, H.; Cortes Maldonado, I.; Fernandez Tellez, A.; Martinez, M. I.; Rodriguez Cahuantzi, M.; Tejeda Munoz, G.; Vargas, A.; Limon, S. Vergara] Benemerita Univ Autonoma Puebla, Puebla, Mexico. 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S.; Norman, J.; Romita, R.] Univ Liverpool, Liverpool L69 3BX, Merseyside, England. [Castro, A. J.; Mazer, J.; Nattrass, C.; Read, K. F.; Scott, R.; Sharma, N.; Sorensen, S.] Univ Tennessee, Knoxville, TN USA. [Vilakazi, Z.] Univ Witwatersrand, Johannesburg, South Africa. [Gunji, T.; Hamagaki, H.; Hayashi, S.; Sekiguchi, Y.; Terasaki, K.; Tsuji, T.; Watanabe, Y.] Univ Tokyo, Tokyo, Japan. [Bhom, J.; Busch, O.; Chujo, T.; Esumi, S.; Inaba, M.; Kobayashi, T.; Masui, H.; Miake, Y.; Sano, M.; Tanaka, N.; Watanabe, D.; Yokoyama, H.] Univ Tsukuba, Tsukuba, Ibaraki, Japan. [Erhardt, F.; Planinic, M.; Poljak, N.; Simatovic, G.; Utrobicic, A.] Univ Zagreb, Zagreb 41000, Croatia. [Cheshkov, C.; Cheynis, B.; Ducroux, L.; Grossiord, J. -Y.; Teyssier, B.; Tieulent, R.; Uras, A.] Univ Lyon 1, CNRS, IN2P3, IPN Lyon, F-69622 Villeurbanne, France. [Altsybeev, I.; Feofilov, G.; Kolojvari, A.; Kondratiev, V.; Kovalenko, V.; Vechernin, V.; Vinogradov, L.; Zarochentsev, A.] St Petersburg State Univ, V Fock Inst Phys, St Petersburg 199034, Russia. [Ahammed, Z.; Alam, S. N.; Basu, S.; Chattopadhyay, S.; Choudhury, S.; Dubey, A. K.; Ghosh, P.; Kar, S.; Khan, S. A.; Mitra, J.; Mohanty, B.; Muhuri, S.; Mukherjee, M.; Nayak, T. K.; Pal, S. K.; Saini, J.; Sarkar, D.; Singaraju, R.; Singh, R.; Singha, S.; Singhal, V.; Viyogi, Y. P.] Ctr Variable Energy Cyclotron, Kolkata, India. [Milosevic, J.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Graczykowski, L. K.; Janik, M. A.; Kisiel, A.; Oleniacz, J.; Pluta, J.; Szymanski, M.; Zaborowska, A.; Zbroszczyk, H.] Warsaw Univ Technol, Warsaw, Poland. [Belmont, R.; Bianchin, C.; Loggins, V. R.; Pan, J.; Pruneau, C. A.; Pujahari, P.; Putschke, J.; Reed, R. J.; Saleh, M. A.; Verweij, M.; Yaldo, C. G.] Wayne State Univ, Detroit, MI USA. [Barnafoeldi, G. 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RI Martinez Hernandez, Mario Ivan/F-4083-2010; Ferretti, Alessandro/F-4856-2013; Vickovic, Linda/F-3517-2017; Fernandez Tellez, Arturo/E-9700-2017; Naru, Muhammad Umair/N-5547-2015; Graczykowski, Lukasz/O-7522-2015; Janik, Malgorzata/O-7520-2015; Pshenichnov, Igor/A-4063-2008; Sevcenco, Adrian/C-1832-2012; Barnby, Lee/G-2135-2010; feofilov, grigory/A-2549-2013; Kucera, Vit/G-8459-2014; Krizek, Filip/G-8967-2014; Bielcikova, Jana/G-9342-2014; Vajzer, Michal/G-8469-2014; Ferencei, Jozef/H-1308-2014; Natal da Luz, Hugo/F-6460-2013; Bregant, Marco/I-7663-2012; Karasu Uysal, Ayben/K-3981-2015; HAMAGAKI, HIDEKI/G-4899-2014; Guber, Fedor/I-4271-2013; Kovalenko, Vladimir/C-5709-2013; Zarochentsev, Andrey/J-6253-2013; Altsybeev, Igor/K-6687-2013; Vinogradov, Leonid/K-3047-2013; Kondratiev, Valery/J-8574-2013; Vechernin, Vladimir/J-5832-2013; Nattrass, Christine/J-6752-2016; Usai, Gianluca/E-9604-2015; Cosentino, Mauro/L-2418-2014; Suaide, Alexandre/L-6239-2016; Peitzmann, Thomas/K-2206-2012; Fachbereich14, Dekanat/C-8553-2015; Castillo Castellanos, Javier/G-8915-2013; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ferreiro, Elena/C-3797-2017; Armesto, Nestor/C-4341-2017; Sumbera, Michal/O-7497-2014; Adamova, Dagmar/G-9789-2014; Christensen, Christian/D-6461-2012; De Pasquale, Salvatore/B-9165-2008; Chinellato, David/D-3092-2012; Felea, Daniel/C-1885-2012; de Cuveland, Jan/H-6454-2016; Kurepin, Alexey/H-4852-2013; Jena, Deepika/P-2873-2015; Jena, Satyajit/P-2409-2015; Akindinov, Alexander/J-2674-2016; Takahashi, Jun/B-2946-2012 OI Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Ferretti, Alessandro/0000-0001-9084-5784; Vickovic, Linda/0000-0002-9820-7960; Fernandez Tellez, Arturo/0000-0003-0152-4220; Naru, Muhammad Umair/0000-0001-6489-0784; Janik, Malgorzata/0000-0002-3356-3438; Pshenichnov, Igor/0000-0003-1752-4524; Sevcenco, Adrian/0000-0002-4151-1056; Barnby, Lee/0000-0001-7357-9904; feofilov, grigory/0000-0003-3700-8623; Natal da Luz, Hugo/0000-0003-1177-870X; Karasu Uysal, Ayben/0000-0001-6297-2532; Guber, Fedor/0000-0001-8790-3218; Kovalenko, Vladimir/0000-0001-6012-6615; Zarochentsev, Andrey/0000-0002-3502-8084; Altsybeev, Igor/0000-0002-8079-7026; Vinogradov, Leonid/0000-0001-9247-6230; Kondratiev, Valery/0000-0002-0031-0741; Vechernin, Vladimir/0000-0003-1458-8055; Nattrass, Christine/0000-0002-8768-6468; Usai, Gianluca/0000-0002-8659-8378; Cosentino, Mauro/0000-0002-7880-8611; Suaide, Alexandre/0000-0003-2847-6556; Peitzmann, Thomas/0000-0002-7116-899X; Castillo Castellanos, Javier/0000-0002-5187-2779; Ferreiro, Elena/0000-0002-4449-2356; Armesto, Nestor/0000-0003-0940-0783; Sumbera, Michal/0000-0002-0639-7323; Christensen, Christian/0000-0002-1850-0121; De Pasquale, Salvatore/0000-0001-9236-0748; Chinellato, David/0000-0002-9982-9577; Felea, Daniel/0000-0002-3734-9439; de Cuveland, Jan/0000-0003-0455-1398; Kurepin, Alexey/0000-0002-1851-4136; Jena, Deepika/0000-0003-2112-0311; Jena, Satyajit/0000-0002-6220-6982; Akindinov, Alexander/0000-0002-7388-3022; Takahashi, Jun/0000-0002-4091-1779 FU Worldwide LHC Computing Grid (WLCG); Grid centres; State Committee of Science; World Federation of Scientists (WFS); Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under European Community's Seventh Framework Programme; Helsinki Institute of Physics; Academy of Finland; French CNRS-IN2P3, France; Region Pays de Loire, France; Region Alsace, France; Region Auvergne, France; CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung und Technologie (BMBF); Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian Orszagos Tudomanyos Kutatasi Alappgrammok (OTKA); National Office for Research and Technology (NKTH); Department of Atomic Energy; Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN), Italy; Centro Fermi - Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT), Mexico; Direccion General de Asuntos del Personal Academico(DGAPA), Mexico; Amerique Latine Formation academique - European Commission(ALFA-EC); EPLANET Program (European Particle Physics Latin American Network) Stichting voor Fundamenteel Onderzoek der Materie (FOM); Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics; Consiliul National al Cercetarii Stiintifice - Executive Agency for Higher Education Research Development and Innovation Funding (CNCS-UEFISCDI) - Romania; Ministry of Education and Science of Russian Federation; Russian Academy of Sciences; Russian Federal Agency of Atomic Energy; Russian Federal Agency for Science and Innovations; Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT); E-Infrastructure shared between Europe and Latin America (EELA); Ministerio de Economia y Competitividad (MINECO) of Spain; Xunta de Galicia (Conselleria de Educacion); Centro de Aplicaciones Tecnologicas y Desarrollo Nuclear (CEADEN), Cuba; Cubaenergia, Cuba; IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); United States Department of Energy; United States National Science Foundation; State of Texas; State of Ohio; Ministry of Science, Education and Sports of Croatia; Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India FX The ALICE Collaboration would like to thank all its engineers and technicians for their invaluable contributions to the construction of the experiment and the CERN accelerator teams for the outstanding performance of the LHC complex. The ALICE Collaboration gratefully acknowledges the resources and support provided by all Grid centres and the Worldwide LHC Computing Grid (WLCG) collaboration.; The ALICE Collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector: State Committee of Science, World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia, Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE) and the Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council, the Carlsberg Foundation and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics and the Academy of Finland; French CNRS-IN2P3, the 'Region Pays de Loire', 'Region Alsace', 'Region Auvergne' and CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung und Technologie (BMBF) and the Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian Orszagos Tudomanyos Kutatasi Alappgrammok (OTKA) and National Office for Research and Technology (NKTH); Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi - Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; MEXT Grant-in-Aid for Specially Promoted Research, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT), Direccion General de Asuntos del Personal Academico(DGAPA), Mexico, Amerique Latine Formation academique - European Commission(ALFA-EC) and the EPLANET Program (European Particle Physics Latin American Network) Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics and Consiliul National al Cercetarii Stiintifice - Executive Agency for Higher Education Research Development and Innovation Funding (CNCS-UEFISCDI) - Romania; Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations and The Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT), E-Infrastructure shared between Europe and Latin America (EELA), Ministerio de Economia y Competitividad (MINECO) of Spain, Xunta de Galicia (Conselleria de Educacion), Centro de Aplicaciones Tecnologicas y Desarrollo Nuclear (CEADEN), Cubaenergia, Cuba, and IAEA (International Atomic Energy Agency); Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); The United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio; Ministry of Science, Education and Sports of Croatia and Unity through Knowledge Fund, Croatia. Council of Scientific and Industrial Research (CSIR), New Delhi, India NR 87 TC 8 Z9 8 U1 3 U2 57 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JUL 10 PY 2015 IS 7 AR 051 DI 10.1007/JHEP07(2015)051 PG 33 WC Physics, Particles & Fields SC Physics GA CM8ES UT WOS:000357931400001 ER PT J AU Adamczyk, L Adkins, JK Agakishiev, G Aggarwal, MM Ahammed, Z Alekseev, I Alford, J Anson, CD Aparin, A Arkhipkin, D Aschenauer, EC Averichev, GS Banerjee, A Beavis, DR Bellwied, R Bhasin, A Bhati, AK Bhattarai, P Bichsel, H Bielcik, J Bielcikova, J Bland, LC Bordyuzhin, IG Borowski, W Bouchet, J Brandin, AV Brovko, SG Bultmann, S Bunzarov, I Burton, TP Butterworth, J Caines, H Sanchez, MCD Cebra, D Cendejas, R Cervantes, MC Chaloupka, P Chang, Z Chattopadhyay, S Chen, HF Chen, JH Chen, L Cheng, J Cherney, M Chikanian, A Christie, W Chwastowski, J Codrington, MJM Contin, G Cramer, JG Crawford, HJ Cui, X Das, S Leyva, AD De Silva, LC Debbe, RR Dedovich, TG Deng, J Derevschikov, AA de Souza, RD Dhamija, S di Ruzza, B Didenko, L Dilks, C Ding, F Djawotho, P Dong, X Drachenberg, JL Draper, JE Du, CM Dunkelberger, LE Dunlop, JC Efimov, LG Engelage, J Engle, KS Eppley, G Eun, L Evdokimov, O Eyser, O Fatemi, R Fazio, S Fedorisin, J Filip, P Finch, E Fisyak, Y Flores, CE Gagliardi, CA Gangadharan, DR Garand, D Geurts, F Gibson, A Girard, M Gliske, S Greiner, L Grosnick, D Gunarathne, DS Guo, Y Gupta, A Gupta, S Guryn, W Haag, B Hamed, A Han, LX Haque, R Harris, JW Heppelmann, S Hirsch, A Hoffmann, GW Hofman, DJ Horvat, S Huang, B Huang, HZ Huang, X Huck, P Humanic, TJ Igo, G Jacobs, WW Jang, H Judd, EG Kabana, S Kalinkin, D Kang, K Kauder, K Ke, HW Keane, D Kechechyan, A Kesich, A Khan, ZH Kikola, DP Kisel, I Kisiel, A Koetke, DD Kollegger, T Konzer, J Koralt, I Kosarzewski, LK Kotchenda, L Kraishan, AF Kravtsov, P Krueger, K Kulakov, I Kumar, L Kycia, RA Lamont, MAC Landgraf, JM Landry, KD Lauret, J Lebedev, A Lednicky, R Lee, JH LeVine, MJ Li, C Li, W Li, X Li, X Li, Y Li, ZM Lisa, MA Liu, F Ljubicic, T Llope, WJ Lomnitz, M Longacre, RS Luo, X Ma, GL Ma, YG Don, DMMDM Mahapatra, DP Majka, R Margetis, S Markert, C Masui, H Matis, HS McDonald, D McShane, TS Minaev, NG Mioduszewski, S Mohanty, B Mondal, MM Morozov, DA Mustafa, MK Nandi, BK Nasim, M Nayak, TK Nelson, JM Nigmatkulov, G Nogach, LV Noh, SY Novak, J Nurushev, SB Odyniec, G Ogawa, A Oh, K Ohlson, A Okorokov, V Oldag, EW Olvitt, DL Pachr, M Page, BS Pal, SK Pan, YX Pandit, Y Panebratsev, Y Pawlak, T Pawlik, B Pei, H Perkins, C Peryt, W Pile, P Planinic, M Pluta, J Poljak, N Poniatowska, K Porter, J Poskanzer, AM Pruthi, NK Przybycien, M Pujahari, PR Putschke, J Qiu, H Quintero, A Ramachandran, S Raniwala, R Raniwala, S Ray, RL Riley, CK Ritter, HG Roberts, JB Rogachevskiy, OV Romero, JL Ross, JF Roy, A Ruan, L Rusnak, J Rusnakova, O Sahoo, NR Sahu, PK Sakrejda, I Salur, S Sandweiss, J Sangaline, E Sarkar, A Schambach, J Scharenberg, RP Schmah, AM Schmidke, WB Schmitz, N Seger, J Seyboth, P Shah, N Shahaliev, E Shanmuganathan, PV Shao, M Sharma, B Shen, WQ Shi, SS Shou, QY Sichtermann, EP Singaraju, RN Skoby, MJ Smirnov, D Smirnov, N Solanki, D Sorensen, P Spinka, HM Srivastava, B Stanislaus, TDS Stevens, JR Stock, R Strikhanov, M Stringfellow, B Sumbera, M Sun, X Sun, XM Sun, Y Sun, Z Surrow, B Svirida, DN Symons, TJM Szelezniak, MA Takahashi, J Tang, AH Tang, Z Tarnowsky, T Thomas, JH Timmins, AR Tlusty, D Tokarev, M Trentalange, S Tribble, RE Tribedy, P Trzeciak, BA Tsai, OD Turnau, J Ullrich, T Underwood, DG Van Buren, G van Nieuwenhuizen, G Vandenbroucke, M Vanfossen, JA Varma, R Vasconcelos, GMS Vasiliev, AN Vertesi, R Videbaek, F Viyogi, YP Vokal, S Vossen, A Wada, M Wang, F Wang, G Wang, H Wang, JS Wang, XL Wang, Y Wang, Y Webb, G Webb, JC Westfall, GD Wieman, H Wissink, SW Witt, R Wu, YF Xiao, Z Xie, W Xin, K Xu, H Xu, J Xu, N Xu, QH Xu, Y Xu, Z Yan, W Yang, C Yang, Y Yang, Y Ye, Z Yepes, P Yi, L Yip, K Yoo, IK Yu, N Zawisza, Y Zbroszczyk, H Zha, W Zhang, JB Zhang, JL Zhang, S Zhang, XP Zhang, Y Zhang, ZP Zhao, F Zhao, J Zhong, C Zhu, X Zhu, YH Zoulkarneeva, Y Zyzak, M AF Adamczyk, L. Adkins, J. K. Agakishiev, G. Aggarwal, M. M. Ahammed, Z. Alekseev, I. Alford, J. Anson, C. D. Aparin, A. Arkhipkin, D. Aschenauer, E. C. Averichev, G. S. Banerjee, A. Beavis, D. R. Bellwied, R. Bhasin, A. Bhati, A. K. Bhattarai, P. Bichsel, H. Bielcik, J. Bielcikova, J. Bland, L. C. Bordyuzhin, I. G. Borowski, W. Bouchet, J. Brandin, A. V. Brovko, S. G. Bueltmann, S. Bunzarov, I. Burton, T. P. Butterworth, J. Caines, H. Sanchez, M. Calderon de la Barca Cebra, D. Cendejas, R. Cervantes, M. C. Chaloupka, P. Chang, Z. Chattopadhyay, S. Chen, H. F. Chen, J. H. Chen, L. Cheng, J. Cherney, M. Chikanian, A. Christie, W. Chwastowski, J. Codrington, M. J. M. Contin, G. Cramer, J. G. Crawford, H. J. Cui, X. Das, S. Leyva, A. Davila De Silva, L. C. Debbe, R. R. Dedovich, T. G. Deng, J. Derevschikov, A. A. Derradi de Souza, R. Dhamija, S. di Ruzza, B. Didenko, L. Dilks, C. Ding, F. Djawotho, P. Dong, X. Drachenberg, J. L. Draper, J. E. Du, C. M. Dunkelberger, L. E. Dunlop, J. C. Efimov, L. G. Engelage, J. Engle, K. S. Eppley, G. Eun, L. Evdokimov, O. Eyser, O. Fatemi, R. Fazio, S. Fedorisin, J. Filip, P. Finch, E. Fisyak, Y. Flores, C. E. Gagliardi, C. A. Gangadharan, D. R. Garand, D. Geurts, F. Gibson, A. Girard, M. Gliske, S. Greiner, L. Grosnick, D. Gunarathne, D. S. Guo, Y. Gupta, A. Gupta, S. Guryn, W. Haag, B. Hamed, A. Han, L-X. Haque, R. Harris, J. W. Heppelmann, S. Hirsch, A. Hoffmann, G. W. Hofman, D. J. Horvat, S. Huang, B. Huang, H. Z. Huang, X. Huck, P. Humanic, T. J. Igo, G. Jacobs, W. W. Jang, H. Judd, E. G. Kabana, S. Kalinkin, D. Kang, K. Kauder, K. Ke, H. W. Keane, D. Kechechyan, A. Kesich, A. Khan, Z. H. Kikola, D. P. Kisel, I. Kisiel, A. Koetke, D. D. Kollegger, T. Konzer, J. Koralt, I. Kosarzewski, L. K. Kotchenda, L. Kraishan, A. F. Kravtsov, P. Krueger, K. Kulakov, I. Kumar, L. Kycia, R. A. Lamont, M. A. C. Landgraf, J. M. Landry, K. D. Lauret, J. Lebedev, A. Lednicky, R. Lee, J. H. LeVine, M. J. Li, C. Li, W. Li, X. Li, X. Li, Y. Li, Z. M. Lisa, M. A. Liu, F. Ljubicic, T. Llope, W. J. Lomnitz, M. Longacre, R. S. Luo, X. Ma, G. L. Ma, Y. G. Don, D. M. M. D. Madagodagettige Mahapatra, D. P. Majka, R. Margetis, S. Markert, C. Masui, H. Matis, H. S. McDonald, D. McShane, T. S. Minaev, N. G. Mioduszewski, S. Mohanty, B. Mondal, M. M. Morozov, D. A. Mustafa, M. K. Nandi, B. K. Nasim, Md. Nayak, T. K. Nelson, J. M. Nigmatkulov, G. Nogach, L. V. Noh, S. Y. Novak, J. Nurushev, S. B. Odyniec, G. Ogawa, A. Oh, K. Ohlson, A. Okorokov, V. Oldag, E. W. Olvitt, D. L., Jr. Pachr, M. Page, B. S. Pal, S. K. Pan, Y. X. Pandit, Y. Panebratsev, Y. Pawlak, T. Pawlik, B. Pei, H. Perkins, C. Peryt, W. Pile, P. Planinic, M. Pluta, J. Poljak, N. Poniatowska, K. Porter, J. Poskanzer, A. M. Pruthi, N. K. Przybycien, M. Pujahari, P. R. Putschke, J. Qiu, H. Quintero, A. Ramachandran, S. Raniwala, R. Raniwala, S. Ray, R. L. Riley, C. K. Ritter, H. G. Roberts, J. B. Rogachevskiy, O. V. Romero, J. L. Ross, J. F. Roy, A. Ruan, L. Rusnak, J. Rusnakova, O. Sahoo, N. R. Sahu, P. K. Sakrejda, I. Salur, S. Sandweiss, J. Sangaline, E. Sarkar, A. Schambach, J. Scharenberg, R. P. Schmah, A. M. Schmidke, W. B. Schmitz, N. Seger, J. Seyboth, P. Shah, N. Shahaliev, E. Shanmuganathan, P. V. Shao, M. Sharma, B. Shen, W. Q. Shi, S. S. Shou, Q. Y. Sichtermann, E. P. Singaraju, R. N. Skoby, M. J. Smirnov, D. Smirnov, N. Solanki, D. Sorensen, P. Spinka, H. M. Srivastava, B. Stanislaus, T. D. S. Stevens, J. R. Stock, R. Strikhanov, M. Stringfellow, B. Sumbera, M. Sun, X. Sun, X. M. Sun, Y. Sun, Z. Surrow, B. Svirida, D. N. Symons, T. J. M. Szelezniak, M. A. Takahashi, J. Tang, A. H. Tang, Z. Tarnowsky, T. Thomas, J. H. Timmins, A. R. Tlusty, D. Tokarev, M. Trentalange, S. Tribble, R. E. Tribedy, P. Trzeciak, B. A. Tsai, O. D. Turnau, J. Ullrich, T. Underwood, D. G. Van Buren, G. van Nieuwenhuizen, G. Vandenbroucke, M. Vanfossen, J. A., Jr. Varma, R. Vasconcelos, G. M. S. Vasiliev, A. N. Vertesi, R. Videbaek, F. Viyogi, Y. P. Vokal, S. Vossen, A. Wada, M. Wang, F. Wang, G. Wang, H. Wang, J. S. Wang, X. L. Wang, Y. Wang, Y. Webb, G. Webb, J. C. Westfall, G. D. Wieman, H. Wissink, S. W. Witt, R. Wu, Y. F. Xiao, Z. Xie, W. Xin, K. Xu, H. Xu, J. Xu, N. Xu, Q. H. Xu, Y. Xu, Z. Yan, W. Yang, C. Yang, Y. Yang, Y. Ye, Z. Yepes, P. Yi, L. Yip, K. Yoo, I-K. Yu, N. Zawisza, Y. Zbroszczyk, H. Zha, W. Zhang, J. B. Zhang, J. L. Zhang, S. Zhang, X. P. Zhang, Y. Zhang, Z. P. Zhao, F. Zhao, J. Zhong, C. Zhu, X. Zhu, Y. H. Zoulkarneeva, Y. Zyzak, M. CA STAR Collaboration TI Beam-energy-dependent two-pion interferometry and the freeze-out eccentricity of pions measured in heavy ion collisions at the STAR detector SO PHYSICAL REVIEW C LA English DT Article ID QUARK-GLUON PLASMA; RELATIVISTIC NUCLEAR COLLISIONS; BOSE-EINSTEIN CORRELATIONS; TRANSVERSE-MOMENTUM; COULOMB CORRECTIONS; PB+PB COLLISIONS; PHASE-TRANSITION; CRITICAL-POINT; SPS ENERGIES; QCD AB We present results of analyses of two-pion interferometry in Au + Au collisions at root s(NN) = 7.7, 11.5, 19.6, 27, 39, 62.4, and 200 GeV measured in the STAR detector as part of the BNL Relativistic Heavy Ion Collider Beam Energy Scan program. The extracted correlation lengths (Hanbury-Brown-Twiss radii) are studied as a function of beam energy, azimuthal angle relative to the reaction plane, centrality, and transverse mass (m(T)) of the particles. The azimuthal analysis allows extraction of the eccentricity of the entire fireball at kinetic freeze-out. The energy dependence of this observable is expected to be sensitive to changes in the equation of state. A new global fit method is studied as an alternate method to directly measure the parameters in the azimuthal analysis. The eccentricity shows a monotonic decrease with beam energy that is qualitatively consistent with the trend from all model predictions and quantitatively consistent with a hadronic transport model. C1 [Adamczyk, L.; Przybycien, M.] AGH Univ Sci & Technol, Krakow, Poland. [Gliske, S.; Krueger, K.; Spinka, H. M.; Underwood, D. G.] Argonne Natl Lab, Argonne, IL 60439 USA. [Nelson, J. M.] Univ Birmingham, Birmingham, W Midlands, England. [Arkhipkin, D.; Aschenauer, E. C.; Beavis, D. R.; Bland, L. C.; Burton, T. P.; Christie, W.; Debbe, R. R.; di Ruzza, B.; Didenko, L.; Dunlop, J. C.; Eyser, O.; Fazio, S.; Fisyak, Y.; Guryn, W.; Huang, B.; Ke, H. W.; Lamont, M. A. C.; Landgraf, J. M.; Lauret, J.; Lebedev, A.; Lee, J. H.; LeVine, M. J.; Ljubicic, T.; Longacre, R. S.; Ogawa, A.; Pile, P.; Ruan, L.; Schmidke, W. B.; Smirnov, D.; Sorensen, P.; Tang, A. H.; Ullrich, T.; Van Buren, G.; Videbaek, F.; Wang, H.; Webb, J. C.; Xu, Z.; Yip, K.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Crawford, H. J.; Engelage, J.; Judd, E. G.; Perkins, C.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Brovko, S. G.; Sanchez, M. Calderon de la Barca; Cebra, D.; Ding, F.; Draper, J. E.; Flores, C. E.; Haag, B.; Kesich, A.; Romero, J. L.; Sangaline, E.] Univ Calif Davis, Davis, CA 95616 USA. [Dunkelberger, L. E.; Huang, H. Z.; Igo, G.; Landry, K. D.; Pan, Y. X.; Shah, N.; Trentalange, S.; Tsai, O. D.; Wang, G.; Zhao, F.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [Derradi de Souza, R.; Takahashi, J.; Vasconcelos, G. M. S.] Univ Estadual Campinas, Sao Paulo, Brazil. [Chen, L.; Huck, P.; Li, Z. M.; Liu, F.; Luo, X.; Pei, H.; Wu, Y. F.; Xu, J.; Yang, Y.; Yu, N.; Zhang, J. B.; Zhao, J.] Cent China Normal Univ HZNU, Wuhan 430079, Peoples R China. [Evdokimov, O.; Hofman, D. J.; Kauder, K.; Khan, Z. H.; Pandit, Y.; Wang, Y.; Ye, Z.] Univ Illinois, Chicago, IL 60607 USA. [Kycia, R. A.] Cracow Univ Technol, Krakow, Poland. [Cherney, M.; De Silva, L. C.; Don, D. M. M. D. Madagodagettige; McShane, T. S.; Ross, J. F.; Seger, J.] Creighton Univ, Omaha, NE 68178 USA. [Bielcik, J.; Chaloupka, P.; Pachr, M.; Rusnakova, O.; Trzeciak, B. A.] Czech Tech Univ, Fac Nucl Sci & Phys Engn, CR-11519 Prague, Czech Republic. [Bielcikova, J.; Rusnak, J.; Sumbera, M.; Tlusty, D.; Vertesi, R.] Nucl Phys Inst AS CR, Rez 25068, Czech Republic. [Kisel, I.; Kollegger, T.; Kulakov, I.; Stock, R.; Zyzak, M.] Frankfurt Inst Adv Studies FIAS, Frankfurt, Germany. [Das, S.; Mahapatra, D. P.; Sahu, P. K.] Inst Phys, Bhubaneswar 751005, Orissa, India. [Nandi, B. K.; Pujahari, P. R.; Sarkar, A.; Varma, R.] Indian Inst Technol, Bombay 400076, Maharashtra, India. [Dhamija, S.; Jacobs, W. W.; Page, B. S.; Skoby, M. J.; Vossen, A.; Wissink, S. W.] Indiana Univ, Bloomington, IN 47408 USA. [Alekseev, I.; Bordyuzhin, I. G.; Kalinkin, D.; Svirida, D. N.] Alikhanov Inst Theoret & Expt Phys, Moscow, Russia. [Bhasin, A.; Gupta, A.; Gupta, S.] Univ Jammu, Jammu 180001, India. [Agakishiev, G.; Aparin, A.; Averichev, G. S.; Bunzarov, I.; Dedovich, T. G.; Efimov, L. G.; Fedorisin, J.; Filip, P.; Kechechyan, A.; Lednicky, R.; Panebratsev, Y.; Rogachevskiy, O. V.; Shahaliev, E.; Tokarev, M.; Vokal, S.; Zoulkarneeva, Y.] Joint Inst Nucl Res, Dubna 141980, Russia. [Alford, J.; Bouchet, J.; Keane, D.; Lomnitz, M.; Margetis, S.; Quintero, A.; Shanmuganathan, P. V.; Vanfossen, J. A., Jr.] Kent State Univ, Kent, OH 44242 USA. [Adkins, J. K.; Fatemi, R.; Ramachandran, S.; Webb, G.] Univ Kentucky, Lexington, KY 40506 USA. [Jang, H.; Noh, S. Y.] Korea Inst Sci & Technol Informat, Taejon, South Korea. [Du, C. M.; Sun, Z.; Wang, J. S.; Xu, H.; Yang, Y.] Inst Modern Phys, Lanzhou, Peoples R China. [Contin, G.; Dong, X.; Eun, L.; Greiner, L.; Masui, H.; Matis, H. S.; Mustafa, M. K.; Odyniec, G.; Porter, J.; Poskanzer, A. M.; Qiu, H.; Ritter, H. G.; Sakrejda, I.; Salur, S.; Schmah, A. M.; Shi, S. S.; Sichtermann, E. P.; Sun, X.; Sun, X. M.; Symons, T. J. M.; Szelezniak, M. A.; Thomas, J. H.; Wieman, H.; Xu, N.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Stevens, J. R.; van Nieuwenhuizen, G.] MIT, Cambridge, MA 02139 USA. [Schmitz, N.; Seyboth, P.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Novak, J.; Tarnowsky, T.; Westfall, G. D.] Michigan State Univ, E Lansing, MI 48824 USA. [Brandin, A. V.; Kotchenda, L.; Kravtsov, P.; Nigmatkulov, G.; Okorokov, V.; Strikhanov, M.] Moscow Engn Phys Inst, Moscow 115409, Russia. [Haque, R.; Kumar, L.; Mohanty, B.; Nasim, Md.] Natl Inst Sci Educ & Res, Bhubaneswar 751005, Orissa, India. [Anson, C. D.; Gangadharan, D. R.; Humanic, T. J.; Lisa, M. A.] Ohio State Univ, Columbus, OH 43210 USA. [Bueltmann, S.; Koralt, I.] Old Dominion Univ, Norfolk, VA 23529 USA. [Pawlik, B.; Turnau, J.] Inst Nucl Phys PAN, Krakow, Poland. [Aggarwal, M. M.; Bhati, A. K.; Pruthi, N. K.; Sharma, B.] Panjab Univ, Chandigarh 160014, India. [Cendejas, R.; Dilks, C.; Heppelmann, S.] Penn State Univ, University Pk, PA 16802 USA. [Chwastowski, J.] Polish Acad Sci, Inst Nucl Sci, PL-31342 Krakow, Poland. [Derevschikov, A. A.; Minaev, N. G.; Morozov, D. A.; Nogach, L. V.; Nurushev, S. B.; Vasiliev, A. N.] Inst High Energy Phys, Protvino, Russia. [Garand, D.; Hirsch, A.; Konzer, J.; Li, X.; Scharenberg, R. P.; Srivastava, B.; Stringfellow, B.; Wang, F.; Xie, W.; Yi, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Oh, K.; Yoo, I-K.] Pusan Natl Univ, Pusan 609735, South Korea. [Raniwala, R.; Raniwala, S.; Solanki, D.] Univ Rajasthan, Jaipur 302004, Rajasthan, India. [Butterworth, J.; Eppley, G.; Geurts, F.; Llope, W. J.; Roberts, J. B.; Xin, K.; Yepes, P.] Rice Univ, Houston, TX 77251 USA. [Chen, H. F.; Cui, X.; Guo, Y.; Li, C.; Shao, M.; Sun, Y.; Tang, Z.; Wang, X. L.; Xu, Y.; Yang, C.; Zawisza, Y.; Zha, W.; Zhang, Y.; Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Deng, J.; Xu, Q. H.; Zhang, J. L.] Shandong Univ, Jinan 250100, Shandong, Peoples R China. [Chen, J. H.; Han, L-X.; Li, W.; Ma, G. L.; Ma, Y. G.; Shen, W. Q.; Shou, Q. Y.; Zhang, S.; Zhong, C.; Zhu, Y. H.] Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China. [Borowski, W.; Kabana, S.] SUBATECH, Nantes, France. [Gunarathne, D. S.; Kraishan, A. F.; Li, X.; Olvitt, D. L., Jr.; Surrow, B.; Vandenbroucke, M.] Temple Univ, Philadelphia, PA 19122 USA. [Cervantes, M. C.; Chang, Z.; Djawotho, P.; Gagliardi, C. A.; Hamed, A.; Mioduszewski, S.; Mondal, M. M.; Sahoo, N. R.; Tribble, R. E.] Texas A&M Univ, College Stn, TX 77843 USA. [Bhattarai, P.; Codrington, M. J. M.; Leyva, A. Davila; Hoffmann, G. W.; Markert, C.; Oldag, E. W.; Ray, R. L.; Schambach, J.; Wada, M.] Univ Texas Austin, Austin, TX 78712 USA. [Bellwied, R.; McDonald, D.; Timmins, A. R.] Univ Houston, Houston, TX 77204 USA. [Cheng, J.; Huang, X.; Kang, K.; Li, Y.; Wang, Y.; Xiao, Z.; Yan, W.; Zhang, X. P.; Zhu, X.] Tsinghua Univ, Beijing 100084, Peoples R China. [Engle, K. S.; Witt, R.] US Naval Acad, Annapolis, MD 21402 USA. [Drachenberg, J. L.; Gibson, A.; Grosnick, D.; Koetke, D. D.; Stanislaus, T. D. S.] Valparaiso Univ, Valparaiso, IN 46383 USA. [Ahammed, Z.; Banerjee, A.; Chattopadhyay, S.; Nayak, T. K.; Pal, S. K.; Roy, A.; Singaraju, R. N.; Tribedy, P.; Viyogi, Y. P.] Ctr Variable Energy Cyclotron, Kolkata 700064, India. [Girard, M.; Kikola, D. P.; Kisiel, A.; Kosarzewski, L. K.; Pawlak, T.; Peryt, W.; Pluta, J.; Poniatowska, K.; Zbroszczyk, H.] Warsaw Univ Technol, Warsaw, Poland. [Bichsel, H.; Cramer, J. G.] Univ Washington, Seattle, WA 98195 USA. [Putschke, J.] Wayne State Univ, Detroit, MI 48201 USA. [Caines, H.; Chikanian, A.; Finch, E.; Harris, J. W.; Horvat, S.; Majka, R.; Ohlson, A.; Riley, C. K.; Sandweiss, J.; Smirnov, N.] Yale Univ, New Haven, CT 06520 USA. [Planinic, M.; Poljak, N.] Univ Zagreb, HR-10002 Zagreb, Croatia. RP Adamczyk, L (reprint author), AGH Univ Sci & Technol, Krakow, Poland. RI Kycia, Radoslaw/J-4397-2015; Fazio, Salvatore /G-5156-2010; Svirida, Dmitry/R-4909-2016; Rusnak, Jan/G-8462-2014; Bielcikova, Jana/G-9342-2014; Sumbera, Michal/O-7497-2014; Chaloupka, Petr/E-5965-2012; Takahashi, Jun/B-2946-2012; Huang, Bingchu/H-6343-2015; Derradi de Souza, Rafael/M-4791-2013; Xin, Kefeng/O-9195-2016; Yi, Li/Q-1705-2016; Alekseev, Igor/J-8070-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Okorokov, Vitaly/C-4800-2017; Ma, Yu-Gang/M-8122-2013; Gunarathne, Devika/C-4903-2017; OI Kycia, Radoslaw/0000-0002-6390-4627; Sumbera, Michal/0000-0002-0639-7323; Takahashi, Jun/0000-0002-4091-1779; Huang, Bingchu/0000-0002-3253-3210; Derradi de Souza, Rafael/0000-0002-2084-7001; Xin, Kefeng/0000-0003-4853-9219; Yi, Li/0000-0002-7512-2657; Alekseev, Igor/0000-0003-3358-9635; Okorokov, Vitaly/0000-0002-7162-5345; Ma, Yu-Gang/0000-0002-0233-9900; Gunarathne, Devika/0000-0002-7155-7418; Ke, Hongwei/0000-0003-1463-7291; Sorensen, Paul/0000-0001-5056-9391; Thomas, James/0000-0002-6256-4536 FU RHIC Operations Group; RCF at BNL; NERSC Center at LBNL; KISTI Center in Korea; Open Science Grid consortium; Office of NP within the US DOE Office of Science; Office of HEP within the US DOE Office of Science; US NSF; CNRS/IN2P3; FAPESP CNPq of Brazil; Ministry of Education and Science of the Russian Federation; NNSFC; CAS; MoST; MoE of China; Korean Research Foundation; GA of the Czech Republic; MSMT of the Czech Republic; FIAS of Germany; DAE; DST; CSIR of India; National Science Centre of Poland; National Research Foundation of the Republic of Croatia, Ministry of Science, Education and Sports of the Republic of Croatia; RosAtom of Russia FX We thank the RHIC Operations Group and RCF at BNL, the NERSC Center at LBNL, the KISTI Center in Korea, and the Open Science Grid consortium for providing resources and support. This work was supported in part by the Offices of NP and HEP within the US DOE Office of Science, the US NSF, CNRS/IN2P3; FAPESP CNPq of Brazil; Ministry of Education and Science of the Russian Federation; NNSFC, CAS, MoST, and MoE of China; the Korean Research Foundation; GA and MSMT of the Czech Republic; FIAS of Germany; DAE, DST, and CSIR of India; National Science Centre of Poland; National Research Foundation of the Republic of Croatia, Ministry of Science, Education and Sports of the Republic of Croatia; and RosAtom of Russia. NR 87 TC 8 Z9 8 U1 2 U2 36 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JUL 10 PY 2015 VL 92 IS 1 AR 014904 DI 10.1103/PhysRevC.92.014904 PG 27 WC Physics, Nuclear SC Physics GA CM6OI UT WOS:000357807800003 ER PT J AU Aursjo, O Pride, SR AF Aursjo, Olav Pride, Steven R. TI Lattice Boltzmann method for diffusion-limited partial dissolution of fluids SO PHYSICAL REVIEW E LA English DT Article ID LIQUID-MIXTURES; SURFACE-TENSION; BINARY-FLUID; SIMULATIONS; SYSTEMS; MODEL; ENERGY AB A lattice Boltzmann model for two partially miscible fluids is developed. By partially miscible we mean that, although there is a definite interfacial region separating the two fluids with a surface tension force acting at all points of the transition region, each fluid can nonetheless accept molecules from the other fluid up to a set solubility limit. We allow each fluid to diffuse into the other with the solubility and diffusivity in each fluid being input parameters. The approach is to define two regions within the fluid: one interfacial region having finite width, across which most of the concentration change occurs, and in which a surface tension force and color separation step are allowed for and one miscible fluid region where the concentration of the binary fluids follows an advection-diffusion equation and the mixture as a whole obeys the Navier-Stokes incompressible flow equations. Numerical examples are presented in which the algorithm produces results that are quantitatively compared to exact analytical results as well as qualitatively examined for their reasonableness. The model has the ability to simulate how bubbles of one fluid flow through another while dissolving their contents as well as to simulate a range of practical invasion problems such as injecting supercritical CO2 into a porous material saturated with water for sequestration purposes. C1 [Aursjo, Olav] IRIS AS, N-4068 Stavanger, Norway. [Aursjo, Olav; Pride, Steven R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Aursjo, O (reprint author), IRIS AS, POB 8046, N-4068 Stavanger, Norway. EM olav.aursjo@iris.no; srpride@lbl.gov FU Center for Nanoscale Control of Geologic CO2, an Energy Frontier Research Center - US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-05CH11231]; US Department of Energy, at the Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Geosciences Research Program of the DOE Office of Basic Energy Sciences, Divisions of Chemical Sciences, Geosciences and Biosciences FX The work of O.A. was supported as part of the Center for Nanoscale Control of Geologic CO2, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Grant No. DE-AC02-05CH11231. The work of S.R.P. was performed under the auspices of the US Department of Energy, at the Lawrence Berkeley National Laboratory, under Contract No. DE-AC02-05CH11231. Support was provided specifically by the Geosciences Research Program of the DOE Office of Basic Energy Sciences, Divisions of Chemical Sciences, Geosciences and Biosciences. NR 35 TC 1 Z9 1 U1 2 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD JUL 10 PY 2015 VL 92 IS 1 AR 013306 DI 10.1103/PhysRevE.92.013306 PG 14 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA CM6OY UT WOS:000357809400008 PM 26274306 ER PT J AU Terzyan, SS Burgett, AWG Heroux, A Smith, CA Mooers, BHM Hanigan, MH AF Terzyan, Simon S. Burgett, Anthony W. G. Heroux, Annie Smith, Clyde A. Mooers, Blaine H. M. Hanigan, Marie H. TI Human gamma-Glutamyl Transpeptidase 1 STRUCTURES OF THE FREE ENZYME, INHIBITOR-BOUND TETRAHEDRAL TRANSITION STATES, AND GLUTAMATE-BOUND ENZYME REVEAL NOVEL MOVEMENT WITHIN THE ACTIVE SITE DURING CATALYSIS SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article ID MACROMOLECULAR STRUCTURES; GLUTATHIONE METABOLISM; SUBSTRATE-SPECIFICITY; ESCHERICHIA-COLI; ACID; IDENTIFICATION; TRANSFERASE; RESISTANCE; MECHANISM; CISPLATIN AB gamma-Glutamyl transpeptidase 1 (GGT1) is a cell surface, N-terminal nucleophile hydrolase that cleaves glutathione and other g-glutamyl compounds. GGT1 expression is essential in cysteine homeostasis, and its induction has been implicated in the pathology of asthma, reperfusion injury, and cancer. In this study, we report four new crystal structures of human GGT1 (hGGT1) that show conformational changes within the active site as the enzyme progresses from the free enzyme to inhibitor-bound tetrahedral transition states and finally to the glutamate-bound structure prior to the release of this final product of the reaction. The structure of the apoenzyme shows flexibility within the active site. The serine-borate-bound hGGT1 crystal structure demonstrates that serine-borate occupies the active site of the enzyme, resulting in an enzyme-inhibitor complex that replicates the enzyme's tetrahedral intermediate/transition state. The structure of GGsTop-bound hGGT1 reveals its interactions with the enzyme and why neutral phosphonate diesters are more potent inhibitors than monoanionic phosphonates. These structures are the first structures for any eukaryotic GGT that include a molecule in the active site covalently bound to the catalytic Thr-381. The glutamate-bound structure shows the conformation of the enzyme prior to release of the final product and reveals novel information regarding the displacement of the main chain atoms that form the oxyanion hole and movement of the lid loop region when the active site is occupied. These data provide new insights into the mechanism of hGGT1-catalyzed reactions and will be invaluable in the development of new classes of hGGT1 inhibitors for therapeutic use. C1 [Terzyan, Simon S.] Univ Oklahoma, Hlth Sci Ctr, Dept Biochem & Mol Biol, Macromol Crystallog Lab, Oklahoma City, OK 73104 USA. [Burgett, Anthony W. G.] Univ Oklahoma, Dept Chem & Biochem, Norman, OK 73019 USA. [Heroux, Annie] Brookhaven Natl Lab, Photon Sci Div, Energy Sci Directorate, Upton, NY 11973 USA. [Smith, Clyde A.] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Mooers, Blaine H. M.] Univ Oklahoma, Hlth Sci Ctr, Dept Biochem & Mol Biol, Oklahoma City, OK 73104 USA. [Hanigan, Marie H.] Univ Oklahoma, Hlth Sci Ctr, Dept Cell Biol, Stanton L Young Biomed Res Ctr, Oklahoma City, OK 73104 USA. RP Hanigan, MH (reprint author), Univ Oklahoma, Hlth Sci Ctr, Dept Cell Biol, Stanton L Young Biomed Res Ctr, Rm 264,975 NE 10th St, Oklahoma City, OK 73104 USA. EM marie-hanigan@ouhsc.edu RI Regan, Clinton/E-6250-2012 FU National Institutes of Health (NIH) from the NIGMS [P20GM103640]; National Institutes of Health (NIH) [R01AI088011]; United States Department of Energy Offices of Biological and Environmental Research and Basic Energy Sciences [DE-AC02-98CH10886, E-SC0012704]; NIH [P41RR012408, P41GM103473, P41-GM111244]; United States Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]; Department of Energy Office of Biological and Environmental Research; NIH, NIGMS [P41GM103393] FX This work was supported, in whole or in part, by National Institutes of Health (NIH) Grants P20GM103640 (an Institutional Development Award (IDeA) from the NIGMS) and R01AI088011 (to B. H. M. M.). X-ray diffraction data were collected at the National Synchrotron Light Source, for which financial support comes principally from the United States Department of Energy Offices of Biological and Environmental Research and Basic Energy Sciences Grants DE-AC02-98CH10886 and E-SC0012704 and from NIH Grants P41RR012408, P41GM103473, and P41-GM111244. X-ray diffraction data were also collected at the Stanford Synchrotron Radiation Light source, the use of which was supported by the United States Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract DE-AC02-76SF00515. The Stanford Synchrotron Radiation Lightsource Structural Molecular Biology Program is supported by the Department of Energy Office of Biological and Environmental Research and by NIH, NIGMS, Grant P41GM103393. The authors declare that they have no conflicts of interest with the contents of this article. NR 33 TC 7 Z9 7 U1 0 U2 8 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD JUL 10 PY 2015 VL 290 IS 28 BP 17576 EP 17586 DI 10.1074/jbc.M115.659680 PG 11 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CM5MB UT WOS:000357730900048 PM 26013825 ER PT J AU Hochberg, Y Kuflik, E Murayama, H Volansky, T Wacker, JG AF Hochberg, Yonit Kuflik, Eric Murayama, Hitoshi Volansky, Tomer Wacker, Jay G. TI Model for Thermal Relic Dark Matter of Strongly Interacting Massive Particles SO PHYSICAL REVIEW LETTERS LA English DT Article ID GALAXY CLUSTER 1E-0657-56; INTERACTION CROSS-SECTION; LATTICE GAUGE-THEORY; 2-COLOR QCD; COSMOLOGICAL SIMULATIONS; CURRENT-ALGEBRA; TEMPERATURE; CONSTRAINTS; SUBHALOES; ALIGNMENT AB A recent proposal is that dark matter could be a thermal relic of 3 -> 2 scatterings in a strongly coupled hidden sector. We present explicit classes of strongly coupled gauge theories that admit this behavior. These are QCD-like theories of dynamical chiral symmetry breaking, where the pions play the role of dark matter. The number-changing 3 -> 2 process, which sets the dark matter relic abundance, arises from the Wess-Zumino-Witten term. The theories give an explicit relationship between the 3 -> 2 annihilation rate and the 2 -> 2 self-scattering rate, which alters predictions for structure formation. This is a simple calculable realization of the strongly interacting massive-particle mechanism. C1 [Hochberg, Yonit; Murayama, Hitoshi] Univ Calif Berkeley, Ernest Orlando Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Hochberg, Yonit; Murayama, Hitoshi] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Kuflik, Eric] Cornell Univ, LEPP, Dept Phys, Ithaca, NY 14853 USA. [Murayama, Hitoshi] Univ Tokyo, Inst Adv Study, Kavli Inst Phys & Math Univ WPI, Kashiwa, Chiba 2778583, Japan. [Volansky, Tomer] Tel Aviv Univ, Dept Phys, IL-6997801 Tel Aviv, Israel. [Wacker, Jay G.] Quora, Mountain View, CA 94041 USA. [Wacker, Jay G.] Stanford Univ, Stanford Inst Theoret Phys, Stanford, CA 94305 USA. RP Hochberg, Y (reprint author), Univ Calif Berkeley, Ernest Orlando Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM yonit.hochberg@berkeley.edu; kuflik@cornell.edu; hitoshi@berkeley.edu; tomerv@post.tau.ac.il; jgwacker@stanford.edu OI Kuflik, Eric/0000-0003-0455-0467 FU U.S. National Science Foundation [PHY-1002399]; Awardee of the Weizmann Institute of Science-National Postdoctoral Award Program for Advancing Women in Science; NSF [PHY-1002399, PHY-1316222, PHY-1316783, PHY-0756174, PHYS-1066293]; U.S. DOE [DE-AC02-05CH11231]; JSPS [26400241, 26105507]; EU-FP7 Marie Curie, CIG Fellowship; I-CORE Program of the Planning Budgeting Committee; Israel Science Foundation [1937/12]; WPI, MEXT, Japan; US-Israel Binational Science Foundation FX The work of Y. H. is supported by the U.S. National Science Foundation under Grant No. PHY-1002399. Y. H. received support as an Awardee of the Weizmann Institute of Science-National Postdoctoral Award Program for Advancing Women in Science. E. K. is supported by the NSF under Grant No. PHY-1316222. H. M. was supported by the U.S. DOE under Contract No. DE-AC02-05CH11231, and by the NSF under Grants No. PHY-1002399 and No. PHY-1316783. H. M. was also supported by the JSPS Grant-in-Aid for Scientific Research (C) (Grant No. 26400241), Scientific Research on Innovative Areas (Grant No. 26105507), and by WPI, MEXT, Japan. T. V. is supported by the US-Israel Binational Science Foundation, by the EU-FP7 Marie Curie, CIG Fellowship, and by the I-CORE Program of the Planning Budgeting Committee and the Israel Science Foundation (Grant No. 1937/12). J. G. W. is supported in part by the NSF under Grant No. PHY-0756174. This work was supported in part by the NSF under Grant No. PHYS-1066293 and the hospitality of the Aspen Center for Physics. NR 48 TC 38 Z9 38 U1 2 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 10 PY 2015 VL 115 IS 2 AR 021301 DI 10.1103/PhysRevLett.115.021301 PG 5 WC Physics, Multidisciplinary SC Physics GA CM6PG UT WOS:000357810300003 PM 26207457 ER PT J AU Kennefick, D Blume, M AF Kennefick, Daniel Blume, Martin TI Reviewing Einstein SO SCIENCE LA English DT Letter C1 [Kennefick, Daniel] Univ Arkansas, Dept Phys, Fayetteville, AR 72701 USA. [Blume, Martin] Brookhaven Natl Lab, CMPMS Dept, Upton, NY 11973 USA. RP Kennefick, D (reprint author), Univ Arkansas, Dept Phys, Fayetteville, AR 72701 USA. EM danielk@uark.edu NR 1 TC 0 Z9 0 U1 1 U2 9 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JUL 10 PY 2015 VL 349 IS 6244 BP 149 EP 149 PG 1 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CM4OM UT WOS:000357664300029 PM 26160937 ER PT J AU Pascolo, L Borelli, V Canzonieri, V Gianoncelli, A Birarda, G Bedolla, DE Salome, M Vaccari, L Calligaro, C Cotte, M Hesse, B Luisi, F Zabucchi, G Melato, M Rizzardi, C AF Pascolo, Lorella Borelli, Violetta Canzonieri, Vincenzo Gianoncelli, Alessandra Birarda, Giovanni Bedolla, Diana E. Salome, Murielle Vaccari, Lisa Calligaro, Carla Cotte, Marine Hesse, Bernhard Luisi, Fernando Zabucchi, Giuliano Melato, Mauro Rizzardi, Clara TI Differential protein folding and chemical changes in lung tissues exposed to asbestos or particulates SO SCIENTIFIC REPORTS LA English DT Article ID COAL-WORKERS PNEUMOCONIOSIS; BODIES; BODY; IRON; SPECTROSCOPY; TOXICITY; FERRITIN; CELLS AB Environmental and occupational inhalants may induce a large number of pulmonary diseases, with asbestos exposure being the most risky. The mechanisms are clearly related to chemical composition and physical and surface properties of materials. A combination of X-ray fluorescence (mu XRF) and Fourier Transform InfraRed (mu FTIR) microscopy was used to chemically characterize and compare asbestos bodies versus environmental particulates (anthracosis) in lung tissues from asbestos exposed and control patients. mu XRF analyses revealed heterogeneously aggregated particles in the anthracotic structures, containing mainly Si, K, Al and Fe. Both asbestos and particulates alter lung iron homeostasis, with a more marked effect in asbestos exposure. mu FTIR analyses revealed abundant proteins on asbestos bodies but not on anthracotic particles. Most importantly, the analyses demonstrated that the asbestos coating proteins contain high levels of beta-sheet structures. The occurrence of conformational changes in the proteic component of the asbestos coating provides new insights into long-term asbestos effects. C1 [Pascolo, Lorella; Melato, Mauro] IRCCS Burlo Garofolo, Inst Maternal & Child Hlth, Trieste, Italy. [Borelli, Violetta; Zabucchi, Giuliano] Univ Trieste, Dept Life Sci, Trieste, Italy. [Canzonieri, Vincenzo] Natl Canc Inst, IRCCS, CRO, Div Pathol, Aviano, PN, Italy. [Gianoncelli, Alessandra; Birarda, Giovanni; Bedolla, Diana E.; Vaccari, Lisa] Elettra Sincrotrone Trieste, Trieste, Italy. [Birarda, Giovanni] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Bedolla, Diana E.] Univ Trieste, Dept Phys, Trieste, Italy. [Salome, Murielle; Cotte, Marine; Hesse, Bernhard] European Synchrotron Radiat Facil, F-38043 Grenoble 9, France. [Calligaro, Carla] Univ Udine, Serv Diagnost Vet, I-33100 Udine, Italy. [Luisi, Fernando] Inail, Sovrintendenza Med Reg, Trieste, Italy. [Rizzardi, Clara] Univ Trieste, Dept Med Surg & Hlth Sci, Trieste, Italy. RP Pascolo, L (reprint author), IRCCS Burlo Garofolo, Inst Maternal & Child Hlth, Trieste, Italy. EM lorella.pascolo@gmail.com OI Bedolla Orozco, Diana Eva/0000-0003-1902-1517; Borelli, Violetta/0000-0002-8166-3513; RIZZARDI, CLARA/0000-0003-2018-9835 FU Friuli Venezia Giulia Region -Commissione Amianto FVG; regional INAIL grant; ESRF FX The authors acknowledge a grant from Friuli Venezia Giulia Region -Commissione Amianto FVG - 2011 and a regional INAIL grant 2013, and ESRF for granting beamtimes (experiments MD 546; MD 710; MD 799). We thank Dr. Kevin Prince for a careful reading of the manuscript. NR 36 TC 3 Z9 3 U1 5 U2 16 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUL 10 PY 2015 VL 5 AR 12129 DI 10.1038/srep12129 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CM5HL UT WOS:000357717800001 PM 26159651 ER PT J AU Merkli, M Song, HF Berman, GP AF Merkli, Marco Song, Haifeng Berman, Gennady P. TI Multiscale dynamics of open three-level quantum systems with two quasi-degenerate levels SO JOURNAL OF PHYSICS A-MATHEMATICAL AND THEORETICAL LA English DT Article DE open quantum system; reduced dynamics; quasi degenerate energies; overlapping resonances; quasi stationary states ID ELECTRON-TRANSFER; MODEL; TEMPERATURE AB We consider a three-level quantum system interacting with a bosonic thermal reservoir. Two energy levels of the system are nearly degenerate but well separated from the third one. The system-reservoir interaction constant is larger than the energy difference of the degenerate levels, but it is smaller than the separation between the latter and the remaining level. We show that the quasi-degeneracy of energy levels leads to the existence of a manifold of quasi-stationary states, and the dynamics exhibits two characteristic time scales. On the first, shorter one, initial states approach the quasi-stationary manifold. Then, on the much longer second time scale, the final unique equilibrium is reached. C1 [Merkli, Marco; Song, Haifeng] Mem Univ Newfoundland, Dept Math & Stat, St John, NF A1C 5S7, Canada. [Berman, Gennady P.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87544 USA. [Berman, Gennady P.] New Mexico Consortium, Los Alamos, NM 87544 USA. RP Merkli, M (reprint author), Mem Univ Newfoundland, Dept Math & Stat, St John, NF A1C 5S7, Canada. EM merkli@mun.ca; song_haifeng@126.com; bgennady@newmexicoconsortium.org FU NSERC; Center for Nonlinear Studies of LANL FX M M and H S have been supported by NSERC through a Discovery Grant. M M is grateful for the hospitality and financial support of the Center for Nonlinear Studies of LANL, where part of this work was carried out. We are grateful to two anonymous referees for a very careful reading of our paper and for giving us valuable comments. NR 18 TC 3 Z9 3 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1751-8113 EI 1751-8121 J9 J PHYS A-MATH THEOR JI J. Phys. A-Math. Theor. PD JUL 10 PY 2015 VL 48 IS 27 AR 275304 DI 10.1088/1751-8113/48/27/275304 PG 25 WC Physics, Multidisciplinary; Physics, Mathematical SC Physics GA CK6MX UT WOS:000356343300008 ER PT J AU Bunn, JK Fang, RL Albing, MR Mehta, A Kramer, MJ Besser, MF Hattrick-Simpers, JR AF Bunn, Jonathan Kenneth Fang, Randy L. Albing, Mark R. Mehta, Apurva Kramer, Matthew J. Besser, Matthew F. Hattrick-Simpers, Jason R. TI A high-throughput investigation of Fe-Cr-Al as a novel high-temperature coating for nuclear cladding materials SO NANOTECHNOLOGY LA English DT Article DE high-throughput materials science; oxidation resistance; big data; in situ synchrotron diffraction; nuclear cladding materials ID X-RAY-DIFFRACTION; WATER-VAPOR; FLUORESCENCE SPECTROSCOPY; MATERIALS LIBRARIES; FECRAL ALLOY; OXIDATION; COMBINATORIAL; SCALES; IDENTIFICATION; BEHAVIOR AB High-temperature alloy coatings that can resist oxidation are urgently needed as nuclear cladding materials to mitigate the danger of hydrogen explosions during meltdown. Here we apply a combination of computationally guided materials synthesis, high-throughput structural characterization and data analysis tools to investigate the feasibility of coatings from the Fe-Cr-Al alloy system. Composition-spread samples were synthesized to cover the region of the phase diagram previous bulk studies have identified as forming protective oxides. The metallurgical and oxide phase evolution were studied via in situ synchrotron glancing incidence x-ray diffraction at temperatures up to 690 K. A composition region with an Al concentration greater than 3.08 at%, and between 20.0 at% and 32.9 at% Cr showed the least overall oxide growth. Subsequently, a series of samples were deposited on stubs and their oxidation behavior at 1373 K was observed. The continued presence of a passivating oxide was confirmed in this region over a period of 6 h. C1 [Bunn, Jonathan Kenneth; Fang, Randy L.; Albing, Mark R.; Hattrick-Simpers, Jason R.] Univ S Carolina, Dept Chem Engn, Columbia, SC 29208 USA. [Bunn, Jonathan Kenneth; Fang, Randy L.; Albing, Mark R.; Hattrick-Simpers, Jason R.] Univ S Carolina, Smart State Ctr Strateg Approaches Generat Elect, Columbia, SC 29208 USA. [Mehta, Apurva] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Kramer, Matthew J.; Besser, Matthew F.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. RP Bunn, JK (reprint author), Univ S Carolina, Dept Chem Engn, Columbia, SC 29208 USA. EM simpers@cec.sc.edu FU Critical Materials Institute, an Energy Innovation Hub - US Department of Energy (DOE), Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office; DOE [DE-AC02-07CH11358]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]; South Carolina Honors College Science Undergraduate Research Funding Program; South Carolina SmartState T center for Strategic Approaches to the Generation of Electricity (SAGE) FX This work is supported by the Critical Materials Institute, an Energy Innovation Hub funded by the US Department of Energy (DOE), Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office. The Ames Laboratory is operated by Iowa State University under DOE Contract No. DE-AC02-07CH11358. Use of the Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, is supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515. This work was supported in part by the South Carolina Honors College Science Undergraduate Research Funding Program (RLF). We would like to acknowledge the support of the South Carolina SmartState T center for Strategic Approaches to the Generation of Electricity (SAGE). NR 33 TC 5 Z9 5 U1 9 U2 46 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD JUL 10 PY 2015 VL 26 IS 27 AR 274003 DI 10.1088/0957-4484/26/27/274003 PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA CK7XH UT WOS:000356449100004 PM 26086841 ER PT J AU Bu, LT Himmel, ME Crowley, MF AF Bu, Lintao Himmel, Michael E. Crowley, Michael F. TI The molecular origins of twist in cellulose I-beta SO CARBOHYDRATE POLYMERS LA English DT Article DE Cellulose; Twist; Modeling; Dynamics; Microfibril; Cell wall ID SYNCHROTRON X-RAY; NEUTRON FIBER DIFFRACTION; HYDROGEN-BONDING SYSTEM; FORCE-FIELD; CRYSTALLINE CELLULOSE; DYNAMICS SIMULATIONS; MICROFIBRIL TWIST; CHARMM; ALPHA; ENERGETICS AB The observation of twisted microfibrils in cellulose I beta both in imaging and in molecular simulations has been reported and studied for years. This article reports a computational modeling study of cellulose I beta twist showing its strong dependence on fibril diameter and no dependence on fibril length. We report that an important contribution to the twist in the model, empirically and analytically, is the hydrogen bonding that spans the glycosidic linkage, and that the characteristics of the chiral centers involved in the trans-glycosidic-linkage hydrogen bonding determine the directions if those interactions and cause observed right-handed twist. Other crystalline forms of cellulose show evidence of twisting at the microfibril scale, but less than I beta. The minimal twist in other forms of cellulose was shown previously to be due to inter-layer hydrogen bonds; this study shows it is also partially due to the primary alcohol not occurring in the TG orientation in those forms. Thus, only cellulose I has the primary alcohol in TG orientation, which leads to formation of the twist-causing hydrogen bonds. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Himmel, Michael E.; Crowley, Michael F.] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA. [Bu, Lintao] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. RP Crowley, MF (reprint author), Natl Renewable Energy Lab, Biosci Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM Lintao.bu@NREL.gov; Mike.Himmel@NREL.gov; Michael.Crowley@NREL.gov FU Center for Direct Catalytic Conversion of Biomass to Biofuels (C3Bio), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0000997]; U.S. Department of Energy [DE-AC36-08-GO28308] FX This work was supported by the Center for Direct Catalytic Conversion of Biomass to Biofuels (C3Bio), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0000997. The National Renewable Energy Laboratory (NREL) is operated for the U.S. Department of Energy under Contract No. DE-AC36-08-GO28308. The authors acknowledge the generous allocation of computer time on the National Renewable Energy Laboratory (NREL) supercomputer, Peregrine, for all the MD simulations run for this manuscript. NR 45 TC 7 Z9 7 U1 3 U2 39 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0144-8617 EI 1879-1344 J9 CARBOHYD POLYM JI Carbohydr. Polym. PD JUL 10 PY 2015 VL 125 BP 146 EP 152 DI 10.1016/j.carbpol.2015.02.023 PG 7 WC Chemistry, Applied; Chemistry, Organic; Polymer Science SC Chemistry; Polymer Science GA CG8ZM UT WOS:000353604200017 PM 25857969 ER PT J AU Howe, A Chain, PSG AF Howe, Adina Chain, Patrick S. G. TI Challenges and opportunities in understanding microbial communities with metagenome assembly (accompanied by IPython Notebook tutorial) SO FRONTIERS IN MICROBIOLOGY LA English DT Review DE metagenomes; assembly; review; challenges; tutorial ID GENOMES; RECONSTRUCTION; ENVIRONMENT AB Metagenomic investigations hold great promise for informing the genetics, physiology, and ecology of environmental microorganisms. Current challenges for metagenomic analysis are related to our ability to connect the dots between sequencing reads, their population of origin, and their encoding functions. Assembly-based methods reduce dataset size by extending overlapping reads into larger contiguous sequences (contigs), providing contextual information for genetic sequences that does not rely on existing references. These methods, however, tend to be computationally intensive and are again challenged by sequencing errors as well as by genomic repeats While numerous tools have been developed based on these methodological concepts, they present confounding choices and training requirements to metagenomic investigators. To help with accessibility to assembly tools, this review also includes an IPython Notebook metagenomic assembly tutorial. This tutorial has instructions for execution any operating system using Amazon Elastic Cloud Compute and guides users through downloading, assembly, and mapping reads to contigs of a mock microbiome metagenome. Despite its challenges, metagenomic analysis has already revealed novel insights into many environments on Earth. As software, training, and data continue to emerge, metagenomic data access and its discoveries will to grow. C1 [Howe, Adina] Iowa State Univ, Dept Agr & Biosyst Engn, GERMS Lab, Ames, IA 50011 USA. [Chain, Patrick S. G.] Los Alamos Natl Lab, Biosci Div, Bioinformat & Analyt Team, Los Alamos, NM USA. RP Howe, A (reprint author), Iowa State Univ, Dept Agr & Biosyst Engn, GERMS Lab, 3346 Flings Hall, Ames, IA 50011 USA. EM adina@iastate.edu OI Chain, Patrick/0000-0003-3949-3634 NR 32 TC 5 Z9 5 U1 6 U2 43 PU FRONTIERS RESEARCH FOUNDATION PI LAUSANNE PA PO BOX 110, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD JUL 9 PY 2015 VL 6 AR 678 DI 10.3389/fmicb.2015.00678 PG 4 WC Microbiology SC Microbiology GA CN4EW UT WOS:000358384100001 PM 26217314 ER PT J AU Cohen, MF Gurung, S Birarda, G Holman, HYN Yamasaki, H AF Cohen, Michael F. Gurung, Sushma Birarda, Giovanni Holman, Hoi-Ying N. Yamasaki, Hideo TI Bimodal effect of hydrogen peroxide and oxidative events in nitrite-induced rapid root abscission by the water fern Azolla pinnata SO FRONTIERS IN PLANT SCIENCE LA English DT Article DE root abscission; apoplast; free radical cleavage; FTIR spectromicroscopy; hydrogen peroxide; nitric oxide; nitrite; plant cell wall loosening ID HYDROXYL RADICALS; IN-VITRO; ELONGATION GROWTH; CELLS; OXIDE; VIVO; POLYSACCHARIDES; GENERATION; SEPARATION; CHEMISTRY AB In the genus Azolla rapid abscission of roots from floating fronds occurs within minutes in response to a variety of stresses, including exposure to nitrite. We found that hydrogen peroxide, though itself not an inducer of root abscission, modulates nitrite-induced root abscission by Azolla pinnata in a dose-dependent manner, with 2 mM H2O2 significantly diminishing the responsiveness to 2 mM NaNO2, and 10 mM H2O2 slightly enhancing it. Hypoxia, which has been found in other plants to result in autogenic production of H2O2, dramatically stimulated root abscission of A. pinnata in response to nitrite, especially for plants previously cultivated in medium containing 5 mM KNO3 compared to plants cultivated under N-2-fixing conditions without combined nitrogen. Plants, including Azolla, produce the small signaling molecule nitric oxide (NO) from nitrite using nitrate reductase. We found Azolla plants to display dose-dependent root abscission in response to the NO donor spermine NONOate. Treatment of plants with the thiol-modifying agents S-methyl methanethiosulfonate or glutathione inhibited the nitrite-induced root abscission response. Synchrotron radiation-based Fourier transform infrared spectromicroscopy revealed higher levels of carbonylation in the abscission zone of dropped roots, indicative of reaction products of polysaccharides with potent free radical oxidants. We hypothesize that metabolic products of nitrite and NO react with H2O2 in the apoplast leading to free-radical-mediated cleavage of structural polysaccharides and consequent rapid root abscission. C1 [Cohen, Michael F.] Sonoma State Univ, Dept Biol, Rohnert Pk, CA 94928 USA. [Cohen, Michael F.] Okinawa Inst Sci & Technol, Biol Syst Unit, Onna, Okinawa, Japan. [Gurung, Sushma; Yamasaki, Hideo] Univ Ryukyus, Fac Sci, Nishihara, Okinawa 90301, Japan. [Birarda, Giovanni; Holman, Hoi-Ying N.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Ctr Environm Biotechnol, Berkeley, CA 94720 USA. RP Cohen, MF (reprint author), Sonoma State Univ, Dept Biol, 1801 East Cotati Ave, Rohnert Pk, CA 94928 USA. EM cohenm@sonoma.edu RI Holman, Hoi-Ying/N-8451-2014 OI Holman, Hoi-Ying/0000-0002-7534-2625 FU Berkeley Synchrotron Infrared Structural Biology (BSISB) Program; U.S. Department of Energy Office of Biological and Environmental Research (DOE/BER); Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank Jon Fukuto, My Vu Ngyuen, Tamas Torok, and Naoko Watanabe for technical assistance. Support for this work was provided in part by the Berkeley Synchrotron Infrared Structural Biology (BSISB) Program which is funded by the U.S. Department of Energy Office of Biological and Environmental Research (DOE/BER). The Advanced Light Source is supported by the Director, Office of Science of the U.S. Department of Energy under contract No. DE-AC02-05CH11231. NR 40 TC 0 Z9 0 U1 1 U2 7 PU FRONTIERS RESEARCH FOUNDATION PI LAUSANNE PA PO BOX 110, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. PD JUL 9 PY 2015 VL 6 AR 518 DI 10.3389/fpls.2015.00518 PG 8 WC Plant Sciences SC Plant Sciences GA CN4WJ UT WOS:000358430900002 PM 26217368 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Ochesanu, S Rougny, R Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Van Parijs, I Barria, P Caillol, C Clerbaux, B De Lentdecker, G Delannoy, H Dobur, D Fasanella, G Favart, L Gay, APR Grebenyuk, A Leonard, A Mohammadi, A Pernie, L Randleconde, A Reis, T Seva, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Zenoni, F Beernaert, K Benucci, L Cimmino, A Crucy, S Fagot, A Garcia, G Gul, M Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Diblen, SS Sigamani, M Strobbe, N Thyssen, F Tytgat, M Van Driessche, W Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bondu, O Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Mertens, A Nuttens, C Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Beliy, N Hammad, GH Alda, WL Alves, GA Brito, L Martins, MC Martins, TD Hensel, C Herrera, CM Moraes, A Pol, ME Teles, PR Das Chagas, EBB Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Guativa, LMH Malbouisson, H Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santaolalla, J Santoro, A Sznajder, A Manganote, EJT Pereira, AV Ahuja, S Bernardes, CA Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Novaes, SF Padula, SS Abad, DR Vargas, JCR Aleksandrov, A Genchev, V Hadjiiska, R Iaydjiev, P Marinov, A Piperov, S Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Ahmad, M Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Plestina, R Romeo, F Shaheen, SM Tao, J Wang, C Wang, Z Asawatangtrakuldee, C Ban, Y Chen, G Li, Q Liu, S Mao, Y Qian, SJ Wang, D Wang, M Wang, Q Xu, Z Yang, D Zhang, F Zhang, L Zhang, Z Zou, W Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Bodlak, M Finger, M Finger, M Ali, A Aly, R Aly, S Elgammal, S Kamel, AE Lotfy, A Mahmoud, MA Masod, R Radi, A Calpas, B Kadastik, M Murumaa, M Raidal, M Tiko, A Veelken, C Eerola, P Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Talvitie, J Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Favaro, C Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Rander, J Rosowsky, A Titov, M Zghiche, A Baffioni, S Beaudette, F Busson, P Cadamuro, L Chapon, E Charlot, C Dahms, T Davignon, O Filipovic, N Florent, A de Cassagnac, RG Mastrolorenzo, L Mine, P Naranjo, IN Nguyen, M Ochando, C Ortona, G Paganini, P Regnard, S Salerno, R Sauvan, JB Sirois, Y Strebler, T Yilmaz, Y Zabi, A Agram, JL Andrea, J Aubin, A Bloch, D Brom, JM Buttignol, M Chabert, EC Chanon, N Collard, C Conte, E Fontaine, JC Gele, D Goerlach, U Goetzmann, C Le Bihan, AC Merlin, JA Skovpen, K Van Hove, P Gadrat, S Beauceron, S Beaupere, N Bernet, C Boudoul, G Bouvier, E Brochet, S Montoya, CAC Chasserat, J Chierici, R Contardo, D Courbon, B Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Laktineh, IB Lethuillier, M Mirabito, L Pequegnot, AL Perries, S Alvarez, JDR Sabes, D Sgandurra, L Sordini, V Vander Donckt, M Verdier, P Viret, S Xiao, H Lomidze, D Autermann, C Beranek, S Bontenackels, M Edelhoff, M Feld, L Heister, A Kiesel, MK Klein, K Lipinski, M Ostapchuk, A Preuten, M Raupach, F Sammet, J Schael, S Schulte, JF Verlage, T Weber, H Wittmer, B Zhukov, V Ata, M Brodski, M Dietz-Laursonn, E Duchardt, D Endres, M Erdmann, M Erdweg, S Esch, T Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Millet, P Olschewski, M Padeken, K Papacz, P Pook, T Radziej, M Reithler, H Rieger, M Schmitz, SA Sonnenschein, L Teyssier, D Thur, S Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Ahmad, WH Hoehle, F Kargoll, B Kress, T Kuessel, Y Kunsken, A Lingemann, J Nowack, A Nugent, IM Pistone, C Pooth, O Stahl, A Martin, MA Asin, I Bartosik, N Behnke, O Behrens, U Bell, AJ Borras, K Burgmeier, A Cakir, A Calligaris, L Campbell, A Choudhury, S Costanza, F Pardos, CD Dolinska, G Dooling, S Dorland, T Eckerlin, G Eckstein, D Eichhorn, T Flucke, G Garcia, JG Geiser, A Gizhko, A Gunnellini, P Hauk, J Hempel, M Jung, H Kalogeropoulos, A Karacheban, O Kasemann, M Katsas, P Kieseler, J Kleinwort, C Korol, I Lange, W Leonard, J Lipka, K Lobanov, A Mankel, R Marfin, I Melzer-Pellmann, IA Meyer, AB Mittag, G Mnich, J Mussgiller, A Naumann-Emme, S Nayak, A Ntomari, E Perrey, H Pitzl, D Placakyte, R Raspereza, A Cipriano, PMR Roland, B Sahin, MO Salfeld-Nebgen, J Saxena, P Schoerner-Sadenius, T Schroder, M Seitz, C Spannagel, S Wissing, C Blobel, V Vignali, MC Draeger, AR Erfle, J Garutti, E Goebel, K Gonzalez, D Gorner, M Haller, J Hoffmann, M Hoing, RS Junkes, A Kirschenmann, H Klanner, R Kogler, R Lapsien, T 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CA CMS Collaboration TI Search for third-generation scalar leptoquarks in the t tau channel in proton-proton collisions at root s=8 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering; Beyond Standard Model ID CROSS-SECTION; ASSOCIATION; FORCES; UNITY; BOSON; PAIR AB A search for pair production of third-generation scalar leptoquarks decaying to top quark and tau lepton pairs is presented using proton-proton collision data at a center-of-mass energy of root s=8TeV collected with the CMS detector at the LHC and corresponding to an integrated luminosity of 19.7 fb(-1). The search is performed using events that contain an electron or a muon, a hadronically decaying tau lepton, and two or more jets. The observations are found to be consistent with the standard model predictions. Assuming that all leptoquarks decay to a top quark and a tau lepton, the existence of pair produced, charge -1/3, third-generation leptoquarks up to a mass of 685 GeV is excluded at 95% confidence level. This result constitutes the first direct limit for leptoquarks decaying into a top quark and a tau lepton, and may also be applied directly to the pair production of bottom squarks decaying predominantly via the R-parity violating coupling lambda'(333) . C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hartl, C.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Knuenz, V.; Koenig, A.; Krammer, M.; Kraetschmer, I.; Liko, D.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, H.; Schieck, J.; Schoefbeck, R.; Strauss, J.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] Inst Hochenergiephys OeAW, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. [Alderweireldt, S.; Cornelis, T.; De Wolf, E. A.; Janssen, X.; Knutsson, A.; Lauwers, J.; Luyckx, S.; Ochesanu, S.; Rougny, R.; Van De Klundert, M.; Van Haevermaet, H.; Van Mechelen, P.; Van Remortel, N.; Van Spilbeeck, A.] Univ Antwerp, Antwerp, Belgium. [Abu Zeid, S.; Blekman, F.; D'Hondt, J.; Daci, N.; De Bruyn, I.; Deroover, K.; Heracleous, N.; Keaveney, J.; Lowette, S.; Moreels, L.; Olbrechts, A.; Python, Q.; Strom, D.; Tavernier, S.; Van Doninck, W.; Van Mulders, P.; Van Onsem, G. P.; Van Parijs, I.] Vrije Univ Brussel, Brussels, Belgium. [Barria, P.; Caillol, C.; Clerbaux, B.; De Lentdecker, G.; Delannoy, H.; Dobur, D.; Fasanella, G.; Favart, L.; Gay, A. P. R.; Grebenyuk, A.; Leonard, A.; Mohammadi, A.; Pernie, L.; Randleconde, A.; Reis, T.; Seva, T.; Thomas, L.; Vander Velde, C.; Vanlaer, P.; Wang, J.; Zenoni, F.] Univ Libre Bruxelles, Brussels, Belgium. [Beernaert, K.; Benucci, L.; Cimmino, A.; Crucy, S.; Fagot, A.; Garcia, G.; Gul, M.; Mccartin, J.; Rios, A. A. Ocampo; Poyraz, D.; Ryckbosch, D.; Diblen, S. Salva; Sigamani, M.; Strobbe, N.; Thyssen, F.; Tytgat, M.; Van Driessche, W.; Yazgan, E.; Zaganidis, N.] Univ Ghent, B-9000 Ghent, Belgium. [Basegmez, S.; Beluffi, C.; Bondu, O.; Bruno, G.; Castello, R.; Caudron, A.; Ceard, L.; Da Silveira, G. G.; Delaere, C.; du Pree, T.; Favart, D.; Forthomme, L.; Giammanco, A.; Hollar, J.; Jafari, A.; Jez, P.; Komm, M.; Lemaitre, V.; Mertens, A.; Nuttens, C.; Perrini, L.; Pin, A.; Piotrzkowski, K.; Popov, A.; Quertenmont, L.; Selvaggi, M.; Marono, M. Vidal] Catholic Univ Louvain, Louvain, Belgium. [Beliy, N.; Hammad, G. H.] Univ Mons, B-7000 Mons, Belgium. [Alda Junior, W. L.; Alves, G. A.; Brito, L.; Correa Martins Junior, M.; Dos Reis Martins, T.; Hensel, C.; Mora Herrera, C.; Moraes, A.; Pol, M. E.; Rebello Teles, P.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. [Belchior Batista Das Chagas, E.; Carvalho, W.; Chinellato, J.; Custodio, A.; Da Costa, E. M.; De Jesus Damiao, D.; De Oliveira Martins, C.; Fonseca De Souza, S.; Huertas Guativa, L. M.; Malbouisson, H.; Matos Figueiredo, D.; Mundim, L.; Nogima, H.; Prado Da Silva, W. L.; Santaolalla, J.; Santoro, A.; Sznajder, A.; Tonelli Manganote, E. J.; Vilela Pereira, A.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Dogra, S.; Fernandez Perez Tomei, T. R.; Novaes, S. F.; Padula, Sandra S.] Univ Estadual Paulista, Sao Paulo, Brazil. [Bernardes, C. A.; Gregores, E. M.; Mercadante, P. G.] Univ Fed ABC, Sao Paulo, Brazil. [Aleksandrov, A.; Genchev, V.; Hadjiiska, R.; Iaydjiev, P.; Marinov, A.; Piperov, S.; Rodozov, M.; Stoykova, S.; Sultanov, G.; Vutova, M.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy, Sofia, Bulgaria. [Dimitrov, A.; Glushkov, I.; Litov, L.; Pavlov, B.; Petkov, P.] Univ Sofia, BU-1126 Sofia, Bulgaria. [Ahmad, M.; Bian, J. G.; Chen, G. M.; Chen, H. S.; Chen, M.; Cheng, T.; Du, R.; Jiang, C. H.; Plestina, R.; Romeo, F.; Shaheen, S. M.; Tao, J.; Wang, C.; Wang, Z.] Inst High Energy Phys, Beijing 100039, Peoples R China. [Asawatangtrakuldee, C.; Ban, Y.; Chen, G.; Li, Q.; Liu, S.; Mao, Y.; Qian, S. J.; Wang, D.; Wang, M.; Wang, Q.; Xu, Z.; Yang, D.; Zhang, F.; Zhang, L.; Zhang, Z.; Zou, W.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Avila, C.; Cabrera, A.; Chaparro Sierra, L. F.; Florez, C.; Gomez, J. P.; Gomez Moreno, B.; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia. [Godinovic, N.; Lelas, D.; Polic, D.; Puljak, I.] Univ Split, Fac Elect Engn Mech Engn & Naval Architecture, Split, Croatia. [Antunovic, Z.; Kovac, M.] Univ Split, Fac Sci, Split, Croatia. [Brigljevic, V.; Kadija, K.; Luetic, J.; Sudic, L.] Rudjer Boskovic Inst, Zagreb, Croatia. [Attikis, A.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.; Rykaczewski, H.] Univ Cyprus, Nicosia, Cyprus. [Bodlak, M.; Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic. [Ali, A.; Aly, R.; Aly, S.; Elgammal, S.; Kamel, A. Ellithi; Lotfy, A.; Mahmoud, M. A.; Masod, R.; Radi, A.] Acad Sci Res & Technol Arab Republ Egypt, Egyptian Network High Energy Phys, Cairo, Egypt. [Giammanco, A.; Calpas, B.; Kadastik, M.; Murumaa, M.; Raidal, M.; Tiko, A.; Veelken, C.] NICPB, Tallinn, Estonia. [Eerola, P.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Harkonen, J.; Karimaki, V.; Kinnunen, R.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Talvitie, J.; Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Couderc, F.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Favaro, C.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Malcles, J.; Rander, J.; Rosowsky, A.; Titov, M.; Zghiche, A.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Baffioni, S.; Beaudette, F.; Busson, P.; Cadamuro, L.; Chapon, E.; Charlot, C.; Dahms, T.; Davignon, O.; Filipovic, N.; Florent, A.; de Cassagnac, R. Granier; Mastrolorenzo, L.; Mine, P.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Ortona, G.; Paganini, P.; Regnard, S.; Salerno, R.; Sauvan, J. 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Ruiz; Sabes, D.; Sgandurra, L.; Sordini, V.; Vander Donckt, M.; Verdier, P.; Viret, S.; Xiao, H.] Univ Lyon 1, CNRS IN2P3, Inst Phys Nucl Lyon, F-69622 Villeurbanne, France. [Lomidze, D.] Tbilisi State Univ, Inst High Energy Phys & Informatizat, GE-380086 Tbilisi, Rep of Georgia. [Autermann, C.; Beranek, S.; Bontenackels, M.; Edelhoff, M.; Feld, L.; Heister, A.; Kiesel, M. K.; Klein, K.; Lipinski, M.; Ostapchuk, A.; Preuten, M.; Raupach, F.; Sammet, J.; Schael, S.; Schulte, J. F.; Verlage, T.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Ata, M.; Brodski, M.; Dietz-Laursonn, E.; Duchardt, D.; Endres, M.; Erdmann, M.; Erdweg, S.; Esch, T.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Millet, P.; Olschewski, M.; Padeken, K.; Papacz, P.; Pook, T.; Radziej, M.; Reithler, H.; Rieger, M.; Schmitz, S. A.; Sonnenschein, L.; Teyssier, D.; Thuer, S.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Kunsken, A.; Lingemann, J.; Nowack, A.; Nugent, I. M.; Pistone, C.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B 3, Aachen, Germany. [Martin, M. Aldaya; Asin, I.; Bartosik, N.; Behnke, O.; Behrens, U.; Bell, A. J.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. Diez; Dolinska, G.; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Garcia, J. Garay; Geiser, A.; Gizhko, A.; Gunnellini, P.; Hauk, J.; Hempel, M.; Jung, H.; Kalogeropoulos, A.; Karacheban, O.; Kasemann, M.; Katsas, P.; Kieseler, J.; Kleinwort, C.; Korol, I.; Lange, W.; Leonard, J.; Lipka, K.; Lobanov, A.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mittag, G.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Nayak, A.; Ntomari, E.; Perrey, H.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Cipriano, P. M. Ribeiro; Roland, B.; Sahin, M. Oe.; Salfeld-Nebgen, J.; Saxena, P.; Schoerner-Sadenius, T.; Schroeder, M.; Seitz, C.; Spannagel, S.; Wissing, C.] DESY, Hamburg, Germany. [Blobel, V.; Vignali, M. Centis; Draeger, A. R.; Erfle, J.; Garutti, E.; Goebel, K.; Gonzalez, D.; Goerner, M.; Haller, J.; Hoffmann, M.; Hoeing, R. S.; Junkes, A.; Kirschenmann, H.; Klanner, R.; Kogler, R.; Lapsien, T.; Lenz, T.; Marchesini, I.; Marconi, D.; Meyer, M.; Nowatschin, D.; Ott, J.; Peiffer, T.; Perieanu, A.; Pietsch, N.; Poehlsen, J.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Seidel, M.; Sola, V.; Stadie, H.; Steinbrueck, G.; Tholen, H.; Troendle, D.; Usai, E.; Vanelderen, L.; Vanhoefer, A.] Univ Hamburg, Hamburg, Germany. [Akbiyik, M.; Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; Colombo, F.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Frensch, F.; Giffels, M.; Gilbert, A.; Hartmann, F.; Husemann, U.; Katkov, I.; Kornmayer, A.; Pardo, P. Lobelle; Mozer, M. U.; Mueller, T.; Mueller, Th.; Plagge, M.; Quast, G.; Rabbertz, K.; Roecker, S.; Roscher, F.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Woehrmann, C.; Wolf, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Markou, A.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, Inst Nucl & Particle Phys INPP, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Tziaferi, E.] Univ Athens, Athens, Greece. [Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Loukas, N.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hazi, A.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Bartok, M.; Makovec, A.; Raics, P.; Trocsanyi, Z. L.] Univ Debrecen, Debrecen, Hungary. [Mal, P.; Mandal, K.; Sahoo, N.; Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Bansal, S.; Beri, S. B.; Bhatnagar, V.; Chawla, R.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, A.; Kaur, M.; Kumar, R.; Mehta, A.; Mittal, M.; Nishu, N.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Bhardwaj, A.; Choudhary, B. C.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Sharma, R.; Sharma, V.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dey, S.; Dutta, S.; Gomber, B.; Jain, Sa.; Jain, Sh.; Khurana, R.; Majumdar, N.; Modak, A.; Mondal, K.; Mukherjee, S.; Mukhopadhyay, S.; Roy, A.; Roy, D.; Chowdhury, S. Roy; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Jha, V.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Mumbai 400085, Maharashtra, India. [Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Sur, N.; Sutar, B.; Wickramage, N.] Tata Inst Fundamental Res, Mumbai 400005, Maharashtra, India. [Sharma, S.] Indian Inst Sci Educ & Res IISER, Pune, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Ranieri, A.; Selvaggi, G.; Sharma, A.; Silvestris, L.; Venditti, R.; Verwilligen, P.] INFN Sez Bari, Bari, Italy. [Abbrescia, M.; Calabria, C.; Caputo, C.; Chhibra, S. S.; Cristella, L.; De Palma, M.; Miniello, G.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Battilana, C.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] INFN Sez Bologna, Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] INFN Sez Catania, Catania, Italy. [Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Giordano, F.] CSFNSM, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.; Viliani, L.] INFN Sez Firenze, Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.; Viliani, L.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.] INFN Lab Nazl Frascati, Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Robutti, E.; Tosi, S.] INFN Sez Genova, Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] INFN Sez Milano Bicocca, Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.] INFN Sez Napoli, Naples, Italy. [Esposito, M.; Iorio, A. O. M.; Sciacca, C.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, I-85100 Potenza, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; De Oliveira, A. Carvalho Antunes; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Montecassiano, F.; Passaseo, M.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] INFN Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; De Oliveira, A. Carvalho Antunes; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. Univ Trento, Trento, Italy. [Gabusi, M.; Magnani, A.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] INFN Sez Pavia, Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Solestizi, L. Alunni; Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] INFN Sez Perugia, Perugia, Italy. [Solestizi, L. Alunni; Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fedi, G.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] INFN Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Fiori, F.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Soffi, L.; Traczyk, P.] INFN Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Micheli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Covarelli, R.; De Remigis, P.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Roberts, J.] INFN Sez Torino, Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Pacher, L.; Angioni, G. L. Pinna; Romero, A.; Sacchi, R.; Solano, A.] Univ Torino, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.; Zanetti, A.] INFN Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.; Zanetti, A.] Univ Trieste, Trieste, Italy. [Chang, S.; Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Daegu, South Korea. [Kim, H.; Kim, T. J.; Ryu, M. S.] Chonbuk Natl Univ, Jeonju, South Korea. [Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Lee, S.; Kim, H.; Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Jo, M.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.; Vaitkus, J.] Vilnius Univ, Vilnius, Lithuania. [Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Ramirez Sanchez, G.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Carpinteyro, S.; Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Ahmad, A.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Toriashvili, T.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Baskakov, A.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Lokhtin, I.; Myagkov, I.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; Duarte Campderros, J.; Gomez, G.; Graziano, A.; Lopez Virto, A.; Marco, J.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Vila, I.] CSIC Univ Cantabria, Inst Fis Cantabria IFCA, Santander, Spain. [Rabady, D.; Genchev, V.; Merlin, J. A.; Boudoul, G.; Lingemann, J.; Hartmann, F.; Kornmayer, A.; Mohanty, A. K.; Radogna, R.; Silvestris, L.; Giordano, F.; Gennai, S.; Lucchini, M. T.; Marzocchi, B.; Di Guida, S.; Meola, S.; Paolucci, P.; Azzi, P.; Ciangottini, D.; Spiezia, A.; Donato, S.; Traczyk, P.; Finco, L.; Candelise, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Marrouche, J.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Zagozdzinska, A.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Abdulsalam, A.; Bachmair, F.; Baeni, L.; Bianchini, L.; Buchmann, M. A.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marini, A. C.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Mohr, N.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Peruzzi, M.; Quittnat, M.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.; Weber, H. A.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Salerno, D.; Taroni, S.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Ferro, C.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.; Wilken, R.] Natl Taiwan Univ NTU, Taipei, Taiwan. [Asavapibhop, B.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Cerci, S.; Dozen, C.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Tali, B.; Topakli, H.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Albayrak, E. A.; Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Gunaydin, Y. O.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Ball, F.; Beck, L.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Heath, G. P.; Heath, H. F.; Jacob, J.; Lucas, C.; Newbold, D. M.; Poll, A.; Smith, D.] Univ Bristol, Bristol, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Citron, M.; Colling, D.; Corpe, L.; Cripps, N.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Sharp, P.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Pastika, N.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Cutts, D.; Demiragli, Z.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Sagir, S.; Sinthuprasith, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Saltzberg, D.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Rikova, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Sumowidagdo, S.; Wei, H.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Kovalskyi, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Justus, C.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Smith, J. G.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Skinnari, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Hu, Z.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Kwan, S.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Whitbeck, A.; Yang, F.; Yin, H.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Di Giovanni, G. P.; Field, R. D.; Fisher, M.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Kypreos, T.; Low, J. F.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rank, D.; Rinkevicius, A.; Shchutska, L.; Snowball, M.; Sperka, D.; Wang, S. J.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Bhopatkar, V.; Hohlmann, M.; Kalakhety, H.; Mareskas-palcek, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.] Univ Illinois, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Sen, S.; Snyder, C.; Tan, P.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Abdulsalam, A.; Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Nash, K.; Osherson, M.; Swartz, M.; Xiao, M.; Xin, Y.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Gray, J.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Chakaberia, I.; Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Skhirtladze, N.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Abdulsalam, A.; Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Mignerey, A. C.; Pedro, K.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Baty, A.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Mcginn, C.; Niu, X.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Sumorok, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Finkel, A.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Nourbakhsh, S.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. 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RI Ogul, Hasan/S-7951-2016; ciocci, maria agnese /I-2153-2015; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Paulini, Manfred/N-7794-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Stahl, Achim/E-8846-2011; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Sznajder, Andre/L-1621-2016; Vilela Pereira, Antonio/L-4142-2016; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Horani, Hafeez /L-2414-2015; Calvo Alamillo, Enrique/L-1203-2014; Flix, Josep/G-5414-2012; Hernandez Calama, Jose Maria/H-9127-2015; Cerrada, Marcos/J-6934-2014; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Novaes, Sergio/D-3532-2012; Della Ricca, Giuseppe/B-6826-2013; Chinellato, Jose Augusto/I-7972-2012; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Vinogradov, Alexey/O-2375-2015; Petrushanko, Sergey/D-6880-2012; Cakir, Altan/P-1024-2015; Montanari, Alessandro/J-2420-2012; Matorras, Francisco/I-4983-2015; Gennai, Simone/P-2880-2015; TUVE', Cristina/P-3933-2015; Dudko, Lev/D-7127-2012; KIM, Tae Jeong/P-7848-2015; Menasce, Dario/A-2168-2016; Paganoni, Marco/A-4235-2016; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Lo Vetere, Maurizio/J-5049-2012; Moraes, Arthur/F-6478-2010; Manganote, Edmilson/K-8251-2013; Lokhtin, Igor/D-7004-2012; Fano, Livio/K-2460-2015; Grandi, Claudio/B-5654-2015; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; VARDARLI, Fuat Ilkehan/B-6360-2013; Hoorani, Hafeez/D-1791-2013; Dogra, Sunil /B-5330-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015 OI Ogul, Hasan/0000-0002-5121-2893; ciocci, maria agnese /0000-0003-0002-5462; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Stahl, Achim/0000-0002-8369-7506; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Seixas, Joao/0000-0002-7531-0842; Sznajder, Andre/0000-0001-6998-1108; Vilela Pereira, Antonio/0000-0003-3177-4626; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Calvo Alamillo, Enrique/0000-0002-1100-2963; Flix, Josep/0000-0003-2688-8047; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Cerrada, Marcos/0000-0003-0112-1691; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; Chinellato, Jose Augusto/0000-0002-3240-6270; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Montanari, Alessandro/0000-0003-2748-6373; Matorras, Francisco/0000-0003-4295-5668; TUVE', Cristina/0000-0003-0739-3153; Dudko, Lev/0000-0002-4462-3192; KIM, Tae Jeong/0000-0001-8336-2434; Menasce, Dario/0000-0002-9918-1686; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Lo Vetere, Maurizio/0000-0002-6520-4480; Moraes, Arthur/0000-0002-5157-5686; Fano, Livio/0000-0002-9007-629X; Grandi, Claudio/0000-0001-5998-3070; Rovelli, Tiziano/0000-0002-9746-4842; FU BMWFW (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia); ERC IUT (Estonia); ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP (Republic of Korea); NRF (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (U.S.A.); NSF (U.S.A.); Marie-Curie program (European Union); European Research Council (European Union); EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS program of the Foundation for Polish Science; European Union, Regional Development Fund; Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR project (Italy) [20108T4XTM]; Thalis program - EU-ESF; Aristeia program - EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP and NRF (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (U.S.A.).; Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF; and the National Priorities Research Program by Qatar National Research Fund. NR 61 TC 12 Z9 12 U1 8 U2 55 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JUL 9 PY 2015 IS 7 AR 042 DI 10.1007/JHEP07(2015)042 PG 44 WC Physics, Particles & Fields SC Physics GA CM8ET UT WOS:000357931600001 ER PT J AU Bao, J Xu, W Bhattacharya, P Stewart, M Zhang, JG Pan, WX AF Bao, Jie Xu, Wu Bhattacharya, Priyanka Stewart, Mark Zhang, Ji-Guang Pan, Wenxiao TI Discharge Performance of Li-O-2 Batteries Using a Multiscale Modeling Approach SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID LITHIUM AIR BATTERIES; ELECTROLYTE FUEL-CELLS; LI-ION BATTERY; 3-DIMENSIONAL MICROSTRUCTURE; CATHODE MICROSTRUCTURE; TRANSPORT-PROPERTIES; OXYGEN BATTERIES; LI/AIR BATTERIES; CATALYST LAYERS; MECHANISMS AB To study the discharge performance of Li-O-2 batteries, we propose a multiscale modeling framework that links models in an upscaling fashion from the nanoscale to mesoscale and finally to the device scale. We have effectively reconstructed the microstructure of a Li-O-2 air electrode in silico, conserving the porosity, surface-to-volume ratio, and pore size distribution of the real air electrode structure. The mechanism of rate-dependent morphology of Li2O2 growth is incorporated into the mesoscale model. The correlation between the active-surface-to-volume ratio and averaged Li2O2 concentration is derived to link different scales. The proposed approach's accuracy is first demonstrated by comparing the predicted discharge curves of Li-O-2 batteries with experimental results at the high current density. Next, the validated modeling approach effectively captures the significant improvement in discharge capacity due to the formation of Li2O2 particles. Finally, it predicts the discharge capacities of Li-O-2 batteries with different air electrode microstructure designs and operating conditions. C1 [Pan, Wenxiao] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. [Bao, Jie; Xu, Wu; Bhattacharya, Priyanka; Stewart, Mark; Zhang, Ji-Guang] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. RP Zhang, JG (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. EM jiguang.zhang@pnnl.gov; wenxiao.pan@pnnl.gov FU Applied Mathematics Program within the U.S. Department of Energy (DOE), Office of Advanced Scientific Computing Research (ASCR) as part of the Collaboratory on Mathematics for Mesoscopic Modeling of Materials [CM4]; DOE's Energy Efficiency and Renewable Energy, Office of Vehicle Technology; Linus Pauling Distinguished Postdoctoral Fellowship at Pacific Northwest National Laboratory (PNNL); DOE [DE-AC05-76RL01830] FX W. Pan and J. Bao were supported by the Applied Mathematics Program within the U.S. Department of Energy (DOE), Office of Advanced Scientific Computing Research (ASCR) as part of the Collaboratory on Mathematics for Mesoscopic Modeling of Materials (CM4). W. Xu and J.-G. Zhang acknowledge financial support from the Assistant Secretary of DOE's Energy Efficiency and Renewable Energy, Office of Vehicle Technology. P. Bhattacharya is grateful for support from a Linus Pauling Distinguished Postdoctoral Fellowship at Pacific Northwest National Laboratory (PNNL). PNNL is operated by Battelle for the DOE under Contract DE-AC05-76RL01830. The finite volume code was adapted from the massive parallel computational fluid dynamics (CFD) program, ParaFlow, developed and provided by David Rector and Mark Stewart. W. Pan additionally thanks Xiaoliang Wei and Eduard Nasybulin for their valuable advice and helpful discussions about this work. NR 49 TC 1 Z9 1 U1 3 U2 45 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 9 PY 2015 VL 119 IS 27 BP 14851 EP 14860 DI 10.1021/acs.jpcc.5b01441 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CM8PU UT WOS:000357964900005 ER PT J AU Shkrob, IA Wishart, JF Abraham, DP AF Shkrob, Ilya A. Wishart, James F. Abraham, Daniel P. TI What Makes Fluoroethylene Carbonate Different? SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID LI-ION BATTERIES; ELECTRON-SPIN-RESONANCE; PICOSECOND PULSE-RADIOLYSIS; THIN-FILM ELECTRODE; PROPYLENE CARBONATE; SI ANODES; REDUCTION-MECHANISMS; SILICON ELECTRODES; ETHYLENE CARBONATE; GRAPHITE ANODES AB Rechargeable lithium-ion batteries containing silicon-based negative electrodes have the potential to revolutionize electrical energy storage, but the cyclic and acyclic organic carbonate solvents (such as ethylene and propylene carbonates) that are commonly used in graphite Li-ion batteries yield unsatisfactory performance when used with such Li alloying electrodes. It has been found by trial and error that additions of the closely related carbonate additive, fluoroethylene carbonate (FEC), to conventional electrolytes yields a robust solid electrolyte interphase (SEI) on the LixSiy alloy surface. Several mechanisms for this protective action have been considered in the literature and modeled theoretically; however, at present these mechanisms remain hypothetical. In this study, we use radiolysis, laser photoionization, electron paramagnetic resonance, and transient absorption spectroscopy to establish the redox chemistry of FEC. While the oxidation chemistry is similar to that of other organic carbonates, the reduction chemistry of the fluorinated molecule is strikingly different. Specifically, one-electron reduction of bulk FEC causes the fission of two (instead of one) C-O bonds, resulting in concerted defluorination and decarboxylation; in contrast, the reduction of the ethylene and propylene carbonate results in ring-opening and the formation of a radical anion. For FEC, the reduction yields the vinoxyl radical that can abstract an H atom from another FEC molecule, initiating both the chain reaction causing FEC decomposition and radical polymerization involving the reaction products. The resulting polymer can further defluorinate yielding the interior radicals that migrate and recombine to produce a highly cross-linked network This feature implies that the outer SEI resulting from FEC reduction may exhibit elastomeric properties, which would account for its cohesion during expansion and contraction of silicon particles in the course of Li alloying/dealloying cycling. C1 [Shkrob, Ilya A.; Abraham, Daniel P.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Wishart, James F.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Shkrob, IA (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM shkrob@anl.gov; abraham@anl.gov RI Wishart, James/L-6303-2013 OI Wishart, James/0000-0002-0488-7636 FU U.S. Department of Energy Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-AC02-06CH11357, DE-SC0012704] FX I.A.S. thanks K. Quigley, R. Lowers, and S. Chemerisov for technical support. D.P.A. thanks Solvay for providing the FEC used in this study and K. Pupek, S. Trask, M. Klett, and J. Gilbert for technical support. J.F.W. thanks S. D. P. Dhiman for assistance with the pulse radiolysis experiments. This article is based upon work supported by the U.S. Department of Energy Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences under Awards DE-AC02-06CH11357 (Argonne) and DE-SC0012704 (Brookhaven), which also supported use of the LEAF Facility of the Brookhaven Accelerator Center for Energy Research. The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory. The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. NR 56 TC 22 Z9 22 U1 18 U2 118 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 9 PY 2015 VL 119 IS 27 BP 14954 EP 14964 DI 10.1021/acs.jpcc.5b03591 PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CM8PU UT WOS:000357964900016 ER PT J AU Park, JB Luo, XY Lu, J Shin, CD Yoon, CS Amine, K Sun, YK AF Park, Jin-Bum Luo, Xiangyi Lu, Jun Shin, Chang Dae Yoon, Chong Seung Amine, Khalil Sun, Yang-Kook TI Improvement of Electrochemical Properties of Lithium Oxygen Batteries Using a Silver Electrode SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID NONAQUEOUS LI-O-2 BATTERIES; AIR BATTERIES; LIMITATIONS; STABILITY; METALS; CELLS AB Silver (Ag) electrodes are prepared by an electrodeposition method at -0.25 V versus SCE. To evaluate the effect of particle size on Li-air cells, deposition times are 3, 10, 30, and 300 s. When cycled at a current density of 0.032 mA cm(-2), the Ag-deposited electrode for 300 s shows very low polarization corresponding to the oxygen evolution reaction potential at 3.6 V. X-ray diffraction studies confirm that the main discharge product is Li2O2, and the results of scanning electron microscopy and transmission electron microscopy of the discharged electrodes show lithium peroxides at different positions due to the limitation of active sites on silver particles. C1 [Park, Jin-Bum; Shin, Chang Dae; Sun, Yang-Kook] Hanyang Univ, Dept Energy Engn, Seoul 133791, South Korea. [Yoon, Chong Seung] Hanyang Univ, Dept Mat Sci & Engn, Seoul 133791, South Korea. [Luo, Xiangyi; Lu, Jun; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Lu, J (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. EM junlu@anl.gov; yksun@hanyang.ac.kr RI Luo, Xiangyi/K-6058-2015 OI Luo, Xiangyi/0000-0002-4817-1461 FU Korea Institute of Energy Technology Evaluation and Planning (KETEP) - Korea government Ministry of Trade, Industry and Energy [20124010203310]; National Research Foundation of Korea (NRF) - Korea government (MEST) [2014R1A2A1A13050479] FX This work was supported by the Human Resources Development program (No. 20124010203310) of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant funded by the Korea government Ministry of Trade, Industry and Energy, and by the National Research Foundation of Korea (NRF) grant funded by the Korea government (MEST) (No. 2014R1A2A1A13050479). NR 19 TC 4 Z9 4 U1 6 U2 47 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 9 PY 2015 VL 119 IS 27 BP 15036 EP 15040 DI 10.1021/acs.jpcc.5b04653 PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CM8PU UT WOS:000357964900025 ER PT J AU Li, WZ Gao, F Li, Y Walter, ED Liu, J Peden, CHF Wang, Y AF Li, Wei-Zhen Gao, Feng Li, Yan Walter, Eric D. Liu, Jun Peden, Charles H. F. Wang, Yong TI Nanocrystalline Anatase Titania-Supported Vanadia Catalysts: Facet-Dependent Structure of Vanadia SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID X-RAY PHOTOELECTRON; EXPOSED 001 FACETS; PEROXOTITANIUM COMPLEX; TIO2 NANOCRYSTALS; OXIDE CATALYSTS; SELECTIVE OXIDATION; SPECTROSCOPY; PHASE; REACTIVITY; NANORODS AB Titania-supported vanadia, a classic heterogeneous catalyst for redox reactions, typically has nonhomogeneous vanadia species on various titania facets, making it challenging not only to determine and quantify each species but also to decouple their catalytic contributions. We prepared truncated tetragonal bipyramidal (TiO2-TTB) and rod-like (TiO2-Rod) anatase titania with only {101} and {001} facets at ratios of about 80:20 and 93:7, respectively, and used them as supports of submonolayer vanadia. The structure and redox properties of supported vanadia were determined by XRD, TEM, XPS, EPR, Raman, FTIR and TPR, and so on. It was found that vanadia preferentially occupy TiO2 {001} facets and form isolated O=V4+(OTi)(2) species, and with further increase in vanadia surface coverage, isolated O=V5+(OTi)(3) and oligomerized O=V5+(OM)(3) (M = Ti or V) species form on TiO2 {101} facets. The discovery on support facet-dependent structure of vanadia on anatase titania is expected to enable the elucidation of structurefunction correlations on high-surface-area TiO2 supported vanadia catalysts. C1 [Li, Wei-Zhen; Gao, Feng; Walter, Eric D.; Liu, Jun; Peden, Charles H. F.; Wang, Yong] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. [Li, Yan; Wang, Yong] Washington State Univ, Gene & Linda Voiland Sch Chem Engn & Bioengn, Pullman, WA 99164 USA. RP Gao, F (reprint author), Pacific NW Natl Lab, Inst Integrated Catalysis, POB 999, Richland, WA 99352 USA. EM feng.gao@pnnl.gov; yong.wang@pnnl.gov RI Li, Wei-Zhen/A-9715-2015; Walter, Eric/P-9329-2016 OI Li, Wei-Zhen/0000-0002-2298-1423; FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences; DOE Office of Biological and Environmental Research FX This work was supported by U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences. The research was performed in the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the DOE Office of Biological and Environmental Research, and located at Pacific Northwest National Laboratory (PNNL). PNNL is operated for DOE by Battelle. NR 47 TC 3 Z9 3 U1 4 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 9 PY 2015 VL 119 IS 27 BP 15094 EP 15102 DI 10.1021/acs.jpcc.5b01486 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CM8PU UT WOS:000357964900032 ER PT J AU Makaremi, M Jordan, KD Guthrie, GD Myshakin, EM AF Makaremi, Meysam Jordan, Kenneth D. Guthrie, George D. Myshakin, Evgeniy M. TI Multiphase Monte Carlo and Molecular Dynamics Simulations of Water and CO2 Intercalation in Montmorillonite and Beidellite SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SUPERCRITICAL CARBON-DIOXIDE; VAPOR-LIQUID-EQUILIBRIA; SWELLING CLAY-MINERALS; X-RAY-DIFFRACTION; GIBBS-ENSEMBLE; NA-MONTMORILLONITE; IN-SITU; SODIUM MONTMORILLONITE; COMPUTER-SIMULATION; AQUEOUS-SOLUTIONS AB Multiphase Gibbs ensemble Monte Carlo simulations were carried out to compute the free energy of swelling for Na montmorillonite and Na-beidellite interacting with CO2 and H2O at pressure and temperature conditions relevant for geological storage aquifers. The calculated swelling free energy curves show stable monolayer and bilayer configurations of the interlayer species for Na-montmorillonite, while only the monolayer structure is found to be stable for Na-beidellite. The calculations show that CO2 is intercalated into hydrated clay phases at concentrations greatly exceeding its solubility in bulk water. This suggests that expandable clay minerals are good candidates for storing carbon dioxide in interlayer regions. For Na-beidellite the CO2 molecule distribution is mainly controlled by the position of the isomorphic substitutions, while for Na-montmorillonite the hydrated sodium ions play an important role in establishing the CO2 distribution. C1 [Makaremi, Meysam; Jordan, Kenneth D.; Guthrie, George D.; Myshakin, Evgeniy M.] Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. [Makaremi, Meysam; Jordan, Kenneth D.] Univ Pittsburgh, Dept Chem, Pittsburgh, PA 15260 USA. [Makaremi, Meysam] Univ Pittsburgh, Dept Mech Engn, Pittsburgh, PA 15260 USA. [Myshakin, Evgeniy M.] AECOM, Pittsburgh, PA 15236 USA. RP Myshakin, EM (reprint author), Natl Energy Technol Lab, 626 Cochrans Mill Rd, Pittsburgh, PA 15236 USA. EM evgeniy.myshakin@netl.doe.gov FU National Energy Technology Laboratory under the RES [DE-FE0004000] FX This technical effort was performed in support of the National Energy Technology Laboratory's ongoing research under the RES contract DE-FE0004000. The simulations were carried out on NETL's High-Performance Computer for Energy and the Environment (HPCEE) and on computers in the University of Pittsburgh's Center for Simulation and Modeling. NR 90 TC 8 Z9 8 U1 4 U2 40 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 9 PY 2015 VL 119 IS 27 BP 15112 EP 15124 DI 10.1021/acs.jpcc.5b01754 PG 13 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CM8PU UT WOS:000357964900034 ER PT J AU Machesky, ML Predota, M Ridley, MK Wesolowski, DJ AF Machesky, Michael L. Predota, Milan Ridley, Moira K. Wesolowski, David J. TI Constrained Surface Complexation Modeling: Rutile in RbCl, NaCl, and NaCF3SO3 Media to 250 degrees C SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ELECTRIC DOUBLE-LAYER; MOLECULAR-DYNAMICS SIMULATION; OXIDE-WATER INTERFACE; MUSIC MODEL; CHARGE-DISTRIBUTION; ION ADSORPTION; HYDRATION; 250-DEGREES-C; PROTONATION; TITRATIONS AB A comprehensive set of molecular-level results, primarily from classical molecular dynamics (CMD) simulations, are used to constrain CD-MUSIC surface complexation model (SCM) parameters describing rutile powder titrations conducted in RbCl, NaCl, and NaTr (Tr = triflate, CF3SO3-) electrolyte media from 25 to 250 degrees C. Rb+ primarily occupies the innermost tetradentate binding site on the rutile (110) surface at all temperatures (25, 150, 250 degrees C) and negative charge conditions (-0.1 and -0.2 C/m(2)) probed via CMD simulations, reflecting the small hydration energy of this large, monovalent cation. Consequently, variable SCM parameters (Stern-layer capacitance values and intrinsic Rb+ binding constants) were adjusted relatively easily to satisfactorily match the CMD and titration data. The larger hydration energy of Na+ results in a more complex inner-sphere distribution, which shifts from bidentate to tetradentate binding with increasing negative charge and temperature, and this distribution was not matched well for both negative charge conditions, which may reflect limitations in the CMD and/or SCM approaches. In particular, the CMD axial density profiles for Rh+ and Na+ reveal that peak binding distances shift toward the surface with increasing negative charge, suggesting that the CD-MUSIC framework may be improved by incorporating CD or Stern-layer capacitance values that vary with charge. C1 [Machesky, Michael L.] Univ Illinois, Illinois State Water Survey, Champaign, IL 61820 USA. [Predota, Milan] Univ South Bohemia, Fac Sci, Inst Phys & Biophys, Ceske Budejovice 37005, Czech Republic. [Ridley, Moira K.] Texas Tech Univ, Dept Geosci, Lubbock, TX 79409 USA. [Wesolowski, David J.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Machesky, ML (reprint author), Univ Illinois, Illinois State Water Survey, 2204 Griffith Dr, Champaign, IL 61820 USA. EM machesky@illinois.edu RI Predota, Milan/A-2256-2009 OI Predota, Milan/0000-0003-3902-0992 FU Division of Chemical Sciences, Geoscience and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy; National Science Foundation [EAR-0842526]; Czech Science Foundation [13-08651S] FX M.L.M. and D.J.W. were supported by the Division of Chemical Sciences, Geoscience and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy. M.K.R. acknowledges the support of the National Science Foundation (EAR-0842526). M.P. was supported by the Czech Science Foundation (13-08651S). The comments of two anonymous reviewers were greatly appreciated and resulted in an improved final manuscript. NR 43 TC 1 Z9 1 U1 4 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 9 PY 2015 VL 119 IS 27 BP 15204 EP 15215 DI 10.1021/acs.jpcc.5b02841 PG 12 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CM8PU UT WOS:000357964900043 ER PT J AU Wu, D Guo, XF Sun, H Navrotsky, A AF Wu, Di Guo, Xiaofeng Sun, Hui Navrotsky, Alexandra TI Energy Landscape of Water and Ethanol on Silica Surfaces SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID MINERAL OXIDE SURFACES; MESOPOROUS SILICA; DRUG-DELIVERY; POROUS SILICA; THERMODYNAMIC COMPLEXITY; CONTROLLED-RELEASE; MANGANESE OXIDES; NANOPARTICLES; ADSORPTION; ENERGETICS AB Fundamental understanding of small molecule silica surface interactions at their interfaces is essential for the scientific, technological, and medical communities. We report direct enthalpy of adsorption (Delta h(ads)) measurements for ethanol and water vapor on porous silica glass (CPG-10), in both hydroxylated and dehydroxylated (hydrophobic) forms. The results suggest a spectrum of energetics as a function of coverage, stepwise for ethanol but continuous for water. The zero-coverage enthalpy of adsorption for hydroxylated silica shows the most exothermic enthalpies for both water (-72.7 +/- 3.1 kJ/mol water) and ethanol (-78.0 +/- 1.9 kJ/mol ethanol). The water adsorption enthalpy becomes less exothermic gradually until reaching its only plateau (-20.7 +/- 2.2 kJ/mol water) reflecting water clustering on a largely hydrophobic surface, while the enthalpy of ethanol adsorption profile presents two well separated plateaus, corresponding to strong chemisorption of ethanol on adsorbate-free silica surface (-66.4 +/- 4.8 kJ/rnol ethanol), and weak physisorption of ethanol on ethanol covered silica (-4.0 +/- 1.6 kJ/mol ethanol). On the other hand, dehydroxylation leads to missing water-silica interactions, whereas the number of ethanol binding sites is not impacted. The isotherms and partial molar properties of adsorption suggest that water may only bind strongly onto the silanols (which are a minor species on silica glass), whereas ethanol can interact strongly with both silanols and the hydrophobic areas of the silica surface. C1 [Wu, Di; Guo, Xiaofeng; Navrotsky, Alexandra] Univ Calif Davis, Peter A Rock Thermochem Lab, Davis, CA 95616 USA. [Wu, Di; Guo, Xiaofeng; Navrotsky, Alexandra] Univ Calif Davis, NEAT ORU, Davis, CA 95616 USA. [Guo, Xiaofeng] Los Alamos Natl Lab, Earth Syst Observat, Earth & Environm Sci Div, Los Alamos, NM 87545 USA. [Sun, Hui] E China Univ Sci & Technol, State Key Lab Chem Engn, Shanghai 200237, Peoples R China. RP Navrotsky, A (reprint author), Univ Calif Davis, Peter A Rock Thermochem Lab, One Shields Ave, Davis, CA 95616 USA. EM anavrotsky@ucdavis.edu RI Wu, Di/A-3039-2014 OI Wu, Di/0000-0001-6879-321X FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-FG02-97ER14749] FX The calorimetric work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Grant DE-FG02-97ER14749. The authors thank Bruce C. Gates for invaluable discussion during Di Wu's Ph.D. exit seminar, which initiated this study. We also thank Krasen Kovachev and Sergey V. Ushakov for instrumental support. NR 59 TC 2 Z9 2 U1 4 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 9 PY 2015 VL 119 IS 27 BP 15428 EP 15433 DI 10.1021/acs.jpcc.5b04271 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CM8PU UT WOS:000357964900067 ER PT J AU Hook, A Murayama, H AF Hook, Anson Murayama, Hitoshi TI Low-energy supersymmetry breaking without the gravitino problem SO PHYSICAL REVIEW D LA English DT Article ID GAUGE MEDIATION; HIGGS-BOSON; MODEL; MASS; PARTICLE; LHC AB In models of low-energy gauge mediation, the observed Higgs mass is in tension with the cosmological limit on the gravitino mass m(3/2) less than or similar to 16 eV. We present an alternative mediation mechanism of supersymmetry breaking via a U(1) D term with an E-6-inspired particle content, which we call vector mediation. The gravitino mass can be in the eV range. The sfermion masses are at the 10 TeV scale, while gauginos are around a TeV. This mechanism also greatly ameliorates the mu problem. C1 [Hook, Anson] Inst Adv Study, Sch Nat Sci, Princeton, NJ 08540 USA. [Murayama, Hitoshi] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Murayama, Hitoshi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. [Murayama, Hitoshi] Univ Tokyo, Todai Inst Adv Study, Kavli Inst Phys & Math Univ WPI, Kashiwa, Chiba 2778583, Japan. RP Hook, A (reprint author), Inst Adv Study, Sch Nat Sci, Einstein Dr, Princeton, NJ 08540 USA. EM hook@ias.edu; hitoshi@berkeley.edu FU National Science Foundation [1066293, PHY-1002399]; U.S. Department of Energy [DE-SC0009988, DE-AC03-76SF00098]; JSPS [26400241, 26105507]; WPI, MEXT, Japan FX H. M. thanks T. T. Yanagida for discussions. We thank the Aspen Center for Physics and the National Science Foundation Grant No. 1066293 for hospitality during the Aspen Winter Conference "Exploring the Physics Frontier with Circular Colliders, where our collaboration began. The work of A. H. is supported by the U.S. Department of Energy Grant No. DE-SC0009988. H. M. is supported in part by the U.S. Department of Energy under Contract No. DE-AC03-76SF00098, in part by the National Science Foundation under Grant No. PHY-1002399, in part by the JSPS Grant-in-Aid for Scientific Research (C) (No. 26400241), Scientific Research on Innovative Areas (No. 26105507), and by WPI, MEXT, Japan. NR 36 TC 1 Z9 1 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JUL 9 PY 2015 VL 92 IS 1 AR 015004 DI 10.1103/PhysRevD.92.015004 PG 5 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CM4EX UT WOS:000357638300007 ER PT J AU Pal, B Schwartz, AJ Abdesselam, A Adachi, I Aihara, H Al Said, S Arinstein, K Asner, DM Aulchenko, V Aushev, T Ayad, R Babu, V Badhrees, I Bakich, AM Bobrov, A Bonvicini, G Bozek, A Bracko, M Browder, TE Cervenkov, D Chang, MC Chekelian, V Chen, A Cheon, BG Cho, K Chobanova, V Choi, Y Cinabro, D Dalseno, J Dolezal, Z Drasal, Z Drutskoy, A Dutta, D Eidelman, S Farhat, H Fast, JE Ferber, T Frost, O Fulsom, BG Gaur, V Gabyshev, N Ganguly, S Garmash, A Getzkow, D Gillard, R Glattauer, R Goh, YM Golob, B Grzymkowska, O Hara, T Hayasaka, K Hayashii, H He, XH Hou, WS Huschle, M Hyun, HJ Iijima, T Ishikawa, A Itoh, R Iwasaki, Y Jaegle, I Julius, T Kang, KH Kato, E Kiesling, C Kim, DY Kim, JB Kim, JH Kim, KT Kim, MJ Kim, SH Kim, YJ Kinoshita, K Ko, BR Kodys, P Korpar, S Krizan, P Krokovny, P Kuhr, T Kumita, T Kuzmin, A Kwon, YJ Lange, JS Lee, DH Lee, IS Li, Y Gioi, LL Libby, J Liventsev, D Lukin, P Matvienko, D Miyata, H Mohanty, GB Moll, A Moon, HK Nakamura, KR Nakano, E Nakao, M Nanut, T Natkaniec, Z Nayak, M Nishida, S Ogawa, S Okuno, S Pakhlov, P Pakhlova, G Park, CW Park, H Pedlar, TK Pesantez, L Petric, M Piilonen, LE Pulvermacher, C Ribezl, E Ritter, M Rostomyan, A Ryu, S Sakai, Y Sandilya, S Santel, D Santelj, L Sanuki, T Sato, Y Schneider, O Schnell, G Schwanda, C Senyo, K Seon, O Sevior, ME Shapkin, M Shebalin, V Shen, CP Shibata, TA Shiu, JG Sibidanov, A Simon, F Sohn, YS Solovieva, E Stanic, S Staric, M Sumihama, M Sumisawa, K Sumiyoshi, T Tamponi, U Teramoto, Y Thorne, F Uchida, M Uehara, S Unno, Y Uno, S Usov, Y Van Hulse, C Vanhoefer, P Varner, G Vinokurova, A Vorobyev, V Vossen, A Wagner, MN Wang, CH Wang, MZ Wang, P Wang, XL Watanabe, Y Won, E Yamamoto, H Yamaoka, J Yashchenko, S Zhang, ZP Zhilich, V Zhulanov, V Zupanc, A AF Pal, B. Schwartz, A. J. Abdesselam, A. Adachi, I. Aihara, H. Al Said, S. Arinstein, K. Asner, D. M. Aulchenko, V. Aushev, T. Ayad, R. Babu, V. Badhrees, I. Bakich, A. M. Bobrov, A. Bonvicini, G. Bozek, A. Bracko, M. Browder, T. E. Cervenkov, D. Chang, M. -C. Chekelian, V. Chen, A. Cheon, B. G. Cho, K. Chobanova, V. Choi, Y. Cinabro, D. Dalseno, J. Dolezal, Z. Drasal, Z. Drutskoy, A. Dutta, D. Eidelman, S. Farhat, H. Fast, J. E. Ferber, T. Frost, O. Fulsom, B. G. Gaur, V. Gabyshev, N. Ganguly, S. Garmash, A. Getzkow, D. Gillard, R. Glattauer, R. Goh, Y. M. Golob, B. Grzymkowska, O. Hara, T. Hayasaka, K. Hayashii, H. He, X. H. Hou, W. -S. Huschle, M. Hyun, H. J. Iijima, T. Ishikawa, A. Itoh, R. Iwasaki, Y. Jaegle, I. Julius, T. Kang, K. H. Kato, E. Kiesling, C. Kim, D. Y. Kim, J. B. Kim, J. H. Kim, K. T. Kim, M. J. Kim, S. H. Kim, Y. J. Kinoshita, K. Ko, B. R. Kodys, P. Korpar, S. Krizan, P. Krokovny, P. Kuhr, T. Kumita, T. Kuzmin, A. Kwon, Y. -J. Lange, J. S. Lee, D. H. Lee, I. S. Li, Y. Gioi, L. Li Libby, J. Liventsev, D. Lukin, P. Matvienko, D. Miyata, H. Mohanty, G. B. Moll, A. Moon, H. K. Nakamura, K. R. Nakano, E. Nakao, M. Nanut, T. Natkaniec, Z. Nayak, M. Nishida, S. Ogawa, S. Okuno, S. Pakhlov, P. Pakhlova, G. Park, C. W. Park, H. Pedlar, T. K. Pesantez, L. Petric, M. Piilonen, L. E. Pulvermacher, C. Ribezl, E. Ritter, M. Rostomyan, A. Ryu, S. Sakai, Y. Sandilya, S. Santel, D. Santelj, L. Sanuki, T. Sato, Y. Schneider, O. Schnell, G. Schwanda, C. Senyo, K. Seon, O. Sevior, M. E. Shapkin, M. Shebalin, V. Shen, C. P. Shibata, T. -A. Shiu, J. -G. Sibidanov, A. Simon, F. Sohn, Y. -S. Solovieva, E. Stanic, S. Staric, M. Sumihama, M. Sumisawa, K. Sumiyoshi, T. Tamponi, U. Teramoto, Y. Thorne, F. Uchida, M. Uehara, S. Unno, Y. Uno, S. Usov, Y. Van Hulse, C. Vanhoefer, P. Varner, G. Vinokurova, A. Vorobyev, V. Vossen, A. Wagner, M. N. Wang, C. H. Wang, M. -Z. Wang, P. Wang, X. L. Watanabe, Y. Won, E. Yamamoto, H. Yamaoka, J. Yashchenko, S. Zhang, Z. P. Zhilich, V. Zhulanov, V. Zupanc, A. CA Belle Collaboration TI Evidence for the decay B-0 -> eta pi(0) SO PHYSICAL REVIEW D LA English DT Article ID B MESON DECAYS; BELLE DETECTOR; PACKAGE; SEARCH; ETA' AB We report a search for the charmless hadronic decay B-0 -> eta pi(0) with a data sample corresponding to an integrated luminosity of 694 fb(-1) containing 753 x 10(6) BB pairs. The data were collected by the Belle experiment running on the Upsilon(4S) resonance at the KEKB e(+)e(-) collider. We measure a branching fraction B(B-0 > eta pi(0)) = (4.1(-1.5-0.7)(+1.75+0.5)) x 10(-7), where the first unceminty is statistical and the second is systematic. Our measurement gives an upper limit of beta(B-0 -> n pi(0)) < 6.5 x 10(-7) at 90% confidence level. The signal has a significance of 3.0 standard deviations and constitutes the first evidence for this decay mode. C1 [Schnell, G.; Van Hulse, C.] Univ Basque Country UPV EHU, Bilbao 48080, Spain. [Shen, C. P.] Beihang Univ, Beijing 100191, Peoples R China. [Pesantez, L.] Univ Bonn, D-53115 Bonn, Germany. [Arinstein, K.; Aulchenko, V.; Bobrov, A.; Eidelman, S.; Gabyshev, N.; Garmash, A.; Krokovny, P.; Kuzmin, A.; Lukin, P.; Matvienko, D.; Shebalin, V.; Usov, Y.; Vinokurova, A.; Vorobyev, V.; Zhilich, V.; Zhulanov, V.] SB RAS, Budker Inst Nucl Phys, Novosibirsk 630090, Russia. [Arinstein, K.; Aulchenko, V.; Bobrov, A.; Eidelman, S.; Gabyshev, N.; Garmash, A.; Krokovny, P.; Kuzmin, A.; Lukin, P.; Matvienko, D.; Shebalin, V.; Usov, Y.; Vinokurova, A.; Vorobyev, V.; Zhilich, V.; Zhulanov, V.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Cervenkov, D.; Dolezal, Z.; Drasal, Z.; Kodys, P.] Charles Univ Prague, Fac Math & Phys, Prague 12116, Czech Republic. [Pal, B.; Schwartz, A. J.; Kinoshita, K.; Santel, D.] Univ Cincinnati, Cincinnati, OH 45221 USA. [Ferber, T.; Frost, O.; Rostomyan, A.; Yashchenko, S.] DESY, D-22607 Hamburg, Germany. [Getzkow, D.; Lange, J. S.; Wagner, M. N.] Univ Giessen, D-35392 Giessen, Germany. [Sumihama, M.] Gifu Univ, Gifu 5011193, Japan. [Adachi, I.; Hara, T.; Itoh, R.; Nakao, M.; Nishida, S.; Sakai, Y.; Sumisawa, K.; Uehara, S.; Uno, S.] Grad Univ Adv Studies, SOKENDAI, Hayama 2400193, Japan. [Cheon, B. G.; Goh, Y. M.; Kim, S. H.; Lee, I. S.; Unno, Y.] Hanyang Univ, Seoul 133791, South Korea. [Browder, T. E.; Jaegle, I.; Varner, G.] Univ Hawaii, Honolulu, HI 96822 USA. [Adachi, I.; Hara, T.; Hayasaka, K.; Itoh, R.; Iwasaki, Y.; Nakamura, K. R.; Nakao, M.; Nishida, S.; Sakai, Y.; Santelj, L.; Sumisawa, K.; Uehara, S.; Uno, S.] High Energy Accelerator Res Org KEK, Tsukuba, Ibaraki 3050801, Japan. [Schnell, G.] Basque Fdn Sci, IKERBASQUE, Bilbao 48013, Spain. [Dutta, D.] Indian Inst Technol, Gauhati 781039, Assam, India. [Libby, J.; Nayak, M.] Indian Inst Technol, Madras 600036, Tamil Nadu, India. [Vossen, A.] Indiana Univ, Bloomington, IN 47408 USA. [Wang, P.] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Glattauer, R.; Schwanda, C.; Thorne, F.] Inst High Energy Phys, A-1050 Vienna, Austria. [Shapkin, M.] Inst High Energy Phys, Protvino 142281, Russia. [Tamponi, U.] INFN, Sez Torino, I-10125 Turin, Italy. [Aushev, T.; Drutskoy, A.; Pakhlov, P.; Pakhlova, G.; Solovieva, E.] Inst Theoret & Expt Phys, Moscow 117218, Russia. [Bracko, M.; Golob, B.; Korpar, S.; Krizan, P.; Nanut, T.; Petric, M.; Ribezl, E.; Staric, M.; Zupanc, A.] Jozef Stefan Inst, Ljubljana 1000, Slovenia. [Okuno, S.; Watanabe, Y.] Kanagawa Univ, Yokohama, Kanagawa 2218686, Japan. [Huschle, M.; Kuhr, T.; Pulvermacher, C.] Karlsruhe Inst Technol, Inst Expt Kernphys, D-76131 Karlsruhe, Germany. [Badhrees, I.] King Abdulaziz City Sci & Technol, Riyadh 11442, Saudi Arabia. [Al Said, S.] King Abdulaziz Univ, Fac Sci, Dept Phys, Jeddah 21589, Saudi Arabia. [Cho, K.; Kim, J. H.; Kim, Y. J.] Korea Inst Sci & Technol Informat, Taejon 305806, South Korea. [Kim, J. B.; Kim, K. T.; Ko, B. R.; Lee, D. H.; Moon, H. K.; Won, E.] Korea Univ, Seoul 136713, South Korea. [Hyun, H. J.; Kang, K. H.; Kim, M. J.; Park, H.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Schneider, O.] Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland. [Aushev, T.; Golob, B.; Krizan, P.] Univ Ljubljana, Fac Math & Phys, Ljubljana 1000, Slovenia. [Pedlar, T. K.] Luther Coll, Decorah, IA 52101 USA. [Bracko, M.; Korpar, S.] Univ Maribor, Maribor 2000, Slovenia. [Chekelian, V.; Chobanova, V.; Dalseno, J.; Kiesling, C.; Gioi, L. Li; Moll, A.; Ritter, M.; Simon, F.; Vanhoefer, P.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Julius, T.; Sevior, M. E.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Drutskoy, A.; Pakhlov, P.] Moscow Engn Phys Inst, Moscow 115409, Russia. [Pakhlova, G.] Moscow Inst Phys & Technol, Dolgoprudnyi 141700, Moscow Region, Russia. [Iijima, T.; Sato, Y.; Seon, O.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648602, Japan. [Iijima, T.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648602, Japan. [Hayashii, H.] Nara Womens Univ, Nara 6308506, Japan. [Wang, C. H.] Natl Cent Univ, Chungli 32054, Taiwan. [Wang, C. H.] Natl United Univ, Miaoli 36003, Taiwan. [Hou, W. -S.; Shiu, J. -G.; Wang, M. -Z.] Natl Taiwan Univ, Dept Phys, Taipei 10617, Taiwan. [Bozek, A.; Grzymkowska, O.; Natkaniec, Z.] H Niewodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. [Miyata, H.] Niigata Univ, Niigata 9502181, Japan. [Stanic, S.] Univ Nova Gorica, Nova Gorica 5000, Slovenia. [Nakano, E.; Teramoto, Y.] Osaka City Univ, Osaka 5588585, Japan. [Asner, D. M.; Fast, J. E.; Fulsom, B. G.; Yamaoka, J.] Pacific NW Natl Lab, Richland, WA 99352 USA. [He, X. H.] Peking Univ, Beijing 100871, Peoples R China. [Zhang, Z. P.] Univ Sci & Technol China, Anhua 230026, Peoples R China. [Ryu, S.] Seoul Natl Univ, Seoul 151742, South Korea. [Kim, D. Y.] Soongsil Univ, Seoul 156743, South Korea. [Choi, Y.; Park, C. W.] Sungkyunkwan Univ, Suwon 440746, South Korea. [Bakich, A. M.; Sibidanov, A.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdesselam, A.; Al Said, S.; Ayad, R.; Badhrees, I.] Univ Tabuk, Fac Sci, Dept Phys, Tabuk 71451, Saudi Arabia. [Babu, V.; Gaur, V.; Mohanty, G. B.; Sandilya, S.] Tata Inst Fundamental Res, Mumbai 400005, Maharashtra, India. [Dalseno, J.; Moll, A.; Simon, F.] Tech Univ Munich, Excellence Cluster Universe, D-85748 Garching, Germany. [Ogawa, S.] Toho Univ, Funabashi, Chiba 2748510, Japan. [Ishikawa, A.; Kato, E.; Sanuki, T.; Yamamoto, H.] Tohoku Univ, Sendai, Miyagi 9808578, Japan. [Aihara, H.] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Shibata, T. -A.; Uchida, M.] Tokyo Inst Technol, Tokyo 1528550, Japan. [Kumita, T.; Sumiyoshi, T.] Tokyo Metropolitan Univ, Tokyo 1920397, Japan. [Tamponi, U.] Univ Turin, I-10124 Turin, Italy. [Li, Y.; Liventsev, D.; Piilonen, L. E.; Wang, X. L.] Virginia Polytech Inst & State Univ, CNP, Blacksburg, VA 24061 USA. [Bonvicini, G.; Cinabro, D.; Farhat, H.; Ganguly, S.; Gillard, R.] Wayne State Univ, Detroit, MI 48202 USA. [Senyo, K.] Yamagata Univ, Yamagata 9908560, Japan. [Kwon, Y. -J.; Sohn, Y. -S.] Yonsei Univ, Seoul 120749, South Korea. [Chang, M. -C.] Fu Jen Catholic Univ, Dept Phys, Taipei 24205, Taiwan. RP Pal, B (reprint author), Univ Cincinnati, Cincinnati, OH 45221 USA. RI Aihara, Hiroaki/F-3854-2010; Pakhlova, Galina/C-5378-2014; Pakhlov, Pavel/K-2158-2013; Krokovny, Pavel/G-4421-2016; EPFL, Physics/O-6514-2016; Drutskoy, Alexey/C-8833-2016; Cervenkov, Daniel/D-2884-2017; Solovieva, Elena/B-2449-2014; Faculty of, Sciences, KAU/E-7305-2017 OI Aihara, Hiroaki/0000-0002-1907-5964; Pakhlova, Galina/0000-0001-7518-3022; Pakhlov, Pavel/0000-0001-7426-4824; Krokovny, Pavel/0000-0002-1236-4667; Drutskoy, Alexey/0000-0003-4524-0422; Cervenkov, Daniel/0000-0002-1865-741X; Solovieva, Elena/0000-0002-5735-4059; FU Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan; Japan Society for the Promotion of Science (JSPS); Tau-Lepton Physics Research Center of Nagoya University; Australian Research Council; Australian Department of Industry, Innovation, Science and Research; Austrian Science Fund [P 22742-N16, P 26794-N20]; National Natural Science Foundation of China [10575109, 10775142, 10875115, 11175187, 11475187]; Ministry of Education, Youth and Sports of the Czech Republic [LG14034]; Carl Zeiss Foundation; Deutsche Forschungsgemeinschaft; VolkswagenStiftung; Department of Science and Technology of India; Istituto Nazionale di Fisica Nucleare of Italy; National Research Foundation (NRF) of Korea [2011-0029457, 2012-0008143, 2012R1A1A2008330, 2013R1A1A3007772, 2014R1A2A2A01005286, 2014R1A2A2A01002734, 2014R1A1A2006456]; Basic Research Lab program under NRF [KRF-2011-0020333, KRF-2011-0021196]; Center for Korean J-PARC Users [NRF-2013K1A3A7A06056592]; Brain Korea 21-Plus program; Global Science Experimental Data Hub Center of the Korea Institute of Science and Technology Information; Polish Ministry of Science and Higher Education; National Science Center; Ministry of Education and Science of the Russian Federation; Russian Foundation for Basic Research; Slovenian Research Agency; Basque Foundation for Science (IKERBASQUE); Euskal Herriko Unibertsitatea (UPV/EHU) (Spain) [UFI 11/55]; Swiss National Science Foundation; National Science Council; Ministry of Education of Taiwan; U.S. Department of Energy; National Science Foundation; MEXT for Science Research in a Priority Area; JSPS for Creative Scientific Research FX We thank the KEKB group for the excellent operation of the accelerator; the KEK cryogenics group for the efficient operation of the solenoid; and the KEK computer group, the National Institute of Informatics, and the PNNL/EMSL computing group for valuable computing and SINET4 network support. We acknowledge support from the Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan, the Japan Society for the Promotion of Science (JSPS), and the Tau-Lepton Physics Research Center of Nagoya University; the Australian Research Council and the Australian Department of Industry, Innovation, Science and Research; Austrian Science Fund under Grants No. P 22742-N16 and No. P 26794-N20; the National Natural Science Foundation of China under Contracts No. 10575109, No. 10775142, No. 10875115, No. 11175187, and No. 11475187; the Ministry of Education, Youth and Sports of the Czech Republic under Contract No. LG14034; the Carl Zeiss Foundation, the Deutsche Forschungsgemeinschaft and the VolkswagenStiftung; the Department of Science and Technology of India; the Istituto Nazionale di Fisica Nucleare of Italy; National Research Foundation (NRF) of Korea Grants No. 2011-0029457, No. 2012-0008143, No. 2012R1A1A2008330, No. 2013R1A1A3007772, No. 2014R1A2A2A01005286, No. 2014R1A2A2A01002734, and No. 2014R1A1A2006456; the Basic Research Lab program under NRF Grants No. KRF-2011-0020333 and No. KRF-2011-0021196, Center for Korean J-PARC Users, Grant No. NRF-2013K1A3A7A06056592; the Brain Korea 21-Plus program and the Global Science Experimental Data Hub Center of the Korea Institute of Science and Technology Information; the Polish Ministry of Science and Higher Education and the National Science Center; the Ministry of Education and Science of the Russian Federation and the Russian Foundation for Basic Research; the Slovenian Research Agency; the Basque Foundation for Science (IKERBASQUE) and the Euskal Herriko Unibertsitatea (UPV/EHU) under program UFI 11/55 (Spain); the Swiss National Science Foundation; the National Science Council and the Ministry of Education of Taiwan; and the U.S. Department of Energy and the National Science Foundation. This work is supported by a Grant-in-Aid from MEXT for Science Research in a Priority Area ("New Development of Flavor Physics") and from JSPS for Creative Scientific Research ("Evolution of Tau-lepton Physics"). NR 42 TC 1 Z9 1 U1 2 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 9 PY 2015 VL 92 IS 1 AR 011101 DI 10.1103/PhysD.92.011101 PG 7 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CM4EX UT WOS:000357638300001 ER PT J AU Lewicki, JP Fox, CA Worsley, MA AF Lewicki, James P. Fox, Christina A. Worsley, Marcus A. TI On the synthesis and structure of resorcinol-formaldehyde polymeric networks - Precursors to 3D-carbon macroassemblies SO POLYMER LA English DT Article DE Organic sol-gels; NMR; Resorcinol-formaldehyde ID NUCLEAR-MAGNETIC-RESONANCE; SOL-GEL CHEMISTRY; CARBON AEROGEL; RESINS AB With the new impetus towards the development of hierarchical graphene and CNT macro-assemblies for application in fields such as advanced energy storage, catalysis and electronics; there is much renewed interest in organic carbon-based sol-gel processes as a synthetically convenient and versatile means of forming three dimensional, covalently bonded organic/inorganic networks. Such matrices can act as highly effective precursors, scaffolds or molecular 'glues' for the assembly of a wide variety of functional carbon macro-assemblies. However, despite the utility and broad use of organic sol-gel processes - such as the ubiquitous resorcinol-formaldehyde (RF) reaction, there are details of the reaction chemistries of these important sol-gel processes that remain poorly understood at present. It is therefore both timely and necessary to examine these reactions in more detail using modern analytical techniques in order to gain a more rigorous understanding of the mechanisms by which these organic networks form. The goal of such studies is to obtain improved and rational control over the organic network structure, in order to better direct and tailor the architecture of the final inorganic carbon matrix. In this study we have investigated in detail, the mechanism of the organic sol-gel network forming reaction of resorcinol and formaldehyde from a structural and kinetic standpoint, by using a combination of real-time high field solution state nuclear magnetic resonance (NMR), low field NMR relaxometry and differential scanning calorimetry (DSC). These investigations have allowed us to track the network formation processes in real-time, gain both detailed structural information on the mechanisms of the RF solegel process and a quantitative assessment of the kinetics of the global network formation process. It has been shown that the mechanism, by which the RF organic network forms, proceeds via an initial exothermic step correlated to the formation of a free aromatic aldehyde. The network growth reaction then proceeds in a statistical manner following a first order Arrhenius type kinetic relationship - characteristic of a typical thermoset network poly-condensation process. And despite the relative complexity and ill-defined nature of the formaldehyde staring material, the final network structure is to a large extent, governed by the substitution pattern of the resorcinol molecule. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Lewicki, James P.; Fox, Christina A.; Worsley, Marcus A.] Lawrence Livermore Natl Lab, Livermore, CA 94510 USA. RP Lewicki, JP (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94510 USA. EM lewicki1@llnl.gov OI Worsley, Marcus/0000-0002-8012-7727 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. The authors would also like to gratefully acknowledge Mark Pearson (LLNL) for his assistance in carrying out the TGA of the materials studied. NR 32 TC 2 Z9 2 U1 10 U2 76 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0032-3861 EI 1873-2291 J9 POLYMER JI Polymer PD JUL 9 PY 2015 VL 69 BP 45 EP 51 PG 7 WC Polymer Science SC Polymer Science GA CM9AM UT WOS:000357997300006 ER PT J AU Brown, CT Hug, LA Thomas, BC Sharon, I Castelle, CJ Singh, A Wilkins, MJ Wrighton, KC Williams, KH Banfield, JF AF Brown, Christopher T. Hug, Laura A. Thomas, Brian C. Sharon, Itai Castelle, Cindy J. Singh, Andrea Wilkins, Michael J. Wrighton, Kelly C. Williams, Kenneth H. Banfield, Jillian F. TI Unusual biology across a group comprising more than 15% of domain Bacteria SO NATURE LA English DT Article ID RIBOSOMAL-RNA GENES; STRUCTURE PREDICTION; UNCULTURED BACTERIA; SINGLE-CELL; DARK-MATTER; PROTEIN; SEQUENCE; ORGANISMS; ALIGNMENT; DATABASE AB A prominent feature of the bacterial domain is a radiation of major lineages that are defined as candidate phyla because they lack isolated representatives. Bacteria from these phyla occur in diverse environments(1) and are thought to mediate carbon and hydrogen cycles(2). Genomic analyses of a few representatives suggested that metabolic limitations have prevented their cultivation(2-6). Here we reconstructed 8 complete and 789 draft genomes from bacteria representing >35 phyla and documented features that consistently distinguish these organisms from other bacteria. We infer that this group, which may comprise >(1)5% of the bacterial domain, has shared evolutionary history, and describe it as the candidate phyla radiation (CPR). All CPR genomes are small and most lack numerous biosynthetic pathways. Owing to divergent 16S ribosomal RNA (rRNA) gene sequences, 50-100% of organisms sampled from specific phyla would evade detection in typical cultivation-independent surveys. CPR organisms often have self-splicing introns and proteins encoded within their rRNA genes, a feature rarely reported in bacteria. Furthermore, they have unusual ribosome compositions. All are missing a ribosomal protein often absent in symbionts, and specific lineages are missing ribosomal proteins and biogenesis factors considered universal in bacteria. This implies different ribosome structures and biogenesis mechanisms, and underlines unusual biology across a large part of the bacterial domain. C1 [Brown, Christopher T.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Hug, Laura A.; Thomas, Brian C.; Sharon, Itai; Castelle, Cindy J.; Singh, Andrea; Banfield, Jillian F.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Wilkins, Michael J.] Ohio State Univ, Sch Earth Sci, Columbus, OH 43210 USA. [Wilkins, Michael J.; Wrighton, Kelly C.] Ohio State Univ, Dept Microbiol, Columbus, OH 43210 USA. [Williams, Kenneth H.; Banfield, Jillian F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Banfield, Jillian F.] Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. RP Banfield, JF (reprint author), Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. EM jbanfield@berkeley.edu RI Wilkins, Michael/A-9358-2013; Williams, Kenneth/O-5181-2014 OI Williams, Kenneth/0000-0002-3568-1155 FU US Department of Energy (DOE), Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231, DE-SC0004918]; Natural Sciences and Engineering Research Council postdoctoral fellowship; DOE FX We thank J. Cate and S. Moore for input into the ribosomal protein analysis, J. Doudna and E. Nawrocki for suggestions on the rRNA insertion analysis, and M. Markillie and R. Taylor for assistance with RNA sequencing. Research was supported by the US Department of Energy (DOE), Office of Science, Office of Biological and Environmental Research under award number DE-AC02-05CH11231 (Sustainable Systems Scientific Focus Area and DOE-JGI) and award number DE-SC0004918 (Systems Biology Knowledge Base Focus Area). L.A.H. was partially supported by a Natural Sciences and Engineering Research Council postdoctoral fellowship. DNA sequencing was conducted at the DOE Joint Genome Institute, a DOE Office of Science User Facility, via the Community Science Program. RNA sequencing was performed at the DOE-supported Environmental Molecular Sciences Laboratory at Pacific Northwest National Laboratory. NR 62 TC 111 Z9 111 U1 32 U2 118 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD JUL 9 PY 2015 VL 523 IS 7559 BP 208 EP U173 DI 10.1038/nature14486 PG 18 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CM4ZO UT WOS:000357695900034 PM 26083755 ER PT J AU Aznauryan, IG Burkert, VD AF Aznauryan, I. G. Burkert, V. D. TI Extracting meson-baryon contributions to the electroexcitation of the N(1675)5/2(-) nucleon resonance SO PHYSICAL REVIEW C LA English DT Article ID SINGLE PION-PHOTOPRODUCTION; RELATIVISTIC QUARK-MODEL; TRANSITION FORM-FACTORS; REGION; ELECTROPRODUCTION AB We report on the determination of the electrocouplings for the transition from the proton to the N(1675)5/2(-) resonance state using recent differential cross section data on ep -> e pi(+) n by the CLAS collaboration at 1.8 <= Q(2) < 4.5 GeV2. The data have been analyzed using two different approaches, the unitary isobar model and fixed-t dispersion relations. The extracted gamma* p -> N(1675)5/2(-) helicity amplitudes show considerable coupling through the A(1/2)(p) amplitude, that is significantly larger than the predicted three-quark contribution to this amplitude. The amplitude A(3/2)(p) is much smaller. Both results are consistent with the predicted sizes of the meson-baryon contributions at Q(2) >= 1.8 GeV2 from the dynamical coupled-channel model. C1 [Aznauryan, I. G.; Burkert, V. D.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Aznauryan, I. G.] Yerevan Phys Inst, AI Alikhanian Natl Sci Lab, Yerevan 0036, Armenia. RP Aznauryan, IG (reprint author), Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. FU State Committee of Science of Republic of Armenia [13-1C023]; U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC05-06OR23177] FX This work was supported by the State Committee of Science of Republic of Armenia, Grant No. 13-1C023, and the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Contract No. DE-AC05-06OR23177. NR 38 TC 4 Z9 4 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JUL 9 PY 2015 VL 92 IS 1 AR 015203 DI 10.1103/PhysRevC.92.015203 PG 4 WC Physics, Nuclear SC Physics GA CM4EP UT WOS:000357637500004 ER PT J AU Liu, YL Pan, ZH Zhuang, QL Miralles, DG Teuling, AJ Zhang, TL An, PL Dong, ZQ Zhang, JT He, D Wang, LW Pan, XB Bai, W Niyogi, D AF Liu, Yaling Pan, Zhihua Zhuang, Qianlai Miralles, Diego G. Teuling, Adriaan J. Zhang, Tonglin An, Pingli Dong, Zhiqiang Zhang, Jingting He, Di Wang, Liwei Pan, Xuebiao Bai, Wei Niyogi, Dev TI Agriculture intensifies soil moisture decline in Northern China SO SCIENTIFIC REPORTS LA English DT Article ID CLIMATE-CHANGE; WATER AVAILABILITY; LOESS PLATEAU; LAND-USE; FERTILIZER; MANAGEMENT; DROUGHT; WHEAT; CROP; IMPACTS AB Northern China is one of the most densely populated regions in the world. Agricultural activities have intensified since the 1980s to provide food security to the country. However, this intensification has likely contributed to an increasing scarcity in water resources, which may in turn be endangering food security. Based on in-situ measurements of soil moisture collected in agricultural plots during 1983-2012, we find that topsoil (0-50 cm) volumetric water content during the growing season has declined significantly (p < 0.01), with a trend of -0.011 to -0.015 m(3) m(-3) per decade. Observed discharge declines for the three large river basins are consistent with the effects of agricultural intensification, although other factors (e.g. dam constructions) likely have contributed to these trends. Practices like fertilizer application have favoured biomass growth and increased transpiration rates, thus reducing available soil water. In addition, the rapid proliferation of water-expensive crops (e.g., maize) and the expansion of the area dedicated to food production have also contributed to soil drying. Adoption of alternative agricultural practices that can meet the immediate food demand without compromising future water resources seem critical for the sustainability of the food production system. C1 [Liu, Yaling; Pan, Zhihua; An, Pingli; Dong, Zhiqiang; Zhang, Jingting; He, Di; Wang, Liwei; Pan, Xuebiao] China Agr Univ, Coll Resources & Environm Sci, Beijing 100193, Peoples R China. [Liu, Yaling; Zhuang, Qianlai; Niyogi, Dev] Purdue Univ, Dept Earth Atmospher & Planetary Sci, W Lafayette, IN 47907 USA. [Liu, Yaling] Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD 20740 USA. [Zhuang, Qianlai; Niyogi, Dev] Purdue Univ, Dept Agron, W Lafayette, IN 47907 USA. [Miralles, Diego G.] Vrije Univ Amsterdam, Dept Earth Sci, NL-1081 HV Amsterdam, Netherlands. [Miralles, Diego G.] Univ Ghent, Lab Hydrol & Water Management, B-9000 Ghent, Belgium. [Teuling, Adriaan J.] Wageningen Univ, Hydrol & Quantitat Water Management Grp, NL-6708 PB Wageningen, Netherlands. [Zhang, Tonglin] Purdue Univ, Dept Stat, W Lafayette, IN 47907 USA. [Bai, Wei] China Ctr Urban Dev, Beijing 100045, Peoples R China. RP Pan, ZH (reprint author), China Agr Univ, Coll Resources & Environm Sci, Beijing 100193, Peoples R China. EM panzhihua@cau.edu.cn; qzhuang@purdue.edu RI Miralles, Diego/K-8857-2013; OI Miralles, Diego/0000-0001-6186-5751; Teuling, Adriaan/0000-0003-4302-2835 FU National Basic Research Program of China [2012CB956204]; National Natural Science Foundation of China [41371232, 41271110]; National Science and Technology Support Program of China [2012BAD09B02]; National Non-profit Research Foundation for Agriculture of China [201103039]; NASA Land Use and Land Cover Change program [NASA-NNX09AI26G, NN-H-04-Z-YS-005-N, NNX09AM55G]; Department of Energy [DE-FG02-08ER64599]; National Science Foundation [NSF-1028291, NSF-0919331, NSF-CAREER AGS-0847472]; NSF Carbon and Water in the Earth Program [NSF-0630319]; Netherlands Organization for Scientific Research (NWO) [863.14.004]; Belgian Science Policy Office (BELSPO) [SR/00/306] FX This research is supported by the National Basic Research Program of China (No. 2012CB956204), the National Natural Science Foundation of China (Grant Nos. 41371232 and 41271110), the National Science and Technology Support Program of China (No. 2012BAD09B02), the National Non-profit Research Foundation for Agriculture of China (201103039), the NASA Land Use and Land Cover Change program (NASA-NNX09AI26G, NN-H-04-Z-YS-005-N, and NNX09AM55G to Q.Z.), the Department of Energy (DE-FG02-08ER64599 to Q.Z.), the National Science Foundation (NSF-1028291 and NSF-0919331 to Q.Z., NSF-CAREER AGS-0847472 to D.N.), the NSF Carbon and Water in the Earth Program (NSF-0630319 to Q.Z.). We acknowledge Chinese Meteorological Administration, Ministry of Water Resources of China and National Bureau of Statistics of China for provision of data used in this study. D.G.M. acknowledges financial support from Netherlands Organization for Scientific Research (NWO) through grant 863.14.004, and the Belgian Science Policy Office (BELSPO) in the frame of the STEREO III programme, project SAT-EX (SR/00/306). This research was primarily conducted when the lead author Yaling Liu worked at China Agricultural University and Purdue University and was revised during her ongoing affiliation with Pacific Northwest National Laboratory. NR 57 TC 7 Z9 8 U1 6 U2 33 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUL 9 PY 2015 VL 5 AR 11261 DI 10.1038/srep11261 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CM4GR UT WOS:000357643200001 PM 26158774 ER PT J AU Musah, RA Espinoza, EO Cody, RB Lesiak, AD Christensen, ED Moore, HE Maleknia, S Drijfhout, FP AF Musah, Rabi A. Espinoza, Edgard O. Cody, Robert B. Lesiak, Ashton D. Christensen, Earl D. Moore, Hannah E. Maleknia, Simin Drijfhout, Falko P. TI A High Throughput Ambient Mass Spectrometric Approach to Species Identification and Classification from Chemical Fingerprint Signatures SO SCIENTIFIC REPORTS LA English DT Article ID VOLATILE ORGANIC-COMPOUNDS; REAL-TIME; CUTICULAR HYDROCARBONS; GEOGRAPHICAL ORIGIN; TROPANE ALKALOIDS; DART-MS; DIFFERENTIATION; DISCRIMINATION; SPECTROSCOPY; IONIZATION AB A high throughput method for species identification and classification through chemometric processing of direct analysis in real time (DART) mass spectrometry-derived fingerprint signatures has been developed. The method entails introduction of samples to the open air space between the DART ion source and the mass spectrometer inlet, with the entire observed mass spectral fingerprint subjected to unsupervised hierarchical clustering processing. A range of both polar and non-polar chemotypes are instantaneously detected. The result is identification and species level classification based on the entire DART-MS spectrum. Here, we illustrate how the method can be used to: (1) distinguish between endangered woods regulated by the Convention for the International Trade of Endangered Flora and Fauna (CITES) treaty; (2) assess the origin and by extension the properties of biodiesel feedstocks; (3) determine insect species from analysis of puparial casings; (4) distinguish between psychoactive plants products; and (5) differentiate between Eucalyptus species. An advantage of the hierarchical clustering approach to processing of the DART-MS derived fingerprint is that it shows both similarities and differences between species based on their chemotypes. Furthermore, full knowledge of the identities of the constituents contained within the small molecule profile of analyzed samples is not required. C1 [Musah, Rabi A.; Lesiak, Ashton D.] SUNY Albany, Dept Chem, Albany, NY 12222 USA. [Espinoza, Edgard O.] US Natl Fish & Wildlife Forens Lab, Ashland, OR 97520 USA. [Cody, Robert B.] JEOL USA Inc, Peabody, MA 01960 USA. [Christensen, Earl D.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Moore, Hannah E.; Drijfhout, Falko P.] Keele Univ, Sch Phys & Geog Sci, Dept Chem Ecol, Keele ST5 5BG, Staffs, England. [Maleknia, Simin] Univ New S Wales, Sch Biol Earth & Environm Sci, Sydney, NSW, Australia. RP Musah, RA (reprint author), SUNY Albany, Dept Chem, 1400 Washington Ave, Albany, NY 12222 USA. EM rmusah@albany.edu FU Research Foundation of SUNY; U.S. National Science Foundation [1310350]; Winston Churchill Memorial trust; Keele University; U.S. Department of Energy, Office of Vehicle Technologies [DEAC36-99GO10337]; National Renewable Energy Laboratory FX The support of the Research Foundation of SUNY, a grant from the U.S. National Science Foundation to RAM and RBC (grant #1310350), a fellowship from the Winston Churchill Memorial trust as well as financial support from Keele University for HM, and the support of the U.S. Department of Energy, Office of Vehicle Technologies under Contract DEAC36-99GO10337 with the National Renewable Energy Laboratory, are appreciated. The assistance of Justine Giffen with preparation of the Eucalypt samples and Dr. Bryan Moser of the USDA in supplying biodiesel samples is gratefully acknowledged. Thanks are also extended to Professors Jeffery Tomberlin and Eric Benbow who supplied the puparial cases. The findings and conclusions in this article are those of the authors and do not necessarily represent the views of the U.S. Fish and Wildlife Service. NR 63 TC 6 Z9 6 U1 4 U2 28 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUL 9 PY 2015 VL 5 AR 11520 DI 10.1038/srep11520 PG 16 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CM4HG UT WOS:000357644700001 PM 26156000 ER PT J AU Stenfeldt, C Pacheco, JM Singanallur, NB Ferreira, HCD Vosloo, W Rodriguez, LL Arzt, J AF Stenfeldt, Carolina Pacheco, Juan M. Singanallur, Nagendrakumar B. Ferreira, Helena C. de Carvalho Vosloo, Wilna Rodriguez, Luis L. Arzt, Jonathan TI Clinical and virological dynamics of a serotype O 2010 South East Asia lineage foot-and-mouth disease virus in sheep using natural and simulated natural inoculation and exposure systems SO VETERINARY MICROBIOLOGY LA English DT Article DE FMDV; Foot-and-mouth disease; Virus; Sheep; Pathogenesis; Infection ID UNITED-KINGDOM; 2001 EPIDEMIC; CATTLE; INFECTION; PATHOGENESIS; IDENTIFICATION; DIAGNOSIS; ANTIBODY; SWINE; ASSAY AB Within-host infection dynamics of a recent field isolate of foot-and-mouth disease virus (FMDV), serotype O, topotype South East Asia, lineage Myamar'98 were evaluated in sheep using four different systems for virus exposure. Two novel, simulated natural, inoculation systems consisting of intra-nasopharyngeal (INP) deposition and aerosol inoculation were evaluated in comparison with two conventional systems: coronary band inoculation and direct contact exposure. All four exposure systems were efficient in generating consistently severe, generalized FMD with synchronous clinical characteristics within exposure groups, indicating that this Myanmar98 strain is highly virulent in sheep. Clinical and virological dynamics were similarly rapid following INP- and coronary band inoculation, with both systems leading to significantly earlier detection of virus shedding when compared to aerosol inoculation and contact exposure. The data presented herein support application of the two optimized simulated natural inoculation systems as valid alternatives to conventionally used exposure systems for studies of FMDV pathogenesis and vaccinology in sheep. Furthermore, the data suggest that targeted exposure of the ovine pharynx is highly efficient for generating consistent FMDV infection, which supports critical involvement of this anatomic region as a site of primary virus replication in sheep. Published by Elsevier B.V. C1 [Stenfeldt, Carolina; Pacheco, Juan M.; Ferreira, Helena C. de Carvalho; Rodriguez, Luis L.; Arzt, Jonathan] ARS, Plum Isl Anim Dis Ctr, Foreign Anim Dis Res Unit, USDA, Greenport, NY 11944 USA. [Stenfeldt, Carolina; Ferreira, Helena C. de Carvalho] PIADC Res Participat Program, Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. [Singanallur, Nagendrakumar B.; Vosloo, Wilna] CSIRO, Australian Anim Hlth Lab, Geelong, Vic, Australia. RP Arzt, J (reprint author), ARS, Plum Isl Anim Dis Ctr, Foreign Anim Dis Res Unit, USDA, Greenport, NY 11944 USA. EM Jonathan.Arzt@ars.usda.gov OI Stenfeldt, Carolina/0000-0002-2074-3886; Pacheco, Juan/0000-0001-5477-0201; Arzt, Jonathan/0000-0002-7517-7893 FU CSIRO-Australian Animals Health Laboratory [58-1940-3-004]; Agricultural Research Service, USDA [58-1940-3-004]; CSIRO; Australian Government [PSH 0652]; ARS-CRIS Project [1940- 32000-057-00D]; Plum Island Animal Disease Center Research Participation Program fellowships; Cattle Council of Australia; Australian Dairy Farmers; Australian Lot Feeders Association; Wool Producers Australia; Sheepmeat Council of Australia; Australian Pork Limited; Goat Industry Council of Australia through the Meat and Livestock Australia Donor Company FX This study was a collaboration between the CSIRO-Australian Animals Health Laboratory and the Agricultural Research Service, USDA, who co-funded the work under collaborative agreement 58-1940-3-004. Funding through CSIRO was provided in part by the livestock industries in Australia through the Cattle Council of Australia, Australian Dairy Farmers, Australian Lot Feeders Association, Wool Producers Australia, Sheepmeat Council of Australia, Australian Pork Limited and the Goat Industry Council of Australia through the Meat and Livestock Australia Donor Company matching arrangements with the Australian Government (Project PSH 0652). Animal Health Australia provided the project management service for all relevant industries. Additional funding came from ARS-CRIS Project 1940- 32000-057-00D. CS and HCF are recipients of Plum Island Animal Disease Center Research Participation Program fellowships, administered by the Oak Ridge Institute for Science and Education (ORISE) through an interagency agreement with the US Department of Energy. None of the funding sources had influence upon design or performance of experimental study, interpretation of results or writing of the manuscript. The Korean FMDV isolate was provided by Dr. Kwang-Nyeong Lee, Animal and Plant Quarantine Agency, Ministry of Agriculture, Food and Rural Affairs Republic of Korea. The authors thank Elizabeth Bishop, Ethan Hartwig and George Smoliga for processing of samples and Erin Howey for immunomicroscopy support. NR 35 TC 5 Z9 5 U1 4 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-1135 EI 1873-2542 J9 VET MICROBIOL JI Vet. Microbiol. PD JUL 9 PY 2015 VL 178 IS 1-2 BP 50 EP 60 DI 10.1016/j.vetmic.2015.04.004 PG 11 WC Microbiology; Veterinary Sciences SC Microbiology; Veterinary Sciences GA CL2BU UT WOS:000356749400006 PM 25937316 ER PT J AU Caron, E Espona, L Kowalewski, DJ Schuster, H Ternette, N Alpizar, A Schittenhelm, RB Ramarathinam, SH Arlehamn, CSL Koh, CC Gillet, LC Rabsteyn, A Navarro, P Kim, S Lam, H Sturm, T Marcilla, M Sette, A Campbell, DS Deutsch, EW Moritz, RL Purcell, AW Rammensee, HG Stevanovic, S Aebersold, R AF Caron, Etienne Espona, Lucia Kowalewski, Daniel J. Schuster, Heiko Ternette, Nicola Alpizar, Adan Schittenhelm, Ralf B. Ramarathinam, Sri H. Arlehamn, Cecilia S. Lindestam Koh, Ching Chiek Gillet, Ludovic C. Rabsteyn, Armin Navarro, Pedro Kim, Sangtae Lam, Henry Sturm, Theo Marcilla, Miguel Sette, Alessandro Campbell, David S. Deutsch, Eric W. Moritz, Robert L. Purcell, Anthony W. Rammensee, Hans-Georg Stevanovic, Stefan Aebersold, Ruedi TI An open-source computational and data resource to analyze digital maps of immunopeptidomes SO ELIFE LA English DT Article ID SWATH-MASS-SPECTROMETRY; CANCER-IMMUNOTHERAPY; BINDING PREDICTIONS; TARGETED ANALYSIS; MS DATA; PEPTIDES; PROTEOMICS; SEARCH; IDENTIFICATIONS; REPERTOIRE AB We present a novel mass spectrometry-based high-throughput workflow and an open-source computational and data resource to reproducibly identify and quantify HLA-associated peptides. Collectively, the resources support the generation of HLA allele-specific peptide assay libraries consisting of consensus fragment ion spectra, and the analysis of quantitative digital maps of HLA peptidomes generated from a range of biological sources by SWATH mass spectrometry (MS). This study represents the first community-based effort to develop a robust platform for the reproducible and quantitative measurement of the entire repertoire of peptides presented by HLA molecules, an essential step towards the design of efficient immunotherapies. C1 [Caron, Etienne; Espona, Lucia; Koh, Ching Chiek; Gillet, Ludovic C.; Sturm, Theo; Aebersold, Ruedi] ETH, Inst Mol Syst Biol, Dept Biol, Zurich, Switzerland. [Kowalewski, Daniel J.; Schuster, Heiko; Rabsteyn, Armin; Rammensee, Hans-Georg; Stevanovic, Stefan] Univ Tubingen, Dept Immunol, Interfac Inst Cell Biol, Tubingen, Germany. [Kowalewski, Daniel J.; Schuster, Heiko; Rammensee, Hans-Georg; Stevanovic, Stefan] German Canc Consortium, DKFZ Partner Site Tubingen, Tubingen, Germany. [Ternette, Nicola] Univ Oxford, Target Discovery Inst, Mass Spectrometry Lab, Oxford, England. [Alpizar, Adan; Marcilla, Miguel] Spanish Natl Biotechnol Ctr, Prote Unit, Madrid, Spain. [Schittenhelm, Ralf B.; Ramarathinam, Sri H.; Purcell, Anthony W.] Monash Univ, Dept Biochem & Mol Biol, Clayton, Vic, Australia. [Arlehamn, Cecilia S. Lindestam; Sette, Alessandro] La Jolla Inst Allergy & Immunol, La Jolla, CA USA. [Navarro, Pedro] Johannes Gutenberg Univ Mainz, Inst Immunol, Univ Med Ctr, Mainz, Germany. [Kim, Sangtae] Pacific NW Natl Lab, Richland, WA 99352 USA. [Lam, Henry] Hong Kong Univ Sci & Technol, Div Biomed Engn, Hong Kong, Hong Kong, Peoples R China. [Lam, Henry] Hong Kong Univ Sci & Technol, Dept Chem & Biomol Engn, Hong Kong, Hong Kong, Peoples R China. [Campbell, David S.; Deutsch, Eric W.; Moritz, Robert L.] Inst Syst Biol, Seattle, WA USA. [Aebersold, Ruedi] Univ Zurich, Fac Sci, Zurich, Switzerland. RP Caron, E (reprint author), ETH, Inst Mol Syst Biol, Dept Biol, Zurich, Switzerland. EM caron@imsb.biol.ethz.ch; aebersold@imsb.biol.ethz.ch RI Ramarathinam, Sri/G-2278-2012; OI Ramarathinam, Sri/0000-0002-2787-1282; Gillet, Ludovic/0000-0002-1001-3265; Ternette, Nicola/0000-0002-9283-0743; Purcell, Anthony/0000-0003-0532-8331; Marcilla, Miguel/0000-0001-9171-5076; Lindestam Arlehamn, Cecilia/0000-0001-7302-8002 FU National Health and Medical Research Council (NHMRC) [1022509, 1085017]; National Institutes of Health (NIH) [HHSN272201200010C, HHSN272200900044C]; European Research Council (ERC) [ERC-2008-AdG_20080422]; Schweizerische Nationalfonds zur Forderung der Wissenschaftlichen Forschung [3100A0-688 107679]; European Commission (EC) [241587]; German Cancer Consortium (DKTK); Bundesministerium fur Bildung und Forschung [0316179C]; Forschungszentrum Immuntherapie (FZI) of the Johannes Gutenberg University Mainz; Ministerio de Economia y Competitividad Carlos III Health Institute (ISCIII) (ProteoRed-PRB2) [PT13/0001]; European Commission (EC); Schweizerische Nationalfonds zur Forderung der Wissenschaftlichen Forschung; National Institute of General Medical Sciences (NIGMS) [R01GM087221, 2P50GM076547] FX National Health and Medical Research Council (NHMRC) 1022509 and 1085017 Anthony W Purcell; National Institutes of Health (NIH) HHSN272201200010C and HHSN272200900044C Cecilia S Lindestam Arlehamn, Alessandro Sette; European Research Council (ERC) ERC-2008-AdG_20080422 Ruedi Aebersold; Schweizerische Nationalfonds zur Forderung der Wissenschaftlichen Forschung 3100A0-688 107679 Ruedi Aebersold; European Commission (EC) SysteMtb, 241587 Ruedi Aebersold; German Cancer Consortium (DKTK) Daniel J Kowalewski, Heiko Schuster, Hans-Georg Rammensee, Stefan Stevanovic; Bundesministerium fur Bildung und Forschung e:Bio Express2Present, 0316179C Pedro Navarro; Forschungszentrum Immuntherapie (FZI) of the Johannes Gutenberg University Mainz Pedro Navarro; Ministerio de Economia y Competitividad Carlos III Health Institute (ISCIII) (ProteoRed-PRB2, PT13/0001) Miguel Marcilla; European Commission (EC) Marie Curie Intra-European Fellowship Etienne Caron; Schweizerische Nationalfonds zur Forderung der Wissenschaftlichen Forschung Postdoc Mobility Fellowship Ralf B Schittenhelm; National Institute of General Medical Sciences (NIGMS) R01GM087221 and 2P50GM076547/Center for Systems Biology David S Campbell, Eric W Deutsch, Robert L Moritz NR 50 TC 16 Z9 16 U1 4 U2 14 PU ELIFE SCIENCES PUBLICATIONS LTD PI CAMBRIDGE PA SHERATON HOUSE, CASTLE PARK, CAMBRIDGE, CB3 0AX, ENGLAND SN 2050-084X J9 ELIFE JI eLife PD JUL 8 PY 2015 VL 4 AR e07661 DI 10.7554/eLife.07661 PG 17 WC Biology SC Life Sciences & Biomedicine - Other Topics GA CN2KW UT WOS:000358250900001 ER PT J AU Bamgbade, BA Wu, Y Burgess, WA Tapriyal, D Gamwo, IK Baled, HO Enick, RM McHugh, MA AF Bamgbade, Babatunde A. Wu, Yue Burgess, Ward A. Tapriyal, Deepak Gamwo, Isaac K. Baled, Hseen O. Enick, Robert M. McHugh, Mark A. TI High-Temperature, High-Pressure Volumetric Properties of Propane, Squalane, and Their Mixtures: Measurement and PC-SAFT Modeling SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID EQUATION-OF-STATE; BINARY-LIQUID MIXTURES; PERTURBED-CHAIN SAFT; N-OCTANE; 298.15 K; ELEVATED-TEMPERATURES; EXPERIMENTAL DENSITY; REFRACTIVE-INDEXES; ORGANIC LIQUIDS; 265 MPA AB This study reports the high-temperature, high-pressure density data for propane, squalane, and their binary mixtures for five compositions at temperatures to 520 K and pressures to 260 MPa. The density measurements are obtained with a floating-piston, variable-volume, high-pressure view cell. From the density data, the isothermal and isobaric excess molar volumes upon mixing are computed. For the mixture compositions studied here, the excess volume is mostly negative, showing a minimum at 0.6550 mole fraction of propane and becomes less negative as the propane concentration increases. The perturbed-chain statistical associating fluid theory (PC-SAFT) equation of state (EoS) provides good representation for the experimental data. A mean absolute percent deviation (delta) of 1.4% is obtained with the PC-SAFT EoS when using propane and squalane pure component parameters fit to density data at high-temperature, high-pressure conditions. C1 [Bamgbade, Babatunde A.; Wu, Yue; Burgess, Ward A.; Tapriyal, Deepak; Gamwo, Isaac K.; Baled, Hseen O.; Enick, Robert M.; McHugh, Mark A.] US DOE, Natl Energy Technol Lab, Off Res & Dev, Pittsburgh, PA 15236 USA. [Bamgbade, Babatunde A.; Wu, Yue; McHugh, Mark A.] Virginia Commonwealth Univ, Dept Chem & Life Sci Engn, Richmond, VA 23284 USA. [Tapriyal, Deepak] URS, Pittsburgh, PA 15236 USA. [Baled, Hseen O.; Enick, Robert M.] Univ Pittsburgh, Swanson Sch Engn, Dept Chem & Petr Engn, Pittsburgh, PA 15261 USA. RP Bamgbade, BA (reprint author), Virginia Commonwealth Univ, Dept Chem & Life Sci Engn, 601 W Main St, Richmond, VA 23220 USA. EM bamgbadeba@vcu.edu FU National Energy Technology Laboratory's Office of Research and Development of the Strategic Center for Natural Gas and Oil under RES [DE-FE0004000] FX This technical effort was performed in support of the National Energy Technology Laboratory's Office of Research and Development support of the Strategic Center for Natural Gas and Oil under RES Contract DE-FE0004000. NR 44 TC 2 Z9 2 U1 3 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD JUL 8 PY 2015 VL 54 IS 26 BP 6804 EP 6811 DI 10.1021/acs.iecr.5b01173 PG 8 WC Engineering, Chemical SC Engineering GA CM8PN UT WOS:000357964200022 ER PT J AU Zhou, Y Lu, Q Zhuang, ZB Hutchings, GS Kattel, S Yan, YS Chen, JGG Xiao, JQ Jiao, F AF Zhou, Yang Lu, Qi Zhuang, Zhongbin Hutchings, Gregory S. Kattel, Shyam Yan, Yushan Chen, Jingguang G. Xiao, John Q. Jiao, Feng TI Oxygen Reduction at Very Low Overpotential on Nanoporous Ag Catalysts SO ADVANCED ENERGY MATERIALS LA English DT Article ID MEMBRANE FUEL-CELLS; SILVER NANOWIRES; AIR BATTERIES; CARBON; ELECTROCATALYSTS; ELECTROREDUCTION; HYDROXIDE; OXIDATION C1 [Zhou, Yang; Xiao, John Q.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [Lu, Qi; Chen, Jingguang G.] Columbia Univ, Dept Chem Engn, New York, NY 10027 USA. [Lu, Qi; Zhuang, Zhongbin; Hutchings, Gregory S.] Univ Delaware, Dept Chem & Biomol Engn, Newark, DE 19716 USA. [Kattel, Shyam; Chen, Jingguang G.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Chen, JGG (reprint author), Columbia Univ, Dept Chem Engn, New York, NY 10027 USA. EM jgchen@columbia.edu; jqx@udel.edu; jiao@udel.edu RI Zhuang, e/H-8164-2016; Hutchings, Gregory/B-5620-2012; Lu, Qi/P-7477-2016; OI Zhuang, e/0000-0001-7187-1266; Hutchings, Gregory/0000-0002-0819-9654; Jiao, Feng/0000-0002-3335-3203 FU National Science Foundation Faculty Early Career Development (CAREER) Program [CBET-1350911]; University of Delaware Research Foundation Strategic Initiatives (UDRF-SI) Grant; US Department of Energy [DE-FG02-13ER16381] FX Y.Z. and Q.L. contributed equally to this work. The authors at University of Delaware are grateful for financial support from the National Science Foundation Faculty Early Career Development (CAREER) Program (Award No. CBET-1350911) and the University of Delaware Research Foundation Strategic Initiatives (UDRF-SI) Grant. The authors at Columbia University acknowledge support from the US Department of Energy (DE-FG02-13ER16381). NR 26 TC 9 Z9 9 U1 18 U2 83 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD JUL 8 PY 2015 VL 5 IS 13 AR 1500149 DI 10.1002/aenm.201500149 PG 4 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA CM7NG UT WOS:000357880100003 ER PT J AU Wills, AW Michalak, DJ Ercius, P Rosenberg, ER Perciano, T Ushizima, D Runser, R Helms, BA AF Wills, Andrew W. Michalak, David J. Ercius, Peter Rosenberg, Ethan R. Perciano, Talita Ushizima, Daniela Runser, Rory Helms, Brett A. TI Block Copolymer Packing Limits and Interfacial Reconfigurability in the Assembly of Periodic Mesoporous Organosilicas SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article DE block copolymers; directed self-assembly; periodic mesoporous organosilicas; thin films ID LOW DIELECTRIC-CONSTANT; SUPERIOR MECHANICAL-PROPERTIES; HYBRID THIN-FILMS; DIBLOCK COPOLYMERS; ORGANIC GROUPS; SILICA; FRAMEWORKS; NANOCRYSTALS; TRANSPORT; TEXTURE AB Here poly(N,N-dimethylacrylamide)-block-poly(styrene) block copolymer micelles (BCPs) are advanced and applied to assemble periodic mesoporous organosilicas (PMOs) with noncylindrical pores. Using these BCP micelles, it is found that pore dimensions (11-23 nm), wall thicknesses (5-9 nm), and overall porosities (26%-78%) are independently programable, depending only on relative inputs for BCP and matrix former. Notably, the degree of order in all films improves as BCP loading approaches a packing limit of 63 vol%. Beyond this limit and regardless of pore dimensions, both porogen packing in the film and pore structure after thermal processing show significant deviations away from spherical close-packed lattices. The surprising absence of film collapse in this regime allows here to quantify the evolution of pore structure through the thermally driven interfacial reconfigurability of BCP micelles in the hybrid films when porogen loading exceeds the packing limit by using both scattering techniques and scanning transmission electron microscopy tomography. Finally, the PMOs here give dielectric constants of 1.2 and 1.5 above and below the BCP packing limit, respectivelythe lowest ever reported for this matrix material. C1 [Wills, Andrew W.; Ercius, Peter; Rosenberg, Ethan R.; Runser, Rory; Helms, Brett A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Michalak, David J.] Intel Corp, Hillsboro, OR 97124 USA. [Ercius, Peter] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Natl Ctr Elect Microscopy, Berkeley, CA 94720 USA. [Perciano, Talita; Ushizima, Daniela] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. RP Wills, AW (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. EM bahelms@lbl.gov RI Foundry, Molecular/G-9968-2014; Perciano, Talita/I-5977-2012; OI Perciano, Talita/0000-0002-2388-1803; Helms, Brett/0000-0003-3925-4174 FU WFO; U.S. Department of Energy, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS); Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]; Office of Science, Advanced Scientific Computing Research, of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors thank C. Zhu and A. Hexemer for helpful discussions regarding GISAXS. Some ellipsometric porosimetry and all determinations of dielectric constant, dielectric breakdown voltage, and PMO hydrophobicity were performed at Intel Corporation (Hillsboro, OR). A. W. Wills and E. R. Rosenberg were supported by a WFO contract between Intel Corporation and B. A. Helms. E. R. Rosenberg also received partial support from the U.S. Department of Energy, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Science Undergraduate Laboratory Internship (SULI) program. Synthesis of block copolymer architecture-directing agents, PMO assembly, and aspects of PMO film characterization were carried out as part of a User Project at the Molecular Foundry, which is supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. GISAXS of PMO films assembled with the smaller BCPs was carried out at beamline 7.3.3 of the Advanced Light Source, which is supported by the Director of the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under the same contract. STEM tomography was performed at the National Center for Electron Microscopy, Molecular Foundry, Lawrence Berkeley National Laboratory, which is supported by the U.S. Department of Energy also under the same contract. GISAXS of PMO films assembled with the largest BCP was carried out at beamline 1-5 at the Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, which is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515. T. Perciano and D. Ushizima are supported by the Director, Office of Science, Advanced Scientific Computing Research, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The image analysis project is a part of the Center for Applied Mathematics for Energy Research Applications (CAMERA) at Lawrence Berkeley National Laboratory. P. Ercius and B. A. Helms are supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 68 TC 8 Z9 8 U1 4 U2 41 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD JUL 8 PY 2015 VL 25 IS 26 BP 4120 EP 4128 DI 10.1002/adfm.201501059 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CM6QC UT WOS:000357812500016 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyka, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andreia, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arika, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Auerbach, B Augsten, K Aurousseau, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Balek, P Balestri, T Balli, F Banas, E Banerjee, S Bannoura, AAE Bansil, HS Barak, L Baranov, SP Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, M Becker, S Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C 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Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Bruschi, M Bryngemark, L Buanes, T Buat, Q Buchholz, P Buckley, AG Buda, SI Budagov, IA Buehrer, F Bugge, L Bugge, MK Bulekov, O Burckhart, H Burdin, S Burghgrave, B Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Buszello, CP Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Buzykaev, R Urban, SC Caforio, D Cakira, O Calafiura, P Calandri, A Calderini, G Calfayan, P Caloba, LP Calvet, D Calvet, S Toro, RC Camarda, S Cameron, D Caminada, LM Armadans, RC Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Cardarelli, R Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Caudron, J Cavaliere, V Cavallia, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, BC Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chang, P Chapleau, B Chapman, JD Charlton, DG Chau, CC Barajas, CAC Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A Cheremushkina, E El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Childers, JT Chiodinia, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Choi, K Chouridou, S Chow, BKB Christodoulou, V Chromek-Burckhart, D Chu, ML Chudoba, J Chuinard, AJ Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Cinca, D Cindro, V Cioara, IA Ciocio, A Citron, ZH Ciubancana, M Clark, A Clark, BL Clark, PJ Clarke, RN Cleland, W Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Cogan, JG Cole, B Cole, S Colijn, AP Collot, J Colombo, T Compostella, G Muino, PC Coniavitis, E Connell, 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KD Fiolhais, MCN Fiorini, L Firan, A Fischer, A Fischer, C Fischer, J Fisher, WC Fitzgerald, EA Flechl, M Fleck, I Fleischmann, P Fleischmann, S Fletcher, GT Fletcher, G Flick, T Floderus, A Castillo, LRF Flowerdew, MJ Formica, A Forti, A Fournier, D Fox, H Fracchia, S Francavilla, P Franchini, M Francis, D Franconi, L Franklin, M Fraternali, M Freeborn, D French, ST Friedrich, F Froidevaux, D Frost, JA Fukunaga, C Torregrosa, EF Fulsom, BG Fuster, J Gabaldon, C Gabizon, O Gabrielli, A Gabrielli, A Gadatsch, S Gadomski, S Gagliardi, G Gagnon, P Galea, C Galhardo, B Gallas, EJ Gallop, BJ Gallus, P Galster, G Gan, KK Gao, J Gao, Y Gao, YS Walls, FMG Garberson, F Garcia, C Navarro, JEG Garcia-Sciveres, M Gardner, RW Garelli, N Garonne, V Gatti, C Gaudiello, A Gaudio, G Gaur, B Gauthier, L Gauzzi, P Gavrilenko, IL Gay, C Gaycken, G Gazis, EN Ge, P Gecse, Z Gee, CNP Geerts, DAA Geich-Gimbel, C Geisler, MP Gemme, C Genest, MH Gentile, S George, M George, S Gerbaudo, D Gershon, A Ghazlane, H 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CA ATLAS Collaboration TI Search for supersymmetry in events containing a same-flavour opposite-sign dilepton pair, jets, and large missing transverse momentum in root s=8TeV pp collisions with the ATLAS detector SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID SUPERGAUGE TRANSFORMATIONS; FORTRAN CODE; MODEL; GENERATORS; PARTICLE; CURRENTS; LEPTONS; PHYSICS; ENERGY; SQUARK AB Two searches for supersymmetric particles in final states containing a same-flavour opposite-sign lepton pair, jets and large missing transverse momentum are presented. The proton-proton collision data used in these searches were collected at a centre-of-mass energy root s = 8TeV by the ATLAS detector at the Large Hadron Collider and corresponds to an integrated luminosity of 20.3 fb(-1). Two leptonic production mechanisms are considered: decays of squarks and gluinos with Z bosons in the final state, resulting in a peak in the dilepton invariant mass distribution around the Z-boson mass; and decays of neutralinos (e.g.. (chi) over tilde (0)(2) -> l(+)l(-) (chi) over tilde (0)(1)), resulting in a kinematic endpoint in the dilepton invariant mass distribution. For the former, an excess of events above the expected Standard Model background is observed, with a significance of three standard deviations. In the latter case, the data are well-described by the expected Standard Model background. The results from each channel are interpreted in the context of several supersymmetric models involving the production of squarks and gluinos. C1 [Davies, E.; Jackson, P.; Lee, L.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. 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M.; Beringer, J.; Brandt, G.; Brosamer, J.; Calafiura, P.; Caminada, L. M.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Axen, B.; Barnett, R. M.; Beringer, J.; Brandt, G.; Brosamer, J.; Calafiura, P.; Caminada, L. M.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Dietrich, J.; Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Herrberg-Schubert, R.; Hristova, I.; Kind, O. M.; Kolanoski, H.; Lacker, H.; Lohse, T.; Nikiforov, A.; Rehnisch, L.; Rieck, P.; Schulz, H.; Stamm, S.; zur Nedden, M.] Humboldt Univ, Dept Phys, Berlin, Germany. [Agustoni, M.; Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Agustoni, M.; Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allbrooke, B. M. M.; Bella, L. Aperio; Bansil, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Owen, R. E.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arika, M.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Alberghi, G. L.; Bellagamba, L.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Corradi, M.; DeCastro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstrom, P.; Lasagni Manghi, F.; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] INFN Sez Bologna, Bologna, Italy. [Alberghi, G. L.; DeCastro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstrom, P.; Lasagni Manghi, F.; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Cioara, I. A.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Hageboeck, S.; Hansen, M. C.; Hellmich, D.; Hohn, D.; Huegging, F.; Janssen, J.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mergelmeyer, S.; Mijovic, L.; Mueller, K.; Obermann, T.; Pohl, D.; Ricken, O.; Sarrazin, B.; Schaepe, S.; Schopf, E.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Seema, P.; Stillings, J. A.; Tannoury, N.; Therhaag, J.; Uhlenbrock, M.; Velz, T.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Zimmermann, R.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Fitzgerald, E. A.; Sciolla, G.; Venturini, A.; Zambito, S.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio De Janeiro COPPE EE IF, Rio De Janeiro, Brazil. [Manhaes De Andrade Filho, L.] Fed Univ Juiz de Fora UFJF, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; La Rosa Navarro, J. L.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Mountricha, E.; Nevski, P.; Nilsson, P.; Oliveira Damazio, D.; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M-A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancana, M.; Constantinescu, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Iengo, P.; Jaekel, M. R.; Jakobsen, S.; Jenni, P.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. 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Y.; Xu, L.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.; Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Romano Saez, S. M.; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Clermont Univ, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Romano Saez, S. M.; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Romano Saez, S. M.; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Thompson, E. N.; Tuts, P. M.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] INFN Grp Collegato Cosenza, Lab Nazl Frascati, Frascati, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyka, L.; Bold, T.; Dabrowskia, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Naranjo Garcia, R. F.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Naranjo Garcia, R. F.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Olivares Pino, S. A.; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA, Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] INFN Lab Nazl Frascati, Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dao, V.; Di Simone, A.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koencke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Picazio, A.; Ristic, B.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] INFN Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Oropeza Barrera, C.; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Bindi, M.; Blumenschein, U.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Moreno Llacer, M.; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, Lab Phys Subatom & Cosmol, CNRS IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andreia, V.; Baas, A. E.; Brandta, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E-E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Pok Fu Lam, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R. W.; Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, S.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodinia, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] INFN Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Allport, P. P.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Price, J.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Teixeira Dias Castanheira, M.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Kempster, J. J.; Panduro Vazquez, J. G.; Pastore, Fr.; Savage, G.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Pilkington, A. D.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Moritz, S.; Poettgen, R.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Meyer, C.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Merino, J. Llorente; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Ticse Torres, R. E.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Merino, J. Llorente; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Ticse Torres, R. E.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Vazquez Schroeder, T.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Hu, X.; Levin, D.; Long, J. D.; Lu, N.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavallia, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Villaplana Perez, M.] INFN Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Turra, R.; Villaplana Perez, M.] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Moser, H. G.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] INFN Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Koenig, A. C.; Nektarijevic, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; W. H. Hopkins; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS IN2P3, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pachal, K.; Pickering, M. A.; Ryder, N. C.; Sawyer, C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] INFN Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Spalla, M.; Volpi, G.; White, S.] INFN Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Galhardo, B.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Pilcher, J. E.; Sankey, D. P. C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] INFN Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] INFN Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Di Ciaccio, A.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Stanescu, C.; Taccini, C.; Trovatelli, M.] INFN Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Taccini, C.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddade, N.; Idrissie, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Lanon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] Commissariat Energie Atom & Energies Alternat, CEA Saclay, DSM IRFU Inst Rech Lois Fondamentales Univers, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Vickey Boeriu, O. E.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; O'Neil, D. C.; Stelzer, B.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Mount, R.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urbanb, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.; Meehan, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Govender, N.; Lee, C. A.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hamity, G. N.; Hsu, C.; March, L.; Mellado Garcia, B. R.; Ruan, X.] Univ Witwatersrand, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Astron & Chem, Stony Brook, NY 11794 USA. [Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Santoyo Castillo, I.; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G-Y.; Limosani, A.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Hsu, P. J.; Jamin, D. O.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Munwes, Y.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Paredes Hernandez, D.; Petridou, C.; Sampsonidis, D.; Sotiropoulou, C. L.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Ilic, N.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. 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[Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Ferrer, J. A. 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M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Ctr Calcul, Inst Natl Phys Nucl & Phys Particules IN2P3, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London WC2R 2LS, England. [Anisenkov, A. V.; Bobrovnikov, V. S.; Buzykaev, R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. 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[Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tikhomirov, V. O.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Xu, L.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; La Rosa Navarro, Jose Luis/K-4221-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; Staroba, Pavel/G-8850-2014; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; White, Ryan/E-2979-2015; Mitsou, Vasiliki/D-1967-2009; Grancagnolo, Sergio/J-3957-2015; Zhukov, Konstantin/M-6027-2015; Doyle, Anthony/C-5889-2009; Livan, Michele/D-7531-2012; spagnolo, stefania/A-6359-2012; Di Domenico, Antonio/G-6301-2011; Negrini, Matteo/C-8906-2014; Tassi, Enrico/K-3958-2015; Ferrando, James/A-9192-2012; Boyko, Igor/J-3659-2013; Shmeleva, Alevtina/M-6199-2015; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Smirnova, Oxana/A-4401-2013; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Vranjes Milosavljevic, Marija/F-9847-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Snesarev, Andrey/H-5090-2013; Gavrilenko, Igor/M-8260-2015; Veneziano, Stefano/J-1610-2012; Tikhomirov, Vladimir/M-6194-2015; Villa, Mauro/C-9883-2009; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Brooks, William/C-8636-2013; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; De, Kaushik/N-1953-2013; Carvalho, Joao/M-4060-2013; Fabbri, Laura/H-3442-2012; Gerbaudo, Davide/J-4536-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Monzani, Simone/D-6328-2017 OI Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; White, Ryan/0000-0003-3589-5900; Mitsou, Vasiliki/0000-0002-1533-8886; Grancagnolo, Sergio/0000-0001-8490-8304; Doyle, Anthony/0000-0001-6322-6195; Livan, Michele/0000-0002-5877-0062; spagnolo, stefania/0000-0001-7482-6348; Di Domenico, Antonio/0000-0001-8078-2759; Negrini, Matteo/0000-0003-0101-6963; Ferrando, James/0000-0002-1007-7816; Boyko, Igor/0000-0002-3355-4662; Mashinistov, Ruslan/0000-0001-7925-4676; Smirnova, Oxana/0000-0003-2517-531X; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Veneziano, Stefano/0000-0002-2598-2659; Tikhomirov, Vladimir/0000-0002-9634-0581; Villa, Mauro/0000-0002-9181-8048; Warburton, Andreas/0000-0002-2298-7315; Brooks, William/0000-0001-6161-3570; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; De, Kaushik/0000-0002-5647-4489; Carvalho, Joao/0000-0002-3015-7821; Fabbri, Laura/0000-0002-4002-8353; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Monzani, Simone/0000-0002-0479-2207 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; RGC, Hong Kong SAR, China; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, UK; Royal Society, UK; Leverhulme Trust, UK; DOE, USA; NSF, USA FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; RGC, Hong Kong SAR, China; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, UK; DOE and NSF, USA. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 91 TC 15 Z9 15 U1 8 U2 63 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JUL 8 PY 2015 VL 75 IS 7 AR 318 DI 10.1140/epjc/s10052-015-3518-2 PG 40 WC Physics, Particles & Fields SC Physics GA CM4WJ UT WOS:000357686000001 ER PT J AU Perras, FA Kobayashi, T Pruski, M AF Perras, Frederic A. Kobayashi, Takeshi Pruski, Marek TI Natural Abundance O-17 DNP Two-Dimensional and Surface-Enhanced NMR Spectroscopy SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID DYNAMIC NUCLEAR-POLARIZATION; SOLID-STATE NMR; ANGLE-SPINNING NMR; MAGNETIC-RESONANCE; DISTANCE MEASUREMENTS; NEUTRON-DIFFRACTION; MOLECULAR-DYNAMICS; BOND LENGTHS; MAS NMR; NANOPARTICLES AB Due to its extremely low natural abundance and quadrupolar nature, the O-17 nuclide is very rarely used for spectroscopic investigation of solids by NMR without isotope enrichment. Additionally, the applicability of dynamic nuclear polarization (DNP), which leads to O-17 sensitivity enhancements of 2 orders of magnitude, to 130 is wrought with challenges due to the lack of spin diffusion and low polarization transfer efficiency from H-1. Here, we demonstrate new DNP-based measurements that extend O-17 solid-state NMR beyond its current capabilities. The use of the PRESTO technique instead of conventional H-1-O-17 cross-polarization greatly improves the sensitivity and enables the facile measurement of undistorted line shapes and two-dimensional H-1-O-17 HETCOR NMR spectra as well as accurate internuclear distance measurements at natural abundance. This was applied for distinguishing hydrogen-bonded and lone O-17 sites on the surface of silica gel; the one-dimensional spectrum of which could not be used to extract such detail. Lastly, this greatly enhanced sensitivity has enabled, for the first time, the detection of surface hydroxyl sites on mesoporous silica at natural abundance, thereby extending the concept of DNP surface-enhanced NMR spectroscopy to the O-17 nuclide. C1 [Perras, Frederic A.; Kobayashi, Takeshi; Pruski, Marek] US DOE, Ames Lab, Ames, IA 50011 USA. [Pruski, Marek] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. RP Pruski, M (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. EM mpruski@iastate.edu FU U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Division of Materials Science and Engineering; Division of Chemical Sciences, Geosciences, and Biosciences; LDRD program; DOE [DE-AC02-07CH11358] FX We thank M. Carravetta and I. M. Haies for sharing their PRESTO-II pulse program, I. I. Slowing for synthesizing silica SBA-15, and J. Stebbins for 17O-enriched silica gel sample. This research is supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Division of Materials Science and Engineering (methods development), and Division of Chemical Sciences, Geosciences, and Biosciences (specific applications). Support for F.P. is through a Spedding Fellowship funded by the LDRD program. Ames Laboratory is operated for the DOE by Iowa State University under Contract No. DE-AC02-07CH11358. NR 43 TC 25 Z9 25 U1 13 U2 66 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUL 8 PY 2015 VL 137 IS 26 BP 8336 EP 8339 DI 10.1021/jacs.5b03905 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA CM8PP UT WOS:000357964400006 PM 26098846 ER PT J AU Wei, Y Zheng, JX Cui, SH Song, XH Su, YT Deng, WJ Wu, ZZ Wang, XW Wang, WD Rao, MM Lin, Y Wang, CM Amine, K Pan, F AF Wei, Yi Zheng, Jiaxin Cui, Suihan Song, Xiaohe Su, Yantao Deng, Wenjun Wu, Zhongzhen Wang, Xinwei Wang, Weidong Rao, Mumin Lin, Yuan Wang, Chongmin Amine, Khalil Pan, Feng TI Kinetics Tuning of Li-Ion Diffusion in Layered Li(NixMnyCoz)O-2 SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID RECHARGEABLE LITHIUM BATTERIES; POSITIVE ELECTRODE MATERIALS; MINIMUM ENERGY PATHS; ELASTIC BAND METHOD; ELECTROCHEMICAL PROPERTIES; COBALT SUBSTITUTION; CATHODE MATERIAL; SADDLE-POINTS; PERFORMANCE; LINI0.5MN0.5O2 AB Using ab initio calculations combined with experiments, we clarified how the kinetics of Li-ion diffusion can be tuned in LiNixMnyCozO2 (NMC, x + y + z = 1) materials. It is found that Li-ions tend to choose oxygen dumbbell hopping (ODH) at the early stage of charging (delithiation), and tetrahedral site hopping (TSH) begins to dominate when more than 1/3 Li-ions are extracted. In both ODH and TSH, the Li-ions surrounded by nickel (especially with low valence state) are more likely to diffuse with low activation energy and form an advantageous path. The Li slab space, which also contributes to the effective diffusion barriers, is found to be closely associated with the delithiation process (Ni oxidation) and the contents of Ni, Co, and Mn. C1 [Wei, Yi; Zheng, Jiaxin; Cui, Suihan; Song, Xiaohe; Su, Yantao; Deng, Wenjun; Wu, Zhongzhen; Wang, Xinwei; Lin, Yuan; Pan, Feng] Peking Univ, Shenzhen Grad Sch, Sch Adv Mat, Shenzhen 518055, Peoples R China. [Wang, Weidong] Shenzhen Tianjiao Technol Dev Co Ltd, Shenzhen 518119, Peoples R China. [Rao, Mumin] Shenzhen OptimumNano Energy Co Ltd, Shenzhen 518118, Peoples R China. [Wang, Chongmin] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Electrochem Technol Program, Argonne, IL 60439 USA. RP Pan, F (reprint author), Peking Univ, Shenzhen Grad Sch, Sch Adv Mat, Shenzhen 518055, Peoples R China. EM panfeng@pkusz.edu.cn RI Wang, Xinwei/I-2850-2012; lin, yuan/G-9390-2013 OI Wang, Xinwei/0000-0002-1191-8162; lin, yuan/0000-0003-3410-3588 FU National Project for EV Batteries, OptimumNano, Shenzhen [20121110]; Guangdong Innovation Team Project [2013N080]; Shenzhen Science and Technology Research Grant [ZDSY20130331145131323, CXZZ20120829172325895, JCYJ20120614150338154, JCYJ20130329181509637, JCYJ20140417144423201]; National Natural Science Foundation of China [51302007] FX The work was financially supported by National Project for EV Batteries (20121110, OptimumNano, Shenzhen), Guangdong Innovation Team Project (No. 2013N080), Shenzhen Science and Technology Research Grant (Nos. ZDSY20130331145131323, CXZZ20120829172325895, JCYJ20120614150338154, JCYJ20130329181509637, and JCYJ20140417144423201), and the National Natural Science Foundation of China (No. 51302007). NR 26 TC 36 Z9 36 U1 27 U2 152 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUL 8 PY 2015 VL 137 IS 26 BP 8364 EP 8367 DI 10.1021/jacs.5b04040 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA CM8PP UT WOS:000357964400013 PM 26098282 ER PT J AU Britto, S Leskes, M Hua, X Hebert, CA Shin, HS Clarke, S Borkiewicz, O Chapman, KW Seshadri, R Cho, J Grey, CP AF Britto, Sylvia Leskes, Michal Hua, Xiao Hebert, Claire-Alice Shin, Hyeon Suk Clarke, Simon Borkiewicz, Olaf Chapman, Karena W. Seshadri, Ram Cho, Jaephil Grey, Clare P. TI Multiple Redox Modes in the Reversible Lithiation of High-Capacity, Peierls-Distorted Vanadium Sulfide SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID SOLID-STATE NMR; KRISTALLSTRUKTUR DES PATRONITS; RAY-ABSORPTION SPECTROSCOPY; INITIO MOLECULAR-DYNAMICS; AUGMENTED-WAVE METHOD; RECHARGEABLE BATTERIES; CONVERSION REACTION; REACTION-MECHANISM; LITHIUM BATTERIES; CATHODE MATERIALS AB Vanadium sulfide VS4 in the patronite mineral structure is a linear chain compound comprising vanadium atoms coordinated by disulfide anions [S-2](2-). V-51 NMR shows that the material, despite having V formally in the d(1) configuration, is diamagnetic, suggesting potential dimerization through metal metal bonding associated with a Peierls distortion of the linear chains. This is supported by density functional calculations, and is also consistent with the observed alternation in V V distances of 2.8 and 3.2 angstrom along the chains. Partial lithiation results in reduction of the disulfide ions to sulfide S2-, via an internal redox process whereby an electron from V4+ is transferred to [S-2](2-) in oxidation of V4+ to V5+ and reduction of the [S-2](2-) to S2- to form Li3VS4 containing tetrahedral [VS4](3-) anions. On further lithiation this is followed by reduction of the V5+ in Li3VS4 to form Li3+xVS4 (x = 0.5-1), a mixed valent V4+/V5+ compound. Eventually reduction to Li2S plus elemental V occurs. Despite the complex redox processes involving both the cation and the anion occurring in this material, the system is found to be partially reversible between 0 and 3 V. The unusual redox processes in this system are elucidated using a suite of short-range characterization tools including V-51 nuclear magnetic resonance spectroscopy (NMR), S K-edge X-ray absorption near edge spectroscopy (XANES), and pair distribution function (PDF) analysis of X-ray data. C1 [Britto, Sylvia; Leskes, Michal; Hua, Xiao; Grey, Clare P.] Univ Cambridge, Dept Chem, Cambridge CB2 1EW, England. [Shin, Hyeon Suk] Ulsan Natl Inst Sci & Technol, Dept Chem, Ulsan, South Korea. [Shin, Hyeon Suk] Ulsan Natl Inst Sci & Technol, Dept Energy Engn, Ulsan, South Korea. [Hebert, Claire-Alice] Univ Calif Santa Barbara, Coll Creat Studies, Santa Barbara, CA 93106 USA. [Borkiewicz, Olaf; Chapman, Karena W.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Seshadri, Ram] Univ Calif Santa Barbara, Adv Mat Res Lab, Mitsubishi Chem Ctr, Santa Barbara, CA 93106 USA. [Cho, Jaephil] Ulsan Natl Inst Sci & Technol, Interdisciplinary Sch Green Energy, Nano Energy Mat Lab, Ulsan, South Korea. [Clarke, Simon] Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford OX1 3QR, England. RP Grey, CP (reprint author), Univ Cambridge, Dept Chem, Lensfield Rd, Cambridge CB2 1EW, England. EM cpg27@cam.ac.uk RI Leskes, Michal/J-4674-2015; Cho, Jaephil/E-4265-2010; Shin, Hyeon Suk/E-5901-2010; Seshadri, Ram/C-4205-2013; Hua, Xiao/M-4896-2015 OI Leskes, Michal/0000-0002-7172-9689; Seshadri, Ram/0000-0001-5858-4027; Hua, Xiao/0000-0002-8673-5678 FU Schlumberger Stichting Fund; European Research Council (EU ERC); California Nanosystems Institute [NSF CNS-0960316]; Hewlett-Packard; Materials Research Laboratory [DMR-1121053]; DOE Office of Science [DE-AC02-06CH11357] FX S.B. acknowledges Schlumberger Stichting Fund and European Research Council (EU ERC) for funding. J.C. thanks BK21 plus project of Korea. We thank Phoebe Allan and Andrew J. Morris, University of Cambridge, for useful discussions. We also thank Trudy Bolin and Tianpin Wu of Beamline 9-BM, Argonne National Laboratory, for help with XANES measurements. The DFT calculations were performed at the UCSB Center for Scientific Computing at UC Santa Barbara, supported by the California Nanosystems Institute (NSF CNS-0960316), Hewlett-Packard, and the Materials Research Laboratory (DMR-1121053). This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 56 TC 5 Z9 5 U1 21 U2 113 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUL 8 PY 2015 VL 137 IS 26 BP 8499 EP 8508 DI 10.1021/jacs.5b03395 PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA CM8PP UT WOS:000357964400035 PM 26053432 ER PT J AU Bainsla, L Mallick, AI Raja, MM Coelho, AA Nigam, AK Johnson, DD Alam, A Suresh, KG AF Bainsla, Lakhan Mallick, A. I. Raja, M. Manivel Coelho, A. A. Nigam, A. K. Johnson, D. D. Alam, Aftab Suresh, K. G. TI Origin of spin gapless semiconductor behavior in CoFeCrGa: Theory and Experiment SO PHYSICAL REVIEW B LA English DT Article ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET AB Despite a plethora of materials suggested for spintronic applications, a new class of materials has emerged, namely spin gapless semiconductors (SGS), which offers potentially more advantageous properties than existing ones. These magnetic semiconductors exhibit a finite band gap for one spin channel and a closed gap for the other. Here, supported by electronic-structure calculations, we report evidence of SGS behavior in equiatomic quaternary CoFeCrGa, having a cubic Heusler (prototype LiMgPdSn) structure but exhibiting chemical disorder (DO3 structure). CoFeCrGa is found to transform from SGS to half-metallic phase under pressure, which is attributed to unique electronic-structure features. The saturation magnetization (M-S) obtained at 8K agrees with the Slater-Pauling rule and the Curie temperature (T-C) is found to exceed 400 K. Carrier concentration (up to 250 K) and electrical conductivity are observed to be nearly temperature independent, prerequisites for SGS. The anomalous Hall coefficient is estimated to be 185 S/cm at 5K. Considering the SGS properties and high T-C, this material appears to be promising for spintronic applications. C1 [Bainsla, Lakhan; Mallick, A. I.; Alam, Aftab; Suresh, K. G.] Indian Inst Technol, Dept Phys, Bombay 400076, Maharashtra, India. [Raja, M. Manivel] Def Met Res Lab, Hyderabad 500058, Andhra Pradesh, India. [Coelho, A. A.] Univ Estadual Campinas UNICAMP, Inst Fis Gleb Wataghin, BR-13083970 Campinas, SP, Brazil. [Nigam, A. K.] Tata Inst Fundamental Res, DCMPMS, Bombay 4000005, Maharashtra, India. [Johnson, D. D.] US DOE, Ames Lab, Ames, IA 50011 USA. [Johnson, D. D.] Iowa State Univ Sci & Technol, Dept Mat Sci & Engn, Ames, IA 50011 USA. RP Suresh, KG (reprint author), Indian Inst Technol, Dept Phys, Bombay 400076, Maharashtra, India. EM suresh@phy.iitb.ac.in RI Bainsla, Lakhan/A-7315-2016; Inst. of Physics, Gleb Wataghin/A-9780-2017; OI Bainsla, Lakhan/0000-0001-9626-4278; Johnson, Duane/0000-0003-0794-7283 FU UGC, Government of India; ISRO, Government of India; TAP fellowship under the SEED Grant [13IRCCSG020]; U.S. Department of Energy (DOE), Office of Science, Basic Energy Science, Materials Sciences and Engineering Division; U.S. DOE [DE-AC02-07CH11358] FX One of the authors, L.B., would like to thank UGC, Government of India, for financial support through senior research fellowship (SRF). The authors convey their thanks to D. Buddhikot for his help in the resistivity measurements. K.G.S. thanks ISRO, Government of India, for the financial support. A.I.M. acknowledges the support from the TAP fellowship under the SEED Grant (project code No. 13IRCCSG020). Support, including computing resources, at Ames Laboratory (D.D.J.) was funded by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Science, Materials Sciences and Engineering Division. The Ames Laboratory is operated for the U.S. DOE by Iowa State University under Contract No. DE-AC02-07CH11358. NR 24 TC 7 Z9 7 U1 3 U2 31 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 8 PY 2015 VL 92 IS 4 AR 045201 DI 10.1103/PhysRevB.92.045201 PG 5 WC Physics, Condensed Matter SC Physics GA CM4EA UT WOS:000357635900004 ER PT J AU Gangadharan, D AF Gangadharan, Dhevan TI Techniques for multiboson interferometry SO PHYSICAL REVIEW C LA English DT Article ID BOSE-EINSTEIN CORRELATIONS; RELATIVISTIC NUCLEAR COLLISIONS; HEAVY-ION GENERATOR; COULOMB CORRECTIONS; DISTRIBUTIONS; INTERFERENCE; THERMINATOR; PARTICLES; SYSTEMS; DECAY AB The quantum statistics (QS) correlations of identical bosons are well known to be sensitive to the space-time extent and dynamics of the particle emitting source in high-energy collisions. While two-pion correlations are most often experimentally measured, the QS correlations of three pions and higher are rarely explored. A set of techniques to isolate and analyze three-and four-pion QS correlations is presented. In particular, the technique of built correlation functions allows one to more easily study the effects of quantum coherence at finite relative momenta instead of at the unmeasured intercept of correlation functions. C1 Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. RP Gangadharan, D (reprint author), Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM dhevan.raja.gangadharan@cern.ch FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX I would like to thank Sergiy Akkelin, Richard Lednicky and Constantin Loizides for numerous helpful discussions. This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 46 TC 2 Z9 2 U1 0 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD JUL 8 PY 2015 VL 92 IS 1 AR 014902 DI 10.1103/PhysRevC.92.014902 PG 18 WC Physics, Nuclear SC Physics GA CM4EL UT WOS:000357637100002 ER PT J AU Zhao, PW Itagaki, N Meng, J AF Zhao, P. W. Itagaki, N. Meng, J. TI Rod-shaped Nuclei at Extreme Spin and Isospin SO PHYSICAL REVIEW LETTERS LA English DT Article ID ROTATION; STATES; CLUSTER; DY-152; MG-24; O-16; LINE AB The anomalous rod shape in carbon isotopes has been investigated in the framework of the cranking covariant density functional theory, and two mechanisms to stabilize such a novel shape with respect to the bending motion, extreme spin, and isospin are simultaneously discussed for the first time in a self-consistent and microscopic way. By adding valence neutrons and rotating the system, we have found the mechanism stabilizing the rod shape; i.e., the sigma orbitals (parallel to the symmetry axis) of the valence neutrons, important for the rod shape, are lowered by the rotation due to the Coriolis term. The spin and isospin effects enhance the stability of the rod-shaped configuration. This provides a strong hint that a rod shape could be realized in nuclei towards extreme spin and isospin. C1 [Zhao, P. W.; Itagaki, N.] Kyoto Univ, Yukawa Inst Theoret Phys, Kyoto 6068502, Japan. [Zhao, P. W.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Zhao, P. W.; Meng, J.] Peking Univ, Sch Phys, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Meng, J.] Beihang Univ, Sch Phys & Nucl Energy Engn, Beijing 100191, Peoples R China. [Meng, J.] Univ Stellenbosch, Dept Phys, ZA-7602 Stellenbosch, South Africa. RP Zhao, PW (reprint author), Kyoto Univ, Yukawa Inst Theoret Phys, Kyoto 6068502, Japan. EM mengj@pku.edu.cn RI Meng, Jie/B-8548-2009; Zhao, Pengwei/F-9107-2010 OI Meng, Jie/0000-0002-0977-5318; Zhao, Pengwei/0000-0001-8243-2381 FU Chinese Major State 973 Program [2013CB834402]; NSFC [11175002, 11105005, 11335002]; U.S. Department of Energy (DOE), Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357] FX This work is partly supported by the Chinese Major State 973 Program 2013CB834402, by the NSFC (Grants No. 11175002, No. 11105005, and No. 11335002), and by U.S. Department of Energy (DOE), Office of Science, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357. Numerical computation was carried out at the Yukawa Institute Computer Facility and the computing resources of the Laboratory Computing Resource Center at Argonne National Laboratory. NR 48 TC 16 Z9 16 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 8 PY 2015 VL 115 IS 2 AR 022501 DI 10.1103/PhysRevLett.115.022501 PG 6 WC Physics, Multidisciplinary SC Physics GA CM4HJ UT WOS:000357645000006 PM 26207464 ER PT J AU Yachdav, G Goldberg, T Wilzbach, S Dao, D Shih, I Choudhary, S Crouch, S Franz, M Garcia, A Garcia, LJ Gruning, BA Inupakutika, D Sillitoe, I Thanki, AS Vieira, B Villaveces, JM Schneider, MV Lewis, S Pettifer, S Rost, B Corpas, M AF Yachdav, Guy Goldberg, Tatyana Wilzbach, Sebastian Dao, David Shih, Iris Choudhary, Saket Crouch, Steve Franz, Max Garcia, Alexander Garcia, Leyla J. Gruening, Bjorn A. Inupakutika, Devasena Sillitoe, Ian Thanki, Anil S. Vieira, Bruno Villaveces, Jose M. Schneider, Maria V. Lewis, Suzanna Pettifer, Steve Rost, Burkhard Corpas, Manuel TI Anatomy of BioJS, an open source community for the life sciences SO ELIFE LA English DT Article ID BIOLOGICAL DATA; 3D STRUCTURES; CATH AB BioJS is an open source software project that develops visualization tools for different types of biological data. Here we report on the factors that influenced the growth of the BioJS user and developer community, and outline our strategy for building on this growth. The lessons we have learned on BioJS may also be relevant to other open source software projects. C1 [Yachdav, Guy; Goldberg, Tatyana; Wilzbach, Sebastian; Dao, David; Shih, Iris; Rost, Burkhard] Tech Univ Munich, Bioinformat, Garching, Germany. [Yachdav, Guy; Goldberg, Tatyana; Rost, Burkhard] Tech Univ Munich, Grad Sch, Ctr Doctoral Studies Informat & Its Applicat, Garching, Germany. [Yachdav, Guy; Rost, Burkhard] Biosof LLC, New York, NY USA. [Choudhary, Saket] Univ So Calif, Mol & Computat Biol, Los Angeles, CA USA. [Crouch, Steve; Inupakutika, Devasena] Univ Southampton, Web & Internet Sci, Southampton, Hants, England. [Franz, Max] Univ Toronto, Banting & Best Dept Med Res, Donnelly Ctr Cellular & Biomol Res, Toronto, ON, Canada. [Garcia, Alexander] Linkingdata IO LLC, Austin, TX USA. [Garcia, Leyla J.] European Bioinformat Inst, European Mol Biol Lab, Cambridge, England. [Gruening, Bjorn A.] Univ Freiburg, Dept Comp Sci, Bioinformat Grp, D-79106 Freiburg, Germany. [Gruening, Bjorn A.] Univ Freiburg, Ctr Biol Syst Anal, D-79106 Freiburg, Germany. [Sillitoe, Ian] UCL, Inst Struct & Mol Biol, London, England. [Thanki, Anil S.; Schneider, Maria V.; Corpas, Manuel] Genome Anal Ctr, Norwich, Norfolk, England. [Vieira, Bruno] Queen Mary Univ London, Sch Biol & Chem Sci, London, England. [Villaveces, Jose M.] Max Planck Inst Biochem, Planegg, Germany. [Lewis, Suzanna] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Pettifer, Steve] Univ Manchester, Sch Comp Sci, Manchester, Lancs, England. RP Yachdav, G (reprint author), Tech Univ Munich, Bioinformat, Garching, Germany. EM gyachdav@bio-sof.com; manuel.corpas@tgac.ac.uk RI Choudhary, Saket/H-8655-2014; OI Choudhary, Saket/0000-0001-5202-7633; Vieira, Bruno/0000-0002-4878-6431; Wilzbach, Sebastian/0000-0002-0083-9987; Thanki, Anil/0000-0002-8941-444X; Gruning, Bjorn/0000-0002-3079-6586 FU Biotechnology and Biological Sciences Research Council (BBSRC); Google; Engineering and Physical Sciences Research Council (EPSRC) [EP/H043160/1] FX Biotechnology and Biological Sciences Research Council (BBSRC) Manuel Corpas, Anil S Thanki, Maria V Schneider; Google Sebastian Wilzbach, David Dao; Engineering and Physical Sciences Research Council (EPSRC) EP/H043160/1 Steve Crouch, Devasena Inupakutika NR 22 TC 5 Z9 5 U1 0 U2 2 PU ELIFE SCIENCES PUBLICATIONS LTD PI CAMBRIDGE PA SHERATON HOUSE, CASTLE PARK, CAMBRIDGE, CB3 0AX, ENGLAND SN 2050-084X J9 ELIFE JI eLife PD JUL 8 PY 2015 VL 4 AR e07009 DI 10.7554/eLife.07009 PG 7 WC Biology SC Life Sciences & Biomedicine - Other Topics GA CM3OD UT WOS:000357590900001 ER PT J AU Crowhurst, JC Jeffries, JR Aberg, D Zaug, JM Dai, ZR Siekhaus, WJ Teslich, NE Holliday, KS Knight, KB Nelson, AJ Hutcheon, ID AF Crowhurst, J. C. Jeffries, J. R. Aberg, D. Zaug, J. M. Dai, Z. R. Siekhaus, W. J. Teslich, N. E. Holliday, K. S. Knight, K. B. Nelson, A. J. Hutcheon, I. D. TI A combined theoretical and experimental investigation of uranium dioxide under high static pressure SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE UO2; high pressure; Raman spectroscopy; electrical transport; optical transmission; DFT ID INDUCED PHASE-TRANSFORMATION; INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; RAMAN-SPECTROSCOPY; FLUORITE STRUCTURE; GPA; UO2; OXIDATION; OXIDES AB We have investigated the behavior of uranium dioxide (UO2) under high static pressure using a combination of experimental and theoretical techniques. We have made Raman spectroscopic measurements up to 87 GPa, electrical transport measurements up to 50 GPa from 10K to room temperature, and optical transmission measurements up to 28 GPa. We have also carried out theoretical calculations within the GGA+U framework. We find that Raman frequencies match to a large extent, theoretical predictions for the cotunnite (Pnma) structure above 30 GPa, but at higher pressures some behavior is not captured theoretically. The Raman measurements also imply that the low-pressure fluorite phase coexists with the cotunnite phase up to high pressures, consistent with earlier reports. Electrical transport measurements show that the resistivity decreases by more than six orders of magnitude with increasing pressure up to 50 GPa but that the material never adopts archetypal metallic behavior. Optical transmission spectra show that while UO2 becomes increasingly opaque with increasing pressure, a likely direct optical band gap of more than 1 eV exists up to at least 28 GPa. Together with the electrical transport measurements, we conclude that the high pressure electrical conductivity of UO2 is mediated by variable-range hopping. C1 [Crowhurst, J. C.; Jeffries, J. R.; Aberg, D.; Zaug, J. M.; Dai, Z. R.; Siekhaus, W. J.; Teslich, N. E.; Holliday, K. S.; Knight, K. B.; Nelson, A. J.; Hutcheon, I. D.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94551 USA. RP Crowhurst, JC (reprint author), Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94551 USA. EM crowhurst1@llnl.gov FU US Department of Energy by Lawrence Livermore National Security, LLC [DE-AC52-07NA27344]; Laboratory Directed Research and Development Program at LLNL [10-SI-016] FX First and foremost we would like to acknowledge the deep debt we owe our friend and colleague, Dr Ian D Hutcheon, for the benefit of his tremendous expertise as well as his unflagging support and enthusiasm. He will be greatly missed. We are grateful to K Syassen, AF Goncharov, HF Shaw, and PG Allen for reading earlier versions of the manuscript and for much useful advice. We are also grateful to Z Jenei, MR Armstrong, G C Allen, J G Tobin, L E Fried, W J Evans, and M A Wall. We are grateful to R J Gross for polishing our samples. This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Security, LLC under Contract DE-AC52-07NA27344 and supported by the Laboratory Directed Research and Development Program (10-SI-016) at LLNL. NR 42 TC 0 Z9 0 U1 6 U2 47 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD JUL 8 PY 2015 VL 27 IS 26 AR 265401 DI 10.1088/0953-8984/27/26/265401 PG 13 WC Physics, Condensed Matter SC Physics GA CL0FU UT WOS:000356616700006 PM 26053594 ER PT J AU Dane, M Kim, SK Surh, MP Aberg, D Benedict, LX AF Daene, Markus Kim, Soo Kyung Surh, Michael P. Aberg, Daniel Benedict, Lorin X. TI Density functional theory calculations of magnetocrystalline anisotropy energies for (Fe1-xCox)(2)B SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE magnetocrystalline anisotropy; denisty functional theory; permanent magnet; curie temperature ID AUGMENTED-WAVE METHOD; INITIO MOLECULAR-DYNAMICS; BASIS-SET; ALLOYS; METALS AB We present and discuss density functional theory calculations of magnetic properties of the family of ferromagnetic compounds, (Fe1-xCox)(2)B, focusing specifically on the magnetocrystalline anisotropy energy (MAE). Using periodic supercells of various sizes (up to 96 atoms), it is shown that the general qualitative features of the composition dependence of the MAE is in agreement with experimental findings, while our predicted magnitudes are larger than those of experiment. We find that the use of small supercells (6 and 12-atom) favors larger MAE values relative to a statistical sample of configurations constructed with 96-atom supercells. The effect of lattice relaxations is shown to be small. Calculations of the Curie temperature for this alloy are also presented. C1 [Daene, Markus; Surh, Michael P.; Aberg, Daniel; Benedict, Lorin X.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Kim, Soo Kyung] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA. RP Dane, M (reprint author), Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94551 USA. EM daene1@unl.gov FU Laboratory Directed Research and Development (LDRD) Program at LLNL [13-ERD-044]; Critical Materials Institute (CMI); Energy Innovation Hub - US Department of Energy; US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We thank B Sadigh for many helpful suggestions. This work was supported by the Laboratory Directed Research and Development (LDRD) Program at LLNL under tracking code No. 13-ERD-044, and the Critical Materials Institute (CMI), an Energy Innovation Hub funded by the US Department of Energy. Tc and 96-atom supercell MAE calculations were performed under the LDRD, and 12-atom supercell MAE calculations were performed within the CMI. Investigations of the local spin moments were performed under both LDRD (VASP calculations), and CMI (KKR-ASA calculations). This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 35 TC 2 Z9 2 U1 1 U2 10 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD JUL 8 PY 2015 VL 27 IS 26 AR 266002 DI 10.1088/0953-8984/27/26/266002 PG 11 WC Physics, Condensed Matter SC Physics GA CL0FU UT WOS:000356616700014 PM 26075465 ER PT J AU Huang, L Cong, DY Wang, ZL Nie, ZH Dong, YH Zhang, Y Ren, Y Wang, YD AF Huang, L. Cong, D. Y. Wang, Z. L. Nie, Z. H. Dong, Y. H. Zhang, Y. Ren, Y. Wang, Y. D. TI Direct evidence for stress-induced transformation between coexisting multiple martensites in a Ni-Mn-Ga multifunctional alloy SO JOURNAL OF PHYSICS D-APPLIED PHYSICS LA English DT Article DE magnetic shape memory alloy; martensitic transformation; external-field-induced structural transformation ID SHAPE-MEMORY ALLOYS; FIELD-INDUCED STRAIN; CRYSTAL-STRUCTURE; PHASE-TRANSFORMATION; NIMNGA ALLOYS; SN ALLOYS; X-RAY; DEPENDENCE AB The structural response of coexisting multiple martensites to stress field in a Ni-Mn-Ga multifunctional alloy was investigated by the in situ high-energy x-ray diffraction technique. Stress-induced transformation between coexisting multiple martensites was observed at 110 K, at which five-layered modulated (5M), seven-layered modulated (7M) and non-modulated (NM) martensites coexist. We found that a tiny stress of as low as 0.5 MPa could trigger the transformation from 5M and 7M martensites to NM martensite and this transformation is partly reversible. Besides the transformation between coexisting multiple martensites, rearrangement of martensite variants also occurs during loading, at least at high stress levels. The present study is instructive for designing advanced multifunctional alloys with easy actuation. C1 [Huang, L.; Cong, D. Y.; Dong, Y. H.; Zhang, Y.; Wang, Y. D.] Univ Sci & Technol Beijing, State Key Lab Adv Met & Mat, Beijing 100083, Peoples R China. [Huang, L.; Wang, Z. L.; Nie, Z. H.] Beijing Inst Technol, Sch Mat Sci & Engn, Beijing 100081, Peoples R China. [Ren, Y.] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Cong, DY (reprint author), Univ Sci & Technol Beijing, State Key Lab Adv Met & Mat, 30 Xueyuan Rd, Beijing 100083, Peoples R China. EM dycong@ustb.edu.cn; ydwang@ustb.edu.cn RI wang, yandong/G-9404-2013; ZHANG, Yong/B-7928-2009; Nie, Zhihua/G-9459-2013 OI ZHANG, Yong/0000-0002-6355-9923; Nie, Zhihua/0000-0002-2533-933X FU National Basic Research Program of China (973 Program) [2012CB619405]; National Natural Science Foundation of China [51471030, 11305008]; National 863 Program of China [2015AA034101]; Fundamental Research Funds for the Central Universities [06111023, 06111020]; NPL, CAEP [2013DB02]; Beijing Higher Education Young Elite Teacher Project [YETP0410]; State Key Laboratory for Advanced Metals and Materials [2014Z-01, 2014Z-02]; US Department of Energy, Office of Science, Office of Basic Energy Science [DE-AC02-06CH11357] FX We acknowledge the support from the National Basic Research Program of China (973 Program) under Contract No. 2012CB619405, the National Natural Science Foundation of China (Nos. 51471030 and 11305008), the National 863 Program of China (Grant No. 2015AA034101), the Fundamental Research Funds for the Central Universities (Nos. 06111023 and 06111020), the NPL, CAEP (Project No. 2013DB02), the Beijing Higher Education Young Elite Teacher Project (No. YETP0410), and the financial support (Grant Nos. 2014Z-01 and 2014Z-02) by the State Key Laboratory for Advanced Metals and Materials. Use of the Advanced Photon Source was supported by the US Department of Energy, Office of Science, Office of Basic Energy Science, under Contract No. DE-AC02-06CH11357. NR 41 TC 3 Z9 3 U1 4 U2 39 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0022-3727 EI 1361-6463 J9 J PHYS D APPL PHYS JI J. Phys. D-Appl. Phys. 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Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Search for low-scale gravity signatures in multi-jet final states with the ATLAS detector at root s=8 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Exotics; Hadron-Hadron Scattering ID MILLIMETER; DIMENSIONS; HIERARCHY; LHC AB A search for evidence of physics beyond the Standard Model in final states with multiple high-transverse-momentum jets is performed using 20.3 fb(-1) of proton-proton collision data at root s = 8TeV recorded by the ATLAS detector at the LHC. No significant excess of events beyond Standard Model expectations is observed, and upper limits on the visible cross sections for non-Standard Model production of multi-jet final states are set. A wide variety of models for black hole and string ball production and decay are considered, and the upper limit on the cross section times acceptance is as low as 0.16 fb at the 95% confidence level. 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L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Garzon, G. Otero Y.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Gonzalez, B. Alvarez; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Iengo, P.; Jaekel, M. R.; Jakobsen, S.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pomme, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Pezoa, R.; Prokoshin, F.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China. [Chen, S.; Guo, J.; Li, Y.; Wang, C.] Nanjing Univ, Dept Phys, Nanjing 210008, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Theveneaux-Pelzer, T.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Thompson, E. N.; Tuts, P. M.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Lab Nazl Frascati, INFN Grp Collegato Cosenza, Arcavacata Di Rende, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Curatolo, M.; Esposito, B.; Gatti, C.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Ancu, L. S.; Barone, G.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Paolozzi, L.; Picazio, A.; Ristic, B.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Izzo, V.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R. W.; Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Jansky, R. W.; Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.; Usanova, A.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, S.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] INFN Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Allport, P. P.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Aloisio, A.; Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Poettgen, R.; Rave, S.; Sander, H. G.; Schaeffer, J.; Afer, U. Sch; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Hughes, E. W.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Hu, X.; Levin, D.; Long, J. D.; Lu, N.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Napoli, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Koenig, A. C.; Nektarijevic, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Tanaka, R.; Zerwas, D.] CNRS IN2P3, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Berta, P.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Sawyer, C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, I-56010 Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Hong, T. M.; Kuze, M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Fac Ciencias & Tecnol, Caparica, Portugal. Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.; Trovatelli, M.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] Commissariat Energie Atom & Energies Alternat, CEA Saclay, IRFU, DSM, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Mount, R.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnuclear Phys, Kosice 04353, Slovakia. [Hamilton, A.; Meehan, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Govender, N.; Lee, C. A.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hamity, G. N.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Astron & Chem, Stony Brook, NY 11794 USA. [Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Hsu, P. J.; Jamin, D. O.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Munwes, Y.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Ilic, N.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Jovicevic, J.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] INFN Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Neubauer, M. S.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Brost, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, IFIC, Valencia, Spain. [Aloisio, A.; Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, IMB, CNM, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Swedish, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.; Turgeman, D.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Aloisio, A.; Bannoura, A. A. E.; Beermann, T. A.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Thomsen, L. A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London, England. [Ahmadov, F.; Huseynov, N.; Javadov, N.] Azerbaijan Acad Sci, Inst Phys, Baku, Azerbaijan. [Anisenkov, A. V.; Bawa, H. S.; Bobrovnikov, V. S.; Buzykaev, A. R.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Azuelos, G.; Gingrich, D. M.; Oakham, F. G.; Savard, P.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Gao, Y. S.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beck, H. P.] Univ Fribourg, Dept Phys, CH-1700 Fribourg, Switzerland. [Castro, N. F.] Univ Porto, Fac Ciencias, Dept Fis & Astron, P-4100 Oporto, Portugal. [Chelkov, G. A.] Tomsk State Univ, Tomsk 634050, Russia. [Chen, L.] Aix Marseille Univ, CPPM, Marseille, France. [Chen, L.] CNRS IN2P3, Marseille, France. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] Inst Particle Phys, Toronto, ON, Canada. [Davies, E.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Barcelona, Spain. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu 30013, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Jenni, P.] CERN, Geneva, Switzerland. [Khubua, J.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellen Open Univ, Patras, Greece. [Li, B.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Li, Y.] Univ Paris 11, LAL, Orsay, France. [Li, Y.] CNRS IN2P3, Orsay, France. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Liu, B.] Shandong Univ, Sch Phys, Jian, Shandong, Peoples R China. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] State Univ, Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tikhomirov, V. O.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Xu, L.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Mitsou, Vasiliki/D-1967-2009; Smirnova, Oxana/A-4401-2013; Doyle, Anthony/C-5889-2009; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Boyko, Igor/J-3659-2013; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Chekulaev, Sergey/O-1145-2015; Gerbaudo, Davide/J-4536-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Martinez, Mario /I-3549-2015; Peleganchuk, Sergey/J-6722-2014; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Tikhomirov, Vladimir/M-6194-2015; Snesarev, Andrey/H-5090-2013; Kantserov, Vadim/M-9761-2015; Villa, Mauro/C-9883-2009; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; Staroba, Pavel/G-8850-2014; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Warburton, Andreas/N-8028-2013; spagnolo, stefania/A-6359-2012; Buttar, Craig/D-3706-2011; Brooks, William/C-8636-2013; Di Domenico, Antonio/G-6301-2011; Gorelov, Igor/J-9010-2015; Livan, Michele/D-7531-2012; Gladilin, Leonid/B-5226-2011; Carvalho, Joao/M-4060-2013; White, Ryan/E-2979-2015; Mashinistov, Ruslan/M-8356-2015 OI Mitsou, Vasiliki/0000-0002-1533-8886; Smirnova, Oxana/0000-0003-2517-531X; Doyle, Anthony/0000-0001-6322-6195; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Boyko, Igor/0000-0002-3355-4662; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Tikhomirov, Vladimir/0000-0002-9634-0581; Kantserov, Vadim/0000-0001-8255-416X; Villa, Mauro/0000-0002-9181-8048; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Camarri, Paolo/0000-0002-5732-5645; Warburton, Andreas/0000-0002-2298-7315; spagnolo, stefania/0000-0001-7482-6348; Brooks, William/0000-0001-6161-3570; Di Domenico, Antonio/0000-0001-8078-2759; Gorelov, Igor/0000-0001-5570-0133; Livan, Michele/0000-0002-5877-0062; Gladilin, Leonid/0000-0001-9422-8636; Carvalho, Joao/0000-0002-3015-7821; White, Ryan/0000-0003-3589-5900; Mashinistov, Ruslan/0000-0001-7925-4676 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; RGC, China; Hong Kong SAR, China; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; RGC, Hong Kong SAR, China; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 43 TC 1 Z9 1 U1 8 U2 53 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JUL 7 PY 2015 IS 7 AR 032 DI 10.1007/JHEP07(2015)032 PG 38 WC Physics, Particles & Fields SC Physics GA CU4LR UT WOS:000363501800003 ER PT J AU Sali, A Berman, HM Schwede, T Trewhella, J Kleywegt, G Burley, SK Markley, J Nakamura, H Adams, P Bonvin, AMJJ Chiu, W Dal Peraro, M Di Maio, F Ferrin, TE Grunewald, K Gutmanas, A Henderson, R Hummer, G Iwasaki, K Johnson, G Lawson, CL Meiler, J Marti-Renom, MA Montelione, GT Nilges, M Nussinov, R Patwardhan, A Rappsilber, J Read, RJ Saibil, H Schroder, GF Schwieters, CD Seidel, CAM Svergun, D Topf, M Ulrich, EL Velankar, S Westbrook, JD AF Sali, Andrej Berman, Helen M. Schwede, Torsten Trewhella, Jill Kleywegt, Gerard Burley, Stephen K. Markley, John Nakamura, Haruki Adams, Paul Bonvin, Alexandre M. J. J. Chiu, Wah Dal Peraro, Matteo Di Maio, Frank Ferrin, Thomas E. Gruenewald, Kay Gutmanas, Aleksandras Henderson, Richard Hummer, Gerhard Iwasaki, Kenji Johnson, Graham Lawson, Catherine L. Meiler, Jens Marti-Renom, Marc A. Montelione, Gaetano T. Nilges, Michael Nussinov, Ruth Patwardhan, Ardan Rappsilber, Juri Read, Randy J. Saibil, Helen Schroeder, Gunnar F. Schwieters, Charles D. Seidel, Claus A. M. Svergun, Dmitri Topf, Maya Ulrich, Eldon L. Velankar, Sameer Westbrook, John D. TI Outcome of the First wwPDB Hybrid/Integrative Methods Task Force Workshop SO STRUCTURE LA English DT News Item ID ANGLE SCATTERING DATA; PROTEIN DATA-BANK; X-RAY-SCATTERING; MASS-SPECTROMETRY; BINDING-PROTEIN; CROSS-LINKING; ELECTRON-MICROSCOPY; STRUCTURAL BIOLOGY; NMR-SPECTROSCOPY; NUCLEIC-ACID AB Structures of biomolecular systems are increasingly computed by integrative modeling that relies on varied types of experimental data and theoretical information. We describe here the proceedings and conclusions from the first wwPDB Hybrid/Integrative Methods Task Force Workshop held at the European Bioinformatics Institute in Hinxton, UK, on October 6 and 7, 2014. At the workshop, experts in various experimental fields of structural biology, experts in integrative modeling and visualization, and experts in data archiving addressed a series of questions central to the future of structural biology. How should integrative models be represented? How should the data and integrative models be validated? What data should be archived? How should the data and models be archived? What information should accompany the publication of integrative models? C1 [Sali, Andrej] Univ Calif San Francisco, Dept Bioengn & Therapeut Sci, Dept Pharmaceut Chem, Calif Inst Quantitat Biosci, San Francisco, CA 94158 USA. [Berman, Helen M.; Burley, Stephen K.; Lawson, Catherine L.; Westbrook, John D.] Rutgers State Univ, Ctr Integrat Prote Res, Res Collaboratory Struct Bioinformat Prot Data Ba, Piscataway, NJ 08854 USA. [Schwede, Torsten] Univ Basel, Swiss Inst Bioinformat Biozentrum, CH-4056 Basel, Switzerland. [Trewhella, Jill] Univ Sydney, Sch Mol Biosci, Sydney, NSW 2006, Australia. [Kleywegt, Gerard; Gutmanas, Aleksandras; Patwardhan, Ardan; Velankar, Sameer] European Bioinformat Inst, Protein Data Bank Europe, European Mol Biol Lab, Cambridge CB10 1SD, England. [Burley, Stephen K.] Univ Calif San Diego, Skaggs Sch Pharm & Pharmaceut Sci, La Jolla, CA 92093 USA. [Burley, Stephen K.] Univ Calif San Diego, San Diego Supercomp Ctr, La Jolla, CA 92093 USA. [Markley, John; Ulrich, Eldon L.] Univ Wisconsin, Dept Biochem, BioMagResBank, Madison, WI 53706 USA. [Nakamura, Haruki] Osaka Univ, Inst Prot Res, Protein Data Bank Japan, Suita, Osaka 5650871, Japan. [Adams, Paul] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Adams, Paul] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Bonvin, Alexandre M. J. J.] Univ Utrecht, Fac Sci Chem, Bijvoet Ctr Biomol Res, NL-3584 CH Utrecht, Netherlands. [Chiu, Wah] Baylor Coll Med, Natl Ctr Macromol Imaging, Houston, TX 77030 USA. [Dal Peraro, Matteo] Ecole Polytech Fed Lausanne, Sch Life Sci, Inst Bioengn, CH-1015 Lausanne, Switzerland. [Dal Peraro, Matteo] Swiss Inst Bioinformat, CH-1015 Lausanne, Switzerland. [Di Maio, Frank] Univ Washington, Dept Biochem, Seattle, WA 98195 USA. [Ferrin, Thomas E.] Univ Calif San Francisco, Dept Pharmaceut Chem, San Francisco, CA 94158 USA. [Ferrin, Thomas E.; Johnson, Graham] Univ Calif San Francisco, Dept Bioengn & Therapeut Sci, Calif Inst Quantitat Biosci, San Francisco, CA 94158 USA. [Gruenewald, Kay] Univ Oxford, Wellcome Trust Ctr Human Genet, Div Struct Biol, Oxford OX3 7BN, England. [Henderson, Richard] MRC Lab Mol Biol, Cambridge CB2 0QH, England. [Hummer, Gerhard] Max Planck Inst Biophys, Dept Theoret Biophys, D-60438 Frankfurt, Germany. [Iwasaki, Kenji] Osaka Univ, Inst Prot Res, Suita, Osaka 5650871, Japan. [Meiler, Jens] Vanderbilt Univ, Struct Biol Ctr, Dept Chem, Nashville, TN 37235 USA. [Marti-Renom, Marc A.] Ctr Genom Regulat, Genome Biol Grp, CNAG, Gene Regulat Stem Cells & Canc Program, Barcelona 08028, Spain. [Marti-Renom, Marc A.] ICREA, Barcelona 08028, Spain. [Montelione, Gaetano T.] Rutgers State Univ, Ctr Adv Biotechnol & Med, Dept Mol Biol & Biochem, Piscataway, NJ 08854 USA. [Montelione, Gaetano T.] Rutgers State Univ, Robert Wood Johnson Med Sch, Dept Biochem, Piscataway, NJ 08854 USA. [Nilges, Michael] Inst Pasteur, Unite Bioinformat Struct, Dept Biol Struct & Chim, F-75015 Paris, France. [Nilges, Michael] Ctr Natl Rech Sci, Unite Mixte Rech 3258, F-75015 Paris, France. [Nussinov, Ruth] NCI, Canc & Inflammat Program, Leidos Biomed Res Inc, Frederick Natl Lab, Frederick, MD 21702 USA. [Nussinov, Ruth] Tel Aviv Univ, Sackler Sch Med, Dept Human Mol Genet & Biochem, IL-69978 Tel Aviv, Israel. [Rappsilber, Juri] Univ Edinburgh, Inst Cell Biol, Wellcome Trust Ctr Cell Biol, Edinburgh EH9 3BF, Midlothian, Scotland. [Rappsilber, Juri] Tech Univ Berlin, Inst Biotechnol, Dept Bioanalyt, D-13355 Berlin, Germany. [Read, Randy J.] Univ Cambridge, Dept Haematol, Cambridge Inst Med Res, Cambridge CB2 0XY, England. [Saibil, Helen; Topf, Maya] Birkbeck Coll, Dept Biol Sci, Inst Struct & Mol Biol, London WC1E 7HX, England. [Schroeder, Gunnar F.] Forschungszentrum Julich, Inst Complex Syst ICS 6, D-52425 Julich, Germany. [Schroeder, Gunnar F.] Univ Dusseldorf, Phys Dept, D-40225 Dusseldorf, Germany. [Schwieters, Charles D.] NIH, Ctr Informat Technol, Div Computat Biosci, Bethesda, MD 20892 USA. [Seidel, Claus A. M.] Univ Dusseldorf, Chair Mol Phys Chem, D-40225 Dusseldorf, Germany. [Svergun, Dmitri] European Mol Biol Lab, Hamburg Unit, D-22607 Hamburg, Germany. RP Sali, A (reprint author), Univ Calif San Francisco, Dept Bioengn & Therapeut Sci, Dept Pharmaceut Chem, Calif Inst Quantitat Biosci, Byers Hall Room 503B,1700 4th St, San Francisco, CA 94158 USA. EM sali@salilab.org RI Bonvin, Alexandre/A-5420-2009; Read, Randy/L-1418-2013; Schroder, Gunnar/H-5261-2013; Hummer, Gerhard/A-2546-2013; Nilges, Michael/E-4803-2011; Seidel, Claus/A-3682-2012; OI Kleywegt, Gerard J./0000-0002-4670-0331; Patwardhan, Ardan/0000-0001-7663-9028; Velankar, Sameer/0000-0002-8439-5964; Grunewald, Kay/0000-0002-4788-2691; Rappsilber, Juri/0000-0001-5999-1310; Bonvin, Alexandre/0000-0001-7369-1322; Gutmanas, Aleksandras/0000-0001-6311-0176; Read, Randy/0000-0001-8273-0047; Schroder, Gunnar/0000-0003-1803-5431; Hummer, Gerhard/0000-0001-7768-746X; Nilges, Michael/0000-0002-1451-8092; Seidel, Claus/0000-0002-5171-149X; Marti-Renom, Marc A./0000-0002-0151-4279; Meiler, Jens/0000-0001-8945-193X FU Wellcome Trust [088944]; NSF DBI [1338415]; JST-NBDC; NLM [P41 LM05799]; NIH [GM079429]; wwPDB outreach activities FX The workshop was supported by funding to PDBe by Wellcome Trust 088944; RCSB PDB by NSF DBI 1338415; PDBj by JST-NBDC; BMRB by NLM P41 LM05799; EMDataBank by NIH GM079429; and tax-deductible donations made to the wwPDB Foundation in support of wwPDB outreach activities. NR 73 TC 26 Z9 26 U1 5 U2 20 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0969-2126 EI 1878-4186 J9 STRUCTURE JI Structure PD JUL 7 PY 2015 VL 23 IS 7 BP 1156 EP 1167 DI 10.1016/j.str.2015.05.013 PG 12 WC Biochemistry & Molecular Biology; Biophysics; Cell Biology SC Biochemistry & Molecular Biology; Biophysics; Cell Biology GA CQ0UG UT WOS:000360312200004 PM 26095030 ER PT J AU Segrest, JP Jones, MK Catte, A Manchekar, M Datta, G Zhang, L Zhang, R Li, L Patterson, JC Palgunachari, MN Oram, JF Ren, G AF Segrest, Jere P. Jones, Martin K. Catte, Andrea Manchekar, Medha Datta, Geeta Zhang, Lei Zhang, Robin Li, Ling Patterson, James C. Palgunachari, Mayakonda N. Oram, Jack F. Ren, Gang TI Surface Density-Induced Pleating of a Lipid Monolayer Drives Nascent High-Density Lipoprotein Assembly SO STRUCTURE LA English DT Article ID APOLIPOPROTEIN-A-I; COMPUTATIONAL-EXPERIMENTAL-APPROACH; CASSETTE TRANSPORTER 1; TANGIER-DISEASE; ELECTRON-MICROSCOPY; CELLULAR CHOLESTEROL; PLASMA-LIPOPROTEINS; MOLECULAR-DYNAMICS; NEUTRON-SCATTERING; AMPHIPATHIC HELIX AB Biogenesis of high-density lipoproteins (HDL) is coupled to the transmembrane protein, ATP-binding cassette transporter A1 (ABCA1), which transports phospholipid (PL) from the inner to the outer membrane monolayer. Using a combination of computational and experimental approaches, we show that increased outer lipid monolayer surface density, driven by excess PL or membrane insertion of amphipathic helices, results in pleating of the outer monolayer to form membrane-attached discoidal bilayers. Apolipoprotein (apo) A-I accelerates and stabilizes the pleats. In the absence of apoA-I, pleats collapse to form vesicles. These results mimic cells overexpressing ABCA1 that, in the absence of apoA-I, form and release vesicles. We conclude that the basic driving force for nascent discoidal HDL assembly is a PL pump-induced surface density increase that produces lipid monolayer pleating. We then argue that ABCA1 forms an extracellular reservoir containing an isolated pressurized lipid monolayer decoupled from the transbilayer density buffering of cholesterol. C1 [Segrest, Jere P.; Jones, Martin K.; Catte, Andrea; Manchekar, Medha; Datta, Geeta; Li, Ling; Palgunachari, Mayakonda N.] Univ Alabama Birmingham, Dept Med, Birmingham, AL 35294 USA. [Segrest, Jere P.; Jones, Martin K.; Catte, Andrea; Manchekar, Medha; Datta, Geeta; Li, Ling; Palgunachari, Mayakonda N.] Univ Alabama Birmingham, Atherosclerosis Res Unit, Birmingham, AL 35294 USA. [Segrest, Jere P.; Jones, Martin K.; Catte, Andrea] Univ Alabama Birmingham, Ctr Computat & Struct Dynam, Birmingham, AL 35294 USA. [Patterson, James C.] Univ Alabama Birmingham, Dept Chem, Birmingham, AL 35294 USA. [Zhang, Lei; Zhang, Robin; Ren, Gang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Oram, Jack F.] Univ Washington, Dept Med, Seattle, WA 98109 USA. RP Segrest, JP (reprint author), Univ Alabama Birmingham, Dept Med, Birmingham, AL 35294 USA. EM segrest@uab.edu RI Foundry, Molecular/G-9968-2014; Zhang, Lei/G-6427-2012 OI Zhang, Lei/0000-0002-4880-824X FU NIH [P01HL34343, R01HL102515]; Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231] FX Thanks to UAB Information Technology and Department of Mechanical Engineering for use of the cluster Cheaha. A.C. thanks Manjula Chaddha, G.M. Anantharamaiah, and Vinod Mishra for helpful discussions. Thanks also to J.C. Gumbart of the Georgia Institute of Technology School of Physics for helpful discussions about lipid pressure profiles. Work supported by NIH grants P01HL34343 and R01HL102515 to J.P.S. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 48 TC 7 Z9 7 U1 1 U2 5 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0969-2126 EI 1878-4186 J9 STRUCTURE JI Structure PD JUL 7 PY 2015 VL 23 IS 7 BP 1214 EP 1226 DI 10.1016/j.str.2015.05.010 PG 13 WC Biochemistry & Molecular Biology; Biophysics; Cell Biology SC Biochemistry & Molecular Biology; Biophysics; Cell Biology GA CQ0UG UT WOS:000360312200009 PM 26095027 ER PT J AU Schivley, G Ingwersen, WW Marriott, J Hawkins, TR Skone, TJ AF Schivley, Greg Ingwersen, Wesley W. Marriott, Joe Hawkins, Troy R. Skone, Timothy J. TI Identifying/Quantifying Environmental Trade-offs Inherent in GHG Reduction Strategies for Coal-Fired Power SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID FLUIDIZED-BED COMBUSTION; METHANE LEAKAGE; NATURAL-GAS; AIR-QUALITY; BIOMASS; EMISSIONS; LIFE; US; ELECTRICITY; LCA AB Improvements to coal power plant technology and the cored combustion :of biomass promise direct greenhouse gas (GHG) reductions for existing coal-fired power plants. Questions remain as to what the reduction potentials are from a life cycle perspective and if it will result in unintended increases in impacts to air and water quality and human health. This study provides a Unique analysis of the potential environmental impact reductions froth upgrading existing subcritical pulverized coal power plants to increase their efficiency, improving environmental controls, cofiring biomass, and exporting steam for industrial use. The climate impacts are examined in both a traditional-100 year GWP-method and a time series analysis that accounts for emission and uptake timing over the life of the power plant. Compared to fleet average pulverized bed boilers (33% efficiency), we find that circulating fluidized bed boilers (39% efficiency) may provide GHG reductions of about 13% when using 100% coal and reductions of about 20-37% when cofiring with 30% biomass. Additional greenhouse gas reductions from combined heat and power are minimal if the steam coproduct displaces steam from an efficient natural gas boiler. These upgrades and cofiring biomass can also reduce other life cycle impacts, although there may be increased impacts to water quality (eutrophication) when using biomass from an intensely cultivated source. Climate change impacts are sensitive to the timing of emissions and carbon sequestration as well as the time horizon over which impacts are considered, particularly for long growth woody biomass. C1 [Schivley, Greg; Marriott, Joe] Booz Allen Hamilton, Pittsburgh, PA 15220 USA. [Ingwersen, Wesley W.; Hawkins, Troy R.] US EPA, Natl Risk Management Res Lab, Off Res & Dev, Cincinnati, OH 45220 USA. [Skone, Timothy J.] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. RP Schivley, G (reprint author), Booz Allen Hamilton, Pittsburgh, PA 15220 USA. EM schivley_greg@bah.com OI Schivley, Greg/0000-0002-8947-694X FU Air, Climate, and Energy Research Program of the U.S. Environmental Protection Agency, Office of Research and Development; Booz Allen Hamilton under DOE NETL [DE-FE0004001] FX We thank Chris Sherry, Greg Cooney, Matt Jamieson, James Littlefield, Francesco Cherubini, Rebecca Dodder, Carlos Nunez, and Michael Gonzalez for their assistance and insight. Research support provided by the Air, Climate, and Energy Research Program of the U.S. Environmental Protection Agency, Office of Research and Development. This work was performed as a collaboration between EPA NRML and DOE NETL staff with support from Booz Allen Hamilton under DOE NETL Contract Number DE-FE0004001. NR 49 TC 5 Z9 5 U1 7 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUL 7 PY 2015 VL 49 IS 13 BP 7562 EP 7570 DI 10.1021/acs.est.5b01118 PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CM6ZN UT WOS:000357840300010 PM 26001040 ER PT J AU Harding-Marjanovic, KC Houtz, EF Yi, S Field, JA Sedlak, DL Alvarez-Cohen, L AF Harding-Marjanovic, Katie C. Houtz, Erika F. Yi, Shan Field, Jennifer A. Sedlak, David L. Alvarez-Cohen, Lisa TI Aerobic Biotransformation of Fluorotelomer Thioether Amido Sulfonate (Lodyne) in AFFF-Amended Microcosms SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID FILM-FORMING FOAM; FIRE-TRAINING AREA; PERFLUOROALKYL ACIDS; PERFLUORINATED SURFACTANTS; ALCOHOL BIODEGRADATION; ACCIDENTAL RELEASE; FIREFIGHTING FOAM; ETOBICOKE CREEK; US MILITARY; GROUNDWATER AB The aerobic biotransformation pathways of 4:2, 6:2, and 8:2 fluorotelomer thioether amido sulfonate (FtTAoS) were characterized by determining the fate of the compounds in soil and medium microcosms amended with an aqueous film-forming foam (AFFF) solution. The biotransformation of FtTAoS occurred in live microcosms over approximately 40 days and produced 4:2, 6:2, and 8:2 fluorotelomer sulfonate (FtS), 6:2 fluorotelomer unsaturated carboxylic acid (FtUCA.), 5:3 fluorotelomer carboxylic acid (FtCA), and C-4 to C-8 perfluorinated carboxylic acids (PFCAs). Two biotransformation products corresponding to singly and doubly oxygenated forms of 6:2 FtTAoS were also identified through high resolution mass spectrometry (MS) analysis and liquid chromatography tandem-MS. An oxidative assay was used to indirectly quantify the total concentration of polyfluorinated compounds and check the mass balance. The assay produced near complete mass recovery of FtTAoS after biotransformation, with 10% (mol/mol) of the amended FtTAoS accounted for in FtS, FtCA, and PFCA products. The transformation rates of identified products appear to be slow relative to FtTAoS, indicating that some intermediates may persist in the environment. This study confirms some of the sources of FtS and PFCAs in groundwater and soil at AFFF-impacted sites and suggests that fluorinated intermediates that are not routinely measured during the biotransformation of PFASs may accumulate. C1 [Harding-Marjanovic, Katie C.; Houtz, Erika F.; Yi, Shan; Sedlak, David L.; Alvarez-Cohen, Lisa] Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA. [Field, Jennifer A.] Oregon State Univ, Dept Environm & Mol Toxicol, Corvallis, OR 97331 USA. [Alvarez-Cohen, Lisa] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Alvarez-Cohen, L (reprint author), Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA. EM alvarez@ce.berkeley.edu RI Yi, Shan/I-4589-2012 OI Yi, Shan/0000-0003-1371-0418 FU Strategic Environmental Research and Development Program (SERDP) [ER-2128] FX This study was supported by the Strategic Environmental Research and Development Program (SERDP), grant number ER-2128. The authors thank Professor Chris Higgins, Keenan Christensen, and Jennifer Guelfo at Colorado School of Mines for providing the soil used to conduct these experiments. NR 40 TC 11 Z9 11 U1 15 U2 62 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUL 7 PY 2015 VL 49 IS 13 BP 7666 EP 7674 DI 10.1021/acs.est.5b01219 PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CM6ZN UT WOS:000357840300022 PM 26042823 ER PT J AU Shao, HB Qafoku, NP Lawter, AR Bowden, ME Brown, CF AF Shao, Hongbo Qafoku, Nikolla P. Lawter, Amanda R. Bowden, Mark E. Brown, Christopher F. TI Coupled Geochemical Impacts of Leaking CO2 and Contaminants from Subsurface Storage Reservoirs on Groundwater Quality SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID FRESH-WATER RESOURCES; BATCH-REACTION EXPERIMENT; GEOLOGICAL STORAGE; SEQUESTRATION CONDITIONS; CARBON SEQUESTRATION; SITE SELECTION; CLIMATE-CHANGE; METAL RELEASE; LEAKAGE; SHALLOW AB The leakage of CO2 and: the concomitant brine from deep storage reservoirs to overlying groundwater aquifers is considered one of the major potential risks associated with geologic CO2 sequestration (GCS). In this work both batch and column experiments were Conducted to determine the fate of trace metals in groundwater in the scenarios of CO2 and metal-contaminated brine leakage. The sediments for this study were from an unconsolidated sand and gravel aquifer in Kansas, containing 0-4 wt % carbonates. Cd (114 mu g/L) and As (40 mu g/L) were spiked into the reaction system to represent potential contaminants from the reservoir brine. Through this research we demonstrated that Cd and As were adsorbed on the sediments, in spite of the lowered pH due to CO2 dissolution in the groundwater: Cd concentrations in the effluent were below the Cd MCL, even for sediments without detectable carbonate to buffer the pH. Arsenic concentrations in the effluent were also significantly lower than the influent concentration, suggesting that the sediments tested have the capacity to mitigate the coupled adverse effects of CO2 leakage and brine intrusion. The mitigation capacity of sediment is a function of its geochemical properties (e.g., the presence of carbonate minerals, adsorbed As, and phosphate). C1 [Shao, Hongbo; Qafoku, Nikolla P.; Lawter, Amanda R.; Bowden, Mark E.; Brown, Christopher F.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Shao, HB (reprint author), Illinois State Geol Survey, 615 East Peabody Dr,MC 650, Champaign, IL 61820 USA. EM hbshao@illinois.edu FU National Risk Assessment Partnership (NRAP) in the U.S. DOE Office of Fossil Energy under DOE Contract [DE AC05 76RL01830]; Department of Energy's Office of Biological and Environmental Research FX Funding for this research was provided by the National Risk Assessment Partnership (NRAP) in the U.S. DOE Office of Fossil Energy under DOE Contract Number DE AC05 76RL01830. XRD analyses were performed in the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at PNNL. NR 54 TC 6 Z9 6 U1 4 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUL 7 PY 2015 VL 49 IS 13 BP 8202 EP 8209 DI 10.1021/acs.est.5b01004 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CM6ZN UT WOS:000357840300084 PM 26039150 ER PT J AU Cai, H Brandt, AR Yeh, S Englander, JG Han, J Elgowainy, A Wang, MQ AF Cai, Hao Brandt, Adam R. Yeh, Sonia Englander, Jacob G. Han, Jeongwoo Elgowainy, Amgad Wang, Michael Q. TI Well-to-Wheels Greenhouse Gas Emissions of Canadian Oil Sands Products: Implications for US Petroleum Fuels SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID QUALITY; ENERGY; CARBON; MODEL AB Greenhouse gas (GHG) regulations affecting U.S. transportation fuels require holistic examination of the life-cycle emissions of U.S. petroleum feedstocks. With an expanded system boundary that included land disturbance-induced GHG emissions, we estimated well-to-wheels (WTW) GHG emissions of U.S. production of gasoline and diesel sourced from Canadian oil sands. Our analysis was based on detailed characterization of the energy intensities of 27 oil sands projects, representing industrial practices and technological advances since 2008. Four major oil sands production pathways were examined, including bitumen and synthetic crude oil (SCO) from both surface mining and in situ projects. Pathway-average GHG emissions from oil sands extraction, separation, and upgrading ranged from, similar to 6.1 to similar to 27.3 g CO2 equivalents per megajoule (in lower heating value, CO(2)e/MJ). This range can be compared to similar to 4.4 g CO(2)e/MJ for U.S. conventional crude oil recovery. Depending on the extraction technology and product type output of oil sands projects, the WTW GHG emissions for gasoline and diesel produced from bitumen and SCO in U.S. refineries were in the range of 100-115 and 99-117 g CO(2)e/MJ, respectively, representing, on average, about 18% and 21% higher emissions than those derived from U.S. conventional crudes. WTW GHG emissions of gasoline and diesel derived from diluted bitumen ranged from 97 to 103 and 96 to 104 g CO(2)e/M1 respectively, showing the effect of diluent use on fuel emissions. C1 [Cai, Hao; Han, Jeongwoo; Elgowainy, Amgad; Wang, Michael Q.] Argonne Natl Lab, Div Energy Syst, Syst Assessment Grp, Lemont, IL 60439 USA. [Brandt, Adam R.; Englander, Jacob G.] Stanford Univ, Dept Energy Resources Engn, Stanford, CA 94305 USA. [Yeh, Sonia] Univ Calif Davis, Inst Transportat Studies, Davis, CA 95616 USA. RP Cai, H (reprint author), Argonne Natl Lab, Div Energy Syst, Syst Assessment Grp, 9700 S Cass Ave, Lemont, IL 60439 USA. EM hcai@anl.gov RI Cai, Hao/A-1975-2016; OI Yeh, Sonia/0000-0002-4852-1177 FU Vehicle Technologies Office of the U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy; Bioenergy Technologies Office of the U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy [DE-AC02-06CH11357] FX This research effort was supported by the Vehicle Technologies Office and the Bioenergy Technologies Office of the U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy under Contract DE-AC02-06CH11357. We thank the anonymous reviewers of this paper for their helpful comments. The authors are solely responsible for the contents and results of the paper. NR 22 TC 10 Z9 10 U1 1 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUL 7 PY 2015 VL 49 IS 13 BP 8219 EP 8227 DI 10.1021/acs.est.5b01255 PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CM6ZN UT WOS:000357840300086 PM 26054375 ER PT J AU Im, J Walshe-Langford, GE Moon, JW Loffler, FE AF Im, Jeongdae Walshe-Langford, Gillian E. Moon, Ji-Won Loeffler, Frank E. TI Response to Comment on "Environmental Fate of the Next Generation Refrigerant 2,3,3,3-Tetrafluoropropene (HFO-1234yf)". SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Editorial Material ID GROUNDWATER C1 [Im, Jeongdae; Walshe-Langford, Gillian E.; Loeffler, Frank E.] Univ Tennessee, Ctr Environm Biotechnol, Knoxville, TN 37996 USA. [Im, Jeongdae; Walshe-Langford, Gillian E.; Loeffler, Frank E.] Univ Tennessee, Dept Microbiol, Knoxville, TN 37996 USA. [Moon, Ji-Won; Loeffler, Frank E.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Loeffler, Frank E.] Univ Tennessee & Oak Ridge Natl Lab UT ORNL Joint, Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Loeffler, Frank E.] Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN 37996 USA. RP Loffler, FE (reprint author), Univ Tennessee, Ctr Environm Biotechnol, Knoxville, TN 37996 USA. EM frank.loeffler@utk.edu RI Moon, Ji-Won/A-9186-2011 OI Moon, Ji-Won/0000-0001-7776-6889 NR 5 TC 1 Z9 1 U1 0 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUL 7 PY 2015 VL 49 IS 13 BP 8265 EP 8266 DI 10.1021/acs.est.5b01970 PG 2 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CM6ZN UT WOS:000357840300092 PM 26066073 ER PT J AU Charlton, JJ Jones, NC Wallace, RA Smithwick, RW Bradshaw, JA Kravchenko, II Lavrik, NV Sepaniak, MJ AF Charlton, Jennifer J. Jones, Natalie C. Wallace, Ryan A. Smithwick, Robert W. Bradshaw, James A. Kravchenko, Ivan I. Lavrik, Nickolay V. Sepaniak, Michael J. TI Nanopillar Based Enhanced-Fluorescence Detection of Surface-Immobilized Beryllium SO ANALYTICAL CHEMISTRY LA English DT Article ID CAPILLARY-ELECTROPHORESIS; SELECTIVE DETERMINATION; SILICON NANOPILLARS; ARRAYS; ION; CHROMATOGRAPHY; REAGENT; PROBE; FIELD AB The unique properties associated with beryllium metal ensures the continued use in many industries despite the documented health and environmental risks. While engineered safeguards and personal protective equipment can reduce risks associated with working with the metal, it has been mandated by the Environmental Protection Agency (EPA) and Occupational Safety and Health Administration (OSHA) that the workplace air and surfaces must be monitored for toxic levels. While many methods have been developed to monitor levels down to the low mu g/m(3), the complexity and expense of these methods have driven the investigation into alternate methodologies. Herein, we use a combination of the previously developed fluorescence Be(II) ion detection reagent, 10-hydroxybenzo[h]quinoline (HBO), with an optical field enhanced silicon nanopillar array, creating a new surface immobilized (si-HBQ) platform. The si-HBQ platform allows the positive control of the reagent for demonstrated reusability and a pillar diameter based tunable enhancement. Furthermore, native silicon nanopillars are overcoated with thin layers of porous silicon oxide to develop an analytical platform capable of a 0.0006 mu g/L limit of detection (LOD) using sub-mu L sample volumes. Additionally, we demonstrate a method to multiplex the introduction of the sample to the platform, with minimal 5.2% relative standard deviation (RSD) at 0.1 mu g/L, to accommodate the potentially large number of samples needed to maintain industrial compliance. The minimal sample and reagent volumes and lack of complex and highly specific instrumentation, as well as positive control and reusability of traditionally consumable reagents, create a platform that is accessible and economically advantageous. C1 [Charlton, Jennifer J.; Wallace, Ryan A.; Bradshaw, James A.; Sepaniak, Michael J.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Charlton, Jennifer J.; Jones, Natalie C.; Smithwick, Robert W.; Bradshaw, James A.] Analyt Chem Org, Oak Ridge, TN 37830 USA. [Kravchenko, Ivan I.; Lavrik, Nickolay V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37830 USA. [Jones, Natalie C.] No Arizona Univ, Coll Engn Forestry & Nat Sci, Flagstaff, AZ 86011 USA. RP Sepaniak, MJ (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. EM msepaniak@utk.edu RI Kravchenko, Ivan/K-3022-2015; Lavrik, Nickolay/B-5268-2011 OI Kravchenko, Ivan/0000-0003-4999-5822; Lavrik, Nickolay/0000-0002-9543-5634 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; National Science Foundation [CHE-1144947]; University of Tennessee; Y-12 National Security Complex Plant Directed Research and Development fund FX Substrate design, patterning, and fabrication were conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. This material is based on work supported in part by The National Science Foundation under Grant CHE-1144947 with the University of Tennessee. This work was supported in part by the Y-12 National Security Complex Plant Directed Research and Development fund. NR 33 TC 2 Z9 2 U1 5 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD JUL 7 PY 2015 VL 87 IS 13 BP 6814 EP 6821 DI 10.1021/acs.analchem.5b01035 PG 8 WC Chemistry, Analytical SC Chemistry GA CM6ZH UT WOS:000357839700058 PM 26041094 ER PT J AU Brown, BL Martinez, P Zakhidov, AA Shaner, EA Lee, M AF Brown, Brian L. Martinez, Patricia Zakhidov, Anvar A. Shaner, Eric A. Lee, Mark TI Microwave conductance properties of aligned multiwall carbon nanotube textile sheets SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID TRANSPORT; TEMPERATURES; TRANSPARENT; PERFORMANCE; GRAPHENE; FILMS; WALL AB Understanding the conductance properties of multi-walled carbon nanotube (MWNT) textile sheets in the microwave regime is essential for their potential use in high-speed and high-frequency applications. To expand current knowledge, complex high-frequency conductance measurements from 0.01 to 50 GHz and across temperatures from 4.2K to 300K and magnetic fields up to 2 T were made on textile sheets of highly aligned MWNTs with strand alignment oriented both parallel and perpendicular to the microwave electric field polarization. Sheets were drawn from 329 and 520 mu m high MWNT forests that resulted in different DC resistance anisotropy. For all samples, the microwave conductance can be modeled approximately by a shunt capacitance in parallel with a frequency-independent conductance, but with no inductive contribution. This is consistent with diffusive Drude conduction as the primary transport mechanism up to 50 GHz. Further, it is found that the microwave conductance is essentially independent of both temperature and magnetic field. (C) 2015 AIP Publishing LLC. C1 [Brown, Brian L.; Zakhidov, Anvar A.; Lee, Mark] Univ Texas Dallas, Dept Phys, Richardson, TX 75080 USA. [Martinez, Patricia; Zakhidov, Anvar A.] Univ Texas Dallas, Alan G McDiarmid NanoTech Inst, Richardson, TX 75080 USA. [Martinez, Patricia] Univ Texas Dallas, Dept Mat Sci & Engn, Richardson, TX 75080 USA. [Shaner, Eric A.] Sandia Natl Labs, Albuquerque, NM 87123 USA. RP Brown, BL (reprint author), Univ Texas Dallas, Dept Phys, Richardson, TX 75080 USA. FU DOE Office of Basic Energy Sciences; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Welch Foundation [AT 16-17]; Mexican CONACYT graduate fellowship FX Work at Sandia and UTD Department of Physics was supported by the DOE Office of Basic Energy Sciences. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. Work at the UTD McDiarmid NanoTech Institute was supported by the Welch Foundation via Grant No. AT 16-17. P.M. acknowledges the support of a Mexican CONACYT graduate fellowship. NR 44 TC 0 Z9 0 U1 0 U2 6 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 7 PY 2015 VL 118 IS 1 AR 014308 DI 10.1063/1.4926379 PG 9 WC Physics, Applied SC Physics GA CM7LC UT WOS:000357873100022 ER PT J AU Choi, SG Manandhar, P Picraux, ST AF Choi, S. G. Manandhar, P. Picraux, S. T. TI Vapor-liquid-solid epitaxial growth of Si1-xGex alloy nanowires: Composition dependence on precursor reactivity and morphology control for vertical forests SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID SILICON-GERMANIUM NANOWIRES; ORIENTATION CONTROL; CHEMISTRY; NANOSTRUCTURES; SHAPE AB Growth of high-density group IV alloy nanowire forests is critical for exploiting their unique functionalities in many applications. Here, the compositional dependence on precursor reactivity and optimized conditions for vertical growth are studied for Si1-xGex alloy nanowires grown by the vapor-liquid-solid method. The nanowire composition versus gas partial-pressure ratio for germane-silane and germane-disilane precursor combinations is obtained at 350 degrees C over a wide composition range (0.05 <= x <= 0.98) and a generalized model to predict composition for alloy nanowires is developed based on the relative precursor partial pressures and reactivity ratio. In combination with germane, silane provides more precise compositional control at high Ge concentrations (x > 0.7), whereas disilane greatly increases the Si concentration for a given gas ratio and enables more precise alloy compositional control at small Ge concentrations (x < 0.3). Vertically oriented, non-kinking nanowire forest growth on Si (111) substrates is then discussed for silane/germane over a wide range of compositions, with temperature and precursor partial pressure optimized by monitoring the nanowire growth front using in-situ optical reflectance. For high Ge compositions (x approximate to 0.9), a "two-step" growth approach with nucleation at higher temperatures results in nanowires with high-density and uniform vertical orientation. With increasing Si content (x approximate to 0.8), the optimal growth window is shifted to higher temperatures, which minimizes nanowire kinking morphologies. For Si-rich Si1-xGex alloys (x approximate to 0.25), vertical nanowire growth is enhanced by single-step, higher-temperature growth at reduced pressures. (C) 2015 AIP Publishing LLC. C1 [Choi, S. G.; Manandhar, P.; Picraux, S. T.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. RP Picraux, ST (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol, POB 1663, Los Alamos, NM 87545 USA. EM picraux@lanl.gov FU Laboratory Directed Research and Development Program at Los Alamos National Laboratory; Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility at Los Alamos National Laboratory [DE-AC52-06NA25396]; Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility at Sandia National Laboratories [DE-AC04-94AL85000] FX Transmission electron microscopy analyses and valuable discussions with Jian Yu Huang are gratefully acknowledged. This research was funded in part by the Laboratory Directed Research and Development Program at Los Alamos National Laboratory and performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility at Los Alamos National Laboratory (Contract No. DE-AC52-06NA25396) and Sandia National Laboratories (Contract No. DE-AC04-94AL85000). NR 41 TC 0 Z9 0 U1 4 U2 17 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 7 PY 2015 VL 118 IS 1 AR 014303 DI 10.1063/1.4923355 PG 11 WC Physics, Applied SC Physics GA CM7LC UT WOS:000357873100017 ER PT J AU Fleming, RM Seager, CH Lang, DV Campbell, JM AF Fleming, R. M. Seager, C. H. Lang, D. V. Campbell, J. M. TI Injection deep level transient spectroscopy: An improved method for measuring capture rates of hot carriers in semiconductors SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID IRRADIATED SILICON; IMPLANTED SILICON; ELECTRON; TRAPS; PROFILES; LIFETIME; VACANCY; DEFECT; FIELD; GAAS AB An improved method for measuring the cross sections for carrier trapping at defects in semiconductors is described. This method, a variation of deep level transient spectroscopy (DLTS) used with bipolar transistors, is applied to hot carrier trapping at vacancy-oxygen, carbon-oxygen, and three charge states of divacancy centers (V-2) in n-and p-type silicon. Unlike standard DLTS, we fill traps by injecting carriers into the depletion region of a bipolar transistor diode using a pulse of forward bias current applied to the adjacent diode. We show that this technique is capable of accurately measuring a wide range of capture cross sections at varying electric fields due to the control of the carrier density it provides. Because this technique can be applied to a variety of carrier energy distributions, it should be valuable in modeling the effect of radiation-induced generation-recombination currents in bipolar devices. (C) 2015 AIP Publishing LLC. C1 [Fleming, R. M.; Seager, C. H.; Lang, D. V.; Campbell, J. M.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Fleming, RM (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RI Fleming, Robert/B-1248-2008; OI Fleming, Robert/0000-0003-2092-2152 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX We thank Don King for irradiating these samples at the Little Mountain Linac. We thank Gary Hennigan, Normand Modine, Sam Myers, Marty Shaneyfelt, George Vizkelethy, and Bill Wampler for helpful discussions. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 26 TC 0 Z9 0 U1 3 U2 24 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 7 PY 2015 VL 118 IS 1 AR 015703 DI 10.1063/1.4923358 PG 8 WC Physics, Applied SC Physics GA CM7LC UT WOS:000357873100037 ER PT J AU Liu, J Pecharsky, VK Gschneidner, KA AF Liu, J. Pecharsky, V. K. Gschneidner, K. A., Jr. TI Metamagnetic transition and magnetothermal properties of ErCo4Ge2 SO JOURNAL OF APPLIED PHYSICS LA English DT Article AB Polycrystalline ErCo4Ge2 was investigated by magnetic susceptibility and heat capacity measurements. The results show that ErCo4Ge2 undergoes a transition from the paramagnetic to the antiferromagnetic (AFM) state around 2.6 K. The second order character of this magnetic transition is confirmed from the lambda-like peak of the heat capacity data. Both chi' and chi '' of ErCo4Ge2 are strongly dependent on the ac magnetic field frequency and bias dc magnetic field. A field induced metamagnetic transition from AFM to ferromagnetic state is observed below T-N. Under a magnetic field change of 50 kOe, the maximum value of the magnetic entropy change (magnetocaloric effect) -Delta S-M is 14.2 J/kg K at 2.75K and the adiabatic temperature change Delta T-ad is 5.7 K. In particular, a large -Delta S-M value of 11.7 J/kg K is achieved for a low magnetic field change of 20 kOe. (C) 2015 AIP Publishing LLC. C1 [Liu, J.; Pecharsky, V. K.; Gschneidner, K. A., Jr.] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. [Liu, J.; Pecharsky, V. K.; Gschneidner, K. A., Jr.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. RP Liu, J (reprint author), Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. EM anneliu0@gmail.com FU U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; U.S. DOE [DE-AC02-07CH11358] FX This work was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. The research was performed at the Ames Laboratory, which is operated for the U.S. DOE by Iowa State University under Contract No. DE-AC02-07CH11358. NR 16 TC 1 Z9 1 U1 3 U2 15 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 7 PY 2015 VL 118 IS 1 AR 013904 DI 10.1063/1.4923414 PG 5 WC Physics, Applied SC Physics GA CM7LC UT WOS:000357873100012 ER PT J AU Liu, P Yang, SM Jain, A Wang, QG Jiang, HW Song, JM Koschny, T Soukoulis, CM Dong, L AF Liu, Peng Yang, Siming Jain, Aditya Wang, Qiugu Jiang, Huawei Song, Jiming Koschny, Thomas Soukoulis, Costas M. Dong, Liang TI Tunable meta-atom using liquid metal embedded in stretchable polymer SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID SPLIT-RING RESONATORS; SILICON INTEGRATED-CIRCUITS; TERAHERTZ METAMATERIALS; TRANSISTORS; ELECTRONICS; COMPOSITE; CLOAKING; ANTENNAS; DEVICES; MATRIX AB Reconfigurable metamaterials have great potential to alleviate complications involved in using passive metamaterials to realize emerging electromagnetic functions, such as dynamical filtering, sensing, and cloaking. This paper presents a new type of tunable meta-atoms in the X-band frequency range (8-12 GHz) toward reconfigurable metamaterials. The meta-atom is made of all flexible materials compliant to the surface of an interaction object. It uses a liquid metal-based split-ring resonator as its core constituent embedded in a highly flexible elastomer. We demonstrate that simple mechanical stretching of the meta-atom can lead to the great flexibility in reconfiguring its resonance frequency continuously over more than 70% of the X-band frequency range. The presented meta-atom technique provides a simple approach to dynamically tune response characteristics of metamaterials over a broad frequency range. (C) 2015 AIP Publishing LLC. C1 [Liu, Peng; Yang, Siming; Jain, Aditya; Wang, Qiugu; Jiang, Huawei; Song, Jiming; Dong, Liang] Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA. [Jain, Aditya; Koschny, Thomas; Soukoulis, Costas M.] US DOE, Ames Lab, Ames, IA 50011 USA. [Jain, Aditya; Koschny, Thomas; Soukoulis, Costas M.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Dong, L (reprint author), Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA. EM ldong@iastate.edu RI Soukoulis, Costas/A-5295-2008; OI Wang, Qiugu/0000-0003-2662-7736 FU National Science Foundation [ECCS-0954765]; Iowa Department of Transportation; Iowa Highway Research Board; China Scholarship Council; U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering; U.S. Department of Energy [DE-AC02-07CH11358] FX The work was partially supported by the National Science Foundation under the Grant No. ECCS-0954765, the Iowa Department of Transportation, the Iowa Highway Research Board, and the China Scholarship Council. The work at Ames Laboratory was partially supported by the U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. NR 49 TC 7 Z9 7 U1 4 U2 34 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 7 PY 2015 VL 118 IS 1 AR 014504 DI 10.1063/1.4926417 PG 8 WC Physics, Applied SC Physics GA CM7LC UT WOS:000357873100027 ER PT J AU Yadav, SK Sharma, V Ramprasad, R AF Yadav, S. K. Sharma, V. Ramprasad, R. TI Controlling electronic structure through epitaxial strain in ZnSe/ZnTe nano-heterostructures SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID NANOCRYSTALS; INTERFACES; GROWTH AB Using first-principles computations, we study the effect of epitaxial strains on electronic structure variations across ZnSe/ZnTe nano-heterostructures. Epitaxial strains of various types are modeled using pseudomorphic ZnSe/ZnTe heterostructures. We find that a wide range of band gaps (spanning the visible solar spectrum) and band offsets (0-1.5 eV) is accessible across the heterostructures in a controllable manner via reasonable levels of epitaxial strain. In addition to quantum confinement effects, strain in ZnSe/ZnTe heterostructures may thus be viewed as a powerful degree of freedom that can enable the rational design of optoelectronic devices. (C) 2015 AIP Publishing LLC. C1 [Yadav, S. K.; Sharma, V.; Ramprasad, R.] Univ Connecticut, Mat Sci & Engn, Storrs, CT 06269 USA. [Yadav, S. K.] Los Alamos Natl Lab, Mat Sci & Technol Div, MST 8, Los Alamos, NM 87545 USA. RP Yadav, SK (reprint author), Univ Connecticut, Mat Sci & Engn, Storrs, CT 06269 USA. EM syadav@lanl.gov RI Yadav, Satyesh/M-6588-2014; sharma, Vinit/K-3407-2015 FU National Science Foundation (NSF) FX Financial support of this work through a grant from the National Science Foundation (NSF) and computational support through a NSF Teragrid Resource Allocation are acknowledged. Authors would like to acknowledge a critical reading of the manuscript by Ghanshyam Pilania and Arun Mannodi-Kanakkithodi. NR 27 TC 2 Z9 2 U1 3 U2 17 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 7 PY 2015 VL 118 IS 1 AR 015701 DI 10.1063/1.4923385 PG 4 WC Physics, Applied SC Physics GA CM7LC UT WOS:000357873100035 ER PT J AU Hernandez-Ortiz, JP de Pablo, JJ AF Hernandez-Ortiz, Juan P. de Pablo, Juan J. TI Self-consistent description of electrokinetic phenomena in particle-based simulations SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID SPHERICAL COLLOIDAL PARTICLES; ACCELERATED STOKESIAN DYNAMICS; FLOWING POLYMER-SOLUTIONS; DOUBLE-LAYER INTERACTION; SMOOTHED PROFILE METHOD; HYDRODYNAMIC INTERACTIONS; ELECTROPHORETIC MOBILITY; BROWNIAN DYNAMICS; LATTICE-BOLTZMANN; MOLECULAR-DYNAMICS AB A new computational method is presented for study suspensions of charged particles undergoing fluctuating hydrodynamic and electrostatic interactions. The proposed model is appropriate for polymers, proteins, and porous particles embedded in a continuum electrolyte. A self-consistent Langevin description of the particles is adopted in which hydrodynamic and electrostatic interactions are included through a Green's function formalism. An Ewald-like split is adopted in order to satisfy arbitrary boundary conditions for the Stokeslet and Poisson Green functions, thereby providing a formalism that is applicable to any geometry and that can be extended to deformable objects. The convection-diffusion equation for the continuum ions is solved simultaneously considering Nernst-Planck diffusion. The method can be applied to systems at equilibrium and far from equilibrium. Its applicability is demonstrated in the context of electrokinetic motion, where it is shown that the ionic clouds associated with individual particles can be severely altered by the flow and concentration, leading to intriguing cooperative effects. (C) 2015 AIP Publishing LLC. C1 [Hernandez-Ortiz, Juan P.] Univ Nacl Colombia, Dept Mat & Minerales, Sede Medellin, Medellin, Colombia. [Hernandez-Ortiz, Juan P.; de Pablo, Juan J.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. [Hernandez-Ortiz, Juan P.] Univ Wisconsin, UW Biotechnol Ctr, Lab Mol & Computat Genom, Madison, WI 53706 USA. [de Pablo, Juan J.] Argonne Natl Lab, Mat Sci Div, Argonne, IL 60349 USA. RP Hernandez-Ortiz, JP (reprint author), Univ Nacl Colombia, Dept Mat & Minerales, Sede Medellin, Medellin, Colombia. EM jphernandezo@unal.edu.co; depablo@uchicago.edu OI Hernandez-Ortiz, Juan/0000-0003-0404-9947 FU Department of Energy, Basic Energy Sciences, Materials Science and Engineering Division. Argonne, a U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357]; COL-CIENCIAS; NIH National Human Genome Research Institute [HG000225] FX This work was supported by the Department of Energy, Basic Energy Sciences, Materials Science and Engineering Division. Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. An award of computer time was provided by the Innovative and Novel Computational Impact on Theory and Experiment (INCITE) program of the Argonne Leadership Computing Facility at Argonne National Laboratory. Additional development work was performed using the Argonne Laboratory Resource Computing Center (LCRC) and University of Chicago Midway cluster. J.P.H.O. is thankful to COL-CIENCIAS and the NIH National Human Genome Research Institute Grant No. HG000225 (UW-Madison) for partial support of this research. NR 93 TC 3 Z9 3 U1 3 U2 27 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUL 7 PY 2015 VL 143 IS 1 AR 014108 DI 10.1063/1.4923342 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CM7LJ UT WOS:000357873900012 PM 26156466 ER PT J AU Li, Z Yazdani, A Tartakovsky, A Karniadakis, GE AF Li, Zhen Yazdani, Alireza Tartakovsky, Alexandre Karniadakis, George Em TI Transport dissipative particle dynamics model for mesoscopic advection-diffusion-reaction problems SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID RED-BLOOD-CELLS; SLIP BOUNDARY-CONDITIONS; ENERGY-CONSERVATION; SIMULATION; SHAPES; FLOWS AB We present a transport dissipative particle dynamics (tDPD) model for simulating mesoscopic problems involving advection-diffusion-reaction (ADR) processes, along with a methodology for implementation of the correct Dirichlet and Neumann boundary conditions in tDPD simulations. tDPD is an extension of the classic dissipative particle dynamics (DPD) framework with extra variables for describing the evolution of concentration fields. The transport of concentration is modeled by a Fickian flux and a random flux between tDPD particles, and the advection is implicitly considered by the movements of these Lagrangian particles. An analytical formula is proposed to relate the tDPD parameters to the effective diffusion coefficient. To validate the present tDPD model and the boundary conditions, we perform three tDPD simulations of one-dimensional diffusion with different boundary conditions, and the results show excellent agreement with the theoretical solutions. We also performed two-dimensional simulations of ADR systems and the tDPD simulations agree well with the results obtained by the spectral element method. Finally, we present an application of the tDPD model to the dynamic process of blood coagulation involving 25 reacting species in order to demonstrate the potential of tDPD in simulating biological dynamics at the mesoscale. We find that the tDPD solution of this comprehensive 25-species coagulation model is only twice as computationally expensive as the conventional DPD simulation of the hydrodynamics only, which is a significant advantage over available continuum solvers. (C) 2015 AIP Publishing LLC. C1 [Li, Zhen; Yazdani, Alireza; Karniadakis, George Em] Brown Univ, Div Appl Math, Providence, RI 02912 USA. [Tartakovsky, Alexandre] Pacific NW Natl Lab, Computat Math Grp, Richland, WA 99352 USA. RP Li, Z (reprint author), Brown Univ, Div Appl Math, Providence, RI 02912 USA. EM george_karniadakis@brown.edu RI Li, Zhen/B-2722-2013 OI Li, Zhen/0000-0002-0936-6928 FU NIH [1U01HL116323-01]; DOE Center on Mathematics for Mesoscopic Modeling of Materials (CM4); TACC/STAMPEDE through the XSEDE Grant [TG-DMS140007] FX This work was primarily supported by NIH (Grant No. 1U01HL116323-01) and the DOE Center on Mathematics for Mesoscopic Modeling of Materials (CM4). Computational resources were provided by the Innovative and Novel Computational Impact on Theory and Experiment (INCITE) program and TACC/STAMPEDE through the XSEDE Grant (Grant No. TG-DMS140007). Z. Li would like to acknowledge helpful discussions with Dr. Wenxiao Pan and Professor Bruce Caswell. A. Yazdani would like to thank Dr. Hessam Babaee for the support he gave for the spectral element solver. NR 36 TC 6 Z9 6 U1 2 U2 25 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUL 7 PY 2015 VL 143 IS 1 AR 014101 DI 10.1063/1.4923254 PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CM7LJ UT WOS:000357873900005 PM 26156459 ER PT J AU Walen, H Liu, DJ Oh, J Lim, H Evans, JW Kim, Y Thiel, PA AF Walen, Holly Liu, Da-Jiang Oh, Junepyo Lim, Hyunseob Evans, J. W. Kim, Yousoo Thiel, P. A. TI Self-organization of S adatoms on Au(111): root 3R30 degrees rows at low coverage SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID SCANNING-TUNNELING-MICROSCOPY; ADSORBATE-ADSORBATE INTERACTIONS; FORMED SULFUR ADLAYERS; PHASE-DIAGRAM; SURFACE; GOLD; DENSITY; STM; RECONSTRUCTION; TEMPERATURE AB Using scanning tunneling microscopy, we observe an adlayer structure that is dominated by short rows of S atoms, on unreconstructed regions of a Au(111) surface. This structure forms upon adsorption of low S coverage (less than 0.1 monolayer) on a fully reconstructed clean surface at 300 K, then cooling to 5 K for observation. The rows adopt one of three orientations that are rotated by 30 degrees from the close-packed directions of the Au(111) substrate, and adjacent S atoms in the rows are separated by root 3 times the surface lattice constant, a. Monte Carlo simulations are performed on lattice-gas models, derived using a limited cluster expansion based on density functional theory energetics. Models which include long-range pairwise interactions (extending to 5a), plus selected trio interactions, successfully reproduce the linear rows of S atoms at reasonable temperatures. (C) 2015 AIP Publishing LLC. C1 [Walen, Holly; Thiel, P. A.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Liu, Da-Jiang; Evans, J. W.; Thiel, P. A.] US DOE, Ames Lab, Ames, IA 50011 USA. [Oh, Junepyo; Lim, Hyunseob; Kim, Yousoo] RIKEN Surface & Interface Sci Lab, Wako, Saitama 3510198, Japan. [Evans, J. W.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Thiel, P. A.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. RP Walen, H (reprint author), Iowa State Univ, Dept Chem, Ames, IA 50011 USA. EM hwalen@iastate.edu RI Lim, Hyunseob /K-1692-2015; Oh, Junepyo/M-3244-2016 OI Lim, Hyunseob /0000-0002-4956-4208; Oh, Junepyo/0000-0003-2452-3386 FU U.S., NSF [CHE-1111500]; Japan, Ministry of Education, Culture, Sports, Science, and Technology (MEXT); Division of Chemical Sciences, Basic Energy Sciences, U.S. Department of Energy (USDOE); Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX The experimental component of this work was supported by three sources. From the U.S., it was NSF Grant No. CHE-1111500. From Japan, support was provided by a Grant-in-Aid for Scientific Research on Priority Areas "Electron Transport Through a Linked Molecule in Nano-scale" and a Grant-in-Aid for Scientific Research(S) "Single Molecule Spectroscopy using Probe Microscope" from the Ministry of Education, Culture, Sports, Science, and Technology (MEXT). The theoretical component of this work was supported by the Division of Chemical Sciences, Basic Energy Sciences, U.S. Department of Energy (USDOE), and it utilized resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy (Contract No. DE-AC02-05CH11231). NR 51 TC 5 Z9 5 U1 5 U2 23 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUL 7 PY 2015 VL 143 IS 1 AR 014704 DI 10.1063/1.4922929 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CM7LJ UT WOS:000357873900035 PM 26156489 ER PT J AU White, AJ Gorshkov, VN Tretiak, S Mozyrsky, D AF White, Alexander J. Gorshkov, Vyacheslav N. Tretiak, Sergei Mozyrsky, Dmitry TI Non-adiabatic molecular dynamics by accelerated semiclassical Monte Carlo SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID QUANTUM-CLASSICAL DYNAMICS; PATH-INTEGRAL TREATMENT; EXCITED-STATE DYNAMICS; AB-INITIO; SCATTERING THEORY; ENERGY-TRANSFER; SIMULATIONS; DECOHERENCE; RELAXATION; SYSTEMS AB Non-adiabatic dynamics, where systems non-radiatively transition between electronic states, plays a crucial role in many photo-physical processes, such as fluorescence, phosphorescence, and photoisomerization. Methods for the simulation of non-adiabatic dynamics are typically either numerically impractical, highly complex, or based on approximations which can result in failure for even simple systems. Recently, the Semiclassical Monte Carlo (SCMC) approach was developed in an attempt to combine the accuracy of rigorous semiclassical methods with the efficiency and simplicity of widely used surface hopping methods. However, while SCMC was found to be more efficient than other semiclassical methods, it is not yet as efficient as is needed to be used for large molecular systems. Here, we have developed two new methods: the accelerated-SCMC and the accelerated-SCMC with re-Gaussianization, which reduce the cost of the SCMC algorithm up to two orders of magnitude for certain systems. In most cases shown here, the new procedures are nearly as efficient as the commonly used surface hopping schemes, with little to no loss of accuracy. This implies that these modified SCMC algorithms will be of practical numerical solutions for simulating non-adiabatic dynamics in realistic molecular systems. (C) 2015 AIP Publishing LLC. C1 [White, Alexander J.; Tretiak, Sergei; Mozyrsky, Dmitry] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [White, Alexander J.; Tretiak, Sergei] Los Alamos Natl Lab, Ctr Nonlinear Studies CNLS, Los Alamos, NM 87545 USA. [Gorshkov, Vyacheslav N.] Natl Tech Univ Ukraine, UA-03056 Kiev, Ukraine. [Tretiak, Sergei] Los Alamos Natl Lab, Ctr Integrated Nanotechnol CINT, Los Alamos, NM 87545 USA. RP White, AJ (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM serg@lanl.gov; mozyrsky@lanl.gov RI White, Alexander/D-8754-2014; Tretiak, Sergei/B-5556-2009; OI White, Alexander/0000-0002-7771-3899; Tretiak, Sergei/0000-0001-5547-3647; Mozyrsky, Dima/0000-0001-5305-4617 FU U.S. Department of Energy through the Los Alamos National Laboratory (LANL) LDRD Program; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396]; Center for Nonlinear Studies (CNLS); Center for Integrated Nanotechnology (CINT) at LANL; Texas A&M University at Qatar via the NPRP from the Qatar National Research Fund [6-021-1-005] FX We acknowledge support of the U.S. Department of Energy through the Los Alamos National Laboratory (LANL) LDRD Program. LANL is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. We acknowledge support of the Center for Nonlinear Studies (CNLS) and the Center for Integrated Nanotechnology (CINT) at LANL. V.G. gratefully acknowledges support from Texas A&M University at Qatar via the NPRP Grant No. 6-021-1-005 from the Qatar National Research Fund. NR 71 TC 7 Z9 7 U1 2 U2 22 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUL 7 PY 2015 VL 143 IS 1 AR 014115 DI 10.1063/1.4923473 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CM7LJ UT WOS:000357873900019 PM 26156473 ER PT J AU Kim, HS Liu, WS Chen, G Chua, CW Ren, ZF AF Kim, Hee Seok Liu, Weishu Chen, Gang Chua, Ching-Wu Ren, Zhifeng TI Relationship between thermoelectric figure of merit and energy conversion efficiency SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE thermoelectrics; engineering figure of merit; engineering power factor; conversion efficiency; cumulative temperature dependence ID POWER-GENERATION; PERFORMANCE; CRYSTALS; ALLOYS AB The formula for maximum efficiency (eta(max)) of heat conversion into electricity by a thermoelectric device in terms of the dimensionless figure of merit (ZT) has been widely used to assess the desirability of thermoelectric materials for devices. Unfortunately, the eta(max) values vary greatly depending on how the average ZT values are used, raising questions about the applicability of ZT in the case of a large temperature difference between the hot and cold sides due to the neglect of the temperature dependences of the material properties that affect ZT. To avoid the complex numerical simulation that gives accurate efficiency, we have defined an engineering dimensionless figure of merit (ZT)(eng) and an engineering power factor (PF)(eng) as functions of the temperature difference between the cold and hot sides to predict reliably and accurately the practical conversion efficiency and output power, respectively, overcoming the reporting of unrealistic efficiency using average ZT values. C1 [Kim, Hee Seok; Liu, Weishu; Chua, Ching-Wu; Ren, Zhifeng] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Kim, Hee Seok; Liu, Weishu; Chua, Ching-Wu; Ren, Zhifeng] Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. [Chen, Gang] MIT, Dept Mech Engn, Cambridge, MA 02139 USA. [Chua, Ching-Wu] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Chen, G (reprint author), MIT, Dept Mech Engn, Cambridge, MA 02139 USA. EM gchen2@mit.edu; cwchu@uh.edu; zren@uh.edu RI Chen, Gang/J-1325-2014; Kim, Hee Seok/N-1080-2014; Liu, WeiShu/E-7098-2011 OI Chen, Gang/0000-0002-3968-8530; Liu, WeiShu/0000-0001-8643-822X FU US Department of Energy (DOE) [DOE DE-FG02-13ER46917/DE-SC0010831]; Solid State Solar Thermal Energy Conversion Center (S3TEC), an Energy Frontier Research Center - US DOE, Office of Science, Office of Basic Energy Science [DE-SC0001299]; US Air Force Office of Scientific Research [FA9550-09-1-0656]; T. L. L. Temple Foundation; John J. and Rebecca Moores Endowment; State of Texas through the Texas Center for Superconductivity at the University of Houston FX This work was partially supported by the US Department of Energy (DOE) under Contract DOE DE-FG02-13ER46917/DE-SC0010831 (the part without the Thomson effect) and also partially by Solid State Solar Thermal Energy Conversion Center (S3TEC), an Energy Frontier Research Center funded by the US DOE, Office of Science, Office of Basic Energy Science under Award DE-SC0001299 (the part considering the Thomson effect). The work is also supported in part by US Air Force Office of Scientific Research Grant FA9550-09-1-0656, the T. L. L. Temple Foundation, the John J. and Rebecca Moores Endowment, and the State of Texas through the Texas Center for Superconductivity at the University of Houston. NR 34 TC 39 Z9 39 U1 7 U2 76 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUL 7 PY 2015 VL 112 IS 27 BP 8205 EP 8210 DI 10.1073/pnas.1510231112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CM2QU UT WOS:000357527600038 PM 26100905 ER PT J AU Meinecke, J Tzeferacos, P Bell, A Bingham, R Clarke, R Churazov, E Crowston, R Doyle, H Drake, RP Heathcote, R Koenig, M Kuramitsu, Y Kuranz, C Lee, D MacDonald, M Murphy, C Notley, M Park, HS Pelka, A Ravasio, A Reville, B Sakawa, Y Wan, W Woolsey, N Yurchak, R Miniati, F Schekochihin, A Lamb, D Gregori, G AF Meinecke, Jena Tzeferacos, Petros Bell, Anthony Bingham, Robert Clarke, Robert Churazov, Eugene Crowston, Robert Doyle, Hugo Drake, R. Paul Heathcote, Robert Koenig, Michel Kuramitsu, Yasuhiro Kuranz, Carolyn Lee, Dongwook MacDonald, Michael Murphy, Christopher Notley, Margaret Park, Hye-Sook Pelka, Alexander Ravasio, Alessandra Reville, Brian Sakawa, Youichi Wan, Willow Woolsey, Nigel Yurchak, Roman Miniati, Francesco Schekochihin, Alexander Lamb, Don Gregori, Gianluca TI Developed turbulence and nonlinear amplification of magnetic fields in laboratory and astrophysical plasmas SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE galaxy clusters; laboratory analogues; lasers; magnetic fields; turbulence ID LARGE-SCALE STRUCTURE; SHOCK-WAVES; COLLISIONLESS SHOCKS; WEIBEL INSTABILITY; GALAXY CLUSTER; GAS-DENSITY; GENERATION; HYDRODYNAMICS; CODE; MAGNETOHYDRODYNAMICS AB The visible matter in the universe is turbulent and magnetized. Turbulence in galaxy clusters is produced by mergers and by jets of the central galaxies and believed responsible for the amplification of magnetic fields. We report on experiments looking at the collision of two laser-produced plasma clouds, mimicking, in the laboratory, a cluster merger event. By measuring the spectrum of the density fluctuations, we infer developed, Kolmogorov-like turbulence. From spectral line broadening, we estimate a level of turbulence consistent with turbulent heating balancing radiative cooling, as it likely does in galaxy clusters. We show that the magnetic field is amplified by turbulent motions, reaching a nonlinear regime that is a precursor to turbulent dynamo. Thus, our experiment provides a promising platform for understanding the structure of turbulence and the amplification of magnetic fields in the universe. C1 [Meinecke, Jena; Bell, Anthony; Doyle, Hugo; Schekochihin, Alexander; Gregori, Gianluca] Univ Oxford, Dept Phys, Oxford OX1 3PU, England. [Tzeferacos, Petros; Lamb, Don; Gregori, Gianluca] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Bingham, Robert; Clarke, Robert; Heathcote, Robert; Notley, Margaret] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bingham, Robert] Univ Strathclyde, Dept Phys, Glasgow G4 0NG, Lanark, Scotland. [Churazov, Eugene] Max Planck Inst Astrophys, D-85741 Garching, Germany. [Churazov, Eugene] Space Res Inst, Moscow 117997, Russia. [Crowston, Robert; Murphy, Christopher; Woolsey, Nigel] Univ York, Dept Phys, York YO10 5D, N Yorkshire, England. [Drake, R. Paul; Kuranz, Carolyn; MacDonald, Michael; Wan, Willow] Univ Michigan, Atmospher Ocean & Space Sci, Ann Arbor, MI 48109 USA. [Koenig, Michel; Pelka, Alexander; Ravasio, Alessandra; Yurchak, Roman] Univ Paris 06, Lab Utilisat Lasers Intenses, Commissariat Energie Atom & Energies Alternat, UMR7605,CNRS,Ecole Polytech, F-91128 Palaiseau, France. [Kuramitsu, Yasuhiro] Natl Cent Univ, Dept Phys, Taoyuan 320, Taiwan. [Kuramitsu, Yasuhiro; Sakawa, Youichi] Osaka Univ, Inst Laser Engn, Osaka 5650871, Japan. [Lee, Dongwook] Univ Calif Santa Cruz, Appl Math & Stat, Santa Cruz, CA 96064 USA. [Park, Hye-Sook] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Pelka, Alexander] Helmholtz Zentrum Dresden Rossendorf, Inst Radiat Phys, D-01314 Dresden, Germany. [Reville, Brian] Queens Univ Belfast, Sch Math & Phys, Belfast BT7 1NN, Antrim, North Ireland. [Miniati, Francesco] ETH, Dept Phys, CH-8093 Zurich, Switzerland. RP Meinecke, J (reprint author), Univ Oxford, Dept Phys, Oxford OX1 3PU, England. EM jena.meinecke@physics.ox.ac.uk; g.gregori1@physics.ox.ac.uk RI Churazov, Eugene/A-7783-2013; Sakawa, Youichi/J-5707-2016; Drake, R Paul/I-9218-2012; OI Sakawa, Youichi/0000-0003-4165-1048; Drake, R Paul/0000-0002-5450-9844; MacDonald, Michael/0000-0002-6295-6978 FU European Research Council (ERC) under the European Community [256973, 247039]; US Department of Energy [B591485, DE-NA0001840]; National Institutes of Health; Science and Technology Facilities Council; Engineering and Physical Sciences Research Council of the United Kingdom [EP/G007187/1]; Biological Sciences Division of the University of Chicago; Argonne National Laboratory [S10 RR029030-01] FX We thank the Vulcan technical team at the Central Laser Facility of the Rutherford Appleton Laboratory for their support during the experiments. The research leading to these results has received funding from the European Research Council (ERC) under the European Community's Seventh Framework Programme (FP7/2007-2013)/ERC Grant Agreements 256973 and 247039, and the US Department of Energy under Contract B591485 to Lawrence Livermore National Laboratory and Field Work Proposal 57789 to Argonne National Laboratory. This work was supported in part by National Institutes of Health through resources provided by the Computation Institute and the Biological Sciences Division of the University of Chicago and Argonne National Laboratory, under Grant S10 RR029030-01. Partial support from the Science and Technology Facilities Council and the Engineering and Physical Sciences Research Council of the United Kingdom (Grant EP/G007187/1) is also acknowledged. The work of R.P.D, C.K., M.M., and W.W. was supported by the US Department of Energy under Grant DE-NA0001840. NR 51 TC 8 Z9 8 U1 0 U2 20 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUL 7 PY 2015 VL 112 IS 27 BP 8211 EP 8215 DI 10.1073/pnas.1502079112 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CM2QU UT WOS:000357527600039 PM 26100873 ER PT J AU Iberi, V Vlassiouk, I Zhang, XG Matola, B Linn, A Joy, DC Rondinone, AJ AF Iberi, Vighter Vlassiouk, Ivan Zhang, X. -G. Matola, Brad Linn, Allison Joy, David C. Rondinone, Adam J. TI Maskless Lithography and in situ Visualization of Conductivity of Graphene using Helium Ion Microscopy SO SCIENTIFIC REPORTS LA English DT Article ID MODEL AB The remarkable mechanical and electronic properties of graphene make it an ideal candidate for next generation nanoelectronics. With the recent development of commercial-level single-crystal graphene layers, the potential for manufacturing household graphene-based devices has improved, but significant challenges still remain with regards to patterning the graphene into devices. In the case of graphene supported on a substrate, traditional nanofabrication techniques such as e-beam lithography (EBL) are often used in fabricating graphene nanoribbons but the multi-step processes they require can result in contamination of the graphene with resists and solvents. In this letter, we report the utility of scanning helium ion lithography for fabricating functional graphene nanoconductors that are supported directly on a silicon dioxide layer, and we measure the minimum feature size achievable due to limitations imposed by thermal fluctuations and ion scattering during the milling process. Further we demonstrate that ion beams, due to their positive charging nature, may be used to observe and test the conductivity of graphene-based nanoelectronic devices in situ. C1 [Iberi, Vighter; Zhang, X. -G.; Matola, Brad; Linn, Allison; Joy, David C.; Rondinone, Adam J.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Vlassiouk, Ivan] Oak Ridge Natl Lab, Energy & Transportat Sci, Oak Ridge, TN 37831 USA. [Zhang, X. -G.] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. [Zhang, X. -G.] Univ Florida, Quantum Theory Project, Gainesville, FL 32611 USA. [Joy, David C.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Rondinone, AJ (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM rondinoneaj@ornl.gov RI Rondinone, Adam/F-6489-2013; Vlassiouk, Ivan/F-9587-2010 OI Rondinone, Adam/0000-0003-0020-4612; Vlassiouk, Ivan/0000-0002-5494-0386 NR 15 TC 8 Z9 8 U1 6 U2 36 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUL 7 PY 2015 VL 5 AR 11952 DI 10.1038/srep11952 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CM1OR UT WOS:000357450700001 PM 26150202 ER PT J AU Mangeri, J Heinonen, O Karpeyev, D Nakhmanson, S AF Mangeri, John Heinonen, Olle Karpeyev, Dmitry Nakhmanson, Serge TI Influence of Elastic and Surface Strains on the Optical Properties of Semiconducting Core-Shell Nanoparticles SO PHYSICAL REVIEW APPLIED LA English DT Article ID PHOTOCATALYTIC ACTIVITY; ZNO NANOTUBES; ZINC-OXIDE; SYSTEMS; NANOSTRUCTURES; MICROSPHERES; IRRADIATION; FABRICATION; PARTICLES; CELLS AB Core-shell nanoparticle systems of Zn-ZnO and ZnO-TiO2 are studied computationally using finite-element methods. The inclusion of a surface free energy and the elastic mismatch of the core and shell create an imprinting effect within the shell structure that produces a wide variation of strains. Due to this diversity of strains, the sharp, direct, band-gap edges of the bulk semiconductor are observed to be broadened. We show that a variety of factors, such as particle size, core-to-shell volume ratio, applied hydrostatic pressure, shell microstructure, as well as the effect of elastic anisotropy, can influence the distribution of optical band-gap values throughout the particle. C1 [Mangeri, John; Nakhmanson, Serge] Univ Connecticut, Dept Phys, Storrs, CT 06269 USA. [Heinonen, Olle] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. [Heinonen, Olle] Northwestern Univ, Ctr Hierarch Mat Design, Northwestern Argonne Inst Sci & Engn, Evanston, IL 60208 USA. [Karpeyev, Dmitry] Univ Chicago, Computat Inst, Chicago, IL 60637 USA. [Nakhmanson, Serge] Univ Connecticut, Dept Mat Sci & Engn, Storrs, CT 06269 USA. [Nakhmanson, Serge] Univ Connecticut, Inst Mat Sci, Storrs, CT 06269 USA. RP Mangeri, J (reprint author), Univ Connecticut, Dept Phys, Storrs, CT 06269 USA. EM mangeri@phys.uconn.edu OI Heinonen, Olle/0000-0002-3618-6092 FU U.S. Department of Commerce, National Institute of Standards and Technology as part of the Center for Hierarchical Material Design (CHiMaD) [70NANB14H012]; U.S. Department of Energy FX Part of the work by O. H. was performed under Award No. 70NANB14H012 from U.S. Department of Commerce, National Institute of Standards and Technology as part of the Center for Hierarchical Material Design (CHiMaD). The authors gratefully acknowledge the computing resources provided on Blues, a high-performance computing cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory, and on the Hornet cluster hosted by the Taylor L. Booth Engineering Center for Advanced Technology (BECAT) located at the University of Connecticut at Storrs. Part of the work at Argonne was funded by the U.S. Department of Energy. The authors are also indebted to Prof. Luyi Sun for many useful discussions and help with providing references for this paper. NR 63 TC 1 Z9 1 U1 4 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2331-7019 J9 PHYS REV APPL JI Phys. Rev. Appl. PD JUL 7 PY 2015 VL 4 IS 1 AR 014001 DI 10.1103/PhysRevApplied.4.014001 PG 10 WC Physics, Applied SC Physics GA CM2IB UT WOS:000357502200001 ER PT J AU Niclis, JC Murphy, SV Parkinson, DY Zedan, A Sathananthan, AH Cram, DS Heraud, P AF Niclis, J. C. Murphy, S. V. Parkinson, D. Y. Zedan, A. Sathananthan, A. H. Cram, D. S. Heraud, P. TI Three-dimensional imaging of human stem cells using soft X-ray tomography SO JOURNAL OF THE ROYAL SOCIETY INTERFACE LA English DT Article DE stem cells; transmission soft X-ray microscopy; three-dimensional; human ID MICRO-COMPUTED TOMOGRAPHY; BIOLOGICAL SPECIMENS; ELECTRON TOMOGRAPHY; SPATIAL-RESOLUTION; MOUSE; DIFFERENTIATION; TRANSPLANTATION; ULTRASTRUCTURE; RECONSTRUCTION; EXPRESSION AB Three-dimensional imaging of human stem cells using transmission soft X-ray tomography (SXT) is presented for the first time. Major organelle types-nuclei, nucleoli, mitochondria, lysosomes and vesicles were discriminated at approximately 50 nm spatial resolution without the use of contrast agents, on the basis of measured linear X-ray absorption coefficients and comparison of the size and shape of structures to transmission electron microscopy (TEM) images. In addition, SXT was used to visualize the distribution of a cell surface protein using gold-labelled antibody staining. We present the strengths of SXT, which include excellent spatial resolution (intermediate between that of TEM and light microscopy), the lack of the requirement for fixative or contrast agent that might perturb cellular morphology or produce imaging artefacts, and the ability to produce three-dimensional images of cells without microtome sectioning. Possible applications to studying the differentiation of human stem cells are discussed. C1 [Niclis, J. C.; Sathananthan, A. H.; Cram, D. S.; Heraud, P.] Monash Univ, Monash Inst Med Res, Dept Anat & Dev Biol, Clayton, Vic 3800, Australia. [Murphy, S. V.] Monash Univ, Monash Inst Med Res, Ritchie Ctr, Clayton, Vic 3800, Australia. [Niclis, J. C.] Univ Melbourne, Florey Inst Neurosci & Mental Hlth, Parkville, Vic 3052, Australia. [Murphy, S. V.] Wake Forest Inst Regenerat Med, Wake Forest Baptist Med Ctr, Winston Salem, NC USA. [Parkinson, D. Y.; Zedan, A.] US DOE, Adv Light Source, Lawrence Berkeley Natl Lab, Berkeley, CA USA. [Heraud, P.] Monash Univ, Sch Chem, Ctr Biospectroscopy, Melbourne, Vic 3004, Australia. RP Heraud, P (reprint author), Monash Univ, Monash Inst Med Res, Dept Anat & Dev Biol, Clayton, Vic 3800, Australia. EM phil.heraud@monash.edu FU National Institute of General Medical Sciences of the National Institutes of Health [P41GM103445]; US Department of Energy, Office of Biological and Environmental Research [DE-AC02-05CH11231]; Australian Synchrotron's International Synchrotron Access Program, NHMRC Project [491145]; Monash University; Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231] FX The NCXT is supported by the National Institute of General Medical Sciences of the National Institutes of Health (P41GM103445) and the US Department of Energy, Office of Biological and Environmental Research (contract no. DE-AC02-05CH11231). Financial assistance to attend the beamtime at the ALS and perform the measurements was provided by the Australian Synchrotron's International Synchrotron Access Program, NHMRC Project grant no. 491145 and support from Monash University. The ALS is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under contract no. DE-AC02-05CH11231. NR 59 TC 0 Z9 0 U1 2 U2 9 PU ROYAL SOC PI LONDON PA 6-9 CARLTON HOUSE TERRACE, LONDON SW1Y 5AG, ENGLAND SN 1742-5689 EI 1742-5662 J9 J R SOC INTERFACE JI J. R. Soc. Interface PD JUL 6 PY 2015 VL 12 IS 108 AR 20150252 DI 10.1098/rsif.2015.0252 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CO0FD UT WOS:000358824600025 PM 26063819 ER PT J AU Arion, T Neppl, S Roth, F Shavorskiy, A Bluhm, H Hussain, Z Gessner, O Eberhardt, W AF Arion, Tiberiu Neppl, Stefan Roth, Friedrich Shavorskiy, Andrey Bluhm, Hendrik Hussain, Zahid Gessner, Oliver Eberhardt, Wolfgang TI Site-specific probing of charge transfer dynamics in organic photovoltaics (vol 106, 121602, 2015) SO APPLIED PHYSICS LETTERS LA English DT Correction C1 [Arion, Tiberiu; Roth, Friedrich; Eberhardt, Wolfgang] Ctr Free Electron Laser Sci DESY, D-22607 Hamburg, Germany. [Neppl, Stefan; Shavorskiy, Andrey; Bluhm, Hendrik; Gessner, Oliver] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Hussain, Zahid; Eberhardt, Wolfgang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, ALS, Berkeley, CA 94720 USA. [Eberhardt, Wolfgang] TU Berlin, Inst Opt & Atom Phys, D-10623 Berlin, Germany. RP Arion, T (reprint author), Ctr Free Electron Laser Sci DESY, Notkestr 85, D-22607 Hamburg, Germany. NR 1 TC 0 Z9 0 U1 1 U2 10 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUL 6 PY 2015 VL 107 IS 1 AR 019903 DI 10.1063/1.4926838 PG 1 WC Physics, Applied SC Physics GA CM6TX UT WOS:000357824200065 ER PT J AU Chen, Y Cai, L Liu, ZC dela Cruz, CR Liang, CD An, K AF Chen, Yan Cai, Lu Liu, Zengcai dela Cruz, Clarina R. Liang, Chengdu An, Ke TI Correlation of anisotropy and directional conduction in beta-Li3PS4 fast Li+ conductor SO APPLIED PHYSICS LETTERS LA English DT Article ID SITU NEUTRON-DIFFRACTION; CRYSTAL-STRUCTURE; IONIC-CONDUCTIVITY; THERMAL-EXPANSION; PHASE-TRANSITION; BEHAVIOR; ELECTROLYTES; LI3PS4 AB This letter reports the correlation of anisotropy and directional conduction in the fast Li-1 conductor beta-Li3PS4, one of the low-symmetry crystalline electrolyte candidates. The material has both high conductivity and good stability that serves well for the large-scale energy storage applications of all-solid-state lithium ion batteries. The anisotropic physical properties, demonstrated here by the thermal expansion coefficients, are crucial for compatibility in the solid-state system and battery performance. Neutron and X-ray powder diffraction measurements were done to determine the crystal structure and thermal stability. The crystallographic b-axis was revealed as a fast expansion direction, while negligible thermal expansion was observed along the a-axis around the battery operating temperatures. The anisotropic behavior has its structural origin from the Li-1 conduction channels with incomplete Li occupancy and a flexible connection of LiS4 and PS4 tetrahedra within the framework. This indicates a strong correlation in the direction of the ionic transport in the low-symmetry Li-1 conductor. (C) 2015 AIP Publishing LLC. C1 [Chen, Yan; Cai, Lu; An, Ke] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Liu, Zengcai; Liang, Chengdu] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [dela Cruz, Clarina R.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP An, K (reprint author), Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. EM kean@ornl.gov RI An, Ke/G-5226-2011; Chen, Yan/H-4913-2014; dela Cruz, Clarina/C-2747-2013 OI An, Ke/0000-0002-6093-429X; Chen, Yan/0000-0001-6095-1754; dela Cruz, Clarina/0000-0003-4233-2145 FU Division of Materials Science and Engineering, Office of Basic Energy Sciences (BES), U.S. Department of Energy (DOE); Scientific User Facilities Division, BES, DOE FX This work was supported by the Division of Materials Science and Engineering, Office of Basic Energy Sciences (BES), U.S. Department of Energy (DOE). Neutron scattering experiments were carried out at the Spallation Neutron Source (SNS) and High Flux Isotope Reactor (HFIR) at Oak Ridge National Laboratory. X-ray diffraction experiments were performed at the Center for Nanophase Materials Sciences (CNMS). SNS, HFIR, and CNMS are national user facilities sponsored by the Scientific User Facilities Division, BES, DOE. The authors thank Dr. E. A. Payzant from SNS and Ms. K. Andrews from HFIR for their technical support of the neutron experiments. The authors thank Mrs. Gumin Zhu for the technical support. NR 28 TC 5 Z9 5 U1 11 U2 62 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUL 6 PY 2015 VL 107 IS 1 AR 013904 DI 10.1063/1.4926725 PG 5 WC Physics, Applied SC Physics GA CM6TX UT WOS:000357824200055 ER PT J AU Resnik, B Nussdorf, B AF Resnik, Bennett Nussdorf, Benjamin TI Innovation addresses US environmental regulations; more needed SO OIL & GAS JOURNAL LA English DT Article C1 [Resnik, Bennett] Vermont Law Sch, South Royalton, VT 05068 USA. [Nussdorf, Benjamin] US DOE, Washington, DC USA. RP Resnik, B (reprint author), Vermont Law Sch, South Royalton, VT 05068 USA. EM resnikbe@gmail.com; nussdorf@american.edu NR 4 TC 0 Z9 0 U1 0 U2 0 PU PENNWELL PUBL CO ENERGY GROUP PI TULSA PA 1421 S SHERIDAN RD PO BOX 1260, TULSA, OK 74112 USA SN 0030-1388 EI 1944-9151 J9 OIL GAS J JI Oil Gas J. PD JUL 6 PY 2015 VL 113 IS 7 BP 70 EP 73 PG 4 WC Energy & Fuels; Engineering, Petroleum SC Energy & Fuels; Engineering GA CN1MY UT WOS:000358185300018 ER PT J AU Zhu, L Chen, K Hao, J Wei, ZY Zhang, HC Yin, PC Wei, YG AF Zhu, Li Chen, Kun Hao, Jian Wei, Zheyu Zhang, Haocheng Yin, Panchao Wei, Yongge TI Synthesis and Crystallization Behavior of Surfactants with Hexamolybdate as the Polar Headgroup SO INORGANIC CHEMISTRY LA English DT Article ID POLYOXOMETALATE-ORGANIC HYBRID; CLUSTERS; NANOSCALE; CATALYSTS; DEVICES; DESIGN AB Alkyl chains with different lengths were covalently grafted onto the surface of hexamolybdate through the postfunctionalization protocol of polyoxometalates. The obtained compounds represent typical structures of the so-called giant surfactants. Unexpectedly, those surfactants with hexamolybdates as polar headgroups are able to crystallize, while single-crystal X-ray diffraction reveals that the crystallization behavior of the surfactants is highly dependent on the length of the alkyl chains. For surfactants with comparatively short alkyl chains (C6 and C10), the alkyl chains prefer to interact with tetrabutylammonium, the countercation of hexamolybdate. However, the alkyl chains tend to pack with each other to form a domain of alkyl chains in the surfactant with a longer alkyl chain (C18). The possible mechanism is that a long alkyl chain cannot be fully compatible with the short chain (C4) of tetrabutylammonium. C1 [Zhu, Li] Beijing Union Univ, Beijing 100101, Peoples R China. [Zhu, Li; Chen, Kun; Hao, Jian; Wei, Zheyu; Zhang, Haocheng; Wei, Yongge] Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China. [Yin, Panchao] Oak Ridge Natl Lab, Chem & Engn Mat Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. [Wei, Yongge] Peking Univ, State Key Lab Nat & Biomimet Drugs, Beijing 100191, Peoples R China. RP Yin, PC (reprint author), Oak Ridge Natl Lab, Chem & Engn Mat Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. EM yinp@ornl.gov; yonggewei@mail.tsinghua.edu.cn RI Yin, Panchao/J-3322-2013; Wei, Yen/H-5329-2012 OI Yin, Panchao/0000-0003-2902-8376; FU Neutron Sciences Directorate at Oak Ridge National Laboratory; Office of Science of the U.S. Department of Energy [DE-AC0500OR22725]; National Natural Science Foundation of China (NSFC) [21225103, 21221062]; Tsinghua University Initiative Foundation Research Program [20131089204] FX We acknowledge the Clifford G. Shull Fellowship support from the Neutron Sciences Directorate at Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract DE-AC0500OR22725, and the support from the National Natural Science Foundation of China (NSFC Grants 21225103 and 21221062) and the Tsinghua University Initiative Foundation Research Program 20131089204. NR 23 TC 7 Z9 7 U1 7 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUL 6 PY 2015 VL 54 IS 13 BP 6075 EP 6077 DI 10.1021/acs.inorgchem.5b00903 PG 3 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CM5DA UT WOS:000357705800005 PM 26067891 ER PT J AU Mednikov, EG Ivanov, SA Dahl, LF AF Mednikov, Evgueni G. Ivanov, Sergei A. Dahl, Lawrence F. TI Nanosized {Pd-4(mu(4)-C)}Pd-32(CO)(28)(PMe3)(14) Containing Tetrahedrally Deformed Pd-4 Cage with Encapsulated Carbide Atom: Formal Substitution of Geometrically Analogous Interior Au-4 Entity in Isostructural Au4Pd32(CO)(28)(PMe3)(14) by Electronically Equivalent Pd-4(mu(4)-C) and Computational/Catalytic Implications SO INORGANIC CHEMISTRY LA English DT Article ID VINYL-ACETATE SYNTHESIS; CARBONYL CLUSTER COMPLEXES; CRYSTAL-STRUCTURE; MOLECULAR-STRUCTURES; METAL CLUSTER; STRUCTURAL-CHARACTERIZATION; CARBIDOCARBONYL CLUSTERS; CHIROPTICAL PROPERTIES; INTERSTITIAL CARBON; GROWTH-PATTERNS AB This first homopalladium carbido cluster, {Pd-4(mu C4-)}Pd-32(CO)(28)(PMe3)(14) (1), was isolated (3-7% yields) from an ultimately simplified procedure the reaction of CHCl3 under N-2 with either Pd-8(CO)(8)(PMe3)(7) or Pd-10(CO)(12)(PMe3)(6) at room temperature. Charge-coupled device (CCD) X-ray diffraction data at 100 K for 1.2.5 C6H14 (1a) and 1.3 CHCl3 (1b) produced closely related molecular parameters for 1. This {Pd4C}Pd-32 cluster (1) possesses a highly unusual tetracoordinated carbide atom that causes a major distortion of a central regular Pd-4 tetrahedron into a new symmetry type of encapsulated Pd-4 cage of pseudo-D-2 (222) symmetry. Mean Pd-Pd distances for the three pairs of opposite twofold-equivalent Pd-Pd tetrahedral-like edges for Ia are 2.71, 2.96, and 3.59 angstrom; the mean of the four Pd-C distances [range, 1.87(2)-1.94(2) angstrom] is 1.91 angstrom. An astonishing molecular feature is that this {Pd4C}Pd-32 cluster (1) is an isostructural and electronically equivalent analogue of the nanosized Au4Pd32(CO)(28)(PMe3)(14) (2). Cluster 2, likewise a pseudo-D-2 molecule, contains a geometrically analogous tetrahedrally deformed interior Au, entity encapsulated within an identical Pd-32(CO)(28)(PMe3)(14) shell; mean distances for the three corresponding symmetry-equivalent pairs of slightly smaller opposite tetrahedral-distorted Au-Au edges are 2.64, 2.90, and 3.51 angstrom. A computational study by both a natural population analysis (NPA) and an atoms-in-molecules (AIM) method performed on model analogues {Pd14C}Pd-32(CO)(28)(PH3)(14) (1-mod) and Au4Pd32(CO)(28)(PH3)(14) (2-mod) suggested that the negatively charged Au-4 entity in 2-mod may be described as two weakly interacting electron-pair Au-2 intradimers. In contrast, an NPA of the {Pd4C} entity in 1-mod revealed that two similarly oriented identical Pd-2 intradimers of 2.71 angstrom are primarily stabilized by Pd-C bonding with a negatively charged carbide atom. The isostructural stabilizations of 1 and 2 are then attributed to the similar sizes, shapes, and overall negative charge distributions of the electronically equivalent interior {Pd4C} and Au-4 entities. This resulting remarkable structural/electronic equivalency between 1 and 2 is consistent with the greatly improved performances of commercial palladium catalysts for vinyl acetate synthesis by gold-atom incorporation to suppress carbonization of the Pd atoms, namely, that the extra Au 6s(1) valence electron of each added Au atom provides an effective "negative charge protection" against electron-donating carbon atoms forming Pd carbido species such as {Pd4C}. C1 [Mednikov, Evgueni G.; Dahl, Lawrence F.] Univ Wisconsin, Dept Chem, Madison, WI 53706 USA. [Ivanov, Sergei A.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. RP Mednikov, EG (reprint author), Univ Wisconsin, Dept Chem, 1101 Univ Ave, Madison, WI 53706 USA. EM mednikov@chem.wisc.edu; dahl@chem.wisc.edu RI Ivanov, Sergei/B-5505-2011 FU Univ. of Wisconsin-Madison; Hilldale Foundation (UW-Madison); National Science Foundation [CHE-9310428] FX This research was supported by the Univ. of Wisconsin-Madison and the Hilldale Foundation (UW-Madison). The SMART 1000 CCD X-ray area-detector system was purchased, in part, from National Science Foundation Grant No. CHE-9310428. Structural drawings were prepared with Crystal Maker Software (D. C. Palmer, Centre for Innovation & Enterprise, Begbroke Science Park, Bldg 5, Sandy Lane, Yarnton, Oxfordshire OX5 1PF, U.K.). We are grateful to Prof. John F. Berry (Chem. Dept.; UW-Madison) and Prof. June Dahl (Dept. of Neuroscience; UW School of Medicine & Public Health) for helpful comments. We also thank Dr. Ilia Guzei (Chem. Dept.; UW-Madison) for crystallographic advice and the use of the Departmental X-ray Crystallographic Facilities. NR 92 TC 0 Z9 0 U1 1 U2 6 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUL 6 PY 2015 VL 54 IS 13 BP 6157 EP 6168 DI 10.1021/acs.inorgchem.5b00208 PG 12 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CM5DA UT WOS:000357705800016 PM 25946428 ER PT J AU Niklas, J Westwood, M Mardis, KL Brown, TL Pitts-McCoy, AM Hopkins, MD Poluektov, OG AF Niklas, Jens Westwood, Mark Mardis, Kristy L. Brown, Tiara L. Pitts-McCoy, Anthony M. Hopkins, Michael D. Poluektov, Oleg G. TI X-ray Crystallographic, Multifrequency Electron Paramagnetic Resonance, and Density Functional Theory Characterization of the Ni((P2N2tBu)-N-Cy)(2)(n+)) Hydrogen Oxidation Catalyst in the Ni(I) Oxidation State SO INORGANIC CHEMISTRY LA English DT Article ID PENDANT AMINES; MOLECULAR ELECTROCATALYSTS; SOLAR-ENERGY; EPR; SPECTROSCOPY; SOFTWARE; REDUCTION; COMPLEXES; DELIVERY; SOLVENT AB The Ni(I) hydrogen oxidation catalyst [Ni-((P2N2tBu)-N-Cy)(2)](+) (1(+); (P2Nt2Bu)-N-Cy = 1,5-di(tert-butyl)-3,7-dicyclohexyl-1,5-diaza-3,7-diphosphacyclooctane) has been studied using a combination of electron paramagnetic resonance (EPR) techniques (X-, Q-, and D-band, electron nuclear double resonance, hyperfine sublevel correlation spectroscopy), X-ray crystallography, and density functional theory (DFT) calculations. Crystallographic and DFT studies indicate that the molecular structure of 1(+) is highly symmetrical. EPR spectroscopy has allowed determination of the electronic g tensor and the spin density distribution on the ligands, and revealed that the Ni(I) center does not interact strongly with the potentially coordinating solvents acetonitrile and butyronitrile. The EPR spectra and magnetic parameters of 1(+) are found to be distinctly different from those for the related compound [Ni((P2N2Ph)-N-Ph)(2)](+) (4(+)). One significant contributor to these differences is that the molecular structure of 4(+) is unsymmetrical, unlike that of 1(+). DFT calculations on derivatives in which the Rand R' groups are systematically varied have allowed elucidation of structure/substituent relationships and their corresponding influence on the magnetic resonance parameters. C1 [Niklas, Jens; Poluektov, Oleg G.] Argonne Natl Lab, Div Chem Sci & Engn, Argonne, IL 60439 USA. [Westwood, Mark; Hopkins, Michael D.] Univ Chicago, Dept Chem, Chicago, IL 60637 USA. [Mardis, Kristy L.; Brown, Tiara L.; Pitts-McCoy, Anthony M.] Chicago State Univ, Dept Chem & Phys, Chicago, IL 60628 USA. RP Hopkins, MD (reprint author), Univ Chicago, Dept Chem, 5735 S Ellis Ave, Chicago, IL 60637 USA. EM mhopkins@uchicago.edu; oleg@anl.gov RI Niklas, Jens/I-8598-2016; OI Niklas, Jens/0000-0002-6462-2680; Mardis, Kristy/0000-0003-2633-9304 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-AC02-06CH11357, DE-FG02-07-ER15910]; Illinois Space Grant Consortium; National Institutes of Health National Institute of General Medical Sciences (NIGMS) [R25 GM59218] FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, under Contract Numbers DE-AC02-06CH11357 at Argonne National Laboratory (J.N. and O.G.P.) and DE-FG02-07-ER15910 (M.W. and M.D.H.). K.L.M. was supported by the Illinois Space Grant Consortium, and T.L.B. and A.M.P.-M. were supported by a National Institutes of Health National Institute of General Medical Sciences (NIGMS) Grant (R25 GM59218). We thank Dr. Ian Steele and Dr. Alex Filatov for determining the crystal structure. NR 56 TC 3 Z9 3 U1 2 U2 11 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUL 6 PY 2015 VL 54 IS 13 BP 6226 EP 6234 DI 10.1021/acs.inorgchem.5b00445 PG 9 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CM5DA UT WOS:000357705800023 PM 26098955 ER PT J AU Reichert, MD White, MA Thompson, MJ Miller, GJ Vela, J AF Reichert, Malinda D. White, Miles A. Thompson, Michelle J. Miller, Gordon J. Vela, Javier TI Preparation and Instability of Nanocrystalline Cuprous Nitride SO INORGANIC CHEMISTRY LA English DT Article ID AUGMENTED-WAVE METHOD; COPPER NITRIDE; THIN-FILMS; SOLVOTHERMAL SYNTHESIS; THERMAL-STABILITY; CU3N; CUO; NANOCUBES; AMMONIA; CU2O AB Low-dimensional cuprous, nitride (Cu3N) was synthesized by nitridation (ammonolysis) of cuprous oxide (Cu2O) nanocrystals using either ammonia (NH3) or urea (H2NCONH2) as the nitrogen source. The resulting nanocrystalline Cu3N spontaneously decomposes to nanocrystalline CuO in the presence of both water and oxygen from air at. room temperature. Ammonia was produced in 60% chemical yield during Cu3N decomposition, as measured using the colorimetric indophenol Method. Because Cu3N decomposition requites H2O and produces substoichiometric amounts of NH3, we conclude that this reaction proceeds through a complex stoichiometry that involves the concomitant release of both N-2 and NH3. This is a thermodynamically unfavorable outcome, strongly indicating that H2O (and thus NH3 production) facilitate the kinetics of the reaction by lowering the energy barrier for Cu3N decomposition. The three different Cu2O, Cu3N, and CuO nano crystalline phases were characterized by a combination of optical absorption, powder X-ray diffraction, transmission electron microscopy, and electronic density of states obtained from electronic structure calculations on the bulk solids. The relative ease of interconversion between these interesting and inexpensive materials bears possible implications for catalytic and optoelectronic applications. C1 [Vela, Javier] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. Ames Lab, Ames, IA 50011 USA. RP Vela, J (reprint author), Iowa State Univ, Dept Chem, Ames, IA 50011 USA. EM vela@iastate.edu RI Vela, Javier/I-4724-2014 OI Vela, Javier/0000-0001-5124-6893 FU National Science Foundation through the Division of Materials Research, Solid State and Materials Chemistry program [NSF-DMR-1309510] FX J.V. gratefully acknowledges the National Science Foundation for funding of this work through the Division of Materials Research, Solid State and Materials Chemistry program (NSF-DMR-1309510). M.A.W. thanks Yuemei Zhang for assistance with calculations. NR 50 TC 1 Z9 1 U1 5 U2 53 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUL 6 PY 2015 VL 54 IS 13 BP 6356 EP 6362 DI 10.1021/acs.inorgchem.5b00679 PG 7 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CM5DA UT WOS:000357705800037 PM 26091284 ER PT J AU Zhang, SG Bullock, RM AF Zhang, Shaoguang Bullock, R. Morris TI Molybdenum Hydride and Dihydride Complexes Bearing Diphosphine Ligands with a Pendant Amine: Formation of Complexes with Bound Amines SO INORGANIC CHEMISTRY LA English DT Article ID TRANSITION-METAL HYDRIDES; N-HETEROCYCLIC CARBENE; CATALYTIC IONIC HYDROGENATIONS; HETEROLYTIC CLEAVAGE; CARBONYL HYDRIDES; DIHYDROGEN COMPLEXES; STRUCTURAL-CHARACTERIZATION; MOLECULAR ELECTROCATALYSTS; AZADITHIOLATE COFACTOR; PROTON-TRANSFER AB CpMo(CO)(PNP)H complexes (PNP = (R2PCH2)(2)NMe, R = Et or Ph) were synthesized by displacement of two CO ligands of CpMo(CO)(3)H by the PNP ligand; these complexes were characterized by IR and variable temperature H-1 and P-31 NIVIR spectroscopy. CpMo(CO)(PNP)H complexes are formed as mixture of cis- and trans-isomers. The structures of both cis-CpMo (CO)((PNPEt)-N-Et-P-Me)H and trans-CpMo(CO)((PNPPh)-N-Ph-P-Me) H were determined by single crystal X-ray diffraction. Electrochemical oxidation of CpMo(CO)((PNPEt)-N-Et-P-Me)H and CpMo(CO)-((PNPPh)-N-Ph-P-Me)H in CH3CN are both irreversible at slow scan rates and quasireversible at higher scan rates, with E-1/2 = -0.36 V (vs Cp2Fe+/0) for CpMo(CO)((PNPEt)-N-Et-P-Me)H and E-1/2 = -0.18 V for CpMo (CO) ((PNPPh)-N-Ph-P-Me)H. Hydride abstraction from CpMo-(CO)(PNP)H with [Ph3C](+)[A](-) (A = B(C6F5)(4) or BAr4F; [Ar-F = 3,5-bis(trifluoromethyl)phenyl]) afforded "tuck-in" [CpMo(CO)(kappa(3)-(PNPEt)-N-Et-P-Me)](+) complexes that feature the amine bound to the metal. Displacement of the kappa(3) Mo-N bond by CD3CN gives [CpMo(CO)(PNP)(CD3CN)](+). The kinetics of this reaction were studied by 31P{H-1} NMR spectroscopy for [CpMo(CO)(kappa(3)-(PNPEt)-N-Et-P-Me)](+), providing the activation parameters Delta H-double dagger = 21.6 +/- 2.8 kcal/mol, Delta S-double dagger = -0.3 +/- 9.8 cal/(mol K), E-a = 22.1 +/- 2.8 kcal/mol. Protonation of CpMo(CO)((PNPEt)-N-Et-P-Me)H affords the Mo dihydride complex [CpMo(CO)(kappa(2)-(PNPEt)-N-Et-P-Me)(H)(2)](+), which loses H-2 to generate [CpMo (CO)(kappa(3)-(PNPEt)-N-Et-P-Me)](+) at room temperature. Our results show that the pendant amine has a strong driving force to form stable "tuck-in" [CpMo(CO)(kappa(3)-PNP)](+) complexes, and also promotes hydrogen elimination from [CpMo(CO)(PNP)(H)(2)](+) complexes by formation of a Mo-N dative bond. CpMo(CO)(dppp)H (dppp = 1,3-bis(diphenylphosphino)propane) was studied as a Mo diphosphine analogue without a pendant amine, and the product of protonation of this complex gives [CpMo(CO)(dppp)(H)(2)](+). C1 [Zhang, Shaoguang; Bullock, R. Morris] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP Bullock, RM (reprint author), Pacific NW Natl Lab, Div Phys Sci, POB 999,K2-12, Richland, WA 99352 USA. EM Morris.Bullock@pnnl.gov RI Bullock, R. Morris/L-6802-2016 OI Bullock, R. Morris/0000-0001-6306-4851 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences FX We thank the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences for support. Pacific Northwest National Laboratory is operated by Battelle for the U.S. Department of Energy. Appel for helpful discussions; and Ming Fang for assistance on the electrochemical experiments. NR 109 TC 4 Z9 4 U1 3 U2 23 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUL 6 PY 2015 VL 54 IS 13 BP 6397 EP 6409 DI 10.1021/acs.inorgchem.5b00728 PG 13 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CM5DA UT WOS:000357705800042 PM 26054002 ER PT J AU Inoue, T Janes, DW Ren, JX Suh, HS Chen, XX Ellison, CJ Nealey, PF AF Inoue, Takejiro Janes, Dustin W. Ren, Jiaxing Suh, Hyo Seon Chen, Xuanxuan Ellison, Christopher J. Nealey, Paul F. TI Molecular Transfer Printing of Block Copolymer Patterns over Large Areas with Conformal Layers SO ADVANCED MATERIALS INTERFACES LA English DT Article ID DIBLOCK COPOLYMER; FILMS; GRAPHOEPITAXY; STRESS; NANOFABRICATION; ORIENTATION; ROUGHNESS; DOMAINS; DEVICE AB Areal defect frequency in patterns formed by the directed self-assembly of block copolymers can likely be minimized by using 1:1 chemical nanopatterns. Here, a transfer printing technique is demonstrated by using conformal layers that generates continuous, sub-15 nm resolution, 1:1 chemical nanopatterns over large areas. C1 [Inoue, Takejiro; Ren, Jiaxing; Suh, Hyo Seon; Chen, Xuanxuan; Nealey, Paul F.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. [Janes, Dustin W.; Ellison, Christopher J.] Univ Texas Austin, McKetta Dept Chem Engn, Austin, TX 78712 USA. [Suh, Hyo Seon; Nealey, Paul F.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Nealey, PF (reprint author), Univ Chicago, Inst Mol Engn, 5801 South Ellis Ave, Chicago, IL 60637 USA. EM nealey@uchicago.edu FU U.S. DOE [DE-AC02-06CH11357]; Toray Industries, Inc.; Welch Foundation [F-1709] FX The authors thank Paulina Rincon and Roel Gronheid of IMEC for providing chemically patterned substrates for DSA, and Merck KGaA for providing materials. Use of the Center for Nanoscale Materials (CNM) and Advanced Photon Source (APS), an Office of Science User Facility operated for the U.S. DOE Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. The authors thank Christopher J. Thode for making SiO2 coated fingerprint patterns used during the early stages of this work. T. Inoue acknowledges financial support from Toray Industries, Inc. C.J.E. acknowledges partial financial support from the Welch Foundation (Grant No. F-1709). NR 36 TC 5 Z9 5 U1 4 U2 30 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2196-7350 J9 ADV MATER INTERFACES JI Adv. Mater. Interfaces PD JUL 6 PY 2015 VL 2 IS 10 AR 1500133 DI 10.1002/admi.201500133 PG 9 WC Chemistry, Multidisciplinary; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CM4WO UT WOS:000357686600008 ER PT J AU Jones, JL LeBeau, JM Nikkel, J Oni, AA Dycus, JH Cozzan, C Lin, FY Chernatynskiy, A Nino, JC Sinnott, SB Mhin, S Brennecka, GL Ihlefeld, J AF Jones, Jacob L. LeBeau, James M. Nikkel, Jason Oni, Adedapo A. Dycus, J. Houston Cozzan, Clayton Lin, Fang-Yin Chernatynskiy, Aleksandr Nino, Juan C. Sinnott, Susan B. Mhin, Sungwook Brennecka, Geoff L. Ihlefeld, Jon TI Combined Experimental and Computational Methods Reveal the Evolution of Buried Interfaces during Synthesis of Ferroelectric Thin Films SO ADVANCED MATERIALS INTERFACES LA English DT Article ID LEAD-ZIRCONATE-TITANATE; CHEMICAL SOLUTION DEPOSITION; ELECTRICAL-PROPERTIES; TEXTURE EVOLUTION; PHASE; CRYSTALLIZATION; PT/TI/SIO2/SI; SILICON; OXIDE; MICROSTRUCTURE AB Understanding interfaces between dissimilar materials is crucial to the development of modern technologies, for example, semiconductor-dielectric and thermoelectric-semiconductor interfaces in emerging electronic devices. However, the structural characterization of buried interfaces is challenging because many measurement techniques are surface sensitive by design. When interested in interface evolution during synthesis, the experimental challenges multiply and often necessitate in situ techniques. For solution-derived lead zirconate titanate (PZT) ferroelectric thin films, the evolution of buried interfaces during synthesis (including dielectric-metal and metal-metal) is thought to dramatically influence the resultant dielectric and ferroelectric properties. In the present work, multiple experimental and computational methods are combined to characterize interface evolution during synthesis of ferroelectric PZT films on platinized Si wafers-including in situ X-ray diffraction during thermal treatment, aberration-corrected scanning transmission electron microscopy of samples quenched from various synthesis states, and calculations using density functional theory. Substantial interactions at buried interfaces in the PZT/Pt/Ti/SiOx/Si heterostructure are observed and discussed relative to their role(s) in the synthesis process. The results prove that perovskite PZT nucleates directly from the platinum (111)-oriented bottom electrode and reveal the roles of Pb and O diffusion and intermetallic Pt3Pb and Pt3Ti phases. C1 [Jones, Jacob L.; LeBeau, James M.; Nikkel, Jason; Oni, Adedapo A.; Dycus, J. Houston] N Carolina State Univ, Dept Mat Sci & Engn, Raleigh, NC 27695 USA. [Cozzan, Clayton; Lin, Fang-Yin; Chernatynskiy, Aleksandr; Nino, Juan C.; Sinnott, Susan B.] Univ Florida, Dept Mat Sci & Engn, Gainesville, FL 32611 USA. [Mhin, Sungwook] Korea Inst Ind Technol KITECH, Heat Treatment Technol R&BD Grp, Inchon 406840, South Korea. [Brennecka, Geoff L.] Colorado Sch Mines, Dept Met & Mat Engn, Golden, CO 80401 USA. [Ihlefeld, Jon] Sandia Natl Labs, Elect Opt & Nanostruct Mat Dept, Albuquerque, NM 87185 USA. RP Jones, JL (reprint author), N Carolina State Univ, Dept Mat Sci & Engn, Box 7907, Raleigh, NC 27695 USA. EM jacobjones@ncsu.edu RI Nino, Juan/A-6496-2008; Brennecka, Geoff/J-9367-2012; OI Nino, Juan/0000-0001-8256-0535; Brennecka, Geoff/0000-0002-4476-7655; Chernatynskiy, Aleksandr/0000-0001-7431-7201; Cozzan, Clayton/0000-0003-3409-0377 FU NSF [DMR-1207293]; National Science Foundation; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors acknowledge support for this work under NSF award number DMR-1207293 and the use of the Analytical Instrumentation Facility (AIF) at North Carolina State University, which is supported by the State of North Carolina and the National Science Foundation. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract no. DE-AC04-94AL85000. NR 48 TC 1 Z9 1 U1 3 U2 37 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2196-7350 J9 ADV MATER INTERFACES JI Adv. Mater. Interfaces PD JUL 6 PY 2015 VL 2 IS 10 AR 1500181 DI 10.1002/admi.201500181 PG 10 WC Chemistry, Multidisciplinary; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CM4WO UT WOS:000357686600011 ER PT J AU Kim, JH Pieczonka, NPW Lu, P Liu, ZY Qiao, RM Yang, WL Tessema, MM Sun, YK Powell, BR AF Kim, Jung-Hyun Pieczonka, Nicholas P. W. Lu, Peng Liu, Zhongyi Qiao, Ruimin Yang, Wanli Tessema, Misle M. Sun, Yang-Kook Powell, Bob R. TI In Situ Formation of a Cathode-Electrolyte Interface with Enhanced Stability by Titanium Substitution for High Voltage Spinel Lithium-Ion Batteries SO ADVANCED MATERIALS INTERFACES LA English DT Article ID LI-ION; ELECTROCHEMICAL PROPERTIES; LIMN1.5NI0.5-XMXO4 M; NEGATIVE ELECTRODES; LINI0.5MN1.5O4; GRAPHITE; PERFORMANCE; CELLS; DISSOLUTION; CHEMISTRY AB Although LiNi0.5Mn1.5O4 (LNMO) high-voltage spinel is a promising candidate for a next generation cathode material, LNMO/graphite full cells experience severe capacity fading caused by degradation reactions at electrode/electrolyte interfaces and consequent active Li+ loss in the cells. In this study, it is first reported that in situ formation of a Ti-O enriched cathode/electrolyte interfacial (CEI) layer on a Ti-substituted LiNi0.5Mn1.2Ti0.3O4 (LNMTO) spinel cathode effectively mitigates electrolyte oxidation and transition metal dissolution, which improves the Coulombic efficiency and cycle life of LNMTO/graphite full cells. The Ti-O enriched CEI layer is produced in situ during an initial cycling of LNMTO as a result of selective Mn and Ni dissolution at its surface, as evidenced by various surface characterizations using X-ray photoelectron spectroscopy, transmission electron microscopy, time-of-flight secondary ion mass spectrometry, Raman spectroscopy, and synchrotron-based soft X-ray absorption spectroscopy. The Ti-O enriched CEI has an advantage over traditional LNMO powder coatings, namely the formation of conformal CEI without compromising electronic conduction pathways between cathode particles. C1 [Kim, Jung-Hyun; Lu, Peng; Liu, Zhongyi; Powell, Bob R.] Gen Motors Global R&D Ctr, Chem & Mat Syst Lab, Warren, MI 48090 USA. [Pieczonka, Nicholas P. W.] Optimal CAE Inc, Plymouth, MI 48170 USA. [Qiao, Ruimin; Yang, Wanli] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Tessema, Misle M.] GM Global Powertrain, Engn Operat, Warren, MI 48090 USA. [Sun, Yang-Kook] Hanyang Univ, Dept Energy Engn, Seoul 133791, South Korea. RP Kim, JH (reprint author), Gen Motors Global R&D Ctr, Chem & Mat Syst Lab, Warren, MI 48090 USA. EM junghyun.kim@gm.com; yksun@hanyang.ac.kr RI Qiao, Ruimin/E-9023-2013; Yang, Wanli/D-7183-2011; Kim, Jung-Hyun/I-5273-2013 OI Yang, Wanli/0000-0003-0666-8063; Kim, Jung-Hyun/0000-0002-4598-4686 NR 57 TC 8 Z9 8 U1 10 U2 91 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2196-7350 J9 ADV MATER INTERFACES JI Adv. Mater. Interfaces PD JUL 6 PY 2015 VL 2 IS 10 AR 1500109 DI 10.1002/admi.201500109 PG 13 WC Chemistry, Multidisciplinary; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CM4WO UT WOS:000357686600007 ER PT J AU Huang, TC Petriello, F AF Huang, Ting-Chung Petriello, Frank TI Rare exclusive decays of the Z boson revisited SO PHYSICAL REVIEW D LA English DT Article ID QUANTUM CHROMODYNAMICS; FORM-FACTORS; MESON AB The realization that first- and second-generation Yukawa couplings can be probed by decays of the Higgs boson to a meson in association with a photon has renewed interest in such rare exclusive decays. We present here a detailed study of the rare Z-boson processes Z -> J/psi + gamma, Z -> gamma + gamma, and Z -> phi + gamma that can serve as benchmarks for the analogous Higgs-boson decays. We include both direct-production and fragmentation contributions to these decays and consider the leading QCD corrections and the relativistic corrections to the J/(if and 7 processes. We present numerical predictions for the branching ratios that include a careful accounting of the theoretical uncertainties. C1 [Huang, Ting-Chung; Petriello, Frank] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60201 USA. [Petriello, Frank] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. RP Huang, TC (reprint author), Northwestern Univ, Dept Phys & Astron, Evanston, IL 60201 USA. EM tingchunghuang2014@u.northwestern.edu; f-petriello@northwestern.edu FU DOE [DE-FG02-91ER40684, DE-AC02-06CH11357] FX We thank K. Nikolopoulos for helpful discussions and for encouraging us to pursue this calculation. We also thank A. Chisholm, S. Stoynev, and M. Velasco for useful discussions. This work is supported in part by the DOE Contract No. DE-FG02-91ER40684 and Grant No. DE-AC02-06CH11357. NR 28 TC 3 Z9 3 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. 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Gershtein, Y. Gray, R. Halkiadakis, E. Hidas, D. Kaplan, S. Lath, A. Panwalkar, S. Park, M. Patel, R. Salur, S. Schnetzer, S. Somalwar, S. Stone, R. Thomas, S. Thomassen, P. Walker, M. Rose, K. Spanier, S. York, A. Bouhali, O. Hernandez, A. Castaneda Eusebi, R. Flanagan, W. Gilmore, J. Kamon, T. Khotilovich, V. Krutelyov, V. Montalvo, R. Osipenkov, I. Pakhotin, Y. Perloff, A. Roe, J. Rose, A. Safonov, A. Sakuma, T. Suarez, I. Tatarinov, A. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kovitanggoon, K. Kunori, S. Lee, S. W. Libeiro, T. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Johns, W. Maguire, C. Mao, Y. Melo, A. Sharma, M. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Arenton, M. W. Boutle, S. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Wood, J. Clarke, C. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Sturdy, J. Belknap, D. A. Carlsmith, D. Cepeda, M. Dasu, S. Dodd, L. Duric, S. Friis, E. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Lanaro, A. Lazaridis, C. Levine, A. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Sarangi, T. Savin, A. Smith, W. H. Taylor, D. Verwilligen, P. Vuosalo, C. Woods, N. CA CMS Collaboration TI Measurement of diffractive dissociation cross sections in pp collisions at root s=7 TeV SO PHYSICAL REVIEW D LA English DT Article ID TRANSVERSE-MOMENTUM SPECTRA; LHC DATA; COLLIDER; MODEL; SCATTERING; PHYSICS; ISR AB Measurements of diffractive dissociation cross sections in pp collisions at root s = 7 TeV are presented in kinematic regions defined by the masses M-X and M-Y of the two final-state hadronic systems separated by the largest rapidity gap in the event. Differential cross sections are measured as a function of xi= M-X(2)/s in the region -5.5 < log(10)xi 10(X) < -2.5, for logio M-Y < 0.5, dominated by single dissociation (SD), and 0.5 < log(10)M(Y) < 1.1, dominated by double dissociation (DD), where M-x and M-y are given in GeV. The inclusive pp cross section is also measured as a function of the width of the central pseudorapidity gap Delta eta for Delta eta > 3, logio M-X > 1.1, and logioMy > 1.1, a region dominated by DD. The cross sections integrated over these regions are found to be, respectively, 2.99 0.02(staf)12392(sysf) mb, 1.18 +/- 0.02(stat) +/- 0.13(syst) mh, and 0.58 +/- 0.01(stat)(-0.11)(+0.13) (syst) mh, and are used to extract extrapolated total SD and DD cross sections. In addition, the inclusive differential cross section, d sigma/d Delta eta(F), for events with a pseudorapidity gap adjacent to the edge of the detector, is measured over Delta eta F = 8.4 units of pseudorapidity. 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Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. CSFNSM, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Ferretti, R.; Ferro, F.; Lo Vetere, M.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Ferretti, R.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, Rome, Italy. [Iorio, A. O. M.] Univ Naples Federico II, Rome, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, Rome, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Dall'Osso, M.; Dorigo, T.; Galanti, M.; Gasparini, F.; Giubilato, P.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Montecassiano, F.; Passaseo, M.; Pazzini, J.; Pegoraro, M.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Triossi, A.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, I-38050 Trento, Italy. [Bisello, D.; Branca, A.; Dall'Osso, M.; Galanti, M.; Gasparini, F.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Trento, Italy. [Kanishchev, K.] Univ Trent, Trento, Italy. [Gabusi, M.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Grassi, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Ortona, G.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, Novara, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Finco, L.; Migliore, E.; Monaco, V.; Ortona, G.; Pacher, L.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Novara, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Son, D. C.] Kvungpook Natl Univ, Daegu, South Korea. [Kim, T. J.] Chonbuk Natl Univ, Jeonju, South Korea. [Kim, J. Y.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, I. C.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Komaragiri, J. R.; Ali, M. A. B. Md] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Nat Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Wolszczak, W.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz e Silva, C.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Karjavin, V.; Konoplyanikov, V.; Korenkov, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Matveev, V.; Mitsyn, V. V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Smirnov, V.; Tikhonenko, E.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Belyaev, A.; Boos, E.; Ershov, A.; Gribushin, A.; Khein, L.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Lukina, O.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Maestre, J. Alcaraz; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Marrouche, J.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Musella, P.; Orsini, L.; Pape, L.; Perez, E.; Perrozzi, L.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Rolandi, G.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Tsirou, A.; Veres, G. 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Millan; Ngadiuba, J.; Robmann, P.; Ronga, F. J.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.; Chang, P.] Natl Cent Univ, Chungli 32054, Taiwan. [Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W-S; Kao, K. Y.; Lei, Y. J.; Liu, Y. F.; Lu, R-S; Majumder, D.; Petrakou, E.; Tzeng, Y. M.; Wilken, R.] NTU, Taipei, Taiwan. [Asavapibhop, B.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Gamsizkan, H.; Karapinar, G.; Ocalan, K.; Sekmen, S.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Dunne, P.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Hall, G.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A-M; Malik, S.; Mathias, B.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Imperial Coll, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL 35487 USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Lawson, P.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Miceli, T.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Rikova, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Negrete, M. Olmedo; Shrinivas, A.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Evans, D.; Holzner, A.; Kelley, R.; Klein, D.; Lebourgeois, M.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Welke, C.; Wuerthwein, F.; Yagil, A.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Incandela, J.; Justus, C.; Mccoll, N.; Richman, J.; Stuart, D.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Skinnari, L.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY 14853 USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kreis, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Sharma, S.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Yang, F.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carver, M.; Cheng, T.; Curry, D.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Field, R. D.; Fisher, M.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Snowball, M.; Sperka, D.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL 32611 USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL 60607 USA. [Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Haytmyradov, M.; Merlo, J-P; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA 52242 USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.] Johns Hopkins Univ, Baltimore, MD 21218 USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Kenny, R. P., III; Malek, M.; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Skhirtladze, N.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Baden, A.; Belloni, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y-J; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN 55455 USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS 38677 USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.; Zvada, M.] Univ Nebraska, Lincoln, NE 68588 USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; Trocino, D.; Wang, R-J; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL 60208 USA. [Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Pearson, T.; Planer, M.; Ruchti, R.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hebda, P.; Hunt, A.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08542 USA. [Brownson, E.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR 00681 USA. [Barnes, V. E.; Benedetti, D.; Bortoletto, D.; De Mattia, M.; Gutay, L.; Hu, Z.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, IN 46323 USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX 77251 USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Khukhunaishvili, A.; Petrillo, G.; Vishnevskiy, D.] Univ Rochester, Rochester, NY 14627 USA. [Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Kaplan, S.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Salur, S.; Schnetzer, S.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ 08854 USA. [Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN 37996 USA. [Bouhali, O.; Hernandez, A. Castaneda; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Krutelyov, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Rose, A.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.] Texas A&M Univ, College Stn, TX 77843 USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kovitanggoon, K.; Kunori, S.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA 22904 USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI 48202 USA. [Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Dodd, L.; Duric, S.; Friis, E.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Lazaridis, C.; Levine, A.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. H.; Taylor, D.; Verwilligen, P.; Vuosalo, C.; Woods, N.] Univ Wisconsin, Madison, WI 53706 USA. [Fabjan, C.; Fruehwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C-E] Vienna Univ Technol, A-1040 Vienna, Austria. 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RI Hoorani, Hafeez/D-1791-2013; Dogra, Sunil /B-5330-2013; VARDARLI, Fuat Ilkehan/B-6360-2013; Leonidov, Andrey/M-4440-2013; Lokhtin, Igor/D-7004-2012; Ragazzi, Stefano/D-2463-2009; Lo Vetere, Maurizio/J-5049-2012; Manganote, Edmilson/K-8251-2013; Fano, Livio/K-2460-2015; Grandi, Claudio/B-5654-2015; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Andreev, Vladimir/M-8665-2015; Vinogradov, Alexey/O-2375-2015; Petrushanko, Sergey/D-6880-2012; Cakir, Altan/P-1024-2015; Montanari, Alessandro/J-2420-2012; Matorras, Francisco/I-4983-2015; Gennai, Simone/P-2880-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Menasce, Dario/A-2168-2016; Paganoni, Marco/A-4235-2016; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Horani, Hafeez /L-2414-2015; Sguazzoni, Giacomo/J-4620-2015; Ligabue, Franco/F-3432-2014; Benussi, Luigi/O-9684-2014; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Paulini, Manfred/N-7794-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ogul, Hasan/S-7951-2016; ciocci, maria agnese /I-2153-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Seixas, Joao/F-5441-2013; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Calvo Alamillo, Enrique/L-1203-2014; Flix, Josep/G-5414-2012; Hernandez Calama, Jose Maria/H-9127-2015; Cerrada, Marcos/J-6934-2014; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Novaes, Sergio/D-3532-2012; Della Ricca, Giuseppe/B-6826-2013; Chinellato, Jose Augusto/I-7972-2012; Tomei, Thiago/E-7091-2012; Stahl, Achim/E-8846-2011; Kirakosyan, Martin/N-2701-2015 OI Ragazzi, Stefano/0000-0001-8219-2074; Lo Vetere, Maurizio/0000-0002-6520-4480; Fano, Livio/0000-0002-9007-629X; Grandi, Claudio/0000-0001-5998-3070; Rovelli, Tiziano/0000-0002-9746-4842; Montanari, Alessandro/0000-0003-2748-6373; Matorras, Francisco/0000-0003-4295-5668; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Menasce, Dario/0000-0002-9918-1686; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Androsov, Konstantin/0000-0003-2694-6542; Fiorendi, Sara/0000-0003-3273-9419; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Korenkov, Vladimir/0000-0002-2342-7862; Giubilato, Piero/0000-0003-4358-5355; Gallinaro, Michele/0000-0003-1261-2277; Tabarelli de Fatis, Tommaso/0000-0001-6262-4685; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Boccali, Tommaso/0000-0002-9930-9299; Gerosa, Raffaele/0000-0001-8359-3734; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Sguazzoni, Giacomo/0000-0002-0791-3350; Casarsa, Massimo/0000-0002-1353-8964; Ligabue, Franco/0000-0002-1549-7107; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Ghezzi, Alessio/0000-0002-8184-7953; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Ogul, Hasan/0000-0002-5121-2893; ciocci, maria agnese /0000-0003-0002-5462; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Calvo Alamillo, Enrique/0000-0002-1100-2963; Flix, Josep/0000-0003-2688-8047; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Cerrada, Marcos/0000-0003-0112-1691; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; Chinellato, Jose Augusto/0000-0002-3240-6270; Tomei, Thiago/0000-0002-1809-5226; Stahl, Achim/0000-0002-8369-7506; FU Austrian Federal Ministry of Science, Research and Economy; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; CNPq; CAPES; FAPERJ; FAPESP; Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences, Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research; Estonian Research Council [IUT23-4, IUT23-6]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules/CNRS; Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA; Bundesministerium fur Bildung und Forschung; Deutsche Forschungsgemeinschaft; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation; National Innovation Office; Hungary; Department of Atomic Energy and the Department of Science and Technology. India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleate, Italy; Ministry of Science. ICT and Future Planning; National Research Foundation (NRF), Republic of Korea; Lithuanian Academy of Sciences; Ministry' of Education, and University of Malaya (Malaysia); CINVESTAV; CONACYT; SEP; UASLP-FAI; Ministry of Business; Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry' of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; ETH Board; ETH Zurich; PSI; SNF; UniZH; Canton Zurich; SER; Ministry of Science and Technology, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine; State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, UK; US Department of Energy; US National Science Foundation; Marie-Curie program; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education. Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS program of the Foundation for Polish Science; European Union, Regional Development Fund; Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR (Italy) [20108T4XTM]; Thalis and Aristeia programs; EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology; and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via IUT23-4 and IUT23-6 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules/CNRS; and Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA; France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft; and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation; and National Innovation Office; Hungary; the Department of Atomic Energy and the Department of Science and Technology. India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleate, Italy; the Ministry of Science.; ICT and Future Planning, and National Research Foundation (NRF), Republic of Korea; the Lithuanian Academy of Sciences; the Ministry' of Education, and University of Malaya (Malaysia); the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business; Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation; the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry' of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF; UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics; the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine, and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, UK; the US Department of Energy, and the US National Science Foundation. Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium): the Ministry of Education. Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF; and the National Priorities Research Program by Qatar National Research Fund. NR 46 TC 8 Z9 8 U1 7 U2 45 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD JUL 6 PY 2015 VL 92 IS 1 AR 012003 DI 10.1103/PhysRevD.92.012003 PG 32 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CM2EN UT WOS:000357492700001 ER PT J AU Tobin, JG Yu, SW Booth, CH Tyliszczak, T Shuh, DK van der Laan, G Sokaras, D Nordlund, D Weng, TC Bagus, PS AF Tobin, J. G. Yu, S. -W. Booth, C. H. Tyliszczak, T. Shuh, D. K. van der Laan, G. Sokaras, D. Nordlund, D. Weng, T. -C. Bagus, P. S. TI Oxidation and crystal field effects in uranium SO PHYSICAL REVIEW B LA English DT Article ID X-RAY-ABSORPTION; ELECTRONIC-STRUCTURE; PLUTONIUM INTERMETALLICS; EMISSION SPECTROSCOPY; GROUND-STATE; 5F ORBITALS; SPECTRA; DIOXIDE; OXIDES; PHOTOELECTRON AB An extensive investigation of oxidation in uranium has been pursued. This includes the utilization of soft x-ray absorption spectroscopy, hard x-ray absorption near-edge structure, resonant (hard) x-ray emission spectroscopy, cluster calculations, and a branching ratio analysis founded on atomic theory. The samples utilized were uranium dioxide (UO2), uranium trioxide (UO3), and uranium tetrafluoride (UF4). A discussion of the role of nonspherical perturbations, i.e., crystal or ligand field effects, will be presented. C1 [Tobin, J. G.; Yu, S. -W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Booth, C. H.; Tyliszczak, T.; Shuh, D. K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [van der Laan, G.] Diamond Light Source, Magnet Spect Grp, Didcot, Oxon, England. [Sokaras, D.; Nordlund, D.; Weng, T. -C.] Stanford Synchrotron Radiat Lightsource, Stanford, CA 94025 USA. [Bagus, P. S.] Univ N Texas, Dept Chem, Denton, TX 76203 USA. RP Tobin, JG (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM tobin1@llnl.gov RI Bagus, Paul/M-1273-2015; Tobin, James/O-6953-2015; van der Laan, Gerrit/Q-1662-2015; Nordlund, Dennis/A-8902-2008 OI van der Laan, Gerrit/0000-0001-6852-2495; Nordlund, Dennis/0000-0001-9524-6908 FU U. S. Department of Energy, National Nuclear Security Administration [DE-AC52-07NA27344]; Office of Science, Office of Basic Energy Sciences (OBES), Division of Chemical Sciences, Geosciences, and Biosciences (CSGB), Heavy Element Chemistry (HEC) Program of U. S. Department of Energy [DE-AC02-05CH11231]; Office of Science, OBES of U. S. Department of Energy at LBNL [DE-AC02-05CH11231]; Office of Science, OBES, CSGB Condensed Phase and Interfacial Molecular Sciences and HEC programs, U. S. Department of Energy at LBNL [DE-AC02-05CH11231]; Geosciences Research Program, Office of Basic Energy Sciences, U. S. DOE; [DE-FG02-04ER15508] FX Lawrence Livermore National Laboratory is operated by Lawrence Livermore National Security, LLC, for the U. S. Department of Energy, National Nuclear Security Administration under Contract No. DE-AC52-07NA27344. Work at Lawrence Berkeley National Laboratory (C.H.B., D.K.S.) was supported by the Director, Office of Science, Office of Basic Energy Sciences (OBES), Division of Chemical Sciences, Geosciences, and Biosciences (CSGB), Heavy Element Chemistry (HEC) Program of the U. S. Department of Energy under Contract No. DE-AC02-05CH11231. The XANES and RXES data were collected at BL-6-2 and BL-11-2 at SSRL. The ALS and T.T. are supported by the Director, Office of Science, OBES of the U. S. Department of Energy at LBNL under Contract No. DE-AC02-05CH11231. MES Beamline 11.0.2 is supported by the Director, Office of Science, OBES, CSGB Condensed Phase and Interfacial Molecular Sciences and HEC programs, both of the U. S. Department of Energy at LBNL under Contract No. DE-AC02-05CH11231. P.S.B. acknowledges support by the Geosciences Research Program, Office of Basic Energy Sciences, U. S. DOE; the support for P.S.B. is through Grant No. DE-FG02-04ER15508. The Stanford Synchrotron Radiation Lightsource is a national user facility operated by Stanford University on behalf of the DOE, Office of Basic Energy Sciences. The UF4 sample was originally prepared at Oak Ridge National Laboratory and provided to LLNL by J. S. Morrell of Y12 [4]. J.G.T. wishes to thank (1) G. Fox and the PRT Program at LLNL for support during his sabbatical at LBNL; (2) D.K.S. for his hosting of the sabbatical at GTSC/LBNL; and (3) C.H.B. for the opportunity to learn new hard x-ray skills. We thank E. D. Bauer and M. T. Paffett of LANL for making the UO2 sample available to us and we thank W. Lukens for many enlightening discussions about crystal field theory. NR 57 TC 7 Z9 7 U1 7 U2 48 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 6 PY 2015 VL 92 IS 3 AR 035111 DI 10.1103/PhysRevB.92.035111 PG 12 WC Physics, Condensed Matter SC Physics GA CM2CA UT WOS:000357486100005 ER PT J AU Toft-Petersen, R Reehuis, M Jensen, TBS Andersen, NH Li, JY Le, MD Laver, M Niedermayer, C Klemke, B Lefmann, K Vaknin, D AF Toft-Petersen, Rasmus Reehuis, Manfred Jensen, Thomas B. S. Andersen, Niels H. Li, Jiying Le, Manh Duc Laver, Mark Niedermayer, Christof Klemke, Bastian Lefmann, Kim Vaknin, David TI Anomalous magnetic structure and spin dynamics in magnetoelectric LiFePO4 SO PHYSICAL REVIEW B LA English DT Article ID LICOPO4; LINIPO4; FERROELECTRICITY; MULTIFERROICS; DIFFRACTION; SCATTERING; MECHANISM; CAPACITY; CRYSTAL; BATTERY AB We report significant details of the magnetic structure and spin dynamics of LiFePO4 obtained by single-crystal neutron scattering. Our results confirm a previously reported collinear rotation of the spins away from the principal b axis, and they determine that the rotation is toward the a axis. In addition, we find a significant spin-canting component along c. The possible causes of these components are discussed, and their significance for the magnetoelectric effect is analyzed. Inelastic neutron scattering along the three principal directions reveals a highly anisotropic hard plane consistent with earlier susceptibility measurements. Using a spin Hamiltonian, we show that the spin dimensionality is intermediate between XY- and Ising-like, with an easy b axis and a hard c axis. It is shown that both next-nearest neighbor exchange couplings in the bc plane are in competition with the strongest nearest neighbor coupling. C1 [Toft-Petersen, Rasmus; Reehuis, Manfred; Le, Manh Duc; Klemke, Bastian] Helmholtz Zentrum Berlin Mat & Energie, D-14109 Berlin, Germany. [Jensen, Thomas B. S.; Andersen, Niels H.; Laver, Mark] Tech Univ Denmark, Dept Phys, DK-2800 Lyngby, Denmark. [Li, Jiying; Vaknin, David] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Li, Jiying; Vaknin, David] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Le, Manh Duc] Ctr Correlated Electron Syst, Inst Basic Sci, Seoul 151747, South Korea. [Laver, Mark; Niedermayer, Christof] Paul Scherrer Inst, Lab Neutron Scattering & Imaging, CH-5232 Villigen, Switzerland. [Laver, Mark] Univ Birmingham, Dept Met & Mat, Birmingham B15 2TT, W Midlands, England. [Lefmann, Kim] Univ Copenhagen, Niels Bohr Inst, Nanosci Ctr, DK-2100 Copenhagen, Denmark. RP Toft-Petersen, R (reprint author), Helmholtz Zentrum Berlin Mat & Energie, D-14109 Berlin, Germany. EM rasmus.toft-petersen@helmholtz-berlin.de RI Reehuis, Manfred/J-3383-2013; Lefmann, Kim/M-9228-2014; Le, Manh Duc/D-9901-2011; Vaknin, David/B-3302-2009 OI Reehuis, Manfred/0000-0002-6461-4074; Lefmann, Kim/0000-0003-4282-756X; Le, Manh Duc/0000-0003-3012-6053; Vaknin, David/0000-0002-0899-9248 FU Danish Agency for Science, Technology and Innovation under DANSCATT; Swiss NSF [PP002-102831]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-07CH11358] FX Jens Jensen of the University of Copenhagen is greatly acknowledged for illuminating discussions. Work was supported by the Danish Agency for Science, Technology and Innovation under DANSCATT and by the Swiss NSF via Contract No. PP002-102831. Research at Ames Laboratory is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Contract No. DE-AC02-07CH11358. Neutron experiments were performed at the Helmholtz-Zentrum Berlin fur Materialien und Energie, and at the SINQ neutron spallation source at the Paul Scherrer Institute, Switzerland. We thank HZB and PSI for the allocation of neutron radiation beam time. NR 55 TC 6 Z9 6 U1 6 U2 44 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 6 PY 2015 VL 92 IS 2 AR 024404 DI 10.1103/PhysRevB.92.024404 PG 9 WC Physics, Condensed Matter SC Physics GA CM2BR UT WOS:000357485100008 ER PT J AU Zhao, YF Liu, HW Yan, JQ An, W Liu, J Zhang, X Wang, HC Liu, Y Jiang, H Li, Q Wang, Y Li, XZ Mandrus, D Xie, XC Pan, MH Wang, J AF Zhao, Yanfei Liu, Haiwen Yan, Jiaqiang An, Wei Liu, Jun Zhang, Xi Wang, Huichao Liu, Yi Jiang, Hua Li, Qing Wang, Yong Li, Xin-Zheng Mandrus, David Xie, X. C. Pan, Minghu Wang, Jian TI Anisotropic magnetotransport and exotic longitudinal linear magnetoresistance in WTe2 crystals SO PHYSICAL REVIEW B LA English DT Article ID MAGNETIC-FIELD; TRANSITION; LIQUIDS; PHASE AB The WTe2 semimetal, as a typical layered transition-metal dichalcogenide, has recently attracted much attention due to an extremely large, nonsaturating parabolic magnetoresistance in the perpendicular field. Here, we report a systematic study of the angular dependence of the magnetoresistance in a WTe2 single crystal. The significant anisotropic magnetotransport behavior in different magnetic field directions and violation of the Kohler's rule are observed. Unexpectedly, when the applied field and excitation current are both parallel to the tungsten chains of WTe2, an exotic large longitudinal linear magnetoresistance as high as 1200% at 15 T and 2 K is identified. Our results imply that the WTe2 semimetal, due to its balanced hole and electron populations, seems to be the first material for which a large longitudinal linear magnetoresistance appears when the external magnetic field is parallel to the applied current. Our work may stimulate studies of double-carrier correlated materials and the corresponding quantum physics. C1 [Zhao, Yanfei; Liu, Haiwen; Zhang, Xi; Wang, Huichao; Liu, Yi; Xie, X. C.; Wang, Jian] Peking Univ, Sch Phys, Int Ctr Quantum Mat, Beijing 100871, Peoples R China. [Zhao, Yanfei; Liu, Haiwen; An, Wei; Zhang, Xi; Wang, Huichao; Liu, Yi; Li, Xin-Zheng; Xie, X. C.; Wang, Jian] Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China. [Yan, Jiaqiang; Mandrus, David] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Yan, Jiaqiang; Mandrus, David] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [An, Wei; Li, Xin-Zheng] Peking Univ, Sch Phys, Beijing 100871, Peoples R China. [Liu, Jun; Wang, Yong] Zhejiang Univ, Ctr Elect Microscopy, Dept Mat Sci & Engn, State Key Lab Silicon Mat, Hangzhou 310027, Zhejiang, Peoples R China. [Jiang, Hua] Soochow Univ, Coll Phys Optoelect & Energy, Suzhou 215006, Peoples R China. [Li, Qing] Soochow Univ, Inst Funct Nano & Soft Mat FUNSOM, Suzhou 215123, Jiangsu, Peoples R China. [Li, Qing] Soochow Univ, Collaborat Innovat Ctr Suzhou Sci & Technol, Suzhou 215123, Jiangsu, Peoples R China. [Pan, Minghu] Huazhong Univ Sci & Technol, Sch Phys, MOE Key Lab Fundamental Phys Quant Measurements, Wuhan 430074, Peoples R China. RP Pan, MH (reprint author), Huazhong Univ Sci & Technol, Sch Phys, MOE Key Lab Fundamental Phys Quant Measurements, Wuhan 430074, Peoples R China. EM mhupan@gmail.com; jianwangphysics@pku.edu.cn RI Wang, Yong/A-7766-2010; Liu, Haiwen/F-2518-2014; jiang, hua/F-2478-2011 OI Wang, Yong/0000-0002-9893-8296; Liu, Haiwen/0000-0002-0007-3117; jiang, hua/0000-0001-5735-4465 FU National Basic Research Program of China [2013CB934600, 2012CB921300]; National Natural Science Foundation of China [11222434, 11174007]; Research Fund for the Doctoral Program of Higher Education (RFDP) of China; Gordon and Betty Moore Foundation's EPiQS Initiative [GBMF4416]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; Natural Science Foundation of China [11174244]; Zhejiang Provincial Natural Science Foundation of China [LR12A04002] FX We acknowledge Qian Niu, Fa Wang, and Hua Chen for helpful discussions. This work was financially supported by the National Basic Research Program of China (Grants No. 2013CB934600 and No. 2012CB921300), the National Natural Science Foundation of China (No. 11222434 and No. 11174007), and the Research Fund for the Doctoral Program of Higher Education (RFDP) of China. D.G.M. acknowledges support from the Gordon and Betty Moore Foundation's EPiQS Initiative through Grant No. GBMF4416. J.Q.Y. acknowledges support from the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. Y.W. acknowledges support from the Natural Science Foundation of China (11174244) and Zhejiang Provincial Natural Science Foundation of China (LR12A04002). NR 32 TC 26 Z9 26 U1 16 U2 133 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD JUL 6 PY 2015 VL 92 IS 4 AR 041104 DI 10.1103/PhysRevB.92.041104 PG 7 WC Physics, Condensed Matter SC Physics GA CM2CJ UT WOS:000357487000003 ER PT J AU Zhuang, HLL Xie, Y Kent, PRC Ganesh, P AF Zhuang, Houlong L. Xie, Yu Kent, P. R. C. Ganesh, P. TI Computational discovery of ferromagnetic semiconducting single-layer CrSnTe3 SO PHYSICAL REVIEW B LA English DT Article ID AUGMENTED-WAVE METHOD; ENERGY; CR2SI2TE6; COMPOUND AB Despite many single-layer materials being reported in the past decade, few of them exhibit magnetism. Here we perform first-principles calculations using accurate hybrid density functional methods (HSE06) to predict that single-layer CrSnTe3 (CST) is a ferromagnetic semiconductor, with band gaps of 0.9 and 1.2 eV for the majority and minority spin channels, respectively. We determine the Curie temperature as 170 K, significantly higher than that of single-layer CrSiTe3 (90 K) and CrGeTe3 (130 K). This is due to the enhanced ionicity of the Sn-Te bond, which in turn increases the superexchange coupling between the magnetic Cr atoms. We further explore the mechanical and dynamical stability and strain response of this single-layer material for possible epitaxial growth. Our study provides an intuitive approach to understand and design single-layer magnetic semiconductors for a wide range of spintronics and energy applications. C1 [Zhuang, Houlong L.; Xie, Yu; Kent, P. R. C.; Ganesh, P.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Kent, P. R. C.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. RP Zhuang, HLL (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM zhuanghl@ornl.gov RI Ganesh, Panchapakesan/E-3435-2012; Kent, Paul/A-6756-2008; Zhuang, Houlong/D-8801-2014 OI Ganesh, Panchapakesan/0000-0002-7170-2902; Kent, Paul/0000-0001-5539-4017; Zhuang, Houlong/0000-0002-3845-4601 FU Texas Advanced Computing Center [TG-DMR140067] FX This research was conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. A part of this research used computational resources of the Texas Advanced Computing Center under Contract No. TG-DMR140067. A part of this material is based upon work performed using computational resources supported by the University of Tennessee and Oak Ridge National Laboratory's Joint Institute for Computational Sciences (http://www.jics.utk.edu). We thank Kai Xiao and Richard Hennig for helpful discussions. NR 36 TC 12 Z9 12 U1 18 U2 66 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 6 PY 2015 VL 92 IS 3 AR 035407 DI 10.1103/PhysRevB.92.035407 PG 6 WC Physics, Condensed Matter SC Physics GA CM2CA UT WOS:000357486100011 ER PT J AU Plagemann, KU Ruter, HR Bornath, T Shihab, M Desjarlais, MP Fortmann, C Glenzer, SH Redmer, R AF Plagemann, Kai-Uwe Rueter, Hannes R. Bornath, Thomas Shihab, Mohammed Desjarlais, Michael P. Fortmann, Carsten Glenzer, Siegfried H. Redmer, Ronald TI Ab initio calculation of the ion feature in x-ray Thomson scattering SO PHYSICAL REVIEW E LA English DT Article ID AUGMENTED-WAVE METHOD; WARM DENSE MATTER; MOLECULAR-DYNAMICS; LIQUID-METALS; PLASMAS; APPROXIMATION AB The spectrum of x-ray Thomson scattering is proportional to the dynamic structure factor. An important contribution is the ion feature which describes elastic scattering of x rays off electrons. We apply an ab initio method for the calculation of the form factor of bound electrons, the slope of the screening cloud of free electrons, and the ion-ion structure factor in warm dense beryllium. With the presented method we can calculate the ion feature from first principles. These results will facilitate a better understanding of x-ray scattering in warm dense matter and an accurate measurement of ion temperatures which would allow determining nonequilibrium conditions, e.g., along shock propagation. C1 [Plagemann, Kai-Uwe; Rueter, Hannes R.; Bornath, Thomas; Shihab, Mohammed; Redmer, Ronald] Univ Rostock, Inst Phys, D-18051 Rostock, Germany. [Shihab, Mohammed] Tanta Univ, Fac Sci, Dept Phys, Tanta 31527, Egypt. [Desjarlais, Michael P.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Fortmann, Carsten] Quantumwise AS, DK-2100 Copenhagen, Denmark. [Glenzer, Siegfried H.] SLAC Natl Accelerator Lab, High Energy Dens Sci, Menlo Pk, CA 94025 USA. RP Plagemann, KU (reprint author), Univ Rostock, Inst Phys, D-18051 Rostock, Germany. EM kai-uwe.plagemann@uni-rostock.de FU U.S. Department of Energy, Office of Science, Fusion Energy Science [FWP 100182]; DFG [SFB 652]; BMBF [FSP 302] FX We thank the operators of the supercomputing center HLRN and the computing center of the University of Rostock for assistance. We thank W.-D. Kraeft and P. Neumayer for helpful discussions. S.G. acknowledges support by U.S. Department of Energy, Office of Science, Fusion Energy Science under contract FWP 100182. This study was supported by the DFG within the SFB 652 and by the BMBF within the FSP 302. NR 39 TC 10 Z9 10 U1 4 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD JUL 6 PY 2015 VL 92 IS 1 AR 013103 DI 10.1103/PhysRevE.92.013103 PG 8 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA CM2GL UT WOS:000357497800029 PM 26274290 ER PT J AU Jha, PK Ni, XJ Wu, CH Wang, Y Zhang, X AF Jha, Pankaj K. Ni, Xingjie Wu, Chihhui Wang, Yuan Zhang, Xiang TI Metasurface-Enabled Remote Quantum Interference SO PHYSICAL REVIEW LETTERS LA English DT Article ID PLASMONIC METASURFACES; META-SURFACES; LIGHT; REFLECTION; OPTICS; ATOM AB An anisotropic quantum vacuum (AQV) opens novel pathways for controlling light-matter interaction in quantum optics, condensed matter physics, etc. Here, we theoretically demonstrate a strong AQV over macroscopic distances enabled by a judiciously designed array of subwavelength-scale nanoantennas-a metasurface. We harness the phase-control ability and the polarization-dependent response of the metasurface to achieve strong anisotropy in the decay rate of a quantum emitter located over distances of hundreds of wavelengths. Such an AQV induces quantum interference among radiative decay channels in an atom with orthogonal transitions. Quantum vacuum engineering with metasurfaces holds promise for exploring new paradigms of long-range light-matter interaction for atom optics, solid-state quantum optics, quantum information processing, etc. C1 [Jha, Pankaj K.; Ni, Xingjie; Wu, Chihhui; Wang, Yuan; Zhang, Xiang] Univ Calif Berkeley, NSF Nanoscale Sci & Engn Ctr NSEC, Berkeley, CA 94720 USA. [Zhang, Xiang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Zhang, X (reprint author), Univ Calif Berkeley, NSF Nanoscale Sci & Engn Ctr NSEC, 3112 Etcheverry Hall, Berkeley, CA 94720 USA. EM xiang@berkeley.edu RI Ni, Xingjie/I-2235-2012; Wang, Yuan/F-7211-2011; Zhang, Xiang/F-6905-2011 OI Ni, Xingjie/0000-0001-7405-5678; FU Multidisciplinary University Research Initiative from the Air Force Office of Scientific Research (AFOSR MURI Award) [FA9550-12-1-0488] FX The authors acknowledge funding support from the Multidisciplinary University Research Initiative from the Air Force Office of Scientific Research (AFOSR MURI Award No. FA9550-12-1-0488). P. K. J. conceived the idea, performed the atomic analytical and numerical calculations. X. N. designed the metasurface, conducted numerical simulations and decay rate calculations. X. Z. and Y. W. guided the research. All authors contributed to discussions and wrote the Letter. NR 46 TC 16 Z9 16 U1 10 U2 55 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 6 PY 2015 VL 115 IS 2 AR 025501 DI 10.1103/PhysRevLett.115.025501 PG 5 WC Physics, Multidisciplinary SC Physics GA CM2HL UT WOS:000357500500005 PM 26207477 ER PT J AU Lee, J Jeon, H Oh, DG Szanyi, J Kwak, JH AF Lee, Jaekyoung Jeon, Himchan Oh, Dong Gun Szanyi, Janos Kwak, Ja Hun TI Morphology-dependent phase transformation of gamma-Al2O3 SO APPLIED CATALYSIS A-GENERAL LA English DT Article DE gamma-Al2O3; Phase transformation; Morphology; TEM; Ethanol-TPD ID ALUMINA THIN-FILMS; GAMMA-ALUMINA; SURFACE-AREA; HYDROTHERMAL SYNTHESIS; TRANSITIONAL ALUMINAS; ETHANOL DEHYDRATION; THERMAL EVOLUTION; PARTICLE-SIZE; BOEHMITE; NANOPARTICLES AB The phase transformations of platelet- and rod-shaped gamma-Al2O3 were investigated and compared to that of a commercial sample by XRD, BET surface area measurements, transmission electron microscopy (TEM), solid state Al-27-NMR, and ethanol temperature programmed desorption (TPD) after sequential annealing in air up to 1100 degrees C. After annealing at 1100 degrees C, commercial gamma-Al2O3 mostly transformed into alpha-Al2O3 with drastic surface area reduction (from 200 m(2)/g to 25 m(2)/g). Interestingly, platelet- and rod-shaped gamma-Al2O3 which showed exactly the same XRD patterns transformed into different phases upon the high temperature calcinations. Platelet-shaped gamma-Al2O3 transformed into theta-phase while the rod-shaped gamma-Al2O3 transformed into the delta-phase and not to the alpha-polymorph. Both platelet- and rod-shaped aluminas retained significantly higher surface area (similar to 60 m(2)/g) than the commercial one after the same treatment at 1100 degrees C. These results suggest that the phase transformation in gamma-Al2O3 is strongly affected by not only the crystal structure of the starting material, but its morphology as well. Ethanol TPD from platelet- and rod-shaped alumina after 1100 degrees C annealing, showed significantly different desorption profiles which suggest different surface characteristics even though they had almost the same surface areas. These different phase transformations were also supported by solid state Al-27-NMR. After 1100 degrees C annealing commercial alumina showed the presence of mostly octahedral Al3+ ions, but the other two samples displayed even higher number of tetrahedral Al3+ ions than the initial gamma-Al2O3. Morphological changes were also confirmed by TEM. All these results consistently suggest the morphology-dependent phase transformations of gamma-Al2O3 and the improved thermal stability of platelet- and rod-shaped gamma-Al2O3 in comparison to a commercial gamma-Al2O3. (C) 2015 Elsevier B.V. All rights reserved. C1 [Lee, Jaekyoung; Jeon, Himchan; Oh, Dong Gun; Kwak, Ja Hun] UNIST, Sch Energy & Chem Engn, Dept Chem Engn, Ulsan 689798, South Korea. [Szanyi, Janos] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. RP Kwak, JH (reprint author), UNIST, Sch Energy & Chem Engn, Dept Chem Engn, 100 Banyeon Ri, Ulsan 689798, South Korea. EM jhkwak@unist.ac.kr FU Basic Science Research Program through the National Research Foundation of Korea (NRF) - Ministry of Education, Science and Technology [2013R1A1A2009307]; U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES), Division of Chemical Sciences, Geosciences Biosciences FX This research was supported by Basic Science Research Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Education, Science and Technology (Grant number 2013R1A1A2009307). J. Sz. acknowledges the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES), Division of Chemical Sciences, Geosciences & Biosciences for the support of this work. NR 43 TC 9 Z9 9 U1 6 U2 59 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0926-860X EI 1873-3875 J9 APPL CATAL A-GEN JI Appl. Catal. A-Gen. PD JUL 5 PY 2015 VL 500 BP 58 EP 68 DI 10.1016/j.apcata.2015.03.040 PG 11 WC Chemistry, Physical; Environmental Sciences SC Chemistry; Environmental Sciences & Ecology GA CL7GY UT WOS:000357141700008 ER PT J AU Tian, HJ Fisher, JC AF Tian, Hanjing Fisher, James C., II TI Isotopic steam investigations of hematite (Fe2O3) for chemical looping combustion of methane SO CATALYSIS COMMUNICATIONS LA English DT Article DE Isotopic mechanistic study; Methane combustion/reforming; Steam effect ID OXYGEN CARRIERS; NICKEL; IRON AB The effect of steam on the chemical looping combustion of methane over hematite (Fe2O3) is studied by the isotopic exchange method coupled with mass spectroscopy. Traditional steam was replaced with deuterium-oxide providing interesting mechanistic information not previously reported. The rapid kinetics of steam reforming were established before complete combustion reaction, and adsorption of deuterium into the iron structure was observed. Additionally, the presence of deuterium-oxide drastically reduced the combustion conversion of methane to carbon dioxide. (C) 2015 Elsevier B.V. All rights reserved. C1 [Tian, Hanjing; Fisher, James C., II] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. [Tian, Hanjing] W Virginia Univ, Dept Chem Engn, Morgantown, WV 26506 USA. RP Tian, HJ (reprint author), POB 6102,Engn Sci Bldg Rm 435, Morgantown, WV 26506 USA. EM htian@mail.wvu.edu FU National Energy Technology Laboratory under RES [DE-FE0004000] FX This technical effort was performed in support of the National Energy Technology Laboratory's ongoing research under the RES contract DE-FE0004000. NR 8 TC 1 Z9 2 U1 7 U2 42 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1566-7367 EI 1873-3905 J9 CATAL COMMUN JI Catal. Commun. PD JUL 5 PY 2015 VL 67 BP 83 EP 86 DI 10.1016/j.catcom.2015.04.015 PG 4 WC Chemistry, Physical SC Chemistry GA CI9AJ UT WOS:000355062500018 ER PT J AU Scullin, C Cruz, AG Chuang, YD Simmons, BA Loque, D Singh, S AF Scullin, Chessa Cruz, Alejandro G. Chuang, Yi-De Simmons, Blake A. Loque, Dominique Singh, Seema TI Restricting lignin and enhancing sugar deposition in secondary cell walls enhances monomeric sugar release after low temperature ionic liquid pretreatment SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Arabidopsis; Biofuels; Cell wall; Lignin; Saccharification; Ionic liquid ID CORN STOVER; BIOSYNTHESIS PERTURBATIONS; LIGNOCELLULOSIC BIOMASS; TRANSCRIPTION FACTORS; ARABIDOPSIS-THALIANA; ENZYMATIC-HYDROLYSIS; SACCHARIFICATION; CELLULOSE; DIGESTIBILITY; RECALCITRANCE AB Background: Lignocellulosic biomass has the potential to be a major source of renewable sugar for biofuel production. Before enzymatic hydrolysis, biomass must first undergo a pretreatment step in order to be more susceptible to saccharification and generate high yields of fermentable sugars. Lignin, a complex, interlinked, phenolic polymer, associates with secondary cell wall polysaccharides, rendering them less accessible to enzymatic hydrolysis. Herein, we describe the analysis of engineered Arabidopsis lines where lignin biosynthesis was repressed in fiber tissues but retained in the vessels, and polysaccharide deposition was enhanced in fiber cells with little to no apparent negative impact on growth phenotype. Results: Engineered Arabidopsis plants were treated with the ionic liquid (IL) 1-ethyl-3-methylimidazolium acetate 1-ethyl-3-methylimidazolium acetate ([C(2)C(1)im][OAc]) at 10 % wt biomass loading at either 70 degrees C for 5 h or 140 degrees C for 3 h. After pretreatment at 140 degrees C and subsequent saccharification, the relative peak sugar recovery of similar to 26.7 g sugar per 100 g biomass was not statistically different for the wild type than the peak recovery of similar to 25.8 g sugar per 100 g biomass for the engineered plants (84 versus 86 % glucose from the starting biomass). Reducing the pretreatment temperature to 70 degrees C for 5 h resulted in a significant reduction in the peak sugar recovery obtained from the wild type to 16.2 g sugar per 100 g biomass, whereas the engineered lines with reduced lignin content exhibit a higher peak sugar recovery of 27.3 g sugar per 100 g biomass and 79 % glucose recoveries. Conclusions: The engineered Arabidopsis lines generate high sugar yields after pretreatment at 70 degrees C for 5 h and subsequent saccharification, while the wild type exhibits a reduced sugar yield relative to those obtained after pretreatment at 140 degrees C. Our results demonstrate that employing cell wall engineering efforts to decrease the recalcitrance of lignocellulosic biomass has the potential to drastically reduce the energy required for effective pretreatment. C1 [Scullin, Chessa; Cruz, Alejandro G.; Simmons, Blake A.; Singh, Seema] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, Deconstruct Div, Berkeley, CA 94720 USA. [Scullin, Chessa; Simmons, Blake A.; Singh, Seema] Sandia Natl Labs, Biol & Mat Sci Ctr, Livermore, CA USA. [Cruz, Alejandro G.; Chuang, Yi-De] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Loque, Dominique] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Feedstocks Div, Joint BioEnergy Inst, Berkeley, CA 94720 USA. [Loque, Dominique] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Singh, Seema] Joint BioEnergy Inst, Emeryville, CA 94608 USA. RP Singh, S (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, Deconstruct Div, Berkeley, CA 94720 USA. EM seesing@sandia.gov RI Loque, Dominique/A-8153-2008 FU Office of Science, Office of Biological and Environmental Research, of the US Department of Energy [DE-AC02-05CH11231] FX This work, conducted by the Joint BioEnergy Institute, was supported by the Office of Science, Office of Biological and Environmental Research, of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 37 TC 2 Z9 2 U1 3 U2 94 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD JUL 4 PY 2015 VL 8 AR 95 DI 10.1186/s13068-015-0275-2 PG 12 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA CM4IP UT WOS:000357648400001 PM 26161139 ER PT J AU Price, T Roloff, P Strube, J Tanabe, T AF Price, T. Roloff, P. Strube, J. Tanabe, T. TI Full simulation study of the top Yukawa coupling at the ILC at TeV SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID HADRON-COLLISIONS; E&E ANNIHILATION; E+E ANNIHILATION; HEAVY QUARKS; O(ALPHA(2)(S)); ALGORITHM; BOSON; JETS; LHC AB We present a study of the expected precision for the measurement of the top Yukawa coupling, , in collisions at a center-of-mass energy of 1 TeV. Independent analyses of final states containing at least six hadronic jets are performed, based on detailed simulations of SiD and ILD, the two candidate detector concepts for the ILC. We estimate that a statistical precision on of 4.5 % can be obtained with an integrated luminosity of 1 that is split equally between two configurations for the beam polarization , and . This estimate improves to if the 1 sample is assumed to be fully in the configuration. C1 [Price, T.] Univ Birmingham, Birmingham, W Midlands, England. [Roloff, P.] CERN, CH-1211 Geneva 23, Switzerland. [Strube, J.] Tohoku Univ, Aoba Ku, Sendai, Miyagi 9808578, Japan. [Tanabe, T.] Univ Tokyo, ICEPP, Bunkyo Ku, Tokyo 1130033, Japan. [Strube, J.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Price, T (reprint author), Univ Birmingham, Birmingham, W Midlands, England. EM t.price@bham.ac.uk; philipp.roloff@cern.ch; jan.strube@pnnl.gov; tomohiko@icepp.s.u-tokyo.ac.jp FU JSPS KAKENHI [23000002] FX The authors would like to thank their colleagues in the Linear Collider community for their help in facilitating this work; in particular, T. Barklow, M. Berggren, and A. Miyamoto for generating the Monte-Carlo samples; J. Engels, C. Grefe, and S. Poss for the production on the Grid. The authors also thank K. Fujii, N. Watson, and V. Martin for the helpful discussions and suggestions. This work was partially supported by JSPS KAKENHI Grant Number 23000002. NR 41 TC 1 Z9 1 U1 0 U2 1 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JUL 4 PY 2015 VL 75 IS 7 AR 309 DI 10.1140/epjc/s10052-015-3532-4 PG 9 WC Physics, Particles & Fields SC Physics GA CM1ZI UT WOS:000357478800001 ER PT J AU Wilbanks, TJ Fernandez, SJ Allen, MR AF Wilbanks, Thomas J. Fernandez, Steven J. Allen, Melissa R. TI Extreme Weather Events and Interconnected Infrastructures: TOWARD MORE COMPREHENSIVE CLIMATE CHANGE PLANNING SO ENVIRONMENT LA English DT Article C1 [Wilbanks, Thomas J.; Allen, Melissa R.] Oak Ridge Natl Lab, Oak Ridge, TN 37830 USA. [Fernandez, Steven J.; Allen, Melissa R.] Univ Tennessee, Knoxville, TN 37996 USA. [Fernandez, Steven J.] Los Alamos Natl Lab, Natl Infrastruct Simulat & Anal Ctr Efforts Elect, Los Alamos, NM 87545 USA. [Fernandez, Steven J.] Idaho Natl Lab, Idaho Falls, ID 83401 USA. RP Wilbanks, TJ (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37830 USA. NR 20 TC 1 Z9 1 U1 1 U2 12 PU ROUTLEDGE JOURNALS, TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXFORDSHIRE, ENGLAND SN 0013-9157 EI 1939-9154 J9 ENVIRONMENT JI Environment PD JUL 4 PY 2015 VL 57 IS 4 BP 4 EP 15 DI 10.1080/00139157.2015.1048134 PG 12 WC Environmental Sciences; Environmental Studies SC Environmental Sciences & Ecology GA CL1HZ UT WOS:000356694700002 ER PT J AU Bansal, P Cremaschi, L AF Bansal, Pradeep Cremaschi, Lorenzo TI Advances in refrigeration and heat transfer engineering SO SCIENCE AND TECHNOLOGY FOR THE BUILT ENVIRONMENT LA English DT Editorial Material C1 [Bansal, Pradeep] Oak Ridge Natl Lab, R&D Staff, Oak Ridge, TN 37831 USA. [Cremaschi, Lorenzo] Oklahoma State Univ, Mech & Aerosp Engn, Stillwater, OK 74078 USA. RP Bansal, P (reprint author), Oak Ridge Natl Lab, R&D Staff, Oak Ridge, TN 37831 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 2374-4731 EI 2374-474X J9 SCI TECHNOL BUILT EN JI Sci. Technol. Built Environ. PD JUL 4 PY 2015 VL 21 IS 5 SI SI BP 481 EP 482 DI 10.1080/23744731.2015.1048623 PG 2 WC Thermodynamics; Construction & Building Technology; Engineering, Mechanical SC Thermodynamics; Construction & Building Technology; Engineering GA CP1TP UT WOS:000359659300001 ER PT J AU Bansal, P Shen, B AF Bansal, Pradeep Shen, Bo TI Analysis of environmentally friendly refrigerant options for window air conditioners SO SCIENCE AND TECHNOLOGY FOR THE BUILT ENVIRONMENT LA English DT Article ID HORIZONTAL TUBES; CONDENSATION AB This article presents a technical assessment of environmentally friendly refrigerants as alternatives to R410A for window air conditioners. The alternative refrigerants that are studied for its replacement include R32, a mixture of R32/R125 with 90%/10% molar concentration, R600a, R290, R1234yf, R1234ze, and R134a. Baseline experiments were performed on a window unit charged with R410A. The heat pump design model was modified and calibrated with the baseline data and was used to evaluate the comparative performance of the window air conditioner with alternative refrigerants. The article discusses the advantages and disadvantages of each refrigerant and their suitability for window air conditioners. Among all of the refrigerants studied, R32 offers the best efficiency improvement over R410A and has a 67.5% lower global warming potential. C1 [Bansal, Pradeep; Shen, Bo] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. RP Bansal, P (reprint author), Oak Ridge Natl Lab, Energy & Transportat Sci Div, One Bethel Valley Rd,POB 2008,MS6070, Oak Ridge, TN 37831 USA. EM bansalpk@ornl.gov FU Building Technologies Office of the US Department of Energy [DE-AC05-00OR22725]; UT-Battelle FX The authors gratefully acknowledge the support of the Building Technologies Office of the US Department of Energy under contract DE-AC05-00OR22725 with UT-Battelle for their financial support and industry partner for their in-kind and technical support. NR 11 TC 1 Z9 1 U1 0 U2 0 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 2374-4731 EI 2374-474X J9 SCI TECHNOL BUILT EN JI Sci. Technol. Built Environ. PD JUL 4 PY 2015 VL 21 IS 5 SI SI BP 483 EP 490 DI 10.1080/23744731.2015.1016364 PG 8 WC Thermodynamics; Construction & Building Technology; Engineering, Mechanical SC Thermodynamics; Construction & Building Technology; Engineering GA CP1TP UT WOS:000359659300002 ER PT J AU Komatsu, K Munakata, K Matsubayashi, K Uwatoko, Y Yokoyama, Y Sugiyama, K Matsuda, M AF Komatsu, Kazuki Munakata, Koji Matsubayashi, Kazuyuki Uwatoko, Yoshiya Yokoyama, Yoshihiko Sugiyama, Kazumasa Matsuda, Masaaki TI Zr-based bulk metallic glass as a cylinder material for high pressure apparatuses SO HIGH PRESSURE RESEARCH LA English DT Article DE bulk metallic glass; piston-cylinder; neutron scattering; magnetic property measurement ID CRYSTAL NEUTRON-DIFFRACTION; 10 GPA; CELL; TEMPERATURE AB Zirconium-based bulk metallic glass (Zr-based BMG) has outstanding properties as a cylinder material for piston-cylinder high pressure apparatuses and is especially useful for neutron scattering. The piston-cylinder consisting of a Zr-based BMG cylinder with outer/inner diameters of 8.8/2.5mm sustains pressures up to 1.81GPa and ruptured at 2.0GPa, with pressure values determined by the superconducting temperature of lead. The neutron attenuation of Zr-based BMG is similar to that of TiZr null-scattering alloy and more transparent than that of CuBe alloy. No contamination of sharp Bragg reflections is observed in the neutron diffraction pattern for Zr-based BMG. The magnetic susceptibility of Zr-based BMG is similar to that of CuBe alloy; this leads to a potential application for measurements of magnetic properties under pressure. C1 [Komatsu, Kazuki] Univ Tokyo, Grad Sch Sci, Geochem Res Ctr, Tokyo 113, Japan. [Munakata, Koji] Comprehens Res Org Sci & Soc, Tokai, Ibaraki, Japan. [Matsubayashi, Kazuyuki; Uwatoko, Yoshiya] Univ Tokyo, Inst Solid State Phys, Kashiwa, Chiba, Japan. [Yokoyama, Yoshihiko; Sugiyama, Kazumasa] Tohoku Univ, Inst Mat Res, Aoba Ku, Sendai, Miyagi 980, Japan. [Matsuda, Masaaki] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN USA. RP Komatsu, K (reprint author), Univ Tokyo, Grad Sch Sci, Geochem Res Ctr, Tokyo 113, Japan. EM kom@eqchem.s.u-tokyo.ac.jp RI Matsuda, Masaaki/A-6902-2016; Komatsu, Kazuki/B-8165-2013; Matsubayashi, Kazuyuki/F-7696-2013; Sugiyama, Kazumasa/B-3447-2010 OI Matsuda, Masaaki/0000-0003-2209-9526; Komatsu, Kazuki/0000-0003-3573-9174; FU JSPS KAKENHI [19GS0205, 20103001-4, 25870182, 26246039]; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; US-Japan Cooperative Program on Neutron Scattering FX This study was supported by JSPS KAKENHI [grant number 19GS0205], [grant number 20103001-4], [grant number 25870182], [grant number 26246039]. Research conducted at ORNL's High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. This study was supported in part by the US-Japan Cooperative Program on Neutron Scattering. NR 15 TC 2 Z9 2 U1 2 U2 20 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 0895-7959 EI 1477-2299 J9 HIGH PRESSURE RES JI High Pressure Res. PD JUL 3 PY 2015 VL 35 IS 3 BP 254 EP 262 DI 10.1080/08957959.2015.1041939 PG 9 WC Physics, Multidisciplinary SC Physics GA CP3ZV UT WOS:000359822700005 ER PT J AU Vohra, YK Samudrala, GK Moore, SL Montgomery, JM Tsoi, GM Velisavljevic, N AF Vohra, Yogesh K. Samudrala, Gopi K. Moore, Samuel L. Montgomery, Jeffrey M. Tsoi, Georgiy M. Velisavljevic, Nenad TI High pressure studies using two-stage diamond micro-anvils grown by chemical vapor deposition SO HIGH PRESSURE RESEARCH LA English DT Article DE high pressure techniques; diamond growth; micro X-ray diffraction; rare-earth metals ID GPA AB Ultra-high static pressures have been achieved in the laboratory using a two-stage micro-ball nanodiamond anvils as well as a two-stage micro-paired diamond anvils machined using a focused ion-beam system. The two-stage diamond anvils' designs implemented thus far suffer from a limitation of one diamond anvil sliding past another anvil at extreme conditions. We describe a new method of fabricating two-stage diamond micro-anvils using a tungsten mask on a standard diamond anvil followed by microwave plasma chemical vapor deposition (CVD) homoepitaxial diamond growth. A prototype two-stage diamond anvil with 300 mu m culet and with a CVD diamond second stage of 50 mu m in diameter was fabricated. We have carried out preliminary high pressure X-ray diffraction studies on a sample of rare-earth metal lutetium sample with a copper pressure standard to 86GPa. The micro-anvil grown by CVD remained intact during indentation of gasket as well as on decompression from the highest pressure of 86GPa. C1 [Vohra, Yogesh K.; Samudrala, Gopi K.; Moore, Samuel L.; Montgomery, Jeffrey M.; Tsoi, Georgiy M.] Univ Alabama Birmingham, Dept Phys, Birmingham, AL 35294 USA. [Velisavljevic, Nenad] Los Alamos Natl Lab, Los Alamos, NM 87544 USA. RP Vohra, YK (reprint author), Univ Alabama Birmingham, Dept Phys, Birmingham, AL 35294 USA. EM ykvohra@uab.edu FU Department of Energy-National Nuclear Security Administration [DE-NA0002014]; DOE-NNSA [DE-AC52-06NA25396, DE-NA0001974]; LANL Science Campaigns 2; DOE-BES [DE-FG02-99ER45775, DE-AC02-06CH11357]; NSF; US DOE [DE-AC02-06CH11357] FX This material is based upon work supported by the Department of Energy-National Nuclear Security Administration under Award Number DE-NA0002014. Los Alamos National Laboratory (LANL) is operated by LANS, LLC for the DOE-NNSA under contract no. DE-AC52-06NA25396. NV acknowledges funding support from LANL Science Campaigns 2. Portions of this work were performed at HPCAT (Sector 16), Advanced Photon Source (APS), Argonne National Laboratory. HPCAT operations are supported by DOE-NNSA under Award No. DE-NA0001974 and DOE-BES under Award No. DE-FG02-99ER45775, with partial instrumentation funding by NSF. APS is supported by DOE-BES, under Contract No. DE-AC02-06CH11357. Use of the APS, an Office of Science User Facility operated for the US Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the US DOE under Contract No. DE-AC02-06CH11357. NR 8 TC 3 Z9 3 U1 4 U2 16 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 0895-7959 EI 1477-2299 J9 HIGH PRESSURE RES JI High Pressure Res. PD JUL 3 PY 2015 VL 35 IS 3 BP 282 EP 288 DI 10.1080/08957959.2015.1053881 PG 7 WC Physics, Multidisciplinary SC Physics GA CP3ZV UT WOS:000359822700008 ER PT J AU Hanson, DE Barber, JL AF Hanson, David E. Barber, John L. TI A new paradigm for the molecular basis of rubber elasticity SO CONTEMPORARY PHYSICS LA English DT Article DE natural rubber; elasticity theory; networks; polymer modeling ID POLYMER NETWORKS; NATURAL-RUBBER; STATISTICAL-MECHANICS; INTERNAL-ROTATION; STRESSED RUBBER; RETRACTION; DYNAMICS; DEFORMATION; TEMPERATURE; STRENGTH AB The molecular basis for rubber elasticity is arguably the oldest and one of the most important questions in the field of polymer physics. The theoretical investigation of rubber elasticity began in earnest almost a century ago with the development of analytic thermodynamic models, based on simple, highly-symmetric configurations of so-called Gaussian chains, i.e. polymer chains that obey Markov statistics. Numerous theories have been proposed over the past 90years based on the ansatz that the elastic force for individual network chains arises from the entropy change associated with the distribution of end-to-end distances of a free polymer chain. There are serious conceptual objections to this assumption and others, such as the assumption that all network nodes undergo a simple volume-preserving linear motion and that all of the network chains have the same length. Recently, a new paradigm for elasticity in rubber networks has been proposed that is based on mechanisms that originate at the molecular level. Using conventional statistical mechanics analyses, Quantum Chemistry, and Molecular Dynamics simulations, the fundamental entropic and enthalpic chain extension forces for polyisoprene (natural rubber) have been determined, along with estimates for the basic force constants. Concurrently, the complex morphology of natural rubber networks (the joint probability density distributions that relate the chain end-to-end distance to its contour length) has also been captured in a numerical model (EPnet). When molecular chain forces are merged with the network structure in this model, it is possible to study the mechanical response to tensile and compressive strains of a representative volume element of a polymer network. As strain is imposed on a network, pathways of connected taut chains, that completely span the network along strain axis, emerge. Although these chains represent only a few percent of the total, they account for nearly all of the elastic stress at high strain. Here we provide a brief review of previous elasticity theories and their deficiencies, and present a new paradigm with an emphasis on experimental comparisons. C1 [Hanson, David E.; Barber, John L.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87544 USA. RP Hanson, DE (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87544 USA. EM deh@lanl.gov FU Laboratory Directed Research and Development, under the Los Alamos National Laboratory [20060226ER]; National Nuclear Security Administration of the US Department of Energy [DE-AC52-06NA25396]; US DOE-DOD Joint Munitions Program FX Some of this work was supported by Laboratory Directed Research and Development [grant number 20060226ER], under the auspices of Los Alamos National Laboratory, which is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the US Department of Energy under contract [DE-AC52-06NA25396]. We wish to gratefully acknowledge the support of the US DOE-DOD Joint Munitions Program. NR 59 TC 1 Z9 1 U1 2 U2 28 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 0010-7514 EI 1366-5812 J9 CONTEMP PHYS JI Contemp. Phys. PD JUL 3 PY 2015 VL 56 IS 3 BP 319 EP 337 DI 10.1080/00107514.2015.1006810 PG 19 WC Physics, Multidisciplinary SC Physics GA CP2IF UT WOS:000359700000004 ER PT J AU Osborn, DL Taatjes, CA AF Osborn, David L. Taatjes, Craig A. TI The physical chemistry of Criegee intermediates in the gas phase SO INTERNATIONAL REVIEWS IN PHYSICAL CHEMISTRY LA English DT Review DE Criegee intermediate; carbonyl oxide; ozonolysis ID CONFORMER-DEPENDENT REACTIVITY; SUBSTITUTED CARBONYL OXIDES; DIRECT KINETIC MEASUREMENTS; INFRARED MATRIX-ISOLATION; OH RADICAL PRODUCTS; WATER-VAPOR; SULFUR-DIOXIDE; FORMIC-ACID; ATMOSPHERIC CHEMISTRY; ABSORPTION-SPECTRUM AB Carbonyl oxides, also known as Criegee intermediates, are key intermediates in both gas phase ozonolysis of unsaturated hydrocarbons in the troposphere and solution phase organic synthesis via ozonolysis. Although the study of Criegee intermediates in both arenas has a long history, direct studies in the gas phase have only recently become possible through new methods of generating stabilised Criegee intermediates in sufficient quantities. This advance has catalysed a large number of new experimental and theoretical investigations of Criegee intermediate chemistry. In this article we review the physical chemistry of Criegee intermediates, focusing on their molecular structure, spectroscopy, unimolecular and bimolecular reactions. These recent results have overturned conclusions from some previous studies, while confirming others, and have clarified areas of investigation that will be critical targets for future studies. In addition to expanding our fundamental understanding of Criegee intermediates, the rapidly expanding knowledge base will support increasingly predictive models of their impacts on society. C1 [Osborn, David L.; Taatjes, Craig A.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. RP Osborn, DL (reprint author), Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. EM dlosbor@sandia.gov FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; National Nuclear Security Administration [DE-AC04-94AL85000] FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the National Nuclear Security Administration, under contract DE-AC04-94AL85000. NR 129 TC 26 Z9 26 U1 24 U2 125 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 0144-235X EI 1366-591X J9 INT REV PHYS CHEM JI Int. Rev. Phys. Chem. PD JUL 3 PY 2015 VL 34 IS 3 BP 309 EP 360 DI 10.1080/0144235X.2015.1055676 PG 52 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CO4VY UT WOS:000359160200001 ER PT J AU Chen, SM Mercado, BQ Bergman, RG Ellman, JA AF Chen, Shuming Mercado, Brandon Q. Bergman, Robert G. Ellman, Jonathan A. TI Regio- and Diastereoselective Synthesis of Highly Substituted, Oxygenated Piperidines from Tetrahydropyridines SO JOURNAL OF ORGANIC CHEMISTRY LA English DT Article ID M-CHLOROPERBENZOIC ACID; C-H ACTIVATION; STEREOSELECTIVE-SYNTHESIS; POLYSUBSTITUTED PIPERIDINES; NITROGEN-HETEROCYCLES; ALKENYLAMMONIUM SALTS; ASYMMETRIC-SYNTHESIS; HOMOALLYLIC AMINES; AZOMETHINE YLIDES; EPOXIDE REACTIONS AB Diastereoselective epoxidation and regioselective ring-opening methods were developed for the synthesis of densely substituted, oxygenated piperidines from two classes of tetrahydropyridines with distinct stereochemical displays of functionalities. A new and practical in situ prepared epoxidation reagent was developed for the diastereoselective epoxidation of one class of sterically hindered tetrahydropyridines. The novel bifunctional epoxidation reagent, 2-carboperoxy-3,4,5,6-tetrafluorobenzoic acid; was designed to incorporate highly reactive percarboxy acid and pendant carboxylic acid groups, which through hydrogen bonding to the amino group successfully overrode steric effects and directed epoxidation to occur at the more hindered face of the tetrahydropyridine. Nucleophilic ring-opening of the epoxides with water, alcohols, and HE proceeded with high regioselectivity, affording piperidinol products with adjacent tetrasubstituted carbons. C1 [Chen, Shuming; Mercado, Brandon Q.; Ellman, Jonathan A.] Yale Univ, Dept Chem, New Haven, CT 06520 USA. [Bergman, Robert G.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Bergman, Robert G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Ellman, JA (reprint author), Yale Univ, Dept Chem, 225 Prospect St, New Haven, CT 06520 USA. EM jonathan.ellman@yale.edu RI Ellman, Jonathan/C-7732-2013 FU NIH [GM069559]; Office of Basic Energy Sciences, Chemical Sciences Division, U.S. DOE [DE-AC02-05CH11231] FX This work was supported by the NIH Grant GM069559 (to J.A.E.). R.G.B. acknowledges funding from the Office of Basic Energy Sciences, Chemical Sciences Division, U.S. DOE, under Contract DE-AC02-05CH11231. We are grateful to Prof. Scott Miller for helpful discussions. NR 52 TC 3 Z9 3 U1 1 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0022-3263 J9 J ORG CHEM JI J. Org. Chem. PD JUL 3 PY 2015 VL 80 IS 13 BP 6660 EP 6668 DI 10.1021/acs.joc.5b00816 PG 9 WC Chemistry, Organic SC Chemistry GA CM3ZN UT WOS:000357624100016 PM 26098485 ER PT J AU Hamada, MS AF Hamada, M. S. TI Bayesian Analysis of Step-Stress Accelerated Life Tests and Its Use in Planning SO QUALITY ENGINEERING LA English DT Article DE simulation; cumulative damage; credible interval; Metropolis-Hastings algorithm; Weibull distribution; lifetime quantile ID MODEL AB A Bayesian analysis of step-stress accelerated life test data is introduced and illustrated by an experiment on cryogenic cables. A cumulative damage model is used to describe the cumulative distribution function of Weibull lifetimes. The analysis methodology can then be used to evaluate a step-stress accelerated life test plan through simulation and calculation of appropriate criteria. Such planning is illustrated with the cryogenic cable example. C1 Los Alamos Natl Lab, Stat Sci Grp, Los Alamos, NM 87545 USA. RP Hamada, MS (reprint author), Los Alamos Natl Lab, Stat Sci Grp, Mail Stop F600, Los Alamos, NM 87545 USA. EM hamada@lanl.gov NR 14 TC 2 Z9 2 U1 3 U2 10 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 0898-2112 EI 1532-4222 J9 QUAL ENG JI Qual. Eng. PD JUL 3 PY 2015 VL 27 IS 3 SI SI BP 276 EP 282 DI 10.1080/08982112.2015.1038357 PG 7 WC Engineering, Industrial; Statistics & Probability SC Engineering; Mathematics GA CK7RB UT WOS:000356428700002 ER PT J AU Lu, L Anderson-Cook, CM AF Lu, Lu Anderson-Cook, Christine M. TI Improving Reliability Understanding Through Estimation and Prediction with Usage Information SO QUALITY ENGINEERING LA English DT Article DE population reliability; auxiliary information; Bayesian analysis; individual reliability ID POPULATION AB Using information about the usage or exposure of a complex system in addition to its age can provide additional understanding about mechanisms driving change in reliability as well as potentially improve the prediction. Both the individual reliability of particular units as well as population reliability can be improved with the inclusion of additional explanatory factors. In this article we consider an example based on a complex munition system. Using age alone to predict reliability can provide some information, but differences between units of the same age cannot be discerned. Subpopulations of the stockpile can be identified to help improve estimation, but the largest gains in understanding of the mechanisms driving change in reliability and prediction of future performance come from incorporating usage information. C1 [Lu, Lu] Univ S Florida, Dept Math & Stat, Tampa, FL USA. [Anderson-Cook, Christine M.] Los Alamos Natl Lab, Stat Sci Grp, Los Alamos, NM 87545 USA. RP Anderson-Cook, CM (reprint author), Los Alamos Natl Lab, Stat Sci Grp, POB 1663,MS F600, Los Alamos, NM 87545 USA. EM c-and-cook@lanl.gov NR 4 TC 1 Z9 1 U1 0 U2 3 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 0898-2112 EI 1532-4222 J9 QUAL ENG JI Qual. Eng. PD JUL 3 PY 2015 VL 27 IS 3 SI SI BP 304 EP 316 DI 10.1080/08982112.2014.990033 PG 13 WC Engineering, Industrial; Statistics & Probability SC Engineering; Mathematics GA CK7RB UT WOS:000356428700006 ER PT J AU Xu, CC Chinte, U Chen, LR Yao, QQ Meng, Y Zhou, D Bi, LJ Rose, J Adang, MJ Wang, BC Yu, ZN Sun, M AF Xu, Chengchen Chinte, Unmesh Chen, Lirong Yao, Qingqing Meng, Ying Zhou, Dayong Bi, Li-Jun Rose, John Adang, Michael J. Wang, Bi-Cheng Yu, Ziniu Sun, Ming TI Crystal structure of Cry51Aa1: A potential novel insecticidal aerolysin-type beta-pore-forming toxin from Bacillus thuringiensis SO BIOCHEMICAL AND BIOPHYSICAL RESEARCH COMMUNICATIONS LA English DT Article DE Bacillus thuringiensis; Crystal structure; Insecticidal; Pore-forming toxin ID PROTEIN; SIMILARITY; PARASPORIN; MECHANISM; BINDING AB The structures of several Bacillus thuringiensis (Bt) insecticidal crystal proteins have been determined by crystallographic methods and a close relationship has been explicated between specific toxicities and conserved three-dimensional architectures. In this study, as a representative of the coleopteran- and hemipteran-specific Cry51A group, the complete structure of Cry51Aa1 protoxin has been determined by X-ray crystallography at 1.65 angstrom resolution. This is the first report of a coleopteran-active Bt insecticidal toxin with high structural similarity to the aerolysin-type beta-pore forming toxins (beta-FFTs). Moreover, study of featured residues and structural elements reveal their possible roles in receptor binding and pore formation events. This study provides new insights into the action of aerolysin-type (beta-PFTs from a structural perspective, and could be useful for the control of coleopteran and hemipteran insect pests in agricultures. (C) 2015 Elsevier Inc. All rights reserved. C1 [Xu, Chengchen; Meng, Ying; Yu, Ziniu; Sun, Ming] Huazhong Agr Univ, Coll Life Sci & Technol, State Key Lab Agr Microbiol, Wuhan 430070, Hubei, Peoples R China. [Xu, Chengchen; Chinte, Unmesh; Chen, Lirong; Zhou, Dayong; Rose, John; Adang, Michael J.; Wang, Bi-Cheng] Univ Georgia, Dept Biochem & Mol Biol, Athens, GA 30602 USA. [Chinte, Unmesh; Rose, John; Wang, Bi-Cheng] Univ Georgia, SER CAT, Argonne, IL 60439 USA. [Chinte, Unmesh; Rose, John; Wang, Bi-Cheng] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Yao, Qingqing] Fudan Univ, Sch Life Sci, Dept Biochem, Shanghai 200438, Peoples R China. [Bi, Li-Jun] Chinese Acad Sci, Inst Biophys, Natl Lab Biomacromol, Beijing 100101, Peoples R China. [Adang, Michael J.] Univ Georgia, Dept Entomol, Athens, GA 30602 USA. RP Yu, ZN (reprint author), Huazhong Agr Univ, Coll Life Sci & Technol, State Key Lab Agr Microbiol, Wuhan 430070, Hubei, Peoples R China. EM wang@bcl1.bmb.uga.edu; yz41@mail.hzau.edu.cn; m98sun@mail.hzau.edu.cn RI Ming, Sun/Q-1497-2015 FU State Key Program of National Natural Science of China [30930004, 31170047]; National High Technology Research and Development Program (863) of China [2011AA10A203]; China 948 Program of Ministry of Agriculture [2011-G25]; Georgia Research Alliance and the University of Georgia Research Foundation; U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [W-31-109-Eng-38] FX This project was supported by the State Key Program of National Natural Science of China (Grant No. 30930004 and 31170047), the National High Technology Research and Development Program (863) of China (2011AA10A203), the China 948 Program of Ministry of Agriculture (2011-G25), the Georgia Research Alliance and the University of Georgia Research Foundation. Use of the Advanced Photon Source was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. W-31-109-Eng-38." NR 28 TC 10 Z9 11 U1 2 U2 34 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0006-291X EI 1090-2104 J9 BIOCHEM BIOPH RES CO JI Biochem. Biophys. Res. Commun. PD JUL 3 PY 2015 VL 462 IS 3 BP 184 EP 189 DI 10.1016/j.bbrc.2015.04.068 PG 6 WC Biochemistry & Molecular Biology; Biophysics SC Biochemistry & Molecular Biology; Biophysics GA CK6DY UT WOS:000356319900003 PM 25957471 ER PT J AU Harvey, CA Carter, JC Ertel, JR Alviso, CT Chinn, SC Maxwell, RS AF Harvey, Chris A. Carter, J. Chance Ertel, John R. Alviso, Cindy T. Chinn, Sarah C. Maxwell, Robert S. TI Fiber-based solid phase microextraction using fused silica lined bottles to collect, store, and stabilize a multianalyte headspace gas sample for offline analyses SO JOURNAL OF CHROMATOGRAPHY A LA English DT Article DE Fiber SPME; GC-MS; Gas chromatography; Fused silica lined bottle; In situ HS-SPME; Headspace gas analysis; Material outgassing; Internal standard; External standard; Magnetic translation ID SPME-GC-MS; ORGANIC-COMPOUNDS; WATER; QUANTIFICATION; OPTIMIZATION; EXTRACTION; RESIDUES; DESIGN AB We have developed a solid phase microextraction (SPME) sampling method using fused silica lined bottles (400 ml) to collect, store, and stabilize a headspace subsample from the source for subsequent offline, repetitive analyses of the gas using fiber-based SPME. The method enables long-term stability for repeated offline analysis of the organic species collected from the source headspace and retains all the advantages of fiber SPME sampling (e.g. rapid extraction, solvent free, simple and inexpensive) while providing additional advantages. Typically, the analytes collected on the SPME fiber must be desorbed and analyzed immediately to mitigate analyte loss or contamination. The new SPME sampling method, conducted offline using carboxen/polydimethylsiloxane (carboxen/PDMS 85 mu m) coated fibers, has been shown to be identical to in situ SPME sampling of a headspace acquired from an 80 component organic matrix with reproducibility demonstrated to be less than %RSD = 7.0% for replicate samples measured over a 30-day period. In addition, repetitive samplings from one headspace aliquot are possible using one or more fibers and fiber types as well as quantitative options such as internal standard addition as demonstrated in a feasibility study using a benzene/toluene/xylene (BTX; 1 ppmv) certified gas standard, in which the SAME measurement precision (%RSD) was improved by a factor of 1.5-1.9 compared to the use of an external standard. (C) 2015 Elsevier B.V. All rights reserved. C1 [Harvey, Chris A.; Carter, J. Chance; Ertel, John R.; Alviso, Cindy T.; Chinn, Sarah C.; Maxwell, Robert S.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Harvey, CA (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. EM harvey11@llnl.gov FU LLNL [DE-AC52-07NA27344] FX The authors would like to express thanks to Linda Domeier of Sandia National Laboratory Livermore, CA for her cooperation and contributions during the multi-material compatibility test. Prepared by LLNL under Contract DE-AC52-07NA27344. NR 23 TC 2 Z9 2 U1 5 U2 25 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0021-9673 EI 1873-3778 J9 J CHROMATOGR A JI J. Chromatogr. A PD JUL 3 PY 2015 VL 1401 BP 1 EP 8 DI 10.1016/j.chroma.2015.04.032 PG 8 WC Biochemical Research Methods; Chemistry, Analytical SC Biochemistry & Molecular Biology; Chemistry GA CK9HI UT WOS:000356550800001 PM 26008594 ER PT J AU Jankovic, J Zontek, TL Ogle, BR Hollenbeck, S AF Jankovic, John Zontek, Tracy L. Ogle, Burton R. Hollenbeck, Scott TI Analytical Performance Issues Direct Reading Particle Counters: Calibration Verification and Multiple Instrument Agreement via Bump Testing SO JOURNAL OF OCCUPATIONAL AND ENVIRONMENTAL HYGIENE LA English DT Article C1 [Jankovic, John; Hollenbeck, Scott] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN USA. [Zontek, Tracy L.; Ogle, Burton R.] Western Carolina Univ, Environm Hlth Program, Cullowhee, NC 28723 USA. RP Zontek, TL (reprint author), Western Carolina Univ, 4121 Little Savannah Rd, Cullowhee, NC 28723 USA. EM zontek@email.wcu.edu FU DOE Higher Education Research Experience (HERE) FX Additionally, this research was supported by the DOE Higher Education Research Experience (HERE) and was administered by the Oak Ridge Institute for Science and Education (ORISE). NR 8 TC 0 Z9 0 U1 0 U2 1 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 1545-9624 EI 1545-9632 J9 J OCCUP ENVIRON HYG JI J. Occup. Environ. Hyg. PD JUL 3 PY 2015 VL 12 IS 7 BP D116 EP D122 PG 7 WC Environmental Sciences; Public, Environmental & Occupational Health SC Environmental Sciences & Ecology; Public, Environmental & Occupational Health GA CK4MF UT WOS:000356197200002 ER PT J AU Jankovic, J Zontek, TL Ogle, BR Hollenbeck, S AF Jankovic, John Zontek, Tracy L. Ogle, Burton R. Hollenbeck, Scott TI Direct Reading Particle Counters: Calibration Verification and Multiple Instrument Agreement via Bump Testing SO JOURNAL OF OCCUPATIONAL AND ENVIRONMENTAL HYGIENE LA English DT Article DE condensation particle counter; air monitoring; calibration; nanoscale material AB The calibration records of two direct reading instruments designated as condensation particle counters were examined to determine the number of times they were found to be out of tolerance at annual manufacturer's recalibration. Both instruments were found to be out of tolerance more times than within tolerance. And, it was concluded that annual calibration alone was insufficient to provide operational confidence in an instrument's response. Therefore, a method based on subsequent agreement with data gathered from a newly calibrated instrument was developed to confirm operational readiness between annual calibrations, hereafter referred to as bump testing. The method consists of measuring source particles produced by a gas grille spark igniter in a gallon-size jar. Sampling from this chamber with a newly calibrated instrument to determine the calibrated response over the particle concentration range of interest serves as a reference. Agreement between this reference response and subsequent responses at later dates implies that the instrument is performing as it was at the time of calibration. Side-by-side sampling allows the level of agreement between two or more instruments to be determined. This is useful when simultaneously collected data are compared for differences, i.e., background with process aerosol concentrations. A reference set of data was obtained using the spark igniter. The generation system was found to be reproducible and suitable to form the basis of calibration verification. The bump test is simple enough to be performed periodically throughout the calibration year or prior to field monitoring. C1 [Jankovic, John; Hollenbeck, Scott] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN USA. [Zontek, Tracy L.; Ogle, Burton R.] Western Carolina Univ, Environm Hlth Program, Cullowhee, NC 28723 USA. RP Zontek, TL (reprint author), Western Carolina Univ, 4121 Little Savannah Rd, Cullowhee, NC 28723 USA. EM zontek@email.wcu.edu FU DOE Higher Education Research Experience (HERE) FX Additionally, this research was supported by the DOE Higher Education Research Experience (HERE) and was administered by the Oak Ridge Institute for Science and Education (ORISE). NR 8 TC 0 Z9 0 U1 0 U2 4 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 1545-9624 EI 1545-9632 J9 J OCCUP ENVIRON HYG JI J. Occup. Environ. Hyg. PD JUL 3 PY 2015 VL 12 IS 7 BP D116 EP D122 DI 10.1080/15459624.2015.1009990 PG 7 WC Environmental Sciences; Public, Environmental & Occupational Health SC Environmental Sciences & Ecology; Public, Environmental & Occupational Health GA CK4MM UT WOS:000356197900002 ER PT J AU Song, M Chu, JH Zhou, J Tongay, S Liu, K Suh, J Chen, H Kang, JS Zou, XC You, L AF Song, Min Chu, Jiun-Haw Zhou, Jian Tongay, Sefaattin Liu, Kai Suh, Joonki Chen, Henry Kang, Jeong Seuk Zou, Xuecheng You, Long TI Magnetoresistance oscillations in topological insulator Bi2Te3 nanoscale antidot arrays SO NANOTECHNOLOGY LA English DT Article DE topological insulator; antidot array; magnetoresistance; coherence length; surface states; reactive ion etching ID CROSSOVER; SYSTEMS AB Nanoscale antidot arrays were fabricated on a single-crystal microflake of topological insulator Bi2Te3. The introduction of antidot arrays significantly increased the resistance of the microflake, yet the temperature dependence of the resistance remains metallic. We observed that small oscillations that are periodic in magnetic field B appeared on top of the weak anti-localization magnetoresistance. Since the electron coherence length at low temperature becomes comparable to the feature size in our device, we argued that the magnetoresistance oscillations are the manifestation of quantum interference induced by the nanostructure. Our work demonstrates that the transport of topological insulators could indeed be controlled by artificially created nanostructures, and paves the way for future technological applications of this class of materials. C1 [Song, Min; Zou, Xuecheng; You, Long] Huazhong Univ Sci & Technol, Sch Opt & Elect Informat, Wuhan 430074, Hubei, Peoples R China. [Chu, Jiun-Haw] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Zhou, Jian; Tongay, Sefaattin; Liu, Kai; Suh, Joonki; Kang, Jeong Seuk] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Chen, Henry] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [You, Long] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. RP Song, M (reprint author), Huazhong Univ Sci & Technol, Sch Opt & Elect Informat, Wuhan 430074, Hubei, Peoples R China. EM Jiun-Haw.Chu@stanford.edu; long@eecs.berkeley.edu RI Liu, Kai/A-4754-2012 OI Liu, Kai/0000-0002-0638-5189 NR 15 TC 1 Z9 1 U1 4 U2 38 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD JUL 3 PY 2015 VL 26 IS 26 AR 265301 DI 10.1088/0957-4484/26/26/265301 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA CK7XE UT WOS:000356448700005 PM 26059087 ER PT J AU Mhamdi, R Ardley, J Tian, R Seshadri, R Reddy, TBK Pati, A Woyke, T Markowitz, V Ivanova, N Kyrpides, N Reeve, W AF Mhamdi, Ridha Ardley, Julie Tian, Rui Seshadri, Rekha Reddy, T. B. K. Pati, Amrita Woyke, Tanja Markowitz, Victor Ivanova, Natalia Kyrpides, Nikos Reeve, Wayne TI High-quality permanent draft genome sequence of Ensifer meliloti strain 4H41, an effective salt- and drought-tolerant microsymbiont of Phaseolus vulgaris SO STANDARDS IN GENOMIC SCIENCES LA English DT Article DE Root-nodule bacteria; Nitrogen fixation; Alphaproteobacteria; Ensifer; Phaseolus vulgaris ID SINORHIZOBIUM-MELILOTI; RHIZOBIUM-MELILOTI; MICROBIAL GENOMES; TUNISIAN SOILS; ROOT-NODULE; SP-NOV; COMMON; SYSTEM; L.; MEDITERRANENSE AB Ensifer meliloti 4H41 is an aerobic, motile, Gram-negative, non-spore-forming rod that can exist as a soil saprophyte or as a legume microsymbiont of common bean (Phaseolus vulgaris). Strain 4H41 was isolated in 2002 from root nodules of P. vulgaris grown in South Tunisia from the oasis of Rjim-Maatoug. Strain 4H41 is salt-and drought-tolerant and highly effective at fixing nitrogen with P. vulgaris. Here we describe the features of E. meliloti 4H41, together with genome sequence information and its annotation. The 6,795,637 bp high-quality permanent draft genome is arranged into 47 scaffolds of 47 contigs containing 6,350 protein-coding genes and 72 RNA-only encoding genes, and is one of the rhizobial genomes sequenced as part of the DOE Joint Genome Institute 2010 Genomic Encyclopedia for Bacteria and Archaea-Root Nodule Bacteria (GEBA-RNB) project proposal. C1 [Mhamdi, Ridha] Ctr Biotechnol Borj Cedria, Lab Legumes, Hammam Lif 2050, Tunisia. [Ardley, Julie; Tian, Rui; Reeve, Wayne] Murdoch Univ, Ctr Rhizobium Studies, Murdoch, WA 6150, Australia. [Seshadri, Rekha; Reddy, T. B. K.; Pati, Amrita; Woyke, Tanja; Ivanova, Natalia; Kyrpides, Nikos] DOE Joint Genome Inst, Walnut Creek, CA USA. [Markowitz, Victor] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Data Management & Technol Ctr, Berkeley, CA 94720 USA. [Kyrpides, Nikos] King Abdulaziz Univ, Fac Sci, Dept Biol Sci, Jeddah 21413, Saudi Arabia. RP Reeve, W (reprint author), Murdoch Univ, Ctr Rhizobium Studies, Murdoch, WA 6150, Australia. EM W.Reeve@murdoch.edu.au RI Mhamdi, Ridha/D-9378-2013; Kyrpides, Nikos/A-6305-2014; Fac Sci, KAU, Biol Sci Dept/L-4228-2013; Faculty of, Sciences, KAU/E-7305-2017 OI Ivanova, Natalia/0000-0002-5802-9485; Mhamdi, Ridha/0000-0002-2999-7604; Kyrpides, Nikos/0000-0002-6131-0462; FU US Department of Energy's Office of Science, Biological and Environmental Research Program; University of California, Lawrence Berkeley National Laboratory [DE-AC02-05CH11231] FX This work was performed under the auspices of the US Department of Energy's Office of Science, Biological and Environmental Research Program, and by the University of California, Lawrence Berkeley National Laboratory under contract No. DE-AC02-05CH11231. We thank Gordon Thompson (Murdoch University) for the preparation of SEM and TEM photos. NR 54 TC 1 Z9 1 U1 1 U2 2 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD JUL 2 PY 2015 VL 10 AR 34 DI 10.1186/s40793-015-0005-1 PG 7 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DA7MQ UT WOS:000367988800001 PM 26380038 ER PT J AU Groza, T Kohler, S Moldenhauer, D Vasilevsky, N Baynam, G Zemojtel, T Schriml, LM Kibbe, WA Schofield, PN Beck, T Vasant, D Brookes, AJ Zankl, A Washington, NL Mungall, CJ Lewis, SE Haendel, MA Parkinson, H Robinson, PN AF Groza, Tudor Koehler, Sebastian Moldenhauer, Dawid Vasilevsky, Nicole Baynam, Gareth Zemojtel, Tomasz Schriml, Lynn Marie Kibbe, Warren Alden Schofield, Paul N. Beck, Tim Vasant, Drashtti Brookes, Anthony J. Zankl, Andreas Washington, Nicole L. Mungall, Christopher J. Lewis, Suzanna E. Haendel, Melissa A. Parkinson, Helen Robinson, Peter N. TI The Human Phenotype Ontology: Semantic Unification of Common and Rare Disease SO AMERICAN JOURNAL OF HUMAN GENETICS LA English DT Article ID GENOME-WIDE ASSOCIATION; RISK LOCI; GENETIC-VARIANTS; IDENTIFICATION; DISORDERS; DATABASE; SUSCEPTIBILITY; MUTATIONS; MEDICINE; RESOURCE AB The Human Phenotype Ontology (HPO) is widely used in the rare disease community for differential diagnostics, phenotype-driven analysis of next-generation sequence-variation data, and translational research, but a comparable resource has not been available for common disease. Here, we have developed a concept-recognition procedure that analyzes the frequencies of HPO disease annotations as identified in over five million Pub Med abstracts by employing an iterative procedure to optimize precision and recall of the identified terms. We derived disease models for 3,145 common human diseases comprising a total of 132,006 HPO annotations. The HPO now comprises over 250,000 phenotypic annotations for over 10,000 rare and common diseases and can be used for examining the phenotypic overlap among common diseases that share risk alleles, as well as between Mendelian diseases and common diseases linked by genomic location. The annotations, as well as the HPO itself, are freely available. C1 [Groza, Tudor] Univ Queensland, Sch Informat Technol & Elect Engn, St Lucia, Qld 4072, Australia. [Groza, Tudor; Zankl, Andreas] Garvan Inst Med Res, Sydney, NSW 2010, Australia. [Koehler, Sebastian; Moldenhauer, Dawid; Zemojtel, Tomasz; Robinson, Peter N.] Charite, Inst Med & Human Genet, D-13353 Berlin, Germany. [Moldenhauer, Dawid] Univ Appl Sci, D-35390 Giessen, Germany. [Vasilevsky, Nicole] Oregon Hlth & Sci Univ, Lib, Portland, OR 97239 USA. [Baynam, Gareth] Univ Western Australia, Sch Paediat & Child Hlth, Perth, WA 6840, Australia. [Baynam, Gareth] Murdoch Univ, Inst Immunol & Infect Dis, Perth, WA 6150, Australia. [Baynam, Gareth] Off Populat Hlth Genom, Publ Hlth & Clin Serv Div, Dept Hlth, Perth, WA 6004, Australia. [Baynam, Gareth] King Edward Mem Hosp, Genet Serv Western Australia, Perth, WA 6008, Australia. [Baynam, Gareth] Telethon Kids Inst, Perth, WA 6008, Australia. [Zemojtel, Tomasz] Polish Acad Sci, Inst Bioorgan Chem, PL-61704 Poznan, Poland. [Schriml, Lynn Marie] Univ Maryland, Sch Med, Dept Epidemiol & Publ Hlth, Baltimore, MD 21201 USA. [Schriml, Lynn Marie] Univ Maryland, Sch Med, Inst Genome Sci, Baltimore, MD 21201 USA. [Kibbe, Warren Alden] NCI, Ctr Biomed Informat & Informat Technol, Rockville, MD 20850 USA. [Schofield, Paul N.] Univ Cambridge, Dept Physiol Dev & Neurosci, Cambridge CB2 3EG, England. [Schofield, Paul N.] Jackson Lab, Bar Harbor, ME 04609 USA. [Beck, Tim; Brookes, Anthony J.] Univ Leicester, Dept Genet, Leicester LE1 7RH, Leics, England. [Vasant, Drashtti; Parkinson, Helen] European Bioinformat Inst, European Mol Biol Lab, Cambridge CB10 1SD, England. [Zankl, Andreas] Childrens Hosp Westmead, Acad Dept Med Genet, Sydney, NSW 2145, Australia. [Zankl, Andreas] Univ Sydney, Discipline Genet Med, Sydney Med Sch, Sydney, NSW 2145, Australia. [Washington, Nicole L.; Mungall, Christopher J.; Lewis, Suzanna E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Genom Div, Berkeley, CA 94720 USA. [Robinson, Peter N.] Max Planck Inst Mol Genet, D-14195 Berlin, Germany. [Robinson, Peter N.] Charite, Berlin Brandenburg Ctr Regenerat Therapies, D-13353 Berlin, Germany. [Robinson, Peter N.] Free Univ Berlin, Dept Math & Comp Sci, Inst Bioinformat, D-14195 Berlin, Germany. RP Robinson, PN (reprint author), Charite, Inst Med & Human Genet, Augustenburger Pl 1, D-13353 Berlin, Germany. EM peter.robinson@charite.de OI Parkinson, Helen/0000-0003-3035-4195; Kohler, Sebastian/0000-0002-5316-1399; Lewis, Suzanna/0000-0002-8343-612X; Schriml, Lynn/0000-0001-8910-9851; Vasilevsky, Nicole/0000-0001-5208-3432 FU Bundesministerium fur Bildung und Forschung [0313911]; European Commission [602300]; Raine Clinician Research Fellowship [20140101]; National Health and Medical Research Council of Australia [APP1055319, 305444]; NIH Office of the Director [1R24OD011883-01]; Australian Research Council Discovery Early Career Researcher Award [DE120100508]; BioMedBridges project - Research Infrastructures of the FP7 [284209]; European Molecular Biology Laboratory Core Funds; Basic Energy Sciences, Office of Science, US Department of Energy [DE-AC02-05CH11231]; NIH [1R24OD011883-01]; US Government FX This work was supported by the Bundesministerium fur Bildung und Forschung (project 0313911), the European Commission Seventh Framework Programme (FP7; grant 602300; SYBIL project), the Raine Clinician Research Fellowship (20140101), and the National Health and Medical Research Council of Australia (grant APP1055319, which is partnered with FP7 grant 305444). Oregon Health and Science University acknowledges the support of grant 1R24OD011883-01 from the NIH Office of the Director. T.G. was supported by an Australian Research Council Discovery Early Career Researcher Award (DE120100508). D.V. was supported in part by the BioMedBridges project funded by Research Infrastructures of the FP7 (grant 284209). H.P. was supported by European Molecular Biology Laboratory Core Funds. This work was supported by the director, Basic Energy Sciences, Office of Science, US Department of Energy under contract DE-AC02-05CH11231 and NIH contract 1R24OD011883-01. This document was prepared as an account of work sponsored by the US Government. While this document is believed to contain correct information, neither the US Government nor any agency thereof, nor the Regents of the University of California, nor any of their employees makes any warranty, express or implied, or assumes any legal responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed or represents that its use would not infringe privately owned rights. The views and opinions of authors expressed herein do not necessarily state or reflect those of the US Government or any agency thereof or the Regents of the University of California. NR 85 TC 34 Z9 35 U1 2 U2 14 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0002-9297 EI 1537-6605 J9 AM J HUM GENET JI Am. J. Hum. Genet. PD JUL 2 PY 2015 VL 97 IS 1 BP 111 EP 124 DI 10.1016/j.ajhg.2015.05.020 PG 14 WC Genetics & Heredity SC Genetics & Heredity GA CN1OO UT WOS:000358189500010 PM 26119816 ER PT J AU Aad, G Collaboration, A Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Auerbach, B Augsten, K Aurousseau, M Avolio, G Axen, B Azuelos, G Azuma, Y Baak, MA Baas, AE Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Balek, P Balli, F Banas, E Banerjee, S Bannoura, AAE Bansil, HS Barak, L Baranov, SP Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Bartsch, V Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Battistin, M Bauer, F Bawa, HS Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Becot, C Beddall, AJ Bedikian, S Beddall, A Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, K Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernat, P Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biesiada, J Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boddy, CR Boehler, M Boek, TT Bogaerts, JA Bogdanchikov, AG Bogouch, A Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borri, M Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boterenbrood, H Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutouil, S Boveia, A Boyd, J Boyko, IR Bozic, I Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brelier, B Brendlinger, K Brennan, AJ Brenner, R Bressler, S Bristow, K Bristow, TM Britton, D Brochu, FM Brock, I Brock, R Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Brunet, S Bruni, A Bruni, G Bruschi, M Bryngemark, L Buanes, T Buat, Q Bucci, F Buchholz, P Buckley, AG Buda, SI Budagov, IA Buehrer, F Bugge, L Bugge, MK Bulekov, O Bundock, AC Burckhart, H Burdin, S Burghgrave, B Burke, S Burmeister, I Busato, E Buescher, D Buescher, V Bussey, P Buszello, CP Butler, B Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Byszewski, M Urban, SC Caforio, D Cakir, O Calafiura, P Calandri, A Calderini, G Calfayan, P Calkins, R Caloba, LP Calvet, D Calvet, S Toro, RC Camarda, S Cameron, D Caminada, LM Armadans, RC Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Cardarelli, R Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Cattani, G Caudron, J Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, BC Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chang, P Chapleau, B Chapman, JD Charfeddine, D Charlton, DG Chau, CC Barajas, CAC Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiefari, G Childers, JT Chilingarov, A Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Chouridou, S Chow, BKB Chromek-Burckhart, D Chu, ML Chudoba, J Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Ciftci, R Cinca, D Cindro, V Ciocio, A Citron, ZH Citterio, M Ciubancan, M Clark, A Clark, PJ Clarke, RN Cleland, W Clemens, JC Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Cogan, JG Cole, B Cole, S Colijn, AP Collot, J Colomboc, T Compostella, G Muino, PC Coniavitis, E Connellb, SH Connelly, IA Consonni, SM Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cooper-Smith, NJ Copic, K Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cote, D Cottin, G Cowan, G Cox, BE Cranmer, K Cree, G Crepe-Renaudin, S Crescioli, F Cribbs, WA Ortuzar, MC Cristinziani, M Croft, V Crosetti, G Donszelmann, TC Cummings, J Curatolo, M Cuthbert, C Czirr, H Czodrowski, P D'Auria, S D'Onofrio, M De Sousa, MJDS Da Via, C Dabrowski, W Dafinca, A Dai, T Dale, O Dallaire, F Dallapiccola, C Dam, M Daniells, AC Hoffmann, MD Dao, V Darbo, G Darmora, S Dassoulas, J Dattagupta, A Davey, W David, C Davidek, T Davies, E Davies, M Davignon, O Davison, AR Davison, P Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Castro, S De Cecco, S De Groot, N De Jong, P De la Torre, H De Lorenzi, F De Nooij, L De Pedis, D De Salvo, A De Sanctis, U De Santo, A De Regie, JBD Dearnaley, WJ Debbe, R Debenedetti, C Dechenaux, B Dedovich, DV Deigaard, I Del Peso, J Del Prete, T Deliot, F Delitzsch, CM Deliyergiyev, M Dell'Acqua, A Dell'Asta, L Dell'Orso, M Della Pietra, M Della Volpe, D Delmastro, M Delsart, PA Deluca, C DeMarco, DA Demers, S Demichev, M Demilly, A Denisov, SP Derendarz, D Derkaoui, JE Derue, F Dervan, P Desch, K Deterre, C Deviveiros, PO Dewhurst, A Dhaliwal, S Di Ciaccio, A Di Ciaccio, L Di Domenico, A Di Donato, C Di Girolamo, A Di Girolamo, B Di Mattia, A Di Micco, B Di Nardo, R Di Simone, A Di Sipio, R Di Valentino, D Dias, FA Diaz, MA Diehl, EB Dietrich, J Dietzsch, TA Diglio, S Dimitrievska, A Dingfelder, J Dita, P Dita, S Dittus, F Djama, F Djobava, T Djuvsland, JI do Vale, MAB Dobos, D Doglioni, C Doherty, T Dohmae, T Dolejsi, J Dolezal, Z Dolgoshein, BA Donadelli, M Donati, S Dondero, P Donini, J Dopke, J Doria, A Dova, MT Doyle, AT Dris, M Dubbert, J Dube, S Dubreuil, E Duchovni, E Duckeck, G Ducu, OA Duda, D Dudarev, A Dudziak, F Duflot, L Duguid, L 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TI Identification and energy calibration of hadronically decaying tau leptons with the ATLAS experiment in pp collisions at root s=8 TeV SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID CROSS-SECTION; MONTE-CARLO; DETECTOR; NUCLEUS; SEARCH AB This paper describes the trigger and offline reconstruction, identification and energy calibration algorithms for hadronic decays of tau leptons employed for the data collected from pp collisions in 2012 with the ATLAS detector at the LHC center-of-mass energy root s = 8 TeV. The performance of these algorithms is measured in most cases with Z decays to tau leptons using the full 2012 dataset, corresponding to an integrated luminosity of 20.3 fb(-1). An uncertainty on the offline reconstructed tau energy scale of 2-4%, depending on transverse energy and pseudorapidity, is achieved using two independent methods. The offline tau identification efficiency is measured with a precision of 2.5% for hadronically decaying tau leptons with one associated track, and of 4% for the case of three associated tracks, inclusive in pseudorapidity and for a visible transverse energy greater than 20 GeV. For hadronic tau lepton decays selected by offline algorithms, the tau trigger identification efficiency is measured with a precision of 2-8%, depending on the transverse energy. The performance of the tau algorithms, both offline and at the trigger level, is found to be stable with respect to the number of concurrent proton-proton interactions and has supported a variety of physics results using hadronically decaying tau leptons at ATLAS. C1 [Jackson, P.; Lee, L.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Gingrich, D. M.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Ciftci, R.; Yildiz, H. Duran] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Yilmaz, M.] Gazi Univ, Dept Phys, Ankara, Turkey. [Kuday, S.; Cakir, I. Turk] Istanbul Aydin Univ, Istanbul, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. [Barnovska, Z.; Berger, N.; Delmastro, M.; Di Ciaccio, L.; Elles, S.; Goy, C.; Hryn'ova, T.; Jezequel, S.; Keoshkerian, H.; Koletsou, I.; Lafaye, R.; Leveque, J.; Lombardo, V. P.; Massol, N.; Przysiezniak, H.; Sauvage, G.; Sauvan, E.; Schwoerer, M.; Simard, O.; Todorov, T.; Wingerter-Seez, I.] CNRS, IN2P3, LAPP, Annecy Le Vieux, France. [Barnovska, Z.; Berger, N.; Delmastro, M.; Di Ciaccio, L.; Elles, S.; Goy, C.; Hryn'ova, T.; Jezequel, S.; Keoshkerian, H.; Koletsou, I.; Lafaye, R.; Leveque, J.; Lombardo, V. P.; Massol, N.; Przysiezniak, H.; Sauvage, G.; Sauvan, E.; Schwoerer, M.; Simard, O.; Todorov, T.; Wingerter-Seez, I.] Univ Savoie, Annecy Le Vieux, France. [Asquith, L.; Auerbach, B.; Blair, R. E.; Chekanov, S.; Childers, J. T.; Feng, E. J.; LeCompte, T.; Love, J.; Malon, D.; Nguyen, D. H.; Nodulman, L.; Paramonov, A.; Price, L. E.; Proudfoot, J.; Stanek, R. W.; Van Gemmeren, P.; Vaniachine, A.; Yoshida, R.; Zhang, J.] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Cheu, E.; Johns, K. A.; Kaushik, V.; Lampen, C. L.; Lampl, W.; Lei, X.; Leone, R.; Loch, P.; Nayyar, R.; O'grady, F.; Rutherfoord, J. P.; Shupe, M. A.; Varnes, E. W.; Veatch, J.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Brandt, A.; Cote, D.; Darmora, S.; De, K.; Farbin, A.; Griffiths, J.; Hadavand, H. K.; Heelan, L.; Kim, H. Y.; Maeno, M.; Ozturk, N.; Pravahan, R.; Sosebee, M.; Stradling, A. R.; Usai, G.; Vartapetian, A.; White, A.; Yu, J.] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA. [Angelidakis, S.; Antonaki, A.; Chouridou, S.; Fassouliotis, D.; Giokaris, N.; Ioannou, P.; Iordanidou, K.; Kourkoumelis, C.; Manousakis-Katsikakis, A.; Tsirintanis, N.] Univ Athens, Dept Phys, Athens, Greece. [Alexopoulos, T.; Byszewski, M.; Dris, M.; Gazis, E. N.; Iakovidis, G.; Karakostas, K.; Karastathis, N.; Leontsinis, S.; Maltezos, S.; Ntekas, K.; Panagiotopoulou, E.; Papadopoulou, Th. D.; Tsipolitis, G.; Vlachos, S.] Natl Tech Univ Athens, Dept Phys, Zografos, Greece. [Abdinov, O.; Khalil-Zada, F.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Anjos, N.; Bosman, M.; Armadans, R. Caminal; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fracchia, S.; Giangiobbe, V.; Parra, G. Gonzalez; Grinstein, S.; Rozas, A. Juste; Korolkov, I.; Le Menedeu, E.; Paz, I. Lopez; Martinez, M.; Mir, L. M.; Berlingen, J. Montejo; Pages, A. Pacheco; Aranda, C. Padilla; Bueso, X. Portell; Riu, I.; Rubbo, F.; Sorin, V.; Succurro, A.; Tripiana, M. 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N.; Cooke, M.; Copic, K.; Dube, S.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Holmes, T. R.; Hurwitz, M.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Virzi, J.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Dietrich, J.; Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Herrberg-Schubert, R.; Hristova, I.; Kind, O.; Kolanoski, H.; Lacker, H.; Lohse, T.; Nikiforov, A.; Rehnisch, L.; Rieck, P.; Schulz, H.; Stamm, S.; Wendland, D.; zur Nedden, M.] Humboldt Univ, Dept Phys, Berlin, Germany. [Agustoni, M.; Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Kruker, T.; Marti, L. F.; Meloni, F.; Schneider, B.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Agustoni, M.; Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Kruker, T.; Marti, L. F.; Meloni, F.; Schneider, B.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allbrooke, B. M. M.; Bella, L. Aperio; Bansil, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Palmer, J. D.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Alberghi, G. L.; Bellagamba, L.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Caforio, D.; Corradi, M.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Acharya, B. S.; Ahmadov, F.; Huseynov, N.; Javadov, N.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Hageboeck, S.; Hellmich, D.; Huegging, F.; Janssen, J.; Khoriauli, G.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mergelmeyer, S.; Mijovic, L.; Mueller, K.; Nanava, G.; Nattermann, T.; Obermann, T.; Pohl, D.; Sarrazin, B.; Schaepe, S.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Seema, P.; Stillings, J. A.; Tannoury, N.; Therhaag, J.; Uchida, K.; Uhlenbrock, M.; Velz, T.; Vogel, A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Fitzgerald, E. A.; Sciolla, G.; Venturini, A.; Zambito, S.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE, EE, IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; de Andrade Filho, L. Manhaes] Univ Fed Juiz de Fora, Elect Circuits Dept, Juiz de Fora, Brazil. [do Vale, M. A. B.] Univ Fed Sao Joao del Rei, Sao Joao del Rei, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M-A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Schovancova, J.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Ducu, O. A.; Jinaru, A.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; Marchand, J. F.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Battistin, M.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; DHrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Franchino, S.; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. 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A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; Van der Ster, D.; Van Eldik, N.; Van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Cheng, Y.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Shandong, Peoples R China. [Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Podlyski, F.; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Podlyski, F.; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Podlyski, F.; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Guo, J.; Hu, D.; Hughes, E. W.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Wulf, E.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Nazl Frascati Lab, Grp Coll Cosenza, I-00044 Frascati, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Kopernya, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Lou, X.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Camarda, S.; Deterre, C.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Moenig, K.; Morton, A.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Camarda, S.; Deterre, C.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Moenig, K.; Morton, A.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Prokofiev, K.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dao, V.; Di Simone, A.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Kneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Madar, R.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ronzani, M.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Vuanh, T.; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; Della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; LaRosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nektarijevic, S.; Nikolics, K.; Picazio, A.; Pohl, M.; Rosbach, K.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; O'Shea, V.; Barrera, C. Oropeza; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.; Wright, M.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Bierwagen, K.; Bindi, M.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Keil, M.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.; Della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Dietzsch, T. A.; Djuvsland, J. I.; Dunford, M.; Hanke, P.; Jongmanns, J.; Khomich, A.; Kluge, E-E.; Laier, H.; Lang, V. S.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H-C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colomboc, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. Univ Hong Kong, Dept Phys, Pok Fu Lam, Hong Kong, Peoples R China. Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Brunet, S.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Glonti, G. L.; Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Morange, N.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Pluth, D.; Prell, S.; Shrestha, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Topilin, N. D.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dassoulas, J.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Readioff, N. P.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Egham, Surrey, England. [Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Cooper, B. D.; Davison, A. R.; Davison, P.; Falla, R. J.; Gregersen, K.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Sircar, A.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; LeDortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; LeDortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; LeDortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Goeringer, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Knig, S.; Koepke, L.; Lin, T. H.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Mueller, T.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Barnes, S. L.; Borri, M.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Hallewell, G. D.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. 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A.; Mantifel, R.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Jennens, D.; Kubota, T.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Harper, D.; Hu, X.; Levin, D.; Liu, L.; Long, J. D.; Lu, N.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Panikashvili, N.; Qian, J.; Schwarz, T. A.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Perini, L.; Pizio, C.; Ragusa, F.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. 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A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Heller, C.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Knig, A. C.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; De Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; Van der Geer, R.; Van der Graaf, H.; Van der Leeuw, R.; Van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; De Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; Van der Geer, R.; Van der Graaf, H.; Van der Leeuw, R.; Van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Burghgrave, B.; Calkins, R.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Kharlamov, A.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Tannenwald, B. B.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Behr, K.; Boddy, C. R.; Cooper-Sarkar, A. M.; Crispin Ortuzar, M.; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Lester, C. M.; Lipeles, E.; Meyer, C.; Ospanov, R.; Saxon, J.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis Fermi E, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Mueller, J.; Prieur, D.; Sapp, K.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; De Sousa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; De Sousa, M. J. Da Cunha Sargedas; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Aloisio, A.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Stanescu, C.; Taccini, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Taccini, C.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Pinto Firmino Da Costa, J. Goncalves; Guyot, C.; Hanna, R.; Hassani, S.; Kozanecki, W.; Lanon, E.; Laporte, J. F.; Maiani, C.; Mal, P.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay, DSM IRFU Inst Rech Lois Fondamentales Univer, Commissariat Energie Atom & Energies Alternat, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S-C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; Horton, A. J.; O'Neil, D. C.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. 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D.; Jeng, G-Y.; Limosani, A.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; LoSterzo, F.; Mazini, R.; Ren, Z. L.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. 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Vranjes Milosavljevic, Marija/F-9847-2016; Perrino, Roberto/B-4633-2010; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Shmeleva, Alevtina/M-6199-2015; Gavrilenko, Igor/M-8260-2015; Veneziano, Stefano/J-1610-2012; Tikhomirov, Vladimir/M-6194-2015; Villa, Mauro/C-9883-2009; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Brooks, William/C-8636-2013; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; De, Kaushik/N-1953-2013; Mitsou, Vasiliki/D-1967-2009; Zhukov, Konstantin/M-6027-2015; Grancagnolo, Sergio/J-3957-2015; Doyle, Anthony/C-5889-2009; Livan, Michele/D-7531-2012; spagnolo, stefania/A-6359-2012; Di Domenico, Antonio/G-6301-2011; Negrini, Matteo/C-8906-2014; Tassi, Enrico/K-3958-2015; Ferrando, James/A-9192-2012; Boyko, Igor/J-3659-2013; Ciubancan, Liviu Mihai/L-2412-2015; White, Ryan/E-2979-2015 OI Belanger-Champagne, Camille/0000-0003-2368-2617; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Pina, Joao /0000-0001-8959-5044; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Smirnova, Oxana/0000-0003-2517-531X; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Perrino, Roberto/0000-0002-5764-7337; SULIN, VLADIMIR/0000-0003-3943-2495; Veneziano, Stefano/0000-0002-2598-2659; Tikhomirov, Vladimir/0000-0002-9634-0581; Villa, Mauro/0000-0002-9181-8048; Warburton, Andreas/0000-0002-2298-7315; Brooks, William/0000-0001-6161-3570; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; De, Kaushik/0000-0002-5647-4489; Mitsou, Vasiliki/0000-0002-1533-8886; Grancagnolo, Sergio/0000-0001-8490-8304; Doyle, Anthony/0000-0001-6322-6195; Livan, Michele/0000-0002-5877-0062; spagnolo, stefania/0000-0001-7482-6348; Di Domenico, Antonio/0000-0001-8078-2759; Negrini, Matteo/0000-0003-0101-6963; Ferrando, James/0000-0002-1007-7816; Boyko, Igor/0000-0002-3355-4662; Ciubancan, Liviu Mihai/0000-0003-1837-2841; White, Ryan/0000-0003-3589-5900 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET; ERC; NSRF; European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; RGC, Hong Kong SAR, China; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia; NRC KI; Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, UK; Royal Society, UK; Leverhulme Trust, UK; DOE, USA; NSF, USA FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; RGC, Hong Kong SAR, China; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, UK; DOE and NSF, USA. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 49 TC 3 Z9 3 U1 6 U2 51 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JUL 2 PY 2015 VL 75 IS 7 AR 303 DI 10.1140/epjc/s10052-015-3500-z PG 33 WC Physics, Particles & Fields SC Physics GA CL9SH UT WOS:000357317900001 ER PT J AU Alekhin, S Behnke, O Belov, P Borroni, S Botje, M Britzger, D Camarda, S Cooper-Sarkar, AM Daum, K Diaconu, C Feltesse, J Gizhko, A Glazov, A Guffanti, A Guzzi, M Hautmann, F Jung, A Jung, H Kolesnikov, V Kowalski, H Kuprash, O Kusina, A Levonian, S Lipka, K Lobodzinski, B Lohwasser, K Luszczak, A Malaescu, B McNulty, R Myronenko, V Naumann-Emme, S Nowak, K Olness, F Perez, E Pirumov, H Placakyte, R Rabbertz, K Radescu, V Sadykov, R Salam, GP Sapronov, A Schoning, A Schorner-Sadenius, T Shushkevich, S Slominski, W Spiesberger, H Starovoitov, P Sutton, M Tomaszewska, J Turkot, O Vargas, A Watt, G Wichmann, K AF Alekhin, S. Behnke, O. Belov, P. Borroni, S. Botje, M. Britzger, D. Camarda, S. Cooper-Sarkar, A. M. Daum, K. Diaconu, C. Feltesse, J. Gizhko, A. Glazov, A. Guffanti, A. Guzzi, M. Hautmann, F. Jung, A. Jung, H. Kolesnikov, V. Kowalski, H. Kuprash, O. Kusina, A. Levonian, S. Lipka, K. Lobodzinski, B. Lohwasser, K. Luszczak, A. Malaescu, B. McNulty, R. Myronenko, V. Naumann-Emme, S. Nowak, K. Olness, F. Perez, E. Pirumov, H. Placakyte, R. Rabbertz, K. Radescu, V. Sadykov, R. Salam, G. P. Sapronov, A. Schoening, A. Schoerner-Sadenius, T. Shushkevich, S. Slominski, W. Spiesberger, H. Starovoitov, P. Sutton, M. Tomaszewska, J. Turkot, O. Vargas, A. Watt, G. Wichmann, K. TI HERAFitter SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID DEEP-INELASTIC-SCATTERING; HIGH-ENERGY FACTORIZATION; HEAVY FLAVOR PRODUCTION; UNINTEGRATED PARTON DISTRIBUTIONS; PRODUCTION CROSS-SECTION; INITIAL-STATE RADIATION; W LEPTON ASYMMETRY; SMALL-X; QCD ANALYSIS; PERTURBATION-THEORY AB HERAFitter is an open-source package that provides a framework for the determination of the parton distribution functions (PDFs) of the proton and for many different kinds of analyses in Quantum Chromodynamics (QCD). It encodes results from a wide range of experimental measurements in lepton-proton deep inelastic scattering and proton-proton (proton-antiproton) collisions at hadron colliders. These are complemented with a variety of theoretical options for calculating PDF-dependent cross section predictions corresponding to the measurements. The framework covers a large number of the existing methods and schemes used for PDF determination. The data and theoretical predictions are brought together through numerous methodological options for carrying out PDF fits and plotting tools to help to visualise the results. While primarily based on the approach of collinear factorisation, HERAFitter also provides facilities for fits of dipole models and transverse-momentum dependent PDFs. The package can be used to study the impact of new precise measurements from hadron colliders. This paper describes the general structure of HERAFitter and its wide choice of options. C1 [Alekhin, S.; Lohwasser, K.] Deutsch Elektronen Synchrotron DESY, D-15738 Zeuthen, Germany. [Alekhin, S.] Inst High Energy Phys, Protvino 142281, Moscow Region, Russia. [Behnke, O.; Belov, P.; Borroni, S.; Britzger, D.; Camarda, S.; Gizhko, A.; Glazov, A.; Guffanti, A.; Guzzi, M.; Jung, H.; Kowalski, H.; Kuprash, O.; Levonian, S.; Lipka, K.; Lohwasser, K.; Myronenko, V.; Naumann-Emme, S.; Nowak, K.; Pirumov, H.; Placakyte, R.; Radescu, V.; Schoerner-Sadenius, T.; Shushkevich, S.; Starovoitov, P.; Turkot, O.; Vargas, A.; Wichmann, K.] Deutsch Elektronen Synchrotron DESY, Hamburg, Germany. [Botje, M.] Nikhef, Amsterdam, Netherlands. [Cooper-Sarkar, A. M.; Nowak, K.] Univ Oxford, Dept Phys, Oxford, England. [Daum, K.] Univ Wuppertal, Fachbereich C, Wuppertal, Germany. [Daum, K.] Univ Wuppertal, Rechenzentrum, Wuppertal, Germany. [Diaconu, C.] Aix Marseille Univ, CNRS IN2P3, CPPM UMR 7346, F-13288 Marseille, France. [Feltesse, J.] CEA, DSM Irfu, CE Saclay, Gif Sur Yvette, France. [Guffanti, A.] Univ Copenhagen, Niels Bohr Inst, Niels Bohr Int Acad & Discovery Ctr, DK-2100 Copenhagen, Denmark. [Hautmann, F.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Hautmann, F.] Rutherford Appleton Lab, Chilton OX11 0QX, England. [Hautmann, F.] Univ Oxford, Dept Theoret Phys, Oxford OX1 3NP, England. [Jung, A.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Jung, H.] Univ Antwerp, Elementaire Deeltjes Fys, B-2020 Antwerp, Belgium. [Kolesnikov, V.; Sadykov, R.; Sapronov, A.] JINR, Dubna 141980, Moscow Region, Russia. [Kusina, A.; Olness, F.] So Methodist Univ, Dallas, TX 75275 USA. [Lobodzinski, B.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Luszczak, A.] T Kosciuszko Univ Technol, Krakow, Poland. [Malaescu, B.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Malaescu, B.] Univ Paris Diderot, Paris, France. [Malaescu, B.] CNRS IN2P3, Paris, France. [McNulty, R.] Univ Coll Dublin, Dublin 4, Ireland. [Perez, E.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Rabbertz, K.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Salam, G. P.] CERN, PH TH, CH-1211 Geneva 23, Switzerland. [Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Slominski, W.] Jagiellonian Univ, Inst Phys, PL-30059 Krakow, Poland. [Spiesberger, H.] Johannes Gutenberg Univ Mainz, Inst Phys WA THEP, PRISMA Cluster Excellence, D-55099 Mainz, Germany. [Sutton, M.] Univ Sussex, Dept Phys & Astron, Brighton BN1 9RH, E Sussex, England. [Tomaszewska, J.] Warsaw Univ Technol, Fac Phys, PL-00662 Warsaw, Poland. [Watt, G.] Univ Durham, Inst Particle Phys Phenomenol, Durham DH1 3LE, England. RP Alekhin, S (reprint author), Deutsch Elektronen Synchrotron DESY, Platanenallee 6, D-15738 Zeuthen, Germany. EM herafitter-help@desy.de; herafitter-help@desy.de RI Levonian, Sergey/M-8693-2015; Belov, Pavel/N-2871-2015; Guffanti, Alberto/A-6201-2016; OI Belov, Pavel/0000-0002-4004-7001; Guffanti, Alberto/0000-0001-6092-1221; Watt, Graeme/0000-0003-0775-6604 FU Helmholtz Alliance "Physics at the Terascale" of the Helmholtz Association; DESY IT department; H1 and ZEUS Collaborations; BMBF-JINR; Heisenberg-Landau program, the RFBR [12-02-91526-CERN a]; Polish NSC [DEC-2011/03/B/ST2/00220]; Initiative and Networking Fond of Helmholtz Association [SO-072] FX HERAFitter developers team acknowledges the kind hospitality of DESY and funding by the Helmholtz Alliance "Physics at the Terascale" of the Helmholtz Association. We are grateful to the DESY IT department for their support of the HERAFitter developers. We thank the H1 and ZEUS Collaborations for the support in the initial stage of the project. Additional support was received from the BMBF-JINR cooperation program, the Heisenberg-Landau program, the RFBR Grant 12-02-91526-CERN a, the Polish NSC project DEC-2011/03/B/ST2/00220 and a dedicated funding of the Initiative and Networking Fond of Helmholtz Association SO-072. We also acknowledge Nathan Hartland with Luigi Del Debbio for contributing to the implementation of the Bayesian Reweighting technique and would like to thank R. Thorne for fruitful discussions. NR 148 TC 25 Z9 25 U1 3 U2 5 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JUL 2 PY 2015 VL 75 IS 7 AR 304 DI 10.1140/epjc/s10052-015-3480-z PG 17 WC Physics, Particles & Fields SC Physics GA CL9SH UT WOS:000357317900002 ER PT J AU Wu, D Guo, XF Sun, H Navrotsky, A AF Wu, Di Guo, Xiaofeng Sun, Hui Navrotsky, Alexandra TI Thermodynamics of Methane Adsorption on Copper HKUST-1 at Low Pressure SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID METAL-ORGANIC FRAMEWORKS; CARBON-DIOXIDE; STORAGE; HYDROGEN; ENERGY; SIMULATION; EMISSIONS; DESIGN; OXIDES AB Metal-organic frameworks (MOFs) can be engineered as natural gas storage materials by tuning the pore structures and surface properties. Here we report the direct measurement of CH4 adsorption enthalpy on a paddlewheel MOF (Cu HKUST-1) using gas adsorption calorimetry at 25 degrees C at low pressures (below 1 bar). In this pressure region, the CH4-CH4 intermolecular interactions are minimized and the energetics solely reflects the CH4-MOF interactions. Our results suggest moderately exothermic physisorption with an enthalpy of -21.1 +/- 1.1 kJ/mol CH4 independent of coverage. This calorimetric investigation complements previous computational and crystallographic studies by providing zero coverage enthalpies of CH4 adsorption. The analysis of the new and literature data suggests that in initial stages of adsorption the CH4-HKUST-1 interaction tends to be more sensitive to the pore dimension than to the guest polarizability, suggesting a less specific chemical binding role for the open Cu site. C1 [Wu, Di; Guo, Xiaofeng; Navrotsky, Alexandra] Univ Calif Davis, Peter A Rock Thermochem Lab, Davis, CA 95616 USA. [Wu, Di; Guo, Xiaofeng; Navrotsky, Alexandra] Univ Calif Davis, NEAT ORU, Davis, CA 95616 USA. [Guo, Xiaofeng] Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. [Sun, Hui] E China Univ Sci & Technol, State Key Lab Chem Engn, Shanghai 200237, Peoples R China. RP Navrotsky, A (reprint author), Univ Calif Davis, Peter A Rock Thermochem Lab, One Shields Ave, Davis, CA 95616 USA. EM anavrotsky@ucdavis.edu RI Wu, Di/A-3039-2014 OI Wu, Di/0000-0001-6879-321X FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-FG02-05ER15667]; National Natural Science Foundation of China under National Natural Science Fund [21201063]; Ministry of Education of Republic of China under Research Fund for the Doctoral Program of Higher Education of China (RFDP) [20110074120020]; Fundamental Research Funds for the Central Universities; China Scholarship Council for the State Scholarship Fund [201308310077] FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Grant DE-FG02-05ER15667. H.S. thanks the National Natural Science Foundation of China for financial support under the National Natural Science Fund for Young Scholar (No. 21201063), the Ministry of Education of Republic of China for financial support under the Research Fund for the Doctoral Program of Higher Education of China (RFDP) (No. 20110074120020) and the Fundamental Research Funds for the Central Universities, and the China Scholarship Council for the State Scholarship Fund (No. 201308310077). We thank Manas K. Bhunia and James T. Hughes for providing the MOF material. NR 38 TC 2 Z9 2 U1 8 U2 49 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JUL 2 PY 2015 VL 6 IS 13 BP 2439 EP 2443 DI 10.1021/acs.jpclett.5b00893 PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CM4AN UT WOS:000357626700006 PM 26266715 ER PT J AU McCarthy, RF Schaller, RD Gosztola, DJ Wiederrecht, GP Martinson, ABF AF McCarthy, Robert F. Schaller, Richard D. Gosztola, David J. Wiederrecht, Gary P. Martinson, Alex B. F. TI Photoexcited Carrier Dynamics of In2S3 Thin Films SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID V-SUBSTITUTED IN2S3; INDIUM SULFIDE; INTERMEDIATE BAND; BUFFER LAYERS; CU(IN,GA)SE-2 AB Indium sulfide (In2S3) is a promising absorber base for substitutionally doped intermediate band photovoltaics (IBPV); however, the dynamics of charge carriers traversing the electronic density of states that determine the optical and electronic response of thin films under stimuli have yet to be explored. The kinetics of photophysical processes in In2S3 grown by oxygen-free atomic layer deposition are deduced from photoconductivity, photoluminescence (PL), and transient absorption spectroscopy. We develop a map of excited-state dynamics for polycrystalline thin films including a secondary conduction band similar to 2.1 eV above the first, plus sulfur vacancy and indium interstitial defect levels resulting in long-lived (similar to 100 ns) transients. Band-edge recombination produces PL and stimulated emission, which both intensify and red-shift as deposition temperature and grain size increase. The effect of rapid conduction band electron relaxation (<30 ps) and deep defect levels on IBPV employing In2S3-based absorbers is finally considered. C1 [McCarthy, Robert F.; Martinson, Alex B. F.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Schaller, Richard D.; Gosztola, David J.; Wiederrecht, Gary P.] Argonne Natl Lab, Nanosci & Technol Div, Argonne, IL 60439 USA. RP Martinson, ABF (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM martinson@anl.gov RI Gosztola, David/D-9320-2011; OI Gosztola, David/0000-0003-2674-1379; Martinson, Alex/0000-0003-3916-1672 FU U.S. Department of Energy [DE-AC02-06CH11357]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX Work at Argonne National Laboratory was supported under U.S. Department of Energy contract DE-AC02-06CH11357. Use of the Center for Nanoscale Materials, an Office of Science user facility, including resources in the Electron Microscopy Center, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract no. DE-AC02-06CH11357 NR 23 TC 4 Z9 4 U1 2 U2 18 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JUL 2 PY 2015 VL 6 IS 13 BP 2554 EP 2561 DI 10.1021/acs.jpclett.5b00935 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CM4AN UT WOS:000357626700024 PM 26266733 ER PT J AU Li, GL Cherqui, C Wu, YY Bigelow, NW Simmons, PD Rack, PD Masiello, DJ Camden, JP AF Li, Guoliang Cherqui, Charles Wu, Yueying Bigelow, Nicholas W. Simmons, Philip D. Rack, Philip D. Masiello, David J. Camden, Jon P. TI Examining Substrate-Induced Plasmon Mode Splitting and Localization in Truncated Silver Nanospheres with Electron Energy Loss Spectroscopy SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID ENHANCED RAMAN-SCATTERING; NANOPARTICLE ARRAYS; METAL NANOPARTICLES; GOLD NANOPARTICLES; SURFACE-PLASMONS; RESONANCE; TIO2; NANORODS; SEMICONDUCTOR; ABSORPTION AB Motivated by the need to study the size dependence of nanoparticle-substrate systems, we present a combined experimental and theoretical electron energy loss spectroscopy (EELS) study of the plasmonic spectrum of substrate-supported truncated silver nanospheres. This work spans the entire classical range of plasmonic behavior probing particles of 20-1000 nm in diameter, allowing us to map the evolution of localized surface plasmons into surface plasmon polaritons and study the size dependence of substrate-induced mode splitting. This work constitutes the first nanoscopic characterization and imaging of these effects in truncated nanospheres, setting the stage for the systematic study of plasmon-mediated energy transfer in nanoparticle-substrate systems. C1 [Li, Guoliang; Camden, Jon P.] Univ Notre Dame, Dept Chem & Biochem, Notre Dame, IN 46556 USA. [Cherqui, Charles; Bigelow, Nicholas W.; Masiello, David J.] Univ Washington, Dept Chem, Seattle, WA 98195 USA. [Wu, Yueying; Rack, Philip D.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Simmons, Philip D.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Rack, Philip D.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Masiello, DJ (reprint author), Univ Washington, Dept Chem, Seattle, WA 98195 USA. EM masiello@chem.washington.edu; jon.camden@nd.edu RI Li, Guoliang/M-6614-2014; OI Li, Guoliang/0000-0003-3798-8422; Rack, Philip/0000-0002-9964-3254 FU U.S. National Science Foundation [CHE-1253775]; U.S. National Science Foundation through XSEDE [PHY-130045]; National Science Foundation [CBET-1235651]; U.S. Department of Energy, Basic Energy Sciences [DE-SC0010536]; Notre Dame Energy postdoctoral fellowship FX This work was supported by the U.S. National Science Foundation's CAREER program under award number CHE-1253775 and through XSEDE resources under award number PHY-130045 (D.J.M., C.C., N.W.B.). This work is supported by National Science Foundation under grant number CBET-1235651 (P.D.R.). P.D.R. acknowledges that part of the pulsed laser-induced dewetting synthesis and dielectric constants measurements (measured with Dr. Bradley Lokitz) were performed at the Center for Nanophase Materials Science, which is a DOE Office of Science User Facility. This work was also supported by the U.S. Department of Energy, Basic Energy Sciences under award number DE-SC0010536 (J.P.C., G.L., Y.W.). G.L. was supported by a Notre Dame Energy postdoctoral fellowship. NR 62 TC 7 Z9 7 U1 5 U2 51 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JUL 2 PY 2015 VL 6 IS 13 BP 2569 EP 2576 DI 10.1021/acs.jpclett.5b00961 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CM4AN UT WOS:000357626700026 PM 26266735 ER PT J AU Grimaldo, M Roosen-Runge, F Hennig, M Zanini, F Zhang, FJ Zamponi, M Jalarvo, N Schreiber, F Seydel, T AF Grimaldo, Marco Roosen-Runge, Felix Hennig, Marcus Zanini, Fabio Zhang, Fajun Zamponi, Michaela Jalarvo, Niina Schreiber, Frank Seydel, Tilo TI Salt-Induced Universal Slowing Down of the Short-Time Self-Diffusion of a Globular Protein in Aqueous Solution SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID EQUILIBRIUM CLUSTERS; LYSOZYME SOLUTIONS; DISEASE; CRYSTALLIZATION; SCATTERING; DYNAMICS; CELLS AB The short-time self-diffusion D of the globular model protein bovine serum albumin in aqueous (D2O) solutions has been measured comprehensively as a function of the protein and trivalent salt (YCl3) concentration, noted c(p) and c(s), respectively. We observe that D follows a universal master curve D(c(s),c(p)) = D(c(s) = 0,c(p)) g(c(s)/c(p)), where D(c(s) = 0,c(p)) is the diffusion coefficient in the absence of salt and g(c(s)/c(p)) is a scalar function solely depending on the ratio of the salt and protein concentration. This observation is consistent with a universal scaling of the bonding probability in a picture of cluster formation of patchy particles. The finding corroborates the predictive power of the description of proteins as colloids with distinct attractive ion-activated surface patches. C1 [Grimaldo, Marco; Roosen-Runge, Felix; Hennig, Marcus; Seydel, Tilo] Inst Max von Laue Paul Langevin ILL, F-38042 Grenoble, France. [Grimaldo, Marco; Hennig, Marcus; Zanini, Fabio; Zhang, Fajun; Schreiber, Frank] Univ Tubingen, Inst Angew Phys, D-72076 Tubingen, Germany. [Zamponi, Michaela; Jalarvo, Niina] Forschungszentrum Julich, JCNS, D-52425 Julich, Germany. [Zamponi, Michaela] MLZ, JCNS Outstn, D-85747 Garching, Germany. [Jalarvo, Niina] Oak Ridge Natl Lab, Neutron Sci Directorate, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Jalarvo, Niina] Oak Ridge Natl Lab, JCNS Outstn, SNS, Oak Ridge, TN 37831 USA. RP Seydel, T (reprint author), Inst Max von Laue Paul Langevin ILL, CS 20156,71 Ave Martyrs, F-38042 Grenoble, France. EM seydel@ill.eu RI Roosen-Runge, Felix/A-9107-2013; Schreiber, Frank/J-3311-2014; Jalarvo, Niina/Q-1320-2015 OI Roosen-Runge, Felix/0000-0001-5106-4360; Schreiber, Frank/0000-0003-3659-6718; Jalarvo, Niina/0000-0003-0644-6866 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Julich Center for Neutron Science (JCNS), Germany; JCNS; Institut Laue-Langevin (ILL); ILL; DFG FX The research at Oak Ridge National Laboratory's Spoliation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. The spectrometer BASIS is supported by the Julich Center for Neutron Science (JCNS), Germany, via the partner user programme and M.G. and F.Za. acknowledge travel funding by JCNS to conduct the experiments as well as a student grant by the Institut Laue-Langevin (ILL). M.H., M.G. and T.S. have obtained travel funding by ILL to conduct the experiments. We acknowledge E. Mamontov, M. Oettel, R. Roth, and H. Schober for fruitful discussions and R Moody and V. Glenisson for assistance. We further acknowledge financial support by the DFG. NR 42 TC 2 Z9 2 U1 1 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JUL 2 PY 2015 VL 6 IS 13 BP 2577 EP 2582 DI 10.1021/acs.jpclett.5b01073 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CM4AN UT WOS:000357626700027 PM 26266736 ER PT J AU Arslan, I Roehling, JD Ogino, I Batenburg, KJ Zones, SI Gates, BC Katz, A AF Arslan, Ilke Roehling, John D. Ogino, Isao Batenburg, K. Joost Zones, Stacey I. Gates, Bruce C. Katz, Alexander TI Genesis of De laminated-Zeolite Morphology: 3-D Characterization of Changes by STEM Tomography SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID EXTRA-LARGE-PORE; CATALYTIC APPLICATIONS; MESOPOROUS MATERIALS; DELAMINATED ZEOLITE; MOLECULAR-SIEVES; CRYSTALLINE; PRECURSORS; NANOSHEETS; MICRO AB Zeolite delamination increases the external surface area available for catalyzing the conversion of bulky molecules, but a fundamental understanding of the delamination process remains unknown. Here we report morphological changes accompanying delamination on the length scale of individual zeolite clusters determined by 3-D imaging in scanning transmission electron microscopy. The results are tomograms that demonstrate delamination as it proceeds on the nanoscale through two distinct key steps: a chemical treatment that leads to a swelled material and a subsequent calcination that leads to curling and peeling off of delaminated zeolite sheets over hundreds of nanometers. These results characterize the direct, local, 3-D morphological changes accompanying delaminated materials synthesis and, with corroboration by mercury porosimetry, provide unique insight into the morphology of these materials, which is difficult to obtain with any other technique. C1 [Arslan, Ilke] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. [Roehling, John D.; Gates, Bruce C.] Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA. [Ogino, Isao; Katz, Alexander] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Batenburg, K. Joost] Ctr Wiskunde & Informat, NL-1098 XG Amsterdam, Netherlands. [Zones, Stacey I.] Chevron Energy Technol Co, Richmond, CA 94804 USA. RP Arslan, I (reprint author), Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, 902 Battelle Blvd, Richland, WA 99352 USA. EM ilke.arslan@pnnl.gov FU U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences [DE-SC0005822]; LDRD program at the Pacific Northwest National Laboratory (PNNL); Department of Energy's Office of Biological and Environmental Research; DOE [DE-AC05-76RL01830] FX We acknowledge support from the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Grant DE-SC0005822, and the LDRD program at the Pacific Northwest National Laboratory (PNNL). The experiments were performed in the Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at PNNL. PNNL is operated by Battelle for the DOE under contract DE-AC05-76RL01830. NR 31 TC 0 Z9 0 U1 8 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JUL 2 PY 2015 VL 6 IS 13 BP 2598 EP 2602 DI 10.1021/acs.jpclett.5b01004 PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CM4AN UT WOS:000357626700031 PM 26266740 ER PT J AU McFarland, HL Ahmed, T Zhu, JX Balatsky, AV Haradsen, JT AF McFarland, Hannah L. Ahmed, Towfiq Zhu, Jian-Xin Balatsky, Alexander V. Haradsen, Jason T. TI First-Principles Investigation of Nanopore Sequencing Using Variable Voltage Bias on Graphene-Based Nanoribbons SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID SINGLE DNA-MOLECULES; HUMAN-GENOME-PROJECT; CANCER; METHYLATION AB In this study, we examine the mechanism of nanopore-based DNA sequencing using a voltage bias across a graphene nanoribbon. Using density function theory and a nonequilibrium Green's function approach, we determine the transmission spectra and current profile for adenine, guanine, cytosine, thymine, and uracil as a function of bias voltage in an energy minimized configuration. Utilizing the transmission current, we provide a general methodology for the development of a three nanopore graphene-based device that can be used to distinguish between the various nucleobases for DNA/RNA sequencing. From our analysis, we deduce that it is possible to use different transverse currents across a multinanopore device to differentiate between nucleobases using various voltages of 0.5, 1.3, and 1.6 V. Overall, our goal is to improve nanopore design to further DNA/RNA nucleobase sequencing and biomolecule identification techniques. C1 [McFarland, Hannah L.] James Madison Univ, Dept Biol, Harrisonburg, VA 22802 USA. [Ahmed, Towfiq; Zhu, Jian-Xin] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Zhu, Jian-Xin] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Balatsky, Alexander V.] Los Alamos Natl Lab, Inst Mat Sci, Los Alamos, NM 87545 USA. [Balatsky, Alexander V.] KTH Royal Inst Technol, Nord Inst Theoret Phys, S-10691 Stockholm, Sweden. [Balatsky, Alexander V.] Stockholm Univ, S-10691 Stockholm, Sweden. [Haradsen, Jason T.] James Madison Univ, Dept Phys & Astron, Harrisonburg, VA 22802 USA. RP Haradsen, JT (reprint author), James Madison Univ, Dept Phys & Astron, Harrisonburg, VA 22802 USA. EM j.t.haraldsen@unf.edu FU James Madison University; U.S. DOE; NNSA [DEAC52-06NA25396]; U.S. DOE Basic Energy Sciences Office; Center for Integrated Nanotechnologies, a U.S. DOE Office of Basic Energy Sciences; ERC [DM 321031]; Knut and Alice Wallenberg (KAW) foundation FX H.L.M. and J.T.H. thank the support of James Madison University and useful discussions with J.-H. Kim. The work at Los Alamos National Laboratory was ad out under the auspice of the U.S. DOE and NNSA under Contract No. DEAC52-06NA25396 and supported by U.S. DOE Basic Energy Sciences Office (T.A. and A.V.B.). This work was also, in part, supported by the Center for Integrated Nanotechnologies, a U.S. DOE Office of Basic Energy Sciences user facility (J.-X.Z). Work at the Nordic Institute for Theoretical Physics was supported by ERC DM 321031 and the Knut and Alice Wallenberg (KAW) foundation. NR 39 TC 4 Z9 4 U1 5 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JUL 2 PY 2015 VL 6 IS 13 BP 2616 EP 2621 DI 10.1021/acs.jpclett.5b01014 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CM4AN UT WOS:000357626700034 PM 26266743 ER PT J AU Fulton, JL Govind, N Huthwelker, T Bylaska, EJ Vjunov, A Pin, S Smurthwaite, TD AF Fulton, John L. Govind, Niranjan Huthwelker, Thomas Bylaska, Eric J. Vjunov, Aleksei Pin, Sonia Smurthwaite, Tricia D. TI Electronic and Chemical State of Aluminum from the Single- (K) and Double-Electron Excitation (KLII&III, KLI) X-ray Absorption Near-Edge Spectra of alpha-Alumina, Sodium Aluminate, Aqueous Al3+center dot(H2O)(6), and Aqueous Al(OH)(4)(-) SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID NORM-CONSERVING PSEUDOPOTENTIALS; FINE-STRUCTURE; MULTIELECTRON EXCITATIONS; THEORETICAL-ANALYSIS; MOLECULAR-DYNAMICS; SPECTROSCOPY; DENSITY; CL; CHANNELS; ELEMENTS AB We probe, at high energy resolution, the double electron excitation (KLII&II) X-ray absorption region that lies approximately 115 eV above the main Al K-edge (1566 eV) of alpha-alumina and sodium aluminate. The two solid standards, alpha-alumina (octahedral) and sodium aluminate (tetrahedral), are compared to aqueous species that have the same Al coordination symmetries, Al3+center dot 6H(2)O (octahedral) and Al(OH)(4)(-) (tetrahedral). For the octahedral species, the edge height of the KLII&III-edge is approximately 10% of the main K-edge; however, the edge height is much weaker (3% of K-edge height) for Al species with tetrahedral symmetry. For the a-alumina and aqueous Al3+center dot 6H(2)O the KLII&III spectra contain white line features and extended absorption fine structure (EXAFS) that mimics the K-edge spectra. The KLII&III-edge feature interferes with an important region in the EXAFS spectra of the crystalline and aqueous standards. The K-edge spectra and K-edge energy positions are predicted using time-dependent density functional theory (TDDFT). The TDDFT calculations for the K-edge X-ray absorption near-edge spectra (XANES) reproduce the observed transitions in the experimental spectra of the four Al species. The KLII&II and KLI onsets and their corresponding chemical shifts for the four standards are estimated using the delta self-consistent field (Delta SCF) method. C1 [Fulton, John L.] Pacific NW Natl Lab, Phys Sci Div, Richland, WA 99352 USA. [Govind, Niranjan; Bylaska, Eric J.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Vjunov, Aleksei] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. [Smurthwaite, Tricia D.] Pacific NW Natl Lab, Energy Proc & Mat, Richland, WA 99352 USA. [Huthwelker, Thomas; Pin, Sonia] Paul Scherrer Inst, Lab Catalysis & Sustainable Chem LSK, Swiss Light Source, CH-5232 Villigen, Switzerland. RP Fulton, JL (reprint author), Pacific NW Natl Lab, Phys Sci Div, POB 999, Richland, WA 99352 USA. EM john.fulton@pnnl.gov; niri.govind@pnnl.gov FU U.S. Department of Energy's (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences; U.S. Department of Energy's Office of Biological and Environmental Research; DOE [DE-AC06-76RL0-1830] FX The Al XAFS measurements were performed at the PHOENIX beamline of the Swiss Light Source, Paul Scherrer Institute, Villigen, Switzerland. Research by J.L.F., N.G., E.J.B., A.V., and T.D.S. was supported by U.S. Department of Energy's (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences. N.G. thanks Amity Andersen for help with the alpha-Al2O3 and tetrahedral sodium aluminate (NaAlO2) clusters. All the calculations were performed using the Molecular Science Computing Capability at EMSL, a national scientific user facility sponsored by the U.S. Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). PNNL is a multiprogram national laboratory operated for DOE by Battelle Memorial Institute under Contract # DE-AC06-76RL0-1830. NR 59 TC 3 Z9 3 U1 3 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JUL 2 PY 2015 VL 119 IS 26 BP 8380 EP 8388 DI 10.1021/jp511602n PG 9 WC Chemistry, Physical SC Chemistry GA CM3ZG UT WOS:000357623400016 PM 26036606 ER PT J AU March, AM Assefa, TA Bressler, C Doumy, G Galler, A Gawelda, W Kanter, EP Nemeth, Z Papai, M Southworth, SH Young, L Vanko, G AF March, Anne Marie Assefa, Tadesse A. Bressler, Christian Doumy, Gilles Galler, Andreas Gawelda, Wojciech Kanter, Elliot P. Nemeth, Zoltan Papai, Matyas Southworth, Stephen H. Young, Linda Vanko, Gyoergy TI Feasibility of Valence-to-Core X-ray Emission Spectroscopy for Tracking Transient Species SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID EXCITED-STATE CHEMISTRY; METAL-LIGAND COVALENCY; ABSORPTION SPECTROSCOPY; ELECTRONIC EXCITATIONS; COORDINATION-COMPLEXES; FERROCYANIDE ION; AQUEOUS-SOLUTION; IRON COMPLEXES; DIRECT PROBE; IDENTIFICATION AB X-ray spectroscopies, when combined in laser-pump, X-ray-probe measurement schemes, can be powerful tools for tracking the electronic and geometric structural changes that occur during the course of a photoinitiated chemical reaction. X-ray absorption spectroscopy (XAS) is considered an established technique for such measurements, and X-ray emission spectroscopy (XES) of the strongest core-to-core emission lines (K alpha and K beta) is now being utilized. Flux demanding valence-to-core XES promises to be an important addition to the time-resolved spectroscopic toolkit. In this paper we present measurements and density functional theory calculations on laser-excited, solution-phase ferrocyanide that demonstrate the feasibility of valence-to-core XES for time-resolved experiments. We discuss technical improvements that will make valence-to-core XES a practical pump-probe technique. C1 [March, Anne Marie; Doumy, Gilles; Kanter, Elliot P.; Southworth, Stephen H.; Young, Linda] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Assefa, Tadesse A.; Bressler, Christian; Galler, Andreas; Gawelda, Wojciech] European XFEL, D-22761 Hamburg, Germany. [Bressler, Christian] Hamburg Ctr Ultrafast Imaging, D-22761 Hamburg, Germany. [Nemeth, Zoltan; Papai, Matyas; Vanko, Gyoergy] Hungarian Acad Sci, Wigner Res Ctr Phys, H-1525 Budapest, Hungary. RP March, AM (reprint author), Argonne Natl Lab, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM arnarch@anl.gov; vanko.gyorgy@wigner.mta.hu RI Vanko, Gyorgy/B-8176-2012; Gawelda, Wojciech/B-7878-2014; OI Vanko, Gyorgy/0000-0002-3095-6551; Gawelda, Wojciech/0000-0001-7824-9197; Papai, Matyas Imre/0000-0002-4819-0611 FU European Research Council [ERC-StG-259709]; Hungarian Academy of Sciences; European XFEL; Deutsche Forschungsgemeinschaft [SFB925]; Hamburg Centre of Ultrafast Imaging; U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES) [DE-AC02-06CH11357]; DOE Office of Science [DE-AC02-06CH11357] FX This project was supported by the European Research Council via contract ERC-StG-259709, the 'Lendulet' (Momentum) Program of the Hungarian Academy of Sciences, and the European XFEL. Z.N. acknowledges support from the Bolyai Fellowship of the Hungarian Academy of Sciences. W.G., T. A., A.G., and C. B. acknowledge funding by the Deutsche Forschungsgemeinschaft via SFB925 and by the Hamburg Centre of Ultrafast Imaging. Work by A.M.M., G.D., L.Y., E.P.K., and S.H.S was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), under Contract No. DE-AC02-06CH11357. This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 71 TC 13 Z9 13 U1 17 U2 52 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 2 PY 2015 VL 119 IS 26 SI SI BP 14571 EP 14578 DI 10.1021/jp511838q PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CM3ZH UT WOS:000357623500013 ER PT J AU Biswas, M Libera, JA Darling, SB Elam, JW AF Biswas, Mahua Libera, Joseph A. Darling, Seth B. Elam, Jeffrey W. TI Kinetics for the Sequential Infiltration Synthesis of Alumina in Poly(methyl methacrylate): An Infrared Spectroscopic Study SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ATOMIC LAYER DEPOSITION; BLOCK-COPOLYMERS; FILMS; TRIMETHYLALUMINUM; POLYSTYRENE; POLYMERS; FTIR; PMMA AB Sequential infiltration synthesis (SIS) is a method for growing inorganic materials within polymers in an atomically controlled fashion. This technique can increase the etch resistance of optical, electron-beam, and block copolymer (BCP) lithography resists and is also a flexible strategy for nanomaterials synthesis. Despite this broad utility, the kinetics of SIS remain poorly understood, and this knowledge gap must be bridged in order to gain firm control over the growth of inorganic materials inside polymer films at a large scale. In this paper, we explore the reaction kinetics for Al2O3 SIS in PMMA using in situ Fourier transform infrared spectroscopy. First, we establish the kinetics for saturation adsorption and desorption of trimethyl aluminum (TMA) in PMMA over a range of PMMA film thicknesses deposited on silicon substrates. These observations guide the selection of TMA dose and purge times during SIS lithography to achieve robust organic/inorganic structures. Next, we examine the effects of TMA desorption on BCP lithography by performing SIS on silicon surfaces coated with polystyrene-block-poly(methyl methacrylate) films. After etching the organic components, the substrates are examined using scanning electron microcopy to evaluate the resulting Al2O3 patterns. Finally, we examine the effects of temperature on Al2O3 SIS in PMMA. to elucidate the infiltration kinetics. The insights provided by these measurements will help extend SIS lithography to larger substrate sizes for eventual commercialization and expand our knowledge of precursor polymer interactions that will benefit the SIS of a wide range of inorganic materials in the future. C1 [Biswas, Mahua; Libera, Joseph A.; Elam, Jeffrey W.] Argonne Natl Lab, Energy Syst Div, Argonne, IL 60439 USA. [Darling, Seth B.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Darling, Seth B.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. RP Darling, SB (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. EM darling@anl.gov; jelam@anl.gov FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Technology Maturation Grant through the Technology Development and Commercialization Division at Argonne FX Use of the Center for Nanoscale Materials was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. The authors want to thank Dr. Wei Chen from Materials Science Division, Argonne National Laboratory for providing PS-r-PMMA polymer. The authors gratefully acknowledge support from a Technology Maturation Grant through the Technology Development and Commercialization Division at Argonne. NR 26 TC 11 Z9 11 U1 6 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 2 PY 2015 VL 119 IS 26 SI SI BP 14585 EP 14592 DI 10.1021/jp511939j PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CM3ZH UT WOS:000357623500015 ER PT J AU Eren, B Lichtenstein, L Wu, CH Bluhm, H Somorjai, GA Salmeron, M AF Eren, Baran Lichtenstein, Leonid Wu, Cheng Hao Bluhm, Hendrik Somorjai, Gabor A. Salmeron, Miquel TI Reaction of CO with Preadsorbed Oxygen on Low-Index Copper Surfaces: An Ambient Pressure X-ray Photoelectron Spectroscopy and Scanning Tunneling Microscopy Study SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID IN-SITU; CARBON-MONOXIDE; OXIDATION; CU(110); ADSORPTION; STM; RECONSTRUCTION; CHEMISTRY; DYNAMICS; CATALYST AB The reaction of CO with chemisorbed oxygen on three low-index faces of copper was studied using ambient pressure X-ray photoelectron spectroscopy (XPS) and high-pressure scanning tunneling microscopy. At room temperature, the chemisorbed oxide can be removed by reaction with gas-phase CO in the 0.01-0.20 Torr pressure range. The reaction rates were determined by measuring the XPS peak intensities of O and CO as a function of time, pressure, and temperature. On Cu(111) the rate was found to be one order of magnitude faster than that on Cu(100) and two orders of magnitude faster than that on Cu(110). The apparent activation energies for CO oxidation were measured as 0.24 eV for O/Cu(111), 0.29 eV for O/Cu(100), and 0.51 eV for O/Cu(110) in the temperature range between 298 and 473 K. These energies are correlated to the oxygen binding energies on each surface. C1 [Eren, Baran; Lichtenstein, Leonid; Wu, Cheng Hao; Salmeron, Miquel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Bluhm, Hendrik; Somorjai, Gabor A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Wu, Cheng Hao; Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Salmeron, Miquel] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Salmeron, M (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM mbsalmeron@lbl.gov RI Eren, Baran/A-9644-2013 FU Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering, of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231]; Swiss National Research Funds (SNF); Alexander von Humboldt Foundation; ALS Doctoral Fellowship in Residence FX This work was supported by the Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering, of the U.S. Department of Energy (DOE) under Contract DE-AC02-05CH11231, through the Chemical and Mechanical Properties of Surfaces, Interfaces and Nanostructures program. B.E. acknowledges the Early Postdoc Mobility fellowship from the Swiss National Research Funds (SNF). L.L. acknowledges support by the Alexander von Humboldt Foundation. C.H.W. acknowledges the ALS Doctoral Fellowship in Residence. NR 35 TC 15 Z9 15 U1 11 U2 59 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 2 PY 2015 VL 119 IS 26 SI SI BP 14669 EP 14674 DI 10.1021/jp512831f PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CM3ZH UT WOS:000357623500022 ER PT J AU Ford, DC Zapol, P Cooley, LD AF Ford, Denise C. Zapol, Peter Cooley, Lance D. TI First-Principles Study of Carbon and Vacancy Structures in Niobium SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID BCC TRANSITION-METALS; AUGMENTED-WAVE METHOD; ALPHA-IRON; DIFFUSION; SUPERCONDUCTIVITY; HYDROGEN; CARBIDE; DENSITY; ENERGY; MIGRATION AB The interstitial chemical impurities hydrogen, oxygen, nitrogen, and carbon are important for niobium metal production and particularly for the optimization of niobium SRF technology. These atoms are present in refined sheets and can be absorbed into niobium during processing treatments, resulting in changes to the residual resistance and the performance of SRF cavities. A first-principles approach is taken to study the properties of carbon in niobium, and the results are compared and contrasted with the properties of the other interstitial impurities. The results indicate that C will likely form precipitates or atmospheres around defects rather than strongly bound complexes with other impurities. On the basis of the analysis of carbon and hydrogen near niobium lattice vacancies and small vacancy chains and clusters, the formation of extended carbon chains and hydrocarbons is not likely to occur. Association of carbon with hydrogen atoms can, however, occur through the strain fields created by interstitial binding of the impurity atoms. Calculated electronic densities of states indicate that interstitial C may have a similar effect as interstitial O on the superconducting transition temperature of Nb. C1 [Ford, Denise C.; Zapol, Peter] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Cooley, Lance D.] Fermilab Natl Accelerator Lab, Tech Div, Batavia, IL 60510 USA. RP Cooley, LD (reprint author), Fermilab Natl Accelerator Lab, Tech Div, Mail Stop 315,POB 500, Batavia, IL 60510 USA. EM ldcooley@fnal.gov OI Cooley, Lance/0000-0003-3488-2980 FU [DE-AC02-06CH11357] FX We acknowledge computer resources from Fermilab, Argonne LCRC, and Argonne Center for Nanoscale Materials. Argonne National Laboratory, a U.S. Department of Energy Office of Science laboratory, is operated under contract no. DE-AC02-06CH11357. NR 62 TC 0 Z9 0 U1 4 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 2 PY 2015 VL 119 IS 26 SI SI BP 14728 EP 14736 DI 10.1021/acs.jpcc.5b00372 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CM3ZH UT WOS:000357623500030 ER PT J AU Nakayama, M Xue, M An, W Liu, P White, MG AF Nakayama, Mild Xue, Meng An, Wei Liu, Ping White, Michael G. TI Influence of Cluster-Support Interactions on Reactivity of Size-Selected NbxOy Clusters SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID WATER-GAS SHIFT; METAL-OXIDE CLUSTERS; OXYGEN-INDUCED RECONSTRUCTIONS; SCANNING-TUNNELING-MICROSCOPY; TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; NIOBIUM OXIDE; ELECTRONIC-STRUCTURE; HYDROGEN-PRODUCTION; CU(110) SURFACE AB Size-selected niobium Oxide nanoclusters (Nb3O5, Nb3O7, Nb4O7, and Nb4O10) were deposited at room temperature onto a Cu(111) surface and a thin film of Cu2O on Cu(111), and their interfacial electronic interactions and reactivity toward water dissociation were examined. These clusters were specifically chosen to elucidate the effects of the oxidation state of the metal centers; Nb3O5 and Nb4O7 are the reduced counterparts of Nb3O7 and Nb4O10, respectively. From two-photon photoemission spectroscopy (2PPE) measurements, we found that the work function increases upon cluster adsorption in all cases, indicating a negative interfacial dipole moment with the positive end pointing into the surface. The amount of increase was greater for the clusters with more metal centers and higher oxidation state. Further analysis with DFT calculations of the clusters on Cu(111) indicated that the reduced clusters donate electrons to the substrate, indicating that the intrinsic cluster dipole moment makes a larger contribution to the overall interfacial dipole moment than charge transfer. X-ray photoelectron spectroscopy (XPS) measurements showed that the Nb atoms of Nb3O7 and Nb4O10 are primarily Nb5+ on Cu(111), while for the reduced Nb3O5 and Nb4O7 clusters, a mixture of oxidation states was observed on Cu(111). Temperature-programmed desorption (TPD) experiments with D2O showed that water dissociation occurred on all systems except for the oxidized Nb3O7 and Nb4O10 clusters on the Cu2O film. A comparison of our XPS and TPD results suggests that Nb5+ cations associated with Nb=O terminal groups act as Lewis acid sites which are key for water binding and subsequent dissociation. TPD measurements of 2-propanol dehydration also show that the clusters active toward water dissociation are indeed acidic. DFT calculations of water dissociation on Nb3O7 support our TPD results, but the use of bulk Cu2O(111) as a model for the Cu2O film merits future scrutiny in terms of interfacial charge transfer. The combination of our experimental and theoretical results suggests that both Lewis acidity and metal reducibility are important for water dissociation. C1 [Nakayama, Mild; An, Wei; Liu, Ping; White, Michael G.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11974 USA. [Xue, Meng; White, Michael G.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. RP White, MG (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11974 USA. EM mgwhite@bnl.gov FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10086] FX This work was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract DE-AC02-98CH10086. The DFT calculations were performed using computational resources at the Center for Functional Nanomaterials which is a DOE Office of Science User Facility located at Brookhaven National Laboratory. M.N. graciously acknowledges Prof. Sibener's guidance and support throughout her graduate studies at the University of Chicago. NR 86 TC 4 Z9 4 U1 7 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 2 PY 2015 VL 119 IS 26 SI SI BP 14756 EP 14768 DI 10.1021/acs.jpcc.5b00691 PG 13 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CM3ZH UT WOS:000357623500034 ER PT J AU Farina, R Laugel, N Yu, J Tirrell, M AF Farina, Robert Laugel, Nicolas Yu, Jing Tirrell, Matthew TI Reversible Adhesion with Polyelectrolyte Brushes Tailored via the Uptake and Release of Trivalent Lanthanum Ions SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID AMPHIPHILIC DIBLOCK COPOLYMERS; POLYMER BRUSHES; MULTIVALENT COUNTERIONS; ADSORPTION MECHANISMS; ELECTROLYTE-SOLUTIONS; FORCES; SURFACES; LUBRICATION; INTERFACE; BEHAVIOR AB Applications of end-tethered polyelectrolyte "brushes" to modify solid surfaces have been developed and studied for their colloidal stabilization and high lubrication properties. Current efforts have expanded into biological realms and stimuli-responsive materials. Our work explores responsive and reversible aspects of polyelectrolyte brush behavior when polyelectrolyte chains interact with oppositely charged multivalent ions and complexes, which act as counterions. There is a significant void in the polyelectrolyte literature regarding interactions with multivalent species. This paper demonstrates that interactions between solid surfaces bearing negatively charged polyelectrolyte brushes are highly sensitive to the presence of trivalent lanthanum, La3+. Lanthanum cations have unique interactions with polyelectrolyte chains, in part due to their small size and hydration radius which results in a high local charge density. Using La3+ in conjunction with the surface forces apparatus (SFA), adhesion has been observed to reversibly appear and disappear upon the uptake and release, respectively, of these multivalent cations acting as counterions. In media of fixed ionic strength set by monovalent sodium salt, at I-0 = 0.003 M and I-0 = 0.3 M, the sign of the interaction forces between overlapping brushes changes from repulsive to attractive when La3+ concentrations reach 0.1 mol % of the total ion concentration. These results are also shown to be generally consistent with, but subtlety different from, previous polyelectrolyte brush experiments using trivalent ruthenium hexamine in the role of the multivalent counterion. C1 [Farina, Robert; Laugel, Nicolas] Univ Calif Santa Barbara, Dept Chem Engn, Santa Barbara, CA 93106 USA. [Yu, Jing; Tirrell, Matthew] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. [Yu, Jing; Tirrell, Matthew] Argonne Natl Lab, Inst Mol Engn, Argonne, IL 60439 USA. RP Tirrell, M (reprint author), Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. EM mtirrell@uchicago.edu RI Yu, Jing/C-4138-2017 OI Yu, Jing/0000-0002-4288-951X FU U.S. Department of Energy, Office of Science, Program in Basic Energy Sciences, Division of Materials Science and Engineering FX We gratefully acknowledge the contribution of Ms. Cui Fan to some of the experimental work reported here. This work was supported by the U.S. Department of Energy, Office of Science, Program in Basic Energy Sciences, Division of Materials Science and Engineering. NR 44 TC 6 Z9 6 U1 6 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 2 PY 2015 VL 119 IS 26 SI SI BP 14805 EP 14814 DI 10.1021/acs.jpcc.5b02121 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CM3ZH UT WOS:000357623500038 ER PT J AU Martin, LB Rutqvist, J Birkholzer, JT AF Martin, Laura Blanco Rutqvist, Jonny Birkholzer, Jens T. TI Long-term modeling of the thermal-hydraulic-mechanical response of a generic salt repository for heat-generating nuclear waste SO ENGINEERING GEOLOGY LA English DT Article DE Nuclear waste disposal; Natural salt; Crushed salt; Large strains; Numerical modeling; Coupled processes ID ROCK-SALT; CONSTITUTIVE MODEL; POROUS SOLIDS; COUPLED FLOW; GEOMECHANICS; PERMEABILITY; DEFORMATION; CONVERGENCE; FORMULATION; SIMULATION AB A modeling effort has been undertaken to investigate the long-term response of a generic salt repository for heat-generating nuclear waste, including processes that could affect the geological (natural salt host rock) and geotechnical (backfill) barriers. For this purpose, the TOUGH-FLAC sequential simulator for coupled thermal hydraulic mechanical processes modeling has recently been provided with a capability for large strains and creep. The responses of the saliferous host rock and the crushed salt backfill are modeled using dedicated constitutive relationships. Similarly, the coupling between the geomechanics and the flow sub-problems is performed on the basis of theoretical and experimental studies. The repository investigated in this work considers in-drift emplacement of the waste packages and subsequent backfill of the drifts with run-of-mine salt. Using the updated TOUGH-FLAC, the compaction of the bacicfill and the evolution of its properties as porosity decreases can be modeled. Additionally, different processes that may influence the initial tightness of the host rock can be investigated. On the basis of state-of-the-art phenomenological models, our simulation results show that, in order to evaluate the barriers integrity, it is necessary to consider full coupling between thermal, hydraulic and mechanical processes. A base case scenario that accounts for these coupled processes is presented and compared to a case in which the mechanical processes are disregarded. Also, we investigate the sensitivity of the coupled numerical predictions to two factors: the initial saturation within the host rock and the capillary forces. Although the outcome of these simulations is preliminary and will be improved as the understanding of relevant processes moves forward, the numerical tools required to perform the target predictions have been significantly improved. (C) 2015 Elsevier B.V. All rights reserved. C1 [Martin, Laura Blanco; Rutqvist, Jonny; Birkholzer, Jens T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Martin, LB (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, 1 Cyclotron Rd,MS 74R316C, Berkeley, CA 94720 USA. EM lblancomartin@lbl.gov; jrutqvist@lbl.gov; jtbirkholzer@lbl.gov RI Birkholzer, Jens/C-6783-2011; Rutqvist, Jonny/F-4957-2015; Blanco Martin, Laura/G-1512-2015 OI Birkholzer, Jens/0000-0002-7989-1912; Rutqvist, Jonny/0000-0002-7949-9785; Blanco Martin, Laura/0000-0003-1794-3227 FU Used Fuel Disposition Campaign, Office of Nuclear Energy of the U.S. Department of Energy [DE-AC02-05CH11231]; Lawrence Berkeley National Laboratory FX The authors gratefully acknowledge Stefan Finsterle and Victor Vilarrasa for their careful review of a draft manuscript. The cooperation with Prof. Lux's team at the Department of Waste Disposal and Geomechanics, Clausthal University of Technology, is kindly appreciated. The constructive comments issued from the anonymous review process have significantly improved the quality of this paper. Funding for this work has been provided by the Used Fuel Disposition Campaign, Office of Nuclear Energy of the U.S. Department of Energy, under Contract Number DE-AC02-05CH11231 with Lawrence Berkeley National Laboratory. NR 92 TC 5 Z9 5 U1 0 U2 17 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0013-7952 EI 1872-6917 J9 ENG GEOL JI Eng. Geol. PD JUL 2 PY 2015 VL 193 BP 198 EP 211 DI 10.1016/j.enggeo.2015.04.014 PG 14 WC Engineering, Geological; Geosciences, Multidisciplinary SC Engineering; Geology GA CM0EA UT WOS:000357350000016 ER PT J AU Zhu, L Gong, HL Li, XJ Wang, R Chen, BB Dai, ZX Teatini, P AF Zhu, Lin Gong, Huili Li, Xiaojuan Wang, Rong Chen, Beibei Dai, Zhenxue Teatini, Pietro TI Land subsidence due to groundwater withdrawal in the northern Beijing plain, China SO ENGINEERING GEOLOGY LA English DT Article DE Land subsidence; Groundwater level; Compressible layer; Building; PSI; GIS ID XI-CHANG AREA; SCATTERER SAR INTERFEROMETRY; RADAR INTERFEROMETRY; YANGTZE DELTA; DEFORMATION; SYSTEM; SIMULATION; CITY; COMPRESSIBILITY; DISPLACEMENTS AB Beijing is an international metropolis, where over-exploration of water resource makes land subsidence becoming more and more serious. The related problems cannot be avoided in the coming years because of the giant increase of population. The aims of this study are to quantify land subsidence over the period 2003 to 2010, grasp the evolution of the process, and investigate the relation with the triggering factors in the northern area of the Beijing plain. Various data, including deep compaction from vertical multiple borehole extensometers, land subsidence from Persistent Scatterer Interferometry and leveling surveys, groundwater levels, hydrogeological setting from wellbores, and Landsat TM image were collected and effectively used to detect the spatial and temporal features of land subsidence and its possible relation with groundwater level changes, compressible layer thickness, and urban development. Results show that land subsidence is unevenly distributed and continuously increased from 2003 to 2010. The average loss of elevation over the monitoring period amounted to 92.5 mm, with rates up to 52 mm/y. The distribution of the subsidence bowl is only partially consistent with that of the groundwater depression cone because of the variable thickness of the most compressible fine deposits. In fact, extensometers reveal that silty-clay layers account for the larger contribution to land subsidence, with the 15 m thick silty-clay layer between 102 and 117 m depth accounting for about 25% of the total subsidence. Finally, no clear correlation has been observed between the subsidence rates and the increase of the load on the land surface connected to the impressive urban development. This study represents a first step toward the development of a physically-based model of the subsidence occurrence to be used for planning remediation strategies in the northern Beijing plain. (C) 2015 Elsevier B.V. All rights reserved. C1 [Zhu, Lin; Gong, Huili; Li, Xiaojuan; Chen, Beibei] Capital Normal Univ, Beijing Key Lab Resource Environm & Geog Informat, Coll Resource Environm & Tourism, Beijing 10048, Peoples R China. [Teatini, Pietro] Univ Padua, Dept Civil Environm & Architectural Engn, I-23124 Padua, Italy. [Wang, Rong] Beijing Inst Hydrogeol & Engn Geol, Beijing 100195, Peoples R China. [Dai, Zhenxue] Los Alamos Natl Lab, Earth & Environm Sci Div, Los Alamos, NM 87545 USA. RP Gong, HL (reprint author), Capital Normal Univ, Beijing Key Lab Resource Environm & Geog Informat, Coll Resource Environm & Tourism, Beijing 10048, Peoples R China. EM hi-zhulin@163.com OI Teatini, Pietro/0000-0001-9525-4561; Dai, Zhenxue/0000-0002-0805-7621 FU National Natural Science [41201420, 41130744]; Beijing Nova Program [Z111106054511097]; Beijing Young Talent Program; Beijing Science and Technology Program [Z131100005613022] FX This work was supported by the National Natural Science (No.41201420, 41130744), the Beijing Nova Program (No.Z111106054511097), the Beijing Young Talent Program, and the Beijing Science and Technology Program (Z131100005613022). NR 54 TC 20 Z9 24 U1 14 U2 46 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0013-7952 EI 1872-6917 J9 ENG GEOL JI Eng. Geol. PD JUL 2 PY 2015 VL 193 BP 243 EP 255 DI 10.1016/j.enggeo.2015.04.020 PG 13 WC Engineering, Geological; Geosciences, Multidisciplinary SC Engineering; Geology GA CM0EA UT WOS:000357350000020 ER PT J AU Anheier, NC AF Anheier, Norm C. TI NANOTECHNOLOGY Colourful particles for spectrometry SO NATURE LA English DT Editorial Material C1 Pacific NW Natl Lab, Richland, WA 99352 USA. RP Anheier, NC (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM norm.anheier@pnnl.gov NR 7 TC 1 Z9 1 U1 4 U2 30 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD JUL 2 PY 2015 VL 523 IS 7558 BP 39 EP 40 PG 2 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CL7RN UT WOS:000357169500023 PM 26135442 ER PT J AU Charest, MRJ Canfield, TR Morgan, NR Waltz, J Wohlbier, JG AF Charest, Marc R. J. Canfield, Thomas R. Morgan, Nathaniel R. Waltz, Jacob Wohlbier, John G. TI A high-order vertex-based central ENO finite-volume scheme for three-dimensional compressible flows SO COMPUTERS & FLUIDS LA English DT Article DE Numerical algorithms; Computational fluid dynamics; High-order methods; Compressible flows; Shock hydrodynamics ID ESSENTIALLY NONOSCILLATORY SCHEMES; DISCONTINUOUS GALERKIN METHOD; COMPUTATIONAL FLUID-DYNAMICS; HYPERBOLIC CONSERVATION-LAWS; SHOCK-CAPTURING SCHEMES; UNSTRUCTURED GRIDS; ELEMENT-METHOD; EFFICIENT IMPLEMENTATION; EULER EQUATIONS; MESHES AB High-order discretization methods offer the potential to reduce the computational cost associated with modeling compressible flows. However, it is difficult to obtain accurate high-order discretizations of conservation laws that do not produce spurious oscillations near discontinuities, especially on multi-dimensional unstructured meshes. A novel, high-order, central essentially non-oscillatory (CENO) finite-volume method that does not have these difficulties is proposed for tetrahedral meshes. The proposed unstructured method is vertex-based, which differs from existing cell-based CENO formulations, and uses a hybrid reconstruction procedure that switches between two different solution representations. It applies a high-order k-exact reconstruction in smooth regions and a limited linear reconstruction when discontinuities are encountered. Both reconstructions use a single, central stencil for all variables, making the application of CENO to arbitrary unstructured meshes relatively straightforward. The new approach was applied to the conservation equations governing compressible flows and assessed in terms of accuracy and computational cost. For all problems considered, which included various function reconstructions and idealized flows, CENO demonstrated excellent reliability and robustness. Up to fifth-order accuracy was achieved in smooth regions and essentially non-oscillatory solutions were obtained near discontinuities. The high-order schemes were also more computationally efficient for high-accuracy solutions, i.e., they took less wall time than the lower-order schemes to achieve a desired level of error. In one particular case, it took a factor of 24 less wall-time to obtain a given level of error with the fourth-order CENO scheme than to obtain the same error with the second-order scheme. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Charest, Marc R. J.; Canfield, Thomas R.; Morgan, Nathaniel R.; Waltz, Jacob; Wohlbier, John G.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Charest, MRJ (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM charest@lanl.gov FU United States Department of Energy, through Advanced Simulation & Computing (ASC); Metropolis postdoctoral fellowship program FX This research was supported by the United States Department of Energy, through the Advanced Simulation & Computing (ASC) and Metropolis postdoctoral fellowship programs. NR 84 TC 2 Z9 2 U1 1 U2 14 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0045-7930 EI 1879-0747 J9 COMPUT FLUIDS JI Comput. Fluids PD JUL 2 PY 2015 VL 114 BP 172 EP 192 DI 10.1016/j.compfluid.2015.03.001 PG 21 WC Computer Science, Interdisciplinary Applications; Mechanics SC Computer Science; Mechanics GA CH6IX UT WOS:000354141400016 ER PT J AU Tumuluru, JS AF Tumuluru, Jaya Shankar TI High moisture corn stover pelleting in a flat die pellet mill fitted with a 6 mm die: physical properties and specific energy consumption SO ENERGY SCIENCE & ENGINEERING LA English DT Article DE High moisture corn stover; pellet properties; pelleting; specific energy consumption ID SINGLE-SCREW EXTRUSION; LIGNOCELLULOSIC BIOMASS; PROCESS VARIABLES; DENSIFICATION; FUEL; SWITCHGRASS; DURABILITY; PRESSURE; PELLETIZATION; TORREFACTION AB The quality and specific energy consumption (SEC) of the biomass pellets produced depend upon pelleting process conditions. The present study includes understanding the effect of feedstock moisture in the range of 28-38% (wet basis [w. b.]) and preheating in the range of 30-110 degrees C at two die speeds of 40 and 60 Hz on the physical properties and SEC. A flat die pellet mill fitted with a 6 mm die was used in the present study. The physical properties of pellets such as moisture content, unit, bulk and tapped density, durability, and expansion ratio and SEC of the pelleting process are measured. The results indicate that the pellets produced have durability values in the range of 87-98%, and unit bulk and tapped density in the range of 670-1100, 375-575, and 420-620 kg/m(3). Increasing the feedstock moisture content from 33% to 38% (w. b) decreased the unit, bulk and tapped density by about 30-40%. Increasing feedstock moisture content increased the expansion ratio and decreased the density values. A higher feedstock moisture content of 38% (w. b.) and higher preheating temperature of 110 degrees C resulted in lower density and a higher expansion ratio, which can be attributed to flash off of moisture as the material extrudes out of the die. The SEC was in the range of 75-275 kWh/ton. Higher feedstock moisture content of 38% (w. b.) and a lower die speed of 40 Hz increased the SEC, whereas lower to medium preheating temperature (30-70 degrees C), medium feedstock moisture content of 33% (w. b.), and a higher die speed of 60 Hz minimized the SEC to <100 kWh/ton. C1 [Tumuluru, Jaya Shankar] Idaho Natl Lab, Biofuels & Renewable Energy Technol Dept, 750 Univ Blvd, Idaho Falls, ID 83415 USA. RP Tumuluru, JS (reprint author), Idaho Natl Lab, Biofuels & Renewable Energy Technol Dept, 750 Univ Blvd, Idaho Falls, ID 83415 USA. EM JayaShankar.Tumuluru@inl.gov FU Department of Energy, Office of Energy Efficiency, and Renewable Energy under the Department of Energy Idaho Operations Office [DE-AC07-05ID14517] FX This work was supported by the Department of Energy, Office of Energy Efficiency, and Renewable Energy under the Department of Energy Idaho Operations Office Contract DE-AC07-05ID14517. NR 51 TC 4 Z9 4 U1 3 U2 4 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2050-0505 J9 ENERGY SCI ENG JI Energy Sci. Eng. PD JUL PY 2015 VL 3 IS 4 BP 327 EP 341 DI 10.1002/ese3.74 PG 15 WC Energy & Fuels SC Energy & Fuels GA DJ8CN UT WOS:000374440200005 ER PT J AU Melchionna, R Iapicca, P Di Modugno, F Trono, P Gualtieri, N Diodoro, MG Mottolese, M Grazi, GL Fassan, M Scarpa, A Bissell, MJ Nistico, P AF Melchionna, Roberta Iapicca, Pierluigi Di Modugno, Francesca Trono, Paola Gualtieri, Novella Diodoro, Maria Grazia Mottolese, Marcella Grazi, Gian Luca Fassan, Matteo Scarpa, Aldo Bissell, Mina J. Nistico, Paola TI The hMENA Splicing Program: An important regulator of TGF beta 1-driven EMT and invasiveness in pancreatic cancer SO CANCER RESEARCH LA English DT Meeting Abstract CT AACR Special Conference on Pancreatic Cancer - Innovations in Research and Treatment CY MAY 18-21, 2014-2015 CL New Orleans, LA SP Amer Assoc Canc Res C1 [Melchionna, Roberta; Iapicca, Pierluigi; Di Modugno, Francesca; Trono, Paola; Gualtieri, Novella; Diodoro, Maria Grazia; Mottolese, Marcella; Grazi, Gian Luca; Nistico, Paola] Regina Elena Inst Canc Res, Rome, Italy. [Fassan, Matteo; Scarpa, Aldo] ARC NET Res Ctr, Verona, Italy. [Bissell, Mina J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. NR 0 TC 0 Z9 0 U1 1 U2 1 PU AMER ASSOC CANCER RESEARCH PI PHILADELPHIA PA 615 CHESTNUT ST, 17TH FLOOR, PHILADELPHIA, PA 19106-4404 USA SN 0008-5472 EI 1538-7445 J9 CANCER RES JI Cancer Res. PD JUL 1 PY 2015 VL 75 SU 13 MA A60 DI 10.1158/1538-7445.PANCA2014-A60 PG 2 WC Oncology SC Oncology GA DF3RL UT WOS:000371263900058 ER PT J AU Parrish, DA Kramer, S Windler, GK Chavez, DE Leonard, PW AF Parrish, Damon A. Kramer, Stephanie Windler, G. Kenneth Chavez, David E. Leonard, Philip W. TI Crystal structure of 2-diazoimidazole-4,5-dicarbonitrile SO ACTA CRYSTALLOGRAPHICA SECTION E-CRYSTALLOGRAPHIC COMMUNICATIONS LA English DT Article DE crystal structure; diazo; imidazole; carbonitrile AB In the title compound, C5N6, all the atoms are approximately coplanar. In the crystal, molecules are packed with short contact distances of 2.885 (2) (between the diazo N atom connected to the ring and a cyano N atom on a neighboring molecule) and 3.012 (2) angstrom (between the terminal diazo N atom and an N atom of a neighboring imidazole ring). C1 [Parrish, Damon A.; Kramer, Stephanie] Naval Res Lab, CBMSE, Washington, DC 20375 USA. [Windler, G. Kenneth; Chavez, David E.; Leonard, Philip W.] Los Alamos Natl Lab, POB 1663 MS C920, Los Alamos, NM 87545 USA. RP Leonard, PW (reprint author), Los Alamos Natl Lab, POB 1663 MS C920, Los Alamos, NM 87545 USA. EM philipl@lanl.gov NR 11 TC 2 Z9 2 U1 1 U2 6 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 2056-9890 J9 ACTA CRYSTALLOGR E JI Acta Crystallogr. Sect. E.-Crystallogr. Commun. PD JUL PY 2015 VL 71 BP O491 EP + DI 10.1107/S2056989015010944 PN 7 PG 6 WC Crystallography SC Crystallography GA DD5RD UT WOS:000369981000035 PM 26279924 ER PT J AU Mittal, S Vetter, JS AF Mittal, Sparsh Vetter, Jeffrey S. TI AYUSH: A Technique for Extending Lifetime of SRAM-NVM Hybrid Caches SO IEEE COMPUTER ARCHITECTURE LETTERS LA English DT Article DE Non-volatile memory (NVM); hybrid cache; SRAM-NVM cache; device lifetime; write endurance ID ENERGY; MODEL AB Recently, researchers have explored way-based hybrid SRAM-NVM (non-volatile memory) last level caches (LLCs) to bring the best of SRAM and NVM together. However, the limited write endurance of NVMs restricts the lifetime of these hybrid caches. We present AYUSH, a technique to enhance the lifetime of hybrid caches, which works by using data-migration to preferentially use SRAM for storing frequently-reused data. Microarchitectural simulations confirm that AYUSH achieves larger improvement in lifetime than a previous technique and also maintains performance and energy efficiency. For single, dual and quad-core workloads, the average increase in cache lifetime with AYUSH is 6.90, 24.06 and 47.62x, respectively. C1 [Mittal, Sparsh; Vetter, Jeffrey S.] Oak Ridge Natl Lab, Div Math & Comp Sci, Oak Ridge, TN 37831 USA. RP Mittal, S (reprint author), Oak Ridge Natl Lab, Div Math & Comp Sci, Oak Ridge, TN 37831 USA. EM mittals@ornl.gov; vetter@ornl.gov OI Mittal, Sparsh/0000-0002-2908-993X NR 17 TC 5 Z9 5 U1 0 U2 0 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 1556-6056 EI 1556-6064 J9 IEEE COMPUT ARCHIT L JI IEEE Comput. Archit. Lett. PD JUL-DEC PY 2015 VL 14 IS 2 BP 115 EP 118 DI 10.1109/LCA.2014.2355193 PG 4 WC Computer Science, Hardware & Architecture SC Computer Science GA CZ7DC UT WOS:000367259100008 ER PT J AU Guo, Z Zhou, TJ Wang, MH Qian, Y AF Guo, Zhun Zhou, Tianjun Wang, Minghuai Qian, Yun TI Impact of cloud radiative heating on East Asian summer monsoon circulation SO ENVIRONMENTAL RESEARCH LETTERS LA English DT Article DE East Asian summer monsoon; cloud radiative heating; numerical experiments ID COMMUNITY ATMOSPHERE MODEL; CLIMATE SIMULATIONS; CONVECTION; PRECIPITATION; LONGWAVE; REGION; CHINA; RRTM AB The impacts of cloud radiative heating on the East Asian Summer Monsoon (EASM) over southeastern China (105 degrees-125 degrees E, 20 degrees-35 degrees N) are addressed by using the Community Atmosphere Model version 5 (CAM5). Sensitivity experiments demonstrate that the radiative heating of clouds leads to a positive effect on the local EASM circulation over southeastern China. Without the radiative heating of clouds, the EASM circulation and precipitation would be much weaker than that in normal conditions. The longwave heating of clouds dominates the changes of EASM circulation. The positive effect of clouds on EASM circulation is explained by the thermodynamic energy equation, i.e. the different heating rate between cloud base and cloud top enhances the convective instability over southeastern China, which consequently enhances updraft. The strong updraft would further result in a southward meridional wind above the center of the updraft through Sverdrup vorticity balance. C1 [Guo, Zhun; Zhou, Tianjun] Chinese Acad Sci, Inst Atmospher Phys, LASG, Beijing, Peoples R China. [Guo, Zhun; Zhou, Tianjun] Chinese Acad Sci, Climate Change Res Ctr, Beijing, Peoples R China. [Guo, Zhun; Wang, Minghuai] Nanjing Univ, Inst Climate & Global Change Res, Nanjing 210093, Jiangsu, Peoples R China. [Guo, Zhun; Wang, Minghuai] Nanjing Univ, Sch Atmospher Sci, Nanjing 210093, Jiangsu, Peoples R China. [Wang, Minghuai; Qian, Yun] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Guo, Z (reprint author), Chinese Acad Sci, Inst Atmospher Phys, LASG, Beijing, Peoples R China. EM zhoutj@lasg.iap.ac.cn RI qian, yun/E-1845-2011; Wang, Minghuai/E-5390-2011; ZHOU, Tianjun/C-3195-2012 OI Wang, Minghuai/0000-0002-9179-228X; ZHOU, Tianjun/0000-0002-5829-7279 FU National Natural Science Foundation of China [41405103, 41330423]; National Science Fund for Distinguished Young Scholars [41125017]; Jiangsu Specially-appointed professorship grant; US Department of Energy, Office of Science, Biological and Environmental Research, as part of the Earth System Modeling Program; DOE [DE-AC06-76RLO1830] FX This work is supported by the National Natural Science Foundation of China under grant 41405103, 41330423 and the National Science Fund for Distinguished Young Scholars under grant 41125017. MW is supported by the Jiangsu Specially-appointed professorship grant. The contribution of authors from PNNL in this manuscript are supported by the US Department of Energy, Office of Science, Biological and Environmental Research, as part of the Earth System Modeling Program. The Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under contract DE-AC06-76RLO1830. NR 23 TC 1 Z9 1 U1 1 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-9326 J9 ENVIRON RES LETT JI Environ. Res. Lett. PD JUL PY 2015 VL 10 IS 7 AR 074014 DI 10.1088/1748-9326/10/7/074014 PG 7 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA CY9XH UT WOS:000366759200017 ER PT J AU Zan, YL Boutchko, R Huang, Q Li, B Chen, KW Gullberg, GT AF Zan, Yunlong Boutchko, Rostyslav Huang, Qiu Li, Biao Chen, Kewei Gullberg, Grant T. TI Longitudinal Evaluation of Sympathetic Nervous System and Perfusion in Normal and Spontaneously Hypertensive Rat Hearts with Dynamic Single-Photon Emission Computed Tomography SO MOLECULAR IMAGING LA English DT Article ID ALTERED INVITRO UPTAKE; MYOCARDIAL BLOOD-FLOW; CARDIAC-HYPERTROPHY; METAIODOBENZYLGUANIDINE UPTAKE; CARDIOVASCULAR TISSUES; VASOSPASTIC ANGINA; UPTAKE MECHANISMS; SPECT; NOREPINEPHRINE; TL-201 AB The objective of this work was to evaluate the sympathetic nervous system and structure remodeling during the progression of heart failure in a rodent model using dynamic cardiac single-photon emission computed tomography (SPECT). The spontaneously hypertensive rat (SHR) model was used to study changes in the nervous system innervation and perfusion in the left ventricular (LV) myocardium with the progression of left ventricular hypertrophy (LVH) to heart failure. Longitudinal dynamic SPECT studies were performed with seven SHR and seven Wistar-Kyoto (WKY) rats over 1.5 years using a dual-head SPECT scanner with pinhole collimators. Time-activity curves (TACs) of the I-123-MIBG and (TI)-T-201 distribution in the LV blood pool and myocardium were extracted from dynamic SPECT data and fitted to compartment models to determine the influx rate, washout rate, and distribution volume (DV) of I-123-MIBG and (TI)-T-201 in the LV myocardium. The standardized uptake values (SUVs) of I-123-MIBG and (TI)-T-201 in the LV myocardium were also calculated from the static reconstructed images. The influx and washout rates of I-123-MIBG did not show a significant difference between SHRs and WKY rats. The DVs of I-123-MIBG were greater in the SHRs than in the WKY rats (p = .0028). Specifically, the DV of I-123-MIBG became greater in the SHRs by 6 months of age (p = .0017) and was still significant at the age of 22 months. The SUV of I-123-MIBG in SHRs exhibited abnormal values compared to WKY rats from the age of 18 months. There was no difference in the influx rate and the washout rate of (TI)-T-201 between the SHRs and WKY rats. The SHRs exhibited greater DV of (TI)-T-201 than WKY rats after the age of 18 months (p = .034). The SUV of (TI)-T-201 in SHRs did not show any significant difference from WKY at all ages. The higher DV of I-123-MIBG in the LV myocardium reveals abnormal nervous system activity of the SHRs at an age of 6 months, whereas a greater DV of (TI)-T-201 in the LV myocardium can only be detected at an age of 18 months. The results show that the abnormal nervous system activity appears earlier than perfusion. Furthermore, the comparison between the DV and the SUV indicates that dynamic SPECT with I-123-MIBG and (TI)-T-201 with the kinetic parameter DV is capable of detecting abnormalities of the LV at an early age. C1 Shanghai Jiao Tong Univ, Sch Biomed Engn, Shanghai 200030, Peoples R China. Shanghai Jiao Tong Univ, Rui Jin Hosp, Sch Med, Shanghai 200030, Peoples R China. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. Banner Good Samaritan Med Ctr, Phoenix, AZ USA. RP Huang, Q (reprint author), 1954 Huashan Rd, Shanghai 200030, Peoples R China. EM qiuhuang@sjtu.edu.cn; lb10363@rjh.com.cn; gtgullberg@lbl.gov FU National Science Foundation of China [81201114, 81271610, 91330102]; National Institutes of Health of the U.S. Department of Health and Human Services [R01-EB007219]; Office of Science, Office of Biological and Environmental Research of the U.S. Department of Energy [DE-AC02-05CH11231] FX This study was supported by the National Science Foundation of China (Nos. 81201114, 81271610, and 91330102); the National Institutes of Health of the U.S. Department of Health and Human Services under grant R01-EB007219; and the Director, Office of Science, Office of Biological and Environmental Research of the U.S. Department of Energy under contract DE-AC02-05CH11231. NR 48 TC 0 Z9 0 U1 2 U2 3 PU B C DECKER INC PI HAMILTON PA 69 JOHN STREET SOUTH, STE 310, HAMILTON, ONTARIO L8N 2B9, CANADA SN 1535-3508 EI 1536-0121 J9 MOL IMAGING JI Mol. Imaging PD JUL PY 2015 VL 14 BP 373 EP 384 DI 10.2310/7290.2015.00012 PG 12 WC Biochemical Research Methods; Radiology, Nuclear Medicine & Medical Imaging SC Biochemistry & Molecular Biology; Radiology, Nuclear Medicine & Medical Imaging GA CX3KH UT WOS:000365597200003 PM 26162232 ER PT J AU Ren, XX Yan, D Hong, TZ AF Ren, Xiaoxin Yan, Da Hong, Tianzhen TI Data mining of space heating system performance in affordable housing SO BUILDING AND ENVIRONMENT LA English DT Article DE Data mining; Space heating; Affordable housing; Occupant behavior; Clustering; Decision tree ID ENERGY-CONSUMPTION; RESIDENTIAL BUILDINGS; SIMULATION; BEHAVIOR; MODEL; GAS AB The space heating in residential buildings accounts for a considerable amount of the primary energy use. Therefore, understanding the operation and performance of space heating systems becomes crucial in improving occupant comfort while reducing energy use. This study investigated the behavior of occupants adjusting their thermostat settings and heating system operations in a 62-unit affordable housing complex in Revere, Massachusetts, USA. The data mining methods, including clustering approach and decision trees, were used to ascertain occupant behavior patterns. Data tabulating ON/OFF space heating states was assessed, to provide a better understanding of the intermittent operation of space heating systems in terms of system cycling frequency and the duration of each operation. The decision tree was used to verify the link between room temperature settings, house and heating system characteristics and the heating energy use. The results suggest that the majority of apartments show fairly constant room temperature profiles with limited variations during a day or between weekday and weekend. Data clustering results revealed six typical patterns of room temperature profiles during the heating season. Space heating systems cycled more frequently than anticipated due to a tight range of room thermostat settings and potentially oversized heating capacities. The results from this study affirm data mining techniques are an effective method to analyze large datasets and extract hidden patterns to inform design and improve operations. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Ren, Xiaoxin; Yan, Da] Tsinghua Univ, Sch Architecture, Beijing 100084, Peoples R China. [Hong, Tianzhen] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Hong, TZ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM thong@lbl.gov OI Hong, Tianzhen/0000-0003-1886-9137 FU U.S. Department of Energy [DE-AC02-05CH11231]; China Ministry of Housing and Urban-Rural Development; Ministry of Science & Technology under the U.S.-China Clean Energy Research Center for Building Energy Efficiency [2010DFA72740-02]; Twelfth Five Year National Science and Technology [2012BAJ12B00] FX This work was sponsored by the U.S. Department of Energy (Contract No. DE-AC02-05CH11231), and the China Ministry of Housing and Urban-Rural Development and the Ministry of Science & Technology (Grant No. 2010DFA72740-02) under the U.S.-China Clean Energy Research Center for Building Energy Efficiency. The work was also supported by the Twelfth Five Year National Science and Technology Support Program "Research on a framework to support energy efficiency technologies in buildings" (Grant No. 2012BAJ12B00). The authors appreciate Fraunhofer for sharing the dataset and answered our questions. This work is part of the research in IEA EBC ANNEX 66, Definition and Simulation of Occupant Behavior in Buildings. NR 40 TC 7 Z9 7 U1 4 U2 14 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-1323 EI 1873-684X J9 BUILD ENVIRON JI Build. Environ. PD JUL PY 2015 VL 89 BP 1 EP 13 DI 10.1016/j.buildenv.2015.02.009 PN 1 PG 13 WC Construction & Building Technology; Engineering, Environmental; Engineering, Civil SC Construction & Building Technology; Engineering GA CV7GO UT WOS:000364440600001 ER PT J AU DeForest, N Shehabi, A O'Donnell, J Garcia, G Greenblatt, J Lee, ES Selkowitz, S Milliron, DJ AF DeForest, Nicholas Shehabi, Arman O'Donnell, James Garcia, Guillermo Greenblatt, Jeffery Lee, Eleanor S. Selkowitz, Stephen Milliron, Delia J. TI United States energy and CO2 savings potential from deployment of near-infrared electrochromic window glazings SO BUILDING AND ENVIRONMENT LA English DT Article DE Dynamic windows; Electrochromic glazings; NIR-Switching; National energy reduction; Solar heat gain ID PERFORMANCE AB This paper presents a simulation study of the energy and CO2 benefits of a transparent, near-infrared switching electrochromic (NEC) glazing for building applications. NEC glazings are an emerging dynamic window technology that can modulate the transmission of NIR heat without affecting transmission of visible light. In this study, a hypothetical NEC glazing is simulated on clear and tinted glass in six building type models in 16 U.S. climate regions using Energy Plus 7.1. The total annual energy consumption for lighting, heating, cooling, and ventilation for the NEC glazings are compared with high performance static windows and conventional tungsten-oxide EC glazings. Using regional CO2 intensities and building stock totals, the results from individual building model simulations are scaled up to national totals. The U.S. national savings from NEC deployment is found to be 167 TWh/yr (600 PJ/yr) compared to the existing building stock, but only 8 TWh/yr (29 PJ/yr) or 1.56 million tonnes of CO2 per year when compared to high performance static glazings with lighting controls installed. NEC performance varied significantly by building type and location. This analysis reveals that 50% of the total energy savings can be realized by deploying NEC glazings in only 18% of the total window stock, and 75% of the savings in only 39% of the stock. The best performing locations include medium offices and midrise residential buildings in northern climates, where energy savings per unit window area range from 50 to 200 kWh/m(2)-yr. (C) 2015 Elsevier Ltd. All rights reserved. C1 [DeForest, Nicholas; Shehabi, Arman; O'Donnell, James; Greenblatt, Jeffery; Lee, Eleanor S.; Selkowitz, Stephen] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [O'Donnell, James] Univ Coll Dublin, Sch Mech & Mat Engn, Elect Res Ctr, Dublin 4, Ireland. [Garcia, Guillermo] Heliotrope Technol, Berkeley, CA 94705 USA. [Milliron, Delia J.] Univ Texas Austin, McKetta Dept Chem Engn, Austin, TX 78712 USA. RP DeForest, N (reprint author), 1 Cyclotron Rd,MS 90-1121,Bldg 90 Room 1139, Berkeley, CA 94720 USA. EM ndeforest@lbl.gov RI Milliron, Delia/D-6002-2012 FU Laboratory Directed Research and Development funding at the Lawrence Berkeley National Laboratory; US Department of Energy [DE-AC02-05CH11231] FX This research was supported by Laboratory Directed Research and Development funding at the Lawrence Berkeley National Laboratory. Lawrence Berkeley National Laboratory is operated for US Department of Energy under Contract Grant No. DE-AC02-05CH11231. NR 31 TC 11 Z9 11 U1 9 U2 17 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-1323 EI 1873-684X J9 BUILD ENVIRON JI Build. Environ. PD JUL PY 2015 VL 89 BP 107 EP 117 DI 10.1016/j.buildenv.2015.02.021 PN 1 PG 11 WC Construction & Building Technology; Engineering, Environmental; Engineering, Civil SC Construction & Building Technology; Engineering GA CV7GO UT WOS:000364440600009 ER PT J AU Qian, JF Xu, W Bhattacharya, P Engelhard, M Henderson, WA Zhang, YH Zhang, JG AF Qian, Jiangfeng Xu, Wu Bhattacharya, Priyanka Engelhard, Mark Henderson, Wesley A. Zhang, Yaohui Zhang, Ji-Guang TI Dendrite-free Li deposition using trace-amounts of water as an electrolyte additive SO NANO ENERGY LA English DT Article DE Li deposition; Dendrite free; Water additive; LiF; SEI layer ID FREE LITHIUM DEPOSITION; NONAQUEOUS ELECTROLYTES; METAL ANODES; ELECTROCHEMICAL DEPOSITION; ION BATTERIES; CELLS; SALTS; HYDROLYSIS; MECHANISMS; MICROSCOPY AB Residual water (H2O) presents in nonaqueous electrolytes has been widely regarded as a detrimental factor for lithium (Li) batteries. This is because H2O is highly reactive with the commonly used LiPF6 salt leading to the formation of HF which subsequently corrodes battery materials. In this work, we demonstrate that a controlled trace-amount of H2O (25-50 ppm) can be an effective electrolyte additive for achieving dendrite-free Li metal deposition in LiPF6-based electrolytes, while avoid detrimental effects. Detailed analyses revealed that the trace amount of HF derived from the decomposition reaction of LiPF6 with H2O is electrochemically reduced during the initial Li deposition process to form a uniform and dense LIF-rich solid electrolyte interphase (SEI) layer on the surface of the substrate. This LiF-rich SEI layer leads to a uniform distribution of the electric field on the substrate surface thereby enabling uniform and dendrite-free Li deposition. Meanwhile, the detrimental effect of HF on the other cell components is diminished due to the consumption of the HF in the LiF formation process. Microscopic analysis reveals that the as-deposited, dendrite-free Li films exhibit a self-aligned and highlycompact Li nanorod structure which is consistent with a vivid blue color due to structural coloration. These findings clearly demonstrate a novel approach to control the nucleation and grow processes of Li metal films using a well-controlled, trace-amount of H2O, as well as illuminate the effect of H2O on other electrodeposition processes. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Qian, Jiangfeng; Xu, Wu; Bhattacharya, Priyanka; Henderson, Wesley A.; Zhang, Yaohui; Zhang, Ji-Guang] Pacific NW Natl Lab, Joint Ctr Energy Storage Res, Energy & Environm Directorate, Richland, WA 99354 USA. [Engelhard, Mark] Pacific NW Natl Lab, Joint Ctr Energy Storage Res, Environm & Mol Sci Lab, Richland, WA 99354 USA. [Zhang, Yaohui] Harbin Inst Technol, Dept Phys, Harbin 150001, Heilongjiang, Peoples R China. RP Xu, W (reprint author), Pacific NW Natl Lab, Joint Ctr Energy Storage Res, Energy & Environm Directorate, Richland, WA 99354 USA. EM wu.xu@pnnl.gov; jiguang.zhang@pnnl.gov OI Engelhard, Mark/0000-0002-5543-0812; Xu, Wu/0000-0002-2685-8684 FU Joint Center for Energy Storage Research (JCESR), an Energy Innovation - Basic Energy Sciences, Office of Science of the U.S. DOE [70084]; DOE's Office of Biological and Environmental Research; Linus Pau ling Distinguished Postdoctoral Fellowship at PNNL FX This work was supported by the Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub funded by the Basic Energy Sciences, Office of Science of the U.S. DOE under grant # EDCHEE, 70084. The SEM and EDX measurements were performed in the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility located at PNNL and sponsored by the DOE's Office of Biological and Environmental Research. PB is grateful for support from a Linus Pau ling Distinguished Postdoctoral Fellowship at PNNL. NR 42 TC 19 Z9 19 U1 42 U2 139 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2211-2855 EI 2211-3282 J9 NANO ENERGY JI Nano Energy PD JUL PY 2015 VL 15 BP 135 EP 144 DI 10.1016/j.nanoen.2015.04.009 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CV9AE UT WOS:000364578900014 ER PT J AU Zhao, TL Li, L Chen, RJ Wu, HM Zhang, XX Chen, S Xie, M Wu, F Lu, J Amine, K AF Zhao, Taolin Li, Li Chen, Renjie Wu, Huiming Zhang, Xiaoxiao Chen, Shi Xie, Man Wu, Feng Lu, Jun Amine, Khalil TI Design of surface protective layer of LiF/FeF3 nanoparticles in Li-rich cathode for high-capacity Li-ion batteries SO NANO ENERGY LA English DT Article DE Lithium-ion battery; Nanoparticle; Surface protective layer; Iron fluoride; Li[Li0.2Ni0.2Mn0.6]O-2 ID METAL FLUORIDE NANOCOMPOSITES; RECHARGEABLE LITHIUM BATTERIES; ELECTRODE MATERIALS; ELECTROCHEMICAL PERFORMANCE; CONVERSION REACTION; IRON FLUORIDE; MN; OXIDES; CHALLENGES; NICKEL AB Advanced lithium-ion batteries for renewable energy storage applications have become a major research interest in recent years. Much better performance can be realized by improvements in the material surface design, especially for the cathode materials. Here, we present a new design for a surface protective layer formed via a facile aqueous solution process in which a nano-architectured layer of LiF/FeF3 is epitaxially grown on bulk hierarchical Li-rich cathode Li [Li0.2Ni0.2Mn0.6]O-2. Coin cell tests of this material in the voltage range of 2-4.8 V indicated a high reversible capacity (260.1 mA h g(-1) at 0.1 C), superior rate performance (129.9 mA h g(-1) at 20 C), and excellent capacity retention. Differential scanning calorimetry showed good thermal stability. The enhanced capacity and cycling stability are attributed to the suppression of interfacial side reactions as well as the conversion reaction resulting from the introduction of LiF/FeF3 as a surface protective layer. Published by Elsevier Ltd. C1 [Zhao, Taolin; Li, Li; Chen, Renjie; Zhang, Xiaoxiao; Chen, Shi; Xie, Man; Wu, Feng] Beijing Inst Technol, Beijing Key Lab Environm Sci & Engn, Sch Mat Sci & Engn, Beijing 100081, Peoples R China. [Li, Li; Chen, Renjie; Chen, Shi; Wu, Feng] Collaborat Innovat Ctr Elect Vehicles, Beijing, Peoples R China. [Wu, Huiming; Lu, Jun; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Chen, RJ (reprint author), Beijing Inst Technol, Beijing Key Lab Environm Sci & Engn, Sch Mat Sci & Engn, Beijing 100081, Peoples R China. EM chenrj@bit.edu.cn; wufeng863@bit.edu.cn; junlu@anl.gov; amine@anl.gov FU Chinese National 973 Program [2015CB251100]; National Science Foundation of China [NSFC51302014]; Beijing Nova Program [Z121103002512029]; Beijing Excellent Talents Plan funding; New Century Educational Talents Plan of the Chinese Education Ministry [NCET-12-0050]; U.S. Department of Energy [DE-AC0206CH11357]; Vehicle Technologies Office, Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy (EERE) FX The experimental work of this study was supported by the Chinese National 973 Program (2015CB251100), the National Science Foundation of China (NSFC51302014), Beijing Nova Program (Z121103002512029), Beijing Excellent Talents Plan funding and the New Century Educational Talents Plan of the Chinese Education Ministry (NCET-12-0050). This work was also supported by the U.S. Department of Energy under Contract DE-AC0206CH11357 with the main support provided by the Vehicle Technologies Office, Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy (EERE). The authors especially thank US-China Electric Vehicle and Battery Technology between Beijing Institute of Technology and Argonne National Laboratory. NR 45 TC 28 Z9 28 U1 36 U2 95 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2211-2855 EI 2211-3282 J9 NANO ENERGY JI Nano Energy PD JUL PY 2015 VL 15 BP 164 EP 176 DI 10.1016/j.nanoen.2015.04.013 PG 13 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CV9AE UT WOS:000364578900017 ER PT J AU Xu, R Zhang, XF Chamoun, R Shui, JL Li, JCM Lu, J Amine, K Belharouak, I AF Xu, Rui Zhang, Xiaofeng Chamoun, Rita Shui, Jianglan Li, James C. M. Lu, Jun Amine, Khalil Belharouak, Ilias TI Enhanced rate performance of LiNi0.5Mn1.5O4 fibers synthesized by electrospinning SO NANO ENERGY LA English DT Article DE Electrospinning; Nanofiber; High voltagespinel; Cathode; Lithium-ion battery ID LITHIUM-ION BATTERIES; HIGH-RATE CAPABILITIES; ELECTROCHEMICAL CHARACTERISTICS; MESOPOROUS NANOCOMPOSITE; POLYMER NANOFIBERS; ELECTRODE MATERIAL; CARBON NANOFIBERS; ENERGY-CONVERSION; SPINEL LI4TI5O12; STORAGE DEVICES AB Spinel LiNi0.5Mn1.5O4 (LNMO) provides a high working potential as a cathode material for lithium-ion batteries. Yet there is a phase transition from cubic to tetragonal structure in LNMO during the similar to 3-V charge/discharge region. To suppress the large volume change and capacity fade inherent with bulk-sized LNMO particles when discharged to below 3.0 V, one-dimensional nano-structured LNMO was prepared by an electrospinning method and a subsequent heat treatment. The well-separated nanofiber precursors combat the growth and aggregation of LNMO particles during the heating procedure and lead to improved capacity, better cycling stability, and improved rate capability of the final LMNO nanofibers. The as-prepared LMNO nanofibers have a diameter as thin as 50-100 nm, which is the thinnest of this kind of complex compounds that contain multi-transition metal elements produced through the electrospinning method. In coin cell tests of this material at a current density of 27 mA g(-1), the initial discharge capacity was 130 mAh g(-1) over a voltage range of 3.54.8 V and 300 mAh g(-1) over a voltage range of 2.04.8 V. Published by Elsevier Ltd. C1 [Xu, Rui; Zhang, Xiaofeng; Shui, Jianglan; Lu, Jun; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Chamoun, Rita; Belharouak, Ilias] Qatar Fdn, Qatar Environm & Energy Res Inst, Doha, Qatar. [Xu, Rui; Li, James C. M.] Univ Rochester, Dept Mech Engn, Rochester, NY 14627 USA. RP Lu, J (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 South Cass Ave, Argonne, IL 60439 USA. EM junlu@anl.gov; amine@anl.gov; ibelharouak@qf.org.qa FU U.S. Department of Energy, Freedom CAR; Vehicle Technologies Office; U.S. Department of Energy Office of Science Laboratory [DE-AC02-06CH11357] FX This research was funded by the U.S. Department of Energy, Freedom CAR, and Vehicle Technologies Office. The electron microscopy was accomplished at the Electron Microscopy Center for Materials Research at the Argonne National Laboratory, a U.S. Department of Energy Office of Science Laboratory operated under Contract no. DE-AC02-06CH11357 by UChicago Argonne, LLC. NR 38 TC 6 Z9 6 U1 7 U2 68 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2211-2855 EI 2211-3282 J9 NANO ENERGY JI Nano Energy PD JUL PY 2015 VL 15 BP 616 EP 624 DI 10.1016/j.nanoen.2015.05.023 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CV9AE UT WOS:000364578900059 ER PT J AU Black, JM Okatan, MB Feng, G Cummings, PT Kalinin, SV Balke, N AF Black, Jennifer M. Okatan, M. Baris Feng, Guang Cummings, Peter T. Kalinin, Sergei V. Balke, Nina TI Topological defects in electric double layers of ionic liquids at carbon interfaces SO NANO ENERGY LA English DT Article DE Ionic liquid; Carbon; Electric double layer; Defect; Atomic force microscopy ID ATOMIC-FORCE MICROSCOPY; SURFACE-STRUCTURE; SOLID INTERFACE; GRAPHITE; AFM; SIMULATIONS; CAPACITANCE; AU(111); SYSTEMS; EWALD AB The structure and properties of the electrical double layer in ionic liquids is of interest in a wide range of areas including energy storage, catalysis, lubrication, and many more. Theories describing the electrical double layer for ionic liquids have been proposed; however, a full molecular level description of the double layer is lacking. To date, studies have been predominantly focused on ion distributions normal to the surface; however, the 3D nature of the electrical double layer in ionic liquids requires a full picture of the double layer structure not only normal to the surface, but also in plane. Here we utilize 3D force mapping to probe the in plane structure of an ionic liquid at a graphite interface and report the direct observation of the structure and properties of topological defects. The observation of ion layering at structural defects such as step-edges, reinforced by molecular dynamics simulations, defines the spatial resolution of the method. Observation of defects allows for the establishment of the universality of ionic liquid behavior vs. separation from the carbon surface and to map internal defect structure. These studies offer a universal pathway for probing the internal structure of topological defects in soft condensed matter on the nanometer level in three dimensions. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Black, Jennifer M.; Okatan, M. Baris; Kalinin, Sergei V.; Balke, Nina] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Feng, Guang] Huazhong Univ Sci & Technol, Sch Energy & Power Engn, State Key Lab Coal Combust, Wuhan 430074, Peoples R China. [Cummings, Peter T.] Vanderbilt Univ, Dept Chem & Biomol Engn, Nashville, TN 37235 USA. [Cummings, Peter T.] Vanderbilt Univ, Multiscale Modeling & Simulat Ctr, Nashville, TN 37235 USA. RP Feng, G (reprint author), Huazhong Univ Sci & Technol, Sch Energy & Power Engn, State Key Lab Coal Combust, Wuhan 430074, Peoples R China. EM gfeng@hust.edu.ch; balken@ornl.gov RI Balke, Nina/Q-2505-2015; Kalinin, Sergei/I-9096-2012; Feng, Guang/D-8989-2011; Okatan, M. Baris/E-1913-2016 OI Balke, Nina/0000-0001-5865-5892; Kalinin, Sergei/0000-0001-5354-6152; Okatan, M. Baris/0000-0002-9421-7846 FU Fluid Interface Reactions, Structures and Transport (FIRST); Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division through the Office of Science Early Career Research Program; Center for Nanophase Materials Sciences; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; National Natural Science Foundation of China [51406060] FX The experimental and modeling efforts of JB, GF, and PTC were supported by the Fluid Interface Reactions, Structures and Transport (FIRST), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. Additional support was provided by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division through the Office of Science Early Career Research Program (NB) and the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. (MBO and SVK). We thank the computational resource from the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. G.F. also acknowledges the support from National Natural Science Foundation of China (51406060). NR 43 TC 8 Z9 8 U1 17 U2 41 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2211-2855 EI 2211-3282 J9 NANO ENERGY JI Nano Energy PD JUL PY 2015 VL 15 BP 737 EP 745 DI 10.1016/j.nanoen.2015.05.037 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CV9AE UT WOS:000364578900072 ER PT J AU Raju, MR AF Raju, M. R. TI Glimpses of evolutionary developments of radiotherapy and challenges in meeting the needs of cancer patients, especially in rural India SO JOURNAL OF CANCER RESEARCH AND THERAPEUTICS LA English DT Editorial Material C1 [Raju, M. R.] Mahatma Gandhi Mem Med Trust, Int Canc Ctr, Bhimavaram 534204, Andhra Pradesh, India. [Raju, M. R.] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM USA. RP Raju, MR (reprint author), Mahatma Gandhi Mem Med Trust, Int Canc Ctr, Bhimavaram 534204, Andhra Pradesh, India. EM mgmtrust2@gmail.com NR 9 TC 0 Z9 0 U1 1 U2 1 PU MEDKNOW PUBLICATIONS & MEDIA PVT LTD PI MUMBAI PA B-9, KANARA BUSINESS CENTRE, OFF LINK RD, GHAKTOPAR-E, MUMBAI, 400075, INDIA SN 0973-1482 EI 1998-4138 J9 J CANCER RES THER JI J. Canc. Res. Ther. PD JUL-SEP PY 2015 VL 11 IS 3 BP 503 EP 507 DI 10.4103/0973-1482.165990 PG 5 WC Oncology SC Oncology GA CU3JG UT WOS:000363420200001 PM 26458574 ER PT J AU Dobrzynski, L Fornalski, KW Feinendegen, LE AF Dobrzynski, Ludwik Fornalski, Krzysztof W. Feinendegen, Ludwig E. TI Cancer Mortality Among People Living in Areas With Various Levels of Natural Background Radiation SO DOSE-RESPONSE LA English DT Article DE natural radiation; background radiation; HBRA; HNBR; low radiation; cancer; hormesis ID LUNG-CANCER; CHROMOSOME-ABERRATIONS; SOUTHWEST COAST; RADON EXPOSURE; DNA-DAMAGE; RISK; LYMPHOCYTES; KERALA; INDIA; CHINA AB There are many places on the earth, where natural background radiation exposures are elevated significantly above about 2.5 mSv/year. The studies of health effects on populations living in such places are crucially important for understanding the impact of low doses of ionizing radiation. This article critically reviews some recent representative literature that addresses the likelihood of radiation-induced cancer and early childhood death in regions with high natural background radiation. The comparative and Bayesian analysis of the published data shows that the linear no-threshold hypothesis does not likely explain the results of these recent studies, whereas they favor the model of threshold or hormesis. Neither cancers nor early childhood deaths positively correlate with dose rates in regions with elevated natural background radiation. C1 [Dobrzynski, Ludwik] Natl Ctr Nucl Res NCBJ, PL-05400 Otwock, Poland. [Fornalski, Krzysztof W.] PGE EJ 1 Sp Zoo, Warsaw, Poland. [Feinendegen, Ludwig E.] Univ Dusseldorf, Dusseldorf, Germany. [Feinendegen, Ludwig E.] Brookhaven Natl Lab, BECS Dept, Upton, NY 11973 USA. RP Dobrzynski, L (reprint author), Natl Ctr Nucl Res NCBJ, Ul Soltana 7, PL-05400 Otwock, Poland. EM ludwik.dobrzynski@ncbj.gov.pl NR 56 TC 3 Z9 3 U1 4 U2 10 PU SAGE PUBLICATIONS INC PI THOUSAND OAKS PA 2455 TELLER RD, THOUSAND OAKS, CA 91320 USA SN 1559-3258 J9 DOSE-RESPONSE JI Dose-Response PD JUL-SEP PY 2015 VL 13 IS 3 AR 1559325815592391 DI 10.1177/1559325815592391 PG 10 WC Pharmacology & Pharmacy; Radiology, Nuclear Medicine & Medical Imaging; Toxicology SC Pharmacology & Pharmacy; Radiology, Nuclear Medicine & Medical Imaging; Toxicology GA CS9XR UT WOS:000362447500005 PM 26674931 ER PT J AU Acciarri, R Adamowski, M Artrip, D Baller, B Bromberg, C Cavanna, F Carls, B Chen, H Deptuch, G Epprecht, L Dharmapalan, R Foreman, W Hahn, A Johnson, M Jones, BJP Junk, T Lang, K Lockwitz, S Marchionni, A Mauger, C Montanari, C Mufson, S Nessi, M Back, HO Petrillo, G Pordes, S Raaf, J Rebel, B Sinins, G Soderberg, M Spooner, NJC Stancari, M Strauss, T Terao, K Thorn, C Tope, T Toups, M Urheim, J Van de Water, R Wang, H Wasserman, R Weber, M Whittington, D Yang, T AF Acciarri, R. Adamowski, M. Artrip, D. Baller, B. Bromberg, C. Cavanna, F. Carls, B. Chen, H. Deptuch, G. Epprecht, L. Dharmapalan, R. Foreman, W. Hahn, A. Johnson, M. Jones, B. J. P. Junk, T. Lang, K. Lockwitz, S. Marchionni, A. Mauger, C. Montanari, C. Mufson, S. Nessi, M. Back, H. Olling Petrillo, G. Pordes, S. Raaf, J. Rebel, B. Sinins, G. Soderberg, M. Spooner, N. J. C. Stancari, M. Strauss, T. Terao, K. Thorn, C. Tope, T. Toups, M. Urheim, J. Van de Water, R. Wang, H. Wasserman, R. Weber, M. Whittington, D. Yang, T. TI Summary of the second workshop on liquid argon time projection chamber research and development in the United States SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Particle tracking detectors; Calorimeters; Neutrino detectors; Time projection chambers ID 300 K; LIFETIME; DETECTOR; DEPENDENCE; STRENGTH AB The second workshop to discuss the development of liquid argon time projection chambers (LArTPCs) in the United States was held at Fermilab on July 8-9, 2014. The workshop was organized under the auspices of the Coordinating Panel for Advanced Detectors, a body that was initiated by the American Physical Society Division of Particles and Fields. All presentations at the workshop were made in six topical plenary sessions: i) Argon Purity and Cryogenics, ii) TPC and High Voltage, iii) Electronics, Data Acquisition and Triggering, iv) Scintillation Light Detection, v) Calibration and Test Beams, and vi) Software. This document summarizes the current efforts in each of these areas. It primarily focuses on the work in the US, but also highlights work done elsewhere in the world. C1 [Acciarri, R.; Adamowski, M.; Baller, B.; Cavanna, F.; Carls, B.; Deptuch, G.; Hahn, A.; Johnson, M.; Junk, T.; Lockwitz, S.; Marchionni, A.; Pordes, S.; Raaf, J.; Rebel, B.; Soderberg, M.; Stancari, M.; Tope, T.; Yang, T.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Bromberg, C.] Michigan State Univ, E Lansing, MI 48824 USA. [Cavanna, F.] Yale Univ, New Haven, CT 06520 USA. [Chen, H.; Thorn, C.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Epprecht, L.] ETH, CH-8092 Zurich, Switzerland. [Dharmapalan, R.] Argonne Natl Lab, Argonne, IL 60439 USA. [Foreman, W.] Univ Chicago, Chicago, IL 60637 USA. [Jones, B. J. P.] MIT, Cambridge, MA 02139 USA. [Lang, K.] Univ Texas Austin, Austin, TX 78712 USA. [Mauger, C.; Sinins, G.; Van de Water, R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Montanari, C.; Toups, M.] Ist Nazl Fis Nucl, I-27100 Pavia 6, Italy. [Mufson, S.; Urheim, J.; Whittington, D.] Indiana Univ, Bloomington, IN 47405 USA. [Nessi, M.] CERN, CH-1217 Meyrin, Switzerland. [Back, H. Olling] Princeton Univ, Princeton, NJ 08544 USA. [Petrillo, G.] Univ Rochester, Rochester, NY 14627 USA. [Soderberg, M.] Syracuse Univ, Syracuse, NY 13210 USA. [Spooner, N. J. C.] Univ Sheffield, Sheffield S10 2TN, S Yorkshire, England. [Strauss, T.; Weber, M.] Univ Bern, CH-3012 Bern, Switzerland. [Terao, K.] Columbia Univ, New York, NY 10027 USA. [Wang, H.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [Wasserman, R.] Colorado State Univ, Ft Collins, CO 80523 USA. RP Rebel, B (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM brebel@fnal.gov OI Van de Water, Richard/0000-0002-1573-327X; Weber, Michele/0000-0002-2770-9031 FU U.S. Department of Energy Office of Science [DE-FG02-91ER40661]; Brookhaven National Laboratory [BNL 240296]; National Science Foundation; LDRD program FX We thank the ICARUS collaboration for sharing their experiences and lessons learned in building and operating the first large LArTPC. The High Energy Astrophysics Group at Indiana University is supported by the U.S. Department of Energy Office of Science with grant DE-FG02-91ER40661 to Indiana University and LBNE project funding from Brookhaven National Laboratory with grant BNL 240296 to Indiana University. The LArIAT collaboration is supported by the U.S. Department of Energy Office of Science and the National Science Foundation. The CAPTAIN detector has been designed and is being built by the Physics and the Theory divisions of Los Alamos National Laboratory under the auspices of the LDRD program. T. Strauss spoke on behalf of the Albert Einstein Center, Laboratory of High Energy Physics of the University of Bern. The MicroBooNE and LBNE collaborations have participated in the development of cold electronics as supported by the U.S. Department of Energy Office of Science. NR 45 TC 1 Z9 1 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD JUL PY 2015 VL 10 AR T07006 DI 10.1088/1748-0221/10/07/T07006 PG 49 WC Instruments & Instrumentation SC Instruments & Instrumentation GA CS7LR UT WOS:000362265600044 ER PT J AU Bromberg, C Carls, B Edmunds, D Hahn, A Jaskierny, W Jostlein, H Kendziora, C Lockwitz, S Pahlka, B Pordes, S Rebel, B Shooltz, D Stancari, M Tope, T Yang, T AF Bromberg, C. Carls, B. Edmunds, D. Hahn, A. Jaskierny, W. Jostlein, H. Kendziora, C. Lockwitz, S. Pahlka, B. Pordes, S. Rebel, B. Shooltz, D. Stancari, M. Tope, T. Yang, T. TI Design and operation of LongBo: a 2 m long drift liquid argon TPC SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Time projection Chambers (TPC); Noble liquid detectors (scintillation, ionization, double-phase) AB In this paper, we report on the design and operation of the LongBo time projection chamber in the Liquid Argon Purity Demonstrator cryostat. This chamber features a 2 m long drift distance. We measure the electron drift lifetime in the liquid argon using cosmic ray muons and the lifetime is at least 14 ms at 95% confidence level. LongBo is equipped with preamplifiers mounted on the detector in the liquid argon. Of the 144 channels, 128 channels were readout by preamplifiers made with discrete circuitry and 16 channels were readout by ASIC preamplifiers. For the discrete channels, we measure a signal-to-noise (S/N) ratio of 30 at a drift field of 350 V/cm. The measured S/N ratio for the ASIC channels was 1.4 times larger than that measured for the discrete channels. C1 [Bromberg, C.; Edmunds, D.; Shooltz, D.] Michigan State Univ, E Lansing, MI 48824 USA. [Carls, B.; Hahn, A.; Jaskierny, W.; Jostlein, H.; Kendziora, C.; Lockwitz, S.; Pahlka, B.; Pordes, S.; Rebel, B.; Stancari, M.; Tope, T.; Yang, T.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Yang, T (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM tjyang@fnal.gov FU US DOE; NSF [1068318, 1410972]; United States Department of Energy [De-AC02-07CH11359] FX We would like to thank Tom Junk for the useful discussions on statistical analysis. This work was supported by the US DOE, and by the NSF through Grants 1068318 and 1410972, to Michigan State University. We thank the staff at Fermilab for their technical assistance in running the LAPD experiment. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. De-AC02-07CH11359 with the United States Department of Energy. NR 14 TC 0 Z9 0 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD JUL PY 2015 VL 10 AR P07015 DI 10.1088/1748-0221/10/07/P07015 PG 19 WC Instruments & Instrumentation SC Instruments & Instrumentation GA CS7LR UT WOS:000362265600034 ER PT J AU Haupt, J O'Connor, P AF Haupt, J. O'Connor, P. TI Design of a single-star optical emulator for a fast telescope SO JOURNAL OF INSTRUMENTATION LA English DT Article; Proceedings Paper CT Conference on Precision Astronomy with Fully Depleted CCDs CY DEC 04-05, 2014 CL Brookhaven Natl Lab, Upton, NY HO Brookhaven Natl Lab DE Optics; Photon detectors for UV, visible and IR photons (solid-state) (PIN diodes, APDs, Si-PMTs, G-APDs, CCDs, EBCCDs, EMCCDs etc); Photon detectors for UV, visible and IR photons (solid-state); Overall mechanics design (support structures and materials, vibration analysis etc) AB The design of a simple lens system is described capable of projecting a diffraction limited f1/.2 point of light through a variety of plane parallel vacuum windows. The system was built for the purpose of testing prototype CCDs for the Large Synpotic Survey Telescope in which lab testing drove the desire to create a beam that matches the telescope's f-ratio and obstruction, and which would have sufficient back-focal distance to allow imaging onto a sensor at least 50 mm away in various dewars with various window thicknesses. Also used as the final optic in an atmospheric turbulence simulator, the lens can simulate the real-world star PSF as it will appear on the Large Synoptic Survey Telescope (LSST) focal plane. C1 [Haupt, J.; O'Connor, P.] Brookhaven Natl Lab, Instrumentat Div, Upton, NY 11973 USA. RP Haupt, J (reprint author), Brookhaven Natl Lab, Instrumentat Div, Bldg 535, Upton, NY 11973 USA. EM jhaupt@bnl.gov FU Department of Energy [DE-SC0012704, DE-AC02-76-SFO0515]; Brookhaven National Laboratory; National Science Foundation [0809409]; SLAC National Accelerator Laboratory; LSSTC FX This manuscript has been co-authored by employees of Brookhaven Science Associates, LLC., Portions of this work are supported by the Department of Energy under contract DE-SC0012704 with Brookhaven National Laboratory. LSST project activities are supported in part by the National Science Foundation through Governing Cooperative Agreement 0809409 managed by the Association of Universities for Research in Astronomy (AURA), and the Department of Energy under contract DE-AC02-76-SFO0515 with the SLAC National Accelerator Laboratory. Additional LSST funding comes from private donations, grants to universities, and in-kind support from LSSTC Institutional Members. NR 5 TC 0 Z9 0 U1 1 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD JUL PY 2015 VL 10 AR C07003 DI 10.1088/1748-0221/10/07/C07003 PG 12 WC Instruments & Instrumentation SC Instruments & Instrumentation GA CS7LR UT WOS:000362265600003 ER PT J AU Best, DM Cox, BA AF Best, Daniel M. Cox, B. Ann TI Clique: Situational Awareness through Behavior SO IT PROFESSIONAL LA English DT Editorial Material C1 [Best, Daniel M.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Cox, B. Ann] US Dept Homeland Secur Sci & Technol Directorate, Washington, DC USA. RP Best, DM (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM daniel.best@pnnl.gov; ann.cox@hq.dhs.gov NR 4 TC 0 Z9 0 U1 2 U2 3 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 1520-9202 EI 1941-045X J9 IT PROF JI IT Prof. PD JUL-AUG PY 2015 VL 17 IS 4 BP 66 EP 68 PG 3 WC Computer Science, Information Systems; Computer Science, Software Engineering; Telecommunications SC Computer Science; Telecommunications GA CS2MY UT WOS:000361906500011 ER PT J AU Szecsody, JE Truex, MJ Zhong, LR McKinley, JP Qafoku, NP Lee, BD Saurey, SD AF Szecsody, Jim E. Truex, Mike J. Zhong, Lirong McKinley, James P. Qafoku, Nikolla P. Lee, Brady D. Saurey, Sabrina D. TI Remediation of Technetium in Vadose Zone Sediments Using Ammonia and Hydrogen Sulfide Gases SO VADOSE ZONE JOURNAL LA English DT Article ID RAY-ABSORPTION SPECTROSCOPY; TANK WASTE PLUMES; SUBSURFACE SEDIMENTS; CONTAMINATED SEDIMENTS; HIGHLY ALKALINE; HANFORD SITE; PERTECHNETATE; REDUCTION; URANIUM; DISSOLUTION AB Technetium-99 is a mobile, long-lived radionuclide and environmental risk driver at some nuclear waste sites. The feasibility of decreasing Tc-99 mobility in vadose zone sediments using H2S and NH3 gases was evaluated in laboratory experiments. In untreated sediments, 75 to 95% of the Tc-99 was leachable. Using combinations of H2S and NH3 gases, the Tc-99 mobility was reduced to 14 to 48%. Individual H2S or NH3 gas treatment of sediments had little lasting effect. For the combined gas treatment, the H2S gas created reducing conditions at the pore water-mineral interface, which temporarily reduced and precipitated Tc-99, while the NH3 gas created alkaline pore water that caused mineral dissolution. As the pH neutralized, subsequent aluminosilicate precipitation probably coated Tc-99 precipitates and rendered them less mobile. Surface phase analysis showed that Tc-99 was associated with weathered basalt clasts and S, possibly from the precipitation of TcSx. Treatment performance was nearly the same at different Tc-99 concentrations (1.3-240.5 Bq g(-1)), water contents (1-8%), and gas injection rates but was sensitive to gas concentrations. Low gas concentrations (<3%) had insufficient reductant or slower mineral dissolution. High gas concentrations (>30%) formed an NH4SH precipitate. The 14 to 48% mobile Tc-99 remaining after gas treatment may have been caused by the limited time for aluminosilicates to precipitate in our experiments. Degradation of added NH3 was not observed during the 3-mo experiment. Overall, this study showed that combined H2S and NH3 gas treatment of low-water-content sediments can be applied to significantly decrease Tc-99 mobility. C1 [Szecsody, Jim E.; Truex, Mike J.; Zhong, Lirong; McKinley, James P.; Qafoku, Nikolla P.; Lee, Brady D.; Saurey, Sabrina D.] Pacific NW Natl Lab, Richland, WA 99354 USA. RP Szecsody, JE (reprint author), Pacific NW Natl Lab, POB 999, Richland, WA 99354 USA. EM jim.szecsody@pnnl.gov OI Qafoku, Nikolla P./0000-0002-3258-5379 FU USDOE Richland Operations Office under the Deep Vadose Zone-Applied Field Research Initiative; USDOE [DE-AC05-76RL01830] FX Funding for this work was provided by the USDOE Richland Operations Office under the Deep Vadose Zone-Applied Field Research Initiative. The Pacific Northwest National Laboratory is operated by Battelle Memorial Institute for the USDOE under Contract DE-AC05-76RL01830. NR 56 TC 0 Z9 0 U1 5 U2 12 PU SOIL SCI SOC AMER PI MADISON PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA SN 1539-1663 J9 VADOSE ZONE J JI Vadose Zone J. PD JUL PY 2015 VL 14 IS 7 DI 10.2136/vzj2014.09.0134 PG 12 WC Environmental Sciences; Soil Science; Water Resources SC Environmental Sciences & Ecology; Agriculture; Water Resources GA CS4SC UT WOS:000362065200009 ER PT J AU Jung, HS Tsai, HZ Wong, D Germany, C Kahn, S Kim, Y Aikawa, AS Desai, DK Rodgers, GF Bradley, AJ Velasco, J Watanabe, K Taniguchi, T Wang, F Zettl, A Crommie, MF AF Jung, Han Sae Tsai, Hsin-Zon Wong, Dillon Germany, Chad Kahn, Salman Kim, Youngkyou Aikawa, Andrew S. Desai, Dhruv K. Rodgers, Griffin F. Bradley, Aaron J. Velasco, Jairo, Jr. Watanabe, Kenji Taniguchi, Takashi Wang, Feng Zettl, Alex Crommie, Michael F. TI Fabrication of Gate-tunable Graphene Devices for Scanning Tunneling Microscopy Studies with Coulomb Impurities SO JOVE-JOURNAL OF VISUALIZED EXPERIMENTS LA English DT Article DE Engineering; Issue 101; Physics; graphene; electrostatic gating; scanning tunneling microscopy (STM); Coulomb impurity; chemical vapor deposition (CVD); poly(methyl methacrylate) (PMMA) transfer; wire bonding ID COPPER FOILS; BORON-NITRIDE; HIGH-QUALITY; SPECTROSCOPY; SINGLE; SURFACE; FILMS AB Owing to its relativistic low-energy charge carriers, the interaction between graphene and various impurities leads to a wealth of new physics and degrees of freedom to control electronic devices. In particular, the behavior of graphene's charge carriers in response to potentials from charged Coulomb impurities is predicted to differ significantly from that of most materials. Scanning tunneling microscopy (STM) and scanning tunneling spectroscopy (STS) can provide detailed information on both the spatial and energy dependence of graphene's electronic structure in the presence of a charged impurity. The design of a hybrid impurity-graphene device, fabricated using controlled deposition of impurities onto a back-gated graphene surface, has enabled several novel methods for controllably tuning graphene's electronic properties. (1-8) Electrostatic gating enables control of the charge carrier density in graphene and the ability to reversibly tune the charge(2) and/or molecular(5) states of an impurity. This paper outlines the process of fabricating a gate-tunable graphene device decorated with individual Coulomb impurities for combined STM/STS studies. (2-5) These studies provide valuable insights into the underlying physics, as well as signposts for designing hybrid graphene devices. C1 [Jung, Han Sae; Tsai, Hsin-Zon; Wong, Dillon; Germany, Chad; Kahn, Salman; Kim, Youngkyou; Aikawa, Andrew S.; Desai, Dhruv K.; Rodgers, Griffin F.; Bradley, Aaron J.; Velasco, Jairo, Jr.; Wang, Feng; Zettl, Alex; Crommie, Michael F.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Jung, Han Sae] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Kim, Youngkyou] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Watanabe, Kenji; Taniguchi, Takashi] Natl Inst Mat Sci Japan, Tsukuba, Ibaraki, Japan. [Wang, Feng; Zettl, Alex; Crommie, Michael F.] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA USA. [Wang, Feng; Zettl, Alex; Crommie, Michael F.] Univ Calif Berkeley, Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. [Wang, Feng; Zettl, Alex; Crommie, Michael F.] Lawrence Berkeley Natl Lab, Berkeley, CA USA. RP Crommie, MF (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM crommie@berkeley.edu RI Tsai, Hsin-Zon/J-1682-2016; TANIGUCHI, Takashi/H-2718-2011; WATANABE, Kenji/H-2825-2011; Zettl, Alex/O-4925-2016; wang, Feng/I-5727-2015; OI Tsai, Hsin-Zon/0000-0003-2097-0170; WATANABE, Kenji/0000-0003-3701-8119; Zettl, Alex/0000-0001-6330-136X; Kahn, Salman/0000-0002-0012-3305 FU Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy sp2 Program [DE-AC02-05CH11231]; Office of Naval Research; NSF [CMMI-1235361]; Department of Defense (DoD) through National Defense Science & Engineering Graduate Fellowship (NDSEG) Program [32 CFR 168a] FX Our research was supported by the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy sp2 Program under contract no. DE-AC02-05CH11231 (STM instrumentation development and device integration); the Office of Naval Research (device characterization), and NSF award no. CMMI-1235361 (dI/dV imaging). STM data were analyzed and rendered using WSxM software.33 D. W. and A.J.B. were supported by the Department of Defense (DoD) through the National Defense Science & Engineering Graduate Fellowship (NDSEG) Program, 32 CFR 168a. NR 33 TC 1 Z9 1 U1 3 U2 19 PU JOURNAL OF VISUALIZED EXPERIMENTS PI CAMBRIDGE PA 1 ALEWIFE CENTER, STE 200, CAMBRIDGE, MA 02140 USA SN 1940-087X J9 JOVE-J VIS EXP JI J. Vis. Exp. PD JUL PY 2015 IS 101 AR e52711 DI 10.3791/52711 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CR7ND UT WOS:000361536200019 PM 26273961 ER PT J AU Lamprou, A Wang, HX Saeed, A Svec, F Britt, D Maya, F AF Lamprou, Alexandros Wang, Hongxia Saeed, Adeela Svec, Frantisek Britt, David Maya, Fernando TI Preparation of Highly Porous Coordination Polymer Coatings on Macroporous Polymer Monoliths for Enhanced Enrichment of Phosphopeptides SO JOVE-JOURNAL OF VISUALIZED EXPERIMENTS LA English DT Article DE Chemistry; Issue 101; Porous materials; hybrid materials; polymer monoliths; porous coordination polymers; flow-through supports; phosphopeptide enrichment; mass spectrometry ID METAL-ORGANIC FRAMEWORK; LIQUID-CHROMATOGRAPHIC SEPARATION; CAPILLARY; CHEMISTRY; PROTEINS; PHASE; OXIDE AB We describe a protocol for the preparation of hybrid materials based on highly porous coordination polymer coatings on the internal surface of macroporous polymer monoliths. The developed approach is based on the preparation of a macroporous polymer containing carboxylic acid functional groups and the subsequent step-by-step solution-based controlled growth of a layer of a porous coordination polymer on the surface of the pores of the polymer monolith. The prepared metal-organic polymer hybrid has a high specific micropore surface area. The amount of iron(III) sites is enhanced through metal-organic coordination on the surface of the pores of the functional polymer support. The increase of metal sites is related to the number of iterations of the coating process. The developed preparation scheme is easily adapted to a capillary column format. The functional porous polymer is prepared as a self-contained single-block porous monolith within the capillary, yielding a flow-through separation device with excellent flow permeability and modest back-pressure. The metal-organic polymer hybrid column showed excellent performance for the enrichment of phosphopeptides from digested proteins and their subsequent detection using matrix-assisted laser desorption/ionization time-of-flight mass spectrometry. The presented experimental protocol is highly versatile, and can be easily implemented to different organic polymer supports and coatings with a plethora of porous coordination polymers and metal-organic frameworks for multiple purification and/or separation applications. C1 [Lamprou, Alexandros; Wang, Hongxia; Svec, Frantisek; Britt, David] EO Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Saeed, Adeela] Bahauddin Zakariya Univ, Inst Chem Sci, Multan, Pakistan. [Maya, Fernando] Univ Balearic Isl, Dept Chem, Palma De Mallorca, Spain. [Wang, Hongxia] Beijing Univ Chem Technol, Coll Life Sci & Technol, Beijing Key Lab Bioproc, Beijing, Peoples R China. RP Britt, D (reprint author), EO Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. EM davidkbritt@gmail.com RI Britt, David/D-4675-2009 FU Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division of the US Department of Energy [DE-AC02-05CH11231]; ME-Fulbright fellowship; Higher Education Commission of Pakistan FX This work has been performed at the Molecular Foundry, Lawrence Berkeley National Laboratory and supported by the Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division of the US Department of Energy, under Contract No. DE-AC02-05CH11231. The financial support of F.M. by a ME-Fulbright fellowship and A.S. by Higher Education Commission of Pakistan are gratefully acknowledged. NR 25 TC 0 Z9 0 U1 4 U2 34 PU JOURNAL OF VISUALIZED EXPERIMENTS PI CAMBRIDGE PA 1 ALEWIFE CENTER, STE 200, CAMBRIDGE, MA 02140 USA SN 1940-087X J9 JOVE-J VIS EXP JI J. Vis. Exp. PD JUL PY 2015 IS 101 AR e52926 DI 10.3791/52926 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CR7ND UT WOS:000361536200045 PM 26273850 ER PT J AU Chylek, LA Harris, LA Faeder, JR Hlavacek, WS AF Chylek, Lily A. Harris, Leonard A. Faeder, James R. Hlavacek, William S. TI Modeling for (physical) biologists: an introduction to the rule-based approach SO PHYSICAL BIOLOGY LA English DT Article DE rule-based modeling; systems biology; cell signaling ID GROWTH-FACTOR RECEPTOR; BIOCHEMICAL REACTION NETWORKS; BIOMOLECULAR SITE DYNAMICS; FC-EPSILON-RI; SIGNAL-TRANSDUCTION; CELL-SURFACE; STOCHASTIC SIMULATION; SYSTEMS BIOLOGY; COMBINATORIAL COMPLEXITY; COMPUTATIONAL MODEL AB Models that capture the chemical kinetics of cellular regulatory networks can be specified in terms of rules for biomolecular interactions. A rule defines a generalized reaction, meaning a reaction that permits multiple reactants, each capable of participating in a characteristic transformation and each possessing certain, specified properties, which may be local, such as the state of a particular site or domain of a protein. In other words, a rule defines a transformation and the properties that reactants must possess to participate in the transformation. A rule also provides a rate law. A rule-based approach to modeling enables consideration of mechanistic details at the level of functional sites of biomolecules and provides a facile and visual means for constructing computational models, which can be analyzed to study how system-level behaviors emerge from component interactions. C1 [Chylek, Lily A.] Cornell Univ, Dept Chem & Chem Biol, Ithaca, NY 14853 USA. [Chylek, Lily A.; Hlavacek, William S.] Los Alamos Natl Lab, Div Theoret, Theoret Biol & Biophys Grp, Los Alamos, NM 87545 USA. [Chylek, Lily A.; Hlavacek, William S.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Harris, Leonard A.] Vanderbilt Univ, Sch Med, Dept Canc Biol, Nashville, TN 37212 USA. [Faeder, James R.] Univ Pittsburgh, Sch Med, Dept Computat & Syst Biol, Pittsburgh, PA 15260 USA. [Hlavacek, William S.] New Mexico Consortium, Los Alamos, NM 87544 USA. RP Chylek, LA (reprint author), Cornell Univ, Dept Chem & Chem Biol, Ithaca, NY 14853 USA. EM faeder@pitt.edu; wish@lanl.gov OI Hlavacek, William/0000-0003-4383-8711; Harris, Leonard/0000-0003-2112-6940 FU National Institute of General Medical Sciences (NIGMS) of the National Institutes of Health (NIH) [R25GM105608, P50GM085273, P41GM103712]; National Science Foundation (NSF) [0926181] FX This work was supported by grants R25GM105608, P50GM085273, and P41GM103712 from the National Institute of General Medical Sciences (NIGMS) of the National Institutes of Health (NIH) and by an Expeditions in Computing Grant (award 0926181) from the National Science Foundation (NSF). NR 143 TC 4 Z9 4 U1 2 U2 16 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1478-3967 EI 1478-3975 J9 PHYS BIOL JI Phys. Biol. PD JUL PY 2015 VL 12 IS 4 AR 045007 DI 10.1088/1478-3975/12/4/045007 PG 24 WC Biochemistry & Molecular Biology; Biophysics SC Biochemistry & Molecular Biology; Biophysics GA CS1OW UT WOS:000361837200007 PM 26178138 ER PT J AU Gao, K Chung, ET Gibson, RL Fu, SB Efendiev, Y AF Gao, Kai Chung, Eric T. Gibson, Richard L., Jr. Fu, Shubin Efendiev, Yalchin TI A numerical homogenization method for heterogeneous, anisotropic elastic media based on multiscale theory SO GEOPHYSICS LA English DT Article ID ACOUSTIC-WAVE EQUATION; FINITE-DIFFERENCE; ELEMENT METHOD; HOOKES LAW; PROPAGATION; ROCKS; STATISTICS; CONTINUUM; SOLIDS; SCALAR AB The development of reliable methods for upscaling fine-scale models of elastic media has long been an important topic for rock physics and applied seismology. Several effective medium theories have been developed to provide elastic parameters for materials such as finely layered media or randomly oriented or aligned fractures. In such cases, the analytic solutions for upscaled properties can be used for accurate prediction of wave propagation. However, such theories cannot be applied directly to homogenize elastic media with more complex, arbitrary spatial heterogeneity. Therefore, we have proposed a numerical homogenization algorithm based on multiscale finite-element methods for simulating elastic wave propagation in heterogeneous, anisotropic elastic media. Specifically, our method used multiscale basis functions obtained from a local linear elasticity problem with appropriately defined boundary conditions. Homogenized, effective medium parameters were then computed using these basis functions, and the approach applied a numerical discretization that was similar to the rotated staggered-grid finite-difference scheme. Comparisons of the results from our method and from conventional, analytical approaches for finely layered media showed that the homogenization reliably estimated elastic parameters for this simple geometry. Additional tests examined anisotropic models with arbitrary spatial heterogeneity in which the average size of the heterogeneities ranged from several centimeters to several meters, and the ratio between the dominant wavelength and the average size of the arbitrary heterogeneities ranged from 10 to 100. Comparisons to finite-difference simulations proved that the numerical homogenization was equally accurate for these complex cases. C1 [Gao, Kai; Gibson, Richard L., Jr.] Texas A&M Univ, Dept Geol & Geophys, College Stn, TX USA. [Chung, Eric T.] Chinese Univ Hong Kong, Dept Math, Shatin, Hong Kong, Peoples R China. [Fu, Shubin; Efendiev, Yalchin] Texas A&M Univ, Dept Math, College Stn, TX 77843 USA. [Efendiev, Yalchin] King Abdullah Univ Sci & Technol, Numer Porous Media SRI Ctr NumPor, Thuwal, Saudi Arabia. RP Gao, K (reprint author), Los Alamos Natl Lab, Geophys Grp, Los Alamos, NM 87544 USA. EM kaigao87@gmail.com; tschung@math.cuhk.edu.hk; gibson@tamu.edu; shubinfu89@gmail.com; efendiev@math.tamu.edu FU Saudi Aramco; U.S. Department of Energy [DE-FG03-00ER15034]; Hong Kong RGC General Research Fund [400411]; CUHK Faculty of Science Research Incentive Fund FX The project is partially supported by Saudi Aramco, and partially by the U.S. Department of Energy under grant no. DE-FG03-00ER15034. E. Chung's research is partially supported by the Hong Kong RGC General Research Fund (project no. 400411) and the CUHK Faculty of Science Research Incentive Fund. We appreciate editor E. Slob, assistant editor J. Shragge, associate editor E. Saenger, and the four anonymous reviewers for their valuable comments and suggestions that have greatly improved the quality of the manuscript. NR 50 TC 6 Z9 6 U1 4 U2 9 PU SOC EXPLORATION GEOPHYSICISTS PI TULSA PA 8801 S YALE ST, TULSA, OK 74137 USA SN 0016-8033 EI 1942-2156 J9 GEOPHYSICS JI Geophysics PD JUL-AUG PY 2015 VL 80 IS 4 BP D385 EP D401 DI 10.1190/GEO2014-0363.1 PG 17 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CR3GL UT WOS:000361219200013 ER PT J AU Fu, HH Wang, YQ Um, ES Fang, JR Wei, TP Huang, XM Yang, GW AF Fu, Haohuan Wang, Yingqiao Um, Evan Schankee Fang, Jiarui Wei, Tengpeng Huang, Xiaomeng Yang, Guangwen TI A parallel finite-element time-domain method for transient electromagnetic simulation SO GEOPHYSICS LA English DT Article ID SUBSPACE PROJECTION; DIFFERENCE; DIFFUSION; GERMANY; EARTH; AREA AB The finite-difference time-domain (FDTD) method has been widely used to perform transient electromagnetic simulation. Compared to the traditional FDTD method, the finite-element time-domain (FETD) method with unstructured meshes and an adaptive time-stepping scheme has the potential to dramatically cut down the number of unknowns and the number of time steps. However, with a need to solve a large-scale unstructured sparse matrix at every time step, the FETD method is generally difficult to scale with the available parallel computing resources. To make efficient use of the multicore resources in current computing platforms, we designed a parallel FETD method that used multiple threads to accelerate the key steps for solving a large sparse matrix, including the construction of the preconditioner and matrix-vector multiplication. Using a customized incomplete Cholesky preconditioner, we achieved faster convergence than many existing preconditioners and a scalable parallel performance over multiple cores. To further reduce the total calculation time, we implemented an overlapping scheme and a preconditioner-reusing scheme. The overlapping scheme executed the solver computation and the preconditioner computation concurrently using different parts of the parallel resources. The preconditioner reusing scheme reduced the need to recompute preconditioners when increasing the time-step size, thus reducing the frequency of the less scalable preconditioner computations. It brought performance benefits by reducing the frequency of less scalable preconditioner computation. Computed parallel FETD results showed the same level of accuracy as FDTD results. In terms of parallel performance, using eight cores, the method cut execution time by a factor of 4 (i.e., 50 parallel efficiency). For a realistic salt model, we simulated TEM responses from 0.01 s to 30 s in 5 min, using hundreds of CPU cores. C1 [Fu, Haohuan; Huang, Xiaomeng] Tsinghua Univ, Minist Educ, Key Lab Earth Syst Modeling, Beijing 100084, Peoples R China. [Fu, Haohuan; Huang, Xiaomeng] Tsinghua Univ, Ctr Earth Syst Sci, Beijing 100084, Peoples R China. [Wang, Yingqiao; Fang, Jiarui; Wei, Tengpeng; Yang, Guangwen] Tsinghua Univ, Dept Comp Sci & Technol, Beijing 100084, Peoples R China. [Um, Evan Schankee] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Fu, HH (reprint author), Tsinghua Univ, Minist Educ, Key Lab Earth Syst Modeling, Beijing 100084, Peoples R China. EM haohuan@tsinghua.edu.cn; wangyingqiao11@mails.tsinghua.edu.cn; evanum@gmail.com; fang_jiarui@163.com; tpwei07@gmail.com; hxm@tsinghua.edu.cn; ygw@tsinghua.edu.cn RI Um, Evan/E-9414-2015 FU National Natural Science Foundation of China [41374113] FX This work was supported by the National Natural Science Foundation of China (grant no. 41374113). We would also like to thank editor Aria Abubakar (Schlumberger) and three anonymous reviewers for constructive comments that helped us to improve the paper. NR 29 TC 4 Z9 4 U1 0 U2 4 PU SOC EXPLORATION GEOPHYSICISTS PI TULSA PA 8801 S YALE ST, TULSA, OK 74137 USA SN 0016-8033 EI 1942-2156 J9 GEOPHYSICS JI Geophysics PD JUL-AUG PY 2015 VL 80 IS 4 BP E213 EP E224 DI 10.1190/GEO2014-0067.1 PG 12 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CR3GL UT WOS:000361219200015 ER EF