FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Kiraly, B Jacobberger, RM Mannix, AJ Campbell, GP Bedzyk, MJ Arnold, MS Hersam, MC Guisinger, NP AF Kiraly, Brian Jacobberger, Robert M. Mannix, Andrew J. Campbell, Gavin P. Bedzyk, Michael J. Arnold, Michael S. Hersam, Mark C. Guisinger, Nathan P. TI Electronic and Mechanical Properties of Graphene-Germanium Interfaces Grown by Chemical Vapor Deposition SO NANO LETTERS LA English DT Article DE Epitaxy; surface reconstruction; chemical vapor deposition; scanning tunneling microscopy; scanning tunneling spectroscopy; Raman spectroscopy ID SCANNING-TUNNELING-MICROSCOPY; HEXAGONAL BORON-NITRIDE; X-RAY PHOTOEMISSION; HIGH-QUALITY; EPITAXIAL GRAPHENE; LARGE-AREA; MONOLAYER GRAPHENE; GRAIN-BOUNDARIES; DIRAC FERMIONS; LAYER GRAPHENE AB Epitaxially oriented wafer-scale graphene grown directly on semiconducting Ge substrates is of high interest for both fundamental science and electronic device applications. To date, however, this material system remains relatively unexplored structurally and electronically, particularly at the atomic scale. To further understand the nature of the interface between graphene and Ge, we utilize ultrahigh vacuum scanning tunneling microscopy (STM) and scanning tunneling spectroscopy (STS) along with Raman and X-ray photoelectron spectroscopy to probe interfacial atomic structure and chemistry. STS reveals significant differences in electronic interactions between graphene and Ge(110)/Ge(111), which is consistent with a model of stronger interaction on Ge(110) leading to epitaxial growth. Raman spectra indicate that the graphene is considerably strained after growth, with more point-to-point variation on Ge(111). Furthermore, this native strain influences the atomic structure of the interface by inducing metastable and previously unobserved Ge surface reconstructions following annealing. These nonequilibrium reconstructions cover >90% of the surface and, in turn, modify both the electronic and mechanical properties of the graphene overlayer. Finally, graphene on Ge(001) represents the extreme strain case, where graphene drives the reorganization of the Ge surface into [107] facets. From this work, it is clear that the interaction between graphene and the underlying Ge is not only dependent on the substrate crystallographic orientation, but is also tunable and strongly related to the atomic reconfiguration of the graphene-Ge interface. C1 [Kiraly, Brian; Mannix, Andrew J.; Campbell, Gavin P.; Bedzyk, Michael J.; Hersam, Mark C.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Kiraly, Brian; Mannix, Andrew J.; Guisinger, Nathan P.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Jacobberger, Robert M.; Arnold, Michael S.] Univ Wisconsin, Dept Mat Sci & Engn, Madison, WI 53706 USA. [Bedzyk, Michael J.] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [Hersam, Mark C.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. RP Hersam, MC (reprint author), Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. EM m-hersam@northwestem.edu; nguisinger@anl.gov RI Hersam, Mark/B-6739-2009; Bedzyk, Michael/B-7503-2009; Arnold, Michael/L-9112-2015 FU Center for Nanoscale Materials, a U.S. Department of Energy Office of Science User Facility [DE-AC02-06CH11357]; U.S. Department of Energy SISGR [DE-FG02-09ER16109]; Office of Naval Research [N00014-14-1-0669]; National Science Foundation [DGE-0824162, DGE-1324585]; Department of Energy (DOE) Office of Science Early Career Research Program through the Office of Basic Energy Sciences [DE-SC0006414]; Department Of Defense (DOD) Air Force Office of Scientific Research through the National Defense Science and Engineering Graduate Fellowship [32 CFR 168a]; Northwestern University MRSEC from the National Science Foundation [DMR-1121262] FX The authors would like to thank Brandon Fisher for technical support. This work was performed, in part, at the Center for Nanoscale Materials, a U.S. Department of Energy Office of Science User Facility under Contract No. DE-AC02-06CH11357. This work was supported by the U.S. Department of Energy SISGR contract No. DE-FG02-09ER16109, the Office of Naval Research (Grant No. N00014-14-1-0669), and the National Science Foundation Graduate Fellowship DGE-0824162 and DGE-1324585. R.M.J. and M.S.A. acknowledge support from the Department of Energy (DOE) Office of Science Early Career Research Program through the Office of Basic Energy Sciences (No. DE-SC0006414) for graphene synthesis, and R.M.J. also acknowledges support from the Department Of Defense (DOD) Air Force Office of Scientific Research through the National Defense Science and Engineering Graduate Fellowship (No. 32 CFR 168a). G.P.C. and M.J.B. acknowledge support from the Northwestern University MRSEC (Award No. DMR-1121262 from the National Science Foundation). NR 55 TC 6 Z9 6 U1 21 U2 87 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1530-6984 EI 1530-6992 J9 NANO LETT JI Nano Lett. PD NOV PY 2015 VL 15 IS 11 BP 7414 EP 7420 DI 10.1021/acs.nanolett.5b02833 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CW1BU UT WOS:000364725400037 PM 26506006 ER PT J AU Zhou, X Wenger, J Viscomi, FN Le Cunff, L Beal, J Kochtcheev, S Yang, X Wiederrecht, GP des Francs, GC Bisht, AS Jradi, S Caputo, R Demir, HV Schaller, RD Plain, J Vial, A Sun, XW Bachelot, R AF Zhou, Xuan Wenger, Jeremie Viscomi, Francesco N. Le Cunff, Loic Beal, Jeremie Kochtcheev, Serguei Yang, Xuyong Wiederrecht, Gary P. des Francs, Gerard Colas Bisht, Anu Singh Jradi, Safi Caputo, Roberto Demir, Hilmi Volkan Schaller, Richard D. Plain, Jerome Vial, Alexandre Sun, Xiao Wei Bachelot, Renaud TI Two-Color Single Hybrid Plasmonic Nanoemitters with Real Time Switchable Dominant Emission Wavelength SO NANO LETTERS LA English DT Article DE nanoemitter; hybrid nanostructures; fluorescence spectroscopy; nanophotonics; surface plasmons; photopolymerization ID MOLECULAR FLUORESCENCE; OPTICAL-PROPERTIES; GOLD NANOPARTICLE; ENERGY-TRANSFER; ENHANCEMENT; NANOSTRUCTURES; NANOANTENNAS; NANOLASER; NANOCUBES; NANORODS AB We demonstrate two-color nanoemitters that enable the selection of the dominant emitting wavelength by varying the polarization of excitation light The nanoemitters were fabricated via surface plasmon-triggered two-photon polymerization. By using two polymerizable solutions with different quantum dots, emitters of different colors can be positioned selectively in different orientations in the close vicinity of the metal nanoparticles. The dominant emission wavelength of the metal/polymer anisotropic hybrid nanoemitter thus can be selected by altering the incident polarization. C1 [Zhou, Xuan; Wenger, Jeremie; Viscomi, Francesco N.; Le Cunff, Loic; Beal, Jeremie; Kochtcheev, Serguei; Bisht, Anu Singh; Jradi, Safi; Plain, Jerome; Vial, Alexandre; Bachelot, Renaud] Univ Technol Troyes, CNRS UMR 6281, Lab Nanotechnol & Instrumentat Opt, ICD, F-10004 Troyes, France. [Viscomi, Francesco N.; Caputo, Roberto] Univ Calabria, Dept Phys, I-87036 Cosenza, Italy. [Viscomi, Francesco N.; Caputo, Roberto] Univ Calabria, CNR NANOTEC, I-87036 Cosenza, Italy. [Yang, Xuyong; Demir, Hilmi Volkan] Nanyang Technol Univ, Sch Elect & Elect Engn, Singapore 639798, Singapore. [Wiederrecht, Gary P.; Schaller, Richard D.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [des Francs, Gerard Colas] Univ Bourgogne, Lab Interdisciplinaire Carnot Bourgogne ICB, F-2178 Dijon, France. [des Francs, Gerard Colas] Univ Bourgogne, UMR CNRS 6303, F-2178 Dijon, France. RP Sun, XW (reprint author), Nanyang Technol Univ, Sch Elect & Elect Engn, Nanyang Ave, Singapore 639798, Singapore. EM exwsun@ntu.edu.sg; renaud.bachelot@utt.fr RI Vial, Alexandre/I-7894-2012 OI Vial, Alexandre/0000-0002-7701-0413 FU Agence Nationale de la Recherche (ANR) [ANR-12-BS10-0016]; Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science and Office of Basic Energy Sciences User Facility [DE-AC02-06CH11357]; National Research Foundation of Singapore under Competitive Research Program [NRF-CRP11-2012-01, NRF-CRP6-2010-2]; COST Action [IC1208]; Labex ACTION program [ANR-11-LABX-01-01] FX The authors would like to thank the platform Nano'mat and the HAPPLE project (ANR-12-BS10-0016) funded by Agence Nationale de la Recherche (ANR). R.B. would like to thank the members of the HAPPLE consortium for fruitful discussion. This work was supported, in part (R.D.S. and G.P.W.), by the Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science and Office of Basic Energy Sciences User Facility under Contract No. DE-AC02-06CH11357. X.W.S. would like to thank the support from the National Research Foundation of Singapore under its Competitive Research Program No. NRF-CRP11-2012-01 and No. NRF-CRP6-2010-2. The authors would like to give thanks to Dr. Prashant K. Jain for suggestions. The author would also like to acknowledge networking support by the COST Action IC1208, www.ic1208.com. This work has been done in the general context of the Labex ACTION program (ANR-11-LABX-01-01). NR 57 TC 4 Z9 4 U1 15 U2 62 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1530-6984 EI 1530-6992 J9 NANO LETT JI Nano Lett. PD NOV PY 2015 VL 15 IS 11 BP 7458 EP 7466 DI 10.1021/acs.nanolett.5b02962 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CW1BU UT WOS:000364725400043 PM 26437118 ER PT J AU Cui, F Yu, Y Dou, LT Sun, JW Yang, Q Schildknecht, C Schierle-Arndt, K Yang, PD AF Cui, Fan Yu, Yi Dou, Letian Sun, Jianwei Yang, Qin Schildknecht, Christian Schierle-Arndt, Kerstin Yang, Peidong TI Synthesis of Ultrathin Copper Nanowires Using Tris(trimethylsilyl)silane for High-Performance and Low-Haze Transparent Conductors SO NANO LETTERS LA English DT Article DE Ultrathin copper nanowires; tris(trimethylsilyl)silane; growth mechanism; transparent conductor; reduced haze ID LARGE-SCALE SYNTHESIS; SILVER NANOWIRES; FILMS; ELECTRODES; NANORODS; NETWORKS; GROWTH; OXIDE; LONG AB Colloidal metal nanowire based transparent conductors are excellent candidates to replace indium-tin-oxide (ITO) owing to their outstanding balance between transparency and conductivity, flexibility, and solution-processabllity. Copper stands out as a promising material candidate due to its high intrinsic conductivity and earth abundance. Here, we report a new synthetic approach, using tris(trimethylsilyl)silane as a mild reducing reagent, for synthesizing high-quality, ultrathin, and monodispersed copper nanowires, with an average diameter of 17.5 nm and a mean length of 17 mu m. A study of the growth mechanism using high-resolution transmission electron microscopy reveals that the copper nano-wires adopt a five-fold twinned structure and evolve from decahedral nanoseeds. Fabricated transparent conducting films exhibit excellent transparency and conductivity. An additional advantage of our nanowire transparent conductors is highlighted through reduced optical haze factors (forward light scattering) due to the small nanowire diameter. C1 [Cui, Fan; Yu, Yi; Dou, Letian; Sun, Jianwei; Yang, Qin; Yang, Peidong] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Cui, Fan; Dou, Letian; Schildknecht, Christian; Schierle-Arndt, Kerstin; Yang, Peidong] BASF Corp, Calif Res Alliance CARA, Berkeley, CA 94720 USA. [Cui, Fan; Yu, Yi; Dou, Letian; Sun, Jianwei; Yang, Peidong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Yang, Peidong] Univ Calif Berkeley, Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. [Yang, Peidong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Yang, Peidong] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Yang, PD (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM p_yang@berkeley.edu FU BASF Corporation [20131459]; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was financially supported by BASF Corporation (Funding 20131459). We thank Dr. Sam Eaton, Mr. Nick Kornienko, and Dr. Anthony Fu for proofreading the manuscript. Work at the NCEM, Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 38 TC 25 Z9 25 U1 17 U2 122 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1530-6984 EI 1530-6992 J9 NANO LETT JI Nano Lett. PD NOV PY 2015 VL 15 IS 11 BP 7610 EP 7615 DI 10.1021/acs.nanolett.5b03422 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CW1BU UT WOS:000364725400065 PM 26496181 ER PT J AU Huang, XJ Yang, WG Harder, R Sun, YG Lu, M Chu, YS Robinson, IK Mao, HK AF Huang, Xiaojing Yang, Wenge Harder, Ross Sun, Yugang Lu, Ming Chu, Yong S. Robinson, Ian K. Mao, Ho-kwang TI Deformation Twinning of a Silver Nanocrystal under High Pressure SO NANO LETTERS LA English DT Article DE Nanocrystal; deformation twinning; coherent diffractive imaging; X-ray imaging ID LATTICE DEFORMATION; PHASE RETRIEVAL; ICE; NANOPARTICLES; NANOSCALE; CRYSTAL; STRAIN; LIMIT; GOLD AB Within a high-pressure environment, crystal deformation is controlled by complex processes such as dislocation motion, twinning, and phase transitions, which change materials' microscopic morphology and alter their properties. Understanding a crystal's response to external stress provides a unique opportunity for rational tailoring of its functionalities. It is very challenging to track the strain evolution and physical deformation from a single nanoscale crystal under high-pressure stress. Here, we report an in situ three-dimensional mapping of morphology and strain evolutions in a single-crystal silver nanocube within a high-pressure environment using the Bragg Coherent Diffractive Imaging (CDI) method. We observed a continuous lattice distortion, followed by a deformation twining process at a constant pressure. The ability to visualize stress-introduced deformation of nanocrystals with high spatial resolution and prominent strain sensitivity provides an important route for interpreting and engineering novel properties of nanomaterials. C1 [Huang, Xiaojing; Chu, Yong S.] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. [Lu, Ming] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Huang, Xiaojing; Yang, Wenge] Carnegie Inst Sci, Geophys Lab, HPSynC, Argonne, IL 60439 USA. [Yang, Wenge; Mao, Ho-kwang] Ctr High Pressure Sci & Technol Adv Res, Shanghai 201203, Peoples R China. [Harder, Ross] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Sun, Yugang] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Robinson, Ian K.] UCL, London Ctr Nanotechnol, London WC1H 0AH, England. [Robinson, Ian K.] Res Complex Harwell, Didcot OX11 0DE, Oxon, England. [Mao, Ho-kwang] Carnegie Inst Sci, Geophys Lab, Washington, DC 20015 USA. RP Huang, XJ (reprint author), Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. EM xjhuang@bnl.gov; yangwg@hpstar.ac.cn RI Sun, Yugang /A-3683-2010; Huang, Xiaojing/K-3075-2012 OI Sun, Yugang /0000-0001-6351-6977; Huang, Xiaojing/0000-0001-6034-5893 FU DOE-BES X-ray Scattering Core Program [DE-FG02-99ER45775]; NSAF [U1530402]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0012704]; ERC [227711]; US National Science Foundation [DMR-9724294]; US Department of Energy, Office of Basic Energy Sciences [DE-AC0206CH11357] FX This work was supported by DOE-BES X-ray Scattering Core Program under grant number DE-FG02-99ER45775 and NSAF (Grant No. U1530402). Work at the National Synchrotron Light Source II, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-SC0012704. I.K.R. is supported by the ERC "nanosculpture" advanced grant 227711. The measurements were carried out at APS beamline 34-ID-C, built with US National Science Foundation grant DMR-9724294 and operated by the US Department of Energy, Office of Basic Energy Sciences, under contract no. DE-AC0206CH11357. NR 35 TC 4 Z9 4 U1 6 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1530-6984 EI 1530-6992 J9 NANO LETT JI Nano Lett. PD NOV PY 2015 VL 15 IS 11 BP 7644 EP 7649 DI 10.1021/acs.nanolett.5b03568 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CW1BU UT WOS:000364725400071 PM 26484941 ER PT J AU Jin, HE Zueger, C Chung, WJ Wong, WN Lee, BY Lee, SW AF Jin, Hyo-Eon Zueger, Chris Chung, Woo-Jae Wong, Winnie Lee, Byung Yang Lee, Seung-Wuk TI Selective and Sensitive Sensing of Flame Retardant Chemicals Through Phage Display Discovered Recognition Peptide SO NANO LETTERS LA English DT Article DE Phage display; polybrominated diphenyl ether; environmental toxicant; biosensor ID POLYBROMINATED DIPHENYL ETHERS; CHROMATOGRAPHY-MASS SPECTROMETRY; HOUSE-DUST; PBDES; EXTRACTION; EXPOSURE; SAMPLES AB We report a highly selective and sensitive biosensor for the detection of an environmentally toxic molecule, decabrominated diphenyl ether (DBDE), one of the most common congeners of the polybrominated frame retardants (polybrominated diphenyl ether (PBDE)), using newly discovered DBDE peptide receptors integrated with carbon nanotube field-effect transistors (CNT-FET). The specific DBDE peptide receptor was identified using a high-throughput screening process of phage library display. The resulting binding peptide carries an interesting consensus binding pocket with two Trp-His/Asn-Trp repeats, which binds to the DBDE in a multivalent manner. We integrated the novel DBDE binding peptide onto the CNT-FET using polydiacetylene coating materials linked through cysteine-maleimide click chemistry. The resulting biosensor could detect the desired DBDE selectively with a 1 fM detection limit. Our combined approaches of selective receptor discovery, material nanocoating through click chemistry, and integration onto a sensitive CNT-FET electronic sensor for desired target chemicals will pave the way toward the rapid development of portable and easy-to-use biosensors for desired chemicals to protect our health and environment. C1 [Jin, Hyo-Eon; Chung, Woo-Jae; Wong, Winnie; Lee, Byung Yang; Lee, Seung-Wuk] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Zueger, Chris] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. [Jin, Hyo-Eon; Zueger, Chris; Chung, Woo-Jae; Wong, Winnie; Lee, Byung Yang; Lee, Seung-Wuk] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Lee, Byung Yang] Korea Univ, Dept Mech Engn, Seoul 136713, South Korea. RP Lee, BY (reprint author), Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. EM blee@korea.ac.kr; leesw@berkeley.edu OI Lee, Byung Yang/0000-0003-0125-2501 FU Center of Integrated Nanomechanical Systems (COINS) of the National Science Foundation [EEC-0832819]; National Research Foundation (NRF) - Korea government (MSIP) [2015R1A2A2A04002733, 2013R1A1A1010802] FX This work was supported by Center of Integrated Nanomechanical Systems (COINS) of the National Science Foundation (Grant EEC-0832819). B.Y.L. acknowledges the support from the National Research Foundation (NRF) funded by the Korea government (MSIP) (Grants 2015R1A2A2A04002733 and 2013R1A1A1010802). NR 29 TC 2 Z9 2 U1 18 U2 57 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1530-6984 EI 1530-6992 J9 NANO LETT JI Nano Lett. PD NOV PY 2015 VL 15 IS 11 BP 7697 EP 7703 DI 10.1021/acs.nanolett.5b03678 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CW1BU UT WOS:000364725400079 PM 26455834 ER PT J AU Kalinin, SV Morozovska, AN AF Kalinin, Sergei V. Morozovska, Anna N. TI MULTIFERROICS Focusing light on flexoelectricity SO NATURE NANOTECHNOLOGY LA English DT Editorial Material ID FERROELECTRIC THIN-FILMS; POLARIZATION; PHASES C1 [Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Morozovska, Anna N.] Natl Acad Sci Ukraine, Inst Phys, UA-03028 Kiev, Ukraine. RP Kalinin, SV (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM sergei2@ornl.gov RI Kalinin, Sergei/I-9096-2012 OI Kalinin, Sergei/0000-0001-5354-6152 NR 28 TC 8 Z9 8 U1 3 U2 28 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1748-3387 EI 1748-3395 J9 NAT NANOTECHNOL JI Nat. Nanotechnol. PD NOV PY 2015 VL 10 IS 11 BP 917 EP 918 PG 2 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CV8IY UT WOS:000364528300006 ER PT J AU Wong, D Velasco, J Ju, L Lee, J Kahn, S Tsai, HZ Germany, C Taniguchi, T Watanabe, K Zettl, A Wang, F Crommie, MF AF Wong, Dillon Velasco, Jairo, Jr. Ju, Long Lee, Juwon Kahn, Salman Tsai, Hsin-Zon Germany, Chad Taniguchi, Takashi Watanabe, Kenji Zettl, Alex Wang, Feng Crommie, Michael F. TI Characterization and manipulation of individual defects in insulating hexagonal boron nitride using scanning tunnelling microscopy SO NATURE NANOTECHNOLOGY LA English DT Article ID POINT-DEFECTS; SINGLE-CRYSTALS; GRAPHENE; SPECTROSCOPY; BN; SUBSTRATE; RESONANCE; GAAS; EPR AB Defects play a key role in determining the properties and technological applications of nanoscale materials and, because they tend to be highly localized, characterizing them at the singledefect level is of particular importance. Scanning tunnelling microscopy has long been used to image the electronic structure of individual point defects in conductors(1), semiconductors(2-4) and ultrathin films(5-9), but such single-defect electronic characterization remains an elusive goal for intrinsic bulk insulators. Here, we show that individual native defects in an intrinsic bulk hexagonal boron nitride insulator can be characterized and manipulated using a scanning tunnelling microscope. This would typically be impossible due to the lack of a conducting drain path for electrical current. We overcome this problem by using a graphene/boron nitride heterostructure, which exploits the atomically thin nature of graphene to allow the visualization of defect phenomena in the underlying bulk boron nitride. We observe three different defect structures that we attribute to defects within the bulk insulating boron nitride. Using scanning tunnelling spectroscopy we obtain charge and energy-level information for these boron nitride defect structures. We also show that it is possible to manipulate the defects through voltage pulses applied to the scanning tunnelling microscope tip. C1 [Wong, Dillon; Velasco, Jairo, Jr.; Ju, Long; Lee, Juwon; Kahn, Salman; Tsai, Hsin-Zon; Germany, Chad; Zettl, Alex; Wang, Feng; Crommie, Michael F.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Taniguchi, Takashi; Watanabe, Kenji] Natl Inst Mat Sci, Tsukuba, Ibaraki 3050044, Japan. [Zettl, Alex; Wang, Feng; Crommie, Michael F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Zettl, Alex; Wang, Feng; Crommie, Michael F.] Univ Calif Berkeley, Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. [Zettl, Alex; Wang, Feng; Crommie, Michael F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Crommie, MF (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM crommie@berkeley.edu RI Foundry, Molecular/G-9968-2014; Tsai, Hsin-Zon/J-1682-2016; TANIGUCHI, Takashi/H-2718-2011; WATANABE, Kenji/H-2825-2011; Zettl, Alex/O-4925-2016; wang, Feng/I-5727-2015; OI Tsai, Hsin-Zon/0000-0003-2097-0170; WATANABE, Kenji/0000-0003-3701-8119; Zettl, Alex/0000-0001-6330-136X; Kahn, Salman/0000-0002-0012-3305 FU sp2 programme; LBNL Molecular Foundry; Office of Science, Office of Basic Energy Sciences of the US Department of Energy [DE-AC02-05CH11231]; National Science Foundation [CMMI-1235361]; UC President's Postdoctoral Fellowship; Department of Defense (DoD) through the National Defense Science & Engineering Graduate Fellowship (NDSEG) Program; Qualcomm Scholars Research Fellowship FX The authors thank P. Jarillo-Herrero, N. Gabor, A. Young, P. Yu and A. Rubio for discussions. This research was supported by the sp2 programme (STM measurement and device fabrication) and the LBNL Molecular Foundry (graphene growth characterization) funded by the Director, Office of Science, Office of Basic Energy Sciences of the US Department of Energy (contract no. DE-AC02-05CH11231). Support was also provided by National Science Foundation award CMMI-1235361 (device characterization, image analysis). J.V.J. acknowledges support from the UC President's Postdoctoral Fellowship. D.W. was supported by the Department of Defense (DoD) through the National Defense Science & Engineering Graduate Fellowship (NDSEG) Program. S.K. acknowledges support from the Qualcomm Scholars Research Fellowship. NR 33 TC 23 Z9 23 U1 24 U2 87 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1748-3387 EI 1748-3395 J9 NAT NANOTECHNOL JI Nat. Nanotechnol. PD NOV PY 2015 VL 10 IS 11 BP 949 EP U192 DI 10.1038/NNANO.2015.188 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CV8IY UT WOS:000364528300011 PM 26301901 ER PT J AU Wang, F Kivelson, SA Lee, DH AF Wang, Fa Kivelson, Steven A. Lee, Dung-Hai TI Nematicity and quantum paramagnetism in FeSe SO NATURE PHYSICS LA English DT Article ID HEISENBERG MODELS; VALENCE-BOND; GROUND-STATES; SPIN; ANTIFERROMAGNETS AB In common with other iron-based high-temperature superconductors, Fe Se exhibits a transition to a 'nematic' phase below 90 K in which the crystal rotation symmetry is spontaneously broken. However, the absence of strong low-frequency magnetic fluctuations near or above the transition has been interpreted as implying the primacy of orbital ordering. In contrast, we establish that quantum fluctuations of spin-1 local moments with strongly frustrated exchange interactions can lead to a nematic quantum paramagnetic phase consistent with the observations in Fe Se. We show that this phase is a fundamental expression of the existence of a Berry's phase associated with the topological defects of a Neel antiferromagnet, in a manner analogous to that which gives rise to valence bond crystal order for spin-1/2 systems. We present an exactly solvable model realizing the nematic quantum paramagnetic phase, discuss its relation with the spin-1 J(1)-J(2) model, and construct a field theory of the Landau-forbidden transition between the Neel state and this nematic quantum paramagnet. C1 [Wang, Fa] Peking Univ, Sch Phys, Int Ctr Quantum Mat, Beijing 100871, Peoples R China. [Wang, Fa] Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China. [Kivelson, Steven A.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Lee, Dung-Hai] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Lee, Dung-Hai] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Lee, DH (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM dunghai@berkeley.edu RI Wang, Fa/D-3817-2015 OI Wang, Fa/0000-0002-6220-5349 FU National Key Basic Research Program of China [2014CB920902]; National Science Foundation of China [11374018]; US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division [DE-AC02-76SF00515, DE-AC02-05CH11231]; National Science Foundation [NSF PHY11-25915] FX We thank H. Jiang and T. Xiang for useful discussions. F.W. was supported by the National Key Basic Research Program of China (Grant No. 2014CB920902) and the National Science Foundation of China (Grant No. 11374018). S.A.K. was supported in part by the US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division, grant DE-AC02-76SF00515 at Stanford. D.-H.L. was supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division grant DE-AC02-05CH11231. D.-H.L. and S.A.K. would like to thank KITP for hospitality, supported in part by the National Science Foundation under Grant No. NSF PHY11-25915, where the collaboration started. NR 35 TC 46 Z9 46 U1 16 U2 64 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1745-2473 EI 1745-2481 J9 NAT PHYS JI Nat. Phys. PD NOV PY 2015 VL 11 IS 11 BP 959 EP 963 DI 10.1038/NPHYS3456 PG 5 WC Physics, Multidisciplinary SC Physics GA CW2DF UT WOS:000364800600022 ER PT J AU Bukac, M Layton, W Moraiti, M Tran, H Trenchea, C AF Bukac, Martina Layton, William Moraiti, Marina Tran, Hoang Trenchea, Catalin TI Analysis of Partitioned Methods for the Biot System SO NUMERICAL METHODS FOR PARTIAL DIFFERENTIAL EQUATIONS LA English DT Article DE Biot system; partitioned methods; poroelasticity ID STOKES-DARCY MODEL; STABILITY; EXPLICIT; FLOW AB In this work, we present a comprehensive study of several partitioned methods for the coupling of flow and mechanics. We derive energy estimates for each method for the fully-discrete problem. We write the obtained stability conditions in terms of a key control parameter defined as a ratio of the coupling strength and the speed of propagation. Depending on the parameters in the problem, give the choice of the partitioned method which allows the largest time step. (C) 2015 Wiley Periodicals, Inc. C1 [Bukac, Martina] Univ Notre Dame, Dept Appl & Computat Math & Stat, Notre Dame, IN 46556 USA. [Layton, William; Moraiti, Marina; Trenchea, Catalin] Univ Pittsburgh, Dept Math, Pittsburgh, PA 15260 USA. [Tran, Hoang] Oak Ridge Natl Lab, Div Math & Comp Sci, Oak Ridge, TN 37831 USA. RP Bukac, M (reprint author), Univ Notre Dame, Dept Appl & Computat Math & Stat, Notre Dame, IN 46556 USA. EM mbukac@nd.edu FU AFOSR [FA 9550-12-1-0191]; [DMS-1216465]; [DMS-1318763] FX Contract grant sponsor: DMS-1216465 (W.L., M.M., and H.T.); Contract grant sponsor: DMS-1318763 (M.B.); Contract grant sponsor: AFOSR (W.L., M.M., H.T., and C.T.); contract grant number: FA 9550-12-1-0191 NR 25 TC 0 Z9 0 U1 1 U2 2 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0749-159X EI 1098-2426 J9 NUMER METH PART D E JI Numer. Meth. Part Differ. Equ. PD NOV PY 2015 VL 31 IS 6 BP 1769 EP 1813 DI 10.1002/num.21968 PG 45 WC Mathematics, Applied SC Mathematics GA CW0DK UT WOS:000364659400003 ER PT J AU Campione, S Luk, TS Liu, S Sinclair, MB AF Campione, Salvatore Luk, Ting S. Liu, Sheng Sinclair, Michael B. TI Optical properties of transiently-excited semiconductor hyperbolic metamaterials SO OPTICAL MATERIALS EXPRESS LA English DT Article ID TOPOLOGICAL TRANSITIONS; NEGATIVE REFRACTION; ABSORPTION; RADIATION; GAAS AB Ultrafast optical excitation of photocarriers has the potential to transform undoped semiconductor superlattices into semiconductor hyperbolic metamaterials (SHMs). In this paper, we investigate the optical properties associated with such ultrafast topological transitions. We first show reflectance, transmittance, and absorption under TE and TM plane wave incidence. In the unpumped state, the superlattice exhibits a frequency region with high reflectance (>80%) and a region with low reflectance (<1%) for both TE and TM polarizations over a wide range of incidence angles. In contrast, in the photopumped state, the reflectance for both frequencies and polarizations is very low (<1%) for a similar range of angles. Interestingly, this system can function as an all-optical reflection switch on ultrafast timescales. Furthermore, for TM incidence and close to the epsilon-near-zero point of the longitudinal permittivity, directional perfect absorption on ultrafast timescales may also be achieved. Finally, we discuss the onset of negative refraction in the photopumped state. (C) 2015 Optical Society of America C1 [Campione, Salvatore; Luk, Ting S.; Liu, Sheng] Sandia Natl Labs, Ctr Integrated Nanotechnol CINT, Albuquerque, NM 87185 USA. [Campione, Salvatore; Luk, Ting S.; Liu, Sheng; Sinclair, Michael B.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Campione, S (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol CINT, POB 5800, Albuquerque, NM 87185 USA. EM sncampi@sandia.gov; mbsincl@sandia.gov FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering and performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 31 TC 3 Z9 3 U1 5 U2 12 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 2159-3930 J9 OPT MATER EXPRESS JI Opt. Mater. Express PD NOV 1 PY 2015 VL 5 IS 11 BP 2385 EP 2394 DI 10.1364/OME.5.002385 PG 10 WC Materials Science, Multidisciplinary; Optics SC Materials Science; Optics GA CV7PY UT WOS:000364467700001 ER PT J AU Ye, M Sun, LB Hu, XL Shi, B Zeng, BB Wang, LS Zhao, J Yang, SM Tai, RZ Fecht, HJ Jiang, JZ Zhang, DX AF Ye, Ming Sun, Libin Hu, Xiaolin Shi, Bin Zeng, Beibei Wang, Liansheng Zhao, Jun Yang, Shumin Tai, Renzhong Fecht, Hans-Jorg Jiang, Jian-Zhong Zhang, Dong-Xian TI Angle-insensitive plasmonic color filters with randomly distributed silver nanodisks SO OPTICS LETTERS LA English DT Article ID EXTRAORDINARY OPTICAL-TRANSMISSION; SUBWAVELENGTH HOLE ARRAYS; LIGHT; DIMERS; FILMS; LIMIT AB Plasmonic color filters inherently suffer from angular sensitiveness, which hinder them from practical applications. Here, we present a plasmonic subtractive color filter incorporating two-dimensional randomly distributed silver nanodisks on top of a glass substrate. Due to the elimination of structural periodicity, the proposed plasmonic color filter works via localized surface plasmon resonances (LSPRs) and thus enables excellent angle-insensitive (up to 60 degrees) performance. In addition, uncoupled LSPRs between nanodisks guarantee stability and reproducibility of the color filter. Finally, a palette of colors across the visible region was obtained with the proposed color filters by simply varying the diameter of nanodisks, exhibiting a promising and robust applicability in digital imaging and sensing industries. (C) 2015 Optical Society of America C1 [Ye, Ming; Sun, Libin; Hu, Xiaolin; Shi, Bin; Zhang, Dong-Xian] Zhejiang Univ, State Key Lab Modern Opt Instrumentat, Hangzhou 310027, Zhejiang, Peoples R China. [Zeng, Beibei] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Wang, Liansheng; Zhao, Jun; Yang, Shumin; Tai, Renzhong] Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201204, Peoples R China. [Fecht, Hans-Jorg] Univ Ulm, Dept Mat, D-89081 Ulm, Germany. [Jiang, Jian-Zhong] Zhejiang Univ, Int Ctr New Struct Mat, State Key Lab Silicon Mat, Hangzhou 310027, Zhejiang, Peoples R China. [Jiang, Jian-Zhong] Zhejiang Univ, Sch Mat Sci & Engn, Hangzhou 310027, Zhejiang, Peoples R China. RP Zhang, DX (reprint author), Zhejiang Univ, State Key Lab Modern Opt Instrumentat, Hangzhou 310027, Zhejiang, Peoples R China. EM zhangdx@zju.edu.cn RI Zhejiang University, Dep. Optical Eng./G-9022-2011 FU China Scholarship Council (CSC) [201400260166]; National Key Basic Research Program of China [2012CB825700]; National Natural Science Foundation of China (NSFC) [51371157, U1432105, U1432110] FX China Scholarship Council (CSC) (201400260166); National Key Basic Research Program of China (2012CB825700); National Natural Science Foundation of China (NSFC) (51371157, U1432105, U1432110). NR 27 TC 7 Z9 7 U1 5 U2 34 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 0146-9592 EI 1539-4794 J9 OPT LETT JI Opt. Lett. PD NOV 1 PY 2015 VL 40 IS 21 BP 4979 EP 4982 DI 10.1364/OL.40.004979 PG 4 WC Optics SC Optics GA CV7QH UT WOS:000364468600040 PM 26512498 ER PT J AU Gift, TL Haderxhanaj, LT Torrone, EA Behl, AS Romaguera, RA Leichliter, JS AF Gift, Thomas L. Haderxhanaj, Laura T. Torrone, Elizabeth A. Behl, Ajay S. Romaguera, Raul A. Leichliter, Jami S. TI Estimating the Size and Cost of the STD Prevention Services Safety Net SO PUBLIC HEALTH REPORTS LA English DT Article ID TRANSMITTED-DISEASE SERVICES; CHLAMYDIA-TRACHOMATIS; REPEAT INFECTION; UNITED-STATES; GONORRHEA; WOMEN; MEN; TRENDS AB The Patient Protection and Affordable Care Act is expected to reduce the number of uninsured people in the United States during the next eight years, but more than 10% are expected to remain uninsured. Uninsured people are one of the main populations using publicly funded safety net sexually transmitted disease (STD) prevention services. Estimating the proportion of the uninsured population expected to need STD services could help identify the potential demand for safety net STD services and improve program planning. In 2013, an estimated 8.27 million people met the criteria for being in need of STD services. In 2023, 4.70 million uninsured people are expected to meet the criteria for being in need of STD services. As an example, the cost in 2014 U.S. dollars of providing chlamydia screening to these people was an estimated $271.1 million in 2013 and is estimated to be $153.8 million in 2023. A substantial need will continue to exist for safety net STD prevention services in coming years. C1 [Gift, Thomas L.; Torrone, Elizabeth A.; Romaguera, Raul A.; Leichliter, Jami S.] Ctr Dis Control & Prevent, Div STD Prevent, Atlanta, GA 30333 USA. [Haderxhanaj, Laura T.] Ctr Dis Control & Prevent, ORISE, Atlanta, GA 30333 USA. [Behl, Ajay S.] Hlth Partners Inst Res & Educ, Minneapolis, MN USA. RP Gift, TL (reprint author), Ctr Dis Control & Prevent, Div STD Prevent, 1600 Clifton Rd NE,MS E-80, Atlanta, GA 30333 USA. EM tgift@cdc.gov NR 30 TC 1 Z9 1 U1 1 U2 1 PU ASSOC SCHOOLS PUBLIC HEALTH PI WASHINGTON PA 1900 M ST NW, STE 710, WASHINGTON, DC 20036 USA SN 0033-3549 J9 PUBLIC HEALTH REP JI Public Health Rep. PD NOV-DEC PY 2015 VL 130 IS 6 BP 602 EP 609 PG 8 WC Public, Environmental & Occupational Health SC Public, Environmental & Occupational Health GA CV8CI UT WOS:000364503700008 PM 26556931 ER PT J AU Juhas, P Farrow, CL Yang, XH Knox, KR Billinge, SJL AF Juhas, Pavol Farrow, Christopher L. Yang, Xiaohao Knox, Kevin R. Billinge, Simon J. L. TI Complex modeling: a strategy and software program for combining multiple information sources to solve ill posed structure and nanostructure inverse problems SO ACTA CRYSTALLOGRAPHICA A-FOUNDATION AND ADVANCES LA English DT Article DE complex modeling; nanostructure analysis; Python software framework ID PAIR DISTRIBUTION FUNCTION; NANOPARTICLES; SCATTERING; NANOSCALE; FRAMEWORK AB A strategy is described for regularizing ill posed structure and nanostructure scattering inverse problems (i.e. structure solution) from complex material structures. This paper describes both the philosophy and strategy of the approach, and a software implementation, DiffPy Complex Modeling Infrastructure (DiffPy-CMI). C1 [Juhas, Pavol; Knox, Kevin R.; Billinge, Simon J. L.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Farrow, Christopher L.; Yang, Xiaohao; Billinge, Simon J. L.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. RP Billinge, SJL (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. EM sb2896@columbia.edu OI Juhas, Pavol/0000-0001-8751-4458 FU US National Science Foundation [DMR-0520547]; Laboratory Directed Research and Development (LDRD) Program (Complex Modeling) at Brookhaven National Laboratory - US Department of Energy Office of Basic Energy Sciences [12007, DE-SC00112704] FX Early development of the software was carried out under the DANSE software development project funded by the US National Science Foundation through award DMR-0520547. Since 2012, the project has been funded as Laboratory Directed Research and Development (LDRD) Program 12007 (Complex Modeling) at Brookhaven National Laboratory, which is funded by the US Department of Energy Office of Basic Energy Sciences grant DE-SC00112704. NR 40 TC 11 Z9 11 U1 2 U2 12 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 2053-2733 J9 ACTA CRYSTALLOGR A JI Acta Crystallogr. Sect. A PD NOV PY 2015 VL 71 BP 562 EP 568 DI 10.1107/S2053273315014473 PN 6 PG 7 WC Chemistry, Multidisciplinary; Crystallography SC Chemistry; Crystallography GA CV4GX UT WOS:000364226200002 PM 26522405 ER PT J AU Breault, RW Monazam, ER Carpenter, JT AF Breault, Ronald W. Monazam, Esmail R. Carpenter, Jared T. TI Analysis of hematite re-oxidation in the chemical looping process SO APPLIED ENERGY LA English DT Article DE Chemical Looping Combustion; Fixed bed reactor; Hematite re-oxidation ID OXYGEN CARRIER; IRON-OXIDE; COMBUSTION; REDUCTION; PARTICLES; KINETICS AB Very little attention has been dedicated to the carrier re-oxidation in chemical looping systems. The work presented in this paper is for the re-oxidation of partially reduced hematite from a cyclic chemical looping fixed bed process. The underlying purpose of this work is to develop engineering rates and mechanisms for the re-oxidation of partially reduced hematite that can be included in CFD models for a chemical looping process. To this end, experiments were run using nominally 1000 g of hematite material in a fixed bed reactor cycling between reduction and re-oxidation. The cyclic processing began with the reduction step then proceeded to the oxidation step repeating this analysis for several cycles ranging from 5 to 10. The re-oxidation process was conducted at temperatures ranging from 745 degrees C to 825 degrees C and oxygen concentrations ranging between 9% and 11%. The reduction was carried out at the same temperature as the re-oxidation step at various CH4 concentrations from 5% to 9%. In this paper, cyclic induced variations in performance are presented as well as the kinetic parameters for the first cycle. The re-oxidation of the depleted hematite occurs through a 2 step parallel process in which oxygen reacts to fill the surface of each grain within the particles and then migrates through oxygen vacancy diffusion to the depleted cores of each grain. Published by Elsevier Ltd. C1 [Breault, Ronald W.; Carpenter, Jared T.] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. [Monazam, Esmail R.] REM Engn Serv PLLC, Morgantown, WV 26507 USA. RP Breault, RW (reprint author), NETL DoE, POB 880, Morgantown, WV 26507 USA. EM ronald.breault@netl.doe.gov FU Department of Energy through the office of Fossil Energy FX The authors acknowledge the Department of Energy for funding the research through the office of Fossil Energy's Gasification Technology and Advanced Research funding programs. Special thanks go to Duane Miller and Rich Eddy of URS Energy & Construction, Inc. for their assistance with experimental work and data collection and to Dave Huckaby and Justin Weber for their insight on the kinetic discussion. NR 36 TC 1 Z9 1 U1 3 U2 16 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD NOV 1 PY 2015 VL 157 BP 174 EP 182 DI 10.1016/j.apenergy.2015.08.015 PG 9 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA CV4PO UT WOS:000364249200016 ER PT J AU Siriwardane, R Tian, HJ Miller, D Richards, G AF Siriwardane, Ranjani Tian, Hanjing Miller, Duane Richards, George TI Fluidized bed testing of commercially prepared MgO-promoted hematite and CuO-Fe2O3 mixed metal oxide oxygen carriers for methane and coal chemical looping combustion SO APPLIED ENERGY LA English DT Article DE Oxygen carriers; Chemical looping combustion; Commercial scale preparation of oxygencarriers; Fluidized bed testing of oxygen carriers ID SYNTHESIS GAS; REACTOR; NI; KINETICS; HYDROGEN; FE; CU; REDUCTION; PARTICLES; FE2O3 AB Performance data of two commercially prepared oxygen carriers, MgO-promoted natural mineral hematite (Fe2O3) and synthetic mixed metal cuO-Fe2O3/alumina, are described in this paper. Large, 180-kg (400-pound) batches of both oxygen carriers were successfully prepared at a commercial catalyst preparation facility. These carriers have shown excellent reactivity and stable performance during cyclic chemical-looping combustion (CLC) tests conducted with methane/air at 700-850 degrees C in an atmospheric fluid bed reactor. Attrition resistance of both oxygen carriers with particle size of 100-150 gm, measured using the ASTM 5757D method, was better than that of standard fluidized bed cracking catalysts. The presence of MgO on the hematite oxygen carrier significantly improved the oxygen utilization of hematite for methane CLC. The CuO-Fe2O3/alumina oxygen carrier showed excellent performance during the 25-cycle fluidized bed CLC test conducted at 800 degrees C with methane and air. Full combustion of methane to CO2 and stable oxygen transfer capacity were observed during all the cycles. The fluidization of this material was easy, with no particle agglomeration as is traditionally observed with CuO-containing materials. Fluidized bed temperature programmed reaction tests with coal were also conducted with both materials. Published by Elsevier Ltd. C1 [Siriwardane, Ranjani; Tian, Hanjing; Miller, Duane; Richards, George] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. [Tian, Hanjing] W Virginia Univ, Dept Chem Engn, Morgantown, WV 26506 USA. RP Siriwardane, R (reprint author), US DOE, Natl Energy Technol Lab, 3610 Collins Ferry Rd, Morgantown, WV 26507 USA. EM ranjani.siriwardane@netl.doe.gov NR 42 TC 3 Z9 4 U1 8 U2 34 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD NOV 1 PY 2015 VL 157 BP 348 EP 357 DI 10.1016/j.apenergy.2015.04.042 PG 10 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA CV4PO UT WOS:000364249200033 ER PT J AU Saxena, S MacDonald, J Moura, S AF Saxena, Samveg MacDonald, Jason Moura, Scott TI Charging ahead on the transition to electric vehicles with standard 120 V wall outlets SO APPLIED ENERGY LA English DT Article DE Electric vehicles; Range anxiety; EV charging; EV range; Clean transportation ID INFRASTRUCTURE; CONSUMPTION; RECHARGE; IMPACTS AB Electrification of transportation is needed soon and at significant scale to meet climate goals, but electric vehicle adoption has been slow and there has been little systematic analysis to show that today's electric vehicles meet the needs of drivers. We apply detailed physics-based models of electric vehicles with data on how drivers use their cars on a daily basis. We show that the energy storage limits of today's electric vehicles are outweighed by their high efficiency and the fact that driving in the United States seldom exceeds 100 km of daily travel. When accounting for these factors, we show that the normal daily travel of 85-89% of drivers in the United States can be satisfied with electric vehicles charging with standard 120 V wall outlets at home only. Further, we show that 77-79% of drivers on their normal daily driving will have over 60 km of buffer range for unexpected trips. We quantify the sensitivities to terrain, high ancillary power draw, and battery degradation and show that an extreme case with all trips on a 3% uphill grade still shows the daily travel of 70% of drivers being satisfied with electric vehicles. These findings show that today's electric vehicles can satisfy the daily driving needs of a significant majority of drivers using only 120 V wall outlets that are already the standard across the United States. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Saxena, Samveg; MacDonald, Jason] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Moura, Scott] Univ Calif Berkeley, Berkeley, CA 94720 USA. RP Saxena, S (reprint author), Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM samveg@berkeley.edu FU Laboratory Directed Research & Development program at Lawrence Berkeley National Laboratory; Office of Science, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported with funding through the Laboratory Directed Research & Development program at Lawrence Berkeley National Laboratory, by the Director, Office of Science, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 31 TC 9 Z9 9 U1 0 U2 7 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD NOV 1 PY 2015 VL 157 BP 720 EP 728 DI 10.1016/j.apenergy.2015.05.005 PG 9 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA CV4PO UT WOS:000364249200070 ER PT J AU Gao, ZM Curran, SJ Parks, JE Smith, DE Wagner, RM Daw, CS Edwards, KD Thomas, JF AF Gao, Zhiming Curran, Scott J. Parks, James E., II Smith, David E. Wagner, Robert M. Daw, C. Stuart Edwards, K. Dean Thomas, John F. TI Drive cycle simulation of high efficiency combustions on fuel economy and exhaust properties in light-duty vehicles SO APPLIED ENERGY LA English DT Article DE Fuel economy; Emissions; Engine efficiency; Hybrid vehicle; Drive cycle ID COMPRESSION IGNITION; GDI ENGINE; EMISSIONS; GASOLINE; DIESEL; SYSTEM; IMPACT AB Results from computational simulations of fuel economy and engine-out emissions are presented for light-duty conventional and hybrid vehicles powered by conventional and high-efficiency combustion engines, including use of port fuel-injected, lean gasoline direct injection, reactivity controlled compression ignition, and conventional diesel combustion. The results indicate that multimode operation with conventional diesel combustion plus reactivity controlled compression ignition, conventional diesel combustion only, and lean gasoline direct injection has the potential to significantly exceed port fuel-injected fuel economy. In all cases, hybridization is predicted to significantly improve fuel economy by permitting the maximum exploitation of high efficiency engine combustion states. Predicted engine-out emissions vary considerably with combustion mode, with reactivity controlled compression ignition generating the highest carbon monoxide and hydrocarbon emissions. On the other hand, reactivity controlled compression ignition is predicted to generate the lowest emissions of nitrogen oxides. Importantly, lean gasoline direct injection and reactivity controlled compression ignition combustion modes are expected to dramatically decrease exhaust temperatures, especially for reactivity controlled compression ignition, which can potentially limit aftertreatment performance. While all results presented are from simulations, the results provide prediction of important details and trends for advanced vehicles that are currently extremely difficult to experimentally study. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Gao, Zhiming; Curran, Scott J.; Parks, James E., II; Smith, David E.; Wagner, Robert M.; Daw, C. Stuart; Edwards, K. Dean; Thomas, John F.] Oak Ridge Natl Lab, Natl Transportat Res Ctr, Knoxville, TN 37932 USA. RP Gao, ZM (reprint author), Oak Ridge Natl Lab, Natl Transportat Res Ctr, 2360 Cherahala Blvd, Knoxville, TN 37932 USA. EM gaoz@ornl.gov OI Curran, Scott/0000-0002-4665-0231; Gao, Zhiming/0000-0002-7139-7995 FU Office of Vehicle Technologies in the U.S. Department of Energy; U.S. Department of Energy [DE-AC05-00OR22725]; United States Government FX We are indebted to the Office of Vehicle Technologies in the U.S. Department of Energy for supporting this research. We are also grateful to our colleagues at ORNL, who contributed helpful suggestions and insights. Thanks also go to the reviewers for their time and effort.; This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http:// energy.gov/downloads/doe-public-access-plan). NR 43 TC 2 Z9 2 U1 6 U2 16 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD NOV 1 PY 2015 VL 157 BP 762 EP 776 DI 10.1016/j.apenergy.2015.03.070 PG 15 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA CV4PO UT WOS:000364249200074 ER PT J AU Erchinger, JL Aalseth, CE Bernacki, BE Douglas, M Fuller, ES Keillor, ME Morley, SM Mullen, CA Orrell, JL Panisko, ME Warren, GA Williams, RO Wright, ME AF Erchinger, J. L. Aalseth, C. E. Bernacki, B. E. Douglas, M. Fuller, E. S. Keillor, M. E. Morley, S. M. Mullen, C. A. Orrell, J. L. Panisko, M. E. Warren, G. A. Williams, R. O. Wright, M. E. TI Development of a low background liquid scintillation counter for a shallow underground laboratory SO APPLIED RADIATION AND ISOTOPES LA English DT Article DE Liquid scintillation counting; Low background; Shallow underground laboratory ID SPECTROMETRY; CONSTRUCTION; IMPURITIES; AC-227 AB Pacific Northwest National Laboratory has recently opened a shallow underground laboratory intended for measurement of low-concentration levels of radioactive isotopes in samples collected from the environment. The development of a low-background liquid scintillation counter is currently underway to further augment the measurement capabilities within this underground laboratory. Liquid scintillation counting is especially useful for measuring charged particle (e.g., beta and alpha) emitting isotopes with no (or very weak) gamma-ray yields. The combination of high-efficiency detection of charged particle emission in a liquid scintillation cocktail coupled with the low-background environment of an appropriately designed shield located in a clean underground laboratory provides the opportunity for increased-sensitivity measurements of a range of isotopes. To take advantage of the 35 m-water-equivalent overburden of the underground laboratory, a series of simulations have evaluated the scintillation counter's shield design requirements to assess the possible background rate achievable. This report presents the design and background evaluation for a shallow underground, low background liquid scintillation counter design for sample measurements. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Erchinger, J. L.; Aalseth, C. E.; Bernacki, B. E.; Douglas, M.; Fuller, E. S.; Keillor, M. E.; Morley, S. M.; Mullen, C. A.; Orrell, J. L.; Panisko, M. E.; Warren, G. A.; Williams, R. O.; Wright, M. E.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Erchinger, J. L.] Texas A&M Univ, College Stn, TX 77840 USA. [Williams, R. O.] Wittenberg Univ, Springfield, OH 45504 USA. RP Erchinger, JL (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM jennifer.erchinger@pnnl.gov RI Orrell, John/E-9313-2015; OI Orrell, John/0000-0001-7968-4051; Keillor, Martin/0000-0001-7828-5868; Douglas, Matthew/0000-0001-9708-1780 NR 29 TC 2 Z9 2 U1 0 U2 3 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0969-8043 J9 APPL RADIAT ISOTOPES JI Appl. Radiat. Isot. PD NOV PY 2015 VL 105 BP 209 EP 218 DI 10.1016/j.apradiso.2015.08.027 PG 10 WC Chemistry, Inorganic & Nuclear; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging SC Chemistry; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging GA CV4RK UT WOS:000364254000035 PM 26334781 ER PT J AU McManamay, RA Peoples, BK Orth, DJ Dolloff, CA Matthews, DC AF McManamay, Ryan A. Peoples, Brandon K. Orth, Donald J. Dolloff, Charles A. Matthews, David C. TI Isolating causal pathways between flow and fish in the regulated river hierarchy SO CANADIAN JOURNAL OF FISHERIES AND AQUATIC SCIENCES LA English DT Article ID LIFE-HISTORY STRATEGIES; MODIFYING DAM OPERATIONS; UNITED-STATES; STREAM FISHES; POPULATION REGULATION; ECOLOGICAL RESPONSES; ENVIRONMENTAL FLOWS; ASSEMBLAGE RESPONSE; HABITAT USE; REGIMES AB Unregulated river systems are organized in a hierarchy in which large-scale factors (i.e., landscape and segment scales) influence local habitats (i.e., reach, meso-, and microhabitat scales), and both differentially exert selective pressures on biota. Dams, however, create discontinua in these processes and change the hierarchical structure. We examined the relative roles of hydrology and other instream factors, within a hierarchical landscape context, in organizing fish communities in regulated and unregulated tributaries to the Upper Tennessee River, USA. We used multivariate regression trees to identify factors that partition fish assemblages based on trait similarities, irrespective of spatial scale. We then used classical path analysis and structural equation modeling to evaluate the most plausible hierarchical causal structure of specific trait-based community components, given the data. Both statistical approaches suggested that river regulation affects stream fishes through a variety of reach-scale variables, not always through hydrology itself. Although we observed different changes in flow, temperature, and biotic responses according to regulation types, the most predominant path in which dam regulation affected biota was via temperature alterations. Diversion dams had the strongest effects on fish assemblages. Diversion dams reduced flow magnitudes, leading to declines in fish richness but increased temperatures, leading to lower abundances in equilibrium species and nest guarders. Peaking and run-of-river dams increased flow variability, leading to lower abundances in nest-guarding fishes. Flow displayed direct relationships with biotic responses; however, results indicated that changes in temperature and substrate had equal, if not stronger, effects on fish assemblage composition. The strength and nature of relationships depended on whether flow metrics were standardized for river size. We suggest that restoration efforts in regulated rivers focus on improving flow conditions in conjunction with temperature and substrate restoration. C1 [McManamay, Ryan A.] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Peoples, Brandon K.; Orth, Donald J.] Virginia Tech, Dept Fish & Wildlife Conservat, Blacksburg, VA 24061 USA. [Dolloff, Charles A.] US Forest Serv, USDA, Dept Fish & Wildlife Conservat, Virginia Tech, Blacksburg, VA 24061 USA. [Matthews, David C.] Tennessee Valley Author, Knoxville, TN 37902 USA. RP McManamay, RA (reprint author), Oak Ridge Natl Lab, Div Environm Sci, POB 2008 MS6351, Oak Ridge, TN 37831 USA. EM mcmanamayra@ornl.gov OI Orth, Donald/0000-0002-9236-0147 FU Cheoah Fund Board; USDA Forest Service; US Department of Energy [DE-AC05-00OR22725] FX This work was funded by the Cheoah Fund Board, a multiagency collaboration between Alcoa Power, USDA Forest Service, US Fish and Wildlife Service, North Carolina Wildlife Resources Commission, and the NC Division of Water Resources-DENR, and by other grants provided by the USDA Forest Service. We are thankful for the valuable input from Paul Angermeier and Emmanuel Frimpong on earlier versions of this work. In addition, we thank Charles Saylor for his comments concerning fish assemblage sampling procedures. We also thank Tyler Young, Toby Coyner, David Belkoski, and Adam Hart for their assistance with field work. This manuscript has been authored by an employee of UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the US Department of Energy. The publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 95 TC 3 Z9 3 U1 8 U2 35 PU CANADIAN SCIENCE PUBLISHING, NRC RESEARCH PRESS PI OTTAWA PA 65 AURIGA DR, SUITE 203, OTTAWA, ON K2E 7W6, CANADA SN 0706-652X EI 1205-7533 J9 CAN J FISH AQUAT SCI JI Can. J. Fish. Aquat. Sci. PD NOV PY 2015 VL 72 IS 11 BP 1731 EP 1748 DI 10.1139/cjfas-2015-0227 PG 18 WC Fisheries; Marine & Freshwater Biology SC Fisheries; Marine & Freshwater Biology GA CV2RL UT WOS:000364104300012 ER PT J AU Liu, YN Hussaini, Y Okten, G AF Liu, Yaning Hussaini, Yousuff Oekten, Giray TI Global sensitivity analysis for the Rothermel model based on high-dimensional model representation SO CANADIAN JOURNAL OF FOREST RESEARCH LA English DT Article DE Rothermel fire spread model; global sensitivity analysis; high-dimensional model representation; Monte Carlo methods; ANOVA ID PARAMETRIC UNCERTAINTY; FIRE; INDEXES AB Rothermel's wildland surface fire spread model is widely used in North America. The model outputs depend on a number of input parameters, which can be broadly categorized as fuel model, fuel moisture, terrain, and wind parameters. Due to the inevitable presence of uncertainty in the input parameters, knowing the sensitivity of the model output to a given input parameter can be very useful for understanding and controlling the sources of parametric uncertainty. Instead of obtaining the local sensitivity indices, we perform a global sensitivity analysis that considers the synchronous changes of parameters in their respective ranges. The global sensitivity indices corresponding to different parameter groups are computed by constructing the truncated ANOVA - high dimensional model representation for the model outputs with a polynomial expansion approach. We apply global sensitivity analysis to six standard fuel models, namely short grass, tall grass, chaparral, hardwood litter, timber, and light logging slash. Our sensitivity results show similarities, as well as differences, between fuel models. For example, the sensitivities of the input parameters, i.e., fuel depth, low heat content, and wind, are large in all fuel models and as high as 85% of the total model variance in the fuel model light logging slash. On the other hand, the fuel depth explains around 40% of the total variance in the fuel model light logging slash but only 12% of the total variance in the fuel model short grass. The quantification of the importance of parameters across fuel models helps identify the parameters for which additional resources should be used to lower their uncertainty, leading to effective fire management. C1 [Liu, Yaning] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Hussaini, Yousuff; Oekten, Giray] Florida State Univ, Dept Math, Tallahassee, FL 32306 USA. RP Okten, G (reprint author), Florida State Univ, Dept Math, Tallahassee, FL 32306 USA. EM okten@math.fsu.edu RI Liu, Yaning/K-8547-2014 NR 27 TC 1 Z9 1 U1 1 U2 4 PU CANADIAN SCIENCE PUBLISHING, NRC RESEARCH PRESS PI OTTAWA PA 65 AURIGA DR, SUITE 203, OTTAWA, ON K2E 7W6, CANADA SN 0045-5067 EI 1208-6037 J9 CAN J FOREST RES JI Can. J. For. Res. PD NOV PY 2015 VL 45 IS 11 BP 1474 EP 1479 DI 10.1139/cjfr-2015-0148 PG 6 WC Forestry SC Forestry GA CV0KF UT WOS:000363938900004 ER PT J AU Firdous, T Vick, D Belov, M Sani, FF McDermott, A Losby, JE Bazylinski, DA Prozorov, T Potter, DK Freeman, MR AF Firdous, T. Vick, D. Belov, M. Sani, F. Fani McDermott, A. Losby, J. E. Bazylinski, D. A. Prozorov, T. Potter, D. K. Freeman, M. R. TI Nanomechanical torque magnetometry of an individual aggregate of similar to 350 nanoparticles SO CANADIAN JOURNAL OF PHYSICS LA English DT Article ID MAGNETIC NANOPARTICLES; MAGNETOTACTIC BACTERIA; SENSORS; RESONATORS; ASSEMBLIES AB The measurements of magnetic hysteresis for aggregates of nanoparticles deposited on a surface are reported. Magnetite nanoparticles derived from magnetotactic bacteria are studied using nanomechanical torque magnetometry. The nanoparticles are deposited on high-stress Si3N4 membranes, to allow inspection by electron microscopy, followed by focused ion-beam milling of torsional resonators precisely located to capture selected aggregates within the membrane area. Torque magnetometry is performed using the resonators. We investigate also the magnetic torque-driven AC resonant modes of the modified supporting membrane. The observations are compared to numerical simulations of the mechanical modes, and to micromagnetic modeling of the hysteresis of a specific measured cluster of similar to 350 nanoparticles. C1 [Firdous, T.; Sani, F. Fani; McDermott, A.; Losby, J. E.; Potter, D. K.; Freeman, M. R.] Univ Alberta, Dept Phys, Edmonton, AB T6G 2E1, Canada. [Firdous, T.; Vick, D.; Belov, M.; Sani, F. Fani; Losby, J. E.; Freeman, M. R.] Natl Inst Nanotechnol, Edmonton, AB T6G 2M9, Canada. [Bazylinski, D. A.] Univ Nevada, Sch Life Sci, Las Vegas, NV 89154 USA. [Prozorov, T.] US DOE, Ames Lab, Ames, IA 50011 USA. RP Freeman, MR (reprint author), Univ Alberta, Dept Phys, 4-181 CCIS, Edmonton, AB T6G 2E1, Canada. EM freemanm@ualberta.ca FU Alberta Innovates - Technology Futures iCORE iCiNano Project; National Institute for Nanotechnology; Natural Sciences and Engineering Research Council, Canada FX This work was supported by Alberta Innovates - Technology Futures iCORE iCiNano Project, the National Institute for Nanotechnology, and the Natural Sciences and Engineering Research Council, Canada. NR 30 TC 1 Z9 1 U1 1 U2 8 PU CANADIAN SCIENCE PUBLISHING, NRC RESEARCH PRESS PI OTTAWA PA 65 AURIGA DR, SUITE 203, OTTAWA, ON K2E 7W6, CANADA SN 0008-4204 EI 1208-6045 J9 CAN J PHYS JI Can. J. Phys. PD NOV PY 2015 VL 93 IS 11 BP 1252 EP 1256 DI 10.1139/cjp-2014-0722 PG 5 WC Physics, Multidisciplinary SC Physics GA CV2RI UT WOS:000364103900006 ER PT J AU Devereux, M AF Devereux, Michael TI Reduction of the atomic wavefunction in the Stern-Gerlach magnetic field SO CANADIAN JOURNAL OF PHYSICS LA English DT Article ID QUANTUM-MECHANICS; INTERFEROMETRY; QUANTIZATION AB Observation of two separated beam spots at a detection screen downstream of a Stern-Gerlach magnet does not, in fact, demonstrate that the wavefunction of a neutral spin one-half particle has remained in a spin superposition while traveling through that magnetic field. The wavefunction may have been reduced to just one spin-direction eigenfunction, as D. Bohm suggested, by immediate momentum and energy transfer with the magnet, rather than by subsequent, which-way determination at the screen. The same two beam spots at the detector screen will result. Einsteinian relativity, and the understanding of Schrodinger evolution applicability through a static potential, forbid continuation of a spin superposition through the Stern-Gerlach field. A calculation for single wavepacket development there conforms to observations from the Stern-Gerlach experiment. And several experiments corroborate immediate reduction to a single spin eigenfunction in the magnetic field. Additionally, Ramsey's separated, oscillating fields observations, and related experiments, do not rebut this understanding. C1 [Devereux, Michael] Los Alamos Natl Lab, Los Alamos, NM 87544 USA. RP Devereux, M (reprint author), 1373 40th St, Los Alamos, NM 87544 USA. EM d_bar_x@centurylink.net NR 41 TC 3 Z9 3 U1 1 U2 9 PU CANADIAN SCIENCE PUBLISHING, NRC RESEARCH PRESS PI OTTAWA PA 65 AURIGA DR, SUITE 203, OTTAWA, ON K2E 7W6, CANADA SN 0008-4204 EI 1208-6045 J9 CAN J PHYS JI Can. J. Phys. PD NOV PY 2015 VL 93 IS 11 BP 1382 EP 1390 DI 10.1139/cjp-2015-0031 PG 9 WC Physics, Multidisciplinary SC Physics GA CV2RI UT WOS:000364103900027 ER PT J AU Bruno, C Sankaran, V Kolla, H Chen, JH AF Bruno, Claudio Sankaran, Vaidyanathan Kolla, Hemanth Chen, Jacqueline H. TI Impact of multi-component diffusion in turbulent combustion using direct numerical simulations SO COMBUSTION AND FLAME LA English DT Article DE Premixed turbulent combustion; Molecular diffusion; Multi-component diffusion ID PREMIXED CH4/AIR FLAMES; DIFFERENTIAL DIFFUSION; PREFERENTIAL TRANSPORT; SPONTANEOUS RAMAN; SCATTERING; CHEMISTRY; FLOWS AB This paper presents the results of DNS of a partially premixed turbulent syngas/air flame at atmospheric pressure. The objective was to assess the importance and possible effects,of molecular transport on flame behavior and structure. To this purpose DNS were performed at with two proprietary DNS codes and with three different molecular diffusion transport models: fully multi-component, mixture averaged, and imposing the Lewis number of all species to be unity. Results indicate that 1. At the Reynolds numbers of the simulations (Re-turb = 600, Re = 8000) choice of molecular diffusion models affects significantly the temperature and concentration fields; 2. Assuming Le = 1 for all species predicts temperatures up to 250 K higher than the physically realistic multi-component model; 3. Faster molecular transport of lighter species changes the local concentration field and affects reaction pathways and chemical kinetics. A possible explanation for these observations is provided in terms of species diffusion velocity that is a strong function of gradients: thus, at sufficiently large Reynolds numbers, gradients and their effects tend to be large. The preliminary conclusion from these simulations seems to indicate molecular diffusion as the third important mechanism active in flames besides convective transport and kinetics. If confirmed by further DNS and measurements, molecular transport in high intensity turbulent flames will have to be realistically modeled to accurately predict emissions (gaseous and particulates) and other combustor performance metrics. (C) 2015 Published by Elsevier Inc. on behalf of The Combustion Institute. C1 [Bruno, Claudio; Sankaran, Vaidyanathan] United Technol Res Ctr, E Hartford, CT 06108 USA. [Kolla, Hemanth; Chen, Jacqueline H.] Sandia Natl Labs, Livermore, CA USA. RP Bruno, C (reprint author), United Technol Res Ctr, 411 Silver Lane, E Hartford, CT 06108 USA. EM brunoc@utrc.utc.com FU US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences; US Department of Energy [DE-AC04-94-AL85000]; Office of Science of the US DOE [DE-AC02-05CH11231, DE-AC05-00OR22725] FX The authors wish to thank Dr. Catalin Fotache and Dr. Joe Sangiovanni for supporting this work internally and for useful technical discussions. The authors also wish to thank Dr. Jeremiah Lee for many in-depth discussions on the subject of SGS models of multicomponent diffusion. Special thanks are due to Dr. Robert Barlow at Sandia National Laboratories, Livermore, CA for information and clarification of experimental data found by his team. The research at UTRC was supported by the Director's funding and the research at Sandia was sponsored by the US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences. Sandia National Laboratories is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the US Department of Energy, under Contract DE-AC04-94-AL85000. This research used computational resources of the National Energy Research Computing Center (NERSC) and of the National Center for Computational Sciences at Oak Ridge National Laboratory (NCCS/ORNL) supported by The Office of Science of the US DOE under Contract Nos. DE-AC02-05CH11231 and DE-AC05-00OR22725 and through the director's discretionary access computer time awarded to UTRC. NR 42 TC 3 Z9 3 U1 3 U2 6 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0010-2180 EI 1556-2921 J9 COMBUST FLAME JI Combust. Flame PD NOV PY 2015 VL 162 IS 11 BP 4313 EP 4330 DI 10.1016/j.combustflame.2015.07.013 PG 18 WC Thermodynamics; Energy & Fuels; Engineering, Multidisciplinary; Engineering, Chemical; Engineering, Mechanical SC Thermodynamics; Energy & Fuels; Engineering GA CV1FE UT WOS:000363998300020 ER PT J AU Beckman, P AF Beckman, Pete TI Our Dynamic Future SO COMPUTING IN SCIENCE & ENGINEERING LA English DT Editorial Material C1 [Beckman, Pete] Argonne Natl Lab, Argonne, IL 60439 USA. [Beckman, Pete] Northwestern Univ, Evanston, IL 60208 USA. RP Beckman, P (reprint author), Argonne Natl Lab, Argonne, IL 60439 USA. EM beckman@anl.gov NR 0 TC 0 Z9 0 U1 1 U2 1 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 1521-9615 EI 1558-366X J9 COMPUT SCI ENG JI Comput. Sci. Eng. PD NOV-DEC PY 2015 VL 17 IS 6 BP 88 EP 90 PG 3 WC Computer Science, Interdisciplinary Applications SC Computer Science GA CV4IE UT WOS:000364229600014 ER PT J AU Hoversten, GM Commer, M Haber, E Schwarzbach, C AF Hoversten, G. Michael Commer, Michael Haber, Eldad Schwarzbach, Christoph TI Hydro-frac monitoring using ground time-domain electromagnetics SO GEOPHYSICAL PROSPECTING LA English DT Article AB As motivation for considering new electromagnetic techniques for hydraulic fracture monitoring, we develop a simple financial model for the net present value offered by geophysical characterization to reduce the error in stimulated reservoir volume calculations. This model shows that even a 5% improvement in stimulated reservoir volume for a 1 billion barrel (bbl.) field results in over 1 billion U.S. dollars (US$) in net present value over 24 years for US$100/bbl. oil and US$0.5 billion for US$50/bbl. oil. The application of conductivity upscaling, often used in electromagnetic modeling to reduce mesh size and thus simulation runtimes, is shown to be inaccurate for the high electrical contrasts needed to represent steel-cased wells in the earth. Fine-scale finite-difference modeling with 12.22-mm cells to capture the steel casing and fractures shows that the steel casing provides a direct current pathway to a created fracture that significantly enhances the response compared with neglecting the steel casing. We consider conductively enhanced proppant, such as coke-breeze-coated sand, and a highly saline brine solution to produce electrically conductive fractures. For a relatively small frac job at a depth of 3 km, involving 5,000 bbl. of slurry and a source midpoint to receiver separation of 50 m, the models show that the conductively enhanced proppant produces a 15% increase in the electric field strength (in-line with the transmitter) in a 10-m background. In a 100-m background, the response due to the proppant increases to 213%. Replacing the conductive proppant by brine with a concentration of 100,000-ppm NaCl, the field strength is increased by 23% in the 100-m background and by 2.3% in the 10-m background. All but the 100,000-ppm NaCl brine in a 10-m background produce calculated fracture-induced electric field increases that are significantly above 2%, a value that has been demonstrated to be observable in field measurements. C1 [Hoversten, G. Michael] Chevron Energy Technol Co, San Ramon, CA 94583 USA. [Commer, Michael] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Haber, Eldad; Schwarzbach, Christoph] Univ British Columbia, Dept Earth & Ocean Sci, Vancouver, BC V6T 1Z4, Canada. RP Hoversten, GM (reprint author), Chevron Energy Technol Co, 6001 Bollinger Canyon Rd,Build K1010, San Ramon, CA 94583 USA. EM hovg@chevron.com RI Commer, Michael/G-3350-2015 OI Commer, Michael/0000-0003-0015-9217 NR 18 TC 0 Z9 0 U1 1 U2 11 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0016-8025 EI 1365-2478 J9 GEOPHYS PROSPECT JI Geophys. Prospect. PD NOV PY 2015 VL 63 IS 6 BP 1508 EP 1526 DI 10.1111/1365-2478.12300 PG 19 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CU9TA UT WOS:000363886900013 ER PT J AU Hamada, Y Grippo, MA AF Hamada, Yuki Grippo, Mark A. TI Erosion Resistance Index (ERI) to Assess Surface Stability in Desert Environments SO IEEE GEOSCIENCE AND REMOTE SENSING LETTERS LA English DT Article DE Arid environments; desert; erosion; multispectral remote sensing; soil stability; spectral index; very high resolution ID SOLAR-ENERGY; CALIFORNIA; IMAGERY; FIELD AB A spectral index, i.e., the erosion resistance index (ERI), was developed to assess erosion risks in desert landscapes. The index was developed by applying trigonometry to the combination of the green-red band ratio and the green-near-infrared band ratio from very high spatial resolution multispectral imagery. The resultant ERI maps showed spatially cohesive distributions of high and low index values across the study areas. High index values were observed over areas that were resistant to erosion (such as desert pavement and dense vegetation), whereas low index values overlapped with areas that were likely dominated by loose sandy soils, such as stream beds and access roads. Although further investigation is warranted, this spectral index, i.e., the ERI, shows promise for the assessment of erosion risks in desert regions. C1 [Hamada, Yuki; Grippo, Mark A.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Hamada, Y (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM yhamada@anl.gov FU U.S. Department of Energy through the SunShot Initiative [27239] FX This work was supported by the U.S. Department of Energy through the SunShot Initiative under Grant 27239. NR 18 TC 0 Z9 0 U1 2 U2 10 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1545-598X EI 1558-0571 J9 IEEE GEOSCI REMOTE S JI IEEE Geosci. Remote Sens. Lett. PD NOV PY 2015 VL 12 IS 11 BP 2193 EP 2197 DI 10.1109/LGRS.2015.2451613 PG 5 WC Geochemistry & Geophysics; Engineering, Electrical & Electronic; Remote Sensing; Imaging Science & Photographic Technology SC Geochemistry & Geophysics; Engineering; Remote Sensing; Imaging Science & Photographic Technology GA CV4DG UT WOS:000364215500003 ER PT J AU Hacke, P Spataru, S Terwilliger, K Perrin, G Glick, S Kurtz, S Wohlgemuth, J AF Hacke, Peter Spataru, Sergiu Terwilliger, Kent Perrin, Greg Glick, Stephen Kurtz, Sarah Wohlgemuth, John TI Accelerated Testing and Modeling of Potential-Induced Degradation as a Function of Temperature and Relative Humidity SO IEEE JOURNAL OF PHOTOVOLTAICS LA English DT Article DE Photovoltaic (PV) modules; potential-induced degradation (PID); silicon; solar cells ID SYSTEM VOLTAGE STRESS; MODULES AB An acceleration model based on the Peck equation was applied to power performance of crystalline silicon cell modules as a function of time and of temperature and humidity, which are the two main environmental stress factors that promote potential-induced degradation (PID). This model was derived from module power degradation data obtained semicontinuously and statistically by in-situ dark current-voltage measurements in an environmental chamber. The modeling enables prediction of degradation rates and times as functions of temperature and humidity. Power degradation could be modeled linearly as a function of time to the second power; additionally, we found that the quantity of electric charge transferred from the active cell circuit to ground during the stress test is approximately linear with time. Therefore, the power loss could be linearized as a function of coulombs squared. With this result, we observed that when the module face was completely grounded with a condensed phase conductor, leakage current exceeded the anticipated corresponding degradation rate relative to the other tests performed in damp heat. C1 [Hacke, Peter; Terwilliger, Kent; Perrin, Greg; Glick, Stephen; Kurtz, Sarah; Wohlgemuth, John] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Spataru, Sergiu] Aalborg Univ, DK-9220 Aalborg, Denmark. RP Hacke, P (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM peter.hacke@nrel.gov; ssp@et.aau.dk; kent.terwilliger@nrel.gov; greg.perrin@nrel.gov; stephen.glick@nrel.gov; sarah.kurtz@nrel.gov; john.wohlgemuth@nrel.gov OI Spataru, Sergiu/0000-0001-8112-2779 FU U.S. Department of Energy [DE-AC36-08GO28308] FX This work performed at the National Renewable Energy Laboratory was supported by the U.S. Department of Energy under Contract DE-AC36-08GO28308. NR 25 TC 6 Z9 6 U1 3 U2 20 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2156-3381 J9 IEEE J PHOTOVOLT JI IEEE J. Photovolt. PD NOV PY 2015 VL 5 IS 6 BP 1549 EP 1553 DI 10.1109/JPHOTOV.2015.2466463 PG 5 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA CV2PJ UT WOS:000364098400007 ER PT J AU Osterwald, CR Campanelli, M Moriarty, T Emery, KA Williams, R AF Osterwald, Carl R. Campanelli, Mark Moriarty, Tom Emery, Keith A. Williams, Rafell TI Temperature-Dependent Spectral Mismatch Corrections SO IEEE JOURNAL OF PHOTOVOLTAICS LA English DT Article DE Characterization; metrology; measurement; photovoltaic (PV) cells; PV modules; solar cells; short-circuit current; spectral irradiance; temperature coefficient (TC) ID PERFORMANCE AB This paper develops the mathematical foundation for a translation of solar cell short-circuit current from one thermal and spectral irradiance operating condition to another without the use of ill-defined and error-prone temperature coefficients typically employed in solar cell metrology. Using the partial derivative of quantum efficiency with respect to temperature, the conventional isothermal expression for spectral mismatch corrections is modified to account for changes of current due to temperature; this modification completely eliminates the need for short-circuit-current temperature coefficients. An example calculation is provided to demonstrate use of the new translation. C1 [Osterwald, Carl R.; Campanelli, Mark; Moriarty, Tom; Emery, Keith A.; Williams, Rafell] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Osterwald, CR (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM carl.osterwald@nrel.gov; mark.campanelli@nrel.gov; tom.moriarty@nrel.gov; keith.emery@nrel.gov; rafell.williams@nrel.gov NR 12 TC 3 Z9 3 U1 1 U2 2 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2156-3381 J9 IEEE J PHOTOVOLT JI IEEE J. Photovolt. PD NOV PY 2015 VL 5 IS 6 BP 1692 EP 1697 DI 10.1109/JPHOTOV.2015.2459914 PG 6 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA CV2PJ UT WOS:000364098400028 ER PT J AU Deceglie, MG Silverman, TJ Marion, B Kurtz, SR AF Deceglie, Michael G. Silverman, Timothy J. Marion, Bill Kurtz, Sarah R. TI Real-Time Series Resistance Monitoring in PV Systems Without the Need for I-V Curves SO IEEE JOURNAL OF PHOTOVOLTAICS LA English DT Article DE Monitoring; photovoltaic; reliability; series resistance AB We apply the physical principles of a familiar method, suns-V-oc, to a new application: the real-time detection of series resistance changes in modules and systems operating outside. The real-time series resistance (RTSR) method that we describe avoids the need for collecting I-V curves or constructing full series-resistance-free I-V curves. RTSR is most readily deployable at the module level on microinverters or module-integrated electronics, but it can also be extended to full strings. Automated detection of series resistance increases can provide early warnings of some of the most common reliability issues, which also pose fire risks, including broken ribbons, broken solder bonds, and contact problems in the junction or combiner box. We describe the method in detail and describe a sample application to data collected from modules operating in the field. C1 [Deceglie, Michael G.; Silverman, Timothy J.; Marion, Bill; Kurtz, Sarah R.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Deceglie, MG (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM michael.deceglie@nrel.gov; timothy.silverman@nrel.gov; bill.marion@nrel.gov; Sarah.Kurtz@nrel.gov FU U.S. Department of Energy [DE-AC36-08GO28308]; National Renewable Energy Laboratory FX This work was supported by the U.S. Department of Energy under Contract DE-AC36-08GO28308 with the National Renewable Energy Laboratory. The U.S. Government retains and the publisher, by accepting the article for publication, acknowledges that the U.S. Government retains a nonexclusive, paid up, irrevocable, worldwide license to publish or reproduce the published form of this work, or allow others to do so, for U.S. Government purposes. NR 11 TC 2 Z9 2 U1 1 U2 2 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2156-3381 J9 IEEE J PHOTOVOLT JI IEEE J. Photovolt. PD NOV PY 2015 VL 5 IS 6 BP 1706 EP 1709 DI 10.1109/JPHOTOV.2015.2478070 PG 4 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA CV2PJ UT WOS:000364098400030 ER PT J AU Kanevce, A Moseley, J Al-Jassim, M Metzger, WK AF Kanevce, Ana Moseley, John Al-Jassim, Mowafak Metzger, Wyatt K. TI Quantitative Determination of Grain-Boundary Recombination Velocity in CdTe by Cathodoluminescence Measurements and Numerical Simulations SO IEEE JOURNAL OF PHOTOVOLTAICS LA English DT Article DE Cathodoluminescence; CdTe; grain boundaries; numerical simulations ID FILM SOLAR-CELLS AB We present a 2-D numerical model simulating cathodoluminescence (CL) measurements on CdTe. The model is used to analyze the impact of material parameters on the measured CL intensity to establish when grain-boundary (GB) recombination velocity S-GB can be determined accurately from CL contrast. In addition to GB recombination, grain size and its ratio to the carrier diffusion length can impact CL measurements. Holding the grain interior and GB recombination rates constant, we find that as the grain size increases and exceeds the diffusion length, the observed CL contrast increases. For small-grain-size material, surface recombination lowers the overall intensity of the CL signal but does not significantly impact CL contrast. For large grains, high-surface recombination velocity can decrease the CL contrast. The model is combined with experimental results to quantify the S-GB in polycrystalline CdTe before and after the CdCl2 treatment and to predict the impact of GB recombination on device performance. C1 [Kanevce, Ana; Moseley, John; Al-Jassim, Mowafak; Metzger, Wyatt K.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Moseley, John] Colorado Sch Mines, Golden, CO 80401 USA. RP Kanevce, A (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM Ana.Kanevce@nrel.gov; john.moseley@nrel.gov; Mowafak.Al-Jassim@nrel.gov; wyatt.metzger@nrel.gov FU U.S. Department of Energy [DE-AC36-08GO28308]; USDOE Office of Energy Efficiency and Renewable Energy Solar Energy Technologies Program; National Renewable Energy Laboratory FX This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08GO28308 with the National Renewable Energy Laboratory. Funding provided by "applicable DOE Office and Program," [e.g., USDOE Office of Energy Efficiency and Renewable Energy Solar Energy Technologies Program]. NR 18 TC 3 Z9 3 U1 2 U2 14 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2156-3381 J9 IEEE J PHOTOVOLT JI IEEE J. Photovolt. PD NOV PY 2015 VL 5 IS 6 BP 1722 EP 1726 DI 10.1109/JPHOTOV.2015.2478061 PG 5 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA CV2PJ UT WOS:000364098400033 ER PT J AU Silverman, TJ Deceglie, MG Sun, XS Garris, RL Alam, MA Deline, C Kurtz, S AF Silverman, Timothy J. Deceglie, Michael G. Sun, Xingshu Garris, Rebekah L. Alam, Muhammad Ashraful Deline, Chris Kurtz, Sarah TI Thermal and Electrical Effects of Partial Shade in Monolithic Thin-Film Photovoltaic Modules SO IEEE JOURNAL OF PHOTOVOLTAICS LA English DT Article AB Photovoltaic cells can be damaged by reverse bias stress, which arises during service when a monolithically integrated thin-film module is partially shaded. We introduce a model for describing a module's internal thermal and electrical state, which cannot normally be measured. Using this model and experimental measurements, we present several results with relevance for reliability testing and module engineering: Modules with a small breakdown voltage experience less stress than those with a large breakdown voltage, with some exceptions for modules having light-enhanced reverse breakdown. Masks leaving a small part of the masked cells illuminated can lead to very high temperature and current density compared with masks covering entire cells. C1 [Silverman, Timothy J.; Deceglie, Michael G.; Garris, Rebekah L.; Deline, Chris; Kurtz, Sarah] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Sun, Xingshu; Alam, Muhammad Ashraful] Purdue Univ, W Lafayette, IN 47907 USA. RP Silverman, TJ (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM timothy.silverman@nrel.gov; michael.deceglie@nrel.gov; sunxingshu@gmail.com; rebekah.garris@nrel.gov; alam@purdue.edu; chris.deline@nrel.gov; sarah.kurtz@nrel.gov FU U.S. Department of Energy [DE-AC36-08GO28308] FX This work was supported by the U.S. Department of Energy under Contract DE-AC36-08GO28308 with the National Renewable Energy Laboratory. Some of the data in this report were obtained using equipment at the Energy Systems Integration Facility (a national user facility sponsored by the U.S. DOE Office of Energy Efficiency and Renewable Energy) located at the National Renewable Energy Laboratory. The U.S. Government retains and the publisher, by accepting the article for publication, acknowledges that the U.S. Government retains a nonexclusive, paid up, irrevocable, worldwide license to publish or reproduce the published form of this work, or allow others to do so, for U.S. Government purposes. NR 9 TC 4 Z9 4 U1 0 U2 4 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2156-3381 J9 IEEE J PHOTOVOLT JI IEEE J. Photovolt. PD NOV PY 2015 VL 5 IS 6 BP 1742 EP 1747 DI 10.1109/JPHOTOV.2015.2478071 PG 6 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA CV2PJ UT WOS:000364098400036 ER PT J AU Song, T Kanevce, A Sites, JR AF Song, Tao Kanevce, Ana Sites, James R. TI Design of Epitaxial CdTe Solar Cells on InSb Substrates SO IEEE JOURNAL OF PHOTOVOLTAICS LA English DT Article DE CdTe; epitaxial; InSb; single-crystal; solar cells; substrate ID EFFICIENCY; GAAS; GE AB Epitaxial CdTe has been shown by others to have a radiative recombination rate approaching unity, high carrier concentration, and low defect density. It has, therefore, become an attractive candidate for high-efficiency solar cells, perhaps becoming competitive with GaAs. The choice of substrate is a key design feature for epitaxial CdTe solar cells, and several possibilities (CdTe, Si, GaAs, and InSb) have been investigated by others. All have challenges, and these have generally been addressed through the addition of intermediate layers between the substrate and CdTe absorber. InSb is an attractive substrate choice for CdTe devices, because it has a close lattice match with CdTe, it has low resistivity, and it is easy to contact. However, the valence-band alignment between InSb and p-type CdTe, which can both impede hole current and enhance forward electron current, is not favorable. Three strategies to address the band-offset problem are investigated by numerical simulation: heavy doping of the back part of the CdTe layer, incorporation of an intermediate CdMgTe or CdZnTe layer, and the formation of an InSb tunnel junction. Each of these strategies is predicted to be helpful for higher cell performance, but a combination of the first two should be most effective. C1 [Song, Tao; Sites, James R.] Colorado State Univ, Dept Phys, Ft Collins, CO 80523 USA. [Kanevce, Ana] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Song, T (reprint author), Colorado State Univ, Dept Phys, Ft Collins, CO 80523 USA. EM tsong241@rams.colostate.edu; Ana.Kanevce@nrel.gov; James.Sites@colostate.edu FU National Renewable Energy Laboratory [UGA-0-41027-18]; U.S. Department of Energy SunShot program FX This work was supported by the National Renewable Energy Laboratory Subcontract UGA-0-41027-18 with funding from the U.S. Department of Energy SunShot program. NR 28 TC 3 Z9 3 U1 6 U2 23 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2156-3381 J9 IEEE J PHOTOVOLT JI IEEE J. Photovolt. PD NOV PY 2015 VL 5 IS 6 BP 1762 EP 1768 DI 10.1109/JPHOTOV.2015.2466471 PG 7 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA CV2PJ UT WOS:000364098400039 ER PT J AU Mansfield, LM Kuciauskas, D Dippo, P Li, JV Bowers, K To, B DeHart, C Ramanathan, K AF Mansfield, Lorelle M. Kuciauskas, Darius Dippo, Patricia Li, Jian V. Bowers, Karen To, Bobby DeHart, Clay Ramanathan, Kannan TI Optoelectronic Investigation of Sb-Doped Cu(In,Ga)Se-2 SO IEEE JOURNAL OF PHOTOVOLTAICS LA English DT Article DE Admittance spectroscopy; Cu(In, Ga)Se-2 (CIGS); defects; photovoltaic cells; photoluminescence; Sb doping; thin films ID SOLAR-CELLS; EFFICIENCY AB In this study, we incorporated Sb into the precursor that was subsequently converted to Cu(In,Ga)Se-2 (CIGS) by a selenization process. We observed enhanced grain size and improved device performance compared with similarly processed CIGS films made without Sb. The optoelectronic properties of the Sb-doped CIGS films were examined with photoluminescence (PL) and admittance spectroscopy. These techniques allowed us to explore the changes in native defect compensation and evaluate the origin of a lower energy PL peak that is not typically seen in CIGS. C1 [Mansfield, Lorelle M.; Kuciauskas, Darius; Dippo, Patricia; Li, Jian V.; Bowers, Karen; To, Bobby; DeHart, Clay; Ramanathan, Kannan] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Mansfield, LM (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM lorelle.mansfield@nrel.gov; darius.kuciauskas@nrel.gov; pat.dippo@nrel.gov; jian.li@nrel.gov; karen.bowers@nrel.gov; bobby.to@nrel.gov; clay.dehart@nrel.gov; kannan.ramanathan@nrel.gov RI Li, Jian/B-1627-2016 FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory FX This work was supported by the U.S. Department of Energy under Contract DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. The U.S. Government retains and the publisher, by accepting the article for publication, acknowledges that the U.S. Government retains a nonexclusive, paid up, irrevocable, worldwide license to publish or reproduce the published form of this work, or allow others to do so, for U.S. Government purposes. NR 16 TC 0 Z9 0 U1 8 U2 30 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2156-3381 J9 IEEE J PHOTOVOLT JI IEEE J. Photovolt. PD NOV PY 2015 VL 5 IS 6 BP 1769 EP 1774 DI 10.1109/JPHOTOV.2015.2470082 PG 6 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA CV2PJ UT WOS:000364098400040 ER PT J AU Geisz, JF Steiner, MA Garcia, I France, RM McMahon, WE Osterwald, CR Friedman, DJ AF Geisz, John F. Steiner, Myles A. Garcia, Ivan France, Ryan M. McMahon, William E. Osterwald, Carl R. Friedman, Daniel J. TI Generalized Optoelectronic Model of Series-Connected Multijunction Solar Cells SO IEEE JOURNAL OF PHOTOVOLTAICS LA English DT Article DE Electroluminescence (EL); luminescent coupling (LC); multijunction solar cells; photoluminescence (PL) ID QUANTUM EFFICIENCY MEASUREMENTS; P-N JUNCTION; MEASUREMENT ARTIFACTS; CARRIER GENERATION; BIAS; RECOMBINATION; LUMINESCENCE; ELIMINATION; DESIGN; LIMIT AB The emission of light from each junction in a series-connected multijunction solar cell both complicates and elucidates the understanding of its performance under arbitrary conditions. Bringing together many recent advances in this understanding, we present a general 1-D model to describe luminescent coupling that arises from both voltage-driven electroluminescence and voltage-independent photoluminescence in nonideal junctions that include effects such as Sah-Noyce-Shockley (SNS) recombination with n not equal 2, Auger recombination, shunt resistance, reverse-bias breakdown, series resistance, and significant dark area losses. The individual junction voltages and currents are experimentally determined from measured optical and electrical inputs and outputs of the device within the context of the model to fit parameters that describe the devices performance under arbitrary input conditions. Techniques to experimentally fit the model are demonstrated for a four-junction inverted metamorphic solar cell, and the predictions of the model are compared with concentrator flash measurements. C1 [Geisz, John F.; Steiner, Myles A.; Garcia, Ivan; France, Ryan M.; McMahon, William E.; Osterwald, Carl R.; Friedman, Daniel J.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Garcia, Ivan] Univ Politecn Madrid, Inst Energia Solar, E-28040 Madrid, Spain. RP Geisz, JF (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM john.geisz@nrel.gov; myles.steiner@nrel.gov; igarcia@ies-def.upm.es; ryan.france@nrel.gov; bill.mcmahon@nrel.gov; Carl.Osterwald@nrel.gov; daniel.friedman@nrel.gov RI Garcia, Ivan/L-1547-2014 OI Garcia, Ivan/0000-0002-9895-2020 FU U.S. Department of Energy [DE-AC36-08GO28308]; IOF Grant from People Program (Marie Curie Actions) of European Union's Seventh Framework Program under REA Grant [299878] FX The work was supported by the U.S. Department of Energy under Contract DE-AC36-08GO28308 with the National Renewable Energy Laboratory. The work of I. Garcia was supported by an IOF Grant from the People Program (Marie Curie Actions) of the European Union's Seventh Framework Program (FP7/2007-2013) under REA Grant 299878. The U.S. Government retains and the publisher, by accepting the article for publication, acknowledges that the U.S. Government retains a nonexclusive, paid up, irrevocable, worldwide license to publish or reproduce the published form of this work, or allow others to do so, for U.S. Government purposes. NR 53 TC 10 Z9 10 U1 6 U2 20 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2156-3381 J9 IEEE J PHOTOVOLT JI IEEE J. Photovolt. PD NOV PY 2015 VL 5 IS 6 BP 1827 EP 1839 DI 10.1109/JPHOTOV.2015.2478072 PG 13 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA CV2PJ UT WOS:000364098400048 ER PT J AU Fan, YW Zhang, ZH Trinkle, M Dimitrovski, AD Bin Song, J Li, HS AF Fan, Yawen Zhang, Zhenghao Trinkle, Matthew Dimitrovski, Aleksandar D. Bin Song, Ju Li, Husheng TI A Cross-Layer Defense Mechanism Against GPS Spoofing Attacks on PMUs in Smart Grids SO IEEE TRANSACTIONS ON SMART GRID LA English DT Article DE Cross-layer mechanism; global positioning system (GPS) spoofing; multiple attacks detection; phasor measurement units (PMU) ID PHASOR MEASUREMENT UNITS; SYSTEM AB Recent investigations have revealed the susceptibility of phasor measurement units (PMUs) to the time synchronization attack by spoofing its global positioning system (GPS). This paper proposes a cross-layer detection mechanism to fight against simultaneous attacks toward multiple PMUs. In the physical layer, we propose a GPS carrier-to-noise ratio (C/No) based spoofing detection technique. We apply the patch-monopole hybrid antenna to two GPS receivers and compute the difference between the standard deviation of each receiver's C/No. The priori probability of spoofing is calculated from the distributions of the difference. A counter is embedded in the physical layer to identify the most suspicious PMU. In the upper layer, the spoofing attack is considered similarly to the bad data injection toward the power system. A trustworthiness evaluation, which is based on both the physical layer information and power grid measurements, is applied to identify the PMU being attacked. An experiment has been carried to validate the proposed algorithm. C1 [Fan, Yawen; Li, Husheng] Univ Tennessee, Knoxville, TN 37996 USA. [Li, Husheng] Kyung Hee Univ, Int Scholar, Seoul, South Korea. [Zhang, Zhenghao] Ji Nan Univ, Guangzhou 510632, Guangdong, Peoples R China. [Trinkle, Matthew] Univ Adelaide, Adelaide, SA 5005, Australia. [Dimitrovski, Aleksandar D.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Bin Song, Ju] Kyung Hee Univ, Seoul, South Korea. RP Li, HS (reprint author), Univ Tennessee, Knoxville, TN 37996 USA. EM husheng@eecs.utk.edu RI Dimitrovski, Aleksandar/G-5897-2016 OI Dimitrovski, Aleksandar/0000-0001-9109-621X FU National Science Foundation [CNS-1116826, CNS-1237834, CNS-1239366]; University of Tennessee-Battelle [R011344513] FX The work of Y. Fan and H. Li was supported in part by the National Science Foundation under Grant CNS-1116826, Grant CNS-1237834, and Grant CNS-1239366, and in part by the University of Tennessee-Battelle under Grant R011344513. NR 24 TC 4 Z9 6 U1 2 U2 10 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1949-3053 EI 1949-3061 J9 IEEE T SMART GRID JI IEEE Trans. Smart Grid PD NOV PY 2015 VL 6 IS 6 BP 2659 EP 2668 DI 10.1109/TSG.2014.2346088 PG 10 WC Engineering, Electrical & Electronic SC Engineering GA CV1TF UT WOS:000364040300009 ER PT J AU Lu, XN Sun, K Guerrero, JM Vasquez, JC Huang, LP Wang, JH AF Lu, Xiaonan Sun, Kai Guerrero, Josep M. Vasquez, Juan C. Huang, Lipei Wang, Jianhui TI Stability Enhancement Based on Virtual Impedance for DC Microgrids With Constant Power Loads SO IEEE TRANSACTIONS ON SMART GRID LA English DT Article DE Constant power load (CPL); dc microgrid; stability; virtual impedance ID ENERGY-STORAGE SYSTEMS; DROOP CONTROL METHOD; HIERARCHICAL CONTROL; CONVERTER; INVERTERS; DESIGN; STABILIZATION; INSTABILITY; OPERATION; PARALLEL AB In this paper, a converter-based dc microgrid is studied. By considering the impact of each component in dc microgrids on system stability, a multistage configuration is employed, which includes the source stage, interface converter stage between buses, and common load stage. In order to study the overall stability of the above dc microgrid with constant power loads (CPLs), a comprehensive small-signal model is derived by analyzing the interface converters in each stage. The instability issue induced by the CPLs is revealed by using the criteria of impedance matching. Meanwhile, virtual-impedance-based stabilizers are proposed in order to enhance the damping of dc microgrids with CPLs and guarantee the stable operation. Since droop control is commonly used to reach proper load power sharing in dc microgrids, its impact is taken into account when testing the proposed stabilizers. By using the proposed stabilizers, virtual impedances are employed in the output filters of the interface converters in the second stage of the multistage configuration. In particular, one of the virtual impedances is connected in series with the filter capacitor, and the other one is connected at the output path of the converter. It can be seen that by using the proposed stabilizers, the unstable poles induced by the CPLs are forced to move into the stable region. The proposed method is verified by the MATLAB/Simulink model of multistage dc microgrids with three distributed power generation units. C1 [Lu, Xiaonan; Wang, Jianhui] Argonne Natl Lab, Div Energy Syst, Lemont, IL 60439 USA. [Sun, Kai; Huang, Lipei] Tsinghua Univ, Dept Elect Engn, State Key Lab Power Syst, Beijing 100084, Peoples R China. [Guerrero, Josep M.; Vasquez, Juan C.] Aalborg Univ, Dept Energy Technol, DK-9220 Aalborg, Denmark. RP Sun, K (reprint author), Tsinghua Univ, Dept Elect Engn, State Key Lab Power Syst, Beijing 100084, Peoples R China. EM sun-kai@mail.tsinghua.edu.cn RI Vasquez, Juan/J-2247-2014; Guerrero, Josep/D-5519-2014 OI Vasquez, Juan/0000-0001-6332-385X; Guerrero, Josep/0000-0001-5236-4592 FU National Natural Science Foundation of China [51177083]; State Key Laboratory of Power Systems Tsinghua University, China [SKLD14M01]; U.S. Department of Energy Office of Electricity Delivery and Energy Reliability FX This work was supported in part by the National Natural Science Foundation of China under Grant 51177083, and in part by the State Key Laboratory of Power Systems Tsinghua University, China, under Grant SKLD14M01. The work of X. Lu and J. Wang was supported by the U.S. Department of Energy Office of Electricity Delivery and Energy Reliability. NR 40 TC 8 Z9 8 U1 4 U2 17 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1949-3053 EI 1949-3061 J9 IEEE T SMART GRID JI IEEE Trans. Smart Grid PD NOV PY 2015 VL 6 IS 6 BP 2770 EP 2783 DI 10.1109/TSG.2015.2455017 PG 14 WC Engineering, Electrical & Electronic SC Engineering GA CV1TF UT WOS:000364040300019 ER PT J AU Jalowicka, A Duan, R Huczkowski, P Chyrkin, A Gruner, D Pint, BA Unocic, KA Quadakkers, WJ AF Jalowicka, A. Duan, R. Huczkowski, P. Chyrkin, A. Gruner, D. Pint, B. A. Unocic, K. A. Quadakkers, W. J. TI Effect of Specimen Thickness on Microstructural Changes During Oxidation of the NiCrW Alloy 230 at 950-1050 degrees C SO JOM LA English DT Article ID HIGH-TEMPERATURE OXIDATION; COOLED REACTOR APPLICATIONS; NICKEL-BASE SUPERALLOYS; CHROMIA SCALES; 602 CA; DEPLETION PROFILES; HIGH-STRENGTH; WATER-VAPOR; BEHAVIOR; CR AB An accurate procedure for predicting oxidation-induced damage and lifetime limits is crucial for the reliable operation of high-temperature metallic components in practical applications. In order to develop a predictive oxidation lifetime model for Ni-Cr alloys, specimens of wrought NiCrW alloy 230 with different thicknesses were cyclically oxidized in air at 950-1050 degrees C for up to 3000 h. After prolonged exposure, two types of carbides as well as a Cr-rich nitride (pi-phase) precipitated in the gamma-Ni matrix. The oxidation-induced loss of Cr from the alloy resulted in the formation of subscale zones, which were free of the Cr-rich carbide and nitride but also of the Ni-W rich M6C. The width of the M6C-free zone was smaller than that free of the Cr-rich precipitates. Thermodynamic and diffusion calculations of the observed time- and temperature-dependent Cr depletion processes identified that back diffusion of C occurred which resulted in an increased volume fraction of M23C6 in the specimen core. With increasing time and temperature, the amount of pi-phase in the specimen core increased. The subscale depletion of the initially present Cr-nitrides and the formation of Cr-nitrides in the specimen center is believed to be related to a mechanism which is qualitatively similar to that described for the Cr carbide enrichment. However, with increasing time and decreasing specimen thickness, N uptake from the atmosphere becomes apparent. As a result, the precipitates present in the specimen center eventually consisted almost exclusively of nitrides. C1 [Jalowicka, A.; Duan, R.; Huczkowski, P.; Chyrkin, A.; Gruner, D.; Quadakkers, W. J.] Forschungszentrum Julich, IEK 2, Inst Energy & Climate Res, D-52425 Julich, Germany. [Pint, B. A.; Unocic, K. A.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Jalowicka, A (reprint author), Forschungszentrum Julich, IEK 2, Inst Energy & Climate Res, D-52425 Julich, Germany. EM a.jalowicka@fz-juelich.de RI Pint, Bruce/A-8435-2008; OI Pint, Bruce/0000-0002-9165-3335; Chyrkin, Anton/0000-0002-4355-3030 FU Bundesministerium fur Bildung und Forschung (BMBF) [03EK3032]; U.S. Department of Energy; Advanced Manufacturing Office (Combined Heat and Power Program); U.S. Assistant Secretary for Energy Efficiency and Renewable Energy FX The authors would like to acknowledge Dr. K. Ohla from Haynes International for supplying the material. The authors would also like to acknowledge the Bundesministerium fur Bildung und Forschung (BMBF) for funding part of this work under Grant No. 03EK3032. Assistance with ICP-OES analysis provided by H. Lippert and V. Nischwitz from the Central Institute for Engineering, Electronics and Analytics, ZEA-3, Forschungszentrum Julich GmbH is greatly appreciated. The authors are grateful to the following colleagues in the Institute of Energy and Climate Research of the Forschungszentrum Julich GmbH IEK-2 for assistance in the experimental work: R. Mahnke, H. Cosler, and A. Kick for the oxidation experiments, V. Gutzeit and J. Bartsch for metallographic studies, Dr. E. Wessel for EBSD investigations and Dr. Nowak for GDOES analyses. At ORNL, G. Garner, T. Lowe and T. Jordan assisted with the experimental work and the research was sponsored by the U.S. Department of Energy, U.S. Assistant Secretary for Energy Efficiency and Renewable Energy, Advanced Manufacturing Office (Combined Heat and Power Program). NR 48 TC 2 Z9 2 U1 2 U2 6 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1047-4838 EI 1543-1851 J9 JOM-US JI JOM PD NOV PY 2015 VL 67 IS 11 BP 2573 EP 2588 DI 10.1007/s11837-015-1645-8 PG 16 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering; Mineralogy; Mining & Mineral Processing SC Materials Science; Metallurgy & Metallurgical Engineering; Mineralogy; Mining & Mineral Processing GA CV0JG UT WOS:000363936400012 ER PT J AU Pint, BA Keiser, JR AF Pint, B. A. Keiser, J. R. TI Initial Assessment of Ni-Base Alloy Performance in 0.1 MPa and Supercritical CO2 SO JOM LA English DT Article ID CARBON-DIOXIDE; MATERIALS TECHNOLOGY; OXIDATION BEHAVIOR; INTERNAL OXIDATION; STAINLESS-STEEL; CORROSION; SCALES; HEAT; CYCLES; POWER AB There is considerable interest in increasing the working temperature of both open and closed supercritical CO2 (sCO(2)) cycles to a parts per thousand yen700A degrees C. At these temperatures, it is unlikely that Fe-base alloys have suitable strength and therefore the focus is on Ni-base alloys for this application. To begin addressing the lack of sCO(2) materials compatibility data under these conditions, initial work exposed a wide range of candidate alloys for 500 h at 20 MPa (200 bar) CO2 at 650-750A degrees C in high-purity CO2. In general, the reaction products were thin and protective in these exposures. A smaller group of alloy coupons focusing on chromia- and alumina-forming alloys was exposed for 500 h in 0.1 MPa (1 bar) air, CO2, CO2 + O-2 and CO2 + H2O for comparison. The thin surface oxides formed were very similar to those formed at high pressure and no clear detrimental effect of CO2 oxidation or O-2 or H2O impurities could be observed in these exposures. C1 [Pint, B. A.; Keiser, J. R.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Corros Sci & Technol Grp, Oak Ridge, TN 37831 USA. RP Pint, BA (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Corros Sci & Technol Grp, Oak Ridge, TN 37831 USA. EM pintba@ornl.gov RI Pint, Bruce/A-8435-2008 OI Pint, Bruce/0000-0002-9165-3335 FU U. S. Department of Energy, Office of Fossil Energy; Office of Coal and Power RD FX The research shown was sponsored by the U. S. Department of Energy, Office of Fossil Energy, Office of Coal and Power R&D. M. Howell, M. Stephens, T. Lowe, T. Jordan, R. Brese and D. Leonard assisted with the experimental work. M. P. Brady provided helpful comments on the manuscript. NR 29 TC 4 Z9 4 U1 5 U2 13 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1047-4838 EI 1543-1851 J9 JOM-US JI JOM PD NOV PY 2015 VL 67 IS 11 BP 2615 EP 2620 DI 10.1007/s11837-015-1661-8 PG 6 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering; Mineralogy; Mining & Mineral Processing SC Materials Science; Metallurgy & Metallurgical Engineering; Mineralogy; Mining & Mineral Processing GA CV0JG UT WOS:000363936400016 ER PT J AU Gao, MC Carney, CS Dogan, AN Jablonksi, PD Hawk, JA Alman, DE AF Gao, M. C. Carney, C. S. Dogan, A-N. Jablonksi, P. D. Hawk, J. A. Alman, D. E. TI Design of Refractory High-Entropy Alloys SO JOM LA English DT Article ID BULK METALLIC GLASSES; MULTICOMPONENT ALLOYS; PHASE-FORMATION; ELEMENT; EXPLORATION; ENTHALPY AB This report presents a design methodology for refractory high-entropy alloys with a body-centered cubic (bcc) structure using select empirical parameters (i.e., enthalpy of mixing, atomic size difference, Omega-parameter, and electronegativity difference) and CALPHAD approach. Sixteen alloys in equimolar compositions ranging from quinary to ennead systems were designed with experimental verification studies performed on two alloys using x-ray diffraction, energy-dispersive spectroscopy, and scanning electron microscopy. Two bcc phases were identified in the as-cast HfMoNbTaTiVZr, whereas multiple phases formed in the as-cast HfMoNbTaTiVWZr. Observed elemental segregation in the alloys qualitatively agrees with CALPHAD prediction. Comparisons of the thermodynamic mixing properties for liquid and bcc phases using the Miedema model and CALPHAD are presented. This study demonstrates that CALPHAD is more effective in predicting HEA formation than empirical parameters, and new single bcc HEAs are suggested: HfMoNbTiZr, HfMoTaTiZr, NbTaTiVZr, HfMoNbTaTiZr, HfMoTaTiVZr, and MoNbTaTiVZr. C1 [Gao, M. C.; Carney, C. S.; Dogan, A-N.; Jablonksi, P. D.; Hawk, J. A.; Alman, D. E.] Natl Energy Technol Lab, Albany, OR 97321 USA. [Gao, M. C.; Carney, C. S.] AECOM, Albany, OR 97321 USA. RP Gao, MC (reprint author), Natl Energy Technol Lab, Albany, OR 97321 USA. EM michael.gao@netl.doe.gov FU Cross-Cutting Technologies Program at the National Energy Technology Laboratory (NETL)-Strategic Center for Coal; RES [DE-FE-0004000] FX This work was funded by the Cross-Cutting Technologies Program at the National Energy Technology Laboratory (NETL)-Strategic Center for Coal, managed by Robert Romanosky (Technology Manager) and Charles Miller (Technology Monitor). The Research was executed through NETL's Office of Research and Development's Innovative Process Technologies (IPT) Field Work Proposal. Research performed by AECOM Staff was conducted under the RES contract DE-FE-0004000. The authors thank Ed Argetsinger (AECOM) for making the ingots, Paul Danielson (NETL) for performing optical microscopy, Chris Powell (AECOM) for performing hardness tests, Richard Chin (NETL) for performing WDXRF analysis, and Kyle Rozman (NETL/ORISE) performing x-ray diffraction. M.C.G. thanks from Andreas Markstrom, Huahai Mao, and Chao Jiang from Thermo-Calc for providing technical support. NR 32 TC 10 Z9 10 U1 16 U2 54 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1047-4838 EI 1543-1851 J9 JOM-US JI JOM PD NOV PY 2015 VL 67 IS 11 BP 2653 EP 2669 DI 10.1007/s11837-015-1617-z PG 17 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering; Mineralogy; Mining & Mineral Processing SC Materials Science; Metallurgy & Metallurgical Engineering; Mineralogy; Mining & Mineral Processing GA CV0JG UT WOS:000363936400022 ER PT J AU Knezevic, M Zecevic, M Beyerlein, IJ Bhattacharyya, A McCabe, RJ AF Knezevic, Marko Zecevic, Miroslav Beyerlein, Irene J. Bhattacharyya, Abhishek McCabe, Rodney J. TI Predicting Texture Evolution in Ta and Ta-10W Alloys Using Polycrystal Plasticity SO JOM LA English DT Article ID TANTALUM-TUNGSTEN ALLOYS; STRAIN-RATE; HCP/BCC COMPOSITES; DEFORMATION; TEMPERATURE; BEHAVIOR; MODEL; SIMULATION; NIOBIUM; RHENIUM AB We present results of texture characterization and predictions of a multiscale physically based constitutive law developed to predict the mechanical response and texture evolution of body-centered cubic metals. The model is unique in the sense that single crystal deformation results not only from the resolved shear stress along the direction of slip (Schmid law) but also from shear stresses resolved along directions orthogonal to the slip direction as well as the three normal stress components (non-Schmid effects). The single crystal model is implemented into a visco-plastic self-consistent homogenization scheme containing a hardening law for crystallographic slip. The polycrystal model is calibrated using a set of mechanical test data collected on a tantalum-tungsten alloy, Ta-10W, in tension and compression and pure tantalum, Ta, in tension, compression, and cross-rolling. We demonstrate that the model effectively captures the texture evolution in all cases. We show that alloying has the effect of increasing the dislocation friction stress, the trapping rate of dislocations, and activation barrier for recovery. C1 [Knezevic, Marko; Zecevic, Miroslav] Univ New Hampshire, Dept Mech Engn, Durham, NH 03824 USA. [Beyerlein, Irene J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Bhattacharyya, Abhishek] HC Starck, Newton, MA 02461 USA. [McCabe, Rodney J.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. RP Knezevic, M (reprint author), Univ New Hampshire, Dept Mech Engn, 33 Acad Way,Kingsbury Hall,W119, Durham, NH 03824 USA. EM marko.knezevic@unh.edu OI McCabe, Rodney /0000-0002-6684-7410 FU H.C. Starck, Newton, MA, USA; Laboratory Directed Research and Development Program Award [20140348ER] FX Support for this research was provided by H.C. Starck, Newton, MA, 02461, USA. I. J. Beyerlein would like to acknowledge support by a Laboratory Directed Research and Development Program Award Number 20140348ER. NR 20 TC 7 Z9 7 U1 3 U2 8 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1047-4838 EI 1543-1851 J9 JOM-US JI JOM PD NOV PY 2015 VL 67 IS 11 BP 2670 EP 2674 DI 10.1007/s11837-015-1613-3 PG 5 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering; Mineralogy; Mining & Mineral Processing SC Materials Science; Metallurgy & Metallurgical Engineering; Mineralogy; Mining & Mineral Processing GA CV0JG UT WOS:000363936400023 ER PT J AU Lopez, RE Gonzalez, WD Vasylinnas, V Richardson, IG Cid, C Echer, E Reeves, GD Brandt, PC AF Lopez, R. E. Gonzalez, W. D. Vasylinnas, V. Richardson, I. G. Cid, C. Echer, E. Reeves, G. D. Brandt, P. C. TI Decrease in SYM-H during a storm main phase without evidence of a ring current injection SO JOURNAL OF ATMOSPHERIC AND SOLAR-TERRESTRIAL PHYSICS LA English DT Article DE Magnetic storms; Ring current; Substorm particle injections; Polar cap flux ID TAIL CURRENT CONTRIBUTION; CORONAL MASS EJECTIONS; SOLAR-CYCLE 23; GEOMAGNETIC STORMS; MAGNETIC STORMS; POLAR-CAP; MHD SIMULATIONS; GROWTH-PHASE; FIELD; DST AB Changes in the Dst index, or the similarly constructed high-resolution SYM-H index, are thought to indicate changes in the total energy content of the ring current. However, this is not always the case. In this paper we examine an intense (SYM-H similar to -435 nT) magnetic storm that occurred on March 31, 2001. The arrival at Earth of strongly southward IMF produced an immediate negative response in the SYM-H index. While energetic particle and magnetometer data from geosynchronous orbit and inner magnetosphere energetic neutral atom imaging indicate that two substorm injections took place during the main phase, there was about one hour when the SYM-H decreased more than 200 nT with no evidence in the data for ring current enhancement. Instead the near-Earth magnetotail exhibited a growth phase indicative of a strong, growing cross-tail current, with the large substorm expansion phase and the associated injection of energetic particles coming significantly later. Data from the DMSP spacecraft demonstrate that the polar cap flux grew rapidly in response to the strongly southward IMF. We present observations showing that the decrease in SYM-H occurred when polar cap flux was increasing and there was no evidence of injection into the ring current. Our findings strongly support the relationship between Dst and the polar cap flux proposed by theoretical studies that determined that the tail current system could be a significant contributor to Dst (C) 2015 Elsevier Ltd. All rights reserved. C1 [Lopez, R. E.] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA. [Gonzalez, W. D.; Echer, E.] INPE, Sao Jose Dos Campos, Brazil. [Vasylinnas, V.] Max Planck Inst Sonnensyst Forsch, Gottingen, Germany. [Richardson, I. G.] Univ Maryland, CRESST, College Pk, MD 20742 USA. [Richardson, I. G.] Univ Maryland, Dept Astron, College Pk, MD 20742 USA. [Richardson, I. G.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Cid, C.] Univ Alcala de Henares, Dept Fis & Matemat, Space Res Grp Space Weather, E-28871 Alcala De Henares, Spain. [Reeves, G. D.] Los Alamos Natl Lab, Los Alamos, NM USA. [Brandt, P. C.] Johns Hopkins Appl Phys Lab, Laurel, MD USA. RP Lopez, RE (reprint author), Univ Texas Arlington, Dept Phys, POB 19059, Arlington, TX 76019 USA. EM relopez@uta.edu RI Brandt, Pontus/N-1218-2016; OI Brandt, Pontus/0000-0002-4644-0306; CID, CONSUELO/0000-0002-2863-3745; Richardson, Ian/0000-0002-3855-3634; Reeves, Geoffrey/0000-0002-7985-8098; Lopez, Ramon/0000-0001-5881-1365 FU CISM - STC Program of the National Science Foundation [ATM-0120950]; NASA [NNX09AI63G]; NSF [ATM-0900920, AGS1303646]; Brazilian CNPq agency [301233/2011-0, 303329/2011-4]; FAPESP [2012/066734]; Comision Interministerial de Ciencia y Tecnologia (CICYT) of Spain [PN-AYA2009-08662]; Junta de Comunidades de Castilla-La Mancha of Spain [PPII10-0183-7802] FX This paper is based upon work supported by CISM, which is funded by the STC Program of the National Science Foundation under agreement ATM-0120950, NASA grant NNX09AI63G, NSF grants ATM-0900920 and AGS1303646, Brazilian CNPq agency contract numbers 301233/2011-0 and 303329/2011-4, FAPESP agency contract number 2012/066734, grant PN-AYA2009-08662 from the Comision Interministerial de Ciencia y Tecnologia (CICYT) of Spain, and grant PPII10-0183-7802 from the Junta de Comunidades de Castilla-La Mancha of Spain. We acknowledge use of NASA/GSFC Space Physics Data Facility OMNIWeb and CDAWeb service, and OMNI data. We thank Los Alamos National Laboratory for providing the geosynchronous particle data. The DMSP particle detectors were designed by Dave Hardy of AFRL, and the data and plots were obtained from JHU/APL. The results presented in this paper rely on data collected at magnetic observatories. We thank the national institutes that support them and INTERMAGNET for promoting high standards of magnetic observatory practice (www.intermagnet.org). This work was initially discussed during the Brazil 9 Workshop on Magnetic Storms held at the Universidad de Alcala, Alcala, Spain in October, 2011. NR 56 TC 2 Z9 2 U1 1 U2 7 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1364-6826 EI 1879-1824 J9 J ATMOS SOL-TERR PHY JI J. Atmos. Sol.-Terr. Phys. PD NOV PY 2015 VL 134 BP 118 EP 129 DI 10.1016/j.jastp.2015.09.016 PG 12 WC Geochemistry & Geophysics; Meteorology & Atmospheric Sciences SC Geochemistry & Geophysics; Meteorology & Atmospheric Sciences GA CV4SV UT WOS:000364257700012 ER PT J AU Gao, F Washton, NM Wang, YL Kollar, M Szanyi, J Peden, CHF AF Gao, Feng Washton, Nancy M. Wang, Yilin Kollar, Marton Szanyi, Janos Peden, Charles H. F. TI Effects of Si/Al ratio on Cu/SSZ-13 NH3-SCR catalysts: Implications for the active Cu species and the roles of Bronsted acidity SO JOURNAL OF CATALYSIS LA English DT Article DE Selective catalytic reduction; Cu/SSZ-13; Si/Al ratio; NMR; Temperature-programmed desorption; Reaction kinetics ID FE-EXCHANGED ZEOLITES; SSZ-13 ZEOLITE; NO OXIDATION; NITRIC-OXIDE; REDUCTION; AMMONIA; CU-SSZ-13; NH3; MECHANISM; SITES AB Cu/SSZ-13 catalysts with three Si/Al ratios of 6, 12 and 35 were synthesized with Cu incorporation via solution ion exchange. The implications of varying Si/Al ratios on the nature of the multiple Cu species that can be present in the SSZ-13 zeolite are a major focus of this work, as highlighted by the results of a variety of catalyst characterization and reaction kinetics measurements. Specifically, catalysts were characterized with surface area/pore volume measurements, temperature programmed reduction by H-2 (H-2-TPR), NH3 temperature programmed desorption (NH3-TPD), and DRIFTS and solid-state nuclear magnetic resonance (NMR) spectroscopies. Catalytic properties were examined using NO oxidation, ammonia oxidation, and standard ammonia selective catalytic reduction (NH3-SCR) reactions on selected catalysts under differential conditions. Besides indicating the possibility of multiple active Cu species for these reactions, the measurements are also used to untangle some of the complexities caused by the interplay between redox of Cu ion centers and Bronsted acidity. All three reactions appear to follow a redox reaction mechanism, yet the roles of Bronsted acidity are quite different. For NO oxidation, increasing Si/Al ratio lowers Cu redox barriers, thus enhancing reaction rates. Bronsted acidity appears to play essentially no role for this reaction. For standard NH3-SCR, residual Bronsted acidity plays a significant beneficial role at both low- and high-temperature regimes. For NH3 oxidation, no clear trend is observed suggesting both Cu ion center redox and Bronsted acidity play important and perhaps competing roles. (C) 2015 Elsevier Inc. All rights reserved. Agreement signed 2015 C1 [Gao, Feng; Washton, Nancy M.; Wang, Yilin; Kollar, Marton; Szanyi, Janos; Peden, Charles H. F.] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. RP Gao, F (reprint author), Pacific NW Natl Lab, Inst Integrated Catalysis, POB 999, Richland, WA 99352 USA. EM feng.gao@pnnl.gov; chuck.peden@pnnl.gov FU US Department of Energy (DOE), Energy Efficiency and Renewable Energy, Vehicle Technologies Office; DOE's Office of Biological and Environmental Research FX The authors gratefully acknowledge the US Department of Energy (DOE), Energy Efficiency and Renewable Energy, Vehicle Technologies Office for the support of this work. The research described in this paper was performed in the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). PNNL is operated for the US DOE by Battelle. The authors also thank Shari Li (PNNL) for surface area/pore volume measurements, and Bruce W. Arey (PNNL) for SEM measurements. Discussions with Drs. A. Yezerets, K. Kamasamudram, J.H. Li, N. Currier and J.Y. Luo from Cummins, Inc., and H.Y. Chen and H. Hess from Johnson-Matthey are greatly appreciated. NR 54 TC 16 Z9 16 U1 30 U2 135 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9517 EI 1090-2694 J9 J CATAL JI J. Catal. PD NOV PY 2015 VL 331 BP 25 EP 38 DI 10.1016/j.jcat.2015.08.004 PG 14 WC Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA CV4QE UT WOS:000364250800003 ER PT J AU Zhang, H Sun, JM Liu, CJ Wang, Y AF Zhang, He Sun, Junming Liu, Changjun Wang, Yong TI Distinct water activation on polar/non-polar facets of ZnO nanoparticles SO JOURNAL OF CATALYSIS LA English DT Article DE Facet; Water dissociation; ZnO; Ketonization; Ethanol ID DEFINED SURFACE PLANES; ZNXZRYOZ MIXED OXIDES; HIGH CO2 SELECTIVITY; AMMONIA-SYNTHESIS; DIRECT CONVERSION; LOW-TEMPERATURE; BIO-ETHANOL; METHANOL; CATALYSTS; NANOCRYSTALS AB ZnO nanoparticles with differing dominant facets were prepared and characterized by a complimentary of techniques such as X-ray diffraction, electron microscopy, temperature programmed desorption of H2O, and Fourier transform infrared spectroscopy analysis of adsorbed D2O. For the first time, water interaction/activation is compared on ZnO polar and non-polar facets. We report that non-polar facets exhibit high activity in water activation, which favors reactions such as ketonization and steam reforming in which dissociated water is involved. The distinct water dissociation on ZnO non-polar facets could be related to its facile formation of oxygen vacancies under realistic reaction conditions. (C) 2015 Elsevier Inc. All rights reserved. C1 [Zhang, He; Sun, Junming; Liu, Changjun; Wang, Yong] Washington State Univ, Gene & Linda Voiland Sch Chem Engn & Bioengn, Pullman, WA 99164 USA. [Wang, Yong] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. RP Sun, JM (reprint author), Washington State Univ, Gene & Linda Voiland Sch Chem Engn & Bioengn, Pullman, WA 99164 USA. EM junming.sun@wsu.edu; yong.wang@pnnl.gov RI Sun, Junming/B-3019-2011; Liu, Changjun/M-3272-2013 OI Sun, Junming/0000-0002-0071-9635; Liu, Changjun/0000-0003-3735-4112 FU U.S. Department of Energy [DE-FG02-05ER15712]; Department of Energy's Office of Biological and Environmental Research FX We greatly acknowledge the financial support by the U.S. Department of Energy (Grant No. DE-FG02-05ER15712). Part of the research was performed at Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). We thank the Franceschi Microscopy and Imaging Center (FMIC) at Washington State University for the access to SEM. J. Sun thanks Dr. Chongmin Wang (PNNL) and Dr. Renqin Zhang (WSU) for the helpful discussions. NR 29 TC 2 Z9 2 U1 9 U2 38 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9517 EI 1090-2694 J9 J CATAL JI J. Catal. PD NOV PY 2015 VL 331 BP 57 EP 62 DI 10.1016/j.jcat.2015.08.016 PG 6 WC Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA CV4QE UT WOS:000364250800006 ER PT J AU Sabnis, KD Cui, YR Akatay, MC Shekhar, M Lee, WS Miller, JT Delgass, WN Ribeiro, FH AF Sabnis, Kaiwalya D. Cui, Yanran Akatay, M. Cem Shekhar, Mayank Lee, Wen-Sheng Miller, Jeffrey T. Delgass, W. Nicholas Ribeiro, Fabio H. TI Water-gas shift catalysis over transition metals supported on molybdenum carbide SO JOURNAL OF CATALYSIS LA English DT Article DE Molybdenum carbide; Water-gas shift; In situ X-ray absorption ID FUEL-CELL APPLICATIONS; HETEROGENEOUS CATALYSIS; GOLD NANOPARTICLES; SIZE; HYDROGENATION; OXIDATION; SITES; MODEL AB We report here that WGS rates per total surface area at 120 degrees C, 7% CO, 22% H2O, 8.5% CO2, 37% H-2 for Pt, Au, Pd and Ni supported over MO2C were 4-8 times higher than those of the commercial Cu/ZnO/Al2O3 catalyst. In agreement with previous literature, the WGS rate per total moles of Pt over Pt/MO2C at 120 degrees C has been shown to be higher than on any Pt/Metal oxide catalyst. We have made use of systematic changes in the apparent kinetic parameters with various admetals (decrease in apparent CO order and apparent activation energy and increase in apparent H2O order compared to unpromoted MO2C) to conclude that the function of the rate-promoting admetals is to enhance the relative surface concentration of the adsorbed CO, thereby leading to a promotion in the WGS rate per total surface area of the catalyst. Temperature programmed desorption of CO was used to show that the CO adsorption properties of MO2C were modified by the various admetals by creating new metallic sites. In situ X-ray absorption on Pt and Au and STEM-EELS experiments showed that the supported Au nanoparticles over MO2C decrease in average particle size from similar to 9 nm to 3 nm after a 600 degrees C carburization pretreatment. Pt was also shown to have assumed a stable structure at 600 degrees C in the form of a Pt-Mo alloy. We suggest that MO2C can be used to synthesize thermally robust supported metal catalysts. (C) 2015 Elsevier Inc. All rights reserved. C1 [Sabnis, Kaiwalya D.; Cui, Yanran; Shekhar, Mayank; Lee, Wen-Sheng; Miller, Jeffrey T.; Delgass, W. Nicholas; Ribeiro, Fabio H.] Purdue Univ, Sch Chem Engn, W Lafayette, IN 47907 USA. [Akatay, M. Cem] Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. [Miller, Jeffrey T.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Ribeiro, FH (reprint author), Purdue Univ, Sch Chem Engn, 480 Stadium Mall Dr, W Lafayette, IN 47907 USA. EM fabio@purdue.edu FU U.S. Department of Energy, Office of Basic Energy Sciences, through the Catalysis Science [DE-FG02-03ER15466]; U.S. Department of Energy, Office of Science [DE-AC02-06CH11357]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357, DE-AC02-98CH10886]; Department of Energy; MRCAT member institutions FX Support for this research was provided by the U.S. Department of Energy, Office of Basic Energy Sciences, through the Catalysis Science Grant No. DE-FG02-03ER15466. Use of the Advanced Photon Source is supported by the U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. MRCAT operations are supported by the Department of Energy and the MRCAT member institutions. Scanning transmission electron microscopy was carried out at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 34 TC 8 Z9 8 U1 23 U2 133 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9517 EI 1090-2694 J9 J CATAL JI J. Catal. PD NOV PY 2015 VL 331 BP 162 EP 171 DI 10.1016/j.jcat.2015.08.017 PG 10 WC Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA CV4QE UT WOS:000364250800017 ER PT J AU Myers, AT Mckee, CF Li, PS AF Myers, Andrew T. Mckee, Christopher F. Li, Pak Shing TI The CH+ abundance in turbulent, diffuse molecular clouds SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE astrochemistry; ISM: abundances; ISM: clouds ID RAY IONIZATION RATE; PHOTON-DOMINATED REGIONS; INTER-STELLAR SHOCKS; INTERSTELLAR CLOUDS; PHYSICAL CONDITIONS; COSMIC-RAY; MHD TURBULENCE; MAGNETOHYDRODYNAMIC TURBULENCE; AMBIPOLAR DIFFUSION; TRANSLUCENT LINES AB The intermittent dissipation of interstellar turbulence is an important energy source in the diffuse interstellar medium. Though on average smaller than the heating rates due to cosmic rays and the photoelectric effect on dust grains, the turbulent cascade can channel large amounts of energy into a relatively small fraction of the gas that consequently undergoes significant heating and chemical enrichment. In particular, this mechanism has been proposed as a solution to the long-standing problem of the high abundance of CH+ along diffuse molecular sight lines, which steady-state, low-temperature models underproduce by over an order of magnitude. While much work has been done on the structure and chemistry of these small-scale dissipation zones, comparatively little attention has been paid to relating these zones to the properties of the large-scale turbulence. In this paper, we attempt to bridge this gap by estimating the temperature and CH+ column density along diffuse molecular sight lines by post-processing three-dimensional magnetohydrodynamic(s) turbulence simulations. Assuming reasonable values for the cloud density ((n) over bar (H) = 30 cm(-3)), size (L = 20 pc), and velocity dispersion (sigma(v) = 2.3 km s(-1)), we find that our computed abundances compare well with CH+ column density observations, as well as with observations of emission lines from rotationally excited H-2 molecules. C1 [Myers, Andrew T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Mckee, Christopher F.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Mckee, Christopher F.; Li, Pak Shing] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. RP Myers, AT (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM atmyers2@gmail.com FU NASA through NASA ATP [NNX09AK31G, NNX13AB84G]; NSF [AST-0908553, AST-1211729]; US Department of Energy at the Lawrence Livermore National Laboratory [LLNL-B569409]; National Center of Supercomputing Application [TG-MCA00N020] FX ATM wishes to thank the anonymous referee for a thoughtful report that improved this paper. Support for this research was provided by NASA through NASA ATP grants NNX09AK31G and NNX13AB84G (CFM and PSL), the NSF through grants AST-0908553 and AST-1211729 (ATM and CFM), and the US Department of Energy at the Lawrence Livermore National Laboratory under grant LLNL-B569409 (A.T.M.). This research was also supported by grants of high performance computing resources from the National Center of Supercomputing Application through grant TG-MCA00N020. We have used yt3 (Turk et al. 2011) as well as the SCIPY4 family of PYTHON libraries for data analysis and plotting. Our analysis and visualization scripts are available online at https://bitbucket.org/atmyers/chplus. NR 67 TC 4 Z9 4 U1 0 U2 1 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD NOV 1 PY 2015 VL 453 IS 3 BP 2747 EP 2758 DI 10.1093/mnras/stv1782 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CU6NL UT WOS:000363649000041 ER PT J AU Johnson, JL AF Johnson, Jarrett L. TI The chemical signature of surviving Population III stars in the Milky Way SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE radiation: dynamics; stars: low-mass; stars: Population III; Galaxy: stellar content; cosmology: theory; early Universe ID METAL-POOR STARS; INITIAL MASS FUNCTION; POROUS INTERSTELLAR GRAINS; 1ST STARS; DUST GRAINS; RADIATION PRESSURE; OPTICAL-PROPERTIES; PROTOPLANETARY DISKS; STELLAR ARCHAEOLOGY; EARLY UNIVERSE AB Cosmological simulations of Population (Pop) III star formation suggest that the primordial initial mass function may have extended to subsolar masses. If Pop III stars with masses <= 0.8 M-circle dot did form, then they should still be present in the Galaxy today as either mainsequence or red giant stars. Despite broad searches, however, no primordial stars have yet been identified. It has long been recognized that the initialmetal-free nature of primordial stars could be masked due to accretion of metal-enriched material from the interstellar medium (ISM). Here, we point out that while gas accretion from the ISM may readily occur, the accretion of dust from the ISM can be prevented due to the pressure of the radiation emitted from low-mass stars. This implies a possible unique chemical signature for stars polluted only via accretion, namely an enhancement in gas phase elements relative to those in the dust phase. Using Pop III stellar models, we outline the conditions in which this signature could be exhibited, and we derive the expected signature for the case of accretion from the local ISM. Intriguingly, due to the large fraction of iron depleted into dust relative to that of carbon and other elements, this signature is similar to that observed in many of the so-called carbon-enhanced metal-poor (CEMP) stars. We therefore suggest that some fraction of the observed CEMP stars may, in fact, be accretion-polluted Pop III stars. C1 Los Alamos Natl Lab, Theoret Design 10, Los Alamos, NM 87545 USA. RP Johnson, JL (reprint author), Los Alamos Natl Lab, Theoret Design 10, POB 1663, Los Alamos, NM 87545 USA. EM jlj@lanl.gov FU National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396] FX Work at LANL was done under the auspices of the National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. JLJ would like to thank George Becker, Joe Smidt and Joyce Guzik for helpful discussion, as well as Thomas Greif and Volker Bromm for valuable feedback on an early version of this work. The author is thankful to an anonymous reviewer for helpful comments on the role of Coulomb drag in coupling gas and dust grains, as well as to another anonymous reviewer for insightful comments and suggestions. NR 89 TC 1 Z9 1 U1 2 U2 3 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD NOV 1 PY 2015 VL 453 IS 3 BP 2771 EP 2778 DI 10.1093/mnras/stv1815 PG 8 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CU6NL UT WOS:000363649000043 ER PT J AU Eftekharzadeh, S Myers, AD White, M Weinberg, DH Schneider, DP Shen, Y Font-Ribera, A Ross, NP Paris, I Streblyanska, A AF Eftekharzadeh, Sarah Myers, Adam D. White, Martin Weinberg, David H. Schneider, Donald P. Shen, Yue Font-Ribera, Andreu Ross, Nicholas P. Paris, Isabelle Streblyanska, Alina TI Clustering of intermediate redshift quasars using the final SDSS III-BOSS sample SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE galaxies: quasars: general; cosmology: observations; dark matter; large-scale; structure of Universe ID DIGITAL-SKY-SURVEY; OSCILLATION SPECTROSCOPIC SURVEY; HALO OCCUPATION DISTRIBUTION; SUPERMASSIVE BLACK-HOLES; ACTIVE GALACTIC NUCLEI; PHOTOMETRICALLY CLASSIFIED QUASARS; DATA RELEASE 9; BARYON ACOUSTIC-OSCILLATIONS; STAR-FORMING GALAXIES; DARK-MATTER HALOS AB We measure the two-point clustering of spectroscopically confirmed quasars from the final sample of the Baryon Oscillation Spectroscopic Survey (BOSS) on comoving scales of 4 less than or similar to s less than or similar to 22 h(-1) Mpc. The sample covers 6950 deg(2) [19 (h(-1)Gpc)(3)] and, over the redshift range 2.2 <= z <= 2.8, contains 55 826 homogeneously selected quasars, which is twice as many as in any similar work. We deduce b(Q) = 3.54 +/- 0.10; the most precise measurement of quasar bias to date at these redshifts. This corresponds to a host halo mass of similar to 2 x 10(12) h(-1)M(circle dot) with an implied quasar duty cycle of similar to 1 per cent. The real-space projected correlation function is well fitted by a power law of index 2 and correlation length r(0) = (8.12 +/- 0.22) h(-1)Mpc over scales of 4 less than or similar to r(p) less than or similar to 25 h(-1) Mpc. To better study the evolution of quasar clustering at moderate redshift, we extend the redshift range of our study to z similar to 3.4 and measure the bias and correlation length of three subsamples over 2.2 <= z <= 3.4. We find no significant evolution of r(0) or bias over this range, implying that the host halo mass of quasars decreases somewhat with increasing redshift. We find quasar clustering remains similar over a decade in luminosity, contradicting a scenario in which quasar luminosity is monotonically related to halo mass at z approximate to 2.5. Our results are broadly consistent with previous BOSS measurements, but they yield more precise constraints based upon a larger and more uniform data set. C1 [Eftekharzadeh, Sarah; Myers, Adam D.] Univ Wyoming, Dept Phys & Astron, Laramie, WY 82071 USA. [White, Martin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [White, Martin] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [White, Martin] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Weinberg, David H.] Ohio State Univ, Dept Astron, Columbus, OH 43210 USA. [Weinberg, David H.] Ohio State Univ, CCAPP, Columbus, OH 43210 USA. [Schneider, Donald P.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Schneider, Donald P.] Penn State Univ, Inst Gravitat & Cosmos, University Pk, PA 16802 USA. [Shen, Yue] Carnegie Observ, Pasadena, CA 91101 USA. [Shen, Yue] Peking Univ, Kavli Inst Astron & Astrophys, Beijing 100871, Peoples R China. [Font-Ribera, Andreu] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Ross, Nicholas P.] Drexel Univ, Dept Phys, Philadelphia, PA 19104 USA. [Ross, Nicholas P.] Univ Edinburgh, Astron Inst, Royal Observ, Edinburgh EH9 3HJ, Midlothian, Scotland. [Paris, Isabelle] Osserv Astron Trieste, INAF, I-34131 Trieste, Italy. [Streblyanska, Alina] Inst Astrofis Canarias, E-38200 Tenerife, Spain. [Streblyanska, Alina] Univ La Laguna, Dept Astrofis, E-38205 Tenerife, Spain. RP White, M (reprint author), Univ Wyoming, Dept Phys & Astron, 1000 Univ Ave, Laramie, WY 82071 USA. EM seftekha@uwyo.edu RI White, Martin/I-3880-2015 OI White, Martin/0000-0001-9912-5070 FU Alfred P. Sloan Foundation; National Science Foundation; US Department of Energy Office of Science; NASA through ADAP award [NNX12AE38G]; EPSCoR award [NNX11AM18A]; National Science Foundation [1211112] FX Funding for SDSS-III8 has been provided by the Alfred P. Sloan Foundation, the Participating Institutions, the National Science Foundation, and the US Department of Energy Office of Science. SDSS-III is managed by the Astrophysical Research Consortium for the Participating Institutions of the SDSS-III Collaboration including the University of Arizona, the Brazilian Participation Group, Brookhaven National Laboratory, University of Cambridge, Carnegie Mellon University, University of Florida, the French Participation Group, the German Participation Group, Harvard University, the Instituto de Astrosica de Canarias, the Michigan State/ Notre Dame/ JINA Participation Group, Johns Hopkins University, Lawrence Berkeley National Laboratory, Max Planck Institute for Astrophysics, Max Planck Institute for Extraterrestrial Physics, New Mexico State University, New York University, Ohio State University, Pennsylvania State University, University of Portsmouth, Princeton University, the Spanish Participation Group, University of Tokyo, University of Utah, Vanderbilt University, University of Virginia, University of Washington, and Yale University.; SE and ADM were partially supported by NASA through ADAP award NNX12AE38G and EPSCoR award NNX11AM18A and by the National Science Foundation through grant number 1211112. NR 127 TC 17 Z9 17 U1 0 U2 0 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD NOV 1 PY 2015 VL 453 IS 3 BP 2779 EP 2798 DI 10.1093/mnras/stv1763 PG 20 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CU6NL UT WOS:000363649000044 ER PT J AU Yakut, K Eggleton, PP Kalomeni, B Tout, CA Eldridge, JJ AF Yakut, K. Eggleton, P. P. Kalomeni, B. Tout, C. A. Eldridge, J. J. TI A turn-off detached binary star V568 Lyr in the Kepler field of the oldest open cluster (NGC 6791) in the Galaxy SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE binaries: close; binaries: eclipsing; stars: fundamental parameters; stars: individual: V568 Lyr; stars: low-mass; open clusters and associations: individual: NGC 6791 ID DWARF COOLING SEQUENCE; RICH OPEN CLUSTER; VARIABLE-STARS; CLOSE-BINARY; BOLOMETRIC CORRECTIONS; HELIUM CONTENT; NGC-6791; ABUNDANCES; EVOLUTION; AGE AB We present the Kepler photometric light-variation analysis of the late-type double-lined binary system V568 Lyr that is in the field of the high metallicity old open cluster NGC 6791. The radial velocity and the high-quality short-cadence light curve of the system are analysed simultaneously. The masses, radii and luminosities of the component stars are M-1 = 1.0886 +/- 0.0031 M-circle dot, M-2 = 0.8292 +/- 0.0026 M-circle dot, R-1 = 1.4203 +/- 0.0058 R-circle dot, R-2 = 0.7997 +/- 0.0015 R-circle dot, L-1 = 1.85 +/- 0.15 L-circle dot, L-2 = 0.292 +/- 0.018 L-circle dot and their separation is a = 31.060 +/- 0.025 R-circle dot. The distance to NGC 6791 is determined to be 4.260 +/- 0.290 kpc by analysis of this binary system. We fit the components of this well-detached binary system with evolution models made with the Cambridge STARS and EV(TWIN) codes to test low-mass binary star evolution. We find a good fit with a metallicity of Z = 0.04 and an age of 7.704 Gyr. The standard tidal dissipation, included in EV(TWIN) is insufficient to arrive at the observed circular orbit unless it formed rather circular to begin with. C1 [Yakut, K.; Eggleton, P. P.; Kalomeni, B.] Univ Ege, Dept Astron & Space Sci, TR-35100 Izmir, Turkey. [Yakut, K.; Eggleton, P. P.; Tout, C. A.; Eldridge, J. J.] Univ Cambridge, Inst Astron, The Observ, Cambridge CB3 0HA, England. [Eggleton, P. P.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Kalomeni, B.; Eldridge, J. J.] MIT, Kavli Inst Astrophys & Space Res, Cambridge, MA 02139 USA. Univ Auckland, Dept Phys, Auckland, New Zealand. RP Yakut, K (reprint author), Univ Ege, Dept Astron & Space Sci, TR-35100 Izmir, Turkey. EM kadri.yakut@ege.edu.tr; eggleton1@llnl.gov; belinda.kalomeni@ege.edu.tr FU Turkish Scientific and Research Council [TUBITAK 111T270, 112T766, 113F097]; Churchill College FX We acknowledge the Kepler team for giving public access to their corrected light curves and thank the anonymous referee for the careful reading and for suggestions. This research has made use of the SIMBAD database, operated at CDS, Strasbourg, France. This study was supported by the Turkish Scientific and Research Council (TUBITAK 111T270, 112T766, and 113F097). CAT thanks Churchill College for his fellowship. NR 44 TC 0 Z9 0 U1 0 U2 0 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD NOV 1 PY 2015 VL 453 IS 3 BP 2937 EP 2942 DI 10.1093/mnras/stv1773 PG 6 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CU6NL UT WOS:000363649000056 ER PT J AU Amanullah, R Johansson, J Goobar, A Ferretti, R Papadogiannakis, S Petrushevska, T Brown, PJ Cao, Y Contreras, C Dahle, H Elias-Rosa, N Fynbo, JPU Gorosabel, J Guaita, L Hangard, L Howell, DA Hsiao, EY Kankare, E Kasliwal, M Leloudas, G Lundqvist, P Mattila, S Nugent, P Phillips, MM Sandberg, A Stanishev, V Sullivan, M Taddia, F Ostlin, G Asadi, S Herrero-Illana, R Jensen, JJ Karhunen, K Lazarevic, S Varenius, E Santos, P Sridhar, SS Wallstrom, SHJ Wiegert, J AF Amanullah, R. Johansson, J. Goobar, A. Ferretti, R. Papadogiannakis, S. Petrushevska, T. Brown, P. J. Cao, Y. Contreras, C. Dahle, H. Elias-Rosa, N. Fynbo, J. P. U. Gorosabel, J. Guaita, L. Hangard, L. Howell, D. A. Hsiao, E. Y. Kankare, E. Kasliwal, M. Leloudas, G. Lundqvist, P. Mattila, S. Nugent, P. Phillips, M. M. Sandberg, A. Stanishev, V. Sullivan, M. Taddia, F. Ostlin, G. Asadi, S. Herrero-Illana, R. Jensen, J. J. Karhunen, K. Lazarevic, S. Varenius, E. Santos, P. Sridhar, S. Seethapuram Wallstrom, S. H. J. Wiegert, J. TI Diversity in extinction laws of Type Ia supernovae measured between 0.2 and 2 mu m SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE circumstellar matter; supernovae: general; supernovae: individual: SNe 2012cg; supernovae: individual: 2012cu; dust, extinction ID HUBBLE-SPACE-TELESCOPE; SODIUM D ABSORPTION; LIGHT-CURVE SHAPES; SN 2011FE; ULTRAVIOLET OBSERVATIONS; CIRCUMSTELLAR MATERIAL; LEGACY SURVEY; ABSOLUTE MAGNITUDES; IMPROVED DISTANCES; INFRARED-EMISSION AB We present ultraviolet (UV) observations of six nearby Type Ia supernovae (SNe Ia) obtained with the Hubble Space Telescope, three of which were also observed in the near-IR (NIR) with Wide-Field Camera 3. UV observations with the Swift satellite, as well as ground-based optical and NIR data provide complementary information. The combined data set covers the wavelength range 0.2-2 mu m. By also including archival data of SN 2014J, we analyse a sample spanning observed colour excesses up to E(B - V) = 1.4 mag. We study the wavelength-dependent extinction of each individual SN and find a diversity of reddening laws when characterized by the total-to-selective extinction R-V. In particular, we note that for the two SNe with E(B - V) greater than or similar to 1 mag, for which the colour excess is dominated by dust extinction, we find R-V = 1.4 +/- 0.1 and R-V = 2.8 +/- 0.1. Adding UV photometry reduces the uncertainty of fitted R-V by similar to 50 per cent allowing us to also measure R-V of individual low-extinction objects which point to a similar diversity, currently not accounted for in the analyses when SNe Ia are used for studying the expansion history of the Universe. C1 [Amanullah, R.; Johansson, J.; Goobar, A.; Ferretti, R.; Papadogiannakis, S.; Petrushevska, T.; Hangard, L.] Stockholm Univ, Dept Phys, Oskar Klein Ctr, SE-10691 Stockholm, Sweden. [Brown, P. J.] Texas A&M Univ, George P & Cynthia Woods Mitchell Inst Fundamenta, Dept Phys & Astron, College Stn, TX 77843 USA. [Cao, Y.; Phillips, M. M.] CALTECH, Cahill Ctr Astrophys, Pasadena, CA 91125 USA. [Contreras, C.; Hsiao, E. Y.] Las Campanas Observ, Carnegie Observ, La Serena, Chile. [Dahle, H.; Santos, P.] Univ Oslo, Inst Theoret Astrophys, N-0315 Oslo, Norway. [Elias-Rosa, N.] Osserv Astron Padova, INAF, I-35122 Padua, Italy. [Fynbo, J. P. U.; Leloudas, G.; Jensen, J. J.] Univ Copenhagen, Niels Bohr Inst, Dark Cosmol Ctr, DK-2100 Copenhagen O, Denmark. [Gorosabel, J.; Herrero-Illana, R.] CSIC, Inst Astrofis Andalucia, E-18008 Granada, Spain. [Gorosabel, J.] Univ Basque Country, UPV EHU, Unidad Asociada Grp Ciencias Planetarias IAA CSIC, Dept Fis Aplicada 1,ETS Ingn, E-48013 Bilbao, Spain. [Guaita, L.] Osserv Astron Roma, INAF, I-00040 Rome, Italy. [Howell, D. A.] Las Cumbres Observ Global Telescope Network, Goleta, CA 93117 USA. [Howell, D. A.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Hsiao, E. Y.] Aarhus Univ, Dept Phys & Astron, DK-8000 Aarhus C, Denmark. [Kankare, E.] Queens Univ Belfast, Sch Math & Phys, Astrophys Res Ctr, Belfast BT7 1NN, Antrim, North Ireland. [Kasliwal, M.] Observ Carnegie Inst Sci, Pasadena, CA 91101 USA. [Leloudas, G.] Weizmann Inst Sci, Fac Phys, Benoziyo Ctr Astrophys, IL-76100 Rehovot, Israel. [Lundqvist, P.; Sandberg, A.; Taddia, F.; Ostlin, G.; Asadi, S.] Stockholm Univ, Dept Astron, Oskar Klein Ctr, SE-10691 Stockholm, Sweden. [Mattila, S.] Univ Turku, Finnish Ctr Astron ESO FINCA, FI-21500 Piikkio, Finland. [Nugent, P.] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Nugent, P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Cosmol Ctr, Berkeley, CA 94720 USA. [Stanishev, V.] Inst Super Tecn, CENTRA Ctr Multidisciplinar Astrofis, P-1049001 Lisbon, Portugal. [Sullivan, M.] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. [Karhunen, K.] Univ Turku, Dept Phys & Astron, Tuorla Observ, FI-21500 Piikkio, Finland. [Lazarevic, S.] Univ Belgrade, Fac Math, Dept Astron, Belgrade 11000, Serbia. [Varenius, E.; Wallstrom, S. H. J.; Wiegert, J.] Chalmers, Onsala Space Observ, Dept Earth & Space Sci, SE-43992 Onsala, Sweden. [Sridhar, S. Seethapuram] ASTRON, NL-7990 AA Dwingeloo, Netherlands. [Sridhar, S. Seethapuram] Univ Groningen, Kapteyn Astron Inst, NL-9700 AV Groningen, Netherlands. RP Amanullah, R (reprint author), Stockholm Univ, Dept Phys, Oskar Klein Ctr, SE-10691 Stockholm, Sweden. EM rahman@fysik.su.se RI Elias-Rosa, Nancy/D-3759-2014; OI Elias-Rosa, Nancy/0000-0002-1381-9125; Herrero-Illana, Ruben/0000-0002-7758-8717; Ferretti, Raphael/0000-0001-7814-5814 FU Swedish Research Council; Swedish Space Board; NASA's Astrophysics Data Analysis Program [NNX13AF35G]; FCT - Fundacao para a Ciencia e Tecnologia [SFRH/BD/62075/2009]; Fundacao para a Ciencia e a Tecnologia; European Union [267251]; Danish Agency for Science and Technology and Innovation through a Sapere Aude Level 2 grant; DNRF; European Research Council under the European Union [EGGS-278202]; National Aeronautics and Space Administration; [PTDC/CTE-AST/112582/2009] FX We would like to thank Denise Taylor at Space Telescope Science Institute for advising and assisting us in carrying out this programme. We would also like to thank Livia Vallini for carrying out observations of SN 2012cg during the Nordic Millimetre and Optical/NIR Astronomy Summer School 2012. We are grateful to the anonymous referee for thoroughly going through the manuscript and providing us with many useful comments. RA and AG acknowledge support from the Swedish Research Council and the Swedish Space Board. PJB and the Swift Optical/Ultraviolet Supernova Archive (SOUSA) are supported by NASA's Astrophysics Data Analysis Program through grant NNX13AF35G. The work of PS is sponsored by FCT - Fundacao para a Ciencia e Tecnologia, under the grant SFRH/BD/62075/2009. VS acknowledges support from Fundacao para a Ciencia e a Tecnologia (Ciencia 2008) and grant PTDC/CTE-AST/112582/2009. NER acknowledges the support from the European Union Seventh Framework Programme (FP7/2007-2013) under grant agreement no. 267251 'Astronomy Fellowships in Italy' (AstroFIt). The Oskar Klein Centre is funded by the Swedish Research Council. EYH acknowledge the generous support provided by the Danish Agency for Science and Technology and Innovation through a Sapere Aude Level 2 grant. The Dark Cosmology Centre is funded by the DNRF. The research leading to these results has received funding from the European Research Council under the European Union's Seventh Framework Programme (FP7/2007-2013)/ERC Grant agreement no. EGGS-278202. Observations were made with the Hubble Space Telescope; the NOT, operated by the Nordic Optical Telescope Scientific Association at the Observatorio del Roque de los Muchachos, La Palma, Spain. The data presented here were obtained in part with ALFOSC, which is provided by the Instituto de Astrofisica de Andalucia (IAA) under a joint agreement with the University of Copenhagen and NOTSA. STSDAS and PyRAF is a product of the Space Telescope Science Institute, which is operated by AURA for NASA. This research has made use of the NASA/IPAC Extragalactic Database (NED) which is operated by the Jet Propulsion Laboratory, California Institute of Technology, under contract with the National Aeronautics and Space Administration. NR 185 TC 12 Z9 12 U1 1 U2 6 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD NOV 1 PY 2015 VL 453 IS 3 BP 3300 EP 3328 DI 10.1093/mnras/stv1505 PG 29 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CU6NL UT WOS:000363649000085 ER PT J AU Ryu, T Spatola, B Delabaere, L Bowlin, K Hopp, H Kunitake, R Karpen, GH Chiolo, I AF Ryu, Taehyun Spatola, Brett Delabaere, Laetitia Bowlin, Katherine Hopp, Hannah Kunitake, Ryan Karpen, Gary H. Chiolo, Irene TI Heterochromatic breaks move to the nuclear periphery to continue recombinational repair SO NATURE CELL BIOLOGY LA English DT Article ID DOUBLE-STRAND BREAK; DROSOPHILA-MELANOGASTER HETEROCHROMATIN; UBIQUITIN E3 LIGASE; DNA-DAMAGE RESPONSE; SUMO LIGASE; SACCHAROMYCES-CEREVISIAE; CHECKPOINT KINASE; GENOME STABILITY; INDUCED FOCI; HUMAN-CELLS AB Heterochromatin mostly comprises repeated sequences prone to harmful ectopic recombination during double-strand break (DSB) repair. In Drosophila cells, 'safe' homologous recombination (HR) repair of heterochromatic breaks relies on a specialized pathway that relocalizes damaged sequences away from the heterochromatin domain before strand invasion. Here we show that heterochromatic DSBs move to the nuclear periphery to continue HR repair. Re localization depends on nuclear pores and inner nuclear membrane proteins (INMPs) that anchor repair sites to the nuclear periphery through the Smc5/6-interacting proteins STUbL/RENi. Both the initial block to HR progression inside the heterochromatin domain, and the targeting of repair sites to the nuclear periphery, rely on SUMO and SUMO E3 ligases. This study reveals a critical role for SUMOylation in the spatial and temporal regulation of HR repair in heterochromatin, and identifies the nuclear periphery as a specialized site for heterochromatin repair in a multicellular eukaryote. C1 [Ryu, Taehyun; Spatola, Brett; Delabaere, Laetitia; Bowlin, Katherine; Hopp, Hannah; Chiolo, Irene] Univ So Calif, Mol & Computat Biol Dept, Los Angeles, CA 90089 USA. [Kunitake, Ryan; Karpen, Gary H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Genome Dynam Dept, Berkeley, CA 94720 USA. [Karpen, Gary H.] Univ Calif Berkeley, Mol & Cell Biol Dept, Berkeley, CA 94720 USA. RP Chiolo, I (reprint author), Univ So Calif, Mol & Computat Biol Dept, Los Angeles, CA 90089 USA. EM chiolo@usc.edu FU USC Gold Family Fellowship; USC Research Enhancement Fellowship; USC Provost Fellowship; Rose Hills Foundation [R21ES021541]; [R01GM117376]; [R0IGM086613] FX This work was supported by the USC Gold Family Fellowship and the USC Research Enhancement Fellowship to T.R.; the USC Provost Fellowship to B.S.; R21ES021541, The Rose Hills Foundation, and R01GM117376 to I.C.; R0IGM086613 to G.H.K. We would like to thank S. Keagy, M. Michael, J. Haber and O. Aparicio for insightful comments on the manuscript, and S. Gasser for sharing results before publication. We are grateful to V. Doye (Institut Jacques Monod, France), J. Kadonaga (University of California San Diego, USA), J. Fischer (University of Texas, USA), M. Welts (University of Rochester, USA), A. Orian (Technion, Israel), S. Parkhurst (Fred Hutchinson Cancer Research Center, USA), A. Ashworth (Institute of Cancer Research, UK) and the O. Aparicio laboratory (University of Southern California, USA) for sharing reagents and the Chiolo and Karpen laboratories for helpful discussions. We thank C. Ferraro and N. Brisson for their help with Lamin and SUMO RNAi studies, and J. Swenson for his initial dPIAS RNAi studies. We also thank M. Bonner for generating the mCh-LaminC construct, D. Das, E. Lin and C. Ren for cloning and RNAi reagents, A. Kim, S. Wijelcularatne and N. Saxena for cloning and Smc5 mutant characterization. Fly stocks from BDSC (NIH P40OD018537) and RNAi libraries from DRSC (NIH R01GM067761) were used for this study. NR 70 TC 27 Z9 27 U1 1 U2 10 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1465-7392 EI 1476-4679 J9 NAT CELL BIOL JI Nat. Cell Biol. PD NOV PY 2015 VL 17 IS 11 BP 1401 EP 1411 DI 10.1038/ncb3258 PG 11 WC Cell Biology SC Cell Biology GA CV4XT UT WOS:000364270500006 PM 26502056 ER PT J AU Ye, Y Wong, ZJ Lu, XF Ni, XJ Zhu, HY Chen, XH Wang, Y Zhang, X AF Ye, Yu Wong, Zi Jing Lu, Xiufang Ni, Xingjie Zhu, Hanyu Chen, Xianhui Wang, Yuan Zhang, Xiang TI Monolayer excitonic laser SO NATURE PHOTONICS LA English DT Article ID LAYER MOS2; VALLEY POLARIZATION; ENERGY-CONVERSION; ROOM-TEMPERATURE; PIEZOELECTRICITY; TRANSISTORS; DISULFIDE; DIODES; WSE2 AB Two-dimensional van der Waals materials have opened a new paradigm for fundamental physics exploration and device applications because of their emerging physical properties. Unlike gapless graphene, monolayer transition-metal dichalcogenides (TMDCs) are two-dimensional semiconductors that undergo an indirect-to-direct bandgap transition(1-5), creating new optical functionalities for next-generation ultra-compact photonics and optoelectronics. Although the enhancement of spontaneous emission has been reported on TMDC monolayers integrated with photonic crystals(6,7) and distributed Bragg reflector microcavities(8,9), coherent light emission from a TMDC monolayer has not been demonstrated. Here, we report the realization of a two-dimensional excitonic laser by embedding monolayer WS2 in a microdisk resonator. Using a whispering gallery mode with a high quality factor and optical confinement, we observe bright excitonic lasing at visible wavelengths. This demonstration of a two-dimensional excitonic laser marks a major step towards two-dimensional on-chip optoelectronics for high-performance optical communication and computing applications. C1 [Ye, Yu; Wong, Zi Jing; Ni, Xingjie; Zhu, Hanyu; Wang, Yuan; Zhang, Xiang] Univ Calif Berkeley, NSF Nanoscale Sci & Engn Ctr, Berkeley, CA 94720 USA. [Ye, Yu; Wong, Zi Jing; Ni, Xingjie; Wang, Yuan; Zhang, Xiang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Lu, Xiufang; Chen, Xianhui] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China. [Lu, Xiufang; Chen, Xianhui] Univ Sci & Technol China, Dept Phys, Hefei 230026, Anhui, Peoples R China. [Zhang, Xiang] King Abdulaziz Univ, Dept Phys, Jeddah 21589, Saudi Arabia. RP Zhang, X (reprint author), Univ Calif Berkeley, NSF Nanoscale Sci & Engn Ctr, Berkeley, CA 94720 USA. EM xiang@berkeley.edu RI Zhang, Xiang/F-6905-2011; Wang, Yuan/F-7211-2011 FU US Air Force Office of Scientific Research [FA9550-12-1-0197]; 'Light-Material Interaction in Energy Conversion' Energy Frontier Research Center - US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-05CH11231] FX The authors acknowledge financial support from the US Air Force Office of Scientific Research under award no. FA9550-12-1-0197 (Optical Design and Characterization), and the 'Light-Material Interaction in Energy Conversion' Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under award no. DE-AC02-05CH11231 (Materials Synthesis and Lithography). The authors also thank A. Grine for his help in measuring the passive Q factor of the cavity. NR 36 TC 40 Z9 40 U1 48 U2 190 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1749-4885 EI 1749-4893 J9 NAT PHOTONICS JI Nat. Photonics PD NOV PY 2015 VL 9 IS 11 BP 733 EP 737 DI 10.1038/NPHOTON.2015.197 PG 5 WC Optics; Physics, Applied SC Optics; Physics GA CV1TA UT WOS:000364039800012 ER PT J AU Freudenthal, BD Beard, WA Cuneo, MJ Dyrkheeva, NS Wilson, SH AF Freudenthal, Bret D. Beard, William A. Cuneo, Matthew J. Dyrkheeva, Nadezhda S. Wilson, Samuel H. TI Capturing snapshots of APE1 processing DNA damage SO NATURE STRUCTURAL & MOLECULAR BIOLOGY LA English DT Article ID HUMAN APURINIC/APYRIMIDINIC ENDONUCLEASE; BASE EXCISION-REPAIR; HUMAN ABASIC ENDONUCLEASE; DOUBLE-STRANDED DNA; METAL-BINDING SITE; INCISION ACTIVITY; CATALYTIC MECHANISM; PHOSPHODIESTER-BOND; POLYMERASE-BETA; CPG ISLANDS AB DNA apurinic-apyrimidinic (AP) sites are prevalent noncoding threats to genomic stability and are processed by AP endonuclease 1 (APE1). APE1 incises the AP-site phosphodiester backbone, generating a DNA-repair intermediate that is potentially cytotoxic. The molecular events of the incision reaction remain elusive, owing in part to limited structural information. We report multiple high-resolution human APE1-DNA structures that divulge new features of the APE1 reaction, including the metal-binding site, the nucleophile and the arginine clamps that mediate product release. We also report APE1-DNA structures with a T-G mismatch 5' to the AP site, representing a clustered lesion occurring in methylated CpG dinucleotides. These structures reveal that APE1 molds the T-G mismatch into a unique Watson-Crick-like geometry that distorts the active site, thus reducing incision. These snapshots provide mechanistic clarity for APE1 while affording a rational framework to manipulate biological responses to DNA damage. C1 [Freudenthal, Bret D.; Beard, William A.; Dyrkheeva, Nadezhda S.; Wilson, Samuel H.] NIEHS, Genome Integr & Struct Biol Lab, NIH, Res Triangle Pk, NC 27709 USA. [Cuneo, Matthew J.] Oak Ridge Natl Lab, Neutron Sci Directorate, Oak Ridge, TN USA. RP Wilson, SH (reprint author), NIEHS, Genome Integr & Struct Biol Lab, NIH, POB 12233, Res Triangle Pk, NC 27709 USA. EM wilson5@niehs.nih.gov OI Cuneo, Matthew/0000-0002-1475-6656 FU US National Institutes of Health, National Institute of Environmental Health Sciences [Z01-ES050158, Z01-ES050161]; United States Department of Energy, Office of Basic Energy Sciences; Eli Lilly and Co.; United States Department of State, as part of the United States-Russia Collaboration in the Biomedical Sciences US National Institutes of Health Visiting Fellows Program FX We thank the Collaborative Crystallography group at NIEHS for help with data collection and analysis. We thank L. Pedersen and L. Perera for valuable discussions. This research was supported in part by the Intramural Research Program of the US National Institutes of Health, National Institute of Environmental Health Sciences (project numbers Z01-ES050158 and Z01-ES050161 (S.H.W.)). A part of this research was performed at Oak Ridge National Laboratory's Spallation Neutron Source and the Joint Institute for Neutron Sciences Biophysical Characterization Laboratory, sponsored by the United States Department of Energy, Office of Basic Energy Sciences (M.J.C.). N.S.D is supported in part by Eli Lilly and Co. and the United States Department of State, as part of the United States-Russia Collaboration in the Biomedical Sciences US National Institutes of Health Visiting Fellows Program. NR 57 TC 12 Z9 13 U1 4 U2 13 PU NATURE PUBLISHING GROUP PI NEW YORK PA 75 VARICK ST, 9TH FLR, NEW YORK, NY 10013-1917 USA SN 1545-9993 EI 1545-9985 J9 NAT STRUCT MOL BIOL JI Nat. Struct. Mol. Biol. PD NOV PY 2015 VL 22 IS 11 BP 924 EP 931 DI 10.1038/nsmb.3105 PG 8 WC Biochemistry & Molecular Biology; Biophysics; Cell Biology SC Biochemistry & Molecular Biology; Biophysics; Cell Biology GA CV4ZA UT WOS:000364273800017 PM 26458045 ER PT J AU Howard, TK Marcum, WR Jones, WF AF Howard, T. K. Marcum, W. R. Jones, W. F. TI A novel approach to modeling plate deformations in fluid-structure interactions SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article DE K. Thermal hydraulics ID DYNAMIC HYDROELASTIC INSTABILITIES; FUEL ASSEMBLIES; FLAT PLATES; FLOW; STABILITY; ELEMENTS AB As computational power increases, so does the desire to use computational simulations while designing fuel plates. The downside is multi-physics simulations - or more specifically, fluid-structure interactions (FSI) as addressed herein - require a larger amount of computational resources. Current simulations of a single plate can take weeks on a desktop computer, thus requiring the use of multiple servers or a cluster for FSI simulations. While computational fluid dynamic (CFD) codes coupled to computational structural mechanics (CSM) codes can provide a wealth of information regarding flow patterns, there should be some skepticism in whether or not they are the only means of achieving the desired solution. When the parameters of interest are the onset of plate collapse and the associated fluid channel velocities, coupled CFD-CSM simulations provide superfluous information. The paper provides an alternative approach to solving FSI problems using a 1-D, semi-analytical model derived from first principles. The results are compared and contrasted to the numerical and experimental work performed by Kennedy et al. (2014. Experimental Investigation of Deflection of Flat Aluminium Plates Under Variable Velocity Parallel Flow, Columbia: University of Missouri TherMec Research Group). (C) 2015 Elsevier B.V. All rights reserved. C1 [Howard, T. K.; Marcum, W. R.] Oregon State Univ, Dept Nucl Engn & Radiat Hlth Phys, Corvallis, OR 97331 USA. [Jones, W. F.] Idaho Natl Lab, Nucl Fuels & Mat Dept, Idaho Falls, ID 83415 USA. RP Howard, TK (reprint author), Oregon State Univ, Dept Nucl Engn & Radiat Hlth Phys, 116 Radiat Ctr, Corvallis, OR 97331 USA. EM howartre@onid.oregonstate.edu; marcumw@engr.orst.edu NR 21 TC 0 Z9 0 U1 1 U2 6 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 EI 1872-759X J9 NUCL ENG DES JI Nucl. Eng. Des. PD NOV PY 2015 VL 293 BP 1 EP 15 DI 10.1016/j.nucengdes.2015.06.010 PG 15 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CV3LX UT WOS:000364161800001 ER PT J AU Bahn, CB Oh, YJ Majumdar, S AF Bahn, Chi Bum Oh, Young-Jin Majumdar, Saurin TI Ligament rupture and unstable burst behaviors of axial flaws in steam generator U-bends SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article ID LIMIT LOADS; PRESSURE; TUBES AB Incidents of U-bend cracking in steam generator (SG) tubes have been reported, some of which have led to tube rupture. Experimental and analytical modeling efforts to determine the failure criteria of flawed SG U-bends are limited. To evaluate structural integrity of flawed U-bends, ligament rupture and unstable burst pressure tests were conducted on 57 and 152 mm bend radius U-bends with axial electrical discharge machining notches. In general, the ligament rupture and burst pressures of the U-bends were higher than those of straight tubes with similar notches. To quantitatively address the test data scatter issue, probabilistic models were introduced. All ligament rupture and burst pressures of U-bends were bounded by 90% lower limits of the probabilistic models for straight tubes. It was concluded that the prediction models for straight tubes could be applied to U-bends to conservatively evaluate the ligament rupture and burst pressures of U-bends with axial flaws. (C) 2015 Elsevier B.V. All rights reserved. C1 [Bahn, Chi Bum] Pusan Natl Univ, Busan 609735, South Korea. [Oh, Young-Jin] KEPCO Engn & Construct Co Inc, Songnam 463870, South Korea. [Majumdar, Saurin] Argonne Natl Lab, Lemont, IL 60439 USA. RP Bahn, CB (reprint author), Pusan Natl Univ, 2 Busandaehak Ro 63 Beon Gil, Busan 609735, South Korea. EM bahn@pusan.ac.kr FU Korea Institute of Energy Technology Evaluation and Planning (KETEP) from the Ministry of Trade Industry and Energy [20138530030010] FX The experimental work in this article was supported by the U.S. Nuclear Regulatory Commission. This work was also financially supported by the International Collaborative Energy Technology R&D Program (no. 20138530030010) of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) granted financial resource from the Ministry of Trade Industry and Energy. NR 22 TC 0 Z9 0 U1 1 U2 1 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 EI 1872-759X J9 NUCL ENG DES JI Nucl. Eng. Des. PD NOV PY 2015 VL 293 BP 228 EP 237 DI 10.1016/j.nucengdes.2015.06.019 PG 10 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CV3LX UT WOS:000364161800025 ER PT J AU Mo, K Yun, D Yacout, AM Wright, AE AF Mo, Kun Yun, Di Yacout, Abdellatif M. Wright, Arthur E. TI Heat transfer simulations of the UO2 particle-graphite system in TREAT fuel SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article ID THERMAL-CONDUCTIVITY DEGRADATION; ACCIDENT-TOLERANT FUELS; URANIUM-DIOXIDE; THERMOPHYSICAL PROPERTIES; NEUTRON-IRRADIATION; LOW-TEMPERATURE; MIXED-OXIDE; MODEL; PERFORMANCE; OXIDATION AB In this study, a heat transfer simulation of a UO2 particle-graphite system in highly enriched nuclear fuel at the Transient Reactor Test Facility (TREAT) was performed using the finite element method. Different factors that can impact fuel performance were modeled and implemented in the simulated micro-scale UO2 particle-graphite system. The fission fragments caused an irradiation-induced degradation of the thermal conductivity of the graphite, which added major heat resistance to the irradiated system. The effect of graphite quality and irradiation on the UO2 particles has also been evaluated, but neither has an impact as pronounced as the fission fragment damage to the graphite. By combining these factors, the dynamic temperature profiles were obtained, and the limitations on particle size in the irradiated and unirradiated UO2 particle-graphite systems have been determined. (C) 2015 Published by Elsevier B.V. C1 [Mo, Kun; Yun, Di; Yacout, Abdellatif M.; Wright, Arthur E.] Argonne Natl Lab, Nucl Engn Div, Lemont, IL 60439 USA. RP Mo, K (reprint author), Argonne Natl Lab, Nucl Engn Div, 9700 S Cass Ave, Lemont, IL 60439 USA. EM kunmo@anl.gov FU UChicago Argonne, LLC [DE-AC-02-06CH11357]; Department of Energy [DE-AC-02-06CH11357] FX This work was sponsored by the U.S. Department of Energy, Office of Global Threat Reduction (NA-21), National Nuclear Security Administration, under Contract No. DE-AC-02-06CH11357 between UChicago Argonne, LLC and the Department of Energy. NR 55 TC 0 Z9 0 U1 3 U2 6 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 EI 1872-759X J9 NUCL ENG DES JI Nucl. Eng. Des. PD NOV PY 2015 VL 293 BP 313 EP 322 DI 10.1016/j.nucengdes.2015.08.009 PG 10 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CV3LX UT WOS:000364161800032 ER PT J AU Gamble, KA Williams, AF Chan, PK Wowk, D AF Gamble, Kyle A. Williams, Anthony F. Chan, Paul K. Wowk, Diane TI A feasibility study on the use of the MOOSE computational framework to simulate three-dimensional deformation of CANDU reactor fuel elements SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article ID MULTIDIMENSIONAL MULTIPHYSICS SIMULATION; IRRADIATED UO2 FUEL AB Horizontally oriented fuel bundles, such as those in CANada Deuterium Uranium (CANDU) reactors present unique modeling challenges. After long irradiation times or during severe transients the fuel elements can laterally deform out of plane due to processes known as bow and sag. Bowing is a thermally driven process that causes the fuel elements to laterally deform when a temperature gradient develops across the diameter of the element. Sagging is a coupled mechanical and thermal process caused by deformation of the fuel pin due to creep mechanisms of the sheathing after long irradiation times and or high temperatures. These out-of-plane deformations can lead to reduced coolant flow and a reduction in coolability of the fuel bundle. In extreme cases element-to-element or element-to-pressure tube contact could occur leading to reduced coolant flow in the subchannels or pressure tube rupture leading to a loss of coolant accident. This paper evaluates the capability of the Multiphysics Object-Oriented Simulation Environment (MOOSE) framework developed at the Idaho National Laboratory to model these deformation mechanisms. The material model capabilities of MOOSE and its ability to simulate contact are also investigated. Crown Copyright (C) 2015 Published by Elsevier B.V. All rights reserved. C1 [Gamble, Kyle A.; Chan, Paul K.] Royal Mil Coll Canada, Chem & Chem Engn, Kingston, ON K7K 7B4, Canada. [Williams, Anthony F.] Canadian Nucl Labs, Fuel & Fuel Channel Safety, Chalk River, ON K0J 1J0, Canada. [Wowk, Diane] Royal Mil Coll Canada, Mech & Aerosp Engn, Kingston, ON K7K 7B4, Canada. RP Gamble, KA (reprint author), Idaho Natl Lab, Fuel Modeling & Simulat, POB 1625, Idaho Falls, ID 83415 USA. EM Kyle.Gamble@inl.gov; Tony.Williams@cnl.ca; Paul.Chan@rmc.ca; Diane.Wowk@rmc.ca FU Natural Sciences and Engineering Research Council of Canada (NSERC) under CRDPJ [415247]; MOOSE at the Idaho National Laboratory; BISON at the Idaho National Laboratory FX The authors would like to thank the MOOSE and BISON developers at the Idaho National Laboratory for their support. Thanks are also extended to the Idaho National Laboratory for allowing the use of their fission high performance computer cluster for running the full fuel element analyses. Funding for this research was provided by the Natural Sciences and Engineering Research Council of Canada (NSERC) under CRDPJ #415247. NR 26 TC 1 Z9 1 U1 3 U2 4 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 EI 1872-759X J9 NUCL ENG DES JI Nucl. Eng. Des. PD NOV PY 2015 VL 293 BP 385 EP 394 DI 10.1016/j.nucengdes.2015.07.028 PG 10 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CV3LX UT WOS:000364161800038 ER PT J AU Hugo, J Gertman, D AF Hugo, Jacques Gertman, David TI Selecting HSIs for new nuclear plants SO NUCLEAR ENGINEERING INTERNATIONAL LA English DT Article C1 [Hugo, Jacques; Gertman, David] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Hugo, J (reprint author), Idaho Natl Lab, Idaho Falls, ID 83415 USA. EM jacques.hugo@inl.gov; david.gertman@inl.gov NR 0 TC 0 Z9 0 U1 0 U2 0 PU WILMINGTON PUBL PI SIDCUP PA WILMINGTON HOUSE, MAIDSTONE RD, FOOTS CRAY, SIDCUP DA14 SHZ, KENT, ENGLAND SN 0029-5507 J9 NUCL ENG INT JI Nucl. Eng. Int. PD NOV PY 2015 VL 60 IS 736 BP 34 EP 37 PG 4 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CV2VF UT WOS:000364114600011 ER PT J AU Bzdak, A Skokov, V AF Bzdak, Adam Skokov, Vladimir TI Multi-particle eccentricities in collisions dominated by fluctuations SO NUCLEAR PHYSICS A LA English DT Article DE LHC; p plus A; Quark gluon plasma ID LONG-RANGE; ANGULAR-CORRELATIONS; TRANSVERSE-MOMENTUM; NUCLEUS COLLISIONS; PROTON-NUCLEUS; PB COLLISIONS; SIDE AB We compute analytically the multi-particle eccentricities, epsilon(m) {2n}, for systems dominated by fluctuations, such as proton -nucleus collisions at the Large Hadron Collider. In particular, we derive a general relation for . We further discuss the relations between various multi-particle eccentricities and demonstrate that epsilon(2){2} > epsilon(2){4} similar or equal to 62{6} similar or equal to epsilon(2){8}, in agreement with recent numerical calculations in a Glauber model. (C) 2015 Elsevier B.V. All rights reserved. C1 [Bzdak, Adam] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Bzdak, Adam; Skokov, Vladimir] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Skokov, Vladimir] Western Michigan Univ, Dept Phys, Kalamazoo, MI 49008 USA. RP Bzdak, A (reprint author), AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. EM bzdak@fis.agh.edu.pl; vskokov@quark.phy.bnl.gov FU Ministry of Science and Higher Education (MNiSW); Foundation for Polish Science; National Science Centre [DEC-2014/15/B/ST2/0017, DEC-2013/09/B/ST2100497]; RIKEN-BNL Research Center FX We thank R. Pisarski for valuable comments. A.B. was supported through the RIKEN-BNL Research Center, by the Ministry of Science and Higher Education (MNiSW), by founding from the Foundation for Polish Science, and by the National Science Centre, Grant No. DEC-2014/15/B/ST2/00175, and in part by DEC-2013/09/B/ST2100497. V.S. acknowledges support and hospitality of RIKEN-BNL Research Center, where this work was initiated. NR 44 TC 4 Z9 4 U1 0 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0375-9474 EI 1873-1554 J9 NUCL PHYS A JI Nucl. Phys. A PD NOV PY 2015 VL 943 BP 1 EP 8 DI 10.1016/j.nuclphysa.2015.08.001 PG 8 WC Physics, Nuclear SC Physics GA CV4WN UT WOS:000364267300001 ER PT J AU Boudichevskaia, A Heckwolf, M Kaldenhoff, R AF Boudichevskaia, Anastassia Heckwolf, Marlies Kaldenhoff, Ralf TI T-DNA insertion in aquaporin gene AtPIP1;2 generates transcription profiles reminiscent of a low CO2 response SO PLANT CELL AND ENVIRONMENT LA English DT Article DE Arabidopsis; CO2 diffusion; transcriptome ID ARABIDOPSIS-THALIANA; DROUGHT STRESS; MESOPHYLL CONDUCTANCE; MEMBRANE-DIFFUSION; PLANT AQUAPORINS; QUANTITATIVE PCR; EXPRESSION; WATER; CHANNELS; TOBACCO AB Results from CO2 diffusion studies and characterization of Arabidopsis thaliana aquaporin AtPIP1;2T-DNA insertion lines support the idea that specific aquaporins facilitate the diffusion of CO2 through biological membranes. However, their function as CO2 diffusion facilitators in plant physiology is still a matter of debate. Assuming that a lack of AtPIP1;2 causes a characteristic transcriptional response, we compared data from a AtPIP1;2T-DNA insertion line obtained by Illumina sequencing, Affymetrix chip analysis and quantitative RT-PCR to the transcriptome of plants grown under drought stress or under low CO2 conditions. The plant reaction to the deficit of AtPIP1;2 was unlike drought stress responses but comparable with that of low CO2 conditions. In addition, we observed a phenotype characteristic to plants grown under low CO2. The findings support the hypothesis that the AtPIP1;2 function in plant physiology is not to facilitate water but CO2 diffusion. The results from a transcriptome analysis of an Arabidopsis thaliana T-DNA insertion mutant line provide evidence that the product of the respective gene AtPIP1;2 caused an answer related to a limitation of CO2 diffusion. To our opinion, it provides an important argument to the ongoing debate about the significance of these kinds of aquaporins: whether the protein is a component of drought stress management or facilitates CO2 diffusion. C1 [Boudichevskaia, Anastassia; Heckwolf, Marlies; Kaldenhoff, Ralf] Tech Univ Darmstadt, Appl Plant Sci, D-64287 Darmstadt, Germany. [Heckwolf, Marlies] Univ Wisconsin, Dept Energy, Dept Agron, Great Lakes Bioenergy Res Ctr, Madison, WI 53703 USA. RP Kaldenhoff, R (reprint author), Tech Univ Darmstadt, Appl Plant Sci, D-64287 Darmstadt, Germany. EM kaldenhoff@bio.tu-darmstadt.de NR 58 TC 2 Z9 4 U1 1 U2 21 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0140-7791 EI 1365-3040 J9 PLANT CELL ENVIRON JI Plant Cell Environ. PD NOV PY 2015 VL 38 IS 11 BP 2286 EP 2298 DI 10.1111/pce.12547 PG 13 WC Plant Sciences SC Plant Sciences GA CU9SE UT WOS:000363884600009 PM 25850563 ER PT J AU Degteva, MO Shagina, NB Shishkina, EA Vozilova, AV Volchkova, AY Vorobiova, MI Wieser, A Fattibene, P Della Monaca, S Ainsbury, E Moquet, J Anspaugh, LR Napier, BA AF Degteva, M. O. Shagina, N. B. Shishkina, E. A. Vozilova, A. V. Volchkova, A. Y. Vorobiova, M. I. Wieser, A. Fattibene, P. Della Monaca, S. Ainsbury, E. Moquet, J. Anspaugh, L. R. Napier, B. A. TI Analysis of EPR and FISH studies of radiation doses in persons who lived in the upper reaches of the Techa River SO RADIATION AND ENVIRONMENTAL BIOPHYSICS LA English DT Article DE Dose reconstruction; Environmental contamination; Techa River; Electron paramagnetic resonance; Fluorescence in situ hybridization ID ELECTRON-PARAMAGNETIC-RESONANCE; MAYAK-PRODUCTION-ASSOCIATION; RECONSTRUCTION SYSTEM; DOSIMETRY SYSTEM; CANCER-MORTALITY; TOOTH ENAMEL; POPULATION; TRANSLOCATIONS; EXPOSURE; COHORT AB Waterborne radioactive releases into the Techa River from the Mayak Production Association in Russia during 1949-1956 resulted in significant doses to about 30,000 persons who lived in downstream settlements. The residents were exposed to internal and external radiation. Two methods for reconstruction of the external dose are considered in this paper, electron paramagnetic resonance (EPR) measurements of teeth, and fluorescence in situ hybridization (FISH) measurements of chromosome translocations in circulating lymphocytes. The main issue in the application of the EPR and FISH methods for reconstruction of the external dose for the Techa Riverside residents was strontium radioisotopes incorporated in teeth and bones that act as a source of confounding local exposures. In order to estimate and subtract doses from incorporated Sr-89,Sr-90, the EPR and FISH assays were supported by measurements of Sr-90-body burdens and estimates of Sr-90 concentrations in dental tissues by the luminescence method. The resulting dose estimates derived from EPR to FISH measurements for residents of the upper Techa River were found to be consistent: The mean values vary from 510 to 550 mGy for the villages located close to the site of radioactive release to 130-160 mGy for the more distant villages. The upper bound of individual estimates for both methods is equal to 2.2-2.3 Gy. The EPR- and FISH-based dose estimates were compared with the doses calculated for the donors using the most recent Techa River Dosimetry System (TRDS). The TRDS external dose assessments are based on the data on contamination of the Techa River floodplain, simulation of air kerma above the contaminated soil, age-dependent lifestyles and individual residence histories. For correct comparison, TRDS-based doses were calculated from two sources: external exposure from the contaminated environment and internal exposure from Cs-137 incorporated in donors' soft tissues. It is shown here that the TRDS-based absorbed doses in tooth enamel and muscle are in agreement with EPR- and FISH-based estimates within uncertainty bounds. Basically, this agreement between the estimates has confirmed the validity of external doses calculated with the TRDS. C1 [Degteva, M. O.; Shagina, N. B.; Shishkina, E. A.; Vozilova, A. V.; Volchkova, A. Y.; Vorobiova, M. I.] Urals Res Ctr Radiat Med, Chelyabinsk 454076, Russia. [Wieser, A.] Helmholtz Ctr Munich, Neuherberg, Germany. [Fattibene, P.; Della Monaca, S.] Inst Super Sanita, Rome, Italy. [Ainsbury, E.; Moquet, J.] Publ Hlth England, Chilton, England. [Anspaugh, L. R.] Univ Utah, Salt Lake City, UT USA. [Napier, B. A.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Degteva, MO (reprint author), Urals Res Ctr Radiat Med, 68a Vorovsky St, Chelyabinsk 454076, Russia. EM marina@urcrm.ru; lena@urcrm.ru RI Shishkina, Elena/G-4595-2016; DELLA MONACA, SARA/E-9044-2015 OI Shishkina, Elena/0000-0003-4464-0889; DELLA MONACA, SARA/0000-0002-3109-9344 FU European Commission [FP7-249675]; US Department of Energy's Office of International Health Programs; Federal Medical-Biological Agency of the Russian Federation FX The EPR and FISH studies have been supported by the European Commission under contract number FP7-249675 "Epidemiological Studies of Exposed Southern Urals Populations" (SOLO). The work on development of the Techa River Dosimetry System (TRDS) has been supported by the US Department of Energy's Office of International Health Programs and the Federal Medical-Biological Agency of the Russian Federation. The authors acknowledge the contributions to the study, which were made by Denis Ivanov (IMP, Russia) and Firouz Darroudi (LUMC, the Netherlands). NR 34 TC 4 Z9 4 U1 1 U2 5 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0301-634X EI 1432-2099 J9 RADIAT ENVIRON BIOPH JI Radiat. Environ. Biophys. PD NOV PY 2015 VL 54 IS 4 BP 433 EP 444 DI 10.1007/s00411-015-0611-8 PG 12 WC Biology; Biophysics; Environmental Sciences; Radiology, Nuclear Medicine & Medical Imaging SC Life Sciences & Biomedicine - Other Topics; Biophysics; Environmental Sciences & Ecology; Radiology, Nuclear Medicine & Medical Imaging GA CV1OT UT WOS:000364028400005 PM 26205380 ER PT J AU Cosseddu, P Fraboni, B Scida, A Wang, YQ Nastasi, M Bonfiglio, A AF Cosseddu, P. Fraboni, B. Scida, A. Wang, Y. Q. Nastasi, M. Bonfiglio, A. TI Self-encapsulation of organic thin film transistors by means of ion implantation SO SYNTHETIC METALS LA English DT Article DE Organic thin film transistors; Encapsulation; Ion implantation; Ambient stability ID FIELD-EFFECT TRANSISTORS; PENTACENE; LAYER; SEMICONDUCTORS; PERFORMANCE AB Long-term stability of devices based on organic materials is still impeding the diffusion of these structures in real applications. In this paper we have investigated the effects of low energy, combined, ion implantation (N and Ne) in the evolution of the electrical performances of pentacene-based Organic Thin Film Transistors (OTFTs) over time by means of current-voltage and photocurrent spectroscopy analyses. We have demonstrated that the selected combination of ions allows reducing the degradation of charge carriers mobility, and also stabilization of the devices threshold voltage over a long time (over 2000 h). (c) 2015 Elsevier B.V. All rights reserved. C1 [Cosseddu, P.; Bonfiglio, A.] CNR, Inst Nanosci, S3Ctr, I-41100 Modena, Italy. [Cosseddu, P.; Bonfiglio, A.] Univ Cagliari, Dipartimento Ingn Elettr & Elettron, I-09123 Cagliari, Italy. [Fraboni, B.; Scida, A.] Univ Bologna, Dipartimento Fis & Astron, I-40127 Bologna, Italy. [Wang, Y. Q.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. [Nastasi, M.] Univ Nebraska, Nebraska Ctr Energy Sci Res, Lincoln, NE 68583 USA. RP Cosseddu, P (reprint author), Univ Cagliari, Dept Elect & Elect Engn, I-09123 Cagliari, Italy. EM piero.cosseddu@diee.unica.it OI COSSEDDU, Piero/0000-0003-4896-504X FU National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396]; European Commission [611070] FX This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-AC52-06NA25396.; P.C., B.F, and A.B. acknowledge financial support by the European Commission, under the FP7-ICT Project "I-FLEXIS", G.A. # 611070. NR 25 TC 0 Z9 0 U1 2 U2 2 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0379-6779 J9 SYNTHETIC MET JI Synth. Met. PD NOV PY 2015 VL 209 BP 178 EP 182 DI 10.1016/j.synthmet.2015.07.018 PG 5 WC Materials Science, Multidisciplinary; Physics, Condensed Matter; Polymer Science SC Materials Science; Physics; Polymer Science GA CV4OH UT WOS:000364245900026 ER PT J AU Abdel-Fattah, TM Younes, EM Namkoong, G El-Maghraby, EM Elsayed, AH Elazm, AHA AF Abdel-Fattah, Tarek M. Younes, Enas M. Namkoong, Gon El-Maghraby, E. M. Elsayed, Adly H. Elazm, A. H. Abo TI Stability study of low and high band gap polymer and air stability of PTB7:PC71BM bulk heterojunction organic photovoltaic cells with encapsulation technique SO SYNTHETIC METALS LA English DT Article DE Organic photovoltaics; Bulk heterojunction (BHJ); Low and high band gap polymers stability; Degradation; Sealant glass; Efficiency decay ID SOLAR-CELLS; ZINC-OXIDE; PERFORMANCE; INTERLAYER; EFFICIENT; LIFETIME; DEVICES; LAYER; FILM AB This study describes the air stability of organic photovoltaic (OPV) cells based on low band gap polymer, thieno(3,4-b)-thiophene/benzodithiophene copolymer and [6,6]-phenyl C-71 butyric acid methyl ester (PTB7:PC71BM) bulk heterojunction (BHJ) with titanium oxide (TiOx) layer. The ITO/PEDOT:PSS/PTB7: PC71BM/TiOx/Al device was fabricated and protected via an encapsulation technique. An optical sealant glass was used for encapsulating the device. We succeeded to keep the device in air for 20 days without a significant loss of its initial power conversion efficiency (PCE). After 20 days, the PTB7:PC71BM/TiOx device without encapsulation in air showed a rapid decrease in power conversion efficiency (PCE), losing approximately more than 98.0% of its initial value. The efficiency decays of the encapsulated devices in the nitrogen filled glove box and in air were about 32.3% and 41.7%, respectively. The organic photovoltaic cells based on high band gap polymer, poly(3-hexylthiophene) and [6,6]-phenyl C-71 butyric acid methyl ester (P3HT:PC71BM) BHJ with TiOx layer was fabricated. We compared the stability of P3HT:PC71BM and PTB7:PC71BM OPV devices for 10 days in a glove box with and without TiOx layer. We found that the device based on PTB7:PC71BM/TiOx organic photovoltaic cell has better stability than the P3HT:PC71BM/TiOx organic photovoltaic cell. (C) 2015 Elsevier B.V. All rights reserved. C1 [Abdel-Fattah, Tarek M.; Younes, Enas M.; Namkoong, Gon] Thomas Jefferson Natl Accelerator Facil, Appl Res Ctr, Newport News, VA 23606 USA. [Abdel-Fattah, Tarek M.; Younes, Enas M.] Christopher Newport Univ, Dept Mol Biol & Chem, Newport News, VA 23606 USA. [Younes, Enas M.; El-Maghraby, E. M.] Old Dominion Univ, Dept Elect & Comp Engn, Norfolk, VA 23529 USA. [Younes, Enas M.; Namkoong, Gon] Damanhour Univ, Dept Phys, Fac Sci, Damanhour 22111, Egypt. [Elsayed, Adly H.; Elazm, A. H. Abo] Univ Alexandria, Dept Phys, Fac Sci, Alexandria 21511, Egypt. RP Abdel-Fattah, TM (reprint author), Christopher Newport Univ, Dept Mol Biol & Chem, 12050 Jefferson Ave, Newport News, VA 23606 USA. EM fattah@cnu.edu RI Younes, Enas/F-6945-2015 OI Younes, Enas/0000-0001-9036-6775 FU Egyptian Government via a scholarship from the Culture Affairs and Mission Sector of the Egyptian Ministry of Higher Education FX This work was supported by the Egyptian Government via a scholarship from the Culture Affairs and Mission Sector of the Egyptian Ministry of Higher Education. NR 31 TC 3 Z9 3 U1 4 U2 41 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0379-6779 J9 SYNTHETIC MET JI Synth. Met. PD NOV PY 2015 VL 209 BP 348 EP 354 DI 10.1016/j.synthmet.2015.08.005 PG 7 WC Materials Science, Multidisciplinary; Physics, Condensed Matter; Polymer Science SC Materials Science; Physics; Polymer Science GA CV4OH UT WOS:000364245900050 ER PT J AU Bradshaw, NP Severt, SY Wang, ZY Fengel, CV Larson, JD Zhu, ZH Murphy, AR Leger, JM AF Bradshaw, Nathan P. Severt, Sean Y. Wang, Zhaoying Fengel, Carly V. Larson, Jesse D. Zhu, Zihua Murphy, Amanda R. Leger, Janelle M. TI ToF-SIMS characterization of silk fibroin and polypyrrole composite actuators SO SYNTHETIC METALS LA English DT Article DE ToF-SIMS; Actuator; Polypyrrole; Biocomposite; Bilayer; Artificial muscle ID CLUSTER ION-BEAMS; ELECTROMECHANICAL ACTUATORS; PHOTOCATALYTIC DEGRADATION; CONDUCTING POLYMERS; FREESTANDING FILMS; MASS-SPECTROMETRY; DIODE-ARRAY; CHROMATOGRAPHY; ELECTRODES; TI AB Biocompatible materials capable of controlled actuation under biologically relevant conditions are in high demand for use in a number of biomedical applications. Recently, we demonstrated that a composite material composed of silk biopolymer and the conducting polymer polypyrrole can bend under an applied voltage using a simple bilayer device. Here, further characterization of these bilayer actuators using time-of-flight secondary ion mass spectrometry is presented. The roles of different electrolyte components and factors affecting device performance and stability are clarified. Results of this study are discussed in the context of strategies for optimization of device performance. (C) 2015 Elsevier B.V. All rights reserved. C1 [Bradshaw, Nathan P.; Severt, Sean Y.; Larson, Jesse D.; Murphy, Amanda R.] Western Washington Univ, Dept Chem, Bellingham, WA 98225 USA. [Fengel, Carly V.; Leger, Janelle M.] Western Washington Univ, Dept Phys & Astron, Bellingham, WA 98225 USA. [Wang, Zhaoying; Zhu, Zihua] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Leger, JM (reprint author), Western Washington Univ, Dept Phys & Astron, 516 High St, Bellingham, WA 98225 USA. EM Janelle.Leger@wwu.edu RI Zhu, Zihua/K-7652-2012 FU Western Washington University; M.J. Murdock Charitable Trust; National Science Foundation [DMR-1411292, DMR-1057209]; Office of Biological and Environmental Research FX We are grateful for financial support from Western Washington University, a grant to WWU's Advanced Materials Science and Engineering Center (AMSEC) from the M.J. Murdock Charitable Trust, and the National Science Foundation (DMR-1411292 and DMR-1057209). A portion of the research was performed using EMSL, a DOE Office of Science User Facility sponsored by the Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. NR 26 TC 3 Z9 3 U1 4 U2 22 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0379-6779 J9 SYNTHETIC MET JI Synth. Met. PD NOV PY 2015 VL 209 BP 490 EP 495 DI 10.1016/j.synthmet.2015.08.031 PG 6 WC Materials Science, Multidisciplinary; Physics, Condensed Matter; Polymer Science SC Materials Science; Physics; Polymer Science GA CV4OH UT WOS:000364245900071 ER PT J AU Strmcnik, D Li, DG Lopes, PP Tripkovic, D Kodama, K Stamenkovic, VR Markovic, NM AF Strmcnik, Dusan Li, Dongguo Lopes, Pietro P. Tripkovic, Dusan Kodama, Kensaku Stamenkovic, Vojislav R. Markovic, Nenad M. TI When Small is Big: The Role of Impurities in Electrocatalysis SO TOPICS IN CATALYSIS LA English DT Article DE Electrocatalysis; ORR; CO oxidation; Impurity effect ID SINGLE-CRYSTAL ELECTRODES; OXYGEN EVOLUTION REACTION; SMALL ORGANIC-MOLECULES; FOREIGN METAL ADATOMS; UNDERPOTENTIAL DEPOSITION; NONCOVALENT INTERACTIONS; ACIDIC ENVIRONMENTS; AD-ATOMS; OXIDATION; PLATINUM AB Improvements in the fundamental understanding of electrocatalysis have started to revolutionize the development of electrochemical interfaces for the efficient conversion of chemical energy into electricity, as well as for the utilization of electrons to produce new chemicals that then can be re-used in energy conversion systems. Here, some facets of the role of trace level of impurities (from 10(-7) to 10(-6) M) in electrocatalysis of the oxygen reduction reaction, hydrogen oxidation and evolution reactions, and CO oxidation reactions are explored on well-characterized platinum single crystal surfaces and high surface area materials in alkaline and acidic environments. Of particular interest is the effect of anions (e.g., Cl-, NO3-) and cations (i.e., Cu2+) present in the supporting electrolytes as well as surface defects (i.e., ad-islands) that are present on metal surfaces. The examples presented are chosen to demonstrate that a small level of impurities may play a crucial role in governing the reactivity of electrochemical interfaces. C1 [Strmcnik, Dusan; Li, Dongguo; Lopes, Pietro P.; Tripkovic, Dusan; Kodama, Kensaku; Stamenkovic, Vojislav R.; Markovic, Nenad M.] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60559 USA. RP Markovic, NM (reprint author), Argonne Natl Lab, Div Mat Sci, Lemont, IL 60559 USA. EM nmmarkovic@anl.gov RI Lopes, Pietro/E-2724-2013; Li, Dongguo/O-6253-2016 OI Lopes, Pietro/0000-0003-3211-470X; Li, Dongguo/0000-0001-7578-7811 FU Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences [DE-AC0206CH11357] FX This work is supported by the Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences, under contract DE-AC0206CH11357. NR 45 TC 4 Z9 4 U1 18 U2 64 PU SPRINGER/PLENUM PUBLISHERS PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1022-5528 EI 1572-9028 J9 TOP CATAL JI Top. Catal. PD NOV PY 2015 VL 58 IS 18-20 BP 1174 EP 1180 DI 10.1007/s11244-015-0492-8 PG 7 WC Chemistry, Applied; Chemistry, Physical SC Chemistry GA CV0LC UT WOS:000363941200004 ER PT J AU Vianco, PT Neilsen, MK AF Vianco, P. T. Neilsen, M. K. TI Reliability Analysis of Pin-in-Hole Solder Joints SO WELDING JOURNAL LA English DT Editorial Material C1 [Vianco, P. T.; Neilsen, M. K.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Vianco, PT (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM ptvianc@sandia.gov NR 3 TC 0 Z9 0 U1 1 U2 1 PU AMER WELDING SOC PI MIAMI PA 550 N W LEJEUNE RD, MIAMI, FL 33126 USA SN 0043-2296 J9 WELD J JI Weld. J. PD NOV PY 2015 VL 94 IS 11 BP 56 EP 61 PG 6 WC Metallurgy & Metallurgical Engineering SC Metallurgy & Metallurgical Engineering GA CV4YS UT WOS:000364273000016 ER PT J AU Cholia, S Sun, T AF Cholia, Shreyas Sun, Terence TI The NEWT platform: an extensible plugin framework for creating ReSTful HPC APIs SO CONCURRENCY AND COMPUTATION-PRACTICE & EXPERIENCE LA English DT Article DE ReST; API; HTTP; web; HPC; scientific computing AB This work describes the NEWT platform, a framework for creating ReSTful web APIs for high-performance scientific computing. The NEWT platform is designed to be a customizable framework that can be deployed at a high-performance computing center and enables access to various backend resources and services through a common web API. The goal of this effort is to create a service that can be plugged into multiple backend resources and can easily be extended while presenting a standard interface to the consumer with common semantics. This effort also updates the NEWT API that has been deployed at the National Energy Research Scientific Computing Center since 2010 and provides additional structure and consistency across the API. Copyright (c) 2015 John Wiley & Sons, Ltd. C1 [Cholia, Shreyas; Sun, Terence] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Sun, Terence] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. RP Cholia, S (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM scholia@lbl.gov FU Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX This research used resources of the National Energy Research Scientific Computing Center (NERSC), a DOE Office of Science User Facility supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 14 TC 1 Z9 1 U1 0 U2 0 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1532-0626 EI 1532-0634 J9 CONCURR COMP-PRACT E JI Concurr. Comput.-Pract. Exp. PD NOV PY 2015 VL 27 IS 16 SI SI BP 4304 EP 4317 DI 10.1002/cpe.3517 PG 14 WC Computer Science, Software Engineering; Computer Science, Theory & Methods SC Computer Science GA CU4BK UT WOS:000363470800019 ER PT J AU Madduri, R Chard, K Chard, R Lacinski, L Rodriguez, A Sulakhe, D Kelly, D Dave, U Foster, I AF Madduri, Ravi Chard, Kyle Chard, Ryan Lacinski, Lukasz Rodriguez, Alex Sulakhe, Dinanath Kelly, David Dave, Utpal Foster, Ian TI The Globus Galaxies platform: delivering science gateways as a service SO CONCURRENCY AND COMPUTATION-PRACTICE & EXPERIENCE LA English DT Article DE Cloud Computing; Science Gateways; HPC ID CLOUD AB The use of public cloud computers to host sophisticated scientific data and software is transforming scientific practice by enabling broad access to capabilities previously available only to the few. The primary obstacle to more widespread use of public clouds to host scientific software (cloud-based science gateways') has thus far been the considerable gap between the specialized needs of science applications and the capabilities provided by cloud infrastructures. We describe here a domain-independent, cloud-based science gateway platform, the Globus Galaxies platform, which overcomes this gap by providing a set of hosted services that directly address the needs of science gateway developers. The design and implementation of this platform leverages our several years of experience with Globus Genomics, a cloud-based science gateway that has served more than 200 genomics researchers across 30 institutions. Building on that foundation, we have implemented a platform that leverages the popular Galaxy system for application hosting and workflow execution; Globus services for data transfer, user and group management, and authentication; and a cost-aware elastic provisioning model specialized for public cloud resources. We describe here the capabilities and architecture of this platform, present six scientific domains in which we have successfully applied it, report on user experiences, and analyze the economics of our deployments. Published 2015. This article is a U.S. Government work and is in the public domain in the USA. C1 [Madduri, Ravi; Chard, Kyle; Lacinski, Lukasz; Rodriguez, Alex; Sulakhe, Dinanath; Kelly, David; Dave, Utpal; Foster, Ian] Univ Chicago, Computat Inst, Chicago, IL 60637 USA. [Madduri, Ravi; Chard, Kyle; Lacinski, Lukasz; Rodriguez, Alex; Sulakhe, Dinanath; Kelly, David; Dave, Utpal; Foster, Ian] Argonne Natl Lab, Chicago, IL 60637 USA. [Chard, Ryan] Victoria Univ Wellington, Sch Engn & Comp Sci, Wellington, New Zealand. RP Madduri, R (reprint author), Univ Chicago, Computat Inst, Chicago, IL 60637 USA. EM madduri@mcs.anl.gov OI Madduri, Ravi/0000-0003-2130-2887 FU US Department of Energy [DE-AC02-06CH11357]; NIH [U24 GM104203, R24HL085343]; NIH, Big Data for Discovery Science (BDDS) Center [1U54EB020406-01] FX This work was supported in part by the US Department of Energy under contract DE-AC02-06CH11357 and the NIH through U24 GM104203 Bio-Informatics Research Network Coordinating Center (BIRN-CC) and R24HL085343 Cardiovascular Research Grid (CVRG). We would like to acknowledge generous research credits provided by Amazon Web Services that helped support our work. We also appreciate the support of the Globus and Galaxy teams. This work is supported in part by NIH under contract 1U54EB020406-01, Big Data for Discovery Science (BDDS) Center. NR 28 TC 9 Z9 9 U1 1 U2 4 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1532-0626 EI 1532-0634 J9 CONCURR COMP-PRACT E JI Concurr. Comput.-Pract. Exp. PD NOV PY 2015 VL 27 IS 16 SI SI BP 4344 EP 4360 DI 10.1002/cpe.3486 PG 17 WC Computer Science, Software Engineering; Computer Science, Theory & Methods SC Computer Science GA CU4BK UT WOS:000363470800022 ER PT J AU Montella, R Kelly, D Xiong, W Brizius, A Elliott, J Madduri, R Maheshwari, K Porter, C Vilter, P Wilde, M Zhang, M Foster, I AF Montella, Raffaele Kelly, David Xiong, Wei Brizius, Alison Elliott, Joshua Madduri, Ravi Maheshwari, Ketan Porter, Cheryl Vilter, Peter Wilde, Michael Zhang, Meng Foster, Ian TI FACE-IT: A science gateway for food security research SO CONCURRENCY AND COMPUTATION-PRACTICE & EXPERIENCE LA English DT Article DE science gateways; climate impacts and food security; globus galaxies ID GLOBUS; SERVICES; GENOMICS; MODELS; GALAXY AB Progress in sustainability science is hindered by challenges in creating and managing complex data acquisition, processing, simulation, post-processing, and intercomparison pipelines. To address these challenges, we developed the Framework to Advance Climate, Economic, and Impact Investigations with Information Technology (FACE-IT) for crop and climate impact assessments. This integrated data processing and simulation framework enables data ingest from geospatial archives; data regridding, aggregation, and other processing prior to simulation; large-scale climate impact simulations with agricultural and other models, leveraging high-performance and cloud computing; and post-processing to produce aggregated yields and ensemble variables needed for statistics, for model intercomparison, and to connect biophysical models to global and regional economic models. FACE-IT leverages the capabilities of the Globus Galaxies platform to enable the capture of workflows and outputs in well-defined, reusable, and comparable forms. We describe FACE-IT and applications within the Agricultural Model Intercomparison and Improvement Project and the Center for Robust Decision-making on Climate and Energy Policy. Copyright (c) 2015 John Wiley & Sons, Ltd. C1 [Montella, Raffaele] Univ Naples Parthenope, Dept Sci & Technol, Naples, Italy. [Montella, Raffaele; Kelly, David; Brizius, Alison; Elliott, Joshua; Madduri, Ravi; Vilter, Peter; Wilde, Michael; Foster, Ian] Argonne Natl Lab, Computat Inst, Argonne, IL 60439 USA. [Montella, Raffaele; Kelly, David; Brizius, Alison; Elliott, Joshua; Madduri, Ravi; Vilter, Peter; Wilde, Michael; Foster, Ian] Univ Chicago, Chicago, IL 60637 USA. [Xiong, Wei; Porter, Cheryl; Wilde, Michael] Univ Florida, Dept Agr & Biol Engn, Gainesville, FL USA. [Madduri, Ravi; Maheshwari, Ketan; Wilde, Michael; Foster, Ian] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. [Foster, Ian] Univ Chicago, Dept Comp Sci, Chicago, IL 60637 USA. RP Elliott, J (reprint author), Argonne Natl Lab, Computat Inst, Argonne, IL 60439 USA. EM jelliott@ci.uchicago.edu OI Madduri, Ravi/0000-0003-2130-2887 FU NSF cyberSEES program [ACI-1331782]; NSF Decision Making Under Uncertainty program [0951576]; DOE [DE-AC02-06CH11357] FX We thank the Globus Galaxies, Globus, and Galaxy teams for their outstanding work on those systems and for their assistance with this project. This work was supported by the NSF cyberSEES program award ACI-1331782, the NSF Decision Making Under Uncertainty program award 0951576, and the DOE under contract DE-AC02-06CH11357. EC2 resources have been generously provided by Amazon. NR 21 TC 2 Z9 2 U1 0 U2 5 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1532-0626 EI 1532-0634 J9 CONCURR COMP-PRACT E JI Concurr. Comput.-Pract. Exp. PD NOV PY 2015 VL 27 IS 16 SI SI BP 4423 EP 4436 DI 10.1002/cpe.3540 PG 14 WC Computer Science, Software Engineering; Computer Science, Theory & Methods SC Computer Science GA CU4BK UT WOS:000363470800027 ER PT J AU Johnson, TC Versteeg, RJ Day-Lewis, FD Major, W Lane, JW AF Johnson, Timothy C. Versteeg, Roelof J. Day-Lewis, Frederick D. Major, William Lane, John W., Jr. TI Time-Lapse Electrical Geophysical Monitoring of Amendment-Based Biostimulation SO GROUNDWATER LA English DT Article ID CROSS-BOREHOLE RADAR; RESISTIVITY TOMOGRAPHY; VADOSE ZONE; AQUIFER CHARACTERIZATION; RESISTANCE TOMOGRAPHY; INDUCED POLARIZATION; REDOX CONDITIONS; RIVER-WATER; TRACER; CONDUCTIVITY AB Biostimulation is increasingly used to accelerate microbial remediation of recalcitrant groundwater contaminants. Effective application of biostimulation requires successful emplacement of amendment in the contaminant target zone. Verification of remediation performance requires postemplacement assessment and contaminant monitoring. Sampling-based approaches are expensive and provide low-density spatial and temporal information. Time-lapse electrical resistivity tomography (ERT) is an effective geophysical method for determining temporal changes in subsurface electrical conductivity. Because remedial amendments and biostimulation-related biogeochemical processes often change subsurface electrical conductivity, ERT can complement and enhance sampling-based approaches for assessing emplacement and monitoring biostimulation-based remediation. Field studies demonstrating the ability of time-lapse ERT to monitor amendment emplacement and behavior were performed during a biostimulation remediation effort conducted at the Department of Defense Reutilization and Marketing Office (DRMO) Yard, in Brandywine, Maryland, United States. Geochemical fluid sampling was used to calibrate a petrophysical relation in order to predict groundwater indicators of amendment distribution. The petrophysical relations were field validated by comparing predictions to sequestered fluid sample results, thus demonstrating the potential of electrical geophysics for quantitative assessment of amendment-related geochemical properties. Crosshole radar zero-offset profile and borehole geophysical logging were also performed to augment the data set and validate interpretation. In addition to delineating amendment transport in the first 10 months after emplacement, the time-lapse ERT results show later changes in bulk electrical properties interpreted as mineral precipitation. Results support the use of more cost-effective surface-based ERT in conjunction with limited field sampling to improve spatial and temporal monitoring of amendment emplacement and remediation performance. C1 [Johnson, Timothy C.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. [Versteeg, Roelof J.] Subsurface Insights LLC, Hanover, NH 03755 USA. [Day-Lewis, Frederick D.; Lane, John W., Jr.] US Geol Survey, Off Groundwater, Branch Geophys, Storrs, CT 06269 USA. [Major, William] US Naval Facil, Engn Serv Ctr, Port Hueneme, CA 93043 USA. RP Johnson, TC (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. EM TJ@pnnl.gov; roelof.versteeg@subsurfaceinsights.com; daylewis@usgs.gov; majorwr@gmail.com; jwlane@usgs.gov OI Day-Lewis, Frederick/0000-0003-3526-886X FU Department of Defense Environmental Security Technology Certification Program (ESTCP) [ER-0717]; U.S. Geological Survey Toxic Substances Hydrology and Groundwater Resources Programs FX This research was supported by grant ER-0717 from the Department of Defense Environmental Security Technology Certification Program (ESTCP), with additional support from the U.S. Geological Survey Toxic Substances Hydrology and Groundwater Resources Programs. We are grateful for field assistance from Jessica Teunis, Peter Lapa-Lilly, Eric White, Rory Henderson, Emily Voytek, Jim Rauman, Jason Smith (USGS); Yuxin Wu (Lawrence Berkeley National Labroatory); and Karen Wright (Idaho National Laboratory). We also are grateful to the ESTCP program manager, Andrea Leeson, who provided useful comments on aspects of this project, and to the staff of HGL, Mactec, and Andrews Air Force Base who facilitated our site access and provided useful information regarding the Brandywine remediation effort. Any use of trade, firm, or product names is for descriptive purposes only and does not imply endorsement by the U.S. Government. NR 65 TC 2 Z9 2 U1 1 U2 9 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0017-467X EI 1745-6584 J9 GROUNDWATER JI Groundwater PD NOV-DEC PY 2015 VL 53 IS 6 BP 920 EP 932 DI 10.1111/gwat.12291 PG 13 WC Geosciences, Multidisciplinary; Water Resources SC Geology; Water Resources GA CU9VM UT WOS:000363894200013 PM 25457440 ER PT J AU Silva, CM Snead, LL Hunn, JD Specht, ED Terrani, KA Katoh, Y AF Silva, C. M. Snead, L. L. Hunn, J. D. Specht, E. D. Terrani, K. A. Katoh, Y. TI Application of X-ray microcomputed tomography in the characterization of irradiated nuclear fuel and material specimens SO JOURNAL OF MICROSCOPY LA English DT Article DE carbon-carbon fibre composites; FCM; nuclear-grade graphite; TRISO; X-ray microtomography ID GRAPHITE; MICROSTRUCTURE; PARTICLES AB X-ray microcomputed tomography (CT) was applied in characterizing the internal structures of a number of irradiated materials, including carbon-carbon fibre composites, nuclear-grade graphite and tristructural isotropic-coated fuel particles. Local cracks in carbon-carbon fibre composites associated with their synthesis process were observed with CT without any destructive sample preparation. Pore analysis of graphite samples was performed quantitatively, and qualitative analysis of pore distribution was accomplished. It was also shown that high-resolution CT can be used to probe internal layer defects of tristructural isotropic-coated fuel particles to elucidate the resulting high release of radioisotopes. Layer defects of sizes ranging from 1 to 5 m and up could be isolated by tomography. As an added advantage, CT could also be used to identify regions with high densities of radioisotopes to determine the proper plane and orientation of particle mounting for further analytical characterization, such as materialographic sectioning followed by optical and electron microscopy. In fully ceramic matrix fuel forms, despite the highly absorbing matrix, characterization of tristructural isotropic-coated particles embedded in a silicon carbide matrix was accomplished using CT and related advanced image analysis techniques. Lay Description X-ray tomography was applied in characterizing a number of materials that relate to nuclear fuel industry. These include carbon-carbon (C-C) fibre composites, nuclear-grade graphite and tristructural isotropic (TRISO)-coated fuel particles. Cracks within C-C composites associated with their synthesis process were observed using tomography without damaging the samples. Characteristics of voids in the graphite samples were evaluated qualitatively and quantitatively. Internal layer defects of TRISO-coated fuel particles were also examined. Layer defects of sizes ranging from 1 to 5 m and up could be isolated by tomography. As an added advantage, tomography could be used to identify regions with high densities of radioactive elements to determine the proper way to mount the particles for further characterization using other microscopy techniques. Characterization of TRISO-coated particles embedded in a silicon carbide matrix was accomplished using tomography and related advanced image analysis techniques. C1 [Silva, C. M.; Snead, L. L.; Hunn, J. D.; Specht, E. D.; Terrani, K. A.; Katoh, Y.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Silva, CM (reprint author), Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. EM silvagw@ornl.gov FU US Department of Energy through the Office of Nuclear Energy, Science, and Technology's Fuel Cycle Research and Development Program [DE-AC05-00OR22725]; UT-Battelle, LLC. FX The authors thank Jim Kiggans and Charles Baldwin at ORNL for their support in preparing specimens. This research was sponsored by the US Department of Energy through the Office of Nuclear Energy, Science, and Technology's Fuel Cycle Research and Development Program under contract DE-AC05-00OR22725 with UT-Battelle, LLC. NR 21 TC 0 Z9 0 U1 4 U2 13 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0022-2720 EI 1365-2818 J9 J MICROSC-OXFORD JI J. Microsc.. PD NOV PY 2015 VL 260 IS 2 BP 163 EP 174 DI 10.1111/jmi.12279 PG 12 WC Microscopy SC Microscopy GA CU4UH UT WOS:000363525400006 PM 26243381 ER PT J AU Lu, FY Liu, ZY Zhang, SQ Liu, Y Jacob, R AF Lu, Feiyu Liu, Zhengyu Zhang, Shaoqing Liu, Yun Jacob, Robert TI Strongly Coupled Data Assimilation Using Leading Averaged Coupled Covariance (LACC). Part II: CGCM Experiments SO MONTHLY WEATHER REVIEW LA English DT Article DE Mathematical and statistical techniques; Kalman filters; Models and modeling; Coupled models; Data assimilation; Ensembles ID ENSEMBLE KALMAN FILTER; ATMOSPHERE-OCEAN DATA; CLIMATE MODEL; STATISTICAL ASSESSMENT; PARAMETER-ESTIMATION; DECADAL VARIABILITY; NORTH-ATLANTIC; SYSTEM; PERFORMANCE; HOLOCENE AB This paper uses a fully coupled general circulation model (CGCM) to study the leading averaged coupled covariance (LACC) method in a strongly coupled data assimilation (SCDA) system. The previous study in a simple coupled climate model has shown that, by calculating the coupled covariance using the leading averaged atmospheric states, the LACC method enhances the signal-to-noise ratio and improves the analysis quality of the slow model component compared to both the traditional weakly coupled data assimilation without cross-component adjustments (WCDA) and the regular SCDA using the simultaneous coupled covariance (SimCC).Here in Part II, the LACC method is tested with a CGCM in a perfect-model framework. By adding the observational adjustments from the low-level atmosphere temperature to the sea surface temperature (SST), the SCDA using LACC significantly reduces the SST error compared to WCDA over the globe; it also improves from the SCDA using SimCC, which performs better than the WCDA only in the deep tropics. The improvement in SST analysis is a result of the enhanced signal-to-noise ratio in the LACC method, especially in the extratropical regions. The improved SST analysis also benefits the subsurface ocean temperature and low-level atmosphere temperature analyses through dynamic and statistical processes. C1 [Lu, Feiyu; Liu, Zhengyu; Liu, Yun] Univ Wisconsin, Nelson Inst Ctr Climat Res, Madison, WI USA. [Lu, Feiyu; Liu, Zhengyu; Liu, Yun] Univ Wisconsin, Dept Atmospher & Ocean Sci, Madison, WI USA. [Liu, Zhengyu] Peking Univ, Lab Climate Ocean & Atmosphere Studies, Beijing 100871, Peoples R China. [Zhang, Shaoqing] NOAA, Geophys Fluid Dynam Lab, Princeton, NJ USA. [Jacob, Robert] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. RP Lu, FY (reprint author), Ctr Climat Res, 1225 W Dayton St, Madison, WI 53706 USA. EM flu7@wisc.edu OI Lu, Feiyu/0000-0001-6532-0740 FU NSF [AGS-0968383]; Chinese MOST [2012CB955200] FX We thank Drs. Shu Wu and Xinyao Rong for their work during the early development of our data assimilation code. This research is sponsored by NSF AGS-0968383 and Chinese MOST 2012CB955200. NR 39 TC 2 Z9 2 U1 1 U2 3 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0027-0644 EI 1520-0493 J9 MON WEATHER REV JI Mon. Weather Rev. PD NOV PY 2015 VL 143 IS 11 BP 4645 EP 4659 DI 10.1175/MWR-D-15-0088.1 PG 15 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA CU7DQ UT WOS:000363696800019 ER PT J AU Hunter, GJ Trinh, CH Bonetta, R Stewart, EE Cabelli, DE Hunter, T AF Hunter, Gary J. Trinh, Chi H. Bonetta, Rosalin Stewart, Emma E. Cabelli, Diane E. Hunter, Therese TI The structure of the Caenorhabditis elegans manganese superoxide dismutase MnSOD-3-azide complex SO PROTEIN SCIENCE LA English DT Article DE superoxide dismutase; conformational variation; MnSOD-3-azide complex; catalytic mechanism; product inhibition ID CRYSTAL-STRUCTURE; THERMUS-THERMOPHILUS; ESCHERICHIA-COLI; GENE-EXPRESSION; TYROSINE 34; LIFE-SPAN; EVOLUTIONARY CONSERVATION; FREE-RADICALS; LONGEVITY; RESOLUTION AB C. elegans MnSOD-3 has been implicated in the longevity pathway and its mechanism of catalysis is relevant to the aging process and carcinogenesis. The structures of MnSOD-3 provide unique crystallographic evidence of a dynamic region of the tetrameric interface (residues 41-54). We have determined the structure of the MnSOD-3-azide complex to 1.77-angstrom resolution. Analysis of this complex shows that the substrate analog, azide, binds end-on to the manganese center as a sixth ligand and that it ligates directly to a third and new solvent molecule also positioned within interacting distance to the His30 and Tyr34 residues of the substrate access funnel. This is the first structure of a eukaryotic MnSOD-azide complex that demonstrates the extended, uninterrupted hydrogen-bonded network that forms a proton relay incorporating three outer sphere solvent molecules, the substrate analog, the gateway residues, Gln142, and the solvent ligand. This configuration supports the formation and release of the hydrogen peroxide product in agreement with the 5-6-5 catalytic mechanism for MnSOD. The high product dissociation constant k(4) of MnSOD-3 reflects low product inhibition making this enzyme efficient even at high levels of superoxide. C1 [Hunter, Gary J.; Bonetta, Rosalin; Hunter, Therese] Univ Malta, Fac Med & Surg, Dept Physiol & Biochem, Msida, Malta. [Trinh, Chi H.; Stewart, Emma E.] Univ Leeds, Inst Mol & Cellular Biol, Astbury Ctr Struct Mol Biol, Leeds, W Yorkshire, England. [Cabelli, Diane E.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Hunter, T (reprint author), Univ Malta, Fac Med & Surg, Dept Physiol & Biochem, MSD 2080, Msida, Malta. EM therese.hunter@um.edu.mt FU University of Malta [PHBRP02]; Dean's Research Award [MDSIN08-19, MEDIN08-01]; US Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-AC02-98CH10886] FX Grant sponsor: University of Malta; Grant number: PHBRP02; Grant sponsor: Dean's Research Award; Grant numbers: MDSIN08-19, MEDIN08-01; Grant sponsor: US Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; Grant number: DE-AC02-98CH10886. NR 86 TC 2 Z9 2 U1 3 U2 9 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0961-8368 EI 1469-896X J9 PROTEIN SCI JI Protein Sci. PD NOV PY 2015 VL 24 IS 11 BP 1777 EP 1788 DI 10.1002/pro.2768 PG 12 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CU7NK UT WOS:000363727200008 PM 26257399 ER PT J AU Maniraj, M D'Souza, SW Rai, A Schlagel, DL Lograsso, TA Chakrabarti, A Barman, SR AF Maniraj, M. D'Souza, S. W. Rai, Abhishek Schlagel, D. L. Lograsso, T. A. Chakrabarti, Aparna Barman, S. R. TI Unoccupied electronic structure of Ni2MnGa ferromagnetic shape memory alloy SO SOLID STATE COMMUNICATIONS LA English DT Article DE Ferromagnetic shape memory alloy; Martensite transition; Inverse photoemission spectroscopy; Korriga-Kohn-Rostoker method ID NI-MN-SN; INVERSE-PHOTOEMISSION; PHASE-TRANSFORMATION; MARTENSITIC PHASE; SINGLE-CRYSTAL; NI2+XMN1-XGA; TRANSITIONS; SURFACE AB Momentum resolved inverse photoemission spectroscopy measurements show that the dispersion of the unoccupied bands of Ni(2)MaGa is significant in the austenite phase. In the martensite phase, it is markedly reduced, which is possibly related to the structural transition to an incommensurate modulated state in the martensite phase. Based on the first principle calculations of the electronic structure of Ni-Mn-Ga, we show that the modification of the spectral shape with surface composition is related to change in the hybridization between the Mn 3d and Ni 3d-like states that dominate the unoccupied conduction band. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Maniraj, M.; D'Souza, S. W.; Rai, Abhishek; Barman, S. R.] UGC DAE Consortium Sci Res, Indore 452001, Madhya Pradesh, India. [Schlagel, D. L.; Lograsso, T. A.] Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA. [Lograsso, T. A.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Chakrabarti, Aparna] Raja Ramanna Ctr Adv Technol, Indore 452013, Madhya Pradesh, India. RP Maniraj, M (reprint author), UGC DAE Consortium Sci Res, Khandwa Rd, Indore 452001, Madhya Pradesh, India. EM mr.maniraj@gmail.com RI Roy Barman, Sudipta/B-2026-2010 FU Department of Science and Technology Project [SP/S2/M-06/99]; Council of Scientific and Industrial Research, India; U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; DOE [DE-AC02-07CH11358] FX S. Singh and J. Nayak are thanked for useful discussions and support during the experiment. This work has been performed using the inverse photoemission spectroscopy workstation fabricated under the Department of Science and Technology Project SP/S2/M-06/99. M.M. and S.W.D. are thankful to Council of Scientific and Industrial Research, India for research fellowship. T.A.L. and D.L. acknowledge the support of the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. Ames Laboratory is operated for DOE by Iowa State University under Contract No. DE-AC02-07CH11358. NR 43 TC 0 Z9 0 U1 5 U2 23 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0038-1098 EI 1879-2766 J9 SOLID STATE COMMUN JI Solid State Commun. PD NOV PY 2015 VL 222 BP 1 EP 4 DI 10.1016/j.ssc.2015.08.003 PG 4 WC Physics, Condensed Matter SC Physics GA CU8UG UT WOS:000363819000001 ER PT J AU Cai, QX Wang, JG Wang, YG Mei, DH AF Cai, Qiu-Xia Wang, Jian-Guo Wang, Yang-Gang Mei, Donghai TI Mechanistic insights into the structure-dependent selectivity of catalytic furfural conversion on platinum catalysts SO AICHE JOURNAL LA English DT Article DE catalysis; biomass conversion; structure-dependent selectivity; density functional theory; microkinetic modeling ID TOTAL-ENERGY CALCULATIONS; FINDING SADDLE-POINTS; AUGMENTED-WAVE METHOD; STRUCTURE SENSITIVITY; PD NANOPARTICLES; PARTICLE-SIZE; REACTION PATHWAYS; BASIS-SET; BIO-OIL; HYDROGENATION AB The effects of surface structures on the selectivity of catalytic furfural conversion over platinum (Pt) catalysts in the presence of hydrogen have been studied using first principles density functional theory (DFT) calculations and microkinetic modeling. Three Pt model surface structures, that is, flat Pt(111), stepped Pt(211), and Pt-55 cluster are chosen to represent the terrace, step, and corner sites of Pt nanoparticle. DFT results show that the dominant reaction route (hydrogenation or decarbonylation) in furfural conversion depends strongly on the structures (or reactive sites). Using the size-dependent site distribution rule, our microkinetic modeling results indicate the decarbonylation route prevails over smaller Pt particles less than 1.4 nm while the hydrogenation is the dominant reaction route over larger Pt catalyst particles at T=473 K and PH2=93 kPa. This is in good agreement with the reported experimental observations. (c) 2015 American Institute of Chemical Engineers C1 [Cai, Qiu-Xia; Wang, Jian-Guo] Zhejiang Univ Technol, Coll Chem Engn, Hangzhou 310014, Zhejiang, Peoples R China. [Wang, Yang-Gang; Mei, Donghai] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. [Wang, Yang-Gang; Mei, Donghai] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. RP Wang, JG (reprint author), Zhejiang Univ Technol, Coll Chem Engn, Hangzhou 310014, Zhejiang, Peoples R China. EM jgw@zjut.edu.cn; donghai.mei@pnnl.gov RI Mei, Donghai/D-3251-2011; Mei, Donghai/A-2115-2012 OI Mei, Donghai/0000-0002-0286-4182 FU National Basic Research Program of China (973 Program) [2013CB733501]; National Natural Science Foundation of China [NSFC-21306169, 21176221, 21136001, 21101137, 91334103]; US Department of Energy (DOE), the Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences; DOE's Office of Biological and Environmental Research FX This work was supported by National Basic Research Program of China (973 Program) (2013CB733501) and the National Natural Science Foundation of China (NSFC-21306169, 21176221, 21136001, 21101137, and 91334103). This work was also partially supported by the US Department of Energy (DOE), the Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. Pacific Northwest National Laboratory (PNNL) is a multiprogram national laboratory operated for DOE by Battelle. Computing time was granted by the grand challenge of computational catalysis of the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL). EMSL is a national scientific user facility located at Pacific Northwest National Laboratory (PNNL) and sponsored by DOE's Office of Biological and Environmental Research. NR 44 TC 2 Z9 2 U1 21 U2 84 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0001-1541 EI 1547-5905 J9 AICHE J JI AICHE J. PD NOV PY 2015 VL 61 IS 11 BP 3812 EP 3824 DI 10.1002/aic.14902 PG 13 WC Engineering, Chemical SC Engineering GA CT6YN UT WOS:000362959700021 ER PT J AU Steven, B Kuske, CR Gallegos-Graves, LV Reed, SC Belnap, J AF Steven, Blaire Kuske, Cheryl R. Gallegos-Graves, La Verne Reed, Sasha C. Belnap, Jayne TI Climate Change and Physical Disturbance Manipulations Result in Distinct Biological Soil Crust Communities SO APPLIED AND ENVIRONMENTAL MICROBIOLOGY LA English DT Article ID 16S RIBOSOMAL-RNA; COLORADO PLATEAU; MICROBIAL COMMUNITIES; NITROGEN-FIXATION; ELEVATED CO2; DESERT; CYANOBACTERIA; RAINFALL; PRECIPITATION; ECOSYSTEM AB Biological soil crusts (biocrusts) colonize plant interspaces in many drylands and are critical to soil nutrient cycling. Multiple climate change and land use factors have been shown to detrimentally impact biocrusts on a macroscopic (i.e., visual) scale. However, the impact of these perturbations on the bacterial components of the biocrusts remains poorly understood. We employed multiple long-term field experiments to assess the impacts of chronic physical (foot trampling) and climatic changes (2 degrees C soil warming, altered summer precipitation [wetting], and combined warming and wetting) on biocrust bacterial biomass, composition, and metabolic profile. The biocrust bacterial communities adopted distinct states based on the mechanism of disturbance. Chronic trampling decreased biomass and caused small community compositional changes. Soil warming had little effect on biocrust biomass or composition, while wetting resulted in an increase in the cyanobacterial biomass and altered bacterial composition. Warming combined with wetting dramatically altered bacterial composition and decreased Cyanobacteria abundance. Shotgun metagenomic sequencing identified four functional gene categories that differed in relative abundance among the manipulations, suggesting that climate and land use changes affected soil bacterial functional potential. This study illustrates that different types of biocrust disturbance damage biocrusts in macroscopically similar ways, but they differentially impact the resident soil bacterial communities, and the communities' functional profiles can differ depending on the disturbance type. Therefore, the nature of the perturbation and the microbial response are important considerations for management and restoration of drylands. C1 [Steven, Blaire; Kuske, Cheryl R.; Gallegos-Graves, La Verne] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA. [Reed, Sasha C.; Belnap, Jayne] US Geol Survey, Southwest Biol Sci Ctr, Moab, UT USA. RP Kuske, CR (reprint author), Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA. EM kuske@lanl.gov FU U.S. Department of Energy, Office of Science, Biological and Environmental Research, through a Science Focus Area grant; USGS FX This study was supported by the U.S. Department of Energy, Office of Science, Biological and Environmental Research, through a Science Focus Area grant to C.R.K. DNA sequencing was provided by the Los Alamos National Laboratory through their Laboratory Directed Research and Development program. Field experiments were initiated and maintained through U.S. DOE Terrestrial Ecosystem Science grants to J.B. and S.C.R. and the National Park Service. J.B. thanks the USGS Climate and Land Use and Ecosystem programs for support. NR 54 TC 2 Z9 2 U1 10 U2 61 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0099-2240 EI 1098-5336 J9 APPL ENVIRON MICROB JI Appl. Environ. Microbiol. PD NOV PY 2015 VL 81 IS 21 BP 7448 EP 7459 DI 10.1128/AEM.01443-15 PG 12 WC Biotechnology & Applied Microbiology; Microbiology SC Biotechnology & Applied Microbiology; Microbiology GA CU3YP UT WOS:000363462900012 PM 26276111 ER PT J AU Wang, H Li, HY Gilbert, JA Li, HB Wu, LH Liu, M Wang, LL Zhou, QS Yuan, JX Zhang, ZJ AF Wang, Hang Li, Hongyi Gilbert, Jack A. Li, Haibo Wu, Longhua Liu, Meng Wang, Liling Zhou, Qiansheng Yuan, Junxiang Zhang, Zhijian TI Housefly Larva Vermicomposting Efficiently Attenuates Antibiotic Resistance Genes in Swine Manure, with Concomitant Bacterial Population Changes SO APPLIED AND ENVIRONMENTAL MICROBIOLOGY LA English DT Article ID ESCHERICHIA-COLI STRAINS; MUNICIPAL WASTE-WATER; TETRACYCLINE RESISTANCE; SULFONAMIDE RESISTANCE; TREATMENT SYSTEMS; EASTERN CHINA; FLY DIPTERA; ANTIMICROBIALS; DIVERSITY; SOILS AB Manure from swine treated with antimicrobials as feed additives is a major source for the expansion of the antibiotic resistance gene (ARG) reservoir in the environment. Vermicomposting via housefly larvae (Musca domestica) can be efficiently used to treat manure and regenerate biofertilizer, but few studies have investigated its effect on ARG attenuation. Here, we tracked the abundances of 9 ARGs and the composition and structure of the bacterial communities in manure samples across 6 days of full-scale manure vermicomposting. On day 6, the abundances of genes encoding tetracycline resistance [tet(M), tet(O), tet(Q), and tet(W)] were reduced (P < 0.05), while those of genes encoding sulfonamide resistance (sul1 and sul2) were increased (P < 0.05) when normalized to 16S rRNA. The abundances of tetracycline resistance genes were correlated (P < 0.05) with the changing concentrations of tetracyclines in the manure. The overall diversity and richness of the bacteria significantly decreased during vermicomposting, accompanied by a 100 times increase in the relative abundance of Flavobacteriaceae spp. Variations in the abundances of ARGs were correlated with the changing microbial community structure and the relative abundances of the family Ruminococcaceae, class Bacilli, or phylum Proteobacteria. Vermicomposting, as a waste management practice, can reduce the overall abundance of ARGs. More research is warranted to assess the use of this waste management practice as a measure to attenuate the dissemination of antimicrobial residues and ARGs from livestock production before vermicompost can be safely used as biofertilizer in agroecosystems. C1 [Wang, Hang; Li, Hongyi; Gilbert, Jack A.; Liu, Meng; Zhou, Qiansheng; Yuan, Junxiang; Zhang, Zhijian] Zhejiang Univ, Coll Environm & Resource Sci, Hangzhou 310003, Zhejiang, Peoples R China. [Wang, Hang] Southwest Forestry Univ, Natl Plateau Wetlands Res Ctr, Kunming, Peoples R China. [Gilbert, Jack A.] Argonne Natl Lab, Inst Genom & Syst Biol, Lemont, IL USA. [Gilbert, Jack A.] Univ Chicago, Dept Ecol & Evolut, Chicago, IL 60637 USA. [Li, Haibo; Wang, Liling] Zhejiang Forestry Acad, Inst Ecol, Hangzhou, Zhejiang, Peoples R China. [Wu, Longhua] Chinese Acad Sci, Inst Soil Sci, Nanjing, Jiangsu, Peoples R China. [Zhou, Qiansheng] Tongxiang First High Sch, Tongxiang, Peoples R China. [Zhang, Zhijian] Zhejiang Univ, China Acad West Reg Dev, Hangzhou 310003, Zhejiang, Peoples R China. RP Zhang, ZJ (reprint author), Zhejiang Univ, Coll Environm & Resource Sci, Hangzhou 310003, Zhejiang, Peoples R China. EM zhangzhijian@zju.edu.cn FU National Natural Science Foundation of China [41373074]; National Ministry of Science and Technology [2013GB23600658]; Zhejiang Science and Technology Innovation Program [2013C33001]; U.S. Department of Energy [DE-AC02-06CH11357] FX This work was supported by the National Natural Science Foundation of China (grant 41373074), the National Ministry of Science and Technology (grant 2013GB23600658), and the Zhejiang Science and Technology Innovation Program (grant 2013C33001) and in part by the U.S. Department of Energy under contract DE-AC02-06CH11357. NR 56 TC 1 Z9 1 U1 11 U2 49 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0099-2240 EI 1098-5336 J9 APPL ENVIRON MICROB JI Appl. Environ. Microbiol. PD NOV PY 2015 VL 81 IS 22 BP 7668 EP 7679 DI 10.1128/AEM.01367-15 PG 12 WC Biotechnology & Applied Microbiology; Microbiology SC Biotechnology & Applied Microbiology; Microbiology GA CU3YY UT WOS:000363463800001 PM 26296728 ER PT J AU Anderson, TD Miller, JI Fierobe, HP Clubb, RT AF Anderson, Timothy D. Miller, J. Izaak Fierobe, Henri-Pierre Clubb, Robert T. TI Recombinant Bacillus subtilis That Grows on Untreated Plant Biomass (Retraction of vol 79, pg 867, 2013) SO APPLIED AND ENVIRONMENTAL MICROBIOLOGY LA English DT Correction C1 [Anderson, Timothy D.; Miller, J. Izaak; Clubb, Robert T.] Univ Calif Los Angeles, UCLA DOE Inst Genom & Prote, Los Angeles, CA 90095 USA. [Anderson, Timothy D.; Miller, J. Izaak; Clubb, Robert T.] Univ Calif Los Angeles, Inst Mol Biol, Los Angeles, CA 90024 USA. [Anderson, Timothy D.; Miller, J. Izaak; Clubb, Robert T.] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90024 USA. [Fierobe, Henri-Pierre] IFR88 CNRS, Lab Chim Bacterienne, Marseille, France. RP Anderson, TD (reprint author), Univ Calif Los Angeles, UCLA DOE Inst Genom & Prote, Los Angeles, CA 90095 USA. NR 1 TC 0 Z9 0 U1 2 U2 3 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0099-2240 EI 1098-5336 J9 APPL ENVIRON MICROB JI Appl. Environ. Microbiol. PD NOV PY 2015 VL 81 IS 22 BP 7957 EP 7957 DI 10.1128/AEM.02768-15 PG 1 WC Biotechnology & Applied Microbiology; Microbiology SC Biotechnology & Applied Microbiology; Microbiology GA CU3YY UT WOS:000363463800029 ER PT J AU Mathon, BR Schoonen, MA Riccardi, AL Borda, MJ AF Mathon, B. R. Schoonen, M. A. Riccardi, A. L. Borda, M. J. TI Measuring flow rates and characterizing flow regimes in hot springs SO APPLIED GEOCHEMISTRY LA English DT Article ID LASSEN HYDROTHERMAL SYSTEM; CALCIUM-SULFATE DIHYDRATE; MASS-TRANSFER; DISSOLUTION RATES; NATIONAL-PARK; WATER; GYPSUM; KINETICS; CALIFORNIA; SMOOTH AB Detailed studies were conducted at Big Boiler hot spring in Lassen Volcanic National Park, CA, and Ojo Caliente hot spring in Yellowstone National Park, WY, to measure the flow rate and characterize the flow regime of hot spring drainages. These drainages represent some of the most dynamic interfaces between the hydrosphere and atmosphere with steep temperature gradients and chemical gradients. The rate of thermal disequilibrium and chemical disequilibrium dissipation depends on the flow rate and flow regime. The drainage of each hot spring was divided into ten or more segments and water samples were collected at segment boundaries. Fluid flow velocity throughout the drainage was measured using an in situ flow probe where possible and by determining the advancement of a red food dye tracer through the flow channel. A combination of field and laboratory studies was used to adapt a method based on the transport-controlled dissolution rate of gypsum to characterize the flow regime throughout the drainages. Laboratory experiments as a well as a deployment in an artificial drainage were conducted to validate the application of this method for hot spring environments. The deployment of the gypsum tablets was complemented by using digital videography to record the nature of the flow regime throughout the drainages. In situ flow probe measurements were not possible at all locations. The data obtained with the probe showed a range of values that was in reasonable agreement with the flow rates obtained using the dye tracer. The average flow rate based on advancement of dye tracer determined at Big Boiler was 0.22 m/s in both 2000 and 2001, while in Ojo Caliente flow rate varied from 0.39 m/s in 2001 to 0.45 m/s in 2002. The results of the gypsum dissolution measurement in the field yield boundary layer thicknesses between 8 and 38 mu m, with most values between 15 and 25 mu m, indicating well-developed turbulent flow throughout the drainages. The results, consistent with videography, indicate that gypsum dissolution rates based on the deployment of well-characterized and pure gypsum tablets can be used in hot-spring environments. An analysis of cooling rates within the drainages illustrates the importance of turbulent flow in cooling the waters. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Mathon, B. R.; Schoonen, M. A.; Riccardi, A. L.; Borda, M. J.] SUNY Stony Brook, Dept Geosci, Stony Brook, NY 11794 USA. RP Schoonen, MA (reprint author), Brookhaven Natl Lab, Biol Environm & Climate Sci, Upton, NY 11973 USA. EM martin.schoonen@stonybrook.edu FU NSF-EAR FX This work was supported by awards by NSF-EAR to M. Schoonen. The work benefited from the introduction to YNP and LVNP by Dr. Kirk Nordstrom, USGS, Boulder, CO, with whom Schoonen conducted joint research for several years. This paper benefited from two thorough reviews by anonymous reviewers. NR 39 TC 0 Z9 0 U1 2 U2 9 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0883-2927 J9 APPL GEOCHEM JI Appl. Geochem. PD NOV PY 2015 VL 62 SI SI BP 234 EP 246 DI 10.1016/j.apgeochem.2015.04.007 PG 13 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CU3ZM UT WOS:000363465600019 ER PT J AU Wang, H Liu, L Lu, Y Pan, P Hooker, JM Fowler, JS Tonge, PJ AF Wang, Hui Liu, Li Lu, Yang Pan, Pan Hooker, Jacob M. Fowler, Joanna S. Tonge, Peter J. TI Radiolabelling and positron emission tomography of PT70, a time-dependent inhibitor of InhA, the Mycobacterium tuberculosis enoyl-ACP reductase SO BIOORGANIC & MEDICINAL CHEMISTRY LETTERS LA English DT Article DE Positron emission tomography; InhA enoyl-ACP reductase; Residence time; Carbon-11; PK-PD ID CARRIER PROTEIN REDUCTASE; CATALASE-PEROXIDASE GENE; TIGHT-BINDING INHIBITOR; SLOW-ONSET INHIBITION; DRUG-RESISTANCE; ISONIAZID-RESISTANT; RESIDENCE TIME; TRICLOSAN; KINETICS; STRAINS AB PT70 is a diaryl ether inhibitor of InhA, the enoyl-ACP reductase in the Mycobacterium tuberculosis fatty acid biosynthesis pathway. It has a residence time of 24 min on the target, and also shows antibacterial activity in a mouse model of tuberculosis infection. Due to the interest in studying target tissue pharmacokinetics of PT70, we developed a method to radiolabel PT70 with carbon-11 and have studied its pharmacokinetics in mice and baboons using positron emission tomography. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Wang, Hui; Liu, Li; Lu, Yang; Pan, Pan; Tonge, Peter J.] SUNY Stony Brook, Inst Chem Biol & Drug Discovery, Dept Chem, Stony Brook, NY 11794 USA. [Hooker, Jacob M.; Fowler, Joanna S.] Brookhaven Natl Lab, Biol Environm & Climate Sci Dept, Upton, NY 11973 USA. RP Tonge, PJ (reprint author), SUNY Stony Brook, Inst Chem Biol & Drug Discovery, Dept Chem, Stony Brook, NY 11794 USA. EM peter.tonge@stonybrook.edu OI Lu, Yang/0000-0003-2717-9656 FU National Institutes of Health [GM102864] FX This study was supported by the National Institutes of Health Grant GM102864 to P.J.T. NR 43 TC 1 Z9 1 U1 2 U2 8 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0960-894X EI 1464-3405 J9 BIOORG MED CHEM LETT JI Bioorg. Med. Chem. Lett. PD NOV 1 PY 2015 VL 25 IS 21 BP 4782 EP 4786 DI 10.1016/j.bmcl.2015.07.019 PG 5 WC Chemistry, Medicinal; Chemistry, Organic SC Pharmacology & Pharmacy; Chemistry GA CU1IV UT WOS:000363275400016 PM 26227776 ER PT J AU Birkmann, J Cutter, SL Rothman, DS Welle, T Garschagen, M van Ruijven, B O'Neill, B Preston, BL Kienberger, S Cardona, OD Siagian, T Hidayati, D Setiadi, N Binder, CR Hughes, B Pulwarty, R AF Birkmann, Joern Cutter, Susan L. Rothman, Dale S. Welle, Torsten Garschagen, Matthias van Ruijven, Bas O'Neill, Brian Preston, Benjamin L. Kienberger, Stefan Cardona, Omar D. Siagian, Tiodora Hidayati, Deny Setiadi, Neysa Binder, Claudia R. Hughes, Barry Pulwarty, Roger TI Scenarios for vulnerability: opportunities and constraints in the context of climate change and disaster risk SO CLIMATIC CHANGE LA English DT Article ID ADAPTATION AB Most scientific assessments for climate change adaptation and risk reduction are based on scenarios for climatic change. Scenarios for socio-economic development, particularly in terms of vulnerability and adaptive capacity, are largely lacking. This paper focuses on the utility of socio-economic scenarios for vulnerability, risk and adaptation research. The paper introduces the goals and functions of scenarios in general and reflects on the current global debate around shared socio-economic pathways (SSPs). It examines the options and constraints of scenario methods for risk and vulnerability assessments in the context of climate change and natural hazards. Two case studies are used to contrast the opportunities and current constraints in scenario methods at different scales: the global WorldRiskIndex, based on quantitative data and indicators; and a local participatory scenario development process in Jakarta, showing a qualitative approach. The juxtaposition of a quantitative approach with global data and a qualitative-participatory local approach provides new insights on how different methods and scenario techniques can be applied in vulnerability and risk research. C1 [Birkmann, Joern; Welle, Torsten; Garschagen, Matthias; Setiadi, Neysa] United Nations Univ, Inst Environm & Human Secur, Bonn, Germany. [Cutter, Susan L.] Univ S Carolina, Hazards & Vulnerabil Res Inst, Columbia, SC 29208 USA. [Rothman, Dale S.; Hughes, Barry] Univ Denver, Pardee Ctr Int Futures, Denver, CO USA. [van Ruijven, Bas; O'Neill, Brian] Natl Ctr Atmospher Res, Boulder, CO 80307 USA. [Preston, Benjamin L.] Oak Ridge Natl Lab, Climate Change Sci Inst, Oak Ridge, TN USA. [Kienberger, Stefan] Salzburg Univ, Interfac Dept Geoinformat Z GIS, A-5020 Salzburg, Austria. [Cardona, Omar D.] Univ Nacl Colombia, Inst Estudios Ambientales IDEA, Manizales, Colombia. [Siagian, Tiodora] Govt Indonesia, Stat Indonesia BPS, Jakarta, Indonesia. [Hidayati, Deny] Indonesian Inst Sci LIPI, Jakarta, Indonesia. [Binder, Claudia R.] Univ Munich LMU, Dept Geog, Munich, Germany. [Pulwarty, Roger] NOAA, Earth Syst Res Lab, Boulder, CO USA. RP Birkmann, J (reprint author), United Nations Univ, Inst Environm & Human Secur, Bonn, Germany. EM birkmann@ehs.unu.edu; stefan.kienberger@sbg.ac.at RI O'Neill, Brian/E-6531-2013; Toro, Johan/P-9939-2016; OI Cutter, Susan/0000-0002-7005-8596 NR 35 TC 10 Z9 10 U1 9 U2 34 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0165-0009 EI 1573-1480 J9 CLIMATIC CHANGE JI Clim. Change PD NOV PY 2015 VL 133 IS 1 BP 53 EP 68 DI 10.1007/s10584-013-0913-2 PG 16 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA CU4FW UT WOS:000363483600005 ER PT J AU Ahlstrom, M Ela, E Riesz, J O'Sullivan, J Hobbs, BF O'Malley, M Milligan, M Sotkiewicz, P Caldwell, J AF Ahlstrom, Mark Ela, Erik Riesz, Jenny O'Sullivan, Jonathan Hobbs, Benjamin F. O'Malley, Mark Milligan, Michael Sotkiewicz, Paul Caldwell, Jim TI The Evolution of the Market Designing a Market for High Levels of Variable Generation SO IEEE POWER & ENERGY MAGAZINE LA English DT Article C1 [Ahlstrom, Mark] WindLogics, St Paul, MN 55108 USA. [Ela, Erik] Elect Power Res Inst, Boulder, CO USA. [Riesz, Jenny] Ctr Energy & Environm Markets, Sydney, NSW, Australia. [O'Sullivan, Jonathan] EirGrid Grp, Dublin, Ireland. [Hobbs, Benjamin F.] Johns Hopkins Univ, Baltimore, MD USA. [O'Malley, Mark] Univ Coll Dublin, Dublin, Ireland. [Milligan, Michael] Natl Renewable Energy Lab, Golden, CO USA. [Sotkiewicz, Paul] PJM Interconnect LLC, Audubon, PA USA. [Caldwell, Jim] Low Carbon Grid Study, Sonoma, CA USA. RP Ahlstrom, M (reprint author), WindLogics, St Paul, MN 55108 USA. NR 5 TC 0 Z9 1 U1 0 U2 1 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1540-7977 EI 1558-4216 J9 IEEE POWER ENERGY M JI IEEE Power Energy Mag. PD NOV-DEC PY 2015 VL 13 IS 6 BP 60 EP 66 DI 10.1109/MPE.2015.2458755 PG 7 WC Engineering, Electrical & Electronic SC Engineering GA CT9PJ UT WOS:000363148800006 ER PT J AU Milligan, M Frew, B Kirby, B Schuerger, M Clark, K Lew, D Denholm, P Zavadil, B O'Malley, M Tsuchida, B AF Milligan, Michael Frew, Bethany Kirby, Brendan Schuerger, Matt Clark, Kara Lew, Debbie Denholm, Paul Zavadil, Bob O'Malley, Mark Tsuchida, Bruce TI Alternatives No More Wind and Solar Power Are Mainstays of a Clean, Reliable, Affordable Grid SO IEEE POWER & ENERGY MAGAZINE LA English DT Article C1 [Milligan, Michael; Frew, Bethany; Clark, Kara; Denholm, Paul] NREL, Golden, CO 80401 USA. [Kirby, Brendan] Consult Kirby, Palm City, FL USA. [Schuerger, Matt] Energy Syst Consulting Serv, Minneapolis, MN USA. [Lew, Debbie] GE Energy Consulting, Golden, CO USA. [Zavadil, Bob] EnerNex, Knoxville, TN USA. [O'Malley, Mark] Univ Coll Dublin, Dublin, Ireland. [Tsuchida, Bruce] Brattle Grp, Boston, MA USA. RP Milligan, M (reprint author), NREL, Golden, CO 80401 USA. NR 4 TC 4 Z9 4 U1 2 U2 8 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1540-7977 EI 1558-4216 J9 IEEE POWER ENERGY M JI IEEE Power Energy Mag. PD NOV-DEC PY 2015 VL 13 IS 6 BP 78 EP 87 DI 10.1109/MPE.2015.2462311 PG 10 WC Engineering, Electrical & Electronic SC Engineering GA CT9PJ UT WOS:000363148800008 ER PT J AU Barnett, B Trexler, M Champagne, V AF Barnett, Blake Trexler, Matthew Champagne, Victor TI Cold sprayed refractory metals for chrome reduction in gun barrel liners SO INTERNATIONAL JOURNAL OF REFRACTORY METALS & HARD MATERIALS LA English DT Article DE Tungsten; Alloys & composites; Spray coating; Thermal spray coating AB Modern gun barrel technology faces a number of challenges related to the use of chrome-plated steel at the interior bore surface. The amount of allowable chrome has been significantly reduced due to environmental, health, and safety concerns. Furthermore, current munitions and propellants lead to erosion and condemnation of gun barrels well before their 10,000 round expected lifetime. This has precipitated a search for longer-lasting bore liners, such as refractory metals deposited by explosive bonding. The cost and difficulty associated with shaping these materials have made them impractical choices to date. Gas Dynamic Cold Spray consolidation of refractory metals and alloys was selected as an alternative to extrusion for additive manufacture of donor tubes. Tantalum-10 tungsten alloy donor tubes have been produced by cold spray and tested for compatibility with the cladding process. A 1-meter (3-foot) long tube was produced to test scalability. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Barnett, Blake] US Army Res Lab, Oak Ridge Inst Sci & Educ, Aberdeen Proving Ground, MD 21005 USA. [Trexler, Matthew; Champagne, Victor] US Army Res Lab, Ctr Cold Spray, Aberdeen Proving Ground, MD 21005 USA. RP Barnett, B (reprint author), US Army Res Lab, Oak Ridge Inst Sci & Educ, 4600 Deer Creek Loop, Aberdeen Proving Ground, MD 21005 USA. EM blake.d.barnett.ctr@mail.mil NR 12 TC 0 Z9 0 U1 6 U2 15 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0263-4368 J9 INT J REFRACT MET H JI Int. J. Refract. Met. Hard Mat. PD NOV PY 2015 VL 53 SI SI BP 139 EP 143 DI 10.1016/j.ijrmhm.2015.07.007 PN B PG 5 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA CT8QO UT WOS:000363081300013 ER PT J AU Moore, JAM Jiang, J Patterson, CM Mayes, MA Wang, GS Classen, AT AF Moore, Jessica A. M. Jiang, Jiang Patterson, Courtney M. Mayes, Melanie A. Wang, Gangsheng Classen, Aimee T. TI Interactions among roots, mycorrhizas and free-living microbial communities differentially impact soil carbon processes SO JOURNAL OF ECOLOGY LA English DT Article DE decomposition; extracellular enzyme activity; forest; nutrient cycling; plant-microbe interactions; plant-soil (below-ground) interactions; rhizosphere; simulation model; stable isotope ID ORGANIC-MATTER; TERRESTRIAL ECOSYSTEMS; ECTOMYCORRHIZAL FUNGI; BOREAL FOREST; ELEVATED CO2; BACTERIAL; NITROGEN; BIOMASS; SEQUESTRATION; DECOMPOSITION AB Plant roots, their associated microbial community and free-living soil microbes interact to regulate the movement of carbon from the soil to the atmosphere, one of the most important and least understood fluxes of terrestrial carbon. Our inadequate understanding of how plant-microbial interactions alter soil carbon decomposition may lead to poor model predictions of terrestrial carbon feedbacks to the atmosphere. Roots, mycorrhizal fungi and free-living soil microbes can alter soil carbon decomposition through exudation of carbon into soil. Exudates of simple carbon compounds can increase microbial activity because microbes are typically carbon limited. When both roots and mycorrhizal fungi are present in the soil, they may additively increase carbon decomposition. However, when mycorrhizas are isolated from roots, they may limit soil carbon decomposition by competing with free-living decomposers for resources. We manipulated the access of roots and mycorrhizal fungi to soil insitu in a temperate mixed deciduous forest. We added C-13-labelled substrate to trace metabolized carbon in respiration and measured carbon-degrading microbial extracellular enzyme activity and soil carbon pools. We used our data in a mechanistic soil carbon decomposition model to simulate and compare the effects of root and mycorrhizal fungal presence on soil carbon dynamics over longer time periods. Contrary to what we predicted, root and mycorrhizal biomass did not interact to additively increase microbial activity and soil carbon degradation. The metabolism of C-13-labelled starch was highest when root biomass was high and mycorrhizal biomass was low. These results suggest that mycorrhizas may negatively interact with the free-living microbial community to influence soil carbon dynamics, a hypothesis supported by our enzyme results. Our steady-state model simulations suggested that root presence increased mineral-associated and particulate organic carbon pools, while mycorrhizal fungal presence had a greater influence on particulate than mineral-associated organic carbon pools.Synthesis. Our results suggest that the activity of enzymes involved in organic matter decomposition was contingent upon root-mycorrhizal-microbial interactions. Using our experimental data in a decomposition simulation model, we show that root-mycorrhizal-microbial interactions may have longer-term legacy effects on soil carbon sequestration. Overall, our study suggests that roots stimulate microbial activity in the short term, but contribute to soil carbon storage over longer periods of time. C1 [Moore, Jessica A. M.; Jiang, Jiang; Patterson, Courtney M.; Classen, Aimee T.] Univ Tennessee, Ecol & Evolutionary Biol, Knoxville, TN 37996 USA. [Mayes, Melanie A.; Wang, Gangsheng] Oak Ridge Natl Lab, Climate Change Sci Inst, Oak Ridge, TN 37831 USA. [Mayes, Melanie A.; Wang, Gangsheng] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Classen, Aimee T.] Univ Copenhagen, Nat Hist Museum Denmark, DK-2100 Copenhagen O, Denmark. RP Moore, JAM (reprint author), Univ Tennessee, Ecol & Evolutionary Biol, 569 Dabney Hall,1416 Circle Dr, Knoxville, TN 37996 USA. EM jbryan44@utk.edu RI Jiang, Jiang/H-1080-2012; publist, CMEC/C-3010-2012; Classen, Aimee/C-4035-2008; publicationpage, cmec/B-4405-2017 OI Jiang, Jiang/0000-0001-5058-8664; Classen, Aimee/0000-0002-6741-3470; FU U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, Terrestrial Ecosystem Sciences Program [DE-SC0010562]; University of Tennessee Science Alliance Joint Directed Research and Development grant; Ecology and Evolutionary Biology Department at University of Tennessee FX This work was supported by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, Terrestrial Ecosystem Sciences Program under Award Number DE-SC0010562. A University of Tennessee Science Alliance Joint Directed Research and Development grant to ATC, a Graduate Research grant to JAMM from the Ecology and Evolutionary Biology Department at University of Tennessee contributed to this work. We thank Sneha Patel for assistance with sample collection and analysis, Greg Newman for help with data processing, Aaron Ellison and Nathan Sanders for assistance with statistical analyses, Marisol Sanchez-Garcia and the Matheny Lab at University of Tennessee for assistance with PCR and mycorrhizal sequencing and the University of Tennessee and University of Copenhagen Ecosystem Ecology laboratory groups for comments on the manuscript. The authors declare no conflict of interest. NR 77 TC 5 Z9 6 U1 40 U2 209 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0022-0477 EI 1365-2745 J9 J ECOL JI J. Ecol. PD NOV PY 2015 VL 103 IS 6 BP 1442 EP 1453 DI 10.1111/1365-2745.12484 PG 12 WC Plant Sciences; Ecology SC Plant Sciences; Environmental Sciences & Ecology GA CU2FO UT WOS:000363339300008 ER PT J AU He, ZC Liu, F Wang, C Chen, JH He, LL Nordlund, D Wu, HB Russell, TP Cao, Y AF He, Zhicai Liu, Feng Wang, Cheng Chen, Jihua He, Lilin Nordlund, Dennis Wu, Hongbin Russell, Thomas P. Cao, Yong TI Simultaneous spin-coating and solvent annealing: manipulating the active layer morphology to a power conversion efficiency of 9.6% in polymer solar cells SO MATERIALS HORIZONS LA English DT Article ID SMALL-ANGLE; PHASE AB We developed a simultaneous spin-coating/solvent-annealing process and demonstrated morphology optimization for PTB7 based organic photovoltaics. This novel processing method enhances the edge-on crystalline content in thin films and induces the formation of weak PCBM aggregates. As a result, the efficiency of polymer solar cells increased from 9.2% to a certified high efficiency of 9.61%, owing to an enhanced short-circuit current (J(sc), 18.4 mA cm(-2) vs. 17. 5 mA cm(-2)) and an improved fill factor. C1 [He, Zhicai; Wu, Hongbin; Cao, Yong] S China Univ Technol, Inst Polymer Optoelect Mat & Devices, State Key Lab Luminescent Mat & Devices, Guangzhou 510640, Guangdong, Peoples R China. [Liu, Feng; Russell, Thomas P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Liu, Feng; Russell, Thomas P.] Univ Massachusetts, Dept Polymer Sci & Engn, Amherst, MA 01003 USA. [Wang, Cheng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Chen, Jihua] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [He, Lilin] Oak Ridge Natl Lab, Biol & Soft Matter Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. [Nordlund, Dennis] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Russell, Thomas P.] Tohoku Univ, WPI Adv Inst Mat Res, Aoba Ku, Sendai, Miyagi 9808577, Japan. RP Wu, HB (reprint author), S China Univ Technol, Inst Polymer Optoelect Mat & Devices, State Key Lab Luminescent Mat & Devices, Guangzhou 510640, Guangdong, Peoples R China. EM iamfengliu@gmail.com; hbwu@scut.edu.cn; russell@mail.pse.umass.edu RI Foundry, Molecular/G-9968-2014; Nordlund, Dennis/A-8902-2008; Chen, Jihua/F-1417-2011; Wang, Cheng/A-9815-2014; Liu, Feng/J-4361-2014; OI Nordlund, Dennis/0000-0001-9524-6908; Chen, Jihua/0000-0001-6879-5936; Liu, Feng/0000-0002-5572-8512; He, Lilin/0000-0002-9560-8101 FU National Natural Science Foundation of China [91333206, 51403066, 51225301, 61177022, 5141101251]; Fundamental Research Funds for the Central Universities [2014ZM001]; Innovation Program of Guangdong Province Universities and Colleges [2012KJCX0009]; Polymer-Based Materials for Harvesting Solar Energy (PHaSE), an Energy Frontier Research Centre - US Department of Energy, Office of Basic Energy Sciences [DE-SC0001087]; DOE, Office of Science, and Office of Basic Energy Sciences; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]; Division of Scientific User Facilities, Office of Basic Energy Sciences, US Department of Energy; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy FX H.W. and Z.H. acknowledge financial support from the National Natural Science Foundation of China (no. 91333206, 51403066, 51225301, 61177022 and 5141101251), Fundamental Research Funds for the Central Universities (2014ZM001) and Innovation Program of Guangdong Province Universities and Colleges (2012KJCX0009), and thank M. Yun and X. Wang of CPVT for device performance verification. F.L. and T.P.R. were supported by Polymer-Based Materials for Harvesting Solar Energy (PHaSE), an Energy Frontier Research Centre funded by the US Department of Energy, Office of Basic Energy Sciences under award number DE-SC0001087. Portions of this research were carried out at beamline 7.3.3 and 11.0.1.2 at the Advanced Light Source, and Molecular Foundry, Lawrence Berkeley National Laboratory, which was supported by the DOE, Office of Science, and Office of Basic Energy Sciences. Use of the Stanford Synchrotron Radiation Light source, SLAC National Accelerator Laboratory, was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515. Energy filtered TEM was conducted at the Center for Nanophase Materials Sciences, which was sponsored at Oak Ridge National Laboratory by the Division of Scientific User Facilities, Office of Basic Energy Sciences, US Department of Energy. Research conducted at ORNL's High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. NR 28 TC 7 Z9 7 U1 9 U2 56 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2051-6347 EI 2051-6355 J9 MATER HORIZ JI Mater. Horizons PD NOV PY 2015 VL 2 IS 6 BP 592 EP 597 DI 10.1039/c5mh00076a PG 6 WC Chemistry, Multidisciplinary; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CU0TG UT WOS:000363231000005 ER PT J AU Graham, CF Glenn, TC Mcarthur, AG Boreham, DR Kieran, T Lance, S Manzon, RG Martino, JA Pierson, T Rogers, SM Wilson, JY Somers, CM AF Graham, Carly F. Glenn, Travis C. Mcarthur, Andrew G. Boreham, Douglas R. Kieran, Troy Lance, Stacey Manzon, Richard G. Martino, Jessica A. Pierson, Todd Rogers, Sean M. Wilson, Joanna Y. Somers, Christopher M. TI Impacts of degraded DNA on restriction enzyme associated DNA sequencing (RADSeq) SO MOLECULAR ECOLOGY RESOURCES LA English DT Article DE Coregonus clupeaformis; ddRADSeq; reduced representation libraries; SNP ID WHITEFISH COREGONUS-CLUPEAFORMIS; SINGLE-NUCLEOTIDE POLYMORPHISMS; SALMON ONCORHYNCHUS-TSHAWYTSCHA; GENETIC POPULATION-STRUCTURE; LAKE WHITEFISH; SNP DISCOVERY; CONSERVATION GENOMICS; ANALYSIS REVEALS; SSR MARKERS; DIVERSITY AB Degraded DNA from suboptimal field sampling is common in molecular ecology. However, its impact on techniques that use restriction site associated next-generation DNA sequencing (RADSeq, GBS) is unknown. We experimentally examined the effects of in situDNA degradation on data generation for a modified double-digest RADSeq approach (3RAD). We generated libraries using genomic DNA serially extracted from the muscle tissue of 8 individual lake whitefish (Coregonus clupeaformis) following 0-, 12-, 48- and 96-h incubation at room temperature posteuthanasia. This treatment of the tissue resulted in input DNA that ranged in quality from nearly intact to highly sheared. All samples were sequenced as a multiplexed pool on an Illumina MiSeq. Libraries created from low to moderately degraded DNA (12-48h) performed well. In contrast, the number of RADtags per individual, number of variable sites, and percentage of identical RADtags retained were all dramatically reduced when libraries were made using highly degraded DNA (96-h group). This reduction in performance was largely due to a significant and unexpected loss of raw reads as a result of poor quality scores. Our findings remained consistent after changes in restriction enzymes, modified fold coverage values (2- to 16-fold), and additional read-length trimming. We conclude that starting DNA quality is an important consideration for RADSeq; however, the approach remains robust until genomic DNA is extensively degraded. C1 [Graham, Carly F.; Manzon, Richard G.; Martino, Jessica A.; Somers, Christopher M.] Univ Regina, Dept Biol, Regina, SK S4S 0A2, Canada. [Glenn, Travis C.; Kieran, Troy; Pierson, Todd] Univ Georgia, Coll Publ Hlth, Athens, GA 30602 USA. [Mcarthur, Andrew G.] McMaster Univ, MG DeGroote Inst Infect Dis Res, DeGroote Sch Med, Dept Biochem & Biomed Sci, Hamilton, ON L8S 4K1, Canada. [Boreham, Douglas R.] Northern Ontario Sch Med, Med Sci, Greater Sudbury, ON, Canada. [Lance, Stacey] Univ Georgia, Savannah River Ecol Lab, Athens, GA 30602 USA. [Rogers, Sean M.] Univ Calgary, Dept Biol Sci, Calgary, AB T2N 1N4, Canada. [Wilson, Joanna Y.] McMaster Univ, Dept Biol, Hamilton, ON L8S 4M1, Canada. RP Somers, CM (reprint author), Univ Regina, Dept Biol, Regina, SK S4S 0A2, Canada. EM chris.somers@uregina.ca OI McArthur, Andrew/0000-0002-1142-3063 FU Natural Sciences and Engineering Research Council of Canada; Bruce Power; Canada Research Chairs Program; Canada Foundation for Innovation; McMaster University; University of Regina; U. S. Department of Energy [DE-FC09-07SR22506] FX This research was supported by the Natural Sciences and Engineering Research Council of Canada, Bruce Power, the Canada Research Chairs Program, the Canada Foundation for Innovation, McMaster University, and the University of Regina. We are grateful for in-kind support from the University of Regina's Institute of Environmental Change and Society, and Compute Canada's Westgrid. We would like to thank J. Mee for productive technical discussions and J. Thompson for helpful comments on the manuscript. We are grateful to three anonymous reviewers and the Associate Editor for helpful comments on an earlier version of this manuscript. D. Stefanovic provided technical support for fish rearing. Preparation of this manuscript was partially supported by U. S. Department of Energy under Award Number DE-FC09-07SR22506 to the University of Georgia Research Foundation. NR 99 TC 7 Z9 8 U1 9 U2 76 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1755-098X EI 1755-0998 J9 MOL ECOL RESOUR JI Mol. Ecol. Resour. PD NOV PY 2015 VL 15 IS 6 BP 1304 EP 1315 DI 10.1111/1755-0998.12404 PG 12 WC Biochemistry & Molecular Biology; Ecology; Evolutionary Biology SC Biochemistry & Molecular Biology; Environmental Sciences & Ecology; Evolutionary Biology GA CT5GZ UT WOS:000362838300005 PM 25783180 ER PT J AU Yu, HJ Takeuchi, M LeBarron, J Kantharia, J London, E Bakker, H Haltiwanger, RS Li, HL Takeuchi, H AF Yu, Hongjun Takeuchi, Megumi LeBarron, Jamie Kantharia, Joshua London, Erwin Bakker, Hans Haltiwanger, Robert S. Li, Huilin Takeuchi, Hideyuki TI Notch-modifying xylosyltransferase structures support an S(N)i-like retaining mechanism SO NATURE CHEMICAL BIOLOGY LA English DT Article ID PROTEIN O-GLUCOSYLTRANSFERASE; ENZYMATIC GLYCOSYL TRANSFER; SQUAMOUS-CELL CARCINOMA; GROWTH-FACTOR REPEATS; FACTOR-LIKE DOMAIN; FACTOR-IX; GLYCOSYLTRANSFERASE; ALPHA; RUMI; CONFIGURATION AB A major question remaining in glycobiology is how a glycosyltransferase (GT) that retains the anomeric linkage of a sugar catalyzes the reaction. Xyloside alpha-1,3-xylosyltransferase (XXYLT1) is a retaining GT that regulates Notch receptor activation by adding xylose to the Notch extracellular domain. Here, using natural acceptor and donor substrates and active Mus musculus XXYLT1, we report a series of crystallographic snapshots along the reaction, including an unprecedented natural and competent Michaelis reaction complex for retaining enzymes. These structures strongly support the S(N)i-like reaction as the retaining mechanism for XXYLT1. Unexpectedly, the epidermal growth factor-like repeat acceptor substrate undergoes a large conformational change upon binding to the active site, providing a structural basis for substrate specificity. Our improved understanding of this retaining enzyme will accelerate the design of retaining GT inhibitors that can modulate Notch activity in pathological situations in which Notch dysregulation is known to cause cancer or developmental disorders. C1 [Yu, Hongjun; Li, Huilin] Brookhaven Natl Lab, Biosci Dept, Upton, NY 11973 USA. [Takeuchi, Megumi; Kantharia, Joshua; London, Erwin; Haltiwanger, Robert S.; Li, Huilin; Takeuchi, Hideyuki] SUNY Stony Brook, Dept Biochem & Cell Biol, Stony Brook, NY 11794 USA. [LeBarron, Jamie] SUNY Stony Brook, Dept Physiol & Biophys, Stony Brook, NY 11794 USA. [Bakker, Hans] Hannover Med Sch, Dept Cellular Chem, Hannover, Germany. RP Yu, HJ (reprint author), Brookhaven Natl Lab, Biosci Dept, Upton, NY 11973 USA. EM hli@bnl.gov; takeuchi@uga.edu RI Bakker, Hans/A-1787-2017 OI Bakker, Hans/0000-0002-1364-9154 FU US National Institutes of Health [GM061126, AG029979]; Stony Brook University-Brookhaven National Laboratory Seed grant; German Research Foundation (Deutsche Forschungsgemeinschaft (DFG) [BA4091/5-1]; National Science Foundation [DMR 1404985]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886]; US Department of Energy [DE-FG02-93ER20097] FX We thank members of the Li and Haltiwanger labs for critical comments on this work. The work was supported by US National Institutes of Health grants GM061126 (R.S.H.) and AG029979 (H.L.), Stony Brook University-Brookhaven National Laboratory Seed grant (R.S.H. and H.L.), German Research Foundation (Deutsche Forschungsgemeinschaft (DFG)) grant BA4091/5-1 (H.B.) and National Science Foundation grant DMR 1404985 (E.L.). We acknowledge access to beamlines X25, X29 and X6A at the National Synchrotron Light Source (NSLS) and thank the staff at these beamlines. NSLS were supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract no. DE-AC02-98CH10886. UDP-xylose isolation by the Carbosource Services at the Complex Carbohydrate Research Center, University of Georgia was supported in part by the US Department of Energy grant DE-FG02-93ER20097. The results published here are in part based upon data generated by the Cancer Genome Atlas Research Network (http://cancergenome.nih.gov/). NR 47 TC 6 Z9 6 U1 1 U2 15 PU NATURE PUBLISHING GROUP PI NEW YORK PA 75 VARICK ST, 9TH FLR, NEW YORK, NY 10013-1917 USA SN 1552-4450 EI 1552-4469 J9 NAT CHEM BIOL JI Nat. Chem. Biol. PD NOV PY 2015 VL 11 IS 11 BP 847 EP U61 DI 10.1038/nchembio.1927 PG 10 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CU1HS UT WOS:000363272100010 PM 26414444 ER PT J AU Xu, R Chen, CC Wu, L Scott, MC Theis, W Ophus, C Bartels, M Yang, Y Ramezani-Dakhel, H Sawaya, MR Heinz, H Marks, LD Ercius, P Miao, JW AF Xu, Rui Chen, Chien-Chun Wu, Li Scott, M. C. Theis, W. Ophus, Colin Bartels, Matthias Yang, Yongsoo Ramezani-Dakhel, Hadi Sawaya, Michael R. Heinz, Hendrik Marks, Laurence D. Ercius, Peter Miao, Jianwei TI Three-dimensional coordinates of individual atoms in materials revealed by electron tomography SO NATURE MATERIALS LA English DT Article ID MICROSCOPY; RESOLUTION; STRAIN; DEVICES; SCALE; CRYSTALLOGRAPHY; ENHANCEMENT; CONTRAST; IMAGES; FIELD AB Crystallography, the primary method for determining the 3D atomic positions in crystals, has been fundamental to the development of many fields of science(1). However, the atomic positions obtained from crystallography represent a global average of many unit cells in a crystal(1,2). Here, we report, for the first time, the determination of the 3D coordinates of thousands of individual atoms and a point defect in a material by electron tomography with a precision of similar to 19 pm, where the crystallinity of the material is not assumed. From the coordinates of these individual atoms, we measure the atomic displacement field and the full strain tensor with a 3D resolution of similar to 1 nm(3) and a precision of similar to 10(-3), which are further verifiedby density functional theory calculations and molecular dynamics simulations. The ability to precisely localize the 3D coordinates of individual atoms in materials without assuming crystallinity is expected to find important applications in materials science, nanoscience, physics, chemistry and biology. C1 [Xu, Rui; Chen, Chien-Chun; Wu, Li; Scott, M. C.; Bartels, Matthias; Yang, Yongsoo; Miao, Jianwei] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Xu, Rui; Chen, Chien-Chun; Wu, Li; Scott, M. C.; Bartels, Matthias; Yang, Yongsoo; Miao, Jianwei] Univ Calif Los Angeles, Calif NanoSyst Inst, Los Angeles, CA 90095 USA. [Chen, Chien-Chun] Natl Sun Yat Sen Univ, Dept Phys, Kaohsiung 80424, Taiwan. [Theis, W.] Univ Birmingham, Nanoscale Phys Res Lab, Sch Phys & Astron, Birmingham B15 2TT, W Midlands, England. [Ophus, Colin; Ercius, Peter] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Natl Ctr Electron Microscopy, Mol Foundry, Berkeley, CA 94720 USA. [Ramezani-Dakhel, Hadi; Heinz, Hendrik] Univ Akron, Dept Polymer Engn, Akron, OH 44325 USA. [Sawaya, Michael R.] UCLA DOE Inst Genom & Prote, Howard Hughes Med Inst, Los Angeles, CA 90095 USA. [Marks, Laurence D.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60201 USA. RP Miao, JW (reprint author), Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. EM miao@physics.ucla.edu RI Heinz, Hendrik/E-3866-2010; Yang, Yongsoo/P-7716-2014; Foundry, Molecular/G-9968-2014; Marks, Laurence/B-7527-2009; OI Heinz, Hendrik/0000-0002-6776-7404; Yang, Yongsoo/0000-0001-8654-302X; Sawaya, Michael/0000-0003-0874-9043 FU Office of Basic Energy Sciences of the US Department of Energy [DE-FG02-13ER46943]; NSF [DMR-1437263, DMR-0955071]; ONR MURI [N00014-14-1-0675]; DOE [DE-FG02-01ER45945]; Office of Science, Office of Basic Energy Sciences of the US Department of Energy [DE-AC02-05CH11231] FX We thank U. Dahmen, J. Du, L. Deng, E. J. Kirkland, R. F. Bruinsma and L. A. Vese for stimulating discussions. This work was primarily supported by the Office of Basic Energy Sciences of the US Department of Energy (Grant No. DE-FG02-13ER46943). This work was partially supported by NSF (DMR-1437263 and DMR-0955071) as well as ONR MURI (N00014-14-1-0675). L.D.M. acknowledges support from the DOE (Grant No. DE-FG02-01ER45945). ADF-STEM imaging was performed on TEAM I at the Molecular Foundry, which is supported by the Office of Science, Office of Basic Energy Sciences of the US Department of Energy under Contract No. DE-AC02-05CH11231. H.R.-D. and H.H. acknowledge the allocation of computing resources at the Ohio Supercomputer Center. NR 41 TC 13 Z9 13 U1 16 U2 70 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1476-1122 EI 1476-4660 J9 NAT MATER JI Nat. Mater. PD NOV PY 2015 VL 14 IS 11 BP 1099 EP + DI 10.1038/NMAT4426 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA CU4BU UT WOS:000363471900016 PM 26390325 ER PT J AU Volkow, ND Wang, GJ Smith, L Fowler, JS Telang, F Logan, J Tomasi, D AF Volkow, Nora D. Wang, Gene-Jack Smith, Lisa Fowler, Joanna S. Telang, Frank Logan, Jean Tomasi, Dardo TI Recovery of dopamine transporters with methamphetamine detoxification is not linked to changes in dopamine release SO NEUROIMAGE LA English DT Article DE Addiction; Neurotoxicity; Dopamine terminal; Parkinson's disease ID POSITRON-EMISSION-TOMOGRAPHY; PLACEBO-CONTROLLED TRIAL; PARKINSONS-DISEASE; DOWN-REGULATION; DOUBLE-BLIND; NEUROTOXICITY; BRAIN; RAT; COCAINE; METHYLPHENIDATE AB Methamphetamine's widepread abuse and concerns that it might increase Parkinson's disease led us to assess if the reported loss of dopamine transporters (DAT) in methamphetamine abusers (MA) reflected damage to dopamine neurons. Using PET with [C-11] cocaine to measure DAT, and with [C-11]raclopride to measure dopamine release (assessed as changes in specific binding of [C-11] raclopride between placebo and methylphenidate), which was used as a marker of dopamine neuronal function, we show that MA (n = 16), tested during early detoxification, had lower DAT (20-30%) but overall normal DA release in striatum(except for a small decrease in left putamen), when compared to controls (n = 15). In controls, DAT were positively correlated with DA release (higher DAT associated with larger DA increases), consistent with DAT serving as markers of DA terminals. In contrast, MA showed a trend for a negative correlation (p = 0.07) (higher DAT associated with lower DA increases), consistent with reduced DA re-uptake following DAT downregulation. MA who remained abstinent nine-months later (n = 9) showed significant increases in DAT (20%) but methylphenidate-induced dopamine increases did not change. In contrast, in controls, DAT did not change when retested 9 months later but methylphenidate-induced dopamine increases in ventral striatum were reduced (p = 0.05). Baseline D2/D3 receptors in caudate were lower in MA than in controls and did not change with detoxification, nor did they change in the controls upon retest. The loss of DAT in the MA, which was not associated with a concomitant reduction in dopamine release as would have been expected if DAT loss reflected DA terminal degneration; as well as the recovery of DAT after protracted detoxification, which was not associated with increased dopamine release as would have been expected if DAT increases reflected terminal regeneration, indicate that the loss of DAT in these MA does not reflect degeneration of dopamine terminals. Published by Elsevier Inc. C1 [Volkow, Nora D.; Wang, Gene-Jack; Telang, Frank; Logan, Jean; Tomasi, Dardo] NIAAA, Lab Neuroimaging, Intramural Program, Bethesda, MD USA. [Smith, Lisa] Univ Calif Los Angeles, Dept Psychiat, Los Angeles, CA USA. [Fowler, Joanna S.] Brookhaven Natl Lab, Dept Med, Upton, NY 11973 USA. [Volkow, Nora D.] NIDA, Off Director, Bethesda, MD 20892 USA. RP Volkow, ND (reprint author), NIDA, NIH, 6001 Execut Blvd,Room 5274, Bethesda, MD 20892 USA. EM nvolkow@nida.nih.gov OI Logan, Jean/0000-0002-6993-9994 FU NIH intramural program (NIAAA); Brookhaven National Laboratory (BNL) [DE-AC02-98CH10886] FX This research was supported by the NIH intramural program (NIAAA) and carried out at Brookhaven National Laboratory (BNL) under contract DE-AC02-98CH10886. We thank C. Wong, C Shea, Y. Xu, D Alexoff, P. King, Karen Apelskog and Ruben Baler. NR 54 TC 9 Z9 9 U1 0 U2 9 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 1053-8119 EI 1095-9572 J9 NEUROIMAGE JI Neuroimage PD NOV 1 PY 2015 VL 121 BP 20 EP 28 DI 10.1016/j.neuroimage.2015.07.035 PG 9 WC Neurosciences; Neuroimaging; Radiology, Nuclear Medicine & Medical Imaging SC Neurosciences & Neurology; Radiology, Nuclear Medicine & Medical Imaging GA CT9FK UT WOS:000363122000003 PM 26208874 ER PT J AU Johnson, TD Kulp, WD AF Johnson, T. D. Kulp, W. D. TI Nuclear Data Sheets for A=87* SO NUCLEAR DATA SHEETS LA English DT Article ID NEUTRON EMISSION PROBABILITIES; ISOBARIC-ANALOG RESONANCES; LIVED FISSION-PRODUCTS; GAMMA-RAY ENERGY; HIGH-SPIN STATES; PROTON-TRANSFER-REACTIONS; HALBWERTSZEIT DES RB87; N=46 ISOTONES ZR-86; CORE-COUPLED STATES; DELAYED-NEUTRON AB The evaluated experimental data are presented for 14 known nuclides of mass 87 (Ga, Ge, As, Se, Br, Kr, Rb, Sr, Y, Zr, Nb, Me, Tc, Ru). New datasets have been added for Ga-87, Se-87, Kr-87, Rb-87, Sr-87, Nb-87, and Tc-87. The observation of and new lifetime measurements for As-87 at the NSCL Coupled Cyclotron Facility and the Oak Ridge Isochronous Cyclotron at the HRIBF-ORNL Facility are included in the adopted levels for this isotope. The new evaluation also includes an isomeric level at unknown energy for Tc-87, changes to the adopted levels for Nb-87 based on newly published data including an extension of the high spin levels and new lifetime measurements, and new heavy ion data for Kr-87. New high spin levels for Rb-87 were observed, indicating possible neutron core excitations. In addition, the ground state lifetime of Rb-87 has been revised and a new lifetime measurement for an excited level in Rb-87 indicates a possible proton spin flip. New excitation levels have been observed for the first time in Se-87. New direct and precise measurement of atomic masses of Tc-87, Mo-87, Nb-87, Zr-87, Mo-87 and Tc-87 have greatly improved the Q value landscape in this mass region. This work supersedes the previous A=87 evaluation published in 2002He09, and Q values for all isotopes were updated to incorporate the mass evaluation in 2012Wa38. C1 [Johnson, T. D.; Kulp, W. D.] Brookhaven Natl Lab, Natl Nucl Data Ctr, Upton, NY 11973 USA. RP Johnson, TD (reprint author), Brookhaven Natl Lab, Natl Nucl Data Ctr, Upton, NY 11973 USA. FU Office of Nuclear Physics, Office of Science of the U.S. Department of Energy [DE-AC02-98CH10886] FX Work supported by the Office of Nuclear Physics, Office of Science of the U.S. Department of Energy under contract DE-AC02-98CH10886. NR 339 TC 0 Z9 0 U1 1 U2 7 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD NOV PY 2015 VL 129 BP 1 EP 189 DI 10.1016/j.nds.2015.09.001 PG 189 WC Physics, Nuclear SC Physics GA CU3QC UT WOS:000363438900001 ER PT J AU Bull, D AF Bull, Diana TI An improved understanding of the natural resonances of moonpools contained within floating rigid-bodies: Theory and application to oscillating water column devices SO OCEAN ENGINEERING LA English DT Article DE Moonpool; Natural resonance; Wave energy converter; Oscillating water column; Resistive damping control; BBDB AB The fundamental interactions between waves, a floating rigid-body, and a moonpool that is selectively open to atmosphere or enclosed to purposefully induce pressure fluctuations are investigated. The moonpool hydrodynamic characteristics and the hydrodynamic coupling to the rigid-body are derived implicitly through reciprocity relations on an array of field points. By modeling the free surface of the moonpool in this manner, an explicit hydrodynamic coupling term is included in the equations of motion. This coupling results in the migration of the moonpool's natural resonance frequency from the piston frequency to a new frequency when enclosed in a floating rigid-body. Two geometries that highlight distinct aspects of marine vessels and oscillating water column (OWC) renewable energy devices are analyzed to reveal the coupled natural resonance migration. The power performance of these two OWCs in regular waves is also investigated. The air chamber is enclosed and a three-dimensional, linear, frequency domain performance model that links the rigid-body to the moonpool through a linear resistive control strategy is detailed. An analytic expression for the optimal linear resistive control values in regular waves is presented. (C) 2015 Elsevier Ltd. All rights reserved. C1 Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Bull, D (reprint author), Sandia Natl Labs, POB 5800,MS 1124, Albuquerque, NM 87185 USA. FU U.S. Depai Intent of Energy's Wind and Water Power Technologies Office; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was funded by the U.S. Depai Intent of Energy's Wind and Water Power Technologies Office. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 30 TC 4 Z9 4 U1 7 U2 14 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0029-8018 J9 OCEAN ENG JI Ocean Eng. PD NOV 1 PY 2015 VL 108 BP 799 EP 812 DI 10.1016/j.oceaneng.2015.07.007 PG 14 WC Engineering, Marine; Engineering, Civil; Engineering, Ocean; Oceanography SC Engineering; Oceanography GA CU2HY UT WOS:000363345800068 ER PT J AU Fensin, ML Umbel, M AF Fensin, Michael Lorne Umbel, Marissa TI Testing actinide fission yield treatment in CINDER90 for use in MCNP6 burnup calculations SO PROGRESS IN NUCLEAR ENERGY LA English DT Article DE MCNP6; CINDER90; Fission yield; Burnup ID NUCLEAR-SCIENCE; CODE; LIBRARY AB Most of the development of the MCNPX/6 burnup capability focused on features that were applied to the Boltzman transport or used to prepare coefficients for use in CINDER90, with little change to CINDER90 or the CINDER90 data. Though a scheme exists for best solving the coupled Boltzman and Bateman equations, the most significant approximation is that the employed nuclear data are correct and complete. The CINDER90 library file contains 60 different actinide fission yields encompassing 36 fissionable actinides (thermal, fast, high energy and spontaneous fission). Fission reaction data exists for more than 60 actinides and as a result, fission yield data must be approximated for actinides that do not possess fission yield information. Several types of approximations are used for estimating fission yields for actinides which do not possess explicit fission yield data. The objective of this study is to test whether or not certain approximations of fission yield selection have any impact on predictability of major actinides and fission products. Further we assess which other fission products, available in MCNP6 Tier 3, result in the largest difference in production. Because the CINDER90 library file is in ASCII format and therefore easily amendable, we assess reasons for choosing, as well as compare actinide and major fission product prediction for the H. B. Robinson benchmark for, three separate fission yield selection methods: (1) the current CINDER90 library file method (Base); (2) the element method (Element); and (3) the isobar method (Isobar). Results show that the three methods tested result in similar prediction of major actinides, Tc-99 and Cs-137; however, certain fission products resulted in significantly different production depending on the method of choice. Published by Elsevier Ltd. C1 [Fensin, Michael Lorne; Umbel, Marissa] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Fensin, ML (reprint author), Los Alamos Natl Lab, MS C921, Los Alamos, NM 87545 USA. EM mfensin@lanl.gov RI kiaie, robabeh/I-2157-2016; kiaie, fatemeh/I-6083-2016 OI kiaie, robabeh/0000-0001-5251-3201; NR 24 TC 1 Z9 1 U1 0 U2 2 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0149-1970 J9 PROG NUCL ENERG JI Prog. Nucl. Energy PD NOV PY 2015 VL 85 BP 719 EP 728 DI 10.1016/j.pnucene.2015.09.001 PG 10 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CU2JF UT WOS:000363349100070 ER PT J AU Fox, NK Brenner, SE Chandonia, JM AF Fox, Naomi K. Brenner, Steven E. Chandonia, John-Marc TI The value of protein structure classification informationSurveying the scientific literature SO PROTEINS-STRUCTURE FUNCTION AND BIOINFORMATICS LA English DT Article DE SCOP; CATH; database; curation; resources ID STRUCTURE PREDICTION; STRUCTURE ALIGNMENT; ASTRAL COMPENDIUM; SEQUENCE ALIGNMENT; STRUCTURE DATABASE; HOMOLOGY DETECTION; FUNCTIONAL SITES; GENOME SEQUENCES; CATH DATABASE; DATA-BANK AB The Structural Classification of Proteins (SCOP) and Class, Architecture, Topology, Homology (CATH) databases have been valuable resources for protein structure classification for over 20 years. Development of SCOP (version 1) concluded in June 2009 with SCOP 1.75. The SCOPe (SCOP-extended) database offers continued development of the classic SCOP hierarchy, adding over 33,000 structures. We have attempted to assess the impact of these two decade old resources and guide future development. To this end, we surveyed recent articles to learn how structure classification data are used. Of 571 articles published in 2012-2013 that cite SCOP, 439 actually use data from the resource. We found that the type of use was fairly evenly distributed among four top categories: A) study protein structure or evolution (27% of articles), B) train and/or benchmark algorithms (28% of articles), C) augment non-SCOP datasets with SCOP classification (21% of articles), and D) examine the classification of one protein/a small set of proteins (22% of articles). Most articles described computational research, although 11% described purely experimental research, and a further 9% included both. We examined how CATH and SCOP were used in 158 articles that cited both databases: while some studies used only one dataset, the majority used data from both resources. Protein structure classification remains highly relevant for a diverse range of problems and settings. Proteins 2015; 83:2025-2038. (c) 2015 The Authors. Proteins: Structure, Function, and Bioinformatics Published by Wiley Periodicals, Inc. C1 [Fox, Naomi K.; Brenner, Steven E.; Chandonia, John-Marc] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Brenner, Steven E.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. RP Chandonia, JM (reprint author), Lawrence Berkeley Natl Lab, 1 Cyclotron Rd,Mailstop Donner, Berkeley, CA 94720 USA. EM scope@compbio.berkeley.edu RI Brenner, Steven/A-8729-2008 OI Brenner, Steven/0000-0001-7559-6185 FU National Institutes of Health (NIH) [R01-GM073109]; National Institutes of Health through US Department of Energy [DE-AC02-05CH11231] FX Grant sponsor: National Institutes of Health (NIH); Grant number: R01-GM073109; This work is supported by the National Institutes of Health through the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 78 TC 2 Z9 2 U1 1 U2 6 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0887-3585 EI 1097-0134 J9 PROTEINS JI Proteins PD NOV PY 2015 VL 83 IS 11 BP 2025 EP 2038 DI 10.1002/prot.24915 PG 14 WC Biochemistry & Molecular Biology; Biophysics SC Biochemistry & Molecular Biology; Biophysics GA CU2GN UT WOS:000363342000009 PM 26313554 ER PT J AU Mejia-Alvarez, R Wilson, B Leftwich, MC Martinez, AA Prestridge, KP AF Mejia-Alvarez, R. Wilson, B. Leftwich, M. C. Martinez, A. A. Prestridge, K. P. TI Design of a fast diaphragmless shock tube driver SO SHOCK WAVES LA English DT Article DE Diaphragmless shock tube ID LASER-INDUCED FLUORESCENCE; FAST-ACTING VALVES; PISTON; TEMPERATURE AB In this paper, we developed a one-dimensional compressible flow model to study the behavior of various diaphragmless drivers numerically. We determined that the diameter ratio, , for the discharge orifice of the back chamber controls driver actuation. Driver performance is optimized by accelerating the barrier element before breaching to minimize the opening time of the driver. Our new two-body driver outperforms various designs and exhibits opening times comparable to those of aluminum burst diaphragms. Experimental results verify the effectiveness of the new driver and show that it closely follows the pressure-Mach curve for the ideal case. Planar laser-induced fluorescence images and pressure traces confirm the consistent formation of shock waves about 41 diameters from the driver. C1 [Mejia-Alvarez, R.; Wilson, B.; Martinez, A. A.; Prestridge, K. P.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Leftwich, M. C.] George Washington Univ, Washington, DC 20052 USA. RP Mejia-Alvarez, R (reprint author), Los Alamos Natl Lab, Mailstop H803, Los Alamos, NM 87545 USA. EM rimejal@lanl.gov RI Prestridge, Kathy/C-1137-2012 OI Prestridge, Kathy/0000-0003-2425-5086 NR 28 TC 2 Z9 2 U1 0 U2 7 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0938-1287 EI 1432-2153 J9 SHOCK WAVES JI Shock Waves PD NOV PY 2015 VL 25 IS 6 BP 635 EP 650 DI 10.1007/s00193-015-0579-y PG 16 WC Mechanics SC Mechanics GA CT8IY UT WOS:000363060300006 ER PT J AU Campbell, MF Parise, T Tulgestke, AM Spearrin, RM Davidson, DF Hanson, RK AF Campbell, M. F. Parise, T. Tulgestke, A. M. Spearrin, R. M. Davidson, D. F. Hanson, R. K. TI Strategies for obtaining long constant-pressure test times in shock tubes SO SHOCK WAVES LA English DT Article DE Long test time; Driver insert; Driver gas tailoring; Staged driver gas filling; Reflected shock; Shock tube ID IGNITION DELAY TIMES; CHEMICAL-KINETICS; LOW-TEMPERATURES; MIXTURES; WAVES; ABSORPTION; EXTENSION AB Several techniques have been developed for obtaining long, constant-pressure test times in reflected shock wave experiments in a shock tube, including the use of driver inserts, driver gas tailoring, helium gas diaphragm interfaces, driver extensions, and staged driver gas filling. These techniques are detailed here, including discussion on the most recent strategy, staged driver gas filling. Experiments indicate that this staged filling strategy increases available test time by roughly 20 % relative to single-stage filling of tailored driver gas mixtures, while simultaneously reducing the helium required per shock by up to 85 %. This filling scheme involves firstly mixing a tailored helium-nitrogen mixture in the driver section as in conventional driver filling and, secondly, backfilling a low-speed-of-sound gas such as nitrogen or carbon dioxide from a port close to the end cap of the driver section. Using this staged driver gas filling, in addition to the other techniques listed above, post-reflected shock test times of up to 0.102 s (102 ms) at 524 K and 1.6 atm have been obtained. Spectroscopically based temperature measurements in non-reactive mixtures have confirmed that temperature and pressure conditions remain constant throughout the length of these long test duration trials. Finally, these strategies have been used to measure low-temperature n-heptane ignition delay times. C1 [Campbell, M. F.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. [Parise, T.; Tulgestke, A. M.; Spearrin, R. M.; Davidson, D. F.; Hanson, R. K.] Stanford Univ, Dept Mech Engn, Stanford, CA 94305 USA. RP Campbell, MF (reprint author), Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. EM mfcampb@sandia.gov FU Army Research Office; Division of Chemical Sciences, Geosciences, and Biosciences; Office of Basic Energy Sciences (BES); US Department of Energy (DOE); National Defense Science and Engineering Graduate (NDSEG) Fellowship [32 CFR 168a]; US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the Army Research Office, with Dr. Ralph Anthenien as technical monitor. M.F.C. was supported by the Division of Chemical Sciences, Geosciences, and Biosciences, the Office of Basic Energy Sciences (BES), the US Department of Energy (DOE). Also, during a portion of this work, M.F.C. was supported by a National Defense Science and Engineering Graduate (NDSEG) Fellowship, 32 CFR 168a. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. The authors wish to acknowledge Andrew Lawson and Kaley Boyce for their assistance in the configuration of the shock tube, and further wish to thank the technicians in the Stanford University plumbing shop for assistance in configuration of driver inserts. NR 33 TC 4 Z9 4 U1 0 U2 10 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0938-1287 EI 1432-2153 J9 SHOCK WAVES JI Shock Waves PD NOV PY 2015 VL 25 IS 6 BP 651 EP 665 DI 10.1007/s00193-015-0596-x PG 15 WC Mechanics SC Mechanics GA CT8IY UT WOS:000363060300007 ER PT J AU Di, S Cappello, F AF Di, Sheng Cappello, Franck TI GloudSim: Google trace based cloud simulator with virtual machines SO SOFTWARE-PRACTICE & EXPERIENCE LA English DT Article DE cloud computing; simulation system; Google cluster; Google trace ID OPTIMUM CHECKPOINT INTERVAL; ALGORITHMS; TOOLKIT AB In 2011, Google released a 1-month production trace with hundreds of thousands of jobs running across over 12,000 heterogeneous hosts. In order to perform in-depth research based on the trace, it is necessary to construct a close-to-practice simulation system. In this paper, we devise a distributed cloud simulator (or toolkit) based on virtual machines, with three important features. (1) The dynamic changing resource amounts (such as CPU rate and memory size) consumed by the reproduced jobs can be emulated as closely as possible to the real values in the trace. (2) Various types of events (e.g., kill/evict event) can be emulated precisely based on the trace. (3) Our simulation toolkit is able to emulate more complex and useful cases beyond the original trace to adapt to various research demands. We evaluate the system on a real cluster environment with 16x8=128 cores and 112 virtual machines constructed by XEN hypervisor. To the best of our knowledge, this is the first work to reproduce Google cloud environment with real experimental system setting and real-world large scale production trace. Experiments show that our simulation system could effectively reproduce the real checkpointing/restart events based on Google trace, by leveraging Berkeley Lab Checkpoint/Restart tool. It can simultaneously process up to 1200 emulated Google jobs over the 112 virtual machines. Such a simulation toolkit has been released as a GNU GPL v3 software for free downloading, and it has been successfully applied to the fundamental research on the optimization of checkpoint intervals for Google tasks. Published 2014. This article is a U.S. Government work and is in the public domain in the USA. C1 [Di, Sheng; Cappello, Franck] Argonne Natl Lab, MCS, Lemont, IL 60439 USA. [Cappello, Franck] Univers Illinois Urbana Champaign, Champaign, IL USA. RP Di, S (reprint author), Argonne Natl Lab, MCS Div, Bldg 240,9700 S Cass Ave, Lemont, IL 60439 USA. EM sdi1@anl.gov FU Illinois-INRIA-ANL Joint Laboratory on Petascale Computing, Hong Kong RGC Grant [HKU-716712E]; US Department of Energy, Office of Science [DE-AC02-06CH11357]; [ANR RESCUE 5323] FX This work is supported by the projects ANR RESCUE 5323, Illinois-INRIA-ANL Joint Laboratory on Petascale Computing, Hong Kong RGC Grant HKU-716712E, and also supported in part by the US Department of Energy, Office of Science, under contract DE-AC02-06CH11357. NR 31 TC 4 Z9 4 U1 0 U2 1 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0038-0644 EI 1097-024X J9 SOFTWARE PRACT EXPER JI Softw.-Pract. Exp. PD NOV PY 2015 VL 45 IS 11 BP 1571 EP 1590 DI 10.1002/spe.2303 PG 20 WC Computer Science, Software Engineering SC Computer Science GA CU4LI UT WOS:000363500900006 ER PT J AU Wang, J Lon, HK Lee, SL Burckart, GJ Pisetsky, DS AF Wang, Jian Lon, Hoi-Kei Lee, Shwu-Luan Burckart, Gilbert J. Pisetsky, David S. TI Oligonucleotide-Based Drug Development: Considerations for Clinical Pharmacology and Immunogenicity SO THERAPEUTIC INNOVATION & REGULATORY SCIENCE LA English DT Review DE antisense oligonucleotides; clinical pharmacology; immunogenicity; pharmacokinetics; drug interactions; pharmacodynamics ID SYSTEMIC-LUPUS-ERYTHEMATOSUS; ANTI-DNA ANTIBODIES; KINASE-C-ALPHA; PHASE-II TRIAL; ANTISENSE OLIGONUCLEOTIDE; PROSTATE-CANCER; MESSENGER-RNA; PHARMACOKINETIC INTERACTION; NUCLEIC-ACIDS; SOLID TUMORS AB The field of oligonucleotide (OGN)-based therapeutics has been growing dramatically in the past decade, providing innovative platforms to develop agents for the treatment of a wide variety of clinical conditions. OGN agents have unique physicochemical properties and pharmacokinetic/pharmacodynamic characteristics. This review considers findings from the literature and information on new molecular entities submitted to the US Food and Drug Administration as OGN-based therapeutics. In addition, the article discusses several challenging issues from the perspective of clinical pharmacology, emphasizing the potential of immunogenicity, the effect of renal impairment on OGN exposure, drug-drug interactions, and the utility of pharmacokinetic/pharmacodynamic modeling. The field of OGN-based therapeutics is in evolution and will benefit from further studies as well as clinical experience to formulate guidelines and promote the development of this class of agents. C1 [Wang, Jian; Lon, Hoi-Kei; Burckart, Gilbert J.] US FDA, Off Clin Pharmacol, Silver Spring, MD USA. [Lon, Hoi-Kei] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. [Lee, Shwu-Luan] US FDA, Off Hematol & Oncol Prod, Off New Drugs, Silver Spring, MD USA. [Pisetsky, David S.] Durham VA Med Ctr, Med Res Serv, Durham, NC USA. [Pisetsky, David S.] Duke Univ, Med Ctr, Durham, NC USA. RP Pisetsky, DS (reprint author), 508 Fulton St,151G, Durham, NC 27705 USA. EM david.pisetsky@duke.edu FU US FDA; Oak Ridge Institute for Science and Education FX The author(s) disclosed receipt of the following financial support for the research, authorship, and/or publication of this article: The study was partially supported by the US FDA Regulatory Science and Review Enhancement funding and fellowship support for Dr Lon from Oak Ridge Institute for Science and Education. NR 66 TC 0 Z9 0 U1 2 U2 10 PU SAGE PUBLICATIONS INC PI THOUSAND OAKS PA 2455 TELLER RD, THOUSAND OAKS, CA 91320 USA SN 2168-4790 EI 2168-4804 J9 THER INNOV REGUL SCI JI Ther. Innov. Regul. Sci. PD NOV PY 2015 VL 49 IS 6 BP 861 EP 868 DI 10.1177/2168479015592195 PG 8 WC Medical Informatics; Pharmacology & Pharmacy SC Medical Informatics; Pharmacology & Pharmacy GA CU2DE UT WOS:000363332100011 ER PT J AU Dam, WL Campbell, S Johnson, RH Looney, BB Denham, ME Eddy-Dilek, CA Babits, SJ AF Dam, William L. Campbell, Sam Johnson, Raymond H. Looney, Brian B. Denham, Miles E. Eddy-Dilek, Carol A. Babits, Steven J. TI Refining the site conceptual model at a former uranium mill site in Riverton, Wyoming, USA SO ENVIRONMENTAL EARTH SCIENCES LA English DT Article DE Conceptual site models; Uranium; Unsaturated zone; Groundwater contamination; River flooding; Evaporite mineral deposits ID GROUNDWATER CONTAMINATION; TAILINGS PILE; MIXING MODEL AB Milling activities at a former uranium mill site near Riverton, Wyoming, USA, contaminated the shallow groundwater beneath and downgradient of the site. Although the mill operated for < 6 years (1958-1963), its impact remains an environmental liability. Groundwater modeling predicted that natural flushing would achieve compliance with applicable groundwater protection standards by the year 2098. A decade of groundwater monitoring indicated that contaminant concentrations were declining steadily, which confirmed the conceptual site model (CSM). However, local flooding in 2010 mobilized contaminants that migrated downgradient from the Riverton site and resulted in a dramatic increase in groundwater contaminant concentrations. This observation indicated that the original CSM was inadequate to explain site conditions and needed to be refined. In response to the new observations after the flood, a collaborative investigation to better understand site conditions and processes commenced. This investigation included installing 103 boreholes to collect soil and groundwater samples, sampling and analysis of evaporite minerals along the bank of the Little Wind River, an analysis of evapotranspiration in the shallow aquifer, and sampling naturally organic-rich sediments near groundwater discharge areas. The enhanced characterization revealed that the existing CSM did not account for high uranium concentrations in groundwater remaining on the former mill site and groundwater plume stagnation near the Little Wind River. Observations from the flood and subsequent investigations indicate that additional characterization is still needed to continue refining the CSM and determine the viability of the natural flushing compliance strategy. Additional sampling, analysis, and testing of soil and groundwater are necessary to investigate secondary contaminant sources, mobilization of contaminants during floods, geochemical processes, contaminant plume stagnation, distribution of evaporite minerals and organic-rich sediments, and mechanisms and rates of contaminant transfer from soil to groundwater. Future data collection will be used to continually revise the CSM and evaluate the compliance strategy at the site. C1 [Dam, William L.] US DOE, Off Legacy Management, Grand Junction, CO 81503 USA. [Campbell, Sam; Johnson, Raymond H.] Stoller Newport News Nucl Inc, Grand Junction, CO 81503 USA. [Looney, Brian B.; Denham, Miles E.; Eddy-Dilek, Carol A.] US DOE, Savannah River Natl Lab, Off Environm Management, Ctr Sustainable Groundwater & Soil Solut, Aiken, SC 29808 USA. [Babits, Steven J.] Shoshone & Arapaho Tribes, Lander, WY 82520 USA. RP Dam, WL (reprint author), US DOE, Off Legacy Management, 2597 Legacy Way, Grand Junction, CO 81503 USA. EM William.dam@lm.doe.gov FU US Department of Energy Office of Legacy Management FX This study was funded by the US Department of Energy Office of Legacy Management. The authors wish to thank the people living on the Wind River Indian Reservation for active participation and seeking to differentiate between actual and perceived environmental risks. Kent Bostick provided many helpful technical review comments. NR 20 TC 0 Z9 0 U1 4 U2 11 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1866-6280 EI 1866-6299 J9 ENVIRON EARTH SCI JI Environ. Earth Sci. PD NOV PY 2015 VL 74 IS 10 BP 7255 EP 7265 DI 10.1007/s12665-015-4706-y PG 11 WC Environmental Sciences; Geosciences, Multidisciplinary; Water Resources SC Environmental Sciences & Ecology; Geology; Water Resources GA CT6EA UT WOS:000362903400022 ER PT J AU Hintsala, E Kiener, D Jackson, J Gerberich, WW AF Hintsala, E. Kiener, D. Jackson, J. Gerberich, W. W. TI In-Situ Measurements of Free-Standing, Ultra-Thin Film Cracking in Bending SO EXPERIMENTAL MECHANICS LA English DT Article DE Electron backscatter diffraction; Fracture testing; Electron micrscopy; Steel; Nanomechanics ID FRACTURE-TOUGHNESS; MECHANICAL-PROPERTIES; ALLOY-FILMS; NANOINDENTATION; METAL; TEM; SPECIMENS; ALUMINUM; INTERCONNECTS; DISPLACEMENT AB Metallic thin films are widely used and relied upon for various technologies. Direct measurements of fracture toughness are rare for metallic thin films and existing methods for obtaining these measurements often do not provide characterization of the cracking process for determination of crack growth mechanisms. To rectify this, we explore a new technique which utilizes doubly clamped, in-situ three-point bend testing of micro-scale and nano-scale specimens. This is done by in-situ scanning electron microscopy (SEM) and transmission electron microscopy (TEM) mechanical testing for specimens with thicknesses of 2500 nm (SEM), 500 nm (SEM) and 100 nm (TEM). For in-situ TEM, a novel notching method is employed using the converged electron beam which achieves a notch radius of approximately 5 nm. Additionally, we present supporting characterization using Electron Backscatter Diffraction (EBSD) for 2500 nm thick specimens as a demonstration of the potential of this technique for understanding local deformation. Analysis of the acquired data presents several issues that require addressing, and recommendations for future improvements are given. C1 [Hintsala, E.; Gerberich, W. W.] Univ Minnesota, Dept Chem Engn & Mat Sci, Minneapolis, MN 55455 USA. [Kiener, D.] Univ Leoben, Dept Mat Phys, Leoben, Austria. [Jackson, J.] Idaho Natl Lab, Idaho Falls, ID USA. RP Hintsala, E (reprint author), Univ Minnesota, Dept Chem Engn & Mat Sci, Amundson Hall,421 Washington Ave SE, Minneapolis, MN 55455 USA. EM hints009@umn.edu RI Kiener, Daniel/B-2202-2008 OI Kiener, Daniel/0000-0003-3715-3986 FU INL (DOE) [00109759, DE-AC07-951014517]; Marshall Plan scholarship foundation via Montanuniversitat Leoben; Austrian Science Fund FWF [P25325-N20] FX Funding by INL (DOE) Grant #00109759 (Subcontract to DE-AC07-951014517) and the Marshall Plan scholarship foundation via Montanuniversitat Leoben. The authors would also like to thank Ruth Treml, Peter Imrich and Stefan Wurster for their help on this project. DK acknowledges funding from the Austrian Science Fund FWF (project number P25325-N20). NR 46 TC 1 Z9 1 U1 4 U2 19 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0014-4851 EI 1741-2765 J9 EXP MECH JI Exp. Mech. PD NOV PY 2015 VL 55 IS 9 BP 1681 EP 1690 DI 10.1007/s11340-015-0069-2 PG 10 WC Materials Science, Multidisciplinary; Mechanics; Materials Science, Characterization & Testing SC Materials Science; Mechanics GA CT6ZN UT WOS:000362962700007 ER PT J AU Abraha, M Chen, JQ Chu, HS Zenone, T John, R Su, YJ Hamilton, SK Robertson, GP AF Abraha, Michael Chen, Jiquan Chu, Housen Zenone, Terenzio John, Ranjeet Su, Yahn-Jauh Hamilton, Stephen K. Robertson, G. Philip TI Evapotranspiration of annual and perennial biofuel crops in a variable climate SO GLOBAL CHANGE BIOLOGY BIOENERGY LA English DT Article DE cellulosic biofuel crops; Conservation Reserve Program; conventional agriculture; eddy covariance; grasslands; land use conversion; water use ID ENERGY IMBALANCE PROBLEM; WATER-USE EFFICIENCY; SENSIBLE HEAT-FLUX; EDDY-COVARIANCE; BIOENERGY CROPS; INTERANNUAL VARIATION; GRASSLAND ECOSYSTEMS; SONIC ANEMOMETER; CENTRAL ILLINOIS; MARGINAL LANDS AB Eddy covariance measurements were made in seven fields in the Midwest USA over 4years (including the 2012 drought year) to estimate evapotranspiration (ET) of newly established rain-fed cellulosic and grain biofuel crops. Four of the converted fields had been managed as grasslands under the USDA's Conservation Reserve Program (CRP) for 22years, and three had been in conventional agriculture (AGR) soybean/corn rotation prior to conversion. In 2009, all sites were planted to no-till soybean except one CRP grassland that was left unchanged as a reference site; in 2010, three of the former CRP sites and the three former AGR sites were planted to annual (corn) and perennial (switchgrass and mixed-prairie) grasslands. The annual ET over the 4years ranged from 45% to 77% (mean=60%) of the annual precipitation (848-1063mm; November-October), with the unconverted CRP grassland having the highest ET (622-706mm). In the fields converted to annual and perennial crops, the annual ET ranged between 480 and 639mm despite the large variations in growing-season precipitation and in soil water contents, which had strong effects on regional crop yields. Results suggest that in this humid temperate climate, which represents the US Corn Belt, water use by annual and perennial crops is not greatly different across years with highly variable precipitation and soil water availability. Therefore, large-scale conversion of row crops to perennial biofuel cropping systems may not strongly alter terrestrial water balances. C1 [Abraha, Michael; Chen, Jiquan; John, Ranjeet; Su, Yahn-Jauh] Michigan State Univ, CGCEO Geog, E Lansing, MI 48823 USA. [Abraha, Michael; Chen, Jiquan; Zenone, Terenzio; Hamilton, Stephen K.; Robertson, G. Philip] Michigan State Univ, Great Lakes Bioenergy Res Ctr, Hickory Corners, MI 49060 USA. [Abraha, Michael; Hamilton, Stephen K.; Robertson, G. Philip] Michigan State Univ, WK Kellogg Biol Stn, Hickory Corners, MI 49060 USA. [Chu, Housen; Zenone, Terenzio] Univ Toledo, Landscape Ecol & Ecosyst Sci, Toledo, OH 43606 USA. [Hamilton, Stephen K.] Michigan State Univ, Dept Integrat Biol, E Lansing, MI 48824 USA. [Robertson, G. Philip] Michigan State Univ, Dept Plant Soil & Microbial Sci, E Lansing, MI 48824 USA. RP Abraha, M (reprint author), Michigan State Univ, CGCEO Geog, E Lansing, MI 48823 USA. EM abraha@msu.edu RI Hamilton, Stephen/N-2979-2014; Chu, Housen/Q-6517-2016; Chen, Jiquan/D-1955-2009 OI Hamilton, Stephen/0000-0002-4702-9017; Chu, Housen/0000-0002-8131-4938; FU US Department of Energy's Great Lakes Bioenergy Research Center (DOE Office of Science) [DE-FC02-07ER64494]; US Department of Energy's Great Lakes Bioenergy Research Center (DOE Office of Energy Efficiency and Renewable Energy) [DE-AC05-76RL01830]; US National Science Foundation LTER Program [DEB 1027253]; MSU AgBioResearch FX Financial support for this research was provided by the US Department of Energy's Great Lakes Bioenergy Research Center (DOE Office of Science, DE-FC02-07ER64494 and DOE Office of Energy Efficiency and Renewable Energy, DE-AC05-76RL01830), the US National Science Foundation LTER Program (DEB 1027253), and MSU AgBioResearch. We also gratefully acknowledge assistances from M. Deal, C. Shao, J. Xu, and K. Kahmark for work on towers; S. VanderWulp and P. Jasrotia for field-related activities; and J. Bronson and J. Simmons for agronomic management. NR 67 TC 6 Z9 6 U1 2 U2 29 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1757-1693 EI 1757-1707 J9 GCB BIOENERGY JI GCB Bioenergy PD NOV PY 2015 VL 7 IS 6 BP 1344 EP 1356 DI 10.1111/gcbb.12239 PG 13 WC Agronomy; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA CT5FN UT WOS:000362834200014 ER PT J AU York, WS Urbanowicz, B Moremen, K Pena, MJ Smith, PJ Tuomivaara, S Wang, S Linin, V Alahuhta, P Crowley, M Himmel, M AF York, William S. Urbanowicz, Breeanna Moremen, Kelley Pena, Maria J. Smith, Peter J. Tuomivaara, Sami Wang, Shuo Linin, Vladimir Alahuhta, Petri Crowley, Michael Himmel, Michael TI Hemicellulose biosynthesis is becoming crystal clear SO GLYCOBIOLOGY LA English DT Meeting Abstract CT Annual Meeting of the Society-for-Glycobiology on Glycobiology - Accelerating Impact across the Biomedical Sciences CY DEC 01-04, 2015 CL San Francisco, CA SP Soc Glycobiol C1 [York, William S.; Urbanowicz, Breeanna; Moremen, Kelley; Pena, Maria J.; Smith, Peter J.; Tuomivaara, Sami; Wang, Shuo] Univ Georgia, Complex Carbohydrate Res Ctr, Athens, GA 30602 USA. [Linin, Vladimir; Alahuhta, Petri; Crowley, Michael; Himmel, Michael] Natl Renewable Energy Lab, Golden, CO USA. NR 0 TC 1 Z9 1 U1 0 U2 1 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 0959-6658 EI 1460-2423 J9 GLYCOBIOLOGY JI Glycobiology PD NOV PY 2015 VL 25 IS 11 MA 8 BP 1231 EP 1231 PG 1 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CT7JR UT WOS:000362991500014 ER PT J AU Ebert, B Rautengarten, C Liu, LF Pauly, M Orellana, A Heazlewood, JL Scheller, HV AF Ebert, Berit Rautengarten, Carsten Liu, Lifeng Pauly, Markus Orellana, Ariel Heazlewood, Joshua L. Scheller, Henrik V. TI Identification of the GDP-fucose transporter in plants SO GLYCOBIOLOGY LA English DT Meeting Abstract CT Annual Meeting of the Society-for-Glycobiology on Glycobiology - Accelerating Impact across the Biomedical Sciences CY DEC 01-04, 2015 CL San Francisco, CA SP Soc Glycobiol C1 [Ebert, Berit; Rautengarten, Carsten; Heazlewood, Joshua L.; Scheller, Henrik V.] Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, Phys Biosci Div, Berkeley, CA 94702 USA. [Ebert, Berit] Univ Copenhagen, Dept Plant & Environm Sci, DK-1871 Frederiksberg, Denmark. [Liu, Lifeng; Pauly, Markus; Scheller, Henrik V.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Rautengarten, Carsten; Heazlewood, Joshua L.] Univ Melbourne, Sch BioSci, ARC Ctr Excellence Plant Cell Walls, Melbourne, Vic 3010, Australia. [Orellana, Ariel] Univ Andres Bello, Fac Ciencias Biol, Ctr Biotecnol Vegetal, Santiago, Chile. RI Ebert, Berit/F-1856-2016; Pauly, Markus/B-5895-2008; Scheller, Henrik/A-8106-2008 OI Ebert, Berit/0000-0002-6914-5473; Pauly, Markus/0000-0002-3116-2198; Scheller, Henrik/0000-0002-6702-3560 NR 0 TC 0 Z9 0 U1 0 U2 2 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 0959-6658 EI 1460-2423 J9 GLYCOBIOLOGY JI Glycobiology PD NOV PY 2015 VL 25 IS 11 MA 104 BP 1263 EP 1263 PG 1 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CT7JR UT WOS:000362991500098 ER PT J AU Hu, LY Ramani, S Czako, R Sankaran, B Yu, Y Smith, DF Cummings, RD Estes, MK Prasad, BVV AF Hu, Liya Ramani, Sasirekha Czako, Rita Sankaran, Banumathi Yu, Ying Smith, David F. Cummings, Richard D. Estes, Mary K. Prasad, B. V. Venkataram TI Structural basis of unique glycan recognition in neonate-specific rotaviruses SO GLYCOBIOLOGY LA English DT Meeting Abstract CT Annual Meeting of the Society-for-Glycobiology on Glycobiology - Accelerating Impact across the Biomedical Sciences CY DEC 01-04, 2015 CL San Francisco, CA SP Soc Glycobiol C1 [Hu, Liya; Prasad, B. V. Venkataram] Baylor Coll Med, Verna & Marrs McLean Dept Biochem & Mol Biol, Houston, TX 77030 USA. [Ramani, Sasirekha; Czako, Rita; Estes, Mary K.; Prasad, B. V. Venkataram] Baylor Coll Med, Dept Mol Virol & Microbiol, Houston, TX 77030 USA. [Sankaran, Banumathi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley Ctr Struct Biol, Berkeley, CA 94720 USA. [Yu, Ying; Smith, David F.; Cummings, Richard D.] Emory Univ, Sch Med, Dept Biochem, Atlanta, GA 30322 USA. [Yu, Ying; Smith, David F.; Cummings, Richard D.] Emory Univ, Sch Med, Natl Ctr Funct Glyc, Atlanta, GA 30322 USA. NR 0 TC 0 Z9 0 U1 1 U2 1 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 0959-6658 EI 1460-2423 J9 GLYCOBIOLOGY JI Glycobiology PD NOV PY 2015 VL 25 IS 11 MA 109 BP 1264 EP 1265 PG 2 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CT7JR UT WOS:000362991500103 ER PT J AU Mortimer, JC Ishikawa, T Fang, L Jing, BB Rennie, E Inada, N Yu, XL Lao, J Demura, T Kawai-Yamada, M Scheller, H Dupree, P AF Mortimer, Jenny C. Ishikawa, Toshiki Fang, Lin Jing, Beibei Rennie, Emilie Inada, Noriko Yu, Xiaolan Lao, Jeemeng Demura, Taku Kawai-Yamada, Maki Scheller, Henrik Dupree, Paul TI Glycosylated sphingolipid biosynthesis and function in Arabidopsis SO GLYCOBIOLOGY LA English DT Meeting Abstract CT Annual Meeting of the Society-for-Glycobiology on Glycobiology - Accelerating Impact across the Biomedical Sciences CY DEC 01-04, 2015 CL San Francisco, CA SP Soc Glycobiol C1 [Mortimer, Jenny C.; Fang, Lin; Jing, Beibei; Rennie, Emilie; Lao, Jeemeng; Scheller, Henrik] LBNL, Joint BioEnergy Inst, Berkeley, CA USA. [Ishikawa, Toshiki; Kawai-Yamada, Maki] Saitama Univ, Saitama, Japan. [Inada, Noriko; Demura, Taku] NAIST, Nara, Japan. [Mortimer, Jenny C.; Yu, Xiaolan; Dupree, Paul] Univ Cambridge, Cambridge CB2 1TN, England. [Mortimer, Jenny C.; Demura, Taku] RIKEN Yokohama, Yokohama, Kanagawa, Japan. RI Scheller, Henrik/A-8106-2008 OI Scheller, Henrik/0000-0002-6702-3560 NR 2 TC 0 Z9 0 U1 0 U2 1 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 0959-6658 EI 1460-2423 J9 GLYCOBIOLOGY JI Glycobiology PD NOV PY 2015 VL 25 IS 11 MA 114 BP 1266 EP 1267 PG 2 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CT7JR UT WOS:000362991500108 ER PT J AU Huang, XH Schurman, N Handa, K Hakomori, SI AF Huang, Xiaohua Schurman, Nathan Handa, Kazuko Hakomori, Sen-Itiroh TI Glycosphingolipids involved in contact inhibition of WI38 cell growth SO GLYCOBIOLOGY LA English DT Meeting Abstract CT Annual Meeting of the Society-for-Glycobiology on Glycobiology - Accelerating Impact across the Biomedical Sciences CY DEC 01-04, 2015 CL San Francisco, CA SP Soc Glycobiol C1 [Huang, Xiaohua; Schurman, Nathan; Handa, Kazuko; Hakomori, Sen-Itiroh] Pacific Northwest Res Inst, Div Biomembrane Res, Seattle, WA USA. [Hakomori, Sen-Itiroh] Univ Washington, Dept Pathobiol, Seattle, WA 98195 USA. [Hakomori, Sen-Itiroh] Univ Washington, Dept Global Hlth, Seattle, WA 98195 USA. NR 0 TC 0 Z9 0 U1 1 U2 1 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 0959-6658 EI 1460-2423 J9 GLYCOBIOLOGY JI Glycobiology PD NOV PY 2015 VL 25 IS 11 MA 208 BP 1302 EP 1302 PG 1 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CT7JR UT WOS:000362991500202 ER PT J AU Cordeddu, V Yin, JC Gunnarsson, C Virtanen, C Drunat, S Lepri, F De Luca, A Rossi, C Ciolfi, A Pugh, TJ Bruselles, A Priest, JR Pennacchio, LA Lu, Z Danesh, A Quevedo, R Hamid, A Martinelli, S Pantaleoni, F Gnazzo, M Daniele, P Lissewski, C Bocchinfuso, G Stella, L Odent, S Philip, N Faivre, L Vlckova, M Seemanova, E Digilio, C Zenker, M Zampino, G Verloes, A Dallapiccola, B Roberts, AE Cave, H Gelb, BD Neel, BG Tartaglia, M AF Cordeddu, Viviana Yin, Jiani C. Gunnarsson, Cecilia Virtanen, Carl Drunat, Severine Lepri, Francesca De Luca, Alessandro Rossi, Cesare Ciolfi, Andrea Pugh, Trevor J. Bruselles, Alessandro Priest, James R. Pennacchio, Len A. Lu, Zhibin Danesh, Arnavaz Quevedo, Rene Hamid, Alaa Martinelli, Simone Pantaleoni, Francesca Gnazzo, Maria Daniele, Paola Lissewski, Christina Bocchinfuso, Gianfranco Stella, Lorenzo Odent, Sylvie Philip, Nicole Faivre, Laurence Vlckova, Marketa Seemanova, Eva Digilio, Cristina Zenker, Martin Zampino, Giuseppe Verloes, Alain Dallapiccola, Bruno Roberts, Amy E. Cave, Helene Gelb, Bruce D. Neel, Benjamin G. Tartaglia, Marco TI Activating Mutations Affecting the Dbl Homology Domain of SOS2 Cause Noonan Syndrome SO HUMAN MUTATION LA English DT Article DE genotype-phenotype correlations; Noonan syndrome; RAS signaling; SOS2 ID OF-FUNCTION MUTATIONS; DNA-SEQUENCING DATA; EXCHANGE FACTORS; RAF1 MUTATIONS; RARE VARIANTS; RAS; FRAMEWORK; SPECTRUM; AUTOINHIBITION; SEVENLESS AB The RASopathies constitute a family of autosomal-dominant disorders whose major features include facial dysmorphism, cardiac defects, reduced postnatal growth, variable cognitive deficits, ectodermal and skeletal anomalies, and susceptibility to certain malignancies. Noonan syndrome (NS), the commonest RASopathy, is genetically heterogeneous and caused by functional dysregulation of signal transducers and regulatory proteins with roles in the RAS/extracellular signal-regulated kinase (ERK) signal transduction pathway. Mutations in known disease genes account for approximately 80% of affected individuals. Here, we report that missense mutations altering Son of Sevenless, Drosophila, homolog 2 (SOS2), which encodes a RAS guanine nucleotide exchange factor, occur in a small percentage of subjects with NS. Four missense mutations were identified in five unrelated sporadic cases and families transmitting NS. Disease-causing mutations affected three conserved residues located in the Dbl homology (DH) domain, of which two are directly involved in the intramolecular binding network maintaining SOS2 in its autoinhibited conformation. All mutations were found to promote enhanced signaling from RAS to ERK. Similar to NS-causing SOS1 mutations, the phenotype associated with SOS2 defects is characterized by normal development and growth, as well as marked ectodermal involvement. Unlike SOS1 mutations, however, those in SOS2 are restricted to the DH domain. C1 [Cordeddu, Viviana; Ciolfi, Andrea; Bruselles, Alessandro; Martinelli, Simone; Pantaleoni, Francesca; Tartaglia, Marco] Ist Super Sanita, Dipartimento Ematol Oncol & Med Mol, I-00161 Rome, Italy. [Cordeddu, Viviana] Univ G dAnnunzio, Dipartimento Sci Psicol Salute & Terr, I-66100 Chieti, Italy. [Yin, Jiani C.; Virtanen, Carl; Pugh, Trevor J.; Lu, Zhibin; Danesh, Arnavaz; Quevedo, Rene; Hamid, Alaa; Neel, Benjamin G.] Univ Toronto, Univ Hlth Network, Princess Margaret Canc Ctr, Toronto, ON M5S, Canada. [Yin, Jiani C.; Virtanen, Carl; Pugh, Trevor J.; Lu, Zhibin; Danesh, Arnavaz; Quevedo, Rene; Hamid, Alaa; Neel, Benjamin G.] Univ Toronto, Dept Med Biophys, Toronto, ON M5S, Canada. [Gunnarsson, Cecilia] Linkoping Univ, Fac Hlth Sci, Div Clin Genet, Dept Clin & Expt Med, S-58183 Linkoping, Sweden. [Drunat, Severine; Verloes, Alain; Cave, Helene] Hop Robert Debre, Dept Genet, F-75019 Paris, France. [Lepri, Francesca; Gnazzo, Maria; Digilio, Cristina; Dallapiccola, Bruno; Tartaglia, Marco] Bambino Gesu Pediat Hosp, Ist Ricovero & Cura Carattere Sci, I-00165 Rome, Italy. [De Luca, Alessandro; Daniele, Paola] Casa Sollievo Sofferenza Hosp, Mendel Inst, IRCCS, I-00161 Rome, Italy. [Rossi, Cesare] St Orsola Marcello Malpighi Hosp, UO Genet Med, I-40138 Bologna, Italy. [Priest, James R.] Stanford Univ, Sch Med, Div Pediat Cardiol, Stanford, CA 94305 USA. [Priest, James R.] Stanford Univ, Sch Med, Stanford Cardiovasc Inst, Child Hlth Res Inst, Stanford, CA 94305 USA. [Pennacchio, Len A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Genom Div, Berkeley, CA 94720 USA. [Pennacchio, Len A.] US Dept Energy Joint Genome Inst, Walnut Creek, CA 94598 USA. [Lissewski, Christina; Zenker, Martin] Otto von Guericke Univ, Univ Hosp Magdeburg, Inst Human Genet, D-39106 Magdeburg, Germany. [Bocchinfuso, Gianfranco; Stella, Lorenzo] Univ Roma Tor Vergata, Dipartimento Sci & Tecnol Chim, I-00133 Rome, Italy. [Odent, Sylvie] Hop SUD, Serv Genet Clin, F-35200 Rennes, France. [Philip, Nicole] Hop Enfants la Timone, Dept Med Genet, F-13385 Marseille, France. [Faivre, Laurence] Hop Enfants, Ctr Genet, F-21000 Dijon, France. [Vlckova, Marketa; Seemanova, Eva] Charles Univ Prague, Fac Med 2, Dept Biol & Med Genet, Prague 15006, Czech Republic. [Vlckova, Marketa; Seemanova, Eva] Univ Hosp Motol, Prague 15006, Czech Republic. [Zampino, Giuseppe] Univ Cattolica Sacro Cuore, Ist Pediat, I-00168 Rome, Italy. [Roberts, Amy E.] Boston Childrens Hosp, Dept Cardiol, Boston, MA 02115 USA. [Roberts, Amy E.] Boston Childrens Hosp, Div Genet, Boston, MA 02115 USA. [Cave, Helene] Univ Paris Diderot, Sorbonne Paris Cite, Inst Univ Hematol, INSERM,UMR S1131, F-75205 Paris, France. [Gelb, Bruce D.] Icahn Sch Med Mt Sinai, Mindich Child Hlth & Dev Inst, New York, NY 10029 USA. [Gelb, Bruce D.] Icahn Sch Med Mt Sinai, Dept Pediat, New York, NY 10029 USA. [Gelb, Bruce D.] Icahn Sch Med Mt Sinai, Dept Genet & Genom Sci, New York, NY 10029 USA. [Neel, Benjamin G.] NYU, Sch Med, Laura & Isaac Perlmutter Canc Ctr, New York, NY 10016 USA. RP Neel, BG (reprint author), NYU, Sch Med, Laura & Isaac Perlmutter Canc Ctr, New York, NY 10016 USA. EM bruce.gelb@mssm.edu; Ben-jamin.Neel@nyumc.org; marco.tartaglia@iss.it RI Stella, Lorenzo/A-7996-2010; Philip, Nicole/I-2881-2016; Dallapiccola, Bruno/K-8692-2016; OI Stella, Lorenzo/0000-0002-5489-7381; Lepri, Francesca Romana/0000-0001-5331-0473; Dallapiccola, Bruno/0000-0002-5031-1013; Bocchinfuso, Gianfranco/0000-0002-5556-7691; Tartaglia, Marco/0000-0001-7736-9672 FU National Institutes of Health [R01 HL071207, R01 HL0832732, U01 DE020060, R01 HG003988, U54 HG006997, U54 HG006504]; Telethon-Italy [GGP13107]; AIRC [IG 13360]; Ministry of Health [RF-2011-02349938]; Princess Margaret Cancer Foundation; Ontario Ministry of Health and Long Term Care; CIHR CGS-D FX Contract grant sponsors: National Institutes of Health (R01 HL071207; R01 HL0832732; U01 DE020060, R01 HG003988, and U54 HG006997; U54 HG006504); Telethon-Italy (GGP13107); AIRC (IG 13360); Ministry of Health (RF-2011-02349938); Princess Margaret Cancer Foundation and the Ontario Ministry of Health and Long Term Care; CIHR CGS-D. NR 32 TC 9 Z9 9 U1 2 U2 9 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1059-7794 EI 1098-1004 J9 HUM MUTAT JI Hum. Mutat. PD NOV PY 2015 VL 36 IS 11 BP 1080 EP 1087 DI 10.1002/humu.22834 PG 8 WC Genetics & Heredity SC Genetics & Heredity GA CT7JQ UT WOS:000362991400011 PM 26173643 ER PT J AU Scogland, TRW Feng, WC Rountree, B de Supinski, BR AF Scogland, Thomas R. W. Feng, Wu-Chun Rountree, Barry de Supinski, Bronis R. TI CoreTSAR: Core Task-Size Adapting Runtime SO IEEE TRANSACTIONS ON PARALLEL AND DISTRIBUTED SYSTEMS LA English DT Article DE Heterogeneous; OpenMP; OpenACC; GPU; coscheduling AB Heterogeneity continues to increase at all levels of computing, with the rise of accelerators such as GPUs, FPGAs, and other co-processors into everything from desktops to supercomputers. As a consequence, efficiently managing such disparate resources has become increasingly complex. CoreTSAR seeks to reduce this complexity by adaptively worksharing parallel-loop regions across compute resources without requiring any transformation of the code within the loop. Our results show performance improvements of up to three-fold over a current state-of-the-art heterogeneous task scheduler as well as linear performance scaling from a single GPU to four GPUs for many codes. In addition, CoreTSAR demonstrates a robust ability to adapt to both a variety of workloads and underlying system configurations. C1 [Scogland, Thomas R. W.; Feng, Wu-Chun] Virginia Tech, Dept Comp Sci, Blacksburg, VA 24060 USA. [Rountree, Barry; de Supinski, Bronis R.] Lawrence Livermore Natl Lab, Ctr Appl Sci Comp, Livermore, CA 94551 USA. RP Scogland, TRW (reprint author), Virginia Tech, Dept Comp Sci, Blacksburg, VA 24060 USA. EM tom.scogland@vt.edu; wfeng@vt.edu; rountree@llnl.gov; bronis@llnl.gov FU US Department of Energy's Lawrence Livermore National Laboratory; Office of Science [DE-AC52-07NA27344]; Office of Advanced Scientific Computing Research [LLNL-JRNL-662817]; Air Force Office of Scientific Research (AFOSR) Computational Mathematics Program [FA9550-12-1-0442]; NSF Center for High-Performance Reconfigurable Computing (CHREC) [NSF I/UCRC IIP-1266245]; DoD National Defense Science & Engineering Graduate Fellowship (NDSEG) FX This material is based upon work supported by the US Department of Energy's Lawrence Livermore National Laboratory; Office of Science, under Award number DE-AC52-07NA27344; Office of Advanced Scientific Computing Research (LLNL-JRNL-662817); the Air Force Office of Scientific Research (AFOSR) Computational Mathematics Program via Grant No. FA9550-12-1-0442; NSF I/UCRC IIP-1266245 via the NSF Center for High-Performance Reconfigurable Computing (CHREC); and a DoD National Defense Science & Engineering Graduate Fellowship (NDSEG). NR 20 TC 0 Z9 0 U1 1 U2 1 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 1045-9219 EI 1558-2183 J9 IEEE T PARALL DISTR JI IEEE Trans. Parallel Distrib. Syst. PD NOV PY 2015 VL 26 IS 11 BP 2970 EP 2983 DI 10.1109/TPDS.2014.2365192 PG 14 WC Computer Science, Theory & Methods; Engineering, Electrical & Electronic SC Computer Science; Engineering GA CT4QQ UT WOS:000362792200006 ER PT J AU Tak, T Choe, J Jeong, Y Lee, D Kim, TK Hong, SG AF Tak, Taewoo Choe, Jiwon Jeong, Yongjin Lee, Deokjung Kim, T. K. Hong, Ser Gi TI Feasibility study on ultralong-cycle operation and material performance for compact liquid metal-cooled fast reactors: a review work SO INTERNATIONAL JOURNAL OF ENERGY RESEARCH LA English DT Review DE LMR; SMR; long-cycle operation; breed-and-burn; material performance ID FAST BREEDER-REACTORS; FUEL AB This paper reviews the feasibility of ultralong-cycle operation on a compact liquid metal-cooled fast reactor (LMR) firstly by assessing the operation of a long-life fast reactor core and secondly by evaluating material performance in respect to both long-cycle operation and compact-size fast reactor. Many kinds of reactor concepts have been proposed, and LMR and small modular reactor (SMR) are the issued leading technologies for generation four (Gen-IV) reactor system development. The breed-and-burn strategy was proposed as a core burning strategy to operate a long cycle, and it has been evaluated in this paper with two reactor concepts: constant axial shape of neutron flux, nuclide densities, and power shape during life of energy and ultralong cycle fast reactor. In addition, Super-Safe, Small, and Simple and small modular fast reactor, compact LMR concepts, have been simulated to evaluate their long-life operation strategies. For the other practical issues, the materials for fuel, coolant, and structure have been identified and some of them are selected to have their performance optimized specifically for compact LMR with a long-cycle operation. It is believed that this comprehensive review will propose a proper direction for future reactor development and will be followed by the next step research for a complete reactor model with the other reactor components. Copyright (c) 2015 John Wiley & Sons, Ltd. C1 [Tak, Taewoo; Choe, Jiwon; Jeong, Yongjin; Lee, Deokjung] Ulsan Natl Inst Sci & Technol, Ulsan 689798, South Korea. [Kim, T. K.] Argonne Natl Lab, Lemont, IL 60564 USA. [Hong, Ser Gi] Kyung Hee Univ, Yongin 446701, Gyeonggi Do, South Korea. RP Lee, D (reprint author), Ulsan Natl Inst Sci & Technol, UNIST Gil 50, Ulsan 689798, South Korea. EM deokjung@unist.ac.kr OI Tak, Taewoo/0000-0002-3230-8080 FU National Research Foundation of Korea - Korean government (MSIP) FX This work was supported by a National Research Foundation of Korea grant funded by the Korean government (MSIP). NR 40 TC 3 Z9 3 U1 2 U2 4 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0363-907X EI 1099-114X J9 INT J ENERG RES JI Int. J. Energy Res. PD NOV PY 2015 VL 39 IS 14 BP 1859 EP 1878 DI 10.1002/er.3384 PG 20 WC Energy & Fuels; Nuclear Science & Technology SC Energy & Fuels; Nuclear Science & Technology GA CT5YH UT WOS:000362886500001 ER PT J AU Ibtesham, D Ferreira, KB Arnold, D AF Ibtesham, Dewan Ferreira, Kurt B. Arnold, Dorian TI A checkpoint compression study for high-performance computing systems SO INTERNATIONAL JOURNAL OF HIGH PERFORMANCE COMPUTING APPLICATIONS LA English DT Article DE Fault tolerance; checkpoint; restart; checkpoint compression AB As high-performance computing systems continue to increase in size and complexity, higher failure rates and increased overheads for checkpoint/restart (CR) protocols have raised concerns about the practical viability of CR protocols for future systems. Previously, compression has proven to be a viable approach for reducing checkpoint data volumes and, thereby, reducing CR protocol overhead leading to improved application performance. In this article, we further explore compression-based CR optimization by exploring its baseline performance and scaling properties, evaluating whether improved compression algorithms might lead to even better application performance and comparing checkpoint compression against and alongside other software- and hardware-based optimizations. Our results highlights are that: (1) compression is a very viable CR optimization; (2) generic, text-based compression algorithms appear to perform near optimally for checkpoint data compression and faster compression algorithms will not lead to better application performance; (3) compression-based optimizations fare well against and alongside other software-based optimizations; and (4) while hardware-based optimizations outperform software-based ones, they are not as cost effective. C1 [Ibtesham, Dewan; Arnold, Dorian] Univ New Mexico, Dept Comp Sci, Albuquerque, NM 87131 USA. [Ferreira, Kurt B.] Sandia Natl Labs, Scalable Syst Software Dept, Albuquerque, NM USA. RP Arnold, D (reprint author), Univ New Mexico, Dept Comp Sci, 1 Univ New Mexico,MSC01 1130, Albuquerque, NM 87131 USA. EM darnold@cs.unm.edu FU Sandia National Laboratories [1017357, 1200640, 1321008] FX This work was supported in part by Sandia National Laboratories subcontracts 1017357, 1200640 and 1321008. NR 42 TC 0 Z9 0 U1 2 U2 2 PU SAGE PUBLICATIONS LTD PI LONDON PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND SN 1094-3420 EI 1741-2846 J9 INT J HIGH PERFORM C JI Int. J. High Perform. Comput. Appl. PD NOV PY 2015 VL 29 IS 4 SI SI BP 387 EP 402 DI 10.1177/1094342015570921 PG 16 WC Computer Science, Hardware & Architecture; Computer Science, Interdisciplinary Applications; Computer Science, Theory & Methods SC Computer Science GA CT7LR UT WOS:000362996700001 ER PT J AU Ardeljan, M Knezevic, M Nizolek, T Beyerlein, IJ Mara, NA Pollock, TM AF Ardeljan, Milan Knezevic, Marko Nizolek, Thomas Beyerlein, Irene J. Mara, Nathan A. Pollock, Tresa M. TI A study of microstructure-driven strain localizations in two-phase polycrystalline HCP/BCC composites using a multi-scale model SO INTERNATIONAL JOURNAL OF PLASTICITY LA English DT Article DE Microstructures; Crystal plasticity; Finite elements; Dislocations; Shear banding ID ADIABATIC SHEAR BANDS; CRYSTAL PLASTICITY FEM; CRYSTALLOGRAPHIC TEXTURE EVOLUTION; IMPLICIT FINITE-ELEMENTS; METAL-MATRIX COMPOSITES; PRESSURE-DOUBLE-TORSION; STACKING-FAULT ENERGY; CLOSE-PACKED METALS; ULTRA-HIGH STRENGTH; X-RAY-DIFFRACTION AB In this work, we present a 3D microstructure-based, full-field crystal plasticity finite element (CPFE) model using a thermally activated dislocation-density based constitutive description and apply it to study the deformation of a two-phase hexagonal close packed (HCP)-body center cubic (BCC) Zr/Nb composite. The microstructure models were created using a synthetic grain structure builder (DREAM.3D) and a meshing toolset for the 3D network of grains, grain boundaries, and bimetal interfaces. The crystal orientations, grain shapes, and grain sizes for each phase were initialized based on the measured data. With this novel technique, we aspire to couple the evolution of microstructural heterogeneities with the evolution of spatially resolved mechanical fields during the deformation of complex composites. Here, we apply it to understand the role that microstructure plays in the development of the local concentrations in strain and strain rate that can trigger plastic instabilities, such as shear banding. Our chief findings are that 1) local areas of relatively high (and relatively very low) strain concentration occur at triple junctions or quadruple points and then connect via straining to create a banded configuration that extends across the polycrystalline layer, 2) this event starts in the Zr phase and not in the Nb phase, and 3) the triggering hot spots in strain occur at junctions that join grains with very dissimilar reorientation propensities and vice versa for cold spots. In order to determine how such influential localizations can be prevented during processing via application of intermediate annealing treatments, we used the model to also explore the effects of annealing-induced changes in accumulated dislocation density, crystallographic texture and grain shape on the development of strain localizations during subsequent deformation. We found that while it is difficult to avoid strain localizations at grain junctions, when provided a microstructure containing a few large grains spanning the thickness, elongated grain shapes, and reduced dislocation density, the linkage of hot spots in the form of a band can be postponed. At the end we show that when an additional softening mechanism is introduced, these localized strain concentration areas can lead to shear bands. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Ardeljan, Milan; Knezevic, Marko] Univ New Hampshire, Dept Mech Engn, Durham, NH 03824 USA. [Nizolek, Thomas; Pollock, Tresa M.] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. [Beyerlein, Irene J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Mara, Nathan A.] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. RP Knezevic, M (reprint author), Univ New Hampshire, Dept Mech Engn, 33 Acad Way,Kingsbury Hall,W119, Durham, NH 03824 USA. EM marko.knezevic@unh.edu RI Beyerlein, Irene/A-4676-2011 FU Los Alamos National Laboratory [277871]; UC Lab Fees Research Program [UCD-12-0045.15]; Department of Defense (DoD) through the National Defense Science & Engineering Graduate Fellowship (NDSEG) Program FX MK and MA acknowledge subcontract, NO. 277871, granted by Los Alamos National Laboratory to the University of New Hampshire. IJB, TMP, and NAM wish to acknowledge support by the UC Lab Fees Research Program # UCD-12-0045.15. TN was supported by the Department of Defense (DoD) through the National Defense Science & Engineering Graduate Fellowship (NDSEG) Program. NR 139 TC 21 Z9 21 U1 14 U2 55 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0749-6419 EI 1879-2154 J9 INT J PLASTICITY JI Int. J. Plast. PD NOV PY 2015 VL 74 BP 35 EP 57 DI 10.1016/j.ijplas.2015.06.003 PG 23 WC Engineering, Mechanical; Materials Science, Multidisciplinary; Mechanics SC Engineering; Materials Science; Mechanics GA CT6KS UT WOS:000362922500003 ER PT J AU Bodelot, L Escobedo-Diaz, JP Trujillo, CP Martinez, DT Cerreta, EK Gray, GT Ravichandran, G AF Bodelot, Laurence Escobedo-Diaz, Juan P. Trujillo, Carl P. Martinez, Daniel T. Cerreta, Ellen K. Gray, George T., III Ravichandran, Guruswami TI Microstructural changes and in-situ observation of localization in OFHC copper under dynamic loading SO INTERNATIONAL JOURNAL OF PLASTICITY LA English DT Article DE Dynamics; Polycrystalline material; Electron microscopy; Kolsky bar; Ultra-high-speed imaging ID ADIABATIC SHEAR BANDS; VIRTUAL FIELDS METHOD; HIGH-STRAIN RATES; COMPRESSION SPECIMEN; STAINLESS-STEEL; NUMERICAL VALIDATION; MECHANICAL RESPONSE; GRAIN-SIZE; WIDE-RANGE; BEHAVIOR AB In this paper, we introduce an original experimental protocol that couples microstructural analyses before and after deformation to in-situ grain scale strain measurements in OFHC copper samples during dynamic loading. This analysis is conducted on a modified shear compression specimen (SCS) that exhibits localization within a flat gage section and hence lends itself to ultra-high-speed imaging of the localization evolution. We were thus able to study the influence of the microstructure on strain localization as well as the process of localization in OFHC copper submitted to high-strain rate loading at different rates. We found that in the case of these modified perforated SCS samples, the early stages of localization were geometry driven while grain size and strain-rate dependency only emerged later. For the two smallest grain sizes examined here, a stronger strain-rate dependency was observed. This led to a narrower and more elongated localization of the highest strains at the local scale and to a concurrent harder macroscopic response at higher strain rate. For the largest grain size examined here, the macroscopic response was nearly identical at both strain rates but largely softer than for the smaller grain sizes. This translated into a wider localization pattern in the local strain fields compensating for lower values of maximum local strain. Texture evolution was strongly grain-size-dependent as smaller grain-size samples showed very mild lattice rotation accompanied with dynamic recrystallization into smaller grains, while the large grain-size samples showed a marked texture formation accompanied with both grain growth and stress relaxation phenomena. The introduced experimental protocol can thus give access to data providing new insight into microstructural aspects of localization under dynamic loading; such data is additionally relevant for validating multiscale or crystal plasticity models for dynamic applications. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Bodelot, Laurence; Ravichandran, Guruswami] CALTECH, Grad Aerosp Labs, Pasadena, CA 91125 USA. [Escobedo-Diaz, Juan P.; Trujillo, Carl P.; Martinez, Daniel T.; Cerreta, Ellen K.; Gray, George T., III] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Bodelot, Laurence] Ecole Polytech, Lab Mecan Solides, F-91128 Palaiseau, France. [Escobedo-Diaz, Juan P.] UNSW Australia, Canberra, ACT 2610, Australia. RP Bodelot, L (reprint author), Ecole Polytech, Lab Mecan Solides, Route Saclay, F-91128 Palaiseau, France. EM laurence.bodelot@polytechnique.edu OI Escobedo-Diaz, Juan/0000-0003-2413-7119 FU Department of Energy National Nuclear Security Administration [DE-FC52-08NA28613] FX This paper is based upon work supported by the Department of Energy National Nuclear Security Administration under Award Number DE-FC52-08NA28613, which is gratefully acknowledged. The authors thank Brad St. John, Joe Haggerty and Ali Kiani from GALCIT for machining the SCS samples, as well as Mike Lopez from MST-8 Division in LANL for his technical advice. LB and CT also acknowledge the support of Todd Rumbaugh from Highland Imaging for providing the Shimadzu camera. NR 46 TC 3 Z9 3 U1 3 U2 20 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0749-6419 EI 1879-2154 J9 INT J PLASTICITY JI Int. J. Plast. PD NOV PY 2015 VL 74 BP 58 EP 74 DI 10.1016/j.ijplas.2015.06.002 PG 17 WC Engineering, Mechanical; Materials Science, Multidisciplinary; Mechanics SC Engineering; Materials Science; Mechanics GA CT6KS UT WOS:000362922500004 ER PT J AU Cuevas-Maraver, J Khare, A Kevrekidis, PG Xu, HT Saxena, A AF Cuevas-Maraver, Jesus Khare, Avinash Kevrekidis, Panayotis G. Xu, Haitao Saxena, Avadh TI PT-Symmetric Dimer in a Generalized Model of Coupled Nonlinear Oscillators SO INTERNATIONAL JOURNAL OF THEORETICAL PHYSICS LA English DT Article DE Oscillators; PT-symmetry; Stability; Periodic orbits ID WAVE-GUIDE; LATTICES; STABILITY; GAIN AB In the present work, we explore the case of a general -symmetric dimer in the context of two both linearly and nonlinearly coupled cubic oscillators. To obtain an analytical handle on the system, we first explore the rotating wave approximation converting it into a discrete nonlinear Schrodinger type dimer. In the latter context, the stationary solutions and their stability are identified numerically but also wherever possible analytically. Solutions stemming from both symmetric and anti-symmetric special limits are identified. A number of special cases are explored regarding the ratio of coefficients of nonlinearity between oscillators over the intrinsic one of each oscillator. Finally, the considerations are extended to the original oscillator model, where periodic orbits and their stability are obtained. When the solutions are found to be unstable their dynamics is monitored by means of direct numerical simulations. C1 [Cuevas-Maraver, Jesus] Univ Seville, Escuela Politecn Super, Dept Fis Aplicada 1, Nonlinear Phys Grp, Seville 41011, Spain. [Cuevas-Maraver, Jesus] Univ Seville, Inst Matemat, E-41012 Seville, Spain. [Khare, Avinash] IISER, Pune 411008, Maharashtra, India. [Kevrekidis, Panayotis G.; Xu, Haitao] Univ Massachusetts, Dept Math & Stat, Amherst, MA 01003 USA. [Saxena, Avadh] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Saxena, Avadh] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Cuevas-Maraver, J (reprint author), Univ Seville, Escuela Politecn Super, Dept Fis Aplicada 1, Nonlinear Phys Grp, C Virgen de Africa 7, Seville 41011, Spain. EM jcuevas@us.es RI Cuevas-Maraver, Jesus/A-1255-2008 OI Cuevas-Maraver, Jesus/0000-0002-7162-5759 FU National Science Foundation [CMMI-1000337, DMS-1312856]; FP7-People [IRSES-605096]; US-AFOSR [FA9550-12-10332]; Binational (US-Israel) Science Foundation [2010239]; U.S. Department of Energy; Dept. of Atomic Energy, Govt. of India through a Raja Ramanna Fellowship FX P.G.K. acknowledges support from the National Science Foundation under grants CMMI-1000337, DMS-1312856, from FP7-People under grant IRSES-605096, from the US-AFOSR under grant FA9550-12-10332 and from the Binational (US-Israel) Science Foundation through grant 2010239. This work was supported in part by the U.S. Department of Energy. A.K. acknowledges financial support from Dept. of Atomic Energy, Govt. of India through a Raja Ramanna Fellowship. P.G.K. also acknowledges useful discussions with Igor Barashenkov. NR 44 TC 1 Z9 1 U1 1 U2 10 PU SPRINGER/PLENUM PUBLISHERS PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0020-7748 EI 1572-9575 J9 INT J THEOR PHYS JI Int. J. Theor. Phys. PD NOV PY 2015 VL 54 IS 11 BP 3960 EP 3985 DI 10.1007/s10773-014-2429-6 PG 26 WC Physics, Multidisciplinary SC Physics GA CT5ZI UT WOS:000362889400011 ER PT J AU Childs, BC Poineau, F Czerwinski, KR Sattelberger, AP AF Childs, Bradley C. Poineau, Frederic Czerwinski, Kenneth R. Sattelberger, Alfred P. TI The nature of the volatile technetium species formed during vitrification of borosilicate glass SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article DE Technetium; Volatile; Red; Vitrification; X-ray absorbance spectroscopy ID RAY-ABSORPTION SPECTROSCOPY; FINE-STRUCTURE; WASTE GLASS; RHENIUM; OXIDE AB Vitrification of sodium pertechnetate into borosilicate glass was performed in air at 1100 degrees C. A glass with a composition similar to the one developed for vitrification of the low activity waste at the Hanford site was used. A red volatile species was observed above 600 degrees C. The extended X-ray absorption fine structure results indicate the environment of the absorbing Tc atom consists of 2.9(6) O atoms at 1.73(2) angstrom, 2.2(4) O atoms at 2.02(2) angstrom, and 0.8(2) O atoms at 2.18(2) angstrom. The results are consistent with the presence of a mononuclear species with a structure closely related to TcO3(OH)(H2O)(2). C1 [Childs, Bradley C.; Poineau, Frederic; Czerwinski, Kenneth R.; Sattelberger, Alfred P.] Univ Nevada, Dept Chem, Las Vegas, NV 89154 USA. [Sattelberger, Alfred P.] Argonne Natl Lab, Energy Engn & Syst Anal Directorate, Lemont, IL 60439 USA. RP Childs, BC (reprint author), Univ Nevada, Dept Chem, Las Vegas, NV 89154 USA. EM childsb2@unlv.nevada.edu FU U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX Use of the Advanced Photon Source at Argonne was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. The authors thank Trevor Low, and Julie Bertoia for outstanding health physics support and Dr. Sungsik Lee at the APS for support during XAS experiments. NR 18 TC 4 Z9 4 U1 4 U2 13 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD NOV PY 2015 VL 306 IS 2 BP 417 EP 421 DI 10.1007/s10967-015-4203-5 PG 5 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA CT6XW UT WOS:000362957900010 ER PT J AU Wasserman, G Archibald, R Gelb, A AF Wasserman, Gabriel Archibald, Rick Gelb, Anne TI Image Reconstruction from Fourier Data Using Sparsity of Edges SO JOURNAL OF SCIENTIFIC COMPUTING LA English DT Article DE Fourier data; Edge detection; l(1) regularization; Polynomial annihilation; Convex optimization ID EQUATIONS; BASES; MRI AB Data of piecewise smooth images are sometimes acquired as Fourier samples. Standard reconstruction techniques yield the Gibbs phenomenon, causing spurious oscillations at jump discontinuities and an overall reduced rate of convergence to first order away from the jumps. Filtering is an inexpensive way to improve the rate of convergence away from the discontinuities, but it has the adverse side effect of blurring the approximation at the jump locations. On the flip side, high resolution post processing algorithms are often computationally cost prohibitive and also require explicit knowledge of all jump locations. Recent convex optimization algorithms using regularization exploit the expected sparsity of some features of the image. Wavelets or finite differences are often used to generate the corresponding sparsifying transform and work well for piecewise constant images. They are less useful when there is more variation in the image, however. In this paper we develop a convex optimization algorithm that exploits the sparsity in the edges of the underlying image. We use the polynomial annihilation edge detection method to generate the corresponding sparsifying transform. Our method successfully reduces the Gibbs phenomenon with only minimal blurring at the discontinuities while retaining a high rate of convergence in smooth regions. C1 [Wasserman, Gabriel; Gelb, Anne] Arizona State Univ, Sch Math & Stat Sci, Tempe, AZ 85287 USA. [Archibald, Rick] Oak Ridge Natl Lab, Div Math & Comp Sci, Oak Ridge, TN 37831 USA. RP Gelb, A (reprint author), Arizona State Univ, Sch Math & Stat Sci, Tempe, AZ 85287 USA. EM gabriel.wasserman@asu.edu; archibaldrk@ornl.gov; anne.gelb@asu.edu RI Archibald, Rick/I-6238-2016 OI Archibald, Rick/0000-0002-4538-9780 FU U.S. Government [DE-AC05-00OR22725] FX The submitted manuscript has been authored in part by contractors [UT-Battelle LLC, manager of Oak Ridge National Laboratory (ORNL)] of the U.S. Government under Contract No. DE-AC05-00OR22725. Accordingly, the U.S. Government retains a non-exclusive, royalty-free license to publish or reproduce the published form of this contribution, or allow others to do so, for U.S. Government purposes. NR 14 TC 1 Z9 1 U1 0 U2 8 PU SPRINGER/PLENUM PUBLISHERS PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0885-7474 EI 1573-7691 J9 J SCI COMPUT JI J. Sci. Comput. PD NOV PY 2015 VL 65 IS 2 BP 533 EP 552 DI 10.1007/s10915-014-9973-3 PG 20 WC Mathematics, Applied SC Mathematics GA CT6GR UT WOS:000362911900005 ER PT J AU Xu, X Hong, YK Park, J Lee, W Lane, AM Cui, J AF Xu, Xia Hong, Yang-Ki Park, Jihoon Lee, Woncheol Lane, Alan M. Cui, Jun TI Magnetic self-assembly for the synthesis of magnetically exchange coupled MnBi/Fe-Co composites SO JOURNAL OF SOLID STATE CHEMISTRY LA English DT Article DE MnBi; FeCo; Exchange coupling; Core/shell; Rare-earth-free ID ENERGY PRODUCT; BAFE12O19 SPHERES; 2-PHASE MAGNETS; NANOPARTICLES AB Exchange coupled hard/soft MnBi/Fe-Co core/shell structured composites were synthesized using a magnetic self-assembly process. MnBi particles were prepared by arc-melting, and Fe-Co nanoparticles were synthesized by an oleic acid assisted chemical reduction method. Grinding a mixture of micronsized MnBi and Fe-Co nanoparticles in hexane resulted in MnBi/Fe-Co core/shell structured composites. The MnBi/Fe-Co (95/5 wt%) composites showed smooth magnetic hysteresis loops, enhanced remanent magnetization, and positive values in the Delta M curve, indicating exchange coupling between MnBi and Fe-Co particles. (C) 2015 Elsevier Inc. All rights reserved. C1 [Xu, Xia; Lane, Alan M.] Univ Alabama, Dept Chem & Biol Engn, Tuscaloosa, AL 35487 USA. [Xu, Xia; Hong, Yang-Ki; Park, Jihoon; Lee, Woncheol; Lane, Alan M.] Univ Alabama, MINT Ctr, Tuscaloosa, AL 35487 USA. [Hong, Yang-Ki; Park, Jihoon; Lee, Woncheol] Univ Alabama, Dept Elect & Comp Engn, Tuscaloosa, AL 35487 USA. [Cui, Jun] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99354 USA. RP Hong, YK (reprint author), Univ Alabama, Dept Elect & Comp Engn, Tuscaloosa, AL 35487 USA. EM ykhong@eng.ua.edu RI Xu, Xia/L-5162-2016 OI Xu, Xia/0000-0003-4892-5478 FU U.S. Department of Energy ARPA-E REACT Program [DE-AR0000189] FX This work was supported in part by the U.S. Department of Energy ARPA-E REACT Program under Award no. DE-AR0000189. NR 26 TC 15 Z9 15 U1 12 U2 41 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0022-4596 EI 1095-726X J9 J SOLID STATE CHEM JI J. Solid State Chem. PD NOV PY 2015 VL 231 BP 108 EP 113 DI 10.1016/j.jssc.2015.08.019 PG 6 WC Chemistry, Inorganic & Nuclear; Chemistry, Physical SC Chemistry GA CT5PA UT WOS:000362861100016 ER PT J AU Baker, E Wang, B Bellora, N Peris, D Hulfachor, AB Koshalek, JA Adams, M Libkind, D Hittinger, CT AF Baker, EmilyClare Wang, Bing Bellora, Nicolas Peris, David Hulfachor, Amanda Beth Koshalek, Justin A. Adams, Marie Libkind, Diego Hittinger, Chris Todd TI The Genome Sequence of Saccharomyces eubayanus and the Domestication of Lager-Brewing Yeasts SO MOLECULAR BIOLOGY AND EVOLUTION LA English DT Article DE domestication; hybridization; Saccharomyces eubayanus; lager brewing; genome assembly ID SENSU-STRICTO; EVOLUTIONARY RELATIONSHIPS; MOLECULAR CHARACTERIZATION; DELETERIOUS MUTATIONS; MITOCHONDRIAL GENOME; POPULATION GENOMICS; CLONAL INTERFERENCE; DYNAMIC GENOMES; GENE-EXPRESSION; PROTEIN-KINASE AB The dramatic phenotypic changes that occur in organisms during domestication leave indelible imprints on their genomes. Although many domesticated plants and animals have been systematically compared with their wild genetic stocks, the molecular and genomic processes underlying fungal domestication have received less attention. Here, we present a nearly complete genome assembly for the recently described yeast species Saccharomyces eubayanus and compare it to the genomes of multiple domesticated alloploid hybrids of S. eubayanus x S. cerevisiae (S. pastorianus syn. S. carlsbergensis), which are used to brew lager-style beers. We find that the S. eubayanus subgenomes of lager-brewing yeasts have experienced increased rates of evolution since hybridization, and that certain genes involved in metabolism may have been particularly affected. Interestingly, the S. eubayanus subgenome underwent an especially strong shift in selection regimes, consistent with more extensive domestication of the S. cerevisiae parent prior to hybridization. In contrast to recent proposals that lager-brewing yeasts were domesticated following a single hybridization event, the radically different neutral site divergences between the subgenomes of the two major lager yeast lineages strongly favor at least two independent origins for the S. cerevisiae x S. eubayanus hybrids that brew lager beers. Our findings demonstrate how this industrially important hybrid has been domesticated along similar evolutionary trajectories on multiple occasions. C1 [Baker, EmilyClare; Wang, Bing; Peris, David; Hulfachor, Amanda Beth; Hittinger, Chris Todd] Univ Wisconsin, JF Crow Inst Study Evolut, Wisconsin Energy Inst, Lab Genet,Genome Ctr Wisconsin, Madison, WI 53706 USA. [Bellora, Nicolas; Libkind, Diego] Univ Nacl Comahue, CONICET, Lab Microbiol Aplicada & Biotecnol, Inst Invest Biodiversidad & Medioambiente INIBIOM, San Carlos De Bariloche, Rio Negro, Argentina. [Peris, David; Hittinger, Chris Todd] Univ Wisconsin, DOE Great Lakes Bioenergy Res Ctr, Madison, WI 53706 USA. [Koshalek, Justin A.; Adams, Marie] Univ Wisconsin, Ctr Biotechnol, Madison, WI 53706 USA. RP Hittinger, CT (reprint author), Univ Wisconsin, JF Crow Inst Study Evolut, Wisconsin Energy Inst, Lab Genet,Genome Ctr Wisconsin, Madison, WI 53706 USA. EM cthittinger@wisc.edu OI Peris, David/0000-0001-9912-8802 FU USDA National Institute of Food and Agriculture [1003258]; National Science Foundation [DEB-1253634]; DOE Great Lakes Bioenergy Research Center (DOE Office of Science BER) [DE-FC02-07ER64494]; Project ANPCyT [PICT2011-1814]; Project UNComahue [B171]; NSF-CONICET Argentina [5055/14]; Alexander von Humboldt Foundation; Pew Charitable Trusts FX We thank Paula Goncalves and Jose Paulo Sampaio for critical comments on the manuscript, as well as Dana A. Opulente for providing guidance for statistical analyses. This work was supported by the USDA National Institute of Food and Agriculture (Hatch project 1003258 to C.T.H.); by the National Science Foundation (grant no. DEB-1253634 to C.T.H.); in part by the DOE Great Lakes Bioenergy Research Center (DOE Office of Science BER DE-FC02-07ER64494 to C.T.H.); by Project ANPCyT PICT2011-1814 (D.L.); by Project UNComahue B171 (D.L.); and by a NSF-CONICET Argentina bilateral cooperation agreement (5055/14). C.T.H. is an Alfred Toepfer Faculty Fellow, supported by the Alexander von Humboldt Foundation. C.T.H. is a Pew Scholar in the Biomedical Sciences, supported by the Pew Charitable Trusts. The raw Illumina reads for Saccharomyces eubayanus FM1318 were deposited in NCBI's SRA as BioProject PRJNA243390. The final genome assembly and annotations were deposited in NCBI's GenBank as accession JMCK00000000. NR 88 TC 24 Z9 24 U1 8 U2 39 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0737-4038 EI 1537-1719 J9 MOL BIOL EVOL JI Mol. Biol. Evol. PD NOV PY 2015 VL 32 IS 11 BP 2818 EP 2831 DI 10.1093/molbev/msv168 PG 14 WC Biochemistry & Molecular Biology; Evolutionary Biology; Genetics & Heredity SC Biochemistry & Molecular Biology; Evolutionary Biology; Genetics & Heredity GA CT7YZ UT WOS:000363033100002 PM 26269586 ER PT J AU Swenson, TL Bowen, BP Nico, PS Northen, TR AF Swenson, Tami L. Bowen, Benjamin P. Nico, Peter S. Northen, Trent R. TI Competitive sorption of microbial metabolites on an iron oxide mineral SO SOIL BIOLOGY & BIOCHEMISTRY LA English DT Article DE Ferrihydrite; Sorption; Phosphate; Soil organic matter; Metabolomics ID DISSOLVED ORGANIC-MATTER; TEMPERATURE SENSITIVITY; COMMUNITY COMPOSITION; HUMIC SUBSTANCES; FULVIC-ACID; SOIL; GOETHITE; ADSORPTION; CARBON; DYNAMICS AB A large fraction of soil organic matter (SOM) is composed of small molecules of microbial origin. However, the biotic and abiotic cycling of these nutrients is poorly understood and is a critical component of the global carbon cycle. Although there are many factors controlling the accessibility of SOM to microbes, sorption to mineral surfaces is among the most significant. Here, we investigated the competitive sorption of a complex pool of microbial metabolites on ferrihydrite, an iron oxide mineral, using a lysate prepared from a soil bacterium, Pseudotnonas stutzeri RCH2. After a 24-h incubation with a range of mineral concentrations, more than half of the metabolites showed significant decreases in solution concentration. Phosphate-containing metabolites showed the greatest degree of sorption followed by dicarboxylates and metabolites containing both nitrogen and an aromatic moiety. Similar trends were observed when comparing sorption of metabolites with an equimolar metabolite mixture rather than a bacterial lysate. Interestingly, ectoine, lysine, two disaccharides and uracil were found not to sorb and may be more bioavailable in iron oxide-rich soils. Additionally, the highest-sorbing metabolites were examined for their ability to mobilize mineral-sorbed phosphate. All phosphate-containing metabolites tested and glutathione released phosphate from the mineral surface within 30 min of metabolite addition. These findings of preferential sorption behavior within a complex pool of microbial metabolites may provide insight into the cycling of SOM and specific nutrient availability. Finally, the release of highly-sorptive metabolites may be an underexplored mechanism utilized by microbial communities to gain access to limited environmental nutrients. Published by Elsevier Ltd. C1 [Swenson, Tami L.; Bowen, Benjamin P.; Northen, Trent R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Nico, Peter S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Northen, TR (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM TRNorthen@lbl.gov RI Nico, Peter/F-6997-2010; OI Nico, Peter/0000-0002-4180-9397; Northen, Trent/0000-0001-8404-3259 FU Office of Science Early Career Research Program [DE-AC02-05CH11231]; Office of Biological and Environmental Research; Terrestrial Ecosystem Science, Science Focus Area of the U.S. Department of Energy FX This work was funded by the Office of Science Early Career Research Program (No. DE-AC02-05CH11231), Office of Biological and Environmental Research and P.N. is funded by the Terrestrial Ecosystem Science, Science Focus Area, both of the U.S. Department of Energy under contract to Lawrence Berkeley National Laboratory. NR 52 TC 2 Z9 2 U1 13 U2 60 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0038-0717 J9 SOIL BIOL BIOCHEM JI Soil Biol. Biochem. PD NOV PY 2015 VL 90 BP 34 EP 41 DI 10.1016/j.soilbio.2015.07.022 PG 8 WC Soil Science SC Agriculture GA CT8OI UT WOS:000363075500005 ER PT J AU Zeller, L AF Zeller, Lori TI Potential changes in transportation patterns of New York Islanders fans due to stadium relocation SO TRANSPORTATION LA English DT Article DE Public transit; Mode shift; Accessibility; Survey; Recreational travel ID BUILT ENVIRONMENT; TRAVEL AB In 2015 the New York Islanders, a professional men's ice hockey team in the National Hockey League, will relocate to an arena with more transportation options for fans. The team currently plays at Nassau Coliseum in Uniondale, Long Island, NY, with limited public transportation access. They will move 23 miles west to the Barclays Center, an arena in the heart of Brooklyn, NY, with many public transportation options. This study examined fan characteristics which may influence their likelihood of attending Islanders games at the Barclays Center, including familiarity with public transportation, frequency of game attendance, and demographic factors. An online survey of Islanders fans captured fans' transportation behaviors when traveling to Islanders games at Nassau Coliseum and their projected frequency of attendance after the move, among other variables. Binary and ordered logistic regression models tested the significance of fan characteristics on the likelihood they attended a pre-season Islanders game held at the Barclays Center in September, 2013, and on how frequently respondents reported they will attend future games in Brooklyn. For both models, fans who use regional rail every workday, compared to those who do not, were significantly more likely to have attended the pre-season game and to report they will attend future games. Transit-use variables performed stronger in models than variables representing fans' work locations. The results exemplify the importance of familiarity with public transportation options when making mode choice decisions, bolstering the importance of transportation demand management strategies when opening new or relocating existing large event venues. C1 US EPA, Off Sustainable Communities, ORISE, Washington, DC 20460 USA. RP Zeller, L (reprint author), US EPA, Off Sustainable Communities, ORISE, 1200 Penn Ave,NW Mailcode 1807T, Washington, DC 20460 USA. EM Zeller.Lori@epa.gov FU University Transportation Research Center Region 2 FX This research was made possible by a scholarship from the University Transportation Research Center Region 2. Thank you for this wonderful opportunity. Thank you to all the people who supported this project: Robert Noland, Deva Deka, Mitch Zeller, Paula Zeller, Emily Zeller, Ross Schwarzber, Radha Jagannathan, Orin Puniello, Marc Weiner, Leighann Kimber, Swetha Ramkumar, Joseph Steindam, Kevin Schultz, Rob McGowan, Lisa from IslanderMania, Dan Schack, and all the Islanders fans who responded to the survey and sent personal anecdotes. NR 10 TC 0 Z9 0 U1 3 U2 14 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0049-4488 EI 1572-9435 J9 TRANSPORTATION JI Transportation PD NOV PY 2015 VL 42 IS 6 BP 951 EP 966 DI 10.1007/s11116-015-9652-8 PG 16 WC Engineering, Civil; Transportation; Transportation Science & Technology SC Engineering; Transportation GA CT6CS UT WOS:000362899600004 ER PT J AU Gould, B Greco, A AF Gould, Benjamin Greco, Aaron TI The Influence of Sliding and Contact Severity on the Generation of White Etching Cracks SO TRIBOLOGY LETTERS LA English DT Article DE White etching cracks; Wind turbine gearbox bearings; Bearing failures; Microstructural alterations ID TURBINE GEARBOX BEARINGS; MICROSTRUCTURAL CHANGES; STRUCTURAL ALTERATIONS; FORMATION MECHANISMS; WEC FORMATION; FATIGUE LIFE; HYDROGEN; STEEL; INCLUSIONS; AREA AB White etching cracks (WECs) have been identified as the dominant mechanism of premature failure for bearings within wind turbine gearboxes. Though WECs have been observed in the field for over a decade, the exact mechanisms which lead to this failure are still debated, and benchtop replication has proven difficult. In previously published work, WECs have been replicated only through the use of component level test rigs, where complete bearings are tested. In these tests, the factors that are thought to drive the formation of WECs, such as slide-to-roll ratio (SRR) and lubricant film thickness, cannot not be easily altered or controlled. In this paper, WECs have been replicated on a three ring on roller, benchtop test rig, which allowed for a direct investigation into the influence that SRR magnitude, sliding direction, and the lubricant film thickness have on surface failures and WEC generation. It was determined that WECs were formed in samples that experienced -30 % SRR at various lubrication conditions; however, at lower levels of negative SRR and positive SRR up to 30 %, no white etching cracks were observed. C1 [Gould, Benjamin; Greco, Aaron] Argonne Natl Lab, Div Energy Syst, Lemont, IL 60439 USA. [Gould, Benjamin] Univ Delaware, Dept Mech Engn, Newark, DE 19716 USA. RP Gould, B (reprint author), Argonne Natl Lab, Div Energy Syst, Lemont, IL 60439 USA. EM Bengould@udel.edu OI Gould, Benjamin/0000-0002-4363-6602; Greco, Aaron/0000-0002-2189-0888 FU US Department of Energy Office of Energy Efficiency and Renewable Energy, Wind and Water Power Technology Office [DE-AC02-06CH11357]; US Department of Energy Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work is supported by the US Department of Energy Office of Energy Efficiency and Renewable Energy, Wind and Water Power Technology Office, under Contract No. DE-AC02-06CH11357. The authors are grateful to DOE Project Managers Mr. Michael Derby and Mr. Jim Ahlgrimm for their support and encouragement. The authors would also like to acknowledge the assistance provided by our colleagues at Argonne National Laboratory's Tribology Section, especially Dr. Maria De La Cinta Lorenzo Martin for her assistance with electron microscopy, and Dr. Oyelayo Ajayi for his helpful discussion on metallurgy. As well as Dr. David L. Burris of the University of Delaware's department of Mechanical Engineering for serving as an advisor over the course of this work. The authors would also like to thank PCS Instruments for providing samples for the MPR testing. Use of the Center for Nanoscale Materials an Office of Science user facility was supported by the US Department of Energy Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357. NR 59 TC 6 Z9 7 U1 6 U2 15 PU SPRINGER/PLENUM PUBLISHERS PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1023-8883 EI 1573-2711 J9 TRIBOL LETT JI Tribol. Lett. PD NOV PY 2015 VL 60 IS 2 AR 29 DI 10.1007/s11249-015-0602-6 PG 13 WC Engineering, Chemical; Engineering, Mechanical SC Engineering GA CT8HK UT WOS:000363055600009 ER PT J AU Paris, JL Kamke, FA Xiao, XH AF Paris, Jesse L. Kamke, Frederick A. Xiao, Xianghui TI X-ray computed tomography of wood-adhesive bondlines: attenuation and phase-contrast effects SO WOOD SCIENCE AND TECHNOLOGY LA English DT Article ID DENSITY FIBERBOARD MDF; SYNCHROTRON-RADIATION; IMAGE-ANALYSIS; MICROTOMOGRAPHY; MICROSCOPY; MICROSTRUCTURE; RETRIEVAL; NETWORK; RESIN AB Microscale X-ray computed tomography (XCT) is discussed as a technique for identifying 3D adhesive distribution in wood-adhesive bondlines. Visualization and material segmentation of the adhesives from the surrounding cellular structures require sufficient gray-scale contrast in the reconstructed XCT data. Commercial wood-adhesive polymers have similar chemical characteristics and density to wood cell wall polymers and therefore do not provide good XCT attenuation contrast in their native form. Here, three different adhesive types, namely phenol formaldehyde, polymeric diphenylmethane diisocyanate, and a hybrid polyvinyl acetate, are tagged with iodine such that they yield sufficient X-ray attenuation contrast. However, phase-contrast effects at material edges complicate image quality and segmentation in XCT data reconstructed with conventional filtered backprojection absorption contrast algorithms. A quantitative phase retrieval algorithm, which isolates and removes the phase-contrast effect, was demonstrated. The article discusses and illustrates the balance between material X-ray attenuation and phase-contrast effects in all quantitative XCT analyses of wood-adhesive bondlines. C1 [Paris, Jesse L.; Kamke, Frederick A.] Oregon State Univ, Wood Based Composites Ctr, Dept Wood Sci & Engn, Corvallis, OR 97330 USA. [Xiao, Xianghui] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Paris, JL (reprint author), Oregon State Univ, Wood Based Composites Ctr, Dept Wood Sci & Engn, 119 Richardson Hall, Corvallis, OR 97330 USA. EM jesse.paris@wilvaco.com; fred.kamke@oregonstate.edu FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Wood-Based Composites Center, a National Science Foundation Industry/University Cooperative Research Center [A-04-KA] FX Use of the Advanced Photon Source was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. Financial support was provided by the Wood-Based Composites Center, a National Science Foundation Industry/University Cooperative Research Center; project code A-04-KA. NR 57 TC 2 Z9 2 U1 2 U2 25 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0043-7719 EI 1432-5225 J9 WOOD SCI TECHNOL JI Wood Sci. Technol. PD NOV PY 2015 VL 49 IS 6 BP 1185 EP 1208 DI 10.1007/s00226-015-0750-8 PG 24 WC Forestry; Materials Science, Paper & Wood SC Forestry; Materials Science GA CT8GC UT WOS:000363052000007 ER PT J AU Van Meter, RJ Glinski, DA Henderson, WM Garrison, AW Cyterski, M Purucker, ST AF Van Meter, Robin J. Glinski, Donna A. Henderson, W. Matthew Garrison, A. Wayne Cyterski, Mike Purucker, S. Thomas TI Pesticide Uptake Across the Amphibian Dermis Through Soil and Overspray Exposures SO ARCHIVES OF ENVIRONMENTAL CONTAMINATION AND TOXICOLOGY LA English DT Article ID FROGS LITHOBATES-CLAMITANS; ACUTE TOXICITY; LEGGED FROGS; TERRESTRIAL; GLYPHOSATE; CALIFORNIA; HERBICIDE; DECLINES; CONSERVATION; FORMULATIONS AB For terrestrial amphibians, accumulation of pesticides through dermal contact is a primary route of exposure in agricultural landscapes and may be contributing to widespread amphibian declines. To show pesticide transfer across the amphibian dermis at permitted label application rates, our study was designed to measure pesticide body burdens after two simulated exposure scenarios. We compared direct exposures, where amphibians were present when spraying occurred, to indirect exposures, where amphibians were exposed to soils after pesticide application. During summer 2012, we reared barking (Hyla gratiosa) and green treefrogs (H. cinerea) through 60-90 days post-metamorphosis at a United States Environmental Protection Agency research laboratory. We tested exposure for 8 h to five pesticide active ingredients (imidacloprid, atrazine, triadimefon, fipronil, or pendimethalin) in glass aquaria lined with soil in the laboratory. We quantified total pesticide body burden and soil concentrations using liquid chromatography-mass spectrometry. All individuals in both treatments had measurable body burdens at the end of the study. A randomized block design analysis of variance (n = 18) showed that body burdens (p = 0.03) and bioconcentration factors (BCFs) (p = 0.01) were significantly greater in the direct overspray treatment relative to the indirect soil spray treatment for both species and tested pesticides. BCFs ranged from 0.1 to 1.16 and from 0.013 to 0.78 in the direct and indirect treatments, respectively. Our study shows dermal uptake for multiple pesticides from both direct spray and indirect soil exposures and provides empirical support for the degree to which terrestrial phase amphibians have higher body burdens after overspray pesticide exposure. C1 [Van Meter, Robin J.] US EPA, Oak Ridge Inst Sci & Educ, Athens, GA 30613 USA. [Glinski, Donna A.] US EPA, Student Serv Author Contractor, Athens, GA 30605 USA. [Henderson, W. Matthew; Garrison, A. Wayne; Cyterski, Mike; Purucker, S. Thomas] US EPA, Ecosyst Res Div, Athens, GA 30605 USA. RP Van Meter, RJ (reprint author), Washington Coll, Toll Sci Ctr SG20, Chestertown, MD 21620 USA. EM rvanmeter2@washcoll.edu FU USEPA Ecosystems Research Division, Athens, GA [DW8992298301] FX We gratefully acknowledge the efforts of Jimmy Avants for assistance in developing our amphibian tissue extraction protocol. The USEPA Office of Pesticide Programs provided valuable feedback on study design. Thanks to Fran Rauschenberg and Craig Barber for manuscript review and edits. Many hours of field assistance with tadpoles and metamorphs was given by Craig Barber, Tao Hong, Yin Gu, Katie Price, and Marcia Snyder. This IACUC protocol (A2012 05-018-Y1-A0) received approval from the University of Georgia Institutional Animal Care and Use Committee. This research was supported in part by an appointment to the Post-doctoral Research Program at the USEPA Ecosystems Research Division, Athens, GA, administered by the Oak Ridge Institute for Science and Education through Interagency Agreement No. DW8992298301 between the United States Department of Energy and the United States Environmental Protection Agency. The views expressed in this article are those of the authors and do not necessarily represent the views or policies of the USEPA. NR 41 TC 2 Z9 2 U1 12 U2 35 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0090-4341 EI 1432-0703 J9 ARCH ENVIRON CON TOX JI Arch. Environ. Contam. Toxicol. PD NOV PY 2015 VL 69 IS 4 BP 545 EP 556 DI 10.1007/s00244-015-0183-2 PG 12 WC Environmental Sciences; Toxicology SC Environmental Sciences & Ecology; Toxicology GA CT2WT UT WOS:000362666700017 PM 26135301 ER PT J AU Fichman, Y Gerdes, SY Kovacs, H Szabados, L Zilberstein, A Csonka, LN AF Fichman, Yosef Gerdes, Svetlana Y. Kovacs, Hajnalka Szabados, Laszlo Zilberstein, Aviah Csonka, Laszlo N. TI Evolution of proline biosynthesis: enzymology, bioinformatics, genetics, and transcriptional regulation SO BIOLOGICAL REVIEWS LA English DT Review DE proline; -glutamyl kinase; -glutamyl phosphate reductase; (1)-pyrroline-5-carboxylate reductase; (1)-pyrroline-5-carboxylate synthase; ornithine -aminotransferase; osmotic stress ID GAMMA-GLUTAMYL-KINASE; ORNITHINE-DELTA-AMINOTRANSFERASE; ENCODING DELTA(1)-PYRROLINE-5-CARBOXYLATE SYNTHASE; ARTIFICIAL BIFUNCTIONAL ENZYME; ABIOTIC STRESS TOLERANCE; ORYZA-SATIVA L.; 1ST 2 STEPS; ESCHERICHIA-COLI; ARABIDOPSIS-THALIANA; SALT-STRESS AB Proline is not only an essential component of proteins but it also has important roles in adaptation to osmotic and dehydration stresses, redox control, and apoptosis. Here, we review pathways of proline biosynthesis in the three domains of life. Pathway reconstruction from genome data for hundreds of eubacterial and dozens of archaeal and eukaryotic organisms revealed evolutionary conservation and variations of this pathway across different taxa. In the most prevalent pathway of proline synthesis, glutamate is phosphorylated to -glutamyl phosphate by -glutamyl kinase, reduced to -glutamyl semialdehyde by -glutamyl phosphate reductase, cyclized spontaneously to (1)-pyrroline-5-carboxylate and reduced to proline by (1)-pyrroline-5-carboxylate reductase. In higher plants and animals the first two steps are catalysed by a bi-functional (1)-pyrroline-5-carboxylate synthase. Alternative pathways of proline formation use the initial steps of the arginine biosynthetic pathway to ornithine, which can be converted to (1)-pyrroline-5-carboxylate by ornithine aminotransferase and then reduced to proline or converted directly to proline by ornithine cyclodeaminase. In some organisms, the latter pathways contribute to or could be fully responsible for the synthesis of proline. The conservation of proline biosynthetic enzymes and significance of specific residues for catalytic activity and allosteric regulation are analysed on the basis of protein structural data, multiple sequence alignments, and mutant studies, providing novel insights into proline biosynthesis in organisms. We also discuss the transcriptional control of the proline biosynthetic genes in bacteria and plants. C1 [Fichman, Yosef; Zilberstein, Aviah] Tel Aviv Univ, Dept Mol Biol & Ecol Plants, IL-6997803 Tel Aviv, Israel. [Gerdes, Svetlana Y.] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. [Kovacs, Hajnalka; Szabados, Laszlo] Biol Res Ctr, Inst Plant Biol, H-6726 Szeged, Hungary. [Csonka, Laszlo N.] Purdue Univ, Dept Biol Sci, W Lafayette, IN 47907 USA. RP Csonka, LN (reprint author), Purdue Univ, Dept Biol Sci, W Lafayette, IN 47907 USA. EM csonka@purdue.edu FU US National Science Foundation [IOS-1054977]; Israel Science Foundation [1432/08]; DFG German-Israeli-Palestinian Trilateral Grant [KO 1438/13-1]; IPA [HUSRB/1002/214/036]; OTKA [K81765] FX We are grateful to Erhard Bremer, Andrei Osterman, and Boris Ratnikov for helpful comments on this manuscript, Yuk Fai Leung, Jeffrey R. Lucas, and Michael Rossmann for helpful discussions, and Erhard Bremer for communicating unpublished data to us. Work in L.N.C.'s laboratory was supported by the US National Science Foundation grant IOS-1054977 and in A.Z.'s laboratory by the Israel Science Foundation (Grant no. 1432/08) and the DFG German-Israeli-Palestinian Trilateral Grant (KO 1438/13-1). Research of L.S. was supported by IPA project No. HUSRB/1002/214/036 and OTKA project No. K81765. NR 244 TC 7 Z9 7 U1 10 U2 58 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1464-7931 EI 1469-185X J9 BIOL REV JI Biol. Rev. PD NOV PY 2015 VL 90 IS 4 BP 1065 EP 1099 DI 10.1111/brv.12146 PG 35 WC Biology SC Life Sciences & Biomedicine - Other Topics GA CT3VP UT WOS:000362735300004 PM 25367752 ER PT J AU Morris, JP Chochua, GG Bogdan, AV AF Morris, Joseph P. Chochua, Gocha G. Bogdan, Andrey V. TI An efficient non-newtonian fluid-flow simulator for variable aperture fractures SO CANADIAN JOURNAL OF CHEMICAL ENGINEERING LA English DT Article DE fractures; hydraulic fracturing; numerical methods; CFD; non-Newtonian fluids ID POROUS-MEDIA; YIELD-STRESS; VISCOPLASTIC FLUIDS; MOVING INTERFACE; LAMINAR; DISPLACEMENTS AB Many natural and industrial applications involve non-Newtonian fluids with high effective viscosity ratios flowing between surfaces with spatial variations in aperture. In particular, hydraulic fracturing operations often require pumping sequences of non-Newtonian fluids with yield-stress into a variable-aperture fracture that initially contains water. Numerical methods for this class of problem must deal robustly with the high aspect ratio of the flow domain and large contrasts in effective viscosity while maintaining interfaces between immiscible phases. We avoid the computational burden of a fully three-dimensional approach by introducing an aperture-averaged analytic solution for flow of a Hershel-Bulkley fluid between two plates. We discuss the incorporation of this analytic solution within a simulator of flow within a fracture with spatial variations in aperture. We minimize numerical diffusion through use of a hybrid Lagrangian-Eulerian approach that naturally tracks the multiple fluid phases. We demonstrate effectiveness of the numerical method through comparison with analytic results and one-dimensional finite difference numerical solutions. Benchmarking of the 2-D model against a 3-D model reveals both advantages and shortcomings of a through-aperture averaged method. The two simulations agree on the bulk behaviour of the phases while the 2-D model is two orders of magnitude more efficient. Comparison between predictions of the models after water injection behind the pad reveals that the 3-D model predicts non-uniformity across the fracture aperture. This suggests that while bulk behaviour may be well captured by the 2-D model, improved accuracy could be obtained by introducing multiple fluid layers within each cell of the model. C1 [Morris, Joseph P.] Schlumberger Doll Res Ctr, Cambridge, MA 02139 USA. [Morris, Joseph P.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Chochua, Gocha G.] Schlumberger, Enabling Technol Prod Grp, Sugar Land, TX 77478 USA. [Bogdan, Andrey V.] Schlumberger, Pressure Pumping & Chem, Sugar Land, TX 77478 USA. RP Morris, JP (reprint author), Schlumberger Doll Res Ctr, One Hampshire St, Cambridge, MA 02139 USA. EM morris50@llnl.gov OI Bogdan, Andrey/0000-0001-7582-2007 NR 35 TC 0 Z9 0 U1 2 U2 17 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0008-4034 EI 1939-019X J9 CAN J CHEM ENG JI Can. J. Chem. Eng. PD NOV PY 2015 VL 93 IS 11 BP 1902 EP 1915 DI 10.1002/cjce.22314 PG 14 WC Engineering, Chemical SC Engineering GA CT0AD UT WOS:000362455100003 ER PT J AU Geng, GQ Taylor, R Bae, S Hernandez-Cruz, D Kilcoyne, DA Emwas, AH Monteiro, PJM AF Geng, Guoqing Taylor, Rae Bae, Sungchul Hernandez-Cruz, Daniel Kilcoyne, David A. Emwas, Abdul-Hamid Monteiro, Paulo J. M. TI Atomic and nano-scale characterization of a 50-year-old hydrated C3S paste SO CEMENT AND CONCRETE RESEARCH LA English DT Article DE TEM; NMR; Microstructure; Ca3SiO5; STXM ID C-S-H; CALCIUM-SILICATE-HYDRATE; TRICALCIUM-SILICATE; PORTLAND-CEMENT; EDGE XANES; K-EDGE; QUANTIFICATION; KINETICS; MICRO; PHASE AB This paper investigates the atomic and nano-scale structures of a 50-year-old hydrated alite paste. Imaged by TEM, the outer product C-S-H fibers are composed of particles that are 1.5-2 nm thick and several tens of nanometers long. Si-29 NMR shows 47.9% Q(1) and 52.1% Q(2), with a mean SiO4 tetrahedron chain length (MCL) of 4.18, indicating a limited degree of polymerization after 50 years' hydration. A Scanning Transmission X-ray Microscopy (STXM) study was conducted on this late-age paste and a 1.5 year old hydrated C3S solution. Near Edge X-ray Absorption Fine Structure (NEXAFS) at Ca L-3,L-2-edge indicates that Ca2+ in C-S-H is in an irregular symmetric coordination, which agrees more with the atomic structure of tobermorite than that of jennite. At Si K-edge, multi-scattering phenomenon is sensitive to the degree of polymerization, which has the potential to unveil the structure of the SiO44- tetrahedron chain. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Geng, Guoqing; Taylor, Rae; Bae, Sungchul; Monteiro, Paulo J. M.] Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA. [Kilcoyne, David A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Hernandez-Cruz, Daniel] Univ Autonoma Chiapas, Fac Ingn, Tuxtla Gutierrez 29050, Chiapas, Mexico. [Emwas, Abdul-Hamid] King Abdullah Univ Sci & Technol, NMR Core Lab, Thuwal 23955, Saudi Arabia. RP Monteiro, PJM (reprint author), Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA. EM monteiro@berkeley.edu RI Kilcoyne, David/I-1465-2013 FU China Scholarship Council [201206090127]; National Research Foundation-Prime Minister's office, Republic of Singapore; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX Guoqing GENG's study and research in UC Berkeley are supported by the China Scholarship Council (file No. 201206090127). The authors thank Timothy Teague for the technical help with the SEM and XRD experiments. This research is funded by the National Research Foundation-Prime Minister's office, Republic of Singapore through a grant to the Berkeley Education Alliance for Research in Singapore (BEARS) for the Singapore-Berkeley Building Efficiency and Sustainability in the Tropics (SinBerBEST) Program. BEARS has been established by the University of California, Berkeley as a center for intellectual excellence in research and education in Singapore. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 43 TC 1 Z9 1 U1 3 U2 30 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0008-8846 EI 1873-3948 J9 CEMENT CONCRETE RES JI Cem. Concr. Res. PD NOV PY 2015 VL 77 BP 36 EP 46 DI 10.1016/j.cemconres.2015.06.010 PG 11 WC Construction & Building Technology; Materials Science, Multidisciplinary SC Construction & Building Technology; Materials Science GA CT2EZ UT WOS:000362616100005 ER PT J AU Walsh, JA Romano, PK Forget, B Smith, KS AF Walsh, Jonathan A. Romano, Paul K. Forget, Benoit Smith, Kord S. TI Optimizations of the energy grid search algorithm in continuous-energy Monte Carlo particle transport codes SO COMPUTER PHYSICS COMMUNICATIONS LA English DT Article DE Monte Carlo; Particle transport; Search algorithm; Optimization; Multithreading ID CROSS-SECTIONS; NUCLEAR-DATA; REPRESENTATION AB In this work we propose, implement, and test various optimizations of the typical energy grid-cross section pair lookup algorithm in Monte Carlo particle transport codes. The key feature common to all of the optimizations is a reduction in the length of the vector of energies that must be searched when locating the index of a particle's current energy. Other factors held constant, a reduction in energy vector length yields a reduction in CPU time. The computational methods we present here are physics-informed. That is, they are designed to utilize the physical information embedded in a simulation in order to reduce the length of the vector to be searched. More specifically, the optimizations take advantage of information about scattering kinematics, neutron cross section structure and data representation, and also the expected characteristics of a system's spatial flux distribution and energy spectrum. The methods that we present are implemented in the OpenMC Monte Carlo neutron transport code as part of this work. The gains in computational efficiency, as measured by overall code speedup, associated with each of the optimizations are demonstrated in both serial and multithreaded simulations of realistic systems. Depending on the system, simulation parameters, and optimization method employed, overall code speedup factors of 1.2-1.5, relative to the typical single-nuclide binary search algorithm, are routinely observed. (C) 2015 Elsevier B.V. All rights reserved. C1 [Walsh, Jonathan A.; Forget, Benoit; Smith, Kord S.] MIT, Dept Nucl Sci & Engn, Cambridge, MA 02139 USA. [Romano, Paul K.] Argonne Natl Lab, Math & Comp Sci, Argonne, IL 60439 USA. RP Walsh, JA (reprint author), MIT, Dept Nucl Sci & Engn, 77 Massachusetts Ave,24-107, Cambridge, MA 02139 USA. EM walshjon@mit.edu OI Walsh, Jonathan/0000-0002-2542-1149; Romano, Paul/0000-0002-1147-045X FU Department of Energy Nuclear Energy University Programs Graduate Fellowship; Consortium for Advanced Simulation of Light Water Reactors; U.S. Department of Energy [DE-AC05-000R22725] FX This material is based upon work supported under the first author's appointment to a Department of Energy Nuclear Energy University Programs Graduate Fellowship. This research is partially supported by the Consortium for Advanced Simulation of Light Water Reactors (http://www.casl.gov), an Energy Innovation Hub (http://www.energy.gov/hubs) for Modeling and Simulation of Nuclear Reactors under U.S. Department of Energy Contract No. DE-AC05-000R22725. NR 28 TC 0 Z9 0 U1 3 U2 15 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0010-4655 EI 1879-2944 J9 COMPUT PHYS COMMUN JI Comput. Phys. Commun. PD NOV PY 2015 VL 196 BP 134 EP 142 DI 10.1016/j.cpc.2015.05.025 PG 9 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA CT1ZX UT WOS:000362602900012 ER PT J AU Godfrey, BB Vay, JL AF Godfrey, Brendan B. Vay, Jean-Luc TI Improved numerical Cherenkov instability suppression in the generalized PSTD PIC algorithm SO COMPUTER PHYSICS COMMUNICATIONS LA English DT Article DE Particle-in-cell; Pseudo-Spectral Time-Domain; Relativistic beam; Numerical stability ID LORENTZ-BOOSTED FRAME; PARTICLE CODES; PLASMA; SIMULATIONS; STABILITY AB The family of generalized Pseudo-Spectral Time Domain (including the Pseudo-Spectral Analytical Time Domain) Particle-in-Cell algorithms offers substantial versatility for simulating particle beams and plasmas, and well written codes using these algorithms run reasonably fast. When simulating relativistic beams and streaming plasmas in multiple dimensions, they are, however, subject to the numerical Cherenkov instability. Previous studies have shown that instability growth rates can be reduced substantially by modifying slightly the transverse fields as seen by the streaming particles. Here, we offer an approach which completely eliminates the fundamental mode of the numerical Cherenkov instability while minimizing the transverse field corrections. The procedure, numerically computed residual growth rates (from weaker, higher order instability aliases), and comparisons with simulations using the code Warp are presented. In some instances, there are no numerical instabilities whatsoever, at least in the linear regime. (C) 2015 Elsevier B.V. All rights reserved. C1 [Godfrey, Brendan B.] Univ Maryland, College Pk, MD 20742 USA. [Godfrey, Brendan B.; Vay, Jean-Luc] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Godfrey, BB (reprint author), Univ Maryland, College Pk, MD 20742 USA. EM brendan.godfrey@ieee.org OI Godfrey, Brendan/0000-0003-2311-7060 FU Office of Science, Office of High Energy Physics, US Dept. of Energy [DE-AC02-05CH11231]; US-DOE SciDAC ComPASS collaboration; United States Government FX We thank Irving Haber for suggesting this collaboration and for helpful recommendations. We also are indebted to David Grote for assistance in using the code Warp. This work was supported in part by the Director, Office of Science, Office of High Energy Physics, US Dept. of Energy under Contract No. DE-AC02-05CH11231 and the US-DOE SciDAC ComPASS collaboration, and used resources of the National Energy Research Scientific Computing Center.; This document was prepared as an account of work sponsored in part by the United States Government. While this document is believed to contain correct information, neither the United States Government nor any agency thereof, nor The Regents of the University of California, nor any of their employees, nor the authors makes any warranty, express or implied, or assumes any legal responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by its trade name, trademark, manufacturer, or otherwise, does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof, or The Regents of the University of California. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof or The Regents of the University of California. NR 23 TC 6 Z9 6 U1 2 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0010-4655 EI 1879-2944 J9 COMPUT PHYS COMMUN JI Comput. Phys. Commun. PD NOV PY 2015 VL 196 BP 221 EP 225 DI 10.1016/j.cpc.2015.06.008 PG 5 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA CT1ZX UT WOS:000362602900020 ER PT J AU Cardall, CY Budiardja, RD AF Cardall, Christian Y. Budiardja, Reuben D. TI GENASIS Basics: Object-oriented utilitarian functionality for large-scale physics simulations SO COMPUTER PHYSICS COMMUNICATIONS LA English DT Article DE Simulation framework; Object-oriented programming; Fortran 2003 ID RIEMANN SOLVER; MAGNETOHYDRODYNAMICS; HYDRODYNAMICS; SYSTEMS AB Aside from numerical algorithms and problem setup, large-scale physics simulations on distributed-memory supercomputers require more basic utilitarian functionality, such as physical units and constants; display to the screen or standard output device; message passing; I/O to disk; and runtime parameter management and usage statistics. Here we describe and make available Fortran 2003 classes furnishing extensible object-oriented implementations of this sort of rudimentary functionality, along with individual 'unit test' programs and larger example problems demonstrating their use. These classes compose the Basics division of our developing astrophysics simulation code GsNASIS (General Astrophysical Simulation System), but their fundamental nature makes them useful for physics simulations in many fields. Program summary Program title: GENASIS Catalogue identifier: AEXE_v1_0 Program summary URL: http://cpc.cs.qub.ac.uk/summaries/AEXE_v1_0.html Program obtainable from: CPC Program Library, Queen's University, Belfast, N. Ireland Licensing provisions: Creative Commons Attribution - Non Commercial - ShareALike 4.0 International No. of lines in distributed program, including test data, etc.: 32863 No. of bytes in distributed program, including test data, etc.: 148873 Distribution format: tar.gz Programming language: Fortran 2003 (tested with gfortran 4.9.2, Intel Fortran 15, NAG Fortan 5.3.1, Cray Compiler 8.2.5). Computer: PC, cluster, supercomputer. Operating system: Linux, Unix. RAM: For example problems, depends on user-specified problem size and number of processes. The fluid dynamics problems with 128(3) cells on 8 processes use about 300 MB per process. The molecular dynamics problems with 6912 particles on 12 processes use about 20 MB per process. Classification: 4.14, 6.5, 20. External routines: MPI [1] and Silo [2] Nature of problem: By way of illustrating GENASIS Basics functionality, solve example fluid dynamics and molecular dynamics problems. Solution method: For fluid dynamics examples, finite-volume. For molecular dynamics examples, leapfrog and velocity-Verlet integration. Unusual features: The example problems named above are not ends in themselves, but serve to illustrate our object-oriented approach and the functionality available though GENASIS Basics. In addition to these more substantial examples, we provide individual unit test programs for each of the classes comprised by GENASIS Basics. Additional comments: A version of the GENASIS Basics source code is available from the CPC program library with this publication, and minor revisions will be maintained at http://astro.phys.utk.edu/activities: genasis. Running time: For example problems, depends on user-specified problem size and number of processes. The fluid dynamics problems with 1283 cells on 8 processes take about ten minutes of wall clock time on a Cray XC30. The molecular dynamics problems with 6912 particles for 10000 time steps on 12 processes take a little over an hour on a Cray XC30. References: [1] http://www.mcs.anl.gov/mpi/ [2] https://wci.Ilnl.govisimulation/computer-codes/silo (C) 2015 Elsevier B.V. All rights reserved. C1 [Cardall, Christian Y.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Cardall, Christian Y.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Budiardja, Reuben D.] Univ Tennessee, Natl Inst Computat Sci, Knoxville, TN 37996 USA. RP Cardall, CY (reprint author), Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. EM cardallcy@ornl.gov; reubendb@utk.edu OI Cardall, Christian/0000-0002-0086-105X FU Office of Advanced Scientific Computing of the US Department of Energy; Office of Nuclear Physics of the US Department of Energy FX We acknowledge the support of the Office of Advanced Scientific Computing and the Office of Nuclear Physics of the US Department of Energy. This material is based upon work performed using computational resources supported by the University of Tennessee and Oak Ridge National Laboratory Joint Institute for Computational Sciences (http://www.jics.tennessee.edu). NR 25 TC 1 Z9 1 U1 1 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0010-4655 EI 1879-2944 J9 COMPUT PHYS COMMUN JI Comput. Phys. Commun. PD NOV PY 2015 VL 196 BP 506 EP 534 DI 10.1016/j.cpc.2015.06.001 PG 29 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA CT1ZX UT WOS:000362602900048 ER PT J AU Hyman, JD Karra, S Makedonska, N Gable, CW Painter, SL Viswanathan, HS AF Hyman, Jeffrey D. Karra, Satish Makedonska, Nataliia Gable, Carl W. Painter, Scott L. Viswanathan, Hari S. TI DFNWORKS: A discrete fracture network framework for modeling subsurface flow and transport SO COMPUTERS & GEOSCIENCES LA English DT Article DE Discrete fracture networks; Conforming Delaunay triangulation; Subsurface flow and transport; Fractured porous media; Hydraulic fracturing; CO2 sequestration ID HYBRID MORTAR METHOD; SAFETY ASSESSMENT; ELEMENT METHOD; SOLVING FLOW; SITE; CO2; SEQUESTRATION; SIMULATION; CHALLENGES; ALGORITHM AB DFNWORKS is a parallelized computational suite to generate three-dimensional discrete fracture networks (DFN) and simulate flow and transport. Developed at Los Alamos National Laboratory over the past five years, it has been used to study flow and transport in fractured media at scales ranging from millimeters to kilometers. The networks are created and meshed using DFNGEN, which combines FRAM (the feature rejection algorithm for meshing) methodology to stochastically generate three-dimensional DENs with the LAGRIT meshing toolbox to create a high-quality computational mesh representation. The representation produces a conforming Delaunay triangulation suitable for high performance computing finite volume solvers in an intrinsically parallel fashion. Flow through the network is simulated in DFNFLOW, which utilizes the massively parallel subsurface flow and reactive transport finite volume code PFLOTRAN. A Lagrangian approach to simulating transport through the DFN is adopted within DFNTRANS to determine pathlines and solute transport through the DFN. Example applications of this suite in the areas of nuclear waste repository science, hydraulic fracturing and CO2 sequestration are also included. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Hyman, Jeffrey D.; Karra, Satish; Makedonska, Nataliia; Gable, Carl W.; Viswanathan, Hari S.] Los Alamos Natl Lab, Earth & Environm Sci Div, Computat Earth Sci Grp EES 16, Los Alamos, NM 87544 USA. [Hyman, Jeffrey D.] Los Alamos Natl Lab, Div Theoret, Ctr Nonlinear Studies, Los Alamos, NM USA. [Painter, Scott L.] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. RP Hyman, JD (reprint author), Los Alamos Natl Lab, Earth & Environm Sci Div, Computat Earth Sci Grp EES 16, Los Alamos, NM 87544 USA. EM jhyman@lanl.gov RI Painter, Scott/C-2586-2016; OI Karra, Satish/0000-0001-7847-6293; Painter, Scott/0000-0002-0901-6987; Gable, Carl/0000-0001-7063-0815; Makedonska, Nataliia/0000-0002-4183-5755; Hyman, Jeffrey /0000-0002-4224-2847 FU LANL's DR [20140002DR]; U.S. Department of Energy Strategic Center for Natural Gas and Oil project on 'Fundamentals of Unconventional Reservoirs'; U.S. Department of Energy Used Fuel Disposal campaign; Center for Nonlinear Studies at Los Alamos National Laboratory [DE-AC52-06NA25396] FX The various tools under DFNWORKS and the overall workflow have been developed through the support of various funding programs including LANL's DR research Project # 20140002DR, U.S. Department of Energy Strategic Center for Natural Gas and Oil project on 'Fundamentals of Unconventional Reservoirs' and the U.S. Department of Energy Used Fuel Disposal campaign. Jeffrey Hyman acknowledges the support of the Center for Nonlinear Studies at Los Alamos National Laboratory through Grant # DE-AC52-06NA25396. Satish Karra thanks Glenn Hammond and Gautam Bisht for their help with explicit unstructured grid implementation and corresponding I/O in PFLOTRAN. NR 63 TC 14 Z9 14 U1 7 U2 35 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0098-3004 EI 1873-7803 J9 COMPUT GEOSCI-UK JI Comput. Geosci. PD NOV PY 2015 VL 84 BP 10 EP 19 DI 10.1016/j.cageo.2015.08.001 PG 10 WC Computer Science, Interdisciplinary Applications; Geosciences, Multidisciplinary SC Computer Science; Geology GA CS8AI UT WOS:000362307700002 ER PT J AU Fritz, BG Barnett, JM AF Fritz, Bradley G. Barnett, J. Matthew TI Technical Assessment of Internal Surface Smoothness and Particle Transmission to the American National Standard ANSI/HPS N13.1-2011 SO HEALTH PHYSICS LA English DT Article DE operational topics; aerosols; air sampling; emissions; atmospheric AB Clause 6.4.4 in the American National Standard ANSI/HPS N13.1 standard Sampling and Monitoring Releases of Airborne Radioactive Substances From the Stacks and Ducts of Nuclear Facilities addresses the internal smoothness of sample transport lines present between the nozzle and the analyzer (or collector). The appropriateness of this clause is evaluated by comparing roughness length of various materials against the required relative roughness and by conducting computational fluid dynamic modeling. The results indicate that the inclusion of numerical criteria for the relative roughness of pipe by the ANSI/HPS N13.1-2011 (clause 6.4.4) is not appropriate. Recommended alternatives would be elimination of the numerical criteria or modification of the standard to include a variable criterion for relative roughness. C1 [Fritz, Bradley G.; Barnett, J. Matthew] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Fritz, BG (reprint author), Pacific NW Natl Lab, POB 999,MSIN K7-68, Richland, WA 99352 USA. EM Bradley.Fritz@pnnl.gov NR 5 TC 0 Z9 0 U1 0 U2 2 PU LIPPINCOTT WILLIAMS & WILKINS PI PHILADELPHIA PA TWO COMMERCE SQ, 2001 MARKET ST, PHILADELPHIA, PA 19103 USA SN 0017-9078 EI 1538-5159 J9 HEALTH PHYS JI Health Phys. PD NOV PY 2015 VL 109 SU 3 BP S200 EP S204 DI 10.1097/HP.0000000000000325 PG 5 WC Environmental Sciences; Public, Environmental & Occupational Health; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging SC Environmental Sciences & Ecology; Public, Environmental & Occupational Health; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging GA CS9KA UT WOS:000362408700003 PM 26425982 ER PT J AU King, DA Vitkus, T AF King, David A. Vitkus, Tim TI Lessons Learned on the Presentation of Scan Data SO HEALTH PHYSICS LA English DT Article DE operational topics; contamination; radiation protection; waste management AB Technicians performed a radiological survey of a surplus metal tank to support disposition planning at an Oak Ridge, TN, site. The survey included radiation scans to identify contamination and, if identified, define the boundary and magnitude of contamination. Fixed-point 1-min measurements were also collected at randomly selected locations for comparison against the site's free release limit of 5,000 disintegrations per minute per 100 cm(2) (dpm 100 cm(-2)) (0.83 Bq cm(-2)). Scan data were recorded using a data logger as a means to document surveyor observationlogged data captured at 1-s intervals and converted to counts per minute (cpm) by the data logger software were presented in the project report. Both the qualitative scan data (in cpm) and the quantitative direct measurements (in dpm 100 cm(-2)) were reported for completeness, so stakeholders had all available information to support disposition decisions. However, a new stakeholderintroduced to the project at the reporting phase of workused the instrument efficiency and background data to convert the scan data from cpm to dpm 100 cm(-2), then compared the converted results to the site limit. Many of the converted values exceeded 5,000 dpm 100 cm(-1). This resulted in delays in tank disposition and additional project costs that could have been avoided if the proper use and interpretation of scan data and implications of radon progeny buildup on oxidized metal surfaces had been better communicated. C1 [King, David A.; Vitkus, Tim] Oak Ridge Associated Univ, Oak Ridge, TN 37830 USA. RP King, DA (reprint author), Oak Ridge Associated Univ, 1299 Bethel Valley Rd, Oak Ridge, TN 37830 USA. NR 3 TC 0 Z9 0 U1 0 U2 3 PU LIPPINCOTT WILLIAMS & WILKINS PI PHILADELPHIA PA TWO COMMERCE SQ, 2001 MARKET ST, PHILADELPHIA, PA 19103 USA SN 0017-9078 EI 1538-5159 J9 HEALTH PHYS JI Health Phys. PD NOV PY 2015 VL 109 SU 3 BP S212 EP S218 DI 10.1097/HP.0000000000000358 PG 7 WC Environmental Sciences; Public, Environmental & Occupational Health; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging SC Environmental Sciences & Ecology; Public, Environmental & Occupational Health; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging GA CS9KA UT WOS:000362408700005 PM 26425984 ER PT J AU Rajeev, L Chen, A Kazakov, AE Luning, EG Zane, GM Novichkov, PS Wall, JD Mukhopadhyaya, A AF Rajeev, Lara Chen, Amy Kazakov, Alexey E. Luning, Eric G. Zane, Grant M. Novichkov, Pavel S. Wall, Judy D. Mukhopadhyaya, Aindrila TI Regulation of Nitrite Stress Response in Desulfovibrio vulgaris Hildenborough, a Model Sulfate-Reducing Bacterium SO JOURNAL OF BACTERIOLOGY LA English DT Article ID SULFIDE-OXIDIZING BACTERIA; GENE-EXPRESSION ANALYSIS; HYBRID CLUSTER PROTEINS; ESCHERICHIA-COLI; WOLINELLA-SUCCINOGENES; REDUCTASE-ACTIVITY; OXIDE REDUCTASE; NITRATE; DESULFURICANS; INHIBITION AB Sulfate-reducing bacteria (SRB) are sensitive to low concentrations of nitrite, and nitrite has been used to control SRB-related biofouling in oil fields. Desulfovibrio vulgaris Hildenborough, a model SRB, carries a cytochrome c-type nitrite reductase (nrfHA) that confers resistance to low concentrations of nitrite. The regulation of this nitrite reductase has not been directly examined to date. In this study, we show that DVU0621 (NrfR), a sigma54-dependent two-component system response regulator, is the positive regulator for this operon. NrfR activates the expression of the nrfHA operon in response to nitrite stress. We also show that nrfR is needed for fitness at low cell densities in the presence of nitrite because inactivation of nrfR affects the rate of nitrite reduction. We also predict and validate the binding sites for NrfR upstream of the nrfHA operon using purified NrfR in gel shift assays. We discuss possible roles for NrfR in regulating nitrate reductase genes in nitrate-utilizing Desulfovibrio spp. IMPORTANCE The NrfA nitrite reductase is prevalent across several bacterial phyla and required for dissimilatory nitrite reduction. However, regulation of the nrfA gene has been studied in only a few nitrate-utilizing bacteria. Here, we show that in D. vulgaris, a bacterium that does not respire nitrate, the expression of nrfHA is induced by NrfR upon nitrite stress. This is the first report of regulation of nrfA by a sigma54-dependent two-component system. Our study increases our knowledge of nitrite stress responses and possibly of the regulation of nitrate reduction in SRB. C1 [Rajeev, Lara; Chen, Amy; Kazakov, Alexey E.; Luning, Eric G.; Novichkov, Pavel S.; Mukhopadhyaya, Aindrila] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Zane, Grant M.; Wall, Judy D.] Univ Missouri, Dept Biochem, Columbia, MO USA. RP Mukhopadhyaya, A (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. EM amukhopadhyay@lbl.gov OI Rajeev, Lara/0000-0002-0106-9195 FU U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231] FX This material by ENIGMA (Ecosystems and Networks Integrated with Genes and Molecular Assemblies) (http://enigma.lbl.gov), a scientific focus area program at Lawrence Berkeley National Laboratory, is based on work supported by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, under contract DE-AC02-05CH11231. NR 54 TC 0 Z9 0 U1 10 U2 21 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0021-9193 EI 1098-5530 J9 J BACTERIOL JI J. Bacteriol. PD NOV PY 2015 VL 197 IS 21 BP 3400 EP 3408 DI 10.1128/JB.00319-15 PG 9 WC Microbiology SC Microbiology GA CT1LH UT WOS:000362559300004 PM 26283774 ER PT J AU Lin, TY Santos, TMA Kontur, WS Donohue, TJ Weibel, DB AF Lin, Ti-Yu Santos, Thiago M. A. Kontur, Wayne S. Donohue, Timothy J. Weibel, Douglas B. TI A Cardiolipin-Deficient Mutant of Rhodobacter sphaeroides Has an Altered Cell Shape and Is Impaired in Biofilm Formation SO JOURNAL OF BACTERIOLOGY LA English DT Article ID ESCHERICHIA-COLI-CELLS; BACTERIAL ADHESION; PSEUDOMONAS-AERUGINOSA; CAULOBACTER-CRESCENTUS; ANIONIC PHOSPHOLIPIDS; ACTIN CYTOSKELETON; GENETIC-ANALYSIS; HIGH SALINITY; SURFACES; PROTEIN AB Cell shape has been suggested to play an important role in the regulation of bacterial attachment to surfaces and the formation of communities associated with surfaces. We found that a cardiolipin synthase (Delta cls) mutant of the rod-shaped bacterium Rhodobacter sphaeroides-in which synthesis of the anionic, highly curved phospholipid cardiolipin (CL) is reduced by 90%-produces ellipsoid-shaped cells that are impaired in biofilm formation. Reducing the concentration of CL did not cause significant defects in R. sphaeroides cell growth, swimming motility, lipopolysaccharide and exopolysaccharide production, surface adhesion protein expression, and membrane permeability. Complementation of the CL-deficient mutant by ectopically expressing CL synthase restored cells to their rod shape and increased biofilm formation. Treating R. sphaeroides cells with a low concentration (10 mu g/ml) of the small-molecule MreB inhibitor S-(3,4-dichlorobenzyl) isothiourea produced ellipsoid-shaped cells that had no obvious growth defect yet reduced R. sphaeroides biofilm formation. This study demonstrates that CL plays a role in R. sphaeroides cell shape determination, biofilm formation, and the ability of the bacterium to adapt to its environment. IMPORTANCE Membrane composition plays a fundamental role in the adaptation of many bacteria to environmental stress. In this study, we build a new connection between the anionic phospholipid cardiolipin (CL) and cellular adaptation in Rhodobacter sphaeroides. We demonstrate that CL plays a role in the regulation of R. sphaeroides morphology and is important for the ability of this bacterium to form biofilms. This study correlates CL concentration, cell shape, and biofilm formation and provides the first example of how membrane composition in bacteria alters cell morphology and influences adaptation. This study also provides insight into the potential of phospholipid biosynthesis as a target for new chemical strategies designed to alter or prevent biofilm formation. C1 [Lin, Ti-Yu; Santos, Thiago M. A.; Weibel, Douglas B.] Univ Wisconsin, Dept Biochem, Madison, WI 53705 USA. [Kontur, Wayne S.; Donohue, Timothy J.] Univ Wisconsin, Dept Bacteriol, Madison, WI 53706 USA. [Kontur, Wayne S.; Donohue, Timothy J.] DOE Great Lakes Bioenergy Res Ctr, Madison, WI 53706 USA. [Weibel, Douglas B.] Univ Wisconsin, Dept Chem, Madison, WI 53706 USA. [Weibel, Douglas B.] Univ Wisconsin, Dept Biomed Engn, Madison, WI USA. RP Weibel, DB (reprint author), Univ Wisconsin, Dept Biochem, 420 Henry Mall, Madison, WI 53705 USA. EM weibel@biochem.wisc.edu OI Donohue, Timothy/0000-0001-8738-2467 FU Department of Biochemistry, University of Wisconsin-Madison; National Science Foundation [MCB-1120832, DMR-1121288]; NIH [1DP2OD008735]; USDA [WIS01594]; Department of Energy Office of Science [BER DE-FC02-07ER64494] FX T.-Y. Lin acknowledges a William H. Peterson fellowship from the Department of Biochemistry, University of Wisconsin-Madison. The National Science Foundation (MCB-1120832 and DMR-1121288), NIH (1DP2OD008735), USDA (WIS01594), and Department of Energy Office of Science (BER DE-FC02-07ER64494) supported this research. NR 68 TC 2 Z9 2 U1 1 U2 9 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0021-9193 EI 1098-5530 J9 J BACTERIOL JI J. Bacteriol. PD NOV PY 2015 VL 197 IS 21 BP 3446 EP 3455 DI 10.1128/JB.00420-15 PG 10 WC Microbiology SC Microbiology GA CT1LH UT WOS:000362559300008 PM 26283770 ER PT J AU Lunderberg, JM Zilla, ML Missiakas, D Schneewind, O AF Lunderberg, J. Mark Zilla, Megan Liszewski Missiakas, Dominique Schneewind, Olaf TI Bacillus anthracis tagO Is Required for Vegetative Growth and Secondary Cell Wall Polysaccharide Synthesis SO JOURNAL OF BACTERIOLOGY LA English DT Article ID S-LAYER PROTEINS; STAPHYLOCOCCUS-AUREUS; TEICHOIC-ACID; CHAIN-LENGTH; LINKAGE UNIT; SUBTILIS; SURFACE; BIOSYNTHESIS; BINDING; PEPTIDOGLYCAN AB Bacillus anthracis elaborates a linear secondary cell wall polysaccharide (SCWP) that retains surface (S)-layer and associated proteins via their S-layer homology (SLH) domains. The SCWP is comprised of trisaccharide repeats [-> 4)-beta-ManNAc-(1 -> 4)-beta-GlcNAc-(1 -> 6)-alpha-GlcNAc-(1 ->] and tethered via acid-labile phosphodiester bonds to peptidoglycan. Earlier work identified UDP-GlcNAc 2-epimerases GneY (BAS5048) and GneZ (BAS5117), which act as catalysts of ManNAc synthesis, as well as a polysaccharide deacetylase (BAS5051), as factors contributing to SCWP synthesis. Here, we show that tagO (BAS5050), which encodes a UDP-N-acetylglucosamine: undecaprenyl-P N-acetylglucosaminyl 1-P transferase, the enzyme that initiates the synthesis of murein linkage units, is required for B. anthracis SCWP synthesis and S-layer assembly. Similar to gneY-gneZ mutants, B. anthracis strains lacking tagO cannot maintain cell shape or support vegetative growth. In contrast, mutations in BAS5051 do not affect B. anthracis cell shape, vegetative growth, SCWP synthesis, or S-layer assembly. These data suggest that TagO-mediated murein linkage unit assembly supports SCWP synthesis and attachment to the peptidoglycan via acid-labile phosphodiester bonds. Further, B. anthracis variants unable to synthesize SCWP trisaccharide repeats cannot sustain cell shape and vegetative growth. IMPORTANCE Bacillus anthracis elaborates an SCWP to support vegetative growth and envelope assembly. Here, we show that some, but not all, SCWP synthesis is dependent on tagO-derived murein linkage units and subsequent attachment of SCWP to peptidoglycan. The data implicate secondary polymer modifications of peptidoglycan and subcellular distributions as a key feature of the cell cycle in Gram-positive bacteria and establish foundations for work on the molecular functions of the SCWP and on inhibitors with antibiotic attributes. C1 [Lunderberg, J. Mark; Zilla, Megan Liszewski; Missiakas, Dominique; Schneewind, Olaf] Argonne Natl Lab, Howard Taylor Ricketts Lab, Lemont, IL 60439 USA. [Lunderberg, J. Mark; Zilla, Megan Liszewski; Missiakas, Dominique; Schneewind, Olaf] Univ Chicago, Dept Microbiol, Chicago, IL 60637 USA. RP Schneewind, O (reprint author), Argonne Natl Lab, Howard Taylor Ricketts Lab, Lemont, IL 60439 USA. EM oschnee@bsd.uchicago.edu FU National Institutes of Health (NIH) training grant [GM07281]; NIH Ruth L. Kirschstein National Research Service Award [1F30AI110036]; National Institute of Allergy and Infectious Diseases, Infectious Disease Branch [AI069227] FX J.M.L. and M.L.Z. are trainees of the Medical Scientist Training Program at the University of Chicago and are supported by a National Institutes of Health (NIH) training grant (GM07281). J.M.L. is the recipient of an NIH Ruth L. Kirschstein National Research Service Award (1F30AI110036). This research was supported by grant AI069227 from the National Institute of Allergy and Infectious Diseases, Infectious Disease Branch (to O.S. and D.M.). NR 53 TC 5 Z9 5 U1 0 U2 8 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0021-9193 EI 1098-5530 J9 J BACTERIOL JI J. Bacteriol. PD NOV PY 2015 VL 197 IS 22 BP 3511 EP 3520 DI 10.1128/JB.00494-15 PG 10 WC Microbiology SC Microbiology GA CT1NF UT WOS:000362564500003 PM 26324447 ER PT J AU Ballard, G Demmel, J Grigori, L Jacquelin, M Knight, N Nguyen, HD AF Ballard, G. Demmel, J. Grigori, L. Jacquelin, M. Knight, N. Nguyen, H. D. TI Reconstructing Householder vectors from Tall-Skinny QR SO JOURNAL OF PARALLEL AND DISTRIBUTED COMPUTING LA English DT Article DE QR decomposition; Dense linear algebra; Communication-avoiding algorithms ID COLLECTIVE COMMUNICATION; WY REPRESENTATION; PARALLEL; BROADCAST; NETWORKS AB The Tall-Skinny QR (TSQR) algorithm is more communication efficient than the standard Householder algorithm for QR decomposition of matrices with many more rows than columns. However, TSQR produces a different representation of the orthogonal factor and therefore requires more software development to support the new representation. Further, implicitly applying the orthogonal factor to the trailing matrix in the context of factoring a square matrix is more complicated and costly than with the Householder representation. We show how to perform TSQR and then reconstruct the Householder vector representation with the same asymptotic communication efficiency and little extra computational cost. We demonstrate the high performance and numerical stability of this algorithm both theoretically and empirically. The new Householder reconstruction algorithm allows us to design more efficient parallel QR algorithms, with significantly lower latency cost compared to Householder QR and lower bandwidth and latency costs compared with Communication-Avoiding QR (CAQR) algorithm. Experiments on supercomputers demonstrate the benefits of the communication cost improvements: in particular, our experiments show substantial improvements over tuned library implementations for tall-and-skinny matrices. We also provide algorithmic improvements to the Householder QR and CAQR algorithms, and we investigate several alternatives to the Householder reconstruction algorithm that sacrifice guarantees on numerical stability in some cases in order to obtain higher performance. (C) 2015 Elsevier Inc. All rights reserved. C1 [Ballard, G.] Sandia Natl Labs, Livermore, CA USA. [Demmel, J.; Knight, N.; Nguyen, H. D.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Grigori, L.] INRIA Paris Rocquencourt, Paris, France. [Jacquelin, M.] Lawrence Berkeley Natl Lab, Berkeley, CA USA. RP Knight, N (reprint author), Univ Calif Berkeley, Berkeley, CA 94720 USA. EM gmballa@sandia.gov; demmel@cs.berkeley.edu; laura.grigori@inria.fr; mathias.jacquelin@lbl.gov; knight@cs.berkeley.edu; hdnguyen@cs.berkeley.edu FU Sandia National Laboratories Truman Fellowship in National Security Science and Engineering; Sandia Corporation; U.S. Department of Energy [DE-AC04-94AL85000]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; DOE [DE-SC0008700, DE-SC0010200, AC02-05CH11231]; DARPA [HR0011-12-2-0016] FX Ballard was supported in part by an appointment to the Sandia National Laboratories Truman Fellowship in National Security Science and Engineering, sponsored by Sandia Corporation (a wholly owned subsidiary of Lockheed Martin Corporation) as Operator of Sandia National Laboratories under its U.S. Department of Energy Contract No. DE-AC04-94AL85000. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We also acknowledge DOE grants DE-SC0008700, DE-SC0010200, AC02-05CH11231, and DARPA grant HR0011-12-2-0016. NR 38 TC 1 Z9 1 U1 0 U2 2 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0743-7315 EI 1096-0848 J9 J PARALLEL DISTR COM JI J. Parallel Distrib. Comput. PD NOV PY 2015 VL 85 SI SI BP 3 EP 31 DI 10.1016/j.jpdc.2015.06.003 PG 29 WC Computer Science, Theory & Methods SC Computer Science GA CT2GO UT WOS:000362620200002 ER PT J AU Djidjev, H Chapuis, G Andonov, R Thulasidasan, S Lavenier, D AF Djidjev, Hristo Chapuis, Guillaume Andonov, Rumen Thulasidasan, Sunil Lavenier, Dominique TI All-Pairs Shortest Path algorithms for planar graph for GPU-accelerated clusters SO JOURNAL OF PARALLEL AND DISTRIBUTED COMPUTING LA English DT Article DE All-pairs shortest path problem; Planar graphs; GPGPU; Parallel computing; Floyd-Warshall algorithm; Distributed computing; Algorithm analysis AB We present a new approach for solving the All-Pairs Shortest-Path (APSP) problem for planar graphs that exploits the massive on-chip parallelism available in today's Graphics Processing Units (GPUs). We describe two new algorithms based on our approach. Both algorithms use Floyd-Warshall method, have near optimal complexity in terms of the total number of operations, while their matrix-based structure is regular enough to allow for efficient parallel implementation on the GPUs. By applying a divide-and-conquer approach, we are able to make use of multi-node GPU clusters, resulting in more than an order of magnitude speedup over fastest known Dijkstra-based GPU implementation and a two-fold speedup over a parallel Dijkstra-based CPU implementation. (C) 2015 Elsevier Inc. All rights reserved. C1 [Djidjev, Hristo] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Chapuis, Guillaume] Los Alamos Natl Lab, Informat Sci Grp CCS3, Los Alamos, NM USA. [Thulasidasan, Sunil] Los Alamos Natl Lab, Computat Sci Div, Los Alamos, NM USA. [Andonov, Rumen; Lavenier, Dominique] INRIA IRISA, F-35042 Rennes, France. [Andonov, Rumen; Lavenier, Dominique] Univ Rennes 1, F-35042 Rennes, France. RP Djidjev, H (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM djidjev@lanl.gov; gchapuis@lanl.gov; randonov@irisa.fr; sunil@lanl.gov; lavenier@irisa.fr FU Los Alamos National Laboratory Directed Research and Development Program (LDRD); region of Brittany, France FX We want to thank reviewers for their helpful comments and acknowledge the support provided for this work by the Los Alamos National Laboratory Directed Research and Development Program (LDRD). This work was also partially supported by the region of Brittany, France. NR 26 TC 2 Z9 2 U1 0 U2 13 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0743-7315 EI 1096-0848 J9 J PARALLEL DISTR COM JI J. Parallel Distrib. Comput. PD NOV PY 2015 VL 85 SI SI BP 91 EP 103 DI 10.1016/j.jpdc.2015.06.008 PG 13 WC Computer Science, Theory & Methods SC Computer Science GA CT2GO UT WOS:000362620200007 ER PT J AU Torres-Castro, L Shojan, J Julien, CM Huq, A Dhital, C Paranthaman, MP Katiyar, RS Manivannan, A AF Torres-Castro, Loraine Shojan, Jifi Julien, Christian M. Huq, Ashfia Dhital, Chetan Paranthaman, Mariappan Parans Katiyar, Ram S. Manivannan, Ayyakkannu TI Synthesis, characterization and electrochemical performance of Al-substituted Li2MnO3 SO MATERIALS SCIENCE AND ENGINEERING B-ADVANCED FUNCTIONAL SOLID-STATE MATERIALS LA English DT Article DE Lithium ion battery; Energy storage; Li2MnO3 cathode; Al substitution ID LITHIUM-ION BATTERIES; CATHODE MATERIALS; BEHAVIOR; OXIDES AB Li2MnO3 is known to be electrochemically inactive due to Mn in tetravalent oxidation state. Several compositions such as Li2MnO3, Li1.5Al0.17MnO3, Li1.0Al0.33MnO3 and Li0.3Al0.5MnO3 were synthesized by a sol-gel Pechini method. All the samples were characterized with XRD, Raman, XPS, SEM, Tap density and BET analyzer. XRD patterns indicated the presence of monoclinic phase for pristine Li2MnO3 and mixed monoclinic/spinel phases (Li2-xMn1-yAlx+yO3+z) for Al-substituted Li2MnO3 compounds. The Al substitution seems to occur both at Li and Mn sites, which could explain the presence of spinel phase. XPS analysis for Mn 2p orbital reveals a significant decrease in binding energy for Li1.0Al0.33MnO3 and Li0.5Al0.5MnO3 compounds. Cyclic voltammetry, charge/discharge cycles and electrochemical impedance spectroscopy were also performed. A discharge capacity of 24 mAh g(-1) for Li2MnO3, 68 mAhg(-1) for Li1.5Al0.17MnO3, 58 mAh g(-1) for Li1.0Al0.33MnO3 and 74 mAh g(-1) for Li0.5Al0.5MnO3 were obtained. Aluminum substitutions increased the formation of spinel phase which is responsible for cycling. Published by Elsevier B.V. C1 [Torres-Castro, Loraine; Shojan, Jifi; Katiyar, Ram S.] Univ Puerto Rico, Dept Phys, San Juan, PR 00931 USA. [Torres-Castro, Loraine; Shojan, Jifi; Katiyar, Ram S.] Univ Puerto Rico, Chem Phys Grad Program, San Juan, PR 00931 USA. [Shojan, Jifi; Katiyar, Ram S.] Univ Puerto Rico, Inst Funct Nanomat, San Juan, PR 00931 USA. [Julien, Christian M.] Univ Paris 06, Physicochim Electrolytes Colloides & Sci Analyt, F-75005 Paris, France. [Huq, Ashfia; Dhital, Chetan] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Paranthaman, Mariappan Parans] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Manivannan, Ayyakkannu] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. [Manivannan, Ayyakkannu] W Virginia Univ, Mech & Aerosp Engn, Morgantown, WV 26507 USA. RP Manivannan, A (reprint author), US DOE, Natl Energy Technol Lab, 3610 Collins Ferry Rd,POB 880, Morgantown, WV 26507 USA. EM manivana@netl.doe.gov RI Paranthaman, Mariappan/N-3866-2015; Huq, Ashfia/J-8772-2013; Dhital, Chetan/O-5634-2016 OI Paranthaman, Mariappan/0000-0003-3009-8531; Huq, Ashfia/0000-0002-8445-9649; Dhital, Chetan/0000-0001-8125-6048 FU NASA-CANM [NNX08BA48A]; NASA [NNX10AM80H]; US Department of Energy (DOE) BATT (Batteries for Advanced Transportation Technology) Program; Division of Scientific User Facilities, Office of Basic Energy Sciences, US Department of Energy with UT-Battelle, LLC [DE-AC05-00OR22725] FX Financial support from the NASA-CANM (Grant # NNX08BA48A), NASA Space Grant (Grant # NNX10AM80H) and the US Department of Energy (DOE) BATT (Batteries for Advanced Transportation Technology) Program are acknowledged. We thank Dr. James Poston from the National Energy Technology Laboratory for his continual support with characterization measurements. Financial and technical supports by Spallation Neutron Source user facility are sponsored by the Division of Scientific User Facilities, Office of Basic Energy Sciences, US Department of Energy, under contract DE-AC05-00OR22725 with UT-Battelle, LLC, are gratefully acknowledged. Support (MPP) for neutron characterizations was provided by Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, US Department of Energy. Fruitful discussions with Ms. Maria Abreu-Sepulveda and Dr. Gurpreet Singh are also acknowledged. NR 30 TC 2 Z9 2 U1 12 U2 72 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0921-5107 EI 1873-4944 J9 MATER SCI ENG B-ADV JI Mater. Sci. Eng. B-Adv. Funct. Solid-State Mater. PD NOV PY 2015 VL 201 BP 13 EP 22 DI 10.1016/j.mseb.2015.07.006 PG 10 WC Materials Science, Multidisciplinary; Physics, Condensed Matter SC Materials Science; Physics GA CT2AS UT WOS:000362605000002 ER PT J AU Javni, I Bilic, O Bilic, N Petrovic, ZS Eastwood, EA Zhang, F Ilavsky, J AF Javni, Ivan Bilic, Olivera Bilic, Nikola Petrovic, Zoran S. Eastwood, Eric A. Zhang, Fan Ilavsky, Jan TI Thermoplastic polyurethanes with controlled morphology based on methylenediphenyldiisocyanate/isosorbide/butanediol hard segments SO POLYMER INTERNATIONAL LA English DT Article DE morphology; segmented polyurethanes; isosorbide; chain extender ID X-RAY-SCATTERING; SMALL-ANGLE SCATTERING; ADVANCED PHOTON SOURCE; BLOCK-COPOLYMERS; ELASTOMERS; DIISOCYANATE; SEPARATION; POLYMERS; SYSTEMS; LENGTH AB Isosorbide, a cyclic, rigid and renewable diol, was used as a chain extender in two series of thermoplastic polyurethanes (PUs). Isosorbide was used alone or in combination with butanediol to examine the effects on the morphology of PU. Two series of materials were prepared-one with dispersed hard domains in a matrix of polytetramethylene ether glycol soft segments of molecular weight 1400gmol(-1) (at 70wt% soft segment concentration, SSC) and the other with co-continuous soft and hard phases at 50wt% SSC. We investigated the detailed morphology of these materials with optical and atomic force microscopy, as well as ultra-small-angle X-ray scattering. The atomic force microscopy measurements confirmed the different morphologies in PUs with 50wt% SSC and with 70wt% SSC. Small-angle X-ray scattering data showed that in PU with 70wt% SSC, the hard domain size varied between 2.4 and 2.9nm, and decreased with increasing isosorbide content. In PU with 70wt% SSC, we found that the correlation length and average repeat distances became smaller with increasing isosorbide content. We estimated the thickness of the diffuse phase boundary for PU with 70wt% SSC to be ca 0.5nm, decreasing slightly with increasing isosorbide content. (c) 2015 Society of Chemical Industry C1 [Javni, Ivan; Bilic, Olivera; Bilic, Nikola; Petrovic, Zoran S.] Pittsburg State Univ, Kansas Polymer Res Ctr, Pittsburg, KS 66762 USA. [Eastwood, Eric A.] Honeywell FM&T LLC, Kansas City, MO 61141 USA. [Zhang, Fan] NIST, Mat Measurement Sci Div, Mat Measurement Lab, Gaithersburg, MD 20899 USA. [Ilavsky, Jan] Argonne Natl Lab, X ray Sci Div, Adv Photon Source, Argonne, IL 60439 USA. RP Petrovic, ZS (reprint author), Pittsburg State Univ, Kansas Polymer Res Ctr, 1701 S Broadway, Pittsburg, KS 66762 USA. EM zpetrovic@pittstate.edu RI Ilavsky, Jan/D-4521-2013 OI Ilavsky, Jan/0000-0003-1982-8900 FU Honeywell; Division of Chemistry (CHE); Division of Materials Research (DMR); National Science Foundation [NSF/CHE-1346572]; US DOE [DE-AC02-06CH11357] FX We are grateful to Honeywell for funding this research. ChemMatCARS Sector 15 is principally supported by the Divisions of Chemistry (CHE) and Materials Research (DMR), National Science Foundation, under grant number NSF/CHE-1346572. Use of the Advanced Photon Source, an Office of Science User Facility operated for the US Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the US DOE under contract no. DE-AC02-06CH11357. NR 29 TC 2 Z9 2 U1 2 U2 33 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0959-8103 EI 1097-0126 J9 POLYM INT JI Polym. Int. PD NOV PY 2015 VL 64 IS 11 BP 1607 EP 1616 DI 10.1002/pi.4960 PG 10 WC Polymer Science SC Polymer Science GA CT1NG UT WOS:000362564600015 ER PT J AU Spataru, S Hacke, P Sera, D Packard, C Kerekes, T Teodorescu, R AF Spataru, Sergiu Hacke, Peter Sera, Dezso Packard, Corinne Kerekes, Tamas Teodorescu, Remus TI Temperature-dependency analysis and correction methods of in situ power-loss estimation for crystalline silicon modules undergoing potential-induced degradation stress testing SO PROGRESS IN PHOTOVOLTAICS LA English DT Article DE potential-induced degradation; crystalline silicon; degradation; current-voltage charactersitic; accelerated stress testing; temperature dependency ID CURRENT-VOLTAGE CHARACTERISTICS; SOLAR-CELL PERFORMANCE; DARK CURRENT; PV MODULES; SUPERPOSITION; PARAMETERS; PRINCIPLE; SYSTEM; MODEL AB We propose a method for in situ characterization of the photovoltaic module power at standard test conditions, using superposition of the dark current-voltage (I-V) curve measured at the elevated stress temperature, during potential-induced degradation (PID) testing. PID chamber studies were performed on several crystalline silicon module designs to determine the extent to which the temperature dependency of maximum power is affected by the degradation of the modules. The results using the superposition principle show a mismatch between the power degradation measured at stress temperature and the degradation measured at 25 degrees C, dependent on module design, stress temperature, and level of degradation. We investigate the correction of this mismatch using two maximum-power temperature translation methods found in the literature. For the first method, which is based on the maximum-power temperature coefficient, we find that the temperature coefficient changes as the module degrades by PID, thus limiting its applicability. The second method investigated is founded on the two-diode model, which allows for fundamental analysis of the degradation, but does not lend itself to large-scale data collection and analysis. Last, we propose and validate experimentally a simpler and more accurate maximum-power temperature translation method, by taking advantage of the near-linear relationship between the mismatch and power degradation. This method reduces test duration and cost, avoids stress transients while ramping to and from the stress temperature, eliminates flash testing except at the initial and final data points, and enables significantly faster and more detailed acquisition of statistical data for future application of various statistical reliability models. Copyright (c) 2015 John Wiley & Sons, Ltd. C1 [Spataru, Sergiu; Sera, Dezso; Kerekes, Tamas; Teodorescu, Remus] Aalborg Univ, Energy Technol, Aalborg, Denmark. [Hacke, Peter; Packard, Corinne] Natl Renewable Energy Lab, Golden, CO USA. [Packard, Corinne] Colorado Sch Mines, Met & Mat Engn, Golden, CO 80401 USA. RP Spataru, S (reprint author), Aalborg Univ, Energy Technol, Aalborg, Denmark. EM ssp@et.aau.dk RI Kerekes, Tamas/B-8647-2016; Packard, Corinne/A-9606-2010; Teodorescu, Remus/O-5224-2015; OI Kerekes, Tamas/0000-0001-7594-3298; Packard, Corinne/0000-0002-5815-8586; Teodorescu, Remus/0000-0002-2617-7168; Sera, Dezso/0000-0001-9050-2423; Spataru, Sergiu/0000-0001-8112-2779 FU Energinet.dk, Aalborg University [10648]; U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory FX The authors thank Bill Marion and Sarah Kurtz for helpful discussions; Garry Babbitt for developing the hardware of the experimental setup; Greg Perrin and Kent Terwilliger for their help performing the experiments; Steve Glick and Steve Rummel for module measurements. This work was realized within the research project "Smart photovoltaic systems", project no. 10648 supported by Energinet.dk, Aalborg University, as well as the U.S. Department of Energy under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. NR 34 TC 8 Z9 8 U1 4 U2 15 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1062-7995 EI 1099-159X J9 PROG PHOTOVOLTAICS JI Prog. Photovoltaics PD NOV PY 2015 VL 23 IS 11 BP 1536 EP 1549 DI 10.1002/pip.2587 PG 14 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA CT4SD UT WOS:000362796500011 ER PT J AU Muller, M Kurtz, S Steiner, M Siefer, G AF Muller, Matthew Kurtz, Sarah Steiner, Marc Siefer, Gerald TI Translating outdoor CPV I-V measurements to a CSTC power rating and the associated uncertainty SO PROGRESS IN PHOTOVOLTAICS LA English DT Article DE CSTC; concentrator PV; I-V translation; temperature coefficients; power rating ID SOLAR-CELLS; TEMPERATURE; PERFORMANCE; JUNCTION AB A complete procedure is presented for translating outdoor concentrator photovoltaic (CPV) I-V measurements to the Concentrator Standard Test Conditions (CTSC) (1000W/m(2) and 25 degrees C cell temperature). Methods are demonstrated for measuring all the necessary input parameters for the translation, including outdoor thermal transient measurements and indoor dark I-V curves. Four modules are subjected to the translation method based on multiple months of outdoor data, one module measured at National Renewable Energy Laboratory and three at Fraunhofer ISE. The modules are also characterized under a sun simulator to provide a comparison to the translation approach. The results show that translated CSTC efficiencies are in good agreement with the efficiencies from the solar simulator. Two of the modules agreed within 1%, whereas the other two modules agree within approximately 4%. An uncertainty analysis of the input parameters is discussed in the context of the total uncertainty associated with the translation to CSTC. The reference voltage and efficiency temperature coefficient are the key parameters impacting the translation uncertainty, whereas uncertainty in the outdoor data is driven by spectral and meteorological parameters. Copyright (c) 2015 John Wiley & Sons, Ltd. C1 [Muller, Matthew; Kurtz, Sarah] Natl Renewable Energy Lab, Golden, CO USA. [Steiner, Marc; Siefer, Gerald] Natl Renewable Energy Lab, Golden, CO 80401 USA. Fraunhofer ISE, Freiburg, Germany. RP Muller, M (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM matthew.muller@nrel.gov FU US Department of Energy [DE-AC36-99GO10337] FX The authors wish to thank J. Rodriguez for technical assistance with data collection at NREL. Special thanks are given to Fraunhofer ISE for hosting an exchange scientist from NREL and making the collaborative work presented here possible. This work was completed under Contract No. DE-AC36-99GO10337 with the US Department of Energy. NR 31 TC 12 Z9 12 U1 1 U2 1 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1062-7995 EI 1099-159X J9 PROG PHOTOVOLTAICS JI Prog. Photovoltaics PD NOV PY 2015 VL 23 IS 11 BP 1557 EP 1571 DI 10.1002/pip.2590 PG 15 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA CT4SD UT WOS:000362796500013 ER PT J AU Chu, JP Hsiung, GY Kinsho, M Hseuh, HC Wuest, M Chen, JR Leou, KC Fang, JS AF Chu, Jinn P. Hsiung, Gao-Yu Kinsho, Michikazu Hseuh, Hsiao-Chaun Wueest, Martin Chen, June-Rong Leou, Keh-Chyang Fang, Jau-Shiung TI Preface for VASSCAA7 special issue of VACUUM SO VACUUM LA English DT Editorial Material DE IUVSTA; VASSCAA-7; Taiwan; Vacuum technology; Plasma; Energy; Thin film C1 [Chu, Jinn P.] Natl Taiwan Univ Sci & Technol, Taipei, Taiwan. [Hsiung, Gao-Yu; Chen, June-Rong] Natl Synchrotron Radiat Res Ctr, Taipei, Taiwan. [Kinsho, Michikazu] Japan Atom Energy Agcy, J PARC Ctr, Tokyo, Japan. [Hseuh, Hsiao-Chaun] Brookhaven Natl Lab, NSLS 2, Upton, NY 11973 USA. [Wueest, Martin] INFICON, Zurich, Switzerland. [Chen, June-Rong; Leou, Keh-Chyang] Natl Tsing Hua Univ, Taipei, Taiwan. [Fang, Jau-Shiung] Natl Formosa Univ, Taipei, Taiwan. RP Hsiung, GY (reprint author), Natl Synchrotron Radiat Res Ctr, Taipei, Taiwan. EM hsiung@nsrrc.org.tw NR 0 TC 0 Z9 0 U1 0 U2 0 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0042-207X J9 VACUUM JI Vacuum PD NOV PY 2015 VL 121 BP 236 EP 237 DI 10.1016/j.vacuum.2015.08.004 PG 2 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA CT2GC UT WOS:000362619000038 ER PT J AU Moore, BC Coleman, AM Wigmosta, MS Skaggs, RL Venteris, ER AF Moore, Brandon C. Coleman, Andre M. Wigmosta, Mark S. Skaggs, Richard L. Venteris, Erik R. TI A High Spatiotemporal Assessment of Consumptive Water Use and Water Scarcity in the Conterminous United States SO WATER RESOURCES MANAGEMENT LA English DT Article DE Water demand; Water supply; Energy security; Water-energy nexus; Sustainability; Agriculture; Bioenergy ID HYDROLOGICALLY BASED DATASET; LAND-SURFACE FLUXES AB There is an inextricable link between energy production and food/feed/fiber cultivation with available water resources. Currently in the United States, agriculture represents the largest sector of consumptive water use making up 80.7 % of the total. Electricity generation in the U.S. is projected to increase by 24 % in the next two decades and globally, the production of liquid transportation fuels are forecasted to triple over the next 25-years, having significant impacts on the import/export market and global economies. The tension between local water supply and demand across water use sectors needs to be evaluated with regards to risk evaluation and planning. To this end, we present a systematic method to spatially and temporally disaggregate nationally available 5-year county-scale water use data to a monthly 1/8A degrees scale. Our study suggests that while 81.9 % of the U.S. exhibits unstressed local conditions at the annual scale, 13.7 % is considered water scarce; this value increases to 17.3 % in the summer months. The use of mean annual water scarcity at a coarser basin scale (similar to 373,000 ha) was found to mask information critical for water planning whereas finer spatiotemporal scales revealed local areas that are water stressed or water scarce. Nationally, similar to 1 % of these "unstressed" basins actually contained water stressed or water scarce areas equivalent to at least 30 % and 17 %, respectively, of the basin area. These percentages increase to 34 % and 48 % in the summer months. Additionally, 15 % of basins classified as "unstressed" contained water scarce areas in excess of 10 % during the summer. C1 [Moore, Brandon C.; Coleman, Andre M.; Wigmosta, Mark S.; Skaggs, Richard L.; Venteris, Erik R.] Pacific NW Natl Lab, Hydrol Tech Grp, Richland, WA 99352 USA. [Moore, Brandon C.] Univ Idaho, Dept Geog, Moscow, ID 83844 USA. [Coleman, Andre M.] Clemson Univ, Glenn Dept Civil Engn, Clemson, SC 29634 USA. RP Coleman, AM (reprint author), Pacific NW Natl Lab, Hydrol Tech Grp, MSIN K9-33,POB 999, Richland, WA 99352 USA. EM Andre.Coleman@pnnl.gov FU Analysis and Sustainability Program of the Bioenergy Technology Office under the U.S. Department of Energy's Office of Energy Efficiency & Renewable Energy; U.S. Department of Energy [DE-AC06-76RLO1830] FX Support for this research was provided by the Analysis and Sustainability Program of the Bioenergy Technology Office under the U.S. Department of Energy's Office of Energy Efficiency & Renewable Energy. The Pacific Northwest National Laboratory is operated by Battelle Memorial Institute for the U.S. Department of Energy under contract DE-AC06-76RLO1830. NR 49 TC 2 Z9 2 U1 5 U2 31 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0920-4741 EI 1573-1650 J9 WATER RESOUR MANAG JI Water Resour. Manag. PD NOV PY 2015 VL 29 IS 14 BP 5185 EP 5200 DI 10.1007/s11269-015-1112-x PG 16 WC Engineering, Civil; Water Resources SC Engineering; Water Resources GA CS9PB UT WOS:000362422100017 ER PT J AU Miao, L Massoudi, M AF Miao, Ling Massoudi, Mehrdad TI Heat transfer analysis and flow of a slag-type fluid: Effects of variable thermal conductivity and viscosity SO INTERNATIONAL JOURNAL OF NON-LINEAR MECHANICS LA English DT Article DE Non-Newtonian fluids; Thermal conductivity; Viscosity; Slag; Heat transfer ID STEEL; DEPENDENCE; SPHERES; FOURIER; MODEL; LAYER; LAW AB In this paper we study the effects of variable viscosity and thermal conductivity on the heat transfer and flow of a slag-type non-Newtonian fluid between two horizontal flat plates. We solve the governing equations in their non-dimensional forms and perform a parametric study to see the effects of various dimensionless numbers on the velocity, volume fraction and temperature profiles. The different cases of shear- thinning and thickening, and the effect of the exponent in the Reynolds viscosity model, for the temperature variation in viscosity, are also considered. Published by Elsevier Ltd. C1 [Miao, Ling] Univ Pittsburgh, Dept Mech Engn & Mat Sci, Pittsburgh, PA 15261 USA. [Massoudi, Mehrdad] Natl Energy Technol Lab, US Dept Energy, Pittsburgh, PA 15236 USA. RP Massoudi, M (reprint author), Natl Energy Technol Lab, US Dept Energy, 626 Cochrans Mill Rd,POB 10940, Pittsburgh, PA 15236 USA. EM mehrdad.massoudi@netl.doe.gov NR 46 TC 5 Z9 5 U1 3 U2 13 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0020-7462 EI 1878-5638 J9 INT J NONLIN MECH JI Int. J. Non-Linear Mech. PD NOV PY 2015 VL 76 BP 8 EP 19 DI 10.1016/j.ijnonlinmec.2015.05.001 PG 12 WC Mechanics SC Mechanics GA CS5RL UT WOS:000362135600002 ER PT J AU Sunay, UR Zvanut, ME Allerman, AA AF Sunay, U. R. Zvanut, M. E. Allerman, A. A. TI Reduction in the Number of Mg Acceptors with Al Concentration in Al (x) Ga1-x N SO JOURNAL OF ELECTRONIC MATERIALS LA English DT Article DE Nitride; p-type; GaN; Mg; magnetic resonance ID THREADING DISLOCATIONS; GAN; ALXGA1-XN; ALGAN AB High hole concentrations in Al (x) Ga1-x N become increasingly difficult to obtain as the Al mole fraction increases. The problem is believed to be related to compensation, extended defects, and the band gap of the alloy. Whereas electrical measurements are commonly used to measure hole density, in this work we used electron paramagnetic resonance (EPR) spectroscopy to investigate a defect related to the neutral Mg acceptor. The amount and symmetry of neutral Mg in MOCVD-grown Al (x) Ga1-x N with x = 0 to 0.28 was monitored for films with different dislocation densities and surface conditions. EPR measurements indicated that the amount of neutral Mg decreased by 60% in 900A degrees C-annealed Al (x) Ga1-x N films for x = 0.18 and 0.28 as compared with x = 0.00 and 0.08. A decrease in the angular dependence of the EPR signal accompanied the increased x, suggesting a change in the local environment of the Mg. Neither dislocation density nor annealing conditions contribute to the reduced amount of neutral Mg in samples with the higher Al concentration. Rather, compensation is the simplest explanation of the observations, because a donor could both reduce the number of neutral acceptors and cause the variation in the angular dependence. C1 [Sunay, U. R.; Zvanut, M. E.] Univ Alabama Birmingham, Dept Phys, Birmingham, AL 35294 USA. [Allerman, A. A.] Sandia Natl Labs, Albuquerque, NM 87123 USA. RP Sunay, UR (reprint author), Univ Alabama Birmingham, Dept Phys, 1530 3rd Ave S, Birmingham, AL 35294 USA. EM ustuns1@uab.edu FU National Science foundation [DMR1006163]; US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work is funded by the National Science foundation DMR1006163. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under contract no. DE-AC04-94AL85000. NR 16 TC 1 Z9 1 U1 7 U2 33 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0361-5235 EI 1543-186X J9 J ELECTRON MATER JI J. Electron. Mater. PD NOV PY 2015 VL 44 IS 11 BP 4139 EP 4143 DI 10.1007/s11664-014-3475-9 PG 5 WC Engineering, Electrical & Electronic; Materials Science, Multidisciplinary; Physics, Applied SC Engineering; Materials Science; Physics GA CS2LS UT WOS:000361903000008 ER PT J AU Rohwer, LES Martin, JE AF Rohwer, Lauren E. S. Martin, James E. TI Platelet Composite Coatings for Tin Whisker Mitigation SO JOURNAL OF ELECTRONIC MATERIALS LA English DT Article DE Polymer-matrix composites; electrical properties; thermal properties; tin whisker mitigation; filled conformal coating ID HELIUM GAS-PERMEABILITY; THERMAL-CONDUCTIVITY; TRANSPORT-PROPERTIES; NANOCOMPOSITES; GROWTH; FILMS; SN; BARRIER AB Reliable methods for tin whisker mitigation are needed for applications that utilize tin-plated commercial components. Tin can grow whiskers that can lead to electrical shorting, possibly causing critical systems to fail catastrophically. The mechanisms of tin whisker growth are unclear and this makes prediction of the lifetimes of critical components uncertain. The development of robust methods for tin whisker mitigation is currently the best approach to eliminating the risk of shorting. Current mitigation methods are based on unfilled polymer coatings that are not impenetrable to tin whiskers. In this paper we report tin whisker mitigation results for several filled polymer coatings. The whisker-penetration resistance of the coatings was evaluated at elevated temperature and high humidity and under temperature cycling conditions. The composite coatings comprised Ni and MgF2-coated Al/Ni/Al platelets in epoxy resin or silicone rubber. In addition to improved whisker mitigation, these platelet composites have enhanced thermal conductivity and dielectric constant compared with unfilled polymers. C1 [Rohwer, Lauren E. S.; Martin, James E.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Rohwer, LES (reprint author), Sandia Natl Labs, POB 5800,MS-1425, Albuquerque, NM 87185 USA. EM leshea@sandia.gov FU United States Department of Energy's National Nuclear Safety Administration [DE-AC04-94AL85000]; Joint Department of Defense/Department of Energy Munitions Technology Development Program FX Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed-Martin Company, for the United States Department of Energy's National Nuclear Safety Administration under contract No. DE-AC04-94AL85000. This work was supported in part by the Joint Department of Defense/Department of Energy Munitions Technology Development Program. We thank: Joseph Aragon for components selection and coordinating the fusing, solder dipping, and Pb plating experiments; Bonnie Mckenzie and Ben Thurston for SEM images; Mark Grazier for temperature cycling; John White and Paul Sandoval for temperature-humidity testing; Steve Limmer for tin-plated test coupons; Sylvia Gomez-Vasquez for thermal diffusivity measurements; and Mark Stavig for thermomechanical analysis. NR 41 TC 0 Z9 0 U1 1 U2 10 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0361-5235 EI 1543-186X J9 J ELECTRON MATER JI J. Electron. Mater. PD NOV PY 2015 VL 44 IS 11 BP 4424 EP 4433 DI 10.1007/s11664-015-4026-8 PG 10 WC Engineering, Electrical & Electronic; Materials Science, Multidisciplinary; Physics, Applied SC Engineering; Materials Science; Physics GA CS2LS UT WOS:000361903000046 ER PT J AU Wang, HS Bai, SQ Chen, LD Cuenat, A Joshi, G Kleinke, H Konig, J Lee, HW Martin, J Oh, MW Porter, WD Ren, ZF Salvador, J Sharp, J Taylor, P Thompson, AJ Tseng, YC AF Wang, Hsin Bai, Shengqiang Chen, Lidong Cuenat, Alexander Joshi, Giri Kleinke, Holger Koenig, Jan Lee, Hee Woong Martin, Joshua Oh, Min-Wook Porter, Wallace D. Ren, Zhifeng Salvador, James Sharp, Jeff Taylor, Patrick Thompson, Alan J. Tseng, Y. C. TI International Round-Robin Study of the Thermoelectric Transport Properties of an n-Type Half-Heusler Compound from 300 K to 773 K SO JOURNAL OF ELECTRONIC MATERIALS LA English DT Article DE Thermoelectric; figure of merit; ZT; round-robin ID BULK THERMOELECTRICS; LEAD-TELLURIDE; THERMAL-CONDUCTIVITY; FIGURE; MERIT; CRYSTAL; ZRNISN; SEMICONDUCTOR; SKUTTERUDITES; SUBSTITUTION AB International transport property-measurement round-robins have been conducted by the thermoelectric annex under the International Energy Agency (IEA) Implementing Agreement on Advanced Materials for Transportation (AMT). Two previous round-robins used commercially available bismuth telluride as the test material, with the objectives of understanding measurement issues and developing standard testing procedures. This round-robin extended the measurement temperature range to 773 K. It was designed to meet the increasing demands for reliable transport data for thermoelectric materials used for power-generation applications. Eleven laboratories from six IEA-AMT member countries participated in the study. A half-Heusler (n-type) material prepared by GMZ Energy was selected for the round-robin. The measured transport properties had a narrower distribution of uncertainty than previous round-robin results. The study intentionally included multiple testing methods and instrument types. Over the full temperature range, the measurement discrepancies for the figure of merit, ZT, in this round-robin were +/- 11.5 to +/- 16.4% from the averages. C1 [Wang, Hsin; Porter, Wallace D.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Bai, Shengqiang; Chen, Lidong] Chinese Acad Sci, Shanghai Inst Ceram, Shanghai 200050, Peoples R China. [Cuenat, Alexander] NPL, Teddington, Middx, England. [Joshi, Giri] GMZ Energy, Waltham, MA USA. [Kleinke, Holger] Univ Waterloo, Waterloo, ON N2L 3G1, Canada. [Koenig, Jan] Fraunhofer Inst Phys Measurement Tech, Freiburg, Germany. [Lee, Hee Woong; Oh, Min-Wook] Korea Electrotechnol Res Inst, Anshan, South Korea. [Martin, Joshua] NIST, Gaithersburg, MD 20899 USA. [Ren, Zhifeng] Univ Houston, Houston, TX USA. [Salvador, James] Gen Motors Global R&D, Warren, MI USA. [Sharp, Jeff; Thompson, Alan J.] Marlow Ind, Dallas, TX USA. [Taylor, Patrick] Army Res Lab, Adelphi, MD USA. [Tseng, Y. C.] CanmetMAT, Hamilton, ON, Canada. [Joshi, Giri] Evident Thermoelect, Troy, NY USA. RP Wang, HS (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM wangh2@ornl.gov RI Chen, Lidong/F-2705-2010; Wang, Hsin/A-1942-2013 OI Wang, Hsin/0000-0003-2426-9867 FU International Energy Agency; Natural Resources Canada; International S&T Cooperation Program of China [2015DFA51050]; Oak Ridge National Laboratory [DE-AC 05000OR22725] FX The paper describes work being conducted is part of the Implementing Agreement on Advanced Materials for Transportation under the auspices of the International Energy Agency. The authors would like to acknowledge financial support by Natural Resources Canada for the work conducted at CanmetMATERIALS, the International S&T Cooperation Program of China (2015DFA51050), and the home institution of each participating laboratory. HW would like to thank the assistant secretary for Energy Efficiency and Renewable Energy of the Department of Energy and the Propulsion Materials program under the Vehicle Technologies program, and Oak Ridge National Laboratory managed by UT-Battelle LLC under contract DE-AC 05000OR22725. NR 51 TC 4 Z9 4 U1 9 U2 48 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0361-5235 EI 1543-186X J9 J ELECTRON MATER JI J. Electron. Mater. PD NOV PY 2015 VL 44 IS 11 BP 4482 EP 4491 DI 10.1007/s11664-015-4006-z PG 10 WC Engineering, Electrical & Electronic; Materials Science, Multidisciplinary; Physics, Applied SC Engineering; Materials Science; Physics GA CS2LS UT WOS:000361903000052 ER PT J AU Henager, CH Alvine, KJ Bliss, M Riley, BJ Stave, JA AF Henager, Charles H., Jr. Alvine, Kyle J. Bliss, Mary Riley, Brian J. Stave, Jean A. TI The Influence of Constitutional Supercooling on the Distribution of Te-Particles in Melt-Grown CZT SO JOURNAL OF ELECTRONIC MATERIALS LA English DT Article DE CZT; Te-particles; constitutional supercooling; particle distributions; Rayleigh instability; crystal characterization ID CADMIUM ZINC TELLURIDE; VERTICAL BRIDGMAN GROWTH; CDZNTE RADIATION DETECTORS; CRYSTAL-GROWTH; STIRRED MELTS; CRUCIBLE ROTATION; EXTENDED DEFECTS; DOPED GERMANIUM; CDTE CRYSTALS; CD0.9ZN0.1TE AB A section of a vertical gradient freeze Cd0.9Zn0.1Te boule approximately 2100 mm(3) with a planar area of 300 mm(2) was prepared and examined using transmitted infrared microscopy at various magnifications to determine the three-dimensional spatial and size distributions of Te-particles over large longitudinal and radial length scales. Te-particle density distributions were determined as a function of longitudinal and radial positions in these strips and exhibited a multi-modal log-normal size density distribution that indicated a slight preference for increasing size with longitudinal growth time, while showing a pronounced cellular network structure. Higher magnification images revealed a typical Rayleigh-instability pearl string morphology with large and small satellite droplets. This study includes solidification experiments in small crucibles of 30:70 mixtures of Cd:Te performed over a wide range of cooling rates which clearly demonstrated a growth instability with Te-particle capture that is suggested to be responsible for one of the peaks in the size distribution using size discrimination visualization. The results are discussed with regard to a manifold Te-particle genesis history as Te-particle direct capture from melt-solid growth instabilities due to constitutional supercooling and as Te-particle formation from the breakup of Te-ribbons via a Rayleigh-Plateau instability. C1 [Henager, Charles H., Jr.; Alvine, Kyle J.; Bliss, Mary; Riley, Brian J.; Stave, Jean A.] PNNL, Richland, WA 99352 USA. RP Henager, CH (reprint author), PNNL, POB 999, Richland, WA 99352 USA. EM chuck.henager@pnnl.gov RI Bliss, Mary/G-2240-2012; OI Bliss, Mary/0000-0002-7565-4813; Henager, Chuck/0000-0002-8600-6803; Riley, Brian/0000-0002-7745-6730 FU U.S. Department of Energy [DE-AC06-76RLO 1830]; Office of Defense Nuclear Nonproliferation, Office of Nonproliferation Research and Development, U.S. Department of Energy [NA-22, DE-AC05-00OR-22725]; UT-Battelle, LLC FX PNNL is operated for the U.S. Department of Energy by Battelle Memorial Institute under Contract DE-AC06-76RLO 1830. The Office of Defense Nuclear Nonproliferation, Office of Nonproliferation Research and Development (NA-22), U.S. Department of Energy funded this work at PNNL under contract DE-AC05-00OR-22725 with UT-Battelle, LLC. NR 58 TC 1 Z9 1 U1 5 U2 16 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0361-5235 EI 1543-186X J9 J ELECTRON MATER JI J. Electron. Mater. PD NOV PY 2015 VL 44 IS 11 BP 4604 EP 4621 DI 10.1007/s11664-015-3995-y PG 18 WC Engineering, Electrical & Electronic; Materials Science, Multidisciplinary; Physics, Applied SC Engineering; Materials Science; Physics GA CS2LS UT WOS:000361903000065 ER PT J AU Dempsey, AB Curran, S Wagner, R Cannella, W AF Dempsey, Adam B. Curran, Scott Wagner, Robert Cannella, William TI Effect of Premixed Fuel Preparation for Partially Premixed Combustion With a Low Octane Gasoline on a Light-Duty Multicylinder Compression Ignition Engine SO JOURNAL OF ENGINEERING FOR GAS TURBINES AND POWER-TRANSACTIONS OF THE ASME LA English DT Article AB Gasoline compression ignition (GCI) concepts with the majority of the fuel being introduced early in the cycle are known as partially premixed combustion (PPC). Previous research on single-and multicylinder engines has shown that PPC has the potential for high thermal efficiency with low NOx and soot emissions. A variety of fuel injection strategies have been proposed in the literature. These injection strategies aim to create a partially stratified charge to simultaneously reduce NOx and soot emissions while maintaining some level of control over the combustion process through the fuel delivery system. The impact of the direct injection (DI) strategy to create a premixed charge of fuel and air has not previously been explored, and its impact on engine efficiency and emissions is not well understood. This paper explores the effect of sweeping the direct injected pilot timing from -91 deg to -324 deg ATDC, which is just after the exhaust valve closes (EVCs) for the engine used in this study. During the sweep, the pilot injection consistently contained 65% of the total fuel (based on command duration ratio), and the main injection timing was adjusted slightly to maintain combustion phasing near top dead center. A modern four cylinder, 1.9 l diesel engine with a variable geometry turbocharger (VGT), high pressure common rail injection system, wide included angle injectors, and variable swirl actuations was used in this study. The pistons were modified to an open bowl configuration suitable for highly premixed combustion modes. The stock diesel injection system was unmodified, and the gasoline fuel was doped with a lubricity additive to protect the high pressure fuel pump and the injectors. The study was conducted at a fixed speed/load condition of 2000 rpm and 4.0 bar brake mean effective pressure (BMEP). The pilot injection timing sweep was conducted at different intake manifold pressures, swirl levels, and fuel injection pressures. The gasoline used in this study has relatively high fuel reactivity with a research octane number of 68. The results of this experimental campaign indicate that the highest brake thermal efficiency (BTE) and lowest emissions are achieved simultaneously with the earliest pilot injection timings (i.e., during the intake stroke). C1 [Dempsey, Adam B.; Curran, Scott; Wagner, Robert] Oak Ridge Natl Lab, Fuels Engines & Emiss Res Ctr, Natl Transportat Res Ctr, Knoxville, TN 37932 USA. [Cannella, William] Chevron Energy Technol Co, San Ramon, CA 94583 USA. RP Dempsey, AB (reprint author), Oak Ridge Natl Lab, Fuels Engines & Emiss Res Ctr, Natl Transportat Res Ctr, 2360 Cherahala Blvd, Knoxville, TN 37932 USA. EM dempsab@gmail.com OI Curran, Scott/0000-0002-4665-0231 FU U.S. Department of Energy's Vehicle Technologies Office under Fuel and Lubricant Technologies subprogram; U.S. Department of Energy [DE-AC05-00OR22725] FX This work was supported by the U.S. Department of Energy's Vehicle Technologies Office under the Fuel and Lubricant Technologies subprogram managed by Kevin Stork. The authors would like to thank Jim Szybist, Derek Splitter, Ben Lawler, and Brian Kaul from the Oak Ridge National Laboratory for many helpful discussions about low temperature combustion with gasoline. The fuel used in this study was provided by Chevron. This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. NR 22 TC 2 Z9 2 U1 2 U2 19 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0742-4795 EI 1528-8919 J9 J ENG GAS TURB POWER JI J. Eng. Gas. Turbines Power-Trans. ASME PD NOV PY 2015 VL 137 IS 11 AR 111506 DI 10.1115/1.4030281 PG 12 WC Engineering, Mechanical SC Engineering GA CS3FR UT WOS:000361957800006 ER PT J AU Pei, YJ Mehl, M Liu, W Lu, TF Pitz, WJ Som, S AF Pei, Yuanjiang Mehl, Marco Liu, Wei Lu, Tianfeng Pitz, William J. Som, Sibendu TI A Multicomponent Blend as a Diesel Fuel Surrogate for Compression Ignition Engine Applications SO JOURNAL OF ENGINEERING FOR GAS TURBINES AND POWER-TRANSACTIONS OF THE ASME LA English DT Article ID HIGH-TEMPERATURE OXIDATION; HIGH-PRESSURE; COMBUSTION; MODEL; TOLUENE; XYLENE; SPRAY; COUNTERFLOW; CHEMISTRY; MECHANISM AB A mixture of n-dodecane and m-xylene is investigated as a diesel fuel surrogate for compression ignition (CI) engine applications. Compared to neat n-dodecane, this binary mixture is more representative of diesel fuel because it contains an alkyl-benzene which represents an important chemical class present in diesel fuels. A detailed multicomponent mechanism for n-dodecane and m-xylene was developed by combining a previously developed n-dodecane mechanism with a recently developed mechanism for xylenes.The xylene mechanism is shown to reproduce experimental ignition data from a rapid compression machine (RCM) and shock tube (ST), speciation data from the jet stirred reactor and flame speed data. This combined mechanism was validated by comparing predictions from the model with experimental data for ignition in STs and for reactivity in a flow reactor. The combined mechanism, consisting of 2885 species and 11,754 reactions, was reduced to a skeletal mechanism consisting 163 species and 887 reactions for 3D diesel engine simulations. The mechanism reduction was performed using directed relation graph (DRG) with expert knowledge (DRG-X) and DRG-aided sensitivity analysis (DRGASA) at a fixed fuel composition of 77% of n-dodecane and 23% m-xylene by volume. The sample space for the reduction covered pressure of 1-80 bar, equivalence ratio of 0.5-2.0, and initial temperature of 700-1600K for ignition. The skeletal mechanism was compared with the detailed mechanism for ignition and flow reactor predictions. Finally, the skeletal mechanism was validated against a spray flame dataset under diesel engine conditions documented on the engine combustion network (ECN) website. These multidimensional simulations were performed using a representative interactive flame (RIF) turbulent combustion model. Encouraging results were obtained compared to the experiments with regard to the predictions of ignition delay and lift-off length at different ambient temperatures. C1 [Pei, Yuanjiang; Som, Sibendu] Argonne Natl Lab, Transportat Technol R&D Ctr, Argonne, IL 60439 USA. [Mehl, Marco; Pitz, William J.] Lawrence Livermore Natl Lab, Div Chem Sci, Livermore, CA 94550 USA. [Liu, Wei] Argonne Natl Lab, Chem S&E Div, Argonne, IL 60439 USA. [Lu, Tianfeng] Univ Connecticut, Dept Mech Engn, Storrs, CT 06269 USA. RP Pei, YJ (reprint author), Argonne Natl Lab, Transportat Technol R&D Ctr, 9700 S Cass Ave, Argonne, IL 60439 USA. EM ypei@anl.gov RI Mehl, Marco/A-8506-2009 OI Mehl, Marco/0000-0002-2227-5035 FU U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357]; DOEs Office of Vehicle Technologies, Office of Energy Efficiency and Renewable Energy [DE-AC02-06CH11357]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-AC02-06CH11357]; National Science Foundation; Department of Energy through NSF-DOE Partnership on Advanced Combustion Engines Program [CBET-1258646]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; U.S. Department of Energy, Office of Vehicle Technologies FX The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory (Argonne). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government.; The research was funded by DOEs Office of Vehicle Technologies, Office of Energy Efficiency and Renewable Energy under Contract No. DE-AC02-06CH11357. The authors wish to thank Gurpreet Singh, program manager at DOE, for his support. This work was also supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, under Contract No. DE-AC02-06CH11357.; The work at UCONN was supported by the National Science Foundation and the Department of Energy through the NSF-DOE Partnership on Advanced Combustion Engines Program under Grant No. CBET-1258646.; The LLNL work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344 and was supported by the U.S. Department of Energy, Office of Vehicle Technologies (program manager Gurpreet Singh and Leo Breton). NR 64 TC 7 Z9 7 U1 2 U2 15 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0742-4795 EI 1528-8919 J9 J ENG GAS TURB POWER JI J. Eng. Gas. Turbines Power-Trans. ASME PD NOV PY 2015 VL 137 IS 11 AR 111502 DI 10.1115/1.4030416 PG 9 WC Engineering, Mechanical SC Engineering GA CS3FR UT WOS:000361957800002 ER PT J AU Ding, Y Liu, YZ Pradel, KC Bando, Y Fukata, N Wang, ZL AF Ding, Yong Liu, Yuzi Pradel, Ken C. Bando, Yoshio Fukata, Naoki Wang, Zhong Lin TI Quantifying mean inner potential of ZnO nanowires by off-axis electron holography SO MICRON LA English DT Article DE Off-axis electron holography; Mean inner potential; ZnO; Convergent beam electron diffraction ID NANOPIEZOTRONICS; SEMICONDUCTORS; CRYSTAL AB Off-axis electron holography has been used to quantitatively determine the mean inner potential of ZnO. [0 0 0 1] grown ZnO nanowires with hexagonal cross-sections were chosen as our samples because the angle between the adjacent surfaces is 120 degrees, as confirmed by electron tomography, so the entire geometry of the nanowire could be precisely determined. The acceleration voltage of the transmission electron microscope was accurately calibrated by convergent beam electron diffraction (CBED)-higher-order Laue-zone (HOLZ) analyses. ZnO nanowires were tilted away from zone-axis to avoid strong dynamical diffraction effect, and the tilting angles were determined by CBED patterns. Our experimental data found a mean inner potential of ZnO as 14.30 +/- 0.28 V. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Ding, Yong; Pradel, Ken C.; Wang, Zhong Lin] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA. [Liu, Yuzi] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Bando, Yoshio; Fukata, Naoki] Natl Inst Mat Sci, Int Ctr Mat Nanoarchitecton, Tsukuba, Ibaraki 3050044, Japan. RP Ding, Y (reprint author), Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA. EM yong.ding@mse.gatech.edu RI Wang, Zhong Lin/E-2176-2011; Liu, Yuzi/C-6849-2011; Ding, Yong/F-3705-2017 OI Wang, Zhong Lin/0000-0002-5530-0380; Ding, Yong/0000-0001-5805-347X FU National Science Foundation [DMR-1505319]; MANA, National Institute for Materials Science, Japan; Center for Nanoscale Materials, a U.S. Department of Energy Office of Science User Facility [DE-AC02-06CH11357] FX Research was supported by the National Science Foundation (DMR-1505319), and MANA, National Institute for Materials Science, Japan. This work was performed, in part, at the Center for Nanoscale Materials, a U.S. Department of Energy Office of Science User Facility under Contract No. DE-AC02-06CH11357. NR 22 TC 3 Z9 3 U1 3 U2 37 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0968-4328 J9 MICRON JI Micron PD NOV PY 2015 VL 78 BP 67 EP 72 DI 10.1016/j.micron.2015.07.008 PG 6 WC Microscopy SC Microscopy GA CS1TB UT WOS:000361849500009 PM 26277083 ER PT J AU Zhao, MJ Kim, YS Srebric, J AF Zhao, Mingjie Kim, Yang-Seon Srebric, Jelena TI Occupant perceptions and a health outcome in retail stores SO BUILDING AND ENVIRONMENT LA English DT Article DE Indoor environmental quality; Retail stores; Survey; Field study; Occupant perceptions; Common cold ID INDOOR AIR-QUALITY; LARGE OFFICE BUILDINGS; CO2 CONCENTRATIONS; SHOPPING MALLS; VENTILATION; TEMPERATURE; FORMALDEHYDE; ENVIRONMENT; IRRITATION; RESPONSES AB Indoor Environmental Quality (IEQ) in commercial buildings, such as retail stores, can affect employee satisfaction, productivity, and health. This study administered an IEQ survey to retail employees and found correlations between measured IEQ parameters and the survey responses. The survey included 611 employees in 14 retail stores located in Pennsylvania (climate zone 5A) and Texas (climate zone 2A). The survey questionnaire featured ratings of different aspects of IEQ including thermal comfort, lighting and noise level, indoor smells, overall cleanness, and environmental quality. Simultaneously with the survey, on-site physical measurements were taken to collect data of relative humidity levels, air exchange rates, dry bulb temperatures, and contaminant concentrations. This data was analyzed using multinomial logit regression with independent variables being the measured IEQ parameters, employees' gender, and age. This study found that employee perception of stuffy smells is related to formaldehyde and PM2.5 concentrations. Furthermore, the survey also asked the employees to report an annual frequency of common colds as a health indicator. The regression analysis showed that the cold frequency statistically correlates with the measured air exchange rates, outdoor temperatures, and indoor PM2.5 concentrations. Overall, the air exchange rate is the most influential parameter on the employee perception of the overall environmental quality and self-reported health outcome. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Zhao, Mingjie] Pacific NW Natl Lab, Richland, WA 99352 USA. [Kim, Yang-Seon; Srebric, Jelena] Univ Maryland, Dept Mech Engn, College Pk, MD 20742 USA. RP Srebric, J (reprint author), 3143 Glenn L Martin Hall, College Pk, MD 20742 USA. EM jsrebric@umd.edu OI Srebric, Jelena/0000-0001-6825-5091 FU American Society of Heating Refrigerating and Air Conditioning Engineers (ASHRAE) project "Ventilation and Indoor Air Quality in Retail Stores" [RP-1596]; National Science Foundation (NSF), Division of Emerging Frontiers in Research and Innovation (EFRI) [EFRI-1038264/EFRI-1452045] FX The data collection for this study was suppported by the American Society of Heating Refrigerating and Air Conditioning Engineers (ASHRAE) project RP-1596 project "Ventilation and Indoor Air Quality in Retail Stores." The data analysis for this study was supported by the EFRI-1038264/EFRI-1452045 award from the National Science Foundation (NSF), Division of Emerging Frontiers in Research and Innovation (EFRI). The authors would like to thank the Pennsylvania State University and the University of Texas RP-1596 teams for the measurements that contributed to this paper. The generosity of the store managers and employees are also greatly appreciated. We also would like to acknowledge Dr. Wanyu Chan from the Lawrence Berkley National Laboratory for her valuable comments for the result analysis. NR 35 TC 2 Z9 2 U1 2 U2 12 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-1323 EI 1873-684X J9 BUILD ENVIRON JI Build. Environ. PD NOV PY 2015 VL 93 BP 385 EP 394 DI 10.1016/j.buildenv.2015.05.039 PN 2 PG 10 WC Construction & Building Technology; Engineering, Environmental; Engineering, Civil SC Construction & Building Technology; Engineering GA CR8EM UT WOS:000361583900036 ER PT J AU Mathews, TJ Looney, BB Bryan, AL Smith, JG Miller, CL Southworth, GR Peterson, MJ AF Mathews, Teresa J. Looney, Brian B. Bryan, A. Lawrence Smith, John G. Miller, Carrie L. Southworth, George R. Peterson, Mark J. TI The effects of a stannous chloride-based water treatment system in a mercury contaminated stream SO CHEMOSPHERE LA English DT Article DE Mercury; Tin; Stannous chloride; Remediation; Bioaccumulation ID CHEMICAL-REDUCTION; REMOVE MERCURY; TRACE-ELEMENTS; TIN; FISH; METHYLATION; SEDIMENT; FOOD; LAKE; BAY AB We assessed the impacts of an innovative Hg water treatment system on a small, industrially-contaminated stream in the southeastern United States. The treatment system, installed in 2007, removes Hg from wastewater using tin (Sn) (II) chloride followed by air stripping. Mercury concentrations in the receiving stream, Tims Branch, decreased from >100 to similar to 10 ng/L in the four years following treatment, and Hg body burdens in redfin pickerel (Esox americanus) decreased by 70% at the most contaminated site. Tin concentrations in water and fish increased significantly in the tributary leading to Tims Branch, but concentrations remain below levels of concern for human health or ecological risks. While other studies have shown that Sn may be environmentally methylated and methyltin can transfer its methyl group to Hg, results from our field studies and sediment incubation experiments suggest that the added Sn to the Tims Branch watershed is not contributing to methylmercury (MeHg) production or bioaccumulation in this system. The stannous chloride treatment system installed at Tims Branch was effective at removing Hg inputs and reducing Hg bioaccumulation in the stream, but future studies are needed to assess longer term impacts of Sn on the environment. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Mathews, Teresa J.; Smith, John G.; Miller, Carrie L.; Southworth, George R.; Peterson, Mark J.] Oak Ridge Natl Lab, Oak Ridge, TN 37830 USA. [Looney, Brian B.] Savannah River Natl Lab, Aiken, SC 29808 USA. [Bryan, A. Lawrence] Savannah River Ecol Lab, Aiken, SC 29808 USA. [Miller, Carrie L.] Troy Univ, Troy, AL 36082 USA. RP Mathews, TJ (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37830 USA. EM mathewstj@ornl.gov FU U.S. Department of Energy, Office of Environmental Management under the Remediation of Mercury and Industrial Contaminants Applied Field Research Initiative (RoMIC AFRI) [DE-FC09-96SR18546]; DOE [DE-AC05-00OR22725, DE-AC09-96SR18500, DE-AC09-08SR22470] FX This work was funded by the U.S. Department of Energy, Office of Environmental Management under the Remediation of Mercury and Industrial Contaminants Applied Field Research Initiative (RoMIC AFRI) and through Financial Assistance Award No. DE-FC09-96SR18546 to the University of Georgia Research Foundation. The Oak Ridge National Laboratory is managed by UT-Battelle for the DOE under contract number DE-AC05-00OR22725 and the Savannah River National Laboratory is managed by Savannah River Nuclear Solutions for the DOE under contracts DE-AC09-96SR18500 and DE-AC09-08SR22470. NR 33 TC 1 Z9 1 U1 8 U2 23 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0045-6535 EI 1879-1298 J9 CHEMOSPHERE JI Chemosphere PD NOV PY 2015 VL 138 BP 190 EP 196 DI 10.1016/j.chemosphere.2015.05.083 PG 7 WC Environmental Sciences SC Environmental Sciences & Ecology GA CS0SP UT WOS:000361772800026 PM 26070084 ER PT J AU Meena, AH Kaplan, DI Powell, BA Arai, Y AF Meena, Amanda H. Kaplan, Daniel I. Powell, Brian A. Arai, Yuji TI Chemical stabilization of chromate in blast furnace slag mixed cementitious materials SO CHEMOSPHERE LA English DT Article DE Reduction; Chromium; Technetium; Cement waste form; Blast furnace slag; Immobilization ID CHROMIUM(III) HYDROXIDE; TECHNETIUM SPECIATION; WASTE FORMS; ADSORPTION; INTERFACE; BEHAVIOR; SOILS AB Cement waste form (CWF) technology is among the leading approaches to disposing of metals and liquid low-level nuclear waste in the United States. One such material, saltstone, includes slag, fly ash and Portland cement to enhance the immobilization of contaminants (e.g., Cr, Tc-99) in alkaline liquid wastes. To evaluate the stability of such redox sensitive contaminants in saltstone, the effects of slag as a source of reductant on Cr immobilization was evaluated in aged (<300 d) saltstone monoliths. Specifically, we investigated the effects of artificial cement pore waters on the Cr release and the spatially resolved Cr chemical state analysis using synchrotron based microfocused X-ray microprobe analysis. The microprobe analysis indicated the heterogeneous distribution of insoluble Cr(III)-species in saltstone. Although at most of 20% Cr-total was leached at the top few (2-3) millimeter depth, the release of Cr(VI) was small (<5%) at 5-30 mm with slight changes, indirectly suggesting that Cr is likely present as insoluble Cr(III) species throughout the depths. The study suggests that this saltstone formulation can effectively retain/immobilize Cr under the oxic field condition after <= 300 d of aging time. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Meena, Amanda H.] Clemson Univ, Sch Agr Forest & Environm Sci, Clemson, SC 29634 USA. [Kaplan, Daniel I.] Savannah River Natl Lab, Aiken, SC 29808 USA. [Powell, Brian A.] Clemson Univ, Dept Environm Engn & Earth Sci, Anderson, SC 29625 USA. [Arai, Yuji] Univ Illinois, Dept Nat Resources & Environm Sci, Urbana, IL 61801 USA. RP Arai, Y (reprint author), Univ Illinois, Dept Nat Resources & Environm Sci, Urbana, IL 61801 USA. EM yarai@illinois.edu FU South Carolina Universities Research and Education Foundation [DE-AC09-08SR22470]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515, DE-AC02-06CH11357] FX This research was supported by the South Carolina Universities Research and Education Foundation, Contract No. DE-AC09-08SR22470. Portions of this work were performed at BL2-3 at SSRL and ID-12 at APS. These facilities are supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract Nos. DE-AC02-76SF00515 and DE-AC02-06CH11357, respectively. NR 40 TC 1 Z9 1 U1 7 U2 22 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0045-6535 EI 1879-1298 J9 CHEMOSPHERE JI Chemosphere PD NOV PY 2015 VL 138 BP 247 EP 252 DI 10.1016/j.chemosphere.2015.06.008 PG 6 WC Environmental Sciences SC Environmental Sciences & Ecology GA CS0SP UT WOS:000361772800034 PM 26086810 ER PT J AU Masek, JG Hayes, DJ Hughes, MJ Healey, SP Turner, DP AF Masek, Jeffrey G. Hayes, Daniel J. Hughes, M. Joseph Healey, Sean P. Turner, David P. TI The role of remote sensing in process-scaling studies of managed forest ecosystems SO FOREST ECOLOGY AND MANAGEMENT LA English DT Review DE Remote sensing; Forest ecology; Scaling ID NET PRIMARY PRODUCTION; LANDSAT TIME-SERIES; PHOTOCHEMICAL REFLECTANCE INDEX; NEAREST-NEIGHBOR IMPUTATION; LIGHT-USE EFFICIENCY; CARBON-CYCLE; BIOMASS ESTIMATION; GLOBAL VEGETATION; SATELLITE DATA; FIRE SEVERITY AB Sustaining forest resources requires a better understanding of forest ecosystem processes, and how management decisions and climate change may affect these processes in the future. While plot and inventory data provide our most detailed information on forest carbon, energy, and water cycling, applying this understanding to broader spatial and temporal domains requires scaling approaches. Remote sensing provides a powerful resource for "upscaling" process understanding to regional and continental domains. The increased range of available remote sensing modalities, including interferometric radar, lidar, and hyperspectral imagery, allows the retrieval of a broad range of forest attributes. This paper reviews the application of remote sensing for upscaling forest attributes from the plot scale to regional domains, with particular emphasis on how remote sensing products can support parameterization and validation of ecosystem process models. We focus on four key ecological attributes of forests: composition, structure, productivity and evapotranspiration, and disturbance dynamics. For each attribute, we discuss relevant remote sensing technologies, provide examples of their application, and critically evaluate both strengths and challenges associated with their use. Published by Elsevier B.V. C1 [Masek, Jeffrey G.] NASA, Biospher Sci Lab, Goddard Space Flight Ctr, Greenbelt, MD 20770 USA. [Hayes, Daniel J.] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Hayes, Daniel J.; Hughes, M. Joseph] Univ Tenn, Dept Ecol & Evolutionary Biol, Knoxville, TN USA. [Healey, Sean P.] US Forest Serv, USDA, Rocky Mt Res Stn, Ogden, UT USA. [Turner, David P.] Oregon State Univ, Dept Forest Ecosyst & Soc, Corvallis, OR 97331 USA. RP Masek, JG (reprint author), NASA, Biospher Sci Lab, Goddard Space Flight Ctr, Code 618, Greenbelt, MD 20770 USA. EM Jeffrey.G.Masek@nasa.gov RI Masek, Jeffrey/D-7673-2012 FU NASA; US Forest Service FX This work was supported by the NASA Terrestrial Ecosystems program and the US Forest Service. Dr. Bruce Cook (NASA GSFC) is thanked for providing the G-LiHT lidar example. The authors thank two anonymous reviewers and the editors for their constructive comments on the original version of the manuscript. NR 208 TC 13 Z9 13 U1 18 U2 93 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-1127 EI 1872-7042 J9 FOREST ECOL MANAG JI For. Ecol. Manage. PD NOV 1 PY 2015 VL 355 SI SI BP 109 EP 123 DI 10.1016/j.foreco.2015.05.032 PG 15 WC Forestry SC Forestry GA CS1YL UT WOS:000361864700012 ER PT J AU Pester, NJ Ding, K Seyfried, WE AF Pester, Nicholas J. Ding, Kang Seyfried, William E., Jr. TI Vapor-liquid partitioning of alkaline earth and transition metals in NaCl-dominated hydrothermal fluids: An experimental study from 360 to 465 degrees C, near-critical to halite saturated conditions SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID EAST PACIFIC RISE; MID-ATLANTIC RIDGE; ABSORPTION FINE-STRUCTURE; EQUATION-OF-STATE; DE-FUCA RIDGE; CENTRAL INDIAN RIDGE; MAIN ENDEAVOR FIELD; PHASE-SEPARATION; VENT FLUIDS; SYSTEM NACL-H2O AB Multi-phase fluid flow is a common occurrence in magmatic hydrothermal systems; and extensive modeling efforts using currently established P-V-T-x properties of the NaCl-H2O system are impending. We have therefore performed hydrothermal flow experiments (360-465 degrees C) to observe vapor-liquid partitioning of alkaline earth and first row transition metals in NaCl-dominated source solutions. The data allow extraction of partition coefficients related to the intrinsic changes in both chlorinity and density along the two-phase solvus. The coefficients yield an overall decrease in vapor affinity in the order Cu(I) > Na > Fe(II) > Zn > Ni(II) >= Mg >= Mn(II) > Co(II) > Ca > Sr > Ba, distinguished with 95% confidence for vapor densities greater than similar to 0.2 g/cm(3). The alkaline earth metals are limited to purely electrostatic interactions with Cl ligands, resulting in an excellent linear correlation (R-2 > 0.99) between their partition coefficients and respective ionic radii. Though broadly consistent with this relationship, relative behavior of the transition metals is not well resolved, being likely obscured by complex bonding processes and the potential participation of Na in the formation of tetra-chloro species. At lower densities (at/near halite saturation) partitioning behavior of all metals becomes highly non-linear, where M/Cl ratios in the vapor begin to increase despite continued decreases in chlorinity and density. We refer to this phenomenon as "volatility", which is broadly associated with substantial increases in the HCl/NaCl ratio (eventually to >1) due to hydrolysis of NaCl. Some transition metals (e.g., Fe, Zn) exhibit volatility prior to halite stability, suggesting a potential shift in vapor speciation relative to nearer critical regions of the vapor-liquid solvus. The chemistry of deep-sea hydrothermal fluids appears affected by this process during magmatic events, however, our results do not support suggestions of subseafloor halite precipitation recorded in currently available field data. Ca-Cl systematics in vent fluids are specifically explored, revealing behavior consistent with partitioning due to phase separation. Interestingly, the effect of variable chloride on dissolved Na/Ca ratios associated with plagioclase solubility (in single-phase solutions) appears fundamentally similar to that of phase separation on vapor compositions such that vapors evolved in hydrothermal systems may naturally remain near equilibrium with the host lithology. Conversely, residual liquids/brines left behind in the crust may be undersaturated with metals, enhancing the rate and extent of hydrothermal alteration. Published by Elsevier Ltd. C1 [Pester, Nicholas J.; Ding, Kang; Seyfried, William E., Jr.] Univ Minnesota, Dept Earth Sci, Minneapolis, MN 55455 USA. [Pester, Nicholas J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Pester, NJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM NJPester@lbl.gov RI Pester, Nicholas/G-2424-2015 OI Pester, Nicholas/0000-0002-1852-6663 FU NSF [0927615, 0751771, 0813861] FX We thank Rick Knurr for analysis of the experimental samples, Shijun Wu for drafting Fig. 1, and Robert Jones for helping fabricate the new Ti-alloy reaction vessel. Thoughtful comments from Gleb Pokrovski, Axel Liebscher and two anonymous reviewers greatly improved the clarity and content of the manuscript. Financial support for this research was provided by NSF grants 0927615, 0751771, 0813861 (WES, KD). NR 160 TC 1 Z9 1 U1 9 U2 36 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD NOV 1 PY 2015 VL 168 BP 111 EP 132 DI 10.1016/j.gca.2015.07.028 PG 22 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CS2QR UT WOS:000361916700007 ER PT J AU Messner, MC Barham, MI Kumar, M Barton, NR AF Messner, Mark C. Barham, Matthew I. Kumar, Mukul Barton, Nathan R. TI Wave propagation in equivalent continuums representing truss lattice materials SO INTERNATIONAL JOURNAL OF SOLIDS AND STRUCTURES LA English DT Article DE Meta-materials; Micro-mechanics; Additive manufacturing; Wave propagation; Trusses ID NONLOCAL DISPERSIVE MODEL; HETEROGENEOUS MEDIA; DYNAMIC-RESPONSE; PERIODIC TRUSS; MICRO-INERTIA; ULTRALIGHT; KINEMATICS; MECHANICS; CRYSTALS; DESIGN AB Stiffness scales linearly with density in stretch-dominated lattice meta-materials offering the possibility of very light yet very stiff structures. Current additive manufacturing techniques can assemble structures from lattice materials, but the design of such structures will require accurate, efficient simulation methods. Equivalent continuum models have several advantages over discrete truss models of stretch dominated lattices, including computational efficiency and ease of model construction. However, the development an equivalent model suitable for representing the dynamic response of a periodic truss in the small deformation regime is complicated by microinertial effects. This paper derives a dynamic equivalent continuum model for periodic truss structures suitable for representing long-wavelength wave propagation and verifies it against the full Bloch wave theory and detailed finite element simulations. The model must incorporate microinertial effects to accurately reproduce long wavelength characteristics of the response such as anisotropic elastic soundspeeds. The formulation presented here also improves upon previous work by preserving equilibrium at truss joints for simple lattices and by improving numerical stability by eliminating vertices in the effective yield surface. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Messner, Mark C.; Barham, Matthew I.; Kumar, Mukul; Barton, Nathan R.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Messner, MC (reprint author), Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94551 USA. EM messner6@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344 (LLNL-JRNL-667808)] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 (LLNL-JRNL-667808). The authors thank Greg Schebler for creating the meshes used for the finite element calculations. NR 37 TC 5 Z9 5 U1 7 U2 30 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0020-7683 EI 1879-2146 J9 INT J SOLIDS STRUCT JI Int. J. Solids Struct. PD NOV PY 2015 VL 73-74 BP 55 EP 66 DI 10.1016/j.ijsolstr.2015.07.023 PG 12 WC Mechanics SC Mechanics GA CS1WI UT WOS:000361859200004 ER PT J AU Rycroft, CH Sui, Y Bouchbinder, E AF Rycroft, Chris H. Sui, Yi Bouchbinder, Eran TI An Eulerian projection method for quasi-static elastoplasticity SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Fluid mechanics; Chorin-type projection method; Plasticity; Elastoplasticity ID NAVIER-STOKES EQUATIONS; ELASTIC-PLASTIC SOLIDS; MACH NUMBER COMBUSTION; METALLIC GLASSES; NUMERICAL-SOLUTION; INHOMOGENEOUS DEFORMATION; STRESS; FORMULATION; ALGORITHMS; SIMULATION AB A well-established numerical approach to solve the Navier-Stokes equations for incompressible fluids is Chorin's projection method [1], whereby the fluid velocity is explicitly updated, and then an elliptic problem for the pressure is solved, which is used to orthogonally project the velocity field to maintain the incompressibility constraint. In this paper, we develop a mathematical correspondence between Newtonian fluids in the incompressible limit and hypo-elastoplastic solids in the slow, quasi-static limit. Using this correspondence, we formulate a new fixed-grid, Eulerian numerical method for simulating quasi-static hypo-elastoplastic solids, whereby the stress is explicitly updated, and then an elliptic problem for the velocity is solved, which is used to orthogonally project the stress to maintain the quasi-staticity constraint. We develop a finite-difference implementation of the method and apply it to an elasto-viscoplastic model of a bulk metallic glass based on the shear transformation zone theory. We show that in a two-dimensional plane strain simple shear simulation, the method is in quantitative agreement with an explicit method. Like the fluid projection method, it is efficient and numerically robust, making it practical for a wide variety of applications. We also demonstrate that the method can be extended to simulate objects with evolving boundaries. We highlight a number of correspondences between incompressible fluid mechanics and quasi-static elastoplasticity, creating possibilities for translating other numerical methods between the two classes of physical problems. (C) 2015 Elsevier Inc. All rights reserved. C1 [Rycroft, Chris H.] Harvard Univ, Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USA. [Rycroft, Chris H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Math, Berkeley, CA 94720 USA. [Sui, Yi] Simon Fraser Univ, Dept Math, Burnaby, BC V5A 1S6, Canada. [Bouchbinder, Eran] Weizmann Inst Sci, Dept Chem Phys, IL-76100 Rehovot, Israel. RP Rycroft, CH (reprint author), Harvard Univ, Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USA. EM chr@seas.harvard.edu; eran.bouchbinder@weizmann.ac.il FU National Science Foundation [DMR-1409560]; Office of Science, Computational and Technology Research, U.S. Department of Energy [DE-AC02-05CH11231]; Minerva Foundation; Federal German Ministry for Education and Research; Israel Science Foundation [712/12]; Harold Perlman Family Foundation; William Z. and Eda Bess Novick Young Scientist Fund FX The authors thank Prof. Alexandre J. Chorin (University of California, Berkeley), Prof. Ken Kamrin (Massachusetts Institute of Technology), Prof. James. R. Rice (Harvard University), and Dr. Manish Vasoya (Weizmann Institute of Science) for useful discussions about this work. C.H. Rycroft was supported by the National Science Foundation under Grant No. DMR-1409560, and by the Director, Office of Science, Computational and Technology Research, U.S. Department of Energy under contract number DE-AC02-05CH11231. E. Bouchbinder acknowledges support from the Minerva Foundation with funding from the Federal German Ministry for Education and Research, the Israel Science Foundation (Grant No. 712/12), the Harold Perlman Family Foundation, and the William Z. and Eda Bess Novick Young Scientist Fund. NR 78 TC 3 Z9 3 U1 2 U2 9 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD NOV 1 PY 2015 VL 300 BP 136 EP 166 DI 10.1016/j.jcp.2015.06.046 PG 31 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA CR8AJ UT WOS:000361573200008 ER PT J AU Hoang, TL Marian, J Bulatov, VV Hosemann, P AF Hoang, Tuan L. Marian, Jaime Bulatov, Vasily V. Hosemann, Peter TI Computationally-efficient stochastic cluster dynamics method for modeling damage accumulation in irradiated materials SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Stochastic cluster dynamics; Irradiation damage; Stochastic simulation algorithm; Tau-leaping ID CHEMICALLY REACTING SYSTEMS; SIZE SELECTION; SIMULATION; STIFFNESS; ALGORITHM; EVOLUTION; KINETICS AB An improved version of a recently developed stochastic cluster dynamics (SCD) method (Marian and Bulatov, 2012) [6] is introduced as an alternative to rate theory (RT) methods for solving coupled ordinary differential equation (ODE) systems for irradiation damage simulations. SCD circumvents by design the curse of dimensionality of the variable space that renders traditional ODE-based RT approaches inefficient when handling complex defect population comprised of multiple (more than two) defect species. Several improvements introduced here enable efficient and accurate simulations of irradiated materials up to realistic (high) damage doses characteristic of next-generation nuclear systems. The first improvement is a procedure for efficiently updating the defect reaction-network and event selection in the context of a dynamically expanding reaction-network. Next is a novel implementation of the tau-leaping method that speeds up SCD simulations by advancing the state of the reaction network in large time increments when appropriate. Lastly, a volume rescaling procedure is introduced to control the computational complexity of the expanding reaction-network through occasional reductions of the defect population while maintaining accurate statistics. The enhanced SCD method is then applied to model defect cluster accumulation in iron thin films subjected to triple ion-beam (Fe3+, He+ and H+) irradiations, for which standard RT or spatially-resolved kinetic Monte Carlo simulations are prohibitively expensive. (C) 2015 Elsevier Inc. All rights reserved. C1 [Hoang, Tuan L.; Hosemann, Peter] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Hoang, Tuan L.; Marian, Jaime; Bulatov, Vasily V.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA. [Marian, Jaime] Univ Calif Los Angeles, Dept Mat Sci & Engn, Los Angeles, CA 94720 USA. RP Marian, J (reprint author), Univ Calif Los Angeles, Dept Mat Sci & Engn, Los Angeles, CA 94720 USA. EM jmarian@ucla.edu OI Hosemann, Peter/0000-0003-2281-2213 FU Lawrence Scholar Program; UC Berkeley Chancellor's Fellowship; Nuclear Regulatory Commission Research Fellowship; Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We would like to thank Daryl Chrzan, Athanasios Arsenlis, Alexander Stukowski, David Cereceda, and Ninh Le for many helpful discussions. TLH acknowledges support from the Lawrence Scholar Program, the UC Berkeley Chancellor's Fellowship, and the Nuclear Regulatory Commission Research Fellowship. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 28 TC 2 Z9 2 U1 0 U2 7 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD NOV 1 PY 2015 VL 300 BP 254 EP 268 DI 10.1016/j.jcp.2015.07.061 PG 15 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA CR8AJ UT WOS:000361573200014 ER PT J AU Dai, WW Scannapieco, AJ AF Dai, William W. Scannapieco, Anthony J. TI Interface- and discontinuity-aware numerical schemes for plasma 3-T radiation diffusion in two and three dimensions SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Diffusion; Radiation; 3-T; Coupling; Interface; Implicit ID FINITE-DIFFERENCE METHODS; ADAPTIVE MESH REFINEMENT; NEWTON-KRYLOV METHOD; EQUATIONS; HYDRODYNAMICS; DISCRETIZATION; COEFFICIENTS; SIMULATIONS; CONDUCTION; ACCURACY AB A set of numerical schemes is developed for two- and three-dimensional time-dependent 3-T radiation diffusion equations in systems involving multi-materials. To resolve sub-cell structure, interface reconstruction is implemented within any cell that has more than one material. Therefore, the system of 3-T radiation diffusion equations is solved on two-and three-dimensional polyhedral meshes. The focus of the development is on the fully coupling between radiation and material, the treatment of nonlinearity in the equations, i.e., in the diffusion terms and source terms, treatment of the discontinuity across cell interfaces in material properties, the formulations for both transient and steady states, the property for large time steps, and second order accuracy in both space and time. The discontinuity of material properties between different materials is correctly treated based on the governing physics principle for general polyhedral meshes and full nonlinearity. The treatment is exact for arbitrarily strong discontinuity. The scheme is fully nonlinear for the full nonlinearity in the 3-T diffusion equations. Three temperatures are fully coupled and are updated simultaneously. The scheme is general in two and three dimensions on general polyhedral meshes. The features of the scheme are demonstrated through numerical examples for transient problems and steady states. The effects of some simplifications of numerical schemes are also shown through numerical examples, such as linearization, simple average of diffusion coefficient, and approximate treatment for the coupling between radiation and material. Published by Elsevier Inc. C1 [Dai, William W.; Scannapieco, Anthony J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Dai, WW (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM dai@lanl.gov FU United States Department of Energy ASC program [DE-AC52-06NA25396] FX This research and development are funded by the United States Department of Energy ASC program under the contract DE-AC52-06NA25396. The authors are grateful to Frederick L. Cochran and Chong Chang for discussions about this work. NR 36 TC 0 Z9 0 U1 3 U2 5 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD NOV 1 PY 2015 VL 300 BP 643 EP 664 DI 10.1016/j.jcp.2015.07.041 PG 22 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA CR8AJ UT WOS:000361573200032 ER PT J AU Klapper, H Zaitseva, N Carman, L AF Klapper, Helmut Zaitseva, Natalia Carman, Leslie TI X-ray topographic study of growth defects of trans-stilbene crystals grown from solutions SO JOURNAL OF CRYSTAL GROWTH LA English DT Article DE X-ray topography; Dislocation; Growth from solutions; Aromatic crystal; Trans-stilbene; Organic scintillator ID ORGANIC-CRYSTALS; SCINTILLATION PROPERTIES; RAPID GROWTH; DISLOCATIONS; GENERATION; REFINEMENT; DIBENZYL AB Single crystals of truns-stilbenc, C14H12, with properties suitable for high-energy neutron detection were grown from solution in anisole and toluene by the temperature reduction method with growth rates up to 6 mm/day. From these crystals, slices of appropriate orientation and thickness of 2-4 mm were cut and studied by X-ray diffraction topography applying the Lang method using CuK alpha radiation. The topographs exhibit growth defects such as liquid inclusions, dislocations, striations, and faulty growth-sector boundaries. These defects occur in the same typical arrangements and geometries as is observed in all kinds of crystals grown on habit faces from solution. Besides growth dislocations originating from inclusions and propagating with the growth front, many plastic glide dislocations in the shape of loops or half-loops emitted from inclusions by stress relaxation are observed. The glide system underlying this plasticity is discussed. (c) 2015 Elsevier B.V. All rights reserved. C1 [Klapper, Helmut] Rhein Westfal TH Aachen, Inst Kristallog, D-52066 Aachen, Germany. [Zaitseva, Natalia; Carman, Leslie] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Klapper, H (reprint author), Rhein Westfal TH Aachen, Inst Kristallog, D-52066 Aachen, Germany. EM klapper@xtal.rwth-aachen.de FU US Department of Energy by Lawrence Livermore National Laboratory [DE-AC507NA27344] FX The authors wish to thank Mrs. A. von Berg and Mr. Jan M. Simons (Aachen) for their help in the preparation of figures. The crystal growth work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC507NA27344. NR 31 TC 2 Z9 2 U1 2 U2 14 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-0248 EI 1873-5002 J9 J CRYST GROWTH JI J. Cryst. Growth PD NOV 1 PY 2015 VL 429 BP 74 EP 81 DI 10.1016/j.jcrysgro.2015.07.012 PG 8 WC Crystallography; Materials Science, Multidisciplinary; Physics, Applied SC Crystallography; Materials Science; Physics GA CR9CT UT WOS:000361651500012 ER PT J AU Prisk, TR Sokol, PE AF Prisk, T. R. Sokol, P. E. TI Magnetic Behavior of Solid Ar-O Solutions SO JOURNAL OF LOW TEMPERATURE PHYSICS LA English DT Article DE Oxygen; Solid solutions; Phase transitions ID PHASE DIAGRAM; OXYGEN AB Solid molecular oxygen presents an interesting example of a low-temperature crystal which exists within several different magnetic phases. When solid solutions of argon and oxygen are formed with molar concentrations of oxygen between 60 and 80 %, a new structural and magnetic phase, known as the -phase, appears at low temperatures. In order to investigate the nature of the -phase, we carried out SQUID magnetometry measurements solid argon-oxygen solutions made up of 74 % oxygen and 26 % argon. In particular, we performed measurements of the magnetic susceptibility of the solid solutions over complete temperature cycles and isothermally as a function of time. Taken together, the experimental data demonstrate that that the -phase is not an equilibrium thermodynamic state of the solid solutions, but is instead only a metastable state. C1 [Prisk, T. R.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Sokol, P. E.] Indiana Univ, Dept Phys, Bloomington, IN 47408 USA. RP Prisk, TR (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM prisktr@ornl.gov; pesokol@indiana.edu OI Prisk, Timothy/0000-0002-7943-5175 FU National Institute of Standards and Technology, U.S. Department of Commerce [70NANB5H1163] FX This report was prepared under Grant No. 70NANB5H1163 from the National Institute of Standards and Technology, U.S. Department of Commerce. The statements, findings, conclusions, and recommendations are those of the authors and do not necessarily reflect the views of the National Institute of Standards and Technology or the U.S. Department of Commerce. The authors gratefully thank David Sprinkle for his expert technical assistance. NR 15 TC 0 Z9 0 U1 1 U2 5 PU SPRINGER/PLENUM PUBLISHERS PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0022-2291 EI 1573-7357 J9 J LOW TEMP PHYS JI J. Low Temp. Phys. PD NOV PY 2015 VL 181 IS 3-4 BP 139 EP 146 DI 10.1007/s10909-015-1332-8 PG 8 WC Physics, Applied; Physics, Condensed Matter SC Physics GA CS0MX UT WOS:000361755800004 ER PT J AU Wang, GJ Amman, M Mei, H Mei, DM Irmscher, K Guan, YT Yang, G AF Wang, Guojian Amman, Mark Mei, Hao Mei, Dongming Irmscher, Klaus Guan, Yutong Yang, Gang TI Crystal growth and detector performance of large size High-purity Ge crystals SO MATERIALS SCIENCE IN SEMICONDUCTOR PROCESSING LA English DT Article DE Czochralski method; Semiconducting germanium; Gamma-ray detector ID GERMANIUM DETECTORS; SPECTROSCOPY; DISLOCATION; CONTACTS AB High-purity germanium crystals approximately 12 cm in diameter were grown in a hydrogen atmosphere using the Czochralski method. The dislocation density of the crystals was determined to be in the range of 2000-4200 cm(-2), which meets a requirement for use as a radiation detector. The axial and radial distributions of impurities in the crystals were measured and are discussed. A planar detector was also fabricated from one of the crystals and then evaluated for electrical and spectral performance. Measurements of gamma-ray spectra from Cs-137 and Am-241 sources demonstrate that the detector has excellent energy resolution. Published by Elsevier Ltd. C1 [Wang, Guojian; Mei, Hao; Mei, Dongming; Guan, Yutong; Yang, Gang] Univ S Dakota, Dept Phys, Vermillion, SD 57069 USA. [Amman, Mark] Univ Calif Berkeley, Ernest Orlando Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Irmscher, Klaus] Leibniz Inst Crystal Growth, D-12489 Berlin, Germany. RP Wang, GJ (reprint author), Univ S Dakota, Dept Phys, Vermillion, SD 57069 USA. EM Guojian.Wang@usd.edu FU DOE (Department of Energy) [DE-FG02-10ER46709]; State of South Dakota FX We would like to thank Angela Chiller for a carefully reading of this manuscript and Mike Pietsch for assistance in PTIS measurement. This work is supported by DOE (Department of Energy) Grant DE-FG02-10ER46709 and the State of South Dakota. NR 31 TC 0 Z9 1 U1 1 U2 12 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1369-8001 EI 1873-4081 J9 MAT SCI SEMICON PROC JI Mater. Sci. Semicond. Process PD NOV PY 2015 VL 39 BP 54 EP 60 DI 10.1016/j.mssp.2015.04.044 PG 7 WC Engineering, Electrical & Electronic; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Engineering; Materials Science; Physics GA CS0TC UT WOS:000361774100008 ER PT J AU Mufson, S Baugh, B Bower, C Coan, TE Cooper, J Corwin, L Karty, JA Mason, P Messier, MD Pla-Dalmau, A Proudfoot, M AF Mufson, S. Baugh, B. Bower, C. Coan, T. E. Cooper, J. Corwin, L. Karty, J. A. Mason, P. Messier, M. D. Pla-Dalmau, A. Proudfoot, M. TI Liquid scintillator production for the NOvA experiment SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Liquid scintillator; Neutrino detectors; Neutrino physics ID DETECTOR AB The NOvA collaboration blended and delivered 8.8 kt (2.72M gal) of liquid scintillator as the active detector medium to its near and far detectors. The composition of this scintillator was specifically developed to satisfy NOvA's performance requirements. A rigorous set of quality control procedures was put in place to verify that the incoming components and the blended scintillator met these requirements. The scintillator was blended commercially in Hammond, IN. The scintillator was shipped to the NOvA detectors using dedicated stainless steel tanker trailers cleaned to food grade. (C) 2015 Elsevier B.V. All rights reserved. C1 [Mufson, S.; Baugh, B.; Bower, C.; Karty, J. A.; Messier, M. D.] Indiana Univ, Bloomington, IN 47405 USA. [Coan, T. E.] So Methodist Univ, Dallas, TX 75275 USA. [Cooper, J.; Pla-Dalmau, A.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Corwin, L.] South Dakota Sch Mines & Technol, Rapid City, SD 57701 USA. [Mason, P.] Univ Tennessee, Knoxville, TN 37916 USA. [Proudfoot, M.] Renkert Oil, Morgantown, PA 19543 USA. RP Mufson, S (reprint author), Indiana Univ, Bloomington, IN 47405 USA. EM mufson@indiana.edu OI Corwin, Luke/0000-0001-7143-3821 FU DOE Office of High Energy Physics [DE-SC0010120]; U.S. Department of Energy, Office of Science [DE-AC02-07CH11359] FX This work was supported in part by the DOE Office of High Energy Physics through Grant DE-SC0010120 to Indiana University. Fermi National Accelerator Laboratory (Fermilab) is operated by Fermi Research Alliance, LLC under Contract no. DE-AC02-07CH11359 with the U.S. Department of Energy, Office of Science. The authors wish to thank the many people who helped make this work possible. At IU: B. Adams, F. Busch, C. Canal, M. Gebhard, A. Hansen, T. Harmon, J. Musser, E. Pierson, E. Steele, R. Tayloe, and D. Zipkin; at Fermi lab; E. Baldina, B. Cibic, K. Kephart, D. Pushka, Sarlina, R. Tesarek, and J. VanGemert; at Renkert Oil; S. Kelly and N. Miller; at Wolf Lake: Calarie, N. Cave, J. Hlebek, C. McClellan, J. Patton, and E. Sprenne. NR 12 TC 5 Z9 5 U1 1 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD NOV 1 PY 2015 VL 799 BP 1 EP 9 DI 10.1016/j.nima.2015.07.026 PG 9 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CS2DF UT WOS:000361877300001 ER PT J AU Seiya, K Chaurize, S Drennan, CC Pellico, W Sullivan, T Triplett, AK Waller, AM AF Seiya, K. Chaurize, S. Drennan, C. C. Pellico, W. Sullivan, T. Triplett, A. K. Waller, A. M. TI Development of the beam extraction synchronization system at the Fermilab Booster SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Longitudinal dynamics; RF; Corrector magnets; Feedback AB The new beam extraction synchronization control system called "Magnetic Cogging" was developed at the Fermilab Booster and it replaces a system called "RE Cogging" as part of the Proton Improvement Plan (PIP)[1] The flux throughput goal for the PIP is 2.2 x 10(17) protons per hour, which is double the present flux. The flux increase will be accomplished by doubling the number of beam cycles which, in turn, will double the beam loss in the Booster accelerator if nothing else is done. The Booster accelerates beam from 400 MeV to 8 GeV and extracts it to the Main Injector (MI) or Recycler Ring (RR). Cogging controls the beam extraction gap position which is created early in the Booster cycle and synchronizes the gap to the rising edge of the Booster extraction kicker and the MI/RR injection kicker. The RF Cogging system controls the gap position by changing only the radial position of the beam thus limiting the beam aperture and creating beam loss due to beam scraping. The Magnetic Cogging system controls the gap position with the magnetic field of the dipole correctors while the radial position feedback keeps the beam on a central orbit. Also with Magnetic Cogging the gap creation can occur earlier in the Booster cycle when the removed particles are at a lower energy. Thus Magnetic Cogging reduces the deposited energy of the lost particles (beam energy loss) and results in less beam loss activation. Energy loss was reduced by 40% by moving the gap creation energy from 700 MeV to 400 MeV when the Booster Cogging system was switched from RE Cogging to Magnetic Cogging in March 2015. Published by Elsevier B.V. C1 [Seiya, K.; Chaurize, S.; Drennan, C. C.; Pellico, W.; Sullivan, T.; Triplett, A. K.; Waller, A. M.] Fermilab Natl Accelerator Lab, Accelerator Div, Batavia, IL 60510 USA. RP Seiya, K (reprint author), Fermilab Natl Accelerator Lab, Accelerator Div, POB 500, Batavia, IL 60510 USA. OI Drennan, Craig/0000-0003-3302-3789 FU Fermi Research Alliance, LLC [DE-AC02-07CH11359]; United States Department of Energy FX We would like to thank the Fermilab Accelerator Division for supporting this project, and also thank the Proton Source and Operations departments for their help with the machine studies and commissioning. We also would like to thank T. Boes and D. Dick for their technical support. This work is supported by Fermi Research Alliance, LLC under Contract no. DE-AC02-07CH11359 with the United States Department of Energy. NR 6 TC 0 Z9 0 U1 0 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD NOV 1 PY 2015 VL 799 BP 147 EP 154 DI 10.1016/j.nima.2015.07.035 PG 8 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CS2DF UT WOS:000361877300022 ER PT J AU Carnelli, PFF Almaraz-Calderon, S Rehm, KE Albers, M Alcorta, M Bertone, PF Digiovine, B Esbensen, H Niello, JF Henderson, D Jiang, CL Lai, J Marley, ST Nusair, O Palchan-Hazan, T Pardo, RC Paul, M Ugalde, C AF Carnelli, P. F. F. Almaraz-Calderon, S. Rehm, K. E. Albers, M. Alcorta, M. Bertone, P. F. Digiovine, B. Esbensen, H. Fernandez Niello, J. Henderson, D. Jiang, C. L. Lai, J. Marley, S. T. Nusair, O. Palchan-Hazan, T. Pardo, R. C. Paul, M. Ugalde, C. TI Multi-Sampling Ionization Chamber (MUSIC) for measurements of fusion reactions with radioactive beams SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Active target detector; Multi-Sampling Ionization Chamber; Fusion reactions ID TRACKING PROPORTIONAL CHAMBER; RELATIVISTIC HEAVY-IONS; CROSS-SECTIONS AB A detection technique for high-efficiency measurements of fusion reactions with low-intensity radioactive beams was developed. The technique is based on a Multi-Sampling Ionization Chamber (MUSIC) operating as an active target and detection system, where the ionization gas acts as both target and counting gas. In this way, we can sample an excitation function in an energy range determined by the gas pressure, without changing the beam energy. The detector provides internal normalization to the incident beam and drastically reduces the measuring Lime. In a first experiment we tested the performance of the technique by measuring the C-10,C-13,C-15 + C-12 fusion reactions at energies around the Coulomb barrier. (C) 2015 Elsevier B.V. All rights reserved. C1 [Carnelli, P. F. F.; Almaraz-Calderon, S.; Rehm, K. E.; Albers, M.; Alcorta, M.; Bertone, P. F.; Digiovine, B.; Esbensen, H.; Henderson, D.; Jiang, C. L.; Marley, S. T.; Nusair, O.; Palchan-Hazan, T.; Pardo, R. C.; Ugalde, C.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Carnelli, P. F. F.; Fernandez Niello, J.] Comis Nacl Energia Atom, Lab TANDAR, Buenos Aires, DF, Argentina. [Carnelli, P. F. F.] Consejo Nacl Invest Cient & Tecn, Buenos Aires, DF, Argentina. [Fernandez Niello, J.] Univ Nacl San Martin, Buenos Aires, DF, Argentina. [Lai, J.] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. [Paul, M.] Hebrew Univ Jerusalem, Racah Inst Phys, IL-91904 Jerusalem, Israel. RP Rehm, KE (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. EM rehm@anl.gov OI Pardo, Richard/0000-0002-8264-9430 FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357]; Consejo Nacional de Investigaciones Cientificas y Tecnicas (CONICET), Argentina FX We thank the operations crew of the accelerator for providing the beams used in these experiments. This work was supported by U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Contract Number DE-AC02-06CH11357 (ANL). This research used resources of ANL's ATLAS facility, which is a DOE Office of Science User Facility, Support by the Consejo Nacional de Investigaciones Cientificas y Tecnicas (CONICET), Argentina, is also gratefully acknowledged. NR 25 TC 6 Z9 6 U1 0 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD NOV 1 PY 2015 VL 799 BP 197 EP 202 DI 10.1016/j.nima.2015.07.030 PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CS2DF UT WOS:000361877300028 ER PT J AU Shao, QH Conway, AM Voss, LF Radev, RP Nikolic, RJ Dar, MA Cheung, CL AF Shao, Qinghui Conway, Adam M. Voss, Lars F. Radev, Radoslav P. Nikolic, Rebecca J. Dar, Mushtaq A. Cheung, Chin L. TI Experimental determination of gamma-ray discrimination in pillar-structured thermal neutron detectors under high gamma-ray flux SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Thermal neutron detector; Gamma-ray discrimination; Silicon pillar; Boron ID EFFICIENCY AB In this paper, we demonstrate a detector that has a high neutron-to-gamma discrimination of 8.5 x 10(5) with a high thermal neutron detection efficiency of 39% when exposed to a high gamma-ray held of 10(9) photons/cm(2)s. The detector is based on a silicon pillar structure filled with a neutron converter material (B-10) designed to have high thermal neutron detection efficiency. The pillar dimensions are 50 mu m pillar height, 2 mu m pillar diameter and 2 mu m spacing between adjacent pillars. (C) 2015 Elsevier B.V. All rights reserved. C1 [Shao, Qinghui; Conway, Adam M.; Voss, Lars F.; Radev, Radoslav P.; Nikolic, Rebecca J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Dar, Mushtaq A.] King Saud Univ, Riyadh 11421, Saudi Arabia. [Cheung, Chin L.] Univ Nebraska, Dept Chem, Lincoln, NE 68588 USA. RP Nikolic, RJ (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. EM nikolic1@llnl.gov RI Cheung, Chin Li/B-8270-2013 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344, LLNL-JRNL-641356]; US Department of Homeland Security, Domestic Nuclear Detection Office [HSHQDC-08-X-00874] FX The authors would like to acknowledge Tim Graff and Cathy Reinhardt for their excellent support in the clean room fabrication. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344, LLNL-JRNL-641356. This work has been supported by the US Department of Homeland Security, Domestic Nuclear Detection Office, under competitively awarded IAA HSHQDC-08-X-00874. This support does not constitute an express or implied endorsement on the part of the government. NR 19 TC 0 Z9 0 U1 2 U2 11 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD NOV 1 PY 2015 VL 799 BP 203 EP 206 DI 10.1016/j.nima.2015.07.045 PG 4 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CS2DF UT WOS:000361877300029 ER PT J AU Isotalo, AE Wieselquist, WA AF Isotalo, A. E. Wieselquist, W. A. TI A method for including external feed in depletion calculations with CRAM and implementation into ORIGEN SO ANNALS OF NUCLEAR ENERGY LA English DT Article DE CRAM; ORIGEN; Depletion; External feed; Source term ID SCALE AB A method for including external feed with polynomial time dependence in depletion calculations with the Chebyshev Rational Approximation Method (CRAM) is presented and the implementation of CRAM to the ORIGEN module of the SCALE suite is described. In addition to being able to handle time-dependent feed rates, the new solver also adds the capability to perform adjoint calculations. Results obtained with the new CRAM solver and the original depletion solver of ORIGEN are compared to high precision reference calculations, which shows the new solver to be orders of magnitude more accurate. Furthermore, in most cases, the new solver is up to several times faster due to not requiring similar substepping as the original one. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Isotalo, A. E.; Wieselquist, W. A.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Isotalo, A. E.] Aalto Univ, Dept Appl Phys, FI-00076 Aalto, Finland. RP Isotalo, AE (reprint author), Aalto Univ, Dept Appl Phys, POB 14100, FI-00076 Aalto, Finland. EM aarno.isotalo@aalto.fi FU SAFIR2014, the Finnish Research Program on Nuclear Power Plant Safety; U.S. Department of Energy FX Funding from SAFIR2014, the Finnish Research Program on Nuclear Power Plant Safety, and the Nuclear Energy Advanced Modeling and Simulation (NEAMS) program of the U.S. Department of Energy is acknowledged. NR 15 TC 3 Z9 3 U1 0 U2 1 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0306-4549 J9 ANN NUCL ENERGY JI Ann. Nucl. Energy PD NOV PY 2015 VL 85 BP 68 EP 77 DI 10.1016/j.anucene.2015.04.037 PG 10 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CR5VZ UT WOS:000361413800008 ER PT J AU Wu, HZ Zhao, HH AF Wu, Hsingtzu Zhao, Haihua TI Validation of hydrogen gas stratification and mixing models SO ANNALS OF NUCLEAR ENERGY LA English DT Article DE Hydrogen leaks; Buoyant jets; Enclosure mixing; Hydrogen stratification ID SCALE UNINTENDED RELEASES; INTEGRAL PLUME MODEL; THERMAL STRATIFICATION; CONTAINMENT; SIMULATION; LEAKAGE AB Two validation benchmarks confirm that the BMIX++ code is capable of simulating unintended hydrogen release scenarios efficiently. The BMIX++ (UC Berkeley mechanistic MIXing code in C++) code has been developed to accurately and efficiently predict the fluid mixture distribution and heat transfer in large stratified enclosures for accident analyses and design optimizations. The BMIX++ code uses a scaling based one-dimensional method to achieve large reduction in computational effort compared to a 3-D computational fluid dynamics (CFD) simulation. Two BMIX++ benchmark models have been developed. One is for a single buoyant jet in an open space and another is for a large sealed enclosure with both a jet source and a vent near the floor. Both of them have been validated by comparisons with experimental data. Excellent agreements are observed. The entrainment coefficients of 0.09 and 0.08 are found to fit the experimental data for hydrogen leaks with the Froude number of 99 and 268 best, respectively. In addition, the BIX++ simulation results of the average helium concentration for a enclosure with a vent and a single jet agree with the experimental data within a margin of about 10% for jet flow rates ranging from 1.21 x 10(-4) to 3.29 x 10(-4) m(3)/s. Computing time for each BMIX++ model with a normal desktop computer is less than 5 min. Published by Elsevier Ltd. C1 [Wu, Hsingtzu] Japan Atom Energy Agcy, Tokai, Ibaraki 3191195, Japan. [Zhao, Haihua] Idaho Natl Lab, Thermal Sci & Safety Anal Dept, Idaho Falls, ID 83415 USA. RP Zhao, HH (reprint author), Idaho Natl Lab, Thermal Sci & Safety Anal Dept, POB 1625,MS 3870, Idaho Falls, ID 83415 USA. EM Haihua.Zhao@inl.gov FU U.S. Department of Energy, under Department of Energy Idaho Operations Office [DE-AC07-05ID14517] FX This work is supported by the U.S. Department of Energy, under Department of Energy Idaho Operations Office Contract DE-AC07-05ID14517. Accordingly, the U.S. Government retains a nonexclusive, royalty-free license to publish or reproduce the published form of this contribution, or allow others to do so, for U.S. Government purposes. The BMIX++ code was originally developed at University of California, Berkeley under the advising of Professor Per Peterson. NR 21 TC 1 Z9 1 U1 1 U2 13 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0306-4549 J9 ANN NUCL ENERGY JI Ann. Nucl. Energy PD NOV PY 2015 VL 85 BP 137 EP 144 DI 10.1016/j.anucene.2015.05.003 PG 8 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CR5VZ UT WOS:000361413800013 ER PT J AU Cao, Y Gohar, Y AF Cao, Yan Gohar, Yousry TI Monte Carlo simulations of periodic pulsed reactor with moving geometry parts SO ANNALS OF NUCLEAR ENERGY LA English DT Article DE Periodic pulsed reactor; Monte Carlo method; Movable reactor geometry parts AB In a periodic pulsed reactor, the reactor state varies periodically from slightly subcritical to slightly prompt supercritical for producing periodic power pulses. Such periodic state change is accomplished by a periodic movement of specific reactor parts, such as control rods or reflector sections. The analysis of such reactor is difficult to perform with the current reactor physics computer programs. Based on past experience, the utilization of the point kinetics approximations gives considerable errors in predicting the magnitude and the shape of the power pulse if the reactor has significantly different neutron life times in different zones. To accurately simulate the dynamics of this type of reactor, a Monte Carlo procedure using the transfer function TRCL/TR of the MCNP/MCNPX computer programs is utilized to model the movable reactor parts. In this paper, two algorithms simulating the geometry part movements during a neutron history tracking have been developed. Several test cases have been developed to evaluate these procedures. The numerical test cases have shown that the developed algorithms can be utilized to simulate the reactor dynamics with movable geometry parts. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Cao, Yan; Gohar, Yousry] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. RP Cao, Y (reprint author), Argonne Natl Lab, Nucl Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM ycao@anl.gov; gohar@anl.gov FU Office of Global Nuclear Material Threat Reduction U.S. Department of Energy [DE-AC02-06CH11357] FX This work has been supported by the Office of Global Nuclear Material Threat Reduction U.S. Department of Energy Under Contract DE-AC02-06CH11357. NR 4 TC 0 Z9 0 U1 0 U2 4 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0306-4549 J9 ANN NUCL ENERGY JI Ann. Nucl. Energy PD NOV PY 2015 VL 85 BP 236 EP 244 DI 10.1016/j.anucene.2015.05.020 PG 9 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CR5VZ UT WOS:000361413800024 ER PT J AU Aufiero, M Bidaud, A Hursin, M Leppanen, J Palmiotti, G Pelloni, S Rubiolo, P AF Aufiero, Manuele Bidaud, Adrien Hursin, Mathieu Leppanen, Jaakko Palmiotti, Giuseppe Pelloni, Sandro Rubiolo, Pablo TI A collision history-based approach to sensitivity/perturbation calculations in the continuous energy Monte Carlo code SERPENT SO ANNALS OF NUCLEAR ENERGY LA English DT Article DE Sensitivity; Perturbation; Monte Carlo; SERPENT; Scattering distribution ID PARAMETERS; KINETICS AB In this work, the implementation of a collision history-based approach to sensitivity/perturbation calculations in the Monte Carlo code SERPENT is discussed. The proposed methods allow the calculation of the effects of nuclear data perturbation on several response functions: the effective multiplication factor, reaction rate ratios and bilinear ratios (e.g., effective kinetics parameters). SERPENT results are compared to ERANOS and TSUNAMI Generalized Perturbation Theory calculations for two fast metallic systems and for a PWR pin-cell benchmark. New methods for the calculation of sensitivities to angular scattering distributions are also presented, which adopts fully continuous (in energy and angle) Monte Carlo estimators. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Aufiero, Manuele; Bidaud, Adrien; Rubiolo, Pablo] Univ Grenoble Alpes, CNRS IN2P3, LPSC, F-38026 Grenoble, France. [Hursin, Mathieu; Pelloni, Sandro] Paul Scherrer Inst, Nucl Energy & Safety Dept NES, Reactor Phys & Syst Behav Lab LRS, CH-5232 Villigen, Switzerland. [Leppanen, Jaakko] VTT Tech Res Ctr Finland, FI-02044 Espoo, Vtt, Finland. [Palmiotti, Giuseppe] Idaho Natl Lab, Nucl Syst Design & Anal Div, Idaho Falls, ID 83415 USA. RP Aufiero, M (reprint author), Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. EM manuele.aufiero@berkeley.edu NR 31 TC 9 Z9 9 U1 0 U2 6 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0306-4549 J9 ANN NUCL ENERGY JI Ann. Nucl. Energy PD NOV PY 2015 VL 85 BP 245 EP 258 DI 10.1016/j.anucene.2015.05.008 PG 14 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CR5VZ UT WOS:000361413800025 ER PT J AU Wu, X Kozlowski, T Hales, JD AF Wu, Xu Kozlowski, Tomasz Hales, Jason D. TI Neutronics and fuel performance evaluation of accident tolerant FeCrAl cladding under normal operation conditions SO ANNALS OF NUCLEAR ENERGY LA English DT Article DE FeCrAl; Accident Tolerant Fuel ID HIGH-TEMPERATURE; IRON-ALLOYS; OXIDATION; STEAM AB Neutronics and fuel performance analysis is done for enhanced accident tolerance fuel (ATF), with the Monte Carlo reactor physics code Serpent and INL's fuel performance code BISON. The purpose is to evaluate the most promising ATF candidate material FeCrAl, which has excellent oxidation resistance, as fuel cladding under normal operational conditions. Due to several major disadvantages of FeCrAl coating, such as difficulty in fabrication, diametrical compression from reactor pressurization, coating spallation and inter diffusion with zirconium, a monolithic FeCrAl cladding design is suggested. To overcome the neutron penalty expected when using FeCrAl as cladding for current oxide fuel, an optimized FeCrAl cladding design from a detailed parametric study in literature is adopted, which suggests reducing the cladding thickness and slightly increasing the fuel enrichment. A neutronics analysis is done that implementing this FeCrAl cladding design in a Pressurized Water Reactor (PWR) single assembly. The results show that the PWR cycle length requirements will be matched, with a slight increase in total plutonium production. Fuel performance analysis with BISON code is carried out to investigate the effects with this FeCrAl cladding design. The results demonstrate that the application of FeCrAl cladding could improve performance. For example, the axial temperature profile is flattened. The gap closure is significantly delayed, which means the pellet cladding mechanical interaction is greatly delayed. The disadvantages for monolithic FeCrAl cladding are that: (1) fission gas release is increased: and (2) fuel temperature is increased, but the increase is less than 50 K even at high burnup. The better strength, corrosion, and embrittlement properties of FeCrAl enable the fabrication of FeCrAl cladding with thinner walls. FeCrAl cladding proves to be a good alternate for zircaloy cladding, given the advantages and insignificant disadvantages shown by fuel performance analysis. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Wu, Xu; Kozlowski, Tomasz] Univ Illinois, Dept Nucl Plasma & Radiol Engn, Urbana, IL 61801 USA. [Hales, Jason D.] Idaho Natl Lab, Fuels Modeling & Simulat Dept, Idaho Falls, ID 83415 USA. RP Wu, X (reprint author), Univ Illinois, Dept Nucl Plasma & Radiol Engn, 124 Talbot Lab,104 South Wright St, Urbana, IL 61801 USA. EM xuwu2@illinois.edu; txk@illinois.edu; jason.hales@inl.gov OI Hales, Jason/0000-0003-0836-0476 NR 17 TC 5 Z9 5 U1 5 U2 32 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0306-4549 J9 ANN NUCL ENERGY JI Ann. Nucl. Energy PD NOV PY 2015 VL 85 BP 763 EP 775 DI 10.1016/j.anucene.2015.06.032 PG 13 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CR5VZ UT WOS:000361413800082 ER PT J AU Billings, JJ Deyton, JH Hull, SF Lingerfelt, EJ Wojtowicz, A AF Billings, Jay Jay Deyton, Jordan H. Hull, S. Forest, III Lingerfelt, Eric J. Wojtowicz, Anna TI A domain-specific analysis system for examining nuclear reactor simulation data for light-water and sodium-cooled fast reactors SO ANNALS OF NUCLEAR ENERGY LA English DT Article DE Nuclear reactors; LWR; SFR; Simulation; Modeling; High-performance computing AB Building a new generation of fission reactors in the United States presents many technical and regulatory challenges. One important challenge is the need to share and present results from new high-fidelity, high-performance simulations in an easily usable way. Since modern multiscale, multi-physics simulations can generate petabytes of data, they will require the development of new techniques and methods to reduce the data to familiar quantities of interest (e.g., pin powers, temperatures) with a more reasonable resolution and size. Furthermore, some of the results from these simulations may be new quantities for which visualization and analysis techniques are not immediately available in the community and need to be developed. This paper describes a new system for managing high-performance simulation results in a domain-specific way that naturally exposes quantities of interest for light water and sodium-cooled fast reactors. It describes requirements to build such a system and the technical challenges faced in its development at all levels (simulation, user interface, etc.). An example comparing results from two different simulation suites for a single assembly in a light-water reactor is presented, along with a detailed discussion of the system's requirements and design. (C) 2015 The Authors. Published by Elsevier Ltd. This is an open access article under the CC BY license (http://creativecommons.org/licenses/by/4.0/). C1 [Billings, Jay Jay; Deyton, Jordan H.; Hull, S. Forest, III; Lingerfelt, Eric J.; Wojtowicz, Anna] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Billings, JJ (reprint author), Oak Ridge Natl Lab, POB 2008,MS6173, Oak Ridge, TN 37831 USA. EM billingsjj@ornl.gov OI Billings, Jay/0000-0001-8811-2688 FU NEAMS program; Advanced Reactor Concepts program; CASL program; US Department of Energy, Office of Nuclear Energy; ORNL Postgraduate Research Participation Program - ORNL; US Department of Energy [DE-AC05-00OR22725, DE-AC05-00OR22750] FX The authors are grateful to members of the NEAMS and CASL communities, others whom we have interviewed, and our program managers. The authors are grateful for the assistance of Greg Davidson, Jess Gehin, Andrew Godfrey, Ugur Mertyurek, and John Turner from Oak Ridge National Laboratory (ORNL) and Justin Thomas from Argonne National Laboratory. The authors are also grateful for the financial support provided by the NEAMS, Advanced Reactor Concepts, and CASL programs.; This work has been supported by the US Department of Energy, Office of Nuclear Energy, and by the ORNL Postgraduate Research Participation Program, which is sponsored by ORNL and administered jointly by ORNL and the Oak Ridge Institute for Science and Education (ORISE). ORNL is managed by UT-Battelle, LLC, for the US Department of Energy under contract No. DE-AC05-00OR22725. ORISE is managed by Oak Ridge Associated Universities for the US Department of Energy under contract No. DE-AC05-00OR22750. NR 16 TC 0 Z9 0 U1 1 U2 3 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0306-4549 J9 ANN NUCL ENERGY JI Ann. Nucl. Energy PD NOV PY 2015 VL 85 BP 856 EP 868 DI 10.1016/j.anucene.2015.07.002 PG 13 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CR5VZ UT WOS:000361413800092 ER PT J AU Walter, DJ Kendrick, BK Petrov, V Manera, A Collins, B Downar, T AF Walter, Daniel J. Kendrick, Brian K. Petrov, Victor Manera, Annalisa Collins, Benjamin Downar, Thomas TI Proof-of-principle of high-fidelity coupled CRUD deposition and cycle depletion simulation SO ANNALS OF NUCLEAR ENERGY LA English DT Article DE CRUD; CIPS; Axial offset; High-fidelity; Multiphysics; CILC AB A multiphysics framework for the high-fidelity simulation of CRUD deposition is developed to better understand the coupled physics and their respective feedback mechanisms. This framework includes the primary physics of lattice depletion, computational fluid dynamics, and CRUD chemistry. The three physics are coupled together via the operator-splitting technique, where predictor-corrector and fixed-point iteration schemes are utilized to converge the nonlinear solution. High-fidelity simulations may provide a means to predict and assess potential operating issues, including CRUD induced power shift and CRUD induced localized corrosion, known as CIPS and CILC, respectively. As a proof-of-principle, a coupled 500-day cycle depletion simulation of a pressurized water reactor fuel pin cell was performed using the coupled code suite; a burnup of 31 MWd/kgHM was reached. The simulation recreated the classic striped CRUD pattern often seen on pulled fuel rods containing CRUD. It is concluded that the striping is caused by the flow swirl induced by spacer grid mixing vanes. Two anti-correlated effects contribute to the striping: (1) the flow swirl yields significant azimuthal temperature variations, which impact the locations where CRUD deposits, and (2) the flow swirl is correlated to increased shear stress along the cladding surface and subsequent erosion of the CRUD layer. The CIPS condition of the core is concluded to be primarily controlled by lithium tetraborate precipitation, referred to as boron hideout, which occurs in regions experiencing subcooled nucleate boiling as soluble boron and lithium species reach their solubility limit within the CRUD layer. Subsequently, a localized reduction in power occurs due to the high neutron absorption cross section of boron-10. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Walter, Daniel J.; Petrov, Victor; Manera, Annalisa; Collins, Benjamin; Downar, Thomas] Univ Michigan, Dept Nucl Engn & Radiol Sci, Ann Arbor, MI 48109 USA. [Kendrick, Brian K.] Los Alamos Natl Lab, Theoret Div T1, Los Alamos, NM 87545 USA. RP Walter, DJ (reprint author), Univ Michigan, Dept Nucl Engn & Radiol Sci, 2355 Bonisteel Blvd, Ann Arbor, MI 48109 USA. EM djwalter@umich.edu; bkendric@lanl.gov; petrov@umich.edu; manera@umich.edu; bscollin@umich.edu; downar@umich.edu FU NRC [NRC-HQ-11-G-38-0038]; Consortium for Advanced Simulation of Light Water Reactors an Energy Innovation Hub for Modeling and Simulation of Nuclear Reactors under U.S. Department of Energy [DE-AC05-00OR22725] FX This work was supported by an NRC fellowship, the NRC faculty development grant NRC-HQ-11-G-38-0038, and the Consortium for Advanced Simulation of Light Water Reactors (www.casl.gov), an Energy Innovation Hub (http://www.energy.gov/hubs) for Modeling and Simulation of Nuclear Reactors under U.S. Department of Energy Contract No. DE-AC05-00OR22725. NR 18 TC 2 Z9 2 U1 1 U2 7 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0306-4549 J9 ANN NUCL ENERGY JI Ann. Nucl. Energy PD NOV PY 2015 VL 85 BP 1152 EP 1166 DI 10.1016/j.anucene.2015.07.034 PG 15 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CR5VZ UT WOS:000361413800122 ER PT J AU Wilbanks, TJ AF Wilbanks, Thomas J. TI Putting "Place" in a multiscale context: Perspectives from the sustainability sciences SO ENVIRONMENTAL SCIENCE & POLICY LA English DT Article DE Scale; Multiscale; Place; Sustainability ID CLIMATE CHANGED WORLD; HUMAN DIMENSIONS; SPATIAL-SCALE; GLOBAL CHANGE; ENVIRONMENT; ADAPTATION; GOVERNANCE; KNOWLEDGE; FRAMEWORK; GEOGRAPHY AB This paper summarizes a number of perspectives that have emerged from the sustainability sciences in recent decades that shed light on the role of place in multi-scale sustainability science and vice versa, related to such topics of broad interest as "resilience" and "adaptation" and ranging from the importance of the "co-production" of knowledge for sustainable development to threats to a "sense of place" from global environmental and economic changes. Clearly, scholarly attention to place in a multiscale concept is shared by a number of research communities, especially a rich tradition of research on place as politically contested space. These two traditions intersect in ways that have been little-explored. For example, sustainability science traditions have been focused on challenges in integrating knowledge about nature and society as a research objective, where "scale" is used as one of a number of structural organizing concepts in unraveling natural system - human system interactions in geographical areas from microbial to global, where it has found that a small regional scale is the one where such integrative analysis is often most fruitful but "place" is not usually an organizing concept. Concurrently, the political-economy oriented place traditions have viewed place as a frequent focus of struggles over power, control, and equity, with scale only one of many factors shaping how places work. These intersections, some of them noted below, offer potentials for integrated research that might interest both communities and benefit a number of space/place research discourses. (C) 2015 Elsevier Ltd. All rights reserved. C1 Oak Ridge Natl Lab, Oak Ridge, TN USA. RP Wilbanks, TJ (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN USA. EM wilbankstj@ornl.gov FU Integrated Assessment Research Program of the Office of Science, US Department of Energy FX Valuable contributions from several reviewers are acknowledged; and support from the Integrated Assessment Research Program of the Office of Science, US Department of Energy, is also gratefully acknowledged. NR 93 TC 2 Z9 2 U1 6 U2 33 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1462-9011 EI 1873-6416 J9 ENVIRON SCI POLICY JI Environ. Sci. Policy PD NOV PY 2015 VL 53 SI SI BP 70 EP 79 DI 10.1016/j.envsci.2015.04.009 PN A PG 10 WC Environmental Sciences SC Environmental Sciences & Ecology GA CR3SE UT WOS:000361252600008 ER PT J AU Tan, L Yang, Y AF Tan, L. Yang, Y. TI In situ phase transformation of Laves phase from Chi-phase in Mo-containing Fe-Cr-Ni alloys SO MATERIALS LETTERS LA English DT Article DE Mo-containing stainless steels; TEM; Microstructure; Phase transformation ID AUSTENITIC STAINLESS-STEELS; SIGMA-PHASE; PRECIPITATION AB An in situ phase transformation of the Chi (chi) phase to the Laves phase was observed in a Fe-Cr-Ni-Mo model alloy. The morphology, composition, and crystal structure of the chi and Laves phases, and their orientation relationship with the matrix austenite phase were investigated. The resulted Laves phase has larger lattice mismatch with the matrix phase than the chi phase, leading to the increase of local strain fields and the formation of dislocations. This finding is helpful to understand the precipitation behavior of the intermetallic phases in the Mo-containing austenitic stainless steels. (C) 2015 Elsevier B.V. All rights reserved. C1 [Tan, L.; Yang, Y.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Tan, L (reprint author), One Bethel Valley Rd,POB 2008,MS-6136, Oak Ridge, TN 37831 USA. EM tanl@ornl.gov RI Tan, Lizhen/A-7886-2009; Yang, Ying/E-5542-2017 OI Tan, Lizhen/0000-0002-3418-2450; Yang, Ying/0000-0001-6480-2254 FU U.S. Department of Energy (DOE), Office of Nuclear Energy; Light Water Reactor (LWR) program; Nuclear Engineering Enabling Technology (NEET) Advanced Reactor Material Program Cross-Cut activity [DE-AC05-00OR22725]; UT-Battelle, LLC FX This research was supported by the U.S. Department of Energy (DOE), Office of Nuclear Energy, Light Water Reactor (LWR) program and Nuclear Engineering Enabling Technology (NEET) Advanced Reactor Material Program Cross-Cut activity, under contract DE-AC05-00OR22725 with UT-Battelle, LLC. NR 12 TC 2 Z9 2 U1 2 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-577X EI 1873-4979 J9 MATER LETT JI Mater. Lett. PD NOV 1 PY 2015 VL 158 BP 233 EP 236 DI 10.1016/j.matlet.2015.06.018 PG 4 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA CR3WW UT WOS:000361264800060 ER PT J AU Eisenlohr, J Lee, BG Benick, J Feldmann, F Driessen, M Milenkovic, N Blasi, B Goldschmidt, JC Hermle, M AF Eisenlohr, Johannes Lee, Benjamin G. Benick, Jan Feldmann, Frank Driessen, Marion Milenkovic, Nena Blaesi, Benedikt Goldschmidt, Jan Christoph Hermle, Martin TI Rear side sphere gratings for improved light trapping in crystalline silicon single junction and silicon-based tandem solar cells SO SOLAR ENERGY MATERIALS AND SOLAR CELLS LA English DT Article; Proceedings Paper CT 10th Iberian Conference on Information Systems and Technologies (CISTI) CY JUN 17-20, 2015 CL Univ Aveiro, Sch Technol & Agueda Management, Agueda, PORTUGAL SP Iberian Assoc Syst Informat Technol HO Univ Aveiro, Sch Technol & Agueda Management DE Silicon; Light trapping; Diffraction grating; Passivated contacts; Tandem solar cells; Perovskite ID DIFFRACTION GRATINGS; CONTACTS; ABSORPTION; SIMULATION; EFFICIENCY AB Rear side hexagonal sphere gratings are demonstrated as diffractive structures that enhance the light path length in the near infrared, where crystalline silicon solar cells suffer from weak absorption. Moreover, the rear side sphere grating can be added behind a solar cell with flat rear surface, giving an "electrically flat but optically rough" device with high efficiency potential. Here, a thin passivating tunnel-contact layer electrically separates the sphere grating from the cell's base. Solar cells with the rear side sphere grating have obtained a V-oc of up to 710 mV and a FF of up to 81.9%. External quantum efficiency measurements show a current density gain of 1.4 mA/cm(2) due to the sphere grating. This leads to an overall efficiency of up to 22.1% for the solar cells with planar front side and rear side sphere grating. Estimates for perovskite-silicon and III/V-silicon tandem devices show that the efficiency of tandems can be enhanced by up to 2.4% absolute with a sphere grating on the rear side. Thus, sphere gratings could improve Si-based tandem devices that are limited due to a low current in the Si bottom cell. (C) 2015 Elsevier B.V. All rights reserved. C1 [Eisenlohr, Johannes; Lee, Benjamin G.; Benick, Jan; Feldmann, Frank; Driessen, Marion; Milenkovic, Nena; Blaesi, Benedikt; Goldschmidt, Jan Christoph; Hermle, Martin] Fraunhofer Inst Solar Energy Syst ISE, D-79110 Freiburg, Germany. [Lee, Benjamin G.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Eisenlohr, J (reprint author), Fraunhofer Inst Solar Energy Syst ISE, Heidenhofstr 2, D-79110 Freiburg, Germany. EM johannes.eisenlohr@ise.fraunhofer.de RI Goldschmidt, Jan Christoph/C-1807-2008; Blasi, Benedikt/A-5618-2012 OI Goldschmidt, Jan Christoph/0000-0003-3256-1366; Blasi, Benedikt/0000-0003-1624-1530 FU German Federal Ministry for Economic Affairs and Energy [0325292]; German Federal Ministry of Education and Research in the project "InfraVolt" [03SF0401B]; US Department of Energy SunShot Program to Advance Solar Cell Efficiency II (FPACE) [DE-EE0006336]; Deutsche Bundesstiftung Umwelt (DBU) FX The authors would like to thank A. Leimenstoll, E. Schaffer, F. Schatzle, S. Seitz, N. Weber, T. Rachow and K. Zimmermann for their support with processes and measurements. This work was partially funded by the German Federal Ministry for Economic Affairs and Energy under Contract number 0325292 (ForTeS), by the German Federal Ministry of Education and Research in the project "InfraVolt" (Project number 03SF0401B) as well as by the US Department of Energy SunShot Program to Advance Solar Cell Efficiency II (FPACE) under Award number DE-EE0006336. J. Eisenlohr gratefully acknowledges scholarship support from the Deutsche Bundesstiftung Umwelt (DBU). NR 31 TC 10 Z9 10 U1 5 U2 98 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0248 EI 1879-3398 J9 SOL ENERG MAT SOL C JI Sol. Energy Mater. Sol. Cells PD NOV PY 2015 VL 142 SI SI BP 60 EP 65 DI 10.1016/j.solmat.2015.05.043 PG 6 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA CR8DZ UT WOS:000361582600011 ER PT J AU Chuang, CY Zepeda-Ruiz, LA Han, SM Sinno, T AF Chuang, Claire Y. Zepeda-Ruiz, Luis A. Han, Sang M. Sinno, Talid TI Direct molecular dynamics simulation of Ge deposition on amorphous SiO2 at experimentally relevant conditions SO SURFACE SCIENCE LA English DT Article DE Molecular dynamics; Atomic deposition; Amorphous SiO2; Germanium; Silicon ID KINETIC MONTE-CARLO; HIGH-QUALITY GE; THREADING-DISLOCATION DENSITIES; ISLAND-SIZE DISTRIBUTIONS; THIN-FILM GROWTH; HIGH-PERFORMANCE; SOLAR-CELLS; MORPHOLOGICAL EVOLUTION; NUCLEATION KINETICS; INFREQUENT EVENTS AB Molecular dynamics simulations were used to study Ge island nucleation and growth on amorphous SiO2 substrates. This process is relevant in selective epitaxial growth of Ge on Si, for which SiO2 is often used as a template mask The islanding process was studied over a wide range of temperatures and fluxes, using a recently proposed empirical potential model for the Si-SiO2-Ge system. The simulations provide an excellent quantitative picture of the Ge islanding and compare well with detailed experimental measurements. These quantitative comparisons were enabled by an analytical rate model as a bridge between simulations and experiments despite the fact that deposition fluxes accessible in simulations and experiments are necessarily different by many orders of magnitude. In particular, the simulations led to accurate predictions of the critical island size and the scaling of island density as a function of temperature. The overall approach used here should be useful not just for future studies in this particular system, but also for molecular simulations of deposition in other materials. (C) 2015 Elsevier B.V. All rights reserved. C1 [Chuang, Claire Y.; Sinno, Talid] Univ Penn, Dept Chem & Biomol Engn, Philadelphia, PA 19104 USA. [Zepeda-Ruiz, Luis A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Han, Sang M.] Univ New Mexico, Dept Chem & Biol Engn, Albuquerque, NM 87131 USA. RP Sinno, T (reprint author), Univ Penn, Dept Chem & Biomol Engn, 220 South 33rd St,311A Towne Bldg, Philadelphia, PA 19104 USA. EM yungc@seas.upenn.edu; zepedaruiz1@llnl.gov; meister@unm.edu; talid@seas.upenn.edu FU National Science Foundation [DMR-0907365, DMR-0907112, CMMI-1068841, CMMI-1068970]; US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was supported by the National Science Foundation under Awards DMR-0907365, DMR-0907112, CMMI-1068841, and CMMI-1068970. We also acknowledge computational resources provided by XSEDE (DMR-140059). Part of this work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 (LA.Z.-R.). NR 66 TC 1 Z9 1 U1 7 U2 29 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0039-6028 EI 1879-2758 J9 SURF SCI JI Surf. Sci. PD NOV PY 2015 VL 641 BP 112 EP 120 DI 10.1016/j.susc.2015.04.029 PG 9 WC Chemistry, Physical; Physics, Condensed Matter SC Chemistry; Physics GA CR5UB UT WOS:000361408800016 ER PT J AU Rameshan, C Ng, ML Shavorskiy, A Newberg, JT Bluhm, H AF Rameshan, C. Ng, M. L. Shavorskiy, A. Newberg, J. T. Bluhm, H. TI Water adsorption on polycrystalline vanadium from ultra-high vacuum to ambient relative humidity SO SURFACE SCIENCE LA English DT Article DE Hydroxylation; Ambient pressure photoelectron spectroscopy; Water adsorption; Vanadium; In-situ spectroscopy ID CO OXIDATION; SURFACE SCIENCE; SPECTROSCOPY; OXIDE; THIN; PHOTOEMISSION; NUCLEATION; MICROSCOPY; CATALYSTS; PROBE AB We have studied the reaction of water vapor with a polycrystalline vanadium surface using ambient pressure X-ray photoelectron spectroscopy (AP-XPS) which allows the investigation of the chemical composition of the vanadium/water vapor interface at p(H2O) in the Torr range. Water dissociation on the vanadium surface was studied under isobaric conditions at p(H2O) ranging from 0.01 to 0.50 Torr and temperatures from 625 K to 260 K, i.e. up to a relative humidity (RH) of similar to 15%. Water vapor exposure leads to oxidation and hydroxylation of the vanadium foil already at a pressure of 1 x 10(-6) Torr at 300 K (RH similar to 4 x 10(-6)%). The vanadium oxide layer on the surface has a stoichiometry of V2O3. Initial adsorption of molecular water on the surface is observed at RH > 0.001%. Above a RH of 0.5% the amount of adsorbed water increases markedly. Experiments at increasing temperatures show that the water adsorption process is reversible. Depth profile measurements show a thickness for the vanadium oxide layer of 3-5 mono layers (ML) and for vanadium hydroxide of 1-1.5 ML over the whole RH range in the isobar experiments. The thickness of the adsorbed water layer was found to be in the sub-ML range for the investigated RH's. (C) 2015 Elsevier B.V. All rights reserved. C1 [Rameshan, C.] Vienna Univ Technol, Inst Mat Chem, A-1060 Vienna, Austria. [Ng, M. L.] SLAC Natl Accelerator Lab, SUNCAT Ctr Interface Sci & Catalysis, Menlo Pk, CA 94025 USA. [Shavorskiy, A.; Bluhm, H.] Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Newberg, J. T.] Univ Delaware, Dept Chem & Biochem, Newark, DE 19716 USA. RP Rameshan, C (reprint author), Vienna Univ Technol, Inst Mat Chem, Getreidemarkt 9, A-1060 Vienna, Austria. EM christoph.rameshan@tuwien.ac.at RI Rameshan, Christoph/G-3564-2015 OI Rameshan, Christoph/0000-0002-6340-4147 FU Division of Chemical Sciences, Geosciences, and Biosciences of the US Department of Energy at the Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Austrian Science Fund (FWF) via an Erwin-Schrodinger Scholarship [J3208N-19]; Wenner-Gren Foundations in Stockholm, Sweden; NSF [ANT-1019347] FX The ALS and the MES beamline 11.0.2 are supported by the Director, Office of Science, Office of Basic Energy Sciences, and by the Division of Chemical Sciences, Geosciences, and Biosciences of the US Department of Energy at the Lawrence Berkeley National Laboratory under Contract No. DE-AC02-05CH11231. Christoph Rameshan acknowledges support by the Austrian Science Fund (FWF) via an Erwin-Schrodinger Scholarship [J3208N-19]. May Ling Ng gratefully acknowledges the postdoctoral fellowship from Wenner-Gren Foundations in Stockholm, Sweden. John T. Newberg acknowledges support from an NSF postdoctoral fellowship (ANT-1019347). NR 52 TC 0 Z9 0 U1 1 U2 29 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0039-6028 EI 1879-2758 J9 SURF SCI JI Surf. Sci. PD NOV PY 2015 VL 641 BP 141 EP 147 DI 10.1016/j.susc.2015.06.004 PG 7 WC Chemistry, Physical; Physics, Condensed Matter SC Chemistry; Physics GA CR5UB UT WOS:000361408800020 ER PT J AU Dong, YJ Brooks, JD Chen, TL Mullins, DR Cox, DF AF Dong, Yujung Brooks, John D. Chen, Tsung-Liang Mullins, David R. Cox, David F. TI Reactions of methyl groups on a non-reducible metal oxide: The reaction of iodomethane on stoichiometric alpha-Cr2O3(0001) SO SURFACE SCIENCE LA English DT Article DE Cr2O3; Methyl iodide; XPS; TPD; Dehydrogenation ID TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; PARTIAL OXIDATION; BASIS-SET; SURFACE; OXYGEN; PHOTOCHEMISTRY; AG(111); DECOMPOSITION; RADICALS AB The reaction of iodomethane on the nearly stoichiometric alpha-Cr2O3(0001) surface produces gas phase ethylene, methane, and surface iodine adatoms. The reaction is initiated by the dissociation of iodomethane into surface methyl fragments, -CH3, and iodine adatoms. Methyl fragments bound at surface Cr cation sites undergo a rate-limiting dehydrogenation reaction to methylene, = CH2. The methylene intermediates formed from methyl dehydrogenation can undergo coupling reactions to produce ethylene via two principle reaction pathways: (1) direct coupling of methylene and (2) methylene insertion into the methyl surface bond to form surface ethyl groups which undergo beta-H elimination to produce ethylene. The liberated hydrogen also combines with methyl groups to form methane. Iodine adatoms from the dissociation of iodomethane deactivate the surface by simple site blocking of the surface Cr3+ cations. (C) 2015 Elsevier B.V. All rights reserved. C1 [Dong, Yujung; Brooks, John D.; Cox, David F.] Virginia Polytech Inst & State Univ, Dept Chem Engn, Blacksburg, VA 24061 USA. [Chen, Tsung-Liang; Mullins, David R.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Cox, DF (reprint author), Virginia Polytech Inst & State Univ, Dept Chem Engn, Blacksburg, VA 24061 USA. EM dfcox@vt.edu FU Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy [DE-FG02-97ER14751]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX YD, JDB, and DFC gratefully acknowledge financial support by the Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy through Grant DE-FG02-97ER14751. The efforts of TLC and DRM are sponsored by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. The authors also acknowledge Advanced Research Computing at Virginia Tech for providing computational resources and technical support that have contributed to the results reported within this paper. NR 43 TC 1 Z9 1 U1 0 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0039-6028 EI 1879-2758 J9 SURF SCI JI Surf. Sci. PD NOV PY 2015 VL 641 BP 148 EP 153 DI 10.1016/j.susc.2015.06.003 PG 6 WC Chemistry, Physical; Physics, Condensed Matter SC Chemistry; Physics GA CR5UB UT WOS:000361408800021 ER PT J AU Yi, CW Szanyi, J AF Yi, Cheol-Woo Szanyi, Janos TI The thermal behavior of Pd on graphene/Ru(0001) SO SURFACE SCIENCE LA English DT Article DE Pd/graphene/Ru(0001); Annealing; Agglomeration; Intercalation; IRAS; XPS ID NOX STORAGE MATERIALS; VIBRATIONAL SPECTROSCOPY; SURFACE SCIENCE; CO ADSORPTION; GRAPHENE; CATALYSTS; BAO; NANOPARTICLES; NANOCLUSTERS; INTERFACES AB The thermal behavior of various amounts of palladium deposited onto graphene/Ru(0001) at room temperature was investigated by X-ray photoelectron spectroscopy (XPS) and infrared reflection absorption spectroscopy (IRAS) of adsorbed CO. IRAS spectra of adsorbed CO on palladium deposited onto the graphene layer reveal the formation of defect-rich, highly-stepped and/or nanoparticle-typed palladium clusters. Annealing to temperatures below similar to 900 K, palladium clusters mainly experience agglomeration on the graphene layer, but at higher temperatures intercalation of palladium between the graphene layer and Ru substrate takes place. Eventually, palladium completely desorbs and the graphene layer dissolves into the ruthenium substrate at 1400 K. Even though the annealing induces the intercalation and desorption of palladium, the topmost graphene layer stays intact without any physical damage at and below 1300 K. (C) 2015 Elsevier B.V. All rights reserved. C1 [Yi, Cheol-Woo] Sungshin Womens Univ, Dept Chem, Seoul 142732, South Korea. [Yi, Cheol-Woo] Sungshin Womens Univ, Inst Basic Sci, Seoul 142732, South Korea. [Yi, Cheol-Woo; Szanyi, Janos] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. RP Szanyi, J (reprint author), Pacific NW Natl Lab, Inst Integrated Catalysis, POB 999,MSIN K8-87, Richland, WA 99352 USA. EM janos.szanyi@pnnl.gov RI Yi, Cheol-Woo/B-3082-2010 OI Yi, Cheol-Woo/0000-0003-4549-5433 FU US Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division; DOE Office of Biological and Environmental Research; US DOE [DE-AC05-76RL01830]; Sungshin Women's University FX We gratefully acknowledge the US Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division for the support of this work. The research described in this article was performed at the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the DOE Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). PNNL is operated for the US DOE by Battelle Memorial Institute under contract number DE-AC05-76RL01830. This work was also supported by the Sungshin Women's University Research Grant of 2014. NR 27 TC 1 Z9 1 U1 4 U2 32 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0039-6028 EI 1879-2758 J9 SURF SCI JI Surf. Sci. PD NOV PY 2015 VL 641 BP 154 EP 158 DI 10.1016/j.susc.2015.06.005 PG 5 WC Chemistry, Physical; Physics, Condensed Matter SC Chemistry; Physics GA CR5UB UT WOS:000361408800022 ER PT J AU Thurmer, K Yuan, CQ Kimmel, GA Kay, BD Smith, RS AF Thuermer, Konrad Yuan, Chunqing Kimmel, Greg A. Kay, Bruce D. Smith, R. Scott TI Weak interactions between water and clathrate-forming gases at low pressures SO SURFACE SCIENCE LA English DT Article DE Clathrates; Water; Methane; Isobutane; STM; TPD ID AMORPHOUS SOLID WATER; HYDRATE NUCLEATION; METHANE HYDRATE; CARBON-DIOXIDE; ICE POWDERS; DESORPTION; SURFACE; ADSORPTION; POINT; DISSOCIATION AB Using scanning probe microscopy and temperature programed desorption we examined the interaction between water and two common clathrate-forming gases, methane and isobutane, at low temperature and low pressure. Water co-deposited with up to 10(-1) mbar methane or 10(-5) mbar isobutane at 140 K onto a Pt(111) substrate yielded pure crystalline ice, i.e., the exposure to up to similar to 10(7) gas molecules for each deposited water molecule did not have any detectable effect on the growing films. Exposing metastable, less than 2 molecular layers thick, water films to 10-5 mbar methane does not alter their morphology, suggesting that the presence of the Pt(111) surface is not a strong driver for hydrate formation. This weak water-gas interaction at low pressures is supported by our thermal desorption measurements from amorphous solid water and crystalline ice where 1 ML of methane desorbs near similar to 43 K and isobutane desorbs near similar to 100 K. Similar desorption temperatures were observed for desorption from amorphous solid water. (C) 2015 Elsevier B.V. All rights reserved. C1 [Thuermer, Konrad] Sandia Natl Labs, Livermore, CA 94550 USA. [Yuan, Chunqing; Kimmel, Greg A.; Kay, Bruce D.; Smith, R. Scott] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. RP Thurmer, K (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA. EM kthurme@sandia.gov RI Smith, Scott/G-2310-2015; Thurmer, Konrad/L-4699-2013; OI Smith, Scott/0000-0002-7145-1963; Thurmer, Konrad/0000-0002-3078-7372; Kimmel, Greg/0000-0003-4447-2440 FU Laboratory Directed Research and Development program at Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; DOE' s Office of Biological and Environmental Research FX We gratefully acknowledge the discussions with Laura Stern, Randall Cygan, Margaret Gordon, and Stephanie Teich-McGoldrick. The STM research (KT) was supported by the Laboratory Directed Research and Development program at Sandia National Laboratories. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. The TPD work (CY, GAK, BDK, and RSS) was supported by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences. The research was performed using EMSL, a national scientific user facility sponsored by DOE' s Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory, which is operated by Battelle for the DOE. NR 55 TC 1 Z9 1 U1 5 U2 44 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0039-6028 EI 1879-2758 J9 SURF SCI JI Surf. Sci. PD NOV PY 2015 VL 641 BP 216 EP 223 DI 10.1016/j.susc.2015.07.013 PG 8 WC Chemistry, Physical; Physics, Condensed Matter SC Chemistry; Physics GA CR5UB UT WOS:000361408800032 ER PT J AU Li, BY Ou, LW Dang, Q Meyer, P Jones, S Brown, R Wright, M AF Li, Boyan Ou, Longwen Dang, Qi Meyer, Pimphan Jones, Susanne Brown, Robert Wright, Mark TI Techno-economic and uncertainty analysis of in situ and ex situ fast pyrolysis for biofuel production SO BIORESOURCE TECHNOLOGY LA English DT Article DE Pyrolysis; In situ; Ex situ; Techno-economics analysis; Uncertainty analysis ID CATALYTIC FAST PYROLYSIS; BIOMASS FAST PYROLYSIS; TRANSPORTATION FUELS; BED REACTOR; GASIFICATION; OIL; PATHWAYS; ENERGY AB This study evaluates the techno-economic uncertainty in cost estimates for two emerging technologies for biofuel production: in situ and ex situ catalytic pyrolysis. The probability distributions for the minimum fuel-selling price (MFSP) indicate that in situ catalytic pyrolysis has an expected MFSP of $1.11 per liter with a standard deviation of 0.29, while the ex situ catalytic pyrolysis has a similar MFSP with a smaller deviation ($1.13 per liter and 0.21 respectively). These results suggest that a biorefinery based on ex situ catalytic pyrolysis could have a lower techno-economic uncertainty than in situ pyrolysis compensating for a slightly higher MFSP cost estimate. Analysis of how each parameter affects the NPV indicates that internal rate of return, feedstock price, total project investment, electricity price, biochar yield and bio-oil yield are parameters which have substantial impact on the MFSP for both in situ and ex situ catalytic pyrolysis. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Li, Boyan; Ou, Longwen; Dang, Qi; Brown, Robert; Wright, Mark] Iowa State Univ, Dept Mech Engn, Ames, IA 50010 USA. [Dang, Qi; Brown, Robert; Wright, Mark] Iowa State Univ, Bioecon Inst, Ames, IA 50011 USA. [Meyer, Pimphan; Jones, Susanne] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Wright, M (reprint author), Iowa State Univ, Bioecon Inst, Ames, IA 50011 USA. EM markmw@iastate.edu FU US Department of Energy; Pacific Northwest National Laboratory [167288] FX This project was made possible by support from the US Department of Energy and Pacific Northwest National Laboratory through Contract Number 167288. The authors would like to acknowledge Rajeeva Thilakaratne for developing the baseline process models. NR 34 TC 8 Z9 8 U1 6 U2 42 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0960-8524 EI 1873-2976 J9 BIORESOURCE TECHNOL JI Bioresour. Technol. PD NOV PY 2015 VL 196 BP 49 EP 56 DI 10.1016/j.biortech.2015.07.073 PG 8 WC Agricultural Engineering; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA CR0VD UT WOS:000361040500008 PM 26226581 ER PT J AU Vandamme, D Pohl, PI Beuckels, A Foubert, I Brady, PV Hewson, JC Muylaert, K AF Vandamme, Dries Pohl, Philip I. Beuckels, Annelies Foubert, Imogen Brady, Patrick V. Hewson, John C. Muylaert, Koenraad TI Alkaline flocculation of Phaeodactylum tricornutum induced by brucite and calcite SO BIORESOURCE TECHNOLOGY LA English DT Article DE Coagulation; Marine algae; Enmeshment; Biomass; Autoflocculation ID CHLORELLA-VULGARIS; ALGAL AUTOFLOCCULATION; MICROALGAE; BIOMASS; PH; PRECIPITATION; MAGNESIUM; MECHANISM AB Alkaline flocculation holds great potential as a low-cost harvesting method for marine microalgae biomass production. Alkaline flocculation is induced by an increase in pH and is related to precipitation of calcium and magnesium salts. In this study, we used the diatom Phaeodactylum tricornutum as model organism to study alkaline flocculation of marine microalgae cultured in seawater medium. Flocculation started when pH was increased to 10 and flocculation efficiency reached 90% when pH was 10.5, which was consistent with precipitation modeling for brucite or Mg(OH)(2). Compared to freshwater species, more magnesium is needed to achieve flocculation (>7.5 mM). Zeta potential measurements suggest that brucite precipitation caused flocculation by charge neutralization. When calcium concentration was 12.5 mM, flocculation was also observed at a pH of 10. Zeta potential remained negative up to pH 11.5, suggesting that precipitated calcite caused flocculation by a sweeping coagulation mechanism. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Vandamme, Dries; Beuckels, Annelies; Muylaert, Koenraad] KU Leuven Kulak, Lab Aquat Biol, B-8500 Kortrijk, Belgium. [Pohl, Philip I.; Brady, Patrick V.; Hewson, John C.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Foubert, Imogen] KU Leuven Kulak, Res Unit Food & Lipids, Dept Mol & Microbial Syst Kulak, B-8500 Kortrijk, Belgium. [Foubert, Imogen] Katholieke Univ Leuven, Leuven Food Sci & Nutr Res Ctr LFoRCe, B-3001 Heverlee, Belgium. RP Vandamme, D (reprint author), KU Leuven Kulak, Lab Aquat Biol, Etienne Sabbelaan 53, B-8500 Kortrijk, Belgium. EM dries.vandamme@kuleuven-kulak.be RI Vandamme, Dries/I-7553-2015 OI Vandamme, Dries/0000-0003-0941-2434 FU Research Foundation Flanders Belgium (FWO); Laboratory Directed Research and Development program; BioEnergy Technology Office, U.S. Department of Energy [9.1.1.3_DE-EE0005995]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The research presented in this paper was financially supported by the Research Foundation Flanders Belgium (FWO Postdoctoral Fellowship D. Vandamme, FWO Ph.D. fellowship A. Beuckels). We thank Sina Salim, Prof. Marjan Vermue and Prof. Rene Wijffels, Bio-process Engineering, WUR, Wageningen for the usage of the Malvern Zetasizer during our experiments. We thank Kristin Coorevits and Prof. Erik Smolders, Division of Soil and Water Management, KU Leuven for the ICP-MS analysis. We thank Saul Garcia-Perez and Manel Azzabi for their contribution to this work. This work at Sandia National Laboratories was partially supported by the Laboratory Directed Research and Development program and was partially supported by the BioEnergy Technology Office, U.S. Department of Energy under Award 9.1.1.3_DE-EE0005995. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 30 TC 3 Z9 3 U1 9 U2 33 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0960-8524 EI 1873-2976 J9 BIORESOURCE TECHNOL JI Bioresour. Technol. PD NOV PY 2015 VL 196 BP 656 EP 661 DI 10.1016/j.biortech.2015.08.042 PG 6 WC Agricultural Engineering; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA CR0VD UT WOS:000361040500082 PM 26310384 ER PT J AU Hu, D Liu, Q Tisdale, J Nam, H Park, SY Wang, H Urbas, A Hu, B AF Hu, Dehua Liu, Qing Tisdale, Jeremy Nam, Haerim Park, Soo Young Wang, Hsin Urbas, Augustine Hu, Bin TI Optically tunable Seebeck effect from intramolecular proton-transfer materials in organic vertical thin-film thermoelectric device SO ORGANIC ELECTRONICS LA English DT Article DE Seebeck effect; Proton-transfer; Electron-phonon coupling; Organic semiconductors ID DENSITY-OF-STATES; ELECTRICAL-CONDUCTIVITY; SURFACE POLARIZATION; COEFFICIENT; EFFICIENCY; POLYMER AB This paper reports Seebeck effects from optically-induced intramolecular proton-transfer HPI-Cbz molecules based on vertical electrode/organic film/electrode thin-film devices. We observed large Seebeck coefficients of 428 mu V/K and 390 mu V/K from HPI-Cbz based thin-film devices at 60 degrees C when proton-transfer was induced by the photoexcitation of a 325 nm laser with an intensity of 12 mW/cm(2) and 6 mW/cm(2) respectively. Under dark condition without proton transfer occurring, the Seebeck coefficient was measured to be 342 mu V/K at 60 degrees C. The Seebeck coefficient enhancement by the induced intramolecular charge transfer can be attributed to the enhanced polarization difference between high-and low-temperature surface due to the stronger electron-phonon coupling followed with the proton-transfer in HPI-Cbz under photoexcitation, and the strength of electron-phonon coupling is proportional to the photoexcitation intensity. The enhanced temperature-dependent electrical polarization between the high and low-temperature surfaces acts as an additional driving force to diffuse the majority charge carriers for the development of a large Seebeck effect. Therefore, using intramolecular proton-transfer presents an effective approach of enhancing Seebeck effect in organic materials. (C) 2015 Elsevier B.V. All rights reserved. C1 [Hu, Dehua; Liu, Qing; Tisdale, Jeremy; Hu, Bin] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Nam, Haerim; Park, Soo Young] Seoul Natl Univ, Dept Mat Sci & Engn, ENG445, Seoul 151744, South Korea. [Wang, Hsin] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Urbas, Augustine] Air Force Res Lab, Wright Patterson AFB, OH 45433 USA. [Hu, Dehua] S China Univ Technol, State Key Lab Luminescent Mat & Devices, Inst Polymer Optoelect Mat & Devices, Guangzhou 510640, Guangdong, Peoples R China. RP Hu, B (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. EM bhu@utk.edu RI Park, Soo Young/G-1080-2012; Wang, Hsin/A-1942-2013 OI Park, Soo Young/0000-0002-2272-8524; Wang, Hsin/0000-0003-2426-9867 FU Air Force Office of Scientific Research (AFOSR) [FA 9550-15-1-0064]; National Science Foundation [CBET-1438181]; Sustainable Energy Education and Research Center; Center for Materials Processing at the University of Tennessee; Division of Scientific User Facilities, U.S. Department of Energy [CNMS2012-106, CNMS2012-107, CNMS-2012-108]; National Significant Program [2014CB643506, 2013CB922104]; NSFC Program in China [61475051]; National Science Foundation of China [51403063]; China Postdoctoral Science Fund [2014M562174] FX This research was supported by the financial supports from Air Force Office of Scientific Research (AFOSR) (FA 9550-15-1-0064) and National Science Foundation (CBET-1438181). The authors also acknowledge the support from Sustainable Energy Education and Research Center and Center for Materials Processing at the University of Tennessee. This research was partially conducted at the Center for Nanophase Materials Sciences based on user project (CNMS2012-106, CNMS2012-107, CNMS-2012-108), which is sponsored at Oak Ridge National Laboratory by the Division of Scientific User Facilities, U.S. Department of Energy. The authors also acknowledge the supports from the National Significant Program (2014CB643506, 2013CB922104) and NSFC Program (61475051) in China. The authors also acknowledge the supports from National Science Foundation of China (Grant No. 51403063) and China Postdoctoral Science Fund (Grant No. 2014M562174). NR 31 TC 2 Z9 2 U1 3 U2 58 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1566-1199 EI 1878-5530 J9 ORG ELECTRON JI Org. Electron. PD NOV PY 2015 VL 26 BP 117 EP 120 DI 10.1016/j.orgel.2015.07.029 PG 4 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA CR3IX UT WOS:000361226900019 ER PT J AU Song, B Lu, WY AF Song, Bo Lu, Wei-Yang TI Effect of twist on transverse impact response of ballistic fiber yarns SO INTERNATIONAL JOURNAL OF IMPACT ENGINEERING LA English DT Article DE Transverse impact; Ballistic fiber; Twist; Ballistic performance; Hopkinson bar AB A Hopkinson bar was employed to conduct transverse impact testing of twisted Kevlar KM2 fiber yarns at the same impact speed. The speed of Euler transverse wave generated by the impact was measured utilizing a high speed digital camera. The study included fiber yarns twisted by different amounts. The Euler transverse wave speed was observed to increase with increasing amount of twist of the fiber yarn, within the range of this investigation. The higher transverse wave speeds in the more twisted fiber yarns indicate better ballistic performance in soft body armors for personal protection. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Song, Bo] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Lu, Wei-Yang] Sandia Natl Labs, Livermore, CA 94550 USA. RP Song, B (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM bsong@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 10 TC 0 Z9 0 U1 2 U2 10 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0734-743X EI 1879-3509 J9 INT J IMPACT ENG JI Int. J. Impact Eng. PD NOV PY 2015 VL 85 BP 1 EP 4 DI 10.1016/j.ijimpeng.2015.06.005 PG 4 WC Engineering, Mechanical; Mechanics SC Engineering; Mechanics GA CQ3OS UT WOS:000360512600001 ER PT J AU Rohr, WF Nguyen, K Bunting, BG Qu, J AF Rohr, William F. Nguyen, Ke Bunting, Bruce G. Qu, Jun TI Feasibility of Observing Small Differences in Friction Mean Effective Pressure between Different Lubricating Oil Formulations Using a Small, Single-Cylinder Motored Engine Rig SO TRIBOLOGY TRANSACTIONS LA English DT Article DE Friction Test Methods; Diesel Engine Oils; Diesel Engines; FMEP; Automotive ID PERFORMANCE AB The feasibility of using a motored single-cylinder 517 cc diesel engine to observe small frictional differences between oil formulations is investigated. Friction mean effective pressure (FMEP) is measured and compared for an SAE 10W-30 and an SAE 5W-20 oil in three stages of production: base oil, commercial oil without a friction and wear reducing additive, and fully formulated commercial oil. In addition, a commercial SAE 5W-30 engine oil is investigated. Friction mean effective pressure is plotted versus oil dynamic viscosity to compare the lubricant FMEP at a given viscosity. Linear regressions and average friction mean effective pressure are used as a secondary means of comparing FMEP for the various oil formulations. Differences between the oils are observed with the base oil having higher friction at a given viscosity but a lower average FMEP due to the temperature distribution of the test and lower viscosities reached by the base oil. The commercial oil is shown to have both a higher FMEP at a given viscosity and a higher average FMEP than the commercial oil without a friction and wear reducing additive. The increase in friction for the oil without a friction and wear reduction additive indicates that the operational regime of the engine may be out of the bounds of the optimal regime for the additive or that the additive is more optimized for wear reduction. Results show that it is feasible to observe small differences in FMEP between lubricating oil formulations using a small, single-cylinder motored engine. C1 [Rohr, William F.; Nguyen, Ke] Univ Tennessee, Dept Mech Aerosp & Biomed Engn, Knoxville, TN 37996 USA. [Bunting, Bruce G.] Oak Ridge Natl Lab, Fuels Engines & Emiss Res Ctr, Natl Transportat Res Ctr, Knoxville, TN 37932 USA. [Qu, Jun] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Rohr, WF (reprint author), Univ Tennessee, Dept Mech Aerosp & Biomed Engn, Knoxville, TN 37996 USA. OI Qu, Jun/0000-0001-9466-3179 FU Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Office; ORNL [DE-AC05-00OR22725] FX This work was supported by the Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Office and conducted at ORNL under contract number DE-AC05-00OR22725. NR 23 TC 0 Z9 0 U1 2 U2 18 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 1040-2004 EI 1547-397X J9 TRIBOL T JI Tribol. Trans. PD NOV-DEC PY 2015 VL 58 IS 6 BP 1067 EP 1075 DI 10.1080/10402004.2015.1041627 PG 9 WC Engineering, Mechanical SC Engineering GA CQ5SS UT WOS:000360666600010 ER PT J AU Petrovic, M Sadowski, JT Siber, A Kralj, M AF Petrovic, Marin Sadowski, Jerzy T. Siber, Antonio Kralj, Marko TI Wrinkles of graphene on Ir(111): Macroscopic network ordering and internal multi-lobed structure SO CARBON LA English DT Article ID CHEMICAL-VAPOR-DEPOSITION; LARGE-AREA GRAPHENE; POLYCRYSTALLINE GRAPHENE; ELECTRONIC TRANSPORT; SUPPORTED GRAPHENE; THIN-FILMS; STRAIN; LAYERS; INTERCALATION; REACTIVITY AB The large-scale production of graphene monolayer greatly relies on epitaxial samples which often display stress-relaxation features in the form of wrinkles. Wrinkles of graphene on Ir(111) are found to exhibit a fairly well ordered interconnecting network which is characterized by low-energy electron microscopy (LEEM). The high degree of quasi-hexagonal network arrangement for the graphene aligned to the underlying substrate can be well described as a (non-Poissonian) Voronoi partition of a plane. The results obtained strongly suggest that the wrinkle network is frustrated at low temperatures, retaining the order inherited from elevated temperatures when the wrinkles interconnect in junctions which most often join three wrinkles. Such frustration favors the formation of multi-lobed wrinkles which are found in scanning tunneling microscopy (STM) measurements. The existence of multiple lobes is explained within a model accounting for the interplay of the van der Waals attraction between graphene and iridium and bending energy of the wrinkle. The presented study provides new insights into wrinkling of epitaxial graphene and can be exploited to further expedite its application. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Petrovic, Marin; Siber, Antonio; Kralj, Marko] Inst Fiziku, Zagreb 10000, Croatia. [Sadowski, Jerzy T.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Siber, Antonio; Kralj, Marko] Inst Fiziku, Ctr Excellence Adv Mat & Sensing Devices, Zagreb 10000, Croatia. RP Petrovic, M (reprint author), Inst Fiziku, Bijenicka 46, Zagreb 10000, Croatia. EM mpetrovic@ifs.hr RI Siber, Antonio/B-8881-2008; Petrovic, Marin/N-2473-2013; Kralj, Marko/A-8232-2008; OI Siber, Antonio/0000-0003-1665-6541; Petrovic, Marin/0000-0002-2234-1207; Kralj, Marko/0000-0002-9786-3130; Sadowski, Jerzy/0000-0002-4365-7796 FU Unity Through Knowledge Fund [66/10]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886, DE-SC0012704]; Center of Excellence for Advanced Materials and Sensing Devices FX The financial support by the Unity Through Knowledge Fund (Grant No. 66/10) is gratefully acknowledged. Research has been carried out in part at the Center for Functional Nanomaterials and National Synchrotron Light Source, BNL, which are supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contracts No. DE-AC02-98CH10886 and DE-SC0012704. The financial support through the Center of Excellence for Advanced Materials and Sensing Devices, research unit for Graphene and Related 2D Structures is gratefully acknowledged. NR 58 TC 1 Z9 1 U1 9 U2 74 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0008-6223 EI 1873-3891 J9 CARBON JI Carbon PD NOV PY 2015 VL 94 BP 856 EP 863 DI 10.1016/j.carbon.2015.07.059 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CQ0OD UT WOS:000360294900101 ER PT J AU Oliveira, L Saini, D Gaillard, JB Podila, R Rao, AM Serkiz, SM AF Oliveira, Luciana Saini, Deepika Gaillard, Jay B. Podila, Ramakrishna Rao, Apparao M. Serkiz, Steven M. TI Directed-assembly of carbon structures in a nonpolar dielectric liquid under the influence of DC-generated electric fields SO CARBON LA English DT Article ID TRANSPARENT; NANOTUBES; CRYSTALS; BANDGAP; FILMS AB Externally applied direct current (DC) electric fields have been examined as a means of controllable organization of carbon structures (one-dimensional multi-walled carbon nanotubes of three sizes, quasi two-dimensional exfoliated graphene platelets, and three-dimensional bulk graphite) suspended in a high dielectric strength (i.e., highly resistive) solvent (perfluorocarbon FC-40). The net particle charge of the carbon structures in FC-40 was negligible. This eliminates non-dielectrophoretic (DEP) kinetic motions and allows for examination of isolated DEP forces on the assembly process. At a sufficiently high DC field strength and carbon structure concentration, DEP directed assembly and subsequent formation of electrically conductive networks were observed. The influences of particle size, aspect ratio, concentration, and structure on the assembly and electrical conduction in this system were investigated. Threshold voltage, an operationally defined measure of the applied voltage where current flow first occurred, was used as a characteristic measure of the assembly process. Consistent with charge percolation theory, the threshold voltage was found to be inversely related to the particle concentration and directly proportional to particle size as measured by light scattering. Accordingly, we developed an agglomeration model that accounts for the influence of particle size on the threshold voltage. Published by Elsevier Ltd. C1 [Oliveira, Luciana; Serkiz, Steven M.] Clemson Univ, Sch Mat Sci & Engn, Clemson, SC 29634 USA. [Saini, Deepika; Podila, Ramakrishna; Rao, Apparao M.; Serkiz, Steven M.] Clemson Univ, Dept Phys & Astron, Clemson Nanomat Ctr, Clemson, SC 29634 USA. [Saini, Deepika; Podila, Ramakrishna; Rao, Apparao M.; Serkiz, Steven M.] Clemson Univ, COMSET, Clemson, SC 29634 USA. [Saini, Deepika; Gaillard, Jay B.; Serkiz, Steven M.] Savannah River Natl Lab, Aiken, SC 29808 USA. RP Rao, AM (reprint author), Clemson Univ, Dept Phys & Astron, Clemson Nanomat Ctr, Clemson, SC 29634 USA. EM arao@clemson.edu; steven.serkiz@srnl.doe.gov FU Savanah River National Lab under the U.S. DOE [DE-AC09-96SR18500] FX This work was supported by Savanah River National Lab under the U.S. DOE Contract DE-AC09-96SR18500. NR 23 TC 2 Z9 2 U1 3 U2 32 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0008-6223 EI 1873-3891 J9 CARBON JI Carbon PD NOV PY 2015 VL 93 BP 32 EP 38 DI 10.1016/j.carbon.2015.05.026 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CQ0ND UT WOS:000360292100004 ER PT J AU Zhang, PF Zhang, ZY Chen, JH Dai, S AF Zhang, Pengfei Zhang, Zhiyong Chen, Jihua Dai, Sheng TI Ultrahigh surface area carbon from carbonated beverages: Combining self-templating process and in situ activation SO CARBON LA English DT Article ID ORDERED MESOPOROUS CARBON; OXYGEN REDUCTION REACTION; POROUS CARBON; HYDROTHERMAL CARBONIZATION; ENERGY-STORAGE; NANOPOROUS CARBON; DOPED CARBON; PORE-SIZE; SUPERCAPACITORS; PERFORMANCE AB Ultrahigh surface area carbons (USACs, e.g., >2000 m(2)/g) are attracting tremendous attention due to their outstanding performance in energy-related applications. The state-of-art approaches to USACs involve templating or activation methods and all these techniques show certain drawbacks. In this work, a series of USACs with specific surface areas up to 3633 m(2)/g were prepared in two steps: hydrothermal carbonization (200 degrees C) of carbonated beverages (CBs) and further thermal treatment in nitrogen (600-1000 degrees C). The rich inner porosity is formed by a self-templated process during which acids and polyelectrolyte sodium salts in the beverage formulas make some contribution. This strategy covers various CBs such as Coca Cola (R), Pepsi Cola (R), Dr. Pepper (R), and Fanta (R) and it enables an acceptable product yield (based on sugars), for example: 21 wt% for carbon (2940 m(2)/g) from Coca Cola (R). Being potential electrode materials for supercapacitors, those carbon materials possessed a good specific capacitance (57.2-185.7 F g(-1)) even at a scan rate of 1000 mV s(-1). Thus, a simple and efficient strategy to USACs has been presented. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Zhang, Pengfei; Zhang, Zhiyong; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Chen, Jihua] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Zhang, PF (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM chemistryzpf@163.com; dais@ornl.gov RI Chen, Jihua/F-1417-2011; Zhang, Pengfei/I-5484-2013; Zhang, Zhiyong/H-5611-2012; Dai, Sheng/K-8411-2015 OI Chen, Jihua/0000-0001-6879-5936; Zhang, Zhiyong/0000-0001-7936-9510; Dai, Sheng/0000-0002-8046-3931 FU Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Cente - US Department of Energy, Office of Science, Office of Basic Energy Sciences [ERKCC61] FX This work was supported as part of the Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number ERKCC61. TEM (J.C.) experiments were conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. NR 71 TC 3 Z9 3 U1 11 U2 104 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0008-6223 EI 1873-3891 J9 CARBON JI Carbon PD NOV PY 2015 VL 93 BP 39 EP 47 DI 10.1016/j.carbon.2015.05.019 PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CQ0ND UT WOS:000360292100005 ER PT J AU Schmucker, SW Cress, CD Culbertson, JC Beeman, JW Dubon, OD Robinson, JT AF Schmucker, Scott W. Cress, Cory D. Culbertson, James C. Beeman, Jeffrey W. Dubon, Oscar D. Robinson, Jeremy T. TI Raman signature of defected twisted bilayer graphene SO CARBON LA English DT Article ID VAN-HOVE SINGULARITIES; OPTICAL CONDUCTIVITY; SUPERLATTICES; LAYERS; FILMS; HETEROSTRUCTURES; SPECTROSCOPY; CARBON; WATER; MICA AB Layered two-dimensional crystal systems can exhibit complex interlayer interactions, which are influenced by local crystal structure and/or electronic variations. Here, we study the influence of defects in twisted bilayer graphene (TBG) using Raman spectroscopy. We explore the varied influence of defects on three characteristic Raman modes of both fully-defected TBG, with defects introduced in both layers, and half-defected TBG, with defects introduced in only a single layer. The resonance condition responsible for a strong enhancement of the G peak is sensitive to structural disorder and is quenched within a radius similar to 3 nm of defects, while the twist-angle dependence of the 2D peak is influenced only at the site of structural disorder (similar to 1 nm radius). (C) 2015 Elsevier Ltd. All rights reserved. C1 [Schmucker, Scott W.; Cress, Cory D.; Culbertson, James C.; Robinson, Jeremy T.] US Naval Res Lab, Washington, DC 20375 USA. [Beeman, Jeffrey W.; Dubon, Oscar D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Dubon, Oscar D.] Univ Calif Berkeley, Berkeley, CA 94720 USA. RP Schmucker, SW (reprint author), US Naval Res Lab, Washington, DC 20375 USA. EM scott.schmucker@gmail.com RI Schmucker, Scott/D-8312-2012; OI Schmucker, Scott/0000-0003-2908-5282; Cress, Cory/0000-0001-7563-6693 FU Office of Naval Research; Defense Threat Reduction Agency; NRL Nanoscience Institute FX The work at the Naval Research Laboratory was supported by the Office of Naval Research, the Defense Threat Reduction Agency, and the NRL Nanoscience Institute. This research was performed while S.W. Schmucker held a National Research Council Associateship Award at the Naval Research Laboratory. NR 44 TC 6 Z9 6 U1 6 U2 64 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0008-6223 EI 1873-3891 J9 CARBON JI Carbon PD NOV PY 2015 VL 93 BP 250 EP 257 DI 10.1016/j.carbon.2015.05.076 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CQ0ND UT WOS:000360292100026 ER PT J AU del Pino, AP Gyorgy, E Logofatu, C Puigmarti-Luis, J Gao, W AF Perez del Pino, Angel Gyoergy, Eniko Logofatu, Constantin Puigmarti-Luis, Josep Gao, Wei TI Laser-induced chemical transformation of graphene oxide-iron oxide nanoparticles composites deposited on polymer substrates SO CARBON LA English DT Article ID ELECTRONIC-STRUCTURE; GRAPHITE OXIDE; QUANTUM DOTS; REDUCTION; FE3O4; DEFECTS; FUNCTIONALIZATION; SPECTROSCOPY; WRINKLES; SINGLE AB Ultraviolet laser irradiation of films composed of graphene oxide (GO) and GO-magnetite (Fe3O4) nanoparticles deposited on polydimethylsiloxane substrates is carried out. The irradiations are performed in vacuum and ammonia-rich gas environments. Electron and scanning probe microscopies reveal a rippling process in GO sheets as the accumulation of laser pulses proceeds, being the effect more pronounced with the increase of laser fluence. X-ray photoelectron spectroscopy analyses point to laser-induced chemical reaction pathways in GO completely different depending on the environment and the presence or absence of Fe3O4 nanoparticles. It is demonstrated that GO-based films with diverse type of oxygen- and nitrogen-containing chemical groups can be obtained by means of laser irradiation processes. The sheet resistance of these materials is also correlated to their structure and composition. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Perez del Pino, Angel; Gyoergy, Eniko] Consejo Super Invest Cient ICMAB CSIC, Inst Ciencia Mat Barcelona, Bellaterra 08193, Spain. [Gyoergy, Eniko] Natl Inst Lasers Plasma & Radiat Phys, Bucharest 77125, Romania. [Logofatu, Constantin] Natl Inst Mat Phys, Bucharest 77125, Romania. [Puigmarti-Luis, Josep] Swiss Fed Labs Mat Sci & Technol, CH-9014 St Gallen, Switzerland. [Gao, Wei] N Carolina State Univ, Chem & Sci Dept, Text Engn, Raleigh, NC 27695 USA. [Gao, Wei] Los Alamos Natl Lab, Ctr Integrated Nanotecnol, Los Alamos, NM 87545 USA. RP del Pino, AP (reprint author), Consejo Super Invest Cient ICMAB CSIC, Inst Ciencia Mat Barcelona, Campus UAB, Bellaterra 08193, Spain. EM aperez@icmab.es RI Perez del Pino, Angel/G-3758-2011; Puigmarti-Luis, Josep/A-5302-2015 FU Spanish Ministry of Economy and Competitiveness [ENE2014-56109-C3-3-R]; Executive Unit for Financing Higher Education, Research, Development, and Innovation of the Romanian Ministry of Education, Research, Youth, and Sports [PN-II-PT-PCCA-2011-3.2-1235]; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396]; College of Textiles at North Carolina State University; Ramon y Cajal program from the Spanish Ministry of Economy and Competitiveness [RYC-2011-08071] FX The authors acknowledge the financial support of the Spanish Ministry of Economy and Competitiveness under the project ENE2014-56109-C3-3-R, in addition to the Executive Unit for Financing Higher Education, Research, Development, and Innovation of the Romanian Ministry of Education, Research, Youth, and Sports under the Grant PN-II-PT-PCCA-2011-3.2-1235. This work was also performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-AC52-06NA25396. Wei Gao thanks the start-up funding support from the College of Textiles at North Carolina State University. Josep Puigmarti Luis also acknowledge the Ramon y Cajal program (RYC-2011-08071) from the Spanish Ministry of Economy and Competitiveness. NR 53 TC 4 Z9 4 U1 11 U2 87 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0008-6223 EI 1873-3891 J9 CARBON JI Carbon PD NOV PY 2015 VL 93 BP 373 EP 383 DI 10.1016/j.carbon.2015.05.078 PG 11 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CQ0ND UT WOS:000360292100039 ER PT J AU Azoz, S Gilbertson, LM Hashmi, SM Han, P Sterbinsky, GE Kanaan, SA Zimmerman, JB Pfefferle, LD AF Azoz, Seyla Gilbertson, Leanne M. Hashmi, Sara M. Han, Patrick Sterbinsky, George E. Kanaan, Stacy A. Zimmerman, Julie B. Pfefferle, Lisa D. TI Enhanced dispersion and electronic performance of single-walled carbon nanotube thin films without surfactant: A comprehensive study of various treatment processes SO CARBON LA English DT Article ID CHEMICAL OXIDATION; NETWORKS; CONDUCTIVITY; NEXAFS; SOLUBILIZATION; DISPERSABILITY; TRANSISTORS; AGGREGATION; FABRICATION; CHEMISTRY AB A method for enhancing electronic performance of single-walled carbon nanotube (SWCNT) thin films through enhanced dispersion of SWCNTs in aqueous solutions is presented. The best dispersion enhancement is obtained by covalent attachment of urea to the acid functionalized SWCNTs. Dispersion properties of urea treatment are compared to conventional chemical and physical treatment techniques, such as surfactants. The treatment type and time significantly influence SWCNT surface functionalization, which determines the dispersion effectiveness as described by the SWCNT aggregate size, morphology and stability. The findings suggest that urea-SWCNTs, as compared to surfactant dispersed-SWCNTs, resulted in the most effective dispersion method among chemical treatments, yielding the smallest monodispersed aggregates with the most rod-like morphology that were stable over the greatest range in pH. Thin films prepared with SWCNT samples were evaluated for their transparency and resistance, two metrics that are important for electronics device applications. The urea-SWCNT films exhibited superior optoelectrical properties compared to SWCNT films prepared with conventional chemicals as well as surfactants. This indicates a correlation between degree of dispersibility and optoelectrical properties. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Azoz, Seyla; Gilbertson, Leanne M.; Hashmi, Sara M.; Han, Patrick; Kanaan, Stacy A.; Zimmerman, Julie B.; Pfefferle, Lisa D.] Yale Univ, Dept Chem & Environm Engn, New Haven, CT 06520 USA. [Sterbinsky, George E.] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. [Zimmerman, Julie B.] Yale Univ, Sch Forestry & Environm Studies, New Haven, CT 06520 USA. RP Pfefferle, LD (reprint author), Yale Univ, Dept Chem & Environm Engn, New Haven, CT 06520 USA. EM lisa.pfefferle@yale.edu RI Zimmerman, Julie/K-9572-2013; OI Gilbertson, Leanne M/0000-0003-3396-4204 FU NSF [DMR-0934520, CBET-1264698]; U.S. EPA [RD83558001-0] FX Authors gratefully acknowledge financial support from NSF DMR-0934520, NSF CBET-1264698 and U.S. EPA under Assistance Agreement No: RD83558001-0. The authors acknowledge Dr Dario Arena and NSLS, Brookhaven National Laboratories for use of their facilities. We thank Prof Gary Haller for critical discussions, Magdalena Majewska for help in NEXAFS measurements, Dr Judy Cha for help in TEM imaging, and Melis Emre for assistance with data analysis. NR 55 TC 6 Z9 6 U1 5 U2 44 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0008-6223 EI 1873-3891 J9 CARBON JI Carbon PD NOV PY 2015 VL 93 BP 1008 EP 1020 DI 10.1016/j.carbon.2015.05.087 PG 13 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CQ0ND UT WOS:000360292100103 ER PT J AU Seong, H Choi, S AF Seong, Heeje Choi, Seungmok TI Oxidation-derived maturing process of soot, dependent on O-2-NO2 mixtures and temperatures SO CARBON LA English DT Article ID DIESEL PARTICULATE; CARBON-BLACKS; REACTIVITY; RAMAN; ENGINE; NANOSTRUCTURE; IMPACT; NO2; COMBUSTION; MICROSCOPY AB Oxidizer- and temperature-dependent soot properties were investigated to better understand soot oxidation process. For this work, partially oxidized Printex-U samples as surrogate soot, under three different O-2-NO2 mixtures, were analyzed by using the high resolution-transmission electron microscope, Raman microscope and Fourier transform infrared spectroscopy-attenuated total reflectance. The results show that the maturing process was much dependent on NO2 content in the O-2-NO2 mixture: with no NO2 added, soot oxidized through the internal-burning out process, whereas with increased NO2 in the mixture, soot tended to oxidize through the external burning process. As the NO2 content increased, the preferential oxidation of less-ordered carbon crystallites decreased and as a result the maturing process was delayed. Internal burning-out process by O-2 only was also verified at various temperatures and with actual engine soot such as diesel soot and gasoline direct-injection (GDI) soot by TEM observations. Despite similar internal burning-out process, however, it was shown that oxidation at increased temperature resulted in relatively less-ordered soot, implying that soot maturing process was delayed with temperature. Since soot oxidation rate increased with temperature, the increase in oxidation temperature seems to diminish preference on short-ranged crystallites like more efficient O-2-NO2 cases. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Seong, Heeje; Choi, Seungmok] Argonne Natl Lab, Ctr Transportat Res, Argonne, IL 60439 USA. RP Seong, H (reprint author), Argonne Natl Lab, Ctr Transportat Res, 9700 S Cass Ave, Argonne, IL 60439 USA. EM hseong@anl.gov FU Argonne, a U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357]; Advanced Engine Combustion Program at the U.S. Department of Energy Office of Vehicle Technologies; Corning Inc.; Hyundai motor company; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne''). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. The U.S. government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, perform publicly and display publicly, by or on behalf of the government. The authors thank the Advanced Engine Combustion Program at the U.S. Department of Energy Office of Vehicle Technologies, Corning Inc. and Hyundai motor company for their support. Furthermore, the use of the TEM instruments at the Center for Nanoscale Materials facility and the Electron Microscopy Center was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. NR 35 TC 4 Z9 6 U1 5 U2 25 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0008-6223 EI 1873-3891 J9 CARBON JI Carbon PD NOV PY 2015 VL 93 BP 1068 EP 1076 DI 10.1016/j.carbon.2015.07.008 PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CQ0ND UT WOS:000360292100109 ER PT J AU Forthomme, D Cich, MJ Twagirayezu, S Hall, GE Sears, TJ AF Forthomme, D. Cich, M. J. Twagirayezu, S. Hall, G. E. Sears, T. J. TI Application of the Hartmann-Tran profile to precise experimental data sets of (C2H2)-C-12 SO JOURNAL OF QUANTITATIVE SPECTROSCOPY & RADIATIVE TRANSFER LA English DT Article DE Lineshape modeling; Acetylene; C2H2; Frequency comb referenced spectroscopy; HTP ID WAVE COHERENT TRANSIENTS; SPEED DEPENDENCE; SPECTRAL LINES; BROADENED HF; COLLISIONS; ACETYLENE; DOPPLER; PARAMETERS; VELOCITY; HITRAN AB Self- and nitrogen-broadened line shape data for the P-e(11) line of the v(1) + v(3) band of acetylene, recorded using a frequency comb-Stabilized laser spectrometer, have been analyzed using the Hartmann-Tran profile (HTP) line shape model in a multispectrum fitting. In total, the data included measurements recorded at temperatures between 125 K and 296 K and at pressures between 4 and 760 Ton. New, sub-Doppler, frequency combreferenced measurements of the positions of multiple underlying hot band lines have also been made. These underlying lines significantly affect the P-e(11) line profile at temperatures above 240 K and poorly known frequencies previously introduced errors into the line shape analyses. The behavior of the HTP model was compared to the quadratic speed dependent Voigt profile (QSDVP) expressed in the frequency and time domains. A parameter uncertainty analysis was carried out using a Monte Carlo method based on the estimated pressure, transmittance and frequency measurement errors. From the analyses, the P-e(11) line strength was estimated to be 1.2014(50)x10(-2) in cm molecule(-1) units at 296 K with the standard deviation in parenthesis. For analyzing these data, we found that a reduced form of the HTP, equivalent to the QSDVP, was most appropriate because the additional parameters included in the full HTP were not well determined. As a supplement to this work, expressions for analytic derivatives and a lineshape fitting code written in Matlab for the HTP are available. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Forthomme, D.; Twagirayezu, S.; Hall, G. E.; Sears, T. J.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Cich, M. J.; Sears, T. J.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. RP Sears, TJ (reprint author), Brookhaven Natl Lab, Dept Chem, Bldg 555A,POB 5000, Upton, NY 11973 USA. EM sears@bnl.gov RI Sears, Trevor/B-5990-2013; Hall, Gregory/D-4883-2013; Twagirayezu, Sylvestre/Q-4651-2016 OI Sears, Trevor/0000-0002-5559-0154; Hall, Gregory/0000-0002-8534-9783; FU U.S. Department of Energy, Office of Science [DE-SC0012704]; Division of Chemical Sciences, Geosciences and Biosciences within the Office of Basic Energy Sciences FX We thank Professor Robert Gamache (University of Massachussetts) for discussions that motivated this work. We are also grateful to Professor David Perry (University of Akron) who provided us with the results of the global polyad Hamiltonian for acetylene and to Professor Hiroyuki Sasada (Keio University) who helped us identify several of the hot band lines in our spectra. Work at Brookhaven National Laboratory was carried out under Contract no. DE-SC0012704 with the U.S. Department of Energy, Office of Science, and supported by its Division of Chemical Sciences, Geosciences and Biosciences within the Office of Basic Energy Sciences. NR 41 TC 2 Z9 2 U1 5 U2 13 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0022-4073 EI 1879-1352 J9 J QUANT SPECTROSC RA JI J. Quant. Spectrosc. Radiat. Transf. PD NOV PY 2015 VL 165 BP 28 EP 37 DI 10.1016/j.jqsrt.2015.06.013 PG 10 WC Optics; Spectroscopy SC Optics; Spectroscopy GA CQ3PF UT WOS:000360514100004 ER PT J AU Peterson, JW Gu, BH Seymour, MD AF Peterson, Jonathan W. Gu, Baohua Seymour, Michael D. TI Surface interactions and degradation of a fluoroquinolone antibiotic in the dark in aqueous TiO2 suspensions SO SCIENCE OF THE TOTAL ENVIRONMENT LA English DT Article DE Fluoroquinolone degradation; Titanium oxide nanoparticles; Ofloxacin; Antibiotics in wastewater; PPCP contamination ID TITANIUM-DIOXIDE NANOPARTICLES; STRUCTURALLY RELATED AMINES; WASTE-WATER CONTAMINANTS; ANTIBACTERIAL AGENTS; AQUATIC ENVIRONMENT; NATIONAL RECONNAISSANCE; OXIDE NANOPARTICLES; MASS-SPECTROMETRY; ORGANIC-MATTER; SOIL AB Fluoroquinolone antibiotics (FQs) are important drugs used in human and veterinary medicine. Their detection in natural waters and waste water treatment plants, along with increased resistance to FQs among some bacteria, have generated an increased interest in the fate of these drugs in the environment. Partitioning of FQs between an aqueous solution and attendant substrates depends, in part, on the surface reactivity of the adsorbent, commonly a function of particle size, surface charge, and functional groups. This study investigated the surface interactions between the FQ drug ofloxacin (OFL) and titanium oxide (TiO2), a common catalyst and widely-observed constituent in many consumer products. Raman and fluorescence spectroscopic techniques, as well as LC/MS, were used to determine the OFL moieties present on TiO2 surfaces and in attendant solutions. Raman spectra indicate that the C=O (ketone) group of the quinolone core, the NH+ of the piperazinyl ring, and CH3 of benzoxazine core are the most active in sorption onto the TiO2 surface. Raman spectra also show that the sorbed benzoxazine-quinolone core and piperazinyl moieties are readily desorbed from the surface by re-suspending samples in water. Importantly, we found that OFL could be degraded by reacting with TiO2 even in the dark. Complementary LC/MS analysis of the attendant supernatants indicates the presence of de-piperazinylated and de-carboxylated OFL breakdown products in supernatant solutions. Together, both Raman and LC/MS analyses indicate that TiO2 breaks the compound into piperazinyl and carboxylate groups which attach to the surface, whereas decarboxylated and hydroxylated quinolone moieties remain in solution. The present study thus identifies the sorption mechanisms and breakdown products of OFL during dark reactions with TiO2, which is critically important for understanding the fate and transport of OFL as it enters the soil and aquatic environment. (C) 2015 Elsevier B.V. All rights reserved. C1 [Peterson, Jonathan W.] Hope Coll, Dept Geol & Environm Sci, Holland, MI 49422 USA. [Gu, Baohua] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Seymour, Michael D.] Hope Coll, Dept Chem, Holland, MI 49422 USA. RP Peterson, JW (reprint author), Hope Coll, Dept Geol & Environm Sci, POB 9000, Holland, MI 49422 USA. EM peterson@hope.edu RI Gu, Baohua/B-9511-2012 OI Gu, Baohua/0000-0002-7299-2956 FU Hope College Department of Geological & Environmental Sciences; GLCA-ACM Oak Ridge Science Semester Program; Office of Biological and Environmental Research, Office of Science, US Department of Energy (DOE) [DE-AC05-00OR22725]; DOE [DE-AC05-00OR22725] FX This research was sponsored in part by the Hope College Department of Geological & Environmental Sciences and the GLCA-ACM Oak Ridge Science Semester Program, and by the Office of Biological and Environmental Research, Office of Science, US Department of Energy (DOE) (DE-AC05-00OR22725). Oak Ridge National Laboratory is managed by UT-Battelle LLC for the DOE under contract DE-AC05-00OR22725. Thanks to Xiangping Yin and Xia Lu for their assistance with analysis and instrumentation. NR 44 TC 2 Z9 2 U1 10 U2 67 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0048-9697 EI 1879-1026 J9 SCI TOTAL ENVIRON JI Sci. Total Environ. PD NOV 1 PY 2015 VL 532 BP 398 EP 403 DI 10.1016/j.scitotenv.2015.06.024 PG 6 WC Environmental Sciences SC Environmental Sciences & Ecology GA CQ0LD UT WOS:000360286500039 PM 26086371 ER PT J AU Wei, HL Pal, S Manvatkar, V Lienert, TJ DebRoy, T AF Wei, H. L. Pal, S. Manvatkar, V. Lienert, T. J. DebRoy, T. TI Asymmetry in steel welds with dissimilar amounts of sulfur SO SCRIPTA MATERIALIA LA English DT Article DE Surface active element; Center line shift (CLS); Marangoni flow ID FLUID-FLOW; STAINLESS-STEEL; SURFACE-TENSION; HEAT-TRANSFER; GTA AB During welding of steels containing dissimilar amounts of sulfur, the weld pool is shifted laterally from the original joint interface and rotated at an angle with the interface. The mechanism for this unusual behavior is not known. Here, we show for the first time through comparison of numerically calculated and experimental results that Marangoni convection causes these rotational and translational asymmetries and the reported arc shift is a consequence of asymmetric melting rather than its cause. (C) 2015 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Wei, H. L.; Pal, S.; Manvatkar, V.; DebRoy, T.] Penn State Univ, Dept Mat Sci & Engn, Forest Resources Lab 309, University Pk, PA 16802 USA. [Lienert, T. J.] Los Alamos Natl Lab, Div Mat Sci, Los Alamos, NM 87545 USA. RP DebRoy, T (reprint author), Penn State Univ, Dept Mat Sci & Engn, Forest Resources Lab 309, University Pk, PA 16802 USA. EM debroy@psu.edu RI Wei, Huiliang/B-2265-2017 OI Wei, Huiliang/0000-0003-2373-6603 NR 15 TC 1 Z9 1 U1 2 U2 17 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6462 J9 SCRIPTA MATER JI Scr. Mater. PD NOV PY 2015 VL 108 BP 88 EP 91 DI 10.1016/j.scriptamat.2015.06.024 PG 4 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA CP9YB UT WOS:000360250700022 ER PT J AU Zhang, CX Hu, J Zhang, XD Wang, XK Meng, YD AF Zhang, Chengxu Hu, Jue Zhang, Xiaodong Wang, Xiangke Meng, Yuedong TI Certain nitrogen functionalities on carbon nanofiber support for improving platinum performance SO CATALYSIS TODAY LA English DT Article; Proceedings Paper CT 2nd China-USA Symposium on Energy CY JUN 26-28, 2015 CL Shanghai Jiao Tong, Shanghai, PEOPLES R CHINA HO Shanghai Jiao Tong DE Nitrogen functionalities; Carbon nanofiber; Plasma modification; Platinum electrocatalytic activity; Durability ID OXYGEN REDUCTION REACTION; ELECTROLYTE FUEL-CELLS; DOPED GRAPHENE; EXCHANGE MEMBRANE; NANOTUBES; CATALYST; METHANOL; NANOPARTICLES; SPECTROSCOPY; CLUSTERS AB Nitrogen (N) modification of carbon nanomaterial, which plays a critical role in improving platinum (Pt) performance, has shown fascinating applications. N-doped carbon nanofiber (CNF)-supported platinum catalysts were produced by an approach combined of plasma-enhanced chemical vapor deposition and in situ plasma activation. This approach can successfully introduce nitrogen functionalities into a carbon network, and at the same time, preserve the highly graphitic structure of the carbon support. XPS results indicate that NH3 plasma modification mainly creates pyridinic nitrogen functionalities, while N-2 plasma modification mainly increases the percentage of pyrrolic nitrogen in the carbon network, which suggests a modification of certain nitrogen functionalities on the carbon support. By correlating TEM and XPS data with electrochemical measurements, we conclude that the N-modified CNF exhibits a significant improvement in Pt electrochemical activity and stability than pristine CNF support and Pt/CNF-NH3 electrode with smallest Pt particle size, highest percentage of pyridinic nitrogen, exhibits the highest Pt utilization, electrochemical activity, and poisoning-resistance ability. Our study gives both insights on the influence of N modification of the carbon support in platinum catalytic effectiveness and a route for formation of certain nitrogen functionalities on the carbon support. This will be important for the further development of Pt catalysts. (C) 2015 Elsevier B.V. All rights reserved. C1 [Zhang, Chengxu; Hu, Jue; Zhang, Xiaodong; Wang, Xiangke; Meng, Yuedong] Chinese Acad Sci, Inst Plasma Phys, Hefei 230031, Peoples R China. [Hu, Jue] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Wang, Xiangke] North China Elect Power Univ, Sch Environm & Chem Engn, Beijing 102206, Peoples R China. RP Hu, J (reprint author), Chinese Acad Sci, Inst Plasma Phys, POB 1126, Hefei 230031, Peoples R China. EM hujue@ipp.ac.cn RI Wang, Xiangke/I-5806-2012 OI Wang, Xiangke/0000-0002-3352-1617 FU National Nature Science Foundation of Anhui province [1308085QA09]; National Nature Science Foundation of China [11205202, 21203204, 11175214] FX This research is financially supported by the National Nature Science Foundation of Anhui province (No. 1308085QA09) and National Nature Science Foundation of China (Nos. 11205202, 21203204, 11175214). NR 61 TC 2 Z9 2 U1 7 U2 65 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0920-5861 EI 1873-4308 J9 CATAL TODAY JI Catal. Today PD NOV 1 PY 2015 VL 256 BP 193 EP 202 DI 10.1016/j.cattod.2015.01.026 PN 1 PG 10 WC Chemistry, Applied; Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA CP7RJ UT WOS:000360085300026 ER PT J AU Huskins, EL Cordero, ZC Schuh, CA Schuster, BE AF Huskins, Emily L. Cordero, Zachary C. Schuh, Christopher A. Schuster, Brian E. TI Micropillar compression testing of powders SO JOURNAL OF MATERIALS SCIENCE LA English DT Article ID METALLIC-GLASS; SPHERICAL INDENTATION; MECHANICAL-BEHAVIOR; DEFORMATION MODE; LENGTH SCALES; SIZE; STRENGTH; PLASTICITY; BULK; MICROCOMPRESSION AB An experimental design for microcompression on individual powder particles is proposed as a means of testing novel materials without the challenges associated with consolidation to produce bulk specimens. This framework is demonstrated on an amorphous tungsten alloy powder, and yields reproducible measurements of the yield strength (4.5 +/- A 0.3 GPa) and observations of the deformation mode (in this case, serrated flow by shear localization). C1 Army Res Lab, Oak Ridge Inst Sci & Educ, Postdoctoral Fellowship Program, Aberdeen Proving Ground, MD 21005 USA. [Cordero, Zachary C.; Schuh, Christopher A.] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. [Schuster, Brian E.] Army Res Lab, RDRL WML H, Weap & Mat Res Directorate, Aberdeen Proving Ground, MD 21005 USA. RP Schuster, BE (reprint author), Army Res Lab, RDRL WML H, Weap & Mat Res Directorate, Aberdeen Proving Ground, MD 21005 USA. EM brian.e.schuster.civ@mail.mil FU US Defense Threat Reduction Agency [HDTRA1-11-1-0062]; Oak Ridge Institute for Space and Education (ORISE) Program [1120-1120-99]; Department of Defense through the NDSEG fellowship program; [11-24] FX This study was supported by the US Defense Threat Reduction Agency under Grant No. HDTRA1-11-1-0062. ELH acknowledges support through the Oak Ridge Institute for Space and Education (ORISE) Program #1120-1120-99. ZCC gratefully acknowledges support from the Department of Defense through the NDSEG fellowship program. BES would like to acknowledge support work from the Cooperative Research and Development Agreement #11-24. NR 45 TC 1 Z9 1 U1 3 U2 20 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0022-2461 EI 1573-4803 J9 J MATER SCI JI J. Mater. Sci. PD NOV PY 2015 VL 50 IS 21 BP 7058 EP 7063 DI 10.1007/s10853-015-9260-1 PG 6 WC Materials Science, Multidisciplinary SC Materials Science GA CP3VR UT WOS:000359811300021 ER PT J AU Song, XY McIntyre, D Chen, XQ Barbero, EJ Chen, Y AF Song, Xueyan McIntyre, Dustin Chen, Xueqin Barbero, Ever J. Chen, Yun TI Phase evolution and thermoelectric performance of calcium cobaltite upon high temperature aging SO CERAMICS INTERNATIONAL LA English DT Article DE Electron microscopy; Thermoelectric materials; Calcium cobaltite; Crystal phase transformation ID MISFIT-LAYERED COBALTITE; CA3CO4O9 THIN-FILMS; THERMAL-STABILITY; CRYSTAL-STRUCTURE; OXIDES; MAGNETORESISTANCE; (CAOH)(1.14)COO2; COMPOUND; CERAMICS; CA3CO2O6 AB Crystal phase transformation and their nanostructure evolutions were studied for baseline thermoelectric ceramic Ca3Co4O9, and for a sample aged at 1283 K, which is significantly higher than the Ca3Co4O9 decomposition temperature of 1199 K. X-ray diffraction from both samples only reveals peaks from Ca3Co4O9 phase. TEM examination reveals that in the aged sample, CaO nano-phase exists between neighboring Ca3Co4O9 nano-lamella grains. Moreover, a small amount of Co3O4 and Ca2Co2O5 phase were also observed in the aged sample. The Ca2Co2O5 phase does not exhibit the same lamella nanostructure as Ca3Co4O9 and displayed few crystal defects. Except for Ca3Co4O9, Ca2Co2O5, and Co3O4, no other Ca-Co-O cobaltite phase, such as Ca3Co2O6, was found in the aged sample. Electrical and thermal properties of both baseline and aged sample were measured over the temperature range of 320-1033 K. (C) 2015 Elsevier Ltd All rights reserved. C1 [Song, Xueyan; Chen, Xueqin; Barbero, Ever J.; Chen, Yun] W Virginia Univ, Dept Mech & Aerosp Engn, Morgantown, WV 26506 USA. [McIntyre, Dustin] Natl Energy Technol Lab, Morgantown, WV 26507 USA. RP Song, XY (reprint author), W Virginia Univ, Dept Mech & Aerosp Engn, Evansdale Dr, Morgantown, WV 26506 USA. EM xueyan.song@mail.wvu.edu FU National Science Foundation DMR [1254594] FX Support from the National Science Foundation DMR (1254594) is greatly appreciated. NR 32 TC 1 Z9 1 U1 6 U2 55 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0272-8842 EI 1873-3956 J9 CERAM INT JI Ceram. Int. PD NOV PY 2015 VL 41 IS 9 BP 11069 EP 11074 DI 10.1016/j.ceramint.2015.05.052 PN A PG 6 WC Materials Science, Ceramics SC Materials Science GA CO4XZ UT WOS:000359165500091 ER PT J AU Sprague, MA Purkayastha, A AF Sprague, Michael A. Purkayastha, Avi TI Legendre spectral finite elements for Reissner-Mindlin composite plates SO FINITE ELEMENTS IN ANALYSIS AND DESIGN LA English DT Article DE Composite; Finite element; High order; Numerical methods; Reissner-Mindlin AB Legendre spectral finite elements (LSFEs) are examined in their application to Reissner-Mindlin composite plates for static and dynamic deformation on unstructured grids. LSFEs are high-order Lagrangian-interpolant finite elements whose nodes are located at the Gauss-Lobatto-Legendre quadrature points. Nodal quadrature is employed for mass-matrix calculations, which yields diagonal mass matrices. Full quadrature or mixed-reduced quadrature is used for stiffness-matrix calculations. Solution accuracy is examined in terms of model size, computation time, and memory storage for LSFEs and for quadratic serendipity elements calculated in a commercial finite-element code. Linear systems for both model types were solved with the same sparse-system direct solver. At their best, LSFEs provide many orders of magnitude more accuracy than the quadratic elements for a fixed measure (e.g., computation time). At their worst, LSFEs provide the same accuracy as the quadratic elements for a given measure. The LSFEs were insensitive to shear locking and were shown to be more robust in the thinplate limit than their low-order counterparts. (C) 2015 Elsevier B.V. All rights reserved. C1 [Sprague, Michael A.; Purkayastha, Avi] Natl Renewable Energy Lab, Computat Sci Ctr, Golden, CO 80401 USA. RP Sprague, MA (reprint author), Natl Renewable Energy Lab, Computat Sci Ctr, Golden, CO 80401 USA. EM Michael.A.Sprague@nrel.gov FU U.S. Department of Energy [DE-AC36-08-G028308]; National Renewable Energy Laboratory; NREL Laboratory Directed Research and Development (LDRD) program; Department of Energy's Office of Energy Efficiency and Renewable Energy FX This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08-G028308 with the National Renewable Energy Laboratory. The U.S. Government retains and the publisher, by accepting the article for publication, acknowledges that the U.S. Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this work, or allow others to do so, for U.S. Government purposes. Funding was provided by the NREL Laboratory Directed Research and Development (LDRD) program through the grant "High-Fidelity Computational Modeling of Wind-Turbine Structural Dynamics." The research was performed using computational resources sponsored by the Department of Energy's Office of Energy Efficiency and Renewable Energy and located at the National Renewable Energy Laboratory, We acknowledge insightful comments from the reviewers that led to an improved paper. NR 25 TC 0 Z9 0 U1 2 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-874X EI 1872-6925 J9 FINITE ELEM ANAL DES JI Finite Elem. Anal. Des. PD NOV 1 PY 2015 VL 105 BP 33 EP 43 DI 10.1016/j.final.2015.06.007 PG 11 WC Mathematics, Applied; Mechanics SC Mathematics; Mechanics GA CP1FN UT WOS:000359621800004 ER PT J AU Wu, HY Shahidehpour, M Alabdulwahab, A Abusorrah, A AF Wu, Hongyu Shahidehpour, Mohammad Alabdulwahab, Ahmed Abusorrah, Abdullah TI Thermal Generation Flexibility With Ramping Costs and Hourly Demand Response in Stochastic Security-Constrained Scheduling of Variable Energy Sources SO IEEE TRANSACTIONS ON POWER SYSTEMS LA English DT Article DE Demand response; flexible ramping capability; renewable energy sources; stochastic day-ahead scheduling ID UNIT COMMITMENT; WIND POWER; SCUC AB This paper proposes a stochastic day-ahead scheduling of electric power systems with flexible resources for managing the variability of renewable energy sources (RES). The flexible resources include thermal units with up/down ramping capability, energy storage, and hourly demand response (DR). The Monte Carlo simulation (MCS) is used in this paper for simulating random outages of generation units and transmission lines as well as representing hourly forecast errors of loads and RES. Numerical tests are conducted for a 6-bus system and a modified IEEE 118-bus system and the results demonstrate the benefits of applying demand response as a viable option for managing the RES variability in the least-cost stochastic power system operations. C1 [Wu, Hongyu] Natl Renewable Energy Lab, Power Syst Engn Ctr, Golden, CO 80401 USA. [Shahidehpour, Mohammad] IIT, Robert W Galvin Ctr Elect Innovat, Chicago, IL 60616 USA. [Shahidehpour, Mohammad] King Abdulaziz Univ, Fac Engn, Renewable Energy Res Grp, Jeddah 21413, Saudi Arabia. [Alabdulwahab, Ahmed; Abusorrah, Abdullah] King Abdulaziz Univ, Dept Elect & Comp Engn, Jeddah 21413, Saudi Arabia. RP Wu, HY (reprint author), Natl Renewable Energy Lab, Power Syst Engn Ctr, Golden, CO 80401 USA. EM hongyu.wu@nrel.gov; ms@iit.edu OI Wu, Hongyu/0000-0002-5223-6635 FU NSTIP strategic technologies program in the Kingdom of Saudi Arabia [13-ENE2264-03-R] FX This project was supported in part by the NSTIP strategic technologies program in the Kingdom of Saudi Arabia-Project No. 13-ENE2264-03-R. The authors also acknowledge and appreciate the technical support provided by the Science and Technology Unit at King Abdulaziz University. NR 21 TC 12 Z9 13 U1 3 U2 16 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8950 EI 1558-0679 J9 IEEE T POWER SYST JI IEEE Trans. Power Syst. PD NOV PY 2015 VL 30 IS 6 BP 2955 EP 2964 DI 10.1109/TPWRS.2014.2369473 PG 10 WC Engineering, Electrical & Electronic SC Engineering GA CO7VS UT WOS:000359371600012 ER PT J AU Liu, H Hu, ZC Song, YH Wang, JH Xie, X AF Liu, Hui Hu, Zechun Song, Yonghua Wang, Jianhui Xie, Xu TI Vehicle-to-Grid Control for Supplementary Frequency Regulation Considering Charging Demands SO IEEE TRANSACTIONS ON POWER SYSTEMS LA English DT Article DE Charging demand; electric vehicle (EV); frequency regulation capacity (FRC); supplementary frequency regulation (SFR); vehicle-to-grid (V2G) ID ELECTRIC VEHICLES AB Electric vehicles (EVs) as distributed storage devices have the potential to provide frequency regulation services due to the fast adjustment of charging/discharging power. In our previous research, decentralized vehicle-to-grid (V2G) control methods for EVs were proposed to participate in primary frequency control. In this paper, our attention is on bringing a large number of EVs into the centralized supplementary frequency regulation (SFR) of interconnected power systems. An aggregator is the coordinator between EVs and the power system control center. The aggregator calculates the total frequency regulation capacity (FRC) and expected V2G (EV2G) power of EVs based on the data communicated between the aggregator and individual EVs or EV charging stations. With FRC and EV2G power, a V2G control strategy is proposed for the aggregator to dispatch regulation requirements to EVs and EV charging stations. In individual EV charging stations, the FRC is calculated on the basis of the V2G power at present time, and EV2G power is presented considering both frequency regulation and charging demands. Besides, V2G control strategies are developed to distribute regulation requirements to each EV. Simulations on an interconnected power grid based on a practical power grid in China have demonstrated the effectiveness of the proposed strategies. C1 [Liu, Hui] Jiangsu Univ, Sch Elect & Informat Engn, Zhenjiang, Peoples R China. [Liu, Hui; Hu, Zechun; Song, Yonghua] Tsinghua Univ, Dept Elect Engn, Beijing 100084, Peoples R China. [Wang, Jianhui] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. [Xie, Xu] State Grid Corp China, North China Branch, Beijing 100053, Peoples R China. RP Liu, H (reprint author), Jiangsu Univ, Sch Elect & Informat Engn, Zhenjiang, Peoples R China. EM hughlh@126.com; zechhu@tsinghua.edu.cn; yhsong@tsinghua.edu.cn; jianhui.wang@anl.gov FU National Natural Science Foundation of China [51107054, 51107060]; National High Technology Research and Development of China 863 Program [2011AA05A110] FX This work was supported in part by the National Natural Science Foundation of China (51107054, 51107060) and in part by the National High Technology Research and Development of China 863 Program (2011AA05A110). Paper no. TPWRS-00455-2014. NR 24 TC 14 Z9 16 U1 6 U2 35 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8950 EI 1558-0679 J9 IEEE T POWER SYST JI IEEE Trans. Power Syst. PD NOV PY 2015 VL 30 IS 6 BP 3110 EP 3119 DI 10.1109/TPWRS.2014.2382979 PG 10 WC Engineering, Electrical & Electronic SC Engineering GA CO7VS UT WOS:000359371600028 ER PT J AU Wang, ZY Wang, JH AF Wang, Zhaoyu Wang, Jianhui TI Self-Healing Resilient Distribution Systems Based on Sectionalization Into Microgrids SO IEEE TRANSACTIONS ON POWER SYSTEMS LA English DT Article DE Distributed power generation; microgrid (MG); power distribution; power distribution faults; self-healing; stochastic optimization ID DISTRIBUTION NETWORKS; OPTIMIZATION; GENERATORS; MANAGEMENT; SECURITY; FEEDERS; ERROR AB This paper proposes a novel comprehensive operation and self-healing strategy for a distribution system with both dispatchable and nondispatchable distributed generators (DGs). In the normal operation mode, the control objective of the system is to minimize the operation costs and maximize the revenues. A rolling-horizon optimization method is used to schedule the outputs of dispatchable DGs based on forecasts. In the self-healing mode, the on-outage portion of the distribution system will be optimally sectionalized into networked self-supplied microgrids (MGs) so as to provide reliable power supply to the maximum loads continuously. The outputs of the dispatchable DGs will be rescheduled accordingly too. In order to take into account the uncertainties of DG outputs and load consumptions, we formulate the problems as a stochastic program. A scenario reduction method is applied to achieve a tradeoff between the accuracy of the solution and the computational burden. A modified IEEE 123-node distribution system is used as a test system. The results of case studies demonstrate the effectiveness of the proposed methodology. C1 [Wang, Zhaoyu] Georgia Inst Technol, Sch Elect & Comp Engn, Atlanta, GA 30332 USA. [Wang, Jianhui] Argonne Natl Lab, Argonne, IL 60439 USA. RP Wang, ZY (reprint author), Georgia Inst Technol, Sch Elect & Comp Engn, Atlanta, GA 30332 USA. EM zhaoyuwang@gatech.edu; jianhui.wang@anl.gov FU U.S. Department of Energy Office of Electricity Delivery and Energy Reliability FX The work of J. Wang was supported by the U.S. Department of Energy Office of Electricity Delivery and Energy Reliability. Paper no. TPWRS-00571-2014. NR 35 TC 17 Z9 18 U1 2 U2 13 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8950 EI 1558-0679 J9 IEEE T POWER SYST JI IEEE Trans. Power Syst. PD NOV PY 2015 VL 30 IS 6 BP 3139 EP 3149 DI 10.1109/TPWRS.2015.2389753 PG 11 WC Engineering, Electrical & Electronic SC Engineering GA CO7VS UT WOS:000359371600031 ER PT J AU Li, ZS Wang, JH Sun, HB Guo, QL AF Li, Zhengshuo Wang, Jianhui Sun, Hongbin Guo, Qinglai TI Transmission Contingency Analysis Based on Integrated Transmission and Distribution Power Flow in Smart Grid SO IEEE TRANSACTIONS ON POWER SYSTEMS LA English DT Article DE Contingency analysis; distribution; global power flow; GPF-based transmission CA; master-slave-splitting; transmission ID SECURITY; SYSTEMS AB In future smart grids, with distribution networks having loops more frequently, current transmission contingency analysis (TCA) which usually neglects the distribution power flow variations after a contingency may leave out severe outages. With more distribution management systems deployed on the distribution side, a new transmission CA method based on global power flow (GPF) analysis which integrates both the transmission and distribution power flow is proposed in this paper (named as GTCA) to address the problem. The definition and new features of GTCA are first introduced. Then, the necessity of GTCA is physically illustrated. Difference in the results of GTCA and TCA is mathematically analyzed. A GPF-embedded algorithm of performing GTCA is then provided. The data exchange process and the performance with communication interruptions are discussed. As multiple contingencies are considered in GTCA, several approaches are proposed and discussed to reduce communication burdens and improve the computational efficiency. Plenty of numerical tests are performed in several systems to verify the theoretical analysis. With theoretical analysis and numerical verification, it is suggested that GTCA should be performed instead of TCA to avoid potential false alarms, especially in the condition that DNs are more frequently looped in the future smart grids. C1 [Li, Zhengshuo; Sun, Hongbin; Guo, Qinglai] Tsinghua Univ, Dept Elect Engn, State Key Lab Power Syst, Beijing 100084, Peoples R China. [Wang, Jianhui] Argonne Natl Lab, Argonne, IL 60439 USA. RP Li, ZS (reprint author), Tsinghua Univ, Dept Elect Engn, State Key Lab Power Syst, Beijing 100084, Peoples R China. EM jianhui.wang@anl.gov; shb@tsinghua.edu.cn FU National Key Basic Research Program of China (973 Program) [2013CB228203]; National Science Foundation of China [51025725, 51321005]; Tsinghua University Initiative Scientific Research Program; U.S. Department of Energy Office of Electricity Delivery and Energy Reliability FX Manuscript received July 23, 2014; revised November 13, 2014; accepted December 10, 2014. Date of publication January 06, 2015; date of current version August 03, 2015. This work was supported in part by the National Key Basic Research Program of China (973 Program) (2013CB228203), the National Science Foundation of China (51025725& 51321005), and the Tsinghua University Initiative Scientific Research Program. The work of J. Wang was supported by the U.S. Department of Energy Office of Electricity Delivery and Energy Reliability. Paper no. TPWRS-01001-2014. NR 32 TC 4 Z9 4 U1 2 U2 10 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8950 EI 1558-0679 J9 IEEE T POWER SYST JI IEEE Trans. Power Syst. PD NOV PY 2015 VL 30 IS 6 BP 3356 EP 3367 DI 10.1109/TPWRS.2014.2381879 PG 12 WC Engineering, Electrical & Electronic SC Engineering GA CO7VS UT WOS:000359371600053 ER PT J AU Park, JS An, J Lee, MH Prinz, FB Lee, W AF Park, Joong Sun An, Jihwan Lee, Min Hwan Prinz, Fritz B. Lee, Wonyoung TI Effects of surface chemistry and microstructure of electrolyte on oxygen reduction kinetics of solid oxide fuel cells SO JOURNAL OF POWER SOURCES LA English DT Article DE Solid oxide fuel cells; Cathode; Oxygen reduction kinetics; Grain boundary ID YTTRIA-STABILIZED ZIRCONIA; ATOMIC LAYER DEPOSITION; GRAIN-BOUNDARY; LOW-TEMPERATURE; HIGH-PERFORMANCE; SEGREGATION; EXCHANGE; YSZ; CONDUCTIVITY; SIMULATIONS AB We report systematic investigation of the surface properties of yttria-stabilized zirconia (YSZ) electrolytes with the control of the grain boundary (GB) density at the surface, and its effects on electrochemical activities. The GB density of thin surface layers deposited on single crystal YSZ substrates is controlled by changing the annealing temperature (750-1450 degrees C). Higher oxygen reduction reactions (ORR) kinetics is observed in samples annealed at lower temperatures. The higher ORR activity is ascribed to the higher GB density at the YSZ surface where 'mobile' oxide ion vacancies are more populated. Meanwhile, oxide ion vacancies concurrently created with yttrium segregation at the surface at the higher annealing temperature are considered inactive to oxygen incorporation reactions. Our results provide additional insight into the interplay between the surface chemistry, microstructures, and electrochemical activity. They potentially provide important guidelines for engineering the electrolyte electrode interfaces of solid oxide fuel cells for higher electrochemical performance. (C) 2015 Elsevier B.V. All rights reserved. C1 [Park, Joong Sun] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Park, Joong Sun; An, Jihwan; Prinz, Fritz B.; Lee, Wonyoung] Stanford Univ, Dept Mech Engn, Stanford, CA 94305 USA. [An, Jihwan] Seoul Natl Univ Sci & Technol, Mfg Syst & Design Engn Program, Seoul, South Korea. [Lee, Min Hwan] Univ Calif Merced, Dept Mech Engn, Merced, CA USA. [Prinz, Fritz B.] Stanford Univ, Dept Mat & Sci Engn, Stanford, CA 94305 USA. [Lee, Wonyoung] Sungkyunkwan Univ, Sch Mech Engn, Suwon 440746, South Korea. RP Lee, W (reprint author), Sungkyunkwan Univ, Sch Mech Engn, Suwon 440746, South Korea. EM leewy@skku.edu FU Basic Science Research Program through the National Research Foundation of Korea (NRF) - Ministry of Science, ICT & Future Planning [NRF-2013R1A1A1059845]; Global Frontier R&D Program on Center for Multiscale Energy System - National Research Foundation under the Ministry of Science, ICT & Future Planning, Korea [NRF-2014M3A6A7074784] FX This research was supported by Basic Science Research Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Science, ICT & Future Planning (Grant No. NRF-2013R1A1A1059845), and by the Global Frontier R&D Program on Center for Multiscale Energy System funded by the National Research Foundation under the Ministry of Science, ICT & Future Planning, Korea (Grant No. NRF-2014M3A6A7074784). NR 43 TC 5 Z9 5 U1 5 U2 64 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD NOV 1 PY 2015 VL 295 BP 74 EP 78 DI 10.1016/j.jpowsour.2015.06.149 PG 5 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA CO7HP UT WOS:000359330500010 ER PT J AU Lu, XC Li, GS Kim, JY Meinhardt, KD Sprenkle, VL AF Lu, Xiaochuan Li, Guosheng Kim, Jin Y. Meinhardt, Kerry D. Sprenkle, Vincent L. TI Enhanced sintering of beta"-Al2O3/YSZ with the sintering aids of TiO2 and MnO2 SO JOURNAL OF POWER SOURCES LA English DT Article DE beta"-Al2O3 solid electrolyte; Boehmite; Sintering aid; Titanium oxide; Manganese oxide ID LITHIA-STABILIZED BETA''-ALUMINA; BETA-ALUMINA ELECTROLYTE; SODIUM-BETA; GRAIN-SIZE; POLYCRYSTALLINE; MICROSTRUCTURE; BATTERY; CELL; CRYSTALLIZATION; COMPOSITES AB beta-Al2O3 has been the dominated choice for the electrolyte materials of sodium batteries because of its high ionic conductivity, excellent stability with the electrode materials, satisfactory mechanical strength, and low material cost. To achieve adequate electrical and mechanical performance, sintering of beta-Al2O3 is typically carried out at temperatures above 1600 degrees C with deliberate efforts on controlling the phase, composition, and microstructure. Here, we reported a simple method to fabricate beta-Al2O3/YSZ electrolyte at relatively lower temperatures. With the starting material of boehmite, single phase of "-Al2O3 (3 can be achieved at as low as 1200 degrees C. It was found that TiO2 was extremely effective as a sintering aid for the densification of beta-Al2O3 and similar behavior was observed with MnO2 for YSZ. With the addition of 2 mol% TiO2 and 5 mol% MnO2, the beta-Al203/YSZ composite was able to be densified at as low as 1400 degrees C with a fine microstructure and good electrical/mechanical performance. This study demonstrated a new approach of synthesis and sintering of beta-Al2O3/YSZ composite, which represented a simple and low-cost method for fabrication of high-performance beta-Al2O3/YSZ electrolyte. Published by Elsevier B.V. C1 [Lu, Xiaochuan; Li, Guosheng; Kim, Jin Y.; Meinhardt, Kerry D.; Sprenkle, Vincent L.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Lu, XC (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM Xiaochuan.Lu@pnnl.gov; Jin.Kim@pnnl.gov FU U.S. Department of Energy's (DOE's) Office of Electricity Delivery & Energy Reliability (OE) [57558]; Department of Energy [DE-AC05-76RL01830] FX This work was supported by the U.S. Department of Energy's (DOE's) Office of Electricity Delivery & Energy Reliability (OE) under Contract No. 57558. We appreciate the useful discussions with Dr. I. Gyuk of the DOE-OE Grid Storage Program. PNNL is a multiprogram laboratory operated by Battelle Memorial Institute for the Department of Energy under Contract DE-AC05-76RL01830. NR 41 TC 4 Z9 4 U1 3 U2 38 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD NOV 1 PY 2015 VL 295 BP 167 EP 174 DI 10.1016/j.jpowsour.2015.06.147 PG 8 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA CO7HP UT WOS:000359330500022 ER PT J AU Lewis, AJ Ren, S Ye, X Kim, P Labbe, N Borole, AP AF Lewis, A. J. Ren, S. Ye, X. Kim, P. Labbe, N. Borole, A. P. TI Hydrogen production from switchgrass via an integrated pyrolysis-microbial electrolysis process SO BIORESOURCE TECHNOLOGY LA English DT Article DE Microbial electrolysis cell (MEC); Integrated pyrolysis-MEC; Bio-oil aqueous phase; Integrated hydrogen production ID BIOELECTROCHEMICAL SYSTEMS; FUEL-CELLS; FERMENTATION; CELLULOSE; VOLTAGE; SURFACE; GAS AB A new approach to hydrogen production using an integrated pyrolysis-microbial electrolysis process is described. The aqueous stream generated during pyrolysis of switchgrass was used as a substrate for hydrogen production in a microbial electrolysis cell, achieving a maximum hydrogen production rate of 4.3 L H-2/L anode-day at a loading of 10 g COD/L-anode-day. Hydrogen yields ranged from 50 +/- 3.2% to 76 +/- 0.5% while anode Coulombic efficiency ranged from 54 +/- 6.5% to 96 +/- 0.21%, respectively. Significant conversion of furfural, organic acids and phenolic molecules was observed under both batch and continuous conditions. The electrical and overall energy efficiency ranged from 149-175% and 48-63%, respectively. The results demonstrate the potential of the pyrolysis-microbial electrolysis process as a sustainable and efficient route for production of renewable hydrogen with significant implications for hydrocarbon production from biomass. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Lewis, A. J.; Ren, S.; Ye, X.; Kim, P.; Labbe, N.; Borole, A. P.] Univ Tennessee, Knoxville, TN 37996 USA. [Borole, A. P.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Kim, P.; Labbe, N.] Univ Tennessee, Ctr Renewable Carbon, Knoxville, TN 37996 USA. [Lewis, A. J.; Borole, A. P.] Univ Tennessee, Bredesen Ctr Interdisciplinary Res & Educ, Knoxville, TN 37996 USA. RP Borole, AP (reprint author), Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. EM borolea@ornl.gov OI Borole, Abhijeet/0000-0001-8423-811X FU U.S. Department of Energy, BioEnergy Technologies Office under the Carbon, Hydrogen and Separations Efficiency for Bio-oil Pathways (CHASE) program; Bredesen Center for Interdisciplinary Research and Education; U.S. Department of Energy [DEAC05-00OR22725] FX Funding from the U.S. Department of Energy, BioEnergy Technologies Office under the Carbon, Hydrogen and Separations Efficiency for Bio-oil Pathways (CHASE) program is acknowledged. A.J.L. was partially supported by the Bredesen Center for Interdisciplinary Research and Education. The manuscript has been co-authored by UT-Battelle, LLC, under Contract No. DEAC05-00OR22725 with the U.S. Department of Energy. NR 35 TC 17 Z9 17 U1 6 U2 51 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0960-8524 EI 1873-2976 J9 BIORESOURCE TECHNOL JI Bioresour. Technol. PD NOV PY 2015 VL 195 BP 231 EP 241 DI 10.1016/j.biortech.2015.06.085 PG 11 WC Agricultural Engineering; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA CO8TL UT WOS:000359444600032 PM 26210530 ER PT J AU Meng, XW Lu, SQ Liu, SX Liu, XY Sui, YR Li, XY Pang, MJ Wang, B Ji, Y Hu, MZ AF Meng, Xiangwei Lu, Shiquan Liu, Shouxiu Liu, Xiaoyan Sui, Yingrui Li, Xiuyan Pang, Mingjun Wang, Biao Ji, Yuan Hu, Michael Z. TI Electrochemical characterization of B-site cation-excess Pr2Ni0.75Cu0.25Ga0.05O4+delta cathode for IT-SOFCS SO CERAMICS INTERNATIONAL LA English DT Article DE Solid oxide fuel cell; Cathode; Electrochemical performance ID OXIDE FUEL-CELLS; COMPOSITE CATHODE; PROTON CONDUCTORS; PEROVSKITE OXIDE; PERFORMANCE; ELECTROLYTE; MEMBRANE AB The B-site cation-excess K2NiF4-type structure oxide, Pr2Ni0.75Cu0.25Ga0.05O4+delta (PNCG) is investigated as a cathode for intermediate-temperature solid oxide fuel cells (IT-SOFCs). XRD result shows that PNCG cathode is chemically compatible with the electrolyte Gd0.1Ce0.9O2-delta (GDC) at 900 degrees C for 5 h. The PNCG material exhibits a semiconductor to metal transition around 425 degrees C. The thermal expansion coefficient (TEC) of the PNCG sample is 12.72 x 10(-6) K-1 between 30 and 850 degrees C in air. The polarization resistance (R-p) of PNCG cathode on GDC electrolyte is 0.105, 0.197 and 0.300 Omega cm(2) at 800, 750, 700 degrees C, respectively. A maximum power density of 371 mW cm(-2) is obtained at 800 degrees C for single-cell with 300 mu m thick GDC electrolyte and PNCG cathode. The results of this study demonstrate that PNCG can be a promising cathode material for IT-SOFCs. (C) 2015 Elsevier Ltd and Techna Group S.r.l. All rights reserved. C1 [Meng, Xiangwei; Lu, Shiquan; Liu, Xiaoyan; Sui, Yingrui; Li, Xiuyan] Jilin Normal Univ, Key Lab Funct Mat Phys & Chem, Minist Educ, Siping 136000, Peoples R China. [Meng, Xiangwei; Liu, Shouxiu; Pang, Mingjun; Wang, Biao; Ji, Yuan] Jilin Univ, Coll Phys, Key Lab Phys & Technol Adv Batteries, Minist Educ, Changchun 130012, Peoples R China. [Hu, Michael Z.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Hu, Michael Z.] Univ Tennessee, Knoxville, TN 37930 USA. RP Lu, SQ (reprint author), Jilin Normal Univ, Key Lab Funct Mat Phys & Chem, Minist Educ, Siping 136000, Peoples R China. EM shiquan_lv@126.com; jiyuan@jlu.edu.cn FU Program for the Development of Science and Technology of Jilin province [20140520103JH]; Twentieth Five-Year Program for Science and Technology of Education Department of Jilin Province [20130447]; Program for the Development of Science and Technology of Siping city [2012036] FX The authors gratefully acknowledge the research funding provided by Program for the Development of Science and Technology of Jilin province (No. 20140520103JH), the Twentieth Five-Year Program for Science and Technology of Education Department of Jilin Province (No. 20130447), Program for the Development of Science and Technology of Siping city (No. 2012036). NR 40 TC 2 Z9 2 U1 4 U2 38 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0272-8842 EI 1873-3956 J9 CERAM INT JI Ceram. Int. PD NOV PY 2015 VL 41 IS 9 BP 12107 EP 12114 DI 10.1016/j.ceramint.2015.06.028 PN B PG 8 WC Materials Science, Ceramics SC Materials Science GA CO4XX UT WOS:000359165300068 ER PT J AU Miller, SM Xiao, X Faber, KT AF Miller, S. M. Xiao, X. Faber, K. T. TI Freeze-cast alumina pore networks: Effects of freezing conditions and dispersion medium SO JOURNAL OF THE EUROPEAN CERAMIC SOCIETY LA English DT Article DE Freeze casting; Porous ceramics; Directional solidification; X-ray computed tomography; Modeling ID DENDRITIC SOLIDIFICATION; ARM SPACINGS; TIP RADIUS; CERAMICS; MICROSTRUCTURE; GROWTH; ICE; CONDUCTIVITY; BIOMATERIALS; SUSPENSIONS AB Alumina ceramics were freeze-cast from water- and camphene-based slurries under varying freezing conditions and examined using X-ray computed tomography (XCT). Pore network characteristics, i.e., porosity, pore size, geometric surface area, and tortuosity, were measured from XCT reconstructions and the data were used to develop a model to predict feature size from processing conditions. Classical solidification theory was used to examine relationships between pore size, temperature gradients, and freezing front velocity. Freezing front velocity was subsequently predicted from casting conditions via the two-phase Stefan problem. Resulting models for water-based samples agreed with solidification-based theories predicting lamellar spacing of binary eutectic alloys, and models for camphene-based samples concurred with those for dendritic growth. Relationships between freezing conditions and geometric surface area were also modeled by considering the inverse relationship between pore size and surface area. Tortuosity was determined to be dependent primarily on the type of dispersion medium. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Miller, S. M.; Faber, K. T.] Northwestern Univ, Robert R McCormick Sch Engn & Appl Sci, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Xiao, X.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Faber, KT (reprint author), CALTECH, MC 138-78, Pasadena, CA 91125 USA. EM kfaber@caltech.edu RI Faber, Katherine/B-6741-2009 FU NASA Office of the Chief Technologist; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357]; MRSEC Program of the Materials Research Center at Northwestern University [NSF DMR-1121262]; MRSEC program at the Materials Research Center [NSF DMR-1121262] FX This work was supported by a NASA Office of the Chief Technologist's Space Technology Research Fellowship and used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. This work also made use of the OMM Facility which receives support from the MRSEC Program (NSF DMR-1121262) of the Materials Research Center at Northwestern University and the EPIC facility (NUANCE Center-Northwestern University), which has received support from the MRSEC program (NSF DMR-1121262) at the Materials Research Center; the International Institute for Nanotechnology (UN); and the State of Illinois, through the UN. The authors would like to thank Dr. Fabian Stolzenburg for the suggestion to use a thermoelectric cooler as a cold plate. NR 55 TC 5 Z9 5 U1 9 U2 46 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0955-2219 EI 1873-619X J9 J EUR CERAM SOC JI J. Eur. Ceram. Soc. PD NOV PY 2015 VL 35 IS 13 BP 3595 EP 3605 DI 10.1016/j.jeurceramsoc.2015.05.012 PG 11 WC Materials Science, Ceramics SC Materials Science GA CO3AS UT WOS:000359029300027 ER PT J AU Alammar, T Hamm, I Wark, M Mudringad, AV AF Alammar, Tarek Hamm, Ines Wark, Michael Mudringad, Anja-Verena TI Low-temperature route to metal titanate perovskite nanoparticles for photocatalytic applications SO APPLIED CATALYSIS B-ENVIRONMENTAL LA English DT Article; Proceedings Paper CT 8th European Meeting on Solar Chemistry and Photocatalysis - Environmental Applications (SPEA) CY 2014 CL Thessaloniki, GREECE DE Titanates; Sonochemical synthesis; Photocatalysis; Hydrogen formation; Nitrogen doping ID IONIC LIQUIDS; HYDROTHERMAL SYNTHESIS; SOL-GEL; SRTIO3; POWDERS; BATIO3; CATIO3; SONOCHEMISTRY; PERFORMANCES; FILMS AB MTiO3 (M = Ca, Sr, Ba) nanoparticles were synthesized by a one-step room-temperature ultrasound synthesis in ionic liquid. The obtained samples are characterized by X-ray diffraction, scanning electron microscopy, nitrogen adsorption, UV-vis diffuse reflectance, Raman and IR spectroscopy and their capability in photocatalytic hydrogen evolution and methylene blue degradation was tested. Powder X-ray diffraction and Raman spectroscopic investigations revealed the products to crystallize in the cubic perovskite structure. SEM observations showed that the obtained CaTiO3 consists of nanospheres, BaTiO3 of raspberry-like shaped particles of 20 nm in diameter. SrTiO3 particles have cubic-like morphology with an edge length varying from 100 to 300 nm. SrTiO3 exhibited the highest catalytic activity for photocatalytic H-2 evolution using only 0.025 wt.% Rh as co-catalyst and for the degradation of methylene blue under UV irradiation. The influence of parameters such as synthesis method, calcination temperature, and doping with nitrogen on the morphology, crystallinity, chemical composition, and photocatalytic acivity of SrTiO3 was studied. Heating the as-prepared SrTiO3 to 700 degrees C for extended time leads to a decrease in surface area and catalytic activity. lonothermal prepared SrTiO3 exhibits a higher activity than sonochemically prepared one without co-catalyst due to a synergistic effect of anatase which is present in small amount as a by-phase. After photodeposition of Rh, however, the activity is lower than that of the sonochemically prepared SrTiO3. Nitrogen-doped SrTiO3 showed photocatalytic acivity under visible light irradiation. (C) 2014 Elsevier B.V. All rights reserved. C1 [Alammar, Tarek; Hamm, Ines; Mudringad, Anja-Verena] Ruhr Univ Bochum, Inorgan Chem 3, D-44801 Bochum, Germany. [Hamm, Ines; Wark, Michael] Ruhr Univ Bochum, Lab Ind Chem, D-44801 Bochum, Germany. [Wark, Michael] Carl von Ossietzky Univ Oldenburg, Inst Chem Tech Chem, D-26129 Oldenburg, Germany. [Mudringad, Anja-Verena] Iowa State Univ, Mat Sci & Engn, Ames, IA 50010 USA. [Mudringad, Anja-Verena] Crit Mat Inst, Ames Lab, Ames, IA 50010 USA. RP Wark, M (reprint author), Carl von Ossietzky Univ Oldenburg, Inst Chem Tech Chem, Carl von Ossietzlcy Str 9-11, D-26129 Oldenburg, Germany. EM michael.wark@uni-oldenburg.de; mudring@iastate.edu OI Mudring, Anja/0000-0002-2800-1684 FU German Science Foundation (DFG) [WA 1116/23-1]; DFG Cluster of Excellence RESOLV at the Ruhr-University Bochum, Germany [EXC 1069]; Energy Innovation Hub - U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office; Iowa State University; Critical Materials Institute FX Financial support by the German Science Foundation (DFG) under the project number WA 1116/23-1 and within the DFG Cluster of Excellence RESOLV (EXC 1069) at the Ruhr-University Bochum, Germany, is gratefully acknowledged. We thank Prof. Dr. M. Muhler (Laboratory of Industrial Chemistry, Ruhr-University Bochum, Germany) for his continuous support. This work was supported in part the Critical Materials Institute, an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office and Iowa State University. NR 47 TC 6 Z9 6 U1 25 U2 202 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0926-3373 EI 1873-3883 J9 APPL CATAL B-ENVIRON JI Appl. Catal. B-Environ. PD NOV PY 2015 VL 178 SI SI BP 20 EP 28 DI 10.1016/j.apcatb.2014.11.010 PG 9 WC Chemistry, Physical; Engineering, Environmental; Engineering, Chemical SC Chemistry; Engineering GA CN0II UT WOS:000358096900004 ER PT J AU Colak, K Asa, E Bojarski, M Czarkowski, D Onar, OC AF Colak, Kerim Asa, Erdem Bojarski, Mariusz Czarkowski, Dariusz Onar, Omer C. TI A Novel Phase-Shift Control of Semibridgeless Active Rectifier for Wireless Power Transfer SO IEEE TRANSACTIONS ON POWER ELECTRONICS LA English DT Article DE Pickup circuit; phase shift; receiver control; resonant converter; semibridgeless active rectifier (S-BAR); wireless energy ID TRANSFER SYSTEMS; CHARGING PLATFORM; IPT SYSTEMS; TRANSMISSION; PICKUP; DESIGN; COIL AB A novel phase-shift control of a semibridgeless active rectifier (S-BAR) is investigated in order to utilize the S-BAR in wireless energy transfer applications. The standard receiver-side rectifier topology is developed by replacing rectifier lower diodes with synchronous switches controlled by a phase-shifted PWM signal. Theoretical and simulation results showthat with the proposed control technique, the output quantities can be regulated without communication between the receiver and transmitter. To confirm the performance of the proposed converter and control, experimental results are provided using 8-, 15-, and 23-cm air gap coreless transformer which has dimension of 76 cm x 76 cm, with 120-V input and the output power range of 0 to 1kW with a maximum efficiency of 94.4%. C1 [Colak, Kerim; Asa, Erdem; Bojarski, Mariusz; Czarkowski, Dariusz] NYU, Polytech Sch Engn, Brooklyn, NY 11201 USA. [Onar, Omer C.] Oak Ridge Natl Lab, Power Elect & Elect Machinery Grp, Natl Transportat Res Ctr, Oak Ridge, TN 37831 USA. RP Colak, K (reprint author), Istanbul Ulasim AS, TR-34220 Esenler, Turkey. EM kc1353@nyu.edu; ea1145@nyu.edu; mb4496@nyu.edu; dc1677@nyu.edu; onaroc@ornl.gov RI Nunes, Joao Ricardo/I-8440-2016 NR 27 TC 13 Z9 14 U1 0 U2 26 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8993 EI 1941-0107 J9 IEEE T POWER ELECTR JI IEEE Trans. Power Electron. PD NOV PY 2015 VL 30 IS 11 BP 6288 EP 6297 DI 10.1109/TPEL.2015.2430832 PG 10 WC Engineering, Electrical & Electronic SC Engineering GA CM8LA UT WOS:000357951200030 ER PT J AU Yuan, JY Wang, DL Cheriyadat, AM AF Yuan, Jiangye Wang, Deliang Cheriyadat, Anil M. TI Factorization-Based Texture Segmentation SO IEEE TRANSACTIONS ON IMAGE PROCESSING LA English DT Article DE Matrix factorization; texture segmentation; spectral histogram ID NONNEGATIVE MATRIX FACTORIZATION; LOCAL SPECTRAL HISTOGRAMS; IMAGE SEGMENTATION; MODEL; CLASSIFICATION; SHIFT AB This paper introduces a factorization-based approach that efficiently segments textured images. We use local spectral histograms as features, and construct an M x N feature matrix using M-dimensional feature vectors in an N-pixel image. Based on the observation that each feature can be approximated by a linear combination of several representative features, we factor the feature matrix into two matrices-one consisting of the representative features and the other containing the weights of representative features at each pixel used for linear combination. The factorization method is based on singular value decomposition and nonnegative matrix factorization. The method uses local spectral histograms to discriminate region appearances in a computationally efficient way and at the same time accurately localizes region boundaries. The experiments conducted on public segmentation data sets show the promise of this simple yet powerful approach. C1 [Yuan, Jiangye; Cheriyadat, Anil M.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Wang, Deliang] Ohio State Univ, Dept Comp Sci & Engn, Ctr Cognit & Brain Sci, Columbus, OH 43210 USA. RP Yuan, JY (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM yuanj@ornl.gov; dwang@cse.ohio-state.edu; cheriyadatam@ornl.gov FU U.S. Department of Energy [DE-AC05-00OR22725]; United States Government FX At least one or more of the authors of this manuscript are employees of UT-Battelle, LLC, under contract DE-AC05-00OR22725 with the U.S. Department of Energy. Accordingly, the United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The authors would like to thank Dr. Alper Yilmaz for valuable suggestions. NR 43 TC 4 Z9 4 U1 2 U2 14 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1057-7149 EI 1941-0042 J9 IEEE T IMAGE PROCESS JI IEEE Trans. Image Process. PD NOV PY 2015 VL 24 IS 11 BP 3488 EP 3497 DI 10.1109/TIP.2015.2446948 PG 10 WC Computer Science, Artificial Intelligence; Engineering, Electrical & Electronic SC Computer Science; Engineering GA CM6IZ UT WOS:000357793200009 PM 26087494 ER PT J AU Hemme, CL Tu, QC Shi, Z Qin, YJ Gao, WM Deng, Y Van Nostrand, JD Wu, LY He, ZL Chain, PSG Tringe, SG Fields, MW Rubin, EM Tiedje, JM Hazen, TC Arkin, AP Zhou, JZ AF Hemme, Christopher L. Tu, Qichao Shi, Zhou Qin, Yujia Gao, Weimin Deng, Ye Van Nostrand, Joy D. Wu, Liyou He, Zhili Chain, Patrick S. G. Tringe, Susannah G. Fields, Matthew W. Rubin, Edward M. Tiedje, James M. Hazen, Terry C. Arkin, Adam P. Zhou, Jizhong TI Comparative metagenomics reveals impact of contaminants on groundwater microbiomes SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE metagenomics; bioremediation; groundwater microbiology ID IN-SITU BIOREMEDIATION; COMMUNITY STRUCTURE; ANALYSIS SYSTEM; GENE-TRANSFER; HIGH-NITRATE; URANIUM; SUBSURFACE; GENOMES; AQUIFER; WATER AB To understand patterns of geochemical cycling in pristine versus contaminated groundwater ecosystems, pristine shallow groundwater (FW301) and contaminated groundwater (FW106) samples from the Oak Ridge Integrated Field Research Center (OR-IFRC) were sequenced and compared to each other to determine phylogenetic and metabolic difference between the communities. Proteobacteria (e.g., Burkholderia, Pseudomonas) are the most abundant lineages in the pristine community, though a significant proportion (>55%) of the community is composed of poorly characterized low abundance (individually <1%) lineages. The phylogenetic diversity of the pristine community contributed to a broader diversity of metabolic networks than the contaminated community. In addition, the pristine community encodes redundant and mostly complete geochemical cycles distributed over multiple lineages and appears capable of a wide range of metabolic activities. In contrast, many geochemical cycles in the contaminated community appear truncated or minimized due to decreased biodiversity and dominance by Rhodanobacter populations capable of surviving the combination of stresses at the site. These results indicate that the pristine site contains more robust and encodes more functional redundancy than the stressed community, which contributes to more efficient nutrient cycling and adaptability than the stressed community. C1 [Hemme, Christopher L.; Tu, Qichao; Shi, Zhou; Qin, Yujia; Deng, Ye; Van Nostrand, Joy D.; Wu, Liyou; He, Zhili; Zhou, Jizhong] Univ Oklahoma, Dept Microbiol & Plant Biol, Inst Environm Genom, Norman, OK 73019 USA. [Gao, Weimin] Arizona State Univ, Biodesign Inst, Tempe, AZ USA. [Deng, Ye] Chinese Acad Sci, Res Ctr Ecoenvironm Sci, CAS Key Lab Environm Biotechnol, Beijing, Peoples R China. [Chain, Patrick S. G.] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM USA. [Tringe, Susannah G.; Rubin, Edward M.] US DOE, Joint Genome Inst, Walnut Creek, CA USA. [Fields, Matthew W.] Montana State Univ, Dept Microbiol, Bozeman, MT 59717 USA. [Tiedje, James M.] Michigan State Univ, Ctr Microbial Ecol, E Lansing, MI 48824 USA. [Hazen, Terry C.] Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN USA. [Hazen, Terry C.] Univ Tennessee, Dept Earth & Planetary Sci, Knoxville, TN USA. [Hazen, Terry C.] Univ Tennessee, Dept Microbiol, Knoxville, TN 37996 USA. [Hazen, Terry C.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. [Arkin, Adam P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Bioengn, Berkeley, CA 94720 USA. [Zhou, Jizhong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Zhou, Jizhong] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China. RP Zhou, JZ (reprint author), Univ Oklahoma, Dept Microbiol & Plant Biol, Inst Environm Genom, Norman, OK 73019 USA. EM hemmecl@uri.edu; jzhou@ou.edu RI Van Nostrand, Joy/F-1740-2016; Arkin, Adam/A-6751-2008; Hazen, Terry/C-1076-2012; Gao, Weimin/J-1795-2014; OI Van Nostrand, Joy/0000-0001-9548-6450; Arkin, Adam/0000-0002-4999-2931; Hazen, Terry/0000-0002-2536-9993; Gao, Weimin/0000-0002-6758-9775; ?, ?/0000-0002-7584-0632; Chain, Patrick/0000-0003-3949-3634 FU Office of Science, Office of Biological and Environmental Research, of the U. S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy [DE-FG02-07ER64398]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Office of the Vice President for Research; College of Arts and Sciences; Department of Microbiology and Plant Biology at the University of Oklahoma FX This work conducted by ENIGMA- Ecosystems and Networks Integrated with Genes and Molecular Assemblies was supported by the Office of Science, Office of Biological and Environmental Research, of the U. S. Department of Energy under Contract No. DE-AC02-05CH11231, U.S. Department of Energy Grant DE-FG02-07ER64398. The work conducted by the U.S. Department of Energy joint Genome Institute is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We also wish to acknowledge financial support provided by the Office of the Vice President for Research, the College of Arts and Sciences, and the Department of Microbiology and Plant Biology at the University of Oklahoma. NR 43 TC 4 Z9 4 U1 8 U2 31 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD OCT 31 PY 2015 VL 6 AR 1205 DI 10.3389/fmicb.2015.01205 PG 12 WC Microbiology SC Microbiology GA CV4NA UT WOS:000364242600002 PM 26583008 ER PT J AU Weigand, M Bredeweg, TA Couture, A Gobel Heftrich, T Jandel, M Kappeler, F Lederer, C Kivel, N Korschinek, G Krticka, M O'Donnell, JM Ostermoller, J Plag, R Reifarth, R Schumann, D Ullmann, JL Wallner, A AF Weigand, M. Bredeweg, T. A. Couture, A. Goebel, K. Heftrich, T. Jandel, M. Kaeppeler, F. Lederer, C. Kivel, N. Korschinek, G. Krticka, M. O'Donnell, J. M. Ostermoeller, J. Plag, R. Reifarth, R. Schumann, D. Ullmann, J. L. Wallner, A. TI Ni-63(n,gamma) cross sections measured with DANCE SO PHYSICAL REVIEW C LA English DT Article ID GIANT BRANCH STARS; ASTROPHYSICAL REACTION-RATES; NEUTRON-CAPTURE; S-PROCESS; MASSIVE STARS; SOLAR-SYSTEM; NUCLEOSYNTHESIS; EVOLUTION AB The neutron capture cross section of the s-process branch nucleus Ni-63 affects the abundances of other nuclei in its region, especially (CU)-C-63 and Zn-64. In order to determine the energy-dependent neutron capture cross section in the astrophysical energy region, an experiment at the Los Alamos National Laboratory has been performed using the calorimetric 4 pi BaF2 array DANCE. The (n,gamma) cross section of Ni-63 has been determined relative to the well-known Au-197 standard with uncertainties below 15%. Various Ni-63 resonances have been identified based on the Q value. Furthermore, the s-process sensitivity of the new values was analyzed with the new network calculation tool NETZ. C1 [Weigand, M.; Goebel, K.; Heftrich, T.; Lederer, C.; Ostermoeller, J.; Plag, R.; Reifarth, R.] Goethe Univ Frankfurt, D-60438 Frankfurt, Germany. [Bredeweg, T. A.; Couture, A.; Jandel, M.; O'Donnell, J. M.; Ullmann, J. L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Kaeppeler, F.] Karlsruhe Inst Technol, Inst Kernphys, D-76021 Karlsruhe, Germany. [Kivel, N.; Schumann, D.] Paul Scherrer Inst, Villigen, Switzerland. [Korschinek, G.] Tech Univ Munich, Munich, Germany. [Krticka, M.] Charles Univ Prague, Fac Math & Phys, CZ-18000 Prague 8, Czech Republic. [Wallner, A.] Australian Natl Univ, Dept Nucl Phys, Canberra, ACT 2601, Australia. RP Weigand, M (reprint author), Goethe Univ Frankfurt, Max von Laue Str 1, D-60438 Frankfurt, Germany. EM m.weigand@gsi.de RI Weigand, Mario/R-6517-2016 OI Weigand, Mario/0000-0003-1406-7241 FU Czech Science Foundation [13-07117S]; HIC for FAIR; Helmholtz Young Investigator Project [VH-NG-327]; Nuclear Astrophysics Virtual Institute FX This project was supported through the Nuclear Astrophysics Virtual Institute, the Helmholtz Young Investigator Project (No. VH-NG-327), and HIC for FAIR. M.K. acknowledges support from the Czech Science Foundation (Grant No. 13-07117S). NR 35 TC 1 Z9 1 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD OCT 30 PY 2015 VL 92 IS 4 AR 045810 DI 10.1103/PhysRevC.92.045810 PG 10 WC Physics, Nuclear SC Physics GA CU8KU UT WOS:000363792100005 ER PT J AU Yang, S Oksenberg, N Takayama, S Heo, SJ Poliakov, A Ahituv, N Dubchak, I Boffelli, D AF Yang, Song Oksenberg, Nir Takayama, Sachiko Heo, Seok-Jin Poliakov, Alexander Ahituv, Nadav Dubchak, Inna Boffelli, Dario TI Functionally conserved enhancers with divergent sequences in distant vertebrates SO BMC GENOMICS LA English DT Article ID COMPARATIVE GENOMICS; TRANSCRIPTION FACTORS; REGULATORY ELEMENTS; MAMMALIAN GENOMES; GENE-REGULATION; CONSTRAINT; ZEBRAFISH; EVOLUTION; TOOLS; CIS AB Background: To examine the contributions of sequence and function conservation in the evolution of enhancers, we systematically identified enhancers whose sequences are not conserved among distant groups of vertebrate species, but have homologous function and are likely to be derived from a common ancestral sequence. Our approach combined comparative genomics and epigenomics to identify potential enhancer sequences in the genomes of three groups of distantly related vertebrate species. Results: We searched for sequences that were conserved within groups of closely related species but not between groups of more distant species, and were associated with an epigenetic mark of enhancer activity. To facilitate inferring orthology between non-conserved sequences, we limited our search to introns whose orthology could be unambiguously established by mapping the bracketing exons. We show that a subset of these non-conserved but syntenic sequences from the mouse and zebrafish genomes have homologous functions in a zebrafish transgenic enhancer assay. The conserved expression patterns driven by these enhancers are probably associated with short transcription factor-binding motifs present in the divergent sequences. Conclusions: We have identified numerous potential enhancers with divergent sequences but a conserved function. These results indicate that selection on function, rather than sequence, may be a common mode of enhancer evolution; evidence for selection at the sequence level is not a necessary criterion to define a gene regulatory C1 [Yang, Song; Dubchak, Inna] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Genom Div, Berkeley, CA 94720 USA. [Oksenberg, Nir; Ahituv, Nadav] Univ Calif San Francisco, Dept Bioengn & Therapeut Sci, San Francisco, CA 94158 USA. [Oksenberg, Nir; Ahituv, Nadav] Univ Calif San Francisco, Inst Human Genet, San Francisco, CA 94158 USA. [Takayama, Sachiko; Heo, Seok-Jin; Boffelli, Dario] Childrens Hosp Oakland, Res Inst, Oakland, CA 94609 USA. [Poliakov, Alexander; Dubchak, Inna] US DOE, Joint Genome Inst, Walnut Creek, CA 94598 USA. RP Dubchak, I (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Genom Div, Berkeley, CA 94720 USA. EM ildubchak@lbl.gov; dboffelli@chori.org OI Ahituv, Nadav/0000-0002-7434-8144 FU National Institutes of Health [R01 HL091495]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; NHGRI [R01HG005058, 1R01HG006768]; NICHD [R01HD059862]; NIGMS [GM61390]; NIDDK [1R01DK090382]; NINDS [1R01NS079231] FX We are thankful to Adam Siepel and Melissa Jane Hubisz for their help with the PhastCons analysis, to Ivan Ovcharenko and Leila Taher for numerous helpful discussions. ID and DB were supported by National Institutes of Health (R01 HL091495). The work conducted by the U.S. Department of Energy Joint Genome Institute is supported by the Office of Science of the U.S. Department of Energy under Contract No. (DE-AC02-05CH11231). This work was also supported by NHGRI award R01HG005058 (NA). NA is also supported in part by NHGRI award 1R01HG006768, NICHD award R01HD059862, NIGMS award number GM61390, NIDDK award number 1R01DK090382 and NINDS award number 1R01NS079231. The authors declare no conflict of interest. NR 44 TC 0 Z9 0 U1 1 U2 5 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2164 J9 BMC GENOMICS JI BMC Genomics PD OCT 30 PY 2015 VL 16 AR 882 DI 10.1186/s12864-015-2070-7 PG 13 WC Biotechnology & Applied Microbiology; Genetics & Heredity SC Biotechnology & Applied Microbiology; Genetics & Heredity GA CW8WB UT WOS:000365279000001 PM 26519295 ER PT J AU Bacik, JP Klesmith, JR Whitehead, TA Jarboe, LR Unkefer, CJ Mark, BL Michalczyk, R AF Bacik, John-Paul Klesmith, Justin R. Whitehead, Timothy A. Jarboe, Laura R. Unkefer, Clifford J. Mark, Brian L. Michalczyk, Ryszard TI Producing Glucose 6-Phosphate from Cellulosic Biomass STRUCTURAL INSIGHTS INTO LEVOGLUCOSAN BIOCONVERSION SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article ID LIGNOCELLULOSIC BIOMASS; PSEUDOMONAS-AERUGINOSA; ESCHERICHIA-COLI; ORGANIC-MATTER; KINASE; DYNAMICS; TRIS; CRYSTALLOGRAPHY; PURIFICATION; SPECIFICITY AB The most abundant carbohydrate product of cellulosic biomass pyrolysis is the anhydrosugar levoglucosan (1,6-anhydro-beta-D-glucopyranose), which can be converted to glucose 6-phosphate by levoglucosan kinase (LGK). In addition to the canonical kinase phosphotransfer reaction, the conversion requires cleavage of the 1,6-anhydro ring to allow ATP-dependent phosphorylation of the sugar O6 atom. Using x-ray crystallography, we show that LGK binds two magnesium ions in the active site that are additionally coordinated with the nucleotide and water molecules to result in ideal octahedral coordination. To further verify the metal binding sites, we co-crystallized LGK in the presence of manganese instead of magnesium and solved the structure de novo using the anomalous signal from four manganese atoms in the dimeric structure. The first metal is required for catalysis, whereas our work suggests that the second is either required or significantly promotes the catalytic rate. Although the enzyme binds its sugar substrate in a similar orientation to the structurally related 1,6-anhydro-N-acetylmuramic acid kinase (AnmK), it forms markedly fewer bonding interactions with the substrate. In this orientation, the sugar is in an optimal position to couple phosphorylation with ring cleavage. We also observed a second alternate binding orientation for levoglucosan, and in these structures, ADP was found to bind with lower affinity. These combined observations provide an explanation for the high Km of LGK for levoglucosan. Greater knowledge of the factors that contribute to the catalytic efficiency of LGK can be used to improve applications of this enzyme for levoglucosan-derived biofuel production. C1 [Bacik, John-Paul; Unkefer, Clifford J.; Michalczyk, Ryszard] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA. [Klesmith, Justin R.] Michigan State Univ, Dept Biochem & Mol Biol, E Lansing, MI 48824 USA. [Whitehead, Timothy A.] Michigan State Univ, Dept Chem Engn & Mat Sci, E Lansing, MI 48824 USA. [Whitehead, Timothy A.] Michigan State Univ, Dept Biosyst & Agr Engn, E Lansing, MI 48824 USA. [Jarboe, Laura R.] Iowa State Univ, Dept Chem & Biol Engn, Ames, IA 50011 USA. [Mark, Brian L.] Univ Manitoba, Dept Microbiol, Winnipeg, MB R3T 2N2, Canada. RP Bacik, JP (reprint author), Los Alamos Natl Lab, Biosci Div, TA03,Bldg 4200,MS T007, Los Alamos, NM 87545 USA. EM jbacik@lanl.gov OI Klesmith, Justin/0000-0003-2908-9355; Michalczyk, Ryszard/0000-0001-8839-6473 FU Natural Sciences and Engineering Research Council of Canada (NSERC); National Research Council; Canadian Institutes of Health Research; University of Saskatchewan; U. S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]; DOE Office of Biological and Environmental Research; National Institutes of Health, NIGMS [P41GM103393] FX We thank Shaun Labiuk, Pavel Afonine, and the Canadian Light Source as well as the staff at the SLAC National Accelerator Laboratory for assistance in data collection and processing. We thank the Los Alamos National Laboratory Principal Associate Directorate for Science, Technology and Engineering for institutional investment in key equipment that enabled NMR measurements reported here. The Canadian Light Source is supported by Natural Sciences and Engineering Research Council of Canada (NSERC), the National Research Council, Canadian Institutes of Health Research, and the University of Saskatchewan. Use of the Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, is supported by the U. S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences under Contract DE-AC02-76SF00515. The Stanford Synchrotron Radiation Lightsource Structural Molecular Biology Program is supported by the DOE Office of Biological and Environmental Research, and by the National Institutes of Health, NIGMS (including Grant P41GM103393). We also thank Brian Broom-Peltz for technical assistance and Dr. Virginia A. Unkefer for help with editing the manuscript. NR 52 TC 2 Z9 2 U1 2 U2 13 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD OCT 30 PY 2015 VL 290 IS 44 BP 26638 EP 26648 DI 10.1074/jbc.M115.674614 PG 11 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CW2AO UT WOS:000364793600029 PM 26354439 ER PT J AU Cai, YH Bhuiya, MW Shanklin, J Liu, CJ AF Cai, Yuanheng Bhuiya, Mohammad-Wadud Shanklin, John Liu, Chang-Jun TI Engineering a Monolignol 4-O-Methyltransferase with High Selectivity for the Condensed Lignin Precursor Coniferyl Alcohol SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article ID ITERATIVE SATURATION MUTAGENESIS; ACID O-METHYLTRANSFERASE; DIRECTED EVOLUTION; SWISS-MODEL; STRUCTURAL BASIS; BIOSYNTHESIS; ENZYMES; EFFICIENCY; POPLARS AB Lignin, a rigid biopolymer in plant cell walls, is derived from the oxidative polymerization of three monolignols. The composition of monolignol monomers dictates the degree of lignin condensation, reactivity, and thus the degradability of plant cell walls. Guaiacyl lignin is regarded as the condensed structural unit. Polymerization of lignin is initiated through the deprotonation of the para-hydroxyl group of monolignols. Therefore, preferentially modifying the para-hydroxyl of a specific monolignol to deprive its dehydrogenation propensity would disturb the formation of particular lignin subunits. Here, we test the hypothesis that specific remodeling the active site of a monolignol 4-O-methyltransferase would create an enzyme that specifically methylates the condensed guaiacyl lignin precursor coniferyl alcohol. Combining crystal structural information with combinatorial active site saturation mutagenesis and starting with the engineered promiscuous enzyme, MOMT5(T133L/E165I/F175I/F166W/H169F), we incrementally remodeled its substrate binding pocket by the addition of four substitutions, i.e. M26H, S30R, V33S, and T319M, yielding a mutant enzyme capable of discriminately etherifying the para-hydroxyl of coniferyl alcohol even in the presence of excess sinapyl alcohol. The engineered enzyme variant has a substantially reduced substrate binding pocket that imposes a clear steric hindrance thereby excluding bulkier lignin precursors. The resulting enzyme variant represents an excellent candidate for modulating lignin composition and/or structure in planta. C1 [Cai, Yuanheng; Bhuiya, Mohammad-Wadud; Shanklin, John; Liu, Chang-Jun] Brookhaven Natl Lab, Biol Environm & Climate Sci Dept, Upton, NY 11973 USA. RP Liu, CJ (reprint author), Brookhaven Natl Lab, Biol Environm & Climate Sci Dept, Upton, NY 11973 USA. EM cliu@bnl.gov FU Office of Basic Energy Sciences, United States Department of Energy [DEAC0298CH10886] FX We thank Dr. Eran Pichersky, University of Michigan, for sharing the initial parental enzyme C. breweri IEMT clone. The use of the x-ray beamline X29 and X25 of the National Synchrotron Light source in Brookhaven National Laboratory was supported by the Office of Basic Energy Sciences, United States Department of Energy under Contract DEAC0298CH10886. NR 36 TC 1 Z9 1 U1 6 U2 20 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD OCT 30 PY 2015 VL 290 IS 44 BP 26715 EP 26724 DI 10.1074/jbc.M115.684217 PG 10 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CW2AO UT WOS:000364793600034 PM 26378240 ER PT J AU Song, PA Xu, ZG Lu, Y Guo, QP AF Song, Ping'an Xu, Zhiguang Lu, Yuan Guo, Qipeng TI Bioinspired strategy for tuning thermal stability of PVA via hydrogen-bond crosslink SO COMPOSITES SCIENCE AND TECHNOLOGY LA English DT Article DE Polymers; Thermal properties; Infrared (IR) spectroscopy ID POLY(VINYL ALCOHOL) NANOCOMPOSITES; FLAME-RETARDANT; DEGRADATION; COMPOSITES; FLAMMABILITY; GRAPHENE; POLYMER AB Although many approaches have been employed to enhance thermal stability of PVA, developing a facile and effective strategy remains highly attractive. Herein, we demonstrate a highly effective approach to strikingly improve thermal stability of PVA by selecting the types of multiamines molecules to tune the hydrogen-bond crosslink density. Results show that only adding 0.5 wt% of 2,4,5,6-tetraaminopyrimidine can make the initial degradation temperature (T-i) and maximum degradation temperature (T-max) of PVA increase by similar to 55 degrees C and 98 degrees C due to the formation of 3D physically H-bond crosslinked network, resulting in superior thermal stability property to those of PVA nanocomposites. Moreover, thermal stability strongly depends on the H-bond crosslink density, and T-i and T-max basically obey the linear hydrogen-bond relations despite some deviations. This work opens up a novel biological methodology for creating thermally stable polymeric materials. (C) 2015 Published by Elsevier Ltd. C1 [Song, Ping'an] Zhejiang A&F Univ, Dept Mat, Coll Engn, Hangzhou 311300, Zhejiang, Peoples R China. [Song, Ping'an; Xu, Zhiguang; Guo, Qipeng] Deakin Univ, Inst Frontier Mat, Polymers Res Grp, Geelong, Vic 3220, Australia. [Lu, Yuan] Oak Ridge Natl Lab, Oak Ridge, TN 37830 USA. RP Song, PA (reprint author), Zhejiang A&F Univ, Dept Mat, Coll Engn, Hangzhou 311300, Zhejiang, Peoples R China. EM songyu19800919@163.com; qguo@deakin.edu.au RI Guo, Qipeng/A-8140-2013 OI Guo, Qipeng/0000-0001-7113-651X FU Alfred Deakin Postdoctoral Research Fellowship Scheme; National Science Foundation of China [51303162]; Non-profit Project of Science and Technology Agency of Zhejiang Province of China [2013C32073, 2012C22077] FX P.S. was supported by the Alfred Deakin Postdoctoral Research Fellowship Scheme and by the National Science Foundation of China (Grant No. 51303162) and the Non-profit Project of Science and Technology Agency of Zhejiang Province of China (2013C32073 and 2012C22077). NR 29 TC 6 Z9 6 U1 8 U2 29 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0266-3538 EI 1879-1050 J9 COMPOS SCI TECHNOL JI Compos. Sci. Technol. PD OCT 30 PY 2015 VL 118 BP 16 EP 22 DI 10.1016/j.compscitech.2015.08.006 PG 7 WC Materials Science, Composites SC Materials Science GA CV4RL UT WOS:000364254100003 ER PT J AU Guo, P Danilkin, IV Szczepaniak, AP AF Guo, Peng Danilkin, I. V. Szczepaniak, Adam P. TI Dispersive approaches for three-particle final state interaction SO EUROPEAN PHYSICAL JOURNAL A LA English DT Article ID TREIMAN-TYPE EQUATIONS; PION-PION SCATTERING; PERTURBATION-THEORY; 3-BODY DECAY; FIELD THEORY; UNITARITY; AMPLITUDES; MODEL; ANALYTICITY; PARTICLES AB In this work, we present different representations of the Khuri-Treiman equation and discuss advantages and disadvantages of each representation. In particular we focus on the inversion technique proposed by Pasquier, which, even though developed a long time ago, has not been used in modern analyses of data on three particle decays. We apply the method to a toy model and compare the sensitivity of this and alternative solution methods to the left-hand cut contribution. We also discuss the meaning and applicability of Watson's theorem when three particles in final states are involved. C1 [Guo, Peng; Szczepaniak, Adam P.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Guo, Peng; Szczepaniak, Adam P.] Indiana Univ, Ctr Explorat Energy & Matter, Bloomington, IN 47408 USA. [Guo, Peng; Danilkin, I. V.; Szczepaniak, Adam P.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. RP Guo, P (reprint author), Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. EM pguo@jlab.org FU U.S. Department of Energy [DE-FG0287ER40365, DE-AC05-06OR23177]; Indiana University Collaborative Research Grant; U.S. National Science Foundation [PHY-1205019] FX We thank Michael R. Pennington for many useful discussions, we also thank Andrew W. Jackura for the final proof reading of this manuscript. This research was supported in part by the U.S. Department of Energy under Grant No. DE-FG0287ER40365, the Indiana University Collaborative Research Grant and U.S. National Science Foundation under grant PHY-1205019. We also acknowledge support from U.S. Department of Energy contract DE-AC05-06OR23177, under which Jefferson Science Associates, LLC, manages and operates Jefferson Laboratory. NR 51 TC 2 Z9 2 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6001 EI 1434-601X J9 EUR PHYS J A JI Eur. Phys. J. A PD OCT 30 PY 2015 VL 51 IS 11 BP 1 EP 10 AR 135 DI 10.1140/epja/i2015-15135-7 PG 10 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA CV8EO UT WOS:000364513200001 ER PT J AU Ruszkowski, M Nocek, B Forlani, G Dauter, Z AF Ruszkowski, Milosz Nocek, Boguslaw Forlani, Giuseppe Dauter, Zbigniew TI The structure of Medicago truncatula delta(1)-pyrroline-5-carboxylate reductase provides new insights into regulation of proline biosynthesis in plants SO FRONTIERS IN PLANT SCIENCE LA English DT Article DE protein structure; decamer; coenzyme preference; salt stress; abiotic stress; P5C reductase; P5CR ID OSMOTIC-STRESS; PYRROLINE-5-CARBOXYLATE REDUCTASE; STREPTOCOCCUS-PYOGENES; ARABIDOPSIS-THALIANA; ENHANCED TOLERANCE; CRYSTAL-STRUCTURES; SYNTHETASE GENE; P5C REDUCTASE; ROOT-NODULES; ACCUMULATION AB The two pathways for proline biosynthesis in higher plants share the last step, the conversion of delta(1)-pyrroline-5-carboxylate (P5C) to L-proline, which is catalyzed by P5C reductase (P5OR, EC 1.5.1.2) with the use of NAD(P)H as a coenzyme. There is increasing amount of evidence to suggest a complex regulation of P5CR activity at the post-translational level, yet the molecular basis of these mechanisms is unknown. Here we report the three-dimensional structure of the P5CR enzyme from the model legume Medicago truncatula (Mt). The crystal structures of unliganded MtP5CR decamer, and its complexes with the products NAD+, NADP, and L-proline were refined using x-ray diffraction data (at 1.7, 1.85, 1.95, and 2.1 angstrom resolution, respectively). Based on the presented structural data, the coenzyme preference for NADPH over NADH was explained, and NADPH is suggested to be the only coenzyme used by MtP5CR in vivo. Furthermore, the insensitivity of MtP5CR to feed-back inhibition by proline, revealed by enzymatic analysis, was correlated with structural features. Additionally, a mechanism for the modulation of enzyme activity by chloride anions is discussed, as well as the rationale for the possible development of effective enzyme inhibitors. C1 [Ruszkowski, Milosz; Dauter, Zbigniew] NCI, Synchrotron Radiat Res Sect, Macromol Crystallog Lab, Argonne, IL 60439 USA. [Nocek, Boguslaw] Argonne Natl Lab, Biosci Div, Struct Biol Ctr, Argonne, IL 60439 USA. [Forlani, Giuseppe] Univ Ferrara, Dept Life Sci & Biotechnol, I-44100 Ferrara, Italy. RP Ruszkowski, M (reprint author), NCI, Synchrotron Radiat Res Sect, Macromol Crystallog Lab, Argonne, IL 60439 USA. EM mruszkowski@anl.gov RI Forlani, Giuseppe/B-7869-2009 OI Forlani, Giuseppe/0000-0003-2598-5718 FU NCI, Center for Cancer Research; U.S. Department of Energy, Office of Biological and Environmental Research [DE-AC02-06CH11357] FX This project was supported in part by the Intramural Research Program of the NCI, Center for Cancer Research. Structural results shown in this report are derived from work performed at Argonne National Laboratory, Structural Biology Center at the Advanced Photon Source. Argonne is operated by UChicago Argonne, LLC, for the U.S. Department of Energy, Office of Biological and Environmental Research under contract DE-AC02-06CH11357. NR 70 TC 3 Z9 3 U1 3 U2 15 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. PD OCT 30 PY 2015 VL 6 AR 869 DI 10.3389/fpls.2015.00869 PG 17 WC Plant Sciences SC Plant Sciences GA CV8ZD UT WOS:000364576000001 PM 26579138 ER PT J AU Zheng, LE Rutqvist, J Birkholzer, JT Liu, HH AF Zheng, Liange Rutqvist, Jonny Birkholzer, Jens T. Liu, Hui-Hai TI On the impact of temperatures up to 200 degrees C in clay repositories with bentonite engineer barrier systems: A study with coupled thermal, hydrological, chemical, and mechanical modeling SO ENGINEERING GEOLOGY LA English DT Article DE nuclear waste disposal; Clay; Bentonite; THMC; Modeling; High temperature ID OPALINUS CLAY; COMPACTED BENTONITE; SMECTITE; ILLITIZATION; BEHAVIOR; TRANSPORT; TRANSFORMATION; PERFORMANCE; DISPOSAL; WASTE AB One of the most important design variables for a geological nuclear waste repository is the temperature limit up to which the engineered barrier system (EBS) and the natural geologic environment can be exposed. Up to now, almost all design concepts that involve bentonite-backfilled emplacement tunnels have chosen a maximum allowable temperature of about 100 degrees C. Such a choice is largely based on the consideration that in clay-based materials illitization and the associated mechanical changes in the bentonite (and perhaps the clay host rock) could affect the barrier attributes of the EBS. However, existing experimental and modeling studies on the occurrence of illitization and related performance impacts are not conclusive, in part because the relevant couplings between the thermal, hydrological, chemical, and mechanical (THMC) processes have not been fully represented in the models. This paper presents a fully coupled THMC simulation of a nuclear waste repository in a clay formation with a bentonite-backfilled EBS for 1000 years. Two scenarios were simulated for comparison: a case in which the temperature in the bentonite near the waste canister can reach about 200 degrees C and a case in which the temperature in the bentonite near the waste canister peaks at about 100 degrees C. The model simulations demonstrate some degree of illitization in both the bentonite buffer and the surrounding clay formation. Other chemical alterations include the dissolution of K-feldspar and calcite, and precipitation of quartz, chlorite, and kaolinite. In general, illitization in the bentonite and the clay formation is enhanced at higher temperature. However, the quantity of illitization is affected by many chemical factors and therefore varies a great deal. The most important chemical factors are the concentration of K in the pore water as well as the abundance and dissolution rate of K-feldspar; less important ones are the concentration of sodium and the quartz precipitation rate. In our modeling scenarios, the calculated decrease in smectite volume fraction in bentonite ranges from 1 to 8% of the initial volume fraction of smectite in the 100 degrees C scenario and 1-27% in the 200 degrees C scenario. Chemical changes in the 200 degrees C scenario could also lead to a reduction in swelling stress up to 15-18% whereas those in the 100 degrees C scenario result in about 14-15% reduction in swelling stress for the base case scenario. Model results also show that the 200 degrees C scenario results in a much higher total stress than the 100 degrees C scenario, mostly due to thermal pressurization. While cautions should be taken regarding the model results due to some limitations in the models, the modeling worlds illustrative in light of the relative importance of different processes occurring in EBS bentonite and clay formation at higher than 100 degrees C conditions, and could be of greater use when site specific data are available. (C) 2015 Elsevier B.V. All rights reserved. C1 [Zheng, Liange; Rutqvist, Jonny; Birkholzer, Jens T.; Liu, Hui-Hai] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Zheng, LE (reprint author), Mail Stop 74R316C,1 Cyclotron Rd, Berkeley, CA 94720 USA. EM lzheng@lbl.gov RI Birkholzer, Jens/C-6783-2011; Rutqvist, Jonny/F-4957-2015; zheng, liange/B-9748-2011 OI Birkholzer, Jens/0000-0002-7989-1912; Rutqvist, Jonny/0000-0002-7949-9785; zheng, liange/0000-0002-9376-2535 FU Used Fuel Disposition Campaign, Office of Nuclear Energy, of the U.S. Department of Energy [DE-AC02-05CH11231]; Berkeley Lab FX Funding for this work was provided by the Used Fuel Disposition Campaign, Office of Nuclear Energy, of the U.S. Department of Energy under Contract Number DE-AC02-05CH11231 with Berkeley Lab. NR 60 TC 4 Z9 4 U1 4 U2 22 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0013-7952 EI 1872-6917 J9 ENG GEOL JI Eng. Geol. PD OCT 30 PY 2015 VL 197 BP 278 EP 295 DI 10.1016/j.enggeo.2015.08.026 PG 18 WC Engineering, Geological; Geosciences, Multidisciplinary SC Engineering; Geology GA CV4QR UT WOS:000364252100023 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Aring;kesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Aring;sman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Aurousseau, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Banas, E Banerjee, S Bannoura, AAE Bansil, HS Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, M Becker, S Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Biedermann, D Bieniek, SP Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biondi, S Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehler, M Bogaerts, JA Bogavac, D Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boveia, A Boyd, J Boyko, IR Bozic, I Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Madden, WDB Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, K Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Bruschi, M Bruscino, N Bryngemark, L Buanes, T Buat, Q Buchholz, P Buckley, AG Buda, SI Budagov, IA Buehrer, F Bugge, L Bugge, MK Bulekov, O Bullock, D Burckhart, H Burdin, S Burghgrave, B Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Buzykaev, AR Urban, SC Caforio, D Cairo, VM Cakir, O Calace, N Calafiura, P Calandri, A Calderini, G Calfayan, P Caloba, LP Calvet, D Calvet, S Toro, RC Camarda, S Camarri, P Cameron, D Armadans, RC Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Cardarelli, R Cardillo, F Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Caudron, J Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, BC Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chang, P Chapman, JD Charlton, DG Chau, CC Barajas, CAC Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A Cheremushkina, E El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiarelli, G Childers, JT Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Choi, K Chouridou, S Chow, BKB Christodoulou, V Chromek-Burckhart, D Chudoba, J Chuinard, AJ Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Cinca, D Cindro, V Cioara, IA Ciocio, A Citron, ZH Ciubancan, M Clark, A Clark, BL Clark, PJ Clarke, RN Cleland, W Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Cogan, JG Colasurdo, L Cole, B Cole, S Colijn, AP Collot, J Colombo, T Compostella, G Muino, PC Coniavitis, E Connell, SH Connelly, IA Consonni, SM Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cote, D Cottin, G Cowan, G Cox, BE Cranmer, K Cree, G Crepe-Renaudin, S Crescioli, F Cribbs, WA Ortuzar, MC Cristinziani, M Croft, V Crosetti, G Donszelmann, TC Cummings, J Curatolo, M Cuthbert, C Czirr, H Czodrowski, P D'Auria, S D'Onofrio, M De Sousa, MJDS Da Via, C Dabrowski, W Dafinca, A Dai, T Dale, O Dallaire, F Dallapiccola, C Dam, M Dandoy, JR Dang, NP Daniells, AC Danninger, M Hoffmann, MD Dao, V Darbo, G Darmora, S Dassoulas, J Dattagupta, A Davey, W David, C Davidek, T Davies, E Davies, M Davison, P Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Benedetti, A De Castro, S De Cecco, S De Groot, N de Jong, P De la Torre, H De Lorenzi, F De Nooij, L De Pedis, D De Salvo, A De Sanctis, U De Santo, A De Regie, JBD Dearnaley, WJ Debbe, R Debenedetti, C Dedovich, DV Deigaard, I Del Peso, J Del Prete, T Delgove, D Deliot, F Delitzsch, CM Deliyergiyev, M Dell'Acqua, A Dell'Asta, L Dell'Orso, M Della Pietra, M della Volpe, D Delmastro, M Delsart, PA Deluca, C DeMarco, DA Demers, S Demichev, M Demilly, A Denisov, SP Derendarz, D Derkaoui, JE Derue, F Dervan, P Desch, K Deterre, C Deviveiros, PO Dewhurst, A Dhaliwal, S Di Ciaccio, A Di Ciaccio, L Di Domenico, A Di Donato, C Di Girolamo, A Di Girolamo, B Di Mattia, A Di Micco, B Di Nardo, R Di Simone, A Di Sipio, R Di Valentino, D Diaconu, C Diamond, M Dias, FA Diaz, MA Diehl, EB Dietrich, J Diglio, S Dimitrievska, A Dingfelder, J Dita, P Dita, S Dittus, F Djama, F Djobava, T Djuvsland, JI do Vale, MAB Dobos, D Dobre, M Doglioni, C Dohmae, T Dolejsi, J Dolezal, Z Dolgoshein, BA Donadelli, M Donati, S Dondero, P Donini, J Dopke, J Doria, A Dova, MT Doyle, AT Drechsler, E Dris, M Dubreuil, E Duchovni, E Duckeck, G Ducu, OA Duda, D Dudarev, A Duflot, L Duguid, L Duhrssen, M Dunford, M Yildiz, HD Duren, M Durglishvili, A Duschinger, D Dyndal, M Eckardt, C Ecker, KM Edgar, RC Edson, W Edwards, NC Ehrenfeld, W Eifert, T Eigen, G Einsweiler, K Ekelof, T El Kacimi, M Ellert, M Elles, S Ellinghaus, F Elliot, AA Ellis, N Elmsheuser, J Elsing, M Emeliyanov, D Enari, Y Endner, OC Endo, M Erdmann, J Ereditato, A Ernis, G Ernst, J Ernst, M Errede, S Ertel, E Escalier, M Esch, H Escobar, C Esposito, B Etienvre, AI Etzion, E Evans, H Ezhilov, A Fabbri, L Facini, G Fakhrutdinov, RM Falciano, S Falla, RJ Faltova, J Fang, Y Fanti, M Farbin, A Farilla, A Farooque, T Farrell, S Farrington, SM Farthouat, P Fassi, F Fassnacht, P Fassouliotis, D Giannelli, MF Favareto, A Fayard, L Federic, P Fedin, OL Fedorko, W Feigl, S Feligioni, L Feng, C Feng, EJ Feng, H Fenyuk, AB Feremenga, L Martinez, PF Perez, SF Ferrando, J Ferrari, A Ferrari, P Ferrari, R de Lima, DEF Ferrer, A Ferrere, D Ferretti, C Parodi, AF Fiascaris, M Fiedler, F Filipcic, A Filipuzzi, M Filthaut, F Fincke-Keeler, M Finelli, KD Fiolhais, MCN 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Zhao, Y. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Z boson production in p plus Pb collisions at root S-NN=5.02 TeV measured with the ATLAS detector SO PHYSICAL REVIEW C LA English DT Article ID RANGE ANGULAR-CORRELATIONS; LONG-RANGE; ROOT(NN)-N-S=5.02 TEV; ROOT-S(NN)=5.02 TEV; PPB COLLISIONS; DEPENDENCE; SIDE; LHC AB The ATLAS Collaboration measures the inclusive production of Z bosons via their decays into electron and muon pairs in p + Pb collisions at root S-NN = 5.02 TeV at the Large Hadron Collider. The measurements are made using data corresponding to integrated luminosities of 29.4 and 28.1 nb(-1) for Z -> ee and Z -> mu mu, respectively. The results from the two channels are consistent and combined to obtain a cross section times the Z -> ll branching ratio, integrated over the rapidity region vertical bar y(Z)*vertical bar < 3.5, of 139.8 +/- 4.8 (statistical) +/- 6.2 (systematic) +/- 3.8 (luminosity) nb. Differential cross sections are presented as functions of the Z boson rapidity and transverse momentum and compared with models based on parton distributions both with and without nuclear corrections. The centrality dependence of Z boson production in p + Pb collisions is measured and analyzed within the framework of a standard Glauber model and the model's extension for fluctuations of the underlying nucleon-nucleon scattering cross section. C1 [Jackson, P.; Lee, L.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Yildiz, H. Duran] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Kuday, S.] Istanbul Aydin Univ, Istanbul, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. [Barnovska, Z.; Berger, N.; Delmastro, M.; Di Ciaccio, L.; Elles, S.; Hryn'ova, T.; Jezequel, S.; Koletsou, I.; Lafaye, R.; Leveque, J.; Massol, N.; Sauvage, G.; Sauvan, E.; Simard, O.; Todorov, T.; Wingerter-Seez, I.; Yatsenko, E.] CNRS IN2P3, LAPP, Annecy Le Vieux, France. [Barnovska, Z.; Berger, N.; Delmastro, M.; Di Ciaccio, L.; Elles, S.; Hryn'ova, T.; Jezequel, S.; Koletsou, I.; Lafaye, R.; Leveque, J.; Massol, N.; Sauvage, G.; Sauvan, E.; Simard, O.; Todorov, T.; Wingerter-Seez, I.; Yatsenko, E.] Univ Savoie Mt Blanc, Annecy Le Vieux, France. [Blair, R. E.; Chekanov, S.; Childers, J. T.; Feng, E. J.; LeCompte, T.; Love, J.; Malon, D.; Nguyen, D. H.; Paramonov, A.; Price, L. E.; Proudfoot, J.; van Gemmeren, P.; Vaniachine, A.; Wang, R.; Yoshida, R.; Zhang, J.] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Cheu, E.; Johns, K. A.; Lampen, C. L.; Lampl, W.; Lei, X.; Leone, R.; Loch, P.; Nayyar, R.; O'grady, F.; Rutherfoord, J. P.; Shupe, M. A.; Varnes, E. W.; Veatch, J.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Brandt, A.; Bullock, D.; Carrillo-Montoya, G. D.; Cote, D.; Darmora, S.; De, K.; Farbin, A.; Feremenga, L.; Griffiths, J.; Hadavand, H. K.; Heelan, L.; Kim, H. Y.; Ozturk, N.; Schovancova, J.; Sosebee, M.; Stradling, A. R.; Usai, G.; Vartapetian, A.; White, A.; Yu, J.] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA. [Angelidakis, S.; Chouridou, S.; Fassouliotis, D.; Giokaris, N.; Ioannou, P.; Kourkoumelis, C.; Manousakis-Katsikakis, A.; Tsirintanis, N.] Univ Athens, Dept Phys, Athens, Greece. [Alexopoulos, T.; Benekos, N.; Dris, M.; Gazis, E. N.; Karakostas, K.; Karastathis, N.; Karentzos, E.; Leontsinis, S.; Maltezos, S.; Ntekas, K.; Panagiotopoulou, E.; Papadopoulou, Th D.; Shimojima, M.; Tsipolitis, G.; Vlachos, S.] Natl Tech Univ Athens, Dept Phys, Zografos, Greece. [Abdinov, O.; Khalil-zada, F.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Anjos, N.; Bosman, M.; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fischer, C.; Fracchia, S.; Giangiobbe, V.; Gonzalez Parra, G.; Grinstein, S.; Helsens, C.; Rozas, A. Juste; Korolkov, I.; Lange, J. C.; Le Menedeu, E.; Paz, I. Lopez; Martinez, M.; Mir, L. M.; Berlingen, J. Montejo; Pages, A. Pacheco; Aranda, C. Padilla; Riu, I.; Sorin, V.; Succurro, A.; Tripiana, M. F.; Tsiskaridze, S.; Valery, L.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Anjos, N.; Bosman, M.; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fischer, C.; Fracchia, S.; Giangiobbe, V.; Gonzalez Parra, G.; Grinstein, S.; Helsens, C.; Rozas, A. Juste; Korolkov, I.; Lange, J. C.; Le Menedeu, E.; Paz, I. Lopez; Martinez, M.; Mir, L. M.; Berlingen, J. Montejo; Pages, A. Pacheco; Aranda, C. Padilla; Riu, I.; Sorin, V.; Succurro, A.; Tripiana, M. F.; Tsiskaridze, S.; Valery, L.] Univ Autonoma Barcelona, Dept Fis, E-08193 Barcelona, Spain. [Agatonovic-Jovin, T.; Bogavac, D.; Bozic, I.; Dimitrievska, A.; Krstic, J.; Paredes, B. Lopez; Marjanovic, M.; Orestano, D.; Popovic, D. S.; Sijacki, Dj; Simic, Lj; Vranjes, N.; Milosavljevic, M. Vranjes; Zivkovic, L.] Univ Belgrade, Inst Phys, Belgrade, Serbia. [Buanes, T.; Dale, O.; Eigen, G.; Kastanas, A.; Liebig, W.; Lipniacka, A.; Maeland, S.; Latour, B. Martin Dit; Rosendahl, P. L.; Sjursen, T. B.; Smestad, L.; Stugu, B.; Ugland, M.; Zalieckas, J.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Amadio, B. T.; Annovi, A.; Antonov, A.; Artamonov, A.; Axen, B.; Barnett, R. M.; Basalaev, A.; Bellerive, A.; Beringer, J.; Bhimji, W.; Brosamer, J.; Calafiura, P.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Papageorgiou, K.; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Amadio, B. T.; Annovi, A.; Antonov, A.; Artamonov, A.; Axen, B.; Barnett, R. M.; Beringer, J.; Bhimji, W.; Brosamer, J.; Calafiura, P.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Papageorgiou, K.; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Aloisio, A.; Biedermann, D.; Dietrich, J.; Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Herrberg-Schubert, R.; Hristova, I.; Kind, O. M.; Kolanoski, H.; Lacker, H.; Lohse, T.; Nikiforov, A.; Rehnisch, L.; Rieck, P.; Schulz, H.; Sperlich, D.; Stamm, S.; zur Nedden, M.] Humboldt Univ, Dept Phys, Berlin, Germany. [Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Mullier, G. A.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Mullier, G. A.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Bella, L. Aperio; Baca, M. J.; Bansil, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Owen, R. E.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.; Sahinsoy, M.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Phys Engn, Gaziantep, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Alberghi, G. L.; Bellagamba, L.; Biondi, S.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Corradi, M.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] INFN Sez Bologna, Bologna, Italy. [Alberghi, G. L.; Biondi, S.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Aloisio, A.; Annovi, A.; Arslan, O.; Bernlochner, F. U.; Brock, I.; Bruscino, N.; Cioara, I. A.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch; Gonella, L.; Haefner, P.; Hageboeck, S.; Hansen, M. C.; Hellmich, D.; Hohn, D.; Huegging, F.; Janssen, J.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mergelmeyer, S.; Mijovic, L.; Moles-Valls, R.; Obermann, T.; Pohl, D.; Ricken, O.; Sarrazin, B.; Schaepe, S.; Schopf, E.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Seema, P.; Stillings, J. A.; Tannoury, N.; Uhlenbrock, M.; Velz, T.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Yuen, S. P. Y.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Barone, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Dhaliwal, S.; Fitzgerald, E. A.; Sciolla, G.; Venturini, A.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Amaral Coutinho, Y.; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio De Janeiro COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Fed Univ Juiz de Fora UFJF, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Navarro, J. L. La Rosa; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Aloisio, A.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Horia Hulubei Natl Inst Phys & Nucl Engn, Bucharest 077125, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Gonzalez, B. Alvarez; Anders, G.; Anghinolfi, F.; Annovi, A.; Antonov, A.; Armbruster, A. J.; Arnaez, O.; Artamonov, A.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jaekel, M. R.; Jakobsen, S.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sforza, F.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Shanghai Key Lab Particle Phys & Cosmol, Dept Phys & Astron, Shanghai 200030, Peoples R China. [Chen, X.] Tsinghua Univ, Phys Dept, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] INFN Grp Collegato Cosenza, Lab Nazl Frascati, Cosenza, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Gach, G. P.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Phys Dept, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Phys Dept, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Hamburg, Germany. [Annovi, A.; Antonov, A.; Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] INFN Lab Nazl Frascati, Frascati, Italy. [Amoroso, S.; Annovi, A.; Antonov, A.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Sammel, D.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Calace, N.; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Paolozzi, L.; Picazio, A.; Ristic, B.; Schramm, S.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] INFN Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, D-69115 Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Phys Inst, D-69115 Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Jussel, P.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kishimoto, T.; Kurashige, H.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] INFN Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Allport, P. P.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Tepel, F.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Tepel, F.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Annovi, A.; Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Annovi, A.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Hu, X.; Levin, D.; Liu, H.; Long, J. D.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] INFN Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. 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P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Annovi, A.; Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Fusayasu, T.; Shimojima, M.; Wakabayashi, J.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] INFN Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Konig, A. C.; Nektarijevic, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Annovi, A.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kharlamov, A. G.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kharlamov, A. G.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS IN2P3, Orsay, France. [Endo, M.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] INFN Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Fletcher, R. R. M.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Reichert, J.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] INFN Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Onofre, A.; Palma, A.; Pedro, R.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] INFN Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Salamon, A.; Santonico, R.] INFN Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] INFN Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.; Idrissi, Z.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Cadi Ayyad, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph; Schwemling, Ph; Schwindling, J.] CEA Saclay Commissariat Energie Atom & Energies A, DSM IRFU Inst Rech Lois Fondamentales Univers, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.; Meehan, S.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Govender, N.; Lee, C. A.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hamity, G. N.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Fac Exact Sci, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Jovicevic, J.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] INFN Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Gradin, P. O. J.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Swedish, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.; Trovatelli, M.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kaplan, L. S.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Beermann, T. A.; Braun, H. M.; Cornelissen, T.; Ellinghaus, F.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Thomsen, L. A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. 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Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Rozas, A. Juste; Martinez, M.] ICREA, Barcelona, Spain. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu 30013, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Jenni, P.] CERN, Geneva, Switzerland. [Khubua, J.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellen Open Univ, Patras, Greece. [Li, B.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Li, Y.] Univ Paris 11, LAL, Orsay, France. [Li, Y.] CNRS IN2P3, Orsay, France. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Liu, B.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tikhomirov, V. O.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Xu, L.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. EM yy RI Prokoshin, Fedor/E-2795-2012; Staroba, Pavel/G-8850-2014; Gavrilenko, Igor/M-8260-2015; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Fabbri, Laura/H-3442-2012; Gutierrez, Phillip/C-1161-2011; Gerbaudo, Davide/J-4536-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; SULIN, VLADIMIR/N-2793-2015; Brooks, William/C-8636-2013; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Fedin, Oleg/H-6753-2016; Snesarev, Andrey/H-5090-2013; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; Villa, Mauro/C-9883-2009; Chiarelli, Giorgio/E-8953-2012; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Tripiana, Martin/H-3404-2015; Smirnova, Oxana/A-4401-2013; Savarala, Hari Krishna/A-3516-2015; Doyle, Anthony/C-5889-2009; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Boyko, Igor/J-3659-2013; Vranjes Milosavljevic, Marija/F-9847-2016; Chekulaev, Sergey/O-1145-2015; Zhukov, Konstantin/M-6027-2015; Di Domenico, Antonio/G-6301-2011; Livan, Michele/D-7531-2012; Gladilin, Leonid/B-5226-2011; Mitsou, Vasiliki/D-1967-2009; Andreazza, Attilio/E-5642-2011; Tikhomirov, Vladimir/M-6194-2015; Carvalho, Joao/M-4060-2013; White, Ryan/E-2979-2015; Mashinistov, Ruslan/M-8356-2015; Warburton, Andreas/N-8028-2013; spagnolo, stefania/A-6359-2012; Buttar, Craig/D-3706-2011; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Garcia, Jose /H-6339-2015 OI Prokoshin, Fedor/0000-0001-6389-5399; Gauzzi, Paolo/0000-0003-4841-5822; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; SULIN, VLADIMIR/0000-0003-3943-2495; Brooks, William/0000-0001-6161-3570; Vykydal, Zdenek/0000-0003-2329-0672; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Villa, Mauro/0000-0002-9181-8048; Chiarelli, Giorgio/0000-0001-9851-4816; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Smirnova, Oxana/0000-0003-2517-531X; Savarala, Hari Krishna/0000-0001-6593-4849; Doyle, Anthony/0000-0001-6322-6195; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Boyko, Igor/0000-0002-3355-4662; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Di Domenico, Antonio/0000-0001-8078-2759; Livan, Michele/0000-0002-5877-0062; Gladilin, Leonid/0000-0001-9422-8636; Mitsou, Vasiliki/0000-0002-1533-8886; Andreazza, Attilio/0000-0001-5161-5759; Tikhomirov, Vladimir/0000-0002-9634-0581; Carvalho, Joao/0000-0002-3015-7821; White, Ryan/0000-0003-3589-5900; Mashinistov, Ruslan/0000-0001-7925-4676; Warburton, Andreas/0000-0002-2298-7315; spagnolo, stefania/0000-0001-7482-6348; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; RGC, China; Hong Kong SAR, China; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, The Netherlands; NWO, The Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions, without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC, and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST, and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR, and VSC CR, Czech Republic; DNRF, DNSRC, and Lundbeck Foundation, Denmark; EPLANET, ERC, and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG, and AvH Foundation, Germany; GSRT and NSRF, Greece; RGC, Hong Kong SAR, China; ISF, MINERVA, GIF, I-CORE, and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, The Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF, and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; and DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular, from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (The Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK), and BNL (USA) and in the Tier-2 facilities worldwide. NR 38 TC 5 Z9 5 U1 17 U2 98 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD OCT 30 PY 2015 VL 92 IS 4 AR 044915 DI 10.1103/PhysRevC.92.044915 PG 22 WC Physics, Nuclear SC Physics GA CU8KU UT WOS:000363792100004 ER PT J AU Ali, E Nixon, K Murray, A Ning, CG Colgan, J Madison, D AF Ali, Esam Nixon, Kate Murray, Andrew Ning, Chuangang Colgan, James Madison, Don TI Comparison of experimental and theoretical electron-impact-ionization triple-differential cross sections for ethane SO PHYSICAL REVIEW A LA English DT Article ID LOW-ENERGY E; MOLECULAR-ORBITALS; 2E; 3-SIGMA(G) AB We have recently examined electron-impact ionization of molecules that have one large atom at the center, surrounded by H nuclei (H2O, NH3, CH4). All of these molecules have ten electrons; however, they vary in their molecular symmetry. We found that the triple-differential cross sections (TDCSs) for the highest occupied molecular orbitals (HOMOs) were similar, as was the character of the HOMO orbitals which had a p-type " peanut" shape. In this work, we examine ethane (C2H6) which is a molecule that has two large atoms surrounded by H nuclei, so that its HOMO has a double-peanut shape. The experiment was performed using a coplanar symmetric geometry (equal final-state energies and angles). We find the TDCS for ethane is similar to the single-center molecules at higher energies, and is similar to a diatomic molecule at lower energies. C1 [Ali, Esam; Madison, Don] Missouri Univ Sci & Technol, Dept Phys, Rolla, MO 65409 USA. [Nixon, Kate; Murray, Andrew] Univ Manchester, Sch Phys & Astron, Photon Sci Inst, Manchester M13 9PL, Lancs, England. [Nixon, Kate] Wolverhampton Univ, Sch Biol Chem & Forens Sci, Wolverhampton WV1 1LY, W Midlands, England. [Ning, Chuangang] Tsinghua Univ, Dept Phys, State Key Lab Low Dimens Quantum Phys, Beijing 100084, Peoples R China. [Colgan, James] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Ali, E (reprint author), Missouri Univ Sci & Technol, Dept Phys, Rolla, MO 65409 USA. EM eaagx2@mst.edu RI Nixon, Kate/I-4968-2014 OI Nixon, Kate/0000-0002-1226-1879 FU European commission; US National Science Foundation [PHY-1505819]; National Natural Science Foundation of China [11174175]; Texas Advanced Computing Center [TG-MCA07S029]; US Department of Energy [DE-AC5206NA25396] FX K.N. would like to thank the European commission for a Marie Curie International Incoming Fellowship undertaken at the University of Manchester. We would like to thank the technicians in the Schuster laboratory for providing excellent support for the experimental apparatus. This work was partly supported by the US National Science Foundation under Grant No. PHY-1505819 and by the National Natural Science Foundation of China under Grant No. 11174175. Computational work was performed with Institutional Computing resources made available through the Los Alamos National Laboratory and XSEDE resources provided by the Texas Advanced Computing Center (Grant No. TG-MCA07S029). The Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the US Department of Energy under Contract No. DE-AC5206NA25396. NR 36 TC 4 Z9 4 U1 0 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD OCT 30 PY 2015 VL 92 IS 4 AR 042711 DI 10.1103/PhysRevA.92.042711 PG 6 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CU8JW UT WOS:000363789600005 ER PT J AU Mustafa, JI Coh, S Cohen, ML Louie, SG AF Mustafa, Jamal I. Coh, Sinisa Cohen, Marvin L. Louie, Steven G. TI Automated construction of maximally localized Wannier functions: Optimized projection functions method SO PHYSICAL REVIEW B LA English DT Article ID SIMULTANEOUS DIAGONALIZATION; PSEUDOPOTENTIALS AB Maximally localizedWannier functions are widely used in electronic structure theory for analyses of bonding, electric polarization, orbitalmagnetization, and for interpolation. The state of the art method for their construction is based on the method of Marzari and Vanderbilt. One of the practical difficulties of this method is guessing functions (initial projections) that approximate the final Wannier functions. Here we present an approach based on optimized projection functions that can construct maximally localizedWannier functions without a guess. We describe and demonstrate this approach on several realistic examples. C1 [Mustafa, Jamal I.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Mustafa, JI (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM sglouie@berkeley.edu FU Theory Program at the Lawrence Berkeley National Lab through the Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [DMR15-1508412]; Office of Science of the U.S. Department of Energy FX We thank David Vanderbilt for discussion. This research was supported by the Theory Program at the Lawrence Berkeley National Lab through the Office of Basic Energy Sciences, U.S. Department of Energy under Contract No. DE-AC02-05CH11231 (methods and algorithm developments), and by the National Science Foundation under Grant No. DMR15-1508412 (band structure calculations). Computational resources have been provided by the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy. NR 23 TC 5 Z9 5 U1 5 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 30 PY 2015 VL 92 IS 16 AR 165134 DI 10.1103/PhysRevB.92.165134 PG 9 WC Physics, Condensed Matter SC Physics GA CU8KQ UT WOS:000363791700003 ER PT J AU Soderlind, P Zhou, F Landa, A Klepeis, JE AF Soederlind, Per Zhou, F. Landa, A. Klepeis, J. E. TI Phonon and magnetic structure in delta-plutonium from density-functional theory SO SCIENTIFIC REPORTS LA English DT Article ID 1ST-PRINCIPLES THEORY; PU; METALS; SCATTERING; STABILITY; SPIN AB We present phonon properties of plutonium metal obtained from a combination of density-functional-theory (DFT) electronic structure and the recently developed compressive sensing lattice dynamics (CSLD). The CSLD model is here trained on DFT total energies of several hundreds of quasi-random atomic configurations for best possible accuracy of the phonon properties. The calculated phonon dispersions compare better with experiment than earlier results obtained from dynamical mean-field theory. The density-functional model of the electronic structure consists of disordered magnetic moments with all relativistic effects and explicit orbital-orbital correlations. The magnetic disorder is approximated in two ways: (i) a special quasi-random structure and (ii) the disordered-local-moment method within the coherent potential approximation. Magnetism in plutonium has been debated intensely, but the present magnetic approach for plutonium is validated by the close agreement between the predicted magnetic form factor and that of recent neutron-scattering experiments. C1 [Soederlind, Per; Zhou, F.; Landa, A.; Klepeis, J. E.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Soderlind, P (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM soderlind@llnl.gov RI Zhou, Fei/D-1938-2010 OI Zhou, Fei/0000-0001-9659-4648 FU U.S. DOE by LLNL [DE-AC52-07NA27344] FX We thank B. Sadigh, F. Kormann, and T. Bjorkman for helpful discussions. A. L. thanks A. V. Ruban, L. Vitos, and M. Dehghani for EMTO development. This work was performed under the auspices of the U.S. DOE by LLNL under Contract DE-AC52-07NA27344. NR 35 TC 7 Z9 7 U1 6 U2 27 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 30 PY 2015 VL 5 AR 15958 DI 10.1038/srep15958 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CU7YO UT WOS:000363758000001 PM 26514238 ER PT J AU Ma, EY Cui, YT Ueda, K Tang, SJ Chen, K Tamura, N Wu, PM Fujioka, J Tokura, Y Shen, ZX AF Ma, Eric Yue Cui, Yong-Tao Ueda, Kentaro Tang, Shujie Chen, Kai Tamura, Nobumichi Wu, Phillip M. Fujioka, Jun Tokura, Yoshinori Shen, Zhi-Xun TI Mobile metallic domain walls in an all-in-all-out magnetic insulator SO SCIENCE LA English DT Article ID HUBBARD-MODEL; HARTREE-FOCK AB Magnetic domain walls are boundaries between regions with different configurations of the same magnetic order. In a magnetic insulator, where the magnetic order is tied to its bulk insulating property, it has been postulated that electrical properties are drastically different along the domain walls, where the order is inevitably disturbed. Here we report the discovery of highly conductive magnetic domain walls in a magnetic insulator, Nd2Ir2O7, that has an unusual all-in-all-out magnetic order, via transport and spatially resolved microwave impedance microscopy. The domain walls have a virtually temperature-independent sheet resistance of similar to 1 kilohm per square, show smooth morphology with no preferred orientation, are free from pinning by disorders, and have strong thermal and magnetic field responses that agree with expectations for all-in-all-out magnetic order. C1 [Ma, Eric Yue; Cui, Yong-Tao; Tang, Shujie; Wu, Phillip M.; Shen, Zhi-Xun] Stanford Univ, Geballe Lab Adv Mat, Stanford, CA 94305 USA. [Ma, Eric Yue; Shen, Zhi-Xun] Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA. [Ueda, Kentaro; Fujioka, Jun; Tokura, Yoshinori] Univ Tokyo, Dept Appl Phys, Tokyo 113, Japan. [Ueda, Kentaro; Fujioka, Jun; Tokura, Yoshinori] RIKEN Ctr Emergent Matter Sci CEMS, Saitama, Japan. [Tang, Shujie] SIMIT, State Key Lab Funct Mat Informat, Shanghai, Peoples R China. [Chen, Kai] Xi An Jiao Tong Univ, State Key Lab Mech Behav Mat, Ctr Adv Mat Performance Nanoscale CAMP Nano, Xian 710049, Peoples R China. [Tamura, Nobumichi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source ALS, Berkeley, CA 94720 USA. RP Tokura, Y (reprint author), Univ Tokyo, Dept Appl Phys, 7-3-1 Hongo, Tokyo 113, Japan. EM tokura@riken.jp; zxshen@stanford.edu RI Tokura, Yoshinori/C-7352-2009; xjtu, campnano/Q-1904-2015; Chen, Kai/O-5662-2014; Fujioka, Jun/A-1590-2015; Cui, Yong-Tao/G-8505-2015; OI Chen, Kai/0000-0002-4917-4445; Cui, Yong-Tao/0000-0002-8015-1049; Ma, Eric Yue/0000-0002-0539-1501 FU NSF [DMR-1305731]; Gordon and Betty Moore Foundation [GBMF3133]; Emergent Phenomena in Quantum Systems (EPiQS) initiative [GBMF4546]; Japan Society for the Promotion of Science [80609488, 24224009]; Funding Program in World-Leading Innovative R&D on Science and Technology (FIRST Program); China Scholarship Council [201304910185]; National Young 1000 Talents Program; National Science Foundation of China (NSFC) [51302207]; U.S. Department of Energy at Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; University of California, Berkeley, California FX We thank R. Laughlin for helpful discussions. We thank A. Bestwick, E. Fox, and D. Goldhaber-Gordon for help with the dilution refrigerator measurement. The measurement at Stanford University is supported by NSF grant DMR-1305731, the Gordon and Betty Moore Foundation through grant GBMF3133, and Emergent Phenomena in Quantum Systems (EPiQS) initiative GBMF4546. The crystal growth at University of Tokyo and RIKEN is supported by the Grant-in-Aid for Scientific Research (grant 80609488 and 24224009) from the Japan Society for the Promotion of Science and the Funding Program in World-Leading Innovative R&D on Science and Technology (FIRST Program). S.T. is partly supported by China Scholarship Council (grant 201304910185). K.C. is supported by the National Young 1000 Talents Program and the National Science Foundation of China (NSFC) under contract 51302207. The Advanced Light Source is supported by the director, Office of Science, Office of Basic Energy Sciences, Materials Sciences Division, of the U.S. Department of Energy under contract DE-AC02-05CH11231 at Lawrence Berkeley National Laboratory and University of California, Berkeley, California. All additional data are available in the supplementary materials. Z.-X.S. is a cofounder of PrimeNano Inc., which licensed the sMIM technology from Stanford for commercial instrument. This technology was modified for low-temperature measurement in this report. Stanford University and RIKEN have filed a joint provisional U.S. patent application on memory devices based on conductive magnetic domain walls. NR 30 TC 21 Z9 22 U1 19 U2 93 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD OCT 30 PY 2015 VL 350 IS 6260 BP 538 EP 541 DI 10.1126/science.aac8289 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CU6RG UT WOS:000363660000043 PM 26516280 ER PT J AU Gueroult, R Hobbs, DT Fisch, NJ AF Gueroult, Renaud Hobbs, David T. Fisch, Nathaniel J. TI Plasma filtering techniques for nuclear waste remediation SO JOURNAL OF HAZARDOUS MATERIALS LA English DT Article DE Nuclear waste; Separation; Plasma mass filter; Economic feasibility ID MASS FILTER; SLUDGE AB Nuclear waste cleanup is challenged by the handling of feed stocks that are both unknown and complex. Plasma filtering, operating on dissociated elements, offers advantages over chemical methods in processing such wastes. The costs incurred by plasma mass filtering for nuclear waste pretreatment, before ultimate disposal, are similar to those for chemical pretreatment. However, significant savings might be achieved in minimizing the waste mass. This advantage may be realized over a large range of chemical waste compositions, thereby addressing the heterogeneity of legacy nuclear waste. (C) 2015 Elsevier B.V. All rights reserved. C1 [Gueroult, Renaud; Fisch, Nathaniel J.] Princeton Plasma Phys Lab, Princeton, NJ 08540 USA. [Hobbs, David T.] Savannah River Natl Lab, Aiken, SC 29808 USA. RP Gueroult, R (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08540 USA. EM rgueroul@pppl.gov FU DoE [DE-AC02-09CH11466] FX This work was supported under DoE Contract Number DE-AC02-09CH11466. NR 49 TC 2 Z9 2 U1 2 U2 24 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-3894 EI 1873-3336 J9 J HAZARD MATER JI J. Hazard. Mater. PD OCT 30 PY 2015 VL 297 BP 153 EP 159 DI 10.1016/j.jhazmat.2015.04.058 PG 7 WC Engineering, Environmental; Engineering, Civil; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CQ4SU UT WOS:000360595700019 PM 25956646 ER PT J AU Pezeshki, AM Clement, JT Veith, GM Zawodzinski, TA Mench, MM AF Pezeshki, Alan M. Clement, Jason T. Veith, Gabriel M. Zawodzinski, Thomas A. Mench, Matthew M. TI High performance electrodes in vanadium redox flow batteries through oxygen-enriched thermal activation SO JOURNAL OF POWER SOURCES LA English DT Article DE Vanadium redox flow battery; Carbon paper; Kinetics; Surface area; Thermal activation; Electrode AB The roundtrip electrochemical energy efficiency is improved from 63% to 76% at a current density of 200 mA cm(-2) in an all-vanadium redox flow battery (VRFB) by utilizing modified carbon paper electrodes in the high-performance no-gap design. Heat treatment of the carbon paper electrodes in a 42% oxygen/58% nitrogen atmosphere increases the electrochemically wetted surface area from 0.24 to 51.22 m(2) g(-1), resulting in a 100-140 mV decrease in activation overpotential at operationally relevant current densities. An enriched oxygen environment decreases the amount of treatment time required to achieve high surface area. The increased efficiency and greater depth of discharge doubles the total usable energy stored in a fixed amount of electrolyte during operation at 200 mA cm(-2). (C) 2015 Elsevier B.V. All rights reserved. C1 [Pezeshki, Alan M.; Zawodzinski, Thomas A.] Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA. [Pezeshki, Alan M.] Univ Tennessee, Bredesen Ctr Interdisciplinary Res & Grad Educ, Knoxville, TN 37996 USA. [Pezeshki, Alan M.; Veith, Gabriel M.; Zawodzinski, Thomas A.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Clement, Jason T.; Mench, Matthew M.] Univ Tennessee, Dept Mech Aerosp & Biomed Engn, Knoxville, TN 37996 USA. [Mench, Matthew M.] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. RP Mench, MM (reprint author), Univ Tennessee, 410 Dougherty Eng Bldg, Knoxville, TN 37996 USA. EM mmench@utk.edu FU Office of Naval Research [N00014-12-1-0887]; Tennessee Solar Conversion and Storage using Outreach, Research and Education (TN-SCORE); NSF EPS [1004083]; U.S. Department of Energy's Office of Basic Energy Science (DOE-BES), Division of Materials Sciences and Engineering, under UT-Battelle, LLC. [DE-AC0500OR22725] FX The authors would like to acknowledge Dr. C.-N. Sun for assistance in capacitance measurements, N. Cantillo-Cuello for assistance with BET surface area measurements, and Drs. E.L. Redmond and D.S. Aaron for fruitful discussion. The authors would also like to acknowledge the Office of Naval Research for support of this work under Long Range Broad Agency Announcement (BAA) #N00014-12-1-0887 as well as Tennessee Solar Conversion and Storage using Outreach, Research and Education (TN-SCORE; NSF EPS #1004083). A portion of this work (GMV-XPS) was supported by U.S. Department of Energy's Office of Basic Energy Science (DOE-BES, DE-AC0500OR22725), Division of Materials Sciences and Engineering, under contract with UT-Battelle, LLC. NR 22 TC 18 Z9 18 U1 14 U2 90 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD OCT 30 PY 2015 VL 294 BP 333 EP 338 DI 10.1016/j.jpowsour.2015.05.118 PG 6 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA CO2EI UT WOS:000358968400042 ER PT J AU Vu, A Qin, Y Lin, CK Abouimrane, A Burrell, AK Bloom, S Bass, D Bareno, J Bloom, I AF Anh Vu Qin, Yan Lin, Chi-Kai Abouimrane, Ali Burrell, Anthony K. Bloom, Samuel Bass, Dean Bareno, Javier Bloom, Ira TI Effect of composition on the voltage fade phenomenon in lithium-, manganese-rich xLiMnO(3).(1-x)LiNiaMnbCocO2: A combinatorial synthesis approach SO JOURNAL OF POWER SOURCES LA English DT Article DE Lithium battery; Voltage fade; Combinatorial synthesis ID OXIDE PSEUDOTERNARY SYSTEM; ION BATTERIES; POSITIVE ELECTRODE; HIGH-CAPACITY; MN; NI; TEMPERATURES; CATHODES; LIMNO2 AB The effect of composition on the voltage fade phenomenon was probed using combinatorial synthesis methods. In compositions that have the general formula, (Li2MnO3)(a)(LiNiO2)(b)(LiMnO2)(c)(LiCoO2)d, where 0 <= a <= 0.83, 0.15 <= b <= 0.42, 0 <= c <= 0.85, and 0 <= d <= 0.30 (a + b + c + d =1), the dependence of features in the x-ray diffraction pattern and of voltage fade on composition were identified and mapped. The observed values of voltage fade indicated that it displayed some sensitivity to composition, but that the sensitivity was not large. The values of voltage fade were found to be amenable to statistical modeling. The model indicated that it may be possible to lower the value of voltage fade below 0.01% by adjusting the composition of the system; however, the composition is not expected to have the layered-layered structure. (C) 2015 Elsevier B.V. All rights reserved. C1 [Anh Vu; Qin, Yan; Lin, Chi-Kai; Abouimrane, Ali; Burrell, Anthony K.; Bareno, Javier; Bloom, Ira] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Bloom, Samuel] Univ Maryland, Dept Math, College Pk, MD 20742 USA. [Bass, Dean] Argonne Natl Lab, Analyt Chem Lab, Argonne, IL 60439 USA. RP Bloom, I (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM ira.bloom@anl.gov FU U.S. Department of Energy (DOE), Office of Vehicle Technologies [DE-AC02-06CH11357] FX The authors wish to thank Dr. Magali Ferrandon for using the CM3 combinatorial machine to make samples for this work. They also wish to thank John Osudar for help rendering text using OpenGL. The work at Argonne National Laboratory was performed under the auspices of the U.S. Department of Energy (DOE), Office of Vehicle Technologies, under Contract No. DE-AC02-06CH11357. The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. NR 21 TC 2 Z9 2 U1 5 U2 74 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD OCT 30 PY 2015 VL 294 BP 711 EP 718 DI 10.1016/j.jpowsour.2015.06.100 PG 8 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA CO2EI UT WOS:000358968400089 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorima, A Amoroso, S Amram, N 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CA ATLAS Collaboration TI ATLAS Run 1 searches for direct pair production of third-generation squarks at the Large Hadron Collider SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID DYNAMICAL SYMMETRY-BREAKING; PP COLLISIONS; ROOT-S=7 TEV; B-JETS; SUPERGAUGE TRANSFORMATIONS; SUPERSYMMETRIC PARTICLES; E(+)E(-) COLLISIONS; LOCAL SUPERSYMMETRY; GRAND UNIFICATION; MEASURING MASSES AB This paper reviews and extends searches for the direct pair production of the scalar supersymmetric partners of the top and bottom quarks in proton-proton collisions collected by the ATLAS collaboration during the LHC Run 1. Most of the analyses use 20 fb(-1) of collisions at a centre-of-mass energy of root s = 8 TeV, although in some case an additional 4.7 fb(-1) of collision data at root s = 7 TeV are used. New analyses are introduced to improve the sensitivity to specific regions of the model parameter space. 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[Amaral Coutinho, Y.] Univ Fed Rio de Janeiro, COPPE, EE, IF, Rio De Janeiro, Brazil. [Manhaes de Andrade Filho, L.] Fed Univ Juiz Fora UFJF, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Navarro, L. La Rosa; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, Sao Paulo, Brazil. [Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Boldea, V.; Buda, S. I.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON, Canada. [Aleksa, M.; Gonzalez, B. Alvarez; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conventi, F.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duhrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jaekel, M. R.; Jakobsen, S.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sforza, F.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; TenKate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Carquin, E.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. Shandong Univ, Sch Phys, Guangzhou, Guangdong, Peoples R China. Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai, Peoples R China. Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.] INFN Grp Collegato Cosenza, Lab Nazl Frascati, Frascati, Italy. Univ Calabria, Dipartimento Fis, Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, Y.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Monig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Monig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Gossling, C.; Homann, M.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, L.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Testa, M.; Vilucchi, E.] INFN Lab Nazl Frascati, Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buscher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Ruhr, F.; Rurikova, Z.; Ruthmann, N.; Sammel, D.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Zhang, R.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Calace, N.; Clark, A.; Delitzsch, C. M.; della Volp, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Paolozzi, L.; Picazio, A.; Ristic, B.; Schramm, S.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.] INFN Sez Genova, Genoa, Italy. [Barberis, D.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Khubua, J.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Duren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Phys Inst 2, Giessen, Germany. [Bates, R. L.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, E. Ferreira; Gul, U.; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Denis, R. D. St.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Phys Inst 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, Lab Phys Subatom & Cosmol, CNRS, IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.] Heidelberg Univ, Phys Inst, Heidelberg, Germany. Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Jussel, P.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhong, J.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kishimoto, T.; Kurashige, H.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Ventura, A.] INFN Sez Lecce, Lecce, Italy. Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Allport, P. P.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper-Sarkar, A. M.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; LeDortz, O.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; LeDortz, O.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; LeDortz, O.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buscher, V.; Caputo, R.; Caudron, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Hulsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Kopke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schafer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Buzatu, A.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Schoening, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Buzatu, A.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Schoening, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Hu, X.; Levin, D.; Liu, H.; Long, J. D.; Lu, N.; Marley, D. E.; Mckee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, F.; Zhou, C.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavallia, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] INFN Sez Milano, Milan, Italy. [Andreazza, A.] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Losel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.; Zaitsev, A. M.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.; Zaitsev, A. M.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi, Japan. [Aloisio, A.; Alviggi, M. G.; Canalea, V.; Carlino, G.; Cooke, M.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] INFN Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.] Univ Napoli, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Cheplakov, A.; Colasurdo, L.; De Groot, N.; Filthaut, F.; Galea, C.; Konig, A. C.; Maio, A.; Nektarijevic, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zhang, D.; Zhao, X.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zhang, D.; Zhao, X.] CNRS, IN2P3, Orsay, France. [Endo, M.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhou, B.] Univ Oxford, Dept Phys, Oxford, England. INFN Sez Pavia, Pavia, Italy. Univ Pavia, Dipartimento Fis, Pavia, Italy. [Brendlinger, K.; Fletcher, R. R. M.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Reichert, J.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Natl Res Ctr Kurchatov Inst BP Konstantinov, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.] INFN Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Hong, T. M.; Lee, C. A.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorima, A.; Araque, J. P.] Lab Instrumentacao Fis Expt Particulas LIP, Lisbon, Portugal. [Amorima, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.] Univ Coimbra, Dept Phys, Coimbra, Portugal. Univ Lisbon, Ctr Fis Nucl, Lisbon, Portugal. Univ Minho, Dept Fis, Braga, Portugal. Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zenis, T.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.] INFN Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.] Univ Roma La Sapienza, Dipartimento Fis, Rome, Italy. [Aielli, G.] INFN Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.] Univ Roma Tor Vergata, Dipartimento Fis, Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.] INFN Sez Roma Tre, Rome, Italy. [Bacci, C.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. Univ Mohamed Premier, Fac Sci, Oujda, Morocco. LPTPM, Oujda, Morocco. Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay Commissariat Energie Atom & Energes Al, DSM IRFU Inst Rech Lois Fondament Univers, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys1, Burnaby, BC, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.] Slovak Acad Sci, Inst Expt Phys, Dept Subnuclear Phys, Kosice, Slovakia. Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylunda, O. Bessidskaia; Bohm, C.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylunda, O. Bessidskaia; Petridis, A.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Astron & Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Lerner, G.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; LoSterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, Thessaloniki, Greece. [Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.] Tokyo Inst Technol, Dept Phys, Tokyo, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. TRIUMF, Vancouver, BC, Canada. [Garcia, J. A. Benitez] York Univ, Dept Phys & Astron, Toronto, ON, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.] INFN Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.] Univ Udine, Dipartimento Chim Fis & Ambiente, Udine, Italy. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Gradin, P. O. J.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Alvarez Piqueras, D.; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garc-A, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garc-A, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garc-A, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Alvarez Piqueras, D.; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garc-A, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, IMB CNM, Valencia, Spain. [Alvarez Piqueras, D.; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garc-A, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Swedish, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.; Trovatelli, M.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, Rehovot, Israel. [Banerjee, Sw.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kaplan, L. S.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, H.; Zobernig, G.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Strohmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, Wurzburg, Germany. [Bannoura, A. A. E.; Beermann, T. A.; Braun, H. M.; Cornelissen, T.; Ellinghaus, F.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Mattig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Thomsen, L. A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.; Zhao, Z.] Yerevan Phys Inst, Yerevan, Armenia. [Rahal, G.] Inst Natl Phys Nucl & Phys Particules IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.; Alberghi, G. L.; Aloisio, A.; Annovi, A.; Barberis, D.; Bellagamba, L.; Biondi, S.; Bortolotto, V.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Cairo, V. M.; Calobaa, L. P.; Camarri, P.; Canalea, V.; Canepaa, A.; Cantrill, R.; Caprinia, I.; Caprini, M.; Capua, M.; Cardarelli, R.; Carlino, G.; Carminati, L.; Carquin, E.; Carvalho, J.; Castro, N. F.; Cavallia, D.; Cavasinni, V.; Ceradini, F.; Chafaq, A.; Chekulaev, S. V.; Chiarelli, G.; Chiodini, G.; Chitan, A.; Ciapetti, G.; Ciftci, A. K.; Ciubancan, M.; Clement, C.; Cobal, M.; Muino, P. Conde; Consonni, S. M.; Constantinescu, S.; Conta, C.; Conti, G.; Cooke, M.; Corradi, M.; Costa, G.; Cribbs, W. A.; Crosetti, G.; De Sousa, M. J. Da Cunha Sargedas; Dabrowski, W.; Darbo, G.; Davygora, Y.; de Asmundis, R.; DeCastro, S.; De Pedis, D.; De Salvo, A.; Del Prete, T.; Dell'Orso, M.; Della Pietra, M.; Di Ciaccio, A.; Di Domenico, A.; Di Donato, C.; Di Micco, B.; Diaz, M. A.; Dita, P.; Dita, S.; Djuvsland, J. I.; Dobre, M.; Donati, S.; Dondero, P.; Doria, A.; Ducu, O. A.; Dunford, M.; Yildiz, H. Duran; Dyndal, M.; Fabbri, L.; Falciano, S.; Fang, Y.; Fanti, M.; Farilla, A.; Favareto, A.; Federic, P.; Ferrari, R.; Parodi, A. Ferretto; Fiolhais, M. C. N.; Castillo, L. R. Flores; Franchini, M.; Fraternali, M.; Gabrielli, A.; Gabrielli, A.; Gach, G. P.; Gagliardi, G.; Galhardo, B.; Gaudiello, A.; Gaudio, G.; Gauzzi, P.; Geisler, M. P.; Gemme, C.; Gentile, S.; Giacobbe, B.; Giagu, S.; Giannetti, P.; Giordani, M. P.; Giorgia, F. M.; Giugni, D.; Gomes, A.; Goncalo, R.; Gorini, E.; Grabowska-Bold, I.; Grafstrom, P.; Graziani, E.; Guido, E.; Gustavino, G.; Hamilton, A.; Hanke, P.; Hellman, S.; Hoummadaa, A.; Introzzi, G.; Iodice, M.; Istin, S.; Iuppa, R.; Izzo, V.; Jejelava, J.; Jin, S.; Jinaru, A.; Jon-And, K.; Jongmanns, J.; Jorge, P. M.; Jovicevic, J.; Khandanyan, H.; Kim, H.; Kisielewska, D.; Klimek, P.; Kluge, E. -E.; Koperny, S.; Koutsman, A.; Kowalski, T. Z.; Kuna, M.; La Rotonda, L.; Lacava, F.; Lang, V. S.; Lanza, A.; Lari, T.; Manghi, F. Lasagni; Leone, S.; Liberti, B.; Liu, B.; Livan, M.; Lopes, L.; Lou, X.; Luci, C.; Luminari, L.; Lundberg, O.; Maidantchik, C.; Maio, A.; Mandelli, L.; Maneira, J.; Marroquim, F.; Martoiu, V. S.; Marzano, F.; Massa, I.; Massa, L.; Mastroberardino, A.; Maurer, J.; Mazza, S. M.; Mazzaferro, L.; Meehan, S.; Meier, K.; Mengarelli, A.; Merola, L.; Meroni, C.; Messina, A.; Miglioranzi, S.; Milstead, D. A.; Mindur, B.; Moa, T.; Molander, S.; Monzani, S.; Morettini, P.; Myagkov, A. G.; Negri, A.; Negrini, M.; Nepomuceno, A. A.; Nessi, M.; Nikolaenko, V.; Nisati, A.; Ochoa-Ricoux, J. P.; Olariu, A.; Onofre, A.; Oram, C. J.; Orestano, D.; Osculati, B.; Ouyang, Q.; Ozcan, V. E.; Palma, A.; Pani, P.; Pantea, D.; Parodi, F.; Pasqualucci, E.; Passaggio, S.; Pastore, F.; Pedro, R.; Peng, C.; Codina, E. Perez; Perini, L.; Perrella, S.; Petridis, A.; Petrolo, E.; Petrucci, F.; Piccinini, M.; Pina, J.; Pinamonti, M.; Pinto, B.; Pizio, C.; Plazak, L.; Plucinski, P.; Poettgen, R.; Polesello, G.; Policicchio, A.; Polini, A.; Pontecorvo, L.; Popeneciu, G. A.; Primavera, M.; Przybycien, M.; Puddu, D.; Purohit, M.; Quayle, W. B.; Ragusa, F.; Rebuzzi, D. M.; Ren, H.; Rescigno, M.; Resconi, S.; Rimoldi, A.; Rinaldi, L.; Roda, C.; Romano, M.; Rosati, S.; Rossetti, V.; Rossi, E.; Rossi, L. P.; Rotaru, M.; Tehrani, F. 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[Hanagaki, K.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Tsinghua, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Jenni, P.] CERN, Geneva, Switzerland. [Khubua, J.] GTU, Tbilisi, Rep of Georgia. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellenic Open Univ, Patras, Greece. [Li, B.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Li, Y.] Univ Paris 11, LAL, Orsay, France. [Li, Y.] CNRS, IN2P3, Orsay, France. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Liu, B.] Shandong Univ, Sch Phys, Shandong, Peoples R China. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] M Lomonosov Moscow State Univ, Fac Phys, Moscow, Russia. [Tikhomirov, V. O.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Xu, L.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Tikhomirov, Vladimir/M-6194-2015; Kuday, Sinan/C-8528-2014; Tartarelli, Giuseppe Francesco/A-5629-2016; la rotonda, laura/B-4028-2016; Doyle, Anthony/C-5889-2009; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Owen, Mark/Q-8268-2016; Mashinistov, Ruslan/M-8356-2015; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Chekulaev, Sergey/O-1145-2015; Gerbaudo, Davide/J-4536-2012; Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Monzani, Simone/D-6328-2017; Maleev, Victor/R-4140-2016; Guo, Jun/O-5202-2015; Warburton, Andreas/N-8028-2013; Maneira, Jose/D-8486-2011; Gladilin, Leonid/B-5226-2011; Prokoshin, Fedor/E-2795-2012; Di Domenico, Antonio/G-6301-2011; Brooks, William/C-8636-2013; Boyko, Igor/J-3659-2013; Staroba, Pavel/G-8850-2014; Gavrilenko, Igor/M-8260-2015; Gauzzi, Paolo/D-2615-2009; OI Castro, Nuno/0000-0001-8491-4376; Li, Liang/0000-0001-6411-6107; Farrington, Sinead/0000-0001-5350-9271; Robson, Aidan/0000-0002-1659-8284; Prokofiev, Kirill/0000-0002-2177-6401; Veneziano, Stefano/0000-0002-2598-2659; Lacasta, Carlos/0000-0002-2623-6252; Smirnova, Oxana/0000-0003-2517-531X; Price, Darren/0000-0003-2750-9977; Terzo, Stefano/0000-0003-3388-3906; Smirnov, Sergei/0000-0002-6778-073X; Tikhomirov, Vladimir/0000-0002-9634-0581; Kuday, Sinan/0000-0002-0116-5494; Dell'Asta, Lidia/0000-0002-9601-4225; Sannino, Mario/0000-0001-7700-8383; Della Volpe, Domenico/0000-0001-8530-7447; KUBOTA, TAKASHI/0000-0002-1156-5571; Vari, Riccardo/0000-0002-2814-1337; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Gray, Heather/0000-0002-5293-4716; la rotonda, laura/0000-0002-6780-5829; Coccaro, Andrea/0000-0003-2368-4559; Doyle, Anthony/0000-0001-6322-6195; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Owen, Mark/0000-0001-6820-0488; Mashinistov, Ruslan/0000-0001-7925-4676; Fabbri, Laura/0000-0002-4002-8353; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Monzani, Simone/0000-0002-0479-2207; Guo, Jun/0000-0001-8125-9433; Warburton, Andreas/0000-0002-2298-7315; Maneira, Jose/0000-0002-3222-2738; Gladilin, Leonid/0000-0001-9422-8636; Prokoshin, Fedor/0000-0001-6389-5399; Di Domenico, Antonio/0000-0001-8078-2759; Brooks, William/0000-0001-6161-3570; Boyko, Igor/0000-0002-3355-4662; Gauzzi, Paolo/0000-0003-4841-5822; Belanger-Champagne, Camille/0000-0003-2368-2617 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; RGC, Hong Kong SAR, China; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia; NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, UK; Royal Society, UK; Leverhulme Trust, UK; DOE, USA; NSF, USA FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; RGC, Hong Kong SAR, China; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, UK; DOE and NSF, USA. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 132 TC 12 Z9 12 U1 16 U2 39 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD OCT 29 PY 2015 VL 75 IS 10 AR 510 DI 10.1140/epjc/s10052-015-3726-9 PG 48 WC Physics, Particles & Fields SC Physics GA DQ9FI UT WOS:000379515400001 PM 26549981 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Ochesanu, S Rougny, R Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Daci, N Heracleous, N Keaveney, J Lowette, S Maes, M Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Dobur, D Favart, L Gay, 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Taylor, D. Vuosalo, C. Woods, N. TI Measurements of the ZZ production cross sections in the 2l2 nu channel in proton-proton collisions at root s=7 and 8 TeV and combined constraints on triple gauge couplings SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article AB Measurements of the ZZ production cross sections in proton-proton collisions at center-of-mass energies of 7 and 8 TeV are presented. Candidate events for the leptonic decay mode ZZ -> 2l2 nu. where l denotes an electron or a muon, are reconstructed and selected from data corresponding to an integrated luminosity of 5.1 (19.6) fb(-1) at 7 (8) TeV collected with the CMS experiment. The measured cross sections, sigma(pp -> ZZ) = 5.1(1.4)(+1.5) (stat)(-1.1)(+1.4) (syst) +/- 0.1 (lumi) pb at 7 TeV, and 7.2(-0.8)(+0.8) (stat)(1.5)(+1.9) (syst) +/- 0.2 (lumi) pb at 8 TeV, are in good agreement with the standard model predictions with next-to-leading-order accuracy. The selected data are analyzed to search for anomalous triple gauge couplings involving the ZZ final state. In the absence of any deviation from the standard model predictions, limits are set on the relevant parameters. These limits are then combined with the previously published CMS results for ZZ in 4l final states, yielding the most stringent constraints on the anomalous couplings. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hartl, C.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Kiesenhofer, W.; Knuenz, V.; Krammer, M.; Kraetschmer, I.; Liko, D.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, H.; Schoefbeck, R.; Strauss, J.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] Inst Hochenergiephy OeAW, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. 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[Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Soffi, L.; Traczyk, P.] INFN Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Longo, E.; Margaroli, F.; Micheli, F.; Organtini, G.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Univ Roma, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; De Remigis, P.; Degano, A.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] INFN Sez Torino, Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Finco, L.; Migliore, E.; Monaco, V.; Pacher, L.; Angioni, G. L. Pinna; Romero, A.; Sacchi, R.; Solano, A.] Univ Torino, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.; Zanetti, A.] INFN Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Daegu, South Korea. [Kim, T. J.] Chonbuk Natl Univ, Jeonju, South Korea. [Kim, J. Y.; Moon, D. H.; Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, I. C.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania. [Komaragiri, J. R.; Ali, M. A. B. Md] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] Ctr Invest & Estudios Avanzados IPN, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Golutvin, I.; Karjavin, V.; Konoplyanikov, V.; Korenkov, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Matveev, V.; Mitsyn, V. V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Tikhonenko, E.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow, Russia. [Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys & Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] Ctr Invest Energet Medioambient & Tecnol CIEMAT, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] CSIC Univ Cantabria, Inst Fis Cantabria IFCA, Santander, Spain. [Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Marrouche, J.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Orsini, L.; Pape, L.; Perez, E.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pimia, M.; Piparo, D.; Plagge, M.; Racz, A.; Rolandi, G.; Rovere, M.; Sakulin, H.; Schafer, C.; Schwick, C.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Tsirou, A.; Veres, G. I.; Wardle, N.; Wohri, H. K.; Wollny, H.; Zeuner, W. D.] CERN, European Org Nucl Res, Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Bani, L.; Bianchini, L.; Buchmann, M. A.; Casal, B.; Chanon, N.; Dissertori, G.; Dittmar, M.; Donega, M.; Dunser, M.; Eller, P.; Grab, C.; Hits, D.; Hoss, J.; Lustermann, W.; Mangano, B.; Marini, A. C.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Mohr, N.; Musella, P.; Nageli, C.; Nessi-Tedaldi, F.; Pandolfi, F.; Pauss, F.; Perrozzi, L.; Peruzzi, M.; Quittnat, M.; Rebane, L.; Rossini, M.; Starodumov, A.; Takahashi, M.; Theofilatos, K.; Wallny, R.; Weber, H. A.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Mejias, B. Millan; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli, Taiwan. [Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Kao, K. Y.; Liu, Y. F.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Tzeng, Y. M.; Wilken, R.] NTU, Taipei, Taiwan. [Asavapibhop, B.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Dept Phys, Fac Sci, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Gamsizkan, H.; Isildak, B.; Karapinar, G.; Ocalan, K.; Sekmen, S.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle East Tech Univ, Dept Phys, Ankara, Turkey. [Albayrak, E. A.; Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Vardarli, F. I.] Istanbul Tech Univ, Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Branca, A.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-storey, S. Seif; Senkin, S.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Dauncey, P.; Davies, G.; Della Negra, M.; Dunne, P.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Mathias, B.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Lawson, P.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.] Boston Univ, Boston, MA USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Rikova, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Kovalskyi, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tu, Y.; Vartak, A.; Welke, C.; Wurthwein, F.; Yagil, A.] Univ Calif San Diego, San Diego, CA USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Incandela, J.; Justus, C.; Mccoll, N.; Richman, J.; Stuart, D.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA USA. [Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA USA. [Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Krohn, M.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Skinnari, L.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Grunendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kreis, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Sharma, S.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Yang, F.] Fermilab Natl Accelerator Lab, Batavia, IL USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carver, M.; Curry, D.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Field, R. D.; Fisher, M.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Snowball, M.; Sperka, D.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL USA. [Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL USA. [Baarmand, M. M.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Haytmyradov, M.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Gray, J.; Kenny, R. P., III; Malek, M.; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS USA. [Chakaberia, I.; Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Skhirtladze, N.; Svintradze, I.] Kansas State Univ, Manhattan, KS USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Belloni, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD USA. [Apyan, A.; Barbieri, R.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Nourbakhsh, S.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Ratnikov, F.; Snow, G. R.; Zvada, M.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; Trocino, D.; Wang, R. J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Lynch, S.; Marinelli, N.; Musienko, Y.; Pearson, T.; Planer, M.; Ruchti, R.; Smith, G.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH USA. 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[Popov, A.; Zhukov, V.; Katkov, I.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, Brazil. [Plestina, R.] CNRS, Lab Leprince Ringuet, Ecole Polytechn, IN2P3, Palaiseau, France. [Finger, M., Jr.; Tsamalaidze, Z.] Joint Inst Nucl Res, Dubna, Russia. [Assran, Y.] Suez Univ, Suez, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Radi, A.] British Univ Egypt, Cairo, Egypt. [Radi, A.] Ain Shams Univ, Cairo, Egypt. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Hempel, M.; Lohmann, W.; Marfin, I.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Horvath, D.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Karancsi, J.] Univ Debrecen, Debrecen, Hungary. [Bhowmik, S.; Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. 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[Sphicas, P.] Univ Athens, Athens, Greece. [Nageli, C.; Starodumov, A.] Paul Scherrer Inst, Villigen, Switzerland. [Nikitenko, A.] Inst Theoret & Expt Phys, Moscow, Russia. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.; Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Gamsizkan, H.] Anadolu Univ, Eskisehir, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Ocalan, K.] Necmettin Erbakan Univ, Konya, Turkey. [Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. Marmara Univ, Istanbul, Turkey. [Kaya, M.; Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, T.] Yildiz Tech Univ, Istanbul, Turkey. [Newbold, D. M.; Lucas, R.] Rutherford Appleton Lab, Didcot, Oxon, England. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Milenovic, P.] Univ Belgrade, Vinca Inst Nucl Sci, Fac Phys, Belgrade, Serbia. [Bilki, B.] Argonne Natl Lab, Argonne, IL USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Bouhali, O.] Texas A&M Univ, Doha, Qatar. [Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan, Armenia. RI TUVE', Cristina/P-3933-2015; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Sznajder, Andre/L-1621-2016; Vilela Pereira, Antonio/L-4142-2016; Della Ricca, Giuseppe/B-6826-2013; Lokhtin, Igor/D-7004-2012; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Vogel, Helmut/N-8882-2014; Paulini, Manfred/N-7794-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Manganote, Edmilson/K-8251-2013; Dremin, Igor/K-8053-2015; ciocci, maria agnese /I-2153-2015; Kirakosyan, Martin/N-2701-2015; Benussi, Luigi/O-9684-2014; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Ruiz, Alberto/E-4473-2011; Petrushanko, Sergey/D-6880-2012; Dudko, Lev/D-7127-2012; Govoni, Pietro/K-9619-2016; Andreev, Vladimir/M-8665-2015; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013 OI TUVE', Cristina/0000-0003-0739-3153; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Sznajder, Andre/0000-0001-6998-1108; Vilela Pereira, Antonio/0000-0003-3177-4626; Della Ricca, Giuseppe/0000-0003-2831-6982; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Vogel, Helmut/0000-0002-6109-3023; Paulini, Manfred/0000-0002-6714-5787; ciocci, maria agnese /0000-0003-0002-5462; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Ruiz, Alberto/0000-0002-3639-0368; Dudko, Lev/0000-0002-4462-3192; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; FU Austrian Federal Ministry of Science, Research and Economy; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; CNPq; CAPES; FAPERJ; FAPESP; Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research; Estonian Research Council [IUT23-4, IUT236]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules/CNRS; Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; Bundesministerium fur Bildung und Forschung; Deutsche Forschungsgemeinschaft; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation, Hungary; National Innovation Office, Hungary; Department of Atomic Energy, India; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Ministry of Science, ICT and Future Planning, Republic of Korea; National Research Foundation (NRF), Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education, Malaysia; University of Malaya (Malaysia); CINVESTAV; CONACYT; SEP; UASLP-FAI; Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education, Poland; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion; Desarrollo e Innovacion; Programa Consolider-Ingenio, Spain; ETH Board; ETH Zurich; PSI; SNF; UniZH; Canton Zurich; SER; Ministry of Science and Technology, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine; State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, UK; US Department of Energy; US National Science Foundation; Marie-Curie program; European Research Council; EPLANET(European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS program of Foundation for Polish Science - European Union, Regional Development Fund; Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR (Italy) [20108T4XTM]; Thalis program - EU-ESF; Aristeia program - EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund FX We wish to thank our theoretician colleague Tobias Kasprzik for providing the numerical calculations of the next-to-leading-order electroweak corrections to the ZZ and WZ processes. We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses.; Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via IUT23-4 and IUT236 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules/CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Ministry of Science, ICT and Future Planning, and National Research Foundation (NRF), Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine, and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, UK; the US Department of Energy, and the US National Science Foundation. Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET(European Union); the Leventis Foundation; the A. P.; Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR Project 20108T4XTM (Italy); the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF; and the National Priorities Research Program by Qatar National Research Fund. NR 41 TC 2 Z9 2 U1 16 U2 33 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD OCT 29 PY 2015 VL 75 IS 10 AR 511 DI 10.1140/epjc/s10052-015-3706-0 PG 26 WC Physics, Particles & Fields SC Physics GA DQ9FI UT WOS:000379515400002 ER PT J AU Lohmiller, T Shelby, ML Long, X Yachandra, VK Yano, JK AF Lohmiller, Thomas Shelby, Megan L. Long, Xi Yachandra, Vittal K. Yano, Junko TI Removal of Ca2+ from the Oxygen-Evolving Complex in Photosystem II Has Minimal Effect on the Mn4O5 Core Structure: A Polarized Mn X-ray Absorption Spectroscopy Study SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID ELECTRON-PARAMAGNETIC-RES; PHOTOSYNTHETIC WATER OXIDATION; O BOND FORMATION; MANGANESE COMPLEX; MN4CA CLUSTER; S-2 STATE; SPINACH-CHLOROPLASTS; O-2-EVOLVING COMPLEX; CENTERED OXIDATION; MEMBRANE-PARTICLES AB Ca2+-depleted and Ca2+-reconstituted spinach photosystem II was studied using polarized X-ray absorption spectroscopy of oriented PS II preparations to investigate the structural and functional role of the Ca2+ ion in the Mn4O5Ca cluster of the oxygen-evolving complex (OEC). Samples were prepared by low pH/citrate treatment as one-dimensionally ordered membrane layers and poised in the Ca-2-depleted S-1 (S-1') and S-2 (S-2') states, the S-2'Y-z(center dot) state, at which point the catalytic cycle of water oxidation is inhibited, and the Ca2+-reconstituted S-1 state. Polarized Mn K-edge XANES and EXAFS spectra exhibit pronounced dichroism. Polarized EXAFS data of all states of Ca2+ depleted PS II investigated show only minor changes in distances and orientations of the Mn Mn vectors compared to the Ca2+-containing OEC, 3 which may be attributed to some loss of rigidity of the core structure. Thus, removal of the Ca2+ ion does not lead to fundamental distortion or rearrangement of the tetranudear Mn cluster, which indicates that the Ca2+ ion in the OEC is not critical for structural maintenance of the cluster, at least in the S-1 and S-2 states, but fulfills a crucial catalytic function in the mechanism of the water oxidation reaction. On the basis of this structural information, reasons for the inhibitory effect of Ca2+ removal are discussed, attributing to the Ca2+ ion a fundamental role in organizing the surrounding (substrate) water framework and in proton-coupled electron transfer to Y-z(center dot) (D1-Tyr161). C1 [Lohmiller, Thomas; Shelby, Megan L.; Long, Xi; Yachandra, Vittal K.; Yano, Junko] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Yachandra, VK (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. EM vkyachandra@lbl.gov; jyano@lbl.gov FU NIH [GM 55302]; Office of Science, Office of Basic Energy Sciences (OBES), Division of Chemical Sciences, Geosciences, and Biosciences of the Department of Energy (DOE) [DE-AC02-05CH11231]; NIH National Center for Research Resources, Biomedical Technology Program; DOE Office of Biological and Environmental Research; DOE Office of Basic Energy Science FX This work was supported by the NIH Grant GM 55302, and by the Director, Office of Science, Office of Basic Energy Sciences (OBES), Division of Chemical Sciences, Geosciences, and Biosciences of the Department of Energy (DOE) under Contract DE-AC02-05CH11231. This work was performed at SSRL, which is funded by the DOE Office of Basic Energy Science. The SSRL SMB Program is supported by the NIH National Center for Research Resources, Biomedical Technology Program, and by the DOE Office of Biological and Environmental Research. NR 85 TC 7 Z9 7 U1 4 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD OCT 29 PY 2015 VL 119 IS 43 BP 13742 EP 13754 DI 10.1021/acs.jpcb.5b03559 PG 13 WC Chemistry, Physical SC Chemistry GA CV1DQ UT WOS:000363994000031 PM 25989608 ER PT J AU Poluektov, OG Utschig, LM AF Poluektov, Oleg G. Utschig, Lisa M. TI Directionality of Electron Transfer in Type I Reaction Center Proteins: High-Frequency EPR Study of PS I with Removed Iron-Sulfur Centers SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID CYANOBACTERIAL PHOTOSYSTEM-I; CRYOGENIC TEMPERATURES; HYDROGEN-PRODUCTION; CHARGE SEPARATION; CRYSTAL-STRUCTURE; ACCEPTOR A(0); RESOLUTION; BRANCHES; PAIR; SIDE AB A key step of photosynthetic solar energy conversion involves rapid light-induced sequential electron-transfer steps that result in the formation of a stabilized charge-separated state. These primary reactions take place in large integral membrane reaction center (RC) proteins, wherein a series of donor/acceptor cofactors are specifically positioned for efficient electron transfer. RCs can be divided in two classes, Type I and Type II and examples of both types, photosystem I (PS I) and photosystem II (PS II), are involved in the oxygenic photosynthesis of higher plants, cyanobacteria, and algae. High-resolution X-ray crystal structures reveal that PS I and PS II contain two nearly symmetric branches of redox cofactors, termed the A and B branches. While unidirectional ET along the A branch in Type II RCs is well established, there is still a debate of whether primary photochemistry in Type I RCs is unidirectional along the A branch or bidirectional proceeding down both of the A and B branches. Light-induced electron transfer through the B branch has been observed in genetically modified PS I and in native PS I pretreated with strong reducing conditions to reduce three [4Fe-4S] clusters, the terminal electron acceptors of PS I; however, the extent of asymmetry of ET along both cofactor branches remains an open question. To prove that bidirectional ET in PS I is not simply an artifact of a reducing environment or genetic modification and to determine the degree of PS I ET asymmetry, we have examined biochemically modified Synechococcus leopoliensis PS I RCs, wherein the [4Fe-4S] clusters F-X, F-A, and F-B have been removed to prevent secondary ET from phylloquinones (A(1A)/A(1B)) to F-X. For these Fe-removed proteins, we observe that ET along both the A and B branches occurs with a ratio close to 1. Together with previously reported data, the concomitant structural and kinetic information obtained with HF EPR unambiguously proves the bidirectional nature of ET in PS I over a broad temperature range. C1 [Poluektov, Oleg G.; Utschig, Lisa M.] Argonne Natl Lab, Dept Chem Sci & Engn, Argonne, IL 60439 USA. RP Poluektov, OG (reprint author), Argonne Natl Lab, Dept Chem Sci & Engn, 9700 S Cass Ave, Argonne, IL 60439 USA. EM oleg@anl.gov FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences at Argonne National Laboratory [DE-AC02-06CH11357] FX This material is based on work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, under contract number DE-AC02-06CH11357 at Argonne National Laboratory. NR 41 TC 0 Z9 0 U1 3 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD OCT 29 PY 2015 VL 119 IS 43 BP 13771 EP 13776 DI 10.1021/acs.jpcb.5b04063 PG 6 WC Chemistry, Physical SC Chemistry GA CV1DQ UT WOS:000363994000034 PM 26029974 ER PT J AU Hu, S Lewis, NS Ager, JW Yang, JH McKone, JR Strandwitz, NC AF Hu, Shu Lewis, Nathan S. Ager, Joel W. Yang, Jinhui McKone, James R. Strandwitz, Nicholas C. TI Thin-Film Materials for the Protection of Semiconducting Photoelectrodes in Solar-Fuel Generators SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Review ID ATOMIC LAYER DEPOSITION; VISIBLE-LIGHT IRRADIATION; MICROWIRE-ARRAY PHOTOCATHODES; JUNCTION SILICON ELECTRODES; OXYNITRIDE TAON PHOTOANODE; DRIVEN WATER OXIDATION; HYDROGEN-PRODUCTION; ENERGY-CONVERSION; EFFICIENT SOLAR; N-TYPE AB The electrochemical instability of semiconductors in aqueous electrolytes has impeded the development of robust sunlight-driven water-splitting systems. We review the use of protective thin films to improve the electrochemical stability of otherwise unstable semiconductor photoelectrodes (e.g., Si and GaAs). We first discuss the origins of instability and various strategies for achieving stable and functional photoelectrosynthetic interfaces. We then focus specifically on the use of thin protective films on photoanodes and photocathodes for photosynthetic reactions that include oxygen evolution, halide oxidation, and hydrogen evolution. Finally, we provide an outlook for the future development of thin-layer protection strategies to enable semiconductor-based solar-driven fuel production. C1 [Hu, Shu; Lewis, Nathan S.] CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA. [Hu, Shu; Lewis, Nathan S.] CALTECH, Joint Ctr Artificial Photosynth, Pasadena, CA 91125 USA. [Lewis, Nathan S.] CALTECH, Beckman Inst, Pasadena, CA 91125 USA. [Lewis, Nathan S.] CALTECH, Kavli Nanosci Inst, Pasadena, CA 91125 USA. [Ager, Joel W.; Yang, Jinhui] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. [Ager, Joel W.; Yang, Jinhui] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Sci Mat, Berkeley, CA 94720 USA. [McKone, James R.] Cornell Univ, Dept Chem & Biol Chem, Ithaca, NY 14853 USA. [Strandwitz, Nicholas C.] Lehigh Univ, Dept Mat Sci & Engn, Bethlehem, PA 18015 USA. [Strandwitz, Nicholas C.] Lehigh Univ, Ctr Adv Mat & Nanotechnol, Bethlehem, PA 18015 USA. RP Lewis, NS (reprint author), CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA. EM nslewis@caltech.edu; strand@lehigh.edu RI Hu, Shu/B-8120-2013 FU Lehigh University; U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy through the Sun Shot Initiative; Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub; Office of Science of the U.S. Department of Energy [DE-SC0004993]; National Science Foundation [CHE-I214152]; Department of Energy, Office of Basic Energy Sciences [DE-FG02-03ER15483]; Gordon and Betty Moore Foundation [GBMF1225] FX NCS acknowledges start-up funds from Lehigh University. JRM acknowledges a postdoctoral research award from the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy through the Sun Shot Initiative. SH, NSL, JWA, and JY were supported by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under Award Number DE-SC0004993, and NSL was also supported by the National Science Foundation under Award Number CHE-I214152, the Department of Energy, Office of Basic Energy Sciences under Award Number DE-FG02-03ER15483, and the Gordon and Betty Moore Foundation under Award Number GBMF1225. NR 222 TC 32 Z9 32 U1 30 U2 122 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 29 PY 2015 VL 119 IS 43 BP 24201 EP 24228 DI 10.1021/acs.jpcc.5b05976 PG 28 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CV1DU UT WOS:000363994500001 ER PT J AU Shearer, AJ Suich, DE Caplins, BW Harris, CB AF Shearer, Alex J. Suich, David E. Caplins, Benjamin W. Harris, Charles B. TI Impact of Film Thickness and Temperature on Ultrafast Excess Charge Dynamics in Ionic Liquid Films SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID COMPLETE SOLVATION RESPONSE; ELECTRON SOLVATION; HYDRATED ELECTRON; GREEN SOLVENTS; INTERFACES; FEMTOSECOND; SUPERCAPACITORS; PHOTODETACHMENT; SPECTROSCOPY; EXCITATION AB Ultrafast response of the room temperature ionic liquid (RTIL) 1-butyl-1-methylpyrrolidinium bis-(trifiuoromethylsulfonyl)imide ([Bmpyr][NTf2]) to a photo-injected electron is investigated in few-monolayer films using time- and angle-resolved two-photon photoemission spectroscopy. A delocalized precursor state and a localized solvated state were resolved at early times, but after 200 fs only a single solvated state was observed. The dynamics of film response to this solvated state were shown to depend significantly on film temperature and thickness. Population lifetime measurements demonstrated that the RTIL film can significantly affect the coupling between solvated state and metal substrate, as the solvated state's average lifetime increased from 90 +/- 20 fs in 1 ML films to 195 +/- 83 ps in 3 ML films. Additionally, a temperature dependence of the time-dependent binding energy shift of the solvated state after ca. 500 fs was attributed to a phase change occurring between the two temperature regimes that were investigated. Results from xenon overlayer experiments suggest that the solvation process occurs near the surface of the RTIL film. Finally, film degradation was found to be present, suggesting that the observed solvation response could involve a radical species. C1 [Shearer, Alex J.; Suich, David E.; Caplins, Benjamin W.; Harris, Charles B.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Shearer, Alex J.; Suich, David E.; Caplins, Benjamin W.; Harris, Charles B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Harris, CB (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM cbharris@berkeley.edu FU Office of Science, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy, under Contract No. DE-AC02-05CH11231. NR 62 TC 0 Z9 0 U1 8 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 29 PY 2015 VL 119 IS 43 BP 24417 EP 24424 DI 10.1021/acs.jpcc.5b07262 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CV1DU UT WOS:000363994500024 ER PT J AU Chen, XW Shekiro, J Pschorn, T Sabourin, M Tucker, MP Tao, L AF Chen, Xiaowen Shekiro, Joseph Pschorn, Thomas Sabourin, Marc Tucker, Melvin P. Tao, Ling TI Techno-economic analysis of the deacetylation and disk refining process: characterizing the effect of refining energy and enzyme usage on minimum sugar selling price and minimum ethanol selling price SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Biofuel; Pretreatment; Enzymatic hydrolysis; Deacetylation; Mechanical refining; Disk refining; No acid pretreatment; Clean sugar production AB Background: A novel, highly efficient deacetylation and disk refining (DDR) process to liberate fermentable sugars from biomass was recently developed at the National Renewable Energy Laboratory (NREL). The DDR process consists of a mild, dilute alkaline deacetylation step followed by low-energy-consumption disk refining. The DDR corn stover substrates achieved high process sugar conversion yields, at low to modest enzyme loadings, and also produced high sugar concentration syrups at high initial insoluble solid loadings. The sugar syrups derived from corn stover are highly fermentable due to low concentrations of fermentation inhibitors. The objective of this work is to evaluate the economic feasibility of the DDR process through a techno-economic analysis (TEA). Results: A large array of experiments designed using a response surface methodology was carried out to investigate the two major cost-driven operational parameters of the novel DDR process: refining energy and enzyme loadings. The boundary conditions for refining energy (128-468 kWh/ODMT), cellulase (Novozyme's CTec3) loading (11.6-28.4 mg total protein/g of cellulose), and hemicellulase (Novozyme's HTec3) loading (0-5 mg total protein/g of cellulose) were chosen to cover the most commercially practical operating conditions. The sugar and ethanol yields were modeled with good adequacy, showing a positive linear correlation between those yields and refining energy and enzyme loadings. The ethanol yields ranged from 77 to 89 gallons/ODMT of corn stover. The minimum sugar selling price (MSSP) ranged from $0.191 to $0.212 per lb of 50 % concentrated monomeric sugars, while the minimum ethanol selling price (MESP) ranged from $2.24 to $2.54 per gallon of ethanol. Conclusions: The DDR process concept is evaluated for economic feasibility through TEA. The MSSP and MESP of the DDR process falls within a range similar to that found with the deacetylation/dilute acid pretreatment process modeled in NREL's 2011 design report. The DDR process is a much simpler process that requires less capital and maintenance costs when compared to conventional chemical pretreatments with pressure vessels. As a result, we feel the DDR process should be considered as an option for future biorefineries with great potential to be more cost-effective. C1 [Chen, Xiaowen; Shekiro, Joseph; Tucker, Melvin P.; Tao, Ling] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80127 USA. [Pschorn, Thomas; Sabourin, Marc] Andritz Inc, Springfield, OH USA. RP Chen, XW (reprint author), Natl Renewable Energy Lab, Natl Bioenergy Ctr, 1617 Cole Blvd, Golden, CO 80127 USA. EM Xiaowen.Chen@nrel.gov; Ling.Tao@nrel.gov FU BETO program in DOE EERE FX We would like to acknowledge the funding support from BETO program in DOE EERE. We also want to thank the NREL Biomass Analytical Team for their technical assistance and analysis. NR 16 TC 4 Z9 4 U1 9 U2 15 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD OCT 29 PY 2015 VL 8 AR 173 DI 10.1186/s13068-015-0358-0 PG 13 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA CU7RE UT WOS:000363738300001 PM 26516346 ER PT J AU Crabtree, G AF Crabtree, George TI The energy-storage revolution SO NATURE LA English DT Editorial Material C1 [Crabtree, George] Argonne Natl Lab, Joint Ctr Energy Storage Res, Argonne, IL 60439 USA. [Crabtree, George] Univ Illinois, Chicago, IL USA. RP Crabtree, G (reprint author), Argonne Natl Lab, Joint Ctr Energy Storage Res, Argonne, IL 60439 USA. EM crabtree@anl.gov NR 0 TC 11 Z9 12 U1 12 U2 32 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD OCT 29 PY 2015 VL 526 IS 7575 BP S92 EP S92 PG 1 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CU8ZH UT WOS:000363832100024 PM 26509952 ER PT J AU Posen, S Transtrum, MK Catelani, G Liepe, MU Sethna, JP AF Posen, Sam Transtrum, Mark K. Catelani, Gianluigi Liepe, Matthias U. Sethna, James P. TI Shielding Superconductors with Thin Films as Applied to rf Cavities for Particle Accelerators SO PHYSICAL REVIEW APPLIED LA English DT Article ID MIXED-STATE; FIELDS; NB3SN AB Determining the optimal arrangement of superconducting layers to withstand large-amplitude ac magnetic fields is important for certain applications such as superconducting radio-frequency cavities. In this paper, we evaluate the shielding potential of the superconducting-film-insulating-film-superconductor (SIS') structure, a configuration that could provide benefits in screening large ac magnetic fields. After establishing that, for high-frequency magnetic fields, flux penetration must be avoided, the superheating field of the structure is calculated in the London limit both numerically and, for thin films, analytically. For intermediate film thicknesses and realistic material parameters, we also solve numerically the Ginzburg-Landau equations. It is shown that a small enhancement of the superheating field is possible, on the order of a few percent, for the SIS' structure relative to a bulk superconductor of the film material, if the materials and thicknesses are chosen appropriately. C1 [Posen, Sam; Liepe, Matthias U.] Cornell Univ, Dept Phys, Newman Lab, LEPP, Ithaca, NY 14853 USA. [Transtrum, Mark K.] Brigham Young Univ, Dept Phys & Astron, Provo, UT 84602 USA. [Catelani, Gianluigi] Forschungszentrum Julich, Peter Grunberg Inst PGI 2, D-52425 Julich, Germany. [Sethna, James P.] Cornell Univ, Dept Phys, LASSP, Ithaca, NY 14853 USA. RP Posen, S (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. RI Catelani, Gianluigi/E-7134-2011; OI Catelani, Gianluigi/0000-0002-0421-7325; Transtrum, Mark/0000-0001-9529-9399 FU DOE [DE-SC0002329, DE-SC0008431]; NSF [DMR 1312160]; EU under REA [CIG-618258] FX This work is supported by DOE Awards No. DE-SC0002329 and No. DE-SC0008431, NSF Award No. DMR 1312160, and in part the EU under REA Grant Agreement No. CIG-618258. NR 32 TC 6 Z9 6 U1 1 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2331-7019 J9 PHYS REV APPL JI Phys. Rev. Appl. PD OCT 29 PY 2015 VL 4 IS 4 AR 044019 DI 10.1103/PhysRevApplied.4.044019 PG 8 WC Physics, Applied SC Physics GA CU8MC UT WOS:000363795900001 ER PT J AU Langner, MC Zhou, S Coslovich, G Chuang, YD Zhu, Y Robinson, JS Schlotter, WF Turner, JJ Minitti, MP Moore, RG Lee, WS Lu, DH Doering, D Denes, P Tomioka, Y Tokura, Y Kaindl, RA Schoenlein, RW AF Langner, M. C. Zhou, S. Coslovich, G. Chuang, Y. -D. Zhu, Y. Robinson, J. S. Schlotter, W. F. Turner, J. J. Minitti, M. P. Moore, R. G. Lee, W. S. Lu, D. H. Doering, D. Denes, P. Tomioka, Y. Tokura, Y. Kaindl, R. A. Schoenlein, R. W. TI Ultrafast x-ray and optical signatures of phase competition and separation underlying the photoinduced metallic phase in Pr1-xCaxMnO3 SO PHYSICAL REVIEW B LA English DT Article ID MAGNETIC-FIELD; INSULATOR; MANGANITE; TRANSITIONS; DYNAMICS; ORDER AB The coexistence of ferromagnetic and antiferromagnetic phases and their role in the photoinduced insulator-to-metal transition in Pr1-xCax MnO3 are revealed via ultrafast resonant x-ray diffraction and broadband optical reflectivity measurements. The antiferromagnetic scattering signal and ferromagnetically sensitive reflectivity measurements show similar, strongly temperature dependent time scales. We attribute the common dynamics to an activation barrier between the equilibrium insulating phase and the photoinduced metallic phase related to interactions between the phase-separated ferromagnetic and antiferromagnetic insulating phases. C1 [Langner, M. C.; Zhou, S.; Coslovich, G.; Zhu, Y.; Robinson, J. S.; Kaindl, R. A.; Schoenlein, R. W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Zhou, S.; Chuang, Y. -D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Schlotter, W. F.; Turner, J. J.; Minitti, M. P.] SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA 94720 USA. [Moore, R. G.; Lee, W. S.] Stanford Inst Mat & Energy Sci, SLAC Natl Accelerator Lab, Menlo Pk, CA 94720 USA. [Lu, D. H.] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94720 USA. [Doering, D.; Denes, P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Engn, Berkeley, CA 94720 USA. [Tomioka, Y.] Natl Inst Adv Ind Sci & Technol, Nanoelect Res Inst, Tsukuba, Ibaraki 3058562, Japan. [Tokura, Y.] Univ Tokyo, Dept Appl Phys, Tokyo 1138656, Japan. [Tokura, Y.] Univ Tokyo, Quantum Phase Elect Ctr, Tokyo 1138656, Japan. [Tokura, Y.] RIKEN, Ctr Emergent Matter Sci, Wako, Saitama 3510198, Japan. RP Langner, MC (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RI Tokura, Yoshinori/C-7352-2009; Zhou, Shuyun/A-5750-2009 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (BES) [DEAC02-05CH11231 (LBNL), DE-AC02-76SF00515 (SLAC)]; LCLS, Stanford University through the Stanford Institute for Materials Energy Sciences (SIMES); Advanced Light Source at LBNL, University of Hamburg through the BMBF priority program [FSP 301]; Center for Free Electron Laser Science (CFEL); LBNL provided by the Director, Office of Science, of the U.S. Department of Energy FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (BES) under Contracts No. DEAC02-05CH11231 (LBNL) and No. DE-AC02-76SF00515 (SLAC). Ultrafast X-ray scattering measurements were led by the Ultrafast Materials Program at LBNL and were conducted at the SXR Instrument of the Linac Coherent Light Source (LCLS), a division of SLAC and a DOE Office of Science User Facility (LCLS proposal L336). The SXR Instrument is supported by a consortium whose membership includes the LCLS, Stanford University through the Stanford Institute for Materials Energy Sciences (SIMES), the Advanced Light Source at LBNL, University of Hamburg through the BMBF priority program FSP 301, and the Center for Free Electron Laser Science (CFEL). Data analysis and transient optical spectroscopy were supported by Laboratory Directed Research and Development (LDRD) funding from LBNL provided by the Director, Office of Science, of the U.S. Department of Energy. NR 34 TC 1 Z9 1 U1 4 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 29 PY 2015 VL 92 IS 15 AR 155148 DI 10.1103/PhysRevB.92.155148 PG 7 WC Physics, Condensed Matter SC Physics GA CU8KD UT WOS:000363790400002 ER PT J AU Poudel, N Gooch, M Lorenz, B Chu, CW Kim, JW Cheong, SW AF Poudel, N. Gooch, M. Lorenz, B. Chu, C. W. Kim, J. W. Cheong, S. W. TI Pressure-induced decoupling of rare-earth moments and Mn spins in multiferroic GdMn2O5 SO PHYSICAL REVIEW B LA English DT Article ID FERROELECTRIC POLARIZATION; MAGNETISM; HOMN2O5; OXIDE AB The effects of pressure on the ferroelectric properties of multiferroic GdMn2O5 is studied up to 18.2 kbar. Above a critical pressure of p(c) approximate to 10 kbar, the ferroelectric transition splits into two, with the first transition shifted to higher temperature. The pressure-temperature phase diagram is derived. The results indicate a pressure-induced decoupling of the Gd moments from the Mn spin system. The conclusion is supported by thermal expansion data which show a large increase of the c axis at the ambient-pressure ferroelectric transition. The pressure-induced contraction of the c lattice parameter is considered to be the origin of the decoupling of both magnetic subsystems above p(c). C1 [Poudel, N.; Gooch, M.; Lorenz, B.; Chu, C. W.] Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. [Poudel, N.; Gooch, M.; Lorenz, B.; Chu, C. W.] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Chu, C. W.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Kim, J. W.; Cheong, S. W.] Rutgers State Univ, Rutgers Ctr Emerging Mat, Piscataway, NJ 08854 USA. [Kim, J. W.; Cheong, S. W.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. RP Poudel, N (reprint author), Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. FU US Air Force Office of Scientific Research; Robert A. Welch Foundation [E-1297]; T.L.L. Temple Foundation; J. J. and R. Moores Endowment; State of Texas through the TCSUH; DOE [DOE: DE-FG02-07ER46382] FX This work is supported in part by the US Air Force Office of Scientific Research, the Robert A. Welch Foundation (E-1297), the T.L.L. Temple Foundation, the J. J. and R. Moores Endowment, and the State of Texas through the TCSUH and at LBNL by the DOE. The work at Rutgers University was supported by the DOE under Grant No. DOE: DE-FG02-07ER46382. NR 47 TC 3 Z9 3 U1 0 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD OCT 29 PY 2015 VL 92 IS 14 AR 144430 DI 10.1103/PhysRevB.92.144430 PG 6 WC Physics, Condensed Matter SC Physics GA CU8KB UT WOS:000363790200003 ER PT J AU Glassman, BE Perez-Loureiro, D Wrede, C Allen, J Bardayan, DW Bennett, MB Brown, BA Chipps, KA Febbraro, M Fry, C Hall, MR Hall, O Liddick, SN O'Malley, P Ong, W Pain, SD Schwartz, SB Shidling, P Sims, H Thompson, P Zhang, H AF Glassman, B. E. Perez-Loureiro, D. Wrede, C. Allen, J. Bardayan, D. W. Bennett, M. B. Brown, B. A. Chipps, K. A. Febbraro, M. Fry, C. Hall, M. R. Hall, O. Liddick, S. N. O'Malley, P. Ong, W. Pain, S. D. Schwartz, S. B. Shidling, P. Sims, H. Thompson, P. Zhang, H. TI Revalidation of the isobaric multiplet mass equation for the A=20 quintet SO PHYSICAL REVIEW C LA English DT Article ID NUCLEAR-DATA SHEETS; ENERGY-LEVELS; LIGHT-NUCLEI; T3/Z TERM; MG-20; STATE; SEPARATOR; DECAY; NA20 AB An unexpected breakdown of the isobaric multiplet mass equation in the A = 20, T = 2 quintet was recently reported, presenting a challenge to modern theories of nuclear structure. In the present work, the excitation energy of the lowest T = 2 state in Na-20 has been measured to be 6498.4 +/- 0.2(stat) +/- 0.4(syst) keV by using the superallowed 0(+) -> 0(+) beta decay of Mg-20 to access it and an array of high-purity germanium detectors to detect its gamma-ray deexcitation. This value differs by 27 keV (1.9 standard deviations) from the recommended value of 6525 +/- 14 keV and is a factor of 28 more precise. The isobaric multiplet mass equation is shown to be revalidated when the new value is adopted. C1 [Glassman, B. E.; Wrede, C.; Bennett, M. B.; Brown, B. A.; Fry, C.; Ong, W.; Schwartz, S. B.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Glassman, B. E.; Perez-Loureiro, D.; Wrede, C.; Bennett, M. B.; Brown, B. A.; Fry, C.; Liddick, S. N.; Ong, W.; Schwartz, S. B.; Zhang, H.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Allen, J.; Bardayan, D. W.; Hall, M. R.; Hall, O.; O'Malley, P.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Chipps, K. A.; Febbraro, M.; Pain, S. D.; Thompson, P.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Chipps, K. A.; Febbraro, M.; Thompson, P.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Liddick, S. N.] Michigan State Univ, Dept Chem, E Lansing, MI 48824 USA. [Shidling, P.] Texas A&M Univ, Inst Cyclotron, College Stn, TX 77843 USA. [Sims, H.] Univ Surrey, Guildford GU2 7XH, Surrey, England. RP Glassman, BE (reprint author), Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. EM glassman@nscl.msu.edu; perezlou@nscl.msu.edu; wrede@nscl.msu.edu RI Pain, Steven/E-1188-2011; OI Pain, Steven/0000-0003-3081-688X; Chipps, Kelly/0000-0003-3050-1298; Perez-Loureiro, David/0000-0002-0609-1308 FU National Science Foundation (USA) [PHY-1102511, PHY-1419765, PHY-1404442] FX We gratefully acknowledge the NSCL staff for technical assistance and for providing the 20Mg beam. This work was supported by the National Science Foundation (USA) under Grants No. PHY-1102511, No. PHY-1419765, and No. PHY-1404442. NR 37 TC 5 Z9 5 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 29 PY 2015 VL 92 IS 4 AR 042501 DI 10.1103/PhysRevC.92.042501 PG 4 WC Physics, Nuclear SC Physics GA CU8KS UT WOS:000363791900001 ER PT J AU Bertini, B Essler, FHL Groha, S Robinson, NJ AF Bertini, Bruno Essler, Fabian H. L. Groha, Stefan Robinson, Neil J. TI Prethermalization and Thermalization in Models with Weak Integrability Breaking SO PHYSICAL REVIEW LETTERS LA English DT Article ID MATRIX RENORMALIZATION-GROUP; QUANTUM-SYSTEMS AB We study the effects of integrability-breaking perturbations on the nonequilibrium evolution of manyparticle quantum systems. We focus on a class of spinless fermion models with weak interactions. We employ equation of motion techniques that can be viewed as generalizations of quantum Boltzmann equations. We benchmark our method against time-dependent density matrix renormalization group computations and find it to be very accurate as long as interactions are weak. For small integrability breaking, we observe robust prethermalization plateaux for local observables on all accessible time scales. Increasing the strength of the integrability-breaking term induces a "drift" away from the prethermalization plateaux towards thermal behavior. We identify a time scale characterizing this crossover. C1 [Bertini, Bruno; Essler, Fabian H. L.; Groha, Stefan; Robinson, Neil J.] Univ Oxford, Rudolf Peierls Ctr Theoret Phys, Oxford OX1 3NP, England. [Robinson, Neil J.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Bertini, B (reprint author), Univ Oxford, Rudolf Peierls Ctr Theoret Phys, Oxford OX1 3NP, England. OI Robinson, Neil/0000-0001-6633-5338 FU EPSRC [EP/J014885/1, EP/I032487/1]; U.S. Department of Energy, Office of Basic Energy Sciences [DEAC02-98CH10886, DE-SC0012704]; Clarendon Scholarship fund FX We thank M. Fagotti, A. Gambassi, S. Kehrein, and A. Silva for helpful discussions. This work was supported by the EPSRC under Grants No. EP/J014885/1 and No. EP/I032487/1, by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contracts No. DEAC02-98CH10886 and No. DE-SC0012704 (N. J. R.) and by the Clarendon Scholarship fund (S. G.). NR 64 TC 30 Z9 30 U1 2 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 29 PY 2015 VL 115 IS 18 AR 180601 DI 10.1103/PhysRevLett.115.180601 PG 6 WC Physics, Multidisciplinary SC Physics GA CU8JF UT WOS:000363787600004 PM 26565450 ER PT J AU Jones, BM Grosse, G Arp, CD Miller, E Liu, L Hayes, DJ Larsen, CF AF Jones, Benjamin M. Grosse, Guido Arp, Christopher D. Miller, Eric Liu, Lin Hayes, Daniel J. Larsen, Christopher F. TI Recent Arctic tundra fire initiates widespread thermokarst development SO SCIENTIFIC REPORTS LA English DT Article ID BOREAL FORESTS; CLIMATE-CHANGE; INTERIOR ALASKA; PERMAFROST DEGRADATION; CARBON BALANCE; BURN SEVERITY; VULNERABILITY; ECOSYSTEMS; VEGETATION; WILDFIRE AB Fire-induced permafrost degradation is well documented in boreal forests, but the role of fires in initiating thermokarst development in Arctic tundra is less well understood. Here we show that Arctic tundra fires may induce widespread thaw subsidence of permafrost terrain in the first seven years following the disturbance. Quantitative analysis of airborne LiDAR data acquired two and seven years post-fire, detected permafrost thaw subsidence across 34% of the burned tundra area studied, compared to less than 1% in similar undisturbed, ice-rich tundra terrain units. The variability in thermokarst development appears to be influenced by the interaction of tundra fire burn severity and near-surface, ground-ice content. Subsidence was greatest in severely burned, ice-rich upland terrain (yedoma), accounting for -50% of the detected subsidence, despite representing only 30% of the fire disturbed study area. Microtopography increased by 340% in this terrain unit as a result of ice wedge degradation. Increases in the frequency, magnitude, and severity of tundra fires will contribute to future thermokarst development and associated landscape change in Arctic tundra regions. C1 [Jones, Benjamin M.] US Geol Survey, Alaska Sci Ctr, Anchorage, AK 99508 USA. [Grosse, Guido] Helmholtz Ctr Polar & Marine Res, Alfred Wegener Inst, Potsdam, Germany. [Arp, Christopher D.] Univ Alaska Fairbanks, Water & Environm Res Ctr, Fairbanks, AK 99775 USA. [Miller, Eric] Bur Land Management Alaska Fire Serv, Ft Wainwright, AK 99703 USA. [Liu, Lin] Chinese Univ Hong Kong, Earth Syst Sci Programme, Fac Sci, Hong Kong, Hong Kong, Peoples R China. [Hayes, Daniel J.] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Larsen, Christopher F.] Univ Alaska Fairbanks, Inst Geophys, Fairbanks, AK 99775 USA. RP Jones, BM (reprint author), US Geol Survey, Alaska Sci Ctr, Anchorage, AK 99508 USA. EM bjones@usgs.gov RI Grosse, Guido/F-5018-2011; OI Grosse, Guido/0000-0001-5895-2141; Arp, Christopher/0000-0002-6485-6225 FU USGS Land Remote Sensing program; Land Change Science program; Arctic Landscape Conservation Cooperative FX We thank the USGS Land Remote Sensing program for providing funding for acquisition of the 2014 LiDAR dataset and the USGS Rolla, Missouri Office for working with the vendor on the acquisition of the data. This work was primarily supported by the USGS Land Remote Sensing and Land Change Science programs. Additional support was provided by the Arctic Landscape Conservation Cooperative. Thanks to Kodiak Mapping, Inc. for providing the 2009 LiDAR. Thanks to Crystal Kolden for sharing the Landsat-derived dNBR data. Thanks to Joseph Wheaton and Philip Bailey for assistance with the Geomorphic Change Detection software. Any use of trade, product, or firm names is for descriptive purposes only and does not imply endorsement by the U.S. Government. NR 55 TC 8 Z9 8 U1 6 U2 45 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 29 PY 2015 VL 5 AR 15865 DI 10.1038/srep15865 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CU6DQ UT WOS:000363622200004 PM 26511650 ER PT J AU Lercher, JA AF Lercher, Johannes A. TI New Lewis Acid Catalyzed Pathway to Carbon-Carbon Bonds from Methanol SO ACS CENTRAL SCIENCE LA English DT Editorial Material ID HYDROCARBONS C1 [Lercher, Johannes A.] Tech Univ Munich, Dept Chem, D-85748 Garching, Germany. [Lercher, Johannes A.] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. RP Lercher, JA (reprint author), Tech Univ Munich, Dept Chem, Lichtenbergstr 4, D-85748 Garching, Germany. EM johannes.lercher@ch.tum.de NR 3 TC 2 Z9 2 U1 4 U2 8 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2374-7943 EI 2374-7951 J9 ACS CENTRAL SCI JI ACS Central Sci. PD OCT 28 PY 2015 VL 1 IS 7 BP 350 EP 351 DI 10.1021/acscentsci.5b00311 PG 2 WC Chemistry, Multidisciplinary SC Chemistry GA CX8QU UT WOS:000365969500004 PM 27162993 ER PT J AU Broichhagen, J Damijonaitis, A Levitz, J Sokol, KR Leippe, P Konrad, D Isacoff, EY Trauner, D AF Broichhagen, Johannes Damijonaitis, Arunas Levitz, Joshua Sokol, Kevin R. Leippe, Philipp Konrad, David Isacoff, Ehud Y. Trauner, Dirk TI Orthogonal Optical Control of a G Protein-Coupled Receptor with a SNAP-Tethered Photochromic Ligand SO ACS CENTRAL SCIENCE LA English DT Article ID METABOTROPIC GLUTAMATE RECEPTORS; MOLECULES IN-VIVO; NICOTINIC ACETYLCHOLINE-RECEPTORS; FUSION PROTEINS; O-6-ALKYLGUANINE-DNA ALKYLTRANSFERASE; REMOTE-CONTROL; LIVING CELLS; ION CHANNELS; CHEMISTRY; PHARMACOLOGY AB The covalent attachment of synthetic photoswitches is a general approach to impart light sensitivity onto native receptors. It mimics the logic of natural photoreceptors and significantly expands the reach of optogenetics. Here we describe a novel photoswitch design-the photoswitchable orthogonal remotely tethered ligand (PORTL)-that combines the genetically encoded SNAP-tag with photochromic ligands connected to a benzylguanine via a long flexible linker. We use the method to convert the G protein-coupled receptor mGluR2, a metabotropic glutamate receptor, into a photoreceptor (SNAG-mGluR2) that provides efficient optical control over the neuronal functions of mGluR2: presynaptic inhibition and control of excitability. The PORTL approach enables multiplexed optical control of different native receptors using distinct bioconjugation methods. It should be broadly applicable since SNAP-tags have proven to be reliable, many SNAP-tagged receptors are already available, and photochromic ligands on a long leash are readily designed and synthesized. C1 [Broichhagen, Johannes; Damijonaitis, Arunas; Sokol, Kevin R.; Leippe, Philipp; Konrad, David; Trauner, Dirk] Univ Munich, Dept Chem, D-81377 Munich, Germany. [Broichhagen, Johannes; Damijonaitis, Arunas; Sokol, Kevin R.; Leippe, Philipp; Konrad, David; Trauner, Dirk] Munich Ctr Integrated Prot Sci, D-81377 Munich, Germany. [Levitz, Joshua; Isacoff, Ehud Y.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Isacoff, Ehud Y.] Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA. [Isacoff, Ehud Y.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Trauner, D (reprint author), Univ Munich, Dept Chem, Butenandtstr 5-13, D-81377 Munich, Germany. EM Dirk.Trauner@lmu.de OI Damijonaitis, Arunas/0000-0003-4522-9733 FU NEI NIH HHS [PN2 EY018241] NR 56 TC 6 Z9 6 U1 4 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2374-7943 EI 2374-7951 J9 ACS CENTRAL SCI JI ACS Central Sci. PD OCT 28 PY 2015 VL 1 IS 7 BP 383 EP 393 DI 10.1021/acscentsci.5b00260 PG 11 WC Chemistry, Multidisciplinary SC Chemistry GA CX8QU UT WOS:000365969500009 PM 27162996 ER PT J AU Barabash, RI Voit, SL Aidhy, DS Lee, SM Knight, TW Sprouster, DJ Ecker, LE AF Barabash, Rozaliya I. Voit, Stewart L. Aidhy, Dilpuneet S. Lee, Seung Min Knight, Travis W. Sprouster, David J. Ecker, Lynne E. TI Cation and vacancy disorder in U1-yNdyO2.00-x alloys SO JOURNAL OF MATERIALS RESEARCH LA English DT Review ID PAIR-DISTRIBUTION FUNCTION; FISSION-GAS RELEASE; X-RAY-SCATTERING; MOLECULAR-DYNAMICS SIMULATIONS; URANIUM-DIOXIDE; THERMODYNAMIC PROPERTIES; COORDINATION CHEMISTRY; DEFECT STRUCTURE; IONIC LIQUIDS; HEAT-CAPACITY AB In the present article, the intermixing and clustering of U/Nd, O, and vacancies were studied by both laboratory and synchrotron-based x-ray diffraction in U1-yNdyO2-x alloys. It was found that an increased holding time at the high experimental temperature during initial alloy preparation results in a lower disorder of the Nd distribution in the alloys. Adjustment of the oxygen concentration in the U1-yNdyO2-x alloys with different Nd concentrations was accompanied by the formation of vacancies on the oxygen sublattice and a nanocrystalline component. The lattice parameters in the U1-yNdyO2-x alloys were also found to deviate significantly from Vegard's law when the Nd concentration was high (53%) and decreased with increasing oxygen concentration. Such changes indicate the formation of large vacancy concentrations during oxygen adjustment at these high temperatures. The change in the vacancy concentration after the oxygen adjustment was estimated relative to Nd concentration and oxygen stoichiometry. C1 [Barabash, Rozaliya I.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Voit, Stewart L.] Oak Ridge Natl Lab, Fuel Cycle & Isotopes Div, Oak Ridge, TN 37831 USA. [Aidhy, Dilpuneet S.] Univ Wyoming, Dept Mech Engn, Laramie, WY 82071 USA. [Lee, Seung Min; Knight, Travis W.] Univ S Carolina, Coll Engn & Comp, Dept Nucl Engn, Columbia, SC 29208 USA. [Sprouster, David J.; Ecker, Lynne E.] Brookhaven Natl Lab, Nucl Sci & Technol Dept, Upton, NY 11973 USA. RP Barabash, RI (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM rbarabas@utk.edu; dsprouster@bnl.gov RI Sprouster, David/F-2280-2010 OI Sprouster, David/0000-0002-2689-0721 FU Department of Energy Office of Nuclear Energy, Fuel Cycle Research and Development Program; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; U.S.D.O.E. [DE-AC02-98CH10886] FX Research is sponsored by the Department of Energy Office of Nuclear Energy, Fuel Cycle Research and Development Program. The calculations (DSA) were supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. The National Synchrotron Light Source at Brookhaven National Laboratory is supported under U.S.D.O.E. Grant No. DE-AC02-98CH10886. NR 63 TC 0 Z9 0 U1 3 U2 15 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 EI 2044-5326 J9 J MATER RES JI J. Mater. Res. PD OCT 28 PY 2015 VL 30 IS 20 BP 3026 EP 3040 DI 10.1557/jmr.2015.261 PG 15 WC Materials Science, Multidisciplinary SC Materials Science GA CW9IV UT WOS:000365313300006 ER PT J AU Denton, RE Jordanova, VK Bortnik, J AF Denton, R. E. Jordanova, V. K. Bortnik, J. TI Resonance of relativistic electrons with electromagnetic ion cyclotron waves SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID GEOSYNCHRONOUS ORBIT; EMIC WAVES; SCATTERING AB Relativistic electrons have been thought to more easily resonate with electromagnetic ion cyclotron (EMIC) waves if the total density is large. We show that for a particular EMIC mode, this dependence is weak due to the dependence of the wave frequency and wave vector on the density. A significant increase in relativistic electron minimum resonant energy might occur for the H band EMIC mode only for small density, but no changes in parameters significantly decrease the minimum resonant energy from a nominal value. The minimum resonant energy depends most strongly on the thermal velocity associated with the field line motion of the hot ring current protons that drive the instability. High density due to a plasmasphere or plasmaspheric plume could possibly lead to lower minimum resonance energy by causing the He band EMIC mode to be dominant. We demonstrate these points using parameters from a ring current simulation. C1 [Denton, R. E.] Dartmouth Coll, Dept Phys & Astron, Hanover, NH 03755 USA. [Jordanova, V. K.] Los Alamos Natl Lab, Los Alamos, NM USA. [Bortnik, J.] Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Los Angeles, CA USA. RP Denton, RE (reprint author), Dartmouth Coll, Dept Phys & Astron, Hanover, NH 03755 USA. EM richard.e.denton@dartmouth.edu FU NASA [NNX10AQ60G, NNX13AD65G, NNX08AM58G, NNH13AW83I]; U.S. Department of Energy; NSF [IAA1203460]; NSF/DOE basic plasma physics [DE-SC0010578] FX We thank Mary Hudson and Jay Albert for useful conversations. Work at Dartmouth was supported by NASA grants NNX10AQ60G, NNX13AD65G, and NNX08AM58G. Work at Los Alamos was conducted under the auspices of the U.S. Department of Energy with partial support from NASA grant NNH13AW83I and NSF grant IAA1203460. J.B. would like to acknowledge support from NSF/DOE basic plasma physics grant DE-SC0010578. Numerical data shown in this paper are available from the lead author upon request. NR 24 TC 4 Z9 4 U1 0 U2 10 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD OCT 28 PY 2015 VL 42 IS 20 BP 8263 EP 8270 DI 10.1002/2015GL064379 PG 8 WC Geosciences, Multidisciplinary SC Geology GA CW1WL UT WOS:000364782500001 ER PT J AU Bougamont, M Christoffersen, P Price, SF Fricker, HA Tulaczyk, S Carter, SP AF Bougamont, M. Christoffersen, P. Price, S. F. Fricker, H. A. Tulaczyk, S. Carter, S. P. TI Reactivation of Kamb Ice Stream tributaries triggers century-scale reorganization of Siple Coast ice flow in West Antarctica SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE ice flow modeling; basal processes; subglacial hydrology; West Antarctic ice sheet; mass balance; thermodynamics ID SUBGLACIAL LAKE WHILLANS; GROUNDING-LINE; SHEET DYNAMICS; MASS-BALANCE; STAGNATION; BENEATH; MARGINS; MODEL; RADAR; ROSS AB Ongoing, centennial-scale flow variability within the Ross ice streams of West Antarctica suggests that the present-day positive mass balance in this region may reverse in the future. Here we use a three-dimensional ice sheet model to simulate ice flow in this region over 250years. The flow responds to changing basal properties, as a subglacial till layer interacts with water transported in an active subglacial hydrological system. We show that a persistent weak bed beneath the tributaries of the dormant Kamb Ice Stream is a source of internal ice flow instability, which reorganizes all ice streams in this region, leading to a reduced (positive) mass balance within decades and a net loss of ice within two centuries. This hitherto unaccounted for flow variability could raise sea level by 5mm this century. Better constraints on future sea level change from this region will require improved estimates of geothermal heat flux and subglacial water transport. C1 [Bougamont, M.; Christoffersen, P.] Univ Cambridge, Scott Polar Res Inst, Cambridge CB2 1ER, England. [Price, S. F.] Los Alamos Natl Lab, Fluid Dynam & Solid Mech Grp, Los Alamos, NM USA. [Fricker, H. A.; Carter, S. P.] Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92093 USA. [Tulaczyk, S.] Univ Calif Santa Cruz, Dept Earth & Planetary Sci, Santa Cruz, CA 95064 USA. RP Bougamont, M (reprint author), Univ Cambridge, Scott Polar Res Inst, Cambridge CB2 1ER, England. EM mb627@cam.ac.uk RI Christoffersen, Poul/C-7328-2013; Price, Stephen /E-1568-2013; OI Christoffersen, Poul/0000-0003-2643-8724; Price, Stephen /0000-0001-6878-2553; Bougamont, Marion Heidi/0000-0001-7196-4171 FU Isaac Newton trust; Cecil H., and Ida M. Green Foundation; Natural Environment Research Council [NE/E005950/1, NE/J005800/1]; U.S. Department of Energy Office of Science, Biological and Environmental Research program; National Science Foundation [0338295, ANT-0838885 (Fricker)]; Cryospheric Sciences program of NASA FX This work was carried out with support from the Isaac Newton trust, Cecil H., and Ida M. Green Foundation and Natural Environment Research Council (grants NE/E005950/1 and NE/J005800/1). S.F.P. was supported by the U.S. Department of Energy Office of Science, Biological and Environmental Research program. S.T. acknowledges support from National Science Foundation (grant #0338295). S.P.C. was supported by funding from the Cryospheric Sciences program of NASA, and H.A.F. was supported by funding from NSF (grant ANT-0838885 (Fricker)). The source code for the results presented can be obtained by contacting the corresponding author directly. NR 67 TC 7 Z9 7 U1 4 U2 16 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD OCT 28 PY 2015 VL 42 IS 20 BP 8471 EP 8480 DI 10.1002/2015GL065782 PG 10 WC Geosciences, Multidisciplinary SC Geology GA CW1WL UT WOS:000364782500027 ER PT J AU Fildier, B Collins, WD AF Fildier, Benjamin Collins, William D. TI Origins of climate model discrepancies in atmospheric shortwave absorption and global precipitation changes SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID HYDROLOGICAL CYCLE; CONSTRAINT; RADIATION AB Projected increases in mean precipitation are constrained by the atmospheric energy budget through radiative-convective equilibrium. However, significant differences persist between climate models on the rate of increase in precipitation per unit warming, mostly arising from the clear-sky radiative response. While the intermodel spread in clear-sky longwave cooling has been explained by climate feedbacks, the sources of spread in clear-sky shortwave heating are still unclear. This article focuses on the latter. Since water vapor contributes most of the atmospheric shortwave absorption, both intermodel differences in its spatial distribution and in radiative transfer parameterizations are plausible hypotheses for the spread. This work reestablishes the primary contribution from water vapor relative to other shortwave-absorbing species and evaluates the validity of both hypotheses. It is found that the intermodel spread in shortwave absorption change most likely originates from the radiation schemes, possibly because of simplifications induced by their low spectral resolutions. C1 [Fildier, Benjamin; Collins, William D.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Fildier, Benjamin; Collins, William D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Climate & Ecosyst Sci Div, Berkeley, CA 94720 USA. RP Fildier, B (reprint author), Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. EM benjamin.fildier@berkeley.edu RI Collins, William/J-3147-2014; Fildier, Benjamin/N-9305-2013 OI Collins, William/0000-0002-4463-9848; Fildier, Benjamin/0000-0002-6058-7769 FU Director, Office of Science, Office of Biological and Environmental Research of the U.S. Department of Energy, Earth System Modeling Program [DE-AC02-05CH11231]; National Energy Research Scientific Computing Center (NERSC); Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX The data used in this study are available from the Coupled Model Intercomparison Project Phase 5. This research was supported by the Director, Office of Science, Office of Biological and Environmental Research of the U.S. Department of Energy under contract DE-AC02-05CH11231 as part of their Earth System Modeling Program and used resources of the National Energy Research Scientific Computing Center (NERSC), also supported by the Office of Science of the U.S. Department of Energy, under contract DE-AC02-05CH11231. NR 26 TC 4 Z9 4 U1 1 U2 11 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD OCT 28 PY 2015 VL 42 IS 20 BP 8749 EP 8757 DI 10.1002/2015GL065931 PG 9 WC Geosciences, Multidisciplinary SC Geology GA CW1WL UT WOS:000364782500059 ER PT J AU Feng, R Kremer, F Sprouster, DJ Mirzaei, S Decoster, S Glover, CJ Medling, SA Russo, SP Ridgway, MC AF Feng, R. Kremer, F. Sprouster, D. J. Mirzaei, S. Decoster, S. Glover, C. J. Medling, S. A. Russo, S. P. Ridgway, M. C. TI Structural and electrical properties of In-implanted Ge SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; SELF-INTERSTITIALS; GERMANIUM; SPECTROSCOPY; VACANCIES; IFEFFIT; SI AB We report on the effects of dopant concentration on the structural and electrical properties of In-implanted Ge. For In concentrations of <= 0.2 at. %, extended x-ray absorption fine structure and x-ray absorption near-edge structure measurements demonstrate that all In atoms occupy a substitutional lattice site while metallic In precipitates are apparent in transmission electron micrographs for In concentrations >= 0.6 at. %. Evidence of the formation of In-vacancy complexes deduced from extended x-ray absorption fine structure measurements is complimented by density functional theory simulations. Hall effect measurements of the conductivity, carrier density, and carrier mobility are then correlated with the substitutional In fraction. (C) 2015 AIP Publishing LLC. C1 [Feng, R.; Kremer, F.; Mirzaei, S.; Medling, S. A.; Ridgway, M. C.] Australian Natl Univ, Dept Elect Mat Engn, Res Sch Phys & Engn, Canberra, ACT 0200, Australia. [Sprouster, D. J.] Brookhaven Natl Lab, Nucl Sci & Technol Dept, Upton, NY 11973 USA. [Decoster, S.] Katholieke Univ Leuven, Inst Kern En Stralingsfys, B-3001 Leuven, Belgium. [Glover, C. J.] Australian Synchrotron, Clayton, Vic 3168, Australia. [Russo, S. P.] RMIT Univ, Sch Appl Sci, Dept Appl Phys, Melbourne 3001, Australia. RP Feng, R (reprint author), Australian Natl Univ, Dept Elect Mat Engn, Res Sch Phys & Engn, GPO Box 4, Canberra, ACT 0200, Australia. EM ruixing.feng@anu.edu.au RI Sprouster, David/F-2280-2010; OI Sprouster, David/0000-0002-2689-0721; Russo, Salvy/0000-0003-3589-3040; Kremer, Felipe/0000-0001-6263-7806 FU Australian Research Council; Australian Synchrotron FX We acknowledge access to NCRIS and AMMRF infrastructure at the Australian National University, including the Australian National Fabrication Facility, the Heavy Ion Accelerator Capability, and the Center for Advanced Microscopy. We also thank the Australian Research Council and the Australian Synchrotron for support. NR 42 TC 4 Z9 4 U1 2 U2 14 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 28 PY 2015 VL 118 IS 16 AR 165701 DI 10.1063/1.4934200 PG 8 WC Physics, Applied SC Physics GA CV6VR UT WOS:000364410300051 ER PT J AU McGuire, MA Parker, DS AF McGuire, Michael A. Parker, David S. TI Magnetic and structural properties of ferromagnetic Fe5PB2 and Fe5SiB2 and effects of Co and Mn substitutions SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID X-RAY INVESTIGATIONS; B SYSTEMS ME=MN; FE-SI-B; FEATURES; PHASES AB Crystallographic and magnetic properties of Fe5PB2, Fe4CoPB2, Fe4MnPB2, Fe5SiB2, Fe4CoSiB2, and Fe4MnSiB2 are reported. All adopt the tetragonal Cr5B3 structure-type and are ferromagnetic at room temperature with easy axis of magnetization along the c- axis. The spin reorientation in Fe5SiB2 is observed as an anomaly in the magnetization near 170K and is suppressed by substitution of Co or Mn for Fe. The silicides are found to generally have larger magnetic moments than the phosphides, but the data suggest smaller magnetic anisotropy in the silicides. Cobalt substitution reduces the Curie temperatures by more than 100K and ordered magnetic moments by 16%- 20%, while manganese substitution has a much smaller effect. This suggests Mn moments align ferromagnetically with the Fe and that Co does not have an ordered moment in these structures. Anisotropic thermal expansion is observed in Fe5PB2 and Fe5SiB2, with negative thermal expansion seen along the c-axis of Fe5SiB2. First principles calculations of the magnetic properties of Fe5SiB2 and Fe4MnSiB2 are reported. The results, including the magnetic moment and anisotropy, are in good agreement with experiment. (C) 2015 AIP Publishing LLC. C1 [McGuire, Michael A.; Parker, David S.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP McGuire, MA (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM McGuireMA@ornl.gov RI McGuire, Michael/B-5453-2009 OI McGuire, Michael/0000-0003-1762-9406 FU U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Office, as part of the Propulsion Materials Program; Critical Materials Institute, an Energy Innovation Hub - U.S. Department of Energy, Energy Efficiency and Renewable Energy, Advanced Manufacturing Office; U.S. Department of Energy [DE-AC05-00OR22725] FX Experimental work (M.A.M.) was supported by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Office, as part of the Propulsion Materials Program. Theoretical work (D.S.P.) was supported by the Critical Materials Institute, an Energy Innovation Hub funded by the U.S. Department of Energy, Energy Efficiency and Renewable Energy, Advanced Manufacturing Office. This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable,world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 24 TC 3 Z9 3 U1 6 U2 17 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 28 PY 2015 VL 118 IS 16 AR 163903 DI 10.1063/1.4934496 PG 8 WC Physics, Applied SC Physics GA CV6VR UT WOS:000364410300009 ER PT J AU Vaisakh, CP Mascarenhas, A Kini, RN AF Vaisakh, C. P. Mascarenhas, A. Kini, R. N. TI THz generation mechanisms in the semiconductor alloy, GaAs1-xBix SO JOURNAL OF APPLIED PHYSICS LA English DT Article AB We present measurements of the THz emission from GaAs1-xBix epilayers excited with femtosecond laser pulses (lambda similar to 800 nm). We observed an increase in the peak-to-peak amplitude of the THz electric field with increasing Bi concentration. We also observed a polarity reversal of the THz transient in the epilayers with higher Bi concentration (x greater than or similar to 1.4%). Taking into account the band gap reduction due to Bi incorporation and the excess energy of the carriers, our measurements suggest that there is a cross-over from a predominantly surface field emitter at low Bi concentrations (x less than or similar to 0.5%) to a predominantly photo-Dember field emitter at higher concentrations (x greater than or similar to 1.4%). (C) 2015 AIP Publishing LLC. C1 [Vaisakh, C. P.; Kini, R. N.] Indian Inst Sci Educ & Res Thiruvananthapuram IIS, Thiruvananthapuram, Kerala, India. [Mascarenhas, A.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Kini, RN (reprint author), Indian Inst Sci Educ & Res Thiruvananthapuram IIS, CET Campus,Engn Coll PO, Thiruvananthapuram, Kerala, India. EM rajeevkini@iisertvm.ac.in RI Kini, Rajeev/D-2342-2009 OI Kini, Rajeev/0000-0002-3305-9346 FU Science and Engineering Research Board, Department of Science and Technology, India through Fast Track Scheme for Young Scientists; U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division [DE-AC36-08GO28308] FX Research at IISER-TVM was supported by Science and Engineering Research Board, Department of Science and Technology, India through the Fast Track Scheme for Young Scientists, and the sample growth at NREL was supported by U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division under Contract No. DE-AC36-08GO28308. NR 14 TC 1 Z9 1 U1 6 U2 11 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 28 PY 2015 VL 118 IS 16 AR 165702 DI 10.1063/1.4933290 PG 4 WC Physics, Applied SC Physics GA CV6VR UT WOS:000364410300052 ER PT J AU Han, Y Evans, JW AF Han, Yong Evans, James W. TI Adsorption and diffusion of Ru adatoms on Ru(0001)-supported graphene: Large-scale first-principles calculations SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; ELASTIC BAND METHOD; SURFACE-ENERGY; SADDLE-POINTS; WORK FUNCTION; BASIS-SET; METALS; GRAPHENE/RU(0001) AB Large-scale first-principles density functional theory calculations are performed to investigate the adsorption and diffusion of Ru adatoms on monolayer graphene (G) supported on Ru(0001). The G sheet exhibits a periodic moire-cell superstructure due to lattice mismatch. Within a moire cell, there are three distinct regions: fcc, hcp, and mound, in which the C-6-ring center is above a fcc site, a hcp site, and a surface Ru atom of Ru(0001), respectively. The adsorption energy of a Ru adatom is evaluated at specific sites in these distinct regions. We find the strongest binding at an adsorption site above a C atom in the fcc region, next strongest in the hcp region, then the fcc-hcp boundary (ridge) between these regions, and the weakest binding in the mound region. Behavior is similar to that observed from small-unit-cell calculations of Habenicht et al. [Top. Catal. 57, 69 (2014)], which differ from previous large-scale calculations. We determine the minimum-energy path for local diffusion near the center of the fcc region and obtain a local diffusion barrier of similar to 0.48 eV. We also estimate a significantly lower local diffusion barrier in the ridge region. These barriers and information on the adsorption energy variation facilitate development of a realistic model for the global potential energy surface for Ru adatoms. This in turn enables simulation studies elucidating diffusion-mediated directed-assembly of Ru nanoclusters during deposition of Ru on G/Ru(0001). (C) 2015 AIP Publishing LLC. C1 [Han, Yong] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. Iowa State Univ, US Dept Energy, Ames Lab, Ames, IA 50011 USA. RP Han, Y (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. FU NSF [CHE-1111500]; USDOE Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences through the Ames Laboratory Chemical Physics Program; Ames Laboratory USDOE [DE-AC02-07CH11358] FX Y.H. was supported by NSF Grant No. CHE-1111500. J.W.E. was supported by the USDOE Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences through the Ames Laboratory Chemical Physics Program. Ames Laboratory USDOE is operated by Iowa State University under Contract No. DE-AC02-07CH11358. Computations utilized USDOE NERSC, OLCF, and NSF-supported XSEDE resources. Y.H. thanks Zhengji Zhao for her help in our cNEB calculations at NERSC, Paul Kent at ORNL for the use of his k-point parallelism developmental code, and Hang Liu for his help in our DFT calculations from XSEDE at TACC. NR 51 TC 3 Z9 3 U1 4 U2 21 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD OCT 28 PY 2015 VL 143 IS 16 AR 164706 DI 10.1063/1.4934349 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CV4KN UT WOS:000364235800051 PM 26520542 ER PT J AU Harding, LB Klippenstein, SJ AF Harding, Lawrence B. Klippenstein, Stephen J. TI Comment on "A novel and facile decay path of Criegee intermediates by intramolecular insertion reactions via roaming transition states" [J. Chem. Phys. 142, 124312 (2015)] SO JOURNAL OF CHEMICAL PHYSICS LA English DT Editorial Material ID FORMALDEHYDE; OXYGEN; ATOM C1 [Harding, Lawrence B.; Klippenstein, Stephen J.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Harding, LB (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. OI Klippenstein, Stephen/0000-0001-6297-9187 NR 9 TC 1 Z9 1 U1 4 U2 29 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD OCT 28 PY 2015 VL 143 IS 16 AR 167101 DI 10.1063/1.4934801 PG 2 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CV4KN UT WOS:000364235800067 PM 26520558 ER PT J AU Liu, H Tse, JS Hu, MY Bi, W Zhao, J Alp, EE Pasternak, M Taylor, RD Lashley, JC AF Liu, H. Tse, J. S. Hu, M. Y. Bi, W. Zhao, J. Alp, E. E. Pasternak, M. Taylor, R. D. Lashley, J. C. TI Mechanisms for pressure-induced crystal-crystal transition, amorphization, and devitrification of SnI4 SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID METALLIC AMORPHOUS STATE; ICE-I; SCATTERING; INSTABILITY; DYNAMICS; LIQUID; GLASS AB The pressure-induced amorphization and subsequent recrystallization of SnI4 have been investigated using first principles molecular dynamics calculations together with high-pressure Sn-119 nuclear resonant inelastic x-ray scattering measurements. Above similar to 8 GPa, we observe a transformation from an ambient crystalline phase to an intermediate crystal structure and a subsequent recrystallization into a cubic phase at similar to 64 GPa. The crystalline-to-amorphous transition was identified on the basis of elastic compatibility criteria. The measured tin vibrational density of states shows large amplitude librations of SnI4 under ambient conditions. Although high pressure structures of SnI4 were thought to be determined by random packing of equal-sized spheres, we detected electron charge transfer in each phase. This charge transfer results in a crystal structure packing determined by larger than expected iodine atoms. (C) 2015 AIP Publishing LLC. C1 [Liu, H.; Tse, J. S.] Univ Saskatchewan, Dept Phys & Engn Phys, Saskatoon, SK S7N 5B2, Canada. [Hu, M. Y.; Bi, W.; Zhao, J.; Alp, E. E.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Pasternak, M.] Tel Aviv Univ, Sch Phys & Astron, Ramat Aviv, Israel. [Taylor, R. D.; Lashley, J. C.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Tse, JS (reprint author), Univ Saskatchewan, Dept Phys & Engn Phys, Saskatoon, SK S7N 5B2, Canada. EM john.tse@usask.ca RI Liu, Hanyu/E-9985-2012 OI Liu, Hanyu/0000-0003-2394-5421 FU U.S. DOE [DE-AC02-06CH11357]; National Natural Science Foundation of China [11474126] FX We would like to thank Dongzhou Zhang for help during one of the experiments. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. Calculations were performed at Westgrid Computing Facilities and the Laboratory Computing Resource Center's high-performance computing clusters, Blues and Fusion, at Argonne National Laboratory. John S. Tse and Hanyu Liu acknowledge the National Natural Science Foundation of China (Grant No. 11474126) and support from the University of Saskatchewan research computing group and the use of the HPC resources (Plato machine). NR 39 TC 1 Z9 1 U1 4 U2 22 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD OCT 28 PY 2015 VL 143 IS 16 AR 164508 DI 10.1063/1.4934502 PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CV4KN UT WOS:000364235800037 PM 26520528 ER PT J AU Meyer, ER Ticknor, C Bethkenhagen, M Hamel, S Redmer, R Kress, JD Collins, LA AF Meyer, Edmund R. Ticknor, Christopher Bethkenhagen, Mandy Hamel, Sebastien Redmer, Ronald Kress, Joel D. Collins, Lee A. TI Bonding and structure in dense multi-component molecular mixtures SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; INTERIOR STRUCTURE; DYNAMICS; WATER; URANUS; AMMONIA; METALS; NEPTUNE AB We have performed finite-temperature density functional theory molecular dynamics simulations on dense methane, ammonia, and water mixtures (CH4:NH3:H2O) for various compositions and temperatures (2000 K <= T <= 10 000 K) that span a set of possible conditions in the interiors of ice-giant exoplanets. The equation-of-state, pair distribution functions, and bond autocorrelation functions (BACF) were used to probe the structure and dynamics of these complex fluids. In particular, an improvement to the choice of the cutoff in the BACF was developed that allowed analysis refinements for density and temperature effects. We note the relative changes in the nature of these systems engendered by variations in the concentration ratios. A basic tenet emerges from all these comparisons that varying the relative amounts of the three heavy components (C,N,O) can effect considerable changes in the nature of the fluid and may in turn have ramifications for the structure and composition of various planetary layers. (C) 2015 AIP Publishing LLC. C1 [Meyer, Edmund R.; Ticknor, Christopher; Kress, Joel D.; Collins, Lee A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Bethkenhagen, Mandy; Redmer, Ronald] Univ Rostock, Inst Phys, D-18501 Rostock, Germany. [Hamel, Sebastien] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Meyer, ER (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM meyere@lanl.gov RI Ticknor, Christopher/B-8651-2014; OI Ticknor, Christopher/0000-0001-9972-4524 FU Advanced Simulation and Computing Program (ASC); U.S. DOE [DE-AC52-06NA25396]; Deutsche Forschungsgemeinschaft (DFG) [SFB 652]; North-German Supercomputing Alliance (HLRN) FX The authors E.R.M, C.T, J.D.K, and L.A.C. gratefully acknowledge support from the Advanced Simulation and Computing Program (ASC), science campaigns 1 and 4. LANL is operated by LANS, LLC for the NNSA of the U.S. DOE under Contract No. DE-AC52-06NA25396. M.B. and R.R. thank the Deutsche Forschungsgemeinschaft (DFG) for support within the SFB 652 as well as the North-German Supercomputing Alliance (HLRN) for computation time. NR 44 TC 0 Z9 0 U1 1 U2 12 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD OCT 28 PY 2015 VL 143 IS 16 AR 164513 DI 10.1063/1.4934626 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CV4KN UT WOS:000364235800042 PM 26520533 ER PT J AU Mitra, C Krogel, JT Santana, JA Reboredo, FA AF Mitra, Chandrima Krogel, Jaron T. Santana, Juan A. Reboredo, Fernando A. TI Many-body ab initio diffusion quantum Monte Carlo applied to the strongly correlated oxide NiO SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID PERIODIC BOUNDARY-CONDITIONS; TRANSITION-METAL OXIDES; NARROW ENERGY-BANDS; ELECTRONIC-STRUCTURE; POINT-DEFECTS; EXCITED-STATES; PSEUDOPOTENTIALS; APPROXIMATION; SIMULATIONS; CRYSTALS AB We present a many-body diffusion quantum Monte Carlo (DMC) study of the bulk and defect properties of NiO. We find excellent agreement with experimental values, within 0.3%, 0.6%, and 3.5% for the lattice constant, cohesive energy, and bulk modulus, respectively. The quasiparticle bandgap was also computed, and the DMC result of 4.72 (0.17) eV compares well with the experimental value of 4.3 eV. Furthermore, DMC calculations of excited states at the L, Z, and the gamma point of the Brillouin zone reveal a flat upper valence band for NiO, in good agreement with Angle Resolved Photoemission Spectroscopy results. To study defect properties, we evaluated the formation energies of the neutral and charged vacancies of oxygen and nickel in NiO. A formation energy of 7.2 (0.15) eV was found for the oxygen vacancy under oxygen rich conditions. For the Ni vacancy, we obtained a formation energy of 3.2 (0.15) eV under Ni rich conditions. These results confirm that NiO occurs as a p-type material with the dominant intrinsic vacancy defect being Ni vacancy. (C) 2015 AIP Publishing LLC. C1 [Mitra, Chandrima; Krogel, Jaron T.; Santana, Juan A.; Reboredo, Fernando A.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Mitra, C (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM reboredofa@ornl.gov OI Santana, Juan A./0000-0003-2349-6312; Krogel, Jaron/0000-0002-1859-181X FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division FX This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 64 TC 3 Z9 3 U1 4 U2 23 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD OCT 28 PY 2015 VL 143 IS 16 AR 164710 DI 10.1063/1.4934262 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CV4KN UT WOS:000364235800055 PM 26520546 ER PT J AU Aubrey, ML Long, JR AF Aubrey, Michael L. Long, Jeffrey R. TI A Dual-Ion Battery Cathode via Oxidative Insertion of Anions in a Metal-Organic Framework SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID LAYERED DOUBLE HYDROXIDES; RECHARGEABLE LITHIUM BATTERIES; ELECTRICAL-CONDUCTIVITY; MIXED-VALENCE; ELECTROCHEMICAL INTERCALATION; SECONDARY BATTERIES; ELECTRODE MATERIALS; GRAPHITE; REDOX; POLYMER AB A redox-active metal-organic framework, Fe-2(dobpdc) (dobpdc(4-) = 4,4'-dioxidobiphenyl-3,3'-dicarboxylate), is shown to undergo a topotactic oxidative insertion reaction with a variety of weakly coordinating anions, including BF4- and PF6-. The reaction results in just a minor lattice contraction, and a broad intervalence charge-transfer band emerges, indicative of charge mobility. Although both metal- and ligand-based oxidations can be accessed, only the former were found to be fully reversible and, importantly, proceed stoichiometrically under both chemical and electrochemical conditions. Electrochemical measurements probing the effects of nanoconfinement on the insertion reaction revealed strong anion size and solvent dependences. Significantly, the anion insertion behavior of Fe-2(dobpdc) enabled its use in the construction of a dual-ion battery prototype incorporating a sodium anode. As a cathode, the material displays a particularly high initial reduction potential and is further stable for at least 50 charge/discharge cycles, exhibiting a maximum specific energy of 316 Wh/kg. C1 [Aubrey, Michael L.; Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Aubrey, Michael L.; Long, Jeffrey R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Long, JR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM jrlong@berkeley.edu FU National Science Foundation [DMR-1309066]; Arkema FX This research was supported by the National Science Foundation under award no. DMR-1309066. We would also like to thank Arkema for fellowship support of M.L.A. NR 61 TC 20 Z9 20 U1 52 U2 214 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD OCT 28 PY 2015 VL 137 IS 42 BP 13594 EP 13602 DI 10.1021/jacs.5b08022 PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA CV0DC UT WOS:000363916600027 PM 26436465 ER PT J AU Beyzavi, MH Vermeulen, NA Howarth, AJ Tussupbayev, S League, AB Schweitzer, NM Gallagher, JR Platero-Prats, AE Hafezi, N Sarjeant, AA Miller, JT Chapman, KW Stoddart, JF Cramer, CJ Hupp, JT Farha, OK AF Beyzavi, M. Hassan Vermeulen, Nicolaas A. Howarth, Ashlee J. Tussupbayev, Samat League, Aaron B. Schweitzer, Neil M. Gallagher, James R. Platero-Prats, Ana E. Hafezi, Nema Sarjeant, Amy A. Miller, Jeffrey T. Chapman, Karena W. Stoddart, J. Fraser Cramer, Christopher J. Hupp, Joseph T. Farha, Omar K. TI A Hafnium-Based Metal-Organic Framework as a Nature-Inspired Tandem Reaction Catalyst SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID BIOMIMETIC CATALYSTS; BETA-AZIDO; ALCOHOLS; ACTIVATION; EFFICIENT; COMPLEX; STORAGE AB Tandem catalytic systems, often inspired by biological systems, offer many advantages in the formation of highly functionalized small molecules. Herein, a new metal-organic framework (MOF) with porphyrinic struts and Hf-6 nodes is reported. This MOP demonstrates catalytic efficacy in the tandem oxidation and functionalization of styrene utilizing molecular oxygen as a terminal oxidant. The product, a protected 1,2-aminoalcohol, is formed selectively and with high efficiency using this recyclable heterogeneous catalyst. Significantly, the unusual regioselective transformation occurs only when an Fe-decorated Hf-6 node and the Fe-porphyrin strut work in concert. This report is an example of concurrent orthogonal tandem catalysis. C1 [Beyzavi, M. Hassan; Vermeulen, Nicolaas A.; Howarth, Ashlee J.; Schweitzer, Neil M.; Hafezi, Nema; Sarjeant, Amy A.; Stoddart, J. Fraser; Hupp, Joseph T.; Farha, Omar K.] Northwestern Univ, Dept Chem, IIN, Evanston, IL 60208 USA. [Beyzavi, M. Hassan; Vermeulen, Nicolaas A.; Howarth, Ashlee J.; Schweitzer, Neil M.; Hafezi, Nema; Sarjeant, Amy A.; Stoddart, J. Fraser; Hupp, Joseph T.; Farha, Omar K.] Northwestern Univ, Dept Chem, CCIS, Evanston, IL 60208 USA. [Tussupbayev, Samat; League, Aaron B.; Cramer, Christopher J.] Univ Minnesota, Dept Chem, Chem Theory Ctr, Minneapolis, MN 55455 USA. [Tussupbayev, Samat; League, Aaron B.; Cramer, Christopher J.] Univ Minnesota, Supercomp Inst, Minneapolis, MN 55455 USA. [Gallagher, James R.; Miller, Jeffrey T.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Miller, Jeffrey T.] Purdue Univ, Sch Chem Engn, W Lafayette, IN 47906 USA. [Platero-Prats, Ana E.; Chapman, Karena W.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Farha, Omar K.] King Abdulaziz Univ, Dept Chem, Fac Sci, Jeddah 22254, Saudi Arabia. RP Stoddart, JF (reprint author), Northwestern Univ, Dept Chem, IIN, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM stoddart@northwestern.edu; cramer@umn.edu; j-hupp@northwestern.edu; o-farha@northwestern.edu RI ID, MRCAT/G-7586-2011; Vermeulen, Nicolaas/B-5622-2016; Gallagher, James/E-4896-2014; BM, MRCAT/G-7576-2011; Cramer, Christopher/B-6179-2011; Platero-Prats, Ana Eva/B-2870-2017; OI Vermeulen, Nicolaas/0000-0003-1825-4474; Gallagher, James/0000-0002-5628-5178; Cramer, Christopher/0000-0001-5048-1859; Platero-Prats, Ana Eva/0000-0002-2248-2739; Tussupbayev, Samat/0000-0003-3470-1510 FU Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences [DE-FG02-12ER16362]; Joint Center of Excellence. in Integrated Nano-Systems (JCIN) at King Abdulaziz City for Science and Technology (KACST) [34-944]; Northwestern University (NU) [34-944]; U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences [DE-AC02-06CH11357]; U.S. Department of Energy, Office of Basic Energy Sciences, Chemical Sciences [DE-AC-02-06CH11357]; KACST; NU; DFG FX We thank Dr. Ben Klahr for obtaining the SEM images used and the Integrated Molecular Structure Education and Research Center (IMSERC) at Northwestern University for use of its chemical characterization facilities. O.K.F., C.J.C., and J.T.H.: This work (MOP assembly, experimental characterization, catalysis, and modeling) was supported as part of Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences under Award DE-FG02-12ER16362. J.F.S: This research is part (Project 34-944) of the Joint Center of Excellence. in Integrated Nano-Systems (JCIN) at King Abdulaziz City for Science and Technology (KACST) and Northwestern University (NU). Use of the Advanced Photon Source is supported by the U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. Materials Research Collaborative Access Team (MRCAT, Sectors 10 BM and 10 ID) operations are supported by the Department of Energy and the MRCAT member institutions. J.T.M. and J.R.G. were supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Chemical Sciences under Contract DE-AC-02-06CH11357. We thank both KACST and NU for their continued support of this research. M.H.B. thanks DFG for a Postdoctoral Research Fellowship Award. NR 50 TC 19 Z9 20 U1 35 U2 125 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD OCT 28 PY 2015 VL 137 IS 42 BP 13624 EP 13631 DI 10.1021/jacs.5b03440 PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA CV0DC UT WOS:000363916600030 PM 26434603 ER PT J AU Tang, Z Senkov, ON Parish, CM Zhang, C Zhang, F Santodonato, LJ Wang, GY Zhao, GF Yang, FQ Liaw, PK AF Tang, Zhi Senkov, Oleg N. Parish, Chad M. Zhang, Chuan Zhang, Fan Santodonato, Louis J. Wang, Gongyao Zhao, Guangfeng Yang, Fuqian Liaw, Peter K. TI Tensile ductility of an AlCoCrFeNi multi-phase high-entropy alloy through hot isostatic pressing (HIP) and homogenization SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE High-entropy alloys; Microstructures; Tensile properties; Heat treatment; Thermodynamic modeling; Crack initiation ID PRINCIPAL ELEMENT ALLOYS; V-ZR SYSTEM; MECHANICAL-PROPERTIES; PHASE-STABILITY; SIGMA-PHASE; COMPUTATIONAL THERMODYNAMICS; ELEVATED-TEMPERATURES; CORROSION BEHAVIOR; STAINLESS-STEEL; AL ADDITION AB The microstructure and phase composition of an AlCoCrFeNi high-entropy alloy (HEA) were studied in as-cast (AlCoCrFeNi-AC, AC represents as-cast) and homogenized (AlCoCrFeNi-HP, HP signifies hot iso-static pressed and homogenized) conditions. The AlCoCrFeNi-AC ally has a dendritric structure in the consisting primarily of a nano-lamellar mixture of A2 (disordered body-centered-cubic (BCC)) and B2 (ordered BCC) phases, formed by an eutectic reaction. The homogenization heat treatment, consisting of hot isostatic pressed for 1 h at 1100 degrees C, 207 MPa and annealing at 1150 degrees C for 50 h, resulted in an increase in the volume fraction of the A1 phase and formation of a Sigma (sigma) phase. Tensile properties in as-cast and homogenized conditions are reported at 700 degrees C. The ultimate tensile strength was virtually unaffected by heat treatment, and was 396 +/- 4 MPa at 700 degrees C. However, homogenization produced a noticeable increase in ductility. The AlCoCrFeNi-AC alloy showed a tensile elongation of only 1.0%, while after the heat-treatment, the elongation of AlCoCrFeNi-HP was 11.7%. Thermodynamic modeling of nonequilibrium and equilibrium phase diagrams for the AlCoCrFeNi HEA gave good agreement with the experimental observations of the phase contents in the AlCoCrFeNi-AC and AlCoCrFeNi-HP. The reasons for the improvement of ductility after the heat treatment and the crack initiation subjected to tensile loading were discussed. Published by Elsevier B.V. C1 [Tang, Zhi; Santodonato, Louis J.; Wang, Gongyao; Liaw, Peter K.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Tang, Zhi] Virginia Tech, Dept Mat Sci & Engn, Blacksburg, VA 24061 USA. [Senkov, Oleg N.] Air Force Res Lab, Mat & Mfg Directorate, Wright Patterson AFB, OH 45433 USA. [Parish, Chad M.; Santodonato, Louis J.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Zhang, Chuan; Zhang, Fan] CompuTherrn LLC, Madison, WI 53719 USA. [Zhao, Guangfeng; Yang, Fuqian] Univ Kentucky, Dept Chem & Mat Engn, Lexington, KY 40506 USA. RP Tang, Z (reprint author), Alcoa Tech Ctr, Alloy Technol Div, 100 Tech Dr, Alcoa Ctr, PA 15069 USA. EM Zhi.Tang@alcoa.com; pliaw@utk.edu RI Parish, Chad/J-8381-2013; Santodonato, Louis/A-9523-2015; OI Santodonato, Louis/0000-0002-4600-685X; Senkov, Oleg/0000-0001-5587-415X FU Department of Energy (DOE) Office of Nuclear Energy's Nuclear Energy University Program (NEUP) [00119262]; DOE, Office of Fossil Energy, National Energy Technology Laboratory [DE-FE-0008855, DE-FE-0011194, DE-FE-0024054]; U.S. Army Research Office project [W911NF-13-1-3080438]; United States Air Force (USAF) [FA8650-10-D-5226]; Oak Ridge National Laboratory (ORNL)'s Shared Research Equipment (ShaRE) User Program - Office of Basic Energy Sciences, U.S. Department of Energy FX The authors very much appreciate the original proposed idea of this work from D.B. Miracle of the Air Force Research Laboratory (AFRL) and his many great comments and discussions on this paper. ZT, LJS, GW, and PKL would like to acknowledge the financial support from the Department of Energy (DOE) Office of Nuclear Energy's Nuclear Energy University Program (NEUP) 00119262, and the DOE, Office of Fossil Energy, National Energy Technology Laboratory (DE-FE-0008855, DE-FE-0011194, and DE-FE-0024054), with R.O. Jensen, Jr., L. Tian, V. Cedro, S. Lesica, S. Markovich, J. Mullen, and R. Dunst as program managers. PKL thanks the U.S. Army Research Office project (W911NF-13-1-3080438) with the program manager, S.N. Mathaudhu and D.M. Stepp. The authors also gratefully acknowledge D. Robinson of the Advanced Photon Source CAPS) in the Argonne National Laboratory for assistance with the high-energy X-ray diffraction measurements, D. Fielden, M. Bharadwaj and G. Jones of The University of Tennessee (UT) for the technical support. ZT very much appreciates C.P. Chuang, J.E. Spruiell, and C.D. Lundin of UT, J.S. Hou of the Chinese Academy of Sciences, J.W. Qiao of Taiyuan University of Technology China, M.C. Gao of the National Energy Technology Laboratory (NETL) for helpful discussions. Work at AFRL was supported through the United States Air Force (USAF) Contract no. FA8650-10-D-5226. Research sponsored by the Oak Ridge National Laboratory (ORNL)'s Shared Research Equipment (ShaRE) User Program, which was sponsored by the Office of Basic Energy Sciences, U.S. Department of Energy (C.M. Parish). The authors very much appreciate M.K. Miller of ORNL for his efforts on the atom-probe tomography (APT). NR 77 TC 16 Z9 16 U1 25 U2 70 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD OCT 28 PY 2015 VL 647 BP 229 EP 240 DI 10.1016/j.msea.2015.08.078 PG 12 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA CV4PX UT WOS:000364250100029 ER PT J AU Brewer, LN Bennett, MS Baker, BW Payzant, EA Sochalski-Kolbus, LM AF Brewer, L. N. Bennett, M. S. Baker, B. W. Payzant, E. A. Sochalski-Kolbus, L. M. TI Characterization of residual stress as a function of friction stir welding parameters in oxide dispersion strengthened (ODS) steel MA956 SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE ODS steel; Residual stress; Friction stir welding; X-ray diffraction; Neutron diffraction ID MECHANICAL-PROPERTIES; MICROSTRUCTURE; ALLOY; TEMPERATURE; EVOLUTION; JOINTS; SPEED AB Friction stir welding (FSW) can generate large residual stresses during solid state joining of oxide dispersion strengthened steels. In this work, a plate of MA956 steel was friction stir welded at three conditions: 500 rpm/25 mm per minute (mmpm), 400 rpm/50 mmpm and 400 rpm/100 mmpm. The residual stresses across these welds were measured using both x-ray and neutron diffraction techniques. The distribution and magnitude of the residual stresses agreed well between the two techniques. Longitudinal residual stresses up to eighty percent of the yield strength were observed for the 400 rpm/100 mmpm condition. The surface residual stresses were somewhat larger on the root side of the weld than on the crown side. Increases in the relative heat input during FSW decreased the measured residual stresses in the stir zone and the thermomechanically affected zone (TMAZ). Increasing the traverse rate while holding the rotational speed fixed increased the residual stress levels. The fatigue strength of the material is predicted to decrease by at least twenty percent with cracking most likely in the TMAZ. (C) 2015 Elsevier B.V. All rights reserved. C1 [Brewer, L. N.; Bennett, M. S.; Baker, B. W.] Naval Postgrad Sch, Monterey, CA 93943 USA. [Payzant, E. A.; Sochalski-Kolbus, L. M.] Oak Ridge Natl Lab, Oak Ridge, TN USA. RP Brewer, LN (reprint author), Naval Postgrad Sch, Monterey, CA 93943 USA. EM lnbrewer1@eng.ua.edu RI Payzant, Edward/B-5449-2009 OI Payzant, Edward/0000-0002-3447-2060 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy FX This work was performed in part under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. The two plates measured in this study were provided by Lawrence Livermore National Laboratories. We are grateful for technical assistance from Dr. E.S.K. Menon at NPS and Dr. M. Mahoney at MegaStir Technologies.; Research conducted at ORNL's High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. NR 28 TC 1 Z9 2 U1 3 U2 15 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD OCT 28 PY 2015 VL 647 BP 313 EP 321 DI 10.1016/j.msea.2015.09.020 PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA CV4PX UT WOS:000364250100038 ER PT J AU Muraguchi, H Umezawa, K Niikura, M Yoshida, M Kozaki, T Ishii, K Sakai, K Shimizu, M Nakahori, K Sakamoto, Y Choi, C Ngan, CY Lindquist, E Lipzen, A Tritt, A Haridas, S Barry, K Grigoriev, IV Pukkila, PJ AF Muraguchi, Hajime Umezawa, Kiwamu Niikura, Mai Yoshida, Makoto Kozaki, Toshinori Ishii, Kazuo Sakai, Kiyota Shimizu, Motoyuki Nakahori, Kiyoshi Sakamoto, Yuichi Choi, Cindy Ngan, Chew Yee Lindquist, Eika Lipzen, Anna Tritt, Andrew Haridas, Sajeet Barry, Kerrie Grigoriev, Igor V. Pukkila, Patricia J. TI Strand-Specific RNA-Seq Analyses of Fruiting Body Development in Coprinopsis cinerea SO PLOS ONE LA English DT Article ID BASIDIOMYCETE COPRINUS-CINEREUS; SCHIZOPHYLLUM-COMMUNE; SEXUAL DEVELOPMENT; TRANSCRIPTION FACTORS; LENTINULA-EDODES; GENE-EXPRESSION; MUSHROOM; MORPHOGENESIS; ENCODES; FUNGI AB The basidiomycete fungus Coprinopsis cinerea is an important model system for multicellular development. Fruiting bodies of C. cinerea are typical mushrooms, which can be produced synchronously on defined media in the laboratory. To investigate the transcriptome in detail during fruiting body development, high-throughput sequencing (RNA-seq) was performed using cDNA libraries strand-specifically constructed from 13 points (stages/tissues) with two biological replicates. The reads were aligned to 14,245 predicted transcripts, and counted for forward and reverse transcripts. Differentially expressed genes (DEGs) between two adjacent points and between vegetative mycelium and each point were detected by Tag Count Comparison (TCC). To validate RNA-seq data, expression levels of selected genes were compared using RPKM values in RNA-seq data and qRT-PCR data, and DEGs detected in microarray data were examined in MA plots of RNA-seq data by TCC. We discuss events deduced from GO analysis of DEGs. In addition, we uncovered both transcription factor candidates and antisense transcripts that are likely to be involved in developmental regulation for fruiting. C1 [Muraguchi, Hajime] Akita Prefectural Univ, Fac Bioresource Sci, Dept Biotechnol, Akita 0100195, Japan. [Umezawa, Kiwamu; Niikura, Mai; Yoshida, Makoto] Tokyo Univ Agr & Technol, Dept Environm & Nat Resource Sci, Fac Agr, Fuchu, Tokyo 1838509, Japan. [Kozaki, Toshinori; Ishii, Kazuo] Tokyo Univ Agr & Technol, Fac Agr, Dept Appl Biol Sci, Fuchu, Tokyo 1838509, Japan. [Sakai, Kiyota; Shimizu, Motoyuki] Meijo Univ, Fac Agr, Dept Appl Biol Chem, Nagoya, Aichi 4680073, Japan. [Nakahori, Kiyoshi] Okayama Univ, Grad Sch Nat Sci & Technol, Okayama 7008530, Japan. [Sakamoto, Yuichi] Iwate Biotechnol Res Ctr, Kitakami, Iwate 0240003, Japan. [Choi, Cindy; Ngan, Chew Yee; Lindquist, Eika; Lipzen, Anna; Tritt, Andrew; Haridas, Sajeet; Barry, Kerrie; Grigoriev, Igor V.] US Dept Energy Joint Genome Inst, Walnut Creek, CA 94598 USA. [Pukkila, Patricia J.] Univ N Carolina, Dept Biol, Chapel Hill, NC 27599 USA. RP Muraguchi, H (reprint author), Akita Prefectural Univ, Fac Bioresource Sci, Dept Biotechnol, Akita 0100195, Japan. EM muraguchi@akita-pu.ac.jp RI Yoshida, Makoto/E-8017-2013; Ishii, Kazuo/M-3099-2016 OI Ishii, Kazuo/0000-0002-8363-8266 FU Office of Science of the US Department of Energy [DE-AC02-05CH11231]; Ministry of Agriculture, Forestry and Fisheries of Japan [23053] FX The #326 AmutBmut pab1-1 genome sequencing, assembly and annotation, and the RNA-seq analysis were provided through JGI's Community Sequencing Program "Functional genomics in the model mushroom Coprinopsis cinerea". The work conducted by the US Department of Energy Joint Genome Institute is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. This work was supported in part (preparation of total RNA, and sending the samples from Japna to USA) by a fund from the Ministry of Agriculture, Forestry and Fisheries of Japan (23053). NR 62 TC 4 Z9 4 U1 8 U2 21 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD OCT 28 PY 2015 VL 10 IS 10 AR e0141586 DI 10.1371/journal.pone.0141586 PG 23 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CV0DL UT WOS:000363918100109 PM 26510163 ER PT J AU Ying, S Zeng, DN Chi, L Tan, Y Galzote, C Cardona, C Lax, S Gilbert, J Quan, ZX AF Ying, Shi Zeng, Dan-Ning Chi, Liang Tan, Yuan Galzote, Carlos Cardona, Cesar Lax, Simon Gilbert, Jack Quan, Zhe-Xue TI The Influence of Age and Gender on Skin-Associated Microbial Communities in Urban and Rural Human Populations SO PLOS ONE LA English DT Article ID MOLECULAR ANALYSIS; BODY HABITATS; DIVERSITY; BACTERIAL; SEQUENCES; TAXONOMY; SAMPLES; FLORA; TIME; LIFE AB Differences in the bacterial community structure associated with 7 skin sites in 71 healthy people over five days showed significant correlations with age, gender, physical skin parameters, and whether participants lived in urban or rural locations in the same city. While body site explained the majority of the variance in bacterial community structure, the composition of the skin-associated bacterial communities were predominantly influenced by whether the participants were living in an urban or rural environment, with a significantly greater relative abundance of Trabulsiella in urban populations. Adults maintained greater overall microbial diversity than adolescents or the elderly, while the intragroup variation among the elderly and rural populations was significantly greater. Skin-associated bacterial community structure and composition could predict whether a sample came from an urban or a rural resident similar to 5x greater than random. C1 [Ying, Shi; Zeng, Dan-Ning; Chi, Liang; Quan, Zhe-Xue] Fudan Univ, Dept Microbiol & Microbial Engn, Sch Life Sci, Shanghai 200433, Peoples R China. [Tan, Yuan; Galzote, Carlos] Johnson & Johnson China Ltd, Sci Affairs, Shanghai, Peoples R China. [Cardona, Cesar; Gilbert, Jack] Univ Chicago, Grad Program Biophys Sci, Chicago, IL 60637 USA. [Lax, Simon; Gilbert, Jack] Univ Chicago, Dept Ecol & Evolut, Chicago, IL 60637 USA. [Gilbert, Jack] Argonne Natl Lab, Inst Genom & Syst Biol, Argonne, IL 60439 USA. [Gilbert, Jack] Marine Biol Lab, Woods Hole, MA 02543 USA. [Gilbert, Jack] Zhejiang Univ, Coll Environm & Resource Sci, Hangzhou 310003, Zhejiang, Peoples R China. RP Quan, ZX (reprint author), Fudan Univ, Dept Microbiol & Microbial Engn, Sch Life Sci, Shanghai 200433, Peoples R China. EM quanzx@fudan.edu.cn FU Johnson & Johnson (China); Johnson & Johnson Consumer Companies, Inc. (Skillman, NJ USA) FX This work was supported by a grant from Johnson & Johnson (China). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. The funder provided support in the form of salaries for investigator/authors [YT, CG], but did not have any additional role in the study design, data collection and analysis, decision to publish. The specific roles of these authors are articulated in the 'author contributions' section. Editorial services were provided by Evidence Scientific Solutions (Philadelphia, PA) and were funded by Johnson & Johnson Consumer Companies, Inc. (Skillman, NJ USA). NR 37 TC 9 Z9 9 U1 1 U2 6 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD OCT 28 PY 2015 VL 10 IS 10 AR e0141842 DI 10.1371/journal.pone.0141842 PG 16 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CV0DL UT WOS:000363918100139 PM 26510185 ER PT J AU Song, HS Liu, CX AF Song, Hyun-Seob Liu, Chongxuan TI Dynamic Metabolic Modeling of Denitrifying Bacterial Growth: The Cybernetic Approach SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID MICROBIAL-GROWTH; SUBSTRATE SYSTEMS; CULTURES; PREDICTION; DENITRIFICATION; MULTIPLICITY; PERSPECTIVE; BEHAVIOR; MODES; RATES AB Denitrification is a multistage reduction process converting nitrate ultimately to nitrogen gas, carried out mostly by facultative bacteria. Modeling of the denitrification process is challenging due to the complex metabolic regulation that modulates sequential formation and consumption of a series of nitrogen oxide intermediates, which serve as the final electron acceptors for denitrifying bacteria. In this work, we examined the effectiveness and accuracy of the cybernetic modeling framework in simulating the growth dynamics of denitrifying bacteria in comparison with kinetic models. In four different case studies using the literature data, we successfully simulated diauxic and triauxic growth patterns observed in anoxic and aerobic conditions, only by tuning two or three parameters. In order to understand the regulatory structure of the cybernetic model, we systematically analyzed the effect of cybernetic control variables on simulation accuracy. The results showed that the consideration of both enzyme synthesis and activity control through u- and v-variables is necessary and relevant and that u-variables are of greater importance in comparison to v-variables. In contrast, simple kinetic models were unable to accurately capture dynamic metabolic shifts across alternative electron acceptors, unless an inhibition term was additionally incorporated. Therefore, the denitrification process represents a reasonable example highlighting the criticality of considering dynamic regulation for successful metabolic modeling. C1 [Song, Hyun-Seob; Liu, Chongxuan] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Song, HS (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM hyunseob.song@pnnl.gov RI Liu, Chongxuan/C-5580-2009 FU U.S. Department of Energy (DOE) Office of Biological and Environmental Research (BER), as part of Foundational Scientific Focus Area (SEA); Subsurface Biogeochemistry Research Program's SPA at the Pacific Northwest National Laboratory (PNNL); DOE [DE-AC06-76RLO 1830] FX This research was supported by the U.S. Department of Energy (DOE) Office of Biological and Environmental Research (BER), as part of Foundational Scientific Focus Area (SEA) and Subsurface Biogeochemistry Research Program's SPA at the Pacific Northwest National Laboratory (PNNL). PNNL is operated for the DOE by Battelle Memorial Institute under Contract DE-AC06-76RLO 1830. NR 35 TC 0 Z9 0 U1 4 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD OCT 28 PY 2015 VL 54 IS 42 BP 10221 EP 10227 DI 10.1021/acs.iecr.5b01615 PG 7 WC Engineering, Chemical SC Engineering GA CV0DG UT WOS:000363917000010 ER PT J AU Liu, XP Zhang, HH Nayak, S Parada, G Anderegg, J Feng, SR Nilsen-Hamilton, M Akinc, M Mallapragada, SK AF Liu, Xunpei Zhang, Honghu Nayak, Srikanth Parada, German Anderegg, James Feng, Shuren Nilsen-Hamilton, Marit Akinc, Mufit Mallapragada, Surya K. TI Effect of Surface Hydrophobicity on the Function of the Immobilized Biomineralization Protein Mms6 SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID MULTIFUNCTIONAL MAGNETIC NANOPARTICLES; MAGNETOTACTIC BACTERIUM; BIOMEDICAL APPLICATIONS; MAGNETOSOME FORMATION; IRON-BINDING; GOLD; NANOCRYSTALS; FUNCTIONALIZATION; NANOSTRUCTURES; ADSORPTION AB Magnetotactic bacteria produce magnetic nanocrystals with uniform shapes and sizes in nature, which has inspired in vitro synthesis of uniformly sized magnetite nanocrystals under mild conditions. Mms6, a biomineralization protein from magnetotactic bacteria with a hydrophobic N-terminal domain and a hydrophilic C-terminal domain, can promote formation of magnetite nanocrystals in vitro with well-defined shape and size in gels under mild conditions. Here we investigate the role of surface hydrophobicity on the ability of Mms6 to template magnetite nanoparticle formation on surfaces. Our results confirmed that Mms6 can form a protein network structure on a monolayer of hydrophobic octadecanethiol (ODT)-coated gold surfaces and facilitate magnetite nanocrystal formation with uniform sizes close to those seen in nature, in contrast to its behavior on more hydrophilic surfaces. We propose that this hydrophobicity effect might be due to the amphiphilic nature of the Mms6 protein and its tendency to incorporate the hydrophobic N-terminal domain into the hydrophobic lipid bilayer environment of the magnetosome membrane, exposing the hydrophilic C-terminal domain that promotes biomineralization. Supporting this hypothesis, the larger and well-formed magnetite nanoparticles were found to be preferentially located on ODT surfaces covered with Mms6 as compared to control samples, as characterized by scanning electron microscopy, X-ray diffraction, X-ray photoelectron spectroscopy, and atomic force microscopy studies. A C-terminal domain mutant of this protein did not form the same network structure as wild-type Mms6, suggesting that the network structure is important for the magnetite nanocrystal formation. This study provides valuable insights into the role of surface hydrophilidty on the action of the biomineralization protein Mms6 to synthesize magnetic nanocrystals and provides a facile route to controlling bioinspired nanocrystal synthesis in vitro. C1 [Liu, Xunpei; Zhang, Honghu; Nayak, Srikanth; Anderegg, James; Feng, Shuren; Nilsen-Hamilton, Marit; Akinc, Mufit; Mallapragada, Surya K.] Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA. [Liu, Xunpei; Nayak, Srikanth; Parada, German; Mallapragada, Surya K.] Iowa State Univ, Dept Chem & Biol Engn, Ames, IA 50011 USA. [Zhang, Honghu; Akinc, Mufit] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Feng, Shuren; Nilsen-Hamilton, Marit] Iowa State Univ, Roy J Carver Dept Biochem Biophys & Mol Biol, Ames, IA 50011 USA. RP Mallapragada, SK (reprint author), Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA. EM suryakm@iastate.edu FU U.S. Department of Energy, Office of the Basic Energy Sciences, Division of Materials Sciences and Engineering; U.S. Department of Energy [DE-AC02-07CH11358, DE-AC02-06CH11357] FX S.K.M. is grateful for the inspiration provided by Prof. Doraiswami Ramkrishna through his outstanding body of work and through his graduate teaching at Purdue that directly impacted her. We thank Pierre Palo from M.N.-H.'s group at Ames Laboratory for preparing the Mms6 protein preparations. Research at Ames Laboratory was supported by the U.S. Department of Energy, Office of the Basic Energy Sciences, Division of Materials Sciences and Engineering. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract Number DE-AC02-07CH11358. The use of Magnetic Force Microscopy at the Argonne National Laboratory was supported by the U.S. Department of Energy under Contract Number DE-AC02-06CH11357. NR 47 TC 3 Z9 3 U1 5 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD OCT 28 PY 2015 VL 54 IS 42 BP 10284 EP 10292 DI 10.1021/acs.iecr.5b01413 PG 9 WC Engineering, Chemical SC Engineering GA CV0DG UT WOS:000363917000016 ER PT J AU Lin, RH Ladshaw, A Nan, Y Liu, JX Yiacoumi, S Tsouris, C DePaoli, DW Tavlarides, LL AF Lin, Ronghong Ladshaw, Austin Nan, Yue Liu, Jiuxu Yiacoumi, Sotira Tsouris, Costas DePaoli, David W. Tavlarides, Lawrence L. TI Isotherms for Water Adsorption on Molecular Sieve 3A: Influence of Cation Composition SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID SILICA-GEL; ZEOLITE-A; REMOVAL; VAPOR AB This work is part of our continuing efforts to address engineering issues related to the removal of tritiated water from off-gases produced in used nuclear fuel reprocessing facilities. In the current study, adsorption equilibrium of water on molecular sieve 3A beads was investigated. Adsorption isotherms for water on the UOP molecular sieve 3A were measured by a continuous-flow adsorption system at 298, 313, 333, and 353 K. Experimental data collected were analyzed by the Generalized Statistical Thermodynamic Adsorption (GSTA) isotherm model. The K+/Na+ molar ratio of this particular type of molecular sieve 3A was similar to 4:6. Our results showed that the GSTA isotherm model worked very well to describe the equilibrium behavior of water adsorption on molecular sieve 3A. The optimum number of parameters for the current experimental data was determined to be a set of four equilibrium parameters. This result suggests that the adsorbent crystals contain four energetically distinct adsorption sites. In addition, it was found that water adsorption on molecular sieve 3A follows a three-stage adsorption process. This three-stage adsorption process confirmed different water adsorption sites in molecular sieve crystals. The second adsorption stage is significantly affected by the K+/Na+ molar ratio. In this stage, the equilibrium adsorption capacity at a given water vapor pressure increases as the K+/Na+ molar ratio increases. C1 [Lin, Ronghong; Nan, Yue; Liu, Jiuxu; Tavlarides, Lawrence L.] Syracuse Univ, Dept Biomed & Chem Engn, Syracuse, NY 13244 USA. [Ladshaw, Austin; Yiacoumi, Sotira; Tsouris, Costas] Georgia Inst Technol, Sch Civil & Environm Engn, Atlanta, GA 30332 USA. [Tsouris, Costas; DePaoli, David W.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Tavlarides, LL (reprint author), Syracuse Univ, Dept Biomed & Chem Engn, 329 Link Hall, Syracuse, NY 13244 USA. EM lltavlar@syr.edu RI Tsouris, Costas/C-2544-2016; Lin, Ronghong/D-4187-2011; OI Tsouris, Costas/0000-0002-0522-1027; Lin, Ronghong/0000-0002-4902-0761; Nan, Yue/0000-0001-8731-3568 FU U.S. DOE Office of Nuclear Energy's Nuclear Energy University Programs [NFE-12-03822] FX This research was performed using funding received from the U.S. DOE Office of Nuclear Energy's Nuclear Energy University Programs (Grant No. NFE-12-03822). Grace Davison is acknowledged for providing us molecular sieve 3A samples. NR 20 TC 2 Z9 2 U1 7 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD OCT 28 PY 2015 VL 54 IS 42 BP 10442 EP 10448 DI 10.1021/acs.iecr.5b01411 PG 7 WC Engineering, Chemical SC Engineering GA CV0DG UT WOS:000363917000028 ER PT J AU Bodwin, GT Chung, HS Kim, UR Lee, J AF Bodwin, Geoffrey T. Chung, Hee Sok Kim, U-Rae Lee, Jungil TI Fragmentation contributions to J/psi photoproduction at HERA SO PHYSICAL REVIEW D LA English DT Article ID PLUS JET PHOTOPRODUCTION; GLUON FRAGMENTATION; P(P)OVER-BAR COLLISIONS; PERTURBATION-THEORY; HEAVY QUARKONIUM; MESONS; PHOTON; TEV; SCATTERING; NLO AB We compute leading-power fragmentation corrections to J/psi photoproduction at DESY HERA, making use of the nonrelativistic QCD factorization approach. Our calculations include parton production cross sections through order alpha(2)(s), fragmentation functions though order alpha(2)(s), and leading logarithms of the transverse momentum divided by the charm-quark mass to all orders in as. We find that the leading-power fragmentation corrections, beyond those that are included through next-to-leading order in as, are small relative to the fixed-order contributions through next-to-leading order in as. Consequently, an important discrepancy remains between the experimental measurements of the J/psi photoproduction cross section and predictions that make use of nonrelativistic-QCD long-distance matrix elements that are extracted from the J/psi hadroproduction cross-section and polarization data. C1 [Bodwin, Geoffrey T.; Chung, Hee Sok] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Kim, U-Rae; Lee, Jungil] Korea Univ, Dept Phys, Seoul 136701, South Korea. RP Bodwin, GT (reprint author), Argonne Natl Lab, Div High Energy Phys, 9700 South Cass Ave, Argonne, IL 60439 USA. FU U.S. Department of Energy, Division of High Energy Physics [DE-AC02-06CH11357]; National Research Foundation of Korea [NRF-2012R1A1A2008983] FX We thank Mathias Butenschon and Bernd Kniehl for supplying detailed numerical results from their NLO calculations of the photoproduction SDCs. We also thank Michel Fontannaz for advice regarding the use of the EPHOX code and Michel Fontannaz and Jean-Philippe Guillet for providing a version of the EPHOX code that contains the AFG04 photon parton distributions. The work of G. T. B. and H. S. C. is supported by the U.S. Department of Energy, Division of High Energy Physics, under Contract No. DE-AC02-06CH11357. The work of U-R. K. is supported by the National Research Foundation of Korea under Contract No. NRF-2012R1A1A2008983. J. L. and U-R. K. thank APCTP for its hospitality through the CAT program. The submitted manuscript has been created in part by UChicago Argonne, LLC, Operator of Argonne National Laboratory. Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. NR 42 TC 2 Z9 2 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 28 PY 2015 VL 92 IS 7 AR 074042 DI 10.1103/PhysRevD.92.074042 PG 7 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CU4VC UT WOS:000363527500003 ER PT J AU Ding, HT Mukherjee, S Ohno, H Petreczky, P Schadler, HP AF Ding, H. -T. Mukherjee, Swagato Ohno, H. Petreczky, P. Schadler, H. -P. TI Diagonal and off-diagonal quark number susceptibilities at high temperatures SO PHYSICAL REVIEW D LA English DT Article ID QCD; THERMODYNAMICS; LATTICE AB We present continuum extrapolated lattice QCD results for up to fourth-order diagonal and off-diagonal quark number susceptibilities in the high temperature region of 300-700 MeV. Lattice QCD calculations are performed using 2 + 1 flavors of highly improved staggered quarks with nearly physical quark masses and at four different lattice spacings. Comparisons of our results with recent weak coupling calculations yield reasonably good agreements for the entire temperature range. C1 [Ding, H. -T.] Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China. [Ding, H. -T.] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China. [Mukherjee, Swagato; Ohno, H.; Petreczky, P.; Schadler, H. -P.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Ohno, H.] Univ Tsukuba, Ctr Computat Sci, Tsukuba, Ibaraki 3058577, Japan. [Schadler, H. -P.] Graz Univ, Inst Phys, A-8010 Graz, Austria. RP Ding, HT (reprint author), Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China. OI Mukherjee, Swagato/0000-0002-3824-1008; Ding, Heng-Tong/0000-0003-0590-081X FU U.S. Department of Energy [DE-SC0012704]; FWF [DK W1203] FX This work was supported by U.S. Department of Energy under Contract No. DE-SC0012704. H.-P. Schadler was funded by the FWF DK W1203, "Hadrons in Vacuum, Nuclei and Stars." The authors thank F. Karsch and P. Steinbrecher for interesting discussions. The numerical computations have been carried out on the clusters of USQCD Collaboration, on the BlueGene supercomputers at the New York Center for Computational Sciences and on Vienna Scientific Cluster. The calculations have been performed using the publicly available MILC code. We thank S. Mogliacci and N. Haque for sending the numerical values of their calculations. NR 37 TC 14 Z9 14 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 28 PY 2015 VL 92 IS 7 AR 074043 DI 10.1103/PhysRevD.92.074043 PG 7 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CU4VC UT WOS:000363527500004 ER PT J AU Huang, P Ismail, A Low, I Wagner, CEM AF Huang, Peisi Ismail, Ahmed Low, Ian Wagner, Carlos E. M. TI Same-sign dilepton excesses and light top squarks SO PHYSICAL REVIEW D LA English DT Article ID MODEL HIGGS-BOSON; PP COLLISIONS; SEARCH; MASS; LHC; TEV AB Run 1 data of the Large Hadron Collider (LHC) contain excessive events in the same-sign dilepton channel with b-jets and missing transverse energy (MET), which were observed by five separate analyses from the ATLAS and CMS collaborations. We show that these events could be explained by direct production of top squarks in supersymmetry. In particular, a right-handed top squark with a mass of 550 GeV decaying into 2 t quarks, 2 W bosons, and MET could fit the observed excess without being constrained by other direct search limits from Run 1. We propose kinematic cuts at 13 TeV to enhance the top squark signal, and estimate that top squarks could be discovered with 40 fb(-1) of integrated luminosity at Run 2 of the LHC, when considering only the statistical uncertainty. C1 [Huang, Peisi; Wagner, Carlos E. M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Huang, Peisi; Ismail, Ahmed; Low, Ian; Wagner, Carlos E. M.] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Ismail, Ahmed] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. [Low, Ian] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [Wagner, Carlos E. M.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. RP Huang, P (reprint author), Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. OI Huang, Peisi/0000-0003-3360-2641 FU U.S. Department of Energy [DE-AC02-06CH11357, DE-FG02-12ER41811, DE-FG02-04ER41286, DE-SC0010143] FX We thank Stefania Gori for collaborations in the early stage of this work. Useful discussions with Frank Golf, Ben Hooberman, Aurelio Juste, Kevin Lannon, Jeremy Love, Sasha Paramonov and Michael Ramsey-Musolf are gratefully acknowledged. Work at ANL is supported by the U.S. Department of Energy under Grant No. DE-AC02-06CH11357. A. I. is partially supported in part by the U.S. Department of Energy under Grant No. DE-FG02-12ER41811. P. H. is partially supported by U.S. Department of Energy Grant No. DE-FG02-04ER41286. I. L. is supported in part by the U.S. Department of Energy under Grant No. DE-SC0010143. NR 38 TC 7 Z9 7 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 28 PY 2015 VL 92 IS 7 AR 075035 DI 10.1103/PhysRevD.92.075035 PG 6 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CU4VC UT WOS:000363527500008 ER PT J AU Lees, JP Poireau, V Tisserand, V Grauges, E Palano, A Eigen, G Stugu, B Brown, DN Kerth, LT Kolomensky, YG Lee, MJ Lynch, G Koch, H Schroeder, T Hearty, C Mattison, TS McKenna, JA So, RY Khan, A Blinov, VE Buzykaev, AR Druzhinin, VP Golubev, VB Kravchenko, EA Onuchin, AP Serednyakov, SI Skovpen, YI Solodov, EP Todyshev, KY Lankford, AJ Dey, B Gary, JW Long, O Sevilla, MF Hong, TM Kovalskyi, D Richman, JD West, CA Eisner, AM Lockman, WS Vazquez, WP Schumm, BA Seiden, A Chao, DS Cheng, CH Echenard, B Flood, KT Hitlin, DG Kim, J Miyashita, TS Ongmongkolkul, P Porter, FC Rohrken, M Andreassen, R Huard, Z Meadows, BT Pushpawela, BG Sokoloff, MD Sun, L Ford, WT Smith, JG Wagner, SR Ayad, R Toki, WH Spaan, B Bernard, D Verderi, M Playfer, S Bettoni, D Bozzi, C Calabrese, R Cibinetto, G Fioravanti, E Garzia, I Luppi, E Piemontese, L Santoro, V Calcaterra, A de Sangro, R Finocchiaro, G Martellotti, S Patteri, P Peruzzi, IM Piccolo, M Zallo, A Contri, R Monge, MR Passaggio, S Patrignani, C Bhuyan, B Prasad, V Adametz, A Uwer, U Lacker, HM Mallik, U Chen, C Cochran, J Prell, S Ahmed, H Gritsan, AV Arnaud, N Davier, M Derkach, D Grosdidier, G Le Diberder, F Lutz, AM Malaescu, B Roudeau, P Stocchi, A Wang, LL Wormser, G Lange, DJ Wright, DM Coleman, JP Fry, JR Gabathuler, E Hutchcroft, DE Payne, DJ Touramanis, C Bevan, AJ Di Lodovico, F Sacco, R Cowan, G Brown, DN Davis, CL Denig, AG Fritsch, M Gradl, W Griessinger, K Hafner, A Schubert, KR Barlow, RJ Lafferty, GD Cenci, R Hamilton, B Jawahery, A Roberts, DA Cowan, R Cheaib, R Patel, PM Robertson, SH Neri, N Palombo, F Cremaldi, L Godang, R Summers, DJ Simard, M Taras, P De Nardo, G Onorato, G Sciacca, C Raven, G Jessop, CP LoSecco, JM Honscheid, K Kass, R Margoni, M Morandin, M Posocco, M Rotondo, M Simi, G Simonetto, F Stroili, R Akar, S Ben-Haim, E Bomben, M Bonneaud, GR Briand, H Calderini, G Chauveau, J Leruste, P Marchiori, G Ocariz, J Biasini, M Manoni, E Rossi, A Angelini, C Batignani, G Bettarini, S Carpinelli, M Casarosa, G Chrzaszcz, M Forti, F Giorgi, MA Lusiani, A Oberhof, B Paoloni, E Rama, M Rizzo, G Walsh, JJ Pegna, DL Olsen, J Smith, AJS Anulli, F Faccini, R Ferrarotto, F Ferroni, F Gaspero, M Pilloni, A Piredda, G Bunger, C Dittrich, S Grunberg, O Hess, M Leddig, T Voss, C Waldi, R Adye, T Olaiya, EO Wilson, FF Emery, S Vasseur, G Aston, D Bard, DJ Cartaro, C Convery, MR Dorfan, J Dubois-Felsmann, GP Dunwoodie, W Ebert, M Field, RC Fulsom, BG Graham, MT Hast, C Innes, WR Kim, P Leith, DWGS Luitz, S Luth, V MacFarlane, DB Muller, DR Neal, H Pulliam, T Ratcliff, BN Roodman, A Schindler, RH Snyder, A Su, D Sullivan, MK Va'vra, J Wisniewski, WJ Wulsin, HW Purohit, MV Wilson, JR Randle-Conde, A Sekula, SJ Bellis, M Burchat, PR Puccio, EMT Alam, MS Ernst, JA Gorodeisky, R Guttman, N Peimer, DR Soffer, A Spanier, SM Ritchie, JL Schwitters, RF Izen, JM Lou, XC Bianchi, F De Mori, F Filippi, A Gamba, D Lanceri, L Vitale, L Martinez-Vidal, F Oyanguren, A Albert, J Banerjee, S Beaulieu, A Bernlochner, FU Choi, HHF King, GJ Kowalewski, R Lewczuk, MJ Lueck, T Nugent, IM Roney, JM Sobie, RJ Tasneem, N Gershon, TJ Harrison, PF Latham, TE Band, HR Dasu, S Pan, Y Prepost, R Wu, SL AF Lees, J. P. Poireau, V. Tisserand, V. Grauges, E. Palano, A. Eigen, G. Stugu, B. Brown, D. N. Kerth, L. T. Kolomensky, Yu G. Lee, M. J. Lynch, G. Koch, H. Schroeder, T. Hearty, C. Mattison, T. S. McKenna, J. A. So, R. Y. Khan, A. Blinov, V. E. Buzykaev, A. R. Druzhinin, V. P. Golubev, V. B. Kravchenko, E. A. Onuchin, A. P. Serednyakov, S. I. Skovpen, Yu I. Solodov, E. P. Todyshev, K. Yu Lankford, A. J. Dey, B. Gary, J. W. Long, O. Sevilla, M. Franco Hong, T. M. Kovalskyi, D. Richman, J. D. West, C. A. Eisner, A. M. Lockman, W. S. Vazquez, W. Panduro Schumm, B. A. Seiden, A. Chao, D. S. Cheng, C. H. Echenard, B. Flood, K. T. Hitlin, D. G. Kim, J. Miyashita, T. S. Ongmongkolkul, P. Porter, F. C. Roehrken, M. Andreassen, R. Huard, Z. Meadows, B. T. Pushpawela, B. G. Sokoloff, M. D. Sun, L. Ford, W. T. Smith, J. G. Wagner, S. R. Ayad, R. Toki, W. H. Spaan, B. Bernard, D. Verderi, M. Playfer, S. Bettoni, D. Bozzi, C. Calabrese, R. Cibinetto, G. Fioravanti, E. Garzia, I. Luppi, E. Piemontese, L. Santoro, V. Calcaterra, A. de Sangro, R. Finocchiaro, G. Martellotti, S. Patteri, P. Peruzzi, I. M. Piccolo, M. Zallo, A. Contri, R. Monge, M. R. Passaggio, S. Patrignani, C. Bhuyan, B. Prasad, V. Adametz, A. Uwer, U. Lacker, H. M. Mallik, U. Chen, C. Cochran, J. Prell, S. Ahmed, H. Gritsan, A. V. Arnaud, N. Davier, M. Derkach, D. Grosdidier, G. Le Diberder, F. Lutz, A. M. Malaescu, B. Roudeau, P. Stocchi, A. Wang, L. L. Wormser, G. Lange, D. J. Wright, D. M. Coleman, J. P. Fry, J. R. Gabathuler, E. Hutchcroft, D. E. Payne, D. J. Touramanis, C. Bevan, A. J. Di Lodovico, F. Sacco, R. Cowan, G. Brown, D. N. Davis, C. L. Denig, A. G. Fritsch, M. Gradl, W. Griessinger, K. Hafner, A. Schubert, K. R. Barlow, R. J. Lafferty, G. D. Cenci, R. Hamilton, B. Jawahery, A. Roberts, D. A. Cowan, R. Cheaib, R. Patel, P. M. Robertson, S. H. Neri, N. Palombo, F. Cremaldi, L. Godang, R. Summers, D. J. Simard, M. Taras, P. De Nardo, G. Onorato, G. Sciacca, C. Raven, G. Jessop, C. P. LoSecco, J. M. Honscheid, K. Kass, R. Margoni, M. Morandin, M. Posocco, M. Rotondo, M. Simi, G. Simonetto, F. Stroili, R. Akar, S. Ben-Haim, E. Bomben, M. Bonneaud, G. R. Briand, H. Calderini, G. Chauveau, J. Leruste, Ph Marchiori, G. Ocariz, J. Biasini, M. Manoni, E. Rossi, A. Angelini, C. Batignani, G. Bettarini, S. Carpinelli, M. Casarosa, G. Chrzaszcz, M. Forti, F. Giorgi, M. A. Lusiani, A. Oberhof, B. Paoloni, E. Rama, M. Rizzo, G. Walsh, J. J. Pegna, D. Lopes Olsen, J. Smith, A. J. S. Anulli, F. Faccini, R. Ferrarotto, F. Ferroni, F. Gaspero, M. Pilloni, A. Piredda, G. Buenger, C. Dittrich, S. Gruenberg, O. Hess, M. Leddig, T. Voss, C. Waldi, R. Adye, T. Olaiya, E. O. Wilson, F. F. Emery, S. Vasseur, G. Aston, D. Bard, D. J. Cartaro, C. Convery, M. R. Dorfan, J. Dubois-Felsmann, G. P. Dunwoodie, W. Ebert, M. Field, R. C. Fulsom, B. G. Graham, M. T. Hast, C. Innes, W. R. Kim, P. Leith, D. W. G. S. Luitz, S. Luth, V. MacFarlane, D. B. Muller, D. R. Neal, H. Pulliam, T. Ratcliff, B. N. Roodman, A. Schindler, R. H. Snyder, A. Su, D. Sullivan, M. K. Va'vra, J. Wisniewski, W. J. Wulsin, H. W. Purohit, M. V. Wilson, J. R. Randle-Conde, A. Sekula, S. J. Bellis, M. Burchat, P. R. Puccio, E. M. T. Alam, M. S. Ernst, J. A. Gorodeisky, R. Guttman, N. Peimer, D. R. Soffer, A. Spanier, S. M. Ritchie, J. L. Schwitters, R. F. Izen, J. M. Lou, X. C. Bianchi, F. De Mori, F. Filippi, A. Gamba, D. Lanceri, L. Vitale, L. Martinez-Vidal, F. Oyanguren, A. Albert, J. Banerjee, Sw Beaulieu, A. Bernlochner, F. U. Choi, H. H. F. King, G. J. Kowalewski, R. Lewczuk, M. J. Lueck, T. Nugent, I. M. Roney, J. M. Sobie, R. J. Tasneem, N. Gershon, T. J. Harrison, P. F. Latham, T. E. Band, H. R. Dasu, S. Pan, Y. Prepost, R. Wu, S. L. CA BaBar Collaboration TI Measurement of initial-state-final-state radiation interference in the processes e(+)e(-) -> mu(+)mu(-)gamma and e(+)e(-) -> pi(+)pi(-)gamma SO PHYSICAL REVIEW D LA English DT Article ID BABAR DETECTOR; MONTE-CARLO; TAGGED PHOTONS; B-FACTORIES; DECAYS; ASYMMETRY; PHYSICS AB Charge asymmetry in the processes e(+)e(-) -> mu(+)mu(-)gamma and e(+)e(-) -> pi(+)pi(-)gamma is measured using 232 fb(-1) of data collected with the BABAR detector at e(+)e(-) center-of-mass energies near 10.58 GeV. An observable is introduced and shown to be very robust against detector asymmetries while keeping a large sensitivity to the physical charge asymmetry that results from the interference between initial-and final-state radiation (FSR). The asymmetry is determined as a function of the invariant mass of the final-state tracks from production threshold to a few GeV/c(2). It is compared to the expectation from QED for e(+)e(-) -> mu(+)mu(-)gamma, and from theoretical models for e(+)e(-) -> pi(+)pi(-)gamma. A clear interference pattern is observed in e(+)e(-) -> pi(+)pi(-)gamma, particularly in the vicinity of the f(2)(1270) resonance. The inferred rate of lowest-order FSR production is consistent with the QED expectation for e(+)e(-) -> mu(+)mu(-)gamma, and is negligibly small for e(+)e(-) -> pi(+)pi(-)gamma. C1 [Lees, J. P.; Poireau, V.; Tisserand, V.] Univ Savoie, CNRS, IN2P3, Lab Annecy le Vieux Phys Particules LAPP, F-74941 Annecy Le Vieux, France. [Grauges, E.] Univ Barcelona, Fac Fis, Dept ECM, E-08028 Barcelona, Spain. [Palano, A.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Palano, A.] Univ Bari, Dipartimento Fis, I-70126 Bari, Italy. [Eigen, G.; Stugu, B.] Univ Bergen, Inst Phys, N-5007 Bergen, Norway. [Brown, D. N.; Kerth, L. T.; Kolomensky, Yu G.; Lee, M. J.; Lynch, G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Brown, D. N.; Kerth, L. T.; Kolomensky, Yu G.; Lee, M. J.; Lynch, G.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Koch, H.; Schroeder, T.] Ruhr Univ Bochum, Inst Expt Phys, D-44780 Bochum, Germany. [Hearty, C.; Mattison, T. S.; McKenna, J. A.; So, R. Y.] Univ British Columbia, Vancouver, BC V6T 1Z1, Canada. [Khan, A.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Blinov, V. E.; Buzykaev, A. R.; Druzhinin, V. P.; Golubev, V. B.; Kravchenko, E. A.; Onuchin, A. P.; Serednyakov, S. I.; Skovpen, Yu I.; Solodov, E. P.; Todyshev, K. Yu] RAS, Budker Inst Nucl Phys, SB, Novosibirsk 630090, Russia. [Blinov, V. E.; Druzhinin, V. P.; Golubev, V. B.; Kravchenko, E. A.; Onuchin, A. P.; Serednyakov, S. I.; Skovpen, Yu I.; Solodov, E. P.; Todyshev, K. Yu] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Blinov, V. E.; Onuchin, A. P.] Novosibirsk State Tech Univ, Novosibirsk 630092, Russia. [Lankford, A. 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J.; Touramanis, C.] Univ Liverpool, Liverpool L69 7ZE, Merseyside, England. [Bevan, A. J.; Di Lodovico, F.; Sacco, R.] Univ London, London E1 4NS, England. [Cowan, G.] Univ London Royal Holloway & Bedford New Coll, Egham TW20 0EX, Surrey, England. [Brown, D. N.; Davis, C. L.] Univ Louisville, Louisville, KY 40292 USA. [Denig, A. G.; Fritsch, M.; Gradl, W.; Griessinger, K.; Hafner, A.; Schubert, K. R.] Johannes Gutenberg Univ Mainz, Inst Kernphys, D-55099 Mainz, Germany. [Barlow, R. J.; Lafferty, G. D.] Univ Manchester, Manchester M13 9PL, Lancs, England. [Cenci, R.; Hamilton, B.; Jawahery, A.; Roberts, D. A.] Univ Maryland, College Pk, MD 20742 USA. [Cowan, R.] MIT, Nucl Sci Lab, Cambridge, MA 02139 USA. [Cheaib, R.; Patel, P. M.; Robertson, S. H.] McGill Univ, Montreal, PQ H3A 2T8, Canada. [Neri, N.; Palombo, F.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Palombo, F.] Univ Milan, Dipartimento Fis, I-20133 Milan, Italy. [Cremaldi, L.; Godang, R.; Summers, D. J.] Univ Mississippi, University, MS 38677 USA. [Simard, M.; Taras, P.] Univ Montreal, Phys Particules, Montreal, PQ H3C 3J7, Canada. [De Nardo, G.; Onorato, G.; Sciacca, C.] Ist Nazl Fis Nucl, Sez Napoli, I-80126 Naples, Italy. [De Nardo, G.; Onorato, G.; Sciacca, C.] Univ Naples Federico II, Dipartimento Sci Fis, I-80126 Naples, Italy. [Raven, G.] NIKHEF H, Natl Inst Nucl Phys & High Energy Phys, NL-1009 DB Amsterdam, Netherlands. [Jessop, C. P.; LoSecco, J. M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Honscheid, K.; Kass, R.] Ohio State Univ, Columbus, OH 43210 USA. [Margoni, M.; Morandin, M.; Posocco, M.; Rotondo, M.; Simi, G.; Simonetto, F.; Stroili, R.] Ist Nazl Fis Nucl, Sez Padova, I-35131 Padua, Italy. [Margoni, M.; Simi, G.; Simonetto, F.; Stroili, R.] Univ Padua, Dipartimento Fis, I-35131 Padua, Italy. [Akar, S.; Ben-Haim, E.; Bomben, M.; Bonneaud, G. R.; Briand, H.; Calderini, G.; Chauveau, J.; Leruste, Ph; Marchiori, G.; Ocariz, J.] Univ Paris 07, Univ Paris 06, Lab Phys Nucl & Hautes Energies, IN2P3,CNRS, F-75252 Paris, France. [Biasini, M.; Manoni, E.; Rossi, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06123 Perugia, Italy. [Biasini, M.] Univ Perugia, Dipartimento Fis, I-06123 Perugia, Italy. [Angelini, C.; Batignani, G.; Bettarini, S.; Carpinelli, M.; Casarosa, G.; Chrzaszcz, M.; Forti, F.; Giorgi, M. A.; Lusiani, A.; Oberhof, B.; Paoloni, E.; Rama, M.; Rizzo, G.; Walsh, J. J.] Ist Nazl Fis Nucl, Sez Pisa, I-56127 Pisa, Italy. [Angelini, C.; Batignani, G.; Bettarini, S.; Carpinelli, M.; Casarosa, G.; Forti, F.; Giorgi, M. A.; Oberhof, B.; Paoloni, E.; Rizzo, G.] Univ Pisa, Dipartimento Fis, I-56127 Pisa, Italy. [Lusiani, A.] Scuola Normale Super Pisa, I-56127 Pisa, Italy. [Pegna, D. Lopes; Olsen, J.; Smith, A. J. S.] Princeton Univ, Princeton, NJ 08544 USA. [Anulli, F.; Faccini, R.; Ferrarotto, F.; Ferroni, F.; Gaspero, M.; Pilloni, A.; Piredda, G.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Faccini, R.; Ferroni, F.; Gaspero, M.; Pilloni, A.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Buenger, C.; Dittrich, S.; Gruenberg, O.; Hess, M.; Leddig, T.; Voss, C.; Waldi, R.] Univ Rostock, D-18051 Rostock, Germany. [Adye, T.; Olaiya, E. O.; Wilson, F. F.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Emery, S.; Vasseur, G.] CEA, Irfu, SPP, Ctr Saclay, F-91191 Gif Sur Yvette, France. [Aston, D.; Bard, D. J.; Cartaro, C.; Convery, M. R.; Dorfan, J.; Dubois-Felsmann, G. P.; Dunwoodie, W.; Ebert, M.; Field, R. C.; Fulsom, B. G.; Graham, M. T.; Hast, C.; Innes, W. R.; Kim, P.; Leith, D. W. G. S.; Luitz, S.; Luth, V.; MacFarlane, D. B.; Muller, D. R.; Neal, H.; Pulliam, T.; Ratcliff, B. N.; Roodman, A.; Schindler, R. H.; Snyder, A.; Su, D.; Sullivan, M. K.; Va'vra, J.; Wisniewski, W. J.; Wulsin, H. W.] SLAC Natl Accelerator Lab, Stanford, CA 94309 USA. [Purohit, M. V.; Wilson, J. R.] Univ S Carolina, Columbia, SC 29208 USA. [Randle-Conde, A.; Sekula, S. J.] So Methodist Univ, Dallas, TX 75275 USA. [Bellis, M.; Burchat, P. R.; Puccio, E. M. T.] Stanford Univ, Stanford, CA 94305 USA. [Alam, M. S.; Ernst, J. A.] SUNY Albany, Albany, NY 12222 USA. [Gorodeisky, R.; Guttman, N.; Peimer, D. R.; Soffer, A.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Spanier, S. M.] Univ Tennessee, Knoxville, TN 37996 USA. [Ritchie, J. L.; Schwitters, R. F.] Univ Texas Austin, Austin, TX 78712 USA. [Izen, J. M.; Lou, X. C.] Univ Texas Dallas, Richardson, TX 75083 USA. [Bianchi, F.; De Mori, F.; Filippi, A.; Gamba, D.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Bianchi, F.; De Mori, F.; Gamba, D.] Univ Turin, Dipartimento Fis, I-10125 Turin, Italy. [Lanceri, L.; Vitale, L.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Lanceri, L.; Vitale, L.] Univ Trieste, Dipartimento Fis, I-34127 Trieste, Italy. [Martinez-Vidal, F.; Oyanguren, A.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain. [Albert, J.; Banerjee, Sw; Beaulieu, A.; Bernlochner, F. U.; Choi, H. H. F.; King, G. J.; Kowalewski, R.; Lewczuk, M. J.; Lueck, T.; Nugent, I. M.; Roney, J. M.; Sobie, R. J.; Tasneem, N.] Univ Victoria, Victoria, BC V8W 3P6, Canada. [Gershon, T. J.; Harrison, P. F.; Latham, T. E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Band, H. R.; Dasu, S.; Pan, Y.; Prepost, R.; Wu, S. L.] Univ Wisconsin, Madison, WI 53706 USA. [Carpinelli, M.] Univ Sassari, I-07100 Sassari, Italy. RP Lees, JP (reprint author), Univ Savoie, CNRS, IN2P3, Lab Annecy le Vieux Phys Particules LAPP, F-74941 Annecy Le Vieux, France. RI Patrignani, Claudia/C-5223-2009; Morandin, Mauro/A-3308-2016; Lusiani, Alberto/A-3329-2016; Kravchenko, Evgeniy/F-5457-2015; Di Lodovico, Francesca/L-9109-2016; Calcaterra, Alessandro/P-5260-2015; Rizzo, Giuliana/A-8516-2015 OI Patrignani, Claudia/0000-0002-5882-1747; Morandin, Mauro/0000-0003-4708-4240; Lusiani, Alberto/0000-0002-6876-3288; Di Lodovico, Francesca/0000-0003-3952-2175; Calcaterra, Alessandro/0000-0003-2670-4826; Ebert, Marcus/0000-0002-3014-1512; Bettarini, Stefano/0000-0001-7742-2998; FORD, WILLIAM/0000-0001-8703-6943; Cibinetto, Gianluigi/0000-0002-3491-6231; Rizzo, Giuliana/0000-0003-1788-2866 FU US Department of Energy; National Science Foundation; Natural Sciences and Engineering Research Council (Canada); Commissariat a l'Energie Atomique (France); Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung (Germany); Deutsche Forschungsgemeinschaft (Germany); Istituto Nazionale di Fisica Nucleare (Italy); Foundation for Fundamental Research on Matter (The Netherlands); Research Council of Norway; Ministry of Education (Spain); Science of the Russian Federation, Ministerio de Economia y Competitividad (Spain); Science and Technology Facilities Council (United Kingdom); Binational Science Foundation (U.S.-Israel); Marie-Curie IEF program (European Union); A. P. Sloan Foundation (USA) FX We gratefully acknowledge useful discussions on theoretical issues with H. Czyz, Zhun Lu and B. Pire, and clarifications by A. B. Arbuzov, S. J. Brodsky, R. Gastmans, and R. Kleiss. We thank Henryk Czyz for providing tests with PHOKHARA-V9. We are grateful for the extraordinary contributions of our PEP-II colleagues in achieving the excellent luminosity and machine conditions that have made this work possible. The success of this project also relies critically on the expertise and dedication of the computing organizations that support BABAR. The collaborating institutions wish to thank SLAC for its support and the kind hospitality extended to them. This work is supported by the US Department of Energy and National Science Foundation, the Natural Sciences and Engineering Research Council (Canada), the Commissariat a l'Energie Atomique and Institut National de Physique Nucleaire et de Physique des Particules (France), the Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany), the Istituto Nazionale di Fisica Nucleare (Italy), the Foundation for Fundamental Research on Matter (The Netherlands), the Research Council of Norway, the Ministry of Education and Science of the Russian Federation, Ministerio de Economia y Competitividad (Spain), the Science and Technology Facilities Council (United Kingdom), and the Binational Science Foundation (U.S.-Israel). Individuals have received support from the Marie-Curie IEF program (European Union) and the A. P. Sloan Foundation (USA). NR 32 TC 3 Z9 4 U1 1 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD OCT 28 PY 2015 VL 92 IS 7 AR 072015 DI 10.1103/PhysRevD.92.072015 PG 29 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CU4VC UT WOS:000363527500001 ER PT J AU Rembert, T Battaglia, C Anders, A Javey, A AF Rembert, Thomas Battaglia, Corsin Anders, Andre Javey, Ali TI Room Temperature Oxide Deposition Approach to Fully Transparent, All-Oxide Thin-Film Transistors SO ADVANCED MATERIALS LA English DT Article DE flexible electronics; metal oxides; thin-film transistors; transparent electronics ID INTEGRATED-CIRCUITS; VACUUM-ARC; ZNO; ELECTRONICS; SEMICONDUCTORS; FABRICATION; FIELD; SKIN AB A room temperature cathodic arc deposition technique is used to produce high-mobility ZnO thin films for low voltage thin-film transistors (TFTs) and digital logic inverters. All-oxide, fully transparent devices are fabricated on alkali-free glass and flexible polyimide foil, exhibiting high performance. This provides a practical materials platform for the low-temperature fabrication of all-oxide TFTs on virtually any substrate. C1 [Rembert, Thomas; Battaglia, Corsin; Javey, Ali] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. [Rembert, Thomas; Battaglia, Corsin; Javey, Ali] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Anders, Andre] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Plasma Applicat Grp, Berkeley, CA 94720 USA. RP Javey, A (reprint author), Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. EM ajavey@eecs.berkeley.edu RI Javey, Ali/B-4818-2013; Battaglia, Corsin/B-2917-2010; Anders, Andre/B-8580-2009 OI Anders, Andre/0000-0002-5313-6505 FU ORISE-ORAU [DE-AC05-06OR23100]; Office of Science, Office of Basic Energy Sciences, US Department of Energy [DE-AC02-05CH11231]; Department of Energy Office of Science Graduate Fellowship Program (DOE SCGF) FX T.R. acknowledges the Department of Energy Office of Science Graduate Fellowship Program (DOE SCGF), made possible in part by the American Recovery and Reinvestment Act of 2009, administered by ORISE-ORAU under Contract No. DE-AC05-06OR23100. Materials processing and characterization were supported by the Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract No. DE-AC02-05CH11231. The authors acknowledge Joe Wallig for his help with the cathodic arc chamber maintenance. NR 39 TC 8 Z9 8 U1 23 U2 119 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD OCT 28 PY 2015 VL 27 IS 40 BP 6090 EP 6095 DI 10.1002/adma.201502159 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CU4DF UT WOS:000363476200002 PM 26455916 ER PT J AU Barth, DS Gladden, C Salandrino, A O'Brien, K Ye, ZL Mrejen, M Wang, Y Zhang, X AF Barth, David S. Gladden, Christopher Salandrino, Alessandro O'Brien, Kevin Ye, Ziliang Mrejen, Michael Wang, Yuan Zhang, Xiang TI Macroscale Transformation Optics Enabled by Photoelectrochemical Etching SO ADVANCED MATERIALS LA English DT Article DE gradient index optics; porous silicon; transformation optics; photochemical etching ID POROUS SILICON; INVISIBILITY CLOAK; WAVE-GUIDES; LITHOGRAPHY; METAMATERIALS; WAVELENGTHS; FABRICATION; INDEX; GLASS; LENS AB Photoelectrochemical etching of silicon can be used to form lateral refractive index gradients for transformation optical devices. This technique allows the fabrication of macroscale devices with large refractive index gradients. Patterned porous layers can also be lifted from the substrate and transferred to other materials, creating more possibilities for novel devices. C1 [Barth, David S.; Gladden, Christopher; Salandrino, Alessandro; O'Brien, Kevin; Ye, Ziliang; Mrejen, Michael; Wang, Yuan; Zhang, Xiang] Univ Calif Berkeley, NSF Nanoscale Sci & Engn Ctr NSEC, Berkeley, CA 94720 USA. [Zhang, Xiang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Zhang, Xiang] Univ Calif Berkeley, Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. [Zhang, Xiang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Zhang, Xiang] King Abdulaziz Univ, Dept Phys, Jeddah 21589, Saudi Arabia. RP Zhang, X (reprint author), Univ Calif Berkeley, NSF Nanoscale Sci & Engn Ctr NSEC, Berkeley, CA 94720 USA. EM xiang@berkeley.edu RI Zhang, Xiang/F-6905-2011 FU 'Light-Material Interactions in Energy Conversion' Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-05CH11231]; Office of Naval Research Multidisciplinary University Research Initiative program [N00014-13-1-0649]; DoD, Air Force Office of Scientific Research, National Defense Science and Engineering Graduate (NDSEG) Fellowship [32 CFR 168a] FX D.S.B. and C.G. contributed equally to this work. The authors thank Dr. Rongkuo Zhao and Dr. Xingjie Ni for helpful discussion. The experimental work was supported by the 'Light-Material Interactions in Energy Conversion' Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-AC02-05CH11231 and the simulation part was supported by Office of Naval Research Multidisciplinary University Research Initiative program grant N00014-13-1-0649. D.S.B. acknowledges that this research was conducted with Government support under and awarded by DoD, Air Force Office of Scientific Research, National Defense Science and Engineering Graduate (NDSEG) Fellowship, 32 CFR 168a. NR 35 TC 2 Z9 2 U1 4 U2 32 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD OCT 28 PY 2015 VL 27 IS 40 BP 6131 EP 6136 DI 10.1002/adma.201502322 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CU4DF UT WOS:000363476200008 PM 26332896 ER PT J AU Bodiou, L Gu, QY Guezo, M Delcourt, E Batte, T Lemaitre, J Lorrain, N Guendouz, M Folliot, H Charrier, J Mistry, KS Blackburn, JL Doualan, JL Braud, A Camy, P AF Bodiou, Loic Gu, Qingyuan Guezo, Maud Delcourt, Enguerran Batte, Thomas Lemaitre, Jonathan Lorrain, Nathalie Guendouz, Mohammed Folliot, Herve Charrier, Joel Mistry, Kevin S. Blackburn, Jeffrey L. Doualan, Jean-Louis Braud, Alain Camy, Patrice TI Guided Photoluminescence from Integrated Carbon-Nanotube-Based Optical Waveguides SO ADVANCED MATERIALS LA English DT Article DE carbon nanotubes; photoluminescence; silicon photonics; waveguides ID SELECTIVE DISPERSION; SINGLE; SENSORS; PHOTONICS; GAS AB Thin films and ridge waveguides based on large-diameter semiconducting single-wall carbon nanotubes (s-SWCNTs) dispersed in a polyfluorene derivative are fabricated and optically characterized. Ridge waveguides are designed with appropriate dimensions for single-mode propagation at 1550 nm. Using multimode ridge waveguides, guided s-SWCNT photoluminescence is demonstrated for the first time in the near-infrared telecommunications window. C1 [Bodiou, Loic; Gu, Qingyuan; Guezo, Maud; Delcourt, Enguerran; Batte, Thomas; Lemaitre, Jonathan; Lorrain, Nathalie; Guendouz, Mohammed; Folliot, Herve; Charrier, Joel] Univ Rennes 1, INSA Rennes Enssat, UMR Foton CNRS, F-F22305 Lannion, France. [Mistry, Kevin S.; Blackburn, Jeffrey L.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Doualan, Jean-Louis; Braud, Alain; Camy, Patrice] Univ Caen, UMR CEA CNRS ENSICaen, Ctr Rech Ions Mat & Photon CIMAP, F-14050 Caen, France. RP Bodiou, L (reprint author), Univ Rennes 1, INSA Rennes Enssat, UMR Foton CNRS, F-F22305 Lannion, France. EM loic.bodiou@univ-rennes1.fr FU Lannion Tregor Communaute; RTR SISCom; Region Bretagne; French Ministry of Research; European Regional Development Fund; Solar Photochemistry Program of the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences [DE-AC36-08GO28308] FX This work was supported by Lannion Tregor Communaute, the RTR SISCom, the Region Bretagne, the French Ministry of Research, and the European Regional Development Fund. Guillaume Calvez (ISCR CNRS UMR 6226, INSA Rennes) and Christophe Levallois (Foton CNRS UMR 6082, INSA Rennes) are acknowledged for preliminary optical measurements. J.L.B. and K.S.M. gratefully acknowledge support from the Solar Photochemistry Program of the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences, under Contract No. DE-AC36-08GO28308 to NREL. NR 31 TC 1 Z9 1 U1 8 U2 47 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD OCT 28 PY 2015 VL 27 IS 40 BP 6181 EP 6186 DI 10.1002/adma.201502536 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CU4DF UT WOS:000363476200016 PM 26350035 ER PT J AU Zhao, Q Xiao, ZQ Zhang, FL Ma, JM Qiao, M Meng, YG Lan, CW Li, B Zhou, J Zhang, P Shen, NH Koschny, T Soukoulis, CM AF Zhao, Qian Xiao, Zongqi Zhang, Fuli Ma, Junming Qiao, Ming Meng, Yonggang Lan, Chuwen Li, Bo Zhou, Ji Zhang, Peng Shen, Nian-Hai Koschny, Thomas Soukoulis, Costas M. TI Tailorable Zero-Phase Delay of Subwavelength Particles toward Miniaturized Wave Manipulation Devices SO ADVANCED MATERIALS LA English DT Article DE metamaterials; subwavelength dielectric particles; temperature tunability; wave manipulation; zero-phase delay ID OPTICAL METAMATERIAL; DIFFRACTION LIMIT; REFRACTIVE-INDEX; NEGATIVE-INDEX; NANOPARTICLES; SCATTERING; LIGHT AB Adjustable zero-phase delay and equiphase control are demonstrated in single and multilayer dielectric particle arrays with high index and low loss. The polarization-independent near-zero permeability is the origin of the wave control near the first Mie magnetic resonance. The proposed design paves the way for subwavelength devices and opens up new avenues for the miniaturization and integration of THz and optical components. C1 [Zhao, Qian; Xiao, Zongqi; Ma, Junming; Qiao, Ming; Meng, Yonggang] Tsinghua Univ, Dept Mech Engn, State Key Lab Tribol, Beijing 100084, Peoples R China. [Zhang, Fuli] Northwestern Polytech Univ, Minist Educ, Key Lab Space Appl Phys & Chem, Xian 710072, Peoples R China. [Zhang, Fuli] Northwestern Polytech Univ, Dept Appl Phys Sch Sci, Xian 710072, Peoples R China. [Lan, Chuwen; Li, Bo; Zhou, Ji] Tsinghua Univ, Sch Mat Sci & Engn, State Key Lab New Ceram & Fine Proc, Beijing 100084, Peoples R China. [Zhang, Peng; Shen, Nian-Hai; Koschny, Thomas; Soukoulis, Costas M.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Zhang, Peng; Shen, Nian-Hai; Koschny, Thomas; Soukoulis, Costas M.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Soukoulis, Costas M.] FORTH, IESL, Iraklion 71110, Crete, Greece. RP Zhao, Q (reprint author), Tsinghua Univ, Dept Mech Engn, State Key Lab Tribol, Beijing 100084, Peoples R China. EM zhaoqian@mail.tsinghua.edu.cn RI Soukoulis, Costas/A-5295-2008 FU National High Technology Research and Development Program of China [2012AA030403]; National Natural Science Foundation of China [61275176, 61101044, 11372248, 91123033, 51323006]; Program for New Century Excellent Talents in University [NCET-13-0337]; Chinese State Key Laboratory of Tribology; U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering [DE-AC02-07CH11358]; U.S. Office of Naval Research [N00014-14-1-0474]; European Research Council [320081] FX This work was supported by the National High Technology Research and Development Program of China (Grant No. 2012AA030403), the National Natural Science Foundation of China (Grant Nos. 61275176, 61101044, 11372248, 91123033, and 51323006), the Program for New Century Excellent Talents in University (NCET-13-0337), and the Chinese State Key Laboratory of Tribology. Work at Ames Lab (theory) was partially supported by the U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering under contract No. DE-AC02-07CH11358, the U.S. Office of Naval Research (Simulations) award No. N00014-14-1-0474, and the European Research Council under the ERC Advanced Grant No. 320081 at FORTH. The authors gratefully acknowledge discussions with Dr. L. Kang, J. B. Sun, A. Jain, and Prof. C. W. Qiu. NR 42 TC 7 Z9 8 U1 16 U2 72 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD OCT 28 PY 2015 VL 27 IS 40 BP 6187 EP 6194 DI 10.1002/adma.201502298 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CU4DF UT WOS:000363476200017 PM 26332831 ER PT J AU Li, MM Liu, F Wan, XJ Ni, W Kan, B Feng, HR Zhang, Q Yang, X Wang, YC Zhang, YM Shen, Y Russell, TP Chen, YS AF Li, Miaomiao Liu, Feng Wan, Xiangjian Ni, Wang Kan, Bin Feng, Huanran Zhang, Qian Yang, Xuan Wang, Yunchuang Zhang, Yamin Shen, Yan Russell, Thomas P. Chen, Yongsheng TI Subtle Balance Between Length Scale of Phase Separation and Domain Purification in Small-Molecule Bulk-Heterojunction Blends under Solvent Vapor Treatment SO ADVANCED MATERIALS LA English DT Article DE morphology; small-molecule-based solar cells; solvent vapor annealing ID POLYMER SOLAR-CELLS; POWER CONVERSION EFFICIENCY; OPEN-CIRCUIT VOLTAGE; BENZODITHIOPHENE UNIT; ORGANIC PHOTOVOLTAICS; PERFORMANCE; MORPHOLOGY; RECOMBINATION; 10-PERCENT; LAYER AB A series of solvents with different solubilities for DR3TBDTT and PC71BM, and different boiling points, is used for solvent vapor annealing (SVA) treatment to systematically investigate the solvent-morphologyperformance relationship. The presence of solvent molecules inside bulk-heterojunction (BHJ) thin films promotes the mobility of both donor and acceptor molecules, leading to crystallization and aggregation, which are important in modulating morphology. C1 [Li, Miaomiao; Wan, Xiangjian; Ni, Wang; Kan, Bin; Feng, Huanran; Zhang, Qian; Yang, Xuan; Wang, Yunchuang; Zhang, Yamin; Chen, Yongsheng] Nankai Univ, Coll Chem, Ctr Nanoscale Sci & Technol,Inst Polymer Chem, Collaborat Innovat Ctr Chem Sci & Engn Tianjin,Ke, Tianjin 300071, Peoples R China. [Liu, Feng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Shen, Yan] Huazhong Univ Sci & Technol, Sch Opt & Elect Informat, Wuhan Natl Lab Optoelect, Wuhan 430074, Hubei, Peoples R China. [Russell, Thomas P.] Univ Massachusetts, Dept Polymer Sci & Engn, Amherst, MA 01003 USA. RP Liu, F (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM xjwan@nankai.edu.cn; xjwan@nankai.edu.cn; yschen99@nankai.edu.cn RI Shen, Yan/D-2410-2016; Liu, Feng/J-4361-2014 OI Liu, Feng/0000-0002-5572-8512 FU MoST [2014CB643502]; NSFC [51373078, 51422304, 91433101]; PCSIRT [IRT1257]; Tianjin City [13RCGFGX01121] FX The authors gratefully acknowledge the financial support from MoST (Grant No. 2014CB643502), NSFC (Grant Nos. 51373078, 51422304, and 91433101), PCSIRT (Grant No. IRT1257), and Tianjin City (Grant No. 13RCGFGX01121). NR 43 TC 29 Z9 29 U1 17 U2 110 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD OCT 28 PY 2015 VL 27 IS 40 BP 6296 EP 6302 DI 10.1002/adma.201502645 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CU4DF UT WOS:000363476200034 PM 26333172 ER PT J AU Baranowski, LL McLaughlin, K Zawadzki, P Lany, S Norman, A Hempel, H Eichberger, R Unold, T Toberer, ES Zakutayev, A AF Baranowski, Lauryn L. McLaughlin, Kevin Zawadzki, Pawel Lany, Stephan Norman, Andrew Hempel, Hannes Eichberger, Rainer Unold, Thomas Toberer, Eric S. Zakutayev, Andriy TI Effects of Disorder on Carrier Transport in Cu2SnS3 SO PHYSICAL REVIEW APPLIED LA English DT Article ID THIN-FILMS; STABILITY AB Cu2SnS3 is a promising absorber material that has attracted significant interest in recent years. However, similar to Cu2ZnSn(S, Se)(4) (CZTS), Cu2SnS3 displays cation disorder, which complicates the scientific understanding and technological applications of these materials. In this work, we use postdeposition annealing to convert disordered Cu2SnS3 thin films to the ordered structure. After annealing, we observe crystal structure changes and detect improvements in the majority carrier (hole) transport. However, when the minority carrier (electron) transport is investigated by using optical-pump terahertz-probe spectroscopy, minimal differences are observed in the lifetimes of the photoexcited charge carriers in the ordered and disordered Cu2SnS3. By combining the experimental data with theoretical results from first-principles calculations and Monte Carlo simulations, we are able to conclude that even ostensibly "ordered" Cu2SnS3 displays minority carrier transport properties corresponding to the disordered structure. Transmission electron microscopy investigations reveal only a very low density of planar defects (stacking faults and/or twins) in the annealed film, suggesting that these imperfections can dominate minority carrier transport even at low levels. The results of this study highlight some of the challenges in the development of Cu2SnS3-based photovoltaics and have implications for other disordered multinary semiconductors such as CZTS. C1 [Baranowski, Lauryn L.; Zawadzki, Pawel; Lany, Stephan; Norman, Andrew; Toberer, Eric S.; Zakutayev, Andriy] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Baranowski, Lauryn L.; McLaughlin, Kevin; Toberer, Eric S.] Colorado Sch Mines, Dept Phys, Golden, CO 80401 USA. [Hempel, Hannes; Eichberger, Rainer; Unold, Thomas] Helmholtz Zentrum Berlin Mat & Energie GmbH, D-14109 Berlin, Germany. RP Zakutayev, A (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM andriy.zakutayev@nrel.gov RI Norman, Andrew/F-1859-2010; OI Norman, Andrew/0000-0001-6368-521X; Lany, Stephan/0000-0002-8127-8885; Zakutayev, Andriy/0000-0002-3054-5525 FU U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, as a part of the "Rapid Development of Earth-Abundant Thin Film Solar Cells" [DE-AC36-08GO28308]; Department of Defense through the National Defense Science and Engineering Graduate Fellowship Program; Helmholtz Association Initiative and Network Fund (HNSEI-Project) FX This work is supported by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, as a part of the "Rapid Development of Earth-Abundant Thin Film Solar Cells" agreement, under Contract No. DE-AC36-08GO28308 to NREL. L.L.B. is supported by the Department of Defense through the National Defense Science and Engineering Graduate Fellowship Program. T.U., R.E., and H.H. gratefully acknowledge the support of this work by the Helmholtz Association Initiative and Network Fund (HNSEI-Project). Thanks to Brenden Ortiz at the Colorado School of Mines for the synthesis of SnS and SnS2 powders. Thanks to Lynn Gedvilas and Adam Stokes at the National Renewable Energy Laboratory for Raman spectroscopy and TEM sample preparation. Adele Tamboli at the National Renewable Energy Laboratory provided valuable discussion and input. NR 40 TC 10 Z9 10 U1 11 U2 41 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2331-7019 J9 PHYS REV APPL JI Phys. Rev. Appl. PD OCT 28 PY 2015 VL 4 IS 4 AR 044017 DI 10.1103/PhysRevApplied.4.044017 PG 9 WC Physics, Applied SC Physics GA CU4XS UT WOS:000363535400001 ER PT J AU Chen, J Kondev, FG Ahmad, I Carpenter, MP Greene, JP Janssens, RVF Zhu, S Ehst, D Makarashvili, V Rotsch, D Smith, NA AF Chen, J. Kondev, F. G. Ahmad, I. Carpenter, M. P. Greene, J. P. Janssens, R. V. F. Zhu, S. Ehst, D. Makarashvili, V. Rotsch, D. Smith, N. A. TI Precise absolute gamma-ray and beta(-)-decay branching intensities in the decay of Cu-67(29) SO PHYSICAL REVIEW C LA English DT Article ID NUCLEAR-DATA SHEETS; RADIOIMMUNOTHERAPY AB Absolute gamma-ray emission probabilities in the beta(-)decay of Cu-67 weremeasured by means of gamma-ray and beta(-)-decay singles and beta(-)-gamma coincidences. The new results, together with the known decay scheme of Cu-67, were used to determine absolute beta(-)-decay branching intensities. The present data differ significantly from previously published values. In addition, the half-life of the I-pi = 1/2(-) isomer in Zn-67 was measured as T-1/2 = 9.37( 4) mu s, in a good agreement with earlier measurements. From the analysis of the Fermi-Kurie plots, Q(beta-)(g.s.) = 560.3( 10) keV was deduced, which differs from the previously measured value of 577( 8) keV but is in good agreement with Q(beta-)(g.s.) = 561.3(15) keV recommended in the latest Atomic Mass Evaluation. C1 [Chen, J.; Kondev, F. G.; Ehst, D.; Makarashvili, V.; Rotsch, D.; Smith, N. A.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. [Ahmad, I.; Carpenter, M. P.; Greene, J. P.; Janssens, R. V. F.; Zhu, S.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RP Chen, J (reprint author), Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. EM kondev@anl.gov RI Carpenter, Michael/E-4287-2015; OI Carpenter, Michael/0000-0002-3237-5734; Chen, Jun/0000-0003-0447-7466 FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357]; U.S. Department of Energy Isotope Program; Nuclear Data Section of the International Atomic Energy Agency FX The authors would like to thank Dr. Yan Cao from the Nuclear Engineering Division at Argonne National Laboratory for her help in the Monte Carlo simulations of detector efficiencies. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357. The 67Cu material used in this work was produced using technology developed under a research grant from the U.S. Department of Energy Isotope Program. F.G. Kondev acknowledges support from the Nuclear Data Section of the International Atomic Energy Agency, under the auspices of the Coordinated Research Project on "Nuclear Data for Charged-Particle Monitor Reactions and Medical Isotope Production." NR 19 TC 1 Z9 1 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD OCT 28 PY 2015 VL 92 IS 4 AR 044330 DI 10.1103/PhysRevC.92.044330 PG 5 WC Physics, Nuclear SC Physics GA CU4UN UT WOS:000363526000002 ER PT J AU Kawano, T Talou, P Weidenmuller, HA AF Kawano, T. Talou, P. Weidenmueller, H. A. TI Random-matrix approach to the statistical compound nuclear reaction at low energies using the Monte Carlo technique SO PHYSICAL REVIEW C LA English DT Article ID HAUSER-FESHBACH CALCULATIONS; CROSS-SECTIONS; ENHANCEMENT FACTOR; PHYSICS; FORMULA; AVERAGE; U-238; FLUCTUATIONS; RANGE; CHAOS AB Using a random-matrix approach and Monte Carlo simulations, we generate scattering matrices and cross sections for compound-nucleus reactions. In the absence of direct reactions we compare the average cross sections with the analytic solution given by the Gaussian orthogonal ensemble (GOE) triple integral, and with predictions of statistical approaches such as the ones from Moldauer; Hofmann, Richert, Tepel, and Weidenmuller; and Kawai, Kerman, and McVoy. We find perfect agreement with the GOE triple integral and display the limits of validity of the latter approaches. We establish a criterion for the width of the energy-averaging interval such that the relative difference between the ensemble-averaged and the energy-averaged scattering matrices lies below a given bound. Direct reactions are simulated in terms of an energy-independent background matrix. In that case, cross sections averaged over the ensemble of Monte Carlo simulations fully agree with results from the Engelbrecht-Weidenmuller transformation. The limits of other approximate approaches are displayed. C1 [Kawano, T.; Talou, P.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Weidenmueller, H. A.] Max Planck Inst Kernphys, D-69029 Heidelberg, Germany. RP Kawano, T (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM kawano@lanl.gov FU National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396] FX T.K. and P.T. carried out this work under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. NR 43 TC 4 Z9 4 U1 2 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD OCT 28 PY 2015 VL 92 IS 4 AR 044617 DI 10.1103/PhysRevC.92.044617 PG 16 WC Physics, Nuclear SC Physics GA CU4UN UT WOS:000363526000004 ER PT J AU Sternberg, MG Segel, R Scielzo, ND Savard, G Clark, JA Bertone, PF Buchinger, F Burkey, M Caldwell, S Chaudhuri, A Crawford, JE Deibel, CM Greene, J Gulick, S Lascar, D Levand, AF Li, G Galvan, AP Sharma, KS Van Schelt, J Yee, RM Zabransky, BJ AF Sternberg, M. G. Segel, R. Scielzo, N. D. Savard, G. Clark, J. A. Bertone, P. F. Buchinger, F. Burkey, M. Caldwell, S. Chaudhuri, A. Crawford, J. E. Deibel, C. M. Greene, J. Gulick, S. Lascar, D. Levand, A. F. Li, G. Galvan, A. Perez Sharma, K. S. Van Schelt, J. Yee, R. M. Zabransky, B. J. TI Limit on Tensor Currents from Li-8 beta Decay SO PHYSICAL REVIEW LETTERS LA English DT Article ID ALPHA RADIATIVE CORRECTION; FERMI INTERACTION; NUCLEAR; SCATTERING; MODEL; TRAP AB In the standard model, the weak interaction is formulated with a purely vector-axial-vector (V-A) structure. Without restriction on the chirality of the neutrino, the most general limits on tensor currents from nuclear beta decay are dominated by a single measurement of the beta-(nu) over bar correlation in He-6 beta decay dating back over a half century. In the present work, the beta-(nu) over bar-alpha correlation in the beta decay of Li-8 and subsequent alpha-particle breakup of the Be-8* daughter was measured. The results are consistent with a purely V-A interaction and in the case of couplings to right-handed neutrinos (C-T = -C'(T)) limits the tensor fraction to vertical bar C-T/C-A vertical bar(2) < 0.011 (95.5% C.L.). The measurement confirms the He-6 result using a different nuclear system and employing modern ion-trapping techniques subject to different systematic uncertainties. C1 [Sternberg, M. G.; Savard, G.; Burkey, M.; Caldwell, S.; Van Schelt, J.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Sternberg, M. G.; Savard, G.; Clark, J. A.; Bertone, P. F.; Burkey, M.; Caldwell, S.; Chaudhuri, A.; Greene, J.; Lascar, D.; Levand, A. F.; Li, G.; Galvan, A. Perez; Van Schelt, J.; Zabransky, B. J.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Sternberg, M. G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Segel, R.; Lascar, D.] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [Scielzo, N. D.; Yee, R. M.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA. [Buchinger, F.; Crawford, J. E.; Gulick, S.; Li, G.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Chaudhuri, A.; Sharma, K. S.] Univ Manitoba, Dept Math & Astron, Winnipeg, MB R3T 2N2, Canada. [Deibel, C. M.] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. [Deibel, C. M.] Michigan State Univ, Joint Inst Nucl Astrophys, E Lansing, MI 48824 USA. [Li, G.] Canadian Nucl Labs, Chalk River, ON K0J 1J0, Canada. [Yee, R. M.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. RP Scielzo, ND (reprint author), Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA. EM scielzo1@llnl.gov RI Chaudhuri, Ankur/G-2940-2013 FU NSERC, Canada [216974]; U.S. Department of Energy; Argonne National Laboratory [DE-AC02-06CH11357]; Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We acknowledge the ATLAS staff for their help and support. We thank Dariusz Seweryniak and Calem Hoffman for lending us electronics and providing technical advice. The authors are grateful for discussions with Frederik Wauters on the interpretation of the results of the experiment. This work was carried out under the auspices of the NSERC, Canada, Application No. 216974, and the U.S. Department of Energy, by Argonne National Laboratory under Contract No. DE-AC02-06CH11357 and Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. This research used resources of Argonne National Laboratory's ATLAS facility, which is a DOE Office of Science User Facility. NR 35 TC 4 Z9 4 U1 2 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 28 PY 2015 VL 115 IS 18 AR 182501 DI 10.1103/PhysRevLett.115.182501 PG 6 WC Physics, Multidisciplinary SC Physics GA CU4NT UT WOS:000363507300001 PM 26565463 ER PT J AU van Tilborg, J Steinke, S Geddes, CGR Matlis, NH Shaw, BH Gonsalves, AJ Huijts, JV Nakamura, K Daniels, J Schroeder, CB Benedetti, C Esarey, E Bulanov, SS Bobrova, NA Sasorov, PV Leemans, WP AF van Tilborg, J. Steinke, S. Geddes, C. G. R. Matlis, N. H. Shaw, B. H. Gonsalves, A. J. Huijts, J. V. Nakamura, K. Daniels, J. Schroeder, C. B. Benedetti, C. Esarey, E. Bulanov, S. S. Bobrova, N. A. Sasorov, P. V. Leemans, W. P. TI Active Plasma Lensing for Relativistic Laser-Plasma-Accelerated Electron Beams SO PHYSICAL REVIEW LETTERS LA English DT Article ID Z-PINCH; PARTICLES AB Compact, tunable, radially symmetric focusing of electrons is critical to laser-plasma accelerator (LPA) applications. Experiments are presented demonstrating the use of a discharge-capillary active plasma lens to focus 100-MeV-level LPA beams. The lens can provide tunable field gradients in excess of 3000 T/m, enabling cm-scale focal lengths for GeV-level beam energies and allowing LPA-based electron beams and light sources to maintain their compact footprint. For a range of lens strengths, excellent agreement with simulation was obtained. C1 [van Tilborg, J.; Steinke, S.; Geddes, C. G. R.; Matlis, N. H.; Shaw, B. H.; Gonsalves, A. J.; Huijts, J. V.; Nakamura, K.; Daniels, J.; Schroeder, C. B.; Benedetti, C.; Esarey, E.; Bulanov, S. S.; Leemans, W. P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Shaw, B. H.; Leemans, W. P.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Bobrova, N. A.] Inst Theoret & Expt Phys, Moscow 117218, Russia. [Sasorov, P. V.] MV Keldysh Appl Math Inst, Moscow 125047, Russia. RP van Tilborg, J (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RI Steinke, Sven/D-8086-2011; OI Steinke, Sven/0000-0003-0507-698X; Daniels, Joost/0000-0002-9480-6077; Schroeder, Carl/0000-0002-9610-0166 FU Director, Office of Science, Office of High Energy Physics, of the U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [PHY-1415596]; U.S. Department of Energy National Nuclear Security Administration, Defense Nuclear Nonproliferation RD [NA22] FX This work was supported by the Director, Office of Science, Office of High Energy Physics, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, by the National Science Foundation under Grant No. PHY-1415596, and by the U.S. Department of Energy National Nuclear Security Administration, Defense Nuclear Nonproliferation R&D (NA22). NR 42 TC 13 Z9 13 U1 7 U2 30 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 28 PY 2015 VL 115 IS 18 AR 184802 DI 10.1103/PhysRevLett.115.184802 PG 5 WC Physics, Multidisciplinary SC Physics GA CU4NT UT WOS:000363507300004 PM 26565471 ER PT J AU Iconaru, LI Ban, D Bharatham, K Ramanathan, A Zhang, WX Shelat, AA Zuo, J Kriwacki, RW AF Iconaru, Luigi I. Ban, David Bharatham, Kavitha Ramanathan, Arvind Zhang, Weixing Shelat, Anang A. Zuo, Jian Kriwacki, Richard W. TI Discovery of Small Molecules that Inhibit the Disordered Protein, p27(Kip1) SO SCIENTIFIC REPORTS LA English DT Article ID DRUG DISCOVERY; UNSTRUCTURED PROTEINS; NMR-SPECTROSCOPY; BREAST-CANCER; HAIR-CELLS; CYCLIN-A; C-MYC; BINDING; KINASE; P27 AB Disordered proteins are highly prevalent in biological systems, they control myriad signaling and regulatory processes, and their levels and/or cellular localization are often altered in human disease. In contrast to folded proteins, disordered proteins, due to conformational heterogeneity and dynamics, are not considered viable drug targets. We challenged this paradigm by identifying through NMR-based screening small molecules that bound specifically, albeit weakly, to the disordered cell cycle regulator, p27(Kip1) (p27). Two groups of molecules bound to sites created by transient clusters of aromatic residues within p27. Conserved chemical features within these two groups of small molecules exhibited complementarity to their binding sites within p27, establishing structure-activity relationships for small molecule: disordered protein interactions. Finally, one compound counteracted the Cdk2/cyclin A inhibitory function of p27 in vitro, providing proof-of- principle that small molecules can inhibit the function of a disordered protein (p27) through sequestration in a conformation incapable of folding and binding to a natural regulatory target (Cdk2/cyclin A). C1 [Iconaru, Luigi I.; Ban, David; Zhang, Weixing; Kriwacki, Richard W.] Dept Biol Struct, Memphis, TN 38105 USA. [Iconaru, Luigi I.; Zuo, Jian] Dept Dev Neurobiol, Memphis, TN 38105 USA. [Bharatham, Kavitha; Shelat, Anang A.] St Jude Childrens Res Hosp, Dept Chem Biol & Therapeut, Memphis, TN 38105 USA. [Ramanathan, Arvind] Oak Ridge Natl Lab, Hlth Data Sci Inst, Computat Sci & Engn Div, Oak Ridge, TN 37830 USA. [Kriwacki, Richard W.] Univ Tennessee, Ctr Hlth Sci, Dept Microbiol Immunol & Biochem, Memphis, TN 38163 USA. RP Zuo, J (reprint author), Dept Dev Neurobiol, Memphis, TN 38105 USA. EM jian.zuo@stjude.org; richard.kriwacki@stjude.org FU US National Institutes of Health (NIH) [R01CA082491, 1R01GM083159, 2R01DC006471, 1R21DC013879-01]; Office of Naval Research Grant [N000140911014, N000141210191, N000141210775]; US National Cancer Institute Cancer Center Support Grant (at St. Jude Children's Research Hospital) [P30CA21765]; ALSAC; Garwood Foundation Fellowship from St. Jude Children's Research Hospital; US National Institute of General Medical Science [F32GM113290] FX The authors thank Christy R. Grace for assistance with NMR experiments, Heather Ross for compound library management, and Ariele Viacava Follis for comments on the manuscript. This work was supported by US National Institutes of Health (NIH) grants R01CA082491 and 1R01GM083159 (to R.W.K.), 2R01DC006471 and 1R21DC013879-01 (to J.Z.), Office of Naval Research Grants N000140911014, N000141210191, and N000141210775 (to J.Z.), a US National Cancer Institute Cancer Center Support Grant P30CA21765 (at St. Jude Children's Research Hospital), and ALSAC. L.I.I. was the recipient of the Garwood Foundation Fellowship from St. Jude Children's Research Hospital. D.B. would like to acknowledge support from the US National Institute of General Medical Science (F32GM113290). NR 57 TC 3 Z9 3 U1 3 U2 12 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 28 PY 2015 VL 5 AR 15686 DI 10.1038/srep15686 PG 16 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CU4TH UT WOS:000363522400001 PM 26507530 ER PT J AU Huo, NJ Yang, JH Huang, L Wei, ZM Li, SS Wei, SH Li, JB AF Huo, Nengjie Yang, Juehan Huang, Le Wei, Zhongming Li, Shu-Shen Wei, Su-Huai Li, Jingbo TI Tunable Polarity Behavior and Self-Driven Photoswitching in p-WSe2/n-WS2 Heterojunctions SO SMALL LA English DT Article DE photovoltaics; self-driven photoswitching; tunable polarity; photoswitching; WSe2; WS2 heterojunctions ID DER-WAALS HETEROSTRUCTURES; FIELD-EFFECT TRANSISTORS; P-N DIODES; SINGLE-LAYER; PHOTOCURRENT GENERATION; MONOLAYER MOS2; LIGHT-EMISSION; GRAPHENE; CONTACTS; DEVICES AB Van der Waals (vdW) p-n heterojunctions consisting of various 2D layer compounds are fascinating new artificial materials that can possess novel physics and functionalities enabling the next-generation of electronics and optoelectronics devices. Here, it is reported that the WSe2/WS2 p-n heterojunctions perform novel electrical transport properties such as distinct rectifying, ambipolar, and hysteresis characteristics. Intriguingly, the novel tunable polarity transition along a route of n-anti-bipolar-p-ambipolar is observed in the WSe2/WS2 heterojunctions owing to the successive work of conducting channels of junctions, p-WSe2 and n-WS2 on the electrical transport of the whole systems. The type-II band alignment obtained from first principle calculations and built-in potential in this vdW heterojunction can also facilitate the efficient electron-hole separation, thus enabling the significant photovoltaic effect and a much enhanced self-driven photoswitching response in this system. C1 [Huo, Nengjie; Yang, Juehan; Huang, Le; Wei, Zhongming; Li, Shu-Shen; Li, Jingbo] Chinese Acad Sci, Inst Semicond, State Key Lab Superlattices & Microstruct, Beijing 100083, Peoples R China. [Wei, Su-Huai] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Wei, SH (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM suhuai.wei@nrel.gov; jbli@semi.ac.cn FU National Natural Science Foundation of China [91233120]; National Basic Research Program of China [2011CB921901]; U.S. Department of Energy [DE-AC36-08GO28308] FX This work was supported by the National Natural Science Foundation of China under Grant No. 91233120 and the National Basic Research Program of China (2011CB921901). The work of S.-H. Wei was supported by the U.S. Department of Energy under Contract No. DE-AC36-08GO28308. NR 35 TC 14 Z9 14 U1 11 U2 105 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1613-6810 EI 1613-6829 J9 SMALL JI Small PD OCT 28 PY 2015 VL 11 IS 40 BP 5430 EP 5438 DI 10.1002/smll.201501206 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CU4CP UT WOS:000363474200012 PM 26296851 ER PT J AU Fregoso, BM Coh, S AF Fregoso, Benjamin M. Coh, Sinisa TI Intrinsic surface dipole in topological insulators SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE topological insulators; surface dipole; surface photovoltage; band bending; Schottky barrier solar cell ID TRANSPORT; BI2SE3 AB We calculate the local density of states of two prototypical topological insulators (Bi2Se3 and Bi2Te2Se) as a function of distance from the surface within density functional theory. We find that, in the absence of disorder or doping, there is a 2 nm thick surface dipole the origin of which is the occupation of the topological surface states above the Dirac point. As a consequence, the bottom of the conduction band is bent upward by about 75 meV near the surface, and there is a hump-like feature associated with the top of the valence band. We expect that band bending will occur in all pristine topological insulators as long as the Fermi level does not cross the Dirac point. Our results show that topological insulators are intrinsic Schottky barrier solar cells. C1 [Fregoso, Benjamin M.; Coh, Sinisa] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Coh, Sinisa] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Fregoso, BM (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM benjamin.fregoso@gmail.com FU Conacyt; NSF [DMR-1206513]; NERSC [DE-AC02-05CH11231] FX We thank J Moore, J Analytis, M L Cohen, C Salazar, C Ojeda-Aristizabal and A Drieschova for useful discussions. Support was provided by Conacyt and NSF DMR-1206513, and Computer resources by NERSC under Contract No. DE-AC02-05CH11231. NR 39 TC 4 Z9 4 U1 8 U2 28 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD OCT 28 PY 2015 VL 27 IS 42 AR 422001 DI 10.1088/0953-8984/27/42/422001 PG 5 WC Physics, Condensed Matter SC Physics GA CT1PY UT WOS:000362573500001 PM 26440802 ER PT J AU Matarlo, JS Evans, CE Sharma, I Lavaud, LJ Ngo, SC Shek, R Rajashankar, KR French, JB Tan, DS Tonge, PJ AF Matarlo, Joe S. Evans, Christopher E. Sharma, Indrajeet Lavaud, Lubens J. Ngo, Stephen C. Shek, Roger Rajashankar, Kanagalaghatta R. French, Jarrod B. Tan, Derek S. Tonge, Peter J. TI Mechanism of MenE Inhibition by Acyl-Adenylate Analogues and Discovery of Novel Antibacterial Agents SO BIOCHEMISTRY LA English DT Article ID MENAQUINONE VITAMIN-K2 BIOSYNTHESIS; DOMAIN ALTERNATION MECHANISM; O-SUCCINYLBENZOIC ACID; COENZYME-A LIGASE; MYCOBACTERIUM-TUBERCULOSIS; ESCHERICHIA-COLI; COA SYNTHETASE; FIREFLY LUCIFERASE; ELECTRON-TRANSPORT; BACILLUS-SUBTILIS AB MenE is an o-succinylbenzoyl-CoA (OSB-CoA) synthetase in the bacterial menaquinone biosynthesis pathway and is a promising target for the development of novel antibacterial agents. The enzyme catalyzes CoA ligation via an acyl-adenylate intermediate, and we have previously reported tight-binding inhibitors of MenE based on stable acylsulfonyladenosine analogues of this intermediate, including OSB-AMS (1), which has an IC50 value of <= 25 nM for Escherichia coli MenE. Herein, we show that OSB-AMS reduces menaquinone levels in Staphylococcus aureus, consistent with its proposed mechanism of action, despite the observation that the antibacterial activity of OSB-AMS is similar to 1000-fold lower than the IC50 for enzyme inhibition. To inform the synthesis of MenE inhibitors with improved antibacterial activity, we have undertaken a structure-activity relationship (SAR) study stimulated by the knowledge that OSB-AMS can adopt two isomeric forms in which the OSB side chain exists either as an open-chain keto acid or a cyclic lactol. These studies revealed that negatively charged analogues of the keto acid form bind, while neutral analogues do not, consistent with the hypothesis that the negatively charged keto acid form of OSB-AMS is the active isomer. X-ray crystallography and site-directed mutagenesis confirm the importance of a conserved arginine for binding the OSB carboxylate. Although most lactol isomers tested were inactive, a novel difluoroindanediol inhibitor (11) with improved antibacterial activity was discovered, providing a pathway toward the development of optimized MenE inhibitors in the future. C1 [Matarlo, Joe S.; French, Jarrod B.; Tonge, Peter J.] SUNY Stony Brook, Inst Chem Biol & Drug Discovery, Stony Brook, NY 11794 USA. [Lavaud, Lubens J.; Ngo, Stephen C.; French, Jarrod B.; Tonge, Peter J.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Matarlo, Joe S.; Shek, Roger; French, Jarrod B.] SUNY Stony Brook, Dept Biochem & Cell Biol, Stony Brook, NY 11794 USA. [Evans, Christopher E.; Tan, Derek S.] Mem Sloan Kettering Canc Ctr, Weill Cornell Grad Sch Med Sci, Pharmacol Program, New York, NY 10065 USA. [Sharma, Indrajeet; Tan, Derek S.] Mem Sloan Kettering Canc Ctr, Chem Biol Program, New York, NY 10065 USA. [Tan, Derek S.] Mem Sloan Kettering Canc Ctr, Triinst Res Program, New York, NY 10065 USA. [Rajashankar, Kanagalaghatta R.] Argonne Natl Lab, NE CAT, Argonne, IL 60439 USA. [Rajashankar, Kanagalaghatta R.] Argonne Natl Lab, Dept Chem & Chem Biol, Argonne, IL 60439 USA. RP Tan, DS (reprint author), Mem Sloan Kettering Canc Ctr, Weill Cornell Grad Sch Med Sci, Pharmacol Program, New York, NY 10065 USA. EM tand@mskcc.org; peter.tonge@stonybrook.edu OI French, Jarrod/0000-0002-6762-1309 FU National Institutes of Health (NIH) [R01 GM100477, R01 GM102864, T32 GM073546, P41 GM103403, CCSG P30 CA008748]; NIH [GM-00080]; U.S. Department of Energy [DE-AC02-98CH10886] FX This work was supported by the National Institutes of Health (NIH) (R01 GM100477 to D.S.T., R01 GM102864 to P.J.T., T32 GM073546-Gross to C.E.E., P41 GM103403-Ealick to K.R.R., and CCSG P30 CA008748-Thompson). The National Synchrotron Light Source is supported by NIH Grant GM-00080 (supplement to a PSI program) and U.S. Department of Energy Contract DE-AC02-98CH10886. NR 72 TC 8 Z9 8 U1 3 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD OCT 27 PY 2015 VL 54 IS 42 BP 6514 EP 6524 DI 10.1021/acs.biochem.5b00966 PG 11 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CV0CY UT WOS:000363916200011 PM 26394156 ER PT J AU Moorhead-Rosenberg, Z Huq, A Goodenough, JB Manthiram, A AF Moorhead-Rosenberg, Zach Huq, Ashfia Goodenough, John B. Manthiram, Arumugam TI Electronic and Electrochemical Properties of Li1-xMn1.5Ni0.5O4 Spinel Cathodes As a Function of Lithium Content and Cation Ordering SO CHEMISTRY OF MATERIALS LA English DT Article ID LI-ION BATTERIES; ELECTRICAL-TRANSPORT PROPERTIES; MN3+ CONTENT; KINETIC-PROPERTIES; RATE CAPABILITY; SITE DISORDER; LIMN1.5NI0.5O4; LINI0.5MN1.5O4; LIMN2O4; CONDUCTIVITY AB The electronic and electrochemical properties of the high-voltage spinel LiMn1.5Ni0.5O4 as a function of cation ordering and lithium content have been investigated. Conductivity and activation energy measurements confirm that charge transfer occurs by small polaron hopping and the charge carrier conduction is easier in the Ni:3d band than in the in Mn:3d band. Seebeck coefficient data reveal that the Ni2+/3+. and Ni3+/4+ redox couples are combined in a single,3d band, and that maximum charge carrier concentration occurs where the average Ni oxidation state is close to 3+, corresponding to x = 0.5 in Li Li1-xMn1.5Ni0.5O4. Accordingly, maximum electronic conductivity is found at x = 0.5, regardless of cation ordering. The thermodynamically stable phases formed during cycling were investigated by recording the X-ray diffraction (XRD) of chemically delithiated powders. The more ordered spinels maintained two separate two-phase regions upon lithium extraction, while the more disordered samples exhibited a solid-solubility region from LiMn1.5Ni0.5O4 to Li0.5Mn1.5Ni0.5O4. The conductivity and phase-transformation data of four samples with varying degrees of cation ordering were compared to the electrochemical data collected with lithium cells. Only the most ordered spinel showed inferior rate performance, while the sample annealed for a shorter time performed comparable to the unannealed or disordered samples. The results presented here challenge the most common beliefs about high-voltage spinel: (i) low Mn3+ content is responsible for poor rate performance and (ii) thermodynamically stable solid-solubility is critical for fast kinetics. C1 [Moorhead-Rosenberg, Zach; Goodenough, John B.; Manthiram, Arumugam] Univ Texas Austin, Mat Sci & Engn Program, Austin, TX 78712 USA. [Moorhead-Rosenberg, Zach; Goodenough, John B.; Manthiram, Arumugam] Univ Texas Austin, Texas Mat Inst, Austin, TX 78712 USA. [Huq, Ashfia] Oak Ridge Natl Lab, Chem & Engn Mat Div, Neutron Scattering Directorate, Oak Ridge, TN 37831 USA. RP Manthiram, A (reprint author), Univ Texas Austin, Mat Sci & Engn Program, Austin, TX 78712 USA. EM manth@austin.utexas.edu RI Huq, Ashfia/J-8772-2013 OI Huq, Ashfia/0000-0002-8445-9649 FU National Science Foundation Materials Interdisciplinary Research Team (MIRT) [DMR-1122603]; U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX This work was supported by the National Science Foundation Materials Interdisciplinary Research Team (MIRT) Grant DMR-1122603. Neutron diffraction data collection and analysis was supported by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. Data collection at the Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 45 TC 6 Z9 6 U1 13 U2 104 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD OCT 27 PY 2015 VL 27 IS 20 BP 6934 EP 6945 DI 10.1021/acs.chemmater.5b01356 PG 12 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CV0CM UT WOS:000363915000005 ER PT J AU Bonifacio, CS Carenco, S Wu, CH House, SD Bluhm, H Yang, JC AF Bonifacio, Cecile S. Carenco, Sophie Wu, Cheng Hao House, Stephen D. Bluhm, Hendrik Yang, Judith C. TI Thermal Stability of Core-Shell Nanoparticles: A Combined in Situ Study by XPS and TEM SO CHEMISTRY OF MATERIALS LA English DT Article ID COBALT NANOPARTICLES; SURFACE SEGREGATION; ELECTRON-MICROSCOPY; MAGNETIC-PROPERTIES; OXIDE-FILMS; FUEL-CELL; CATALYSTS; ALLOY; NANOCRYSTALS; DIFFUSION AB In situ techniques of transmission electron microscopy (TEM) and X-ray photoelectron spectroscopy (XPS) were used to investigate the thermal stability of Ni-Co core-shell nanoparticles (NPs). The morphological, structural, and chemical changes involved in the core-shell reconfiguration were studied during in situ annealing through simultaneous imaging and acquisition of elemental maps in the TEM, and acquisition of 0 Is, Ni 3p, and Co 3p XP spectra. The core-shell reconfiguration occurred in a stepwise process of surface oxide removal and metal segregation. Reduction of the stabilizing surface oxide occurred from 320 to 440 degrees C, initiating the core-shell reconfiguration. Above 440 degrees C, the core-shell structure was disrupted through Ni migration from the core to the shell. This resulted in the formation of a homogeneous Ni Co mixed alloy at 600 degrees C. This study provides a mechanistic description of the alteration in the core-shell structures of NPs under vacuum conditions and increasing annealing temperature, which is crucial for understanding these technologically important materials. C1 [Bonifacio, Cecile S.; House, Stephen D.; Yang, Judith C.] Univ Pittsburgh, Dept Chem & Petr Engn, Pittsburgh, PA 15260 USA. [Yang, Judith C.] Univ Pittsburgh, Phys, Pittsburgh, PA 15261 USA. [Carenco, Sophie; Bluhm, Hendrik] Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Carenco, Sophie] Univ Paris 06, Sorbonne Univ, CNRS, Coll France,Lab Chim Matiere Condensee Paris, F-75005 Paris, France. [Wu, Cheng Hao] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Yang, JC (reprint author), Univ Pittsburgh, Dept Chem & Petr Engn & Phys, 208 Benedum Hall,3700 OHara St, Pittsburgh, PA 15261 USA. EM judyyang@pitt.edu RI Carenco, Sophie/D-6512-2011; Foundry, Molecular/G-9968-2014; OI Carenco, Sophie/0000-0002-6164-2053; House, Stephen/0000-0003-2035-6373 FU DOE BES [DE-FG02-03ER15476]; Office of Basic Energy Sciences of the US Department of Energy [DE-AC02-05CH11231] FX C.S.B., S.D.H., and J.C.Y. acknowledge financial support by DOE BES under Contract No. DE-FG02-03ER15476. S.C. acknowledges CNRS, UPMC, and College de France. Electron microscopy was performed at the Molecular Foundry at Lawrence Berkeley National Laboratory, which is supported by the Office of Basic Energy Sciences of the US Department of Energy under Contract No. DE-AC02-05CH11231. C.H.W. acknowledges the ALS doctoral fellowship in residence. We thank Dr. Karen Bustillo for the technical support using the ChemiSTEM and Ross Grieshaber for the careful review of this paper. NR 55 TC 8 Z9 8 U1 13 U2 57 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD OCT 27 PY 2015 VL 27 IS 20 BP 6960 EP 6968 DI 10.1021/acs.chemmater.5b01862 PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CV0CM UT WOS:000363915000007 ER PT J AU Kovarik, L Bowden, M Shi, DC Washton, NM Andersen, A Hu, JZ Lee, J Szanyi, J Kwak, JH Peden, CHF AF Kovarik, Libor Bowden, Mark Shi, Dachuan Washton, Nancy M. Andersen, Amity Hu, Jian Zhi Lee, Jaekyoung Szanyi, Janos Kwak, Ja-Hun Peden, Charles H. F. TI Unraveling the Origin of Structural Disorder in High Temperature Transition Al2O3: Structure of theta-Al2O3 SO CHEMISTRY OF MATERIALS LA English DT Article ID TOTAL-ENERGY CALCULATIONS; GAMMA-ALUMINA SURFACES; WAVE BASIS-SET; DELTA-ALUMINA; ELECTRON-MICROSCOPY; IR SPECTROSCOPIES; THETA-ALUMINA; NMR; DIFFRACTION; EVOLUTION AB The crystallography of transition Al2O3 has been extensively studied in the past, because of the advantageous properties of the oxide in catalytic and a range of other technological applications. However, existing crystallographic models are insufficient to describe the structure of many important Al2O3 polymorphs, because of their highly disordered nature. In this work, we investigate structure and disorder in high-temperature-treated transition Al2O3 and provide a structural description for theta-Al2O3 by using a suite of complementary imaging, spectroscopy, and quantum calculation techniques. Contrary to current understanding, our high-resolution imaging shows that 6-Al2O3 is a disordered composite phase of at least two different end-members. By correlating imaging and spectroscopy results with density functional theory (DFT) calculations, we propose a model that describes O-Al2O3 as a disordered intergrowth of two crystallographic variants at the unit-cell level. One variant is based on beta-Ga2O3, and the other on a monoclinic phase that is closely related to delta-Al2O3. The overall findings and interpretations afford new insight into the origin of poor crystallinity in transition Al2O3, and we also provide new perspectives on structural complexity that can emerge from intergrowth of closely related structural polymorphs. C1 [Kovarik, Libor; Bowden, Mark; Washton, Nancy M.; Andersen, Amity] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Shi, Dachuan; Hu, Jian Zhi; Szanyi, Janos; Peden, Charles H. F.] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. [Lee, Jaekyoung; Kwak, Ja-Hun] UNIST, Dept Chem Engn, Ulsan, South Korea. RP Kovarik, L (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, POB 999, Richland, WA 99352 USA. EM libor.kovarik@pnl.gov RI Hu, Jian Zhi/F-7126-2012; Kovarik, Libor/L-7139-2016 FU U.S. Department of Energy [DE-AC05-76RLO1830]; U.S. DOE, Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences; DOE's Office of Biological and Environmental Research FX The research described in this paper is part of the Chemical Imaging Initiative at Pacific Northwest National Laboratory (PNNL). It was conducted under the Laboratory Directed Research and Development Program at PNNL, a multiprogram national laboratory operated by Battelle Memorial Institute for the U.S. Department of Energy under Contract No. DE-AC05-76RLO1830. Some of the authors (D.S., J.H., J.S., J.H.K., and C.H.F.P.) were supported by the U.S. DOE, Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences. The work was conducted in the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at PNNL. NR 25 TC 5 Z9 5 U1 2 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD OCT 27 PY 2015 VL 27 IS 20 BP 7042 EP 7049 DI 10.1021/acs.chemmater.5b02523 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CV0CM UT WOS:000363915000017 ER PT J AU Wang, ZG Fu, L Ma, G Yan, ECY AF Wang, Zhuguang Fu, Li Ma, Gang Yan, Elsa C. Y. TI Broad-Bandwidth Chiral Sum Frequency Generation Spectroscopy for Probing the Kinetics of Proteins at Interfaces SO LANGMUIR LA English DT Article ID ISLET AMYLOID POLYPEPTIDE; AIR-WATER-INTERFACE; HYDROGEN-EXCHANGE; IN-SITU; VIBRATIONAL SPECTROSCOPY; SECONDARY STRUCTURE; NONLINEAR OPTICS; MOLECULAR-ORIGINS; CYTOCHROME-C; BETA-SHEETS AB The kinetics of proteins at interfaces plays an important role in biological functions and inspires solutions to fundamental problems in biomedical sciences and engineering. Nonetheless, due to the lack of surface-specific and structural-sensitive biophysical techniques, it still remains challenging to probe protein kinetics in situ and in real time without the use of spectroscopic labels at interfaces. Broad-bandwidth chiral sum frequency generation (SFG) spectroscopy has been recently developed for protein kinetic studies at interfaces by tracking the chiral vibrational signals of proteins. In this article, we review our recent progress in kinetic studies of proteins at interfaces using broad-bandwidth chiral SFG spectroscopy. We illustrate the use of chiral SFG signals of protein side chains in the C-H stretch region to monitor self-assembly processes of proteins at interfaces. We also present the use of chiral SFG signals from the protein backbone in the N-H stretch region to probe the real-time kinetics of proton exchange between protein and water at interfaces. In addition, we demonstrate the applications of spectral features of chiral SFG that are typical of protein secondary structures in both the amide I and the N-H stretch regions for monitoring the kinetics of aggregation of amyloid proteins at membrane surfaces. These studies exhibit the power of broad-bandwidth chiral SFG to study protein kinetics at interfaces and the promise of this technique in research areas of surface science to address fundamental problems in biomedical and material sciences. C1 [Wang, Zhuguang; Yan, Elsa C. Y.] Yale Univ, Dept Chem, New Haven, CT 06520 USA. [Fu, Li] Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, Richland, WA 99352 USA. [Ma, Gang] Hebei Univ, Coll Chem & Environm Sci, Minist Educ, Key Lab Med Chem & Mol Diag, Baoding 071002, Peoples R China. RP Yan, ECY (reprint author), Yale Univ, Dept Chem, 225 Prospect St, New Haven, CT 06520 USA. FU Starter Grant Award, Spectroscopy Society of Pittsburgh; National Science Foundation (NSF) [CHE 1213362]; National Institutes of Health (NIH) [1R56DK105381-01] FX E.Y. is the recipient of the Starter Grant Award, Spectroscopy Society of Pittsburgh. This work was supported by the National Science Foundation (NSF) (grant CHE 1213362) and the National Institutes of Health (NIH) (grant 1R56DK105381-01). We thank Ya-Na Chen (Yale University) and Wei Liu (Yale University) for technical assistance. NR 77 TC 0 Z9 0 U1 6 U2 22 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD OCT 27 PY 2015 VL 31 IS 42 BP 11384 EP 11398 DI 10.1021/acs.langmuir.5b02100 PG 15 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CV0CI UT WOS:000363914600002 PM 26196215 ER PT J AU Calder, S Kim, JW Cao, GX Cantoni, C May, AF Cao, HB Aczel, AA Matsuda, M Choi, Y Haskel, D Sales, BC Mandrus, D Lumsden, MD Christianson, AD AF Calder, S. Kim, J. W. Cao, G. -X. Cantoni, C. May, A. F. Cao, H. B. Aczel, A. A. Matsuda, M. Choi, Y. Haskel, D. Sales, B. C. Mandrus, D. Lumsden, M. D. Christianson, A. D. TI Evolution of competing magnetic order in the J(eff)=1/2 insulating state of Sr2Ir1-xRuxO4 SO PHYSICAL REVIEW B LA English DT Article ID TRANSITION; PHASE AB We investigate the magnetic properties of the series Sr2Ir1-xRuxO4 with neutron, resonant x-ray, and magnetization measurements. The results indicate an evolution and coexistence of magnetic structures via a spin-flop transition from ab-plane to c-axis collinear order as the 5d Ir4+ ions are replaced with an increasing concentration of 4d Ru4+ ions. The magnetic structures within the ordered regime of the phase diagram (x < 0.3) are reported. Despite the changes in magnetic structure no alteration of the J(eff) = 1/2 ground state is observed. The behavior of Sr2Ir1-xRuxO4 is consistent with electronic phase separation and diverges from a standard scenario of hole doping. The role of lattice alterations with doping on the magnetic and insulating behavior is considered. The results presented here provide insight into the magnetic insulating states in strong spin-orbit coupled materials and the role perturbations play in altering the behavior. C1 [Calder, S.; Cao, H. B.; Aczel, A. A.; Matsuda, M.; Lumsden, M. D.; Christianson, A. D.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Kim, J. W.; Choi, Y.; Haskel, D.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Cao, G. -X.; Matsuda, M.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Cao, G. -X.; Cantoni, C.; May, A. F.; Sales, B. C.; Mandrus, D.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Christianson, A. D.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RP Calder, S (reprint author), Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. EM caldersa@ornl.gov RI christianson, andrew/A-3277-2016; Aczel, Adam/A-6247-2016; Cao, Huibo/A-6835-2016; Matsuda, Masaaki/A-6902-2016; Mandrus, David/H-3090-2014; May, Andrew/E-5897-2011; Lumsden, Mark/F-5366-2012; OI christianson, andrew/0000-0003-3369-5884; Aczel, Adam/0000-0003-1964-1943; Cao, Huibo/0000-0002-5970-4980; Matsuda, Masaaki/0000-0003-2209-9526; May, Andrew/0000-0003-0777-8539; Lumsden, Mark/0000-0002-5472-9660; Calder, Stuart/0000-0001-8402-3741 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; U.S. DOE [DE-AC02-06CH11357]; U.S. Department of Energy [DE-AC05-00OR22725] FX S.C. thanks A. M. Oles for illuminating discussions. This research at ORNL's High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Part of the work (A.F.M., C.C., D.M., B.C.S., G.C.) was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. DOE Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 29 TC 10 Z9 10 U1 2 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 27 PY 2015 VL 92 IS 16 AR 165128 DI 10.1103/PhysRevB.92.165128 PG 9 WC Physics, Condensed Matter SC Physics GA CU4SU UT WOS:000363521100001 ER PT J AU Gaudet, J Maharaj, DD Sala, G Kermarrec, E Ross, KA Dabkowska, HA Kolesnikov, AI Granroth, GE Gaulin, BD AF Gaudet, J. Maharaj, D. D. Sala, G. Kermarrec, E. Ross, K. A. Dabkowska, H. A. Kolesnikov, A. I. Granroth, G. E. Gaulin, B. D. TI Neutron spectroscopic study of crystalline electric field excitations in stoichiometric and lightly stuffed Yb2Ti2O7 SO PHYSICAL REVIEW B LA English DT Article ID ISING PYROCHLORE MAGNETS; SPIN ICE; TITANATE PYROCHLORES; VISUALIZATION; TRANSITION; HO2TI2O7; OXIDES; IONS AB Time-of-flight neutron spectroscopy has been used to determine the crystalline electric field (CEF) Hamiltonian, eigenvalues and eigenvectors appropriate to the J = 7/2 Yb3+ ion in the candidate quantum spin ice pyrochlore magnet Yb2Ti2O7. The precise ground state (GS) of this exotic, geometrically frustrated magnet is known to be sensitive to weak disorder associated with the growth of single crystals from the melt. Such materials display weak "stuffing," wherein a small proportion, approximate to 2%, of the nonmagnetic Ti4+ sites are occupied by excess Yb3+. We have carried out neutron spectroscopic measurements on a stoichiometric powder sample of Yb2Ti2O7, as well as a crushed single crystal with weak stuffing and an approximate composition of Yb2+xTi2-xO7+y with x = 0.046. All samples display three CEF transitions out of the GS, and the GS doublet itself is identified as primarily composed of m(J) = +/- 1/2, as expected. However, stuffing at low temperatures in Yb2+xTi2-xO7+y induces a similar finite CEF lifetime as is induced in stoichiometric Yb2Ti2O7 by elevated temperature. We conclude that an extended strain field exists about each local " stuffed" site, which produces a distribution of random CEF environments in the lightly stuffed Yb2+xTi2-xO7+y, in addition to producing a small fraction of Yb ions in defective environments with grossly different CEF eigenvalues and eigenvectors. C1 [Gaudet, J.; Maharaj, D. D.; Sala, G.; Kermarrec, E.; Gaulin, B. D.] McMaster Univ, Dept Phys & Astron, Hamilton, ON L8S 4M1, Canada. [Ross, K. A.] Colorado State Univ, Dept Phys, Ft Collins, CO 80523 USA. [Dabkowska, H. A.; Gaulin, B. D.] Brockhouse Inst Mat Res, Hamilton, ON L8S 4M1, Canada. [Kolesnikov, A. I.] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Granroth, G. E.] Oak Ridge Natl Lab, Neutron Data Anal & Visualizat Div, Oak Ridge, TN 37831 USA. [Gaulin, B. D.] Canadian Inst Mat Res, Toronto, ON M5G 1Z8, Canada. RP Gaudet, J (reprint author), McMaster Univ, Dept Phys & Astron, Hamilton, ON L8S 4M1, Canada. EM gaudej@mcmaster.ca RI Kolesnikov, Alexander/I-9015-2012; Granroth, Garrett/G-3576-2012; OI Kolesnikov, Alexander/0000-0003-1940-4649; Granroth, Garrett/0000-0002-7583-8778; Kermarrec, Edwin/0000-0002-3467-5482 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Natural Sciences and Engineering Research Council of Canada (NSERC) FX We would like to acknowledge helpful conversations with M. J. P. Gingras. We would also like to acknowledge T. E. Sherline for technical assistance with the measurements. The neutron scattering data were reduced using Mantid [45] and analyzed using the DAVE software package [46]. Research using ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Work at McMaster University was funded by Natural Sciences and Engineering Research Council of Canada (NSERC). NR 46 TC 10 Z9 10 U1 5 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 27 PY 2015 VL 92 IS 13 AR 134420 DI 10.1103/PhysRevB.92.134420 PG 10 WC Physics, Condensed Matter SC Physics GA CU4RY UT WOS:000363518800001 ER PT J AU Matt, CE Fatuzzo, CG Sassa, Y Mansson, M Fatale, S Bitetta, V Shi, X Pailhes, S Berntsen, MH Kurosawa, T Oda, M Momono, N Lipscombe, OJ Hayden, SM Yan, JQ Zhou, JS Goodenough, JB Pyon, S Takayama, T Takagi, H Patthey, L Bendounan, A Razzoli, E Shi, M Plumb, NC Radovic, M Grioni, M Mesot, J Tjernberg, O Chang, J AF Matt, C. E. Fatuzzo, C. G. Sassa, Y. Mansson, M. Fatale, S. Bitetta, V. Shi, X. Pailhes, S. Berntsen, M. H. Kurosawa, T. Oda, M. Momono, N. Lipscombe, O. J. Hayden, S. M. Yan, J. -Q. Zhou, J. -S. Goodenough, J. B. Pyon, S. Takayama, T. Takagi, H. Patthey, L. Bendounan, A. Razzoli, E. Shi, M. Plumb, N. C. Radovic, M. Grioni, M. Mesot, J. Tjernberg, O. Chang, J. TI Electron scattering, charge order, and pseudogap physics in La1.6-xNd0.4SrxCuO4: An angle-resolved photoemission spectroscopy study SO PHYSICAL REVIEW B LA English DT Article ID HIGH-T-C; TEMPERATURE CUPRATE SUPERCONDUCTORS; FERMI-SURFACE RECONSTRUCTION; COPPER-OXIDE SUPERCONDUCTORS; STRIPE-PHASE ORDER; QUANTUM OSCILLATIONS; SYMMETRY-BREAKING; ENERGY GAPS; UNDERDOPED BI2SR2CACU2O8+DELTA; TRANSITION-TEMPERATURE AB We report an angle-resolved photoemission study of the charge stripe ordered La1.6-xNd0.4SrxCuO4 (Nd-LSCO) system. A comparative and quantitative line-shape analysis is presented as the system evolves from the overdoped regime into the charge ordered phase. On the overdoped side (x = 0.20), a normal-state antinodal spectral gap opens upon cooling below 80 K. In this process, spectral weight is preserved but redistributed to larger energies. A correlation between this spectral gap and electron scattering is found. A different line shape is observed in the antinodal region of charge ordered Nd-LSCO x = 1/8. Significant low-energy spectral weight appears to be lost. These observations are discussed in terms of spectral-weight redistribution and gapping originating from charge stripe ordering. C1 [Matt, C. E.; Sassa, Y.; Shi, X.; Patthey, L.; Bendounan, A.; Razzoli, E.; Shi, M.; Plumb, N. C.; Radovic, M.; Chang, J.] Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland. [Matt, C. E.; Sassa, Y.; Mesot, J.] ETH, Lab Solid State Phys, CH-8093 Zurich, Switzerland. [Fatuzzo, C. G.; Mansson, M.; Fatale, S.; Bitetta, V.; Grioni, M.; Mesot, J.; Chang, J.] Ecole Polytech Fed Lausanne, Inst Condensed Matter Phys, CH-1015 Lausanne, Switzerland. [Sassa, Y.] Uppsala Univ, Dept Phys & Astron, S-75121 Uppsala, Sweden. [Mansson, M.; Berntsen, M. H.; Tjernberg, O.] KTH Royal Inst Technol, Mat Phys, S-16440 Kista, Sweden. [Mansson, M.; Pailhes, S.; Mesot, J.] Paul Scherrer Inst, Lab Neutron Scattering, CH-5232 Villigen, Switzerland. [Pailhes, S.] Univ Lyon 1, Inst Lumiere Matiere, CNRS, UMR5306, F-69622 Villeurbanne, France. [Kurosawa, T.; Oda, M.] Hokkaido Univ, Dept Phys, Sapporo, Hokkaido 0600810, Japan. [Momono, N.] Muroran Inst Technol, Dept Appl Sci, Muroran, Hokkaido 0508585, Japan. [Lipscombe, O. J.; Hayden, S. M.] Univ Bristol, HH Wills Phys Lab, Bristol BS8 1TL, Avon, England. [Yan, J. -Q.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Zhou, J. -S.; Goodenough, J. B.] Univ Texas Austin, Texas Mat Inst, Austin, TX 78712 USA. [Pyon, S.; Takayama, T.; Takagi, H.] Univ Tokyo, Dept Adv Mat, Kashiwa, Chiba 2778561, Japan. [Razzoli, E.] Univ Fribourg, Dept Phys, CH-1700 Fribourg, Switzerland. [Razzoli, E.] Univ Fribourg, Fribourg Ctr Nanomat, CH-1700 Fribourg, Switzerland. [Tjernberg, O.] KTH Royal Inst Technol, Ctr Quantum Mat, S-10691 Stockholm, Sweden. [Tjernberg, O.] Stockholm Univ, S-10691 Stockholm, Sweden. [Chang, J.] Univ Zurich, Inst Phys, CH-8057 Zurich, Switzerland. RP Matt, CE (reprint author), Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland. RI Berntsen, Magnus/B-7529-2012; Hayden, Stephen/F-4162-2011; Mansson, Martin/C-1134-2014; Chang, Johan/F-1506-2014; Plumb, Nicholas/B-8059-2013; EPFL, Physics/O-6514-2016; Sassa, Yasmine/F-3362-2017 OI Berntsen, Magnus/0000-0002-7833-3943; Hayden, Stephen/0000-0002-3209-027X; Mansson, Martin/0000-0002-3086-9642; Chang, Johan/0000-0002-4655-1516; Plumb, Nicholas/0000-0002-2334-8494; FU Swiss National Science Foundation [200020-105151, 200021-137783, 200020_159753/1, BSSGI0_155873]; Ministry of Education and Science of Japan; United Kingdom Engineering and Physical Science Research Council [EP/J015423/1]; Wenner-Gren Stiftelserna; Swedish Research Council; US Department of Energy, BES, Materials Sciences and Engineering Division; US NSF [DMR 1122603]; Marie Sklodowska Curie Action; International Career Grant through the European Union; Swedish Research Council (VR) [INCA-2014-6426] FX This work was supported by the Swiss National Science Foundation [through Grants No. 200020-105151, No. 200021-137783, No. 200020_159753/1, No. BSSGI0_155873 and its NCCR - MaNEP and Sinergia network Mott Physics Beyond the Heisenberg (HPBH) model], the Ministry of Education and Science of Japan, the United Kingdom Engineering and Physical Science Research Council [Grant No. EP/J015423/1], Wenner-Gren Stiftelserna, and the Swedish Research Council. Work at ORNL was supported by the US Department of Energy, BES, Materials Sciences and Engineering Division. J.S.Z. and J.B.G. were supported by the US NSF (Grant No. DMR 1122603) and M.M. was supported by Marie Sklodowska Curie Action, International Career Grant through the European Union and Swedish Research Council (VR), Grant No. INCA-2014-6426. The photoemission experiments were performed at SLS of the Paul Scherrer Institut, Villigen PSI, Switzerland. We thank the X09LA beam-line [33] staff and Xiaoping Wang for technical support. We wish to thank Nicolas Doiron-Leyraud, Paul Freemann, Markus Hucker, Claude Monney, Henrik Ronnow, Louis Taillefer, and Andre-Marie Tremblay for enlightening discussions. NR 107 TC 5 Z9 5 U1 9 U2 37 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 27 PY 2015 VL 92 IS 13 AR 134524 DI 10.1103/PhysRevB.92.134524 PG 10 WC Physics, Condensed Matter SC Physics GA CU4RY UT WOS:000363518800002 ER PT J AU Martinez-Gonzalez, JA Zhou, Y Rahimi, M Bukusoglu, E Abbott, NL de Pablo, JJ AF Martinez-Gonzalez, Jose A. Zhou, Ye Rahimi, Mohammad Bukusoglu, Emre Abbott, Nicholas L. de Pablo, Juan J. TI Blue-phase liquid crystal droplets SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE blue phases; chiral liquid crystals; droplets; confinement ID CHIRAL NEMATIC DROPLETS; STABILIZATION; TRANSITIONS AB Blue phases of liquid crystals represent unique ordered states of matter in which arrays of defects are organized into striking patterns. Most studies of blue phases to date have focused on bulk properties. In this work, we present a systematic study of blue phases confined into spherical droplets. It is found that, in addition to the so-called blue phases I and II, several new morphologies arise under confinement, with a complexity that increases with the chirality of the medium and with a nature that can be altered by surface anchoring. Through a combination of simulations and experiments, it is also found that one can control the wavelength at which blue-phase droplets absorb light by manipulating either their size or the strength of the anchoring, thereby providing a liquid-state analog of nano-particles, where dimensions are used to control absorbance or emission. The results presented in this work also suggest that there are conditions where confinement increases the range of stability of blue phases, thereby providing intriguing prospects for applications. C1 [Martinez-Gonzalez, Jose A.; Zhou, Ye; Rahimi, Mohammad; de Pablo, Juan J.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. [Bukusoglu, Emre; Abbott, Nicholas L.] Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 94720 USA. [de Pablo, Juan J.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP de Pablo, JJ (reprint author), Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. EM depablo@uchicago.edu OI Martinez-Gonzalez, Jose Adrian/0000-0001-7257-8889 FU Department of Energy, Basic Energy Sciences, Materials Science and Engineering Division, Biomaterials Program [DE-SC004025]; Consejo Nacional de Ciencia y Tecnologia (CONACYT) Fellowship [250263] FX This work is supported by the Department of Energy, Basic Energy Sciences, Materials Science and Engineering Division, Biomaterials Program, through DE-SC004025. The calculations reported here were performed on The University of Chicago Research Computing Center. The authors also acknowledge an Innovative and Novel Computational Impact on Theory and Experiment (INCITE) grant at Argonne National Laboratory which permitted additional large-scale simulations of droplets. J.A.M.-G. is grateful for the Consejo Nacional de Ciencia y Tecnologia (CONACYT) Fellowship 250263. NR 49 TC 6 Z9 6 U1 15 U2 49 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 27 PY 2015 VL 112 IS 43 BP 13195 EP 13200 DI 10.1073/pnas.1514251112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CU3WY UT WOS:000363458100039 PM 26460039 ER PT J AU Dong, B Yang, XC Zhu, SB Bassham, DC Fang, N AF Dong, Bin Yang, Xiaochen Zhu, Shaobin Bassham, Diane C. Fang, Ning TI Stochastic Optical Reconstruction Microscopy Imaging of Microtubule Arrays in Intact Arabidopsis thaliana Seedling Roots SO SCIENTIFIC REPORTS LA English DT Article ID STRUCTURED-ILLUMINATION MICROSCOPY; THICK BIOLOGICAL SAMPLES; CORTICAL MICROTUBULES; FLUORESCENT-PROBES; CYTOSKELETAL CONTROL; PLASMA-MEMBRANE; PLANT-CELLS; SUPERRESOLUTION; GROWTH; ORGANIZATION AB Super-resolution fluorescence microscopy has generated tremendous success in revealing detailed subcellular structures in animal cells. However, its application to plant cell biology remains extremely limited due to numerous technical challenges, including the generally high fluorescence background of plant cells and the presence of the cell wall. In the current study, stochastic optical reconstruction microscopy (STORM) imaging of intact Arabidopsis thaliana seedling roots with a spatial resolution of 20-40 nm was demonstrated. Using the super-resolution images, the spatial organization of cortical microtubules in different parts of a whole Arabidopsis root tip was analyzed quantitatively, and the results show the dramatic differences in the density and spatial organization of cortical microtubules in cells of different differentiation stages or types. The method developed can be applied to plant cell biological processes, including imaging of additional elements of the cytoskeleton, organelle substructure, and membrane domains. C1 [Dong, Bin; Zhu, Shaobin] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. [Dong, Bin; Zhu, Shaobin] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Yang, Xiaochen; Bassham, Diane C.] Iowa State Univ, Dept Genet Dev & Cell Biol, Ames, IA 50011 USA. [Bassham, Diane C.] Iowa State Univ, Plant Sci Inst, Ames, IA 50011 USA. [Fang, Ning] Georgia State Univ, Dept Chem, Atlanta, GA 30302 USA. RP Bassham, DC (reprint author), Iowa State Univ, Dept Genet Dev & Cell Biol, Ames, IA 50011 USA. EM bassham@iastate.edu; nfang@gsu.edu FU Iowa State University Plant Sciences Institute; National Science Foundation [IOS-1353867]; Georgia State University FX This work was supported by the Iowa State University Plant Sciences Institute, by grant no. IOS-1353867 to D.C.B. from the National Science Foundation, and by the Start-up Funds provided to N.F. from Georgia State University. We thank Dr. Bo Huang and Jorg Schnitzbauer at the University of California, San Francisco for providing the imaging data analysis program 'Insight3' and for assistance with data analysis. NR 53 TC 0 Z9 0 U1 4 U2 14 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 27 PY 2015 VL 5 AR 15694 DI 10.1038/srep15694 PG 14 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CU3TJ UT WOS:000363447900002 PM 26503365 ER PT J AU Harrison, SE Collins-McIntyre, LJ Schonherr, P Vailionis, A Srot, V van Aken, PA Kellock, AJ Pushp, A Parkin, SSP Harris, JS Zhou, B Chen, YL Hesjedal, T AF Harrison, S. E. Collins-McIntyre, L. J. Schoenherr, P. Vailionis, A. Srot, V. van Aken, P. A. Kellock, A. J. Pushp, A. Parkin, S. S. P. Harris, J. S. Zhou, B. Chen, Y. L. Hesjedal, T. TI Massive Dirac Fermion Observed in Lanthanide-Doped Topological Insulator Thin Films SO SCIENTIFIC REPORTS LA English DT Article ID PHASE-TRANSITION AB The breaking of time reversal symmetry (TRS) in three-dimensional (3D) topological insulators (TIs), and thus the opening of a 'Dirac-mass gap' in the linearly dispersed Dirac surface state, is a prerequisite for unlocking exotic physical states. Introducing ferromagnetic long-range order by transition metal doping has been shown to break TRS. Here, we present the study of lanthanide (Ln) doped Bi2Te3, where the magnetic doping with high-moment lanthanides promises large energy gaps. Using molecular beam epitaxy, single-crystalline, rhombohedral thin films with Ln concentrations of up to similar to 35%, substituting on Bi sites, were achieved for Dy, Gd, and Ho doping. Angle-resolved photoemission spectroscopy shows the characteristic Dirac cone for Gd and Ho doping. In contrast, for Dy doping above a critical doping concentration, a gap opening is observed via the decreased spectral intensity at the Dirac point, indicating a topological quantum phase transition persisting up to room-temperature. C1 [Harrison, S. E.; Collins-McIntyre, L. J.; Schoenherr, P.; Zhou, B.; Chen, Y. L.; Hesjedal, T.] Univ Oxford, Dept Phys, Clarendon Lab, Oxford OX1 3PU, England. [Harrison, S. E.; Harris, J. S.] Stanford Univ, Dept Elect Engn, Stanford, CA 94305 USA. [Vailionis, A.] Stanford Univ, Geballe Lab Adv Mat, Stanford, CA 94305 USA. [Srot, V.; van Aken, P. A.] Max Planck Inst Intelligent Syst, Stuttgart Ctr Electron Microscopy, D-70569 Stuttgart, Germany. [Kellock, A. J.; Pushp, A.; Parkin, S. S. P.; Zhou, B.] IBM Almaden Res Ctr, San Jose, CA 95120 USA. [Zhou, B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Hesjedal, T (reprint author), Univ Oxford, Dept Phys, Clarendon Lab, Oxford OX1 3PU, England. EM thorsten.hesjedal@physics.ox.ac.uk RI Hesjedal, Thorsten/C-6853-2014; Vailionis, Arturas/C-5202-2008 OI Hesjedal, Thorsten/0000-0001-7947-3692; Vailionis, Arturas/0000-0001-5878-1864 FU John Fell Oxford University Press (OUP) Research Fund; DARPA MESO Project [N66001-11-1-4105]; European Union [312483 - ESTEEM2]; VPGE (Stanford University); EPSRC (UK); EPSRC; Corpus Christi College (Oxford); Studienstiftung des deutschen Volkes (Germany) FX This publication arises from research funded by the John Fell Oxford University Press (OUP) Research Fund, a DARPA MESO Project (No. N66001-11-1-4105), and funding from the European Union Seventh Framework Programme under Grant Agreement 312483 - ESTEEM2 (Integrated Infrastructure Initiative I3) and transnational access to MPI-IS (WP13). Part of this work was performed at the Stanford Nano Shared Facilities (SNSF). S.E.H. was supported by the VPGE (Stanford University), L.C.M. by EPSRC (UK), and P.S. acknowledges partial funding from EPSRC, Corpus Christi College (Oxford), and the Studienstiftung des deutschen Volkes (Germany). RCaH is acknowledged for their hospitality. V.S. and P.v.A. thank Birgit Bussmann and Marion Kelsch (both MPI-IS) for developing a novel technique for delaminating sensitive films from substrates and for preparing thin TEM slices using ultramicrotomy. V.S. thanks Prof. Masashi Watanabe (Lehigh University) for the introduction to the MSA software and treatment of EDX data. We thank A.A. Baker for experimental assistance and useful discussions throughout the course of this work. NR 30 TC 5 Z9 5 U1 6 U2 33 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 27 PY 2015 VL 5 AR 15767 DI 10.1038/srep15767 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CU3VD UT WOS:000363453000001 PM 26503435 ER PT J AU Khurshid, H Lampen-Kelley, P Iglesias, O Alonso, J Phan, MH Sun, CJ Saboungi, ML Srikanth, H AF Khurshid, Hafsa Lampen-Kelley, Paula Iglesias, Oscar Alonso, Javier Manh-Huong Phan Sun, Cheng-Jun Saboungi, Marie-Louise Srikanth, Hariharan TI Spin-glass-like freezing of inner and outer surface layers in hollow gamma-Fe2O3 nanoparticles SO SCIENTIFIC REPORTS LA English DT Article ID MAGNETIC NANOPARTICLES; PARTICLE SYSTEM; AGING PHENOMENA; DYNAMICS; TEMPERATURE; BEHAVIOR; SPHERES; GROWTH; MEMORY AB Disorder among surface spins is a dominant factor in the magnetic response of magnetic nanoparticle systems. In this work, we examine time-dependent magnetization in high-quality, monodisperse hollow maghemite nanoparticles (NPs) with a 14.8 +/- 0.5 nm outer diameter and enhanced surface-to-volume ratio. The nanoparticle ensemble exhibits spin-glass-like signatures in dc magnetic aging and memory protocols and ac magnetic susceptibility. The dynamics of the system slow near 50 K, and become frozen on experimental time scales below 20 K. Remanence curves indicate the development of magnetic irreversibility concurrent with the freezing of the spin dynamics. A strong exchange-bias effect and its training behavior point to highly frustrated surface spins that rearrange much more slowly than interior spins. Monte Carlo simulations of a hollow particle corroborate strongly disordered surface layers with complex energy landscapes that underlie both glass-like dynamics and magnetic irreversibility. Calculated hysteresis loops reveal that magnetic behavior is not identical at the inner and outer surfaces, with spins at the outer surface layer of the 15 nm hollow particles exhibiting a higher degree of frustration. Our combined experimental and simulated results shed light on the origin of spin-glass-like phenomena and the important role played by the surface spins in magnetic hollow nanostructures. C1 [Khurshid, Hafsa; Lampen-Kelley, Paula; Alonso, Javier; Manh-Huong Phan; Srikanth, Hariharan] Univ S Florida, Dept Phys, Tampa, FL 33620 USA. [Iglesias, Oscar] Univ Barcelona, Dept Fis Fonamental, E-08028 Barcelona, Spain. [Iglesias, Oscar] Univ Barcelona, Inst Nanociencia & Nanotecnol N2UB, E-08028 Barcelona, Spain. [Alonso, Javier; Saboungi, Marie-Louise] BCMaterials, Derio 48160, Spain. [Sun, Cheng-Jun] Argonne Natl Lab, Adv Photon Source, Argonne, IL USA. [Saboungi, Marie-Louise] Univ Paris 06, F-75252 Paris 05, France. [Saboungi, Marie-Louise] Univ Orleans, F-45067 Orleans, France. RP Phan, MH (reprint author), Univ S Florida, Dept Phys, Tampa, FL 33620 USA. EM phanm@usf.edu; sharihar@usf.edu RI Iglesias, Oscar/A-8274-2008; Phan, Manh-Huong/A-6709-2014 OI Iglesias, Oscar/0000-0002-5526-9491; FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-FG02-07ER46438]; Spanish MINECO [MAT2012-33037]; Catalan DURSI [2009SGR856, 2014SGR220]; European Union FEDER funds (Una manera de hacer Europa); US Department of Energy - Basic Energy Sciences; Canadian Light Source; University of Washington; Advanced Photon Source; U.S. DOE [DE-AC02-06CH11357]; Basque Government; CNRS, Paris, France FX Research at the University of South Florida (NPs synthesis, structural and magnetic studies) was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award No. DE-FG02-07ER46438. Research at the University of Barcelona (Magnetic simulation) was supported by Spanish MINECO (MAT2012-33037), Catalan DURSI (2009SGR856 and 2014SGR220), and European Union FEDER funds (Una manera de hacer Europa). Sector 20 facilities at the Advanced Photon Source, and research at these facilities, are supported by the US Department of Energy - Basic Energy Sciences, the Canadian Light Source and its funding partners, the University of Washington, and the Advanced Photon Source. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. Javier Alonso acknowledges the financial support provided through a postdoctoral fellowship from Basque Government. MLS acknowledges financial support from the CNRS, Paris, France and we thank Tao Li, Bachir Aoun and Yang Ren for their help with the synchrotron measurements. The authors are grateful for technical and human support provided by Inaki Orue from the Magnetic Measurements Service (SGIker) of UPV/EHU. NR 61 TC 13 Z9 13 U1 5 U2 49 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 27 PY 2015 VL 5 AR 15054 DI 10.1038/srep15054 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CU3SS UT WOS:000363446200001 PM 26503506 ER PT J AU Zhong, S Qian, Y Zhao, C Leung, R Yang, XQ AF Zhong, Shi Qian, Yun Zhao, Chun Leung, Ruby Yang, Xiu-Qun TI A case study of urbanization impact on summer precipitation in the Greater Beijing Metropolitan Area: Urban heat island versus aerosol effects SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article AB Convection-resolving ensemble simulations using the WRF-Chem model coupled with a single-layer Urban Canopy Model are conducted to investigate the individual and combined impacts of land use and anthropogenic pollutant emissions from urbanization on a heavy rainfall event in the Greater Beijing Metropolitan Area (GBMA) in China. The simulation with the urbanization effect included generally captures the spatial pattern and temporal variation of the rainfall event. An improvement of precipitation is found in the experiment including aerosol effect on both clouds and radiation. The expanded urban land cover and increased aerosols have an opposite effect on precipitation processes, with the latter playing a more dominant role, leading to suppressed convection and rainfall over the upstream (northwest) area, and enhanced convection and more precipitation in the downstream (southeast) region of the GBMA. In addition, the influence of aerosol indirect effect is found to overwhelm that of direct effect on precipitation in this rainfall event. Increased aerosols lead to more cloud droplets with smaller size, which favor evaporative cooling and reduce updrafts and suppress convection over the upstream (northwest) region in the early stage of the rainfall event. As the rainfall system propagates southeastward, more latent heat is released due to the freezing of larger number of smaller cloud drops that are lofted above the freezing level, which is responsible for the increased updraft strength and convective invigoration over the downstream (southeast) area. C1 [Zhong, Shi; Yang, Xiu-Qun] Nanjing Univ, Sch Atmospher Sci, Nanjing, Jiangsu, Peoples R China. [Zhong, Shi; Qian, Yun; Zhao, Chun; Leung, Ruby] Pacific Northwest Natl Lab, Richland, WA 99352 USA. RP Qian, Y (reprint author), Pacific Northwest Natl Lab, Richland, WA 99352 USA. EM Yun.Qian@pnnl.gov RI qian, yun/E-1845-2011; Zhao, Chun/A-2581-2012; Yang, Michael/G-9716-2013 OI Zhao, Chun/0000-0003-4693-7213; FU National Basic Research program of China [2010CB428504]; Jiangsu Collaborative Innovation Center for Climate Change; China Scholarship Council; U.S. Department of Energy's Office of Science as part of the Atmospheric System Research (ASR) program; Regional and Global Climate Modeling Program; DOE [DE-AC05-76RL01830] FX The contribution of Shi Zhong and Xiu-Qun Yang in this study is supported by the National Basic Research program of China (2010CB428504), Jiangsu Collaborative Innovation Center for Climate Change, and the Scholarship Award for Excellent Doctoral Student granted by China Scholarship Council. The contributions of Yun Qian, Chun Zhao, and Ruby Leung in this study are supported by the U.S. Department of Energy's Office of Science as part of the Atmospheric System Research (ASR) program and the Regional and Global Climate Modeling Program. The Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under contract DE-AC05-76RL01830. This study used computing resources from the PNNL Institutional Computing. All model results are stored at a PNNL cluster and available upon request. Please contact Yun Qian (yun.qian@pnnl.gov). NR 60 TC 1 Z9 1 U1 14 U2 54 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD OCT 27 PY 2015 VL 120 IS 20 BP 10903 EP 10914 DI 10.1002/2015JD023753 PG 12 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA V45WP UT WOS:000209847000020 ER PT J AU Berben, T Sorokin, DY Ivanova, N Pati, A Kyrpides, N Goodwin, LA Woyke, T Muyzer, G AF Berben, Tom Sorokin, Dimitry Y. Ivanova, Natalia Pati, Amrita Kyrpides, Nikos Goodwin, Lynne A. Woyke, Tanja Muyzer, Gerard TI Partial genome sequence of Thioalkalivibrio thiocyanodenitrificans ARhD 1(T), a chemolithoautotrophic haloalkaliphilic sulfur-oxidizing bacterium capable of complete denitrification SO STANDARDS IN GENOMIC SCIENCES LA English DT Article ID SODA LAKES; SP-NOV; TOOL AB Thioalkalivibrio thiocyanodenitrificans strain ARhD 1(T) is a motile, Gram-negative bacterium isolated from soda lakes that belongs to the Gammaproteobacteria. It derives energy for growth and carbon fixation from the oxidation of sulfur compounds, most notably thiocyanate, and so is a chemolithoautotroph. It is capable of complete denitrification under anaerobic conditions. The draft genome sequence consists of 3,746,647 bp in 3 scaffolds, containing 3558 protein-coding and 121 RNA genes. T. thiocyanodenitrificans ARhD 1(T) was sequenced as part of the DOE Joint Genome Institute Community Science Program. C1 [Berben, Tom; Muyzer, Gerard] Univ Amsterdam, Inst Biodivers & Ecosyst Dynam, Dept Aquat Microbiol, Microbial Syst Ecol, Amsterdam, Netherlands. [Sorokin, Dimitry Y.] RAS, Winogradsky Inst Microbiol, Moscow 117901, Russia. [Sorokin, Dimitry Y.] Delft Univ Technol, Dept Biotechnol, Delft, Netherlands. [Ivanova, Natalia; Pati, Amrita; Kyrpides, Nikos; Goodwin, Lynne A.; Woyke, Tanja] Joint Genome Inst, Walnut Creek, CA USA. RP Muyzer, G (reprint author), Univ Amsterdam, Inst Biodivers & Ecosyst Dynam, Dept Aquat Microbiol, Microbial Syst Ecol, Amsterdam, Netherlands. EM g.muijzer@uva.nl RI Kyrpides, Nikos/A-6305-2014; OI Kyrpides, Nikos/0000-0002-6131-0462; Muyzer, Gerard/0000-0002-2422-0732; Berben, Tom/0000-0003-1833-8731; Ivanova, Natalia/0000-0002-5802-9485 FU U.S. Department of Energy Joint Genome Institute, a DOE Office of Science User Facility [DE-AC02-05CH11231]; ERC [322551]; RBFR [13-04-00049] FX The work conducted by the U.S. Department of Energy Joint Genome Institute, a DOE Office of Science User Facility, is supported under Contract No. DE-AC02-05CH11231. Tom Berben and Gerard Muyzer are supported by ERC Advanced Grant PARASOL (No. 322551). Dimitry Sorokin is supported by RBFR grant 13-04-00049. NR 24 TC 1 Z9 2 U1 2 U2 4 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD OCT 26 PY 2015 VL 10 AR 84 DI 10.1186/s40793-015-0080-3 PG 5 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DA7QW UT WOS:000368000200001 PM 26512309 ER PT J AU Berben, T Sorokin, DY Ivanova, N Pati, A Kyrpides, N Goodwin, LA Woyke, T Muyzer, G AF Berben, Tom Sorokin, Dimitry Y. Ivanova, Natalia Pati, Amrita Kyrpides, Nikos Goodwin, Lynne A. Woyke, Tanja Muyzer, Gerard TI Partial genome sequence of the haloalkaliphilic soda lake bacterium Thioalkalivibrio thiocyanoxidans ARh 2(T) SO STANDARDS IN GENOMIC SCIENCES LA English DT Article DE Haloalkaliphilic; Soda lakes; Sulfur-oxidizing bacteria; Thiocyanate ID SULFUR-OXIDIZING BACTERIA; SP-NOV AB Thioalkalivibrio thiocyanoxidans strain ARh 2(T) is a sulfur-oxidizing bacterium isolated from haloalkaline soda lakes. It is a motile, Gram-negative member of the Gammaproteobacteria. Remarkable properties include the ability to grow on thiocyanate as the sole energy, sulfur and nitrogen source, and the capability of growth at salinities of up to 4.3 M total Na+. This draft genome sequence consists of 61 scaffolds comprising 2,765,337 bp, and contains 2616 protein-coding and 61 RNA-coding genes. This organism was sequenced as part of the Community Science Program of the DOE Joint Genome Institute. C1 [Berben, Tom; Muyzer, Gerard] Univ Amsterdam, Inst Biodivers & Ecosyst Dynam, Microbial Syst Ecol, Amsterdam, Netherlands. [Sorokin, Dimitry Y.] RAS, Winogradsky Inst Microbiol, Moscow 117901, Russia. [Sorokin, Dimitry Y.] Delft Univ Technol, Dept Biotechnol, Delft, Netherlands. [Ivanova, Natalia; Pati, Amrita; Kyrpides, Nikos; Goodwin, Lynne A.; Woyke, Tanja] Joint Genome Inst, Walnut Creek, CA USA. RP Muyzer, G (reprint author), Univ Amsterdam, Inst Biodivers & Ecosyst Dynam, Microbial Syst Ecol, Amsterdam, Netherlands. EM g.muijzer@uva.nl RI Kyrpides, Nikos/A-6305-2014; OI Kyrpides, Nikos/0000-0002-6131-0462; Muyzer, Gerard/0000-0002-2422-0732; Berben, Tom/0000-0003-1833-8731; Ivanova, Natalia/0000-0002-5802-9485 FU U.S. Department of Energy Joint Genome Institute, a DOE Office of Science User Facility [DE-AC02-05CH11231]; ERC [322551]; RBFR [13-04-00049] FX The work conducted by the U.S. Department of Energy Joint Genome Institute, a DOE Office of Science User Facility, is supported under Contract No. DE-AC02-05CH11231. Tom Berben and Gerard Muyzer are supported by ERC Advanced Grant PARASOL (No. 322551). Dimitry Sorokin is supported by RBFR Grant 13-04-00049. NR 21 TC 1 Z9 1 U1 2 U2 5 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD OCT 26 PY 2015 VL 10 AR 85 DI 10.1186/s40793-015-0078-x PG 5 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DA7QW UT WOS:000368000200002 PM 26512310 ER PT J AU Eshraghi, L De Meyer, SE Tian, R Seshadri, R Ivanova, N Pati, A Markowitz, V Woyke, T Kyrpides, NC Tiwari, R Yates, R Howieson, J Reeve, W AF Eshraghi, Leila De Meyer, Sofie E. Tian, Rui Seshadri, Rekha Ivanova, Natalia Pati, Amrita Markowitz, Victor Woyke, Tanja Kyrpides, Nikos C. Tiwari, Ravi Yates, Ron Howieson, John Reeve, Wayne TI High-quality permanent draft genome sequence of Bradyrhizobium sp strain WSM1743-an effective microsymbiont of an Indigofera sp growing in Australia SO STANDARDS IN GENOMIC SCIENCES LA English DT Article DE Root-nodule bacteria; Nitrogen fixation; Rhizobia; Alphaproteobacteria; GEBA RNB ID ROOT-NODULE BACTERIA; MICROBIAL GENOMES; ACID TOLERANCE; SYSTEM; JAPONICUM; YUANMINGENSE; RHIZOBIA; DATABASE; GENUS; NOV AB Bradyrhizobium sp. strain WSM1743 is an aerobic, motile, Gram-negative, non-spore-forming rod that can exist as a soil saprophyte or as a legume microsymbiont of an Indigofera sp. WSM1743 was isolated from a nodule recovered from the roots of an Indigofera sp. growing 20 km north of Carnarvon in Australia. It is slow growing, tolerates up to 1 % NaCl and is capable of growth at 37 degrees C. Here we describe the features of Bradyrhizobium sp. strain WSM1743, together with genome sequence information and its annotation. The 8,341,956 bp high-quality permanent draft genome is arranged into 163 scaffolds and 167 contigs, contains 7908 protein-coding genes and 75 RNA-only encoding genes and was sequenced as part of the Root Nodule Bacteria chapter of the Genomic Encyclopedia of Bacteria and Archaea project. C1 [Eshraghi, Leila; De Meyer, Sofie E.; Tian, Rui; Tiwari, Ravi; Howieson, John; Reeve, Wayne] Murdoch Univ, Ctr Rhizobium Studies, Murdoch, WA 6150, Australia. [Eshraghi, Leila] Murdoch Univ, CPSM, Murdoch, WA 6150, Australia. [Seshadri, Rekha; Ivanova, Natalia; Pati, Amrita; Woyke, Tanja; Kyrpides, Nikos C.] DOE Join Genome Inst, Walnut Creek, CA USA. [Markowitz, Victor] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Data Management & Technol Ctr, Berkeley, CA 94720 USA. [Kyrpides, Nikos C.] King Abdulaziz, Dept Biol Sci, Jeddah, Saudi Arabia. [Yates, Ron] Dept Agr & Food, S Perth, WA, Australia. RP Reeve, W (reprint author), Murdoch Univ, Ctr Rhizobium Studies, Murdoch, WA 6150, Australia. EM W.Reeve@murdoch.edu.au RI Kyrpides, Nikos/A-6305-2014; OI Kyrpides, Nikos/0000-0002-6131-0462; Ivanova, Natalia/0000-0002-5802-9485 FU US Department of Energy's Office of Science, Biological and Environmental Research Program; University of California, Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; University of California, Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; University of California, Los Alamos National Laboratory [DE-AC02-06NA25396] FX This work was performed under the auspices of the US Department of Energy's Office of Science, Biological and Environmental Research Program, and by the University of California, Lawrence Berkeley National Laboratory under contract No. DE-AC02-05CH11231, Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344, and Los Alamos National Laboratory under contract No. DE-AC02-06NA25396. NR 38 TC 0 Z9 0 U1 1 U2 2 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD OCT 26 PY 2015 VL 10 AR 87 DI 10.1186/s40793-015-0073-2 PG 7 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DA7QW UT WOS:000368000200004 PM 26512312 ER PT J AU Huntemann, M Ivanova, NN Mavromatis, K Tripp, HJ Paez-Espino, D Palaniappan, K Szeto, E Pillay, M Chen, IMA Pati, A Nielsen, T Markowitz, VM Kyrpides, NC AF Huntemann, Marcel Ivanova, Natalia N. Mavromatis, Konstantinos Tripp, H. James Paez-Espino, David Palaniappan, Krishnaveni Szeto, Ernest Pillay, Manoj Chen, I-Min A. Pati, Amrita Nielsen, Torben Markowitz, Victor M. Kyrpides, Nikos C. TI The standard operating procedure of the DOE-JGI Microbial Genome Annotation Pipeline (MGAP v.4) SO STANDARDS IN GENOMIC SCIENCES LA English DT Article DE Microbial Genome Annotation; SOP; IMG; JGI ID DATABASE; IDENTIFICATION; CLASSIFICATION; RECOGNITION; REPEATS; SYSTEM AB The DOE-JGI Microbial Genome Annotation Pipeline performs structural and functional annotation of microbial genomes that are further included into the Integrated Microbial Genome comparative analysis system. MGAP is applied to assembled nucleotide sequence datasets that are provided via the IMG submission site. Dataset submission for annotation first requires project and associated metadata description in GOLD. The MGAP sequence data processing consists of feature prediction including identification of protein-coding genes, non-coding RNAs and regulatory RNA features, as well as CRISPR elements. Structural annotation is followed by assignment of protein product names and functions. C1 [Huntemann, Marcel; Ivanova, Natalia N.; Mavromatis, Konstantinos; Tripp, H. James; Paez-Espino, David; Pati, Amrita; Nielsen, Torben; Kyrpides, Nikos C.] Joint Genome Inst, Dept Energy, Genome Biol Program, Walnut Creek, CA USA. [Palaniappan, Krishnaveni; Szeto, Ernest; Pillay, Manoj; Chen, I-Min A.; Markowitz, Victor M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Biosci Comp, Berkeley, CA 94720 USA. RP Huntemann, M (reprint author), Joint Genome Inst, Dept Energy, Genome Biol Program, 2800 Mitchell Dr, Walnut Creek, CA USA. EM mhuntemann@lbl.gov RI Kyrpides, Nikos/A-6305-2014; OI Kyrpides, Nikos/0000-0002-6131-0462; Ivanova, Natalia/0000-0002-5802-9485 FU Office of Science, Office of Biological and Environmental Research, Life Sciences Division, U.S. Department of Energy [DE-AC02-05CH11231] FX This work is funded by Director, Office of Science, Office of Biological and Environmental Research, Life Sciences Division, U.S. Department of Energy (Contract No. DE-AC02-05CH11231). NR 21 TC 21 Z9 22 U1 0 U2 0 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD OCT 26 PY 2015 VL 10 AR 86 DI 10.1186/s40793-015-0077-y PG 6 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DA7QW UT WOS:000368000200003 PM 26512311 ER PT J AU Chavez, DE Bottaro, JC Petrie, M Parrish, DA AF Chavez, David E. Bottaro, Jeffery C. Petrie, Mark Parrish, Damon A. TI Synthesis and Thermal Behavior of a Fused, Tricyclic 1,2,3,4-Tetrazine Ring System SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE 1,2,3,4-tetrazines; 1,2,4-triazoles; amination; oxidation; energetic materials ID ENERGETIC MATERIALS; DERIVATIVES AB This study presents the synthesis and characterization of a fused, tricyclic 1,2,3,4-tetrazine ring system. The molecule is synthesized in a three-step process from 5,5-dinitro-bis,1,2,4-triazole via a di-N-amino compound. Oxidation to form the azo-coupled fused tricyclic 1,2,3,4-tetrazine is achieved using tert-butyl hypochlorite as the oxidant. The di-N-amino compound and the desired fused tricyclic 1,2,3,4-triazine display interesting thermal behavior and are predicted to be high-performance energetic materials. C1 [Chavez, David E.] Los Alamos Natl Lab, M Div, Los Alamos, NM 87545 USA. [Bottaro, Jeffery C.; Petrie, Mark] SRI Int, Menlo Pk, CA 94025 USA. [Parrish, Damon A.] Naval Res Lab, Struct Matter Lab, Washington, DC 20375 USA. RP Chavez, DE (reprint author), Los Alamos Natl Lab, M Div, Los Alamos, NM 87545 USA. EM dechavez@lanl.gov FU Joint Munitions Technolgy Development Program; U.S. Department of Energy [DE-AC52-06A25396]; Office of Naval Research [N00014-11-AF-0-0002] FX We would like to thank Stephanie Hagelberg (elemental analysis) for characterization, Hongzhao Tian and Jose G. Archuleta, (sensitivity testing), and Mary Sandstrom (thermal analysis). We would also like to thank the Joint Munitions Technolgy Development Program for funding this work. Los Alamos National Laboratory is operated by Los Alamos National Security (LANS, LLC) under contract No. DE-AC52-06A25396 for the U.S. Department of Energy. The authors also thank the Office of Naval Research (award no. N00014-11-AF-0-0002) NR 23 TC 18 Z9 19 U1 6 U2 27 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD OCT 26 PY 2015 VL 54 IS 44 BP 12973 EP 12975 DI 10.1002/anie.201506744 PG 3 WC Chemistry, Multidisciplinary SC Chemistry GA CU3KM UT WOS:000363423900022 PM 26480332 ER PT J AU Beechem, TE Kowalski, BM Brumbach, MT McDonald, AE Spataru, CD Howell, SW Ohta, T Pask, JA Kalugin, NG AF Beechem, Thomas E. Kowalski, Brian M. Brumbach, Michael T. McDonald, Anthony E. Spataru, Catalin D. Howell, Stephen W. Ohta, Taisuke Pask, Jesse A. Kalugin, Nikolai G. TI Oxidation of ultrathin GaSe SO APPLIED PHYSICS LETTERS LA English DT Article ID EPITAXIAL GA2SE3 LAYERS; MOLECULAR-BEAM EPITAXY; AMORPHOUS SELENIUM; GALLIUM SELENIDE; RAMAN-SCATTERING; CRYSTALS; FILMS AB Oxidation of exfoliated gallium selenide (GaSe) is investigated through Raman, photoluminescence, Auger, and X-ray photoelectron spectroscopies. Photoluminescence and Raman intensity reductions associated with spectral features of GaSe are shown to coincide with the emergence of signatures emanating from the by-products of the oxidation reaction, namely, Ga2Se3 and amorphous Se. Photoinduced oxidation is initiated over a portion of a flake highlighting the potential for laser based patterning of two-dimensional heterostructures via selective oxidation. (C) 2015 AIP Publishing LLC. C1 [Beechem, Thomas E.; Brumbach, Michael T.; McDonald, Anthony E.; Howell, Stephen W.; Ohta, Taisuke] Sandia Natl Labs, Albuquerque, NM 87123 USA. [Kowalski, Brian M.; Pask, Jesse A.; Kalugin, Nikolai G.] New Mexico Inst Min & Technol, Dept Mat & Met Engn, Socorro, NM 87801 USA. [Spataru, Catalin D.] Sandia Natl Labs, Livermore, CA 94551 USA. RP Beechem, TE (reprint author), Sandia Natl Labs, Albuquerque, NM 87123 USA. EM tebeech@sandia.gov FU LDRD program at Sandia National Laboratories (SNL); U.S. DOE National Nuclear Security Administration [DE-AC04-94AL85000] FX Reid Hendricks is appreciated for aid in sample fabrication. Critical review of this work by Jon Ihlefeld of Sandia National Laboratories is greatly appreciated. This work was supported by the LDRD program at Sandia National Laboratories (SNL). Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. DOE National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 36 TC 5 Z9 5 U1 17 U2 50 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 26 PY 2015 VL 107 IS 17 AR 173103 DI 10.1063/1.4934592 PG 4 WC Physics, Applied SC Physics GA CV4JX UT WOS:000364234200038 ER PT J AU Chow, WW Liu, AY Gossard, AC Bowers, JE AF Chow, Weng W. Liu, Alan Y. Gossard, Arthur C. Bowers, John E. TI Extraction of inhomogeneous broadening and nonradiative losses in InAs quantum-dot lasers SO APPLIED PHYSICS LETTERS LA English DT Article ID WELL LASERS; GAIN; THRESHOLD; SPECTRA AB We present a method to quantify inhomogeneous broadening and nonradiative losses in quantum dot lasers by comparing the gain and spontaneous emission results of a microscopic laser theory with measurements made on 1.3 mu m InAs quantum-dot lasers. Calculated spontaneous-emission spectra are first matched to those measured experimentally to determine the inhomogeneous broadening in the experimental samples. This is possible because treatment of carrier scattering at the level of quantum kinetic equations provides the homogeneously broadened spectra without use of free parameters, such as the dephasing rate. We then extract the nonradiative recombination current associated with the quantum-dot active region from a comparison of measured and calculated gain versus current relations. (C) 2015 AIP Publishing LLC. C1 [Chow, Weng W.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Liu, Alan Y.; Gossard, Arthur C.; Bowers, John E.] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. [Gossard, Arthur C.; Bowers, John E.] Univ Calif Santa Barbara, Dept Elect & Comp Engn, Santa Barbara, CA 93106 USA. RP Chow, WW (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM wwchow@sandia.gov FU Sandia LDRD program - U.S. Department of Energy [DE-AC04-94AL85000]; SRC [2014-EP-2576] FX This work was supported by Sandia LDRD program, funded by the U.S. Department of Energy under Contract DE-AC04-94AL85000, and by SRC under Contract 2014-EP-2576. We thank Larry Coldren for helpful discussions. NR 18 TC 2 Z9 2 U1 2 U2 3 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 26 PY 2015 VL 107 IS 17 AR 171106 DI 10.1063/1.4934838 PG 5 WC Physics, Applied SC Physics GA CV4JX UT WOS:000364234200006 ER PT J AU Carter, TJ Wilson, RE AF Carter, Tyler J. Wilson, Richard E. TI Coordination Chemistry of Homoleptic Actinide(IV)-Thiocyanate Complexes SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE actinoids; coordination chemistry; plutonium; thiocyanates ID F-BLOCK COMPLEXES; THIOCYANATE COMPLEXES; STABILITY-CONSTANTS; TRIVALENT ACTINIDES; CRYSTAL-STRUCTURES; MOLECULAR-STRUCTURES; CHLORIDE COMPLEXES; AQUEOUS-SOLUTION; IONIC LIQUIDS; AQUA ION AB The synthesis, X-ray crystal structure, vibrational and optical spectroscopy for the eight-coordinate thiocyanate compounds, [Et4N](4)[Pu-IV(NCS)(8)], [Et4N](4)[Th-IV(NCS)(8)], and [Et4N](4)[Ce-III(NCS)(7)(H2O)] are reported. Thiocyanate was found to rapidly reduce plutonium to Pu-III in acidic solutions (pH<1) in the presence of NCS-. The optical spectrum of [Et4N][SCN] containing Pu-III solution was indistinguishable from that of aquated Pu-III suggesting that inner-sphere complexation with [Et4N][SCN] does not occur in water. However, upon concentration, the homoleptic thiocyanate complex [Et4N](4)[Pu-IV(NCS)(8)] was crystallized when a large excess of [Et4N][NCS] was present. This compound, along with its U-IV analogue, maintains inner-sphere thiocyanate coordination in acetonitrile based on the observation of intense ligand-to-metal charge-transfer bands. Spectroscopic and crystallographic data do not support the interaction of the metal orbitals with the ligand system, but support an enhanced An(IV)-NCS interaction, as the Lewis acidity of the metal ion increases from Th to Pu. C1 [Carter, Tyler J.; Wilson, Richard E.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Wilson, RE (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM rewilson@anl.gov RI Wilson, Richard/H-1763-2011 OI Wilson, Richard/0000-0001-8618-5680 FU United States Department of Energy [DE-AC02-06CH11357]; DOE Office of Basic Energy Sciences, Chemical Sciences, the Heavy Elements Program FX This work was performed at Argonne National Laboratory, operated by UChicagoArgonne LLC for the United States Department of Energy under Contract DE-AC02-06CH11357, and was supported by a DOE Office of Basic Energy Sciences, Chemical Sciences, the Heavy Elements Program. NR 85 TC 1 Z9 1 U1 6 U2 20 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD OCT 26 PY 2015 VL 21 IS 44 BP 15575 EP 15582 DI 10.1002/chem.201502770 PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA CU9SM UT WOS:000363885400021 PM 26493880 ER PT J AU Ginovska, B Autrey, T Parab, K Bowden, ME Potter, RG Camaioni, DM AF Ginovska, Bojana Autrey, Tom Parab, Kshitij Bowden, Mark E. Potter, Robert G. Camaioni, Donald M. TI Heterolysis of H-2 Across a Classical Lewis Pair, 2,6-LutidineBCl(3): Synthesis, Characterization, and Mechanism SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE boron; density functional calculations; frustrated Lewis pairs; hydrodechlorination; hydrogen activation ID ACTIVATION; REACTIVITY; BORANE; BORON AB We report that 2,6-lutidinetrichloroborane (LutBCl(3)) reacts with H-2 in toluene, bromobenzene, dichloromethane, and Lut solvents producing the neutral hydride, LutBHCl(2). The mechanism was modeled with density functional theory, and energies of stationary states were calculated at the G3(MP2)B3 level of theory. LutBCl(3) was calculated to react with H-2 and form the ion pair, [LutH(+)][HBCl3-], with a barrier of H=24.7kcalmol(-1) (G=29.8kcalmol(-1)). Metathesis with a second molecule of LutBCl(3) produced LutBHCl(2) and [LutH(+)][BCl4-]. The overall reaction is exothermic by 6.0kcalmol(-1) ((r)G degrees=-1.1). Alternate pathways were explored involving the borenium cation (LutBCl(2)(+)) and the four-membered boracycle [(CH2{NC5H3Me})BCl2]. Barriers for addition of H-2 across the Lut/LutBCl(2)(+) pair and the boracycle BC bond are substantially higher (G=42.1 and 49.4kcalmol(-1), respectively), such that these pathways are excluded. The barrier for addition of H-2 to the boracycle BN bond is comparable (H=28.5 and G=32kcalmol(-1)). Conversion of the intermediate 2-(BHCl2CH2)-6-Me(C5H3NH) to LutBHCl(2) may occur by intermolecular steps involving proton/hydride transfers to Lut/BCl3. Intramolecular protodeboronation, which could form LutBHCl(2) directly, is prohibited by a high barrier (H=52, G=51kcalmol(-1)). C1 [Ginovska, Bojana; Autrey, Tom; Parab, Kshitij; Bowden, Mark E.; Potter, Robert G.; Camaioni, Donald M.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99354 USA. RP Camaioni, DM (reprint author), Pacific NW Natl Lab, Div Phys Sci, POB 999, Richland, WA 99354 USA. EM donald.camaioni@pnnl.gov FU U.S. Department of Energy's (DOE) Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences, and Geosciences; Department of Energy's Office of Biological and Environmental Research FX We thank Dr. Adrian Houghton for helpful discussions and for providing 1H and 13C NMR spectra of Lut center dot BCl3. We thank a reviewer for suggesting the possibility of adding H2 to the borocycle B-N bond. This work was supported by the U.S. Department of Energy's (DOE) Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences, and Geosciences, and was performed in part using the Molecular Science Computing Facilities in the William R. Wiley Environmental Molecular Sciences Laboratory, a DOE National scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at the Pacific Northwest National Laboratory (PNNL). PNNL is operated by Battelle for DOE. NR 29 TC 1 Z9 1 U1 3 U2 11 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD OCT 26 PY 2015 VL 21 IS 44 BP 15713 EP 15719 DI 10.1002/chem.201501899 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA CU9SM UT WOS:000363885400035 PM 26493883 ER PT J AU Inskeep, WP Jay, ZJ Macur, RE Clingenpeel, S Tenney, A Lovalvo, D Beam, JP Kozubal, MA Shanks, WC Morgan, LA Kan, JJ Gorby, Y Yooseph, SB Nealson, K AF Inskeep, William P. Jay, Zackary J. Macur, Richard E. Clingenpeel, Scott Tenney, Aaron Lovalvo, David Beam, Jacob P. Kozubal, Mark A. Shanks, W. C. Morgan, Lisa A. Kan, Jinjun Gorby, Yuri Yooseph, Shibu Nealson, Kenneth TI Geomicrobiology of sublacustrine thermal vents in Yellowstone Lake: geochemical controls on microbial community structure and function SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE metagenome; Aquificales; Archaea; hydrogen; sulfide; methane; thermophiles; methanotrophs ID SULFUR-OXIDIZING BACTERIUM; NATIONAL-PARK; SP-NOV.; GEOTHERMAL SPRINGS; GEN. NOV.; HOT-SPRINGS; SULFURIHYDROGENIBIUM-AZORENSE; HYDROTHERMAL SYSTEMS; METAGENOME SEQUENCE; ACID CYCLE AB Yellowstone Lake (Yellowstone National Park, WY, USA) is a large high-altitude (2200 m), fresh water lake, which straddles an extensive caldera and is the center of significant geothermal activity. The primary goal of this interdisciplinary study was to evaluate the microbial populations inhabiting thermal vent communities in Yellowstone Lake using 16S rRNA gene and random metagenome sequencing, and to determine how geochemical attributes of vent waters influence the distribution of specific microorganisms and their metabolic potential. Thermal vent waters and associated microbial biomass were sampled during two field seasons (2007-2008) using a remotely operated vehicle (ROV). Sublacustrine thermal vent waters (circa 50-90 degrees C) contained elevated concentrations of numerous constituents associated with geothermal activity including dissolved hydrogen, sulfide, methane and carbon dioxide. Microorganisms associated with sulfur-rich filamentous "streamer" communities of Inflated Plain and West Thumb (pH range 5-6) were dominated by bacteria from the Aquificales, but also contained thermophilic archaea from the Crenarchaeota and Euryarchaeota. Novel groups of methanogens and members of the Korarchaeota were observed in vents from West Thumb and Elliot's Crater (pH 5-6). Conversely, metagenome sequence from Mary Bay vent sediments did not yield large assemblies, and contained diverse thermophilic and nonthermophilic bacterial relatives. Analysis of functional genes associated with the major vent populations indicated a direct linkage to high concentrations of carbon dioxide, reduced sulfur (sulfide and/or elemental S), hydrogen and methane in the deep thermal ecosystems. Our observations show that sublacustrine thermal vents in Yellowstone Lake support novel thermophilic communities, which contain microorganisms with functional attributes not found to date in terrestrial geothermal systems of YNP. C1 [Inskeep, William P.] Montana State Univ, Thermal Biol Inst, Bozeman, MT 59717 USA. [Inskeep, William P.; Jay, Zackary J.; Beam, Jacob P.; Kozubal, Mark A.] Montana State Univ, Land Resources & Environm Sci, Bozeman, MT 59717 USA. [Macur, Richard E.] Montana State Univ, Ctr Biofilm Engn, Bozeman, MT 59717 USA. [Clingenpeel, Scott] DOE Joint Genome Inst, Walnut Creek, CA USA. [Tenney, Aaron; Yooseph, Shibu] J Craig Venter Inst, La Jolla, CA USA. [Lovalvo, David] Eastern Ocean, West Redding, CT USA. [Shanks, W. C.; Morgan, Lisa A.] US Geol Survey, Denver, CO 80225 USA. [Kan, Jinjun; Gorby, Yuri; Nealson, Kenneth] Univ So Calif, Dept Earth Sci, Los Angeles, CA USA. RP Inskeep, WP (reprint author), Montana State Univ, Thermal Biol Inst, Bozeman, MT 59717 USA. EM binskeep@montana.edu FU Gordon and Betty Moore Foundation [1555]; Yellowstone Park Foundation (Bozeman, MT); NSF Integrated Graduate and Education Training Program in Geobiological Systems [0654336]; Center for Resources; Montana Agricultural Experiment Station [911300] FX Authors appreciate collaboration with Dr. Tim McDermott (MSU) and project support (2007-2008) from the Gordon and Betty Moore Foundation (Grant No. 1555), the Yellowstone Park Foundation (Bozeman, MT), the NSF Integrated Graduate and Education Training Program in Geobiological Systems (Ph.D. stipend support for ZJJ and JPB; NSF IGERT 0654336), the Center for Resources (Yellowstone National Park, National Park Service) for permitting and access to facilities necessary to conduct this study, and the Montana Agricultural Experiment Station (Project 911300) for salary support to WPI and REM. NR 64 TC 3 Z9 3 U1 10 U2 39 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD OCT 26 PY 2015 VL 6 AR 1044 DI 10.3389/fmicb.2015.01044 PG 16 WC Microbiology SC Microbiology GA CV3KA UT WOS:000364156900001 PM 26579074 ER PT J AU Kim, Y Kostow, N Demburg, AF AF Kim, Yumi Kostow, Nora Demburg, Abby F. TI The Chromosome Axis Mediates Feedback Control of CHK-2 to Ensure Crossover Formation in C. elegans SO DEVELOPMENTAL CELL LA English DT Article ID SPINDLE ASSEMBLY CHECKPOINT; CAENORHABDITIS-ELEGANS; MEIOTIC PROPHASE; INTERHOMOLOG RECOMBINATION; HOMOLOG ALIGNMENT; CHIASMA FORMATION; CROSSING-OVER; HORMA DOMAIN; DNA-REPAIR; MEIOSIS AB CHK-2 kinase is a master regulator of meiosis in C. elegans. Its activity is required for homolog pairing and synapsis and for double-strand break formation, but how it drives and coordinates these pathways to ensure crossover formation remains unknown. Here we show that CHK-2 promotes pairing and synapsis by phosphorylating a family of zinc finger proteins that bind to specialized regions on each chromosome known as pairing centers, priming their recruitment of the Polo-like kinase PLK-2. This knowledge enabled the development of a phospho-specific antibody as a tool to monitor CHK-2 activity. When either synapsis or crossover formation is impaired, CHK-2 activity is prolonged, and meiotic progression is delayed. We show that this common feedback circuit is mediated by interactions among a network of HORMA domain proteins within the chromosome axis and generates a graded signal. These findings reveal conserved regulatory mechanisms that ensure faithful meiotic chromosome segregation in diverse species. C1 [Kim, Yumi; Kostow, Nora; Demburg, Abby F.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Kim, Yumi; Kostow, Nora; Demburg, Abby F.] Howard Hughes Med Inst, Chevy Chase, MD 20815 USA. [Demburg, Abby F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Dept Genome Dynam, Berkeley, CA 94720 USA. [Demburg, Abby F.] Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. RP Demburg, AF (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. EM afdernburg@berkeley.edu FU NIH [S10RR025622]; NIH Office of Research Infrastructure Programs [P40 OD010440]; Damon Runyon Cancer Research Foundation [DRG 2084-11]; National Institute of Health [GM065591]; Howard Hughes Medical Institute FX We thank Ann Fischer for assistance with Sf9 cell culture. Mass spectrometry was performed by Lori Kohlstaedt in the Proteomics/Mass Spectrometry Laboratory at UC Berkeley, supported in part by NIH S10 Instrumentation Grant S10RR025622. Some strains were provided by the CGC, which is funded by the NIH Office of Research Infrastructure Programs (P40 OD010440). This work was supported by funding from the Damon Runyon Cancer Research Foundation (DRG 2084-11, to Y.K.) and the National Institute of Health (GM065591) and the Howard Hughes Medical Institute (to A.F.D.). NR 61 TC 4 Z9 4 U1 1 U2 2 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 1534-5807 EI 1878-1551 J9 DEV CELL JI Dev. Cell PD OCT 26 PY 2015 VL 35 IS 2 BP 247 EP 261 DI 10.1016/j.devcel.2015.09.021 PG 15 WC Cell Biology; Developmental Biology SC Cell Biology; Developmental Biology GA CU9MJ UT WOS:000363868300011 PM 26506311 ER PT J AU Melnyk, RA Coates, JD AF Melnyk, Ryan A. Coates, John D. TI The Perchlorate Reduction Genomic Island: Mechanisms and Pathways of Evolution by Horizontal Gene Transfer SO BMC GENOMICS LA English DT Article ID PHYLOGENETIC ANALYSIS; CHLORITE DISMUTASE; BACTERIA; IDENTIFICATION; METABOLISM; DIVERSITY; SELECTION; PROTEIN; ENZYME; MODELS AB Background: Perchlorate is a widely distributed anion that is toxic to humans, but serves as a valuable electron acceptor for several lineages of bacteria. The ability to utilize perchlorate is conferred by a horizontally transferred piece of DNA called the perchlorate reduction genomic island (PRI). Methods: We compared genomes of perchlorate reducers using phylogenomics, SNP mapping, and differences in genomic architecture to interrogate the evolutionary history of perchlorate respiration. Results: Here we report on the PRI of 13 genomes of perchlorate-reducing bacteria from four different classes of Phylum Proteobacteria (the Alpha-, Beta-, Gamma- and Epsilonproteobacteria). Among the different phylogenetic classes, the island varies considerably in genetic content as well as in its putative mechanism and location of integration. However, the islands of the densely sampled genera Azospira and Magnetospirillum have striking nucleotide identity despite divergent genomes, implying horizontal transfer and positive selection within narrow phylogenetic taxa. We also assess the phylogenetic origin of accessory genes in the various incarnations of the island, which can be traced to chromosomal paralogs from phylogenetically similar organisms. Conclusion: These observations suggest a complex phylogenetic history where the island is rarely transferred at the class level but undergoes frequent and continuous transfer within narrow phylogenetic groups. This restricted transfer is seen directly by the independent integration of near-identical islands within a genus and indirectly due to the acquisition of lineage-specific accessory genes. The genomic reversibility of perchlorate reduction may present a unique equilibrium for a metabolism that confers a competitive advantage only in the presence of an electron acceptor, which although widely distributed, is generally present at low concentrations in nature. C1 [Melnyk, Ryan A.; Coates, John D.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Melnyk, Ryan A.; Coates, John D.] Univ Calif Berkeley, Energy Biosci Inst, Berkeley, CA 94720 USA. [Melnyk, Ryan A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Coates, JD (reprint author), Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. EM jdcoates@berkeley.edu FU Energy Biosciences Institute; NIH [S10RR029668, S10RR027303] FX Funding for perchlorate research in the lab of J.D.C. comes from the Energy Biosciences Institute. This work used the Vincent J. Coates Genomic Sequencing Laboratory at UC Berkeley, supported by NIH S10 Instrumentation Grants S10RR029668 and S10RR027303. The majority of the computational work described here was carried out using the UC Berkeley Computational Genomics Resource Laboratory under the direction of Ravi Alla, who we would like to acknowledge. We would like to thank Iain Clark for invaluable discussions on computational genomics and sharing his incredibly useful python gene plotting script, among other tools. Finally, the rest of the Coates Lab must be acknowledged for many discussions about perchlorate reduction, from the level of pure culture genetics to evolutionary ecology. NR 47 TC 2 Z9 2 U1 4 U2 13 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2164 J9 BMC GENOMICS JI BMC Genomics PD OCT 26 PY 2015 VL 16 AR 862 DI 10.1186/s12864-015-2011-5 PG 11 WC Biotechnology & Applied Microbiology; Genetics & Heredity SC Biotechnology & Applied Microbiology; Genetics & Heredity GA CU2UM UT WOS:000363379100002 PM 26502901 ER PT J AU Baek, SH Utz, Y Hucker, M Gu, GD Buchner, B Grafe, HJ AF Baek, S-H Utz, Y. Huecker, M. Gu, G. D. Buechner, B. Grafe, H-J TI Magnetic field induced anisotropy of La-139 spin-lattice relaxation rates in stripe ordered La1.875Ba0.125CuO4 SO PHYSICAL REVIEW B LA English DT Article ID TEMPERATURE TETRAGONAL PHASE; SUPERCONDUCTIVITY; LA2-XSRXCUO4; DYNAMICS; LA2-XBAXCUO4; RESONANCE; CUPRATE AB We report La-139 nuclear magnetic resonance studies performed on a La1.875Ba0.125CuO4 single crystal. The data show that the structural phase transitions (high-temperature tetragonal -> low-temperature orthorhombic -> low-temperature tetragonal phase) are of the displacive type in this material. The La-139 spin-lattice relaxation rate T-1(-1) sharply upturns at the charge-ordering temperature T-CO = 54 K, indicating that charge order triggers the slowing down of spin fluctuations. Detailed temperature and field dependencies of the T-1(-1) below the spin-ordering temperature T-SO = 40 K reveal the development of enhanced spin fluctuations in the spin-ordered state for H parallel to [001], which are completely suppressed for large fields along the CuO2 planes. Our results shed light on the unusual spin fluctuations in the charge and spin stripe ordered lanthanum cuprates. C1 [Baek, S-H; Utz, Y.; Buechner, B.; Grafe, H-J] IFW Dresden, Inst Solid State Res, D-01171 Dresden, Germany. [Utz, Y.; Buechner, B.] Tech Univ Dresden, Inst Festkorperphys, D-01062 Dresden, Germany. [Huecker, M.; Gu, G. D.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Baek, SH (reprint author), IFW Dresden, Inst Solid State Res, PF 270116, D-01171 Dresden, Germany. EM sbaek.fu@gmail.com RI Baek, Seung-Ho/F-4733-2011; Buchner, Bernd/E-2437-2016 OI Baek, Seung-Ho/0000-0002-0059-8255; Buchner, Bernd/0000-0002-3886-2680 FU DFG [BA 4927/1-1]; Office of Science, U.S. Department of Energy [DE-AC02-98CH10886] FX This work has been supported by the DFG Research Grant No. BA 4927/1-1. M.H. acknowledges support by the Office of Science, U.S. Department of Energy under Contract No. DE-AC02-98CH10886. NR 42 TC 2 Z9 2 U1 1 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 26 PY 2015 VL 92 IS 15 AR 155144 DI 10.1103/PhysRevB.92.155144 PG 6 WC Physics, Condensed Matter SC Physics GA CU4PT UT WOS:000363512700004 ER PT J AU Wrzesinski, J Lane, GJ Maier, KH Janssens, RVF Dracoulis, GD Broda, R Byrne, AP Carpenter, MP Clark, RM Cromaz, M Fornal, B Lauritsen, T Macchiavelli, AO Rejmund, M Szpak, B Vetter, K Zhu, S AF Wrzesinski, J. Lane, G. J. Maier, K. H. Janssens, R. V. F. Dracoulis, G. D. Broda, R. Byrne, A. P. Carpenter, M. P. Clark, R. M. Cromaz, M. Fornal, B. Lauritsen, T. Macchiavelli, A. O. Rejmund, M. Szpak, B. Vetter, K. Zhu, S. TI High-spin yrast structure of Hg-204 from the decay of a four-hole, 22(+) isomer SO PHYSICAL REVIEW C LA English DT Article ID PO-212; STATE; PB-208; PO212 AB A high-spin isomer with tau > 700 ns has been found in Hg-204, populated in reactions of 1360-MeV Pb-208 and 330-MeV Ca-48 beams with a thick U-238 target and a 1450-MeV Pb-208 beam on a thick Pb-208 target. The observed gamma-ray decay of the isomer has established the yrast states below it, including another isomer with tau = 33(3) ns. The experimental results are compared with shell-model calculations that include four holes in the configuration space between Sn-132 and Pb-208. The available spectroscopic information, including transition strengths, total conversion, and angular correlation coefficients, together with the observed agreement with the calculations, allows spin, parity, and configuration assignments to be proposed for the experimental states. The tau > 700 ns isomer is the 22(+) state of maximum spin available from the alignment of the four valence holes with the configuration pi h(11/2)(-2)nu i(13/2)(-2). C1 [Wrzesinski, J.; Maier, K. H.; Broda, R.; Fornal, B.; Szpak, B.] PAN, Niedwodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. [Lane, G. J.; Maier, K. H.; Dracoulis, G. D.; Byrne, A. P.] Australian Natl Univ, Res Sch Phys Sci & Engn, Dept Nucl Phys, Canberra, ACT 0200, Australia. [Janssens, R. V. F.; Carpenter, M. P.; Lauritsen, T.; Zhu, S.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Clark, R. M.; Cromaz, M.; Macchiavelli, A. O.; Vetter, K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Rejmund, M.] GANIL, F-14076 Caen 5, France. RP Wrzesinski, J (reprint author), PAN, Niedwodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. RI Carpenter, Michael/E-4287-2015; Lane, Gregory/A-7570-2011 OI Carpenter, Michael/0000-0002-3237-5734; Lane, Gregory/0000-0003-2244-182X FU Australian Research Council [FT100100991]; United States Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357, DE-AC0205CH11231] FX This work is supported by Australian Research Council (Grant No. FT100100991) and the United States Department of Energy, Office of Science, Office of Nuclear Physics, under Contracts No. DE-AC02-06CH11357 and No. DE-AC0205CH11231. This research used resources of ANL's ATLAS facility, which is a DOE Office of Science User Facility. NR 23 TC 0 Z9 0 U1 1 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 26 PY 2015 VL 92 IS 4 AR 044327 DI 10.1103/PhysRevC.92.044327 PG 11 WC Physics, Nuclear SC Physics GA CU4UD UT WOS:000363524900004 ER PT J AU Briceno, RA Hansen, MT AF Briceno, Raul A. Hansen, Maxwell T. TI Multichannel 0 -> 2 and 1 -> 2 transition amplitudes for arbitrary spin particles in a finite volume SO PHYSICAL REVIEW D LA English DT Article ID LATTICE QCD; MATRIX-ELEMENTS; PHASE-SHIFTS; STATES; DECAYS AB We present a model-independent, nonperturbative relation between finite-volume matrix elements and infinite-volume 0 -> 2 and 1 -> 2 transition amplitudes. Our result accommodates theories in which the final two-particle state is coupled to any number of other two-body channels, with all angular momentum states included. The derivation uses generic, fully relativistic field theory and is exact up to exponentially suppressed corrections in the lightest particle mass times the box size. This work distinguishes itself from previous studies by accommodating particles with any intrinsic spin. To illustrate the utility of our general result, we discuss how it can be implemented for studies of N + J -> (N pi, N eta, N eta', Sigma K, Lambda K) transitions, where J is a generic external current. The reduction of rotational symmetry, due to the cubic finite volume, manifests in this example through the mixing of S and P waves when the system has nonzero total momentum. C1 [Briceno, Raul A.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Hansen, Maxwell T.] Johannes Gutenberg Univ Mainz, Inst Kernphys, D-55099 Mainz, Germany. [Hansen, Maxwell T.] Johannes Gutenberg Univ Mainz, Helmholz Inst Mainz, D-55099 Mainz, Germany. RP Briceno, RA (reprint author), Thomas Jefferson Natl Accelerator Facil, 12000 Jefferson Ave, Newport News, VA 23606 USA. EM rbriceno@jlab.org; hansen@kph.uni-mainz.de FU U.S. Department of Energy [DE-AC05-06OR23177] FX R. B. acknowledges support from the U.S. Department of Energy Contract No. DE-AC05-06OR23177, under which Jefferson Science Associates, LLC, manages and operates the Jefferson Lab. The authors would like to acknowledge and thank Jozef Dudek, Robert Edwards, Stefan Meinel, Stephen Sharpe, Christian Shultz, Christopher Thomas, Andre Walker-Loud and David Wilson for useful discussion. NR 57 TC 13 Z9 13 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 26 PY 2015 VL 92 IS 7 AR 074509 DI 10.1103/PhysRevD.92.074509 PG 21 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CU4UU UT WOS:000363526700010 ER PT J AU Huschle, M Kuhr, T Heck, M Goldenzweig, P Abdesselam, A Adachi, I Adamczyk, K Aihara, H Al Said, S Arinstein, K Asner, DM Aushev, T Ayad, R Aziz, T Badhrees, I Bakich, AM Bansal, V Barberio, E Bhardwaj, V Bhuyan, B Biswal, J Bobrov, A Bozek, A Bracko, M Browder, TE Cervenkov, D Chang, P Chekelian, V Chen, A Cheon, BG Chilikin, K Chistov, R Cho, K Chobanova, V Choi, Y Cinabro, D Dalseno, J Danilov, M Dolezal, Z Drasal, Z Dutta, D Eidelman, S Epifanov, D Farhat, H Fast, JE Ferber, T Frey, A Fulsom, BG Gaur, V Gabyshev, N Garmash, A Gillard, R Glattauer, R Goh, YM Golob, B Grygier, J Hamer, P Hara, K Hara, T Hasenbusch, J Hayasaka, K Hayashii, H He, XH Heider, M Heller, A Horiguchi, T Hou, WS Hsu, CL Iijima, T Inami, K Inguglia, G Ishikawa, A Itoh, R Iwasaki, Y Jaegle, I Joffe, D Joo, KK Julius, T Kang, KH Kato, E Katrenko, P Kawasaki, T Keck, T Kiesling, C Kim, DY Kim, HJ Kim, JB Kim, JH Kim, KT Kim, MJ Kim, SH Kim, YJ Kinoshita, K Ko, BR Kobayashi, N Kodys, P Korpar, S Krizan, P Krokovny, P Kumita, T Kuzmin, A Kwon, YJ Lee, IS Li, C Li, Y Gioi, LL Libby, J Liventsev, D Lukin, P Masuda, M Matvienko, D Miyabayashi, K Miyake, H Miyata, H Mizuk, R Mohanty, GB Mohanty, S Moll, A Moon, HK Mussa, R Nakamura, KR Nakano, E Nakao, M Nanut, T Nayak, M Nisar, NK Nishida, S Ogawa, S Okuno, S Oswald, C Pakhlova, G Pal, B Park, CW Park, H Pedlar, TK Pesantez, L Pestotnik, R Petric, M Piilonen, LE Pulvermacher, C Ribezl, E Ritter, M Rostomyan, A Sakai, Y Sandilya, S Santelj, L Sanuki, T Sato, Y Savinov, V Schneider, O Schnell, G Schwanda, C Schwartz, AJ Semmler, D Senyo, K Seon, O Sevior, ME Shebalin, V Shen, CP Shibata, TA Shiu, JG Simon, F Sohn, YS Sokolov, A Solovieva, E Stanic, S Staric, M Steder, M Stypula, J Sumihama, M Sumiyoshi, T Tamponi, U Teramoto, Y Trabelsi, K Trusov, V Uchida, M Uglov, T Uno, S Usov, Y Van Hulse, C Vanhoefer, P Varner, G Vinokurova, A Vorobyev, V Wagner, MN Wang, CH Wang, MZ Wang, P Wang, XL Watanabe, M Watanabe, Y Won, E Yamamoto, H Yamaoka, J Yashchenko, S Ye, H Yook, Y Yuan, CZ Yusa, Y Zhang, ZP Zhilich, V Zhulanov, V Zupanc, A AF Huschle, M. Kuhr, T. Heck, M. Goldenzweig, P. Abdesselam, A. Adachi, I. Adamczyk, K. Aihara, H. Al Said, S. Arinstein, K. Asner, D. M. Aushev, T. Ayad, R. Aziz, T. Badhrees, I. Bakich, A. M. Bansal, V. Barberio, E. Bhardwaj, V. Bhuyan, B. Biswal, J. Bobrov, A. Bozek, A. Bracko, M. Browder, T. E. Cervenkov, D. Chang, P. Chekelian, V. Chen, A. Cheon, B. G. Chilikin, K. Chistov, R. Cho, K. Chobanova, V. Choi, Y. Cinabro, D. Dalseno, J. Danilov, M. Dolezal, Z. Drasal, Z. Dutta, D. Eidelman, S. Epifanov, D. Farhat, H. Fast, J. E. Ferber, T. Frey, A. Fulsom, B. G. Gaur, V. Gabyshev, N. Garmash, A. Gillard, R. Glattauer, R. Goh, Y. M. Golob, B. Grygier, J. Hamer, P. Hara, K. Hara, T. Hasenbusch, J. Hayasaka, K. Hayashii, H. He, X. H. Heider, M. Heller, A. Horiguchi, T. Hou, W-S. Hsu, C-L. Iijima, T. Inami, K. Inguglia, G. Ishikawa, A. Itoh, R. Iwasaki, Y. Jaegle, I. Joffe, D. Joo, K. K. Julius, T. Kang, K. H. Kato, E. Katrenko, P. Kawasaki, T. Keck, T. Kiesling, C. Kim, D. Y. Kim, H. J. Kim, J. B. Kim, J. H. Kim, K. T. Kim, M. J. Kim, S. H. Kim, Y. J. Kinoshita, K. Ko, B. R. Kobayashi, N. Kodys, P. Korpar, S. Krizan, P. Krokovny, P. Kumita, T. Kuzmin, A. Kwon, Y-J. Lee, I. S. Li, C. Li, Y. Gioi, L. Li Libby, J. Liventsev, D. Lukin, P. Masuda, M. Matvienko, D. Miyabayashi, K. Miyake, H. Miyata, H. Mizuk, R. Mohanty, G. B. Mohanty, S. Moll, A. Moon, H. K. Mussa, R. Nakamura, K. R. Nakano, E. Nakao, M. Nanut, T. Nayak, M. Nisar, N. K. Nishida, S. Ogawa, S. Okuno, S. Oswald, C. Pakhlova, G. Pal, B. Park, C. W. Park, H. Pedlar, T. K. Pesantez, L. Pestotnik, R. Petric, M. Piilonen, L. E. Pulvermacher, C. Ribezl, E. Ritter, M. Rostomyan, A. Sakai, Y. Sandilya, S. Santelj, L. Sanuki, T. Sato, Y. Savinov, V. Schneider, O. Schnell, G. Schwanda, C. Schwartz, A. J. Semmler, D. Senyo, K. Seon, O. Sevior, M. E. Shebalin, V. Shen, C. P. Shibata, T-A. Shiu, J-G. Simon, F. Sohn, Y. -S. Sokolov, A. Solovieva, E. Stanic, S. Staric, M. Steder, M. Stypula, J. Sumihama, M. Sumiyoshi, T. Tamponi, U. Teramoto, Y. Trabelsi, K. Trusov, V. Uchida, M. Uglov, T. Uno, S. Usov, Y. Van Hulse, C. Vanhoefer, P. Varner, G. Vinokurova, A. Vorobyev, V. Wagner, M. N. Wang, C. H. Wang, M-Z. Wang, P. Wang, X. L. Watanabe, M. Watanabe, Y. Won, E. Yamamoto, H. Yamaoka, J. Yashchenko, S. Ye, H. Yook, Y. Yuan, C. Z. Yusa, Y. Zhang, Z. P. Zhilich, V. Zhulanov, V. Zupanc, A. CA Belle Collaboration TI Measurement of the branching ratio of (B)over-bar -> D-(*())tau(-)(nu)over-bar(tau) relative to (B)over-bar -> D(*)l(-)(nu)over-bar(l) decays with hadronic tagging at Belle SO PHYSICAL REVIEW D LA English DT Article ID MESON DECAYS; B-DECAYS; DETECTOR; QCD AB We report a measurement of the branching fraction ratios R(D)(()*()) of (B) over bar -> D-(*())tau(-)(nu) over bar (tau) relative to (B) over bar -> D-(*())l(-)(nu) over barl (where l = e or mu) using the full Belle data sample of 772 x 10(6)B (B) over bar pairs collected at the Upsilon(4S) resonance with the Belle detector at the KEKB asymmetric-energy e(+)e(-) collider. The measured values are R(D) = 0.375 +/- 0.064(stat) +/- 0.026(syst) and R(D*) = 0.293 +/- 0.038 (stat) +/- 0.015 (syst). The analysis uses hadronic reconstruction of the tag-side B meson and purely leptonic t decays. The results are consistent with earlier measurements and do not show a significant deviation from the standard model prediction. C1 [Schnell, G.; Van Hulse, C.] Univ Basque Country UPV EHU, Bilbao 48080, Spain. [Shen, C. P.] Beihang Univ, Beijing 100191, Peoples R China. [Hasenbusch, J.; Oswald, C.; Pesantez, L.] Univ Bonn, D-53115 Bonn, Germany. [Arinstein, K.; Bobrov, A.; Eidelman, S.; Gabyshev, N.; Garmash, A.; Krokovny, P.; Kuzmin, A.; Lukin, P.; Matvienko, D.; Shebalin, V.; Usov, Y.; Vinokurova, A.; Vorobyev, V.; Zhilich, V.; Zhulanov, V.] Budker Inst Nucl Phys SB RAS, Novosibirsk 630090, Russia. [Cervenkov, D.; Dolezal, Z.; Drasal, Z.; Kodys, P.] Charles Univ Prague, Fac Math & Phys, CR-12116 Prague, Czech Republic. [Joo, K. K.] Chonnam Natl Univ, Kwangju 660701, South Korea. [Kinoshita, K.; Pal, B.; Schwartz, A. J.] Univ Cincinnati, Cincinnati, OH 45221 USA. [Ferber, T.; Inguglia, G.; Rostomyan, A.; Steder, M.; Yashchenko, S.; Ye, H.] DESY, D-22607 Hamburg, Germany. [Semmler, D.; Wagner, M. N.] Univ Giessen, D-35392 Giessen, Germany. [Sumihama, M.] Gifu Univ, Gifu 5011193, Japan. [Frey, A.; Hamer, P.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Adachi, I.; Hara, T.; Itoh, R.; Miyake, H.; Nakao, M.; Nishida, S.; Sakai, Y.; Trabelsi, K.; Uno, S.] SOKENDAI Grad Univ Adv Studies, Hayama 2400193, Japan. [Cheon, B. G.; Goh, Y. M.; Kim, S. H.; Lee, I. S.] Hanyang Univ, Seoul 133791, South Korea. [Browder, T. E.; Jaegle, I.; Varner, G.] Univ Hawaii, Honolulu, HI 96822 USA. [Adachi, I.; Hara, K.; Hara, T.; Itoh, R.; Iwasaki, Y.; Liventsev, D.; Miyake, H.; Nakamura, K. R.; Nakao, M.; Nishida, S.; Sakai, Y.; Santelj, L.; Trabelsi, K.; Uno, S.] High Energy Accelerator Res Org KEK, Tsukuba, Ibaraki 3050801, Japan. [Schnell, G.] Basque Fdn Sci, IKERBASQUE, Bilbao 48013, Spain. [Bhuyan, B.] Indian Inst Technol Guwahati, Gauhati 781039, Assam, India. [Libby, J.; Nayak, M.] Indian Inst Technol, Madras 600036, Tamil Nadu, India. [Wang, P.; Yuan, C. Z.] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Glattauer, R.; Schwanda, C.] Inst High Energy Phys, A-1050 Vienna, Austria. [Sokolov, A.] Inst High Energy Phys, Protvino 142281, Russia. [Mussa, R.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Aushev, T.; Chilikin, K.; Chistov, R.; Danilov, M.; Katrenko, P.; Mizuk, R.; Pakhlova, G.; Solovieva, E.; Uglov, T.] Inst Theoret & Expt Phys, Moscow 117218, Russia. [Biswal, J.; Bracko, M.; Golob, B.; Korpar, S.; Krizan, P.; Nanut, T.; Pestotnik, R.; Petric, M.; Ribezl, E.; Staric, M.; Zupanc, A.] Jozef Stefan Inst, Ljubljana 1000, Slovenia. [Okuno, S.; Watanabe, Y.] Kanagawa Univ, Yokohama, Kanagawa 2218686, Japan. [Huschle, M.; Heck, M.; Goldenzweig, P.; Grygier, J.; Heider, M.; Heller, A.; Keck, T.; Pulvermacher, C.; Trusov, V.] Karlsruher Inst Technol, Inst Expt Kernphys, D-76131 Karlsruhe, Germany. [Joffe, D.] Kennesaw State Univ, Kennesaw, GA 30144 USA. [Badhrees, I.] King Abdulaziz City Sci & Technol, Riyadh 11442, Saudi Arabia. [Al Said, S.] King Abdulaziz Univ, Dept Phys, Fac Sci, Jeddah 21589, Saudi Arabia. [Cho, K.; Kim, J. H.; Kim, Y. J.] Korea Inst Sci & Technol Informat, Daejeon 305806, South Korea. [Kim, J. B.; Kim, K. T.; Ko, B. R.; Moon, H. K.; Won, E.] Korea Univ, Seoul 136713, South Korea. [Kang, K. H.; Kim, H. J.; Kim, M. J.; Park, H.] Kyungpook Natl Univ, Daegu 702701, South Korea. [Schneider, O.] Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland. [Golob, B.; Krizan, P.] Univ Ljubljana, Fac Math & Phys, Ljubljana 1000, Slovenia. [Kuhr, T.] Univ Munich, D-80539 Munich, Germany. [Pedlar, T. K.] Luther Coll, Decorah, IA 52101 USA. [Bracko, M.; Korpar, S.] Univ Maribor, SLO-2000 Maribor, Slovenia. [Chekelian, V.; Chobanova, V.; Dalseno, J.; Kiesling, C.; Gioi, L. Li; Moll, A.; Ritter, M.; Simon, F.; Vanhoefer, P.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Barberio, E.; Hsu, C-L.; Julius, T.; Li, C.; Sevior, M. E.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Danilov, M.; Mizuk, R.] Moscow Phys Engn Inst, Moscow 115409, Russia. [Aushev, T.; Pakhlova, G.; Uglov, T.] Moscow Inst Phys & Technol, Dolgoprudnyi 141700, Moscow Region, Russia. [Iijima, T.; Inami, K.; Sato, Y.; Seon, O.] Nagoya Univ, Sch Sci, Nagoya, Aichi 4648602, Japan. [Hayasaka, K.; Iijima, T.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648602, Japan. [Hayashii, H.; Miyabayashi, K.] Nara Womens Univ, Nara 6308506, Japan. [Chen, A.] Natl Cent Univ, Chungli 32054, Taiwan. [Wang, C. H.] Natl United Univ, Miaoli 36003, Taiwan. [Chang, P.; Hou, W-S.; Shiu, J-G.; Wang, M-Z.] Natl Taiwan Univ, Dept Phys, Taipei 10617, Taiwan. [Adamczyk, K.; Bozek, A.; Stypula, J.] H Niewodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. [Kawasaki, T.; Miyata, H.; Watanabe, M.; Yusa, Y.] Niigata Univ, Niigata 9502181, Japan. [Stanic, S.] Univ Nova Gorica, Nova Gorica 5000, Slovenia. [Arinstein, K.; Bobrov, A.; Eidelman, S.; Gabyshev, N.; Garmash, A.; Krokovny, P.; Kuzmin, A.; Lukin, P.; Matvienko, D.; Shebalin, V.; Usov, Y.; Vinokurova, A.; Vorobyev, V.; Zhilich, V.; Zhulanov, V.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Nakano, E.; Teramoto, Y.] Osaka City Univ, Osaka 5588585, Japan. [Asner, D. M.; Bansal, V.; Fast, J. E.; Fulsom, B. G.; Yamaoka, J.] Pacific NW Natl Lab, Richland, WA 99352 USA. [He, X. H.] Peking Univ, Beijing 100871, Peoples R China. [Savinov, V.] Univ Pittsburgh, Pittsburgh, PA 15260 USA. [Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Kim, D. Y.] Soongsil Univ, Seoul 156743, South Korea. [Bhardwaj, V.] Univ S Carolina, Columbia, SC 29208 USA. [Choi, Y.; Park, C. W.] Sungkyunkwan Univ, Suwon 440746, South Korea. [Bakich, A. M.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdesselam, A.; Al Said, S.; Ayad, R.; Badhrees, I.] Univ Tabuk, Dept Phys, Fac Sci, Tabuk 71451, Saudi Arabia. [Aziz, T.; Dutta, D.; Gaur, V.; Mohanty, G. B.; Mohanty, S.; Nisar, N. K.; Sandilya, S.] Tata Inst Fundamental Res, Bombay 400005, Maharashtra, India. [Dalseno, J.; Moll, A.; Simon, F.] Tech Univ Munich, Excellence Cluster Universe, D-85748 Garching, Germany. [Ogawa, S.] Toho Univ, Funabashi, Chiba 2748510, Japan. [Horiguchi, T.; Ishikawa, A.; Kato, E.; Sanuki, T.; Yamamoto, H.] Tohoku Univ, Sendai, Miyagi 9808578, Japan. [Masuda, M.] Univ Tokyo, Earthquake Res Inst, Tokyo 1130032, Japan. [Aihara, H.; Epifanov, D.] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Kobayashi, N.; Shibata, T-A.; Uchida, M.] Tokyo Inst Technol, Tokyo 1528550, Japan. [Kumita, T.; Sumiyoshi, T.] Tokyo Metropolitan Univ, Tokyo 1920397, Japan. [Tamponi, U.] Univ Turin, I-10124 Turin, Italy. [Mohanty, S.] Utkal Univ, Bhubaneswar 751004, Orissa, India. [Li, Y.; Liventsev, D.; Piilonen, L. E.; Wang, X. L.] Virginia Polytech Inst & State Univ, CNP, Blacksburg, VA 24061 USA. [Cinabro, D.; Farhat, H.; Gillard, R.] Wayne State Univ, Detroit, MI 48202 USA. [Senyo, K.] Yamagata Univ, Yamagata 9908560, Japan. [Kwon, Y-J.; Sohn, Y. -S.; Yook, Y.] Yonsei Univ, Seoul 120749, South Korea. RP Huschle, M (reprint author), Karlsruher Inst Technol, Inst Expt Kernphys, D-76131 Karlsruhe, Germany. RI Solovieva, Elena/B-2449-2014; Aihara, Hiroaki/F-3854-2010; Pakhlova, Galina/C-5378-2014; Uglov, Timofey/B-2406-2014; Danilov, Mikhail/C-5380-2014; Mizuk, Roman/B-3751-2014; Krokovny, Pavel/G-4421-2016; Katrenko, Petr/D-1229-2016; Chilikin, Kirill/B-4402-2014; EPFL, Physics/O-6514-2016; Chistov, Ruslan/B-4893-2014; Cervenkov, Daniel/D-2884-2017 OI Solovieva, Elena/0000-0002-5735-4059; Aihara, Hiroaki/0000-0002-1907-5964; Pakhlova, Galina/0000-0001-7518-3022; Uglov, Timofey/0000-0002-4944-1830; Danilov, Mikhail/0000-0001-9227-5164; Krokovny, Pavel/0000-0002-1236-4667; Katrenko, Petr/0000-0002-8808-1786; Chilikin, Kirill/0000-0001-7620-2053; Chistov, Ruslan/0000-0003-1439-8390; Cervenkov, Daniel/0000-0002-1865-741X FU Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan; Japan Society for the Promotion of Science (JSPS); Tau-Lepton Physics Research Center of Nagoya University; Australian Research Council; Australian Department of Industry, Innovation, Science and Research; Austrian Science Fund [P 22742-N16, P 26794-N20]; National Natural Science Foundation of China [10575109, 10775142, 10875115, 11175187, 11475187]; Ministry of Education, Youth and Sports of the Czech Republic [LG14034]; Carl Zeiss Foundation; Deutsche Forschungsgemeinschaft; Volkswagen Stiftung; Department of Science and Technology of India; Istituto Nazionale di Fisica Nucleare of Italy; National Research Foundation (NRF) of Korea [2011-0029457, 2012-0008143, 2012R1A1A2008330, 2013R1A1A3007772, 2014R1A2A2A01005286, 2014R1A2A2A01002734, 2014R1A1A2006456]; Basic Research Lab program under NRF [KRF-2011-0020333, KRF-2011-0021196]; Center for Korean J-PARC Users [NRF-2013K1A3A7A06056592]; Brain Korea 21-Plus program; Global Science Experimental Data Hub Center of the Korea Institute of Science and Technology Information; Polish Ministry of Science and Higher Education and the National Science Center; Ministry of Education and Science of the Russian Federation; Russian Foundation for Basic Research; Slovenian Research Agency; Basque Foundation for Science (IKERBASQUE); Euskal Herriko Unibertsitatea (UPV/EHU) (Spain) [UFI 11/55]; Swiss National Science Foundation; National Science Council; Ministry of Education of Taiwan; U.S. Department of Energy; National Science Foundation; MEXT for Science Research in a Priority Area (New Development of Flavor Physics); JSPS for Creative Scientific Research (Evolution of Tau-lepton Physics) FX We thank the KEKB group for the excellent operation of the accelerator; the KEK cryogenics group for the efficient operation of the solenoid; and the KEK computer group, the National Institute of Informatics, and the PNNL/EMSL computing group for valuable computing and SINET4 network support. We acknowledge support from the Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan, the Japan Society for the Promotion of Science (JSPS), and the Tau-Lepton Physics Research Center of Nagoya University; the Australian Research Council and the Australian Department of Industry, Innovation, Science and Research; Austrian Science Fund under Grants No. P 22742-N16 and No. P 26794-N20; the National Natural Science Foundation of China under Contracts No. 10575109, No. 10775142, No. 10875115, No. 11175187, and No. 11475187; the Ministry of Education, Youth and Sports of the Czech Republic under Contract No. LG14034; the Carl Zeiss Foundation, the Deutsche Forschungsgemeinschaft and the Volkswagen Stiftung; the Department of Science and Technology of India; the Istituto Nazionale di Fisica Nucleare of Italy; National Research Foundation (NRF) of Korea Grants No. 2011-0029457, No. 2012-0008143, No. 2012R1A1A2008330, No. 2013R1A1A3007772, No. 2014R1A2A2A01005286, No. 2014R1A2A2A01002734, and No. 2014R1A1A2006456; the Basic Research Lab program under NRF Grants No. KRF-2011-0020333 and No. KRF-2011-0021196, Center for Korean J-PARC Users, No. NRF-2013K1A3A7A06056592; the Brain Korea 21-Plus program and the Global Science Experimental Data Hub Center of the Korea Institute of Science and Technology Information; the Polish Ministry of Science and Higher Education and the National Science Center; the Ministry of Education and Science of the Russian Federation and the Russian Foundation for Basic Research; the Slovenian Research Agency; the Basque Foundation for Science (IKERBASQUE) and the Euskal Herriko Unibertsitatea (UPV/EHU) under program UFI 11/55 (Spain); the Swiss National Science Foundation; the National Science Council and the Ministry of Education of Taiwan; and the U.S. Department of Energy and the National Science Foundation. This work is supported by a Grant-in-Aid from MEXT for Science Research in a Priority Area (New Development of Flavor Physics) and from JSPS for Creative Scientific Research (Evolution of Tau-lepton Physics). NR 35 TC 74 Z9 74 U1 2 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD OCT 26 PY 2015 VL 92 IS 7 AR 072014 DI 10.1103/PhysRevD.92.072014 PG 14 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CU4UU UT WOS:000363526700003 ER PT J AU Mkhitaryan, VV Jelezko, F Dobrovitski, VV AF Mkhitaryan, V. V. Jelezko, F. Dobrovitski, V. V. TI Highly selective detection of individual nuclear spins with rotary echo on an electron spin probe SO SCIENTIFIC REPORTS LA English DT Article ID NITROGEN-VACANCY CENTERS; MAGNETIC-RESONANCE; SINGLE SPINS; DIAMOND; MAGNETOMETRY; REGISTER; READOUT; SILICON; QUBITS; SENSOR AB We consider an electronic spin, such as a nitrogen-vacancy center in diamond, weakly coupled to a large number of nuclear spins, and subjected to the Rabi driving with a periodically alternating phase. We show that by switching the driving phase synchronously with the precession of a given nuclear spin, the interaction to this spin is selectively enhanced, while the rest of the bath remains decoupled. The enhancement is of resonant character. The key feature of the suggested scheme is that the width of the resonance is adjustable, and can be greatly decreased by increasing the driving strength. Thus, the resonance can be significantly narrowed, by a factor of 10-100 in comparison with the existing detection methods. Significant improvement in selectivity is explained analytically and confirmed by direct numerical many-spin simulations. The method can be applied to a wide range of solid-state systems. C1 [Mkhitaryan, V. V.; Dobrovitski, V. V.] US DOE, Ames Lab, Ames, IA 50011 USA. [Jelezko, F.] Univ Ulm, Inst Quantum Opt, D-89081 Ulm, Germany. [Jelezko, F.] Univ Ulm, Ctr Integrated Quantum Sci & Technol, D-89081 Ulm, Germany. RP Dobrovitski, VV (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. EM slava@ameslab.gov FU Department of Energy-Basic Energy Sciences [DE-AC02-07CH11358] FX We thank R. Hanson, T. H. Taminiau, M. Raikh, and H. Terletska for helpful and important discussions. This work was supported by the Department of Energy-Basic Energy Sciences under Contract No. DE-AC02-07CH11358. NR 35 TC 4 Z9 4 U1 4 U2 19 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 26 PY 2015 VL 5 AR 15402 DI 10.1038/srep15402 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CU3AA UT WOS:000363394300001 PM 26497777 ER PT J AU Zhao, X Wu, SQ Lv, XB Nguyen, MC Wang, CZ Lin, ZJ Zhu, ZZ Ho, KM AF Zhao, Xin Wu, Shunqing Lv, Xiaobao Nguyen, Manh Cuong Wang, Cai-Zhuang Lin, Zijing Zhu, Zi-Zhong Ho, Kai-Ming TI Exploration of tetrahedral structures in silicate cathodes using a motif-network scheme SO SCIENTIFIC REPORTS LA English DT Article ID LITHIUM-ION BATTERIES; TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; ELECTROCHEMICAL PERFORMANCE; CRYSTAL-STRUCTURE; LI2FESIO4 POLYMORPHS; POSITIVE ELECTRODE; LI2MNSIO4; 1ST-PRINCIPLES; ENERGETICS AB Using a motif-network search scheme, we studied the tetrahedral structures of the dilithium/disodium transition metal orthosilicates A(2)MSiO(4) with A = Li or Na and M = Mn, Fe or Co. In addition to finding all previously reported structures, we discovered many other different tetrahedral-network-based crystal structures which are highly degenerate in energy. These structures can be classified into structures with 1D, 2D and 3D M-Si-O frameworks. A clear trend of the structural preference in different systems was revealed and possible indicators that affect the structure stabilities were introduced. For the case of Na systems which have been much less investigated in the literature relative to the Li systems, we predicted their ground state structures and found evidence for the existence of new structural motifs. C1 [Zhao, Xin; Ho, Kai-Ming] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Wu, Shunqing; Zhu, Zi-Zhong] Xiamen Univ, Dept Phys, Xiamen 361005, Peoples R China. [Lv, Xiaobao; Lin, Zijing] Univ Sci & Technol China, Dept Phys, Hefei 230026, Peoples R China. [Lv, Xiaobao; Lin, Zijing] Univ Sci & Technol China, Collaborat Innovat Ctr Suzhou Nano Sci & Technol, Hefei 230026, Peoples R China. [Nguyen, Manh Cuong; Wang, Cai-Zhuang] US DOE, Ames Lab, Ames, IA 50011 USA. [Ho, Kai-Ming] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Int Ctr Quantum Design Funct Mat ICQD, Hefei 230026, Peoples R China. RP Zhao, X (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. EM xzhao@iastate.edu; wsq@xmu.edu.cn RI Nguyen, Manh Cuong/G-2783-2015; Wu, S.Q./G-3992-2010; OI Nguyen, Manh Cuong/0000-0001-8027-9029; Wu, S.Q./0000-0002-2545-0054; Zhao, Xin/0000-0002-3580-512X FU National Natural Science Foundation of China [21233004, 11004165, 11374272]; Natural Science Foundation of Fujian Province of China [2015J01030]; Fundamental Research Funds for the Central Universities [20720150034]; National Basic Research Program of China (973 program) [2011CB935903]; State Key Development Program for Basic Research of China [2012CB215405]; US Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering [DE-AC02-07CH11358] FX S.Q.W. and Z.Z.Z. acknowledge the financial support from the National Natural Science Foundation of China under grant Nos. 21233004 and 11004165, the Natural Science Foundation of Fujian Province of China (Grant No. 2015J01030), the Fundamental Research Funds for the Central Universities (Grant No. 20720150034) and the National Basic Research Program of China (973 program, Grant No. 2011CB935903). Z.J.L. and X.L. acknowledge the support by the State Key Development Program for Basic Research of China (Grant No. 2012CB215405) and the National Natural Science Foundation of China (Grant No. 11374272). Work at Ames Laboratory was supported by the US Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering, under Contract No. DE-AC02-07CH11358, including a grant of computer time at the National Energy Research Scientific Computing Center (NERSC) in Berkeley, CA. NR 38 TC 4 Z9 4 U1 12 U2 57 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 26 PY 2015 VL 5 AR 15555 DI 10.1038/srep15555 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CU3AX UT WOS:000363396800001 PM 26497381 ER PT J AU Jain, R Poyraz, AS Gamliel, DP Valla, J Suib, SL Maric, R AF Jain, Rishabh Poyraz, Altug S. Gamliel, David P. Valla, Julia Suib, Steven L. Maric, Radenka TI Comparative study for low temperature water-gas shift reaction on Pt/ceria catalysts: Role of different ceria supports SO APPLIED CATALYSIS A-GENERAL LA English DT Article DE Water-gas shift reaction; Flame spray pyrolysis; Pt-ceria interface; Mesoporous ceria; Processing-structure-property relationship ID SPRAY DEPOSITION TECHNOLOGY; FISCHER-TROPSCH SYNTHESIS; FUEL PROCESSING CATALYSTS; CO OXIDATION; DOPED CERIA; MESOPOROUS CERIA; COPRECIPITATION METHOD; ELECTRICAL-PROPERTIES; HYDROGEN-PRODUCTION; RAMAN-SPECTROSCOPY AB Pt on ceria catalysts for water-gas shift (WGS) reaction were prepared by employing three ceria nanopowders synthesized with different processing techniques and having different surface area and porosities. Nano-Pt (similar to 0.5-2 nm) was deposited in the vapor phase onto each of the three ceria supports by Reactive Spray Deposition Technology (RSDT). The catalysts were performance tested for the WGS reaction in the temperature range of 150-450 degrees C at a gas hourly space velocity (GHSV) of 13,360 h(-1). The structure-activity relationship for the ceria-based materials was studied. The most promising catalyst was Pt supported on mesoporous ceria with crystallite size of 5.8 nm and Brunauer-Emmett-Teller (BET) surface area of 187 m(2)/g. This configuration demonstrated complete CO conversion at 225 degrees C. The CO adsorption strength and the ability to dissociate H2O are the two main factors that determine the activity of a particular catalyst site for the water-gas shift (WGS) reaction. This study leads to the,conclusion that the highest water-gas shift reaction activity was obtained on Pt supported on the mesoporous ceria with low crystallite size and high surface area, with well dispersed Pt, leading to enhanced Pt-ceria interaction. (C) 2015 Elsevier B.V. All rights reserved. C1 [Jain, Rishabh; Maric, Radenka] Univ Connecticut, Dept Mat Sci & Engn, Storrs, CT 06269 USA. [Jain, Rishabh; Suib, Steven L.] Univ Connecticut, Inst Mat Sci, Storrs, CT 06269 USA. [Jain, Rishabh; Gamliel, David P.; Valla, Julia; Maric, Radenka] Univ Connecticut, Ctr Clean Energy Engn, Storrs, CT 06269 USA. [Poyraz, Altug S.; Suib, Steven L.] Univ Connecticut, Dept Chem, Storrs, CT 06269 USA. [Poyraz, Altug S.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Gamliel, David P.; Valla, Julia; Maric, Radenka] Univ Connecticut, Dept Chem & Biomol Engn, Storrs, CT 06269 USA. RP Jain, R (reprint author), Univ Connecticut, Dept Mat Sci & Engn, 44 Weaver Rd, Storrs, CT 06269 USA. EM rishabh.jain@uconn.edu OI Jain, Rishabh/0000-0003-0842-1099 FU National Science Foundation [CMMI-1265893]; US Department of Energy, Basic Energy Sciences, Division of Chemical, Geological and Biological Science [DE-FG02-86ER13622.A000]; General Electric (GE) graduate fellowship FX Authors would like to acknowledge financial support from National Science Foundation (award number CMMI-1265893) and US Department of Energy, Basic Energy Sciences, Division of Chemical, Geological and Biological Science (grant DE-FG02-86ER13622.A000). We would also like to acknowledge Dr. George Bollas for providing us access to the in-situ FTIR-DRIFTS equipment. The creative discussion with Mr. Leonard Bonville is highly appreciated. David Kriz is acknowledged for performing the SAXS measurements. R.J. acknowledges the 2015 General Electric (GE) graduate fellowship. NR 103 TC 5 Z9 5 U1 10 U2 54 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0926-860X EI 1873-3875 J9 APPL CATAL A-GEN JI Appl. Catal. A-Gen. PD OCT 25 PY 2015 VL 507 BP 1 EP 13 DI 10.1016/j.apcata.2015.09.041 PG 13 WC Chemistry, Physical; Environmental Sciences SC Chemistry; Environmental Sciences & Ecology GA CV9LL UT WOS:000364608600001 ER PT J AU Allen, AJ Espinal, L Wong-Ng, W Queen, WL Brown, CM Kline, SR Kauffman, KL Culp, JT Matranga, C AF Allen, A. J. Espinal, L. Wong-Ng, W. Queen, W. L. Brown, C. M. Kline, S. R. Kauffman, K. L. Culp, J. T. Matranga, C. TI Flexible metal-organic framework compounds: In situ studies for selective CO2 capture SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE Composite materials; Nanostructured materials; Gas-solid reactions; Microstructure; Phase transitions; Neutron diffraction ID CARBON-DIOXIDE CAPTURE; POROUS COORDINATION POLYMERS; ANGLE NEUTRON-SCATTERING; ADVANCED PHOTON SOURCE; X-RAY-SCATTERING; STRUCTURAL TRANSITIONS; CRYSTAL-STRUCTURE; MOLECULAR-SIEVE; GAS-ADSORPTION; NICKEL(II) DIBENZOYLMETHANATE AB Results are presented that explore the dynamic structural changes occurring in two highly flexible nanocrystalline metal-organic framework (MOF) compounds during the adsorption and desorption of pure gases and binary mixtures. The Ni(1,2-bis(4-pyridyl) ethylene)[Ni(CN)(4)] and catena-bis(dibenzoylmethanato)-(4,4'-bipyridyl) nickel(II) chosen for this study are 3-D and 1-D porous coordination polymers (PCP) with a similar gate opening pressure response for CO2 isotherms at 303 K, but with differing degrees of flexibility for structural change to accommodate guest molecules. As such, they serve as a potential model system for evaluating the complex kinetics associated with dynamic structure changes occurring in response to gas adsorption in flexible MOF systems. Insights into the crystallo-graphic changes occurring as the MOF pore structure expands and contracts in response to interactions with CO2, N-2, and CO2/N-2 mixtures have been obtained from in situ small-angle neutron scattering and neutron diffraction, combined with ex situ X-ray diffraction structure measurements. The role of structure in carbon capture functionality is discussed with reference to the ongoing characterization challenges and a possible materials-by-design approach. Published by Elsevier B.V. C1 [Allen, A. J.; Espinal, L.; Wong-Ng, W.] NIST, Mat Measurement Lab, Gaithersburg, MD 20899 USA. [Queen, W. L.; Brown, C. M.; Kline, S. R.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Queen, W. L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Brown, C. M.] Univ Delaware, Dept Chem & Biomol Engn, Newark, DE 19716 USA. [Kauffman, K. L.; Culp, J. T.; Matranga, C.] US DOE, NETL, Pittsburgh, PA 15236 USA. [Culp, J. T.] URS Corp, South Pk, PA 15219 USA. RP Allen, AJ (reprint author), NIST, Mat Measurement Lab, Gaithersburg, MD 20899 USA. EM andrew.allen@nist.gov RI Brown, Craig/B-5430-2009; Foundry, Molecular/G-9968-2014; OI Brown, Craig/0000-0002-9637-9355; Allen, Andrew/0000-0002-6496-8411 FU National Science Foundation [DMR-0944772]; U.S. DOE [DE-AC02-06CH11357]; National Science Foundation/Department of Energy [NSF/CHE-0822838]; National Energy Technology Laboratory's ongoing research in CO2 capture under the RES [DE-FE0004000] FX The authors thank Juscelino Leao of the NIST Center for Neutron Research and Martin Green of NIST Materials Measurement Science Division for valuable discussions. This work utilized neutron scattering facilities supported in part by the National Science Foundation under Agreement No. DMR-0944772. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. ChemMatCARS Sector 15 is principally supported by the National Science Foundation/Department of Energy under grant number NSF/CHE-0822838. Part of this work was performed in support of the National Energy Technology Laboratory's ongoing research in CO2 capture under the RES contract DE-FE0004000. Supporting Information available online from Elsevier. NR 91 TC 4 Z9 4 U1 6 U2 99 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 EI 1873-4669 J9 J ALLOY COMPD JI J. Alloy. Compd. PD OCT 25 PY 2015 VL 647 BP 24 EP 34 DI 10.1016/j.jallcom.2015.05.148 PG 11 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA CR2JU UT WOS:000361156400005 ER PT J AU Wu, Z Parish, CM Bei, H AF Wu, Z. Parish, C. M. Bei, H. TI Nano-twin mediated plasticity in carbon-containing FeNiCoCrMn high entropy alloys SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE High entropy alloy; Solid solution strengthening; Mechanical properties; Nano-twinning ID STACKING-FAULT ENERGY; AUSTENITIC STAINLESS-STEEL; SOLID-SOLUTION ALLOYS; MECHANICAL-PROPERTIES; PHASE-STABILITY; MICROSTRUCTURAL EVOLUTION; MULTICOMPONENT ALLOYS; TENSILE PROPERTIES; GRAIN-ORIENTATION; DEFORMATION TWINS AB Equiatomic FeNiCoCrMn alloy has been reported to exhibit promising strength and ductility at cryogenic temperature and deformation mediated by nano-twining appeared to be one of the main reasons. We use the FeNiCoCrMn alloy as a base alloy to seek further improvement of its mechanical properties by alloying additional elements, i.e., interstitial carbon. The effects of carbon on microstructures, mechanical properties and twinning activities were investigated in two different temperatures (77 and 293 K). With addition of 0.5 at% C, the high entropy alloy still remains entirely single phase face-centered cubic (FCC) crystal structure. The materials can be cold rolled and recrystallized to produce a microstructure with equiaxed grains. Both strain hardening rate and strength are enhanced while high uniform elongations to fracture (similar to 70% at 77 K and similar to 40% at 293 K) are still maintained. The increased strain hardening and strength could be caused by the promptness of deformation twinning in C-containing high entropy alloys. (C) 2015 Elsevier B.V. All rights reserved. C1 [Wu, Z.; Parish, C. M.; Bei, H.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Wu, Z.] Univ Tennessee, Mat Sci & Engn Dept, Knoxville, TN 37996 USA. RP Bei, H (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM beih@ornl.gov RI Parish, Chad/J-8381-2013; OI Bei, Hongbin/0000-0003-0283-7990 FU US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division FX This work was supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 50 TC 19 Z9 19 U1 14 U2 56 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 EI 1873-4669 J9 J ALLOY COMPD JI J. Alloy. Compd. PD OCT 25 PY 2015 VL 647 BP 815 EP 822 DI 10.1016/j.jallcom.2015.05.224 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA CR2JU UT WOS:000361156400114 ER PT J AU Shi, HL Du, MH Singh, DJ AF Shi, Hongliang Du, Mao-Hua Singh, David J. TI Li2Se:Te as a neutron scintillator SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE Li2Se; Neutron scintillator; Density functional theory; Dopants; Defects ID AUGMENTED-WAVE METHOD; 1ST-PRINCIPLES; SPECTROSCOPY; DETECTOR; DEFECTS; ALLOYS; ZNSE AB We show that Li2Se:Te is a potential neutron scintillator material based on density functional calculations. Li2Se exhibits a number of properties favorable for efficient neutron detection, such as a high Li concentration for neutron absorption, a small effective atomic mass and a low density for reduced sensitivity to background gamma rays, and a small band gap for a high light yield. Our calculations show that Te doping should lead to the formation of deep acceptor complex V-Li-Te-Se, which can facilitate efficient light emission, similar to the emission activation in Te doped ZnSe. (C) 2015 The Authors. Published by Elsevier B.V. C1 [Du, Mao-Hua] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. Oak Ridge Natl Lab, Ctr Radiat Detect Mat & Syst, Oak Ridge, TN 37831 USA. RP Du, MH (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM mhdu@ornl.gov RI Shi, Hongliang/A-7568-2010; Du, Mao-Hua/B-2108-2010 OI Shi, Hongliang/0000-0003-0713-4688; Du, Mao-Hua/0000-0001-8796-167X FU ORNL LDRD fund; Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division FX Initial electronic structure calculations with the modified Becke-Johnson potential were supported by the ORNL LDRD fund. The remainder of the work including optical and defect calculations was supported by the Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 34 TC 1 Z9 1 U1 3 U2 13 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 EI 1873-4669 J9 J ALLOY COMPD JI J. Alloy. Compd. PD OCT 25 PY 2015 VL 647 BP 906 EP 910 DI 10.1016/j.jallcom.2015.06.184 PG 5 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA CR2JU UT WOS:000361156400125 ER PT J AU Huang, L Cong, DY Ma, L Nie, ZH Wang, MG Wang, ZL Suo, HL Ren, Y Wang, YD AF Huang, L. Cong, D. Y. Ma, L. Nie, Z. H. Wang, M. G. Wang, Z. L. Suo, H. L. Ren, Y. Wang, Y. D. TI Large magnetic entropy change and magnetoresistance in a Ni41Co9Mn40Sn10 magnetic shape memory alloy SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE Magnetocaloric effect; Magnetoresistance; Magnetic shape memory alloy; Martensitic transformation; Synchrotron high-energy X-ray diffraction ID PHASE-TRANSFORMATION; TRANSITION AB A polycrystalline Ni41Co9Mn40Sn10 (at. %) magnetic shape memory alloy was prepared by arc melting and characterized mainly by magnetic measurements, in-situ high-energy X-ray diffraction (HEXRD), and mechanical testing. A large magnetoresistance of 53.8% (under 5 T) and a large magnetic entropy change of 31.9 J/(kg K) (under 5 T) were simultaneously achieved. Both of these values are among the highest values reported so far in Ni-Mn-Sn-based Heusler alloys. The large magnetic entropy change, closely related to the structural entropy change, is attributed to the large unit cell volume change across martensitic transformation as revealed by our in-situ HEXRD experiment. Furthermore, good compressive properties were also obtained. The combination of large magnetoresistance, large magnetic entropy change, and good compressive properties, as well as low cost makes this alloy a promising candidate for multifunctional applications. (C) 2015 Elsevier B.V. All rights reserved. C1 [Huang, L.; Cong, D. Y.; Wang, Y. D.] Univ Sci & Technol Beijing, State Key Lab Adv Met & Mat, Beijing 100083, Peoples R China. [Huang, L.; Nie, Z. H.; Wang, Z. L.] Beijing Inst Technol, Sch Mat Sci & Engn, Beijing 100081, Peoples R China. [Ma, L.; Suo, H. L.] Beijing Univ Technol, Coll Mat Sci & Engn, Beijing 100124, Peoples R China. [Wang, M. G.] Northeastern Univ, Coll Sci, Shenyang 110819, Peoples R China. [Ren, Y.] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Cong, DY (reprint author), Univ Sci & Technol Beijing, State Key Lab Adv Met & Mat, 30 Xueyuan Rd, Beijing 100083, Peoples R China. EM dycong@ustb.edu.cn; ydwang@ustb.edu.cn RI wang, yandong/G-9404-2013; Nie, Zhihua/G-9459-2013 OI Nie, Zhihua/0000-0002-2533-933X FU National Basic Research Program of China (973 Program) [2012CB619405]; National Natural Science Foundation of China [51471030, 11305008]; National 863 Program of China [2015AA034101]; Fundamental Research Funds for the Central Universities [06111023, 06111020]; NPL, CAEP [2013DB02]; State Key Laboratory for Advanced Metals and Materials [2014Z-01, 2014Z-02]; U.S. Department of Energy, Office of Science, Office of Basic Energy Science [DE-AC02-06CH11357] FX This work is supported by the National Basic Research Program of China (973 Program) under Contract No. 2012CB619405, the National Natural Science Foundation of China (Nos. 51471030 and 11305008), the National 863 Program of China (Grant No. 2015AA034101), the Fundamental Research Funds for the Central Universities (Nos. 06111023 and 06111020), the NPL, CAEP (Project No. 2013DB02), and the projects (Grant Nos. 2014Z-01 and 2014Z-02) from the State Key Laboratory for Advanced Metals and Materials. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Science, under Contract No. DE-AC02-06CH11357. NR 35 TC 4 Z9 4 U1 9 U2 61 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 EI 1873-4669 J9 J ALLOY COMPD JI J. Alloy. Compd. PD OCT 25 PY 2015 VL 647 BP 1081 EP 1085 DI 10.1016/j.jallcom.2015.06.175 PG 5 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA CR2JU UT WOS:000361156400151 ER PT J AU Afzal, W Liu, XY Prausnitz, JM AF Afzal, Waheed Liu, Xiangyang Prausnitz, John M. TI Physical data for a process to separate krypton from air by selective absorption in an ionic liquid SO FLUID PHASE EQUILIBRIA LA English DT Article DE Selectivity Kr/O-2; Mixture of ionic liquids; Separation; Absorption; Diluent ID SINGLE GASES METHANE; CARBON-DIOXIDE; BIS(2,4,4-TRIMETHYLPENTYL) PHOSPHINATE; PHOSPHONIUM CATION; NITROUS-OXIDE; SOLUBILITY; ETHANE; OXYGEN; O-2; N-2 AB Ionic liquids provide a possible absorption process to extract krypton from air. The feed for such a process is an oxygen stream from a liquid-air plant. An effective ionic liquid is [P(14)666][TMPP]; in that solvent, the solubilities of some pertinent common gases are appreciably larger than those in conventional ionic liquids, and the selectivity Kr/O-2 is close to 3. A nonvolatile ionic liquid is preferred over a hydrocarbon solvent because of safety and simpler solvent recovery. Because, the viscosity of [P(14)666][TMPP] is very high, 20 wt.% [BHMIM][AC] is added to reduce the viscosity by one order of magnitude without significantly reducing solvent capacity and selectivity. This work provides extensive fundamental data (solubility, density and viscosity) required for process design. (C) 2015 Elsevier B.V. All rights reserved. C1 [Afzal, Waheed; Liu, Xiangyang; Prausnitz, John M.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Afzal, Waheed; Prausnitz, John M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Liu, Xiangyang] Xi An Jiao Tong Univ, MOE Key Lab Thermofluid Sci & Engn, Xian 710049, Shaanxi, Peoples R China. [Afzal, Waheed] Univ Aberdeen, Sch Engn, Aberdeen, Scotland. RP Prausnitz, JM (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. EM prausnit@cchem.berkeley.edu OI Afzal, Waheed/0000-0002-2927-0114 FU U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Building Technology, Building Technologies Program of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The authors are grateful to Robert Hart, Dragan Curcija, Alexis Bell, Scott Lynn and co-workers for valuable advice, and to Maogang He for assistance in preparing the manuscript. NR 31 TC 1 Z9 1 U1 8 U2 21 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-3812 EI 1879-0224 J9 FLUID PHASE EQUILIBR JI Fluid Phase Equilib. PD OCT 25 PY 2015 VL 404 BP 124 EP 130 DI 10.1016/j.fluid.2015.06.037 PG 7 WC Thermodynamics; Chemistry, Physical; Engineering, Chemical SC Thermodynamics; Chemistry; Engineering GA CQ8NM UT WOS:000360865000017 ER PT J AU Bowers, RM Clum, A Tice, H Lim, J Singh, K Ciobanu, D Ngan, CY Cheng, JF Tringe, SG Woyke, T AF Bowers, Robert M. Clum, Alicia Tice, Hope Lim, Joanne Singh, Kanwar Ciobanu, Doina Ngan, Chew Yee Cheng, Jan-Fang Tringe, Susannah G. Woyke, Tanja TI Impact of library preparation protocols and template quantity on the metagenomic reconstruction of a mock microbial community SO BMC GENOMICS LA English DT Article DE Low input; Low biomass; Metagenome; Library preparation protocol; Microbiome ID SEQUENCING LIBRARIES; AMPLIFICATION; BIAS; ATMOSPHERE; DIVERSITY; ASSEMBLER; GENOMICS; VIRUSES; SAMPLES; DEEP AB Background: The rapid development of sequencing technologies has provided access to environments that were either once thought inhospitable to life altogether or that contain too few cells to be analyzed using genomics approaches. While 16S rRNA gene microbial community sequencing has revolutionized our understanding of community composition and diversity over time and space, it only provides a crude estimate of microbial functional and metabolic potential. Alternatively, shotgun metagenomics allows comprehensive sampling of all genetic material in an environment, without any underlying primer biases. Until recently, one of the major bottlenecks of shotgun metagenomics has been the requirement for large initial DNA template quantities during library preparation. Results: Here, we investigate the effects of varying template concentrations across three low biomass library preparation protocols on their ability to accurately reconstruct a mock microbial community of known composition. We analyze the effects of input DNA quantity and library preparation method on library insert size, GC content, community composition, assembly quality and metagenomic binning. We found that library preparation method and the amount of starting material had significant impacts on the mock community metagenomes. In particular, GC content shifted towards more GC rich sequences at the lower input quantities regardless of library prep method, the number of low quality reads that could not be mapped to the reference genomes increased with decreasing input quantities, and the different library preparation methods had an impact on overall metagenomic community composition. Conclusions: This benchmark study provides recommendations for library creation of representative and minimally biased metagenome shotgun sequencing, enabling insights into functional attributes of low biomass ecosystem microbial communities. C1 [Bowers, Robert M.; Clum, Alicia; Tice, Hope; Lim, Joanne; Singh, Kanwar; Ciobanu, Doina; Ngan, Chew Yee; Cheng, Jan-Fang; Tringe, Susannah G.; Woyke, Tanja] DOE Joint Genome Inst, Microbial Genom Program, Walnut Creek, CA 94598 USA. RP Woyke, T (reprint author), DOE Joint Genome Inst, Microbial Genom Program, 2800 Mitchell Dr, Walnut Creek, CA 94598 USA. EM twoyke@lbl.gov FU DOE Office of Science User Facility [DE-AC02-05CH11231] FX The work conducted by the U.S. Department of Energy Joint Genome Institute, a DOE Office of Science User Facility, is supported under Contract No. DE-AC02-05CH11231. We would like to thank the JGI production team, including Chia-Lin Wei, Shweta Deshpande and Chris Daum for the sequencing, and Christa Pennacchio, Tatyana Smirnova and Chris Beecroft for assistance with data deposition to the JGI Genome Portal. NR 39 TC 7 Z9 7 U1 6 U2 22 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2164 J9 BMC GENOMICS JI BMC Genomics PD OCT 24 PY 2015 VL 16 AR 856 DI 10.1186/s12864-015-2063-6 PG 12 WC Biotechnology & Applied Microbiology; Genetics & Heredity SC Biotechnology & Applied Microbiology; Genetics & Heredity GA CU2UK UT WOS:000363378900005 PM 26496746 ER PT J AU Bui-Nguyen, TM Baer, CE Lewis, JA Yang, DR Lein, PJ Jackson, DA AF Bui-Nguyen, Tri M. Baer, Christine E. Lewis, John A. Yang, Dongren Lein, Pamela J. Jackson, David A. TI Dichlorvos exposure results in large scale disruption of energy metabolism in the liver of the zebrafish, Danio rerio SO BMC GENOMICS LA English DT Article DE Zebrafish; Dichlorvos; Microarray; Organophosphorus; Fasting ID UNFOLDED PROTEIN RESPONSE; OXIDATIVE STRESS; GENE-EXPRESSION; ORGANOPHOSPHORUS PESTICIDE; CARBOHYDRATE-METABOLISM; ADAPTIVE RESPONSE; ACUTE TOXICITY; CELL-DEATH; L-MALATE; RAT AB Background: Exposure to dichlorvos (DDVP), an organophosphorus pesticide, is known to result in neurotoxicity as well as other metabolic perturbations. However, the molecular causes of DDVP toxicity are poorly understood, especially in cells other than neurons and muscle cells. To obtain a better understanding of the process of non-neuronal DDVP toxicity, we exposed zebrafish to different concentrations of DDVP, and investigated the resulting changes in liver histology and gene transcription. Results: Functional enrichment analysis of genes affected by DDVP exposure identified a number of processes involved in energy utilization and stress response in the liver. The abundance of transcripts for proteins involved in glucose metabolism was profoundly affected, suggesting that carbon flux might be diverted toward the pentose phosphate pathway to compensate for an elevated demand for energy and reducing equivalents for detoxification. Strikingly, many transcripts for molecules involved in beta-oxidation and fatty acid synthesis were down-regulated. We found increases in message levels for molecules involved in reactive oxygen species responses as well as ubiquitination, proteasomal degradation, and autophagy. To ensure that the effects of DDVP on energy metabolism were not simply a consequence of poor feeding because of neuromuscular impairment, we fasted fish for 29 or 50 h and analyzed liver gene expression in them. The patterns of gene expression for energy metabolism in fasted and DDVP-exposed fish were markedly different. Conclusion: We observed coordinated changes in the expression of a large number of genes involved in energy metabolism and responses to oxidative stress. These results argue that an appreciable part of the effect of DDVP is on energy metabolism and is regulated at the message level. Although we observed some evidence of neuromuscular impairment in exposed fish that may have resulted in reduced feeding, the alterations in gene expression in exposed fish cannot readily be explained by nutrient deprivation. C1 [Bui-Nguyen, Tri M.] ORISE, Ft Detrick, MD 21702 USA. [Baer, Christine E.] Excet Inc, Springfield, VA 22151 USA. [Lewis, John A.; Jackson, David A.] US Army Ctr Environm Hlth Res, Ft Detrick, MD 21702 USA. [Yang, Dongren; Lein, Pamela J.] Univ Calif Davis, Sch Vet Med, Mol Biosci, Davis, CA 95616 USA. RP Jackson, DA (reprint author), US Army Ctr Environm Hlth Res, Ft Detrick, MD 21702 USA. EM david.a.jackson17.civ@mail.mil FU National Institute of Environmental Health Sciences (NIEHS) [ES016308]; Military Operational Medicine Research Program of the US Army Medical Research and Materiel Command FX Research was supported by the National Institute of Environmental Health Sciences (NIEHS, grant #ES016308 to PJL) and the Military Operational Medicine Research Program of the US Army Medical Research and Materiel Command. NR 93 TC 2 Z9 2 U1 1 U2 17 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2164 J9 BMC GENOMICS JI BMC Genomics PD OCT 24 PY 2015 VL 16 AR 853 DI 10.1186/s12864-015-1941-2 PG 18 WC Biotechnology & Applied Microbiology; Genetics & Heredity SC Biotechnology & Applied Microbiology; Genetics & Heredity GA CU2UK UT WOS:000363378900002 PM 26499117 ER PT J AU Bagnaschi, EA Buchmueller, O Cavanaugh, R Citron, M De Roeck, A Dolan, MJ Ellis, JR Flacher, H Heinemeyer, S Isidori, G Malik, S Santos, DM Olive, KA Sakurai, K de Vries, KJ Weiglein, G AF Bagnaschi, E. A. Buchmueller, O. Cavanaugh, R. Citron, M. De Roeck, A. Dolan, M. J. Ellis, J. R. Flaecher, H. Heinemeyer, S. Isidori, G. Malik, S. Martinez Santos, D. Olive, K. A. Sakurai, K. de Vries, K. J. Weiglein, G. TI Supersymmetric dark matter after LHC run 1 SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID NONUNIVERSAL HIGGS MASSES; NEUTRALINO RELIC DENSITY; MINIMAL SUPERGRAVITY; STOP COANNIHILATION; STAU COANNIHILATION; BENCHMARK SCENARIOS; YUKAWA UNIFICATION; PARAMETER SPACE; BOSON SEARCHES; MSSM AB Different mechanisms operate in various regions of the MSSM parameter space to bring the relic density of the lightest neutralino, (chi) over bar (0)(1), assumed here to be the lightest SUSY particle (LSP) and thus the dark matter (DM) particle, into the range allowed by astrophysics and cosmology. These mechanisms include coannihilation with some nearly degenerate next-to-lightest supersymmetric particle such as the lighter stau t (tau) over bar (1), stop (t) over bar (1) or chargino (chi) over bar (+/-)(1), resonant annihilation via direct-channel heavy Higgs bosons H/A, the light Higgs boson h or the Z boson, and enhanced annihilation via a larger Higgsino component of the LSP in the focus-point region. These mechanisms typically select lower-dimensional subspaces inMSSMscenarios such as the CMSSM, NUHM1, NUHM2, and pMSSM10. We analyze how future LHC and direct DM searches can complement each other in the exploration of the different DM mechanisms within these scenarios. We find that the (tau) over bar (1) coannihilation regions of the CMSSM, NUHM1, NUHM2 can largely be explored at the LHC via searches for is not an element of(T) events and long-lived charged particles, whereas their H/A funnel, focus-point and (chi) over bar (+/-)(1) coannihilation regions can largely be explored by the LZ and Darwin DM direct detection experiments. We find that the dominant DM mechanism in our pMSSM10 analysis is (chi) over bar (+/-)(1) coannihilation: parts of its parameter space can be explored by the LHC, and a larger portion by future direct DM searches. C1 [Bagnaschi, E. A.; Weiglein, G.] DESY, D-22607 Hamburg, Germany. [Buchmueller, O.; Citron, M.; Malik, S.; de Vries, K. J.] Univ London Imperial Coll Sci Technol & Med, Blackett Lab, High Energy Phys Grp, London SW7 2AZ, England. [Cavanaugh, R.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Cavanaugh, R.] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. [De Roeck, A.; Ellis, J. R.] CERN, Dept Phys, CH-1211 Geneva 23, Switzerland. [De Roeck, A.] Univ Antwerp, B-2610 Antwerp, Belgium. [Dolan, M. J.] SLAC Natl Accelerator Lab, Theory Grp, Menlo Pk, CA 94025 USA. [Dolan, M. J.] Univ Melbourne, Sch Phys, ARC Ctr Excellence Particle Phys Terascale, Parkville, Vic 3010, Australia. [Ellis, J. R.; Sakurai, K.] Kings Coll London, Dept Phys, Theoret Particle Phys & Cosmol Grp, London WC2R 2LS, England. [Flaecher, H.] Univ Bristol, HH Wills Phys Lab, Bristol BS8 1TL, Avon, England. [Heinemeyer, S.] Inst Fis Cantabria CSIC UC, Santander 39005, Spain. [Isidori, G.] Univ Zurich, Inst Phys, CH-8057 Zurich, Switzerland. [Martinez Santos, D.] Univ Santiago de Compostela, Santiago De Compostela 15706, Spain. [Olive, K. A.] Univ Minnesota, Sch Phys & Astron, William I Fine Theoret Phys Inst, Minneapolis, MN 55455 USA. RP Bagnaschi, EA (reprint author), DESY, Notkestr 85, D-22607 Hamburg, Germany. EM olive@physics.umn.edu OI DOLAN, MATTHEW/0000-0003-3420-8718; Bagnaschi, Emanuele Angelo/0000-0002-6827-5022 FU London Centre for Terauniverse Studies (LCTS) from the European Research Council [267352]; National Science Foundation [PHY-1151640]; Fermilab [De-AC02-07CH11359]; United States Department of Energy; Australia Research Council; STFC (UK) [ST/L000326/1]; STFC (UK); CICYT [FPA 2013-40715-P]; Spanish MICINN's Consolider-Ingenio [MultiDark CSD2009-00064]; European Research Council [639068]; DOE [DE-SC0011842]; Collaborative Research Center of the DFG, "Particles, Strings and the early Universe" [SFB676]; European Commission through the "HiggsTools" Initial Training Network [PITN-GA-2012-316704] FX The work of O.B., J.E., S.M., K.A.O., K.S. and K.J.de V. is supported in part by the London Centre for Terauniverse Studies (LCTS), using funding from the European Research Council via the Advanced Investigator Grant 267352. The work of R.C. is supported in part by the National Science Foundation under Grant No. PHY-1151640 at the University of Illinois Chicago and in part by Fermilab, operated by Fermi Research Alliance, LLC under Contract No. De-AC02-07CH11359 with the United States Department of Energy. This work of M.J.D. is supported in part by the Australia Research Council. The work of J.E. is also supported in part by STFC (UK) via the research Grant ST/L000326/1, and the work of H.F. is also supported in part by STFC (UK). The work of S.H. is supported in part by CICYT (Grant FPA 2013-40715-P) and by the Spanish MICINN's Consolider-Ingenio 2010 Program under grant MultiDark CSD2009-00064. The work of D.M.-S. is supported by the European Research Council via Grant BSMFLEET 639068. The work of K.A.O. is supported in part by DOE Grant DE-SC0011842 at the University of Minnesota. The work of G.W. is supported in part by the Collaborative Research Center SFB676 of the DFG, "Particles, Strings and the early Universe", and by the European Commission through the "HiggsTools" Initial Training Network PITN-GA-2012-316704. NR 134 TC 18 Z9 18 U1 1 U2 4 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD OCT 23 PY 2015 VL 75 IS 10 AR 500 DI 10.1140/epjc/s10052-015-3718-9 PG 16 WC Physics, Particles & Fields SC Physics GA CU4WI UT WOS:000363530800001 ER PT J AU Singh, S Michalska, K Bigelow, L Endres, M Kharel, MK Babnigg, G Yennamalli, RM Bingman, CA Joachimiak, A Thorson, JS Phillips, GN AF Singh, Shanteri Michalska, Karolina Bigelow, Lance Endres, Michael Kharel, Madan K. Babnigg, Gyorgy Yennamalli, Ragothaman M. Bingman, Craig A. Joachimiak, Andrzej Thorson, Jon S. Phillips, George N., Jr. TI Structural Characterization of CalS8, a TDP-alpha-D-Glucose Dehydrogenase Involved in Calicheamicin Aminodideoxypentose Biosynthesis SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article ID STREPTOMYCES VIRIDOCHROMOGENES TU57; UDP-GLUCURONIC ACID; ESCHERICHIA-COLI; GENE-CLUSTER; MOLECULAR-REPLACEMENT; POLYMYXIN RESISTANCE; PURIFICATION; CLONING; INHIBITION; PROTEINS AB Classical UDP-glucose 6-dehydrogenases (UGDHs; EC 1.1.1.22) catalyze the conversion of UDP-alpha-D-glucose (UDPGlc) to the key metabolic precursor UDP-alpha-D-glucuronic acid (UDP-GlcA) and display specificity for UDP-Glc. The fundamental biochemical and structural study of the UGDH homolog CalS8 encoded by the calicheamicin biosynthetic gene is reported and represents one of the first studies of a UGDH homolog involved in secondary metabolism. The corresponding biochemical characterization of CalS8 reveals CalS8 as one of the first characterized base-permissive UGDH homologs with a > 15-fold preference for TDP-Glc over UDP-Glc. The corresponding structure elucidations of apo-CalS8 and the CalS8.substrate .cofactor ternary complex (at 2.47 and 1.95 angstrom resolution, respectively) highlight a notably high degree of conservation between CalS8 and classical UGDHs where structural divergence within the intersubunit loop structure likely contributes to the CalS8 base permissivity. As such, this study begins to provide a putative blueprint for base specificity among sugar nucleotide-dependent dehydrogenases and, in conjunction with prior studies on the base specificity of the calicheamicin aminopentosyltransferase CalG4, provides growing support for the calicheamicin aminopentose pathway as a TDP-sugar-dependent process. C1 [Singh, Shanteri; Thorson, Jon S.] Univ Kentucky, Coll Pharm, Ctr Pharmaceut Res & Innovat, Lexington, KY 40536 USA. [Michalska, Karolina; Bigelow, Lance; Endres, Michael; Babnigg, Gyorgy; Joachimiak, Andrzej] Argonne Natl Lab, Midwest Ctr Struct Genom, Argonne, IL 60439 USA. [Michalska, Karolina; Bigelow, Lance; Endres, Michael; Babnigg, Gyorgy; Joachimiak, Andrzej] Argonne Natl Lab, Struct Biol Ctr, Biosci Div, Argonne, IL 60439 USA. [Kharel, Madan K.] Univ Maryland Eastern Shore, Sch Pharm, Princess Anne, MD 21853 USA. [Bingman, Craig A.; Phillips, George N., Jr.] Univ Wisconsin, Dept Biochem, Madison, WI 53706 USA. [Yennamalli, Ragothaman M.; Phillips, George N., Jr.] Rice Univ, Dept Chem, Dept Biosci, Houston, TX 77005 USA. RP Thorson, JS (reprint author), Univ Kentucky, Coll Pharm, Ctr Pharmaceut Res & Innovat, Lexington, KY 40536 USA. EM jsthorson@uky.edu; georgep@rice.edu RI Thorson, Jon/L-3696-2013 OI Thorson, Jon/0000-0002-7148-0721 FU U. S. Department of Energy, Office of Biological and Environmental Research [DE-AC02-06CH11357]; Michigan Economic Development Corporation; Michigan Technology Tri-Corridor FX Use of the Structural Biology Center beamlines was supported by the U. S. Department of Energy, Office of Biological and Environmental Research, under Contract DE-AC02-06CH11357. The Life Sciences Collaborative Access Team (LS-CAT) has been supported by the Michigan Economic Development Corporation and the Michigan Technology Tri-Corridor. NR 63 TC 1 Z9 1 U1 2 U2 15 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD OCT 23 PY 2015 VL 290 IS 43 BP 26249 EP 26258 DI 10.1074/jbc.M115.673459 PG 10 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CU4VA UT WOS:000363527300041 PM 26240141 ER PT J AU Deng, S Hassan, MK Nalawade, A Perry, KA More, KL Mauritz, KA McDonnell, MT Keffer, DJ Mays, JW AF Deng, Shawn Hassan, Mohammad K. Nalawade, Amol Perry, Kelly A. More, Karren L. Mauritz, Kenneth A. McDonnell, Marshall T. Keffer, David J. Mays, Jimmy W. TI High temperature proton exchange membranes with enhanced proton conductivities at low humidity and high temperature based on polymer blends and block copolymers of poly(1,3-cyclohexadiene) and poly(ethylene glycol) SO POLYMER LA English DT Article DE Proton exchange membrane; Poly(ethylene glycol); Poly(1,3-cyclohexadiene) ID FUEL-CELL APPLICATIONS; ELECTROLYTE MEMBRANES; SULFONATED POLYBENZIMIDAZOLES; FLUORINATED POLYMER; POLY(ARYLENE ETHER); MOLECULAR-DYNAMICS; MAIN-CHAIN; TRANSPORT; WATER; MICROSTRUCTURE AB Hot (at 120 degrees C) and dry (20% relative humidity) operating conditions benefit fuel cell designs based on proton exchange membranes (PEMs) and hydrogen due to simplified system design and increasing tolerance to fuel impurities. Presented are preparation, partial characterization, and multi-scale modeling of such PEMs based on cross-linked, sulfonated poly(1,3-cyclohexadiene) (xsPCHD) blends and block copolymers with poly(ethylene glycol) (PEG). These low cost materials have proton conductivities 18 times that of current industry standard Nafion at hot, dry operating conditions. Among the membranes studied, the blend xsPCHD-PEG PEM displayed the highest proton conductivity, which exhibits a morphology with higher connectivity of the hydrophilic domain throughout the membrane. Simulation and modeling provide a molecular level understanding of distribution of PEG within this hydrophilic domain and its relation to proton conductivities. This study demonstrates enhancement of proton conductivity at high temperature and low relative humidity by incorporation of PEG and optimized sulfonation conditions. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Deng, Shawn; Mays, Jimmy W.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Hassan, Mohammad K.; Nalawade, Amol; Mauritz, Kenneth A.] Univ So Mississippi, Sch Polymers & High Performance Mat, Hattiesburg, MS 39406 USA. [Perry, Kelly A.; More, Karren L.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [McDonnell, Marshall T.] Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA. [Keffer, David J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Mays, Jimmy W.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Keffer, DJ (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. EM dkeffer@utk.edu RI More, Karren/A-8097-2016 OI More, Karren/0000-0001-5223-9097 FU U.S. Department of Energy, EERE Program [DE-FG36-06GO16037, DE-FG36-08GO88106]; U.S. Department of Energy's (DOE) Office of Basic Energy Sciences Program [DE-FG02-05ER15723]; National Science Foundation [DGE-0801470]; U.S. National Science Foundation (NSF) [EPS-1004083]; NSF [OCI 07-11134.5] FX We gratefully acknowledge the financial support of this research by the U.S. Department of Energy, EERE Program, under Grants #DE-FG36-06GO16037 and DE-FG36-08GO88106, by the U.S. Department of Energy's (DOE) Office of Basic Energy Sciences Program under Grants #DE-FG02-05ER15723, and by the National Science Foundation under Grant #DGE-0801470. A portion of the work at the University of Tennessee was supported by the U.S. National Science Foundation (NSF EPS-1004083, TN Score Thrust 2). Computational work used resources of the National Institute for Computational Sciences (NICS) supported by NSF under agreement number: OCI 07-11134.5. Microscopy research conducted as part of a user proposal at Oak Ridge National Laboratory's Center for Nanophase Materials Sciences (CNMS), which is an Office of Science User Facility. NR 70 TC 2 Z9 2 U1 6 U2 46 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0032-3861 EI 1873-2291 J9 POLYMER JI Polymer PD OCT 23 PY 2015 VL 77 BP 208 EP 217 DI 10.1016/j.polymer.2015.09.033 PG 10 WC Polymer Science SC Polymer Science GA CU4GC UT WOS:000363484300025 ER PT J AU Freelon, B Liu, YH Chen, JL Craco, L Laad, MS Leoni, S Chen, JQ Tao, L Wang, HD Flauca, R Yamani, Z Fang, MH Chang, CL Guo, JH Hussain, Z AF Freelon, B. Liu, Yu Hao Chen, Jeng-Lung Craco, L. Laad, M. S. Leoni, S. Chen, Jiaqi Tao, Li Wang, Hangdong Flauca, R. Yamani, Z. Fang, Minghu Chang, Chinglin Guo, J. -H. Hussain, Z. TI Mott-Kondo insulator behavior in the iron oxychalcogenides SO PHYSICAL REVIEW B LA English DT Article ID TRANSITION-METAL OXIDES; SUPERCONDUCTOR; SPECTRA; MODEL AB We perform a combined experimental-theoretical study of the Fe-oxychalcogenides (FeO Ch) series La2O2Fe2OM2 (M = S, Se), which are among the latest Fe-based materials with the potential to show unconventional high-T-c superconductivity (HTSC). A combination of incoherent Hubbard features in x-ray absorption and resonant inelastic x-ray scattering spectra, as well as resistivity data, reveal that the parent FeO Ch are correlation-driven insulators. To uncover microscopics underlying these findings, we perform local density approximation-plus-dynamical mean field theory (LDA+DMFT) calculations that reveal a novel Mott-Kondo insulating state. Based upon good agreement between theory and a range of data, we propose that FeO Ch may constitute an ideal testing ground to explore HTSC arising from a strange metal proximate to a novel selective-Mott quantum criticality. C1 [Freelon, B.; Liu, Yu Hao; Chen, Jeng-Lung; Guo, J. -H.; Hussain, Z.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source Div, Berkeley, CA 94720 USA. [Freelon, B.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Chen, Jeng-Lung; Chang, Chinglin] Tamkang Univ, Dept Phys, Tamsui 250, Taiwan. [Craco, L.] Univ Fed Mato Grosso, Inst Fis, BR-78060900 Cuiaba, MT, Brazil. [Laad, M. S.] Inst Math Sci, Madras 600113, Tamil Nadu, India. [Leoni, S.] Cardiff Univ, Sch Chem, Cardiff CF10 3AT, S Glam, Wales. [Chen, Jiaqi; Tao, Li; Wang, Hangdong; Fang, Minghu] Zhejiang Univ, Dept Phys, Hangzhou 310027, Peoples R China. [Flauca, R.; Yamani, Z.] AECL Res, Chalk River Labs, Natl Res Council, Canadian Neutron Beam Ctr, Chalk River, ON K0J 1J0, Canada. RP Freelon, B (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source Div, One Cyclotron Rd, Berkeley, CA 94720 USA. EM freelon@mit.edu; lcraco@fisica.ufmt.br RI Craco, Luis/L-6396-2016 NR 40 TC 4 Z9 4 U1 1 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 23 PY 2015 VL 92 IS 15 AR 155139 DI 10.1103/PhysRevB.92.155139 PG 10 WC Physics, Condensed Matter SC Physics GA CU1PP UT WOS:000363294100002 ER PT J AU Abbar, S Carlson, J Duan, H Reddy, S AF Abbar, Sajad Carlson, Joseph Duan, Huaiyu Reddy, Sanjay TI Quantum Monte Carlo calculations of the thermal conductivity of neutron star crusts SO PHYSICAL REVIEW C LA English DT Article ID ONE-COMPONENT PLASMA; TRANSPORT-PROPERTIES; KS-1731-260; CRYSTALS; DWARFS; ENERGY AB We use quantum Monte Carlo (QMC) techniques to calculate the static structure function S(q) of a one-component ion lattice and use it to calculate the thermal conductivity kappa of high-density solid matter expected in the neutron star crust. By making detailed comparisons with the results for the thermal conductivity obtained using standard techniques based on the one-phonon approximation (OPA) valid at low temperatures and the multiphonon harmonic approximation expected to be valid over a wide range of temperatures, we assess the temperature regime where S(q) from the QMC can be used directly to calculate kappa. We also compare the QMC results to those obtained using the classical Monte Carlo to quantitatively assess the magnitude of the quantum corrections. We found that quantum effects became relevant for the calculation of kappa at a temperature of T less than or similar to 0.3 Omega(P), where Omega(P) is the ion plasma frequency. At T similar or equal to 0.1 Omega(P) the quantum effects suppress kappa by about 30%. The comparison with the results of the OPA indicates that dynamical information beyond the static structure is needed when T similar or equal to 0.1 Omega(P). These quantitative comparisons help to establish QMC as a viable technique to calculate kappa at moderate temperatures in the range of T = 0.1-1 Omega(P) of relevance to the study of accreting neutron stars. This finding is especially important because QMC is the only viable technique so far for calculating kappa in multicomponent systems at low temperatures. C1 [Abbar, Sajad; Duan, Huaiyu] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87109 USA. [Carlson, Joseph] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Reddy, Sanjay] Univ Washington, Inst Nucl Theory, Seattle, WA 98195 USA. RP Abbar, S (reprint author), Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87109 USA. FU U.S. Department of Energy [DE-FG02-00ER41132]; DOE Topical Collaboration on Neutrinos and Nucleosynthesis in Hot and Dense Matter; LANL; NMC FX This collaborative work was supported, in part, by the DOE Topical Collaboration on Neutrinos and Nucleosynthesis in Hot and Dense Matter. H.D. thanks LANL and NMC for providing the start-up funding and the computing resources. S.R. was supported by the U.S. Department of Energy under Contract No. DE-FG02-00ER41132. NR 22 TC 4 Z9 4 U1 2 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 23 PY 2015 VL 92 IS 4 AR 045809 DI 10.1103/PhysRevC.92.045809 PG 8 WC Physics, Nuclear SC Physics GA CU1PU UT WOS:000363294600004 ER PT J AU Appelquist, T Brower, RC Buchoff, MI Fleming, GT Jin, XY Kiskis, J Kribs, GD Neil, ET Osborn, JC Rebbi, C Rinaldi, E Schaich, D Schroeder, C Syritsyn, S Vranas, P Weinberg, E Witzel, O AF Appelquist, T. Brower, R. C. Buchoff, M. I. Fleming, G. T. Jin, X. -Y. Kiskis, J. Kribs, G. D. Neil, E. T. Osborn, J. C. Rebbi, C. Rinaldi, E. Schaich, D. Schroeder, C. Syritsyn, S. Vranas, P. Weinberg, E. Witzel, O. CA Lattice Strong Dynamics LSD TI Stealth dark matter: Dark scalar baryons through the Higgs portal SO PHYSICAL REVIEW D LA English DT Article ID E(+)E(-) COLLISIONS; MASS; PARTICLES; SEARCH; SUPERSYMMETRY; BARYOGENESIS; TECHNICOLOR; ALIGNMENT; SIGNALS; LEPTONS AB We present a new model of stealth dark matter: a composite baryonic scalar of an SU(N-D) strongly coupled theory with even N-D >= 4. All mass scales are technically natural, and dark matter stability is automatic without imposing an additional discrete or global symmetry. Constituent fermions transform in vectorlike representations of the electroweak group that permit both electroweak-breaking and electroweak-preserving mass terms. This gives a tunable coupling of stealth dark matter to the Higgs boson independent of the dark matter mass itself. We specialize to SU(4), and investigate the constraints on the model from dark meson decay, electroweak precision measurements, basic collider limits, and spin-independent direct detection scattering through Higgs exchange. We exploit our earlier lattice simulations that determined the composite spectrum as well as the effective Higgs coupling of stealth dark matter in order to place bounds from direct detection, excluding constituent fermions with dominantly electroweak-breaking masses. A lower bound on the dark baryon mass m(B) greater than or similar to 300 GeV is obtained from the indirect requirement that the lightest dark meson not be observable at LEP II. We briefly survey some intriguing properties of stealth dark matter that are worthy of future study, including collider studies of dark meson production and decay; indirect detection signals from annihilation; relic abundance estimates for both symmetric and asymmetric mechanisms; and direct detection through electromagnetic polarizability, a detailed study of which will appear in a companion paper. C1 [Appelquist, T.; Fleming, G. T.] Yale Univ, Dept Phys, Sloane Lab, New Haven, CT 06520 USA. [Brower, R. C.; Rebbi, C.; Weinberg, E.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Buchoff, M. I.] Univ Washington, Inst Nucl Theory, Seattle, WA 98195 USA. [Jin, X. -Y.; Osborn, J. C.] Argonne Natl Lab, Argonne Leadership Comp Facil, Argonne, IL 60439 USA. [Kiskis, J.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Kribs, G. D.] Univ Oregon, Dept Phys, Eugene, OR 97403 USA. [Neil, E. T.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Neil, E. T.; Syritsyn, S.] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Rinaldi, E.; Schroeder, C.; Vranas, P.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Schaich, D.] Syracuse Univ, Dept Phys, Syracuse, NY 13244 USA. [Witzel, O.] Boston Univ, Ctr Computat Sci, Boston, MA 02215 USA. RP Appelquist, T (reprint author), Yale Univ, Dept Phys, Sloane Lab, New Haven, CT 06520 USA. RI Schaich, David/J-6644-2013; Jin, Xiao-Yong/R-7694-2016; OI Schaich, David/0000-0002-9826-2951; Jin, Xiao-Yong/0000-0002-2346-6861; Rinaldi, Enrico/0000-0003-4134-809X FU LLNL [LDRD 13-ERD-023]; U.S. Department of Energy [DE-SC0008669, DE-SC0009998, DE-SC0010025, DE-FG02-92ER40704, DE-SC0011640, DE-FG02-00ER41132, DE-AC52-07NA27344, DE-AC02-06CH11357, DE-SC0012704]; National Science Foundation [NSF PHY11-00905, OCI-0749300]; Office of Nuclear Physics in the U.S. Department of Energy's Office of Science [DE-AC02-05CH11231] FX We thank S. Chang, O. DeWolfe, and D. B. Kaplan for many valuable discussions during the course of this work. We thank the Lawrence Livermore National Laboratory (LLNL) Multiprogrammatic and Institutional Computing program for Grand Challenge allocations and time on the LLNL BlueGene/Q (rzuseq and vulcan) supercomputer. We thank LLNL for funding from LDRD 13-ERD-023 "Illuminating the Dark Universe with PetaFlops Supercomputing." Computing support for this work comes from the LLNL Institutional Computing Grand Challenge program. This work has been supported by the U.S. Department of Energy under Grants No. DE-SC0008669 and No. DE-SC0009998 (D. S.), No. DE-SC0010025 (R. C. B., C. R., E. W.), No. DE-FG02-92ER40704 (T. A.), No. DE-SC0011640 (G. D. K.), No. DE-FG02-00ER41132 (M. I. B.), and Contracts No. DE-AC52-07NA27344 (LLNL) and No. DE-AC02-06CH11357 (Argonne National Laboratory), and by the National Science Foundation under Grants No. NSF PHY11-00905 (G. F.) and No. OCI-0749300 (O. W.). Brookhaven National Laboratory is supported by the U.S. Department of Energy under Contract No. DE-SC0012704. S. N. S was supported by the Office of Nuclear Physics in the U.S. Department of Energy's Office of Science under Contract No. DE-AC02-05CH11231. NR 94 TC 7 Z9 7 U1 3 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 23 PY 2015 VL 92 IS 7 AR 075030 DI 10.1103/PhysRevD.92.075030 PG 16 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CU1PY UT WOS:000363295000005 ER PT J AU Lee, G Wagner, CEM AF Lee, Gabriel Wagner, Carlos E. M. TI Higgs bosons in heavy supersymmetry with an intermediate m(A) SO PHYSICAL REVIEW D LA English DT Article ID RENORMALIZATION-GROUP EQUATIONS; QUANTUM-FIELD THEORY; STANDARD MODEL; 3 LOOPS; MASS; MSSM; COUPLINGS; SECTOR; LHC; BETA AB The minimal supersymmetric standard model leads to precise predictions of the properties of the light Higgs boson degrees of freedom that depend on only a few relevant supersymmetry-breaking parameters. In particular, there is an upper bound on the mass of the lightest neutral Higgs boson, which for a supersymmetric spectrum of the order of a TeV is barely above the one of the Higgs resonance recently observed at the LHC. This bound can be raised by considering a heavier supersymmetric spectrum, relaxing the tension between theory and experiment. In a previous article, we studied the predictions for the lightest CP-even Higgs mass for large values of the scalar-top and heavy Higgs boson masses. In this article we perform a similar analysis, considering also the case of a CP-odd Higgs boson mass m(A) of the order of the weak scale. We perform the calculation using effective theory techniques, considering a two-Higgs doublet model and a Standard Model-like theory and resumming the large logarithmic corrections that appear at scales above and below m(A), respectively. We calculate the mass and couplings of the lightest CP-even Higgs boson and compare our results with the ones obtained by other methods. C1 [Lee, Gabriel] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Lee, Gabriel; Wagner, Carlos E. M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Lee, Gabriel; Wagner, Carlos E. M.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Wagner, Carlos E. M.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Wagner, Carlos E. M.] Argonne Natl Lab, HEP Div, Argonne, IL 60439 USA. RP Lee, G (reprint author), Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. FU U.S. Department of Energy [DE-AC02-06CH11357]; DOE [DE-FG02-13ER41958]; ICORE Program of Planning and Budgeting Committee; ISF [1937/12]; National Science Foundation [PHY-1066293] FX We are indebted to P. Slavich for his careful reading of the manuscript and many suggestions. We also thank S. Heinemeyer and J. P. Vega for useful discussions, and F. Staub and M. Goodsell for help with SARAH. Work at ANL is supported in part by the U.S. Department of Energy under Contract No. DE-AC02-06CH11357. G. L. acknowledges support from DOE Grant No. DE-FG02-13ER41958, the ICORE Program of Planning and Budgeting Committee, and by ISF Grant No. 1937/12. The authors acknowledge the hospitality of the Munich Institute for Astro- and Particle Physics (MIAPP) of the DFG cluster of excellence "Origin and Structure of the Universe" while this work was being completed. This work was completed while C. W. was at the Aspen Center for Physics, which is supported by National Science Foundation Grant No. PHY-1066293. NR 66 TC 9 Z9 9 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 23 PY 2015 VL 92 IS 7 AR 075032 DI 10.1103/PhysRevD.92.075032 PG 25 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CU1PY UT WOS:000363295000006 ER PT J AU Acconcia, TV Bonanca, MVS Deffner, S AF Acconcia, Thiago V. Bonanca, Marcus V. S. Deffner, Sebastian TI Shortcuts to adiabaticity from linear response theory SO PHYSICAL REVIEW E LA English DT Article AB Ashortcut to adiabaticity is a finite-time process that produces the same final state as would result from infinitely slow driving. We show that such shortcuts can be found for weak perturbations from linear response theory. With the help of phenomenological response functions, a simple expression for the excess work is found-quantifying the nonequilibrium excitations. For two specific examples, i.e., the quantum parametric oscillator and the spin 1/2 in a time-dependent magnetic field, we show that finite-time zeros of the excess work indicate the existence of shortcuts. Finally, we propose a degenerate family of protocols, which facilitates shortcuts to adiabaticity for specific and very short driving times. C1 [Acconcia, Thiago V.; Bonanca, Marcus V. S.] Univ Estadual Campinas Unicamp, Inst Fis Gleb Wataghin, BR-13083859 Sao Paulo, Brazil. [Deffner, Sebastian] Los Alamos Natl Lab, Theoret Div, Los Alamos, NM 87545 USA. [Deffner, Sebastian] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. RP Acconcia, TV (reprint author), Univ Estadual Campinas Unicamp, Inst Fis Gleb Wataghin, Rua Sergio Buarque Holanda 777, BR-13083859 Sao Paulo, Brazil. EM thiagova@ifi.unicamp.br RI Deffner, Sebastian/C-5170-2008; Bonanca, Marcus/C-8478-2012; Acconcia, Thiago/M-9704-2015; Inst. of Physics, Gleb Wataghin/A-9780-2017 OI Deffner, Sebastian/0000-0003-0504-6932; Bonanca, Marcus/0000-0001-7283-3034; Acconcia, Thiago/0000-0002-4113-262X; FU CNPq (Brazil) [134296/2013-3]; Institute of Physics Gleb Wataghin; Capes (Brazil) [1504869]; FAPESP (Brazil) [2012/07429-0]; U.S. Department of Energy FX T.A. acknowledges support from the Institute of Physics Gleb Wataghin, CNPq (Brazil), Project No. 134296/2013-3, and Capes (Brazil), Project No. 1504869. M.B. acknowledges financial support from FAPESP (Brazil), Project No. 2012/07429-0. S.D. acknowledges financial support from the U.S. Department of Energy through a LANL Director's Funded Fellowship. NR 39 TC 6 Z9 6 U1 1 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD OCT 23 PY 2015 VL 92 IS 4 AR 042148 DI 10.1103/PhysRevE.92.042148 PG 8 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA CU1SL UT WOS:000363301500001 PM 26565209 ER PT J AU Appelquist, T Berkowitz, E Brower, RC Buchoff, MI Fleming, GT Jin, XY Kiskis, J Kribs, GD Neil, ET Osborn, JC Rebbi, C Rinaldi, E Schaich, D Schroeder, C Syritsyn, S Vranas, P Weinberg, E Witzel, O AF Appelquist, T. Berkowitz, E. Brower, R. C. Buchoff, M. I. Fleming, G. T. Jin, X. -Y. Kiskis, J. Kribs, G. D. Neil, E. T. Osborn, J. C. Rebbi, C. Rinaldi, E. Schaich, D. Schroeder, C. Syritsyn, S. Vranas, P. Weinberg, E. Witzel, O. CA Lattice Strong Dynamics LSD TI Detecting Stealth Dark Matter Directly through Electromagnetic Polarizability SO PHYSICAL REVIEW LETTERS LA English DT Article ID QCD AB We calculate the spin-independent scattering cross section for direct detection that results from the electromagnetic polarizability of a composite scalar "stealth baryon" dark matter candidate, arising from a dark SU(4) confining gauge theory-"stealth dark matter." In the nonrelativistic limit, electromagnetic polarizability proceeds through a dimension-7 interaction leading to a very small scattering cross section for dark matter with weak-scale masses. This represents a lower bound on the scattering cross section for composite dark matter theories with electromagnetically charged constituents. We carry out lattice calculations of the polarizability for the lightest "baryon" states in SU(3) and SU(4) gauge theories using the background field method on quenched configurations. We find the polarizabilities of SU(3) and SU(4) to be comparable (within about 50%) normalized to the stealth baryon mass, which is suggestive for extensions to larger SU(N) groups. The resulting scattering cross sections with a xenon target are shown to be potentially detectable in the dark matter mass range of about 200-700 GeV, where the lower bound is from the existing LUX constraint while the upper bound is the coherent neutrino background. Significant uncertainties in the cross section remain due to the more complicated interaction of the polarizablity operator with nuclear structure; however, the steep dependence on the dark matter mass, 1/m(B)(6), suggests the observable dark matter mass range is not appreciably modified. We briefly highlight collider searches for the mesons in the theory as well as the indirect astrophysical effects that may also provide excellent probes of stealth dark matter. C1 [Appelquist, T.; Fleming, G. T.] Yale Univ, Dept Phys, Sloane Lab, New Haven, CT 06520 USA. [Berkowitz, E.; Rinaldi, E.; Schroeder, C.; Vranas, P.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Brower, R. C.; Rebbi, C.; Weinberg, E.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Buchoff, M. I.] Univ Washington, Inst Nucl Theory, Seattle, WA 98195 USA. [Jin, X. -Y.; Osborn, J. C.] Argonne Leadership Comp Facil, Argonne, IL 60439 USA. [Kiskis, J.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Kribs, G. D.] Univ Oregon, Dept Phys, Eugene, OR 97403 USA. [Neil, E. T.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Neil, E. T.; Syritsyn, S.] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Schaich, D.] Syracuse Univ, Dept Phys, Syracuse, NY 13244 USA. [Witzel, O.] Boston Univ, Ctr Computat Sci, Boston, MA 02215 USA. RP Appelquist, T (reprint author), Yale Univ, Dept Phys, Sloane Lab, New Haven, CT 06520 USA. RI Schaich, David/J-6644-2013; Jin, Xiao-Yong/R-7694-2016; OI Schaich, David/0000-0002-9826-2951; Jin, Xiao-Yong/0000-0002-2346-6861; Rinaldi, Enrico/0000-0003-4134-809X FU LDRD "Illuminating the Dark Universe with PetaFlops Supercomputing" [13-ERD-023]; Office of Science of the U.S. Department of Energy; U.S. Department of Energy [DE-SC0008669, DE-SC0009998, DE-SC0010025, DE-FG02-92ER-40704, DE-SC0011640, DE-FG02-00ER41132, DE-AC52-07NA27344, DE-AC02-06CH11357, DE-SC0012704]; National Science Foundation [NSF PHY11-00905, OCI-0749300]; Office of Nuclear Physics in the U.S. Department of Energy's Office of Science [DE-AC02-05CH11231, ] FX M. I. B. would like to thank Silas Beane, Paulo Bedaque, Tom Cohen, Jon Engel, Wick Haxton, David B. Kaplan, Jerry Miller, Maxim Pospelov, Sanjay Reddy, Martin Savage, Achim Schwenk, and Luca Vecchi for enlightening discussions on the full complexity of the nuclear physics calculation required for an accurate cross section prediction. We are also indebted to Brian Tiburzi for access to information that allowed for very useful checks of our background field code. We thank the Lawrence Livermore National Laboratory (LLNL) Multiprogrammatic and Institutional Computing program for Grand Challenge allocations and time on the LLNL BlueGene/Q (rzuseq and vulcan) supercomputer. We thank LLNL for funding from LDRD 13-ERD-023 "Illuminating the Dark Universe with PetaFlops Supercomputing." Computing support for this work was provided in part from the LLNL Institutional Computing Grand Challenge program and from the USQCD Collaboration, which is funded by the Office of Science of the U.S. Department of Energy. M. I. B. thanks the University of Oregon and University of Maryland, College Park for hospitality during the course of this work. This work has been supported by the U.S. Department of Energy under Grants No. DE-SC0008669 and No. DE-SC0009998 (D. S.), No. DE-SC0010025 (R. C. B., C. R., E. W.), No. DE-FG02-92ER-40704 (T. A.), No. DE-SC0011640 (G. D. K.), No. DE-FG02-00ER41132 (M. I. B.), and Contracts No. DE-AC52-07NA27344 (LLNL), No. DE-AC02-06CH11357 (Argonne National Laboratory), and by the National Science Foundation under Grants No. NSF PHY11-00905 (G. F.), No. OCI-0749300 (O. W.). Brookhaven National Laboratory is supported by the U.S. Department of Energy under Contract No. DE-SC0012704. S. N. S. was supported by the Office of Nuclear Physics in the U.S. Department of Energy's Office of Science under Contract No. DE-AC02-05CH11231. NR 48 TC 6 Z9 6 U1 3 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 23 PY 2015 VL 115 IS 17 AR 171803 DI 10.1103/PhysRevLett.115.171803 PG 7 WC Physics, Multidisciplinary SC Physics GA CU1TY UT WOS:000363305400003 PM 26551103 ER PT J AU Zhang, XW Zhang, LJ Perkins, JD Zunger, A AF Zhang, Xiuwen Zhang, Lijun Perkins, John D. Zunger, Alex TI Intrinsic Transparent Conductors without Doping SO PHYSICAL REVIEW LETTERS LA English DT Article ID OXIDE AB Transparent conductors (TCs) combine the usually contraindicated properties of electrical conductivity with optical transparency and are generally made by starting with a transparent insulator and making it conductive via heavy doping, an approach that generally faces severe "doping bottlenecks." We propose a different idea for TC design-starting with a metallic conductor and designing transparency by control of intrinsic interband transitions and intraband plasmonic frequency. We identify the specific design principles for three such prototypical intrinsic TC classes and then search computationally for materials that satisfy them. Remarkably, one of the intrinsic TC, Ag3Al22O34, is predicted also to be a prototype 3D compounds that manifest natural 2D electron gas regions with very high electron density and conductivity. C1 [Zhang, Xiuwen; Zhang, Lijun; Zunger, Alex] Univ Colorado, Renewable & Sustainable Energy Inst, Boulder, CO 80309 USA. [Perkins, John D.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Zunger, A (reprint author), Univ Colorado, Renewable & Sustainable Energy Inst, Boulder, CO 80309 USA. EM alex.zunger@colorado.edu RI Zhang, Lijun/F-7710-2011 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division [DE-FG02-13ER46959]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division under Grant No. DE-FG02-13ER46959 to C.U. We thank Liping Yu and Giancarlo Trimarchi for helpful discussions. This work used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 34 TC 2 Z9 2 U1 12 U2 53 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 23 PY 2015 VL 115 IS 17 AR 176602 DI 10.1103/PhysRevLett.115.176602 PG 6 WC Physics, Multidisciplinary SC Physics GA CU1TY UT WOS:000363305400009 PM 26551133 ER PT J AU Wan, WS Brouwer, L Caspi, S Prestemon, S Gerbershagen, A Schippers, JM Robin, D AF Wan, Weishi Brouwer, Lucas Caspi, Shlomo Prestemon, Soren Gerbershagen, Alexander Schippers, Jacobus Maarten Robin, David TI Alternating-gradient canted cosine theta superconducting magnets for future compact proton gantries SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article ID THERAPY; DESIGN AB We present a design of superconducting magnets, optimized for application in a gantry for proton therapy. We have introduced a new magnet design concept, called an alternating-gradient canted cosine theta (AG-CCT) concept, which is compatible with an achromatic layout. This layout allows a large momentum acceptance. The 15 cm radius of the bore aperture enables the application of pencil beam scanning in front of the SC-magnet. The optical and dynamic performance of a gantry based on these magnets has been analyzed using the fields derived (via Biot-Savart law) from the actual windings of the AG-CCT combined with the full equations of motion. The results show that with appropriate higher order correction, a large 3D volume can be rapidly scanned with little beam shape distortion. A very big advantage is that all this can be done while keeping the AG-CCT fields fixed. This reduces the need for fast field ramping of the superconducting magnets between the successive beam energies used for the scanning in depth and it is important for medical application since this reduces the technical risk (e.g., a quench) associated with fast field changes in superconducting magnets. For proton gantries the corresponding superconducting magnet system holds promise of dramatic reduction in weight. For heavier ion gantries there may furthermore be a significant reduction in size. C1 [Wan, Weishi; Brouwer, Lucas; Caspi, Shlomo; Prestemon, Soren; Robin, David] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Brouwer, Lucas] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Gerbershagen, Alexander] Paul Scherrer Inst, CH-5232 Villigen, Switzerland. RP Wan, WS (reprint author), Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM wwan@lbl.gov FU U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [DGE 1106400] FX Some of the authors (W. W., L. B., S. C., S. P. and D. R.) would like to express our deep thanks to Andy Sessler who we had the fortune of working closely with for many years towards the goal of developing technology for ion beam therapy. This work is supported under U.S. Department of Energy under Contract No. DE-AC02-05CH11231 and National Science Foundation under Grant No. DGE 1106400. NR 29 TC 4 Z9 4 U1 4 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD OCT 23 PY 2015 VL 18 IS 10 AR 103501 DI 10.1103/PhysRevSTAB.18.103501 PG 23 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA CU1UB UT WOS:000363305700001 ER PT J AU Chen, X Burnell, FJ Vishwanath, A Fidkowski, L AF Chen, Xie Burnell, F. J. Vishwanath, Ashvin Fidkowski, Lukasz TI Anomalous Symmetry Fractionalization and Surface Topological Order SO PHYSICAL REVIEW X LA English DT Article ID VALENCE-BOND; STATES AB In addition to possessing fractional statistics, anyon excitations of a 2D topologically ordered state can realize symmetry in distinct ways, leading to a variety of symmetry-enriched topological (SET) phases. While the symmetry fractionalization must be consistent with the fusion and braiding rules of the anyons, not all ostensibly consistent symmetry fractionalizations can be realized in 2D systems. Instead, certain "anomalous" SETs can only occur on the surface of a 3D symmetry-protected topological (SPT) phase. In this paper, we describe a procedure for determining whether a SET of a discrete, on-site, unitary symmetry group G is anomalous or not. The basic idea is to gauge the symmetry and expose the anomaly as an obstruction to a consistent topological theory combining both the original anyons and the gauge fluxes. Utilizing a result of Etingof, Nikshych, and Ostrik, we point out that a class of obstructions is captured by the fourth cohomology group H-4 (G, U(1)), which also precisely labels the set of 3D SPT phases, with symmetry group G. An explicit procedure for calculating the cohomology data from a SET is given, with the corresponding physical intuition explained. We thus establish a general bulk-boundary correspondence between the anomalous SET and the 3D bulk SPT whose surface termination realizes it. We illustrate this idea using the chiral spin liquid [U(1)(2)] topological order with a reduced symmetry Z(2) x Z(2) subset of SO(3),which can act on the semion quasiparticle in an anomalous way. We construct exactly solved 3D SPT models realizing the anomalous surface terminations and demonstrate that they are nontrivial by computing three-loop braiding statistics. Possible extensions to antiunitary symmetries are also discussed. C1 [Chen, Xie] CALTECH, Dept Phys, Pasadena, CA 91125 USA. [Chen, Xie] CALTECH, Inst Quantum Informat & Matter, Pasadena, CA 91125 USA. [Chen, Xie; Vishwanath, Ashvin] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Burnell, F. J.] Univ Minnesota, Dept Phys & Astron, Minneapolis, MN 55455 USA. [Vishwanath, Ashvin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Fidkowski, Lukasz] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. RP Chen, X (reprint author), CALTECH, Dept Phys, Pasadena, CA 91125 USA. FU Miller Institute for Basic Research in Science at UC Berkeley; Caltech Institute for Quantum Information and Matter; Walter Burke Institute for Theoretical Physics; [NSF DMR 1206728]; [NSF DMR 1352271] FX We are very grateful for helpful discussions with Meng Cheng, Senthil Todadri, Ryan Thorngren, Alexei Kitaev, Parsa Bonderson, and Netanel Lindner. X. C. is supported by the Miller Institute for Basic Research in Science at UC Berkeley, the Caltech Institute for Quantum Information and Matter, and the Walter Burke Institute for Theoretical Physics. A. V. is supported by Grant No. NSF DMR 1206728, and F. J. B. is supported by Grant No. NSF DMR 1352271. NR 41 TC 21 Z9 21 U1 1 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2160-3308 J9 PHYS REV X JI Phys. Rev. X PD OCT 23 PY 2015 VL 5 IS 4 AR 041013 DI 10.1103/PhysRevX.5.041013 PG 24 WC Physics, Multidisciplinary SC Physics GA CU1SO UT WOS:000363301800002 ER PT J AU Shen, QT Ren, XF Zhang, R Lee, IH Hurley, JH AF Shen, Qing-Tao Ren, Xuefeng Zhang, Rui Lee, Il-Hyung Hurley, James H. TI HIV-1 Nef hijacks clathrin coats by stabilizing AP-1:Arf1 polygons SO SCIENCE LA English DT Article ID CLASS-I MHC; DOWN-REGULATION; MEMBRANE RECRUITMENT; ADAPTER COMPLEXES; PROTEIN COMPLEXES; CYTOPLASMIC TAIL; STRUCTURAL BASIS; GOLGI MEMBRANES; CRYO-EM; MICROSCOPY AB The lentiviruses HIV and simian immunodeficiency virus (SIV) subvert intracellular membrane traffic as part of their replication cycle. The lentiviral Nef protein helps viruses evade innate and adaptive immune defenses by hijacking the adaptor protein 1 (AP-1) and AP-2 clathrin adaptors. We found that HIV-1 Nef and the guanosine triphosphatase Arf1 induced trimerization and activation of AP-1. Here we report the cryo-electron microscopy structures of the Nef- and Arf1-bound AP-1 trimer in the active and inactive states. A central nucleus of three Arf1 molecules organizes the trimers. We combined the open trimer with a known dimer structure and thus predicted a hexagonal assembly with inner and outer faces that bind the membranes and clathrin, respectively. Hexagons were directly visualized and the model validated by reconstituting clathrin cage assembly. Arf1 and Nef thus play interconnected roles in allosteric activation, cargo recruitment, and coat assembly, revealing an unexpectedly intricate organization of the inner AP-1 layer of the clathrin coat. Copyright 2015, American Association for the Advancement of Science. C1 [Shen, Qing-Tao; Ren, Xuefeng; Lee, Il-Hyung; Hurley, James H.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Shen, Qing-Tao; Ren, Xuefeng; Lee, Il-Hyung; Hurley, James H.] Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. [Zhang, Rui; Hurley, James H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. RP Hurley, JH (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. EM jimhurley@berkeley.edu FU HARC Collaborative Opportunity Fund; HARC Collaborative Opportunity Fund (NIH) [P50GM082250]; NIH [R01AI120691] FX We thank E. Nogales for suggestions and advice; J. Bonifacino for discussions; P. Grob, S. Wu, Y. Cheng, and B. LaFrance for assistance at the outset of the project; and A. Johnson for assistance with figure preparation. This work was supported by the HARC Collaborative Opportunity Fund (J.H.H.; subaward of NIH grant P50GM082250 to A. Frankel) and NIH grant R01AI120691 (J.H.H). EM facilities were supported by the Howard Hughes Medical Institute (E. Nogales). All EM maps have been deposited in the Electron Microscopy Data Bank (accession codes: EMD-6385 for closed trimer, EMD-6388 for closed monomer, EMD-6389 for open trimer). NR 48 TC 5 Z9 5 U1 1 U2 23 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD OCT 23 PY 2015 VL 350 IS 6259 AR aac5137 DI 10.1126/science.aac5137 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CU0NG UT WOS:000363213400030 PM 26494761 ER PT J AU Santos-Aberturas, J Dorr, M Waldo, GS Bornscheuer, UT AF Santos-Aberturas, Javier Doerr, Mark Waldo, Geoffrey S. Bornscheuer, Uwe T. TI In-Depth High-Throughput Screening of Protein Engineering Libraries by Split-GFP Direct Crude Cell Extract Data Normalization SO CHEMISTRY & BIOLOGY LA English DT Article ID EVOLUTION; SOLUBILITY; ESTERASE; ASSAYS AB Here, we report a widely and generally applicable strategy to obtain reliable information in high-throughput protein screenings of enzyme mutant libraries. The method is based on the usage of the split-GFP technology for the normalization of the expression level of each individual protein variant combined with activity measurements, thus resolving the important problems associated with the different solubility of each mutant and allowing the detection of previously invisible variants. The small size of the employed protein tag (16 amino acids) required for the reconstitution of the GFP fluorescence reduces possible interferences such as enzyme activity variations or solubility disturbances to a minimum. Specific enzyme activity measurements without purification, in situ soluble protein expression monitoring, and data normalization are the powerful outputs of this methodology, thus enabling the accurate identification of improved protein variants during high-throughput screening by substantially reducing the occurrence of false negatives and false positives. C1 [Santos-Aberturas, Javier; Doerr, Mark; Bornscheuer, Uwe T.] Ernst Moritz Arndt Univ Greifswald, Inst Biochem, Dept Biotechnol & Enzyme Catalysis, D-17487 Greifswald, Germany. [Waldo, Geoffrey S.] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA. RP Santos-Aberturas, J (reprint author), John Innes Ctr, Dept Mol Microbiol, Norwich NR4 7UH, Norfolk, England. EM javier.aberturas@jic.ac.uk; mark.doerr@uni-greifswald.de FU Deustche Forschungsgemeinschaft (DFG) [INST 292/118-1 FUGG]; federal state of Mecklenburg-Vorpommern; European Union [KBBE-2011-5, 289350] FX The authors would like to thank Hau B. Nguyen for the preparation of the pET GFP1-10 plasmid, and Alberto Nobili, Dr. Clare Vickers, Sandy Schmidt, and Moritz Voss for their help with the activity measurements. As a postdoctoral researcher, Javier Santos-Aberturas is deeply grateful to the Alexander von Humboldt foundation for its impeccable support. The authors thank the Deustche Forschungsgemeinschaft (DFG, INST 292/118-1 FUGG) and the federal state of Mecklenburg-Vorpommern for their financial support as well as the European Union (KBBE-2011-5, grant no. 289350, NewProt). G.S.W. is an inventor of the split GFP, which is the subject of pending and allowed patents by Los Alamos National Laboratories. NR 20 TC 2 Z9 2 U1 1 U2 12 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 1074-5521 EI 1879-1301 J9 CHEM BIOL JI Chem. Biol. PD OCT 22 PY 2015 VL 22 IS 10 BP 1406 EP 1414 DI 10.1016/j.chembiol.2015.08.014 PG 9 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CY1BG UT WOS:000366140900012 PM 26441043 ER PT J AU Matzen, LE Trumbo, MC Leach, RC Leshikar, ED AF Matzen, Laura E. Trumbo, Michael C. Leach, Ryan C. Leshikar, Eric D. TI Effects of non-invasive brain stimulation on associative memory SO BRAIN RESEARCH LA English DT Article DE tDCS; Associative memory; Recall; Recognition ID TRANSCRANIAL DC-STIMULATION; HUMAN MOTOR CORTEX; PREFRONTAL CORTEX; EPISODIC MEMORY; RECOGNITION MEMORY; ALZHEIMERS-DISEASE; FACE RECOGNITION; FALSE MEMORIES; WORKING-MEMORY; CUED-RECALL AB Associative memory refers to remembering the association between two items, such as a face and a name. It is a crucial part of daily life, but it is also one of the first aspects of memory performance that is impacted by aging and by Alzheimer's disease. Evidence suggests that transcranial direct current stimulation (tDCS) can improve memory performance, but few tDCS studies have investigated its impact on associative memory. In addition, no prior study of the effects of tDCS on memory performance has systematically evaluated the impact of tDCS on different types of memory assessments, such as recognition and recall tests. In this study, we measured the effects of tDCS on associative memory performance in healthy adults, using both recognition and recall tests. Participants studied face-name pairs while receiving either active (30 min, 2 mA) or sham (30 min, 0.1 mA) stimulation with the anode placed at F9 and the cathode placed on the contralateral upper arm. Participants in the active stimulation group performed significantly better on the recall test than participants in the sham group, recalling 50% more names, on average, and making fewer recall errors. However, the two groups did not differ significantly in terms of their performance on the recognition memory test. This investigation provides evidence that stimulation at the time of study improves associative memory encoding, but that this memory benefit is evident only under certain retrieval conditions. (C) 2015 Elsevier B.V. All rights reserved. C1 [Matzen, Laura E.; Trumbo, Michael C.] Sandia Natl Labs, Cognit Sci & Applicat, Albuquerque, NM 87185 USA. [Trumbo, Michael C.] Univ New Mexico, Albuquerque, NM 87131 USA. [Leach, Ryan C.; Leshikar, Eric D.] Univ Illinois, Chicago, IL USA. RP Matzen, LE (reprint author), Sandia Natl Labs, Cognit Sci & Applicat, POB 5800, Albuquerque, NM 87185 USA. EM lematze@sandia.gov FU Laboratory Directed Research and Development (LDRD) Program at Sandia National Laboratories; Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors thank Dr. Vince Clark for his assistance with this project. This work was funded by the Laboratory Directed Research and Development (LDRD) Program at Sandia National Laboratories. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 54 TC 2 Z9 3 U1 4 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0006-8993 EI 1872-6240 J9 BRAIN RES JI Brain Res. PD OCT 22 PY 2015 VL 1624 BP 286 EP 296 DI 10.1016/j.brainres.2015.07.036 PG 11 WC Neurosciences SC Neurosciences & Neurology GA CW5PY UT WOS:000365050100029 PM 26236022 ER PT J AU Whitney, JC Quentin, D Sawai, S LeRoux, M Harding, BN Ledvina, HE Tran, BQ Robinson, H Goo, YA Goodlett, DR Raunser, S Mougous, JD AF Whitney, John C. Quentin, Dennis Sawai, Shin LeRoux, Michele Harding, Brittany N. Ledvina, Hannah E. Tran, Bao Q. Robinson, Howard Goo, Young Ah Goodlett, David R. Raunser, Stefan Mougous, Joseph D. TI An Interbacterial NAD(P)(+) Glycohydrolase Toxin Requires Elongation Factor Tu for Delivery to Target Cells SO CELL LA English DT Article ID VI SECRETION SYSTEM; PSEUDOMONAS-AERUGINOSA; EF-TU; STRUCTURAL BASIS; BINDING-PROTEIN; EFFECTORS; COMPLEX; PNEUMONIAE; IMMUNITY; RECEPTOR AB Type VI secretion (T6S) influences the composition of microbial communities by catalyzing the delivery of toxins between adjacent bacterial cells. Here, we demonstrate that a T6S integral membrane toxin from Pseudomonas aeruginosa, Tse6, acts on target cells by degrading the universally essential dinucleotides NAD(+) and NADP(+). Structural analyses of Tse6 show that it resembles mono-ADP-ribosyltransferase proteins, such as diphtheria toxin, with the exception of a unique loop that both excludes proteinaceous ADP-ribose acceptors and contributes to hydrolysis. We find that entry of Tse6 into target cells requires its binding to an essential housekeeping protein, translation elongation factor Tu (EF-Tu). These proteins participate in a larger assembly that additionally directs toxin export and provides chaperone activity. Visualization of this complex by electron microscopy defines the architecture of a toxin-loaded T6S apparatus and provides mechanistic insight into intercellular membrane protein delivery between bacteria. C1 [Whitney, John C.; Sawai, Shin; LeRoux, Michele; Harding, Brittany N.; Ledvina, Hannah E.; Mougous, Joseph D.] Univ Washington, Dept Microbiol, Seattle, WA 98195 USA. [Quentin, Dennis; Raunser, Stefan] Max Planck Inst Mol Physiol, Dept Struct Biochem, D-44227 Dortmund, Germany. [Tran, Bao Q.; Goo, Young Ah; Goodlett, David R.] Univ Maryland, Sch Pharm, Dept Pharmaceut Sci, Baltimore, MD 21201 USA. [Robinson, Howard] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. [Mougous, Joseph D.] Howard Hughes Med Inst, Seattle, WA 98195 USA. RP Mougous, JD (reprint author), Univ Washington, Dept Microbiol, Seattle, WA 98195 USA. EM mougous@u.washington.edu OI Raunser, Stefan/0000-0001-9373-3016 FU NIH [AI080609]; University of Maryland Baltimore, School of Pharmacy Mass Spectrometry Center [SOP1841-IQB2014]; Canadian Institutes of Health Research; Chemiefonds fellowship from the Fonds der Chemischen Industrie; Mary Gates Research Scholarship; Investigator in the Pathogenesis of Infectious Disease Award from the Burroughs Wellcome Fund FX The authors would like to thank H. Kulasekara for assistance with membrane fractionation, C. Outten for providing pRSFDuet-1, W. Catterall for use of the ITC instrument, J. Woodward for assistance with radioactivity experiments and for providing Aurodox, C. Ralston for assistance with X-ray data collection, I. Attree for providing alpha-OprF antibody, C. Gatsogiannis for electron microscopy expertise, and S. Dove, C. Goulding, C. Hayes, D. Low, A. Merz, D. Veesler, and members of the S.R. and J.D.M. laboratories for helpful discussions. This work was supported by grants from the NIH (AI080609) (to J.D.M.) and by the University of Maryland Baltimore, School of Pharmacy Mass Spectrometry Center (SOP1841-IQB2014) (to D.R.G.). J.C.W. was supported by a postdoctoral research fellowship from the Canadian Institutes of Health Research, D.Q. was supported by a Chemiefonds fellowship from the Fonds der Chemischen Industrie, S.S. was supported by a Mary Gates Research Scholarship, and J.D.M. holds an Investigator in the Pathogenesis of Infectious Disease Award from the Burroughs Wellcome Fund. NR 46 TC 15 Z9 15 U1 0 U2 10 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0092-8674 EI 1097-4172 J9 CELL JI Cell PD OCT 22 PY 2015 VL 163 IS 3 BP 607 EP 619 DI 10.1016/j.cell.2015.09.027 PG 13 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA CW2NK UT WOS:000364828900015 PM 26456113 ER PT J AU Gebhardt, RS Du, PF Peer, A Rock, M Kessler, MR Biswas, R Ganapathysubramanian, B Chaudhary, S AF Gebhardt, Ryan S. Du, Pengfei Peer, Akshit Rock, Mitch Kessler, Michael R. Biswas, Rana Ganapathysubramanian, Baskar Chaudhary, Sumit TI Utilizing Wide Band Gap, High Dielectric Constant Nanoparticles as Additives in Organic Solar Cells SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID PHOTOVOLTAIC DEVICES; CHARGE-SEPARATION; TERNARY BLENDS; THIN-FILMS; POWDERS AB We experimentally and theoretically investigate the effects of utilizing BaTiO3 nanoparticles as additives in polythiophene/fullerene solar cells. BaTiO3 nanoparticles were chosen because of their multifaceted potential for increasing exciton dissociation (due to their high dielectric constant) and light scattering. To achieve stable suspensions for device fabrication, the nanoparticles were functionalized with organic ligands. Solar cells fabricated in air showed similar to 40% enhancement in the photocurrent primarily due to string-like aggregates of functionalized BaTiO3 particles that increase light absorption without hindering charge collection. Solar cells fabricated in an inert atmosphere yielded overall more efficient devices, but the string-like aggregates were absent and enhancement in photocurrent was up to similar to 6%. Simulations with the excitonic drift-diffusion model demonstrate that a bare nanoparticle significantly increases exciton dissociation, whereas the functional group negates this effect. Simulations utilizing the scattering matrix method reveal that absorption enhancements caused by light scattering increase as the nanoparticles aggregate into string-like structures. These results offer insights for morphological design of ternary-blend bulk-heterojunction organic solar cells. C1 [Gebhardt, Ryan S.; Chaudhary, Sumit] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Gebhardt, Ryan S.; Peer, Akshit; Biswas, Rana; Chaudhary, Sumit] Iowa State Univ, Dept Elect & Comp Engn, Ames, IA USA. [Du, Pengfei; Ganapathysubramanian, Baskar] Iowa State Univ, Dept Mech Engn, Ames, IA USA. [Biswas, Rana] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Rock, Mitch; Kessler, Michael R.] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. [Biswas, Rana] US DOE, Ames Lab, Ames, IA 50011 USA. RP Chaudhary, S (reprint author), Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. EM sumitc@iastate.edu RI Kessler, Michael/C-3153-2008 OI Kessler, Michael/0000-0001-8436-3447 FU National Science Foundation [CBET-1236839, ECCS-1055930, ECCS-1232067, CBET-1336134]; KAUST CRG; NSF [CMMI-1149365]; Ames Laboratory [DE-AC02-07CH11385]; Office of Science of the USDOE [DE-AC02-05CH11231] FX This material is primarily based on work supported by the National Science Foundation under Grants CBET-1236839 and ECCS-1055930. B.G. and P.D. acknowledge partial support from KAUST CRG and NSF Grant CMMI-1149365. R.B. acknowledges partial support from the Ames Laboratory, operated for the Department of Energy (theoretical analysis) by Iowa State University under Contract No. DE-AC02-07CH11385; and the National Science Foundation through Grants ECCS-1232067 and CBET-1336134 (computational work). The research used resources at the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the USDOE under Contract No. DE-AC02-05CH11231. NR 30 TC 0 Z9 0 U1 1 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 22 PY 2015 VL 119 IS 42 BP 23883 EP 23889 DI 10.1021/acs.jpcc.5b08581 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CV0CV UT WOS:000363915900011 ER PT J AU Liu, C Evans, TJ Cheng, L Ninnlos, MR Mukarakate, C Robichaud, DJ Assary, RS Curtiss, LA AF Liu, Cong Evans, Tabitha J. Cheng, Lei Ninnlos, Mark R. Mukarakate, Calvin Robichaud, David J. Assary, Rajeev S. Curtiss, Larry A. TI Catalytic Upgrading of Biomass-Derived Compounds via C-C Coupling Reactions: Computational and Experimental Studies of Acetaldehyde and Furan Reactions in HZSM-5 SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; PYROLYSIS OIL; ZEOLITE CATALYSTS; TRANSPORTATION FUELS; OXYGENATE COMPONENTS; P-XYLENE; CONVERSION; HYDROCARBONS AB Catalytic C-C coupling and deoxygenation reactions are essential for upgrading of biomass-derived oxygenates to fuel-range hydrocarbons. Detailed understanding of mechanistic and energetic aspects of these reactions is crucial to enabling and improving the catalytic upgrading of small oxygenates to useful chemicals and fuels. Using periodic density functional theory (DFT) calculations, we have investigated the reactions of furan and acetaldehyde in an HZSM-5 zeolite catalyst, a representative system associated with the catalytic upgrading of pyrolysis vapors. Comprehensive energy profiles were computed for self-reactions (i.e., acetaldehyde coupling and furan coupling) and cross-reactions (i.e., acetaldehyde + furan) of this representative mixture. Major products proposed from the computations are further confirmed using temperature controlled mass spectra measurements. The computational results show that furan interacts with acetaldehyde in HZSM-5 via an alkylation mechanism, which is more favorable than the self-reactions, indicating that mixing furans with aldehydes could be a promising approach to maximize effective C-C coupling and dehydration while reducing the catalyst deactivation (e.g., coke formation) from aldehyde condensation. C1 [Liu, Cong; Cheng, Lei; Assary, Rajeev S.; Curtiss, Larry A.] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. [Evans, Tabitha J.; Ninnlos, Mark R.; Mukarakate, Calvin; Robichaud, David J.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. RP Assary, RS (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Lemont, IL 60439 USA. EM assary@anl.gov; curtiss@anl.gov RI Surendran Assary, Rajeev/E-6833-2012; OI Surendran Assary, Rajeev/0000-0002-9571-3307; Liu, Cong/0000-0002-2145-5034 FU Bioenergy Technologies Office (BETO) program of Energy Efficiency & Renewable Energy (EERE); Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; ANL; U.S. Department of Energy's Bioenergy Technologies Office (DOE-BETO) [DE-AC36-08GO28308]; National Renewable Energy Laboratory FX This work was conducted as part of the Computational Pyrolysis Consortium (CPC) which is supported by the Bioenergy Technologies Office (BETO) program of Energy Efficiency & Renewable Energy (EERE). We gratefully acknowledge the computing resources provided on "Blues", a computing cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory (ANL). This research used resources of the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Use of the Center for Nanoscale Materials was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. We also thank the support of the Director's Postdoctoral Fellowship from ANL to C.L. D.J.R., T.J.E., C.M., and M.R.N. were supported by the U.S. Department of Energy's Bioenergy Technologies Office (DOE-BETO) Contract No. DE-AC36-08GO28308 with the National Renewable Energy Laboratory. NR 53 TC 5 Z9 5 U1 3 U2 23 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 22 PY 2015 VL 119 IS 42 BP 24025 EP 24035 DI 10.1021/acs.jpcc.5b08141 PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CV0CV UT WOS:000363915900027 ER PT J AU Halliday, MTE Joly, AG Hess, WP Shluger, AL AF Halliday, M. T. E. Joly, A. G. Hess, W. P. Shluger, A. L. TI Photoinduced Br Desorption from CsBr Thin Films Grown on Cu(100) SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ALKALI-HALIDE CRYSTALS; SELF-TRAPPED EXCITON; NACL 100 SURFACES; ELECTRONIC EXCITATION; STIMULATED DESORPTION; ADJUSTABLE-PARAMETERS; HOT PHOTOELECTRONS; ATOMIC DESORPTION; RADIATION-DAMAGE; LASER-DESORPTION AB Thin films of CsBr deposited onto metals such as copper are potential photocathode materials for light sources and other applications. We investigate desorption dynamics of Br atoms from CsBr films grown on insulator (KBr, LiF) and metal (Cu) substrates induced by sub-bandgap 6.4 eV laser pulses. The experimental results demonstrate that the peak kinetic energy of Br atoms desorbed from CsBr/Cu films is much lower than that for the hyperthermal desorption from CsBr/LiF films. Kelvin probe measurements indicate negative charge at the surface following Br desorption from CsBr/Cu films. Our ab initio calculations of excitons at CsBr surfaces demonstrate that this behavior can be explained by an exciton model of desorption including electron trapping at the CsBr surface. Trapped negative charges reduce the energy of surface excitons available for Br desorption. We examine the electron-trapping characteristics of low-coordinated sites at the surface, in particular, divacancies and kink sites. We also provide a model of cation desorption caused by Franck-Hertz excitation of F centers at the surface in the irradiation of CsBr/Cu films. These results provide new insights into the mechanisms of photoinduced structural evolution alkali halide films on metal substrates and activation of metal photocathodes coated with CsBr. C1 [Halliday, M. T. E.; Shluger, A. L.] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Halliday, M. T. E.; Shluger, A. L.] UCL, London Ctr Nanotechnol, London WC1E 6BT, England. [Joly, A. G.; Hess, W. P.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP Shluger, AL (reprint author), UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. EM a.shluger@ucl.ac.uk FU EPSRC; U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosdences; DOE's Office of Biological and Environmental Research; PNNL; EPSRC [EP/F067496] FX M.T.E.H. is grateful to EPSRC for financial support. We acknowledge support from the U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosdences. A portion of this work was performed using EMSL, a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at PNNL. PNNL is a multiprogram national laboratory operated for DOE by Battelle. Access to the Archer facility is provided via our membership of the U.K.'s HPC Materials Chemistry Consortium, which is funded by EPSRC grant EP/F067496. NR 64 TC 1 Z9 1 U1 0 U2 10 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 22 PY 2015 VL 119 IS 42 BP 24036 EP 24045 DI 10.1021/acs.jpcc.5b08275 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CV0CV UT WOS:000363915900028 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Ochesanu, S Rougny, R Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Van Parijs, I Barria, P Caillol, C Clerbaux, B De Lentdecker, G Delannoy, H Dobur, D Fasanella, G Favart, L Gay, APR Grebenyuk, A Leonard, A Mohammadi, A Pernie, L Randle-Conde, A Reis, T Seva, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Zenoni, F Zhang, F Beernaert, K Benucci, L Cimmino, A Crucy, S Fagot, A Garcia, G Gul, M Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Diblen, SS Sigamani, M Strobbe, N Tytgat, M Van Driessche, W Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bondu, O Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Mertens, A Nuttens, C Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Beliy, N Caebergs, T Hammad, GH Alda, WL Alves, GA Brito, L Correa Martins, M Martins, TDR Hensel, C Herrera, CM Moraes, A Pol, ME Teles, PR Das Chagas, EBB Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Guativa, LMH Malbouisson, H Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santaolalla, J Santoro, A Sznajder, A Manganote, EJT Pereira, AV Ahuja, S Bernardes, CA Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Moon, CS Novaes, SF Padula, SS Abad, DR Vargas, JCR Aleksandrov, A Genchev, V Hadjiiska, R Iaydjiev, P Marinov, A Piperov, S Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Ahmad, M Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Plestina, R Romeo, F Shaheen, SM Tao, J Wang, C Wang, Z Zhang, H Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Xu, Z Zou, W Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Bodlak, M Finger, M Finger, M Ali, A Aly, R Aly, S Assran, Y Kamel, AE Lotfy, A Mahmoud, MA Masod, R Radi, A Calpas, B Kadastik, M Murumaa, M Raidal, M Tiko, A Veelken, C Eerola, P Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Pekkanen, J Peltola, T Tuominen, E Tuominiemi, J Tuovi-Nen, E Wendland, L Talvitie, J Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Favaro, C Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Machet, M Maleles, J Rander, J Rosowsky, A Titov, M Zghiche, A Baffioni, S Beaudette, F Busson, P Cadamuro, L Chapon, E Chariot, C Dahms, T Davignon, O Filipovic, N Florent, A de Cassagnac, RG Lisniak, S Mas-Trolorenzo, L Mine, P Naranjo, IN Nguyen, M Ochando, C Ortona, G Paganini, P Regnard, S Salerno, R Sauvan, JB Sirois, Y Strebler, T Yilmaz, Y Zabi, A Agram, JL Andrea, J Aubin, A Bloch, D Brom, JM Buttignol, M Chabert, EC Chanon, N Collard, C Conte, E Fontaine, JC Gele, D Goerlach, U Goetzmann, C Le Bihan, AC Merlin, JA Skovpen, K Van Hove, P Gadrat, S Beauceron, S Beaupere, N Bernet, C Boudoul, G Bouvier, E Brochet, S Montoya, CAC Chasserat, J Chierici, R Contardo, D Courbon, B Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Laktineh, IB Lethuillier, M Mirabito, L Pequegnot, AL Perries, S Alvarez, JDR Sabes, D Sgandurra, L Sordini, V Vander Donckt, M Verdier, P Viret, S Xiao, H Tsamalaidze, Z Autermann, C Beranek, S Edelhoff, M Feld, L Heister, A Kiesel, MK Klein, K Lipinski, M Ostapchuk, A Preuten, M Raupach, F Sammet, J Schael, S Schulte, JF Verlage, T Weber, H Wittmer, B Zhukov, V Ata, M Brodski, M Dietz-Laursonn, E Duchardt, D Endres, M Erdmann, M Erdweg, S Esch, T Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Millet, P Olschewski, M Padeken, K Papacz, P Pook, T Radziej, M Reithler, H Rieger, M Scheuch, F Sonnenschein, L Teyssier, D Thuer, S Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Ahmad, WH Hoehle, F Kargoll, B Kress, T Kuessel, Y Kunsken, A Lingemann, J Nehrkorn, A Nowack, A Nugent, IM Pistone, C Pooth, O Stahl, A Martin, MA Asin, I Bartosik, N Behnke, O Behrens, U Bell, AJ Borras, K Burgmeier, A Cakir, A Calligaris, L Campbell, A Choudhury, S Costanza, F Pardos, CD Dolinska, G Dooling, S Dorland, T Eckerlin, G Eckstein, D Eichhorn, T Flucke, G Gallo, E Garcia, JG Geiser, A Gizhko, A Gunnellini, P Hauk, J Hempel, M Jung, H Kalogeropoulos, A Karacheban, O Kasemann, M Katsas, P Kieseler, J Kleinwort, C Korol, I Lange, W Leonard, J Lipka, K Lobanov, A Lohmann, W Mankel, R Marfin, I Melzer-Pellmann, IA Meyer, AB Mit-Tag, G Mnich, J Mussgiller, A Naumann-Emme, S Nayak, A Ntomari, E Perrey, H Pitzl, D Placakyte, R Raspereza, A Cipriano, PMR Roland, B Sahin, MO Salfeld-Nebgen, J Saxena, P Schoerner-Sadenius, T Schroder, M Spannagel, CSS Trippkewitz, KD Wissing, C Blobel, V Vignali, MC Draeger, AR Erfle, J Garutti, E Goebel, K Gonzalez, D Gorner, M Haller, J Hoffmann, M Hoing, RS Junkes, A Klanner, R Kogler, R Lapsien, T Lenz, T Marchesini, I Marconi, D Nowatschin, D Ott, J Pantaleo, F Peiffer, T Perieanu, A Pietsch, N Poehlsen, J Rathjens, D Sander, C Schettler, H Schleper, P Schlieckau, E Schmidt, A Seidel, M Sola, V Stadie, H Steinbruck, G Tholen, H Troendle, D Usai, E Vanelderen, L Vanhoefer, A Akbiyik, M Barth, C Baus, C Berger, J Boser, C Butz, E Chwalek, T Colombo, F De Boer, W Descroix, A Dierlamm, A Feindt, M Frensch, F Giffels, M Gilbert, A Hartmann, F Husemann, U Kassel, F Katkov, I Kornmayer, A Pardo, PL Mozer, MU Muller, T Muller, T Plagge, M Quast, G Rabbertz, K Rocker, S Roscher, F Simonis, HJ Stober, FM Ulrich, R Wagner-Kuhr, J Wayand, S Weiler, T Wohrmann, C Wolf, R Anagnostou, G Daskalakis, G Geralis, T Giakoumopoulou, VA Kyriakis, A Loukas, D Markou, A Psallidas, A Topsis-Giotis, I Agapitos, A 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Lanaro, A. Levine, A. Long, K. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Ruggles, T. Sarangi, T. Savin, A. Smith, N. Smith, W. H. Taylor, D. Woods, N. CA CMS Collaboration TI Search for a Higgs boson in the mass range from 145 to 1000 GeV decaying to a pair of W or Z bosons SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering; Higgs physics ID WEAK INTERACTIONS; STANDARD MODEL; ATLAS DETECTOR; PP COLLISIONS; PARTON DISTRIBUTIONS; BROKEN SYMMETRIES; GAUGE-THEORIES; HIGH-ENERGIES; HIDDEN HIGGS; FINAL-STATES AB A search for a heavy Higgs boson in the H -> WW and H -> ZZ decay channels is reported. The search is based upon proton-proton collision data samples corresponding to an integrated luminosity of up to 5.1 fb(-1) at root s = 7 TeV and up to 19.7 fb(-1) at root s = 8 TeV, recorded by the CMS experiment at the CERN LHC. Several final states of the H -> WW and H -> ZZ decays are analyzed. The combined upper limit at the 95% confidence level on the product of the cross section and branching fraction exclude a Higgs boson with standard model-like couplings and decays in the range 145 < m(H) < 1000 GeV. We also interpret the results in the context of an electroweak singlet extension of the standard model. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hartl, C.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Knuenz, V.; Koenig, A.; Krammer, M.; Kraetschmer, I.; Liko, D.; Matsushita, T.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, H.; Schieck, J.; Schoefbeck, R.; Strauss, J.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] Inst Hochenergiephys OeAW, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. 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[Beernaert, K.; Benucci, L.; Cimmino, A.; Crucy, S.; Fagot, A.; Garcia, G.; Gul, M.; Mccartin, J.; Rios, A. A. Ocampo; Poyraz, D.; Ryckbosch, D.; Diblen, S. Salva; Sigamani, M.; Strobbe, N.; Tytgat, M.; Van Driessche, W.; Yazgan, E.; Zaganidis, N.] Univ Ghent, B-9000 Ghent, Belgium. [Basegmez, S.; Beluffi, C.; Bondu, O.; Bruno, G.; Castello, R.; Caudron, A.; Ceard, L.; Da Silveira, G. G.; Delaere, C.; du Pree, T.; Favart, D.; Forthomme, L.; Giammanco, A.; Hollar, J.; Jafari, A.; Jez, P.; Komm, M.; Lemaitre, V.; Mertens, A.; Nuttens, C.; Perrini, L.; Pin, A.; Piotrzkowski, K.; Popov, A.; Quertenmont, L.; Selvaggi, M.; Marono, M. Vidal] Catholic Univ Louvain, Louvain, Belgium. [Beliy, N.; Caebergs, T.; Hammad, G. H.] Univ Mons, B-7000 Mons, Belgium. [Alda Junior, W. L.; Alves, G. A.; Brito, L.; Correa Martins Junior, M.; Martins, T. Dos Reis; Hensel, C.; Mora Herrera, C.; Moraes, A.; Pol, M. E.; Teles, P. Rebello] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. [Belchior Batista Das Chagas, E.; Carvalho, W.; Chinellato, J.; Custodio, A.; Da Costa, E. M.; De Jesus Damiao, D.; De Oliveira Martins, C.; Fonseca De Souza, S.; Huertas Guativa, L. M.; Malbouisson, H.; Matos Figueiredo, D.; Mundim, L.; Nogima, H.; Prado Da Silva, W. L.; Santaolalla, J.; Santoro, A.; Sznajder, A.; Tonelli Manganote, E. J.; Vilela Pereira, A.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Dogra, S.; Fernandez Perez Tomei, T. R.; Moon, C. S.; Novaes, S. F.; Padula, Sandra S.] Univ Estadual Paulista, Sao Paulo, Brazil. [Bernardes, C. A.; Gregores, E. M.; Mercadante, P. G.] Univ Fed ABC, Sao Paulo, Brazil. [Aleksandrov, A.; Genchev, V.; Hadjiiska, R.; Iaydjiev, P.; Marinov, A.; Piperov, S.; Rodozov, M.; Stoykova, S.; Sultanov, G.; Vutova, M.] Inst Nucl Energy Res, Sofia, Bulgaria. [Dimitrov, A.; Glushkov, I.; Litov, L.; Pavlov, B.; Petkov, P.] Univ Sofia, BU-1126 Sofia, Bulgaria. [Ahmad, M.; Bian, J. G.; Chen, G. M.; Chen, H. S.; Chen, M.; Cheng, T.; Du, R.; Jiang, C. H.; Plestina, R.; Romeo, F.; Shaheen, S. M.; Tao, J.; Wang, C.; Wang, Z.; Zhang, H.] Inst High Energy Phys, Beijing 100039, Peoples R China. [Zhang, F.; Asawatangtrakuldee, C.; Ban, Y.; Li, Q.; Liu, S.; Mao, Y.; Qian, S. J.; Wang, D.; Xu, Z.; Zou, W.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Avila, C.; Cabrera, A.; Chaparro Sierra, L. F.; Florez, C.; Gomez, J. P.; Gomez Moreno, B.; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia. [Godinovic, N.; Lelas, D.; Polic, D.; Puljak, I.] Univ Split, Fac Elect Engn Mech Engn & Naval Architecture, Split, Croatia. [Antunovic, Z.; Kovac, M.] Univ Split, Fac Sci, Split, Croatia. [Brigljevic, V.; Kadija, K.; Luetic, J.; Sudic, L.] Rudjer Boskovic Inst, Zagreb, Croatia. [Attikis, A.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.; Rykaczewski, H.] Univ Cyprus, Nicosia, Cyprus. 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M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Woehrmann, C.; Wolf, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Markou, A.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Tziaferi, E.; Sphicas, P.] Univ Athens, Athens, Greece. [Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Loukas, N.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hazi, A.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.; Bartok, M.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Bartok, M.; Makovec, A.; Raics, P.; Trocsanyi, Z. 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[Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Gan-guly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Mahakud, B.; Maity, M.; Majumder, G.; Mazumdar, K.; Mitra, S.; Mohanty, G. B.; Parida, B.; Sarkar, T.; Sudhakar, K.; Sur, N.; Sutar, B.; Wickramage, N.] Tata Inst Fundamental Res, Bombay 400005, Maharashtra, India. [Sharma, S.] IISER, Pune, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Ranieri, A.; Selvaggi, G.; Sharma, A.; Silvestris, L.; Venditti, R.; Verwilligen, P.] INFN Sez Bari, Bari, Italy. [Abbrescia, M.; Calabria, C.; Caputo, C.; Chhibra, S. S.; Cristella, L.; De Palma, M.; Miniello, G.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] INFN Sez Bologna, Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] INFN Sez Catania, Catania, Italy. [Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.; Viliani, L.] INFN Sez Firenze, Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.; Viliani, L.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] INFN Lab Nazl Frascati, Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Robutti, E.; Tosi, S.] INFN Sez Genova, Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] INFN Sez Milano Bicocca, Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Manzoni, R. A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.] INFN Sez Napoli, Naples, Italy. [Esposito, M.; Iorio, A. O. M.; Sciacca, C.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, I-85100 Potenza, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Carlin, R.; De Oliveira, A. Carvalho Antunes; Cheechia, P.; Dall'Osso, M.; Dorigo, T.; Dosselli, U.; Gasparini, F.; Gasparini, U.; Gonella, F.; Gozzelino, A.; Laeaprara, S.; Margoni, M.; Meneguzzo, A. T.; Miehelotto, M.; Pazzini, J.; Pozzobon, N.; Ronehese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] INFN Sezi Padova, Padua, Italy. [Bisello, D.; Carlin, R.; De Oliveira, A. Carvalho Antunes; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronehese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. Univ Trento, Trento, Italy. [Braghieri, A.; Gabusi, M.; Magnani, A.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Solestizi, L. Alunni] INFN Sezi Pavia, Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Solestizi, L. Alunni] Univ Pavia, I-27100 Pavia, Italy. [Solestizi, L. Alunni; Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariecia, P.; Mantovani, G.; Meniehelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] INFN Sezi Perugia, Perugia, Italy. [Solestizi, L. Alunni; Biasini, M.; Ciangottini, D.; Fano, L.; Lariecia, P.; Mantovani, G.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] INFN Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Soffi, L.; Traczyk, P.] INFN Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Micheli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Paeher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] INFN Sez Torino, Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Paeher, L.; Angioni, G. L. Pinna; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.; Zanetti, A.] INFN Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Sakharov, A.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. [Kim, H.; Kim, T. J.; Ryu, M. S.] Chonbuk Natl Univ, Jeonju, South Korea. [Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Lee, S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.; Vaitkus, J.] Vilnius Univ, Vilnius, Lithuania. [Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Ramirez Sanchez, G.; Sanchez-Hernandez, A.] Ctr Invest & Estudios Avanzados IPN, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Carpinteyro, S.; Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Mis-iura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varcla, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Finger, M.; Finger, M., Jr.; Tsamalaidze, Z.; Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Toriashvili, T.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Matveev, V.; Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Baskakov, A.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Myagkov, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Fac Phys, YU-11001 Belgrade, Serbia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Maestre, J. Alcaraz; Calvo, E.; Cerrada, M.; Llatas, M. Chamizo; Colino, N.; De la Cruz, B.; Peris, A. Delgado; Vazquez, D. Dominguez; Del Valle, A. Escalante; Bedoya, C. Fernandez; Ramos, J. P. Fernandez; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Lopez, O. Gonzalez; Lopez, S. Goy; Hernandez, J. M.; Josa, M. I.; De Martino, E. Navarro; Yzquierdo, A. Perez-Calero; Pelayo, J. Puerta; Olmeda, A. Quintario; Redondo, I.; Romero, L.; Soares, M. S.] CIEMAT, Madrid, Spain. [Albajar, C.; de Troceniz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Menendez, J. Fernandez; Folgueras, S.; Caballero, I. Gonzalez; Cortezon, E. Palencia; Garcia, J. M. Vizan] Univ Oviedo, Oviedo, Spain. [Cifuentes, J. A. Brochero; Cabrillo, I. J.; Calderon, A.; De Saa, J. R. Castineiras; Campderros, J. Duarte; Fernandez, M.; Gomez, G.; Graziano, A.; Virto, A. Lopez; Marco, J.; Marco, R.; Rivero, C. Martinez; Matorras, F.; Sanchez, F. J. Munoz; Gomez, J. Piedra; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Cortabitarte, R. Vilar] Univ Cantabria, CSIC, IFCA, E-39005 Santander, Spain. [Rabady, D.; Genchev, V.; Merlin, J. A.; Boudoul, G.; Pantaleo, F.; Hartmann, F.; Kassel, F.; Kornmayer, A.; Radogna, R.; Silvestris, L.; Giordano, F.; Gennai, S.; Marzocchi, B.; Di Guida, S.; Meola, S.; Paolucci, P.; Azzi, P.; Ciangottini, D.; Spiezia, A.; Donato, S.; Traczyk, P.; Finco, L.; Candelise, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Marrouche, J.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Tsirou, A.; Veres, G. I.; Wardle, N.; Wohri, H. K.; Zagozdzinska, A.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Buchmann, M. A.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marini, A. C.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Mohr, N.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Peruzzi, M.; Quittnat, M.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.; Weber, H. A.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinz-Mann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Salerno, D.; Taroni, S.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Ferro, C.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.; Wilken, R.] NTU, Taipei, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Onengut, G.; Ozdemir, K.; Polatoz, A.; Cerci, D. Sunar; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Albayrak, E. A.; Guelmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Guenaydin, Y. O.; Vardarh, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Phys & Technol Inst, Natl Sci Ctr, UA-310108 Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Gold-stein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Borzou, A.; Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Pastika, N.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; St. John, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Cutts, D.; Demiragli, Z.; Dhingra, N.; Ferapon-tov, A.; Garabedian, A.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Sagir, S.; Sinthuprasith, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chauhan, S.; Chertok, M.; Con-way, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Saltzberg, D.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Rikova, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Sumowidagdo, S.; Wei, H.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Kovalskyi, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wiirthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Justus, C.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Smith, J. G.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chle-bana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hoober-man, B.; Hu, Z.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Kwant, S.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Whitbeck, A.; Yang, F.; Yin, H.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Di Giovanni, G. P.; Field, R. D.; Fisher, M.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Kypreos, T.; Low, J. F.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rank, D.; Shchutska, L.; Snowball, M.; Sperka, D.; Wang, S. J.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Bhopatkar, V.; Hohlmann, M.; Kalakhety, H.; Mareskas-Palcek, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.] Univ Illinois, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khris-Tenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Sen, S.; Snyder, C.; Tan, P.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Nash, K.; Osherson, M.; Swartz, M.; Xiao, M.; Xin, Y.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Gray, J.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Chakaberia, I.; Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Skhirtladze, N.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Pedro, K.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Baty, A.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. 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Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Trovato, M.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Lynch, S.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Pearson, T.; Planer, M.; Ruchti, R.; Smith, G.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Quan, X.; Saka, H.; Land, D. 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I.] Eotvos Lorand Univ, Budapest, Hungary. [Bhowmik, S.; Maity, M.; Sarkar, T.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Plasma Phys Res Ctr, Sci & Res Branch, Tehran, Iran. [Gele, D.; Androsov, K.; Ciocci, M. A.; Grippo, M. T.; Squillacioti, P.] Univ Siena, I-53100 Siena, Italy. [Ali, M. A. B. Md] Int Islamic Univ Malaysia, Kuala Lumpur, Malaysia. [Heredia-de La Cruz, I.] Consejo Natl Ciencia & Tecnol, Mexico City, DF, Mexico. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst, Moscow 115409, Russia. [Dubinin, M.] CALTECH, Pasadena, CA 91125 USA. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Rolandi, G.] Scuola Normale & Sez INFN, Pisa, Italy. [Zagozdzinska, A.] Warsaw Univ, Inst Elect Syst, Warsaw, Poland. [Starodumov, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.] Gaziosmanpasa Univ, Tokat, Turkey. [Kangal, E. E.] Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. [Cerci, D. Sunar] Adiyaman Univ, Adiyaman, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, T.] Yildiz Tech Univ, Istanbul, Turkey. [Guenaydin, Y. O.] Kahramanmaras Sutcu Imam Univ, TR-46050 Kahramanmaras, Turkey. [Newbold, D. M.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. 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RI Ruiz, Alberto/E-4473-2011; Petrushanko, Sergey/D-6880-2012; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Paulini, Manfred/N-7794-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Dremin, Igor/K-8053-2015; ciocci, maria agnese /I-2153-2015; Ligabue, Franco/F-3432-2014; Sguazzoni, Giacomo/J-4620-2015; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Azarkin, Maxim/N-2578-2015; Chinellato, Jose Augusto/I-7972-2012; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Sznajder, Andre/L-1621-2016; Vilela Pereira, Antonio/L-4142-2016; Paganoni, Marco/A-4235-2016; Ferguson, Thomas/O-3444-2014; de Jesus Damiao, Dilson/G-6218-2012; Dogra, Sunil /B-5330-2013; Leonidov, Andrey/M-4440-2013; Calvo Alamillo, Enrique/L-1203-2014; Hernandez Calama, Jose Maria/H-9127-2015; Cerrada, Marcos/J-6934-2014; Andreev, Vladimir/M-8665-2015; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Novaes, Sergio/D-3532-2012; Della Ricca, Giuseppe/B-6826-2013; Dudko, Lev/D-7127-2012; Moraes, Arthur/F-6478-2010; Manganote, Edmilson/K-8251-2013; KIM, Tae Jeong/P-7848-2015; Menasce, Dario/A-2168-2016; Vinogradov, Alexey/O-2375-2015; VARDARLI, Fuat Ilkehan/B-6360-2013; Lokhtin, Igor/D-7004-2012; Cakir, Altan/P-1024-2015; Montanari, Alessandro/J-2420-2012; Matorras, Francisco/I-4983-2015; Gennai, Simone/P-2880-2015; TUVE', Cristina/P-3933-2015; OI Androsov, Konstantin/0000-0003-2694-6542; Viliani, Lorenzo/0000-0002-1909-6343; ROMERO ABAD, DAVID/0000-0001-5088-9301; ORTONA, Giacomo/0000-0001-8411-2971; Gallinaro, Michele/0000-0003-1261-2277; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; ciocci, maria agnese /0000-0003-0002-5462; Ligabue, Franco/0000-0002-1549-7107; Sharma, Ram Krishna/0000-0003-1181-1426; Preiato, Federico/0000-0003-2996-4105; HSIUNG, YEE/0000-0003-4801-1238; Boccali, Tommaso/0000-0002-9930-9299; Gerosa, Raffaele/0000-0001-8359-3734; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Sguazzoni, Giacomo/0000-0002-0791-3350; Rizzi, Andrea/0000-0002-4543-2718; Martinez Ruiz del Arbol, Pablo/0000-0002-7737-5121; Demaria, Natale/0000-0003-0743-9465; Ciulli, Vitaliano/0000-0003-1947-3396; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Chinellato, Jose Augusto/0000-0002-3240-6270; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Seixas, Joao/0000-0002-7531-0842; Sznajder, Andre/0000-0001-6998-1108; Vilela Pereira, Antonio/0000-0003-3177-4626; Paganoni, Marco/0000-0003-2461-275X; Ferguson, Thomas/0000-0001-5822-3731; de Jesus Damiao, Dilson/0000-0002-3769-1680; Calvo Alamillo, Enrique/0000-0002-1100-2963; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Cerrada, Marcos/0000-0003-0112-1691; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; Dudko, Lev/0000-0002-4462-3192; Moraes, Arthur/0000-0002-5157-5686; KIM, Tae Jeong/0000-0001-8336-2434; Menasce, Dario/0000-0002-9918-1686; Montanari, Alessandro/0000-0003-2748-6373; Matorras, Francisco/0000-0003-4295-5668; TUVE', Cristina/0000-0003-0739-3153; Reis, Thomas/0000-0003-3703-6624; Luukka, Panja/0000-0003-2340-4641; Jacob, Jeson/0000-0001-6895-5493 FU Austrian Federal Ministry of Science, Research and Economy; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; Brazilian Funding Agency (CNPq); Brazilian Funding Agency (CAPES); Brazilian Funding Agency (FAPERJ); Brazilian Funding Agency (FAPESP); Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research; Estonian Research Council [IUT23-4, IUT23-6]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules / CNRS; Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; Bundesministerium fur Bildung und Forschung; Deutsche Forschungsgemeinschaft; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation; National Innovation Office, Hungary; Department of Atomic Energy; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Ministry of Science, ICT and Future Planning; National Research Foundation (NRF), Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education; University of Malaya (Malaysia); Mexican Funding Agency (CINVESTAV); Mexican Funding Agency (CONACYT); Mexican Funding Agency (SEP); Mexican Funding Agency (UASLP-FAI); Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion; Desarrollo e Innovacion; Programa Consolider-Ingenio, Spain; Swiss Funding Agency (ETH Board); Swiss Funding Agency (ETH Zurich); Swiss Funding Agency (PSI); Swiss Funding Agency (SNF); Swiss Funding Agency (UniZH); Swiss Funding Agency (Canton Zurich); Swiss Funding Agency (SER); Ministry of Science and Technology, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine; State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, U.K.; US Department of Energy; US National Science Foundation; Marie-Curie program; European Research Council (European Union); EPLANET (European Union); Leventis Foundation; A.P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS program of the Foundation for Polish Science; European Union, Regional Development Fund; Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR project (Italy) [20108T4XTM]; Thalis program; Aristeia program; EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses.; Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via IUT23-4 and IUT23-6 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules / CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Ministry of Science, ICT and Future Planning, and National Research Foundation (NRF), Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine, and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, U.K.; the US Department of Energy, and the US National Science Foundation.; Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A.P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF; and the National Priorities Research Program by Qatar National Research Fund. NR 123 TC 35 Z9 35 U1 15 U2 62 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD OCT 22 PY 2015 IS 10 AR 144 DI 10.1007/JHEP10(2015)144 PG 52 WC Physics, Particles & Fields SC Physics GA CU5GS UT WOS:000363560700001 ER PT J AU Bethkenhagen, M Cebulla, D Redmer, R Hamel, S AF Bethkenhagen, Mandy Cebulla, Daniel Redmer, Ronald Hamel, Sebastien TI Superionic Phases of the 1:1 Water-Ammonia Mixture SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID INITIO MOLECULAR-DYNAMICS; ALGORITHM; PRESSURE; CRYSTAL; METALS; ICES AB We report four structures for the 1:1 water ammonia mixture showing superionic behavior at high temperature with the space groups P4/nmm, Ima2, Pma2, and Pm, which have been identified from evolutionary random structure search calculations at 0 K. Analyzing the respective pair distribution functions and diffusive properties the superionic phase is found to be stable in a temperature range between 1000 and 6000 K for pressures up to 800 GPa. We propose a high-pressure phase diagram of the water ammonia mixture for the first time and compare the self-diffusion coefficients in the mixture to the ones found in water and ammonia. Finally, possible implications on the interior structure of the giant planets Uranus and Neptune are discussed. C1 [Bethkenhagen, Mandy; Cebulla, Daniel; Redmer, Ronald] Univ Rostock, Inst Phys, D-18059 Rostock, Germany. [Bethkenhagen, Mandy; Hamel, Sebastien] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Hamel, S (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave L-413, Livermore, CA 94550 USA. EM hamel2@llnl.gov FU DFG [SFB 652]; U.S. Department of Energy at the Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; NASA Outer Planet Research program [NNH12AU44I] FX We thank Andreas Becker, Martin French, Clemens Kellermann, Edmund R Meyer, Manuel Schottler, and Nadine Nettelmann for helpful discussions. This work was supported by the DFG within the SFB 652, the U.S. Department of Energy at the Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344, and the NASA Outer Planet Research program (grant no. NNH12AU44I). We are grateful to the North-German Supercomputing Alliance (HLRN) and the ITMZ of the University of Rostock for computation time. NR 49 TC 3 Z9 3 U1 2 U2 13 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD OCT 22 PY 2015 VL 119 IS 42 BP 10582 EP 10588 DI 10.1021/acs.jpca.5b07854 PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CV0DE UT WOS:000363916800014 PM 26390374 ER PT J AU Ankowski, AM Benhar, O Coloma, P Huber, P Jen, CM Mariani, C Meloni, D Vagnoni, E AF Ankowski, A. M. Benhar, O. Coloma, P. Huber, P. Jen, C. -M. Mariani, C. Meloni, D. Vagnoni, E. TI Comparison of the calorimetric and kinematic methods of neutrino energy reconstruction in disappearance experiments SO PHYSICAL REVIEW D LA English DT Article ID LINE-EXPERIMENT-SIMULATOR; OSCILLATION EXPERIMENTS; SPECTRAL-FUNCTION; LEPTON SCATTERING; CROSS-SECTIONS; GEV REGION; DETECTOR; NUCLEI; MODEL AB To be able to achieve their physics goals, future neutrino-oscillation experiments will need to reconstruct the neutrino energy with very high accuracy. In this work, we analyze how the energy reconstruction may be affected by realistic detection capabilities, such as energy resolutions, efficiencies, and thresholds. This allows us to estimate how well the detector performance needs to be determined a priori in order to avoid a sizable bias in the measurement of the relevant oscillation parameters. We compare the kinematic and calorimetric methods of energy reconstruction in the context of two nu(mu) -> nu(mu) disappearance experiments operating in different energy regimes. For the calorimetric reconstruction method, we find that the detector performance has to be estimated with an O(10%) accuracy to avoid a significant bias in the extracted oscillation parameters. On the other hand, in the case of kinematic energy reconstruction, we observe that the results exhibit less sensitivity to an overestimation of the detector capabilities. C1 [Ankowski, A. M.; Benhar, O.; Huber, P.; Jen, C. -M.; Mariani, C.] Virginia Tech, Ctr Neutrino Phys, Blacksburg, VA 24061 USA. [Benhar, O.] Ist Nazl Fis Nucl, I-00185 Rome, Italy. [Benhar, O.] Univ Roma La Sapienza, Dept Phys, I-00185 Rome, Italy. [Coloma, P.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Meloni, D.; Vagnoni, E.] Ist Nazl Fis Nucl, I-00146 Rome, Italy. [Meloni, D.; Vagnoni, E.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. RP Ankowski, AM (reprint author), Virginia Tech, Ctr Neutrino Phys, Blacksburg, VA 24061 USA. EM ankowski@vt.edu RI Mariani, Camillo/J-6070-2015; OI Mariani, Camillo/0000-0003-3284-4681; Coloma, Pilar/0000-0002-1164-9900; Ankowski, Artur/0000-0003-4073-8686 FU National Science Foundation [PHY-1352106]; Fermi Research Alliance [DE-AC02-07CH11359]; U.S. Department of Energy; European Union [PITN-GA-2011-289442]; U.S. Department of Energy [DE-SC0013632]; MIUR (Italy) [RBFR10O36O]; Center for Neutrino Physics of Virginia Tech FX The work of A. M. A., C. M. J., and C. M. was supported by the National Science Foundation under Grant No. PHY-1352106. Fermilab is operated by the Fermi Research Alliance under Contract No. DE-AC02-07CH11359 with the U.S. Department of Energy. P. C. acknowledges partial support from the European Union FP7 ITN INVISIBLES (Marie Curie Actions, Grant No. PITN-GA-2011-289442). P. H. is supported by the U.S. Department of Energy under Contract No. DE-SC0013632. The work of D. M. and E. V. was supported by MIUR (Italy) under the program "Futuro in Ricerca 2010 (RBFR10O36O)." E. V. acknowledges the hospitality and support from Center for Neutrino Physics of Virginia Tech. NR 97 TC 7 Z9 7 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD OCT 22 PY 2015 VL 92 IS 7 AR 073014 DI 10.1103/PhysRevD.92.073014 PG 16 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CU0VS UT WOS:000363237600004 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Ochesanu, S Rougny, R Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Van Parijs, I Barria, P Caillol, C Clerbaux, B De Lentdecker, G Delannoy, H Fasanella, G Favart, L Gay, APR Grebenyuk, A Lenzi, T Leonard, A Maerschalk, T Marinov, A Pernie, L Randle-conde, A Reis, T Seva, T Vander Velde, C Vanlaer, P Yonamine, R Zenoni, F Zhang, F Beernaert, K Benucci, L Cimmino, A Crucy, S Dobur, D Fagot, A Garcia, G Gul, M Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Salva, S Sigamani, M Strobbe, N Tytgat, M Van Driessche, W Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bondu, O Brochet, S Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Mertens, A Nuttens, C Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Beliy, N Hammad, GH Alda, WL Alves, GA Brito, L Martins, MC Hamer, M Hensel, C Herrera, CM Moraes, A Pol, ME Teles, PR Das Chagas, EBB Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DDJ Martins, CDO De Souza, SF Guativa, LMH Malbouisson, H Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Ahuja, S Bernardes, CA Santos, ADS Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Moon, CS Novaes, SF Padula, SS Abad, DR Vargas, JCR Aleksandrov, A Genchev, V Hadjiiska, R Iaydjiev, P Piperov, S Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Ahmad, M Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Plestina, R Romeo, F Shaheen, SM Tao, J Wang, C Wang, Z Zhang, H Zou, W Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Xu, Z Zou, W Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Polic, D Puljak, I Cipriano, PMR Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Micanovic, S Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Bodlak, M Finger, M Finger, M El-khateeb, E Elkafrawy, T Mohamed, A Salama, E Calpas, B Kadastik, M Murumaa, M Raidal, M Tiko, A Veelken, C Eerola, P Pekkanen, J Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Talvitie, J Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Favaro, C Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Machet, M Malcles, J Rander, J Rosowsky, A Titov, M Zghiche, A Antropov, I Baffioni, S Beaudette, F Busson, P Cadamuro, L Chapon, E Charlot, C Dahms, T Davignon, O Filipovic, N Florent, A de Cassagnac, RG Lisniak, S Mastrolorenzo, L Mine, P Naranjo, IN Nguyen, M Ochando, C Ortona, G Paganini, P Regnard, S Salerno, R Sauvan, JB Sirois, Y Strebler, T Yilmaz, Y Zabi, A Agram, JL Andrea, J Aubin, A Bloch, D Brom, JM Buttignol, M Chabert, EC Chanon, N Collard, C Conte, E Coubez, X Fontaine, JC Gele, D Goerlach, U Goetzmann, C Le Bihan, AC Merlin, JA Skovpen, K Van Hove, P Gadrat, S Beauceron, S Bernet, C Boudoul, G Bouvier, E Montoya, CAC Chasserat, J Chierici, R Contardo, D Courbon, B Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Lagarde, F Laktineh, IB Lethuillier, M Mirabito, L Pequegnot, AL Perries, S Alvarez, JDR Sabes, D Sgandurra, L Sordini, V Vander Donckt, M Verdier, P Viret, S Xiao, H Toriashvili, T Tsamalaidze, Z Autermann, C Beranek, S Edelhoff, M Feld, L Heister, A Kiesel, MK Klein, K Lipinski, M Ostapchuk, A Preuten, M Raupach, F Schael, S Schulte, JF Verlage, T Weber, H Wittmer, B Zhukov, V Ata, M Brodski, M Dietz-Laursonn, E Duchardt, D Endres, M Erdmann, M Erdweg, S Esch, T Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Millet, P Olschewski, M Padeken, K Papacz, P Pook, T Radziej, M Reithler, H Rieger, M Scheuch, F Sonnenschein, L Teyssier, D Thuer, S Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Hoehle, F Kargoll, B Kress, T Kuessel, Y Kunsken, A Lingemann, J Nehrkorn, A Nowack, A Nugent, IM Pistone, C Pooth, O Stahl, A Martin, MA Asin, I Bartosik, N Behnke, O Behrens, U Bell, AJ Borras, K Burgmeier, A Cakir, A Calligaris, L Campbell, A Choudhury, S Costanza, F Pardos, CD Dolinska, G Dooling, S Dorland, T Eckerlin, G Eckstein, D Eichhorn, T Flucke, G Gallo, E Garcia, JG Geiser, A Gizhko, A Gunnellini, P Hauk, J Hempel, M Jung, H Kalogeropoulos, A Karacheban, O Kasemann, M Katsas, P Kieseler, J Kleinwort, C Korol, I Lange, W Leonard, J Lipka, K Lobanov, A Lohmann, W Mankel, R Marfin, I Melzer-Pellmann, IA Meyer, AB Mittag, G Mnich, J Mussgiller, A Naumann-Emme, S Nayak, A Ntomari, E Perrey, H Pitzl, D Placakyte, R Raspereza, A Roland, B Sahin, MO Saxena, P Schoerner-Sadenius, T Schroder, M Seitz, C Spannagel, S Trippkewitz, KD Walsh, R Wissing, C Blobel, V Vignali, MC Draeger, AR Erfle, J Garutti, E Goebel, K Gonzalez, D Gorner, M Haller, J Hoffmann, M Hoing, RS 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Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Sturdy, J. Belknap, D. A. Carlsmith, D. Cepeda, M. Christian, A. Dasu, S. Dodd, L. Duric, S. Friis, E. Gomber, B. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Lanaro, A. Levine, A. Long, K. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Ruggles, T. Sarangi, T. Savin, A. Sharma, A. Smith, N. Smith, W. H. Taylor, D. Woods, N. CA CMS Collaboration TI Limits on the Higgs boson lifetime and width from its decay to four charged leptons SO PHYSICAL REVIEW D LA English DT Article ID ATLAS DETECTOR; FINAL-STATES; LHC; SYMMETRIES; MODEL; MASS AB Constraints on the lifetime and width of the Higgs boson are obtained from H -> ZZ -> 4l events using data recorded by the CMS experiment during the LHC run 1 with an integrated luminosity of 5.1 and 19.7 fb(-1) at a center-of-mass energy of 7 and 8 TeV, respectively. The measurement of the Higgs boson lifetime is derived from its flight distance in the CMS detector with an upper bound of tau(H) < 1.9 x 10(-13) s at the 95% confidence level (C.L.), corresponding to a lower bound on the width of Gamma(H) > 3.5 x 10(-9) MeV. The measurement of the width is obtained from an off-shell production technique, generalized to include anomalous couplings of the Higgs boson to two electroweak bosons. From this measurement, a joint constraint is set on the Higgs boson width and a parameter f(Lambda Q) that expresses an anomalous coupling contribution as an on-shell cross-section fraction. The limit on the Higgs boson width is Gamma(H) < 46 MeV with f(Lambda Q) unconstrained and Gamma(H) < 26 MeV for f(Lambda Q) = 0 at the 95% C.L. The constraint f(Lambda Q) < 3.8 x 10(-3) at the 95% C.L. is obtained for the expected standard model Higgs boson width. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hartl, C.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Knuenz, V.; Koenig, A.; Krammer, M.; Kraetschmer, I.; Liko, D.; Matsushita, T.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, H.; Schieck, J.; Schoefbeck, R.; Strauss, J.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] Inst Hochenergiephys OeAW, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. [Alderweireldt, S.; Cornelis, T.; De Wolf, E. A.; Janssen, X.; Knutsson, A.; Lauwers, J.; Luyckx, S.; Ochesanu, S.; Rougny, R.; Van De Klundert, M.; Van Haevermaet, H.; Van Mechelen, P.; Van Remortel, N.; Van Spilbeeck, A.] Univ Antwerp, B-2020 Antwerp, Belgium. [Abu Zeid, S.; Blekman, F.; D'Hondt, J.; Daci, N.; De Bruyn, I.; Deroover, K.; Heracleous, N.; Keaveney, J.; Lowette, S.; Moreels, L.; Olbrechts, A.; Python, Q.; Strom, D.; Tavernier, S.; Van Doninck, W.; Van Mulders, P.; Van Onsem, G. P.; Van Parijs, I.] Vrije Univ Brussel, Brussels, Belgium. [Barria, P.; Caillol, C.; Clerbaux, B.; De Lentdecker, G.; Delannoy, H.; Fasanella, G.; Favart, L.; Gay, A. P. R.; Grebenyuk, A.; Lenzi, T.; Leonard, A.; Maerschalk, T.; Marinov, A.; Pernie, L.; Randle-conde, A.; Reis, T.; Seva, T.; Vander Velde, C.; Vanlaer, P.; Yonamine, R.; Zenoni, F.; Zhang, F.] Univ Libre Bruxelles, Brussels, Belgium. [Beernaert, K.; Benucci, L.; Cimmino, A.; Crucy, S.; Dobur, D.; Fagot, A.; Garcia, G.; Gul, M.; Mccartin, J.; Rios, A. A. Ocampo; Poyraz, D.; Ryckbosch, D.; Salva, S.; Sigamani, M.; Strobbe, N.; Tytgat, M.; Van Driessche, W.; Yazgan, E.; Zaganidis, N.] Univ Ghent, B-9000 Ghent, Belgium. [Basegmez, S.; Beluffi, C.; Bondu, O.; Brochet, S.; Bruno, G.; Castello, R.; Caudron, A.; Ceard, L.; Da Silveira, G. G.; Delaere, C.; Favart, D.; Forthomme, L.; Giammanco, A.; Hollar, J.; Jafari, A.; Jez, P.; Komm, M.; Lemaitre, V.; Mertens, A.; Nuttens, C.; Perrini, L.; Pin, A.; Piotrzkowski, K.; Popov, A.; Quertenmont, L.; Selvaggi, M.; Marono, M. Vidal] Catholic Univ Louvain, Louvain, Belgium. [Beliy, N.; Hammad, G. H.] Univ Mons, B-7000 Mons, Belgium. [Alda Junior, W. L.; Alves, G. A.; Brito, L.; Correa Martins Junior, M.; Hamer, M.; Hensel, C.; Mora Herrera, C.; Moraes, A.; Pol, M. E.; Rebello Teles, P.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. [Belchior Batista Das Chagas, E.; Carvalho, W.; Chinellato, J.; Custodio, A.; Da Costa, E. M.; De Jesus Damiao, D.; De Oliveira Martins, C.; Fonseca De Souza, S.; Huertas Guativa, L. M.; Malbouisson, H.; Matos Figueiredo, D.; Mundim, L.; Nogima, H.; Prado Da Silva, W. L.; Santoro, A.; Sznajder, A.; Tonelli Manganote, E. J.; Vilela Pereira, A.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Chinellato, J.; Tonelli Manganote, E. J.; Ahuja, S.; Dogra, S.; Moon, C. S.; Novaes, S. F.; Padula, Sandra S.; Romero Abad, D.; Ruiz Vargas, J. C.] Univ Estadual Paulista, Sao Paulo, Brazil. [Bernardes, C. A.; De Souza Santos, A.; Gregores, E. M.; Mercadante, P. G.] Univ Fed ABC, Sao Paulo, Brazil. [Aleksandrov, A.; Genchev, V.; Hadjiiska, R.; Iaydjiev, P.; Piperov, S.; Rodozov, M.; Stoykova, S.; Sultanov, G.; Vutova, M.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy, Sofia, Bulgaria. [Dimitrov, A.; Glushkov, I.; Litov, L.; Pavlov, B.; Petkov, P.] Univ Sofia, BU-1126 Sofia, Bulgaria. [Fernandez Perez Tomei, T. R.; Ahmad, M.; Bian, J. G.; Chen, G. M.; Chen, H. S.; Chen, M.; Cheng, T.; Du, R.; Jiang, C. H.; Plestina, R.; Romeo, F.; Shaheen, S. M.; Tao, J.; Wang, C.; Wang, Z.; Zhang, H.] Inst High Energy Phys, Beijing 100039, Peoples R China. [Zhang, F.; Asawatangtrakuldee, C.; Ban, Y.; Li, Q.; Liu, S.; Mao, Y.; Qian, S. J.; Wang, D.; Xu, Z.; Zou, W.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Avila, C.; Cabrera, A.; Chaparro Sierra, L. F.; Florez, C.; Gomez, J. P.; Gomez Moreno, B.; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia. [Godinovic, N.; Lelas, D.; Polic, D.; Puljak, I.; Cipriano, P. M. Ribeiro] Univ Split, Fac Elect Engn Mech Engn & Naval Architecture, Split, Croatia. [Antunovic, Z.; Kovac, M.] Univ Split, Fac Sci, Split, Croatia. [Brigljevic, V.; Kadija, K.; Luetic, J.; Micanovic, S.; Sudic, L.] Rudjer Boskovic Inst, Zagreb *0000, Croatia. [Attikis, A.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.; Rykaczewski, H.] Univ Cyprus, CY-1678 Nicosia, Cyprus. [Bodlak, M.; Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic. [El-khateeb, E.; Elkafrawy, T.; Mohamed, A.; Salama, E.] Acad Sci Res & Technol Arab Republ Egypt, Egyptian Network High Energy Phys, Cairo, Egypt. [Giammanco, A.; Calpas, B.; Kadastik, M.; Murumaa, M.; Raidal, M.; Tiko, A.; Veelken, C.] NICPB, Tallinn, Estonia. [Eerola, P.; Pekkanen, J.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Harkonen, J.; Karimaki, V.; Kinnunen, R.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Talvitie, J.; Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Couderc, F.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Favaro, C.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Machet, M.; Malcles, J.; Rander, J.; Rosowsky, A.; Titov, M.; Zghiche, A.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Plestina, R.; Antropov, I.; Baffioni, S.; Beaudette, F.; Busson, P.; Cadamuro, L.; Chapon, E.; Charlot, C.; Dahms, T.; Davignon, O.; Filipovic, N.; Florent, A.; de Cassagnac, R. Granier; Lisniak, S.; Mastrolorenzo, L.; Mine, P.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Ortona, G.; Paganini, P.; Regnard, S.; Salerno, R.; Sauvan, J. B.; Sirois, Y.; Strebler, T.; Yilmaz, Y.; Zabi, A.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Beluffi, C.; Agram, J. -L.; Andrea, J.; Aubin, A.; Bloch, D.; Brom, J. -M.; Buttignol, M.; Chabert, E. C.; Chanon, N.; Collard, C.; Conte, E.; Coubez, X.; Fontaine, J. -C.; Gele, D.; Goerlach, U.; Goetzmann, C.; Le Bihan, A. -C.; Merlin, J. A.; Skovpen, K.; Van Hove, P.] Univ Haute Alsace Mulhouse, Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, CNRS,IN2P3, Strasbourg, France. [Gadrat, S.] CNRS, Ctr Calcul, IN2P3, Villeurbanne, France. [Beauceron, S.; Bernet, C.; Boudoul, G.; Bouvier, E.; Montoya, C. A. Carrillo; Chasserat, J.; Chierici, R.; Contardo, D.; Courbon, B.; Depasse, P.; El Mamouni, H.; Fan, J.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Lagarde, F.; Laktineh, I. B.; Lethuillier, M.; Mirabito, L.; Pequegnot, A. L.; Perries, S.; Alvarez, J. D. Ruiz; Sabes, D.; Sgandurra, L.; Sordini, V.; Vander Donckt, M.; Verdier, P.; Viret, S.; Xiao, H.] Univ Lyon 1, CNRS, Inst Phys Nucl Lyon, IN2P3, F-69622 Villeurbanne, France. [Toriashvili, T.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Toriashvili, T.; Tsamalaidze, Z.] Tbilisi State Univ, GE-380086 Tbilisi, Rep of Georgia. [Autermann, C.; Beranek, S.; Edelhoff, M.; Feld, L.; Heister, A.; Kiesel, M. K.; Klein, K.; Lipinski, M.; Ostapchuk, A.; Preuten, M.; Raupach, F.; Schael, S.; Schulte, J. F.; Verlage, T.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Phys Inst 1, Aachen, Germany. [Ata, M.; Brodski, M.; Dietz-Laursonn, E.; Duchardt, D.; Endres, M.; Erdmann, M.; Erdweg, S.; Esch, T.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Millet, P.; Olschewski, M.; Padeken, K.; Papacz, P.; Pook, T.; Radziej, M.; Reithler, H.; Rieger, M.; Scheuch, F.; Sonnenschein, L.; Teyssier, D.; Thueer, S.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Kuensken, A.; Lingemann, J.; Nehrkorn, A.; Nowack, A.; Nugent, I. M.; Pistone, C.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B 3, Aachen, Germany. [Martin, M. Aldaya; Asin, I.; Bartosik, N.; Behnke, O.; Behrens, U.; Bell, A. J.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. Diez; Dolinska, G.; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Gallo, E.; Garcia, J. Garay; Geiser, A.; Gizhko, A.; Gunnellini, P.; Hauk, J.; Hempel, M.; Jung, H.; Kalogeropoulos, A.; Karacheban, O.; Kasemann, M.; Katsas, P.; Kieseler, J.; Kleinwort, C.; Korol, I.; Lange, W.; Leonard, J.; Lipka, K.; Lobanov, A.; Lohmann, W.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mittag, G.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Nayak, A.; Ntomari, E.; Perrey, H.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Roland, B.; Sahin, M. Oe.; Saxena, P.; Schoerner-Sadenius, T.; Schroeder, M.; Seitz, C.; Spannagel, S.; Trippkewitz, K. D.; Walsh, R.; Wissing, C.] DESY, Hamburg, Germany. [Blobel, V.; Vignali, M. Centis; Draeger, A. R.; Erfle, J.; Garutti, E.; Goebel, K.; Gonzalez, D.; Goerner, M.; Haller, J.; Hoffmann, M.; Hoeing, R. S.; Junkes, A.; Klanner, R.; Kogler, R.; Lapsien, T.; Lenz, T.; Marchesini, I.; Marconi, D.; Nowatschin, D.; Ott, J.; Pantaleo, F.; Peiffer, T.; Perieanu, A.; Pietsch, N.; Poehlsen, J.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schwandt, J.; Seidel, M.; Sola, V.; Stadie, H.; Steinbrueck, G.; Tholen, H.; Troendle, D.; Usai, E.; Vanelderen, L.; Vanhoefer, A.] Yerevan Phys Inst, Hamburg, Germany. [Akbiyik, M.; Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; Colombo, F.; De Boer, W.; Descroix, A.; Dierlamm, A.; Fink, S.; Frensch, F.; Giffels, M.; Gilbert, A.; Hartmann, F.; Heindl, S. M.; Husemann, U.; Katkov, I.; Kornmayer, A.; Pardo, P. Lobelle; Maier, B.; Mildner, H.; Mozer, M. U.; Mueller, T.; Mueller, Th; Plagge, M.; Quast, G.; Rabbertz, K.; Roecker, S.; Roscher, F.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weber, M.; Weiler, T.; Woehrmann, C.; Wolf, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Tziaferi, E.; Sphicas, P.] Univ Athens, Athens, Greece. [Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Loukas, N.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hazi, A.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.; Bartok, M.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Bartok, M.; Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Mal, P.; Mandal, K.; Sahoo, N.; Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Bansal, S.; Beri, S. B.; Bhatnagar, V.; Chawla, R.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, A.; Kaur, M.; Kumar, R.; Mehta, A.; Mittal, M.; Singh, J. B.; Walia, G.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Bhardwaj, A.; Choudhary, B. C.; Garg, R. B.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Nishu, N.; Ranjan, K.; Sharma, R.; Sharma, V.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dey, S.; Dutta, S.; Jain, Sa; Majumdar, N.; Modak, A.; Mondal, K.; Mukherjee, S.; Mukhopadhyay, S.; Roy, A.; Roy, D.; Chowdhury, S. Roy; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Chudasama, R.; Dutta, D.; Jha, V.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Mahakud, B.; Maity, M.; Majumder, G.; Mazumdar, K.; Mitra, S.; Mohanty, G. B.; Parida, B.; Sarkar, T.; Sudhakar, K.; Sur, N.; Sutar, B.; Wickramage, N.] Tata Inst Fundamental Res, Bombay 400005, Maharashtra, India. [Chauhan, S.; Dube, S.; Sharma, S.] Indian Inst Sci Educ & Res IISER, Pune, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Ranieri, A.; Selvaggi, G.; Silvestris, L.; Venditti, R.; Verwilligen, P.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Calabria, C.; Caputo, C.; Chhibra, S. S.; Cristella, L.; De Palma, M.; Miniello, G.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Battilana, C.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. CSFNSM, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.; Viliani, L.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.; Viliani, L.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Monge, M. R.; Tosi, S.] Univ Genoa, Genoa, Italy. [Brianza, L.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Manzoni, R. A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.; Thyssen, F.] Ist Nazl Fis Nucl, Sez Napoli, Rome, Italy. [Esposito, M.; Iorio, A. O. M.; Sciacca, C.] Univ Naples Federico II, Rome, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, Rome, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; De Oliveira, A. Carvalho Antunes; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Dosselli, U.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Trento, Italy. [Abdulsalam, A.; Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; De Oliveira, A. Carvalho Antunes; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Trento, Italy. [Kanishchev, K.] Univ Trento, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Montagna, P.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Solestizi, L. Alunni; Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Solestizi, L. Alunni; Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fedi, G.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Micheli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Musich, M.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, Novara, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Novara, Italy. [Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Sakharov, A.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. [Cifuentes, J. A. Brochero; Kim, H.; Kim, T. J.; Ryu, M. S.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Lee, S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, H.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.; Vaitkus, J.] Vilnius Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan; Yusli, M. N.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Carpinteyro, S.; Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Leonardo, N.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Finger, M.; Finger, M., Jr.; Tsamalaidze, Z.; Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Matveev, V.; Andreev, Yu; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Bylinkin, A.; Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Baskakov, A.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Myagkov, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.; Albajar, C.] CIEMAT, Madrid, Spain. [de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, E-28049 Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; De Castro Manzano, P.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Merlin, J. A.; Lingemann, J.; Pantaleo, F.; Hartmann, F.; Kornmayer, A.; Mohanty, A. K.; Silvestris, L.; Battilana, C.; Marzocchi, B.; Di Guida, S.; Meola, S.; Paolucci, P.; Azzi, P.; Dall'Osso, M.; Zucchetta, A.; Ciangottini, D.; Donato, S.; D'imperio, G.; Traczyk, P.; Arcidiacono, R.; Finco, L.; Candelise, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Zagozdzinska, A.; Zeuner, W. D.; Ulmer, K. A.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Buchmann, M. A.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marini, A. C.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Peruzzi, M.; Quittnat, M.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Ferro, C.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartek, R.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.] NTU, Taipei, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Dept Phys, Fac Sci, Bangkok, Thailand. [Adiguzel, A.; Cerci, S.; Dozen, C.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Tali, B.; Topakli, H.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Albayrak, E. A.; Guelmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Thomas, L.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Cripps, N.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.; Cole, J. E.; Hobson, P. R.] Univ London Imperial Coll Sci Technol & Med, London, England. [Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Pastika, N.; Charaf, O.] Baylor Univ, Waco, TX 76798 USA. [Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL 35487 USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Cutts, D.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Sagir, S.; Sinthuprasith, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Justus, C.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Smith, J. G.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY 14853 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Hu, Z.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Kwan, S.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Weber, H. A.; Whitbeck, A.; Yang, F.; Yin, H.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Di Giovanni, G. P.; Field, R. D.; Fisher, M.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Low, J. F.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rank, D.; Rossin, R.; Shchutska, L.; Snowball, M.; Sperka, D.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL 32611 USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Bhopatkar, V.; Hohlmann, M.; Kalakhety, H.; Mareskas-palcek, D.; Roy, T.; Yumiceva, F.; Adams, M. R.] Florida Inst Technol, Melbourne, FL 32901 USA. [Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.] Univ Illinois, Chicago, IL 60607 USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tan, P.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA 52242 USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Osherson, M.; Roskes, J.; Sarica, U.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD 21218 USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Gray, J.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Chakaberia, I.; Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. 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RI Menasce, Dario/A-2168-2016; Paganoni, Marco/A-4235-2016; de Jesus Damiao, Dilson/G-6218-2012; Dogra, Sunil /B-5330-2013; Leonidov, Andrey/M-4440-2013; Calvo Alamillo, Enrique/L-1203-2014; Hernandez Calama, Jose Maria/H-9127-2015; Cerrada, Marcos/J-6934-2014; Andreev, Vladimir/M-8665-2015; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Novaes, Sergio/D-3532-2012; Della Ricca, Giuseppe/B-6826-2013; Sguazzoni, Giacomo/J-4620-2015; Ligabue, Franco/F-3432-2014; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Paulini, Manfred/N-7794-2014; Dremin, Igor/K-8053-2015; ciocci, maria agnese /I-2153-2015; Kovac, Marko/D-5817-2017; Vinogradov, Alexey/O-2375-2015; Petrushanko, Sergey/D-6880-2012; VARDARLI, Fuat Ilkehan/B-6360-2013; Cakir, Altan/P-1024-2015; Lokhtin, Igor/D-7004-2012; Montanari, Alessandro/J-2420-2012; Matorras, Francisco/I-4983-2015; Manganote, Edmilson/K-8251-2013; Gennai, Simone/P-2880-2015; TUVE', Cristina/P-3933-2015; Dudko, Lev/D-7127-2012; Moraes, Arthur/F-6478-2010; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Ruiz, Alberto/E-4473-2011; Azarkin, Maxim/N-2578-2015; Chinellato, Jose Augusto/I-7972-2012; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Stahl, Achim/E-8846-2011; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016 OI Reis, Thomas/0000-0003-3703-6624; Luukka, Panja/0000-0003-2340-4641; Jacob, Jeson/0000-0001-6895-5493; Menasce, Dario/0000-0002-9918-1686; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Calvo Alamillo, Enrique/0000-0002-1100-2963; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Cerrada, Marcos/0000-0003-0112-1691; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; Brianza, Luca/0000-0001-5770-6037; Viliani, Lorenzo/0000-0002-1909-6343; ROMERO ABAD, DAVID/0000-0001-5088-9301; ORTONA, Giacomo/0000-0001-8411-2971; Gallinaro, Michele/0000-0003-1261-2277; Gerosa, Raffaele/0000-0001-8359-3734; Bilki, Burak/0000-0001-9515-3306; Sguazzoni, Giacomo/0000-0002-0791-3350; Ligabue, Franco/0000-0002-1549-7107; Rizzi, Andrea/0000-0002-4543-2718; Martinez Ruiz del Arbol, Pablo/0000-0002-7737-5121; Demaria, Natale/0000-0003-0743-9465; Ciulli, Vitaliano/0000-0003-1947-3396; Androsov, Konstantin/0000-0003-2694-6542; HSIUNG, YEE/0000-0003-4801-1238; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; ciocci, maria agnese /0000-0003-0002-5462; Costa, Salvatore/0000-0001-9919-0569; Sharma, Ram Krishna/0000-0003-1181-1426; Malik, Sudhir/0000-0002-6356-2655; Preiato, Federico/0000-0003-2996-4105; Boccali, Tommaso/0000-0002-9930-9299; Montanari, Alessandro/0000-0003-2748-6373; Matorras, Francisco/0000-0003-4295-5668; TUVE', Cristina/0000-0003-0739-3153; Dudko, Lev/0000-0002-4462-3192; Moraes, Arthur/0000-0002-5157-5686; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Ruiz, Alberto/0000-0002-3639-0368; Chinellato, Jose Augusto/0000-0002-3240-6270; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Stahl, Achim/0000-0002-8369-7506; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108 FU Austrian Federal Ministry of Science, Research and Economy; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; Brazilian Funding Agency (CNPq); Brazilian Funding Agency (CAPES); Brazilian Funding Agency (FAPERJ); Brazilian Funding Agency (FAPESP); Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research, Estonia; Estonian Research Council, Estonia [IUT23-4, IUT23-6]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules/CNRS, France; Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; Bundesministerium fur Bildung und Forschung, Germany; Deutsche Forschungsgemeinschaft, Germany; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation, Hungary; National Innovation Office, Hungary; Department of Atomic Energy, India; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Ministry of Science, ICT and Future Planning, Republic of Korea; National Research Foundation (NRF), Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education (Malaysia); University of Malaya (Malaysia); Mexican funding agency (CINVESTAV); Mexican funding agency (CONACYT); Mexican funding agency (SEP); Mexican funding agency (UASLP-FAI); Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education, Poland; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio, Spain; Swiss Funding Agency (ETH Board); Swiss Funding Agency (ETH Zurich); Swiss Funding Agency (PSI); Swiss Funding Agency (SNF); Swiss Funding Agency (UniZH); Swiss Funding Agency (Canton Zurich); Swiss Funding Agency (SER); Ministry of Science and Technology, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine, Ukraine; State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, UK; U.S. Department of Energy; U.S. National Science Foundation; Marie Curie program; European Research Council (European Union); EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS program of the Foundation for Polish Science; European Union, Regional Development Fund; Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR project (Italy) [20108T4XTM]; Thalis program - EU-ESF; Aristeia program - EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); Welch Foundation FX We thank Markus Schulze for optimizing the JHUGen Monte Carlo simulation program and matrix element library for this analysis. We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses.; Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via IUT23-4 and IUT23-6 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules/CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Ministry of Science, ICT and Future Planning, and National Research Foundation (NRF), Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican funding agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine, and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, UK; the U.S. Department of Energy, and the U.S. National Science Foundation. Individuals have received support from the Marie Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P.; Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of the Foundation for Polish Science, cofinanced by the European Union, Regional Development Fund; the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); and the Welch Foundation. NR 72 TC 3 Z9 3 U1 8 U2 47 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 22 PY 2015 VL 92 IS 7 AR 072010 DI 10.1103/PhysRevD.92.072010 PG 28 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CU0VS UT WOS:000363237600001 ER PT J AU Oswald, C Urquijo, P Dingfelder, J Abdesselam, A Adachi, I Aihara, H Al Said, S Asner, DM Aushev, T Ayad, R Babu, V Badhrees, I Bakich, AM Bhardwaj, V Bobrov, A Bonvicini, G Bozek, A Bracko, M Browder, TE Cervenkov, D Chang, MC Chekelian, V Chen, A Cheon, BG Chilikin, K Cho, K Chobanova, V Choi, Y Cinabro, D Dalseno, J Dolezal, Z Drasal, Z Drutskoy, A Dutta, D Eidelman, S Farhat, H Fast, JE Ferber, T Frost, O Fulsom, BG Gaur, V Gabyshev, N Ganguly, S Garmash, A Getzkow, D Gillard, R Glattauer, R Goh, YM Goldenzweig, P Golob, B Grzymkowska, O Hara, T Hasenbusch, J Hayasaka, K Hayashii, H He, XH Hou, WS Huschle, M Hyun, HJ Iijima, T Ishikawa, A Itoh, R Iwasaki, Y Jaegle, I Julius, T Kang, KH Kapusta, P Kato, E Kawasaki, T Kiesling, C Kim, DY Kim, JB Kim, JH Kim, KT Kim, MJ Kim, SH Kim, YJ Kinoshita, K Ko, BR Kodys, P Korpar, S Krizan, P Krokovny, P Kuhr, T Kumita, T Kwon, YJ Lange, JS Lee, DH Lee, IS Li, Y Gioi, LL Libby, J Liventsev, D Lukin, P Matvienko, D Miyata, H Mizuk, R Mohanty, GB Moll, A Moon, HK Nakano, E Nakao, M Nakazawa, H Nanut, T Natkaniec, Z Nayak, M Nishida, S Nozaki, T Okuno, S Pakhlov, P Pakhlova, G Park, CW Park, H Pedlar, TK Pesantez, L Pestotnik, R Petric, M Piilonen, LE Pulvermacher, C Ribezl, E Ritter, M Rostomyan, A Rozanska, M Ryu, S Sakai, Y Sandilya, S Santelj, L Sanuki, T Sato, Y Savinov, V Schneider, O Schnell, G Schwanda, C Semmler, D Senyo, K Seon, O Sevior, ME Shapkin, M Shebalin, V Shen, CP Shibata, TA Shiu, JG Sibidanov, A Simon, F Sohn, YS Solovieva, E Stanic, S Staric, M Stypula, J Sumihama, M Sumiyoshi, T Tamponi, U Teramoto, Y Trabelsi, K Uchida, M Unno, Y Uno, S Usov, Y Van Hulse, C Vanhoefer, P Varner, G Vinokurova, A Vorobyev, V Vossen, A Wagner, MN Wang, CH Wang, MZ Wang, P Wang, XL Watanabe, Y Williams, KM Won, E Yamamoto, H Yashchenko, S Yook, Y Zhang, ZP Zhilich, V Zhulanov, V Zupanc, A AF Oswald, C. Urquijo, P. Dingfelder, J. Abdesselam, A. Adachi, I. Aihara, H. Al Said, S. Asner, D. M. Aushev, T. Ayad, R. Babu, V. Badhrees, I. Bakich, A. M. Bhardwaj, V. Bobrov, A. Bonvicini, G. Bozek, A. Bracko, M. Browder, T. E. Cervenkov, D. Chang, M. -C. Chekelian, V. Chen, A. Cheon, B. G. Chilikin, K. Cho, K. Chobanova, V. Choi, Y. Cinabro, D. Dalseno, J. Dolezal, Z. Drasal, Z. Drutskoy, A. Dutta, D. Eidelman, S. Farhat, H. Fast, J. E. Ferber, T. Frost, O. Fulsom, B. G. Gaur, V. Gabyshev, N. Ganguly, S. Garmash, A. Getzkow, D. Gillard, R. Glattauer, R. Goh, Y. M. Goldenzweig, P. Golob, B. Grzymkowska, O. Hara, T. Hasenbusch, J. Hayasaka, K. Hayashii, H. He, X. H. Hou, W. -S. Huschle, M. Hyun, H. J. Iijima, T. Ishikawa, A. Itoh, R. Iwasaki, Y. Jaegle, I. Julius, T. Kang, K. H. Kapusta, P. Kato, E. Kawasaki, T. Kiesling, C. Kim, D. Y. Kim, J. B. Kim, J. H. Kim, K. T. Kim, M. J. Kim, S. H. Kim, Y. J. Kinoshita, K. Ko, B. R. Kodys, P. Korpar, S. Krizan, P. Krokovny, P. Kuhr, T. Kumita, T. Kwon, Y. -J. Lange, J. S. Lee, D. H. Lee, I. S. Li, Y. Gioi, L. Li Libby, J. Liventsev, D. Lukin, P. Matvienko, D. Miyata, H. Mizuk, R. Mohanty, G. B. Moll, A. Moon, H. K. Nakano, E. Nakao, M. Nakazawa, H. Nanut, T. Natkaniec, Z. Nayak, M. Nishida, S. Nozaki, T. Okuno, S. Pakhlov, P. Pakhlova, G. Park, C. W. Park, H. Pedlar, T. K. Pesantez, L. Pestotnik, R. Petric, M. Piilonen, L. E. Pulvermacher, C. Ribezl, E. Ritter, M. Rostomyan, A. Rozanska, M. Ryu, S. Sakai, Y. Sandilya, S. Santelj, L. Sanuki, T. Sato, Y. Savinov, V. Schneider, O. Schnell, G. Schwanda, C. Semmler, D. Senyo, K. Seon, O. Sevior, M. E. Shapkin, M. Shebalin, V. Shen, C. P. Shibata, T. -A. Shiu, J. -G. Sibidanov, A. Simon, F. Sohn, Y. -S. Solovieva, E. Stanic, S. Staric, M. Stypula, J. Sumihama, M. Sumiyoshi, T. Tamponi, U. Teramoto, Y. Trabelsi, K. Uchida, M. Unno, Y. Uno, S. Usov, Y. Van Hulse, C. Vanhoefer, P. Varner, G. Vinokurova, A. Vorobyev, V. Vossen, A. Wagner, M. N. Wang, C. H. Wang, M. -Z. Wang, P. Wang, X. L. Watanabe, Y. Williams, K. M. Won, E. Yamamoto, H. Yashchenko, S. Yook, Y. Zhang, Z. P. Zhilich, V. Zhulanov, V. Zupanc, A. CA Belle Collaboration TI Semi-inclusive studies of semileptonic B-s decays at Belle SO PHYSICAL REVIEW D LA English DT Article ID MODEL AB We present an analysis of the semi-inclusive decays B-s -> D(s)(-)Xl(+)nu and B-s -> D-s*(-)Xl(+)nu, where X denotes a final state that may consist of additional hadrons or photons and l is an electron or muon. The studied Bs decays are contained in the 121.4 fb(-1) Upsilon(5S) data sample collected by the Belle detector at the KEKB asymmetric-energy e(+)e(-) collider. The branching fractions of the decays are measured to be B(B-s -> D(s)(-)Xl(+)nu) = [8.2 +/- 0.2(stat) +/- 0.6(syst) +/- 1.4(ext)] % and B(B-s -> D-s*(-)Xl(+)nu) = [5.4 +/- 0.4(stat) +/- 0.4(syst) +/- 0.9(ext)] %, where the first two uncertainties are statistical and systematic and the last is due to external parameters. The measurement also provides an estimate of the B-s(()*())(B) over bar (()(s)*()) production cross section, sigma(e(+)e(-) -> B-s(()*())(B) over bar (()(s)*())) = 53.8 +/- 1.4(stat) +/- 4.0(syst) +/- 3.4(ext)] pb, at the center-of-mass energy root s = 10.86 GeV. C1 [Schnell, G.; Van Hulse, C.] Univ Basque Country UPV EHU, Bilbao 48080, Spain. [Shen, C. P.] Beihang Univ, Beijing 100191, Peoples R China. [Oswald, C.; Dingfelder, J.; Hasenbusch, J.; Pesantez, L.] Univ Bonn, D-53115 Bonn, Germany. [Bobrov, A.; Eidelman, S.; Gabyshev, N.; Garmash, A.; Krokovny, P.; Lukin, P.; Matvienko, D.; Shebalin, V.; Usov, Y.; Vinokurova, A.; Vorobyev, V.; Zhilich, V.; Zhulanov, V.] Budker Inst Nucl Phys SB RAS, Novosibirsk 630090, Russia. [Bobrov, A.; Eidelman, S.; Gabyshev, N.; Garmash, A.; Krokovny, P.; Lukin, P.; Matvienko, D.; Shebalin, V.; Usov, Y.; Vinokurova, A.; Vorobyev, V.; Zhilich, V.; Zhulanov, V.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Cervenkov, D.; Dolezal, Z.; Drasal, Z.; Kodys, P.] Charles Univ Prague, Fac Math & Phys, Prague 12116, Czech Republic. [Kinoshita, K.] Univ Cincinnati, Cincinnati, OH 45221 USA. [Ferber, T.; Frost, O.; Rostomyan, A.; Yashchenko, S.] DESY, D-22607 Hamburg, Germany. [Chang, M. -C.] Fu Jen Catholic Univ, Dept Phys, Taipei 24205, Taiwan. [Getzkow, D.; Lange, J. S.; Semmler, D.; Wagner, M. N.] Univ Giessen, D-35392 Giessen, Germany. [Sumihama, M.] Gifu Univ, Gifu 5011193, Japan. [Adachi, I.; Hara, T.; Itoh, R.; Nakao, M.; Nishida, S.; Sakai, Y.; Trabelsi, K.; Uno, S.] Grad Univ Adv Studies, SOKENDAI, Hayama 2400193, Japan. [Cheon, B. G.; Goh, Y. M.; Kim, S. H.; Lee, I. S.; Unno, Y.] Hanyang Univ, Seoul 133791, South Korea. [Browder, T. E.; Jaegle, I.; Varner, G.] Univ Hawaii, Honolulu, HI 96822 USA. [Adachi, I.; Hara, T.; Itoh, R.; Iwasaki, Y.; Nakao, M.; Nishida, S.; Nozaki, T.; Sakai, Y.; Santelj, L.; Trabelsi, K.; Uno, S.] High Energy Accelerator Res Org KEK, Tsukuba, Ibaraki 3050801, Japan. [Schnell, G.] Basque Fdn Sci, IKERBASQUE, Bilbao 48013, Spain. [Libby, J.; Nayak, M.] Indian Inst Technol, Madras 600036, Tamil Nadu, India. [Vossen, A.] Indiana Univ, Bloomington, IN 47408 USA. [Wang, P.] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Glattauer, R.; Schwanda, C.] Inst High Energy Phys, A-1050 Vienna, Austria. [Shapkin, M.] Inst High Energy Phys, Protvino 142281, Russia. [Tamponi, U.] INFN Sez Torino, I-10125 Turin, Italy. [Aushev, T.; Chilikin, K.; Drutskoy, A.; Mizuk, R.; Pakhlov, P.; Pakhlova, G.; Solovieva, E.] Inst Theoret & Expt Phys, Moscow 117218, Russia. [Bracko, M.; Golob, B.; Korpar, S.; Krizan, P.; Nanut, T.; Pestotnik, R.; Petric, M.; Ribezl, E.; Staric, M.; Zupanc, A.] Jozef Stefan Inst, Ljubljana 1000, Slovenia. [Okuno, S.; Watanabe, Y.] Kanagawa Univ, Yokohama, Kanagawa 2218686, Japan. [Goldenzweig, P.; Huschle, M.; Kuhr, T.; Pulvermacher, C.] Karlsruher Inst Technol, Inst Expt Kernphys, D-76131 Karlsruhe, Germany. [Badhrees, I.] King Abdulaziz City Sci & Technol, Riyadh 11442, Saudi Arabia. [Al Said, S.] King Abdulaziz Univ, Dept Phys, Fac Sci, Jeddah 21589, Saudi Arabia. [Cho, K.; Kim, J. H.; Kim, Y. J.] Korea Inst Sci & Technol Informat, Daejeon 305806, South Korea. [Kim, J. B.; Kim, K. T.; Ko, B. R.; Lee, D. H.; Moon, H. K.; Won, E.] Korea Univ, Seoul 136713, South Korea. [Hyun, H. J.; Kang, K. H.; Kim, M. J.; Park, H.] Kyungpook Natl Univ, Daegu 702701, South Korea. [Schneider, O.] Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland. [Golob, B.; Krizan, P.] Univ Ljubljana, Fac Math & Phys, Ljubljana 1000, Slovenia. [Pedlar, T. K.] Luther Coll, Decorah, IA 52101 USA. [Bracko, M.; Korpar, S.] Univ Maribor, SLO-2000 Maribor, Slovenia. [Chekelian, V.; Chobanova, V.; Dalseno, J.; Kiesling, C.; Gioi, L. Li; Moll, A.; Ritter, M.; Simon, F.; Vanhoefer, P.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Urquijo, P.; Julius, T.; Sevior, M. E.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Drutskoy, A.; Mizuk, R.; Pakhlov, P.] Moscow Phys Engn Inst, Moscow 115409, Russia. [Aushev, T.; Pakhlova, G.] Moscow Inst Phys & Technol, Dolgoprudnyi 141700, Moscow Region, Russia. [Iijima, T.; Sato, Y.; Seon, O.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648602, Japan. [Hayasaka, K.; Iijima, T.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648602, Japan. [Hayashii, H.] Nara Womens Univ, Nara 6308506, Japan. [Chen, A.; Nakazawa, H.] Natl Cent Univ, Chungli 32054, Taiwan. [Wang, C. H.] Natl United Univ, Miaoli 36003, Taiwan. [Hou, W. -S.; Shiu, J. -G.; Wang, M. -Z.] Natl Taiwan Univ, Dept Phys, Taipei 10617, Taiwan. [Bozek, A.; Grzymkowska, O.; Kapusta, P.; Natkaniec, Z.; Rozanska, M.; Stypula, J.] H Niewodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. [Kawasaki, T.; Miyata, H.] Niigata Univ, Niigata 9502181, Japan. [Stanic, S.] Univ Nova Gorica, Nova Gorica 5000, Slovenia. [Nakano, E.; Teramoto, Y.] Osaka City Univ, Osaka 5588585, Japan. [Asner, D. M.; Fast, J. E.; Fulsom, B. G.] Pacific NW Natl Lab, Richland, WA 99352 USA. [He, X. H.] Peking Univ, Beijing 100871, Peoples R China. [Savinov, V.] Univ Pittsburgh, Pittsburgh, PA 15260 USA. [Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Ryu, S.] Seoul Natl Univ, Seoul 151742, South Korea. [Kim, D. Y.] Soongsil Univ, Seoul 156743, South Korea. [Bhardwaj, V.] Univ S Carolina, Columbia, SC 29208 USA. [Choi, Y.; Park, C. W.] Sungkyunkwan Univ, Suwon 440746, South Korea. [Bakich, A. M.; Sibidanov, A.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdesselam, A.; Al Said, S.; Ayad, R.; Badhrees, I.] Univ Tabuk, Fac Sci, Dept Phys, Tabuk 71451, Saudi Arabia. [Babu, V.; Dutta, D.; Gaur, V.; Mohanty, G. B.; Sandilya, S.] Inst Fundamental Res, Bombay 400005, Maharashtra, India. [Dalseno, J.; Moll, A.; Simon, F.] Tech Univ Munich, Excellence Cluster Universe, D-85748 Garching, Germany. [Ishikawa, A.; Kato, E.; Sanuki, T.; Yamamoto, H.] Tohoku Univ, Sendai, Miyagi 9808578, Japan. [Aihara, H.] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Shibata, T. -A.; Uchida, M.] Tokyo Inst Technol, Tokyo 1528550, Japan. [Kumita, T.; Sumiyoshi, T.] Tokyo Metropolitan Univ, Tokyo 1920397, Japan. [Tamponi, U.] Univ Turin, I-10124 Turin, Italy. [Li, Y.; Liventsev, D.; Piilonen, L. E.; Wang, X. L.; Williams, K. M.] Virginia Polytech Inst & State Univ, CNP, Blacksburg, VA 24061 USA. [Bonvicini, G.; Cinabro, D.; Farhat, H.; Ganguly, S.; Gillard, R.] Wayne State Univ, Detroit, MI 48202 USA. [Senyo, K.] Yamagata Univ, Yamagata 9908560, Japan. [Kwon, Y. -J.; Sohn, Y. -S.; Yook, Y.] Yonsei Univ, Seoul 120749, South Korea. RP Oswald, C (reprint author), Univ Bonn, D-53115 Bonn, Germany. RI Pakhlov, Pavel/K-2158-2013; Mizuk, Roman/B-3751-2014; Krokovny, Pavel/G-4421-2016; Aihara, Hiroaki/F-3854-2010; Chilikin, Kirill/B-4402-2014; EPFL, Physics/O-6514-2016; Drutskoy, Alexey/C-8833-2016; Cervenkov, Daniel/D-2884-2017; Solovieva, Elena/B-2449-2014; Pakhlova, Galina/C-5378-2014 OI Pakhlov, Pavel/0000-0001-7426-4824; Krokovny, Pavel/0000-0002-1236-4667; Aihara, Hiroaki/0000-0002-1907-5964; Chilikin, Kirill/0000-0001-7620-2053; Drutskoy, Alexey/0000-0003-4524-0422; Cervenkov, Daniel/0000-0002-1865-741X; Solovieva, Elena/0000-0002-5735-4059; Pakhlova, Galina/0000-0001-7518-3022 FU Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan; Japan Society for the Promotion of Science (JSPS); Tau-Lepton Physics Research Center of Nagoya University; Australian Research Council; Australian Department of Industry, Innovation, Science and Research; Austrian Science Fund [P 22742-N16, P 26794-N20]; National Natural Science Foundation of China [10575109, 10775142, 10875115, 11175187, 11475187]; Ministry of Education, Youth and Sports of the Czech Republic [LG14034]; Carl Zeiss Foundation; Deutsche Forschungsgemeinschaft; VolkswagenStiftung; Department of Science and Technology of India; Istituto Nazionale di Fisica Nucleare of Italy; National Research Foundation (NRF) of Korea [2011-0029457, 2012-0008143, 2012R1A1A2008330, 2013R1A1A3007772, 2014R1A2A2A01005286, 2014R1A2A2A01002734, 2014R1A1A2006456]; Basic Research Lab program under NRF Grant [KRF-2011-0020333, KRF-2011-0021196]; Center for Korean J-PARC Users [NRF-2013K1A3A7A06056592]; Brain Korea 21-Plus program; Global Science Experimental Data Hub Center of the Korea Institute of Science and Technology Information; Polish Ministry of Science and Higher Education; National Science Center; Ministry of Education and Science of the Russian Federation; Russian Foundation for Basic Research; Slovenian Research Agency; Basque Foundation for Science (IKERBASQUE); Euskal Herriko Unibertsitatea (UPV/EHU) (Spain) [UFI 11/55]; Swiss National Science Foundation; National Science Council; Ministry of Education of Taiwan; U.S. Department of Energy; National Science Foundation; MEXT; JSPS FX We thank the KEKB group for the excellent operation of the accelerator; the KEK cryogenics group for the efficient operation of the solenoid; and the KEK computer group, the National Institute of Informatics, and the PNNL/EMSL computing group for valuable computing and SINET4 network support. We acknowledge support from the Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan, the Japan Society for the Promotion of Science (JSPS), and the Tau-Lepton Physics Research Center of Nagoya University; the Australian Research Council and the Australian Department of Industry, Innovation, Science and Research; Austrian Science Fund under Grants No. P 22742-N16 and No. P 26794-N20; the National Natural Science Foundation of China under Contracts No. 10575109, No. 10775142, No. 10875115, No. 11175187, and No. 11475187; the Ministry of Education, Youth and Sports of the Czech Republic under Contract No. LG14034; the Carl Zeiss Foundation, the Deutsche Forschungsgemeinschaft and the VolkswagenStiftung; the Department of Science and Technology of India; the Istituto Nazionale di Fisica Nucleare of Italy; National Research Foundation (NRF) of Korea Grants No. 2011-0029457, No. 2012-0008143, No. 2012R1A1A2008330, No. 2013R1A1A3007772, No. 2014R1A2A2A01005286, No. 2014R1A2A2A01002734, No. 2014R1A1A2006456; the Basic Research Lab program under NRF Grant No. KRF-2011-0020333, No. KRF-2011-0021196, Center for Korean J-PARC Users, No. NRF-2013K1A3A7A06056592; the Brain Korea 21-Plus program and the Global Science Experimental Data Hub Center of the Korea Institute of Science and Technology Information; the Polish Ministry of Science and Higher Education and the National Science Center; the Ministry of Education and Science of the Russian Federation and the Russian Foundation for Basic Research; the Slovenian Research Agency; the Basque Foundation for Science (IKERBASQUE) and the Euskal Herriko Unibertsitatea (UPV/EHU) under program UFI 11/55 (Spain); the Swiss National Science Foundation; the National Science Council and the Ministry of Education of Taiwan; and the U.S. Department of Energy and the National Science Foundation. This work is supported by a Grant-in-Aid from MEXT for Science Research in a Priority Area ("New Development of Flavor Physics") and from JSPS for Creative Scientific Research ("Evolution of Tau-lepton Physics"). NR 48 TC 3 Z9 3 U1 0 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 22 PY 2015 VL 92 IS 7 AR 072013 DI 10.1103/PhysRevD.92.072013 PG 13 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CU0VS UT WOS:000363237600003 ER PT J AU Chen, RY Chen, ZG Song, XY Schneeloch, JA Gu, GD Wang, F Wang, NL AF Chen, R. Y. Chen, Z. G. Song, X. -Y. Schneeloch, J. A. Gu, G. D. Wang, F. Wang, N. L. TI Magnetoinfrared Spectroscopy of Landau Levels and Zeeman Splitting of Three-Dimensional Massless Dirac Fermions in ZrTe5 SO PHYSICAL REVIEW LETTERS LA English DT Article ID SEMIMETAL CD3AS2; MOBILITY AB We present a magnetoinfrared spectroscopy study on a newly identified three-dimensional (3D) Dirac semimetal ZrTe5. We observe clear transitions between Landau levels and their further splitting under a magnetic field. Both the sequence of transitions and their field dependence follow quantitatively the relation expected for 3D massless Dirac fermions. The measurement also reveals an exceptionally low magnetic field needed to drive the compound into its quantum limit, demonstrating that ZrTe5 is an extremely clean system and ideal platform for studying 3D Dirac fermions. The splitting of the Landau levels provides direct, bulk spectroscopic evidence that a relatively weak magnetic field can produce a sizable Zeeman effect on the 3D Dirac fermions, which lifts the spin degeneracy of Landau levels. Our analysis indicates that the compound evolves from a Dirac semimetal into a topological line-node semimetal under the current magnetic field configuration. C1 [Chen, R. Y.; Song, X. -Y.; Wang, F.; Wang, N. L.] Peking Univ, Sch Phys, Int Ctr Quantum Mat, Beijing 100871, Peoples R China. [Chen, Z. G.] Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. [Schneeloch, J. A.; Gu, G. D.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Wang, F.; Wang, N. L.] Collaborat Innovat Ctr Quantum Matter, Beijing, Peoples R China. RP Chen, RY (reprint author), Peking Univ, Sch Phys, Int Ctr Quantum Mat, Beijing 100871, Peoples R China. EM wangfa@pku.edu.cn; nlwang@pku.edu.cn RI Wang, Fa/D-3817-2015; Chen, Zhiguo/B-9192-2015 OI Wang, Fa/0000-0002-6220-5349; Chen, Zhiguo/0000-0002-8242-4784 FU National Science Foundation of China [11120101003, 11327806, 11374018]; 973 project of the Ministry of Science and Technology of China [2011CB921701, 2012CB821403, 2014CB920902]; Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, U.S. Department of Energy [DE-SC00112704] FX We acknowledge very helpful discussions with Z. Fang, H. M. Weng, X. C. Xie, D. H. Lee, L. Fu, Q. Li, X. Dai, and H. W. Liu. This work was supported by the National Science Foundation of China (Grants No. 11120101003, No. 11327806, No. 11374018), and the 973 project of the Ministry of Science and Technology of China (Grants No. 2011CB921701, No. 2012CB821403, No. 2014CB920902). Work at Brookhaven is supported by the Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, U.S. Department of Energy under Contract No. DE-SC00112704. NR 29 TC 26 Z9 26 U1 19 U2 101 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 22 PY 2015 VL 115 IS 17 AR 176404 DI 10.1103/PhysRevLett.115.176404 PG 5 WC Physics, Multidisciplinary SC Physics GA CU0YE UT WOS:000363244400009 PM 26551130 ER PT J AU Hogle, CW Tong, XM Martin, L Murnane, MM Kapteyn, HC Ranitovic, P AF Hogle, C. W. Tong, X. M. Martin, L. Murnane, M. M. Kapteyn, H. C. Ranitovic, P. TI Attosecond Coherent Control of Single and Double Photoionization in Argon SO PHYSICAL REVIEW LETTERS LA English DT Article ID 2-PHOTON TRANSITIONS; MOLECULAR-DYNAMICS; LASER CONTROL; IONIZATION; SPECTROSCOPY; REGIME AB Ultrafast high harmonic beams provide new opportunities for coherently controlling excitation and ionization processes in atoms, molecules, and materials on attosecond time scales by employing multiphoton two-pathway electron-wave-packet quantum interferences. Here we use spectrally tailored and frequency tuned vacuum and extreme ultraviolet harmonic combs, together with two phase-locked infrared laser fields, to show how the total single and double photoionization yields of argon can be coherently modulated by controlling the relative phases of both optical and electronic-wave-packet quantum interferences. This Letter is the first to apply quantum control techniques to double photoionization, which is a fundamental process where a single, high-energy photon ionizes two electrons simultaneously from an atom. C1 [Hogle, C. W.; Martin, L.; Murnane, M. M.; Kapteyn, H. C.; Ranitovic, P.] Univ Colorado, JILA, Boulder, CO 80309 USA. [Hogle, C. W.; Martin, L.; Murnane, M. M.; Kapteyn, H. C.; Ranitovic, P.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Hogle, C. W.; Martin, L.; Murnane, M. M.; Kapteyn, H. C.; Ranitovic, P.] NIST, Boulder, CO 80309 USA. [Tong, X. M.] Univ Tsukuba, Div Mat Sci, Fac Pure & Appl Sci, Tsukuba, Ibaraki 3058573, Japan. [Ranitovic, P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Ranitovic, P.] ELI Hu Nkft, ELI ALPS, H-6720 Szeged, Hungary. RP Ranitovic, P (reprint author), Univ Colorado, JILA, Boulder, CO 80309 USA. EM pranitovic@lbl.gov RI Tong, Xiao-Min/A-2748-2011 OI Tong, Xiao-Min/0000-0003-4898-3491 FU Army Research Office; Japan Society for the Promotion of Science [C24540421] FX The authors gratefully acknowledge support from the Army Research Office. X. M. T. was supported by a Grand-in-Aid for Scientific Research (Grant No. C24540421) from the Japan Society for the Promotion of Science. NR 38 TC 1 Z9 1 U1 5 U2 37 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 22 PY 2015 VL 115 IS 17 AR 173004 DI 10.1103/PhysRevLett.115.173004 PG 6 WC Physics, Multidisciplinary SC Physics GA CU0YE UT WOS:000363244400005 PM 26551112 ER PT J AU Zhang, YW Long, E Mihovilovic, M Jin, G Allada, K Anderson, B Annand, JRM Averett, T Ayerbe-Gayoso, C Boeglin, W Bradshaw, P Camsonne, A Canan, M Cates, GD Chen, C Chen, JP Chudakov, E De Leo, R Deng, X Deur, A Dutta, C El Fassi, L Flay, D Frullani, S Garibaldi, F Gao, H Gilad, S Gilman, R Glamazdin, O Golge, S Gomez, J Hansen, O Higinbotham, DW Holmstrom, T Huang, J Ibrahim, H de Jager, CW Jensen, E Jiang, X St John, J Jones, M Kang, H Katich, J Khanal, HP King, P Korsch, W LeRose, J Lindgren, R Lu, HJ Luo, W Markowitz, P Meziane, M Michaels, R Moffit, B Monaghan, P Muangma, N Nanda, S Norum, BE Pan, K Parno, D Piasetzky, E Posik, M Punjabi, V Puckett, AJR Qian, X Qiang, Y Qiu, X Riordan, S Ron, G Saha, A Sawatzky, B Schiavilla, R Schoenrock, B Shabestari, M Shahinyan, A Sirca, S Subedi, R Sulkosky, V Tobias, WA Tireman, W Urciuoli, GM Wang, D Wang, K Wang, Y Watson, J Wojtsekhowski, B Ye, Z Zhan, X Zhang, Y Zheng, X Zhao, B Zhu, L AF Zhang, Y. -W. Long, E. Mihovilovic, M. Jin, G. Allada, K. Anderson, B. Annand, J. R. M. Averett, T. Ayerbe-Gayoso, C. Boeglin, W. Bradshaw, P. Camsonne, A. Canan, M. Cates, G. D. Chen, C. Chen, J. P. Chudakov, E. De Leo, R. Deng, X. Deur, A. Dutta, C. El Fassi, L. Flay, D. Frullani, S. Garibaldi, F. Gao, H. Gilad, S. Gilman, R. Glamazdin, O. Golge, S. Gomez, J. Hansen, O. Higinbotham, D. W. Holmstrom, T. Huang, J. Ibrahim, H. de Jager, C. W. Jensen, E. Jiang, X. St John, J. Jones, M. Kang, H. Katich, J. Khanal, H. P. King, P. Korsch, W. LeRose, J. Lindgren, R. Lu, H. -J. Luo, W. Markowitz, P. Meziane, M. Michaels, R. Moffit, B. Monaghan, P. Muangma, N. Nanda, S. Norum, B. E. Pan, K. Parno, D. Piasetzky, E. Posik, M. Punjabi, V. Puckett, A. J. R. Qian, X. Qiang, Y. Qiu, X. Riordan, S. Ron, G. Saha, A. Sawatzky, B. Schiavilla, R. Schoenrock, B. Shabestari, M. Shahinyan, A. Sirca, S. Subedi, R. Sulkosky, V. Tobias, W. A. Tireman, W. Urciuoli, G. M. Wang, D. Wang, K. Wang, Y. Watson, J. Wojtsekhowski, B. Ye, Z. Zhan, X. Zhang, Y. Zheng, X. Zhao, B. Zhu, L. CA Jefferson Lab Hall A Collaboration TI Measurement of the Target-Normal Single-Spin Asymmetry in Quasielastic Scattering from the Reaction He-3(up arrow) (e,e ') SO PHYSICAL REVIEW LETTERS LA English DT Article ID PROTON SCATTERING AB We report the first measurement of the target single-spin asymmetry, A(y), in quasielastic scattering from the inclusive reaction He-3(up arrow)(e,e') on a He-3 gas target polarized normal to the lepton scattering plane. Assuming time-reversal invariance, this asymmetry is strictly zero for one-photon exchange. A nonzero A(y) can arise from the interference between the one-and two-photon exchange processes which is sensitive to the details of the substructure of the nucleon. An experiment recently completed at Jefferson Lab yielded asymmetries with high statistical precision at Q(2) = 0.13, 0.46, and 0.97 GeV2. These measurements demonstrate, for the first time, that the He-3 asymmetry is clearly nonzero and negative at the 4 sigma-9 sigma level. Using measured proton-to-He-3 cross-section ratios and the effective polarization approximation, neutron asymmetries of -(1-3)% were obtained. The neutron asymmetry at high Q(2) is related to moments of the generalized parton distributions (GPDs). Our measured neutron asymmetry at Q(2) = 0.97 GeV2 agrees well with a prediction based on two-photon exchange using a GPD model and thus provides a new, independent constraint on these distributions. C1 [Zhang, Y. -W.; El Fassi, L.; Gilman, R.] Rutgers State Univ, New Brunswick, NJ 08901 USA. [Zhang, Y. -W.] Univ Penn, Philadelphia, PA 19104 USA. [Long, E.; Anderson, B.] Kent State Univ, Kent, OH 44242 USA. [Mihovilovic, M.; Sirca, S.] Jozef Stefan Inst, SI-1000 Ljubljana, Slovenia. [Jin, G.; Cates, G. D.; Deng, X.; Lindgren, R.; Norum, B. E.; Riordan, S.; Shabestari, M.; Tobias, W. A.; Wang, D.; Wang, K.; Zheng, X.] Univ Virginia, Charlottesville, VA 22908 USA. [Allada, K.; Camsonne, A.; Chen, J. P.; Chudakov, E.; Deur, A.; Gomez, J.; Hansen, O.; Higinbotham, D. W.; de Jager, C. W.; Jones, M.; LeRose, J.; Michaels, R.; Moffit, B.; Nanda, S.; Qiang, Y.; Saha, A.; Sawatzky, B.; Schiavilla, R.; Watson, J.; Wojtsekhowski, B.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Annand, J. R. M.] Univ Glasgow, Glasgow G12 8QQ, Lanark, Scotland. [Averett, T.; Ayerbe-Gayoso, C.; Bradshaw, P.; Katich, J.; Meziane, M.; Zhao, B.] Coll William & Mary, Williamsburg, VA 23187 USA. [Boeglin, W.; Khanal, H. P.; Markowitz, P.] Florida Int Univ, Miami, FL 33181 USA. [Canan, M.; Golge, S.; Schiavilla, R.] Old Dominion Univ, Norfolk, VA 23529 USA. [Chen, C.; Monaghan, P.; Ye, Z.; Zhu, L.] Hampton Univ, Hampton, VA 23669 USA. [De Leo, R.] Univ Bari Aldo, I-70121 Bari, Italy. [Dutta, C.; Korsch, W.] Univ Kentucky, Lexington, KY 40506 USA. [Flay, D.; Posik, M.] Temple Univ, Philadelphia, PA 19122 USA. [Frullani, S.; Garibaldi, F.; Urciuoli, G. M.] Ist Nazl Fis Nucl, INFN Sanita, I-00161 Rome, Italy. [Gao, H.; Qian, X.] Duke Univ, Durham, NC 27708 USA. [Gilad, S.; Huang, J.; Muangma, N.; Pan, K.; Sulkosky, V.; Zhan, X.] MIT, Cambridge, MA 02139 USA. [Glamazdin, O.] Kharkov Inst Phys & Technol, UA-61108 Kharkov, Ukraine. [Holmstrom, T.; St John, J.] Longwood Univ, Farmville, VA 23909 USA. [Huang, J.; Jiang, X.; Puckett, A. J. R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Ibrahim, H.] Cairo Univ, Cairo 12613, Giza, Egypt. [Jensen, E.] Christopher Newport Univ, Newport News, VA 23606 USA. [Kang, H.] Seoul Natl Univ, Seoul 151742, South Korea. [King, P.] Ohio Univ, Athens, OH 45701 USA. [Lu, H. -J.] Huangshan Univ, Huangshan City 245041, Anhui Province, Peoples R China. [Luo, W.; Qiu, X.; Zhang, Y.] Lanzhou Univ, Lanzhou 730000, Gansu, Peoples R China. [Parno, D.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Piasetzky, E.] Tel Aviv Univ, IL-69978 Tel Aviv, Israel. [Punjabi, V.] Norfolk State Univ, Norfolk, VA 23504 USA. [Ron, G.] Hebrew Univ Jerusalem, IL-91904 Jerusalem, Israel. [Schoenrock, B.; Tireman, W.] No Michigan Univ, Marquette, MI 49855 USA. [Shahinyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Sirca, S.] Univ Ljubljana, SI-1000 Ljubljana, Slovenia. [Subedi, R.] George Washington Univ, Washington, DC 20052 USA. [Wang, Y.] Univ Illinois, Urbana, IL 61801 USA. RP Averett, T (reprint author), Rutgers State Univ, New Brunswick, NJ 08901 USA. EM tdaver@wm.edu RI Parno, Diana/B-7546-2017; Ye, Zhihong/E-6651-2017 OI Parno, Diana/0000-0002-9363-0401; Ye, Zhihong/0000-0002-1873-2344 FU U.S. National Science Foundation; U.S. Department of Energy; DOE Contract [DE-AC05-06OR23177]; National Science Foundation of China; UK STFC Grants [57071/1, 50727/1] FX We acknowledge the outstanding support of the Jefferson Lab Hall A technical staff and Accelerator Division in accomplishing this experiment. We wish to thank Drs. A. Deltuva, Vilnius University, A. Afanasev, Jefferson Lab, M. Vanderhaeghen, MAINZ, and J. Arrington, Argonne National Lab for their theoretical guidance and calculations. This work was supported in part by the U.S. National Science Foundation, the U.S. Department of Energy, and DOE Contract No. DE-AC05-06OR23177, under which Jefferson Science Associates, LLC operates the Thomas Jefferson National Accelerator Facility, the National Science Foundation of China, and UK STFC Grants No. 57071/1 and No. 50727/1. NR 28 TC 2 Z9 2 U1 1 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 22 PY 2015 VL 115 IS 17 AR 172502 DI 10.1103/PhysRevLett.115.172502 PG 6 WC Physics, Multidisciplinary SC Physics GA CU0YE UT WOS:000363244400004 PM 26551107 ER PT J AU Xu, B Chen, MJ Yao, MM Ji, XL Mao, ZL Tang, W Qiao, SL Schick, SF Mao, JH Bo, Xia, YK AF Xu, Bo Chen, Minjian Yao, Mengmeng Ji, Xiaoli Mao, Zhilei Tang, Wei Qiao, Shanlei Schick, Suzaynn F. Mao, Jian-Hua Hang, Bo Xia, Yankai TI Metabolomics reveals metabolic changes in male reproductive cells exposed to thirdhand smoke SO SCIENTIFIC REPORTS LA English DT Article ID ENVIRONMENTAL TOBACCO-SMOKE; CIGARETTE-SMOKE; PROFILES DELINEATE; POTENTIAL ROLE; LUNG-CANCER; NICOTINE; GENOTOXICITY; GLUTATHIONE; BIOMARKERS; POLLUTION AB Thirdhand smoke (THS) is a new term for the toxins in cigarette smoke that linger in the environment long after the cigarettes are extinguished. The effects of THS exposure on male reproduction have not yet been studied. In this study, metabolic changes in male germ cell lines (GC-2 and TM-4) were analyzed after THS treatment for 24 h. THS-loaded chromatography paper samples were generated in a laboratory chamber system and extracted in DMEM. At a paper: DMEM ratio of 50 mu g/ml, cell viability in both cell lines was normal, as measured by the MTT assay and markers of cytotoxicity, cell cycle, apoptosis and ROS production were normal as measured by quantitative immunofluorescence. Metabolomic analysis was performed on methanol extracts of GC-2 and TM-4 cells. Glutathione metabolism in GC-2 cells, and nucleic acid and ammonia metabolism in TM-4 cells, was changed significantly by THS treatment. RT-PCR analyses of mRNA for enzyme genes Gss and Ggt in GC-2 cells, and TK, SMS and Glna in TM-4 cells reinforced these findings, showing changes in the levels of enzymes involved in the relevant pathways. In conclusion, exposure to THS at very low concentrations caused distinct metabolic changes in two different types of male reproductive cell lines. C1 [Xu, Bo; Chen, Minjian; Yao, Mengmeng; Ji, Xiaoli; Mao, Zhilei; Qiao, Shanlei; Xia, Yankai] Nanjing Med Univ, Inst Toxicol, State Key Lab Reprod Med, Nanjing 211166, Jiangsu, Peoples R China. [Xu, Bo; Chen, Minjian; Yao, Mengmeng; Ji, Xiaoli; Mao, Zhilei; Qiao, Shanlei; Xia, Yankai] Nanjing Med Univ, Sch Publ Hlth, Minist Educ, Key Lab Modern Toxicol, Nanjing 211166, Jiangsu, Peoples R China. [Tang, Wei] Nanjing Med Univ, Jiangsu Prov Official Hosp, Dept Endocrinol, Nanjing 210024, Jiangsu, Peoples R China. [Schick, Suzaynn F.] Univ Calif San Francisco, Dept Med, Div Occupat & Environm Med, San Francisco, CA 94143 USA. [Mao, Jian-Hua; Hang, Bo] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Dept Canc & DNA Damage Responses, Berkeley, CA 94720 USA. RP Xia, YK (reprint author), Nanjing Med Univ, Inst Toxicol, State Key Lab Reprod Med, Nanjing 211166, Jiangsu, Peoples R China. EM Bo_hang@lbl.gov; yankaixia@njmu.edu.cn FU National 973 Program [2012CBA01305]; National Science Fund for Outstanding Young Scholars [81322039]; National Natural Science Foundation [31371524]; Distinguished Young Scholars of Jiangsu Province [BK20130041]; Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD); New Century Excellent Talents in University [NCET-13-0870]; California Tobacco-Related Disease Research Program (TRDRP) under U.S. Department of Energy [19XT-0070, DE-AC02-05CH11231] FX This study was supported by National 973 Program (2012CBA01305); National Science Fund for Outstanding Young Scholars (81322039); National Natural Science Foundation (31371524); Distinguished Young Scholars of Jiangsu Province (BK20130041); Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD); New Century Excellent Talents in University (NCET-13-0870) and the California Tobacco-Related Disease Research Program (TRDRP) Grant 19XT-0070 (to B.H.) under U.S. Department of Energy (Contract no. DE-AC02-05CH11231). NR 33 TC 4 Z9 4 U1 4 U2 12 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 22 PY 2015 VL 5 AR 15512 DI 10.1038/srep15512 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CT9KV UT WOS:000363136800001 PM 26489853 ER PT J AU Champion, C Quinto, MA Monti, JM Galassi, ME Weck, PF Fojon, OA Hanssen, J Rivarola, RD AF Champion, C. Quinto, M. A. Monti, J. M. Galassi, M. E. Weck, P. F. Fojon, O. A. Hanssen, J. Rivarola, R. D. TI Water versus DNA: new insights into proton track-structure modelling in radiobiology and radiotherapy SO PHYSICS IN MEDICINE AND BIOLOGY LA English DT Article DE proton transport; cross sections; energy transfers; water and DNA; radiobiology; radiotherapy ID LOW-ENERGY ELECTRONS; CROSS-SECTIONS; IONIZATION-POTENTIALS; CHARGE-TRANSFER; STRUCTURE CODES; DNA/RNA BASES; LIQUID WATER; RADIATION; DAMAGE; IONS AB Water is a common surrogate of DNA for modelling the charged particle-induced ionizing processes in living tissue exposed to radiations. The present study aims at scrutinizing the validity of this approximation and then revealing new insights into proton-induced energy transfers by a comparative analysis between water and realistic biological medium. In this context, a self-consistent quantum mechanical modelling of the ionization and electron capture processes is reported within the continuum distorted wave-eikonal initial state framework for both isolated water molecules and DNA components impacted by proton beams. Their respective probability of occurrence-expressed in terms of total cross sections-as well as their energetic signature (potential and kinetic) are assessed in order to clearly emphasize the differences existing between realistic building blocks of living matter and the controverted water-medium surrogate. Consequences in radiobiology and radiotherapy will be discussed in particular in view of treatment planning refinement aiming at better radiotherapy strategies. C1 [Champion, C.] Univ Bordeaux, CNRS IN2P3, Ctr Etudes Nucl Bordeaux, Gradignan, France. [Quinto, M. A.; Monti, J. M.; Galassi, M. E.; Fojon, O. A.; Hanssen, J.; Rivarola, R. D.] Consejo Nacl Invest Cient & Tecn, Inst Fis Rosario, Rosario, Argentina. [Quinto, M. A.; Monti, J. M.; Galassi, M. E.; Fojon, O. A.; Hanssen, J.; Rivarola, R. D.] Univ Nacl Rosario, RA-2000 Rosario, Argentina. [Weck, P. F.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Champion, C (reprint author), Univ Bordeaux, CNRS IN2P3, Ctr Etudes Nucl Bordeaux, Gradignan, France. EM champion@cenbg.in2p3.fr OI , Philippe/0000-0002-7610-2893 FU Agencia Nacional de Promocion Cientifica y Tecnologica from Republica Argentina [PICT 2011-2145]; Consejo Nacional de Investigaciones Cientificas y Tecnicas from Republica Argentina [PIP 1026]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors would like to thank the Mesocentre de Calcul Intensif Aquitain (MCIA, Bordeaux) and the University of Lorraine (Theorie-Modelisation-Simulation group, UMR CNRS 7565) for the free computer time provided. Besides, J M M, M E G, O A F, J H and R D R acknowledge financial support from the Agencia Nacional de Promocion Cientifica y Tecnologica through the project PICT 2011-2145 and from Consejo Nacional de Investigaciones Cientificas y Tecnicas through the project PIP 1026, both institutions from Republica Argentina. Finally, Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 56 TC 8 Z9 8 U1 0 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0031-9155 EI 1361-6560 J9 PHYS MED BIOL JI Phys. Med. Biol. PD OCT 21 PY 2015 VL 60 IS 20 BP 7805 EP 7828 DI 10.1088/0031-9155/60/20/7805 PG 24 WC Engineering, Biomedical; Radiology, Nuclear Medicine & Medical Imaging SC Engineering; Radiology, Nuclear Medicine & Medical Imaging GA CW3SZ UT WOS:000364913500004 PM 26406277 ER PT J AU Modgil, D Rigie, DS Wang, YX Xiao, XH Vargas, PA La Riviere, PJ AF Modgil, Dimple Rigie, David S. Wang, Yuxin Xiao, Xianghui Vargas, Phillip A. La Riviere, Patrick J. TI Material identification in x-ray microscopy and micro CT using multi-layer, multi-color scintillation detectors SO PHYSICS IN MEDICINE AND BIOLOGY LA English DT Article DE x-ray microscopy; micro CT; multi-layer scintillation; multi-color; material identification ID COMPUTED-TOMOGRAPHY AB We demonstrate that a dual-layer, dual-color scintillator construct for microscopic CT, originally proposed to increase sensitivity in synchrotron imaging, can also be used to perform material quantification and classification when coupled with polychromatic illumination. We consider two different approaches to data handling: (1) a data-domain material decomposition whose estimation performance can be characterized by the Cramer-Rao lower bound formalism but which requires careful calibration and (2) an image-domain material classification approach that is more robust to calibration errors. The data-domain analysis indicates that useful levels of SNR (>5) could be achieved in one second or less at typical bending magnet fluxes for relatively large amounts of contrast (several mm path length, such as in a fluid flow experiment) and at typical undulator fluxes for small amount of contrast (tens of microns path length, such as an angiography experiment). The tools introduced could of course be used to study and optimize parameters for a wider range of potential applications. The image domain approach was analyzed in terms of its ability to distinguish different elemental stains by characterizing the angle between the lines traced out in a two-dimensional space of effective attenuation coefficient in the front and back layer images. This approach was implemented at a synchrotron and the results were consistent with simulation predictions. C1 [Modgil, Dimple; Rigie, David S.; Vargas, Phillip A.; La Riviere, Patrick J.] Univ Chicago, Dept Radiol, Chicago, IL 60637 USA. [Wang, Yuxin] Motorola Mobil, Chicago, IL 60654 USA. [Xiao, Xianghui] Argonne Natl Lab, Adv Photon Source, Lemont, IL 60439 USA. RP Modgil, D (reprint author), Univ Chicago, Dept Radiol, Chicago, IL 60637 USA. EM dimple@uchicago.edu FU NIH [R01EB017293, R01CA134680] FX We would like to thank S Rajamani for her help in preparing the stain solutions and J Rajagopal for help in the CRLB analysis. We would also like to thank the anonymous reviewers for their valuable and helpful comments. We would like to acknowledge support from NIH grants R01EB017293 and R01CA134680. NR 26 TC 1 Z9 1 U1 2 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0031-9155 EI 1361-6560 J9 PHYS MED BIOL JI Phys. Med. Biol. PD OCT 21 PY 2015 VL 60 IS 20 BP 8025 EP 8045 DI 10.1088/0031-9155/60/20/8025 PG 21 WC Engineering, Biomedical; Radiology, Nuclear Medicine & Medical Imaging SC Engineering; Radiology, Nuclear Medicine & Medical Imaging GA CW3SZ UT WOS:000364913500016 PM 26422059 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguiar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alex, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Aurousseau, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Balunas, WK Banas, E Banerjee, S Bannoura, AAE Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bance, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beecherle, R Bechtle, P Beck, HP Becker, K Becker, M Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Biedermann, D Bieniek, SP Biesuz, NV Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biondi, S Bjergaard, DM Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Boch, I Blocker, C Blum, W Blumenschein, U Blunier, S Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehler, M Bogaerts, JA Bogavac, D Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutle, SK Boveia, A Boyd, J Boyko, IR Bozic, I Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Madden, WDB Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, K Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E de Renstrom, PAB Bruncko, D Bruneliere, R 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Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, BC Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chang, P Chapman, JD Charlton, DG Chau, CC Barajas, CAC Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, S Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A Cheremushkina, E El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiarelli, G Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Choi, K Chouridou, S Chow, BKB Christodoulou, V Chromek-Burckhart, D Chudoba, J Chuinard, AJ Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Cinca, D Cindro, V Cioara, IA Ciocio, A Cirotto, F Citron, ZH Ciubancan, M Clark, A Clark, BL Clark, PJ Clarke, RN Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Cogan, JG Colasurdo, L Cole, B Cole, S Colijn, AP Collot, J Colombo, T Compostella, G Muino, PC 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Regie, JBD Dearnaley, WJ Debbe, R Debenedetti, C Dedovich, DV Deigaard, I Del Peso, J Del Prete, T Delgove, D Deliot, F Delitzsch, CM Deliyergiyev, M Dell'Acqua, A Dell'Asta, L Dell'Orso, M Della Pietra, M della Volpe, D Delmastro, M Delsart, PA Deluca, C DeMarco, DA Demers, S Demichev, M Demilly, A Denisov, SP Derendarz, D Derkaoui, JE Derue, F Dervan, P Desch, K Deterre, C Deviveiros, PO Dewhurst, A Dhaliwal, S Di Ciaccio, A Di Ciaccio, L Di Domenico, A Di Donato, C Di Girolamo, A Di Girolamo, B Di Mattia, A Di Micco, B Di Nardo, R Di Simone, A Di Sipio, R Di Valentino, D Diaconu, C Diamond, M Dias, FA Diaz, MA Diehl, EB Dietrich, J Diglio, S Dimitrievska, A Dingfelder, J Dita, P Dita, S Dittus, F Djama, F Djobava, T Djuvsland, JI do Vale, MAB Dobos, D Dobre, M Doglioni, C Dohmae, T Dolejsi, J Dolezal, Z Dolgoshein, BA Donadelli, M Donati, S Dondero, P Donini, J Dopke, J Doria, A Dova, MT Doyle, AT Drechsler, E Dris, M Dubreui, E Duchovni, E Duckeck, G Ducu, OA Duda, D Dudarev, A 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Zhang, D. Zhang, F. Zhang, G. Zhang, H. Zhang, J. Zhang, L. Zhang, R. Zhang, X. Zhang, Z. Zhao, X. Zhao, Y. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Summary of the ATLAS experiment's sensitivity to supersymmetry after LHC Run 1-interpreted in the phenomenological MSSM SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID GRAND UNIFIED THEORIES; DYNAMICAL SYMMETRY-BREAKING; NEUTRALINO DARK-MATTER; EVEN HIGGS BOSONS; STANDARD MODEL; SUPERGAUGE TRANSFORMATIONS; COUPLING-CONSTANTS; HADRON COLLIDERS; PROGRAM; UNIFICATION AB A summary of the constraints from the ATLAS experiment on R-parity-conserving supersymmetry is presented. Results from 22 separate ATLAS searches are considered, each based on analysis of up to 20.3 fb(-1) of proton-proton collision data at centre-of-mass energies of root s = 7 and 8TeV at the Large Hadron Collider. The results are interpreted in the context of the 19-parameter phenomenological minimal supersymmetric standard model, in which the lightest supersymmetric particle is a neutralino, taking into account constraints from previous precision electroweak and flavour measurements as well as from dark matter related measurements. The results are presented in terms of constraints on supersymmetric particle masses and are compared to limits from simplified models. The impact of ATLAS searches on parameters such as the dark matter relic density, the couplings of the observed Higgs boson, and the degree of electroweak fine-tuning is also shown. Spectra for surviving supersymmetry model points with low fine-tunings are presented. C1 [Jackson, P.; Lee, L.; Petridis, A.; Soni, N.; White, M. 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V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Xu, L.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. Transilvania Univ Brasov, Brasov, Romania. [Alex, C.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Gonzalez, B. Alvarez; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beermann, T. A.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Carrillo-Montoya, G. D.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Feng, E. J.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Gadatsch, S.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jaekel, M. R.; Jakobsen, S.; Jenni, P.; Klioutchnikova, T.; Krasznahorkay, A.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Ruthmann, N.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sforza, F.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Blunier, S.; Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Loyola, J. E. Salazar; Araya, S. Tapia; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Zhang, G.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, L.; Li, Y.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Liu, B.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreui, E.; Gilles, G.; Gris, Ph; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreui, E.; Gilles, G.; Gris, Ph; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreui, E.; Gilles, G.; Gris, Ph; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Carbone, R. M.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, INFN, Grp Collegato Cosenza, Lab Nazl Frascati, I-87036 Arcavacata Di Rende, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Kisielewska, D.; Kopernya, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Troncona, M. Trzebinski; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Bessner, M.; Boch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Hamburg, Germany. [Asbah, N.; Bessner, M.; Boch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Calace, N.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nessi, M.; Paolozzi, L.; Picazio, A.; Ristic, B.; Schramm, S.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Univ Genoa, INFN, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schutz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolb, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores; Salvucci, A.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Jussel, P.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Univ Salento, INFN, Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Egham, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fys Inst, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Zhang, R.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Zhang, R.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Guo, Y.; Hu, X.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Tollefson, K.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Univ Milan, INFN, Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu; Smirnov, Y.; Soldatov, E. Yu; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Anders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph; Spettel, F.; Stonjck, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Univ Naples Federico II, INFN, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Koenig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; Van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; Van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Fawcett, W. J.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Univ Pavia, INFN, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Machado Miguens, J.; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Natl Res Ctr, Kurchatov Inst, BP Konstantinov Petersburg Nucl Phys Inst, St Petersburg, Russia. [Annovi, A.; Beecherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, INFN, Sez Pisa, Pisa, Italy. [Annovi, A.; Beecherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguiar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguiar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguiar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Castro, N. F.] Univ Nova Lisboa, Dep Fis, Caparica, Portugal. [Castro, N. F.] Univ Nova Lisboa, CEFITEC Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Tarchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bance, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, INFN, Sez Roma, I-00185 Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bance, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, INFN, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Univ Rome Tre, INFN, Sez Roma Tre, I-00146 Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseal Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph; Schwemling, Ph; Schwindling, J.] CEA Saclay Commissariat Energie Atom & Energies A, DSM IRFU Inst Rech Lois Fondamentales Univers, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Hance, M.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Lee, C. A.; Meehan, S.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hsu, C.; Kar, D.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Song, H. Y.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Jovicevic, J.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] INFN, Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Gradin, P. O. J.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Iries Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Iries Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Iries Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Iries Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Iries Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; Gignac, M.; Henkelmann, S.; King, S. B.; Lister, A.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Pearce, J.; Sobie, R.; Trovatelli, M.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.; Spangenberg, M.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kaplan, L. S.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Braun, H. M.; Cornelissen, T.; Ellinghaus, F.; Ernis, G.; Fischer, J.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Thomsen, L. A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] IN2P3, Ctr Calcul, Villeurbanne, France. 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[Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Khubua, J.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellen Open Univ, Patras, Greece. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei 115, Taiwan. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Rizzo, T. G.] SLAC Natl Accelerator Lab, Theory Dept, Stanford, CA USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Prokoshin, Fedor/E-2795-2012; Stabile, Alberto/L-3419-2016; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Gavrilenko, Igor/M-8260-2015; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Fabbri, Laura/H-3442-2012; Gutierrez, Phillip/C-1161-2011; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Brooks, William/C-8636-2013; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Fedin, Oleg/H-6753-2016; Snesarev, Andrey/H-5090-2013; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; Villa, Mauro/C-9883-2009; Chiarelli, Giorgio/E-8953-2012; La Rosa Navarro, Jose Luis/K-4221-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Tripiana, Martin/H-3404-2015; Smirnova, Oxana/A-4401-2013; Savarala, Hari Krishna/A-3516-2015; Doyle, Anthony/C-5889-2009; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Boyko, Igor/J-3659-2013; Vranjes Milosavljevic, Marija/F-9847-2016; Chekulaev, Sergey/O-1145-2015; Zhukov, Konstantin/M-6027-2015; SULIN, VLADIMIR/N-2793-2015; Peleganchuk, Sergey/J-6722-2014; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Garcia, Jose /H-6339-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; la rotonda, laura/B-4028-2016; Mitsou, Vasiliki/D-1967-2009; Di Domenico, Antonio/G-6301-2011; Livan, Michele/D-7531-2012; Gladilin, Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Tikhomirov, Vladimir/M-6194-2015; Carvalho, Joao/M-4060-2013; White, Ryan/E-2979-2015; Mashinistov, Ruslan/M-8356-2015; Warburton, Andreas/N-8028-2013; spagnolo, stefania/A-6359-2012; Buttar, Craig/D-3706-2011 OI Prokoshin, Fedor/0000-0001-6389-5399; Stabile, Alberto/0000-0002-6868-8329; Kukla, Romain/0000-0002-1140-2465; Gauzzi, Paolo/0000-0003-4841-5822; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Brooks, William/0000-0001-6161-3570; Vykydal, Zdenek/0000-0003-2329-0672; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Villa, Mauro/0000-0002-9181-8048; Chiarelli, Giorgio/0000-0001-9851-4816; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Smirnova, Oxana/0000-0003-2517-531X; Savarala, Hari Krishna/0000-0001-6593-4849; Doyle, Anthony/0000-0001-6322-6195; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Boyko, Igor/0000-0002-3355-4662; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Belanger-Champagne, Camille/0000-0003-2368-2617; Sotiropoulou, Calliope-Louisa/0000-0001-9851-1658; Prokofiev, Kirill/0000-0002-2177-6401; Veneziano, Stefano/0000-0002-2598-2659; Lacasta, Carlos/0000-0002-2623-6252; Price, Darren/0000-0003-2750-9977; Terzo, Stefano/0000-0003-3388-3906; Smirnov, Sergei/0000-0002-6778-073X; Coccaro, Andrea/0000-0003-2368-4559; Cristinziani, Markus/0000-0003-3893-9171; Galhardo, Bruno/0000-0003-0641-301X; Della Volpe, Domenico/0000-0001-8530-7447; Pina, Joao /0000-0001-8959-5044; Farrington, Sinead/0000-0001-5350-9271; Robson, Aidan/0000-0002-1659-8284; Weber, Michele/0000-0002-2770-9031; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Gray, Heather/0000-0002-5293-4716; Dell'Asta, Lidia/0000-0002-9601-4225; Sannino, Mario/0000-0001-7700-8383; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; la rotonda, laura/0000-0002-6780-5829; Amorim, Antonio/0000-0003-0638-2321; Mitsou, Vasiliki/0000-0002-1533-8886; Di Domenico, Antonio/0000-0001-8078-2759; Livan, Michele/0000-0002-5877-0062; Gladilin, Leonid/0000-0001-9422-8636; Andreazza, Attilio/0000-0001-5161-5759; Tikhomirov, Vladimir/0000-0002-9634-0581; Carvalho, Joao/0000-0002-3015-7821; White, Ryan/0000-0003-3589-5900; Mashinistov, Ruslan/0000-0001-7925-4676; Warburton, Andreas/0000-0002-2298-7315; spagnolo, stefania/0000-0001-7482-6348; FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; RGC, China; Hong Kong SAR, China; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern, Switzerland; Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; RGC, Hong Kong SAR, China; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 160 TC 20 Z9 20 U1 12 U2 73 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD OCT 21 PY 2015 IS 10 AR 134 DI 10.1007/JHEP10(2015)134 PG 76 WC Physics, Particles & Fields SC Physics GA CU5GP UT WOS:000363560400004 ER PT J AU Vigil, JA Lambert, TN Eldred, K AF Vigil, Julian A. Lambert, Timothy N. Eldred, Kaitlyn TI Electrodeposited MnOx/PEDOT Composite Thin Films for the Oxygen Reduction Reaction SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE catalysis; oxygen reduction reaction; manganese oxide; PEDOT; electrodeposition ID OXIDE ELECTROCATALYSTS; WATER OXIDATION; AQUEOUS-MEDIUM; CATALYST; PEDOT; GRAPHENE AB Manganese oxide (MnOx) was anodically coelectrodeposited with poly(3,4-ethylenedioxythiophene) (PEDOT) from an aqueous solution of Mn(OAc)2, 3,4ethylenedioxythiophene, LiClO4 and sodium dodecyl sulfate to yield a MnOx/PEDOT composite thin film. The MnOx/ PEDOT film showed significant improvement over the MnOx only and PEDOT only films for the oxygen reduction reaction, with a >0.2 V decrease in onset and half-wave overpotential and >1.5 times increase in current density. Furthermore, the MnOx/PEDOT films were competitive with commercial benchmark 20% Pt/C, outperforming it in the half-wave ORR region and exhibiting better electrocatalytic selectivity for the oxygen reduction reaction upon methanol exposure. The high activity of the MnOx/PEDOT composite is attributed to synergistic charge transfer coelectrodepositing MnOx with a conductive polymer while simultaneously achieving intimate substrate capabilities, attained by contact. C1 [Vigil, Julian A.; Lambert, Timothy N.; Eldred, Kaitlyn] Sandia Natl Labs, Dept Mat Devices & Energy Technol, Albuquerque, NM 87185 USA. RP Lambert, TN (reprint author), Sandia Natl Labs, Dept Mat Devices & Energy Technol, POB 5800, Albuquerque, NM 87185 USA. EM tnlambe@sandia.gov FU Laboratory Directed Research and Development program at Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the Laboratory Directed Research and Development program at Sandia National Laboratories, a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration, under contract DE-AC04-94AL85000. Ms. Bonnie McKenzie is thanked for her technical assistance with SEM imaging and EDS elemental analysis. NR 35 TC 7 Z9 7 U1 13 U2 56 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD OCT 21 PY 2015 VL 7 IS 41 BP 22745 EP 22750 DI 10.1021/acsami.5b07684 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CU3PT UT WOS:000363438000003 PM 26444641 ER PT J AU Teng, X Zhan, C Bai, Y Ma, L Liu, Q Wu, C Wu, F Yang, YS Lu, J Amine, K AF Teng, Xin Zhan, Chun Bai, Ying Ma, Lu Liu, Qj Wu, Chuan Wu, Feng Yang, Yusheng Lu, Jun Amine, Khalil TI In Situ Analysis of Gas Generation in Lithium-Ion Batteries with Different Carbonate-Based Electrolytes SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE lithium ion battery; carbonate electrolytes; gas generation; pouch cells; density function theory ID SPECTROSCOPY; MICROSCOPY; ELECTRODES; CELLS; SEI AB Gas generation in lithium-ion batteries is one of the critical issues limiting their safety performance and lifetime. In this work, a set of 900 mAh pouch cells were applied to systematically compare the composition of gases generated from a serial of carbonate-based composite electrolytes, using a self-designed gas analyzing system. Among electrolytes used in this work, the composite gamma-butyrolactone/ethyl methyl carbonate (GBL/EMC) exhibited remarkably less gassing because of the electrochemical stability of the GBL, which makes it a promising electrolyte for battery with advanced safety and lifetime. C1 [Teng, Xin; Bai, Ying; Liu, Qj; Wu, Chuan; Wu, Feng; Yang, Yusheng] Beijing Inst Technol, Sch Mat Sci & Engn, Beijing Key Lab Environm Sci & Engn, Beijing 100081, Peoples R China. [Zhan, Chun; Lu, Jun; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Ma, Lu] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Wu, Chuan; Wu, Feng] Collaborat Innovat Ctr Elect Vehicles Beijing, Beijing 100081, Peoples R China. RP Bai, Y (reprint author), Beijing Inst Technol, Sch Mat Sci & Engn, Beijing Key Lab Environm Sci & Engn, Beijing 100081, Peoples R China. EM membrane@bit.edu.cn; junlu@anl.gov RI wu, chuan/A-1447-2009 FU National Basic Research Program of China [2015CB251100]; New Century Excellent Talents in University [NCET-13-0033]; Beijing Co-construction Project [20150939014]; State Scholarship Fund of China Scholarship Council [201406035025]; Center for Electrical Energy Storage, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX This work is supported by the National Basic Research Program of China (2015CB251100), the Program for New Century Excellent Talents in University (NCET-13-0033), and the Beijing Co-construction Project (20150939014). The authors acknowledge Bryan Wood and Brian Way in BAK Canada for their support in gas components detection. Y.B. acknowledges the support from the State Scholarship Fund (201406035025) of the China Scholarship Council. C.Z, J.L., and K.A. were supported by the Center for Electrical Energy Storage, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. NR 22 TC 4 Z9 4 U1 6 U2 46 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD OCT 21 PY 2015 VL 7 IS 41 BP 22751 EP 22755 DI 10.1021/acsami.5b08399 PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CU3PT UT WOS:000363438000004 PM 26417916 ER PT J AU Petkov, V Prasai, B Shastri, S Chen, TY AF Petkov, Valeri Prasai, Binay Shastri, Sarvjit Chen, Tsan-Yao TI 3D Atomic Arrangement at Functional Interfaces Inside Nanoparticles by Resonant High-Energy X-ray Diffraction SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE composite metallic nanoparticles for catalytic applications; 3D atomic structure; resonant high-energy X-ray diffraction; element specific atomic pair distribution functions; reverse Monte Carlo simulations ID CORE-SHELL NANOPARTICLES; CARBON-MONOXIDE; FUEL-CELLS; METHANOL ELECTROOXIDATION; INTERMETALLIC COMPOUNDS; OXYGEN REDUCTION; RU; CATALYSTS; NANOCRYSTALS; OXIDATION AB With current science and technology moving rapidly into smaller scales, nanometer-sized materials, often referred to as NPs, are produced in increasing numbers and explored for numerous useful applications. Evidence is mounting, however, that useful properties of NPs can be improved further and even new NP functionality achieved by not only controlling the NP size and shape but also interfacing chemically or structurally distinct entities into single, so-called "composite" NPs. A typical example is core shell NPs wherein the synergy of distinct atoms at the core\shell interface endows the NPs with otherwise unachievable functionality. However, though advantageous, the concept of functional interfaces inside NPs is still pursued largely by trial-and-error. That is because it is difficut to assess the interfaces precisely at the atomic level using traditional experimental techniques and, hence, difficult to take control of. Using the core\shell interface in less than 10 nm in size Ru core-Pt shells NPs as an example, we demonstrate that precise knowledge of the 3D atomic arrangement at functional interfaces inside NPs can be obtained by resonant high-energy X-ray diffraction (XRD) coupled to element-specific atomic pair distribution function (PDF) analysis. On the basis of the unique structure knowledge obtained, we scrutinize the still-debatable influence of core\shell interface on the catalytic functionality of Ru core-Pt shell NPs, thus evidencing the usefulness of this nontraditional technique for practical applications. C1 [Petkov, Valeri; Prasai, Binay] Cent Michigan Univ, Dept Phys, Mt Pleasant, MI 48859 USA. [Shastri, Sarvjit] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Chen, Tsan-Yao] Natl Tsing Hua Univ, Dept Engn & Syst Sci, Hsinchu 30013, Taiwan. RP Petkov, V (reprint author), Cent Michigan Univ, Dept Phys, Mt Pleasant, MI 48859 USA. EM petkolvg@cmich.edu FU DOE-BES [DE-SC0006877]; DOE [DEAC02-06CH11357] FX Work for this study was supported by DOE-BES Grant DE-SC0006877. Work at the Advanced Photion Source was supported by DOE under Contract DEAC02-06CH11357. Thanks are due to the group of Prof. C.J. Zhong from SUNY, Binghamton, for providing Pt-Ru alloy NPs. NR 70 TC 0 Z9 0 U1 4 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD OCT 21 PY 2015 VL 7 IS 41 BP 23265 EP 23277 DI 10.1021/acsami.5b07391 PG 13 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CU3PT UT WOS:000363438000062 PM 26415142 ER PT J AU Lu, WB Kumar, P Smoot, GF AF Lu, Wenbin Kumar, Pawan Smoot, George F. TI Probing massive stars around gamma-ray burst progenitors SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE radiation mechanisms: non-thermal; methods: analytical; gamma-ray burst: general ID HIGH-ENERGY EMISSION; EXTRAGALACTIC BACKGROUND LIGHT; CHERENKOV TELESCOPE ARRAY; CORE-COLLAPSE SUPERNOVAE; RELATIVISTIC BLAST WAVES; COMPTON-SCATTERING; POPULATION III; BINARY STARS; GRB 130427A; JETS AB Long gamma-ray bursts (GRBs) are produced by ultra-relativistic jets launched from core collapse of massive stars. Most massive stars form in binaries and/or in star clusters, which means that there may be a significant external photon field (EPF) around the GRB progenitor. We calculate the inverse-Compton scattering of EPF by the hot electrons in the GRB jet. Three possible cases of EPF are considered: the progenitor is (I) in a massive binary system, (II) surrounded by aWolf-Rayet-star wind and (III) in a dense star cluster. Typical luminosities of 10(46)-10(50) erg s(-1) in the 1-100 GeV band are expected, depending on the stellar luminosity, binary separation (I), wind mass-loss rate (II), stellar number density (III), etc. We calculate the light curve and spectrum in each case, taking fully into account the equal-arrival time surfaces and possible pair-production absorption with the prompt gamma-rays. Observations can put constraints on the existence of such EPFs (and hence on the nature of GRB progenitors) and on the radius where the jet internal dissipation process accelerates electrons. C1 [Lu, Wenbin; Kumar, Pawan] Univ Texas Austin, Dept Astron, Austin, TX 78712 USA. [Smoot, George F.] Univ Paris Diderot, Univ Sorbonne Paris Cite, APC, PCCP, F-75013 Paris, France. Univ Calif Berkeley, LBNL, BCCP, Berkeley, CA 94720 USA. Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RP Lu, WB (reprint author), Univ Texas Austin, Dept Astron, RLM 15308, Austin, TX 78712 USA. EM wenbinlu@astro.as.utexas.edu FU Chaire d'Excellence Universite Sorbonne Paris Cite; UnivEarthS Labex program at Universite Sorbonne Paris Cite [ANR-10-LABX-0023, ANR-11-IDEX-0005-02] FX The authors thank M. Milosavljevic, P. Crumley, R. Santana, R. Hernandez for helpful discussions. GFS acknowledges support through his Chaire d'Excellence Universite Sorbonne Paris Cite and the financial support of the UnivEarthS Labex program at Universite Sorbonne Paris Cite (ANR-10-LABX-0023 and ANR-11-IDEX-0005-02). NR 63 TC 1 Z9 1 U1 1 U2 2 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD OCT 21 PY 2015 VL 453 IS 2 BP 1458 EP 1470 DI 10.1093/mnras/stv1677 PG 13 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CU4GQ UT WOS:000363486000023 ER PT J AU Ng, KY Dawson, WA Wittman, D Jee, MJ Hughes, JP Menanteau, F Sifon, C AF Ng, Karen Y. Dawson, William A. Wittman, D. Jee, M. James Hughes, John P. Menanteau, Felipe Sifon, Cristobal TI The return of the merging galaxy subclusters of El Gordo? SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE methods: statistical; galaxies: clusters: individual (ACT-CL J0102-4915); galaxies: high-redshift; cosmology: observations; dark matter ID INTERACTION CROSS-SECTION; CLUSTER RADIO RELICS; ACT-CL J0102-4915; DARK-MATTER; BULLET CLUSTER; COLD FRONTS; COSMOLOGY; MERGERS; 1E-0657-56; SCALE AB Merging galaxy clusters with radio relics provide rare insights to the merger dynamics as the relics are created by the violent merger process. We demonstrate one of the first uses of the properties of the radio relic to reduce the uncertainties of the dynamical variables and determine the three-dimensional (3D) configuration of a cluster merger, ACT-CL J0102-4915, nicknamed El Gordo. From the double radio relic observation and the X-ray observation of a comet-like gas morphology induced by motion of the cool core, it is widely believed that El Gordo is observed shortly after the first core passage of the subclusters. We employ a Monte Carlo simulation to investigate the 3D configuration and dynamics of El Gordo. Using the polarization fraction of the radio relic, we constrain the estimate of the angle between the plane of the sky and the merger axis to be alpha = 21. +/-(9)(11). We find the relative 3D merger speed of El Gordo to be 2400 +/-(400)(200) km s(-1) at pericentre. The two possible estimates of the time since pericentre (TSP) are 0.46 +/-(0.09)(0.16) and 0.91 +/-(0.22)(0.39) Gyr for the outgoing and returning scenario, respectively. We put our estimates of the TSP into context by showing that if the time-averaged shock velocity is approximately equal to or smaller than the pericentre velocity of the corresponding subcluster in the centre-of-mass frame, the two subclusters are more likely to be moving towards, rather than away, from each other, post apocentre. We compare and contrast the merger scenario of El Gordo with that of the Bullet Cluster, and show that this late-stage merging scenario explains why the south-east (SE) dark matter lensing peak of El Gordo is closer to the merger centre than the SE cool core. C1 [Ng, Karen Y.; Wittman, D.; Jee, M. James] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Dawson, William A.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Jee, M. James] Yonsei Univ, Dept Astron, Seoul 120749, South Korea. [Hughes, John P.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Menanteau, Felipe] Univ Illinois, Natl Ctr Supercomp Applicat, Urbana, IL 61801 USA. [Menanteau, Felipe] Univ Illinois, Dept Astron, Urbana, IL 61801 USA. [Sifon, Cristobal] Leiden Univ, Leiden Observ, NL-2300 RA Leiden, Netherlands. RP Ng, KY (reprint author), Univ Calif Davis, Dept Phys, One Shields Ave, Davis, CA 95616 USA. EM karenyng@ucdavis.edu OI Menanteau, Felipe/0000-0002-1372-2534; Sifon, Cristobal/0000-0002-8149-1352; Wittman, David/0000-0002-0813-5888 FU U.S. DOE by LLNL [DE-AC52-07NA27344]; Chandra [GO2-13156X]; Hubble [HST-GO-12755.01-A]; NRF of Korea FX We thank Franco Vazza, Marcus Bruggen and Surajit Paul for sharing their knowledge on the simulated properties of radio relic and merger shocks. We extend our gratitude to Reinout Van Weeren for first proposing the use of radio relic to weight the Monte Carlo realizations. We appreciate the comments from Marusa Bradac about using the position of the relic to break degeneracy of the merger scenario. KN is grateful to Paul Baines and Tom Loredo for discussion of the use of prior information and sensitivity tests. Part of this work was performed under the auspices of the U.S. DOE by LLNL under Contract DE-AC52-07NA27344. JPH gratefully acknowledges support from Chandra (grant number GO2-13156X) and Hubble (grant number HST-GO-12755.01-A). MJJ acknowledges support from NRF of Korea to CGER. We would also like to thank GitHub for providing free repository for version control for our data and analyses. This research made use of APLPY, an open-source plotting package for PYTHON hosted at http://aplpy.github.com; ASTROPY, a community-developed core PYTHON package for Astronomy (Robitaille et al. 2013); ASTROML, a machine learning library for astrophysics (VanderPlas et al. 2012) and IPYTHON, a system for interactive scientific computing, computing in science and engineering (Perez & Granger 2007). NR 43 TC 6 Z9 6 U1 0 U2 0 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD OCT 21 PY 2015 VL 453 IS 2 BP 1531 EP 1549 DI 10.1093/mnras/stv1713 PG 19 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CU4GQ UT WOS:000363486000029 ER PT J AU Ma, XD Baldwin, JKS Hartmann, NF Doorn, SK Htoon, H AF Ma, Xuedan Baldwin, Jon K. S. Hartmann, Nicolai F. Doorn, Stephen K. Htoon, Han TI Solid-State Approach for Fabrication of Photostable, Oxygen-Doped Carbon Nanotubes SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article DE electron beam evaporation; oxygen-doping; photoluminescence; single-photon sources; single-walled carbon nanotubes ID QUANTUM DOTS; AQUEOUS DISPERSIONS; ROOM-TEMPERATURE; PHOTOLUMINESCENCE; SURFACTANTS; SOLUBILIZATION; NANOCRYSTALS; FLUORESCENCE; EMISSION; KINETICS AB A novel procedure for effective fabrication of photostable oxygen-doped single-walled carbon nanotubes (SWCNTs) in solid-state matrices has been developed. SWCNTs drop-cast on various types of substrates are coated with oxide dielectric thin films by electron-beam evaporation. Single tube photoluminescence spectroscopy studies performed at room and cryogenic temperatures reveal that such thin film-coated tubes exhibit characteristic spectral features of oxygen-doped SWCNTs, indicating the oxide thin film coating process leads to oxygen doping of the tubes. It is also found that the doping efficiency can be effectively controlled by the thin film deposition time and by the types of surfactants wrapping the SWCNTs. Moreover, aside from being the doping agent, the oxide thin film also serves as a passivation layer protecting the SWCNTs from the external environment. Comparing the thin film coated SWCNTs with oxygen-doped tubes prepared via ozonolysis, the former exhibit significantly higher photostability and photoluminescence on-time. Therefore, this one-step deposition/oxygen-doping procedure provides a possible route toward scalable, versatile incorporation of highly photostable oxygen-doped SWCNTs in novel optical and optoelectronic devices. C1 [Ma, Xuedan; Baldwin, Jon K. S.; Hartmann, Nicolai F.; Doorn, Stephen K.; Htoon, Han] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. RP Ma, XD (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol, POB 5800, Albuquerque, NM 87185 USA. EM skdoorn@lanl.gov; htoon@lanl.gov OI Hartmann, Nicolai/0000-0002-4174-532X; Htoon, Han/0000-0003-3696-2896 FU Los Alamos National Laboratory (LANL) Directed Research and Development Funds FX This work was conducted at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility and supported in part by Los Alamos National Laboratory (LANL) Directed Research and Development Funds. The authors thank Erik H. Haroz of LANL for insightful discussion on surfactant chemistries of SWCNTs. NR 53 TC 2 Z9 2 U1 4 U2 36 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD OCT 21 PY 2015 VL 25 IS 39 BP 6157 EP 6164 DI 10.1002/adfm.201502580 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CU0LD UT WOS:000363207000001 ER PT J AU Kiriya, D Zhou, YZ Nelson, C Hettick, M Madhvapathy, SR Chen, K Zhao, PD Tosun, M Minor, AM Chrzan, DC Javey, A AF Kiriya, Daisuke Zhou, Yuzhi Nelson, Christopher Hettick, Mark Madhvapathy, Surabhi Rao Chen, Kevin Zhao, Peida Tosun, Mahmut Minor, Andrew M. Chrzan, Daryl C. Javey, Ali TI Oriented Growth of Gold Nanowires on MoS2 SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article DE field effect transistors (FET); nanowires; transition metal dichalcogenides ID DER-WAALS EPITAXY; TRANSITION-METAL DICHALCOGENIDES; CONTROLLED ORIENTATIONS; CARBON NANOTUBES; GUIDED GROWTH; ZNO NANOWIRES; GRAPHENE; NANOSHEETS; NANOSTRUCTURES; NANOCRYSTALS AB Layered 2D materials serve as a new class of substrates for templated synthesis of various nanomaterials even with highly dissimilar crystal structures; thus overcoming the lattice constraints of conventional epitaxial processes. Here, molybdenum disulfide (MoS2) is used as a prototypical model substrate for oriented growth of in-plane Au nanowires (NWs) despite the nearly 8% lattice mismatch between MoS2 and Au. Au NWs on the MoS2 surface are oriented along three symmetrically equivalent directions within the substrate arising from the strong Au-S binding that templates the oriented growth. The kinetics of the growth process are explored through experiments and modeling. Strong charge transfer is observed between Au NWs and MoS2, resulting in degenerate p-doping of MoS2. C1 [Kiriya, Daisuke; Hettick, Mark; Madhvapathy, Surabhi Rao; Chen, Kevin; Zhao, Peida; Tosun, Mahmut; Javey, Ali] Univ Calif Berkeley, Elect Engn & Comp Sci, Berkeley, CA 94720 USA. [Kiriya, Daisuke; Zhou, Yuzhi; Hettick, Mark; Madhvapathy, Surabhi Rao; Chen, Kevin; Zhao, Peida; Tosun, Mahmut; Chrzan, Daryl C.; Javey, Ali] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Kiriya, Daisuke; Hettick, Mark; Chen, Kevin; Zhao, Peida; Tosun, Mahmut; Javey, Ali] Univ Calif Berkeley, Berkeley Sensor & Actuator Ctr, Berkeley, CA 94720 USA. [Zhou, Yuzhi; Minor, Andrew M.; Chrzan, Daryl C.] Univ Calif Berkeley, Mat Sci & Engn, Berkeley, CA 94720 USA. [Nelson, Christopher; Minor, Andrew M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA. RP Kiriya, D (reprint author), Univ Calif Berkeley, Elect Engn & Comp Sci, Berkeley, CA 94720 USA. EM ajavey@berkeley.edu RI Javey, Ali/B-4818-2013 FU Office of Science, Office of Basic Energy Sciences, Material Sciences and Engineering Division of the US Department of Energy [DE-AC02-05CH11231]; Center for Low Energy Systems Technology (LEAST), one of six centers - STARnet phase of the Focus Center Research Program (FCRP), a Semiconductor Research Corporation program - MARCO; Center for Low Energy Systems Technology (LEAST), one of six centers - STARnet phase of the Focus Center Research Program (FCRP), a Semiconductor Research Corporation program - DARPA; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science of the US Department of Energy [DE-SC0004993] FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Material Sciences and Engineering Division of the US Department of Energy under Contract No. DE-AC02-05CH11231. The device fabrication and characterization was funded by the Center for Low Energy Systems Technology (LEAST), one of six centers supported by the STARnet phase of the Focus Center Research Program (FCRP), a Semiconductor Research Corporation program sponsored by MARCO and DARPA. The transmission electron microscopy and XRD were performed at the Molecular Foundry, supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. XPS characterization was performed at the Joint Center for Artificial Photosynthesis, supported through the Office of Science of the US Department of Energy under Award Number DE-SC0004993. NR 45 TC 5 Z9 5 U1 18 U2 104 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD OCT 21 PY 2015 VL 25 IS 39 BP 6257 EP 6264 DI 10.1002/adfm.201502582 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CU0LD UT WOS:000363207000012 ER PT J AU Lu, XC Bowden, ME Sprenkle, VL Liu, J AF Lu, Xiaochuan Bowden, Mark E. Sprenkle, Vincent L. Liu, Jun TI A Low Cost, High Energy Density, and Long Cycle Life Potassium-Sulfur Battery for Grid-Scale Energy Storage SO ADVANCED MATERIALS LA English DT Article DE alkali metal-sulfur batteries; potassium-sulfur batteries; electrolytes; potassium anodes; lower operating temperatures ID BETA-ALUMINA; RAMAN-SPECTROSCOPY; CHLORIDE BATTERY; RESISTANCE RISE; ION-EXCHANGE; SODIUM; TEMPERATURE; ANIONS; CELLS AB A potassium-sulfur battery using K+ conducting beta-alumina as the electrolyte to separate a molten potassium metal anode and a sulfur cathode is presented. The results indicate that the battery can operate at as low as 150 degrees C with excellent performance. This study demon strates a new type of high-performance metal-sulfur battery that is ideal for grid-scale energy-storage applications. C1 [Lu, Xiaochuan; Sprenkle, Vincent L.; Liu, Jun] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. [Bowden, Mark E.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Lu, XC (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. EM Xiaochuan.Lu@pnnl.gov FU US Department of Energy's (DOE's) Office of Electricity Delivery & Energy Reliability (OE); Department of Energy [DE-AC05-76RL01830] FX This work was supported by the US Department of Energy's (DOE's) Office of Electricity Delivery & Energy Reliability (OE). The authors appreciate the useful discussions with Dr. I. Gyuk of the DOE-OE Grid Storage Program. PNNL is a multi-program laboratory operated by Battelle Memorial Institute for the Department of Energy under Contract DE-AC05-76RL01830. NR 42 TC 11 Z9 11 U1 48 U2 141 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD OCT 21 PY 2015 VL 27 IS 39 BP 5915 EP 5922 DI 10.1002/adma.201502343 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CU0KM UT WOS:000363205200009 PM 26305734 ER PT J AU Huang, K Wu, YT Dai, S AF Huang, Kuan Wu, You-Ting Dai, Sheng TI Sigmoid Correlations for Gas Solubility and Enthalpy Change of Chemical Absorption of CO2 SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID FUNCTIONALIZED IONIC LIQUIDS; ESTIMATING ENTROPY CHANGES; CARBON-DIOXIDE CAPTURE; AQUEOUS AMINE SYSTEMS; N-METHYLDIETHANOLAMINE; THERMODYNAMIC ANALYSIS; HYDROGEN-SULFIDE; CAMPBELLS RULE; TEMPERATURE; ANION AB Knowledge of the relationship between gas solubility and enthalpy change of chemical absorption of CO, is very important for exploring energy-efficient absorbents for CO2 capture. To this end, equations that can directly correlate gas solubility with absorption enthalpy were derived through combining the van't Hoff equation with the reaction equilibrium thermodynamic model (RETM). Two typical reaction mechanisms for chemical absorption of CO2 (1:1 and 1:2) were considered for RETM. The variations of gas solubility with enthalpy change were found to be distinctively sigmoid functions, regardless of the investigated temperature and pressure or assumed reaction forms between CO2 and the absorbent molecule. Theoretically calculated variation curves of gas solubility vs enthalpy change agreed well with experimental results reported in literature. On the basis of the trade-off relationship between gas solubility and enthalpy change, criterions for evaluating energy-efficient chemical absorbents for CCO2 capture were proposed. C1 [Huang, Kuan; Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Huang, Kuan; Wu, You-Ting] Nanjing Univ, Sch Chem & Chem Engn, Nanjing 210093, Jiangsu, Peoples R China. [Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Wu, YT (reprint author), Nanjing Univ, Sch Chem & Chem Engn, Nanjing 210093, Jiangsu, Peoples R China. EM ytwu@nju.edu.cn; dais@ornl.org RI Dai, Sheng/K-8411-2015; Huang, Kuan/F-7003-2015 OI Dai, Sheng/0000-0002-8046-3931; Huang, Kuan/0000-0003-1905-3017 FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy [De-AC05-00OR22725]; Oak Ridge National Laboratory; National Natural Science Foundation of China [21376115]; China Scholarship Council FX S.D. was sponsored by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy, under Contract No. De-AC05-00OR22725 with Oak Ridge National Laboratory managed and operated by UT-Battelle, LLC. Y.W. was supported by the National Natural Science Foundation of China under Agreement 21376115. K.H. acknowledges China Scholarship Council for partial financial support. NR 44 TC 2 Z9 2 U1 7 U2 46 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD OCT 21 PY 2015 VL 54 IS 41 BP 10126 EP 10133 DI 10.1021/acs.iecr.5b02145 PG 8 WC Engineering, Chemical SC Engineering GA CU3PY UT WOS:000363438500019 ER PT J AU Mirzaei, S Kremer, F Sprouster, DJ Araujo, LL Feng, R Glover, CJ Ridgway, MC AF Mirzaei, S. Kremer, F. Sprouster, D. J. Araujo, L. L. Feng, R. Glover, C. J. Ridgway, M. C. TI Formation of Ge nanoparticles in SiOxNy by ion implantation and thermal annealing SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID RAMAN-SCATTERING; SIO2 MATRIX; THIN-FILMS; NANOCRYSTALS; SILICON; SPECTRA; GROWTH; LAYERS; DOTS AB Germanium nanoparticles embedded within dielectric matrices hold much promise for applications in optoelectronic and electronic devices. Here we investigate the formation of Ge nanoparticles in amorphous SiO1.67N0.14 as a function of implanted atom concentration and thermal annealing temperature. Using x-ray absorption spectroscopy and other complementary techniques, we show Ge nanoparticles exhibit significant finite-size effects such that the coordination number decreases and structural disorder increases as the nanoparticle size decreases. While the composition of SiO1.67N0.14 is close to that of SiO2, we demonstrate that the addition of this small fraction of N yields a much reduced nanoparticle size relative to those formed in SiO2 under comparable implantation and annealing conditions. We attribute this difference to an increase in an atomic density and a much reduced diffusivity of Ge in the oxynitride matrix. These results demonstrate the potential for tailoring Ge nanoparticle sizes and structural properties in the SiOxNy matrices by controlling the oxynitride stoichiometry. (C) 2015 AIP Publishing LLC. C1 [Mirzaei, S.; Kremer, F.; Feng, R.; Ridgway, M. C.] Australian Natl Univ, Dept Elect Mat Engn, Canberra, ACT 0200, Australia. [Sprouster, D. J.] Brookhaven Natl Lab, Nucl Sci & Technol Dept, Upton, NY 11973 USA. [Araujo, L. L.] Univ Fed Rio Grande do Sul, Inst Fis, Lab Implantacao Ion, BR-91501970 Porto Alegre, RS, Brazil. [Glover, C. J.] Australian Synchrotron, Melbourne, Vic, Australia. RP Mirzaei, S (reprint author), Australian Natl Univ, Dept Elect Mat Engn, GPO Box 4, Canberra, ACT 0200, Australia. EM sahar.mirzaei@anu.edu.au RI Sprouster, David/F-2280-2010; Araujo, Leandro/A-3720-2008; OI Sprouster, David/0000-0002-2689-0721; Araujo, Leandro/0000-0002-9413-8777; Kremer, Felipe/0000-0001-6263-7806 FU Australian Research Council; Australian Synchrotron; Australian Microscopy and Microanalysis Research Facility FX We acknowledge access to NCRIS infrastructure at the Australian National University including the Australian National Fabrication Facility and the Heavy Ion Accelerator Capability. We also thank the Australian Research Council and Australian Synchrotron for support. Access to the facilities of the Centre for Advanced Microscopy, with funding through the Australian Microscopy and Microanalysis Research Facility, is gratefully acknowledged. NR 38 TC 1 Z9 1 U1 2 U2 18 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 21 PY 2015 VL 118 IS 15 AR 154309 DI 10.1063/1.4933396 PG 6 WC Physics, Applied SC Physics GA CU4XW UT WOS:000363535800023 ER PT J AU Reese, MO Perkins, CL Burst, JM Farrell, S Barnes, TM Johnston, SW Kuciauskas, D Gessert, TA Metzger, WK AF Reese, M. O. Perkins, C. L. Burst, J. M. Farrell, S. Barnes, T. M. Johnston, S. W. Kuciauskas, D. Gessert, T. A. Metzger, W. K. TI Intrinsic surface passivation of CdTe SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID TIME-RESOLVED PHOTOLUMINESCENCE; MINORITY-CARRIER LIFETIME; II-VI SEMICONDUCTORS; CSSCDTE SOLAR-CELLS; RECOMBINATION VELOCITY; CADMIUM TELLURIDE; SINGLE-CRYSTALS; CONTACTS; PERFORMANCE; SILICON AB Recombination is critically limiting in CdTe devices such as solar cells and detectors, with much of it occurring at or near the surface. In this work, we explore different routes to passivate p-type CdTe surfaces without any intentional extrinsic passivation layers. To provide deeper insight into the passivation routes, we uniquely correlate a set of characterization methods: surface analysis and time-resolved spectroscopy. We study two model systems: nominally undoped single crystals and large-grain polycrystalline films. We examine several strategies to reduce surface recombination velocity. First, we study the effects of removing surface contaminants while maintaining a near-stoichiometric surface. Then we examine stoichiometric thermally reconstructed surfaces. We also investigate the effects of shifting the surface stoichiometry by both "subtractive" (wet chemical etches) and "additive" (ampoule anneals and epitaxial growth) means. We consistently find for a variety of methods that a highly ordered stoichiometric to Cd-rich surface shows a significant reduction in surface recombination, whereas a Te-rich surface has high recombination and propose a mechanism to explain this. While as-received single crystals and as-deposited polycrystalline films have surface recombination velocities in the range of 10(5)-10(6) cm/s, we find that several routes can reduce surface recombination velocities to <2.5 x 10(4) cm/s. (C) 2015 AIP Publishing LLC. C1 [Reese, M. O.; Perkins, C. L.; Burst, J. M.; Farrell, S.; Barnes, T. M.; Johnston, S. W.; Kuciauskas, D.; Gessert, T. A.; Metzger, W. K.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Reese, MO (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. OI Kuciauskas, Darius/0000-0001-8091-5718 FU U.S. Department of Energy [DE-AC36-08-GO28308]; CdTe Solar program of the Solar Energy Technologies Office, Office of Energy Efficiency and Renewable Energy, U.S. Department of Energy FX The National Renewable Energy Lab was supported by the U.S. Department of Energy under Contract No. DE-AC36-08-GO28308. We acknowledge the support of the CdTe Solar program of the Solar Energy Technologies Office, Office of Energy Efficiency and Renewable Energy, U.S. Department of Energy. The U.S. Government retains and the publisher, by accepting the article for publication, acknowledges that the U.S. Government retains a nonexclusive, paid up, irrevocable, worldwide license to publish or reproduce the published form of this work, or allow others to do so, for U.S. Government purposes. NR 61 TC 8 Z9 8 U1 6 U2 33 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 21 PY 2015 VL 118 IS 15 AR 155305 DI 10.1063/1.4933186 PG 12 WC Physics, Applied SC Physics GA CU4XW UT WOS:000363535800041 ER PT J AU Wickramasinghe, LD Zhou, RW Zong, RF Vo, P Gagnon, KJ Thummel, RP AF Wickramasinghe, Lanka D. Zhou, Rongwei Zong, Ruifa Vo, Pascal Gagnon, Kevin J. Thummel, Randolph P. TI Iron Complexes of Square Planar Tetradentate Polypyridyl-Type Ligands as Catalysts for Water Oxidation SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID HYDROGEN EVOLUTION; RU COMPLEXES; INTERMEDIATE; REACTIVITY AB The tetradentate ligand, 2-(pyrid-2'-yl)-8-(1 '',10 ''-phenanthrolin-2 ''-yl)-quinoline (ppq) embodies a quaterpyridine backbone but with the quinoline C8 providing an additional sp(2) center separating the two bipyridine-like subunits. Thus, the four pyridine rings of ppq present a neutral, square planar host that is well suited to first-row transition metals. When reacted with FeCl3, a mu-oxo-bridged dimer is formed having a water bound to an axial metal site. A similar metal-binding environment is presented by a bis-phenanthroline amine (dpa) which forms a 1:1 complex with FeCl3. Both structures are verified by X-ray analysis. While the Fe-III(dpa) complex shows two reversible one-electron oxidation waves, the Fe-III(ppq) complex shows a clear two-electron oxidation associated with the process H2O-(FeFeIII)-Fe-III -> H2O-(FeFeIV)-Fe-IV -> O=(FeFeIII)-Fe-V. Subsequent disproportionation to an Fe=O species is suggested. When the Fe-III(ppq) complex is exposed to a large excess of the sacrificial electron-acceptor ceric ammonium nitrate at pH 1, copious amounts of oxygen are evolved immediately with a turnover frequency (TOF) = 7920 h(-1). Under the same conditions the mononuclear Fe-III(dpa) complex also evolves oxygen with TOF = 842 h(-1). C1 [Wickramasinghe, Lanka D.; Zhou, Rongwei; Zong, Ruifa; Vo, Pascal; Thummel, Randolph P.] Univ Houston, Dept Chem, Houston, TX 77204 USA. [Gagnon, Kevin J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Thummel, RP (reprint author), Univ Houston, Dept Chem, 112 Fleming Bldg, Houston, TX 77204 USA. EM thummel@uh.edu FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-FG02-07ER15888]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Robert A. Welch Foundation [E-621] FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under award no. DE-FG02-07ER15888, the Advanced Light Source supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under contract no. DE-AC02-05CH11231, and the Robert A. Welch Foundation (Grant E-621) for financial support of this work. We also thank Professor Karl Kadish for a helpful discussion, Ms. Maria A. Vorontsova for conducting dynamic light scattering experiments, and assistance from Dr. Andrew Kopecky. NR 30 TC 18 Z9 18 U1 8 U2 60 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD OCT 21 PY 2015 VL 137 IS 41 BP 13260 EP 13263 DI 10.1021/jacs.5b08856 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA CU3PZ UT WOS:000363438600013 PM 26425866 ER PT J AU Xiang, ZH Mercado, R Huck, JM Wang, H Guo, ZH Wang, WC Cao, DP Haranczyk, M Smit, B AF Xiang, Zhonghua Mercado, Rocio Huck, Johanna M. Wang, Hui Guo, Zhanhu Wang, Wenchuan Cao, Dapeng Haranczyk, Maciej Smit, Berend TI Systematic Tuning and Multifunctionalization of Covalent Organic Polymers for Enhanced Carbon Capture SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID HIGH-SURFACE-AREA; DIOXIDE CAPTURE; CO2 CAPTURE; MICROPOROUS POLYMERS; STORAGE MATERIALS; OXYGEN REDUCTION; METHANE STORAGE; FRAMEWORKS; NETWORKS; DESIGN AB Porous covalent polymers are attracting increasing interest in the fields of gas adsorption, gas separation, and catalysis due to their fertile synthetic polymer chemistry, large internal surface areas, and ultrahigh hydrothermal stabilities. While precisely manipulating the porosities of porous organic materials for targeted applications remains challenging, we show how a large degree of diversity can be achieved in covalent organic polymers by incorporating multiple functionalities into a single framework, as is done for crystalline porous materials. Here, we synthesized 17 novel porous covalent organic polymers (COPs) with finely tuned porosities, a wide range of Brunauer Emmett Teller (BET) specific surface areas of 430-3624 m(2) g(-1), and a broad range of pore volumes of 0.24-3.50 cm(3) g(-1), all achieved by tailoring the length and geometry of building blocks. Furthermore, we are the first to successfully incorporate more than three distinct functional groups into one phase for porous organic materials, which has been previously demonstrated in crystalline metal organic frameworks (MOFs). COPs decorated with multiple functional groups in one phase can lead to enhanced properties that are not simply linear combinations of the pure component properties. For instance, in the dibromobenzene-lined frameworks, the bi- and multifunctionalized COPs exhibit selectivities for carbon dioxide over nitrogen twice as large as any of the singly functionalized COPs. These multifunctionalized frameworks also exhibit a lower parasitic energy cost for carbon capture at typical flue gas conditions than any of the singly functionalized frameworks. Despite the significant improvement, these frameworks do not yet outperform the current state-of-art technology for carbon capture. Nonetheless, the tuning strategy presented here opens up avenues for the design of novel catalysts, the synthesis of functional sensors from these materials, and the improvement in the performance of existing covalent organic polymers by multifunctionalization. C1 [Xiang, Zhonghua; Wang, Hui; Wang, Wenchuan; Cao, Dapeng] Beijing Univ Chem Technol, State Key Lab Organ Inorgan Composites, Beijing 100029, Peoples R China. [Mercado, Rocio; Smit, Berend] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Guo, Zhanhu] Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA. [Wang, Wenchuan] Beijing Univ Chem Technol, Int Res Ctr Soft Matter, Beijing 100029, Peoples R China. [Haranczyk, Maciej] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. [Huck, Johanna M.; Smit, Berend] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Smit, Berend] EPFL, Inst Sci & Ingn Chim Valais, CH-1951 Sion, Switzerland. RP Cao, DP (reprint author), Beijing Univ Chem Technol, State Key Lab Organ Inorgan Composites, Beijing 100029, Peoples R China. EM caodp@mail.buct.edu.cn; berend-smit@berkeley.edu RI Smit, Berend/B-7580-2009; Wang, Wenchuan/G-2961-2010; OI Smit, Berend/0000-0003-4653-8562; Guo, Zhanhu/0000-0003-0134-0210 FU National 863 Programs [2013AA031901, 2012AA101809]; NSF of China [91334203, 21274011, 51502012]; Scientific Research Funding [ZZ1304]; Talent Funding from BUCT [buctrc201420]; Outstanding Talent Funding from BUCT [RC1301]; Talent cultivation of OIC [OIC201403003, OIC201503002]; Fundamental Research Funds for the Central Universities [ZY1508]; Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001015]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work is supported by National 863 Programs (2013AA031901, 2012AA101809), NSF of China (91334203, 21274011, 51502012) Scientific Research Funding (ZZ1304), Talent Funding (buctrc201420) from BUCT, Outstanding Talent Funding (RC1301) from BUCT, Talent cultivation of OIC (Nos. OIC201403003; OIC201503002), and the Fundamental Research Funds for the Central Universities (ZY1508). This research was also supported through the Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award DE-SC0001015. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Z.X. is thankful to Prof. J.F. Chen from IOC and Prof. L. M. Dai from Case Western Reserve University for helpful discussions. NR 46 TC 32 Z9 32 U1 46 U2 279 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD OCT 21 PY 2015 VL 137 IS 41 BP 13301 EP 13307 DI 10.1021/jacs.5b06266 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA CU3PZ UT WOS:000363438600019 PM 26412410 ER PT J AU DeVol, RT Sun, CY Marcus, MA Coppersmith, SN Myneni, SCB Gilbert, PUPA AF DeVol, Ross T. Sun, Chang-Yu Marcus, Matthew A. Coppersmith, Susan N. Myneni, Satish C. B. Gilbert, Pupa U. P. A. TI Nanoscale Transforming Mineral Phases in Fresh Nacre SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID AMORPHOUS CALCIUM-CARBONATE; SEA-URCHIN EMBRYOS; ANISOTROPIC LATTICE-DISTORTIONS; PRECURSOR PILP PROCESS; MOLLUSK SHELL NACRE; PINCTADA-MARGARITIFERA; CRYSTAL-GROWTH; ORGANIC MATRIX; BIOMPHALARIA-GLABRATA; PARTICLE ACCRETION AB Nacre, or mother-of-pearl, the iridescent inner layer of many mollusk shells, is a biomineral lamellar composite of aragonite (CaCO3) and organic sheets. Biomineralization frequently occurs via transient amorphous precursor phases, crystallizing into the final stable biomineral. In nacre, despite extensive attempts, amorphous calcium carbonate (ACC) precursors have remained elusive. They were inferred from non-nacre-forming larval shells, or from a residue of amorphous material surrounding mature gastropod nacre tablets, and have only once been observed in bivalve nacre. Here we present the first direct observation of ACC precursors to nacre formation, obtained from the growth front of nacre in gastropod shells from red abalone (Haliotis rufescens), using synchrotron spectromicroscopy. Surprisingly, the abalone nacre data show the same ACC phases that are precursors to calcite (CaCO3) formation in sea urchin spicules, and not proto-aragonite or poorly crystalline aragonite (pAra), as expected for aragonitic nacre. In contrast, we find pAra in coral. C1 [DeVol, Ross T.; Sun, Chang-Yu; Coppersmith, Susan N.; Gilbert, Pupa U. P. A.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Marcus, Matthew A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Myneni, Satish C. B.] Princeton Univ, Dept Geosci, Princeton, NJ 08544 USA. [Gilbert, Pupa U. P. A.] Univ Wisconsin, Dept Chem, Madison, WI 53706 USA. [Gilbert, Pupa U. P. A.] Harvard Univ, Radcliffe Inst Adv Study, Cambridge, MA 02138 USA. RP Gilbert, PUPA (reprint author), Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. EM pupa@physics.wisc.edu RI Gilbert, Pupa/A-6299-2010 OI Gilbert, Pupa/0000-0002-0139-2099 FU National Science Foundation [DMR-1105167]; U.S. Department of Energy (DOE) [DE-FG02-07ER15899]; US-Israel Binational Science Foundation [BSF-2010065]; Radcliffe Institute for Advanced Study at Harvard University; DOE [DE-AC02-05CH11231] FX We thank Andreas Scholl, Anthony Young, and Richard Celestre for technical support. P.G. acknowledges support from the National Science Foundation (DMR-1105167), the U.S. Department of Energy (DOE grant DE-FG02-07ER15899), US-Israel Binational Science Foundation (BSF-2010065), and the Radcliffe Institute for Advanced Study at Harvard University. PEEM experiments were done at the Advanced Light Source, supported by DOE grant DE-AC02-05CH11231. NR 129 TC 14 Z9 14 U1 14 U2 86 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD OCT 21 PY 2015 VL 137 IS 41 BP 13325 EP 13333 DI 10.1021/jacs.5b07931 PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA CU3PZ UT WOS:000363438600022 PM 26403582 ER PT J AU Dorchies, F Recoules, V Bouchet, J Fourment, C Leguay, PM Cho, BI Engelhorn, K Nakatsutsumi, M Ozkan, C Tschentscher, T Harmand, M Toleikis, S Stormer, M Galtier, E Lee, HJ Nagler, B Heimann, PA Gaudin, J AF Dorchies, F. Recoules, V. Bouchet, J. Fourment, C. Leguay, P. M. Cho, B. I. Engelhorn, K. Nakatsutsumi, M. Ozkan, C. Tschentscher, T. Harmand, M. Toleikis, S. Stoermer, M. Galtier, E. Lee, H. J. Nagler, B. Heimann, P. A. Gaudin, J. TI Time evolution of electron structure in femtosecond heated warm dense molybdenum SO PHYSICAL REVIEW B LA English DT Article ID PHOTOELECTRON-SPECTROSCOPY; TRANSITION; STATE; GOLD AB The time evolution of the electron structure is investigated in a molybdenum foil heated up to the warm dense matter regime by a femtosecond laser pulse, through time-resolved x-ray absorption near-edge spectroscopy. Spectra are measured with independent characterizations of temperature and density. They are successfully compared with ab initio quantum molecular dynamic calculations. We demonstrate that the observed white line in the L-3 edge reveals the time evolution of the electron density of state from the solid to the hot (a few eV) and expanding liquid. The data indicate a highly nonequilibrated state, 5 ps after heating. C1 [Dorchies, F.; Fourment, C.; Leguay, P. M.; Gaudin, J.] Univ Bordeaux, CNRS, CELIA Ctr Lasers Intenses & Applicat, CEA,UMR 5107, F-33400 Talence, France. [Recoules, V.; Bouchet, J.] CEA, DAM, DIF, F-91297 Arpajon, France. [Cho, B. I.] GIST, Dept Phys & Photon Sci, Kwangju, South Korea. [Engelhorn, K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Nakatsutsumi, M.; Ozkan, C.; Tschentscher, T.] European XFEL, Hamburg, Germany. [Harmand, M.; Toleikis, S.] DESY, Hamburg, Germany. [Stoermer, M.] Helmholtz Zentrum Geesthacht, D-21502 Geesthacht, Germany. [Galtier, E.; Lee, H. J.; Nagler, B.; Heimann, P. A.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. RP Dorchies, F (reprint author), Univ Bordeaux, CNRS, CELIA Ctr Lasers Intenses & Applicat, CEA,UMR 5107, F-33400 Talence, France. EM dorchies@celia.u-bordeaux1.fr RI Cho, Byoung-ick/A-6294-2011; harmand, marion/Q-1248-2016 OI harmand, marion/0000-0003-0713-5824 FU French Agence Nationale de la Recherche [ANR-09-BLAN-0206-01, ANR-10-IDEX-03-02]; National Research Foundation of Korea [NRF-2013R1A1A1007084, NRF-2015R1A5A1009962]; TBP research project of GIST; DOE Office of Science, Office of Fusion Energy Sciences [SF00515] FX This work was supported by the French Agence Nationale de la Recherche, under Grant OEDYP (ANR-09-BLAN-0206-01) and Programme IdEx Bordeaux - LAPHIA (ANR-10-IDEX-03-02), and by the GENCI program providing computational time under the Programs GEN6046 and GEN6454. The authors gratefully acknowledge Benoit Chimier and Olivier Peyrusse for fruitful discussions respectively concerning hydrodynamic simulations and XANES spectra calculations, Rodrigue Bouillaud and Laurent Merzeau for their technical assistance, and Frederic Burgy and Fanny Froustey for laser operation at CELIA. The authors thanks Marc Torrent for his great help with ABINIT simulations. B.I.C. acknowledges support from the National Research Foundation of Korea (NRF-2013R1A1A1007084, NRF-2015R1A5A1009962) and the TBP research project of GIST. Portions of this research were carried out at the Linac Coherent Light Source (LCLS) at the SLAC National Accelerator Laboratory. LCLS is an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Stanford University. The MEC instrument has additional support from the DOE Office of Science, Office of Fusion Energy Sciences under Contract No. SF00515. NR 42 TC 4 Z9 4 U1 3 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 21 PY 2015 VL 92 IS 14 AR 144201 DI 10.1103/PhysRevB.92.144201 PG 5 WC Physics, Condensed Matter SC Physics GA CU0UG UT WOS:000363233700006 ER PT J AU Leroux, M Errea, I Le Tacon, M Souliou, SM Garbarino, G Cario, L Bosak, A Mauri, F Calandra, M Rodiere, P AF Leroux, Maxime Errea, Ion Le Tacon, Mathieu Souliou, Sofia-Michaela Garbarino, Gaston Cario, Laurent Bosak, Alexey Mauri, Francesco Calandra, Matteo Rodiere, Pierre TI Strong anharmonicity induces quantum melting of charge density wave in 2H-NbSe2 under pressure SO PHYSICAL REVIEW B LA English DT Article ID DEPENDENT SUPERCONDUCTIVITY; TRANSITIONS; SCATTERING; ORDER; FLUCTUATIONS AB The pressure and temperature dependence of the phonon dispersion of 2H-NbSe2 is measured by inelastic x-ray scattering. A strong temperature dependent soft phonon mode, reminiscent of the charge density wave (CDW), is found to persist up to a pressure as high as 16 GPa, far above the critical pressure at which the CDW disappears at 0 K. By using ab initio calculations beyond the harmonic approximation, we obtain an accurate, quantitative description of the (P, T) dependence of the phonon spectrum. Our results show that the rapid destruction of the CDW under pressure is related to the zero mode vibrations-or quantum fluctuations-of the lattice renormalized by the anharmonic part of the lattice potential. The calculations also show that the low-energy longitudinal acoustic mode that drives the CDW transition barely contributes to superconductivity, explaining the insensitivity of the superconducting critical temperature to the CDW transition. C1 [Leroux, Maxime; Rodiere, Pierre] Univ Grenoble Alpes, CNRS, Inst Neel, F-38000 Grenoble, France. [Errea, Ion] DIPC, Donostia San Sebastian 20018, Basque Country, Spain. [Errea, Ion] Basque Fdn Sci, Ikerbasque, Bilbao 48011, Spain. [Errea, Ion; Mauri, Francesco; Calandra, Matteo] Univ Paris 06, Sorbonne Univ, UMR CNRS 7590, IMPMC,MNHN,IRD, F-75005 Paris, France. [Le Tacon, Mathieu; Souliou, Sofia-Michaela] Max Planck Inst Festkorperforsch, D-70569 Stuttgart, Germany. [Garbarino, Gaston; Bosak, Alexey] European Synchrotron Radiat Facil, F-38043 Grenoble, France. [Cario, Laurent] Univ Nantes, CNRS, Inst Mat Jean Rouxel IMN, F-44322 Nantes, France. RP Leroux, M (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM mleroux@anl.gov; matteo.calandra@upmc.fr; pierre.rodiere@neel.cnrs.fr RI Errea, Ion/J-4237-2014; mauri, francesco/K-5726-2012; Calandra, Matteo/B-6161-2014; Le Tacon, Mathieu/D-8023-2011; Garbarino, Gaston/D-1807-2013; DONOSTIA INTERNATIONAL PHYSICS CTR., DIPC/C-3171-2014; Leroux, Maxime/E-8703-2016 OI Errea, Ion/0000-0002-5719-6580; mauri, francesco/0000-0002-6666-4710; Le Tacon, Mathieu/0000-0002-5838-3724; Leroux, Maxime/0000-0001-9778-323X FU French National Research Agency [ANR-12-JS04-0003-01]; Basque Government [BFI-2011-65]; Spanish Ministry of Economy and Competitiveness [FIS2013-48286-C2-2-P]; Graphene Flagship; Prace [2014102310]; ANR [ANR-13-IS10-0003-01] FX Sabrina Salmon-Bourmand is thanked for her help in the synthesis of 2H-NbSe2 single crystals. P.R. and M.L. acknowledge financial support from the French National Research Agency through Grant No. ANR-12-JS04-0003-01 SUBRISSYME. M.C., F.M., and I.E. acknowledge support from the Basque Government (Grant No. BFI-2011-65), Spanish Ministry of Economy and Competitiveness (FIS2013-48286-C2-2-P), Graphene Flagship and ANR (Contract No. ANR-13-IS10-0003-01), and Prace (2014102310). Calculations were performed at IDRIS, CINES, DIPC, and at CEA TGCC. NR 44 TC 7 Z9 7 U1 18 U2 62 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD OCT 21 PY 2015 VL 92 IS 14 AR 140303 DI 10.1103/PhysRevB.92.140303 PG 6 WC Physics, Condensed Matter SC Physics GA CU0UG UT WOS:000363233700001 ER PT J AU Arnold, R Augier, C Baker, JD Barabash, AS Basharina-Freshville, A Blondel, S Blot, S Bongrand, M Brudanin, V Busto, J Caffrey, AJ Calvez, S Cerna, C Cesar, JP Chapon, A Chauveau, E Duchesneau, D Durand, D Egorov, V Eurin, G Evans, JJ Fajt, L Filosofov, D Flack, R Garrido, X Gomez, H Guillon, B Guzowski, P Hodak, R Huber, A Hubert, P Hugon, C Jullian, S Klimenko, A Kochetov, O Konovalov, SI Kovalenko, V Lalanne, D Lang, K Lemiere, Y Le Noblet, T Liptak, Z Loaiza, P Lutter, G Mamedov, F Marquet, C Mauger, F Morgan, B Mott, J Nemchenok, I Nomachi, M Nova, F Nowacki, F Ohsumi, H Pahlka, RB Perrot, F Piquemal, F Povinec, P Pridal, P Ramachers, YA Remoto, A Reyss, JL Richards, B Riddle, CL Rukhadze, E Saakyan, R Sarazin, X Shitov, Y Simard, L Simkovic, F Smetana, A Smolek, K Smolnikov, A Soldner-Rembold, S Soule, B Stekl, I Suhonen, J Sutton, CS Szklarz, G Thomas, J Timkin, V Torre, S Tretyak, VI Tretyak, VI Umatov, VI Vanushin, I Vilela, C Vorobel, V Waters, D Zukauskas, A AF Arnold, R. Augier, C. Baker, J. D. Barabash, A. S. Basharina-Freshville, A. Blondel, S. Blot, S. Bongrand, M. Brudanin, V. Busto, J. Caffrey, A. J. Calvez, S. Cerna, C. Cesar, J. P. Chapon, A. Chauveau, E. Duchesneau, D. Durand, D. Egorov, V. Eurin, G. Evans, J. J. Fajt, L. Filosofov, D. Flack, R. Garrido, X. Gomez, H. Guillon, B. Guzowski, P. Hodak, R. Huber, A. Hubert, P. Hugon, C. Jullian, S. Klimenko, A. Kochetov, O. Konovalov, S. I. Kovalenko, V. Lalanne, D. Lang, K. Lemiere, Y. Le Noblet, T. Liptak, Z. Loaiza, P. Lutter, G. Mamedov, F. Marquet, C. Mauger, F. Morgan, B. Mott, J. Nemchenok, I. Nomachi, M. Nova, F. Nowacki, F. Ohsumi, H. Pahlka, R. B. Perrot, F. Piquemal, F. Povinec, P. Pridal, P. Ramachers, Y. A. Remoto, A. Reyss, J. L. Richards, B. Riddle, C. L. Rukhadze, E. Saakyan, R. Sarazin, X. Shitov, Yu Simard, L. Simkovic, F. Smetana, A. Smolek, K. Smolnikov, A. Soeldner-Rembold, S. Soule, B. Stekl, I. Suhonen, J. Sutton, C. S. Szklarz, G. Thomas, J. Timkin, V. Torre, S. Tretyak, Vl. I. Tretyak, V. I. Umatov, V. I. Vanushin, I. Vilela, C. Vorobel, V. Waters, D. Zukauskas, A. CA NEMO-3 Collaboration TI Results of the search for neutrinoless double-beta decay in Mo-100 with the NEMO-3 experiment SO PHYSICAL REVIEW D LA English DT Article ID MODES; GE-76 AB The NEMO-3 detector, which had been operating in the Modane Underground Laboratory from 2003 to 2010, was designed to search for neutrinoless double-beta (0 nu beta beta) decay. We report the final results of a search for 0 nu beta beta decays with 6.914 kg of Mo-100 using the entire NEMO-3 data set with a detector live time of 4.96 yr, which corresponds to an exposure of 34.3 kg . yr. We perform a detailed study of the expected background in the 0 nu beta beta signal region and find no evidence of 0 nu beta beta decays in the data. The level of observed background in the 0 nu beta beta signal region [2.8-3.2] MeV is 0.44 +/- 0.13 counts/yr/kg, and no events are observed in the interval [3.2-10] MeV. We therefore derive a lower limit on the half-life of 0 nu beta beta decays in Mo-100 of T-1/2(0 nu beta beta) > 1.1 x 10(24) yr at the 90% confidence level, under the hypothesis of decay kinematics similar to that for light Majorana neutrino exchange. Depending on the model used for calculating nuclear matrix elements, the limit for the effective Majorana neutrino mass lies in the range < m(nu)> < 0.33-0.62 eV. We also report constraints on other lepton-number violating mechanisms for 0 nu beta beta decays. C1 [Arnold, R.; Nowacki, F.] ULP, CNRS, IN2P3, IPHC, F-67037 Strasbourg, France. [Augier, C.; Blondel, S.; Bongrand, M.; Calvez, S.; Eurin, G.; Garrido, X.; Gomez, H.; Jullian, S.; Lalanne, D.; Loaiza, P.; Sarazin, X.; Simard, L.; Szklarz, G.] Univ Paris 11, CNRS, IN2P3, LAL, F-91405 Orsay, France. [Baker, J. D.; Caffrey, A. J.; Riddle, C. L.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Barabash, A. S.; Konovalov, S. I.; Umatov, V. I.; Vanushin, I.] ITEP, Moscow 117218, Russia. [Basharina-Freshville, A.; Eurin, G.; Flack, R.; Mott, J.; Richards, B.; Saakyan, R.; Thomas, J.; Torre, S.; Vilela, C.; Waters, D.] UCL, London WC1E 6BT, England. [Blot, S.; Chauveau, E.; Evans, J. J.; Guzowski, P.; Soeldner-Rembold, S.] Univ Manchester, Manchester M13 9PL, Lancs, England. [Brudanin, V.; Egorov, V.; Filosofov, D.; Klimenko, A.; Kochetov, O.; Kovalenko, V.; Nemchenok, I.; Shitov, Yu; Smolnikov, A.; Timkin, V.; Tretyak, V. I.] Joint Inst Nucl Res, Dubna 141980, Russia. [Busto, J.] Univ Marseille, CNRS, IN2P3, CPPM, F-13288 Marseille, France. [Cerna, C.; Huber, A.; Hubert, P.; Hugon, C.; Lutter, G.; Marquet, C.; Perrot, F.; Piquemal, F.; Soule, B.] Univ Bordeaux, CNRS, IN2P3, CENBG, F-33175 Gradignan, France. [Chapon, A.; Durand, D.; Guillon, B.; Lemiere, Y.; Mauger, F.] Univ Caen, CNRS, IN2P3, LPC Caen,ENSICAEN, F-14050 Caen, France. [Duchesneau, D.; Le Noblet, T.; Remoto, A.] Univ Savoie, CNRS, IN2P3, LAPP, F-74941 Annecy Le Vieux, France. [Fajt, L.; Hodak, R.; Mamedov, F.; Pridal, P.; Rukhadze, E.; Smetana, A.; Smolek, K.; Stekl, I.] Czech Tech Univ, Inst Expt & Appl Phys, CZ-12800 Prague, Czech Republic. [Cesar, J. P.; Lang, K.; Liptak, Z.; Nova, F.; Pahlka, R. B.] Univ Texas Austin, Austin, TX 78712 USA. [Piquemal, F.] Lab Souterrain Modane, F-73500 Modane, France. [Morgan, B.; Ramachers, Y. A.] Univ Warwick, Coventry CV4 7AL, W Midlands, England. [Nomachi, M.] Osaka Univ, Osaka 5600043, Japan. [Ohsumi, H.] Saga Univ, Saga 8408502, Japan. [Povinec, P.; Simkovic, F.] Comenius Univ, FMFI, SK-84248 Bratislava, Slovakia. [Reyss, J. L.] CNRS, LSCE, F-91190 Gif Sur Yvette, France. [Shitov, Yu] Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England. [Simard, L.] Inst Univ France, F-75005 Paris, France. [Suhonen, J.] Univ Jyvaskyla, FIN-40351 Jyvaskyla, Finland. [Sutton, C. S.] Mt Holyoke Coll, S Hadley, MA 01075 USA. [Tretyak, Vl. I.] Inst Nucl Res, UA-03680 Kiev, Ukraine. [Vorobel, V.; Zukauskas, A.] Charles Univ Prague, Fac Math & Phys, CZ-12116 Prague, Czech Republic. [Brudanin, V.] Natl Res Nucl Univ MEPhI, Moscow 115409, Russia. RP Arnold, R (reprint author), ULP, CNRS, IN2P3, IPHC, F-67037 Strasbourg, France. RI Evans, Justin/P-4981-2014; Hodak, Rastislav/O-4243-2016; Barabash, Alexander/S-8851-2016 OI Evans, Justin/0000-0003-4697-3337; Hodak, Rastislav/0000-0001-7640-5643; FU Czech Republic; CNRS/IN2P3 in France; RFBR in Russia; STFC in the U.K; NSF in the U.S FX The authors would like to thank the Modane Underground Laboratory staff for their technical assistance in running the experiment. We acknowledge support by the grants agencies of the Czech Republic, CNRS/IN2P3 in France, RFBR in Russia, STFC in the U.K. and NSF in the U.S. NR 43 TC 10 Z9 10 U1 3 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 21 PY 2015 VL 92 IS 7 AR 072011 DI 10.1103/PhysRevD.92.072011 PG 23 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CU0VQ UT WOS:000363237400002 ER PT J AU Cahill-Rowley, M Hewett, JL Ismail, A Rizzo, TG AF Cahill-Rowley, M. Hewett, J. L. Ismail, A. Rizzo, T. G. TI ATLAS Z plus missing transverse energy excess in the MSSM SO PHYSICAL REVIEW D LA English DT Article ID HADRON COLLIDERS; PP COLLISIONS; SUPERSYMMETRY; PROGRAM; DECAYS; SQUARK; PAIR; LHC; NLO AB We demonstrate that the 3 sigma excess observed by ATLAS in the Z + MET channel can be explained within the context of the MSSM. Using the freedom inherent in the pMSSM, we perform a detailed analysis of the parameter space and find a scenario that describes the excess while simultaneously complying with all other search constraints from the Run I data at 7 and 8 TeV, including the Z + MET analysis by CMS. We generate a small sample of simplified models, using promising models from our existing pMSSM sample as seeds, and study their properties. The successful region is described by the production of 1st/2nd generation squark pairs, followed by their decay into a bino-like neutralino which in turn decays into a Higgsino-like LSP triplet by emitting a Z boson, i.e., (q) over tilde -> (B) over tilde -> (h) over tilde with (q) over tilde = (Q) over tilde (L), (u) over tilde (R), or (d) over tilde (R). The sweet spot for the sparticle spectrum is found to have squark masses in the 500-750 GeV range, with bino masses near 350 GeV with a mass splitting of 150-200 GeV with the Higgsino LSP. If this excess holds, then this scenario predicts that a signal will be observed in the 0l + jets and/or 1l + jets searches in the early operations of Run II. C1 [Cahill-Rowley, M.; Hewett, J. L.; Rizzo, T. G.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Ismail, A.] Argonne Natl Lab, Argonne, IL 60439 USA. [Ismail, A.] Univ Illinois, Chicago, IL 60607 USA. RP Cahill-Rowley, M (reprint author), SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. EM mrowley@slac.stanford.edu; hewett@slac.stanford.edu; aismail@anl.gov; rizzo@slac.stanford.edu FU Department of Energy [DE-AC02-06CH11357, DE-AC02-76SF00515, DE-FG02-12ER41811] FX The authors would like to thank Brian Petersen for communications. This work was supported by the Department of Energy, Contracts No. DE-AC02-06CH11357, No. DE-AC02-76SF00515 and No. DE-FG02-12ER41811. NR 38 TC 7 Z9 7 U1 0 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD OCT 21 PY 2015 VL 92 IS 7 AR 075029 DI 10.1103/PhysRevD.92.075029 PG 12 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CU0VQ UT WOS:000363237400014 ER PT J AU Segovia, J El-Bennich, B Rojas, E Cloet, IC Roberts, CD Xu, SS Zong, HS AF Segovia, Jorge El-Bennich, Bruno Rojas, Eduardo Cloet, Ian C. Roberts, Craig D. Xu, Shu-Sheng Zong, Hong-Shi TI Completing the Picture of the Roper Resonance SO PHYSICAL REVIEW LETTERS LA English DT Article ID DYSON-SCHWINGER EQUATIONS; QUARK-DIQUARK MODEL; NUCLEON RESONANCE; CONTINUUM-QCD; FORM-FACTORS; BARYONS; ELECTROPRODUCTION; COMPONENTS; COVARIANT; LATTICE AB We employ a continuum approach to the three valence-quark bound-state problem in relativistic quantum field theory to predict a range of properties of the proton's radial excitation and thereby unify them with those of numerous other hadrons. Our analysis indicates that the nucleon's first radial excitation is the Roper resonance. It consists of a core of three dressed quarks, which expresses its valence-quark content and whose charge radius is 80% larger than the proton analogue. That core is complemented by a meson cloud, which reduces the observed Roper mass by roughly 20%. The meson cloud materially affects long-wavelength characteristics of the Roper electroproduction amplitudes but the quark core is revealed to probes with Q(2) greater than or similar to 3m(N)(2). C1 [Segovia, Jorge] Univ Salamanca, Grp Fis Nucl, E-37008 Salamanca, Spain. [Segovia, Jorge] Univ Salamanca, IUFFyM, E-37008 Salamanca, Spain. [El-Bennich, Bruno; Rojas, Eduardo] Univ Cruzeiro Sul, Lab Fis Teor & Computac, BR-01506000 Sao Paulo, SP, Brazil. [El-Bennich, Bruno] Univ Estadual Paulista, Inst Fis Teor, BR-01140070 Sao Paulo, SP, Brazil. [Rojas, Eduardo] Univ Antioquia, Inst Fis, Medellin, Colombia. [Cloet, Ian C.; Roberts, Craig D.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Xu, Shu-Sheng; Zong, Hong-Shi] Nanjing Univ, Dept Phys, Nanjing 210093, Jiangsu, Peoples R China. RP Segovia, J (reprint author), Univ Salamanca, Grp Fis Nucl, E-37008 Salamanca, Spain. RI Segovia, Jorge/C-7202-2015 OI Segovia, Jorge/0000-0001-5838-7103 FU Sao Paulo Research Foundation (FAPESP) [2012/03275-8, 2013/16088-4]; CNPq [301190/2014-3, 458371/2014-9]; Patrimonio Autonomo Fondo Nacional de Financiamiento para la Ciencia, la Tecnologia y la Innovacion, Francisco Jose de Caldas and Sostenibilidad-UDEA; U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357]; National Natural Science Foundation of China [11275097, 11475085]; National Basic Research Programme of China [2012CB921504]; Fundamental Research Funds for the Central Universities Programme of China [WK2030040050]; postdoctoral IUFFyM contract at the Universidad de Salamanca FX We are grateful for insightful comments and suggestions from R. Gothe, T.-S. H. Lee, V. Mokeev, and T. Sato. J. S. acknowledges financial support from a postdoctoral IUFFyM contract at the Universidad de Salamanca. This work is also supported by the Sao Paulo Research Foundation (FAPESP) under Grants No. 2012/03275-8 and No. 2013/16088-4; CNPq fellowships (No. 301190/2014-3 and No. 458371/2014-9); Patrimonio Autonomo Fondo Nacional de Financiamiento para la Ciencia, la Tecnologia y la Innovacion, Francisco Jose de Caldas and Sostenibilidad-UDEA 2014-2015; U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357; the National Natural Science Foundation of China (Grants No. 11275097 and No. 11475085); the National Basic Research Programme of China (Grant No. 2012CB921504); and the Fundamental Research Funds for the Central Universities Programme of China (Grant No. WK2030040050). NR 80 TC 18 Z9 18 U1 1 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 21 PY 2015 VL 115 IS 17 AR 171801 DI 10.1103/PhysRevLett.115.171801 PG 6 WC Physics, Multidisciplinary SC Physics GA CU0XY UT WOS:000363243700003 PM 26551101 ER PT J AU Stanier, A Daughton, W Chacon, L Karimabadi, H Ng, J Huang, YM Hakim, A Bhattacharjee, A AF Stanier, A. Daughton, W. Chacon, L. Karimabadi, H. Ng, J. Huang, Y. -M. Hakim, A. Bhattacharjee, A. TI Role of Ion Kinetic Physics in the Interaction of Magnetic Flux Ropes SO PHYSICAL REVIEW LETTERS LA English DT Article ID CURRENT SHEETS; LARGE SYSTEMS; RECONNECTION; COLLISIONLESS; SIMULATIONS; PLASMA; COALESCENCE; DISSIPATION; ISLANDS; HYBRID AB To explain many natural magnetized plasma phenomena, it is crucial to understand how rates of collisionless magnetic reconnection scale in large magnetohydrodynamic (MHD) scale systems. Simulations of isolated current sheets conclude such rates are independent of system size and can be reproduced by the Hall-MHD model, but neglect sheet formation and coupling to MHD scales. Here, it is shown for the problem of flux-rope merging, which includes this formation and coupling, that the Hall-MHD model fails to reproduce the kinetic results. The minimum sufficient model must retain ion kinetic effects, which set the ion diffusion region geometry and give time-averaged rates that reduce significantly with system size, leading to different global evolution in large systems. C1 [Stanier, A.; Daughton, W.; Chacon, L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Karimabadi, H.] SciberQuest Inc, Del Mar, CA 92014 USA. [Ng, J.; Huang, Y. -M.; Hakim, A.; Bhattacharjee, A.] Princeton Plasma Phys Lab, Ctr Heliophys, Princeton, NJ 08543 USA. RP Stanier, A (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM stanier@lanl.gov RI Huang, Yi-Min/G-6926-2011; Daughton, William/L-9661-2013; OI Huang, Yi-Min/0000-0002-4237-2211; Chacon, Luis/0000-0002-4566-8763 FU NSF [AGS-1338944]; U.S. Department of Energy National Nuclear Security Administration [DE-AC52-06NA25396] FX This work is supported by NSF Grant No. AGS-1338944, and used resources provided by the Los Alamos National Laboratory Institutional Computing Program, which is supported by the U.S. Department of Energy National Nuclear Security Administration under Contract No. DE-AC52-06NA25396. NR 39 TC 4 Z9 4 U1 1 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 21 PY 2015 VL 115 IS 17 AR 175004 DI 10.1103/PhysRevLett.115.175004 PG 5 WC Physics, Multidisciplinary SC Physics GA CU0XY UT WOS:000363243700005 PM 26551121 ER PT J AU Qi, B Lougovski, P Pooser, R Grice, W Bobrek, M AF Qi, Bing Lougovski, Pavel Pooser, Raphael Grice, Warren Bobrek, Miljko TI Generating the Local Oscillator "Locally" in Continuous-Variable Quantum Key Distribution Based on Coherent Detection SO PHYSICAL REVIEW X LA English DT Article ID FEEDFORWARD CARRIER RECOVERY; UNCONDITIONAL SECURITY; CRYPTOGRAPHY AB Continuous-variable quantum key distribution (CV-QKD) protocols based on coherent detection have been studied extensively in both theory and experiment. In all the existing implementations of CV-QKD, both the quantum signal and the local oscillator (LO) are generated from the same laser and propagate through the insecure quantum channel. This arrangement may open security loopholes and limit the potential applications of CV-QKD. In this paper, we propose and demonstrate a pilot-aided feedforward data recovery scheme that enables reliable coherent detection using a "locally" generated LO. Using two independent commercial laser sources and a spool of 25-km optical fiber, we construct a coherent communication system. The variance of the phase noise introduced by the proposed scheme is measured to be 0.04 (rad(2)), which is small enough to enable secure key distribution. This technology also opens the door for other quantum communication protocols, such as the recently proposed measurement-device-independent CV-QKD, where independent light sources are employed by different users. C1 [Qi, Bing; Lougovski, Pavel; Pooser, Raphael; Grice, Warren] Oak Ridge Natl Lab, Computat Sci & Engn Div, Quantum Informat Sci Grp, Oak Ridge, TN 37831 USA. [Qi, Bing; Pooser, Raphael] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Bobrek, Miljko] Oak Ridge Natl Lab, Elect & Elect Syst Res Div, RF Commun & Intelligent Syst Grp, Oak Ridge, TN 37831 USA. RP Qi, B (reprint author), Oak Ridge Natl Lab, Computat Sci & Engn Div, Quantum Informat Sci Grp, Oak Ridge, TN 37831 USA. EM qib1@ornl.gov RI Qi, Bing/J-5028-2014; OI Qi, Bing/0000-0001-7723-8998; Grice, Warren/0000-0003-4266-4692; Pooser, Raphael/0000-0002-2922-453X FU U.S. Department of Energy [DE-AC05-00OR22725]; Laboratory Directed Research and Development Program FX We would like to thank Hoi-Kwong Lo and Paul Jouguet for very helpful discussions. This work was performed at Oak Ridge National Laboratory, operated by UT-Battelle for the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. The authors acknowledge support from the Laboratory Directed Research and Development Program. NR 42 TC 10 Z9 10 U1 2 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2160-3308 J9 PHYS REV X JI Phys. Rev. X PD OCT 21 PY 2015 VL 5 IS 4 AR 041009 DI 10.1103/PhysRevX.5.041009 PG 12 WC Physics, Multidisciplinary SC Physics GA CU0XS UT WOS:000363243000001 ER PT J AU Soh, DBS Brif, C Coles, PJ Lutkenhaus, N Camacho, RM Urayama, J Sarovar, M AF Soh, Daniel B. S. Brif, Constantin Coles, Patrick J. Luetkenhaus, Norbert Camacho, Ryan M. Urayama, Junji Sarovar, Mohan TI Self-Referenced Continuous-Variable Quantum Key Distribution Protocol SO PHYSICAL REVIEW X LA English DT Article ID PILOT-CARRIER; STATES AB We introduce a new continuous-variable quantum key distribution (CV-QKD) protocol, self-referenced CV-QKD, that eliminates the need for transmission of a high-power local oscillator between the communicating parties. In this protocol, each signal pulse is accompanied by a reference pulse (or a pair of twin reference pulses), used to align Alice's and Bob's measurement bases. The method of phase estimation and compensation based on the reference pulse measurement can be viewed as a quantum analog of intradyne detection used in classical coherent communication, which extracts the phase information from the modulated signal. We present a proof-of-principle, fiber-based experimental demonstration of the protocol and quantify the expected secret key rates by expressing them in terms of experimental parameters. Our analysis of the secret key rate fully takes into account the inherent uncertainty associated with the quantum nature of the reference pulse(s) and quantifies the limit at which the theoretical key rate approaches that of the respective conventional protocol that requires local oscillator transmission. The self-referenced protocol greatly simplifies the hardware required for CV-QKD, especially for potential integrated photonics implementations of transmitters and receivers, with minimum sacrifice of performance. As such, it provides a pathway towards scalable integrated CV-QKD transceivers, a vital step towards large-scale QKD networks. C1 [Soh, Daniel B. S.; Brif, Constantin; Sarovar, Mohan] Sandia Natl Labs, Livermore, CA 94550 USA. [Soh, Daniel B. S.] Stanford Univ, Edward L Ginzton Lab, Stanford, CA 94305 USA. [Coles, Patrick J.; Luetkenhaus, Norbert] Univ Waterloo, Inst Quantum Comp, Waterloo, ON N2L 3G1, Canada. [Camacho, Ryan M.; Urayama, Junji] Sandia Natl Labs, Albuquerque, NM 87123 USA. RP Soh, DBS (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA. EM dbsoh@sandia.gov; mnsarov@sandia.gov RI Lutkenhaus, Norbert/B-3918-2009 OI Lutkenhaus, Norbert/0000-0002-4897-3376 FU Laboratory Directed Research and Development program at Sandia National Laboratories; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX We are grateful to Chris DeRose (Sandia National Laboratories, SNL), Paul Davids (SNL), Tony Lentine (SNL), and Christian Weedbrook for informative discussions about integrated photonics and CV-QKD. This work was supported by the Laboratory Directed Research and Development program at Sandia National Laboratories. Sandia is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the United States Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 42 TC 11 Z9 11 U1 5 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2160-3308 J9 PHYS REV X JI Phys. Rev. X PD OCT 21 PY 2015 VL 5 IS 4 AR 041010 DI 10.1103/PhysRevX.5.041010 PG 15 WC Physics, Multidisciplinary SC Physics GA CU0XS UT WOS:000363243000002 ER PT J AU Dar, RD Razooky, BS Weinberger, LS Cox, CD Simpson, ML AF Dar, Roy D. Razooky, Brandon S. Weinberger, Leor S. Cox, Chris D. Simpson, Michael L. TI The Low Noise Limit in Gene Expression SO PLOS ONE LA English DT Article ID MESSENGER-RNA DECAY; ESCHERICHIA-COLI; SACCHAROMYCES-CEREVISIAE; TRANSLATION INITIATION; PROTEIN EXPRESSION; SINGLE-CELL; GLOBAL ANALYSIS; YEAST; TRANSCRIPTION; FLUCTUATIONS AB Protein noise measurements are increasingly used to elucidate biophysical parameters. Unfortunately noise analyses are often at odds with directly measured parameters. Here we show that these inconsistencies arise from two problematic analytical choices: (i) the assumption that protein translation rate is invariant for different proteins of different abundances, which has inadvertently led to (ii) the assumption that a large constitutive extrinsic noise sets the low noise limit in gene expression. While growing evidence suggests that transcriptional bursting may set the low noise limit, variability in translational bursting has been largely ignored. We show that genome-wide systematic variation in translational efficiency can-and in the case of E. coli does-control the low noise limit in gene expression. Therefore constitutive extrinsic noise is small and only plays a role in the absence of a systematic variation in translational efficiency. These results show the existence of two distinct expression noise patterns: (1) a global noise floor uniformly imposed on all genes by expression bursting; and (2) high noise distributed to only a select group of genes. C1 [Dar, Roy D.; Weinberger, Leor S.] Gladstone Inst Virol & Immunol, San Francisco, CA USA. [Dar, Roy D.] Univ Illinois, Dept Bioengn, Urbana, IL 61801 USA. [Dar, Roy D.] Univ Illinois, Inst Genom Biol, Urbana, IL 61801 USA. [Razooky, Brandon S.; Simpson, Michael L.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Razooky, Brandon S.; Simpson, Michael L.] Univ Tennessee, Bredesen Ctr Interdisciplinary Res & Grad Educ, Knoxville, TN USA. [Razooky, Brandon S.] Rockefeller Univ, Lab Immune Cell Epigenet & Signaling, New York, NY 10021 USA. [Weinberger, Leor S.] Univ Calif San Francisco, Calif Inst Quantitat Biosci QB3, San Francisco, CA 94143 USA. [Weinberger, Leor S.] Univ Calif San Francisco, Dept Biochem & Biophys, San Francisco, CA 94143 USA. [Cox, Chris D.] Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN USA. [Simpson, Michael L.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Simpson, ML (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM simpsonML1@ornl.gov RI Simpson, Michael/A-8410-2011 OI Simpson, Michael/0000-0002-3933-3457 FU NIH NRSA fellowship [AI104380]; K22 [AI120746]; Collective Phenomena in Nanophases Research Theme at the Center for Nanophase Materials Sciences - Office of Basic Energy Sciences, U.S. Department of Energy; Merck Postdoctoral Fellowship at The Rockefeller University; Pew Scholars Program in the Biomedical Sciences; W.M. Keck Foundation Research Excellence Award; Alfred P. Sloan Research Fellowship; NIH Director's New Innovator Award Program [OD006677] FX RDD was supported by an NIH NRSA fellowship (AI104380) and K22 (AI120746). BSR and MLS were supported by the Collective Phenomena in Nanophases Research Theme at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Office of Basic Energy Sciences, U.S. Department of Energy. BSR was supported in part by funds from a Merck Postdoctoral Fellowship at The Rockefeller University. LSW acknowledges support from the Pew Scholars Program in the Biomedical Sciences, the W.M. Keck Foundation Research Excellence Award, the Alfred P. Sloan Research Fellowship, and the NIH Director's New Innovator Award Program (OD006677). NR 67 TC 1 Z9 1 U1 2 U2 12 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD OCT 21 PY 2015 VL 10 IS 10 AR e0140969 DI 10.1371/journal.pone.0140969 PG 21 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CU0ZM UT WOS:000363248400087 PM 26488303 ER PT J AU Zheng, S Shao, S Zhang, J Wang, YQ Demkowicz, MJ Beyerlein, IJ Mara, NA AF Zheng, Shijian Shao, Shuai Zhang, Jian Wang, Yongqiang Demkowicz, Michael J. Beyerlein, Irene J. Mara, Nathan A. TI Adhesion of voids to bimetal interfaces with non-uniform energies SO SCIENTIFIC REPORTS LA English DT Article ID AUSTENITIC STAINLESS-STEEL; NANOLAYERED COMPOSITES; DEFORMATION MECHANISMS; GRAIN-BOUNDARIES; RADIATION-DAMAGE; BULK; NUCLEATION; BEHAVIOR; ALLOYS AB Interface engineering has become an important strategy for designing radiation-resistant materials. Critical to its success is fundamental understanding of the interactions between interfaces and radiation-induced defects, such as voids. Using transmission electron microscopy, here we report an interesting phenomenon in their interaction, wherein voids adhere to only one side of the bimetal interfaces rather than overlapping them. We show that this asymmetrical void-interface interaction is a consequence of differing surface energies of the two metals and non-uniformity in their interface formation energy. Specifically, voids grow within the phase of lower surface energy and wet only the high-interface energy regions. Furthermore, because this outcome cannot be accounted for by wetting of interfaces with uniform internal energy, our report provides experimental evidence that bimetal interfaces contain non-uniform internal energy distributions. This work also indicates that to design irradiation-resistant materials, we can avoid void-interface overlap via tuning the configurations of interfaces. C1 [Zheng, Shijian; Shao, Shuai; Zhang, Jian; Wang, Yongqiang; Beyerlein, Irene J.; Mara, Nathan A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Zheng, Shijian] Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Beijing 100864, Peoples R China. [Zhang, Jian] Xiamen Univ, Sch Energy Res, Xiamen 361005, Peoples R China. [Demkowicz, Michael J.] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. RP Zheng, S (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM sjzheng@imr.ac.cn FU Center for Materials at Irradiation and Mechanical Extremes, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [2008LANL1026]; "Hundred Talents Project" of Chinese Academy of Sciences; National Natural Science Foundation of China [51401208]; Shenyang National Laboratory for Materials Science [2015RP18] FX This work is supported by the Center for Materials at Irradiation and Mechanical Extremes, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number 2008LANL1026. This work was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy, Office of Science. S. Z. gratefully acknowledges support for this research by "Hundred Talents Project" of Chinese Academy of Sciences, National Natural Science Foundation of China (grant number 51401208), and Shenyang National Laboratory for Materials Science (grant number 2015RP18). NR 40 TC 2 Z9 2 U1 3 U2 27 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 21 PY 2015 VL 5 AR 15428 DI 10.1038/srep15428 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CT9AK UT WOS:000363107800001 PM 26486278 ER PT J AU Wang, ZH Hoffbauer, MA Morris, CL Callahan, NB Adamek, ER Bacon, JD Blatnik, M Brandt, AE Broussard, LJ Clayton, SM Cude-Woods, C Currie, S Dees, EB Ding, X Gao, J Gray, FE Hickerson, KP Holley, AT Ito, TM Liu, CY Makela, M Ramsey, JC Pattie, RW Salvat, DJ Saunders, A Schmidt, DW Schulze, RK Seestrom, SJ Sharapov, EI Sprow, A Tang, Z Wei, W Wexler, J Womack, TL Young, AR Zeck, BA AF Wang, Zhehui Hoffbauer, M. A. Morris, C. L. Callahan, N. B. Adamek, E. R. Bacon, J. D. Blatnik, M. Brandt, A. E. Broussard, L. J. Clayton, S. M. Cude-Woods, C. Currie, S. Dees, E. B. Ding, X. Gao, J. Gray, F. E. Hickerson, K. P. Holley, A. T. Ito, T. M. Liu, C. -Y. Makela, M. Ramsey, J. C. Pattie, R. W., Jr. Salvat, D. J. Saunders, A. Schmidt, D. W. Schulze, R. K. Seestrom, S. J. Sharapov, E. I. Sprow, A. Tang, Z. Wei, W. Wexler, J. Womack, T. L. Young, A. R. Zeck, B. A. TI A multilayer surface detector for ultracold neutrons SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Ultracold neutrons; Multilayer surface detector; B-10 nanometer thin film; Neutron detection efficiency; Low background ID OPTICAL-PROPERTIES; CHAMBER C1 [Wang, Zhehui; Hoffbauer, M. A.; Morris, C. L.; Bacon, J. D.; Broussard, L. J.; Clayton, S. M.; Currie, S.; Gao, J.; Ito, T. M.; Makela, M.; Ramsey, J. C.; Pattie, R. W., Jr.; Salvat, D. J.; Saunders, A.; Schmidt, D. W.; Schulze, R. K.; Seestrom, S. J.; Tang, Z.; Wei, W.; Womack, T. L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Callahan, N. B.; Adamek, E. R.; Liu, C. -Y.; Salvat, D. J.] Indiana Univ, Bloomington, IN 47405 USA. [Blatnik, M.] Cleveland State Univ, Cleveland, OH 44115 USA. [Brandt, A. E.; Cude-Woods, C.; Dees, E. B.; Wexler, J.; Young, A. R.; Zeck, B. A.] N Carolina State Univ, Raleigh, NC 27695 USA. [Ding, X.] Virginia Polytech Inst & State Univ, Blacksburg, VA 24061 USA. [Gray, F. E.] Regis Univ, Denver, CO 80221 USA. [Hickerson, K. P.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [Holley, A. T.] Tennessee Technol Univ, Cookeville, TN 38505 USA. [Sharapov, E. I.] Joint Inst Nucl Res, Dubna 141980, Russia. [Sprow, A.] Univ Kentucky, Lexington, KY 40506 USA. RP Wang, ZH (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM zwang@lanl.gov OI Broussard, Leah/0000-0001-9182-2808; Gray, Frederick/0000-0003-4073-8336; Makela, Mark/0000-0003-0592-3683; Currie, Scott/0000-0002-6164-7321; Morris, Christopher/0000-0003-2141-0255; Ito, Takeyasu/0000-0003-3494-6796; Schulze, Roland/0000-0002-6601-817X FU Los Alamos National Laboratory FX This work was funded by the LORD program of Los Alamos National Laboratory. NR 21 TC 4 Z9 4 U1 2 U2 17 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD OCT 21 PY 2015 VL 798 BP 30 EP 35 DI 10.1016/j.nima.2015.07.010 PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CQ9KO UT WOS:000360933600004 ER PT J AU Gu, X Altinbas, Z Costanzo, M Fischer, W Gassner, DM Hock, J Luo, Y Miller, T Tan, Y Thieberger, P Montag, C Pikin, AI AF Gu, X. Altinbas, Z. Costanzo, M. Fischer, W. Gassner, D. M. Hock, J. Luo, Y. Miller, T. Tan, Y. Thieberger, P. Montag, C. Pikin, A. I. TI Transverse profile of the electron beam for the RHIC electron lenses SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Low energy electron beam; Transverse beam profile; Space charge; Electron lenses; Gaussian beans ID SPACE-CHARGE AB The transverse profile of the electron beam plays a very important role in assuring the success of the electron lens beam-beam compensation, as well as its application in space charge compensation. To compensate for the beam-beam effect in the Relativistic Heavy Ion Collider (RHIC) at Brookhaven National Laboratory, we recently installed and commissioned two electron lenses. In this paper, we describe, via theory and simulations using the code Parmela, the evolution of the density of the electron beam with space charge within an electron lens from the gun to the main solenoid. Our theoretical analysis shows that the change in the beam transverse density is dominated by the effects of the space charge induced longitudinal velocity reduction, not by those of transverse Coulomb collisions. We detail the transverse profile of RHIC electron lens beam, measured via the YAG screen and pinhole detector, and also describe its profile that we assessed from the signal of the electron-backscatter detector (eBSD) via scanning the electron beam with respect to the RHIC beam. We verified, in simulations and experiments, that the distribution of the transverse electron beam is Gaussian throughout its propagation in the RELIC electron lens. (C) 2015 Elsevier B.V. All rights reserved. C1 [Gu, X.; Altinbas, Z.; Costanzo, M.; Fischer, W.; Gassner, D. M.; Hock, J.; Luo, Y.; Miller, T.; Tan, Y.; Thieberger, P.; Montag, C.; Pikin, A. I.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Gu, X (reprint author), Brookhaven Natl Lab, 911 B, Upton, NY 11973 USA. EM xgu@bnl.gov FU Brookhaven Science Associates, LLC [DE-AC02-98CH10886]; U.S. Department of Energy FX The work is supported by Brookhaven Science Associates, LLC under Contract no. DE-AC02-98CH10886 with the U.S. Department of Energy. NR 36 TC 1 Z9 1 U1 1 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD OCT 21 PY 2015 VL 798 BP 36 EP 43 DI 10.1016/j.nima.2015.07.001 PG 8 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CQ9KO UT WOS:000360933600005 ER PT J AU Zholents, A AF Zholents, A. TI A new possibility for production of sub-picosecond x-ray pulses using a time dependent radio frequency orbit deflection SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE X-ray; Synchrotron light source; Short pulse; Deflecting cavity ID FREE-ELECTRON LASER; EXTREME-ULTRAVIOLET; GENERATION; OPERATION AB It is shown that two radio frequency deflecting cavities with slightly different frequencies can be used to produce time-dependent orbit deflection to a few special electron bunches circulating in a synchrotron without affecting the majority of the electron bunches. These special bunches produce an x-ray pulse in which transverse position or angle, or both, are correlated with time. The x-ray pulse is then shortened, either with an asymmetrically cut crystal that acts as a pulse compressor, or with an angular aperture such as a narrow slit positioned downstream. The implementation of this technique creates a highly flexible environment for synchrotrons in which users of most beamlines will be able to easily select between the x-rays originated by the standard electron bunches and the short x-ray pulses originated by the special electron bunches carrying a time-dependent transverse correlation. (C) 2015 Elsevier B.V. All rights reserved. C1 Argonne Natl Lab, Argonne, IL 60439 USA. RP Zholents, A (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. FU Office of Science of the U.S. Department of Energy [DE-AC02-06CH11357] FX Stimulating discussions with T. Berenc, M. Borland, P. Kuske and V. Sajaey are gratefully acknowledged. M. Borland and V. Sajaey also helped in using elegant. This work was supported by the Office of Science of the U.S. Department of Energy under Contract no. DE-AC02-06CH11357. NR 25 TC 3 Z9 3 U1 0 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD OCT 21 PY 2015 VL 798 BP 111 EP 116 DI 10.1016/j.nima.2015.07.016 PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CQ9KO UT WOS:000360933600015 ER PT J AU Aab, A Abreu, P Aglietta, M Ahn, EJ Al Samarai, I Albert, JN Albuquerque, IFM Allekotte, I Allen, J Allison, P Almela, A Castillo, JA Alvarez-Muniz, J Batista, RA Ambrosio, M Aminaei, A Anchordoqui, L Andringa, S Aramo, C Aranda, VM Argiro, S Arisaka, K Arneodo, F Arqueros, F Asch, T Asorey, H Assis, P Aublin, J Ave, M Ag, M Avila, G Awal, N Badescubr, AM Balzer, M Barber, KB Barbosa, A Barenthienal, N Barkhausen, M Baeuml, J Baus, C Beattycj, J Becker, KH Bellidom, JA BenZvi, S Berat, C Bergmann, T Bertaina, ME Biermann, PL Bilhaut, R Billoir, P Blaes, SG Blanco, M Bleve, C Bluemer, H Bohacova, M Bolz, H Boncioli, D Bonifaz, C Bonino, R Boratav, M Borodai, N Bracci, F Brack, J Brancus, I Bridgeman, A Brogueira, P Brown, WC Buchholz, P Bueno, A Buitink, S Buscemi, M Caballero-Mora, KS Caccianiga, B Caccianiga, L Camin, D Candusso, M Caramete, L Caruso, R Castellina, A Castera, A Cataldi, G Cazon, L Cester, R Chavez, AG Chiavassa, A Chinellato, JA Chiosso, M Chudoba, J Cilmo, M Clark, PDJ Clay, RW Cocciolo, G Colalillo, R Coleman, A Collica, L Colombo, E Colonges, S Coluccia, MR Conceicao, R Contreras, F Cooper, MJ Coppens, J Cordier, A Courty, B Coutu, S Covault, CE Cronin, J Curutiu, A Dallier, R Daniel, B Dasso, S Daumiller, K Dawson, BR de Almeida, RM De Domenico, M De Donato, C de Jong, SJ Neto, JRTD De Mitri, I de Oliveira, J de Souza, V de Vries, KD del Peral, L Deligny, O Dembinski, H Dhital, N Di Giulio, C Di Matteo, A Diaz, JC Castro, MLD Diogo, F Dobrigkeit, C Docters, W D'Olivo, C Dolron, P Dorofeev, A Hasankiadeh, QD Dova, MT D'Urso, D Ebr, J Engel, R Epele, LN Erdmann, M Erfani, M Escobar, CO Espadanal, J Etchegoyen, A San Luis, PF Falcke, H Fang, K Farrar, G Fauth, AC Fazzini, N Ferguson, AP Fernandes, M Ferrero, A Fick, B Figueira, JM Filevich, A Filipcic, A Fox, BD Fraenkel, ED Fratu, O Freire, MM Frohlich, U Fuchs, B Fulgione, W Fujii, T Garcia, B Garcia-Gamez, D Garcia-Pinto, D Garilli, G Bravo, AG Gate, F Geenen, H Gemmeke, H Genolini, B Ghia, PL Giaccari, U Giammarchi, M Gibbs, K Giller, M Giudice, N Glaser, C Glass, H Berisso, MG Vitale, PFG Goncalves, P Gonzalez, JG Gonzalez, N Gookin, B Gora, D Gordon, J Gorgi, A Gorham, P Gotink, W Gouffon, P Grebe, S Griffith, N Grillo, AF Grubb, TD Grygar, J Guardone, N Guarino, F Guedes, GP Guglielmi, L Habraken, R Hampel, MR Hansen, P Harari, D Harmsma, S Harrison, TA Hartmann, S Harton, JL Haungs, A Hebbeker, T Heck, D Heimann, P Herve, AE Hill, GC Hojvat, C Hollon, N Holt, E Homola, P Horandel, JR Horneffer, A Horvat, M Horvath, P Hrabovsky, M Huber, D Hucker, H Huege, T Iarlori, M Insolia, A Isar, PG Jandt, I Jansen, S Jarne, C Johnsen, JA Josebachuili, M Kaapa, A Kambeitz, O Kampert, KH Kasper, P Katkov, I Kegl, B Keilhauer, B Keivani, A Kelley, J Kemp, E Kieckhafer, RM Klages, HO Kleifges, M Kleinfeller, J Knapp, J Kopmann, A Krause, R Krohm, N Kromer, O Kuempel, D Kunka, N LaHurd, D Latronico, L Lauer, R Lauscher, M Lautridou, P Le Coz, S Leao, MSAB Lebrun, D Lebrun, P de Oliveira, MAL Letessier-Selvon, A Lhenry-Yvon, I Link, K Lopez, R Casado, AL Louedec, K Bahilo, JL Lu, L Lucero, A Ludwig, M Malacari, M Maldera, S Mallamaci, M Maller, J Mandat, D Mantsch, P Mariazzi, AG Marin, V Maris, IC Marsella, G Martello, D Martina, L Martinez, H Martinez, N Bravo, OM Martraire, D Meza, JJM Mathes, HJ Mathys, S Matthews, J Matthews, JAJ Matthiae, G Maurel, D Maurizio, D Mayotte, E Mazur, PO Medina, C Medina-Tanco, G Meissner, R Melissas, M Mello, VBB Melo, D Menichetti, E Menshikov, A Messina, S Meyhandan, R Micanovic, S Micheletti, MI Middendorf, L Minaya, IA Miramonti, L Mitrica, B Molina-Bueno, L Mollerach, S Monasor, M Montanet, F Morello, C Mostafa, M Moura, CA Muller, MA Muller, G Muller, S Munchmeyer, M Mussa, R Navarra, G Navas, S Necesal, P Nellen, L Nelles, A Neuser, J Nguyen, PH Nicotra, D Niechciol, M Niemietz, L Niggemann, T Nitz, D Nosek, D Novotny, V Nozka, L Ochilo, L Ohnuki, T Oikonomou, F Olinto, A Oliveira, M Olmos-Gilbaja, VM Pacheco, N PakkSelmi-Dei, D Palatka, M Pallotta, J Palmieri, N Papenbreer, P Parente, G Parra, A Patel, M Paul, T Pech, M Pekala, J Pelayo, R Pepe, IM Perrone, L Petermann, E Peters, C Petrera, S Petrinca, P Petrov, Y Phuntsok, J Piegaia, R Pierog, T Pieroni, P Pimenta, M Pirronello, V Platino, M Plum, M Porcelli, A Porowski, C Porter, T Pouryamout, J Pouthas, J Prado, RR Privitera, P Prouza, M Pryke, CL Purrello, V Quel, EJ Querchfeld, S Quinn, S Randriatoamanana, R Rautenberg, J Ravel, O Ravignani, D Revenua, B Ridky, J Risse, M Ristori, P Rizi, V Robbins, S Roberts, M de Carvalho, WR Fernandez, GR Rojo, JR Rodriguez-Frias, MD Rogozin, D Ros, G Rosado, J Rossler, T Roth, M Roulet, E Rovero, AC Saffi, SJ Saftoiu, A Salamida, F Salazar, H Saleh, A Greus, FS Salina, G Sanchez, F Sanchez-Lucas, P Santo, CE Santos, E Santos, EM Sarazin, F Sarkar, B Sarmento, R Sato, R Scharf, N Scherini, V Schieler, H Schiffer, P Schmidt, A Schmidt, D Scholten, O Schoorlemmer, H Schovanek, P Schreuder, F Schroder, FG Schulz, A Schulz, J Schussler, F Schumacher, J Sciutto, SJ Segreto, A Sequeiros, G Settimo, M Shadkam, A Shellard, RC Sidelnik, I Sigl, G Sima, O Smialkowski, A Smida, R Smith, AGK Snow, GR Sommers, P Sorokin, J Speelman, R Spinka, H Squartini, R Srivastava, YN Stanic, S Stapleton, J Stasielak, J Stephan, M Stutz, A Suarez, F Suomijarvi, T Supanitsky, AD Sutherland, MS Sutter, M Swain, J Szadkowski, Z Szuba, M Taborda, OA Tapia, A Tcherniakhovski, D Tepe, A Theodoro, VM Timmermans, C Tkaczyk, W Peixoto, CJT Toma, G Tomankova, L Tome, B Tonachini, A Elipe, GT Machado, DT Travnicek, P Trovato, E Trung, TN Tunnicliffe, V Tusi, E Ulrich, R Unger, M Urban, M Galicia, JFV Valino, I Valore, L van Aar, G van Bodegom, P van den Berg, AM van Velzen, S van Vliet, A Varela, E Cardenas, BV Varnav, DM Varner, G Vasquez, R Vazquez, JR Vazquez, RA Veberic, D Verkooijen, H Verzi, V Vicha, J Videla, M Villasenor, L Vitali, G Vlcek, B Vorenholt, H Vorobiov, S Voyvodic, L Wahlberg, H Wainberg, O Walker, P Walz, D Watson, AA Weber, M Weidenhaupt, K Weindl, A Werner, F Westerhoff, S Widom, A Wiebusch, C Wiencke, L Wijnen, T Wilczynska, B Wilczynski, H Wild, N Winchen, T Wittkowski, D Woerner, G Wundheiler, B Wykes, S Yamamoto, T Yapici, T Yuan, G Yushkov, A Zamorano, B Zas, E Zavrtanik, D Zavrtanik, M Zepeda, A Zhou, J Zhu, Y Silva, MZ Zimmermann, B Ziolkowski, M Zuccarello, F AF Aab, A. Abreu, P. Aglietta, M. Ahn, E. J. Al Samarai, I. Albert, J. N. Albuquerque, I. F. M. Allekotte, I. Allen, J. Allison, P. Almela, A. Alvarez Castillo, J. Alvarez-Muniz, J. Batista, R. Alves Ambrosio, M. Aminaei, A. Anchordoqui, L. Andringa, S. Aramo, C. Aranda, V. M. Argiro, S. Arisaka, K. Arneodo, F. Arqueros, F. Asch, T. Asorey, H. Assis, P. Aublin, J. Ave, M. Avenier, M. Avila, G. Awal, N. Badescu, A. M. Balzer, M. Barber, K. B. Barbosa, A. Barenthien, N. Barkhausen, M. Baeuml, J. Baus, C. Beatty, J. Becker, K. H. Bellido, J. A. BenZvi, S. Berat, C. Bergmann, T. Bertaina, M. E. Biermann, P. L. Bilhaut, R. Billoir, P. Blaes, S. G. Blanco, M. Bleve, C. Bluemer, H. Bohacova, M. Bolz, H. Boncioli, D. Bonifaz, C. Bonino, R. Boratav, M. Borodai, N. Bracci, F. Brack, J. Brancus, I. Bridgeman, A. Brogueira, P. Brown, W. C. Buchholz, P. Bueno, A. Buitink, S. Buscemi, M. Caballero-Mora, K. S. Caccianiga, B. Caccianiga, L. Camin, D. Candusso, M. Caramete, L. Caruso, R. Castellina, A. Castera, A. Cataldi, G. Cazon, L. Cester, R. Chavez, A. G. Chiavassa, A. Chinellato, J. A. Chiosso, M. Chudoba, J. Cilmo, M. Clark, P. D. J. Clay, R. W. Cocciolo, G. Colalillo, R. Coleman, A. Collica, L. Colombo, E. Colonges, S. Coluccia, M. R. Conceicao, R. Contreras, F. Cooper, M. J. Coppens, J. Cordier, A. Courty, B. Coutu, S. Covault, C. E. Cronin, J. Curutiu, A. Dallier, R. Daniel, B. Dasso, S. Daumiller, K. Dawson, B. R. de Almeida, R. M. De Domenico, M. De Donato, C. de Jong, S. J. de Mello Neto, J. R. T. De Mitri, I. de Oliveira, J. de Souza, V. de Vries, K. D. del Peral, L. Deligny, O. Dembinski, H. Dhital, N. Di Giulio, C. Di Matteo, A. Diaz, J. C. Diaz Castro, M. L. Diogo, F. Dobrigkeit, C. Docters, W. D'Olivo, C. Dolron, P. Dorofeev, A. Hasankiadeh, Q. Dorosti Dova, M. T. D'Urso, D. Ebr, J. Engel, R. Epele, L. N. Erdmann, M. Erfani, M. Escobar, C. O. Espadanal, J. Etchegoyen, A. Facal San Luis, P. Falcke, H. Fang, K. Farrar, G. Fauth, A. C. Fazzini, N. Ferguson, A. P. Fernandes, M. Ferrero, A. Fick, B. Figueira, J. M. Filevich, A. Filipcic, A. Fox, B. D. Fraenkel, E. D. Fratu, O. Freire, M. M. Froehlich, U. Fuchs, B. Fulgione, W. Fujii, T. Garcia, B. Garcia-Gamez, D. Garcia-Pinto, D. Garilli, G. Gascon Bravo, A. Gate, F. Geenen, H. Gemmeke, H. Genolini, B. Ghia, P. L. Giaccari, U. Giammarchi, M. Gibbs, K. Giller, M. Giudice, N. Glaser, C. Glass, H. Gomez Berisso, M. Gomez Vitale, P. F. Goncalves, P. Gonzalez, J. G. Gonzalez, N. Gookin, B. Gora, D. Gordon, J. Gorgi, A. Gorham, P. Gotink, W. Gouffon, P. Grebe, S. Griffith, N. Grillo, A. F. Grubb, T. D. Grygar, J. Guardone, N. Guarino, F. Guedes, G. P. Guglielmi, L. Habraken, R. Hampel, M. R. Hansen, P. Harari, D. Harmsma, S. Harrison, T. A. Hartmann, S. Harton, J. L. Haungs, A. Hebbeker, T. Heck, D. Heimann, P. Herve, A. E. Hill, G. C. Hojvat, C. Hollon, N. Holt, E. Homola, P. Hoerandel, J. R. Horneffer, A. Horvat, M. Horvath, P. Hrabovsky, M. Huber, D. Hucker, H. Huege, T. Iarlori, M. Insolia, A. 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Melissas, M. Mello, V. B. B. Melo, D. Menichetti, E. Menshikov, A. Messina, S. Meyhandan, R. Micanovic, S. Micheletti, M. I. Middendorf, L. Minaya, I. A. Miramonti, L. Mitrica, B. Molina-Bueno, L. Mollerach, S. Monasor, M. Montanet, F. Morello, C. Mostafa, M. Moura, C. A. Muller, M. A. Mueller, G. Mueller, S. Muenchmeyer, M. Mussa, R. Navarra, G. Navas, S. Necesal, P. Nellen, L. Nelles, A. Neuser, J. Nguyen, P. H. Nicotra, D. Niechciol, M. Niemietz, L. Niggemann, T. Nitz, D. Nosek, D. Novotny, V. Nozka, L. Ochilo, L. Ohnuki, T. Oikonomou, F. Olinto, A. Oliveira, M. Olmos-Gilbaja, V. M. Pacheco, N. PakkSelmi-Dei, D. Palatka, M. Pallotta, J. Palmieri, N. Papenbreer, P. Parente, G. Parra, A. Patel, M. Paul, T. Pech, M. Pekala, J. Pelayo, R. Pepe, I. M. Perrone, L. Petermann, E. Peters, C. Petrera, S. Petrinca, P. Petrov, Y. Phuntsok, J. Piegaia, R. Pierog, T. Pieroni, P. Pimenta, M. Pirronello, V. Platino, M. Plum, M. Porcelli, A. Porowski, C. Porter, T. Pouryamout, J. Pouthas, J. 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Speelman, R. Spinka, H. Squartini, R. Srivastava, Y. N. Stanic, S. Stapleton, J. Stasielak, J. Stephan, M. Stutz, A. Suarez, F. Suomijaervi, T. Supanitsky, A. D. Sutherland, M. S. Sutter, M. Swain, J. Szadkowski, Z. Szuba, M. Taborda, O. A. Tapia, A. Tcherniakhovski, D. Tepe, A. Theodoro, V. M. Timmermans, C. Tkaczyk, W. Todero Peixoto, C. J. Toma, G. Tomankova, L. Tome, B. Tonachini, A. Torralba Elipe, G. Torres Machado, D. Travnicek, P. Trovato, E. Trung, T. N. Tunnicliffe, V. Tusi, E. Ulrich, R. Unger, M. Urban, M. Valdes Galicia, J. F. Valino, I. Valore, L. van Aar, G. van Bodegom, P. van den Berg, A. M. van Velzen, S. van Vliet, A. Varela, E. Vargas Cardenas, B. Varnav, D. M. Varner, G. Vasquez, R. Vazquez, J. R. Vazquez, R. A. Veberic, D. Verkooijen, H. Verzi, V. Vicha, J. Videla, M. Villasenor, L. Vitali, G. Vlcek, B. Vorenholt, H. Vorobiov, S. Voyvodic, L. Wahlberg, H. Wainberg, O. Walker, P. Walz, D. Watson, A. A. Weber, M. Weidenhaupt, K. Weindl, A. Werner, F. Westerhoff, S. Widom, A. Wiebusch, C. Wiencke, L. Wijnen, T. Wilczynska, B. Wilczynski, H. Wild, N. Winchen, T. Wittkowski, D. Woerner, G. Wundheiler, B. Wykes, S. Yamamoto, T. Yapici, T. Yuan, G. Yushkov, A. Zamorano, B. Zas, E. Zavrtanik, D. Zavrtanik, M. Zepeda, A. Zhou, J. Zhu, Y. Silva, M. Zimbres Zimmermann, B. Ziolkowski, M. Zuccarello, F. TI The Pierre Auger Cosmic Ray Observatory SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Pierre Auger Observatory; High energy cosmic rays; Hybrid observatory; Water Cherenkov detectors; Air fluorescence detectors ID EXTENSIVE AIR-SHOWERS; ULTRA-HIGH ENERGY; ATMOSPHERIC MULTIPLE-SCATTERING; SURFACE DETECTOR ARRAY; FLUORESCENCE YIELD; LOWER IONOSPHERE; LIGHT; RECONSTRUCTION; RADIATION; EMISSION AB The Pierre Auger Observatory, located on a vast, high plain in western Argentina, is the world's largest cosmic ray observatory. The objectives of the Observatory are to probe the origin and characteristics of cosmic rays above 10(17) eV and to study the interactions of these, the most energetic particles observed in nature. The Auger design features an array of 1660 water Cherenkov particle detector stations spread over 3000 km(2) overlooked by 24 air fluorescence telescopes. In addition, three high elevation fluorescence telescopes overlook a 23.5 km(2), 61-detector infilled array with 750 in spacing. The Observatory has been in successful operation since completion in 2008 and has recorded data from an exposure exceeding 40,000 km(2) sr yr. This paper describes the design and performance of the detectors, related subsystems and infrastructure that make up the Observatory. (C) 2015 The Authors. Published by Elsevier B.V. C1 [Allekotte, I.; Asorey, H.; Ave, M.; Gomez Berisso, M.; Harari, D.; Mollerach, S.; Purrello, V.; Roulet, E.; Sidelnik, I.; Taborda, O. A.] Ctr Atom Bariloche, Buenos Aires, DF, Argentina. 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J.; Knapp, J.; Lu, L.; Patel, M.; Tunnicliffe, V.; Walker, P.; Watson, A. A.] Univ Leeds, Sch Phys & Astron, Leeds LS2 9JT, W Yorkshire, England. [Covault, C. E.; Ferguson, A. P.; LaHurd, D.; Quinn, S.] Case Western Reserve Univ, Cleveland, OH 44106 USA. [Johnsen, J. A.; Mayotte, E.; Medina, C.; Sarazin, F.; Wiencke, L.] Colorado Sch Mines, Golden, CO 80401 USA. [Brack, J.; Dorofeev, A.; Gookin, B.; Harton, J. L.; Petrov, Y.] Colorado State Univ, Ft Collins, CO 80523 USA. [Brown, W. C.] Colorado State Univ, Pueblo, CO USA. [Anchordoqui, L.] CUNY Herbert H Lehman Coll, Dept Phys & Astron, New York, NY USA. [Ahn, E. J.; Escobar, C. O.; Fazzini, N.; Glass, H.; Hojvat, C.; Kasper, P.; Lebrun, P.; Mantsch, P.; Mazur, P. O.; Spinka, H.; Voyvodic, L.] Fermilab Natl Accelerator Lab, Batavia, IL USA. [Matthews, J.; Porter, T.; Shadkam, A.; Yuan, G.] Louisiana State Univ, Baton Rouge, LA 70803 USA. [Dhital, N.; Diaz, J. C.; Fick, B.; Kieckhafer, R. M.; Nitz, D.; Yapici, T.] Michigan Technol Univ, Houghton, MI 49931 USA. [Allen, J.; Awal, N.; Farrar, G.; Unger, M.] NYU, New York, NY USA. [Paul, T.; Srivastava, Y. N.; Swain, J.; Widom, A.] Northeastern Univ, Boston, MA 02115 USA. [Allison, P.; Beatty, J.; Gordon, J.; Griffith, N.; Stapleton, J.; Sutherland, M. S.] Ohio State Univ, Columbus, OH 43210 USA. [Coleman, A.; Coutu, S.; Keivani, A.; Mostafa, M.; Oikonomou, F.; Phuntsok, J.; Roberts, M.; Salesa Greus, F.; Sommers, P.] Penn State Univ, University Pk, PA 16802 USA. [Cronin, J.; Facal San Luis, P.; Fang, K.; Fujii, T.; Gibbs, K.; Hollon, N.; Monasor, M.; Olinto, A.; Privitera, P.; Pryke, C. L.; Yamamoto, T.; Zhou, J.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Fox, B. D.; Gorham, P.; Meyhandan, R.; Schoorlemmer, H.; Varner, G.] Univ Hawaii, Honolulu, HI 96822 USA. [Petermann, E.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Lauer, R.; Matthews, J. A. J.] Univ New Mexico, Albuquerque, NM 87131 USA. [Arisaka, K.; Ohnuki, T.] Univ Calif Los Angeles, Los Angeles, CA USA. [BenZvi, S.; Westerhoff, S.] Univ Wisconsin, Madison, WI USA. [Martinez, N.] Univ Autonoma Chiapas, Buenos Aires, DF, Argentina. [Zepeda, A.] Vrije Univ Brussels, Brussels, Belgium. RP Aab, A (reprint author), Univ Siegen, D-57068 Siegen, Germany. RI Sima, Octavian/C-3565-2011; Insolia, Antonio/M-3447-2015; Horvath, Pavel/G-6334-2014; Valino, Ines/J-8324-2012; Ros, German/L-4764-2014; Badescu, Alina/B-6087-2012; Torralba Elipe, Guillermo/A-9524-2015; de souza, Vitor/D-1381-2012; van den Berg, Adriaan/P-6792-2015; Vazquez, Jose Ramon/K-2272-2015; Pech, Miroslav/G-5760-2014; Brogueira, Pedro/K-3868-2012; Martello, Daniele/J-3131-2012; Rodriguez Frias, Maria /A-7608-2015; Wiebusch, Christopher/G-6490-2012; Inst. of Physics, Gleb Wataghin/A-9780-2017; De Mitri, Ivan/C-1728-2017; Mitrica, Bogdan/D-5201-2009; Alves Batista, Rafael/K-6642-2012; dos Santos, Eva/N-6351-2013; Nosek, Dalibor/F-1129-2017; Ridky, Jan/H-6184-2014; Cazon, Lorenzo/G-6921-2014; Conceicao, Ruben/L-2971-2014; Bueno, Antonio/F-3875-2015; Beatty, James/D-9310-2011; Schussler, Fabian/G-5313-2013; de Mello Neto, Joao/C-5822-2013; Guarino, Fausto/I-3166-2012; Colalillo, Roberta/R-5088-2016; Buscemi, Mario/R-5071-2016; Zuccarello, Francesca/R-1834-2016; Bonino, Raffaella/S-2367-2016; Tome, Bernardo/J-4410-2013; Alvarez-Muniz, Jaime/H-1857-2015; Kopmann, Andreas/B-3454-2013; Gouffon, Philippe/I-4549-2012; de Almeida, Rogerio/L-4584-2016; Fauth, Anderson/F-9570-2012; De Domenico, Manlio/B-5826-2014; Sao Carlos Institute of Physics, IFSC/USP/M-2664-2016; Abreu, Pedro/L-2220-2014; Assis, Pedro/D-9062-2013; Navas, Sergio/N-4649-2014; Garcia Pinto, Diego/J-6724-2014; Caramete, Laurentiu/C-2328-2011; Rosado, Jaime/K-9109-2014; Lozano-Bahilo, Julio/F-4881-2016; zas, enrique/I-5556-2015; Chinellato, Jose Augusto/I-7972-2012; Chinellato, Carola Dobrigkeit /F-2540-2011; Arqueros, Fernando/K-9460-2014; De Donato, Cinzia/J-9132-2015; Goncalves, Patricia /D-8229-2013; Moura Santos, Edivaldo/K-5313-2016; Pimenta, Mario/M-1741-2013 OI Insolia, Antonio/0000-0002-9040-1566; Horvath, Pavel/0000-0002-6710-5339; Valino, Ines/0000-0001-7823-0154; Ros, German/0000-0001-6623-1483; Torralba Elipe, Guillermo/0000-0001-8738-194X; Vazquez, Jose Ramon/0000-0001-9217-5219; Brogueira, Pedro/0000-0001-6069-4073; Martello, Daniele/0000-0003-2046-3910; Erdmann, Martin/0000-0002-1653-1303; Zamorano, Bruno/0000-0002-4286-2835; Petrera, Sergio/0000-0002-6029-1255; Rodriguez Frias, Maria /0000-0002-2550-4462; Wiebusch, Christopher/0000-0002-6418-3008; De Mitri, Ivan/0000-0002-8665-1730; Alves Batista, Rafael/0000-0003-2656-064X; dos Santos, Eva/0000-0002-0474-8863; Nosek, Dalibor/0000-0001-6219-200X; Salamida, Francesco/0000-0002-9306-8447; Ridky, Jan/0000-0001-6697-1393; Cazon, Lorenzo/0000-0001-6748-8395; Conceicao, Ruben/0000-0003-4945-5340; Bueno, Antonio/0000-0002-7439-4247; Beatty, James/0000-0003-0481-4952; Schussler, Fabian/0000-0003-1500-6571; de Mello Neto, Joao/0000-0002-3234-6634; Guarino, Fausto/0000-0003-1427-9885; Colalillo, Roberta/0000-0002-4179-9352; Buscemi, Mario/0000-0003-2123-5434; Zuccarello, Francesca/0000-0003-1853-2550; Tome, Bernardo/0000-0002-7564-8392; Alvarez-Muniz, Jaime/0000-0002-2367-0803; Kopmann, Andreas/0000-0002-2362-3943; Gouffon, Philippe/0000-0001-7511-4115; de Almeida, Rogerio/0000-0003-3104-2724; Fauth, Anderson/0000-0001-7239-0288; De Domenico, Manlio/0000-0001-5158-8594; Abreu, Pedro/0000-0002-9973-7314; Assis, Pedro/0000-0001-7765-3606; Navas, Sergio/0000-0003-1688-5758; Garcia Pinto, Diego/0000-0003-1348-6735; Rosado, Jaime/0000-0001-8208-9480; Lozano-Bahilo, Julio/0000-0003-0613-140X; zas, enrique/0000-0002-4430-8117; Chinellato, Jose Augusto/0000-0002-3240-6270; Chinellato, Carola Dobrigkeit /0000-0002-1236-0789; Arqueros, Fernando/0000-0002-4930-9282; De Donato, Cinzia/0000-0002-9725-1281; Goncalves, Patricia /0000-0003-2042-3759; Moura Santos, Edivaldo/0000-0002-2818-8813; Dembinski, Hans/0000-0003-3337-3850; Lauer, Robert/0000-0003-1933-7861; Rodriguez Fernandez, Gonzalo/0000-0002-4683-230X; Del Peral, Luis/0000-0003-2580-5668; Coutu, Stephane/0000-0003-2923-2246; Bonino, Raffaella/0000-0002-4264-1215; Rizi, Vincenzo/0000-0002-5277-6527; Ulrich, Ralf/0000-0002-2535-402X; Novotny, Vladimir/0000-0002-4319-4541; Garcia, Beatriz/0000-0003-0919-2734; Ravignani, Diego/0000-0001-7410-8522; Segreto, Alberto/0000-0001-7341-6603; Aglietta, Marco/0000-0001-8354-5388; Kothandan, Divay/0000-0001-9048-7518; Castellina, Antonella/0000-0002-0045-2467; maldera, simone/0000-0002-0698-4421; Matthews, James/0000-0002-1832-4420; Yuan, Guofeng/0000-0002-1907-8815; Pimenta, Mario/0000-0002-2590-0908 FU Comision Nacional de Energia Atomica; Fundacion Antorchas; Gobierno De La Provincia de Mendoza; Municipalidad de Malargue; NDM Holdings and Valle Las Lenas; Australian Research Council; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Rio de Janeiro (FAPERJ); Sao Paulo Research Foundation (FAPESP) [2010/07359-6, 1999/05404-3]; Ministerio de Ciencia e Tecnologia (MCT), Brazil; MSMT-CR [LG13007, 7AMB14AR005, CZ.1.05/2.1.00/03.0058]; Czech Science Foundation, Czech Republic [14-17501S]; Centre de Calcul IN2P3/CNRS; Centre National de la Recherche Scientifique (CNRS); Conseil Regional Ile-de-France; Departement Physique Nucleaire et Corpusculaire [PNC-IN2P3/CNRS]; Departement Sciences de l'Univers (SDU-INSU/CNRS); Institut Lagrange de Paris; ILP LABEX within the Investissements d'Avenir Programme, France [ANR-11-IDEX-0004-02 ANR-10-LABX-63]; Bundesministerium fur Bildung und Forschung (BMBF); Deutsche Forschungsgemeinschaft (DFG); Finanzministerium Baden-Wurttemberg; Helmholtz Alliance for Astroparticle Physics (HAP); Helmholtz-Gemeinschaft Deutscher Forschungszentren (HGF); Ministerium fur Wissenschaft und Forschung; Nordrhein Westfalen; Ministerium fur Wissenschaft; Forschung und Kunst; Baden-Wurttemberg, Germany; Istituto Nazionale di Astrofisica (INAF); Istituto Nazionale di Fisica Nucleare (INFN); Ministero dell'Istruzione, dell'Universita e della Ricerca (MIUR); Gran Sasso Center for Astroparticle Physics (CFA); CETEMPS Center of Excellence, Italy; Consejo Nacional de Ciencia y Tecnologia (CONACYT), Mexico; Ministerie van Onderwijs; Cultuur en Wetenschap; Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO); Stichting voor Fundamenteel Onderzoek der Materie (FOM), Netherlands; National Centre for Research and Development [ERA-NET-ASPERA/01/11, ERA-NET-ASPERA/02/11]; National Science Centre, Poland [2013/08/M/ST9/00322, 2013/08/M/ST9/00728, HARMONIA 5 - 2013/10/M/ST9/00062]; Portuguese national funds; FEDER funds within COMPETE - Programa Operacional Factores de Competitividade through Fundacao para a Ciencia e a Tecnologia, Portugal; Romanian Authority for Scientific Research ANCS; CNDI-UEFISCDI [20/2012, 194/2012, 1/ASPERA2/2012 ERA-NET, PN-II-RU-PD-2011-3-0145-17, PN-II-RU-PD-2011-3-0062]; Programme for research - Space Technology and Advanced Research - STAR, Romania [83/2013]; Slovenian Research Agency, Slovenia; Comunidad de Madrid; FEDER funds; Ministerio de Educacion y Ciencia; Xunta de Galicia; European Community, Spain [FP7-PEOPLE-2012-IEF-328826]; Science and Technology Facilities Council, United Kingdom; Department of Energy [DE-AC02-07CH11359, DE-FR02-04ER41300, DE-FG02-99ER41107, DE-SC0011689]; National Science Foundation [0450696]; Grainger Foundation, USA; NAFOSTED, Vietnam; Marie Curie-IRSES/EPLANET; European Particle Physics Latin American Network; European Union [PIRSES-2009-GA-246806]; UNESCO FX We are very grateful to the following agencies and organizations for financial support: Comision Nacional de Energia Atomica, Fundacion Antorchas, Gobierno De La Provincia de Mendoza, Municipalidad de Malargue, NDM Holdings and Valle Las Lenas, in gratitude for their continuing cooperation over land access, Argentina; the Australian Research Council; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Rio de Janeiro (FAPERJ), Sao Paulo Research Foundation (FAPESP) Grants # 2010/07359-6 and # 1999/05404-3, Ministerio de Ciencia e Tecnologia (MCT), Brazil; MSMT-CR LG13007, 7AMB14AR005, CZ.1.05/2.1.00/03.0058 and the Czech Science Foundation Grant 14-17501S, Czech Republic; Centre de Calcul IN2P3/CNRS, Centre National de la Recherche Scientifique (CNRS), Conseil Regional Ile-de-France, Departement Physique Nucleaire et Corpusculaire (PNC-IN2P3/CNRS), Departement Sciences de l'Univers (SDU-INSU/CNRS), Institut Lagrange de Paris, ILP LABEX ANR-10-LABX-63, within the Investissements d'Avenir ProgrammeANR-11-IDEX-0004-02, France; Bundesministerium fur Bildung und Forschung (BMBF), Deutsche Forschungsgemeinschaft (DFG), Finanzministerium Baden-Wurttemberg, Helmholtz Alliance for Astroparticle Physics (HAP), Helmholtz-Gemeinschaft Deutscher Forschungszentren (HGF), Ministerium fur Wissenschaft und Forschung, Nordrhein Westfalen, Ministerium fur Wissenschaft, Forschung und Kunst, Baden-Wurttemberg, Germany; Istituto Nazionale di Astrofisica (INAF), Istituto Nazionale di Fisica Nucleare (INFN), Ministero dell'Istruzione, dell'Universita e della Ricerca (MIUR), Gran Sasso Center for Astroparticle Physics (CFA), CETEMPS Center of Excellence, Italy; Consejo Nacional de Ciencia y Tecnologia (CONACYT), Mexico; Ministerie van Onderwijs, Cultuur en Wetenschap, Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Stichting voor Fundamenteel Onderzoek der Materie (FOM), Netherlands; National Centre for Research and Development, Grant nos. ERA-NET-ASPERA/01/11 and ERA-NET-ASPERA/02/11, National Science Centre, Grant nos. 2013/08/M/ST9/00322, and 2013/08/M/ST9/00728 and HARMONIA 5 - 2013/10/M/ST9/00062, Poland; Portuguese national funds and FEDER funds within COMPETE - Programa Operacional Factores de Competitividade through Fundacao para a Ciencia e a Tecnologia, Portugal; Romanian Authority for Scientific Research ANCS, CNDI-UEFISCDI partnership projects nos. 20/2012 and nr.194/2012, project nos. 1/ASPERA2/2012 ERA-NET, PN-II-RU-PD-2011-3-0145-17, and PN-II-RU-PD-2011-3-0062, the Minister of National Education, Programme for research - Space Technology and Advanced Research - STAR, project number 83/2013, Romania; Slovenian Research Agency, Slovenia; Comunidad de Madrid, FEDER funds, Ministerio de Educacion y Ciencia, Xunta de Galicia, European Community 7th Framework Program, Grant no. FP7-PEOPLE-2012-IEF-328826, Spain; Science and Technology Facilities Council, United Kingdom; Department of Energy, Contract no. DE-AC02-07CH11359, DE-FR02-04ER41300, DE-FG02-99ER41107 and DE-SC0011689, National Science Foundation, Grant no. 0450696, The Grainger Foundation, USA; NAFOSTED, Vietnam; Marie Curie-IRSES/EPLANET, European Particle Physics Latin American Network, European Union 7th Framework Program, Grant no. PIRSES-2009-GA-246806; and UNESCO. NR 160 TC 43 Z9 43 U1 18 U2 102 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD OCT 21 PY 2015 VL 798 BP 172 EP 213 DI 10.1016/j.nima.2015.06.058 PG 42 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CQ9KO UT WOS:000360933600025 ER PT J AU Dong, RB Hall, C Rice, K Chiang, E AF Dong, Ruobing Hall, Cassandra Rice, Ken Chiang, Eugene TI SPIRAL ARMS IN GRAVITATIONALLY UNSTABLE PROTOPLANETARY DISKS AS IMAGED IN SCATTERED LIGHT SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE circumstellar matter; planets and satellites: formation; protoplanetary disks; stars: formation; stars: pre-main sequence; stars: variables: T Tauri; Herbig Ae/Be ID 206462 HD 135344B; INDUCED GAP EDGES; TRANSITIONAL DISKS; IMAGING POLARIMETRY; PROTOSTELLAR DISCS; ACCRETION DISCS; GIANT PLANETS; OBSERVATIONAL SIGNATURES; EMBEDDED PLANETS; DUST FILTRATION AB Combining 3D smoothed-particle hydrodynamics and Monte Carlo radiative transfer calculations, we examine the morphology of spiral density waves induced by gravitational instability (GI) in protoplanetary disks, as they would appear in direct images at near-infrared (NIR) wavelengths. We find that systems with disk-to-star-mass ratios q = M-disk/M-star that are similar to 0.25 or more may produce prominent spiral arms in NIR imaging, remarkably resembling features observed in the MWC 758 and SAO 206462 systems. The contrast of GI-induced arms at NIR wavelengths can reach a factor of similar to 3, and their pitch angles are about 10 degrees-15 degrees. The dominant azimuthal wavenumber of GI-induced spiral arms roughly obeys m similar to 1/q in the range 2 less than or similar to 1/q less than or similar to 8. In particular, a massive disk with q approximate to 0.5 can exhibit grand-design m = 2 spirals. GI-induced arms are in approximate corotation with the local disk, and may therefore trap dust particles by pressure drag. Although GI can produce NIR spiral arms with morphologies, contrasts, and pitch angles similar to those reported in recent observations, it also makes other demands that may or may not be satisfied in any given system. A GI origin requires that the spirals be relatively compact, on scales less than or similar to 100 AU; that the disk be massive, q greater than or similar to 0.25; and that the accretion rate M-star be high, on the order of 10(-6) M-circle dot yr(-1). C1 [Dong, Ruobing] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Dong, Ruobing; Chiang, Eugene] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Hall, Cassandra; Rice, Ken] Univ Edinburgh, Inst Astron, Edinburgh EH9 3HJ, Midlothian, Scotland. RP Dong, RB (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM rdong2013@berkeley.edu RI Rice, Ken/H-5084-2011 OI Rice, Ken/0000-0002-6379-9185 FU NASA [HST-HF-51320.01-A, NAS 5-26555]; Space Telescope Science Institute; NSF; UC Berkeley Vice Chancellor for Research; Berkeley Center for Integrative Planetary Science FX R.D. thanks Cathie Clarke and Roman Rafikov for educating him on the subject of GI. We thank Myriam Benisty and Antonio Garufi for kindly sharing with us the VLT/SPHERE image of MWC 758, and the VLT/NACO image of SAO 206462, respectively. We are grateful to the anonymous referee for constructive suggestions that improved the quality of the paper. This project is partially supported by NASA through Hubble Fellowship grant HST-HF-51320.01-A (R.D.) awarded by the Space Telescope Science Institute, which is operated by the Association of Universities for Research in Astronomy, Inc., for NASA, under contract NAS 5-26555. E.C. acknowledges support from NASA and the NSF. Numerical calculations were performed on the SAVIO cluster provided by the Berkeley Research Computing program, supported by the UC Berkeley Vice Chancellor for Research and the Berkeley Center for Integrative Planetary Science. NR 70 TC 0 Z9 0 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD OCT 20 PY 2015 VL 812 IS 2 AR L32 DI 10.1088/2041-8205/812/2/L32 PG 7 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CV7WC UT WOS:000364485600015 ER PT J AU Gonzalez, AH Decker, B Brodwin, M Eisenhardt, PRM Marrone, DP Stanford, SA Stern, D Wylezalek, D Aldering, G Abdulla, Z Boone, K Carlstrom, J Fagrelius, P Gettings, DP Greer, CH Hayden, B Leitch, EM Lin, YT Mantz, AB Muchovej, S Perlmutter, S Zeimann, GR AF Gonzalez, Anthony H. Decker, Bandon Brodwin, Mark Eisenhardt, Peter R. M. Marrone, Daniel P. Stanford, S. A. Stern, Daniel Wylezalek, Dominika Aldering, Greg Abdulla, Zubair Boone, Kyle Carlstrom, John Fagrelius, Parker Gettings, Daniel P. Greer, Christopher H. Hayden, Brian Leitch, Erik M. Lin, Yen-Ting Mantz, Adam B. Muchovej, Stephen Perlmutter, Saul Zeimann, Gregory R. TI THE MASSIVE AND DISTANT CLUSTERS OF WISE SURVEY: MOO J1142+1527, A 10(15) M-circle dot GALAXY CLUSTER AT z=1.19 SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE galaxies: clusters: individual (MOO J1142+1527); galaxies: clusters: intracluster medium ID LESS-THAN 3.2; SPT-SZ SURVEY; SIMILAR-TO 1; SPECTROSCOPIC CONFIRMATION; COSMOLOGICAL PARAMETERS; SKY SURVEY; 1ST; CONSTRAINTS; SAMPLE; TELESCOPE AB We present confirmation of the cluster MOO J1142+1527, a massive galaxy cluster discovered as part of the Massive and Distant Clusters of WISE Survey. The cluster is confirmed to lie at z = 1.19, and using the Combined Array for Research in Millimeter-wave Astronomy we robustly detect the Sunyaev-Zel'dovich (SZ) decrement at 13.2 sigma. The SZ data imply a mass of M-200m = (1.1 +/- 0.2) x 10(15) M-circle dot, making MOO J1142+1527 the most massive galaxy cluster known at z > 1.15 and the second most massive cluster known at z > 1. For a standard Lambda CDM cosmology it is further expected to be one of the similar to 5 most massive clusters expected to exist at z >= 1.19 over the entire sky. Our ongoing Spitzer program targeting similar to 1750 additional candidate clusters will identify comparably rich galaxy clusters over the full extragalactic sky. C1 [Gonzalez, Anthony H.; Gettings, Daniel P.] Univ Florida, Dept Astron, Gainesville, FL 32611 USA. [Decker, Bandon; Brodwin, Mark] Univ Missouri, Dept Phys & Astron, Kansas City, MO 64110 USA. [Eisenhardt, Peter R. M.; Stern, Daniel] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Marrone, Daniel P.; Greer, Christopher H.] Univ Arizona, Steward Observ, Tucson, AZ 85121 USA. [Stanford, S. A.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Stanford, S. A.] Lawrence Livermore Natl Lab, Inst Geophys & Planetary Phys, Livermore, CA 94550 USA. [Wylezalek, Dominika] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Aldering, Greg; Boone, Kyle; Fagrelius, Parker; Hayden, Brian; Perlmutter, Saul] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Abdulla, Zubair; Carlstrom, John; Leitch, Erik M.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Abdulla, Zubair; Carlstrom, John; Leitch, Erik M.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Boone, Kyle; Fagrelius, Parker; Perlmutter, Saul] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Hayden, Brian] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Lin, Yen-Ting] Acad Sinica, Inst Astron & Astrophys, Taipei 115, Taiwan. [Mantz, Adam B.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, Stanford, CA 94305 USA. [Mantz, Adam B.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Muchovej, Stephen] CALTECH, Owens Valley Radio Observ, Big Pine, CA 93513 USA. [Muchovej, Stephen] CALTECH, Dept Astron, Pasadena, CA 91125 USA. [Zeimann, Gregory R.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. RP Gonzalez, AH (reprint author), Univ Florida, Dept Astron, Gainesville, FL 32611 USA. FU NASA [90177]; ADAP grant [NNX12AE15G]; NASA Exoplanet Science Institute [1461527, 1486927]; U. S. Department of Energy [W-7405-ENG-48]; Gordon and Betty Moore Foundation; Kenneth T. and Eileen L. Norris Foundation; James S. McDonnell Foundation; Associates of the California Institute of Technology; University of Chicago; states of California, Illinois, and Maryland; National Science Foundation; NSF [AST-1140019]; CARMA partner universities; [PHY-0114422] FX We thank the anonymous referee for comments that improved the quality of this paper. Support for this research was provided by NASA through Spitzer GO program 90177, ADAP grant NNX12AE15G, and NASA Exoplanet Science Institute grants 1461527 and 1486927. The work by SAS at LLNL was performed under the auspices of the U. S. Department of Energy under Contract No. W-7405-ENG-48.; Support for CARMA construction was derived from the Gordon and Betty Moore Foundation; the Kenneth T. and Eileen L. Norris Foundation; the James S. McDonnell Foundation; the Associates of the California Institute of Technology; the University of Chicago; the states of California, Illinois, and Maryland; and the National Science Foundation. CARMA development and operations were supported by NSF under a cooperative agreement and by the CARMA partner universities; the work at Chicago was supported by NSF grant AST-1140019. Additional support was provided by PHY-0114422. This publication makes use of data products from the Wide-field Infrared Survey Explorer, a joint project of the University of California, Los Angeles, and the Jet Propulsion Laboratory/California Institute of Technology, funded by NASA. This work is based in part on observations made with the Spitzer Space Telescope, which is operated by the Jet Propulsion Laboratory, California Institute of Technology under a contract with NASA. This work is based in part on data obtained at the W. M. Keck and Gemini Observatories. The authors wish to recognize and acknowledge the very significant cultural role and reverence that the summit of Mauna Kea has always had within the indigenous Hawaiian community. We are most fortunate to have the opportunity to conduct observations from this mountain. NR 42 TC 0 Z9 0 U1 3 U2 8 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD OCT 20 PY 2015 VL 812 IS 2 AR L40 DI 10.1088/2041-8205/812/2/L40 PG 6 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CV7WC UT WOS:000364485600023 ER PT J AU Latawiec, P Venkataraman, V Burek, MJ Hausmann, BJM Bulu, I Loncar, M AF Latawiec, Pawel Venkataraman, Vivek Burek, Michael J. Hausmann, Birgit J. M. Bulu, Irfan Loncar, Marko TI On-chip diamond Raman laser SO OPTICA LA English DT Article ID SINGLE-CRYSTAL DIAMOND; SILICON LASER; MU-M; CVD-DIAMOND; THRESHOLD; EFFICIENT; CAVITY; MICROCAVITY; GENERATION; CONVERSION AB Synthetic single-crystal diamond has recently emerged as a promising platform for Raman lasers at exotic wavelengths due to its giant Raman shift, large transparency window, and excellent thermal properties yielding a greatly enhanced figure of merit compared to conventional materials. To date, diamond Raman lasers have been realized using bulk plates placed inside macroscopic cavities, requiring careful alignment and resulting in high threshold powers (W-kW range). Here we demonstrate an on-chip Raman laser based on fully integrated, high-quality-factor, diamond racetrack microresonators embedded in silica. Pumping at telecom wavelengths, we show Stokes output discretely tunable over a similar to 100 nm bandwidth around 2 mu m with output power > 250 mu W, extending the functionality of diamond Raman lasers to an interesting wavelength range at the edge of the mid-infrared spectrum. Continuous-wave operation with only similar to 85 mW pump threshold power in the feeding waveguide is demonstrated along with continuous, mode-hop-free tuning over similar to 7.5 GHz in a compact, integrated-optics platform. (C) 2015 Optical Society of America C1 [Latawiec, Pawel; Venkataraman, Vivek; Burek, Michael J.; Loncar, Marko] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. [Hausmann, Birgit J. M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Hausmann, Birgit J. M.] LBNL, Div Mat Sci, Berkeley, CA 94720 USA. [Bulu, Irfan] Schlumberger Doll Res Ctr, Cambridge, MA 02139 USA. RP Loncar, M (reprint author), Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. EM loncar@seas.harvard.edu FU National Science Foundation (NSF) [ECCS-1202157] FX National Science Foundation (NSF) (ECCS-1202157). NR 32 TC 13 Z9 13 U1 6 U2 13 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 2334-2536 J9 OPTICA JI Optica PD OCT 20 PY 2015 VL 2 IS 11 BP 924 EP 928 DI 10.1364/OPTICA.2.000924 PG 5 WC Optics SC Optics GA CX5JO UT WOS:000365738100003 ER PT J AU Bauer, FE Arevalo, P Walton, DJ Koss, MJ Puccetti, S Gandhi, P Stern, D Alexander, DM Balokovic, M Boggs, SE Brandt, WN Brightman, M Christensen, FE Comastri, A Craig, WW Del Moro, A Hailey, CJ Harrison, FA Hickox, R Luo, B Markwardt, CB Marinucci, A Matt, G Rigby, JR Rivers, E Saez, C Treister, E Urry, CM Zhang, WW AF Bauer, Franz E. Arevalo, Patricia Walton, Dominic J. Koss, Michael J. Puccetti, Simonetta Gandhi, Poshak Stern, Daniel Alexander, David M. Balokovic, Mislav Boggs, Steve E. Brandt, William N. Brightman, Murray Christensen, Finn E. Comastri, Andrea Craig, William W. Del Moro, Agnese Hailey, Charles J. Harrison, Fiona A. Hickox, Ryan Luo, Bin Markwardt, Craig B. Marinucci, Andrea Matt, Giorgio Rigby, Jane R. Rivers, Elizabeth Saez, Cristian Treister, Ezequiel Urry, C. Megan Zhang, William W. TI NuSTAR SPECTROSCOPY OF MULTI-COMPONENT X-RAY REFLECTION FROM NGC 1068 SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: active; galaxies: individual (NGC 1068); X-rays: galaxies ID ACTIVE GALACTIC NUCLEI; NARROW-LINE REGION; SEYFERT 2 GALAXIES; XMM-NEWTON; BROAD-BAND; IONIZED-GAS; MOLECULAR CLOUDS; BLACK-HOLES; REVERBERATION MEASUREMENTS; RESOLVED SPECTROSCOPY AB We report on high-energy X-ray observations of the Compton-thick Seyfert 2 galaxy NGC 1068 with NuSTAR, which provide the best constraints to date on its >10 keV spectral shape. The NuSTAR data are consistent with those from past and current instruments to within cross-calibration uncertainties, and we find no strong continuum or line variability over the past two decades, which is in line with its X-ray classification as a reflection-dominated Compton-thick active galactic nucleus. The combined NuSTAR, Chandra, XMM-Newton, and Swift BAT spectral data set offers new insights into the complex secondary emission seen instead of the completely obscured transmitted nuclear continuum. The critical combination of the high signal-to-noise NuSTAR data and the decomposition of the nuclear and extranuclear emission with Chandra allow us to break several model degeneracies and greatly aid physical interpretation. When modeled as a monolithic (i.e., a single N-H) reflector, none of the common Compton reflection models are able to match the neutral fluorescence lines and broad spectral shape of the Compton reflection hump without requiring unrealistic physical parameters (e.g., large Fe overabundances, inconsistent viewing angles, or poor fits to the spatially resolved spectra). A multi-component reflector with three distinct column densities (e.g., with best-fit values of N-H of 1.4 x 10(23), 5.0 x 10(24), and 10(25) cm(-2)) provides a more reasonable fit to the spectral lines and Compton hump, with near-solar Fe abundances. In this model, the higher N-H component provides the bulk of the flux to the Compton hump, while the lower N-H component produces much of the line emission, effectively decoupling two key features of Compton reflection. We find that approximate to 30% of the neutral Fe K alpha line flux arises from >2 '' (approximate to 140 pc) and is clearly extended, implying that a significant fraction (and perhaps most) of the <10 keV reflected component arises from regions well outside a parsec-scale torus. These results likely have ramifications for the interpretation of Compton-thick spectra from observations with poorer signal-to-noise and/or more distant objects. C1 [Bauer, Franz E.] Pontificia Univ Catolica Chile, Inst Astrofis, Santiago 22, Chile. [Bauer, Franz E.] Millenium Inst Astrophys, Santiago, Chile. [Bauer, Franz E.; Arevalo, Patricia; Treister, Ezequiel] EMBIGGEN Anillo, Concepcion, Chile. [Bauer, Franz E.] Space Sci Inst, Boulder, CO 80301 USA. [Arevalo, Patricia] Univ Valparaiso, Fac Ciencias, Inst Fis & Astron, Valparaiso, Chile. [Walton, Dominic J.; Balokovic, Mislav; Brightman, Murray; Harrison, Fiona A.; Rivers, Elizabeth] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Walton, Dominic J.; Stern, Daniel] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Koss, Michael J.] ETH, Dept Phys, Inst Astron, CH-8093 Zurich, Switzerland. [Puccetti, Simonetta] ASDC ASI, I-00133 Rome, Italy. [Puccetti, Simonetta] Osserv Astron Roma, INAF, I-00040 Monte Porzio Catone, RM, Italy. [Gandhi, Poshak] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. [Alexander, David M.; Del Moro, Agnese] Univ Durham, Dept Phys, Durham DH1 3LE, England. [Boggs, Steve E.; Craig, William W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Brandt, William N.; Luo, Bin] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Brandt, William N.] Penn State Univ, Inst Gravitat & Cosmos, University Pk, PA 16802 USA. [Christensen, Finn E.] Tech Univ Denmark, Natl Space Inst, DTU Space, DK-2800 Lyngby, Denmark. [Comastri, Andrea] Osservatorio Astron Bologna, INAF, I-40127 Bologna, Italy. [Craig, William W.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Hailey, Charles J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Hickox, Ryan] Dartmouth Coll, Dept Phys & Astron, Hanover, NH 03755 USA. [Markwardt, Craig B.; Rigby, Jane R.; Zhang, William W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Marinucci, Andrea; Matt, Giorgio] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Saez, Cristian] Univ Maryland, Dept Astron, College Pk, MD 20742 USA. [Treister, Ezequiel] Univ Concepcion, Dept Astron, Concepcion, Chile. [Urry, C. Megan] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Urry, C. Megan] Yale Univ, Yale Ctr Astron & Astrophys, New Haven, CT 06520 USA. RP Bauer, FE (reprint author), Pontificia Univ Catolica Chile, Inst Astrofis, Santiago 22, Chile. RI Brandt, William/N-2844-2015; Boggs, Steven/E-4170-2015; OI Brandt, William/0000-0002-0167-2453; Boggs, Steven/0000-0001-9567-4224; Puccetti, Simonetta/0000-0002-2734-7835; Comastri, Andrea/0000-0003-3451-9970 FU CONICYT-Chile Basal [CATA PFB-06/2007]; FONDECYT [1141218, 1140304, 1120061]; Anillo grant [ACT1101]; Project "Millennium Institute of Astrophysics (MAS)" - Iniciativa Cientifica Milenio del Ministerio de Economia, Fomento y Turismo [IC120009]; Swiss National Science Foundation through the Ambizione fellowship [PZ00P2_154799/1]; NuSTAR NASA ADP [44A-1092750, NNX10AC99G]; ASI/INAF [I/037/12/0-011/13]; STFC [ST/J003697/1]; NASA [NNG08FD60C]; National Aeronautics and Space Administration FX We thank the anonymous referee for useful comments, which improved the clarity of the paper. We acknowledge financial support from the following: CONICYT-Chile Basal-CATA PFB-06/2007 (FEB, ET), FONDECYT grants 1141218 (FEB), 1140304 (PA), 1120061 (ET), and Anillo grant ACT1101 (FEB, PA, ET); Project IC120009 "Millennium Institute of Astrophysics (MAS)" funded by the Iniciativa Cientifica Milenio del Ministerio de Economia, Fomento y Turismo (FEB); Swiss National Science Foundation through the Ambizione fellowship grant PZ00P2_154799/1 (MK); NuSTAR subcontract 44A-1092750 NASA ADP grant NNX10AC99G (WNB, BL); ASI/INAF grant I/037/12/0-011/13 (SP, AC, AM and GM); and STFC grant ST/J003697/1 (PG). This work was supported under NASA Contract No. NNG08FD60C, and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). This research has made use of data obtained through the High Energy Astrophysics Science Archive Research Center (HEASARC) Online Service, provided by the NASA/Goddard Space Flight Center. NR 120 TC 20 Z9 20 U1 1 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD OCT 20 PY 2015 VL 812 IS 2 AR 116 DI 10.1088/0004-637X/812/2/116 PG 24 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CW7VD UT WOS:000365206600028 ER PT J AU Becerra, L Cipolletta, F Fryer, CL Rueda, JA Ruffini, R AF Becerra, L. Cipolletta, F. Fryer, Chris L. Rueda, Jorge A. Ruffini, Remo TI ANGULAR MOMENTUM ROLE IN THE HYPERCRITICAL ACCRETION OF BINARY-DRIVEN HYPERNOVAE SO ASTROPHYSICAL JOURNAL LA English DT Article DE gamma-ray burst: general ID INDUCED GRAVITATIONAL COLLAPSE; NEUTRON-STAR; MASSIVE STARS; CENTAURUS X-3; BLACK-HOLE; RAY; SUPERNOVA; MATTER; EVOLUTION; FALLBACK AB The induced gravitational collapse paradigm explains a class of energetic, E-iso greater than or similar to 10(52) erg, long-duration gammaray bursts (GRBs) associated with Ic supernovae, recently named binary-driven hypernovae. The progenitor is a tight binary system formed of a carbon-oxygen (CO) core and a neutron star (NS) companion. The supernova ejecta of the exploding CO core trigger a hypercritical accretion process onto the NS, which reaches the critical mass in a few seconds, and gravitationally collapses to a black hole, emitting a GRB. In our previous simulations of this process, we adopted a spherically symmetric approximation to compute the features of the hypercritical accretion process. We here present the first estimates of the angular momentum transported by the supernova ejecta, L-acc, and perform numerical simulations of the angular momentum transfer to the NS during the hyperaccretion process in full general relativity. We show that the NS (1) reaches either the mass-shedding limit or the secular axisymmetric instability in a few seconds depending on its initial mass, (2) reaches a maximum dimensionless angular momentum value, [cJ/(GM(2))](max) approximate to 0.7 (3) max, and (3) can support less angular momentum than the one transported by supernova ejecta, L-acc > J(NS,max), hence there is an angular momentum excess that necessarily leads to jetted emission. C1 [Becerra, L.; Cipolletta, F.; Rueda, Jorge A.; Ruffini, Remo] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Becerra, L.; Cipolletta, F.; Rueda, Jorge A.; Ruffini, Remo] Univ Roma La Sapienza, ICRA, I-00185 Rome, Italy. [Becerra, L.; Cipolletta, F.; Rueda, Jorge A.; Ruffini, Remo] ICRANet, I-65122 Pescara, Italy. [Fryer, Chris L.] Los Alamos Natl Lab, CCS 2, Los Alamos, NM 87545 USA. [Rueda, Jorge A.; Ruffini, Remo] Ctr Brasileiro Pesquisas Fis, ICRANet Rio, BR-22290180 Rio De Janeiro, Brazil. RP Becerra, L (reprint author), Univ Roma La Sapienza, Dipartimento Fis, Ple Aldo Moro 5, I-00185 Rome, Italy. OI Cipolletta, Federico/0000-0001-7894-1028 FU International Cooperation Program CAPES-ICRANet - CAPES; Brazilian Federal Agency; Evaluation of Graduate Education within the Ministry of Education of Brazil FX J.A.R. acknowledges the support by the International Cooperation Program CAPES-ICRANet financed by CAPES, Brazilian Federal Agency for Support and Evaluation of Graduate Education within the Ministry of Education of Brazil. NR 38 TC 5 Z9 5 U1 1 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD OCT 20 PY 2015 VL 812 IS 2 AR 100 DI 10.1088/0004-637X/812/2/100 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CW7VD UT WOS:000365206600012 ER PT J AU Bourgalais, J Capron, M Kailasanathan, RKA Osborn, DL Hickson, KM Loison, JC Wakelam, V Goulay, F Le Picard, SD AF Bourgalais, Jeremy Capron, Michael Kailasanathan, Ranjith Kumar Abhinavam Osborn, David L. Hickson, Kevin M. Loison, Jean-Christophe Wakelam, Valentine Goulay, Fabien Le Picard, Sebastien D. TI THE C(P-3) + NH3 REACTION IN INTERSTELLAR CHEMISTRY. I. INVESTIGATION OF THE PRODUCT FORMATION CHANNELS SO ASTROPHYSICAL JOURNAL LA English DT Article DE astrochemistry; ISM: atoms; ISM: clouds; ISM: molecules; molecular data; molecular processes ID ELECTRONIC-STRUCTURE THEORY; DENSE INTERSTELLAR CLOUDS; NEUTRAL-NEUTRAL REACTIONS; VACUUM ULTRA-VIOLET; RANGE 24-300 K; ATOMIC CARBON; RATE COEFFICIENTS; RATE-CONSTANT; DARK CLOUDS; AB-INITIO AB The product formation channels of ground state carbon atoms, C(P-3), reacting with ammonia, NH3, have been investigated using two complementary experiments and electronic structure calculations. Reaction products are detected in a gas flow tube experiment (330 K, 4 Torr) using tunable vacuum-ultraviolet (VUV) photoionization coupled with time of flight mass spectrometry. Temporal profiles of the species formed and photoionization spectra are used to identify primary products of the C + NH3 reaction. In addition, H-atom formation is monitored by VUV laser induced fluorescence (LIF) from room temperature to 50 K in a supersonic gas flow generated by the Laval nozzle technique. Electronic structure calculations are performed to derive intermediates, transition states, and complexes formed along the reaction coordinate. The combination of photoionization and LIF experiments supported by theoretical calculations indicate that in the temperature and pressure range investigated, the H + H2CN production channel represents 100% of the product yield for this reaction. Kinetics measurements of the title reaction down to 50 K and the effect of the new rate constants on interstellar nitrogen hydride abundances using a model of dense interstellar clouds are reported in Paper II. C1 [Bourgalais, Jeremy; Capron, Michael; Le Picard, Sebastien D.] Univ Rennes 1, UMR CNRS 6251, Inst Phys Rennes, Astrophys Lab, F-35042 Rennes, France. [Kailasanathan, Ranjith Kumar Abhinavam; Goulay, Fabien] W Virginia Univ, Dept Chem, Morgantown, WV 26506 USA. [Osborn, David L.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. [Hickson, Kevin M.; Loison, Jean-Christophe] Univ Bordeaux, Inst Sci Mol, UMR 5255, F-33400 Talence, France. [Hickson, Kevin M.; Loison, Jean-Christophe] CNRS, Inst Sci Mol, UMR 5255, F-33400 Talence, France. [Wakelam, Valentine] Univ Bordeaux, LAB, UMR 5804, F-33270 Floirac, France. [Wakelam, Valentine] CNRS, LAB, UMR 5804, F-33270 Floirac, France. RP Bourgalais, J (reprint author), Univ Rennes 1, UMR CNRS 6251, Inst Phys Rennes, Astrophys Lab, Bat 11C,Campus Beaulieu, F-35042 Rennes, France. EM jean-christophe.loison@u-bordeaux.fr; fabien.goulay@mail.wvu.edu; sebastien.lepicard@univ-rennes1.fr RI Dep. Molecular Physics, Team/B-5839-2016; OI Le Picard, Sebastien/0000-0002-3753-4431 FU Agence Nationale de la Recherche [ANR-11-BS04-024-CRESUSOL-01]; French INSU/CNRS Program "Physique et Chimie du Milieu Interstellaire" (PCMI); Institut National de Physique (INP CNRS); Rgion Bretagne; Universite de Rennes 1; Institut Universitaire de France; American Chemical Society Petroleum Research Fund (PRF) [53105-DN16]; French INSU/CNRS Program PCMI; French INSU/CNRS Program PNP; Division of Chemical Sciences, Geosciences, and Biosciences, the Office of Basic Energy Sciences, the U.S. Department of Energy; Sandia Corporation, a Lockheed Martin Company [DE-AC04-94-AL85000]; ERC Starting Grant 3DICE [336474]; Direct, Office of Science, Office of Basic Energy Sciences; U.S. Department of Energy [DE-AC02-05CH11231] FX The Rennes team acknowledges support from the Agence Nationale de la Recherche, contract ANR-11-BS04-024-CRESUSOL-01, the French INSU/CNRS Program "Physique et Chimie du Milieu Interstellaire" (PCMI), the Institut National de Physique (INP CNRS), the Rgion Bretagne and the Universite de Rennes 1. S.D.L.P. acknowledges financial support from the Institut Universitaire de France. F.G. and R.K.A.K. acknowledge founding by the West Virginia University (startup package) for supply and travel support. Acknowledgement is also made to the Donors of the American Chemical Society Petroleum Research Fund for partial support of this research (PRF#53105-DN16 for R.K.A.K. postdoctoral support). J.C.L. and K.M.H. acknowledge support from the French INSU/CNRS Programs PCMI and PNP. We thank Mr. Howard Johnsen and Dr. John Savee for technical support of this experiment. We also thank Dr. Doug Taube for his help and advice during the carbon suboxide synthesis. D.L.O. and the instrumentation for this work are supported by the Division of Chemical Sciences, Geosciences, and Biosciences, the Office of Basic Energy Sciences, the U.S. Department of Energy. Sandia is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the National Nuclear Security Administration under contract DE-AC04-94-AL85000. V.W. research is supported by the ERC Starting Grant 3DICE (grant agreement 336474) and the the French INSU/CNRS Program "Physique et Chimie du Milieu Interstellaire" (PCMI). This research used resources of the Advanced Light Source, a DOE Office of Science User Facility, which is supported by the Direct, Office of Science, Office of Basic Energy Sciences, the U.S. Department of Energy under contract DE-AC02-05CH11231 at Lawrence Berkeley National Laboratory. NR 89 TC 4 Z9 4 U1 1 U2 12 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD OCT 20 PY 2015 VL 812 IS 2 AR 106 DI 10.1088/0004-637X/812/2/106 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CW7VD UT WOS:000365206600018 ER PT J AU Buenzli, E Marley, MS Apai, D Saumon, D Biller, BA Crossfield, IJM Radigan, J AF Buenzli, Esther Marley, Mark. S. Apai, Daniel Saumon, Didier Biller, Beth A. Crossfield, Ian J. M. Radigan, Jacqueline TI CLOUD STRUCTURE OF THE NEAREST BROWN DWARFS. II. HIGH-AMPLITUDE VARIABILITY FOR LUHMAN 16 A AND B IN AND OUT OF THE 0.99 mu m FeH FEATURE SO ASTROPHYSICAL JOURNAL LA English DT Article DE binaries: visual; brown dwarfs; stars: atmospheres; stars: individual (WISE J104915.57-531906.1, Luhman 16AB); stars: variables: general ID HUBBLE-SPACE-TELESCOPE; FLUX-REVERSAL BINARY; T-DWARFS; L/T TRANSITION; 2 PC; WISE J104915.57-531906.1AB; SPECTROSCOPIC VARIABILITY; EVOLVING WEATHER; TEMPERATURE; GRAVITY AB The re-emergence of the 0.99 mu m FeH feature in brown dwarfs of early-to mid-T spectral type has been suggested as evidence for cloud disruption where flux from deep, hot regions below the Fe cloud deck can emerge. The same mechanism could account for color changes at the L/T transition and photometric variability. We present the first observations of spectroscopic variability of brown dwarfs covering the 0.99 mu m FeH feature. We observed the spatially resolved very nearby brown dwarf binary WISE J104915.57-531906.1 (Luhman 16AB), a late-L and early-T dwarf, with Hubble Space Telescope/WFC3 in the G102 grism at 0.8-1.15 mu m. We find significant variability at all wavelengths for both brown dwarfs, with peak-to-valley amplitudes of 9.3% for Luhman 16B and 4.5% for Luhman 16A. This represents the first unambiguous detection of variability in Luhman 16A. We estimate a rotational period between 4.5 and 5.5 hr, very similar to Luhman 16B. Variability in both components complicates the interpretation of spatially unresolved observations. The probability for finding large amplitude variability in any two brown dwarfs is less than 10%. Our finding may suggest that a common but yet unknown feature of the binary is important for the occurrence of variability. For both objects, the amplitude is nearly constant at all wavelengths except in the deep K I feature below 0.84 mu m. No variations are seen across the 0.99 mu m FeH feature. The observations lend strong further support to cloud height variations rather than holes in the silicate clouds, but cannot fully rule out holes in the iron clouds. We re-evaluate the diagnostic potential of the FeH feature as a tracer of cloud patchiness. C1 [Buenzli, Esther] Max Planck Inst Astron, D-69117 Heidelberg, Germany. [Marley, Mark. S.] NASA, Ames Res Ctr, Moffett Field, CA 94035 USA. [Apai, Daniel] Univ Arizona, Dept Astron, Tucson, AZ 85721 USA. [Apai, Daniel; Crossfield, Ian J. M.] Univ Arizona, Dept Planetary Sci, Tucson, AZ 85721 USA. [Saumon, Didier] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Biller, Beth A.] Univ Edinburgh, Inst Astron, Edinburgh EH9 3HJ, Midlothian, Scotland. [Radigan, Jacqueline] Space Telescope Sci Inst, Baltimore, MD 21218 USA. RP Buenzli, E (reprint author), Max Planck Inst Astron, Konigstuhl 17, D-69117 Heidelberg, Germany. EM buenzli@mpia.de OI Buenzli, Esther/0000-0003-3306-1486 FU Swiss National Science Foundation (SNSF); NASA [NAS 5-26555]; NASA through a grant from the Space Telescope Science Institute [13640] FX We thank the anonymous referee for a helpful report. We thank the staff at the Space Telescope Science Institute (STScI), in particular Amber Armstrong, for the scheduling of the observations. We thank Adam Burgasser, Alexei Kniazev, and Jackie Faherty for providing their published spectra of Luhman 16AB in electronic form. E.B. was supported by the Swiss National Science Foundation (SNSF). Based on observations made with the NASA/ESA Hubble Space Telescope, obtained at the Space Telescope Science Institute, which is operated by the Association of Universities for Research in Astronomy, Inc., under NASA contract NAS 5-26555. These observations are associated with program 13640. Support for program 13640 was provided by NASA through a grant from the Space Telescope Science Institute. This research has made use of the SIMBAD database, operated at CDS, Strasbourg, France, and of NASA's Astrophysics Data System Bibliographic Services. NR 38 TC 5 Z9 5 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD OCT 20 PY 2015 VL 812 IS 2 AR 163 DI 10.1088/0004-637X/812/2/163 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CW7VD UT WOS:000365206600075 ER PT J AU Materese, CK Cruikshank, DP Sandford, SA Imanaka, H Nuevo, M AF Materese, Christopher K. Cruikshank, Dale P. Sandford, Scott A. Imanaka, Hiroshi Nuevo, Michel TI ICE CHEMISTRY ON OUTER SOLAR SYSTEM BODIES: ELECTRON RADIOLYSIS OF N-2-, CH4-, AND CO-CONTAINING ICES SO ASTROPHYSICAL JOURNAL LA English DT Article DE astrochemistry; Kuiper Belt: general; molecular data; molecular processes; planets and satellites: surfaces; solid state: refractory ID HYDROGEN-CYANIDE POLYMERS; ADVANCED LIGHT-SOURCE; BUTYLDIMETHYLSILYL DERIVATIVES; INFRARED-SPECTROSCOPY; SOLID NITROGEN; UV PHOTOLYSIS; ULTRAVIOLET; ANALOGS; TRANSMISSION; IRRADIATION AB Radiation processing of the surface ices of outer Solar System bodies may be an important process for the production of complex chemical species. The refractory materials resulting from radiation processing of known ices are thought to impart to them a red or brown color, as perceived in the visible spectral region. In this work, we analyzed the refractory materials produced from the 1.2-keV electron bombardment of low-temperature N-2-, CH4-, and CO-containing ices (100:1:1), which simulates the radiation from the secondary electrons produced by cosmic ray bombardment of the surface ices of Pluto. Despite starting with extremely simple ices dominated by N-2, electron irradiation processing results in the production of refractory material with complex oxygen-and nitrogen-bearing organic molecules. These refractory materials were studied at room temperature using multiple analytical techniques including Fourier-transform infrared spectroscopy, X-ray absorption near-edge structure (XANES) spectroscopy, and gas chromatography coupled with mass spectrometry (GC-MS). Infrared spectra of the refractory material suggest the presence of alcohols, carboxylic acids, ketones, aldehydes, amines, and nitriles. XANES spectra of the material indicate the presence of carboxyl groups, amides, urea, and nitriles, and are thus consistent with the IR data. Atomic abundance ratios for the bulk composition of these residues from XANES analysis show that the organic residues are extremely N-rich, having ratios of N/C similar to 0.9 and O/C similar to 0.2. Finally, GC-MS data reveal that the residues contain urea as well as numerous carboxylic acids, some of which are of interest for prebiotic and biological chemistries. C1 [Materese, Christopher K.; Cruikshank, Dale P.; Sandford, Scott A.; Imanaka, Hiroshi; Nuevo, Michel] NASA, Ames Res Ctr, Moffett Field, CA 94035 USA. [Materese, Christopher K.] Oak Ridge Associated Univ, Oak Ridge, TN 37831 USA. [Imanaka, Hiroshi] SETI Inst, Mountain View, CA 94043 USA. [Nuevo, Michel] Bay Area Environm Res Inst, Petaluma, CA 94952 USA. RP Materese, CK (reprint author), NASA, Ames Res Ctr, MS 245-6, Moffett Field, CA 94035 USA. OI Materese, Christopher/0000-0003-2146-4288 FU NASA's New Horizons mission program; NASA's Cassini Data Analysis Program; National Aeronautics and Space Administration through the NASA Astrobiology Institute [NNH13ZDA017C]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX C.K.M. acknowledges R.L. Walker (NASA Ames) for technical support, the NASA Postdoctoral Program (NPP) administered by ORAU, and D. Kilcoyne for assistance with ALS beamline 5.3.2.2. D.P.C. acknowledges support from NASA's New Horizons mission program. H.I. acknowledges supports from NASA's Cassini Data Analysis Program. This material is based on work supported by the National Aeronautics and Space Administration through the NASA Astrobiology Institute under Cooperative Agreement Notice NNH13ZDA017C issued through the Science Mission Directorate. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Finally, we also would like to thank an anonymous reviewer for their comments. NR 41 TC 6 Z9 6 U1 0 U2 7 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD OCT 20 PY 2015 VL 812 IS 2 AR 150 DI 10.1088/0004-637X/812/2/150 PG 9 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CW7VD UT WOS:000365206600062 ER PT J AU Mir, A Chen, J Robinson, K Lendy, E Goodman, J Neau, D Golden, BL AF Mir, Aamir Chen, Ji Robinson, Kyle Lendy, Emma Goodman, Jaclyn Neau, David Golden, Barbara L. TI Two Divalent Metal Ions and Conformational Changes Play Roles in the Hammerhead Ribozyme Cleavage Reaction SO BIOCHEMISTRY LA English DT Article ID ACID-BASE CATALYSIS; DELTA VIRUS RIBOZYME; HDV GENOMIC RIBOZYME; ACTIVE-SITE; HAIRPIN RIBOZYME; MECHANISTIC CHARACTERIZATION; MONOVALENT CATIONS; CRYSTAL-STRUCTURE; SELF-CLEAVAGE; BINDING AB The hammerhead ribozyme is a self-cleaving RNA broadly dispersed across all kingdoms of life. Although it was the first of the small, nudeolytic ribozymes discovered, the mechanism by which it catalyzes its reaction remains elusive. The nudeobase of G12 is well positioned to be a general base, but it is unclear if or how this guanine base becomes activated for proton transfer. Metal ions have been implicated in the chemical mechanism, but no interactions between divalent metal ions and the cleavage site have been observed crystallographically. To better understand how this ribozyme functions, we have solved crystal structures of wild-type and G12A mutant ribozymes. We observe a pH-dependent conformational change centered around G12, consistent with this nucleotide becoming deprotonated. Crystallographic and kinetic analysis of the G12A mutant reveals a Zn2+ specificity switch suggesting a direct interaction between a divalent metal ion and the purine at position 12. The metal ion specificity switch and the pH rate profile of the G12A mutant suggest that the minor imino tautomer of A12 serves as the general base in the mutant ribozyme. We propose a model in which the hammerhead ribozyme rearranges prior to the cleavage reaction, positioning two divalent metal ions in the process. The first metal ion, positioned near G12, becomes directly coordinated to the 06 keto oxygen, to lower the pK(a) of the general base and organize the active site. The second metal ion, positioned near G10.1, bridges the N7 of G10.1 and the scissile phosphate and may participate directly in the cleavage reaction. C1 [Mir, Aamir; Chen, Ji; Robinson, Kyle; Lendy, Emma; Goodman, Jaclyn; Golden, Barbara L.] Purdue Univ, Dept Biochem, W Lafayette, IN 47907 USA. [Neau, David] Cornell Univ, Dept Chem & Chem Biol, Northeastern Collaborat Access Team, Argonne Natl Lab, Argonne, IL 60439 USA. RP Golden, BL (reprint author), Purdue Univ, Dept Biochem, W Lafayette, IN 47907 USA. EM barbgolden@purdue.edu FU National Institutes of Health [R01 GM095923, S10 OD012041]; Purdue University Department of Biochemistry; Markey Center for Structural Biology; Purdue University Center for Cancer Research; U.S. Department of Energy (DOE) Office of Science User Facility [DE-AC02-06CH11357]; NIH [P41 GM103403]; NIH-ORIP HEI grant [S10 RR029205]; Michigan Technology Tri-Corridor [085P1000817]; Michigan Economic Development Corporation FX This project was supported by National Institutes of Health Grant R01 GM095923 and S10 OD012041, the Purdue University Department of Biochemistry, the Markey Center for Structural Biology, and the Purdue University Center for Cancer Research. This research used resources of the Advanced Photon Source (a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357), the NE-CAT beamlines [funded by NIH (P41 GM103403)], the Pilatus 6M detector on 24-ID-C beamline [funded by a NIH-ORIP HEI grant (S10 RR029205)] and the LS-CAT Sector 21 beamlines [supported by the Michigan Economic Development Corporation and the Michigan Technology Tri-Corridor (Grant 085P1000817)]. NR 66 TC 7 Z9 7 U1 1 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD OCT 20 PY 2015 VL 54 IS 41 BP 6369 EP 6381 DI 10.1021/acs.biochem.5b00824 PG 13 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CU2IQ UT WOS:000363347600010 PM 26398724 ER PT J AU Leng, XL Kinnun, JJ Marquardt, D Ghefli, M Kucerka, N Katsaras, J Atkinson, J Harroun, TA Feller, SE Wassall, SR AF Leng, Xiaoling Kinnun, Jacob J. Marquardt, Drew Ghefli, Mikel Kucerka, Norbert Katsaras, John Atkinson, Jeffrey Harroun, Thad A. Feller, Scott E. Wassall, Stephen R. TI alpha-Tocopherol Is Well Designed to Protect Polyunsaturated Phospholipids: MD Simulations SO BIOPHYSICAL JOURNAL LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; MAGNETIC-RESONANCE SPECTROSCOPY; LOW-DENSITY-LIPOPROTEIN; STATE H-2 NMR; VITAMIN-E; FATTY-ACIDS; LIPID-BILAYERS; DOCOSAHEXAENOIC ACID; FLIP-FLOP; MEMBRANE-PROPERTIES AB The presumptive function for alpha-tocopherol (alpha toc) in membranes is to protect polyunsaturated lipids against oxidation. Although the chemistry of the process is well established, the role played by molecular structure that we address here with atomistic molecular-dynamics simulations remains controversial. The simulations were run in the constant particle NPT ensemble on hydrated lipid bilayers composed of SDPC (1-stearoyl-2-docosahexaenoylphosphatidylcholine, 18:0-22:6PC) and SOPC (1-stearoyl-2-oleoylphosphatidylcholine, 18:0-18:1 PC) in the presence of 20 mol % alpha toc at 37 degrees C. SDPC with SA (stearic acid) for the sn-1 chain and DHA (docosahexaenoic acid) for the sn-2 chain is representative of polyunsaturated phospholipids, while SOPC with OA (oleic acid) substituted for the sn-2 chain serves as a monounsaturated control. Solid-state H-2 nuclear magnetic resonance and neutron diffraction experiments provide validation. The simulations demonstrate that high disorder enhances the probability that DHA chains at the sn-2 position in SDPC rise up to the bilayer surface, whereby they encounter the chromanol group on alpha toc molecules. This behavior is reflected in the van der Waals energy of interaction between alpha toc and acyl chains, and illustrated by density maps of distribution for acyl chains around alpha toc molecules that were constructed. An ability to more easily penetrate deep into the bilayer is another attribute conferred upon the chromanol group in alpha toc by the high disorder possessed by DHA. By examining the trajectory of single molecules, we found that alpha toc flip-flops across the SDPC bilayer on a submicrosecond timescale that is an order-of-magnitude greater than in SOPC. Our results reveal mechanisms by which the sacrificial hydroxyl group on the chromanol group can trap lipid peroxyl radicals within the interior and near the surface of a polyunsaturated membrane. At the same time, water-soluble reducing agents that regenerate alpha toc can access the chromanol group when it locates at the surface. C1 [Leng, Xiaoling; Kinnun, Jacob J.; Wassall, Stephen R.] Indiana Univ Purdue Univ, Dept Phys, Indianapolis, IN 46205 USA. [Marquardt, Drew; Harroun, Thad A.] Brock Univ, Dept Phys, St Catharines, ON L2S 3A1, Canada. [Marquardt, Drew] Graz Univ, Inst Mol Biosci, Graz, Austria. [Ghefli, Mikel; Atkinson, Jeffrey] Brock Univ, Dept Chem, St Catharines, ON L2S 3A1, Canada. [Kucerka, Norbert] CNR, Canadian Neutron Beam Ctr, Chalk River, ON, Canada. [Kucerka, Norbert] Comenius Univ, Fac Pharm, Bratislava, Slovakia. [Katsaras, John] Oak Ridge Natl Lab, Neutron Sci Directorate, Oak Ridge, TN USA. [Katsaras, John] Joint Inst Neutron Sci, Oak Ridge, TN USA. [Katsaras, John] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Feller, Scott E.] Wabash Coll, Dept Chem, Crawfordsville, IN 47933 USA. RP Wassall, SR (reprint author), Indiana Univ Purdue Univ, Dept Phys, Indianapolis, IN 46205 USA. EM swassall@iupui.edu OI Harroun, Thad/0000-0001-9816-2590 NR 81 TC 5 Z9 5 U1 4 U2 12 PU CELL PRESS PI CAMBRIDGE PA 50 HAMPSHIRE ST, FLOOR 5, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD OCT 20 PY 2015 VL 109 IS 8 BP 1608 EP 1618 DI 10.1016/j.bpj.2015.08.032 PG 11 WC Biophysics SC Biophysics GA CU2NU UT WOS:000363361000014 PM 26488652 ER PT J AU Neale, C Herce, HD Pomes, R Garcia, AE AF Neale, Chris Herce, Henry D. Pomes, Regis Garcia, Angel E. TI Can Specific Protein-Lipid Interactions Stabilize an Active State of the Beta 2 Adrenergic Receptor? SO BIOPHYSICAL JOURNAL LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; BETA-ADRENERGIC-RECEPTOR; NONLAMELLAR-FORMING LIPIDS; PARTICLE MESH EWALD; COUPLED RECEPTOR; BETA(2)-ADRENERGIC RECEPTOR; CRYSTAL-STRUCTURE; FORCE-FIELD; MEMBRANE-PROTEINS; PLASMA-MEMBRANE AB G-protein-coupled receptors are eukaryotic membrane proteins with broad biological and pharmacological relevance. Like all membrane-embedded proteins, their location and orientation are influenced by lipids, which can also impact protein function via specific interactions. Extensive simulations totaling 0.25 ms reveal a process in which phospholipids from the membrane's cytosolic leaflet enter the empty G-protein binding site of an activated (32 adrenergic receptor and form salt-bridge interactions that inhibit ionic lock formation and prolong active-state residency. Simulations of the receptor embedded in an anionic membrane show increased lipid binding, providing a molecular mechanism for the experimental observation that anionic lipids can enhance receptor activity. Conservation of the arginine component of the ionic lock among Rhodopsin-like G-protein-coupled receptors suggests that intracellular lipid ingression between receptor helices H6 and H7 may be a general mechanism for active-state stabilization. C1 [Neale, Chris; Herce, Henry D.; Garcia, Angel E.] Rensselaer Polytech Inst, Dept Phys Appl Phys & Astron, Troy, NY USA. [Pomes, Regis] Hosp Sick Children, Mol Struct & Funct, Toronto, ON M5G 1X8, Canada. [Pomes, Regis] Univ Toronto, Dept Biochem, Toronto, ON, Canada. [Garcia, Angel E.] Rensselaer Polytech Inst, Ctr Biotechnol & Interdisciplinary Studies, Troy, NY USA. RP Garcia, AE (reprint author), Los Alamos Natl Lab, CNLS MSB258, Los Alamos, NM 87545 USA. EM agarcia@lanl.gov FU Canadian Institutes of Health Research [MOP-43998] NR 128 TC 10 Z9 10 U1 7 U2 21 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD OCT 20 PY 2015 VL 109 IS 8 BP 1652 EP 1662 DI 10.1016/j.bpj.2015.08.028 PG 11 WC Biophysics SC Biophysics GA CU2NU UT WOS:000363361000018 PM 26488656 ER PT J AU Abreu-Sepulveda, M Trinh, P Malkhandi, S Narayanan, SR Jorne, J Quesnel, DJ Postonr, JA Manivannan, A AF Abreu-Sepulveda, Maria Trinh, Phong Malkhandi, S. Narayanan, S. R. Jorne, Jacob Quesnel, David J. Postonr, James A., Jr. Manivannan, A. TI Investigation of Oxygen Evolution Reaction at LaRuO3, La3.5Ru4O13, and La2RuO5 SO ELECTROCHIMICA ACTA LA English DT Article DE water electrolyzer; oxygen evolution; noble transition metal perovskites ID METAL-AIR BATTERIES; LI-O-2 BATTERIES; LI2O2 OXIDATION; PEROVSKITE; RUTHENIUM; CATALYSTS; OXIDE; ELECTRODES; REDUCTION; ELECTROCATALYSTS AB Development of electrocatalysts is important for reducing the voltage loss due to the oxygen evolution reaction (OER) in metal-air batteries and water electrolyzers. In the present work, the electrocatalytic activity towards oxygen evolution for a series of lanthanum-ruthenium compounds has been investigated by steady-state current-potential measurements in alkaline media to understand the effect of structure, valence state of the transition metal ion, and the role of surface adsorbed hydroxyl species. Compounds of the perovskite family, LaRuO3, La3.5Ru4O13, and La2RuO5, were prepared by the Pechini process and calcined at different temperatures to obtain the desired phases. X-ray photoelectron spectroscopy of LaRuO3 and La2RuO5 showed shifts of the Ru-3d peaks towards higher binding energies indicative of a highly oxidized surface with possibly high surface hydroxylation. The electrochemical activity of the compounds at 0.8 V vs. NHE was in the order of 10(-6)A/cm(2) and the mass specific activity was about 80 mA/g. Tafel slopes were in the vicinity of 60 mV/decade for LaRuO3 (orthorhombic) and La3.5Ru4O13 (orthorhombic), and about 80 mV/decade for La2RuO5 (monoclinic). In addition FT-IR results indicate high surface coverage by hydroxide species. The reaction order with respect to OH- ions was found to be lower than unity. It is possible that strong interaction of hydroxide groups with ruthenium at the surface of the electrode makes it difficult to dissociate the Ru-OH bond and prevent further interaction with dissolved OH- even at high overpotentials. Published by Elsevier Ltd. C1 [Abreu-Sepulveda, Maria; Jorne, Jacob; Quesnel, David J.] Univ Rochester, Rochester, NY 14627 USA. [Trinh, Phong; Malkhandi, S.; Narayanan, S. R.] Univ So Calif, Los Angeles, CA USA. [Postonr, James A., Jr.; Manivannan, A.] US DOE, NETL, Morgantown, WV 26507 USA. [Manivannan, A.] W Virginia Univ, Mech & Aerosp Engn, Morgantown, WV 26507 USA. RP Manivannan, A (reprint author), US DOE, NETL, Morgantown, WV 26507 USA. EM amanivan@wvu.edu RI Malkhandi, Souradip/C-3582-2009 OI Malkhandi, Souradip/0000-0003-0826-3078 FU NSF-IGERT [DGE-0966089]; University of Rochester, NY; US DOE/ORISE fellowship; US DOE/NETL, Morgantown, WV FX This research has been supported by the NSF-IGERT DGE-0966089, University of Rochester, NY and by the US DOE/ORISE fellowship, US DOE/NETL, Morgantown, WV. Dr. Sungsik Lee at the APS facility in the Argonne National Lab is acknowledged for his assistance with the XANES measurements. NR 29 TC 2 Z9 2 U1 16 U2 63 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD OCT 20 PY 2015 VL 180 BP 401 EP 408 DI 10.1016/j.electacta.2015.08.067 PG 8 WC Electrochemistry SC Electrochemistry GA CU2HR UT WOS:000363345100048 ER PT J AU Dilmore, RM Sams, JI Glosser, D Carter, KM Bain, DJ AF Dilmore, Robert M. Sams, James I., III Glosser, Deborah Carter, Kristin M. Bain, Daniel J. TI Spatial and Temporal Characteristics of Historical Oil and Gas Wells in Pennsylvania: Implications for New Shale Gas Resources SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID DRINKING-WATER WELLS; METHANE EMISSIONS; WELLBORE LEAKAGE; UNITED-STATES; RISK; CO2; MARCELLUS; SITE; CONTAMINATION; INTEGRITY AB Recent large-scale development of oil and gas from low-permeability unconventional formations (e.g., shales, tight sands, and coal seams) has raised concern about potential environmental impacts. If left improperly sealed, legacy oil and gas wells colocated with that new development represent a potential pathway for unwanted migration of fluids (brine, drilling and stimulation fluids, oil, and gas). Uncertainty in the number, location, and abandonment state of legacy wells hinders environmental assessment of exploration and production activity. The objective of this study is to apply publicly available information on Pennsylvania oil and gas wells to better understand their potential to serve as pathways for unwanted fluid migration. This study presents a synthesis of historical reports and digital well records to provide insights into spatial and temporal trends in oil and gas development. Areas with a higher density of wells abandoned prior to the mid-20th century, when more modem well-sealing requirements took effect in Pennsylvania, and areas where conventional oil and gas production penetrated to or through intervals that may be affected by new Marcellus shale development are identified. This information may help to address questions of environmental risk related to new extraction activities. C1 [Dilmore, Robert M.; Sams, James I., III; Glosser, Deborah] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. [Glosser, Deborah] Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37831 USA. [Carter, Kristin M.] Penn Dept Conservat & Nat Resources, Bur Topog & Geol Survey, Econ Geol Div, Pittsburgh, PA 15222 USA. [Bain, Daniel J.] Univ Pittsburgh, Dept Geol & Planetary Sci, Pittsburgh, PA 15260 USA. RP Dilmore, RM (reprint author), US DOE, Natl Energy Technol Lab, 626 Cochrans Mill Rd,POB 10940, Pittsburgh, PA 15236 USA. EM Robert.Dilmore@NETL.DOE.GOV FU URS Corporation FX This work was performed, in part, under a subcontract to the University of Pittsburgh, from URS Corporation. We also wish to acknowledge the contributions and technical guidance of Richard Hammack, Kelly Rose, Jennifer Bauer, Tim Murin, George Guthrie, Ale Hakala, and others in the Pennsylvania Department of Conservation and Natural Resources and the United States Department of Energy's Strategic Center for Natural Gas and Oil. NR 48 TC 1 Z9 1 U1 5 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD OCT 20 PY 2015 VL 49 IS 20 BP 12015 EP 12023 DI 10.1021/acs.est.5b00820 PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CU2JB UT WOS:000363348700004 PM 26267137 ER PT J AU Singh, R Yoon, H Sanford, RA Katz, L Fouke, BW Werth, CJ AF Singh, Rajveer Yoon, Hongkyu Sanford, Robert A. Katz, Lynn Fouke, Bruce W. Werth, Charles J. TI Metabolism-Induced CaCO3 Biomineralization During Reactive Transport in a Micromodel: Implications for Porosity Alteration SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID CALCIUM-CARBONATE PRECIPITATION; TRANSVERSE MIXING ZONE; PORE-SCALE; POROUS-MEDIA; IN-SITU; NITRITE ACCUMULATION; MINERAL FORMATION; BACTERIAL-GROWTH; WASTE-WATER; DENITRIFICATION AB The ability of Pseudomonas stutzeri strain DCP-Ps1 to drive CaCO3 biomineralization has been investigated in a microfluidic flowcell (i.e., micromodel) that simulates subsurface porous media. Results indicate that CaCO3 precipitation occurs during NO3- reduction with a maximum saturation index (SIcalcite) of similar to 1.56, but not when NO3- was removed, inactive biomass remained, and pH and alkalinity were adjusted to SIcalcite similar to 1.56. CaCO3 precipitation was promoted by metabolically active cultures of strain DCP-Ps1, which at similar values of SIcalcite, have a more negative surface charge than inactive strain DCP-Ps1. A two-stage NO3- reduction (NO3- -> NO2- -> N-2) pore-scale reactive transport model was used to evaluate denitrification kinetics, which was observed in the micromodel as upper (NO3- reduction) and lower (NO2- reduction) horizontal zones of biomass growth with CaCO3 precipitation exclusively in the lower zone. Model results are consistent with two biomass growth regions and indicate that precipitation occurred in the lower zone because the largest increase in pH and alkalinity is associated with NO2- reduction. CaCO3 precipitates typically occupied the entire vertical depth of pores and impacted porosity, permeability, and flow. This study provides a framework for incorporating microbial activity in biogeochemistry models, which often base biomineralization only on SI (caused by biotic or abiotic reactions) and, thereby, underpredict the extent of this complex process. These results have wide-ranging implications for understanding reactive transport in relevance to groundwater remediation, CO2 sequestration, and enhanced oil recovery. C1 [Singh, Rajveer] Univ Illinois, Civil & Environm Engn, Urbana, IL 61801 USA. [Singh, Rajveer; Sanford, Robert A.; Fouke, Bruce W.] Univ Illinois, Inst Genom Biol, Urbana, IL 61801 USA. [Sanford, Robert A.; Fouke, Bruce W.] Univ Illinois, Dept Geol, Urbana, IL 61801 USA. [Yoon, Hongkyu] Sandia Natl Labs, Geosci Res & Applicat, Albuquerque, NM 87185 USA. [Katz, Lynn; Werth, Charles J.] Univ Texas Austin, Civil Architectural & Environm Engn, Austin, TX 78712 USA. RP Singh, R (reprint author), Univ Illinois, Civil & Environm Engn, Urbana, IL 61801 USA. EM rajs@illinois.edu FU Energy Bioscience Institute at the University of Illinois Urbana-Champaign; Center for Frontiers of Subsurface Energy Security, an Energy Frontier Research Center (EFRC) - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001114]; U.S. DOE, Office of Science, BES [DE-SC0C12504]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors gratefully acknowledge funding for this research from the Energy Bioscience Institute at the University of Illinois Urbana-Champaign. We are thankful to I.T.G. at the Beckman Institute and CORE facilities at the IGB @ UIUC for their help with Raman, ESEM, EDS, and image analysis. H.Y. is supported as part of the Center for Frontiers of Subsurface Energy Security, an Energy Frontier Research Center (EFRC) funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award DE-SC0001114. Partial support (i.e., analyses of microbial surface charge and model simulation results) for C.J.W. and B.W.F. was provided as part of the Center for Geologic Storage of CO2, an EFRC funded by the U.S. DOE, Office of Science, BES, under Award DE-SC0C12504. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. The authors gratefully acknowledge valuable comments from two reviewers that resulted in a substantially improved manuscript. NR 86 TC 3 Z9 3 U1 8 U2 44 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD OCT 20 PY 2015 VL 49 IS 20 BP 12094 EP 12104 DI 10.1021/acs.est.5b00152 PG 11 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CU2JB UT WOS:000363348700013 PM 26348257 ER PT J AU Miller, CL Watson, DB Lester, BP Howe, JY Phillips, DH He, F Liang, LY Pierce, EM AF Miller, Carrie L. Watson, David B. Lester, Brian P. Howe, Jane Y. Phillips, Debra H. He, Feng Liang, Liyuan Pierce, Eric M. TI Formation of Soluble Mercury Oxide Coatings: Transformation of Elemental Mercury in Soils SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID AQUATIC ENVIRONMENTS; CONTAMINATED SOILS; CHEMICAL EXTRACTIONS; CATALYTIC-OXIDATION; MANGANESE OXIDES; MINAS-GERAIS; SPECIATION; SEDIMENTS; FRACTIONATION; CHROMIUM(III) AB The impact of mercury (Hg) on human and ecological health has been known for decades. Although a treaty signed in 2013 by 147 nations regulates future large-scale mercury emissions, legacy Hg contamination exists worldwide and small-scale releases will continue. The fate of elemental mercury, Hg(0), lost to the subsurface and its potential chemical transformation that can lead to changes in speciation and mobility are poorly understood. Here, we show that Hg(0) beads interact with soil or manganese oxide solids and X-ray spectroscopic analysis indicates that the soluble mercury coatings are HgO. Dissolution studies show that, after reacting with a composite soil, >20 times more Hg is released into water from the coated beads than from a pure liquid mercury bead. An even larger, >700 times, release occurs from coated Hg(0) beads that have been reacted with manganese oxide, suggesting that manganese oxides are involved in the transformation of the Hg(0) beads and creation of the soluble mercury coatings. Although the coatings may inhibit Hg(0) evaporation, the high solubility of the coatings can enhance Hg(II) migration away from the Hg(0)-spill site and result in potential changes in mercury speciation in the soil and increased mercury mobility. C1 [Miller, Carrie L.; Watson, David B.; Lester, Brian P.; Howe, Jane Y.; He, Feng; Liang, Liyuan; Pierce, Eric M.] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Miller, Carrie L.] Troy Univ, Troy, NY 36082 USA. [Howe, Jane Y.] Hitachi High Technol Canada Inc, Toronto, ON M9W 6A4, Canada. [Phillips, Debra H.] Queens Univ Belfast, Belfast BT7 1NN, Antrim, North Ireland. [He, Feng] Zhejiang Univ Technol, Coll Biol & Environm Engn, Hangzhou 310032, Zhejiang, Peoples R China. RP Miller, CL (reprint author), Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. EM millerc@troy.edu; watsondb@ornl.gov RI He, Feng/B-9444-2012; Phillips, Debra/F-1828-2010; Watson, David/C-3256-2016; Howe, Jane/G-2890-2011; Pierce, Eric/G-1615-2011 OI He, Feng/0000-0001-5702-4511; Phillips, Debra/0000-0001-8548-7409; Watson, David/0000-0002-4972-4136; Pierce, Eric/0000-0002-4951-1931 FU Office of Groundwater and Soil Remediation, Office of Environmental Management, U.S. Department of Energy (DOE) as part of the Applied Field Research Initiative Program at ORNL [DE-AC05-00OR22725]; Shared Research Equipment (ShaRE) User Program of ORNL - Office of Basic Energy Sciences, U.S. DOE; U.S. DOE [DE-AC05-00OR22725] FX The authors thank Kenneth Lowe for field sampling assistance and Stephen Field and Terry Cothron of B&W Y-12 for assistance in coordinating the collection of field samples at the Y-12 facility. Roberta Ann Meisner of ORNL conducted the XRD analyses. This research was supported by the Office of Groundwater and Soil Remediation, Office of Environmental Management, U.S. Department of Energy (DOE) as part of the Applied Field Research Initiative Program at ORNL, which is managed by UT-Battelle, LLC for the U.S. DOE under Contract DE-AC05-00OR22725. The SEM work was in part sponsored by the Shared Research Equipment (ShaRE) User Program of ORNL, which is sponsored by the Office of Basic Energy Sciences, U.S. DOE. This manuscript has been authored by UT-Battelle, LLC under Contract DE-AC05-00OR22725 with the U.S. DOE. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript or allow others to do so for United States Government purposes. The DOE will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 48 TC 3 Z9 3 U1 6 U2 40 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD OCT 20 PY 2015 VL 49 IS 20 BP 12105 EP 12111 DI 10.1021/acs.est.5b00263 PG 7 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CU2JB UT WOS:000363348700014 PM 26389816 ER PT J AU Gilson, ER Huang, S van Groos, PGK Scheckel, KG Qafoku, O Peacock, AD Kaplan, DI Jaffe, PR AF Gilson, Emily R. Huang, Shan van Groos, Paul G. Koster Scheckel, Kirk G. Qafoku, Odeta Peacock, Aaron D. Kaplan, Daniel I. Jaffe, Peter R. TI Uranium Redistribution Due to Water Table Fluctuations in Sandy Wetland Mesocosms SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID SAVANNA RIVER SITE; DRINKING-WATER; SEDIMENTS; IMMOBILIZATION; REOXIDATION; SPECIATION; REDUCTION; PLANT AB To understand better the fate and stability of immobilized uranium (U) in wetland sediments, and how intermittent dry periods affect U stability, we dosed saturated sandy wetland mesocosms planted with Scirpus acutus with low levels of uranyl acetate for 4 months before imposing a short drying and rewetting period. Concentrations of U in mesocosm effluent increased after drying and rewetting, but the cumulative amount of U released following the dry period constituted less than 1% of the total U immobilized in the soil during the 4 months prior. This low level of remobilization suggests, and XANES analyses confirm, that microbial reduction was not the primary means of U immobilization, as the U immobilized in mesocosms was primarily U(VI) rather than U(IV). Drying followed by rewetting caused a redistribution of U downward in the soil profile and to root surfaces. Although the U on roots before drying was primarily associated with minerals, the U that relocated to the roots during drying and rewetting was bound diffusely. Results show that short periods of drought conditions in a sandy wetland, which expose reduced sediments to air, may impact U distribution without causing large releases of soil-bound U to surface waters. C1 [Gilson, Emily R.; Huang, Shan; van Groos, Paul G. Koster; Jaffe, Peter R.] Princeton Univ, Princeton, NJ 08540 USA. [Scheckel, Kirk G.] US EPA, Cincinnati, OH 45268 USA. [Qafoku, Odeta] Pacific NW Natl Lab, Richland, WA 99352 USA. [Peacock, Aaron D.] Pace Analyt Energy Serv, Pittsburgh, PA 15238 USA. [Kaplan, Daniel I.] Savannah River Natl Lab, Aiken, SC 29808 USA. RP Jaffe, PR (reprint author), Princeton Univ, Dept Civil & Environm Engn, E Quad, Princeton, NJ 08540 USA. EM jaffe@princeton.edu RI ID, MRCAT/G-7586-2011; OI Scheckel, Kirk/0000-0001-9326-9241 FU Subsurface Biogeochemical Research Program of the U.S. Department of Energy's Office of Biological and Environmental Research [DE-SC0006847]; DOE Office of Science [DE-AC02-06CH11357]; DOE; MRCAT member institutions; EPA; Office of Biological and Environmental Research FX This research was supported through contract DE-SC0006847 by the Subsurface Biogeochemical Research Program of the U.S. Department of Energy's Office of Biological and Environmental Research. A portion of this research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. The Materials Research Collaborative Access Team (MRCAT) operations at the Advanced Photon Source are supported by the DOE and the MRCAT member institutions. Although the U.S. Environmental Protection Agency (EPA) contributed to some of the work described in this document, the research presented was not performed by or funded by EPA and was not subject to EPA's quality system requirements. Consequently, the views, interpretations, and conclusions expressed in this document are solely those of the authors and do not necessarily reflect or represent EPA's views or policies. A portion of this research was performed using Radiochemistry Annex at EMSL, a DOE Office of Science User Facility sponsored by the Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. NR 34 TC 2 Z9 2 U1 3 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD OCT 20 PY 2015 VL 49 IS 20 BP 12214 EP 12222 DI 10.1021/acs.est.5b02957 PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CU2JB UT WOS:000363348700027 PM 26404564 ER PT J AU Kolesar, KR Li, ZY Wilson, KR Cappa, CD AF Kolesar, Katheryn R. Li, Ziyue Wilson, Kevin R. Cappa, Christopher D. TI Heating-Induced Evaporation of Nine Different Secondary Organic Aerosol Types SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID ALPHA-PINENE OZONOLYSIS; VOLATILITY MEASUREMENTS; MASS-SPECTROMETRY; FRAGMENTATION REACTIONS; MOLECULAR COMPOSITION; PARTICLE FORMATION; THERMAL-PROPERTIES; OH OXIDATION; BETA-PINENE; TIME SCALES AB The volatility of the compounds comprising organic aerosol (OA) determines their distribution between the gas and particle phases. However, there is a disconnect between volatility distributions as typically derived from secondary OA (SOA) growth experiments and the effective particle volatility as probed in evaporation experiments. Specifically, the evaporation experiments indicate an overall much less volatile SOA. This raises questions regarding the use of traditional volatility distributions in the simulation and prediction of atmospheric SOA concentrations. Here, we present results from measurements of thermally induced evaporation of SOA for nine different SOA types (i.e., distinct volatile organic compound and oxidant pairs) encompassing both anthropogenic and biogenic compounds and 03 and OH to examine the extent to which the low effective volatility of SOA is a general phenomenon or specific to a subset of SOA types. The observed extents of evaporation with temperature were similar for all the SOA types and indicative of a low effective volatility. Furthermore, minimal variations in the composition of all the SOA types upon heating-induced evaporation were observed. These results suggest that oligomer decomposition likely plays a major role in controlling SOA evaporation, and since the SOA formation time scale in these measurements was less than a minute, the oligomer-forming reactions must be similarly rapid. Overall, these results emphasize the importance of accounting for the role of condensed phase reactions in altering the composition of SOA when assessing particle volatility. C1 [Kolesar, Katheryn R.; Cappa, Christopher D.] Univ Calif Davis, Dept Civil & Environm Engn, Davis, CA 95616 USA. [Li, Ziyue] Univ Calif Davis, Atmospher Sci Grad Grp, Davis, CA 95616 USA. [Wilson, Kevin R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Cappa, CD (reprint author), Univ Calif Davis, Dept Civil & Environm Engn, One Shields Ave, Davis, CA 95616 USA. EM cdcappa@ucdavis.edu FU National Science Foundation [ATM-1151062]; Atmospheric Aerosols and Health program at UC Davis; Office of Science, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy [DE-AC02-05CH1123]; Department of Energy, Early Career Research Program, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank Theodora Nah for experimental assistance and the staff of the ALS for support over the many years these experiments were conducted. This material is based upon work supported by the National Science Foundation under Grant No. ATM-1151062 and by the Atmospheric Aerosols and Health program at UC Davis. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH1123. K.R.W. is supported by Department of Energy, Early Career Research Program, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. This work was performed at Beamline 9.0.2 at the Advanced Light Source at Lawrence Berkeley National Laboratory. NR 75 TC 4 Z9 4 U1 5 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD OCT 20 PY 2015 VL 49 IS 20 BP 12242 EP 12252 DI 10.1021/acs.est.5b03038 PG 11 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CU2JB UT WOS:000363348700030 PM 26393817 ER PT J AU Roth, EJ Gilbert, B Mays, DC AF Roth, Eric J. Gilbert, Benjamin Mays, David C. TI Colloid Deposit Morphology and Clogging in Porous Media: Fundamental Insights Through Investigation of Deposit Fractal Dimension SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID LIGHT-SCATTERING; PARTICLE-SIZE; TRANSPORT; PERMEABILITY; AGGREGATE; GEOMETRY; SURFACE; FLOW AB Experiments reveal a wide discrepancy between the permeability of porous media containing colloid deposits and the available predictive equations. Evidence suggests that this discrepancy results, in part, from the predictive equations failing to account for colloid deposit morphology. This article reports a series of experiments using static light scattering (SLS) to characterize colloid deposit morphology within refractive index matched (RIM) porous media during flow through a column. Real time measurements of permeability, specific deposit, deposit fractal dimension, and deposit radius of gyration, at different vertical positions, were conducted with initially clean porous media at various ionic strengths and fluid velocities. Decreased permeability (i.e., increased clogging) corresponded with higher specific deposit, lower fractal dimension, and smaller radius of gyration. During deposition, fractal dimension, radius of gyration, and permeability decreased with increasing specific deposit. During flushing with colloid-free fluid, these trends reversed, with increased fractal dimension, radius of gyration, and permeability. These observations suggest a deposition scenario in which large and uniform aggregates become deposits, which reduce porosity, lead to higher fluid shear forces, which then decompose the deposits, filling the pore space with small and dendritic fragments of aggregate. C1 [Roth, Eric J.; Mays, David C.] Univ Colorado, Dept Civil Engn, Denver, CO 80217 USA. [Gilbert, Benjamin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Mays, DC (reprint author), Univ Colorado, Dept Civil Engn, Campus Box 113,POB 173364, Denver, CO 80217 USA. EM david.mays@ucdenver.edu RI Mays, David/D-9366-2016; Gilbert, Benjamin/E-3182-2010 OI Mays, David/0000-0002-5218-1670; FU U.S. Department of Energy, Subsurface Biogeochemistry Research Program [DE-SC0006962]; Subsurface Science Scientific Focus Area - U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231] FX We received constructive feedback from three anonymous referees, one of whom provided extensive comments that thoroughly improved the manuscript. This research was supported by the U.S. Department of Energy, Subsurface Biogeochemistry Research Program (award DE-SC0006962). B.G. was supported as part of the Subsurface Science Scientific Focus Area funded by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research (award DE-AC02-05CH11231). NR 47 TC 2 Z9 2 U1 4 U2 10 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD OCT 20 PY 2015 VL 49 IS 20 BP 12263 EP 12270 DI 10.1021/acs.est.5b03212 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CU2JB UT WOS:000363348700032 PM 26412205 ER PT J AU Xu, MY He, ZL Zhang, Q Liu, J Guo, J Sun, GP Zhou, JZ AF Xu, Meiying He, Zhili Zhang, Qin Liu, Jin Guo, Jun Sun, Guoping Zhou, Jizhong TI Responses of Aromatic-Degrading Microbial Communities to Elevated Nitrate in Sediments SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID IN-SITU BIOREMEDIATION; PHYLOGENETIC DIVERSITY; ANAEROBIC DEGRADATION; DENITRIFYING BACTERIA; GENOME SEQUENCE; PURE CULTURES; HYDROCARBONS; METABOLISM; BIODEGRADATION; PHENANTHRENE AB A high number of aromatic compounds that have been released into aquatic ecosystems have accumulated in sediment because of their low solubility and high hydrophobicity, causing significant hazards to the environment and human health. Since nitrate is an essential nitrogen component and a more thermodynamically favorable electron acceptor for anaerobic respiration, nitrate-based bioremediation has been applied to aromatic-contaminated sediments. However, few studies have focused on the response of aromatic-degrading microbial communities to nitrate addition in anaerobic sediments. Here we hypothesized that high nitrate inputs would stimulate aromatic-degrading microbial communities and their associated degrading processes, thus increasing the bioremediation efficiency in aromatic compound-contaminated sediments. We analyzed the changes of key aromatic-degrading genes in the sediment samples from a field-scale site for in situ bioremediation of an aromatic-contaminated creek in the Pearl River Delta before and after nitrate injection using a functional gene array. Our results showed that the genes involved in the degradation of several kinds of aromatic compounds were significantly enriched after nitrate injection, especially those encoding enzymes for central catabolic pathways of aromatic compound degradation, and most of the enriched genes were derived from nitrate-reducing microorganisms, possibly accelerating bioremediation of aromatic-contaminated sediments. The sediment nitrate concentration was found to be the predominant factor shaping the aromatic-degrading microbial communities. This study provides new insights into our understanding of the influences of nitrate addition on aromatic-degrading microbial communities in sediments. C1 [Xu, Meiying; Zhang, Qin; Liu, Jin; Guo, Jun; Sun, Guoping] Guangdong Inst Microbiol, Guangdong Prov Key Lab Microbial Culture Collect, Guangzhou 510070, Guangdong, Peoples R China. [Xu, Meiying; Guo, Jun; Sun, Guoping] State Key Lab Appl Microbiol Southern China, Guangzhou 510070, Guangdong, Peoples R China. [He, Zhili; Zhou, Jizhong] Univ Oklahoma, Inst Environm Genom, Norman, OK 73019 USA. [He, Zhili; Zhou, Jizhong] Univ Oklahoma, Dept Microbiol & Plant Biol, Norman, OK 73019 USA. [Zhou, Jizhong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Zhou, Jizhong] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China. RP Xu, MY (reprint author), Guangdong Inst Microbiol, Guangdong Prov Key Lab Microbial Culture Collect, Guangzhou 510070, Guangdong, Peoples R China. EM xumy@gdim.cn FU National Science Foundation for Excellent Young Scholars of China [51422803]; Guangdong Province-Chinese Academy of Sciences [2013B091500081]; Guangdong Provincial Natural Science Foundation [2014A030308019]; Special Foundation for the Science and Technology Innovation Leaders of Guangdong Province [2014TX01Z038]; Special Fund for Agro-Scientific Research in the Public Interest [201503108]; Guangdong Provincial Innovative Development of Marine Economy Regional Demonstration Projects [GD2012-D01-002] FX This research was supported by the National Science Foundation for Excellent Young Scholars of China (51422803), Guangdong Province-Chinese Academy of Sciences strategic cooperative project (2013B091500081), Guangdong Provincial Natural Science Foundation (2014A030308019), Special Foundation for the Science and Technology Innovation Leaders of Guangdong Province (2014TX01Z038), the Special Fund for Agro-Scientific Research in the Public Interest (201503108), and Guangdong Provincial Innovative Development of Marine Economy Regional Demonstration Projects (GD2012-D01-002). NR 38 TC 2 Z9 2 U1 10 U2 42 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD OCT 20 PY 2015 VL 49 IS 20 BP 12422 EP 12431 DI 10.1021/acs.est.5b03442 PG 10 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CU2JB UT WOS:000363348700050 PM 26390227 ER PT J AU Kelly, JC Sullivan, JL Burnham, A Elgowainy, A AF Kelly, Jarod C. Sullivan, John L. Burnham, Andrew Elgowainy, Amgad TI Impacts of Vehicle Weight Reduction via Material Substitution on Life-Cycle Greenhouse Gas Emissions SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID CLIMATE-CHANGE IMPACTS; AUTOMOTIVE MATERIAL; FUEL CONSUMPTION; KYOTO PROTOCOL; ALUMINUM; SUSTAINABILITY; AUTOMOBILES; BENEFITS; STEEL AB This study examines the vehicle-cycle and vehicle total life-cycle impacts of substituting lightweight materials into vehicles. We determine part-based greenhouse gas (GHG) emission ratios by collecting material substitution data and evaluating that alongside known mass-based GHG ratios (using and updating Argonne National Laboratory's Greet model) associated with material pair substitutions, Several vehicle parts are lightweighted via material substitution, using substitution ratios from a U.S. Department of Energy report, to determine GHG emissions. We then examine fuel-cycle GHG reductions from lightweighting. The fuel reduction value methodology is applied using FRV estimates of 0.15-0.25, and 0.25-0.5 L/(100km.100 kg), with and without powertrain adjustments, respectively. GHG breakeven values are derived for both driving distance and material substitution ratio. While material substitution can reduce vehicle weight, it often increases vehicle-cycle GHGs. It is likely that replacing steel (the dominant vehicle material) with wrought aluminum, carbon fiber reinforced plastic (CRFP), or magnesium will increase vehicle-cycle GHGs. However, lifetime fuel economy benefits often outweigh the vehicle-cycle, resulting in a net total life-cycle GHG benefit. This is the case for steel replaced by wrought aluminum in all assumed cases, and for CFRP and magnesium except for high substitution ratio and low FRV. C1 [Kelly, Jarod C.; Sullivan, John L.; Burnham, Andrew; Elgowainy, Amgad] Argonne Natl Lab, Div Energy Syst, Syst Assessment Grp, Argonne, IL 60439 USA. RP Kelly, JC (reprint author), Argonne Natl Lab, Div Energy Syst, Syst Assessment Grp, 9700 S Cass Ave, Argonne, IL 60439 USA. EM jckelly@anl.gov OI Kelly, Jarod/0000-0002-7804-6506 FU Vehicle Technologies Office of the U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy [DE-AC02-06CH11357] FX This study was supported by the Vehicle Technologies Office of the U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy under Contract Number DE-AC02-06CH11357. We are grateful to Connie Bezanson and Jake Ward of that office for their guidance and support. NR 50 TC 3 Z9 3 U1 7 U2 28 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD OCT 20 PY 2015 VL 49 IS 20 BP 12535 EP 12542 DI 10.1021/acs.est.5b03192 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CU2JB UT WOS:000363348700063 PM 26393414 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Ochesanu, S Rougny, R Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Van Parijs, I Barria, P Caillol, C Clerbaux, B De Lentdecker, G Delannoy, H Dobur, D Fasanella, G Favart, L Gay, APR Grebenyuk, A Leonard, A Mohammadi, A Pernie, L Randleconde, A Reis, T Seva, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Zenoni, F Beernaert, K Benucci, L Cimmino, A Crucy, S Fagot, A Garcia, G Gul, M Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Diblen, SS Sigamani, M Strobbe, N Tytgat, M Van Driessche, W Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bondu, O Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Mertens, A Nuttens, C Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Beliy, N Caebergs, T Hammad, GH Alda, WL Alves, GA Brito, L Martins, MC Martins, TD Hensel, C Herrera, CM Moraes, A Pol, ME Teles, PR Das Chagas, EBB Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Guativa, LMH Malbouisson, H Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santaolalla, J Santoro, A Sznajder, A Manganote, EJT Pereira, AV Ahuja, S Bernardes, CA Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Moon, CS Novaes, SF Padula, SS Abad, DR Vargas, JCR Aleksandrov, A Genchev, V Hadjiiska, R Iaydjiev, P Marinov, A Piperov, S Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Ahmad, M Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Plestina, R Romeo, F Shaheen, SM Tao, J Wang, C Wang, Z Zhang, H Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Xu, Z Zhang, F Zhang, L Zou, W Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Pone, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Bodlak, M Finger, M Finger, M Ali, A Aly, R Aly, S Assran, Y Kamel, AE Lotfy, A Mahmoud, MA Masod, R Radi, A Calpas, B Kadastik, M Murumaa, M Raidal, M Tiko, A Veelken, C Eerola, P Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Talvitie, J Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Favaro, C Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Maleles, J Rander, J Rosowsky, A Titov, M Zghiche, A Baffioni, S Beaudette, F Busson, P Cadamuro, L Chapon, E Charlot, C Dahms, T Davignon, O Filipovic, N Florent, A de Cassagnac, RG Mastrolorenzo, L Mine, P Naranjo, IN Nguyen, M Ochando, C Ortona, G Paganini, P Regnard, S Salerno, R Sauvan, JB Sirois, Y Strebler, T Yilmaz, Y Zabi, A Agram, JL Andrea, J Aubin, A Bloch, D Brom, JM Buttignol, M Chabert, EC Chanon, N Collard, C Conte, E Fontaine, JC Gele, D Goerlach, U Goetzmann, C 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Ruggles, T. Sarangi, T. Savin, A. Smith, N. Smith, W. H. Taylor, D. Woods, N. CA CMS Collaboration TI Comparison of the Z/gamma* plus jets to gamma plus jets cross sections in pp collisions at root s=8 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Jets; Hadron-Hadron Scattering; Beyond Standard Model; QCD; Photon production ID PARTON DISTRIBUTIONS; LHC AB A comparison of the differential cross sections for the processes Z/gamma* + jets and photon (gamma)+ jets is presented. The measurements are based on data collected with the CMS detector at root s = 8TeV corresponding to an integrated luminosity of 19.7 fb(-1). The differential cross sections and their ratios are presented as functions of p(T). The measurements are also shown as functions of the jet multiplicity. Differential cross sections are obtained as functions of the ratio of the Z/gamma* p(T) to the sum of all jet transverse momenta and of the ratio of the Z/gamma* p(T) to the leading jet transverse momentum. 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[Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.; Viliani, L.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Di Guida, S.; Esposito, M.; Iorio, A. O. M.; Sciacca, C.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, I-85100 Potenza, Italy. [Meola, S.] Univ G Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Bellato, M.; Bisello, D.; Carlin, R.; De Oliveira, A. Carvalho Antunes; Cheechia, P.; Dall'Osso, M.; Dorigo, T.; Dosselli, U.; Fantinel, S.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Laeaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronehese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Carlin, R.; De Oliveira, A. Carvalho Antunes; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronehese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. Univ Trent, Trento, Italy. [Braghieri, A.; Gabusi, M.; Magnani, A.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Solestizi, L. Alunni; Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariecia, P.; Mantovani, G.; Meniehelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Solestizi, L. Alunni; Biasini, M.; Ciangottini, D.; Fano, L.; Lariecia, P.; Mantovani, G.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenehini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Fiori, F.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Micheli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliecioni, M.; Angioni, G. L. Pinna; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Pacher, L.; Angioni, G. L. Pinna; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. 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[Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Marrouche, J.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Zagozdzinska, A.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Buchmann, M. A.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marini, A. C.; Marionneau, M.; del Arbol, P. 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J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Citron, M.; Colling, D.; Corpe, L.; Cripps, N.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Sharp, P.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Pastika, N.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Cutts, D.; Demiragli, Z.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Sagir, S.; Sinthuprasith, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Saltzberg, D.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Rikova, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Sumowidagdo, S.; Wei, H.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Kovalskyi, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Justus, C.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Smith, J. G.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Skinnari, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Hu, Z.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Kwan, S.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Whitbeck, A.; Yang, F.; Yin, H.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Di Giovanni, G. P.; Field, R. D.; Fisher, M.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Kypreos, T.; Low, J. F.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rank, D.; Rinkevicius, A.; Shchutska, L.; Snowball, M.; Sperka, D.; Wang, S. J.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Bhopatkar, V.; Hohlmann, M.; Kalakhety, H.; Mareskas-palcek, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.] Univ Illinois, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Sen, S.; Snyder, C.; Tan, P.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovie, P.; Martin, C.; Nash, K.; Osherson, M.; Swartz, M.; Xiao, M.; Xin, Y.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Gray, J.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Chakaberia, I.; Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Skhirtladze, N.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Pedro, K.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Baty, A.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Levin, A.; Luckey, P. D.; Mcginn, C.; Niu, X.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Sumorok, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Finkel, A.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Nourbakhsh, S.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chase, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Trovato, M.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Lynch, S.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Pearson, T.; Planer, M.; Ruchti, R.; Smith, G.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Barnes, V. E.; Benedetti, D.; Bortoletto, D.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Miller, D. H.; Neumeister, N.; Primavera, F.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Zablocki, J.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Hindrichs, O.; Khukhunaishvili, A.; Petrillo, G.; Verzetti, M.; Vishnevskiy, D.] Univ Rochester, Rochester, NY 14627 USA. [Demortier, L.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Fereneek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Hughes, E.; Kaplan, S.; Elayavalli, R. Kunnawalkam; Lath, A.; Panwalkar, S.; Park, M.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Foerster, M.; Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Hernandez, A. Castaneda; Dalchenko, M.; De Mattia, M.; Delgado, A.; Dildick, S.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Krutelyov, V.; Montalvo, R.; Mueller, R.; Osipenkov, I.; Pakhotin, Y.; Patel, R.; Perloff, A.; Roe, J.; Rose, A.; Safonov, A.; Suarez, I.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akehurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kunori, S.; Lamichhane, K.; Lee, S. W.; Libeiro, T.; Undleeb, S.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Janjam, R.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.; Xu, Q.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Wolfe, E.; Wood, J.; Xia, F.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Christian, A.; Dasu, S.; Dodd, L.; Duric, S.; Friis, E.; Gomber, B.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Levine, A.; Long, K.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Ruggles, T.; Sarangi, T.; Savin, A.; Smith, N.; Smith, W. H.; Taylor, D.; Woods, N.] Univ Wisconsin, Madison, WI 53706 USA. [Fruehwirth, R.; Jeitler, M.; Krammer, M.; Schieck, J.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Rabady, D.; Genchev, V.; Merlin, J. A.; Boudoul, G.; Lingemann, J.; Hartmann, F.; Kornmayer, A.; Radogna, R.; Silvestris, L.; Giordano, F.; Gennai, S.; Lucchini, M. T.; Marzocchi, B.; Di Guida, S.; Meola, S.; Paolucci, P.; Azzi, P.; Ciangottini, D.; Spiezia, A.; Donato, S.; Traczyk, P.; Finco, L.; Candelise, V.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Beluffi, C.] Univ Haute Alsace Mulhouse, Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, CNRS IN2P3, Strasbourg, France. [Giammanco, A.] NICPB, Tallinn, Estonia. [Popov, A.; Zhukov, V.; Katkov, I.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, SP, Brazil. [Moon, C. S.] CNRS IN2P3, Paris, France. [Plestina, R.; Bernet, C.] Ecole Polytech, Lab Leprince Ringuet, IN2P3 CNRS, Palaiseau, France. [Zhang, F.] Univ Libre Bruxelles, Brussels, Belgium. [Finger, M., Jr.] Joint Inst Nucl Res, Dubna, Russia. [Ali, A.; Masod, R.; Radi, A.] Ain Shams Univ, Cairo, Egypt. [Ali, A.; Radi, A.] British Univ Egypt, Cairo, Egypt. [Aly, R.; Aly, S.] Helwan Univ, Cairo, Egypt. [Assran, Y.] Suez Univ, Suez, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Lotfy, A.; Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Hempel, M.; Karacheban, O.; Marfin, I.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Horvath, D.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Karancsi, J.] Univ Debrecen, Debrecen, Hungary. [Bartok, M.] Wigner Res Ctr Phys, Budapest, Hungary. [Bhowmik, S.; Maity, M.; Sarkar, T.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.; Squillacioti, P.] Univ Siena, I-53100 Siena, Italy. [Savoy-Navarro, A.] Purdue Univ, W Lafayette, IN 47907 USA. [Ali, M. A. B. Md] Int Islamic Univ Malaysia, Kuala Lumpur, Malaysia. [Heredia-de La Cruz, I.] Consejo Natl Ciencia & Tecnol, Mexico City, DF, Mexico. [Matveev, V.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Toriashvili, T.] Tbilisi State Univ, Inst High Energy Phys & Informatizat, GE-380086 Tbilisi, Rep of Georgia. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Dubinin, M.] CALTECH, Pasadena, CA 91125 USA. [Adzic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Rolandi, G.] Scuola Normale Super Pisa, Pisa, Italy. [Rolandi, G.] Sezione Ist Nazl Fis Nucl, Pisa, Italy. [Sphicas, P.] Univ Athens, Athens, Greece. [Zagozdzinska, A.] Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. [Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.] Gaziosmanpasa Univ, Tokat, Turkey. [Kangal, E. E.] Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Pin Reis Univ, Istanbul, Turkey. [Cerci, D. Sunar] Adiyaman Univ, Adiyaman, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Albayrak, E. A.] Mimar Sinan Univ, Istanbul, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Gunaydin, Y. O.] Kahramanmaras Sutcu Imam Univ, Kahramanmaras, Turkey. [Newbold, D. M.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. [Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI ciocci, maria agnese /I-2153-2015; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Xie, Si/O-6830-2016; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Paulini, Manfred/N-7794-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Dremin, Igor/K-8053-2015; Azarkin, Maxim/N-2578-2015; Chinellato, Jose Augusto/I-7972-2012; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Stahl, Achim/E-8846-2011; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Da Silveira, Gustavo Gil/N-7279-2014; Haj Ahmad, Wael/E-6738-2016; Menasce, Dario/A-2168-2016; Paganoni, Marco/A-4235-2016; de Jesus Damiao, Dilson/G-6218-2012; Dogra, Sunil /B-5330-2013; Leonidov, Andrey/M-4440-2013; Calvo Alamillo, Enrique/L-1203-2014; Hernandez Calama, Jose Maria/H-9127-2015; Cerrada, Marcos/J-6934-2014; Andreev, Vladimir/M-8665-2015; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Novaes, Sergio/D-3532-2012; Della Ricca, Giuseppe/B-6826-2013; Dudko, Lev/D-7127-2012; Moraes, Arthur/F-6478-2010; Manganote, Edmilson/K-8251-2013; Lokhtin, Igor/D-7004-2012; Vinogradov, Alexey/O-2375-2015; Petrushanko, Sergey/D-6880-2012; VARDARLI, Fuat Ilkehan/B-6360-2013; Cakir, Altan/P-1024-2015; Montanari, Alessandro/J-2420-2012; Matorras, Francisco/I-4983-2015; Gennai, Simone/P-2880-2015; TUVE', Cristina/P-3933-2015 OI ciocci, maria agnese /0000-0003-0002-5462; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Chinellato, Jose Augusto/0000-0002-3240-6270; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Stahl, Achim/0000-0002-8369-7506; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Seixas, Joao/0000-0002-7531-0842; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Haj Ahmad, Wael/0000-0003-1491-0446; Menasce, Dario/0000-0002-9918-1686; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Calvo Alamillo, Enrique/0000-0002-1100-2963; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Cerrada, Marcos/0000-0003-0112-1691; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; Dudko, Lev/0000-0002-4462-3192; Moraes, Arthur/0000-0002-5157-5686; Montanari, Alessandro/0000-0003-2748-6373; Matorras, Francisco/0000-0003-4295-5668; TUVE', Cristina/0000-0003-0739-3153 FU BMWFW (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COL-CIENCIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia); ERC IUT (Estonia); ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP (Republic of Korea); NRF (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (U.S.A.); NSF (U.S.A.); Marie-Curie program; European Research Council (European Union); EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS program of the Foundation for Polish Science; European Union, Regional Development Fund; Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR project (Italy) [20108T4XTM]; EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COL-CIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP and NRF (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (U.S.A.).; Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF; and the National Priorities Research Program by Qatar National Research Fund. NR 51 TC 1 Z9 1 U1 9 U2 42 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD OCT 20 PY 2015 IS 10 AR 128 DI 10.1007/JHEP10(2015)128 PG 46 WC Physics, Particles & Fields SC Physics GA CU4PS UT WOS:000363512600001 ER PT J AU Gasparov, VA He, X Dubuis, G Pavuna, D Kushch, ND Yagubskii, EB Schlueter, JA Bozovic, I AF Gasparov, V. A. He, Xi Dubuis, G. Pavuna, D. Kushch, N. D. Yagubskii, E. B. Schlueter, J. A. Bozovic, I. TI Magnetic field, frequency and temperature dependence of complex conductance of ultrathin La1.65Sr0.45CuO4/La2CuO4 films and the organic superconductors kappa-(BEDT-TTF)(2)Cu[N(CN)(2)]Br SO INTERNATIONAL JOURNAL OF MODERN PHYSICS B LA English DT Article; Proceedings Paper CT 10th International Conference on New Theories, Discoveries and Applications of Superconductivity New3SC CY OCT 26-29, 2014 CL Chongqing Sheraton, PEOPLES R CHINA DE Superconducting heterostructures; organic single crystals ID COULOMB-GAS; THIN-FILMS; TRANSITION; MOTION; OXIDES AB We used atomic-layer molecular beam epitaxy (ALL-MBE) to synthesize bilayer films of a cuprate metal (La1.65Sr0.45CuO4, LSCO) and a cuprate insulator (La2CuO4, LCO), in which interface superconductivity occurs in a layer that is just one-half unit cell thick. We have studied the magnetic field and temperature dependence of the complex sheet conductance, sigma(omega), of these films, and compared them to kappa-(BEDT-TTF)(2)Cu[N(CN)(2)] Br single crystals. The magnetic field H was applied both parallel and perpendicular to the 2D conducting layers. Experiments have been carried out at frequencies between 23 kHz and 50 MHz using either two-coil mutual inductance technique, or the LC resonators with spiral or rectangular coils. The real and the imaginary parts of the mutual-inductance M(T,omega) between the coil and the sample were measured and converted to complex conductivity. For H perpendicular to the conducting layers, we observed almost identical behavior in both films and kappa-Br single crystals: (i) the transition onset in the inductive response, L-k(-1) (T) occurs at a temperature lower by 2 K than in Re sigma(T), (ii) this shift is almost constant with magnetic field up to 8 T; (iii) the vortex diffusion constant D(T) is exponential due to pinning of vortex cores. These results can be described by the extended dynamic theory of the Berezinski-Kosterlitz-Thouless (BKT) transition and dynamics of bound vortex-antivortex pairs with short separation lengths. C1 [Gasparov, V. A.] RAS, Inst Solid State Phys, Chernogolovka 142432, Moscow District, Russia. [He, Xi; Dubuis, G.; Bozovic, I.] Brookhaven Natl Lab, Upton, NY 11973 USA. [He, Xi; Dubuis, G.; Pavuna, D.] Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland. [Kushch, N. D.; Yagubskii, E. B.] RAS, Inst Problems Chem Phys, Chernogolovka 142432, Moscow District, Russia. [Schlueter, J. A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. EM vgasparo@issp.ac.ru; xhe@bnl.gov; guydubuis@gmail.com; davor.pavuna@epfl.ch; kushch@icp.ac.ru; yagubskii@icp.ac.ru; jaschlueter@anl.gov; bozovic@bnl.gov RI Dubuis, Guy/A-6849-2012 OI Dubuis, Guy/0000-0002-8199-4953 FU Russian Academy of Sciences; RFFI [12-02-00171]; U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division FX V. G. would like to thank V. F. Gantmakher and R. Huguenin for helpful discussions and A. I. Rodigin and S. Zlobin for experimental aid. This work was supported in part by the Russian Academy of Sciences Program "Quantum mesoscopic and nonhomogeneous systems" and RFFI grant 12-02-00171. The work at Brookhaven National Laboratory was supported by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 21 TC 2 Z9 2 U1 3 U2 22 PU WORLD SCIENTIFIC PUBL CO PTE LTD PI SINGAPORE PA 5 TOH TUCK LINK, SINGAPORE 596224, SINGAPORE SN 0217-9792 EI 1793-6578 J9 INT J MOD PHYS B JI Int. J. Mod. Phys. B PD OCT 20 PY 2015 VL 29 IS 25-26 SI SI AR 1542012 DI 10.1142/S0217979215420126 PG 9 WC Physics, Applied; Physics, Condensed Matter; Physics, Mathematical SC Physics GA CT7FH UT WOS:000362979100013 ER PT J AU Campione, S Liu, S Benz, A Klem, JF Sinclair, MB Brener, I AF Campione, Salvatore Liu, Sheng Benz, Alexander Klem, John F. Sinclair, Michael B. Brener, Igal TI Epsilon-Near-Zero Modes for Tailored Light-Matter Interaction SO PHYSICAL REVIEW APPLIED LA English DT Article ID METAMATERIAL NANOCAVITIES; INTERSUBBAND TRANSITIONS; PERMITTIVITY AB Epsilon-near-zero (ENZ) modes arising from condensed-matter excitations such as phonons and plasmons are a new path for tailoring light-matter interactions at the nanoscale. Complex spectral shaping can be achieved by creating such modes in nanoscale semiconductor layers and controlling their interaction with multiple, distinct, dipole resonant systems. Examples of this behavior are presented at midinfrared frequencies for ENZ modes that are strongly coupled to metamaterial resonators and simultaneously strongly coupled to semiconductor phonons or quantum-well intersubband transitions (ISTs), resulting in double-and triple-polariton branches in transmission spectra. For the double-polariton branch case, we find that the best strategy to maximize the Rabi splitting is to use a combination of a doped layer supporting an ENZ feature and a layer supporting ISTs, with overlapping ENZ and IST frequencies. This design flexibility renders this platform attractive for low-voltage tunable filters, light-emitting diodes, and efficient nonlinear composite materials. C1 [Campione, Salvatore; Liu, Sheng; Benz, Alexander; Klem, John F.; Sinclair, Michael B.; Brener, Igal] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Campione, Salvatore; Liu, Sheng; Benz, Alexander; Brener, Igal] Sandia Natl Labs, Ctr Integrated Nanotechnol CINT, Albuquerque, NM 87185 USA. RP Campione, S (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM sncampi@sandia.gov; ibrener@sandia.gov FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors acknowledge fruitful discussions with Professor Francois Marquier, Institut d'Optique, France. This work is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering and performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy Office of Science. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 34 TC 4 Z9 4 U1 8 U2 29 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2331-7019 J9 PHYS REV APPL JI Phys. Rev. Appl. PD OCT 20 PY 2015 VL 4 IS 4 AR 044011 DI 10.1103/PhysRevApplied.4.044011 PG 7 WC Physics, Applied SC Physics GA CT7WF UT WOS:000363024500002 ER PT J AU Chen, CY Dawson, S Zhang, Y AF Chen, Chien-Yi Dawson, S. Zhang, Yue TI Higgs CP violation from vectorlike quarks SO PHYSICAL REVIEW D LA English DT Article ID ELECTRIC-DIPOLE MOMENT; STANDARD MODEL; HIERARCHY; PHYSICS AB We explore CP violating aspects in the Higgs sector of models where new vectorlike quarks carry Yukawa couplings mainly to the third generation quarks of the Standard Model. We point out that in the simplest model, Higgs CP violating interactions only exist in the hWW channel. At low energy, we find that rare B decays can place similarly strong constraints as those from electric dipole moments on the source of CP violation. These observations offer a new handle to discriminate from other Higgs CP violating scenarios such as scalar sector extensions of the Standard Model, and imply an interesting future interplay among limits from different experiments. C1 [Chen, Chien-Yi; Dawson, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Zhang, Yue] CALTECH, Walter Burke Inst Theoret Phys, Pasadena, CA 91125 USA. RP Chen, CY (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. OI Dawson, Sally/0000-0002-5598-695X; Zhang, Yue/0000-0002-1984-7450 FU U.S. Department of Energy (DOE) [DE-AC02-98CH10886, DE-AC02-76SF00515]; Gordon and Betty Moore Foundation [776]; DOE Grant [DE-FG02-92ER40701]; DOE Early Career Award [DE-SC0010255] FX We thank JiJi Fan, Enrico Lunghi, and Miha Nemevsek for useful discussions. The work of C.-Y. Chen and S. Dawson is supported by the U.S. Department of Energy (DOE) under Grants No. DE-AC02-98CH10886 and Contract No. DE-AC02-76SF00515. This work of Y. Zhang is supported by the Gordon and Betty Moore Foundation through Grant No 776 to the Caltech Moore Center for Theoretical Cosmology and Physics, and by the DOE Grant No. DE-FG02-92ER40701, and also by a DOE Early Career Award under Grant No. DE-SC0010255. NR 53 TC 2 Z9 2 U1 0 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 20 PY 2015 VL 92 IS 7 AR 075026 DI 10.1103/PhysRevD.92.075026 PG 9 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CT7SN UT WOS:000363014900007 ER PT J AU Lees, JP Poireau, V Tisserand, V Grauges, E Palano, A Eigen, G Stugu, B Brown, DN Kerth, LT Kolomensky, YG Lee, MJ Lynch, G Koch, H Schroeder, T Hearty, C Mattison, TS McKenna, JA So, RY Khan, A Blinov, VE Buzykaev, AR Druzhinin, VP Golubev, VB Kravchenko, EA Onuchin, AP Serednyakov, SI Skovpen, YI Solodov, EP Todyshev, KY Lankford, AJ Dey, B Gary, JW Long, O Sevilla, MF Hong, TM Kovalskyi, D Richman, JD West, CA Eisner, AM Lockman, WS Vazquez, WP Schumm, BA Seiden, A Chao, DS Cheng, CH Echenard, B Flood, KT Hitlin, DG Kim, J Miyashita, TS Ongmongkolkul, P Porter, FC Rohrken, M Andreassen, R Huard, Z Meadows, BT Pushpawela, BG Sokoloff, MD Sun, L Ford, WT Smith, JG Wagner, SR Ayad, R Toki, WH Spaan, B Bernard, D Verderi, M Playfer, S Bettoni, D Bozzi, C Calabrese, R Cibinetto, G Fioravanti, E Garzia, I Luppi, E Piemontese, L Santoro, V Calcaterra, A de Sangro, R Finocchiaro, G Martellotti, S Patteri, P Peruzzi, IM Piccolo, M Zallo, A Contri, R Monge, MR Passaggio, S Patrignani, C Bhuyan, B Prasad, V Adametz, A Uwer, U Lacker, HM Mallik, U Chen, C Cochran, J Prell, S Ahmed, H Gritsan, AV Arnaud, N Davier, M Derkach, D Grosdidier, G Le Diberder, F Lutz, AM Malaescu, B Roudeau, P Stocchi, A Wormser, G Lange, DJ Wright, DM Coleman, JP Fry, JR Gabathuler, E Hutchcroft, DE Payne, DJ Touramanis, C Bevan, AJ Di Lodovico, F Sacco, R Cowan, G Brown, DN Davis, CL Denig, AG Fritsch, M Gradl, W Griessinger, K Hafner, A Schubert, KR Barlow, RJ Lafferty, GD Cenci, R Hamilton, B Jawahery, A Roberts, DA Cowan, R Cheaib, R Patel, PM Robertson, SH Neri, N Palombo, F Cremaldi, L Godang, R Summers, DJ Simard, M Taras, P De Nardo, G Onorato, G Sciacca, C Raven, G Jessop, CP LoSecco, JM Honscheid, K Kass, R Margoni, M Morandin, M Posocco, M Rotondo, M Simi, G Simonetto, F Stroili, R Akar, S Ben-Haim, E Bomben, M Bonneaud, GR Briand, H Calderini, G Chauveau, J Leruste, P Marchiori, G Ocariz, J Biasini, M Manoni, E Rossi, A Angelini, C Batignani, G Bettarini, S Carpinelli, M Casarosa, G Chrzaszcz, M Forti, F Giorgi, MA Lusiani, A Oberhof, B Paoloni, E Rama, M Rizzo, G Walsh, JJ Pegna, DL Olsen, J Smith, AJS Anulli, F Faccini, R Ferrarotto, F Ferroni, F Gaspero, M Pilloni, A Piredda, G Bunger, C Dittrich, S Grunberg, O Hess, M Leddig, T Voss, C Waldi, R Adye, T Olaiya, EO Wilson, FF Emery, S Vasseur, G Aston, D Bard, DJ Cartaro, C Convery, MR Dorfan, J Dubois-Felsmann, GP Ebert, M Field, RC Fulsom, BG Graham, MT Hast, C Innes, WR Kim, P Leith, DWGS Luitz, S Luth, V MacFarlane, DB Muller, DR Neal, H Pulliam, T Ratcliff, BN Roodman, A Schindler, RH Snyder, A Su, D Sullivan, MK Va'vra, J Wisniewski, WJ Wulsin, HW Purohit, MV Wilson, JR Randle-Conde, A Sekula, SJ Bellis, M Burchat, PR Puccio, EMT Alam, MS Ernst, JA Gorodeisky, R Guttman, N Peimer, DR Soffer, A Spanier, SM Ritchie, JL Schwitters, RF Izen, JM Lou, XC Bianchi, F De Mori, F Filippi, A Gamba, D Lanceri, L Vitale, L Martinez-Vidal, F Oyanguren, A Albert, J Banerjee, S Beaulieu, A Bernlochner, FU Choi, HHF King, GJ Kowalewski, R Lewczuk, MJ Lueck, T Nugent, IM Roney, JM Sobie, RJ Tasneem, N Gershon, TJ Harrison, PF Latham, TE Band, HR Dasu, S Pan, Y Prepost, R Wu, SL AF Lees, J. P. Poireau, V. Tisserand, V. Grauges, E. Palano, A. Eigen, G. Stugu, B. Brown, D. N. Kerth, L. T. Kolomensky, Yu. G. Lee, M. J. Lynch, G. Koch, H. Schroeder, T. Hearty, C. Mattison, T. S. McKenna, J. A. So, R. Y. Khan, A. Blinov, V. E. Buzykaev, A. R. Druzhinin, V. P. Golubev, V. B. Kravchenko, E. A. Onuchin, A. P. Serednyakov, S. I. Skovpen, Yu. I. Solodov, E. P. Todyshev, K. Yu. Lankford, A. J. Dey, B. Gary, J. W. Long, O. Sevilla, M. Franco Hong, T. M. Kovalskyi, D. Richman, J. D. West, C. A. Eisner, A. M. Lockman, W. S. Vazquez, W. Panduro Schumm, B. A. Seiden, A. Chao, D. S. Cheng, C. H. Echenard, B. Flood, K. T. Hitlin, D. G. Kim, J. Miyashita, T. S. Ongmongkolkul, P. Porter, F. C. Roehrken, M. Andreassen, R. Huard, Z. Meadows, B. T. Pushpawela, B. G. Sokoloff, M. D. Sun, L. Ford, W. T. Smith, J. G. Wagner, S. R. Ayad, R. Toki, W. H. Spaan, B. Bernard, D. Verderi, M. Playfer, S. Bettoni, D. Bozzi, C. Calabrese, R. Cibinetto, G. Fioravanti, E. Garzia, I. Luppi, E. Piemontese, L. Santoro, V. Calcaterra, A. de Sangro, R. Finocchiaro, G. Martellotti, S. Patteri, P. Peruzzi, I. M. Piccolo, M. Zallo, A. Contri, R. Monge, M. R. Passaggio, S. Patrignani, C. Bhuyan, B. Prasad, V. Adametz, A. Uwer, U. Lacker, H. M. Mallik, U. Chen, C. Cochran, J. Prell, S. Ahmed, H. Gritsan, A. V. Arnaud, N. Davier, M. Derkach, D. Grosdidier, G. Le Diberder, F. Lutz, A. M. Malaescu, B. Roudeau, P. Stocchi, A. Wormser, G. Lange, D. J. Wright, D. M. Coleman, J. P. Fry, J. R. Gabathuler, E. Hutchcroft, D. E. Payne, D. J. Touramanis, C. Bevan, A. J. Di Lodovico, F. Sacco, R. Cowan, G. Brown, D. N. Davis, C. L. Denig, A. G. Fritsch, M. Gradl, W. Griessinger, K. Hafner, A. Schubert, K. R. Barlow, R. J. Lafferty, G. D. Cenci, R. Hamilton, B. Jawahery, A. Roberts, D. A. Cowan, R. Cheaib, R. Patel, P. M. Robertson, S. H. Neri, N. Palombo, F. Cremaldi, L. Godang, R. Summers, D. J. Simard, M. Taras, P. De Nardo, G. Onorato, G. Sciacca, C. Raven, G. Jessop, C. P. LoSecco, J. M. Honscheid, K. Kass, R. Margoni, M. Morandin, M. Posocco, M. Rotondo, M. Simi, G. Simonetto, F. Stroili, R. Akar, S. Ben-Haim, E. Bomben, M. Bonneaud, G. R. Briand, H. Calderini, G. Chauveau, J. Leruste, Ph. Marchiori, G. Ocariz, J. Biasini, M. Manoni, E. Rossi, A. Angelini, C. Batignani, G. Bettarini, S. Carpinelli, M. Casarosa, G. Chrzaszcz, M. Forti, F. Giorgi, M. A. Lusiani, A. Oberhof, B. Paoloni, E. Rama, M. Rizzo, G. Walsh, J. J. Pegna, D. Lopes Olsen, J. Smith, A. J. S. Anulli, F. Faccini, R. Ferrarotto, F. Ferroni, F. Gaspero, M. Pilloni, A. Piredda, G. Buenger, C. Dittrich, S. Gruenberg, O. Hess, M. Leddig, T. Voss, C. Waldi, R. Adye, T. Olaiya, E. O. Wilson, F. F. Emery, S. Vasseur, G. Aston, D. Bard, D. J. Cartaro, C. Convery, M. R. Dorfan, J. Dubois-Felsmann, G. P. Ebert, M. Field, R. C. Fulsom, B. G. Graham, M. T. Hast, C. Innes, W. R. Kim, P. Leith, D. W. G. S. Luitz, S. Luth, V. MacFarlane, D. B. Muller, D. R. Neal, H. Pulliam, T. Ratcliff, B. N. Roodman, A. Schindler, R. H. Snyder, A. Su, D. Sullivan, M. K. Va'vra, J. Wisniewski, W. J. Wulsin, H. W. Purohit, M. V. Wilson, J. R. Randle-Conde, A. Sekula, S. J. Bellis, M. Burchat, P. R. Puccio, E. M. T. Alam, M. S. Ernst, J. A. Gorodeisky, R. Guttman, N. Peimer, D. R. Soffer, A. Spanier, S. M. Ritchie, J. L. Schwitters, R. F. Izen, J. M. Lou, X. C. Bianchi, F. De Mori, F. Filippi, A. Gamba, D. Lanceri, L. Vitale, L. Martinez-Vidal, F. Oyanguren, A. Albert, J. Banerjee, Sw. Beaulieu, A. Bernlochner, F. U. Choi, H. H. F. King, G. J. Kowalewski, R. Lewczuk, M. J. Lueck, T. Nugent, I. M. Roney, J. M. Sobie, R. J. Tasneem, N. Gershon, T. J. Harrison, P. F. Latham, T. E. Band, H. R. Dasu, S. Pan, Y. Prepost, R. Wu, S. L. CA BaBar Collaboration TI Study of the e(+)e(-) -> K+K- reaction in the energy range from 2.6 to 8.0 GeV SO PHYSICAL REVIEW D LA English DT Article ID BABAR DETECTOR; QUANTUM CHROMODYNAMICS; RADIATIVE-CORRECTIONS; EXCLUSIVE PROCESSES; E&E ANNIHILATION; PAIR PRODUCTION; NEUTRAL KAON; FORM-FACTORS; MESONS; COLLISIONS AB The e(+)e(-) -> K+K- cross section and charged-kaon electromagnetic form factor are measured in the e(+)e(-) center-of-mass energy range (E) from 2.6 to 8.0 GeV using the initial-state radiation technique with an undetected photon. The study is performed using 469 fb(-1) of data collected with the BABAR detector at the PEP-II2 e(+)e(-) collider at center-of-mass energies near 10.6 GeV. The form factor is found to decrease with energy faster than 1/E-2 and approaches the asymptotic QCD prediction. Production of the K+K- final state through the J/psi and psi(2S) intermediate states is observed. The results for the kaon form factor are used together with data from other experiments to perform a model-independent determination of the relative phases between electromagnetic (single-photon) and strong amplitudes in J/psi and psi(2S). K+K- decays. The values of the branching fractions measured in the reaction e(+)e(-) -> K+K- are shifted relative to their true values due to interference between resonant and nonresonant amplitudes. The values of these shifts are determined to be about +/- 5% for the J/psi meson and +/- 15% for the psi(2S) meson. C1 [Lees, J. P.; Poireau, V.; Tisserand, V.] Univ Savoie, CNRS IN2P3, LAPP, F-74941 Annecy Le Vieux, France. [Grauges, E.] Univ Barcelona, Fac Fis, Dept ECM, E-08028 Barcelona, Spain. [Palano, A.; Buzykaev, A. R.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Palano, A.] Univ Bari, Dipartimento Fis, I-70126 Bari, Italy. [Eigen, G.; Stugu, B.] Univ Bergen, Inst Phys, N-5007 Bergen, Norway. [Brown, D. N.; Kerth, L. T.; Kolomensky, Yu. 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[Lanceri, L.; Vitale, L.] Univ Trieste, Dipartimento Fis, I-34127 Trieste, Italy. [Martinez-Vidal, F.; Oyanguren, A.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain. [Albert, J.; Banerjee, Sw.; Beaulieu, A.; Bernlochner, F. U.; Choi, H. H. F.; King, G. J.; Kowalewski, R.; Lewczuk, M. J.; Lueck, T.; Nugent, I. M.; Roney, J. M.; Sobie, R. J.; Tasneem, N.] Univ Victoria, Victoria, BC V8W 3P6, Canada. [Gershon, T. J.; Harrison, P. F.; Latham, T. E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Band, H. R.; Dasu, S.; Pan, Y.; Prepost, R.; Wu, S. L.] Univ Wisconsin, Madison, WI 53706 USA. RP Lees, JP (reprint author), Univ Savoie, CNRS IN2P3, LAPP, F-74941 Annecy Le Vieux, France. RI Patrignani, Claudia/C-5223-2009; Morandin, Mauro/A-3308-2016; Lusiani, Alberto/A-3329-2016; Kravchenko, Evgeniy/F-5457-2015; Di Lodovico, Francesca/L-9109-2016; Calcaterra, Alessandro/P-5260-2015; Rizzo, Giuliana/A-8516-2015 OI Patrignani, Claudia/0000-0002-5882-1747; Morandin, Mauro/0000-0003-4708-4240; Lusiani, Alberto/0000-0002-6876-3288; Di Lodovico, Francesca/0000-0003-3952-2175; Calcaterra, Alessandro/0000-0003-2670-4826; Bettarini, Stefano/0000-0001-7742-2998; Cibinetto, Gianluigi/0000-0002-3491-6231; Rizzo, Giuliana/0000-0003-1788-2866 FU SLAC; U.S. Department of Energy; National Science Foundation; Natural Sciences and Engineering Research Council (Canada); Commissariat a l'Energie Atomique (France); Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung (Germany); Deutsche Forschungsgemeinschaft (Germany); Istituto Nazionale di Fisica Nucleare (Italy); Foundation for Fundamental Research on Matter (Netherlands); Research Council of Norway; Ministry of Education and Science of the Russian Federation; Ministerio de Economia y Competitividad (Spain); Science and Technology Facilities Council (United Kingdom); Binational Science Foundation (U.S.-Israel); Marie-Curie IEF program (European Union); A. P. Sloan Foundation (USA) FX We thank V. L. Chernyak for useful discussions. We are grateful for the extraordinary contributions of our PEP-II2 colleagues in achieving the excellent luminosity and machine conditions that have made this work possible. The success of this project also relies critically on the expertise and dedication of the computing organizations that support BABAR. The collaborating institutions wish to thank SLAC for its support and the kind hospitality extended to them. This work is supported by the U.S. Department of Energy and National Science Foundation, the Natural Sciences and Engineering Research Council (Canada), the Commissariat a l'Energie Atomique and Institut National de Physique Nucleaire et de Physique des Particules (France), the Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany), the Istituto Nazionale di Fisica Nucleare (Italy), the Foundation for Fundamental Research on Matter (Netherlands), the Research Council of Norway, the Ministry of Education and Science of the Russian Federation, Ministerio de Economia y Competitividad (Spain), the Science and Technology Facilities Council (United Kingdom), and the Binational Science Foundation (U.S.-Israel). Individuals have received support from the Marie-Curie IEF program (European Union) and the A. P. Sloan Foundation (USA). NR 39 TC 2 Z9 2 U1 0 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 20 PY 2015 VL 92 IS 7 AR 072008 DI 10.1103/PhysRevD.92.072008 PG 16 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CT7SN UT WOS:000363014900002 ER PT J AU Qiu, DY Cao, T Louie, SG AF Qiu, Diana Y. Cao, Ting Louie, Steven G. TI Nonanalyticity, Valley Quantum Phases, and Lightlike Exciton Dispersion in Monolayer Transition Metal Dichalcogenides: Theory and First-Principles Calculations SO PHYSICAL REVIEW LETTERS LA English DT Article ID QUASI-PARTICLE; MOS2; STATES; SEMICONDUCTORS; POLARIZATION; DISULFIDE; ENERGY; MASS AB Exciton dispersion as a function of center-of-mass momentum Q is essential to the understanding of exciton dynamics. We use the ab initio GW-Bethe-Salpeter equation method to calculate the dispersion of excitons in monolayer MoS2 and find a nonanalytic lightlike dispersion. This behavior arises from an unusual vertical bar Q vertical bar-term in both the intra- and intervalley exchange of the electron-hole interaction, which concurrently gives rise to a valley quantum phase of winding number two. A simple effective Hamiltonian to Q(2) order with analytic solutions is derived to describe quantitatively these behaviors. C1 [Qiu, Diana Y.; Cao, Ting; Louie, Steven G.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Qiu, Diana Y.; Cao, Ting; Louie, Steven G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Qiu, DY (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM sglouie@berkeley.edu FU Theory Program; U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [DMR15-1508412, ACI-1053575]; NSF Graduate Research Fellowship [DGE 1106400]; Office of Science of the U.S. Department of Energy; Extreme Science and Engineering Discovery Environment (XSEDE) FX We thank F. H. Jornada, F. Bruneval, J. Deslippe, and T. Rangel for fruitful discussions. This research was supported by the Theory Program (which provided the GW-BSE calculations and simulations) and by the SciDAC Program on Excited State Phenomena in Energy Materials (which provided the finite momentum exciton codes) at the Lawrence Berkeley National Lab through the Office of Basic Energy Sciences, U.S. Department of Energy under Contract No. DE-AC02-05CH11231, and by the National Science Foundation under Grant No. DMR15-1508412 (which provided the formulation of the effective Hamiltonian theory). D. Y. Q. acknowledges support from the NSF Graduate Research Fellowship Grant No. DGE 1106400. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy, and the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by National Science Foundation Grant No. ACI-1053575. NR 34 TC 21 Z9 21 U1 5 U2 33 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 20 PY 2015 VL 115 IS 17 AR 176801 DI 10.1103/PhysRevLett.115.176801 PG 5 WC Physics, Multidisciplinary SC Physics GA CT7VX UT WOS:000363023700013 PM 26551134 ER PT J AU Sotty, C Zielinska, M Georgiev, G Balabanski, DL Stuchbery, AE Blazhev, A Bree, N Chevrier, R Das Gupta, S Daugas, JM Davinson, T De Witte, H Diriken, J Gaffney, LP Geibel, K Hadynska-Klek, K Kondev, FG Konki, J Kroll, T Morel, P Napiorkowski, P Pakarinen, J Reiter, P Scheck, M Seidlitz, M Siebeck, B Simpson, G Tornqvist, H Warr, N Wenander, F AF Sotty, C. Zielinska, M. Georgiev, G. Balabanski, D. L. Stuchbery, A. E. Blazhev, A. Bree, N. Chevrier, R. Das Gupta, S. Daugas, J. M. Davinson, T. De Witte, H. Diriken, J. Gaffney, L. P. Geibel, K. Hadynska-Klek, K. Kondev, F. G. Konki, J. Kroell, T. Morel, P. Napiorkowski, P. Pakarinen, J. Reiter, P. Scheck, M. Seidlitz, M. Siebeck, B. Simpson, G. Toernqvist, H. Warr, N. Wenander, F. TI Rb-37(97)60: The Cornerstone of the Region of Deformation around A similar to 100 SO PHYSICAL REVIEW LETTERS LA English DT Article ID NEUTRON-RICH NUCLEI; FISSION FRAGMENTS; DETECTOR; MOMENTS; ZR-100; STATES AB Excited states of the neutron-rich nuclei Rb-97,Rb- 99 were populated for the first time using the multistep Coulomb excitation of radioactive beams. Comparisons of the results with particle-rotor model calculations provide clear identification for the ground-state rotational band of Rb-97 as being built on the pi g(9/2) [431] 3/2(+) Nilsson-model configuration. The ground-state excitation spectra of the Rb isotopes show a marked distinction between single-particle-like structures below N = 60 and rotational bands above. The present study defines the limits of the deformed region around A similar to 100 and indicates that the deformation of Rb-97 is essentially the same as that observed well inside the deformed region. It further highlights the power of the Coulomb-excitation technique for obtaining spectroscopic information far from stability. The Rb-99 case demonstrates the challenges of studies with very short-lived postaccelerated radioactive beams. C1 [Sotty, C.; Georgiev, G.] Univ Paris 11, CSNSM, CNRS IN2P3, UMR8609, F-91405 Orsay, France. [Sotty, C.; Bree, N.; De Witte, H.; Diriken, J.; Gaffney, L. P.] Katholieke Univ Leuven, Inst Kern & Stralingsfys, B-3001 Heverlee, Belgium. [Zielinska, M.; Hadynska-Klek, K.; Napiorkowski, P.] Univ Warsaw, Heavy Ion Lab, PL-02093 Warsaw, Poland. [Zielinska, M.] CEA Saclay, IRFU SPhN, F-91191 Gif Sur Yvette, France. [Balabanski, D. L.] IFIN HH, ELI NP, Bucharest 077125, Magurele, Romania. [Stuchbery, A. E.] Australian Natl Univ, Dept Nucl Phys, RSPE, Canberra, ACT 2601, Australia. [Blazhev, A.; Geibel, K.; Reiter, P.; Seidlitz, M.; Siebeck, B.; Warr, N.] Univ Cologne, Inst Nucl Phys, D-50937 Cologne, Germany. [Chevrier, R.; Daugas, J. M.; Morel, P.] DIF, DAM, CEA, F-91297 Arpajon, France. [Das Gupta, S.] Univ Camerino, Dipartimento Fis, I-62032 Camerino, Italy. [Das Gupta, S.] Ist Nazl Fis Nucl, Sez Perugia, I-06123 Perugia, Italy. [Davinson, T.] Univ Edinburgh, Dept Phys & Astron, Edinburgh EH9 3JZ, Midlothian, Scotland. [Diriken, J.] CEN SCK, Belgian Nucl Res Ctr, B-2400 Mol, Belgium. [Gaffney, L. P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 7ZE, Merseyside, England. [Kondev, F. G.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. [Konki, J.; Pakarinen, J.; Toernqvist, H.; Wenander, F.] CERN, ISOLDE, CH-1211 Geneva 23, Switzerland. [Konki, J.; Pakarinen, J.] Univ Jyvaskyla, Dept Phys, FI-40351 Jyvaskyla, Finland. [Konki, J.; Pakarinen, J.] Univ Helsinki, Helsinki Inst Phys, FI-00014 Helsinki, Finland. [Kroell, T.; Scheck, M.] Tech Univ Darmstadt, Inst Kernphys, D-64289 Darmstadt, Germany. [Simpson, G.] Univ Grenoble 1, LPSC, CNRS IN2P3, INPG, F-38026 Grenoble, France. [Gaffney, L. P.; Scheck, M.] Univ West Scotland, Paisley PA1 2BE, Renfrew, Scotland. [Gaffney, L. P.; Scheck, M.] Scottish Univ Phys Alliance, SUPA, Glasgow G12 8QQ, Lanark, Scotland. RP Georgiev, G (reprint author), Univ Paris 11, CSNSM, CNRS IN2P3, UMR8609, F-91405 Orsay, France. EM Georgi.Georgiev@csnsm.in2p3.fr RI Georgiev, Georgi/C-5110-2008; Gaffney, Liam/G-3169-2014 OI Georgiev, Georgi/0000-0003-1467-1764; Gaffney, Liam/0000-0002-2938-3696 FU European Union [262010]; German BMBF [06KY9136I, 05P12PKFNE, 05P15PKCIA, 06DA9036I, 05P12RDCIA, 05P15RDCIA]; U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357] FX This work was supported by the European Union Seventh Framework through ENSAR (Contract No. 262010), and the German BMBF under Contracts No. 06KY9136I, No. 05P12PKFNE, No. 05P15PKCIA, No. 06DA9036I, No. 05P12RDCIA, and No. 05P15RDCIA. Work at ANL is supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics under Contract No. DE-AC02-06CH11357. NR 34 TC 6 Z9 6 U1 4 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 20 PY 2015 VL 115 IS 17 AR 172501 DI 10.1103/PhysRevLett.115.172501 PG 6 WC Physics, Multidisciplinary SC Physics GA CT7VX UT WOS:000363023700005 PM 26551106 ER PT J AU Squire, J Bhattacharjee, A AF Squire, J. Bhattacharjee, A. TI Generation of Large-Scale Magnetic Fields by Small-Scale Dynamo in Shear Flows SO PHYSICAL REVIEW LETTERS LA English DT Article ID NUMBERS; ELECTRODYNAMICS; TURBULENCE AB We propose a new mechanism for a turbulent mean-field dynamo in which the magnetic fluctuations resulting from a small-scale dynamo drive the generation of large-scale magnetic fields. This is in stark contrast to the common idea that small-scale magnetic fields should be harmful to large-scale dynamo action. These dynamos occur in the presence of a large-scale velocity shear and do not require net helicity, resulting from off-diagonal components of the turbulent resistivity tensor as the magnetic analogue of the "shear-current" effect. Given the inevitable existence of nonhelical small-scale magnetic fields in turbulent plasmas, as well as the generic nature of velocity shear, the suggested mechanism may help explain the generation of large-scale magnetic fields across a wide range of astrophysical objects. C1 [Squire, J.; Bhattacharjee, A.] Princeton Univ, Dept Astrophys Sci, Max Planck & Princeton Ctr Plasma Phys, Princeton, NJ 08543 USA. [Squire, J.; Bhattacharjee, A.] Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Squire, J.] CALTECH, TAPIR, Pasadena, CA 91125 USA. RP Squire, J (reprint author), Princeton Univ, Dept Astrophys Sci, Max Planck & Princeton Ctr Plasma Phys, Princeton, NJ 08543 USA. EM jsquire@caltech.edu FU Procter Fellowship at Princeton University; U.S. Department of Energy [DE-AC02-09-CH11466] FX This work was supported by a Procter Fellowship at Princeton University, and the U.S. Department of Energy Grant No. DE-AC02-09-CH11466. The authors would like to thank A. Schekochihin, J. Krommes, and I. Rogachevskii for enlightening discussion and useful suggestions, as well as G. Lesur for making the SNOOPY code freely available. NR 32 TC 6 Z9 7 U1 1 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 20 PY 2015 VL 115 IS 17 AR 175003 DI 10.1103/PhysRevLett.115.175003 PG 5 WC Physics, Multidisciplinary SC Physics GA CT7VX UT WOS:000363023700009 PM 26551120 ER PT J AU Niu, KY Frolov, T Xin, HL Wang, JL Asta, M Zheng, HM AF Niu, Kaiyang Frolov, Timofey Xin, Huolin L. Wang, Junling Asta, Mark Zheng, Haimei TI Bubble nucleation and migration in a lead-iron hydr(oxide) core-shell nanoparticle SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE bubbles; nucleation; liquid cell; TEM; core-shell nanoparticle ID ELECTRON-IRRADIATION DAMAGE; RADIATION-INDUCED SHRINKAGE; GAS-BUBBLES; VOID FORMATION; BETA-FEOOH; MICROSCOPY; LIQUID; MOLYBDENUM; METALS; GROWTH AB Iron hydroxide is found in a wide range of contexts ranging from biominerals to steel corrosion, and it can transform to anhydrous oxide via releasing O-2 gas and H2O. However, it is not well understood how gases transport through a crystal lattice. Here, we present in situ observation of the nucleation and migration of gas bubbles in iron (hydr)oxide using transmission electron microscopy. We create Pb-FeOOH model core-shell nanoparticles in a liquid cell. Under electron irradiation, iron hydroxide transforms to iron oxide, during which bubbles are generated, and they migrate through the shell to the nanoparticle surface. Geometric phase analysis of the shell lattice shows an inhomogeneous stain field at the bubbles. Our modeling suggests that the elastic interaction between the core and the bubble provides a driving force for bubble migration. C1 [Niu, Kaiyang; Xin, Huolin L.; Zheng, Haimei] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. [Frolov, Timofey; Asta, Mark; Zheng, Haimei] Univ Calif Berkeley, Dept Mat Sci & Engn, Mat Sci Div, Berkeley, CA 94720 USA. [Wang, Junling] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore. RP Zheng, HM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. EM hmzheng@lbl.gov RI WANG, Junling/B-3596-2009; Xin, Huolin/E-2747-2010; OI WANG, Junling/0000-0003-3663-7081; Xin, Huolin/0000-0002-6521-868X; Niu, Kaiyang/0000-0003-3289-1322 FU US Department of Energy (DOE) Basic Energy Sciences [DE-AC02-05CH11231]; University of California (UC), Berkeley; National Research Foundation of Singapore [NRF-CRP5-2009-04]; DOE Office of Science Early Career Research Program FX We acknowledge the facility support of National Center for Electron Microscopy of the Molecular Foundry at Lawrence Berkeley National Laboratory, which is funded by US Department of Energy (DOE) Basic Energy Sciences with Contract DE-AC02-05CH11231. T.F. was supported by a Miller Fellowship of University of California (UC), Berkeley. J.W. acknowledges the funding support of National Research Foundation of Singapore under Project NRF-CRP5-2009-04. H.Z. acknowledges the travel support of SinBeRise BEARS UC Berkeley. H.Z. thanks the support of DOE Office of Science Early Career Research Program. NR 55 TC 2 Z9 2 U1 5 U2 36 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 20 PY 2015 VL 112 IS 42 BP 12928 EP 12932 DI 10.1073/pnas.1510342112 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CT9LN UT WOS:000363138600026 PM 26438864 ER PT J AU Gupta, RK Candler, J Palchoudhury, S Ramasamy, K Gupta, BK AF Gupta, Ram K. Candler, John Palchoudhury, Soubantika Ramasamy, Karthik Gupta, Bipin Kumar TI Flexible and High Performance Supercapacitors Based on NiCo(2)O(4)for Wide Temperature Range Applications SO SCIENTIFIC REPORTS LA English DT Article ID SOLID-STATE SUPERCAPACITORS; HYDROTHERMAL SYNTHESIS; ASYMMETRIC SUPERCAPACITORS; ELECTROCHEMICAL CAPACITORS; ELECTRODE MATERIALS; ENERGY-STORAGE; NICO2O4 NANOSTRUCTURES; OXIDE NANOCOMPOSITE; RUO2 NANOPARTICLES; ARRAYS AB Binder free nanostructured NiCo2O4 were grown using a facile hydrothermal technique. X-ray diffraction patterns confirmed the phase purity of NiCo2O4. The surface morphology and microstructure of the NiCo2O4 analyzed by scanning electron microscopy (SEM) showed flower-like morphology composed of needle-like structures. The potential application of binder free NiCo2O4 as an electrode for supercapacitor devices was investigated using electrochemical methods. The cyclic voltammograms of NiCo2O4 electrode using alkaline aqueous electrolytes showed the presence of redox peaks suggesting pseudocapacitance behavior. Quasi-solid state supercapacitor device fabricated by sandwiching two NiCo2O4 electrodes and separating them by ion transporting layer. The performance of the device was tested using cyclic voltammetry, galvanostatic charge-discharge and electrochemical impedance spectroscopy. The device showed excellent flexibility and cyclic stability. The temperature dependent charge storage capacity was measured for their variable temperature applications. Specific capacitance of the device was enhanced by similar to 150% on raising the temperature from 20 to 60 degrees C. Hence, the results suggest that NiCo2O4 grown under these conditions could be a suitable material for high performance supercapacitor devices that can be operated at variable temperatures. C1 [Gupta, Ram K.; Candler, John] Pittsburg State Univ, Dept Chem, Pittsburg, KS 66762 USA. [Palchoudhury, Soubantika] Univ Alabama, Ctr Mat Informat Technol, Tuscaloosa, AL 35487 USA. [Ramasamy, Karthik] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Albuquerque, NM 87545 USA. [Gupta, Bipin Kumar] Natl Phys Lab, CSIR, New Delhi 110012, India. RP Gupta, RK (reprint author), Pittsburg State Univ, Dept Chem, 1701 S Broadway, Pittsburg, KS 66762 USA. EM ramguptamsu@gmail.com FU Polymer Chemistry Initiative, Pittsburg State University; National Science Foundation [EPS-0903806] FX Synthesis, device fabrication, XRD and electrochemical measurements were carried out at Pittsburg State University. Dr. Ram K. Gupta expresses his sincere acknowledgment to the Polymer Chemistry Initiative, Pittsburg State University for providing financial and research support. This material is based upon work supported by the National Science Foundation under Award No. EPS-0903806 and matching support from the State of Kansas through the Kansas Board of Regents. SEM and TEM characterizations were done at the University of Alabama by Dr. Palchoudhury. NR 62 TC 10 Z9 10 U1 9 U2 95 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 20 PY 2015 VL 5 AR 15265 DI 10.1038/srep15265 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CT7XZ UT WOS:000363030200001 PM 26482921 ER PT J AU Lu, Y Cueva, MC Lara-Curzio, E Ozcan, S AF Lu, Yuan Cueva, Mario Calderon Lara-Curzio, Edgar Ozcan, Soydan TI Improved mechanical properties of polylactide nanocomposites-reinforced with cellulose nanofibrils through interfacial engineering via amine-functionalization SO CARBOHYDRATE POLYMERS LA English DT Article DE Polylactide; Cellulose nanofibrils; Silylation; PAMAM; Aminolysis ID MICROFIBRILLATED CELLULOSE; BIOMEDICAL APPLICATIONS; POLYMER NANOCOMPOSITES; POLY(LACTIC ACID); CARBON NANOTUBES; COMPOSITES; MORPHOLOGY; WHISKERS; SURFACE; NANOCELLULOSE AB One of the main factors responsible for the mechanical and physical properties of nanocomposites is the effectiveness of the interfacial region to transfer loads and mechanical vibrations between the nano-reinforcements and the matrix. Surface functionalization has been the preferred approach to engineer the interfaces in polymer nanocomposites in order to maximize their potential in structural and functional applications. In this study, amine-functionalized cellulose nanofibrils (mCNF-G1) were synthesized via silylation of the hydroxyl groups on the CNF surface using 3-aminopropyltrimethoxysilane (APTMS). To further increase the amine density (mCNF-G2), dendritic polyamidoamine (PAMAM) was grafted onto mCNF-G1 by the Michael addition of methacrylate onto mCNF-G1, followed by the transamidation of the ester groups of methacrylate using ethylenediamine. Compared to native CNF-reinforced, poly(L-lactide) (PLLA) nanocomposites, amine-functionalized CNF exhibited significantly improved dispersion and interfacial properties within the PLLA matrix due to the grafting of PLLA chains via aminolysis. It is also a more effective nucleating agent, with 15% mCNF-G1 leading to a crystallinity of 32.5%, compared to 0.1 and 8.7% for neat PLLA and native CNF-reinforced composites. We have demonstrated that APTMS-functionalized CNF (mCNF-G1) significantly improved the tensile strength compared to native CNF, with 10% mCNF-G1 being the most effective (i.e., >100% increase in tensile strength). However, we also found that excessive amines on the CNF surface (i.e., mCNF-G2) resulted in decreased tensile strength and modulus due to PLLA degradation via aminolysis. These results demonstrate the potential of optimized amine-functionalized CNF for future renewable material applications. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Lu, Yuan; Lara-Curzio, Edgar; Ozcan, Soydan] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Cueva, Mario Calderon] Univ San Francisco Quito, Quito, Ecuador. RP Ozcan, S (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM ozcans@oml.gov OI Ozcan, Soydan/0000-0002-3825-4589 FU Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; U.S. Department of Energy [DE-AC05-00OR22725] FX The authors thank Rich R. Lowden for his assistance in the preparation of the experimental system for tensile testing. The authors gratefully acknowledge the generous assistance and valuable advice of Dr. Harry Meyer on XPS analysis. Thanks to the USDA Forest Service Forest Products Laboratory for providing cellulose nanomaterials as well as information on the properties of cellulosic nanomaterials. This research was sponsored by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy. This article has been authored by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The US government retains and the publisher, by accepting the article for publication, acknowledges that the US government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for US government purposes. NR 52 TC 3 Z9 3 U1 10 U2 81 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0144-8617 EI 1879-1344 J9 CARBOHYD POLYM JI Carbohydr. Polym. PD OCT 20 PY 2015 VL 131 BP 208 EP 217 DI 10.1016/j.carbpol.2015.05.047 PG 10 WC Chemistry, Applied; Chemistry, Organic; Polymer Science SC Chemistry; Polymer Science GA CR2TN UT WOS:000361183600025 PM 26256177 ER PT J AU Santamaria, AD Becton, MK Cooper, NJ Weber, AZ Park, JW AF Santamaria, Anthony D. Becton, Maxwell K. Cooper, Nathanial J. Weber, Adam Z. Park, Jae Wan TI Effect of cross-flow on PEFC liquid-water distribution: An in-situ high-resolution neutron radiography study SO JOURNAL OF POWER SOURCES LA English DT Article DE Fuel cells; Neutron radiography; Permeability; Liquid-water saturation; Gas-diffusion layer; Cross-flow; Breakthrough pressure ID PEM FUEL-CELL; GAS-DIFFUSION-LAYER; POLYMER-ELECTROLYTE; MEMBRANE; TRANSPORT; FIELD; VISUALIZATION; PERFORMANCE; MANAGEMENT; PROFILES AB Liquid-water management in polymer-electrolyte fuel cells (PEFCs) remains an area of ongoing research. To enhance water removal, certain flow-fields induce cross-flow, or flow through the gas-diffusion layer (GDL) via channel-to-channel pressure differences. While beneficial to water removal, cross-flow comes at the cost of higher pumping pressures and may lead to membrane dehydration and other deleterious issues. This paper examines the impact of cross-flow on component saturation levels as determined through in-plane high-resolution neutron radiography. Various humidities and operating conditions are examined, and the results demonstrate that cell saturation levels correlate strongly with the level of cross-flow rate, and lower GDL saturation levels are found to correlate with an increase in permeability at higher flow rates. Effective water removal is found to occur at channel-to-channel pressure gradients greater than the measured breakthrough pressure of the GDL, evidence that similar liquid-water transport mechanisms exist for under-land area transport as in transverse GDL flow. (C) 2015 Elsevier B.V. All rights reserved. C1 [Santamaria, Anthony D.] Western New England Univ, Dept Mech Engn, Springfield, MA 01119 USA. [Becton, Maxwell K.; Cooper, Nathanial J.; Park, Jae Wan] Univ Calif Davis, Dept Mech & Aerosp Engn, Davis, CA 95616 USA. [Weber, Adam Z.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Park, JW (reprint author), Univ Calif Davis, Dept Mech & Aerosp Engn, Davis, CA 95616 USA. EM jwpark@ucdavis.edu FU Research and Development Program of the Korea Institute of Energy Research (KIER) [B3-2413-01] FX The authors would like to acknowledge Dr. Daniel S. Hussey, Dr. David L. Jacobson, and Elias M. Baltic for their help in organizing and carrying out the neutron imaging at NIST. This research is supported by the Research and Development Program of the Korea Institute of Energy Research (KIER) (B3-2413-01). NR 37 TC 7 Z9 7 U1 5 U2 27 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD OCT 20 PY 2015 VL 293 BP 162 EP 169 DI 10.1016/j.jpowsour.2015.05.016 PG 8 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA CN9ZM UT WOS:000358809700021 ER PT J AU Crawford, A Viswanathan, V Stephenson, D Wang, W Thomsen, E Reed, D Li, B Balducci, P Kintner-Meyer, M Sprenkle, V AF Crawford, Alasdair Viswanathan, Vilayanur Stephenson, David Wang, Wei Thomsen, Edwin Reed, David Li, Bin Balducci, Patrick Kintner-Meyer, Michael Sprenkle, Vincent TI Comparative analysis for various redox flow batteries chemistries using a cost performance model SO JOURNAL OF POWER SOURCES LA English DT Article DE Cost; Performance; Flow; Interdigitated; Energy; Power AB The total energy storage system cost is determined by means of a robust performance-based cost model for multiple flow battery chemistries. Systems aspects such as shunt current losses, pumping losses and various flow patterns through electrodes are accounted for. The system cost minimizing objective function determines stack design by optimizing the state of charge operating range, along with current density and current-normalized flow. The model cost estimates are validated using 2-kW stack performance data for the same size electrodes and operating conditions. Using our validated tool, it has been demonstrated that an optimized all-vanadium system has an estimated system cost of < $350 kWh(-1) for 4-h application. With an anticipated decrease in component costs facilitated by economies of scale from larger production volumes, coupled with performance improvements enabled by technology development, the system cost is expected to decrease to 160 kWh(-1) for a 4-h application, and to $100 kWh(-1) for a 10-h application. This tool has been shared with the redox flow battery community to enable cost estimation using their stack data and guide future direction. (C) 2015 Elsevier B.V. All rights reserved. C1 [Crawford, Alasdair; Viswanathan, Vilayanur; Stephenson, David; Wang, Wei; Thomsen, Edwin; Reed, David; Li, Bin; Balducci, Patrick; Kintner-Meyer, Michael; Sprenkle, Vincent] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Viswanathan, V (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd,POB 999, Richland, WA 99352 USA. EM vilayanur.viswanathan@pnl.gov RI Wang, Wei/F-4196-2010 OI Wang, Wei/0000-0002-5453-4695 FU US DOE Office of Electricity Delivery and Energy Reliability (OE) [57558]; US DOE [DE-AC05-76RL01830] FX We acknowledge financial support from the US DOE Office of Electricity Delivery and Energy Reliability (OE) (Contract No. 57558) and the encouragement provided by Dr. Imre Gyuk, the OE Energy Storage and Power Electronics program manager. Valuable discussions with various redox flow battery companies that test drove our model and provided feedback is acknowledged. The authors acknowledge Dr. Lawrence Thaller, a private consultant, who provided the Fe-Cr reports and some of the component cost information for our earlier paper. We acknowledge the guidance provided by Dr. Liyu Li and Dr. Zhenguo Yang, currently at Uni-Energy Technologies, and the contribution of Dr. Soowhan Kim, currently at OCI Company Ltd., to our previous paper. Pacific Northwest National Laboratory is operated for the US DOE by Battelle under Contract DE-AC05-76RL01830. NR 27 TC 9 Z9 9 U1 4 U2 48 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD OCT 20 PY 2015 VL 293 BP 388 EP 399 DI 10.1016/j.jpowsour.2015.05.066 PG 12 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA CN9ZM UT WOS:000358809700047 ER PT J AU Patel, PP Datta, MK Jampani, PH Hong, D Poston, JA Manivannan, A Kumta, PN AF Patel, Prasad Prakash Datta, Moni Kanchan Jampani, Prashanth H. Hong, Daeho Poston, James A. Manivannan, Ayyakkannu Kumta, Prashant N. TI High performance and durable nanostructured TiN supported Pt-50-Ru-50 anode catalyst for direct methanol fuel cell (DMFC) SO JOURNAL OF POWER SOURCES LA English DT Article DE Direct methanol fuel cell; Methanol oxidation; Platinum; Ruthenium; Nanostructured support; Titanium nitride ID ELECTRO-CATALYSTS; TITANIUM NITRIDE; CARBON NANOTUBES; ENERGY-STORAGE; PLATINUM NANOPARTICLES; WATER ELECTROLYSIS; HALIDE APPROACH; OXIDATION; ELECTROOXIDATION; SURFACE AB The design of high performance and durable electro-catalyst has been of particular interest for DMFC anodes. Pt(Ru) has been considered the most active DMFC anode catalyst. In this work, the reaction kinetics of Pt(Ru) electro-catalyst has been improved by synthesizing high active surface area Pt-50(Ru-50) catalyst supported on highly conductive nanostructured titanium nitride, TiN. The Pt(Ru)/TiN has been synthesized by a complexed sal-gel (CSG) process using non-halide precursors of Pt and Ru. High surface area Pt(Ru)/TiN shows promising electrochemical performance for methanol oxidation, showing similar to 52% improved catalytic activity at similar to 0.65 V (vs NHE) and stability/durability in comparison with commercial JM-Pt(Ru). Single cell DMFC performance shows 56% improved maximum power density and superior electrochemical stability for CSG-Pt(Ru)/TiN compared to that of commercial JM-Pt(Ru). This is attributed to the uniform dispersion of Pt(Ru) achieved on the nanostructured TiN (support) yielding higher electrochemical active surface area and lower charge transfer resistance than commercial JM-Pt(Ru). Thus, the present study demonstrates the potential of nanostructured TiN as a support for Pt(Ru) based anode electro-catalyst for DMFC applications. (C) 2015 Elsevier B.V. All rights reserved. C1 [Patel, Prasad Prakash; Kumta, Prashant N.] Univ Pittsburgh, Swanson Sch Engn, Dept Chem & Petr Engn, Pittsburgh, PA 15261 USA. [Datta, Moni Kanchan; Jampani, Prashanth H.; Hong, Daeho; Kumta, Prashant N.] Univ Pittsburgh, Swanson Sch Engn, Dept Bioengn, Pittsburgh, PA 15261 USA. [Datta, Moni Kanchan; Kumta, Prashant N.] Univ Pittsburgh, Ctr Complex Engn Multifunct Mat, Pittsburgh, PA 15261 USA. [Poston, James A.; Manivannan, Ayyakkannu] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. [Kumta, Prashant N.] Univ Pittsburgh, Mech Engn & Mat Sci, Swanson Sch Engn, Pittsburgh, PA 15261 USA. [Kumta, Prashant N.] Univ Pittsburgh, Sch Dent Med, Pittsburgh, PA 15217 USA. RP Kumta, PN (reprint author), Dept Bioengn, 815C Benedum Hall,3700 OHara St, Pittsburgh, PA 15261 USA. EM pkumta@pitt.edu RI Jampani Hanumantha, Prashanth/A-9840-2013 OI Jampani Hanumantha, Prashanth/0000-0001-7159-1993 FU National Science Foundation, CBET [0933141]; Edward R. WeidleinChair Professorship funds; Center for Complex Engineered Multifunctional Materials (CCEMM) FX Research in part supported by the National Science Foundation, CBET - Grant 0933141. PNK also acknowledges the Edward R. WeidleinChair Professorship funds and the Center for Complex Engineered Multifunctional Materials (CCEMM) for support of this research and also for procurement of the electrochemical equipment and facilities used in this research work. NR 50 TC 17 Z9 17 U1 15 U2 108 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD OCT 20 PY 2015 VL 293 BP 437 EP 446 DI 10.1016/j.jpowsour.2015.05.051 PG 10 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA CN9ZM UT WOS:000358809700052 ER PT J AU Myung, ST Amine, K Sun, YK AF Myung, Seung-Taek Amine, Khalil Sun, Yang-Kook TI Nanostructured cathode materials for rechargeable lithium batteries ( vol 283, pg 219, 2015) SO JOURNAL OF POWER SOURCES LA English DT Correction C1 [Myung, Seung-Taek] Sejong Univ, Dept Nano Engn, Seoul 143747, South Korea. [Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA. [Sun, Yang-Kook] Hanyang Univ, Dept Energy Engn, Seoul 133791, South Korea. RP Myung, ST (reprint author), Sejong Univ, Dept Nano Engn, Seoul 143747, South Korea. EM smyung@sejong.ac.kr; amine@anl.gov; yksun@hanyang.ac.kr OI Myung, Seung-Taek/0000-0001-6888-5376 NR 1 TC 0 Z9 0 U1 5 U2 32 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD OCT 20 PY 2015 VL 293 BP 734 EP 734 DI 10.1016/j.jpowsour.2015.06.012 PG 1 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA CN9ZM UT WOS:000358809700086 ER PT J AU Xiao, L Chen, XL Cao, RG Qian, JF Xiang, HF Zheng, JM Zhang, JG Xu, W AF Xiao, Liang Chen, Xilin Cao, Ruiguo Qian, Jiangfeng Xiang, Hongfa Zheng, Jianming Zhang, Ji-Guang Xu, Wu TI Enhanced performance of Li vertical bar LiFePO4 cells using CsPF6 as an electrolyte additive SO JOURNAL OF POWER SOURCES LA English DT Article DE Lithium metal battery; Lithium dendrite suppression; Lithium protection; CsPF6 additive; Li vertical bar LiFePO4 cells ID ELECTROSTATIC SHIELD MECHANISM; FREE LITHIUM DEPOSITION; RECHARGEABLE BATTERIES; AIR BATTERIES; HIGH-ENERGY; PROMISE; ANODES AB The practical application of lithium (Li) metal anode in rechargeable Li batteries is hindered by both the growth of Li dendrites and the low Coulombic efficiency (CE) during repeated charge/discharge cycles. Recently, we have discovered that CsPF6 as an electrolyte additive can significantly suppress Li dendrite growth and lead to highly compacted and well aligned Li nanorod structures during Li deposition on copper substrates. In this paper, the effect of CsPF6 additive on the performance of rechargeable Li metal batteries with lithium iron phosphate (LFP) cathode is further studied. Li vertical bar LFP coin cells with CsPF6 additive in electrolytes show well protected Li anode surface, decreased resistance, enhanced rate capability and extended cycling stability. In Li vertical bar LFP cells, the electrolyte with CsPF6 additive shows excellent long-term cycling stability (at least 500 cycles) at a charge current density of 0.5 mA cm(-2) without internal short circuit. At high charge current densities, the effect of CsPF6 additive becomes less significant. Future work needs to be done to protect Li metal anode, especially at high charge current densities and for long cycle life. (C) 2015 Elsevier B.V. All rights reserved. C1 [Xiao, Liang; Chen, Xilin; Cao, Ruiguo; Qian, Jiangfeng; Xiang, Hongfa; Zheng, Jianming; Zhang, Ji-Guang; Xu, Wu] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99354 USA. [Xiao, Liang] Wuhan Univ Technol, Sch Chem Chem Engn & Life Sci, Wuhan 430070, Hubei, Peoples R China. [Xiang, Hongfa] Hefei Univ Technol, Sch Mat Sci & Engn, Hefei 230009, Anhui, Peoples R China. RP Zhang, JG (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99354 USA. EM jiguang.zhang@pnnl.gov; wu.xu@pnnl.gov RI Zheng, Jianming/F-2517-2014; Cao, Ruiguo/O-7354-2016; Xiang, Hongfa/I-5126-2012 OI Zheng, Jianming/0000-0002-4928-8194; Xiang, Hongfa/0000-0002-6182-1932 FU China Scholarship Council for overseas studies [201208420238]; Fundamental Research Funds for the Central Universities [2014-Ia-031, 2013HGCH0002]; National Science Foundation of China [21006033, 51372060] FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, of the U. S. Department of Energy (DOE) as part of Battery Materials Research (BMR) program. The authors thanked Dr. Eduard Nasybulin for helping in the SEM measurements. Dr. Liang Xiao was grateful for a scholarship from the China Scholarship Council for overseas studies (No. 201208420238) and the support from the Fundamental Research Funds for the Central Universities (No. 2014-Ia-031). Dr. Hongfa Xiang also acknowledged the financial support from National Science Foundation of China (Grant Nos. 21006033 and 51372060) and the Fundamental Research Funds for the Central Universities (2013HGCH0002). NR 17 TC 3 Z9 3 U1 13 U2 77 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD OCT 20 PY 2015 VL 293 BP 1062 EP 1067 DI 10.1016/j.jpowsour.2015.06.044 PG 6 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA CN9ZM UT WOS:000358809700122 ER PT J AU Brumm, P Land, ML Hauser, LJ Jeffries, CD Chang, YJ Mead, DA AF Brumm, Phillip Land, Miriam L. Hauser, Loren J. Jeffries, Cynthia D. Chang, Yun-Juan Mead, David A. TI Complete genome sequences of Geobacillus sp Y412MC52, a xylan-degrading strain isolated from obsidian hot spring in Yellowstone National Park SO STANDARDS IN GENOMIC SCIENCES LA English DT Article DE Geobacillus sp Y412MC52; Obsidian hot spring; Biomass; Arabinan; Xylan; G. thermocatenulatus ID LINE DATABASE GOLD; SP-NOV; THERMUS-AQUATICUS; EXTREME THERMOPHILE; RNA GENES; BACILLUS; GENUS; STEAROTHERMOPHILUS; IDENTIFICATION; PROPOSAL AB Geobacillus sp. Y412MC52 was isolated from Obsidian Hot Spring, Yellowstone National Park, Montana, USA under permit from the National Park Service. The genome was sequenced, assembled, and annotated by the DOE Joint Genome Institute and deposited at the NCBI in December 2011 (CP002835). Based on 16S rRNA genes and average nucleotide identity, Geobacillus sp. Y412MC52 and the related Geobacillus sp. Y412MC61 appear to be members of a new species of Geobacillus. The genome of Geobacillus sp. Y412MC52 consists of one circular chromosome of 3,628,883 bp, an average G + C content of 52 % and one circular plasmid of 45,057 bp and an average G + C content of 45 %. Y412MC52 possesses arabinan, arabinoglucuronoxylan, and aromatic acid degradation clusters for degradation of hemicellulose from biomass. Transport and utilization clusters are also present for other carbohydrates including starch, cellobiose, and alpha- and beta-galactooligosaccharides. C1 [Brumm, Phillip] C5 6 Technol Inc, Middleton, WI 53562 USA. [Land, Miriam L.; Hauser, Loren J.] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Jeffries, Cynthia D.; Chang, Yun-Juan] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM USA. [Mead, David A.] Lucigen Corp, Middleton, WI USA. RP Brumm, P (reprint author), C5 6 Technol Inc, Middleton, WI 53562 USA. EM pbrumm@c56technologies.com RI Land, Miriam/A-6200-2011 OI Land, Miriam/0000-0001-7102-0031 FU DOE Great Lakes Bioenergy Research Center (DOE Office of Science BER) [DE-FC02-07ER64494]; US Department of Energy's Office of Science, Biological and Environmental Research Program; University of California, Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Los Alamos National Laboratory [DE-AC02-06NA25396] FX This work was funded by the DOE Great Lakes Bioenergy Research Center (DOE Office of Science BER DE-FC02-07ER64494). Sequencing work was performed under the auspices of the US Department of Energy's Office of Science, Biological and Environmental Research Program, and by the University of California, Lawrence Berkeley National Laboratory under contract No. DE-AC02-05CH11231, Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344, and Los Alamos National Laboratory under contract No. DE-AC02-06NA25396. NR 51 TC 2 Z9 2 U1 3 U2 7 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD OCT 19 PY 2015 VL 10 DI 10.1186/s40793-015-0075-0 PG 9 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DA7QS UT WOS:000367999700001 ER PT J AU Daniels, MW Guo, W Stocks, GM Xiao, D Xiao, J AF Daniels, Matthew W. Guo, Wei Stocks, G. Malcolm Xiao, Di Xiao, Jiang TI Spin-transfer torque induced spin waves in antiferromagnetic insulators SO NEW JOURNAL OF PHYSICS LA English DT Article DE spintronics; antiferromagnetism; magnonics; magnon; antiferromagnet; surface; spin-transfer torque ID HEISENBERG-ANTIFERROMAGNET; SPINTRONICS; SURFACE; GRAPHENE; NEUTRON AB We explore the possibility of exciting spin waves in insulating antiferromagnetic films by injecting spin current at the surface. We analyze both magnetically compensated and uncompensated interfaces. We find that the spin current induced spin-transfer torque can excite spin waves in insulating antiferromagnetic materials and that the chirality of the excited spin wave is determined by the polarization of the injected spin current. Furthermore, the presence of magnetic surface anisotropy can greatly increase the accessibility of these excitations. C1 [Daniels, Matthew W.; Xiao, Di] Carnegie Mellon Univ, Dept Phys, Pittsburgh, PA 15213 USA. [Guo, Wei; Xiao, Jiang] Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China. [Guo, Wei; Xiao, Jiang] Fudan Univ, State Key Lab Surface Phys, Shanghai 200433, Peoples R China. [Stocks, G. Malcolm] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Xiao, Jiang] Fudan Univ, Collaborat Innovat Ctr Adv Microstruct, Shanghai 200433, Peoples R China. RP Daniels, MW (reprint author), Carnegie Mellon Univ, Dept Phys, Pittsburgh, PA 15213 USA. EM dixiao@cmu.edu; xiaojiang@fudan.edu.cn RI Xiao, Di/B-1830-2008; Xiao, Jiang/B-1832-2008; Stocks, George Malcollm/Q-1251-2016; OI Xiao, Di/0000-0003-0165-6848; Xiao, Jiang/0000-0002-3245-3579; Stocks, George Malcollm/0000-0002-9013-260X; Daniels, Matthew/0000-0002-3390-4714 FU National Science Foundation, Office of Emerging Frontiers in Research and Innovation [EFRI-1433496]; US Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division (GMS); special funds for Major State Basic Research Project of China [2014CB921600, 2011CB925601]; National Natural Science Foundation of China [91121002] FX This work was supported by the National Science Foundation, Office of Emerging Frontiers in Research and Innovation EFRI-1433496 (MWD and DX), the US Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division (GMS), and by the special funds for the Major State Basic Research Project of China (grants No. 2014CB921600, No. 2011CB925601) and the National Natural Science Foundation of China (grant No. 91121002) (WG and JX). NR 39 TC 2 Z9 2 U1 4 U2 22 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD OCT 19 PY 2015 VL 17 AR 103039 DI 10.1088/1367-2630/17/10/103039 PG 10 WC Physics, Multidisciplinary SC Physics GA CZ8DP UT WOS:000367330600003 ER PT J AU Harilal, SS Yeak, J Phillips, MC AF Harilal, S. S. Yeak, J. Phillips, M. C. TI Plasma temperature clamping in filamentation laser induced breakdown spectroscopy SO OPTICS EXPRESS LA English DT Article ID TRANSPARENT MEDIA; ABLATION; AIR; PULSES; LIGHT; LIBS AB Ultrafast laser filament induced breakdown spectroscopy is a very promising method for remote material detection. We present characteristics of plasmas generated in a metal target by laser filaments in air. Our measurements show that the temperature of the ablation plasma is clamped along the filament channel due to intensity clamping in a filament. Nevertheless, significant changes in radiation intensity are noticeable, and this is essentially due to variation in the number density of emitting atoms. The present results also explain the near absence of ion emission but strong atomic neutral emission from plumes produced during fs LIBS in air. (C) 2015 Optical Society of America C1 [Harilal, S. S.; Phillips, M. C.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Yeak, J.] PM & AM Res LLC, Tucson, AZ 85719 USA. RP Harilal, SS (reprint author), Pacific NW Natl Lab, POB 999, Richland, WA 99352 USA. EM hari@pnnl.gov RI Harilal, Sivanandan/B-5438-2014 OI Harilal, Sivanandan/0000-0003-2266-7976 FU DOE/NNSA Office of Nonproliferation and Verification Research and Development [NA-22]; U.S. Department of Energy [DE-AC05-76RL01830] FX This work was supported by the DOE/NNSA Office of Nonproliferation and Verification Research and Development (NA-22). Pacific Northwest National Laboratory, a multi-program national laboratory operated by Battelle for the U.S. Department of Energy under Contract DE-AC05-76RL01830. The authors thank to Dr. Burt Beardsley for technical help as well as lending Echelle spectrograph and Dr. Bret D. Cannon for valuable discussions while preparing the manuscript. NR 28 TC 6 Z9 6 U1 2 U2 22 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD OCT 19 PY 2015 VL 23 IS 21 BP 27113 EP 27122 DI 10.1364/OE.23.027113 PG 10 WC Optics SC Optics GA CY7FR UT WOS:000366574400023 PM 26480372 ER PT J AU Van Nieuwenhove, V De Beenhouwer, J De Carlo, F Mancini, L Marone, F Sijbers, J AF Van Nieuwenhove, Vincent De Beenhouwer, Jan De Carlo, Francesco Mancini, Lucia Marone, Federica Sijbers, Jan TI Dynamic intensity normalization using eigen flat fields in X-ray imaging SO OPTICS EXPRESS LA English DT Article ID ELECTRON TOMOGRAPHY; RING ARTIFACTS; RECONSTRUCTIONS; ALGORITHM; REMOVAL AB In X-ray imaging, it is common practice to normalize the acquired projection data with averaged flat fields taken prior to the scan. Unfortunately, due to source instabilities, vibrating beamline components such as the monochromator, time varying detector properties, or other confounding factors, flat fields are often far from stationary, resulting in significant systematic errors in intensity normalization. In this work, a simple and efficient method is proposed to account for dynamically varying flat fields. Through principal component analysis of a set of flat fields, eigen flat fields are computed. A linear combination of the most important eigen flat fields is then used to individually normalize each X-ray projection. Experiments show that the proposed dynamic flat field correction leads to a substantial reduction of systematic errors in projection intensity normalization compared to conventional flat field correction. (C) 2015 Optical Society of America C1 [Van Nieuwenhove, Vincent; De Beenhouwer, Jan; Sijbers, Jan] Univ Antwerp, Dept Phys, iMinds Vis Lab, B-2020 Antwerp, Belgium. [De Carlo, Francesco] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Mancini, Lucia] Elettra Sincrotrone Trieste SCpA, Trieste, Italy. [Marone, Federica] Paul Scherrer Inst, Swiss Light Source, Villigen, Switzerland. RP Van Nieuwenhove, V (reprint author), Univ Antwerp, Dept Phys, iMinds Vis Lab, B-2020 Antwerp, Belgium. EM Vincent.VanNieuwenhove@uantwerpen.be RI Marone, Federica/J-4420-2013; Sijbers, Jan/H-4324-2015 OI Sijbers, Jan/0000-0003-4225-2487 FU SBO Tomfood project of the Agency for Innovation by Science and Technology in Flanders (IWT); iMinds ICON MetroCT project; EXTREMA COST Action [MP1207]; U.S. Department of Energy (DOE) Office of Science User Facility [DE-AC02-06CH11357] FX This work was supported by the SBO Tomfood project of the Agency for Innovation by Science and Technology in Flanders (IWT). The authors acknowledge financial support from the iMinds ICON MetroCT project. Networking support was provided by the EXTREMA COST Action MP1207. Finally, this research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 22 TC 3 Z9 3 U1 1 U2 2 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD OCT 19 PY 2015 VL 23 IS 21 BP 27975 EP 27989 DI 10.1364/OE.23.027975 PG 15 WC Optics SC Optics GA CY7FR UT WOS:000366574400107 PM 26480456 ER PT J AU Kubec, A Kujala, N Conley, R Bouet, N Zhou, J Mooney, TM Shu, DM Kirchman, J Goetze, K Maser, J Macrander, A AF Kubec, Adam Kujala, Naresh Conley, Raymond Bouet, Nathalie Zhou, Juan Mooney, Tim M. Shu, Deming Kirchman, Jeffrey Goetze, Kurt Maser, Joerg Macrander, Albert TI Diffraction properties of multilayer Laue lenses with an aperture of 102 mu m and WSi2/Al bilayers SO OPTICS EXPRESS LA English DT Article ID X-RAY; PERFORMANCE; FABRICATION AB We report on the characterization of a multilayer Laue lens (MLL) with large acceptance, made of a novel WSi2/Al bilayer system. Fabrication of multilayers with large deposition thickness is required to obtain MLL structures with sufficient apertures capable of accepting the full lateral coherence length of x-rays at typical nanofocusing beamlines. To date, the total deposition thickness has been limited by stress-buildup in the multilayer. We were able to grow WSi2/Al with low grown-in stress, and asses the degree of stress reduction. X-ray diffraction experiments were conducted at beamline 1-BM at the Advanced Photon Source. We used monochromatic x-rays with a photon energy of 12 keV and a bandwidth of Delta E/E = 5.4.10(-4). The MLL was grown with parallel layer interfaces, and was designed to have a large focal length of 9.6 mm. The mounted lens was 2.7 mm in width. We found and quantified kinks and bending of sections of the MLL. Sections with bending were found to partly have a systematic progression in the interface angles. We observed kinking in some, but not all, areas. The measurements are compared with dynamic diffraction calculations made with Coupled Wave Theory. Data are plotted showing the diffraction efficiency as a function of the external tilting angle of the entire mounted lens. This way of plotting the data was found to provide an overview into the diffraction properties of the whole lens, and enabled the following layer tilt analyses. (C) 2015 Optical Society of America C1 [Kubec, Adam; Kujala, Naresh; Conley, Raymond; Mooney, Tim M.; Shu, Deming; Kirchman, Jeffrey; Goetze, Kurt; Maser, Joerg; Macrander, Albert] Argonne Natl Lab, Xray Sci Div, Adv Photon Source, Argonne, IL 60439 USA. [Kubec, Adam] Fraunhofer IWS Dresden, D-01277 Dresden, Germany. [Kujala, Naresh] European XFEL GmbH, D-22761 Hamburg, Germany. [Conley, Raymond; Bouet, Nathalie; Zhou, Juan] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Kubec, A (reprint author), Argonne Natl Lab, Xray Sci Div, Adv Photon Source, Argonne, IL 60439 USA. EM adam.kubec@iws.fraunhofer.de OI Bouet, Nathalie/0000-0002-5816-9429 FU US Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357, DE-SC00112704]; European Union; Free State of Saxony via ESF project [100087859] FX This work was supported by the US Department of Energy, Office of Basic Energy Sciences, under contract No. DE-AC02-06CH11357 and the European Union and the Free State of Saxony via ESF project 100087859, ENano. Work carried out at National Synchrotron Light Source II and the Center for Functional Nanomaterials at Brookhaven National Laboratory was supported by the US Department of Energy, Office of Basic Energy Sciences, under contract No. DE-SC00112704. NR 30 TC 2 Z9 2 U1 2 U2 9 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD OCT 19 PY 2015 VL 23 IS 21 BP 27990 EP 27997 DI 10.1364/OE.23.027990 PG 8 WC Optics SC Optics GA CY7FR UT WOS:000366574400108 PM 26480457 ER PT J AU Theingi, S Guan, TY Kendrick, C Klafehn, G Gorman, BP Taylor, PC Lusk, MT Stradins, P Collins, RT AF Theingi, S. Guan, T. Y. Kendrick, C. Klafehn, G. Gorman, B. P. Taylor, P. C. Lusk, M. T. Stradins, P. Collins, R. T. TI Size dependence of the bandgap of plasma synthesized silicon nanoparticles through direct introduction of sulfur hexafluoride SO APPLIED PHYSICS LETTERS LA English DT Article ID MICROCRYSTALLINE SILICON; RAMAN-SPECTROSCOPY; LIGHT-EMISSION; QUANTUM DOTS; NANOCRYSTALS; PHOTOLUMINESCENCE; LUMINESCENCE; TRANSITIONS; EFFICIENCY; SPECTRUM AB Developing silicon nanoparticle (SiNP) synthesis techniques that allow for straightforward control of nanoparticle size and associated optical properties is critical to potential applications of these materials. In addition, it is, in general, hard to probe the absorption threshold in these materials due to silicon's low absorption coefficient. In this study, size is controlled through direct introduction of sulfur hexafluoride (SF6) into the dilute silane precursor of plasma synthesized SiNPs. Size reduction by nearly a factor of two with high crystallinity independent of size is demonstrated. The optical absorption spectra of the SiNPs in the vicinity of the bandgap are measured using photothermal deflection spectroscopy. Bandgap as a function of size is extracted taking into account the polydispersity of the samples. A systematic blue shift in absorption edge due to quantum confinement in the SiNPs is observed with increasing flow of SF6. Photoluminescence (PL) spectra show a similar blue shift with size. However, a similar to 300 meV difference in energy between emission and absorption for all sizes suggests that PL emission involves a defect related process. This shows that, while PL may allow size-induced shifts in the bandgap of SiNPs to be monitored, it cannot be relied on to give an accurate value for the bandgap as a function of size. (C) 2015 AIP Publishing LLC. C1 [Theingi, S.; Guan, T. Y.; Kendrick, C.; Klafehn, G.; Taylor, P. C.; Lusk, M. T.; Collins, R. T.] Colorado Sch Mines, Dept Phys, Golden, CO 80401 USA. [Theingi, S.; Guan, T. Y.; Kendrick, C.; Klafehn, G.; Taylor, P. C.; Lusk, M. T.; Stradins, P.; Collins, R. T.] Colorado Sch Mines, Renewable Energy Mat Res Sci & Engn Ctr, Golden, CO 80401 USA. [Kendrick, C.] Michigan Technol Univ, Elect & Comp Engn, Houghton, MI 49931 USA. [Gorman, B. P.] Colorado Sch Mines, Met & Mat Engn, Golden, CO 80401 USA. [Stradins, P.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Theingi, S (reprint author), Colorado Sch Mines, Dept Phys, Golden, CO 80401 USA. EM rtcollin@mines.edu RI Collins, Reuben/O-2545-2014; OI Collins, Reuben/0000-0001-7910-3819; Guan, Tianyuan/0000-0001-9084-4351 FU U.S. Department of Energy; National Science Foundation [DE-EE0005326, DMR-0820518]; Solar Energy Research Institute for India and the U.S. (SERIIUS) - U.S. Department of Energy [DE AC36-08G028308]; Office of International Affairs; Government of India [IUSSTF/JCERDC-SERIIUS/2012]; U.S. Government FX This research was based upon work supported by the U.S. Department of Energy and the National Science Foundation under Awards No. DE-EE0005326, DMR-0820518, and was supported in part by the Solar Energy Research Institute for India and the U.S. (SERIIUS) funded jointly by the U.S. Department of Energy subcontract DE AC36-08G028308 (Office of Science, Office of Basic Energy Sciences, and Energy Efficiency and Renewable Energy, Solar Energy Technology Program, with support from the Office of International Affairs) and the Government of India subcontract IUSSTF/JCERDC-SERIIUS/2012 dated 22 November 2012.; This report was prepared as an account of work sponsored by an agency of the U.S. Government. Neither the U.S. Government nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the U.S. Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the U.S. Government or any agency thereof. We would also like to thank Jim Johnson for his support. NR 46 TC 0 Z9 0 U1 5 U2 17 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 19 PY 2015 VL 107 IS 16 AR 163111 DI 10.1063/1.4934570 PG 5 WC Physics, Applied SC Physics GA CU8HG UT WOS:000363781900032 ER PT J AU Wu, PW Zhu, WS Wei, AM Dai, BL Chao, YH Li, CF Li, HM Dai, S AF Wu, Peiwen Zhu, Wenshuai Wei, Aimin Dai, Bilian Chao, Yanhong Li, Changfeng Li, Huaming Dai, Sheng TI Controllable Fabrication of Tungsten Oxide Nanoparticles Confined in Graphene-Analogous Boron Nitride as an Efficient Desulfurization Catalyst SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE Boron; desulfurization; nanoparticles; nitrides; tungsten ID OXIDATIVE DESULFURIZATION; IONIC LIQUID; DEEP DESULFURIZATION; MOLECULAR-OXYGEN; ROOM-TEMPERATURE; WATER OXIDATION; FUELS; TRIOXIDE; SYSTEM; EXTRACTION AB Tungsten oxide nanoparticles (WO(x)NPs) are gaining increasing attention, but low stabiliity and poor dispersion of WO(x)NPs hinder their catalytic applications. Herein, WO(x)NPs were confined in graphene-analogous boron nitride (g-BN) by a one-step, in situ method at high temperature, which can enhance the interactions between WO(x)NPs and the support and control the sizes of WO(x)NPs in a range of about 4-5nm. The as-prepared catalysts were applied in catalytic oxidation of aromatic sulfur compounds in which they showed high catalytic activity. A balance between the W loading and the size distribution of the WO(x)NPs could govern the catalytic activity. Furthermore, a synergistic effect between g-BN and WO(x)NPs also contributed to high catalytic activity. The reaction mechanism is discussed in detail and the catalytic scope was enlarged. C1 [Wu, Peiwen; Li, Changfeng] Jiangsu Univ, Sch Energy & Power Engn, Zhenjiang 212013, Peoples R China. [Zhu, Wenshuai; Wei, Aimin; Dai, Bilian; Chao, Yanhong; Li, Huaming] Jiangsu Univ, Sch Chem & Chem Engn, Zhenjiang 212013, Peoples R China. [Zhu, Wenshuai; Chao, Yanhong; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Zhu, WS (reprint author), Jiangsu Univ, Sch Chem & Chem Engn, 301 Xuefu Rd, Zhenjiang 212013, Peoples R China. EM zhuws@ujs.edu.cn; lihm@ujs.edu.cn RI Dai, Sheng/K-8411-2015 OI Dai, Sheng/0000-0002-8046-3931 FU National Nature Science Foundation of China [21376111, 21276117, 21576122]; Six Big Talent Peak in Jiangasu Province [JNHB-004]; Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy FX We thank the National Nature Science Foundation of China (Nos. 21376111, 21276117, and 21576122) and Six Big Talent Peak in Jiangasu Province (JNHB-004). S.D. was sponsored by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy. NR 45 TC 16 Z9 16 U1 25 U2 102 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. 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Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, R. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Determination of the top-quark pole mass using t(t)over-bar+1-jet events collected with the ATLAS experiment in 7 TeV pp collisions SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering; Top physics ID PARTON DISTRIBUTIONS; HADRON COLLIDERS; LHC; GENERATORS AB The normalized differential cross section for top-quark pair production in association with at least one jet is studied as a function of the inverse of the invariant mass of the t (t) over bar + 1-jet system. This distribution can be used for a precise determination of the top-quark mass since gluon radiation depends on the mass of the quarks. The experimental analysis is based on proton-proton collision data collected by the ATLAS detector at the LHC with a centre-of-mass energy of 7TeV corresponding to an integrated luminosity of 4.6 fb(-1). The selected events were identified using the lepton+jets top-quark-pair decay channel, where lepton refers to either an electron or a muon. The observed distribution is compared to a theoretical prediction at next-to-leading-order accuracy in quantum chromodynamics using the pole-mass scheme. With this method, the measured value of the top-quark pole mass, m(t)(pole), is: m(t)(pole) t = 173.7 +/- 1.5 (stat.) +/- 1.4 (syst.)(-0.5)(+1.0) (theory) GeV. This result represents the most precise measurement of the top-quark pole mass to date. C1 [Jackson, P.; Lee, L.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.; Nanava, G.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. 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L.; Bellagamba, L.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Corradi, M.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstrom, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] INFN Sez Bologna, Bologna, Italy. [Alberghi, G. L.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstrom, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Hageboeck, S.; Hellmich, D.; Hohn, D.; Huegging, F.; Janssen, J.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mergelmeyer, S.; Mijovic, L.; Mueller, K.; Nanava, G.; Nattermann, T.; Obermann, T.; Pohl, D.; Sarrazin, B.; Schaepe, S.; Schopf, E.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Seema, P.; Stillings, J. A.; Tannoury, N.; Therhaag, J.; Uhlenbrock, M.; Velz, T.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Zimmermann, R.] Univ Bonn, Phys Inst, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Dhaliwal, S.; Fitzgerald, E. A.; Sciolla, G.; Venturini, A.; Zambito, S.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio Janeiro COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Filho, L. Manhaes de Andrade] Univ Fed Juiz de Fora, Elect Circuits Dept, Juiz de Fora, Brazil. [do Vale, M. A. B.] Univ Fed Sao Joao del Rei, Sao Joao del Rei, Brazil. [Donadelli, M.; Navarro, J. L. La Rosa; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Acharya, B. S.; Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abulaiti, Y.; Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Castro, N. F.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Favareto, A.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Iengo, P.; Jaekel, M. R.; Jakobsen, S.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Kapliy, A.; Kim, Y.; Krizka, K.; Li, H. L.; Melachrinos, C.; Merritt, F. S.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaza, M. A.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Guo, J.; Li, Y.; Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Liu, B.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Shandong, Peoples R China. [Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Grivaz, J-F.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] INFN Grp Coll Cosenza, Lab Nazl Frascati, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Abulaiti, Y.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Perrella, S.; Reeves, K.] Univ Texas Dallas, Dept Phys, Dallas, TX 75230 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Gossling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Betancourt, C.; Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] INFN Lab Nazl Frascati, Frascati, Italy. [Amoroso, S.; Arnold, H.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dao, V.; Di Simone, A.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fak Mathemat & Phys, D-79106 Freiburg, Germany. [Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrari, A.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nessi, M.; Picazio, A.; Ristic, B.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Ferrari, R.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodia, F.; Passaggio, S.; Rossi, L. P.; Sanninoa, M.; Schiavi, C.] INFN Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Ferrari, R.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodia, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Phys Inst 2, D-35390 Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Fayard, L.; Federic, P.; Ferrag, S.; de Lima, D. E. Ferreira; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; Musto, E.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bindi, M.; Blumenschein, U.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Physikal Inst 2, D-37073 Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Guimaraes da Costa, J. Barreiro; Catastini, P.; Franklin, M.; Huth, J.; Ippolito, V.; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Hanke, P.; Jongmanns, J.; Kluge, E-E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Physikal Inst, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R. W.; Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.; Usanova, A.] Univ Innsbruck, Inst Astro & Teilchenphys, A-6020 Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Hall, D.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Paz, I. Lopez; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.] INFN Sez Lecce, Lecce, Italy. [Chiodini, G.; Gorini, E.; Spagnolo, S.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Price, J.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Hall, D.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Hall, D.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Hall, D.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Hakobyan, H.; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Pilkington, A. D.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Hall, D.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Grivaz, J-F.; Hall, D.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Hall, D.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjoenmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Hall, D.; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koening, S.; Koepke, L.; Lin, T. H.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Poettgen, R.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Feigl, S.; Forti, A.; Grivaz, J-F.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Davies, E.; Della Pietra, M.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Univ Aix Marseille, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Davies, E.; Della Pietra, M.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Feng, H.; Ferrari, P.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Hu, X.; Levin, D.; Liu, L.; Paredes, B. Lopez; Lu, N.; Mc Kee, S. P.; Mcarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Hall, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Pereza, M. Villaplana] INFN Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Turra, R.; Pereza, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Girolamo, B.; Doria, A.; Grivaz, J-F.; Hall, D.; Izzo, V.; Merola, L.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] INFN Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Di Girolamo, B.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartmento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Musto, E.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Koenig, A. C.; Nektarijevic, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Fedorko, W.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Fedorko, W.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adamczyk, L.; Adelman, J.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk 630090, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Haley, J.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.; Hernandez, D. Paredes] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J-F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, CNRS IN2P3, LAL, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pachal, K.; Pickering, M. A.; Ryder, N. C.; Sawyer, C.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Feigl, S.; Fraternali, M.; Gaudio, G.; Livan, M.; Negria, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] INFN Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negria, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Natl Res Ctr, BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Spalla, M.; Volpi, G.; White, S.] INFN Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Fedin, O. L.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr, Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallo, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Di Girolamo, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Mirabelli, G.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] INFN Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Di Girolamo, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonicoa, R.] INFN Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Santonicoa, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Stanescu, C.; Taccini, C.; Trovatelli, M.] INFN Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Taccini, C.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Eseau Univ Phys Hautes Energies, Facult Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Techn Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Cadi Ayyad, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Mourslie, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Aloisio, A.; Alonso, A.; Altheimer, A.; Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J-B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Feigl, S.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Gorisek, A.; Grivaz, J-F.; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay Commissariat Energie Atom & Energies A, DSM IRFU Inst Rech Lois Fondament Univers, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S-C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Kyriazopoulos, D.; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; Horton, A. J.; O'Neil, D. C.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Cribbs, W. A.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Hall, D.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Mount, R.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice, Slovakia. [Hamilton, A.; Meehan, S.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Connell, S. H.; Lee, C. A.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hamity, G. N.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abreu, H.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Eriksson, D.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abreu, H.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; Mckarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; Mckarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G-Y.; Limosani, A.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Hsu, P. J.; Jamin, D. O.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Yang, Y.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, R.; Cheatham, S.; Di Mattia, A.; Kopeliansky, R.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Ninomiya, Y.; Orlando, N.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.; Sotiropoulou, C. L.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Ilic, N.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Qureshi, A.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Abreu, R.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Shaw, K.; Soualah, R.] INFN Grp Coll Udine, Udine, Italy. [Barisonzi, M.; Quayle, W. B.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Fedin, O. L.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Martinez, P. Fernandez; Ferrando, J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Martinez, P. Fernandez; Ferrando, J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Fis Aom Mol & Nucl, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Martinez, P. Fernandez; Ferrando, J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Martinez, P. Fernandez; Ferrando, J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. 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[Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] IPP, Toronto, ON, Canada. [Fedin, O. L.] St Petersburg State Polytechn Univ, Dept Phys, St Petersburg, Russia. [Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Inst Catalana Recerca & Estudis Avancats, Barcelona, Spain. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Khubua, J.] GTU, Tbilisi, Rep of Georgia. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys, Dolgoprudnyi, Russia. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Technol State Univ, Dolgoprudnyi, Russia. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Xu, L.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Univ Aix Marseille, CPPM, Marseille, France. RI Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Staroba, Pavel/G-8850-2014; Gavrilenko, Igor/M-8260-2015; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Mindur, Bartosz/A-2253-2017; Fabbri, Laura/H-3442-2012; Gutierrez, Phillip/C-1161-2011; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Vranjes Milosavljevic, Marija/F-9847-2016; Chekulaev, Sergey/O-1145-2015; Zhukov, Konstantin/M-6027-2015; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Fedin, Oleg/H-6753-2016; Snesarev, Andrey/H-5090-2013; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; Villa, Mauro/C-9883-2009; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; spagnolo, stefania/A-6359-2012; Buttar, Craig/D-3706-2011; Mitsou, Vasiliki/D-1967-2009; Tripiana, Martin/H-3404-2015; Smirnova, Oxana/A-4401-2013; Savarala, Hari Krishna/A-3516-2015; Doyle, Anthony/C-5889-2009; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Boyko, Igor/J-3659-2013; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Livan, Michele/D-7531-2012; Brooks, William/C-8636-2013; Di Domenico, Antonio/G-6301-2011; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Tikhomirov, Vladimir/M-6194-2015; Carvalho, Joao/M-4060-2013; White, Ryan/E-2979-2015; Mashinistov, Ruslan/M-8356-2015; Warburton, Andreas/N-8028-2013 OI Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Villa, Mauro/0000-0002-9181-8048; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; spagnolo, stefania/0000-0001-7482-6348; Mitsou, Vasiliki/0000-0002-1533-8886; Smirnova, Oxana/0000-0003-2517-531X; Savarala, Hari Krishna/0000-0001-6593-4849; Doyle, Anthony/0000-0001-6322-6195; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Boyko, Igor/0000-0002-3355-4662; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Prokofiev, Kirill/0000-0002-2177-6401; Livan, Michele/0000-0002-5877-0062; Brooks, William/0000-0001-6161-3570; Di Domenico, Antonio/0000-0001-8078-2759; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Andreazza, Attilio/0000-0001-5161-5759; Tikhomirov, Vladimir/0000-0002-9634-0581; Carvalho, Joao/0000-0002-3015-7821; White, Ryan/0000-0003-3589-5900; Mashinistov, Ruslan/0000-0001-7925-4676; Warburton, Andreas/0000-0002-2298-7315 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS; MIZS Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 69 TC 2 Z9 2 U1 12 U2 68 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD OCT 19 PY 2015 IS 10 AR 121 DI 10.1007/JHEP10(2015)121 PG 41 WC Physics, Particles & Fields SC Physics GA CU4DM UT WOS:000363476900001 ER PT J AU Tselev, A Klein, A Gassmann, J Jesse, S Li, Q Kalinin, SV Balke, N AF Tselev, Alexander Klein, Andreas Gassmann, Juergen Jesse, Stephen Li, Qian Kalinin, Sergei V. Balke, Nina TI Quantitative Nanometer-Scale Mapping of Dielectric Tunability SO ADVANCED MATERIALS INTERFACES LA English DT Article DE electrostriction; near-field microwave microscopy; piezoresponse force microscopy; permittivity; mapping; dieletrics ID FERROELECTRIC THIN-FILMS; PIEZORESPONSE FORCE MICROSCOPY; MICROWAVE; PERMITTIVITY; POLARIZATION; CAPACITOR AB Two scanning probe microscopy techniquesnear-field scanning microwave microscopy (SMM) and piezoresponse force microscopy (PFM)-are used to characterize and image tunability in a thin (Ba,Sr)TiO3 film with nanometer scale spatial resolution. While sMIM allows direct probing of tunability by measurement of the change in the dielectric constant, in PFM, tunability can be extracted via electrostrictive response. The near-field microwave imaging and PFM provide similar information about dielectric tunability with PFM capable to deliver quantitative information on tunability with a higher spatial resolution close to 15 nm. This is the first time, information about the dielectric tunability is available on such length scales. C1 [Tselev, Alexander; Jesse, Stephen; Li, Qian; Kalinin, Sergei V.; Balke, Nina] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Inst Funct Imaging, Oak Ridge, TN 37831 USA. [Klein, Andreas; Gassmann, Juergen] Tech Univ Darmstadt, Fac Mat Sci, D-64287 Darmstadt, Germany. RP Balke, N (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Inst Funct Imaging, Oak Ridge, TN 37831 USA. EM balken@ornl.gov RI Klein, Andreas/E-6081-2010; Balke, Nina/Q-2505-2015; Kalinin, Sergei/I-9096-2012; Jesse, Stephen/D-3975-2016; OI Klein, Andreas/0000-0001-7463-1495; Balke, Nina/0000-0001-5865-5892; Kalinin, Sergei/0000-0001-5354-6152; Jesse, Stephen/0000-0002-1168-8483; Tselev, Alexander/0000-0002-0098-6696 FU US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division through the Office of Science Early Career Research Program; Division of Materials Sciences and Engineering; Center for Nanophase Materials Sciences, DOE Office of Science User Facility; German Science Foundation (DFG) through the Research Training School (Tunable Integratable Components for Microwaves and Optics) [GRK 1037] FX Support was provided by the US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division through the Office of Science Early Career Research Program (N.B., Q.L.). Additional support (A.T., S.V.K.) was provided by the Division of Materials Sciences and Engineering. This research was conducted at and additional support was provided (S.J.) by the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. Samples were provided by A.K. and J.G., which have been supported by the German Science Foundation (DFG) through the Research Training School GRK 1037 (Tunable Integratable Components for Microwaves and Optics). NR 39 TC 2 Z9 2 U1 5 U2 24 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2196-7350 J9 ADV MATER INTERFACES JI Adv. Mater. Interfaces PD OCT 19 PY 2015 VL 2 IS 15 AR 1500088 DI 10.1002/admi.201500088 PG 10 WC Chemistry, Multidisciplinary; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CU3HP UT WOS:000363415300001 ER PT J AU Zhou, Y Leonard, DN Meyer, HM Luo, HM Qu, J AF Zhou, Yan Leonard, Donovan N. Meyer, Harry M., III Luo, Huimin Qu, Jun TI Does the Use of Diamond-Like Carbon Coating and Organophosphate Lubricant Additive Together Cause Excessive Tribochemical Material Removal? SO ADVANCED MATERIALS INTERFACES LA English DT Article DE Diamond-like carbon (DLC); ionic liquids; lubricants; tribochemical; ZDDP ID MISCIBLE IONIC LIQUID; WEAR MECHANISMS; OIL ADDITIVES; ZDDP; TEMPERATURE; EFFICIENT; FRICTION C1 [Zhou, Yan; Leonard, Donovan N.; Meyer, Harry M., III; Luo, Huimin; Qu, Jun] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Qu, J (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, POB 2008,MS-6063, Oak Ridge, TN 37831 USA. EM qujn@ornl.gov OI Qu, Jun/0000-0001-9466-3179 FU Vehicle Technologies Office, Office of Energy Efficiency and Renewable Energy, U.S. Department of Energy (DOE); U.S. Department of Energy [DE-AC05-00OR22725]; US government grant FX The authors thank Dr. S. Dai from Oak Ridge National Laboratory (ORNL) for results discussion and D.W. Coffey from ORNL for TEM sample preparation. Research was sponsored by the Vehicle Technologies Office, Office of Energy Efficiency and Renewable Energy, U.S. Department of Energy (DOE). Electron microscopy characterization was conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. This paper has been authored by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. This contribution was prepared under a US government grant. The US Government may reproduce, without charge, all or portions of the contribution and may authorize others to do so, for official US Government purposes only, if the US Government contract or grant so requires. NR 25 TC 1 Z9 1 U1 1 U2 13 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2196-7350 J9 ADV MATER INTERFACES JI Adv. Mater. Interfaces PD OCT 19 PY 2015 VL 2 IS 15 AR 1500213 DI 10.1002/admi.201500213 PG 6 WC Chemistry, Multidisciplinary; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CU3HP UT WOS:000363415300006 ER PT J AU Stavretis, SE Atanasov, M Podlesnyak, AA Hunter, SC Neese, F Xue, ZL AF Stavretis, Shelby E. Atanasov, Mihail Podlesnyak, Andrey A. Hunter, Seth C. Neese, Frank Xue, Zi-Ling TI Magnetic Transitions in Iron Porphyrin Halides by Inelastic Neutron Scattering and Ab Initio Studies of Zero-Field Splittings SO INORGANIC CHEMISTRY LA English DT Article ID STATE PERTURBATION-THEORY; BASIS-SETS; MOLECULAR STEREOCHEMISTRY; SCORPIONATE COMPLEXES; ELECTRONIC-STRUCTURE; VALENCE; ANISOTROPY; RESONANCE; METALLOPORPHYRINS; 1ST-PRINCIPLES AB Zero-field splitting (ZFS) parameters of nondeuterated metalloporphyrins [Fe(TPP)X] (X = F, Br, I; H2TPP = tetraphenylporphyrin) have been directly determined by inelastic neutron scattering (INS). The ZFS values are D = 4.49(9) cm(-1) for tetragonal polycrystalline [Fe(TPP)F], and D = 8.8(2) cm(-1), E = 0.1(2) cm(-1) and D = 13.4(6) cm(-1), E = 0.3(6) cm(-1) for monoclinic polycrystalline [Fe(TPP)Br] and [Fe(TPP)I], respectively. Along with our recent report of the ZFS value of D = 6.33(8) cm(-1) for tetragonal polycrystalline [Fe(TPP)Cl], these data provide a rare, complete determination of ZFS parameters in a metalloporphyrin halide series. The electronic structure of [Fe(TPP)X] (X = F, Cl, Br, I) has been studied by multireference ab initio methods: the complete active space self-consistent field (CASSCF) and the N-electron valence perturbation theory (NEVPT2) with the aim of exploring the origin of the large and positive zero-field splitting D of the (6)A(1) ground state. D was calculated from wave functions of the electronic multiplets spanned by the d(5) configuration of Fe(III) along with spin-orbit coupling accounted for by quasi degenerate perturbation theory. Results reproduce trends of D from inelastic neutron scattering data increasing in the order from F, Cl, Br, to I. A mapping of energy eigenvalues and eigenfunctions of the S = 3/2 excited states on ligand field theory was used to characterize the sigma- and pi-antibonding effects decreasing from F to I. This is in agreement with similar results deduced from ab initio calculations on CrX63- complexes and also with the spectrochemical series showing a decrease of the ligand field in the same directions. A correlation is found between the increase of D and decrease of the pi- and sigma-antibonding energies e(lambda)(X) (lambda = sigma, pi) in the series from X = F to I. Analysis of this correlation using second-order perturbation theory expressions in terms of angular overlap parameters rationalizes the experimentally deduced trend. D parameters from CASSCF and NEVPT2 results have been calibrated against those from the INS data, yielding a predictive power of these approaches. Methods to improve the quantitative agreement between ab initio calculated and experimental D and spectroscopic transitions for high-spin Fe(III) complexes are proposed. C1 [Stavretis, Shelby E.; Hunter, Seth C.; Xue, Zi-Ling] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Atanasov, Mihail; Neese, Frank] Max Planck Inst Chem Energy Convers, D-45470 Mulheim An Der Ruhr, Germany. [Atanasov, Mihail] Bulgarian Acad Sci, Inst Gen & Inorgan Chem, Sofia 1113, Bulgaria. [Podlesnyak, Andrey A.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP Atanasov, M (reprint author), Max Planck Inst Chem Energy Convers, Stiftstr 34-36, D-45470 Mulheim An Der Ruhr, Germany. EM mihail.atanasov@cec.mpg.de; podlesnyakaa@ornl.gov; frank.neese@cec.mpg.de; xue@utk.edu RI Neese, Frank/J-4959-2014; Podlesnyak, Andrey/A-5593-2013; Instrument, CNCS/B-4599-2012 OI Neese, Frank/0000-0003-4691-0547; Podlesnyak, Andrey/0000-0001-9366-6319; FU U.S. National Science Foundation [CHE-1362548]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX The work is supported by the U.S. National Science Foundation (CHE-1362548 to Z.-L.X.). Acknowledgment is also made to the Donors of the American Chemical Society Petroleum Research Fund for partial support of this research. Research at Oak Ridge National Laboratory's Spallation Neutron Source was supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. We acknowledge the technical and scientific support from the staff at the SNS. We thank Dr. Jurek Krzystek (National High Magnetic Field Laboratory, Florida State University) and Prof. Joshua Telser (Roosevelt University) for helpful discussions and for communicating HFEPR results on the Fe(TPP)X complexes. NR 69 TC 7 Z9 7 U1 7 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD OCT 19 PY 2015 VL 54 IS 20 BP 9790 EP 9801 DI 10.1021/acs.inorgchem.5b01505 PG 12 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CU0QO UT WOS:000363224000018 PM 26428688 ER PT J AU Chatterjee, S Norton, AE Edwards, MK Peterson, JM Taylor, SD Bryan, SA Andersen, A Govind, N Albrecht-Schmitt, TE Connick, WB Levitskaia, TG AF Chatterjee, Sayandev Norton, Arnie E. Edwards, Matthew K. Peterson, James M. Taylor, Stephen D. Bryan, Samuel A. Andersen, Amity Govind, Niranjan Albrecht-Schmitt, Thomas E. Connick, William B. Levitskaia, Tatiana G. TI Highly Selective Colorimetric and Luminescence Response of a Square-Planar Platinum(II) Terpyridyl Complex to Aqueous TcO4- SO INORGANIC CHEMISTRY LA English DT Article ID SOLVENT-INDUCED AGGREGATION; METAL-METAL INTERACTIONS; EXCITED-STATE; SUPRAMOLECULAR RECOGNITION; -TECHNETIUM(V) COMPLEXES; ELECTRONIC SPECTROSCOPY; CRYSTAL-STRUCTURES; ANION; SALTS; QUANTIFICATION AB Molecular recognition of an aqueous pertechnetate (TcO4-) anion is fundamentally challenging partly due to the charge-diffuse nature of this anion, which hampers design of new technologies for its separation and detection. To address this gap, simple salts of transition metal complexes that undergo a distinct spectroscopic change upon exposure to aqueous anions were explored. The Pt(II) complex [Pt(tpy)-Br]SbF6 (tpy = 2,2';6',2 ''-terpyridine) undergoes a dramatic color change and intense luminescence response upon TcO4- uptake due to concomitant enhancement of Pt center dot center dot center dot Pt interactions. The spectroscopic response was highly selective and quantitative for aqueous TcO4- among other competing anions. Complementary Raman spectroscopy and microscopy techniques, structural determination, and theoretical methods were employed to elucidate the mechanism of this response at the molecular level. C1 [Chatterjee, Sayandev; Edwards, Matthew K.; Peterson, James M.; Bryan, Samuel A.; Levitskaia, Tatiana G.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99354 USA. [Norton, Arnie E.; Taylor, Stephen D.; Connick, William B.] Univ Cincinnati, Dept Chem, Cincinnati, OH 45221 USA. [Andersen, Amity; Govind, Niranjan] Pacific NW Natl Lab, Environm & Mol Sci Lab, Richland, WA 99354 USA. [Albrecht-Schmitt, Thomas E.] Florida State Univ, Dept Chem & Biochem, Tallahassee, FL 32306 USA. RP Chatterjee, S (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99354 USA. EM Sayandev.Chatterjee@pnnl.gov; connicwb@ucmail.uc.edu; Tatiana.Levitskaia@pnnl.gov OI Chatterjee, Sayandev/0000-0003-2218-5635 FU U.S. Department of Energy [DE-AC05-76RL01830]; National Science Foundation [CHE-1152853]; US EPA STAR [FP-91765901]; Office of Science, BER [DE-FG02-07ER64353]; Office of Environmental Management Sciences Program of the U.S. Department of Energy [DE-FG0799ER62331]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Heavy Elements Chemistry Program [DE-FG02-13ER16414] FX This research was supported by (1) the Laboratory Directed Research and Development Program at the Pacific Northwest National Laboratory operated by Battelle for the U.S. Department of Energy under Contract DE-AC05-76RL01830 and (2) the National Science Foundation (CHE-1152853), as well as a to A.E.N. (US EPA STAR, FP-91765901). The initial scoping experiments for the selection of the appropriate platinum complex were performed under support from the Office of Science, BER (Grant No. DE-FG02-07ER64353), and the Office of Environmental Management Sciences Program (Grant No. DE-FG0799ER62331) of the U.S. Department of Energy. Part of this research was performed at EMSL, a national scientific user facility at PNNL managed by the Department of Energy's Office of Biological and Environmental Research. We thank Dr. Zheming Wang for helping with spectroscopy measurements and Mr. Paul Macfarlan for helping with SEM measurements. TEA-S was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Heavy Elements Chemistry Program, under Award Number DE-FG02-13ER16414. NR 77 TC 5 Z9 5 U1 2 U2 30 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD OCT 19 PY 2015 VL 54 IS 20 BP 9914 EP 9923 DI 10.1021/acs.inorgchem.5b01664 PG 10 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CU0QO UT WOS:000363224000032 PM 26447785 ER PT J AU Nguyen, PTK Nguyen, HTD Phamp, HQ Kim, J Cordova, KE Furukawa, H AF Phuong T. K Nguyen Huong T. D. Nguyen Hung Q Phamp Kim, Jaheon Kyle E. Cordova Furukawa, Hiroyasu TI Synthesis and Selective CO2 Capture Properties of a Series of Hexatopic Linker-Based Metal-Organic Frameworks SO INORGANIC CHEMISTRY LA English DT Article ID COORDINATION POLYMERS; TOPOLOGICAL ANALYSIS; STORAGE CAPACITIES; CRYSTAL-STRUCTURES; WATER-ADSORPTION; BUILDING UNITS; CARBON-DIOXIDE; LIGAND; SEPARATION; FUNCTIONALIZATION AB Four crystalline, porous metal organic frameworks (MOFs), based on a new hexatopic linker, 1',2',3',4',5',6'-hexakis(4-carboxyphenyl)benzene (H6CPB), were synthesized and fully characterized. Interestingly, two members of this series exhibited new topologies, namely, htp and hhp, which were previously unseen in MOP chemistry. Gas adsorption measurements revealed that all members exhibited high CO2 selectivity over N-2 and CH4. Accordingly, breakthrough measurements were performed on a representative example, in which the effective separation of CO2 from binary mixtures containing either N-2 or CH4 was demonstrated without any loss in performance over three consecutive cycles. C1 [Phuong T. K Nguyen; Huong T. D. Nguyen; Hung Q Phamp; Kyle E. Cordova] VNU HCM, Univ Sci, Ctr Mol NanoArchitecture, Ho Chi Minh City 721337, Vietnam. [Huong T. D. Nguyen; Hung Q Phamp] VNU HCM, Univ Sci, Fac Chem, Ho Chi Minh City 721337, Vietnam. [Kim, Jaheon] Soongsil Univ, Dept Chem, Seoul 156743, South Korea. [Kyle E. Cordova; Furukawa, Hiroyasu] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Kyle E. Cordova; Furukawa, Hiroyasu] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Kyle E. Cordova; Furukawa, Hiroyasu] Univ Calif Berkeley, Ctr Global Sci Berkeley, Berkeley, CA 94720 USA. [Furukawa, Hiroyasu] King Fahd Univ Petr & Minerals, Dhahran 34464, Saudi Arabia. RP Cordova, KE (reprint author), VNU HCM, Univ Sci, Ctr Mol NanoArchitecture, Ho Chi Minh City 721337, Vietnam. EM kcordova@berkeley.edu; furukawa@berkeley.edu RI Furukawa, Hiroyasu/C-5910-2008; OI Furukawa, Hiroyasu/0000-0002-6082-1738; Cordova, Kyle/0000-0002-4988-0497 FU VNU-HCM [B2011-50-01TD, A2015-50-01-HD-KHCN]; United States Office of Naval Research Global: Naval International Cooperative Opportunities in Science and Technology Program [N62909-15-1N056]; Mid-Career Researcher Program of the National Research Foundation of Korea - Ministry of Science, ICT, and Future Planning [NRF-2014R1A2A1A11054190] FX Prof. O. M. Yaghi is gratefully acknowledged for founding and supporting MANAR. We acknowledge T. T. Ho and A. M. Osborn at MANAR for valuable discussion and assistance on this work. We thank Dr. H. T. C. Ho, Dr. Q. T. Ton, and Prof. H. T. Nguyen at the University of Science (VNU-HCM) for their valuable input. We are indebted to Prof. M. O'Keeffe (Arizona State University) for useful discussion on topological analysis. The work was supported for the synthesis and general adsorption characterization by VNU-HCM (Nos. B2011-50-01TD and A2015-50-01-HD-KHCN), and the dynamic breakthrough measurement was supported by the United States Office of Naval Research Global: Naval International Cooperative Opportunities in Science and Technology Program (No. N62909-15-1N056). J.K. acknowledges support from the Mid-Career Researcher Program of the National Research Foundation of Korea funded by the Ministry of Science, ICT, and Future Planning (NRF-2014R1A2A1A11054190). NR 56 TC 8 Z9 8 U1 11 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD OCT 19 PY 2015 VL 54 IS 20 BP 10065 EP 10072 DI 10.1021/acs.inorgchem.5b01900 PG 8 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CU0QO UT WOS:000363224000049 PM 26445199 ER PT J AU Mason, JA Darago, LE Lukens, WW Long, JR AF Mason, Jarad A. Darago, Lucy E. Lukens, Wayne W., Jr. Long, Jeffrey R. TI Synthesis and O-2 Reactivity of a Titanium(III) Metal-Organic Framework SO INORGANIC CHEMISTRY LA English DT Article ID CARBON-DIOXIDE CAPTURE; IRON(II) COORDINATION SITES; HYDROGEN STORAGE; HYDROCARBON SEPARATIONS; CATALYTIC-PROPERTIES; ELECTRONIC-SPECTRA; POWDER DIFFRACTION; OXO-CLUSTERS; GAS-STORAGE; ACID SITES AB Metal-organic frameworks featuring pores lined with exposed metal cations have received attention for a wide range of adsorption-related applications. While many frameworks with coordinatively unsaturated M-II centers have been reported, there are relatively few examples of porous materials with coordinatively unsaturated M-III centers. Here, we report the synthesis and characterization of Ti3O(OEt)(bdc)(3)(solv)(2) (Ti-MIL-101; bdc(2-) = 1,4-benzenedicarboxylate; solv = N,N-dimethylformamide, tetrahydrofuran), the first metal-organic framework containing exclusively Ti-III centers. Through a combination of gas adsorption, X-ray diffraction, magnetic susceptibility, and electronic and vibrational spectroscopy measurements, this high-surface-area framework is shown to contain five-coordinate Ti-III centers upon desolvation, which irreversibly bind O-2 to form titanium(IV) superoxo and peroxo species. Electronic absorption spectra suggest that the five-coordinate Ti-III sites adopt a distorted trigonal-bipyramidal geometry that effectively shields nuclear charge and inhibits strong adsorption of nonredox-active gases. C1 [Mason, Jarad A.; Darago, Lucy E.; Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Mason, Jarad A.; Darago, Lucy E.; Long, Jeffrey R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Lukens, Wayne W., Jr.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Long, JR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM jrlong@berkeley.edu OI Darago, Lucy/0000-0001-7515-5558 FU Department of Energy, Office of Energy Efficiency and Renewable Energy (DOE-EERE), Fuel Cell Technologies Office; DOE Office of Science User Facility [DE-AC02-06CH11357]; NSF; U.S. DOE, Office of Science, Basic Energy Sciences, Chemical Sciences, Biosciences, and Geosciences Division, Heavy Element Chemistry Program [DE-AC02-05CH11231] FX This research was supported by the Department of Energy, Office of Energy Efficiency and Renewable Energy (DOE-EERE), Fuel Cell Technologies Office. Powder X-ray diffraction data were collected at Beamline 11-BM at the APS, a DOE Office of Science User Facility, operated by Argonne National Laboratory under Contract DE-AC02-06CH11357. We thank Dianne J. Xiao, David Z. Zee, and Gokhan Barin for helpful discussions, and we thank the NSF for providing graduate fellowship support for J.A.M. and L.E.D. EPR studies were supported by the U.S. DOE, Office of Science, Basic Energy Sciences, Chemical Sciences, Biosciences, and Geosciences Division, Heavy Element Chemistry Program, and were performed at Lawrence Berkeley National Laboratory under Contract DE-AC02-05CH11231. NR 97 TC 7 Z9 7 U1 9 U2 62 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD OCT 19 PY 2015 VL 54 IS 20 BP 10096 EP 10104 DI 10.1021/acs.inorgchem.5b02046 PG 9 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CU0QO UT WOS:000363224000052 PM 26439082 ER PT J AU Dobrescu, BA Liu, Z AF Dobrescu, Bogdan A. Liu, Zhen TI Heavy Higgs bosons and the 2 TeV W ' boson SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Higgs Physics; Beyond Standard Model ID RIGHT-SYMMETRICAL MODELS; CP VIOLATION; NEUTRINOS; MASSES; QUARK; PP AB The hints from the LHC for the existence of a W' boson of mass around 1.9TeV point towards a certain SU(2)(L) x SU(2)(R) x U(1)(B-L) gauge theory with an extended Higgs sector. We show that the decays of the W' boson into heavy Higgs bosons have sizable branching fractions. Interpreting the ATLAS excess events in the search for same-sign lepton pairs plus b jets as arising from W' cascade decays, we estimate that the masses of the heavy Higgs bosons are in the 400-700 GeV range. C1 [Dobrescu, Bogdan A.; Liu, Zhen] Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. [Liu, Zhen] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. RP Dobrescu, BA (reprint author), Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. EM bdob@fnal.gov; zliu2@fnal.gov OI Liu, Zhen/0000-0002-3143-1976 FU Fermilab Graduate Student Research Program in Theoretical Physics FX We would like to thank Patrick Fox, Robert Harris, Matthew Low and Andrea Tesi for helpful conversations. We would like to thank Tongyan Lin and the referee for drawing our attention to some errors in an earlier version of section 3. ZL was supported by the Fermilab Graduate Student Research Program in Theoretical Physics. NR 41 TC 37 Z9 37 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD OCT 19 PY 2015 IS 10 AR 118 DI 10.1007/JHEP10(2015)118 PG 18 WC Physics, Particles & Fields SC Physics GA CU0YF UT WOS:000363244500001 ER PT J AU Adare, A Aidala, C Ajitanand, NN Akiba, Y Al-Bataineh, H Alexander, J Alfred, M Angerami, A Aoki, K Apadula, N Aramaki, Y Asano, H Atomssa, ET Averbeck, R Awes, TC Azmoun, B Babintsev, V Bai, M Baksay, G Baksay, L Bandara, NS Bannier, B Barish, KN Bassalleck, B Basye, AT Bathe, S Baublis, V Baumann, C Bazilevsky, A Beaumier, M Beckman, S Belikov, S Belmont, R Bennett, R Berdnikov, A Berdnikov, Y Bhom, JH Blau, DS Bok, JS Boyle, K Brooks, ML Bryslawskyj, J Buesching, H Bumazhnov, V Bunce, G Butsyk, S Campbell, S Caringi, A Chen, CH Chi, CY Chiu, M Choi, IJ Choi, JB Choudhury, RK Christiansen, P Chujo, T Chung, P Chvala, O Cianciolo, V Citron, Z Cole, BA del Valle, ZC Connors, M Csanad, M Csorgo, T Dahms, T Dairaku, S Danchev, I Danley, D Das, K Datta, A Daugherity, MS David, G Dayananda, MK DeBlasio, K Dehmelt, K Denisov, A Deshpande, A Desmond, EJ Dharmawardane, KV Dietzsch, O Dion, A Diss, PB Do, JH Donadelli, M D'Orazio, L Drapier, O Drees, A Drees, KA Durham, JM Durum, A Dutta, D Edwards, S Efremenko, YV Ellinghaus, F Engelmore, T Enokizono, A En'yo, H Esumi, S Fadem, B Feege, N Fields, DE Finger, M Finger, M Fleuret, F Fokin, SL Fraenkel, Z Frantz, JE Franz, A Frawley, AD Fujiwara, K Fukao, Y Fusayasu, T Gal, C Gallus, P Garg, P Garishvili, I Ge, H Giordano, F Glenn, A Gong, H Gonin, M Goto, Y de Cassagnac, RG Grau, N Greene, SV Grim, G Perdekamp, MG Gunji, T Gustafsson, HA Hachiya, T Haggerty, JS Hahn, KI Hamagaki, H Hamblen, J Hamilton, HF Han, R Han, SY Hanks, J Hasegawa, S Haseler, TOS Hashimoto, K Haslum, E Hayano, R He, X Heffner, M Hemmick, TK Hester, T Hill, JC Hohlmann, M Hollis, RS Holzmann, W Homma, K Hong, B Horaguchi, T Hornback, D Hoshino, T Hotvedt, N Huang, J Huang, S Ichihara, T Ichimiya, R Ikeda, Y Imai, K Inaba, M Iordanova, A Isenhower, D Ishihara, M Issah, M Ivanishchev, D Iwanaga, Y Jacak, BV Jezghani, M Jia, J Jiang, X Jin, J Johnson, BM Jones, T Joo, KS Jouan, D Jumper, DS Kajihara, F Kamin, J Kanda, S Kang, JH Kapustinsky, J Karatsu, K Kasai, M Kawall, D Kawashima, M Kazantsev, AV Kempel, T Key, JA Khachatryan, V Khanzadeev, A Kijima, KM Kikuchi, J Kim, A Kim, BI Kim, C Kim, DJ Kim, EJ Kim, GW Kim, M Kim, YJ Kimelman, B Kinney, E Kiss, A Kistenev, E Kitamura, R Klatsky, J Kleinjan, D Kline, P Koblesky, T Kochenda, L Komkov, B Konno, M Koster, J Kotov, D Kral, A Kravitz, A Kunde, GJ Kurita, K Kurosawa, M Kwon, Y Kyle, GS Lacey, R Lai, YS Lajoie, JG Lebedev, A Lee, DM Lee, J Lee, KB Lee, KS Lee, S Lee, SH Leitch, MJ Leite, MAL Li, X Lichtenwalner, P Liebing, P Lim, SH Levy, LAL Liska, T Liu, H Liu, MX Love, B Lynch, D Maguire, CF Makdisi, YI Makek, M Malik, MD Manion, A Manko, VI Mannel, E Mao, Y Masui, H Matathias, F McCumber, M McGaughey, PL McGlinchey, D McKinney, C Means, N Meles, A Mendoza, M Meredith, B Miake, Y Mibe, T Mignerey, AC Miki, K Milov, A Mishra, DK Mitchell, JT Miyasaka, S Mizuno, S Mohanty, AK Montuenga, P Moon, HJ Moon, T Morino, Y Morreale, A Morrison, DP Moukhanova, TV Murakami, T Murata, J Mwai, A Nagamiya, S Nagashima, K Nagle, JL Naglis, M Nagy, MI Nakagawa, I Nakagomi, H Nakamiya, Y Nakamura, KR Nakamura, T Nakano, K Nam, S Nattrass, C Netrakanti, PK Newby, J Nguyen, M Nihashi, M Niida, T Nishimura, S Nouicer, R Novak, T Novitzky, N Nyanin, AS Oakley, C O'Brien, E Oda, SX Ogilvie, CA Oka, M Okada, K Onuki, Y Koop, JDO Osborn, JD Oskarsson, A Ouchida, M Ozawa, K Pak, R Pantuev, V Papavassiliou, V Park, IH Park, JS Park, S Park, SK Park, WJ Pate, SF Patel, M Pei, H Peng, JC Pereira, H Perepelitsa, DV Perera, GDN Peressounko, DY Perry, J Petti, R Pinkenburg, C Pinson, R Pisani, RP Proissl, M Purschke, ML Qu, H Rak, J Ramson, BJ Ravinovich, I Read, KF Rembeczki, S Reygers, K Reynolds, D Riabov, V Riabov, Y Richardson, E Rinn, T Roach, D Roche, G Rolnick, SD Rosati, M Rosen, CA Rosendahl, SSE Rowan, Z Rubin, JG Ruzicka, P Sahlmueller, B Saito, N Sakaguchi, T Sakashita, K Sako, H Samsonov, V Sano, S Sarsour, M Sato, S Sato, T Sawada, S Schaefer, B Schmoll, BK Sedgwick, K Seele, J Seidl, R Sen, A Seto, R Sett, P Sexton, A Sharma, D Shein, I Shibata, TA Shigaki, K Shimomura, M Shoji, K Shukla, P Sickles, A Silva, CL Silvermyr, D Silvestre, C Sim, KS Singh, BK Singh, CP Singh, V Slunecka, M Snowball, M Soltz, RA Sondheim, WE Sorensen, SP Sourikova, IV Stankus, PW Stenlund, E Stepanov, M Stoll, SP Sugitate, T Sukhanov, A Sumita, T Sun, J Sziklai, J Takagui, EM Taketani, A Tanabe, R Tanaka, Y Taneja, S Tanida, K Tannenbaum, MJ Tarafdar, S Taranenko, A Themann, H Thomas, D Thomas, TL Tieulent, R Timilsina, A Todoroki, T Togawa, M Toia, A Tomasek, L Tomasek, M Torii, H Towell, CL Towell, R Towell, RS Tserruya, I Tsuchimoto, Y Vale, C Valle, H van Hecke, HW Vazquez-Zambrano, E Veicht, A Velkovska, J Vertesi, R Virius, M Vrba, V Vznuzdaev, E Wang, XR Watanabe, D Watanabe, K Watanabe, Y Watanabe, YS Wei, F Wei, R Wessels, J White, AS White, SN Winter, D Woody, CL Wright, RM Wysocki, M Xia, B Xue, L Yalcin, S Yamaguchi, YL Yamaura, K Yang, R Yanovich, A Ying, J Yokkaichi, S Yoo, JH Yoon, I You, Z Young, GR Younus, I Yu, H Yushmanov, IE Zajc, WA Zelenski, A Zhou, S Zou, L AF Adare, A. 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CA PHENIX Collaboration TI phi meson production in d plus Au collisions at root s(NN)=200 GeV SO PHYSICAL REVIEW C LA English DT Article ID QUARK-GLUON PLASMA; PB COLLISIONS; LONG-RANGE; ANGULAR-CORRELATIONS; TRANSVERSE-MOMENTUM; NUCLEUS COLLISIONS; ENERGY; COLLABORATION; DEPENDENCE; DETECTOR AB The PHENIX Collaboration has measured phi meson production in d + Au collisions at root s(NN) = 200 GeV using the dimuon and dielectron decay channels. The phi meson is measured in the forward (backward) d-going (Au-going) direction, 1.2 < y < 2.2 (-2.2 < y < -1.2) in the transverse-momentum (pT) range from 1-7 GeV/c and at midrapidity vertical bar y vertical bar < 0.35 in the p(T) range below 7 GeV/c. The phi meson invariant yields and nuclear-modification factors as a function of p(T), rapidity, and centrality are reported. An enhancement of phi meson production is observed in the Au-going direction, while suppression is seen in the d-going direction, and no modification is observed at midrapidity relative to the yield in p + p collisions scaled by the number of binary collisions. Similar behavior was previously observed for inclusive charged hadrons and open heavy flavor, indicating similar cold-nuclear-matter effects. C1 [Basye, A. T.; Daugherity, M. S.; Hamilton, H. F.; Isenhower, D.; Jones, T.; Jumper, D. S.; Pinson, R.; Thomas, D.; Towell, C. L.; Towell, R.; Towell, R. S.; Wright, R. M.] Abilene Christian Univ, Abilene, TX 79699 USA. [Grau, N.] Augustana Coll, Dept Phys, Sioux Falls, SD 57197 USA. [Garg, P.; Singh, B. K.; Singh, C. P.; Singh, V.; Tarafdar, S.] Banaras Hindu Univ, Dept Phys, Varanasi 221005, Uttar Pradesh, India. [Choudhury, R. K.; Dutta, D.; Mishra, D. K.; Mohanty, A. K.; Netrakanti, P. K.; Sett, P.; Shukla, P.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. 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N.; Alexander, J.; Chung, P.; Jia, J.; Lacey, R.; Mwai, A.; Reynolds, D.; Taranenko, A.; Wei, R.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Apadula, N.; Averbeck, R.; Bannier, B.; Bennett, R.; Boyle, K.; Campbell, S.; Chen, C. -H.; Citron, Z.; Connors, M.; Dahms, T.; Dehmelt, K.; Deshpande, A.; Dion, A.; Drees, A.; Durham, J. M.; Feege, N.; Frantz, J. E.; Gal, C.; Ge, H.; Gong, H.; Hanks, J.; Hemmick, T. K.; Jacak, B. V.; Kamin, J.; Khachatryan, V.; Kline, P.; Lee, S. H.; Manion, A.; McCumber, M.; Means, N.; Nguyen, M.; Novitzky, N.; Pantuev, V.; Petti, R.; Proissl, M.; Sahlmueller, B.; Sharma, D.; Sun, J.; Taneja, S.; Themann, H.; Toia, A.; Yalcin, S.; Yamaguchi, Y. L.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Garishvili, I.; Hamblen, J.; Hornback, D.; Nattrass, C.; Read, K. F.; Schmoll, B. K.; Sen, A.; Sorensen, S. P.] Univ Tennessee, Knoxville, TN 37996 USA. [Miyasaka, S.; Nakano, K.; Sakashita, K.; Shibata, T. -A.] Tokyo Inst Technol, Dept Phys, Meguro Ku, Tokyo 1528551, Japan. [Chujo, T.; Esumi, S.; Ikeda, Y.; Inaba, M.; Konno, M.; Masui, H.; Miake, Y.; Miki, K.; Mizuno, S.; Nakagomi, H.; Niida, T.; Oka, M.; Sato, T.; Shimomura, M.; Tanabe, R.; Todoroki, T.; Watanabe, K.] Univ Tsukuba, Inst Phys, Tsukuba, Ibaraki 305, Japan. [Belmont, R.; Danchev, I.; Greene, S. V.; Huang, S.; Issah, M.; Love, B.; Maguire, C. F.; Roach, D.; Schaefer, B.; Valle, H.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Kikuchi, J.; Sano, S.] Waseda Univ, Adv Res Inst Sci & Engn, Shinjuku Ku, Tokyo 1620044, Japan. [Citron, Z.; Fraenkel, Z.; Milov, A.; Naglis, M.; Ravinovich, I.; Sharma, D.; Tarafdar, S.; Tserruya, I.] Weizmann Inst Sci, IL-76100 Rehovot, Israel. [Csoergo, T.; Nagy, M. I.; Novak, T.; Sziklai, J.; Vertesi, R.] Hungarian Acad Sci Wigner RCP, Inst Particle & Nucl Phys, Wigner Res Ctr Phys, RMKI, H-1525 Budapest, Hungary. [Bhom, J. H.; Bok, J. S.; Choi, I. J.; Do, J. H.; Kang, J. H.; Kwon, Y.; Lee, S.; Lim, S. H.; Moon, T.] Yonsei Univ, IPAP, Seoul 120749, South Korea. [Makek, M.] Univ Zagreb, Dept Phys, Fac Sci, HR-10002 Zagreb, Croatia. RP Adare, A (reprint author), Univ Colorado, Boulder, CO 80309 USA. EM morrison@bnl.gov; jamie.nagle@colorado.edu RI Durum, Artur/C-3027-2014; Sen, Abhisek/J-1157-2016; Gu, Yi/B-6101-2016; Nattrass, Christine/J-6752-2016; Sorensen, Soren /K-1195-2016; Hayano, Ryugo/F-7889-2012; Yokkaichi, Satoshi/C-6215-2017; Taketani, Atsushi/E-1803-2017 OI Sen, Abhisek/0000-0003-1192-3938; Gu, Yi/0000-0003-4467-697X; Nattrass, Christine/0000-0002-8768-6468; Sorensen, Soren /0000-0002-5595-5643; Hayano, Ryugo/0000-0002-1214-7806; Taketani, Atsushi/0000-0002-4776-2315 FU Office of Nuclear Physics in the Office of Science of the Department of Energy (U.S.A); National Science Foundation (U.S.A); Abilene Christian University Research Council (U.S.A); Research Foundation of SUNY (U.S.A); Dean of the College of Arts and Sciences, Vanderbilt University (U.S.A); Ministry of Education, Culture, Sports, Science, and Technology (Japan); Japan Society for the Promotion of Science (Japan); Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (Brazil); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (Brazil); Natural Science Foundation of China (Pople's Republic of China); Ministry of Science, Education, and Sports (Croatia); Ministry of Education, Youth and Sports (Czech Republic); Centre National de la Recherche Scientifique (France); Commissariat a l'Energie Atomique (France); Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung (Germany); Deutscher Akademischer Austausch Dienst (Germany); Alexander von Humboldt Stiftung (Germany); National Science Fund (Hungary); OTKA (Hungary); Karoly Robert University College (Hungary); Ch. Simonyi Fund (Hungary); Department of Atomic Energy (India); Department of Science and Technology (India); Israel Science Foundation (Israel); Basic Science Research Program through NRF of the Ministry of Education (Korea); Physics Department, Lahore University of Management Sciences (Pakistan); Ministry of Education and Science, Russian Academy of Sciences, Federal Agency of Atomic Energy (Russia); VR (Sweden); Wallenberg Foundation (Sweden); U.S. Civilian Research and Development Foundation for the Independent States of the Former Soviet Union; Hungarian American Enterprise Scholarship Fund; US-Israel Binational Science Foundation FX We thank the staff of the Collider-Accelerator and Physics Departments at Brookhaven National Laboratory and the staff of the other PHENIX participating institutions for their vital contributions. We acknowledge support from the Office of Nuclear Physics in the Office of Science of the Department of Energy, the National Science Foundation, Abilene Christian University Research Council, Research Foundation of SUNY, and Dean of the College of Arts and Sciences, Vanderbilt University (U.S.A); Ministry of Education, Culture, Sports, Science, and Technology and the Japan Society for the Promotion of Science (Japan); Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (Brazil); Natural Science Foundation of China (Pople's Republic of China); Ministry of Science, Education, and Sports (Croatia); Ministry of Education, Youth and Sports (Czech Republic); Centre National de la Recherche Scientifique, Commissariat a l'Energie Atomique, and Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung, Deutscher Akademischer Austausch Dienst, and Alexander von Humboldt Stiftung (Germany); National Science Fund, OTKA, Karoly Robert University College, and the Ch. Simonyi Fund (Hungary); Department of Atomic Energy and Department of Science and Technology (India); Israel Science Foundation (Israel); Basic Science Research Program through NRF of the Ministry of Education (Korea); Physics Department, Lahore University of Management Sciences (Pakistan); Ministry of Education and Science, Russian Academy of Sciences, Federal Agency of Atomic Energy (Russia); VR and Wallenberg Foundation (Sweden); the U.S. Civilian Research and Development Foundation for the Independent States of the Former Soviet Union, the Hungarian American Enterprise Scholarship Fund, and the US-Israel Binational Science Foundation. NR 54 TC 4 Z9 4 U1 7 U2 25 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 19 PY 2015 VL 92 IS 4 AR 044909 DI 10.1103/PhysRevC.92.044909 PG 14 WC Physics, Nuclear SC Physics GA CT7SF UT WOS:000363014100010 ER PT J AU Allmond, JM Stuchbery, AE Galindo-Uribarri, A Padilla-Rodal, E Radford, DC Batchelder, JC Bingham, CR Howard, ME Liang, JF Manning, B Pain, SD Stone, NJ Varner, RL Yu, CH AF Allmond, J. M. Stuchbery, A. E. Galindo-Uribarri, A. Padilla-Rodal, E. Radford, D. C. Batchelder, J. C. Bingham, C. R. Howard, M. E. Liang, J. F. Manning, B. Pain, S. D. Stone, N. J. Varner, R. L. Yu, C. -H. TI Investigation into the semimagic nature of the tin isotopes through electromagnetic moments SO PHYSICAL REVIEW C LA English DT Article ID RELATIVISTIC QRPA; SN ISOTOPES; STATES; NUCLEI; COLLECTIVITY; SN-116 AB A complete set of electromagnetic moments, B(E2; 0(1)(+) -> 2(1)(+)), Q(2(1)(+)), and g(2(1)(+)), have been measured from Coulomb excitation of semimagic 112,114,116,118,120,122,124Sn (Z = 50) on natural carbon and titanium targets. The magnitude of the B(E2) values, measured to a precision of similar to 4%, disagree with a recent lifetime study [Phys. Lett. B 695, 110 (2011)] that employed the Doppler-shift attenuation method. The B(E2) values show an overall enhancement compared with recent theoretical calculations and a clear asymmetry about midshell, contrary to naive expectations. A new static electric quadrupole moment, Q(2(1)(+)), has been measured for Sn-114. The static quadrupole moments are generally consistent with zero but reveal an enhancement near midshell; this had not been previously observed. The magnetic dipole moments are consistent with previous measurements and show a near monotonic decrease in value with neutron number. The g-factor measurements in Sn-112,Sn-114 establish the recoil-in-vacuum method for states with tau similar to 0.5 ps and hence demonstrate that this method can be used for future g-factor measurements on proton-rich isotopes toward Sn-100. Current theory calculations fail to reproduce the electromagnetic moments of the tin isotopes. The role of 2p-2h and 4p-4h intruders, which are lowest in energy at midshell and outside of current model spaces, needs to be investigated in the future. C1 [Allmond, J. M.; Galindo-Uribarri, A.; Radford, D. C.; Bingham, C. R.; Liang, J. F.; Pain, S. D.; Varner, R. L.; Yu, C. -H.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Stuchbery, A. E.] Australian Natl Univ, Dept Nucl Phys, Canberra, ACT 2601, Australia. [Galindo-Uribarri, A.; Bingham, C. R.; Stone, N. J.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Padilla-Rodal, E.] Univ Nacl Autonoma Mexico, Inst Ciencias Nucl, Mexico City 04510, DF, Mexico. [Batchelder, J. C.] Oak Ridge Associated Univ, UNIRIB, Oak Ridge, TN 37831 USA. [Howard, M. E.; Manning, B.] Rutgers State Univ, Dept Phys & Astron, New Brunswick, NJ 08903 USA. [Stone, N. J.] Univ Oxford, Dept Phys, Oxford OX1 3PU, England. RP Allmond, JM (reprint author), Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. RI Pain, Steven/E-1188-2011; OI Pain, Steven/0000-0003-3081-688X; Allmond, James Mitchell/0000-0001-6533-8721 FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics; Australian Research Council [DP0773273]; CONACyT (Mexico) [CB103366]; National Science Foundation; DOE [DE-AC05-76OR00033, DE-FG02-96ER40963, DE-FG52-08NA28552] FX The authors gratefully acknowledge D. Cline, A.B. Hayes, N. Warr, and J.L. Wood for fruitful discussions, J.P. Greene (Argonne National Laboratory) for making the carbon and titanium targets, and the HRIBF operations staff for providing the beams used in this study. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics and this research used resources of the Holifield Radioactive Ion Beam Facility of Oak Ridge National Laboratory, which is a DOE Office of Science User Facility. This research was also sponsored by the Australian Research Council under Grant No. DP0773273, by CONACyT (Mexico) under Grant No. CB103366, and by the National Science Foundation. In addition, this work was supported in part by the U.S. DOE under Contracts No. DE-AC05-76OR00033 (UNIRIB), No. DE-FG02-96ER40963 (UTK), and No. DE-FG52-08NA28552 (Rutgers). NR 48 TC 7 Z9 7 U1 3 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 19 PY 2015 VL 92 IS 4 AR 041303 DI 10.1103/PhysRevC.92.041303 PG 5 WC Physics, Nuclear SC Physics GA CT7SF UT WOS:000363014100001 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TP Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I 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Y.; Ozturk, N.; Schovancova, J.; Sosebee, M.; Stradling, A. R.; Usai, G.; Vartapetian, A.; White, A.; Yu, J.] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA. [Angelidakis, S.; Chouridou, S.; Fassouliotis, D.; Giokaris, N.; Ioannou, P.; Kourkoumelis, C.; Manousakis-Katsikakis, A.; Tsirintanis, N.] Univ Athens, Dept Phys, Athens, Greece. [Alexopoulos, T.; Benekos, N.; Dris, M.; Gazis, E. N.; Karakostas, K.; Karastathis, N.; Leontsinis, S.; Maltezos, S.; Ntekas, K.; Panagiotopoulou, E.; Papadopoulou, Th. D.; Tsipolitis, G.; Vlachos, S.] Natl Tech Univ Athens, Dept Phys, Zografos, Greece. [Abdinov, O.; Khalil-Zada, F.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Anjos, N.; Bosman, M.; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fischer, C.; Fracchia, S.; Giangiobbe, V.; Parra, G. Gonzalez; Grinstein, S.; Rozas, A. Juste; Korolkov, I.; Lange, J. C.; Le Menedeu, E.; Paz, I. Lopez; Martinez, M.; Mir, L. M.; Berlingen, J. Montejo; Pages, A. Pacheco; Aranda, C. Padilla; Riu, I.; Sorin, V.; Succurro, A.; Tripiana, M. F.; Tsiskaridze, S.; Valery, L.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Anjos, N.; Bosman, M.; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fischer, C.; Fracchia, S.; Giangiobbe, V.; Parra, G. Gonzalez; Grinstein, S.; Rozas, A. Juste; Korolkov, I.; Lange, J. C.; Le Menedeu, E.; Paz, I. Lopez; Martinez, M.; Mir, L. M.; Berlingen, J. Montejo; Pages, A. Pacheco; Aranda, C. Padilla; Riu, I.; Sorin, V.; Succurro, A.; Tripiana, M. F.; Tsiskaridze, S.; Valery, L.] Univ Autonoma Barcelona, Dept Fis, E-08193 Barcelona, Spain. [Agatonovic-Jovin, T.; Bogavac, D.; Bozic, I.; Dimitrievska, A.; Krstic, J.; Marjanovic, M.; Popovic, D. S.; Sijacki, Dj.; Simic, Lj.; Vranjes, N.; Milosavljevic, M. Vranjes; Zivkovic, L.] Univ Belgrade, Inst Phys, Belgrade, Serbia. [Buanes, T.; Dale, O.; Eigen, G.; Kastanas, A.; Liebig, W.; Lipniacka, A.; Maeland, S.; Latour, B. Martin Dit; Rosendahl, P. L.; Sandaker, H.; Sjursen, T. B.; Smestad, L.; Stugu, B.; Ugland, M.; Zalieckas, J.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Amadio, B. T.; Axen, B.; Barnett, R. M.; Beringer, J.; Brosamer, J.; Calafiura, P.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Amadio, B. T.; Axen, B.; Barnett, R. M.; Beringer, J.; Brosamer, J.; Calafiura, P.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Biedermann, D.; Dietrich, J.; Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Herrberg-Schubert, R.; Hristova, I.; Kind, O. M.; Kolanoski, H.; Lacker, H.; Lohse, T.; Nikiforov, A.; Rehnisch, L.; Rieck, P.; Schulz, H.; Stamm, S.; zur Nedden, M.] Humboldt Univ, Dept Phys, Berlin, Germany. [Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Mullier, G. A.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Mullier, G. A.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allbrooke, B. M. M.; Bella, L. Aperio; Bansil, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Owen, R. E.; Slater, M.; Teoh, J. J.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Alberghi, G. L.; Bellagamba, L.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Corradi, M.; Dafinca, A.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, Bologna, Italy. [Alberghi, G. L.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Bruscino, N.; Cioara, I. A.; Cristinziani, M.; Czirr, H.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Hageboeck, S.; Hallewell, G. D.; Hamacher, K.; Hansen, M. C.; Hellmich, D.; Hohn, D.; Huegging, F.; Janssen, J.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mergelmeyer, S.; Mijovic, L.; Mueller, K.; Obermann, T.; Pohl, D.; Ricken, O.; Sarrazin, B.; Schaepe, S.; Schopf, E.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Seema, P.; Stillings, J. A.; Tannoury, N.; Therhaag, J.; Uhlenbrock, M.; Velz, T.; Von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Dhaliwal, S.; Fitzgerald, E. A.; Sciolla, G.; Venturini, A.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE, EE, IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Fed Univ Juiz de Fora UFJF, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Navarro, J. L. La Rosa; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Horia Hulubei Natl Inst Phys & Nucl Engn, Bucharest 077125, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. [Popeneciu, G. A.] Univ Politehn Bucuresti, Bucharest, Romania. [Popeneciu, G. A.] West Univ Timisoara, Timisoara, Romania. [Garzon, G. Otero Y.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Crosetti, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Gonzalez, B. Alvarez; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Iengo, P.; Jaekel, M. R.; Jakobsen, S.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sforza, F.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.; Wang, C.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Shanghai Key Lab Particle Phys & Cosmol, Dept Phys & Astron, Shanghai 200030, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Collegato Cosenza, Lab Nazl Frascati, Frascati, Italy. [Cairo, V. M.; Capua, M.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Hamal, P.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamer, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Yildirim, E.] DESY, Hamburg, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Wasicki, C.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; Von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Ancu, L. S.; Barone, G.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Clark, A.; Delitzsch, C. M.; Della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Paolozzi, L.; Picazio, A.; Ristic, B.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Kareem, M. J.; Kawamura, G.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Donszelmann, T. Cuhadar; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Guimaraes da Costa, J. Barreiro; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E-E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R. W.; Jussel, P.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, S.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Allport, P. P.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Egham, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Cummings, J.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Cummings, J.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Cummings, J.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fys Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. 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M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. 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A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; Von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; Czodrowski, P.; De Groot, N.; Filthaut, F.; Galea, C.; Koenig, A. C.; Nektarijevic, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; De Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; De Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Hamilton, A.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hrabovsky, M.; Jeanty, L.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hakobyan, H.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hakobyan, H.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Cuthbert, C.; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Fletcher, R. R. M.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Techn Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Halladjian, G.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Goncalves Pinto Firmino Da Costa, J.; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, DSM IRFU Inst Rech Lois Fondament Univers, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Mount, R.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Meehan, S.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Govender, N.; Lee, C. A.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Curatolo, M.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Curatolo, M.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Munwes, Y.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. 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[Canepa, A.; Chekulaev, S. V.; Jovicevic, J.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; McPherson, R. A.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Shaw, K.; Soualah, R.; Truong, L.] Ist Nazl Fis Nucl, Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Neubauer, M. S.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. 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RI White, Ryan/E-2979-2015; Mashinistov, Ruslan/M-8356-2015; spagnolo, stefania/A-6359-2012; Buttar, Craig/D-3706-2011; Tripiana, Martin/H-3404-2015; Smirnova, Oxana/A-4401-2013; Savarala, Hari Krishna/A-3516-2015; Doyle, Anthony/C-5889-2009; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Tikhomirov, Vladimir/M-6194-2015; Di Domenico, Antonio/G-6301-2011; Carvalho, Joao/M-4060-2013; Mitsou, Vasiliki/D-1967-2009; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Livan, Michele/D-7531-2012; Brooks, William/C-8636-2013; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Peleganchuk, Sergey/J-6722-2014; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Tartarelli, Giuseppe Francesco/A-5629-2016; la rotonda, laura/B-4028-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; Staroba, Pavel/G-8850-2014; Gavrilenko, Igor/M-8260-2015; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Fabbri, Laura/H-3442-2012; Gutierrez, Phillip/C-1161-2011; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Boyko, Igor/J-3659-2013; Vranjes Milosavljevic, Marija/F-9847-2016; Zhukov, Konstantin/M-6027-2015; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Fedin, Oleg/H-6753-2016; Snesarev, Andrey/H-5090-2013; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; Villa, Mauro/C-9883-2009; BESSON, NATHALIE/L-6250-2015; Vanadia, Marco/K-5870-2016 OI White, Ryan/0000-0003-3589-5900; Mashinistov, Ruslan/0000-0001-7925-4676; spagnolo, stefania/0000-0001-7482-6348; Smirnova, Oxana/0000-0003-2517-531X; Savarala, Hari Krishna/0000-0001-6593-4849; Doyle, Anthony/0000-0001-6322-6195; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Tikhomirov, Vladimir/0000-0002-9634-0581; Di Domenico, Antonio/0000-0001-8078-2759; Carvalho, Joao/0000-0002-3015-7821; Mitsou, Vasiliki/0000-0002-1533-8886; Warburton, Andreas/0000-0002-2298-7315; Livan, Michele/0000-0002-5877-0062; Brooks, William/0000-0001-6161-3570; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Andreazza, Attilio/0000-0001-5161-5759; Sotiropoulou, Calliope-Louisa/0000-0001-9851-1658; Prokofiev, Kirill/0000-0002-2177-6401; Veneziano, Stefano/0000-0002-2598-2659; Lacasta, Carlos/0000-0002-2623-6252; Price, Darren/0000-0003-2750-9977; Terzo, Stefano/0000-0003-3388-3906; Smirnov, Sergei/0000-0002-6778-073X; Belanger-Champagne, Camille/0000-0003-2368-2617; Cristinziani, Markus/0000-0003-3893-9171; Haas, Andrew/0000-0002-4832-0455; Galhardo, Bruno/0000-0003-0641-301X; Castro, Nuno/0000-0001-8491-4376; Della Volpe, Domenico/0000-0001-8530-7447; Pina, Joao /0000-0001-8959-5044; Farrington, Sinead/0000-0001-5350-9271; Robson, Aidan/0000-0002-1659-8284; Grohsjean, Alexander/0000-0003-0748-8494; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Sannino, Mario/0000-0001-7700-8383; Vari, Riccardo/0000-0002-2814-1337; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Gray, Heather/0000-0002-5293-4716; la rotonda, laura/0000-0002-6780-5829; Amorim, Antonio/0000-0003-0638-2321; Coccaro, Andrea/0000-0003-2368-4559; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Gauzzi, Paolo/0000-0003-4841-5822; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Boyko, Igor/0000-0002-3355-4662; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Villa, Mauro/0000-0002-9181-8048; Vanadia, Marco/0000-0003-2684-276X FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF Helmholtz Association, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; RGC, China; Hong Kong SAR, China; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF Helmholtz Association, and AvH Foundation, Germany; GSRT and NSRF, Greece; RGC, Hong Kong SAR, China; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 55 TC 3 Z9 3 U1 13 U2 67 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 19 PY 2015 VL 92 IS 7 AR 072005 DI 10.1103/PhysRevD.92.072005 PG 31 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CT7SL UT WOS:000363014700002 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Knuenz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Ochesanu, S Rougny, R Van de Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F Blyweert, S D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Maes, M Moreels, L Olbrechts, A Python, Q 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Hindrichs, O. Khukhunaishvili, A. Petrillo, G. Verzetti, M. Demortier, L. Arora, S. Barker, A. Chou, J. P. Contreras-Campana, C. Contreras-Campana, E. Duggan, D. Ferencek, D. Gershtein, Y. Gray, R. Halkiadakis, E. Hidas, D. Hughes, E. Kaplan, S. Elayavalli, R. Kunnawalkam Lath, A. Panwalkar, S. Park, M. Salur, S. Schnetzer, S. Sheffield, D. Somalwar, S. Stone, R. Thomas, S. Thomassen, P. Walker, M. Foerster, M. Riley, G. Rose, K. Spanier, S. York, A. Bouhali, O. Hernandez, A. Castaneda Dalchenko, M. De Mattia, M. Delgado, A. Dildick, S. Eusebi, R. Flanagan, W. Gilmore, J. Kamon, T. Krutelyov, V. Montalvo, R. Mueller, R. Osipenkov, I. Pakhotin, Y. Patel, R. Perloff, A. Roe, J. Rose, A. Safonov, A. Tatarinov, A. Ulmer, K. A. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kunori, S. Lamichhane, K. Lee, S. W. Libeiro, T. Undleeb, S. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Janjam, R. Johns, W. Maguire, C. Mao, Y. Melo, A. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Xu, Q. Arenton, M. W. Boutle, S. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Wolfe, E. Wood, J. Xia, F. Clarke, C. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Sturdy, J. Belknap, D. A. Carlsmith, D. Cepeda, M. Christian, A. Dasu, S. Dodd, L. Duric, S. Friis, E. Gomber, B. Grothe, M. Hall-Wilton, R. Herndon, M. Herv, A. Klabbers, P. Lanaro, A. Levine, A. Long, K. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Ruggles, T. Sarangi, T. Savin, A. Sharma, A. Smith, N. Smith, W. H. Taylor, D. Woods, N. CA CMS Collaboration TI Search for supersymmetry with photons in pp collisions at root s=8 TeV SO PHYSICAL REVIEW D LA English DT Article ID MISSING TRANSVERSE-MOMENTUM; PARTON DISTRIBUTIONS; ATLAS DETECTOR; BREAKING; LHC; GRAVITINO; EVENTS; ENERGY; MODELS; SQUARK AB Two searches for physics beyond the standard model in events containing photons are presented. The data sample used corresponds to an integrated luminosity of 19.7 fb(-1) of proton-proton collisions at root s = 8 TeV, collected with the CMS experiment at the CERN LHC. The analyses pursue different inclusive search strategies. One analysis requires at least one photon, at least two jets, and a large amount of transverse momentum imbalance, while the other selects events with at least two photons and at least one jet, and uses the razor variables to search for signal events. The background expected from standard model processes is evaluated mainly from data. The results are interpreted in the context of general gauge-mediated supersymmetry, with the next-to-lightest supersymmetric particle either a bino- or wino-like neutralino, and within simplified model scenarios. Upper limits at the 95% confidence level are obtained for cross sections as functions of the masses of the intermediate supersymmetric particles. C1 [Khachatryan, V.; Sirunyan, A. 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F.; Verlage, T.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Ata, M.; Brodski, M.; Dietz-Laursonn, E.; Duchardt, D.; Endres, M.; Erdmann, M.; Erdweg, S.; Esch, T.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Millet, P.; Olschewski, M.; Padeken, K.; Papacz, P.; Pook, T.; Radziej, M.; Reithler, H.; Rieger, M.; Scheuch, F.; Sonnenschein, L.; Teyssier, D.; Thueer, S.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Kuensken, A.; Lingemann, J.; Nehrkorn, A.; Nowack, A.; Nugent, I. M.; Pistone, C.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B 3, Aachen, Germany. [Martin, M. Aldaya; Asin, I.; Bartosik, N.; Behnke, O.; Behrens, U.; Bell, A. J.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. Diez; Dolinska, G.; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Gallo, E.; Garcia, J. Garay; Geiser, A.; Gizhko, A.; Gunnellini, P.; Hauk, J.; Hempel, M.; Jung, H.; Kalogeropoulos, A.; Karacheban, O.; Kasemann, M.; Katsas, P.; Kieseler, J.; Kleinwort, C.; Korol, I.; Lange, W.; Leonard, J.; Lipka, K.; Lobanov, A.; Lohmann, W.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mittag, G.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Nayak, A.; Ntomari, E.; Perrey, H.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Cipriano, P. M. Ribeiro; Roland, B.; Sahin, M. Oe.; Salfeld-Nebgen, J.; Saxena, P.; Schoerner-Sadenius, T.; Schroeder, M.; Seitz, C.; Spannagel, S.; Trippkewitz, K. D.; Wissing, C.] DESY, Hamburg, Germany. [Blobel, V.; Vignali, M. Centis; Draeger, A. 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Lobelle; Maier, B.; Mildner, H.; Mozer, M. U.; Mueller, T.; Mueller, Th.; Plagge, M.; Printz, M.; Quast, G.; Rabbertz, K.; Roecker, S.; Roscher, F.; Shvetsov, I.; Sieber, G.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Williamson, S.; Woehrmann, C.; Wolf, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Markou, A.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Tziaferi, E.; Sphicas, P.] Univ Athens, GR-10679 Athens, Greece. [Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Loukas, N.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hazi, A.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.; Bartok, M.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Vesztergombi, G.; Bartok, M.; Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.; Veres, G. I.] Univ Debrecen, Debrecen, Hungary. [Mal, P.; Mandal, K.; Sahoo, N.; Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Bansal, S.; Beri, S. B.; Bhatnagar, V.; Chawla, R.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, A.; Kaur, M.; Kumar, R.; Mehta, A.; Mittal, M.; Nishu, N.; Singh, J. B.; Walia, G.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Bhardwaj, A.; Choudhary, B. C.; Garg, R. B.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Sharma, R.; Sharma, V.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dey, S.; Dutta, S.; Jain, Sa.; Jain, Sh.; Khurana, R.; Majumdar, N.; Modak, A.; Mondal, K.; Mukherjee, S.; Mukhopadhyay, S.; Roy, A.; Roy, D.; Chowdhury, S. Roy; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Chudasama, R.; Dutta, D.; Jha, V.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Mumbai 400085, Maharashtra, India. [Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Mahakud, B.; Maity, M.; Majumder, G.; Mazumdar, K.; Mitra, S.; Mohanty, G. B.; Parida, B.; Sarkar, T.; Sudhakar, K.; Sur, N.; Sutar, B.; Wickramage, N.] Tata Inst Fundamental Res, Mumbai 400005, Maharashtra, India. [Sharma, S.] IISER, Pune, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Ranieri, A.; Selvaggi, G.; Silvestris, L.; Venditti, R.; Verwilligen, P.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Calabria, C.; Caputo, C.; Chhibra, S. S.; Cristella, L.; De Palma, M.; Miniello, G.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Battilana, C.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Giordano, F.] CSFNSM, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.; Viliani, L.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.; Viliani, L.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Manzoni, R. A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.; Thyssen, F.] Ist Nazl Fis Nucl, Sez Napoli, Rome, Italy. [Esposito, M.; Iorio, A. O. M.; Sciacca, C.] Univ Naples Federico II, Rome, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, Rome, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Carlin, R.; De Oliveira, A. Carvalho Antunes; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Passaseo, M.; Pazzini, J.; Pegoraro, M.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Trento, Italy. [Bisello, D.; Carlin, R.; De Oliveira, A. Carvalho Antunes; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Trento, Italy. Univ Trento, Trento, Italy. [Braghieri, A.; Gabusi, M.; Magnani, A.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Solestizi, L. Alunni; Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Solestizi, L. Alunni; Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fedi, G.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Micheli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; De Remigis, P.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Musich, M.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.] Ist Nazl Fis Nucl, Sez Torino, Novara, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.] Univ Torino, Novara, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Daegu, South Korea. [Cifuentes, J. A. Brochero; Kim, H.; Kim, T. J.; Ryu, M. S.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Lee, S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.; Vaitkus, J.] Vilnius State Univ, Vilnius, Lithuania. [Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Duran, C.; Heredia-De La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Guisao, J. Mejia; Trejo, R. I. 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[Brona, G.; Bunkowski, K.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Finger, M.; Finger, M., Jr.; Tsamalaidze, Z.; Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Matveev, V.; Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Karapostoli, G.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Bylinkin, A.; Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Baskakov, A.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Myagkov, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Milenovic, P.; Mermerkaya, H.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] CIEMAT, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Genchev, V.; Merlin, J. A.; Lingemann, J.; Pantaleo, F.; Hartmann, F.; Kassel, F.; Kornmayer, A.; Mohanty, A. K.; Silvestris, L.; Battilana, C.; Di Guida, S.; Meola, S.; Paolucci, P.; Azzi, P.; Dall'Osso, M.; Zucchetta, A.; Ciangottini, D.; Donato, S.; D'imperio, G.; Traczyk, P.; Finco, L.; Candelise, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; du Pree, T.; Dupont, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Marrouche, J.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Zagozdzinska, A.; Zeuner, W. D.; Yetkin, T.; Ulmer, K. A.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Rohe, T.; Bachmair, F.; Baeni, L.; Bianchini, L.; Buchmann, M. A.; Casal, B.; Dissertori, G.; Dittmar, M.] Paul Scherrer Inst, Villigen, Switzerland. [Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marini, A. C.; Marionneau, M.; Del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Peruzzi, M.; Quittnat, M.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.; Weber, H. A.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Salerno, D.; Taroni, S.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Ferro, C.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartek, R.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Onengut, G.; Ozdemir, K.; Polatoz, A.; Cerci, D. Sunar; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Surat, U. E.; Yalvac, M.; Zeyrek, M.; Albayrak, E. A.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Guelmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-Storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Thomas, L.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Cripps, N.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Sharp, P.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Borzou, A.; Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL 35487 USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Sagir, S.; Sinthuprasith, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Saltzberg, D.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Sumowidagdo, S.; Wei, H.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Justus, C.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Smith, J. G.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY 14853 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; GrNendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Hu, Z.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Kwan, S.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Whitbeck, A.; Yang, F.; Yin, H.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Di Giovanni, G. P.; Field, R. D.; Fisher, M.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Low, J. F.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rank, D.; Shchutska, L.; Snowball, M.; Sperka, D.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL 32611 USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Bhopatkar, V.; Hohlmann, M.; Kalakhety, H.; Mareskas-Palcek, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.] Univ Illinois, Chicago, IL 60607 USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tan, P.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA 52242 USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Nash, K.; Osherson, M.; Swartz, M.; Xiao, M.; Xin, Y.] Johns Hopkins Univ, Baltimore, MD 21218 USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Gray, J.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Chakaberia, I.; Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Skhirtladze, N.; Svintradze, I.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Pedro, K.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Baty, A.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Mcginn, C.; Niu, X.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Sumorok, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN 55455 USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, University, MS 38677 USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.] Univ Nebraska, Lincoln, NE 68588 USA. [Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Trovato, M.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL 60208 USA. [Brinkerhoff, A.; Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Lynch, S.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Pearson, T.; Planer, M.; Ruchti, R.; Smith, G.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08542 USA. [Savoy-Navarro, A.; Barnes, V. E.; Benedetti, D.; Bortoletto, D.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Miller, D. H.; Neumeister, N.; Primavera, F.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Zablocki, J.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, IN 46323 USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Li, W.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX 77251 USA. [Betchart, B.; Bodek, A.; De Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Hindrichs, O.; Khukhunaishvili, A.; Petrillo, G.; Verzetti, M.] Univ Rochester, Rochester, NY 14627 USA. [Demortier, L.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Hughes, E.; Kaplan, S.; Elayavalli, R. Kunnawalkam; Lath, A.; Panwalkar, S.; Park, M.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ 08854 USA. [Foerster, M.; Riley, G.; Rose, K.; Spanier, S.; York, A.; Bouhali, O.] Univ Tennessee, Knoxville, TN 37996 USA. [Hernandez, A. 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[Radi, A.; Salama, E.; Sayed, A.; Sphicas, P.] British Univ Egypt, Cairo, Egypt. [Tonelli Manganote, E. J.] Univ Haute Alsace, Mulhouse, France. [Hempel, M.; Karacheban, O.; Lohmann, W.; Marfin, I.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Bhowmik, S.; Maity, M.; Sarkar, T.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Plasma Phys Res Ctr, Sci & Res Branch, Tehran, Iran. [Ciocci, M. A.; Grippo, M. T.; Squillacioti, P.] Univ Siena, I-53100 Siena, Italy. [Ali, M. A. B. Md] Int Islamic Univ Malaysia, Kuala Lumpur, Malaysia. [Heredia-De La Cruz, I.] Consejo Nacl Invest Cient & Tecn, Mexico City, DF, Mexico. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Orfanelli, S.] Natl Tech Univ Athens, Athens, Greece. [Racz, A.] Ist Nazl Fis Nucl, Scuola Normale Sez, Pisa, Italy. [Zagozdzinska, A.] Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.] Gaziosmanpasa Univ, Tokat, Turkey. [Kangal, E. E.] Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. [Cerci, D. Sunar] Adiyaman Univ, Adiyaman, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Sen, S.] Hacettepe Univ, Ankara, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Acosta, M. Vazquez] Inst Astrofis Canarias, San Cristobal la Laguna, Spain. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. [Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Sguazzoni, Giacomo/J-4620-2015; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Paulini, Manfred/N-7794-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Dremin, Igor/K-8053-2015; ciocci, maria agnese /I-2153-2015; Lokhtin, Igor/D-7004-2012; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Della Ricca, Giuseppe/B-6826-2013; Azarkin, Maxim/N-2578-2015; Chinellato, Jose Augusto/I-7972-2012; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Stahl, Achim/E-8846-2011; Kirakosyan, Martin/N-2701-2015; Tinoco Mendes, Andre David/D-4314-2011; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Sznajder, Andre/L-1621-2016; Vilela Pereira, Antonio/L-4142-2016; Menasce, Dario/A-2168-2016; Paganoni, Marco/A-4235-2016; Ferguson, Thomas/O-3444-2014; de Jesus Damiao, Dilson/G-6218-2012; Dogra, Sunil /B-5330-2013; Leonidov, Andrey/M-4440-2013; Calvo Alamillo, Enrique/L-1203-2014; Hernandez Calama, Jose Maria/H-9127-2015; Cerrada, Marcos/J-6934-2014; Andreev, Vladimir/M-8665-2015; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Novaes, Sergio/D-3532-2012; TUVE', Cristina/P-3933-2015; Dudko, Lev/D-7127-2012; Manganote, Edmilson/K-8251-2013; Vinogradov, Alexey/O-2375-2015; Petrushanko, Sergey/D-6880-2012; Moraes, Arthur/F-6478-2010; VARDARLI, Fuat Ilkehan/B-6360-2013; Cakir, Altan/P-1024-2015; Montanari, Alessandro/J-2420-2012; Matorras, Francisco/I-4983-2015; Gennai, Simone/P-2880-2015 OI Sguazzoni, Giacomo/0000-0002-0791-3350; Demaria, Natale/0000-0003-0743-9465; Ciulli, Vitaliano/0000-0003-1947-3396; Androsov, Konstantin/0000-0003-2694-6542; Viliani, Lorenzo/0000-0002-1909-6343; ROMERO ABAD, DAVID/0000-0001-5088-9301; Gallinaro, Michele/0000-0003-1261-2277; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; ciocci, maria agnese /0000-0003-0002-5462; Boccali, Tommaso/0000-0002-9930-9299; Gerosa, Raffaele/0000-0001-8359-3734; Bilki, Burak/0000-0001-9515-3306; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982; Chinellato, Jose Augusto/0000-0002-3240-6270; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Stahl, Achim/0000-0002-8369-7506; Tinoco Mendes, Andre David/0000-0001-5854-7699; Seixas, Joao/0000-0002-7531-0842; Sznajder, Andre/0000-0001-6998-1108; Vilela Pereira, Antonio/0000-0003-3177-4626; Menasce, Dario/0000-0002-9918-1686; Paganoni, Marco/0000-0003-2461-275X; Ferguson, Thomas/0000-0001-5822-3731; de Jesus Damiao, Dilson/0000-0002-3769-1680; Calvo Alamillo, Enrique/0000-0002-1100-2963; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Cerrada, Marcos/0000-0003-0112-1691; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; TUVE', Cristina/0000-0003-0739-3153; Dudko, Lev/0000-0002-4462-3192; Moraes, Arthur/0000-0002-5157-5686; Montanari, Alessandro/0000-0003-2748-6373; Matorras, Francisco/0000-0003-4295-5668; FU BMWFW (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia); ERC IUT (Estonia); ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP (Republic of Korea); NRF (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (U.S.A.); NSF (U.S.A.); Marie-Curie program (European Union); European Research Council (European Union); EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS program of the Foundation for Polish Science; European Union; Regional Development Fund; Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR (Italy) [20108T4XTM]; EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); Welch Foundation FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP and NRF (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (U.S.A.). Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR Project No. 20108T4XTM (Italy); the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); and the Welch Foundation. NR 67 TC 0 Z9 0 U1 7 U2 39 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD OCT 19 PY 2015 VL 92 IS 7 AR 072006 DI 10.1103/PhysRevD.92.072006 PG 23 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CT7SL UT WOS:000363014700003 ER PT J AU Steimke, JL Steeper, TJ Colon-Mercado, HR Gorensek, MB AF Steimke, John L. Steeper, Timothy J. Colon-Mercado, Hector R. Gorensek, Maximilian B. TI Development and testing of a PEM SO2-depolarized electrolyzer and an operating method that prevents sulfur accumulation SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Electrolysis; Hybrid sulfur cycle; SO2-depolarized electrolysis; Sulfuric acid ID DIOXIDE DEPOLARIZED ELECTROLYSIS; HYDROGEN-PRODUCTION; ACID; SO2; MEMBRANES; WATER; CYCLE AB The hybrid sulfur (HyS) cycle is being developed as a technology to generate hydrogen by splitting water, using heat and electrical power from a nuclear or solar power plant. A key component is the SO2-depolarized electrolysis (SDE) cell, which reacts SO2 and water to form hydrogen and sulfuric acid. SDE could also be used in once-through operation to consume SO2 and generate hydrogen and sulfuric acid for sale. A proton exchange membrane (PEM) SDE cell based on a PEM fuel cell design was fabricated and tested. Measured cell potential as a function of anolyte pressure and flow rate, sulfuric acid concentration, and cell temperature are presented for this cell. Sulfur accumulation was observed inside the cell, which could have been a serious impediment to further development. A method to prevent sulfur formation was subsequently developed. This was made possible by a testing facility that allowed unattended operation for extended periods. Copyright (C) 2015, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Steimke, John L.; Steeper, Timothy J.; Colon-Mercado, Hector R.; Gorensek, Maximilian B.] Savannah River Natl Lab, Aiken, SC 29808 USA. RP Steimke, JL (reprint author), 1829 Robinson Dr, North Augusta, SC 29841 USA. EM johnsteimke@comcast.net FU US Department of Energy's Office of Nuclear Energy under the Nuclear Hydrogen Initiative; DOE's Office of Environmental Management (DOE-EM) by Savannah River Nuclear Solutions, LLC [DE-A C09-08SR22470] FX The authors gratefully acknowledge funding from the US Department of Energy's Office of Nuclear Energy under the Nuclear Hydrogen Initiative, for which Mr. Carl Sink was the program manager, and thank Dr. William A. Summers, who led SRNL's HyS development effort for his guidance and support. SRNL is operated for the DOE's Office of Environmental Management (DOE-EM) by Savannah River Nuclear Solutions, LLC under contract number DE-A C09-08SR22470. NR 28 TC 1 Z9 1 U1 4 U2 12 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 EI 1879-3487 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD OCT 19 PY 2015 VL 40 IS 39 BP 13281 EP 13294 DI 10.1016/j.ijhydene.2015.08.041 PG 14 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA CT2CB UT WOS:000362608500005 ER PT J AU Rahmani, A AF Rahmani, Armin TI Dynamics of noisy quantum systems in the Heisenberg picture: Application to the stability of fractional charge SO PHYSICAL REVIEW A LA English DT Article ID SOLITONS; STATES; PHASE AB Based on the Heisenberg-picture analog of the master equation, we develop a method for computing the exact time dependence of noise-averaged observables for general noninteracting fermionic systems with noisy fluctuations. Upon noise averaging, these fluctuations generate effective interactions, limiting analytical approaches. While the short-time dynamics can be studied with Langevin-type numerical simulations, the long-time limit is not amenable to such simulations. Our results provide access to this long-time limit. As a simple example, we examine the fate of the fractional charge in cold-atom emulations of polyacetylene after stochastic driving. We find that in a quantum quench to a fluctuating hopping Hamiltonian, the fractional charge remains robust for hopping between different sublattices, while it becomes unstable in the presence of noisy hopping on the same sublattice. C1 [Rahmani, Armin] Los Alamos Natl Lab, Div Theoret, T 4, Los Alamos, NM 87545 USA. [Rahmani, Armin] Los Alamos Natl Lab, CNLS, Los Alamos, NM 87545 USA. RP Rahmani, A (reprint author), Los Alamos Natl Lab, Div Theoret, T 4, POB 1663, Los Alamos, NM 87545 USA. FU U.S. Department of Energy under the LANL/LDRD program; NSERC; Max Planck-UBC Centre for Quantum Materials FX I am grateful to Cristian Batista, Adolfo del Campo, Claudio Chamon, Luca D'Alessio, Eugene Demler, Chang-Yu Hou, Ivar Martin, Anatoli Polkovnikov, and Kun Yang for helpful comments and discussions. This work was supported by the U.S. Department of Energy under the LANL/LDRD program, NSERC, and Max Planck-UBC Centre for Quantum Materials. NR 34 TC 1 Z9 1 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD OCT 19 PY 2015 VL 92 IS 4 AR 042110 DI 10.1103/PhysRevA.92.042110 PG 7 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CT7RI UT WOS:000363011800002 ER PT J AU Yakunin, KN Mezzacappa, A Marronetti, P Yoshida, S Bruenn, SW Hix, WR Lentz, EJ Messer, OEB Harris, JA Endeve, E Blondin, JM Lingerfelt, EJ AF Yakunin, Konstantin N. Mezzacappa, Anthony Marronetti, Pedro Yoshida, Shin'ichirou Bruenn, Stephen W. Hix, W. Raphael Lentz, Eric J. Messer, O. E. Bronson Harris, J. Austin Endeve, Eirik Blondin, John M. Lingerfelt, Eric J. TI Gravitational wave signatures of ab initio two-dimensional core collapse supernova explosion models for 12-25 M-circle dot stars SO PHYSICAL REVIEW D LA English DT Article ID ACCRETION SHOCK INSTABILITY; NEUTRINO-HYDRODYNAMICS SIMULATIONS; ADVECTIVE-ACOUSTIC CYCLE; ROTATING MASSIVE STARS; RELATIVISTIC SIMULATIONS; NEWTONIAN HYDRODYNAMICS; RADIATION HYDRODYNAMICS; NONLINEAR PHASE; 3 DIMENSIONS; CONVECTION AB We present the gravitational waveforms computed in ab initio two-dimensional core collapse supernova models evolved with the CHIMERA code for progenitor masses between 12 and 25 M-circle dot. All models employ multifrequency neutrino transport in the ray-by-ray approximation, state-of-the-art weak interaction physics, relativistic transport corrections such as the gravitational redshift of neutrinos, two-dimensional hydrodynamics with the commensurate relativistic corrections, Newtonian self-gravity with a general-relativistic monopole correction, and the Lattimer-Swesty equation of state with 220 MeV compressibility, and begin with the most recent Woosley-Heger nonrotating progenitors in this mass range. All of our models exhibit robust explosions. Therefore, our waveforms capture all stages of supernova development: 1) a relatively short and weak prompt signal, 2) a quiescent stage, 3) a strong signal due to convection and standing accretion shock instability activity, 4) termination of active accretion onto the proto-neutron star, and 5) a slowly increasing tail that reaches a saturation value. Fourier decomposition shows that the gravitational wave signals we predict should be observable by AdvLIGO for Galactic events across the range of progenitors considered here. The fundamental limitation of these models is in their imposition of axisymmetry. Further progress will require counterpart three-dimensional models, which are underway. C1 [Yakunin, Konstantin N.; Mezzacappa, Anthony; Hix, W. Raphael; Lentz, Eric J.; Messer, O. E. Bronson; Harris, J. Austin; Endeve, Eirik] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Yakunin, Konstantin N.; Mezzacappa, Anthony; Lentz, Eric J.] Oak Ridge Natl Lab, Joint Inst Computat Sci, Oak Ridge, TN 37831 USA. [Yakunin, Konstantin N.; Hix, W. Raphael; Lentz, Eric J.; Lingerfelt, Eric J.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Marronetti, Pedro; Messer, O. E. Bronson] Natl Sci Fdn, Div Phys, Arlington, VA 22230 USA. [Yoshida, Shin'ichirou] Univ Tokyo, Grad Sch Arts & Sci, Dept Earth Sci & Astron, Meguro Ku, Tokyo 1538902, Japan. [Bruenn, Stephen W.] Florida Atlantic Univ, Dept Phys, Boca Raton, FL 33431 USA. [Messer, O. E. Bronson] Oak Ridge Natl Lab, Natl Ctr Computat Sci, Oak Ridge, TN 37831 USA. [Endeve, Eirik; Lingerfelt, Eric J.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Blondin, John M.] N Carolina State Univ, Dept Phys, Raleigh, NC 27695 USA. RP Yakunin, KN (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. EM kyakunin@utk.edu RI Lentz, Eric/M-7173-2015; Hix, William/E-7896-2011; Messer, Bronson/G-1848-2012; Mezzacappa, Anthony/B-3163-2017 OI Lentz, Eric/0000-0002-5231-0532; Hix, William/0000-0002-9481-9126; Messer, Bronson/0000-0002-5358-5415; Mezzacappa, Anthony/0000-0001-9816-9741 FU U.S. Department of Energy Offices of Nuclear Physics and Advanced Scientific Computing Research; NASA [NNH08AH71I, NNH11AQ72I]; National Science Foundation [OCI-0749242, OCI-0749204, OCI-0749248] FX This research was supported by the U.S. Department of Energy Offices of Nuclear Physics and Advanced Scientific Computing Research; the NASA Astrophysics Theory and Fundamental Physics Program (Grants No. NNH08AH71I and NNH11AQ72I); and the National Science Foundation PetaApps Program (Grants No. OCI-0749242, OCI-0749204, and OCI-0749248). P. M. is supported by the National Science Foundation through its employee IR/D program. The opinions and conclusions expressed herein are those of the authors and do not represent the National Science Foundation. The authors would like to acknowledge fruitful discussions with Nelson Christensen. NR 84 TC 8 Z9 8 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD OCT 19 PY 2015 VL 92 IS 8 AR 084040 DI 10.1103/PhysRevD.92.084040 PG 13 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CT7SO UT WOS:000363015000006 ER PT J AU Lu, CH Hahn, EN Remington, BA Maddox, BR Bringa, EM Meyers, MA AF Lu, C-H. Hahn, E. N. Remington, B. A. Maddox, B. R. Bringa, E. M. Meyers, M. A. TI Phase Transformation in Tantalum under Extreme Laser Deformation SO SCIENTIFIC REPORTS LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; SHOCK COMPRESSION; TUNGSTEN ALLOYS; STRAIN-RATE; PRESSURE; METAL AB The structural and mechanical response of metals is intimately connected to phase transformations. For instance, the product of a phase transformation (martensite) is responsible for the extraordinary range of strength and toughness of steel, making it a versatile and important structural material. Although abundant in metals and alloys, the discovery of new phase transformations is not currently a common event and often requires a mix of experimentation, predictive computations, and luck. High-energy pulsed lasers enable the exploration of extreme pressures and temperatures, where such discoveries may lie. The formation of a hexagonal (omega) phase was observed in recovered monocrystalline body-centered cubic tantalum of four crystallographic orientations subjected to an extreme regime of pressure, temperature, and strain-rate. This was accomplished using high-energy pulsed lasers. The omega phase and twinning were identified by transmission electron microscopy at 70 GPa (determined by a corresponding VISAR experiment). It is proposed that the shear stresses generated by the uniaxial strain state of shock compression play an essential role in the transformation. Molecular dynamics simulations show the transformation of small nodules from body-centered cubic to a hexagonal close-packed structure under the same stress state (pressure and shear). C1 [Lu, C-H.; Hahn, E. N.; Meyers, M. A.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Remington, B. A.; Maddox, B. R.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Bringa, E. M.] Univ Nacl Cuyo, Fac Ciencias Exactas & Nat, RA-5500 Mendoza, Argentina. [Bringa, E. M.] Consejo Nacl Invest Cient & Tecn, RA-5500 Mendoza, Argentina. RP Meyers, MA (reprint author), Univ Calif San Diego, La Jolla, CA 92093 USA. EM mameyers@eng.ucsd.edu RI Meyers, Marc/A-2970-2016; OI Meyers, Marc/0000-0003-1698-5396; Hahn, Eric/0000-0002-2305-0532 FU UC Research Laboratories Grant [09-LR-06-118456-MEYM]; National Laser Users Facility (NLUF) Grant [PE-FG52-09NA-29043]; Oak Ridge National Laboratory by the Division of Scientific User Facilities, US Department of Energy; NIH FX This research is funded by the UC Research Laboratories Grant (09-LR-06-118456-MEYM) and the National Laser Users Facility (NLUF) Grant (PE-FG52-09NA-29043). Electron microscopy was conducted at the SHaRE User Facility, which is sponsored at Oak Ridge National Laboratory by the Division of Scientific User Facilities, US Department of Energy. We acknowledge the use of the UCSD Cryo-Electron Microscopy Facility which is supported by NIH grants to Dr. Timothy S. Baker and a gift from the Agouron Institute to UCSD. Computational resources were supported by DOE Office of Science, Office of Advanced Scientific Computing (ASCR) via the Exascale Co-design Center for Materials in Extreme Environments. NR 37 TC 3 Z9 3 U1 4 U2 31 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 19 PY 2015 VL 5 AR 15064 DI 10.1038/srep15064 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CT7IP UT WOS:000362988600001 PM 26478106 ER PT J AU MacLaren, I Sala, B Andersson, SML Pennycook, TJ Xiong, J Jia, QX Choi, EM MacManus-Driscoll, JL AF MacLaren, I. Sala, B. Andersson, S. M. L. Pennycook, T. J. Xiong, J. Jia, Q. X. Choi, E-M MacManus-Driscoll, J. L. TI Strain Localization in Thin Films of Bi(Fe,Mn)O-3 Due to the Formation of Stepped Mn4+-Rich Antiphase Boundaries SO NANOSCALE RESEARCH LETTERS LA English DT Article DE Bismuth ferrite; Scanning transmission electron microscopy (STEM); Strain; Thin films; Multiferroic; Antiphase boundaries AB The atomic structure and chemistry of thin films of Bi(Fe,Mn)O-3 (BFMO) films with a target composition of Bi2FeMnO6 on SrTiO3 are studied using scanning transmission electron microscopy imaging and electron energy loss spectroscopy. It is shown that Mn4+-rich antiphase boundaries are locally nucleated right at the film substrate and then form stepped structures that are approximately pyramidal in three dimensions. These have the effect of confining the material below the pyramids in a highly strained state with an out-of-plane lattice parameter close to 4.1 angstrom. Outside the area enclosed by the antiphase boundaries, the out-of-plane lattice parameter is much closer to bulk values for BFMO. This suggests that to improve the crystallographic perfection of the films whilst retaining the strain state through as much of the film as possible, ways need to be found to prevent nucleation of the antiphase boundaries. Since the antiphase boundaries seem to form from the interaction of Mn with the Ti in the substrate, one route to perform this would be to grow a thin buffer layer of pure BiFeO3 on the SrTiO3 substrate to minimise any Mn-Ti interactions. C1 [MacLaren, I.; Sala, B.; Andersson, S. M. L.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow G12 8QQ, Lanark, Scotland. [Pennycook, T. J.] STFC Daresbury Labs, SuperSTEM Lab, Keckwick Lane, Warrington WA4 4AD, Cheshire, England. [Pennycook, T. J.] Univ Oxford, Dept Mat, Parks Rd, Oxford OX1 3PH, England. [Xiong, J.; Jia, Q. X.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Xiong, J.] Univ Elect Sci & Technol China, State Key Lab Elect Thin Films & Integrated Devic, 4,Sect 2,North Jianshe Rd, Chengdu 610054, Peoples R China. [Choi, E-M; MacManus-Driscoll, J. L.] Univ Cambridge, Dept Mat Sci, 27 Charles Babbage Rd, Cambridge CB3 0FS, England. [Pennycook, T. J.] Univ Vienna, Phys Nanostruct Mat, Fac Phys, Boltzmanngasse 5, A-1090 Vienna, Austria. RP MacLaren, I (reprint author), Univ Glasgow, SUPA Sch Phys & Astron, Glasgow G12 8QQ, Lanark, Scotland. EM ian.maclaren@glasgow.ac.uk RI Pennycook, Timothy/B-4946-2014; MacLaren, Ian/C-1773-2010 OI Pennycook, Timothy/0000-0002-0008-6516; MacLaren, Ian/0000-0002-5334-3010 FU European Research Council [ERC-2009-AdG 247276 NOVOX]; LDRD programme; SUPA; University of Glasgow FX This work was supported by the European Research Council (ERC-2009-AdG 247276 NOVOX). The work at Los Alamos National Laboratory was supported by the LDRD programme and was performed at the Center for Integrated Nanotechnologies (CINT), an Office of Science User Facility operated for the US Department of Energy (DOE) Office of Science. The authors are indebted to the continuing support of the EPSRC for the SuperSTEM facility, which made this work possible. We are also grateful to SUPA and the University of Glasgow for the funding of the JEOL ARM200F, which was also used in this work. The assistance of Mr William (Billy) Smith in the preparation of the FIB specimen is gratefully acknowledged. NR 28 TC 0 Z9 0 U1 2 U2 16 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1556-276X J9 NANOSCALE RES LETT JI Nanoscale Res. Lett. PD OCT 17 PY 2015 VL 10 AR 407 DI 10.1186/s11671-015-1116-8 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA V46EH UT WOS:000209867000001 PM 26474888 ER PT J AU Lizarraga, LE Kaiser, JP Lambert, JC Wesselkamper, SC Zhao, QJ AF Lizarraga, L. E. Kaiser, J. P. Lambert, J. C. Wesselkamper, S. C. Zhao, Q. J. TI Alternative methods in human health risk assessment: Application of a tiered surrogate approach SO TOXICOLOGY LETTERS LA English DT Meeting Abstract CT 51st Congress of the European-Societies-of-Toxicology (EUROTOX) CY SEP 13-16, 2015 CL Portuguese Soc Pharmacol, Sect Toxicol, Porto, PORTUGAL SP European Soc Toxicol HO Portuguese Soc Pharmacol, Sect Toxicol C1 [Lizarraga, L. E.] Oak Ridge Associated Univ, Oak Ridge Inst Sci & Educ, Cincinnati, OH USA. [Kaiser, J. P.; Lambert, J. C.; Wesselkamper, S. C.; Zhao, Q. J.] US EPA, Natl Ctr Environm Assessment, Cincinnati, OH 45268 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER IRELAND LTD PI CLARE PA ELSEVIER HOUSE, BROOKVALE PLAZA, EAST PARK SHANNON, CO, CLARE, 00000, IRELAND SN 0378-4274 EI 1879-3169 J9 TOXICOL LETT JI Toxicol. Lett. PD OCT 16 PY 2015 VL 238 IS 2 SU S MA P03-022 BP S94 EP S95 DI 10.1016/j.toxlet.2015.08.314 PG 2 WC Toxicology SC Toxicology GA DE5SY UT WOS:000370693801151 ER PT J AU De Meyer, SE Parker, M Van Berkum, P Tian, R Seshadri, R Reddy, TBK Markowitz, V Ivanova, N Pati, A Woyke, T Kyrpides, N Howieson, J Reeve, W AF De Meyer, Sofie E. Parker, Matthew Van Berkum, Peter Tian, Rui Seshadri, Rekha Reddy, T. B. K. Markowitz, Victor Ivanova, Natalia Pati, Amrita Woyke, Tanja Kyrpides, Nikos Howieson, John Reeve, Wayne TI High-quality permanent draft genome sequence of the Mimosa asperata - nodulating Cupriavidus sp strain AMP6 SO STANDARDS IN GENOMIC SCIENCES LA English DT Article DE Root-nodule bacteria; Nitrogen fixation; Betaproteobacteria; Texas; Mimosa asperata; GEBA-RNB ID NITROGEN-FIXATION; MICROBIAL GENOMES; BURKHOLDERIA; BACTERIA; SYMBIONTS; TAIWANENSIS; DIVERSITY; NODULES; LEGUMES; SYSTEM AB Cupriavidus sp. strain AMP6 is an aerobic, motile, Gram-negative, non-spore-forming rod that was isolated from a root nodule of Mimosa asperata collected in Santa Ana National Wildlife Refuge, Texas, in 2005. Mimosa asperata is the only legume described so far to exclusively associates with Cupriavidus symbionts. Moreover, strain AMP6 represents an early-diverging lineage within the symbiotic Cupriavidus group and has the capacity to develop an effective nitrogen-fixing symbiosis with three other species of Mimosa. Therefore, the genome of Cupriavidus sp. strain AMP6 enables comparative analyses of symbiotic trait evolution in this genus and here we describe the general features, together with sequence and annotation. The 7,579,563 bp high-quality permanent draft genome is arranged in 260 scaffolds of 262 contigs, contains 7,033 protein-coding genes and 97 RNA-only encoding genes, and is part of the GEBA-RNB project proposal. C1 [De Meyer, Sofie E.; Tian, Rui; Howieson, John; Reeve, Wayne] Murdoch Univ, Ctr Rhizobium Studies, Murdoch, WA 6150, Australia. [Parker, Matthew] SUNY Binghamton, New York, NY USA. [Van Berkum, Peter] ARS, Soybean Genom & Improvement Lab, USDA, Beltsville, MD 20705 USA. [Seshadri, Rekha; Reddy, T. B. K.; Ivanova, Natalia; Pati, Amrita; Woyke, Tanja; Kyrpides, Nikos] DOE Joint Genome Inst, Walnut Creek, CA USA. [Markowitz, Victor] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Data Management & Technol Ctr, Berkeley, CA 94720 USA. King Abdulaziz Univ, Dept Biol Sci, Jeddah 21413, Saudi Arabia. RP Reeve, W (reprint author), Murdoch Univ, Ctr Rhizobium Studies, Murdoch, WA 6150, Australia. EM W.Reeve@murdoch.edu.au RI Kyrpides, Nikos/A-6305-2014; Fac Sci, KAU, Biol Sci Dept/L-4228-2013; OI Kyrpides, Nikos/0000-0002-6131-0462; Ivanova, Natalia/0000-0002-5802-9485 FU US Department of Energy's Office of Science, Biological and Environmental Research Program; University of California, Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; University of California, Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; University of California, Los Alamos National Laboratory [DE-AC02-06NA25396] FX This work was performed under the auspices of the US Department of Energy's Office of Science, Biological and Environmental Research Program, and by the University of California, Lawrence Berkeley National Laboratory under contract No. DE-AC02-05CH11231, Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344, and Los Alamos National Laboratory under contract No. DE-AC02-06NA25396. NR 50 TC 0 Z9 0 U1 3 U2 9 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD OCT 16 PY 2015 VL 10 AR 80 DI 10.1186/s40793-015-0074-1 PG 7 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DA7QQ UT WOS:000367999500002 PM 26478786 ER PT J AU De Meyer, SE Tian, R Seshadri, R Reddy, TBK Markowitz, V Ivanova, N Pati, A Woyke, T Kyrpides, N Yates, R Howieson, J Reeve, W AF De Meyer, Sofie E. Tian, Rui Seshadri, Rekha Reddy, T. B. K. Markowitz, Victor Ivanova, Natalia Pati, Amrita Woyke, Tanja Kyrpides, Nikos Yates, Ron Howieson, John Reeve, Wayne TI High-quality permanent draft genome sequence of the Lebeckia ambigua-nodulating Burkholderia sp strain WSM4176 SO STANDARDS IN GENOMIC SCIENCES LA English DT Article DE Root-nodule bacteria; Nitrogen fixation; Rhizobia; Betaproteobacteria; GEBA-RNB ID BACTERIA; SYSTEM; PREDICTION; LEGUMES; ACID; TOOL AB Burkholderia sp. strain WSM4176 is an aerobic, motile, Gram-negative, non-spore-forming rod that was isolated from an effective N-2-fixing root nodule of Lebeckia ambigua collected in Nieuwoudtville, Western Cape of South Africa, in October 2007. This plant persists in infertile, acidic and deep sandy soils, and is therefore an ideal candidate for a perennial based agriculture system in Western Australia. Here we describe the features of Burkholderia sp. strain WSM4176, which represents a potential inoculant quality strain for L. ambigua, together with sequence and annotation. The 9,065,247 bp high-quality-draft genome is arranged in 13 scaffolds of 65 contigs, contains 8369 protein-coding genes and 128 RNA-only encoding genes, and is part of the GEBA-RNB project proposal (Project ID 882). C1 [De Meyer, Sofie E.; Tian, Rui; Yates, Ron; Howieson, John; Reeve, Wayne] Murdoch Univ, Ctr Rhizobium Studies, Murdoch, WA 6150, Australia. [Seshadri, Rekha; Reddy, T. B. K.; Ivanova, Natalia; Pati, Amrita; Woyke, Tanja; Kyrpides, Nikos] DOE Joint Genome Inst, Walnut Creek, CA USA. [Markowitz, Victor] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Data Management & Technol Ctr, Berkeley, CA 94720 USA. [Kyrpides, Nikos] King Abdulaziz Univ, Dept Biol Sci, Jeddah 21413, Saudi Arabia. [Yates, Ron] Dept Agr & Food, Murdoch, WA, Australia. RP Reeve, W (reprint author), Murdoch Univ, Ctr Rhizobium Studies, Murdoch, WA 6150, Australia. EM W.Reeve@murdoch.edu.au RI Kyrpides, Nikos/A-6305-2014; Fac Sci, KAU, Biol Sci Dept/L-4228-2013; OI Kyrpides, Nikos/0000-0002-6131-0462; Ivanova, Natalia/0000-0002-5802-9485 FU University of California, Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; US Department of Energy Office of Science, Biological and Environmental Research Program; University of California, Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; University of California, Los Alamos National Laboratory [DE-AC02-06NA25396]; Murdoch University Strategic Research Fund through the Crop and Plant Research Institute (CaPRI); Centre for Rhizobium Studies (CRS) at Murdoch University FX This work was performed under the auspices of the US Department of Energy Office of Science, Biological and Environmental Research Program, and by the University of California, Lawrence Berkeley National Laboratory under contract No. DE-AC02-05CH11231, Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344, and Los Alamos National Laboratory under contract No. DE-AC02-06NA25396. We gratefully acknowledge the funding received from the Murdoch University Strategic Research Fund through the Crop and Plant Research Institute (CaPRI) and the Centre for Rhizobium Studies (CRS) at Murdoch University. NR 35 TC 0 Z9 0 U1 0 U2 5 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD OCT 16 PY 2015 VL 10 AR 79 DI 10.1186/s40793-015-0072-3 PG 7 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DA7QQ UT WOS:000367999500001 PM 26478785 ER PT J AU Herman, MF Currier, RP Clegg, SM AF Herman, Michael F. Currier, Robert P. Clegg, Samuel M. TI An isotopic mass effect on the intermolecular potential SO CHEMICAL PHYSICS LETTERS LA English DT Article ID INDEPENDENT FRACTIONATION; CROWN-ETHER; OXYGEN; CHEMISTRY; THERMODYNAMICS; STRONTIUM; INVERSE; ORIGIN; OZONE AB The impact of isotopic variation on the electronic energy and intermolecular potentials is often suppressed when calculating isotopologue thermodynamics. Intramolecular potential energy surfaces for distinct isotopologues are in fact equivalent under the Born-Oppenheimer approximation, which is sometimes used to imply that the intermolecular interactions are independent of isotopic mass. In this communication, the intermolecular dipole-dipole interaction between hetero-nuclear diatomic molecules is considered. It is shown that the intermolecular potential contains mass-dependent terms even though each nucleus moves on a Born-Oppenheimer surface. The analysis suggests that mass dependent variations in intermolecular potentials should be included in comprehensive descriptions of isotopologue thermodynamics. (C) 2015 Elsevier B.V. All rights reserved. C1 [Herman, Michael F.] Tulane Univ, Dept Chem, New Orleans, LA 70118 USA. [Currier, Robert P.; Clegg, Samuel M.] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. RP Currier, RP (reprint author), Los Alamos Natl Lab, Div Chem, POB 1663, Los Alamos, NM 87545 USA. EM mherman@tulane.edu; currier@lanl.gov; sclegg@Lanl.gov OI Clegg, Sam/0000-0002-0338-0948 FU National Nuclear Security Administration Office of Defense Nuclear Nonproliferation Research and Development; DOE [DE-AC52-06NA25396]; US National Energy Technology Laboratory FX SMC and RPC gratefully acknowledge support from the National Nuclear Security Administration Office of Defense Nuclear Nonproliferation Research and Development and the US National Energy Technology Laboratory's Carbon Capture, Use, and Sequestration Program. This research was completed under DOE contract number DE-AC52-06NA25396. Lively and insightful discussions with Travis Peery and Robert Williams of Los Alamos National Laboratory are also acknowledged. NR 45 TC 0 Z9 0 U1 3 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2614 EI 1873-4448 J9 CHEM PHYS LETT JI Chem. Phys. Lett. PD OCT 16 PY 2015 VL 639 BP 266 EP 268 DI 10.1016/j.cplett.2015.09.041 PG 3 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CX6MF UT WOS:000365814400050 ER PT J AU Smith, BE Roder, PB Zhou, XZ Pauzauskie, PJ AF Smith, Bennett E. Roder, Paden B. Zhou, Xuezhe Pauzauskie, Peter J. TI Hot Brownian thermometry and cavity-enhanced harmonic generation with nonlinear optical nanowires SO CHEMICAL PHYSICS LETTERS LA English DT Article ID PHOTODYNAMIC THERAPY; 2-PHOTON EXCITATION; INFRARED-ABSORPTION; ZNO NANOWIRE; LIGHT; KNBO3; NANOPARTICLES; DYNAMICS; LASERS AB The non-linear response of nanoscale materials is affected by phase-matching conditions that are critically dependent on temperature. It has remained a persistent challenge to measure the temperature of individual nonlinear optical nanostructures in situ. Here, we measure the temperature of individual KNbO3 nanowires in an optical trap through analysis of the Brownian dynamics. Additionally, we show Fabry-Perot-type cavity enhancement of second harmonic generation in one-dimensional potassium niobate nanowires (KNNW) using a tunable, continuous wave (CW), near-infrared (NIR) trapping laser. A second co-aligned CW NIR laser is used to extend the range of visible emission through sum frequency generation. (C) 2015 Published by Elsevier B.V. C1 [Smith, Bennett E.] Univ Washington, Dept Chem, Seattle, WA 98195 USA. [Roder, Paden B.; Zhou, Xuezhe; Pauzauskie, Peter J.] Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USA. [Pauzauskie, Peter J.] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA USA. RP Pauzauskie, PJ (reprint author), Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USA. EM peterpz@uw.edu FU Air Force Office of Scientific Research Young Investigator Program [FA95501210400]; University of Washington; NIH [T32CA138312]; NSF [DGE-1256082] FX This research was made possible by a grant from the Air Force Office of Scientific Research Young Investigator Program (contract #FA95501210400) and start-up funding from the University of Washington. B.E.S. acknowledges support from a NIH T32 training grant (T32CA138312). P.B.R. thanks the NSF for a Graduate Research Fellowship under grant number DGE-1256082. XRD and TEM were conducted at the University of Washington NanoTech User Facility, a member of the NSF National Nanotechnology Infrastructure Network (NNIN). XAS was performed at the Advanced Light Source at Lawrence Berkeley National Laboratory. The authors also thank E. James Davis for donating an optical spectrometer with LN2-cooled detector, A.L. David Kilcoyne for help with XAS measurements, and K. Kroy for constructive feedback on the hot Brownian motion analysis. NR 38 TC 3 Z9 3 U1 4 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2614 EI 1873-4448 J9 CHEM PHYS LETT JI Chem. Phys. Lett. PD OCT 16 PY 2015 VL 639 BP 310 EP 314 DI 10.1016/j.cplett.2015.09.047 PG 5 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CX6MF UT WOS:000365814400060 ER PT J AU Fuselier, SA Dayeh, MA Livadiotis, G McComas, DJ Ogasawara, K Valek, P Funsten, HO Petrinec, SM AF Fuselier, S. A. Dayeh, M. A. Livadiotis, G. McComas, D. J. Ogasawara, K. Valek, P. Funsten, H. O. Petrinec, S. M. TI Imaging the development of the cold dense plasma sheet SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE ENA imaging; plasma sheet; solar wind magneotsphere interactions; magnetotail ID NORTHWARD IMF; MAGNETOSPHERE AB The Interstellar Boundary Explorer (IBEX) frequently images the Earth's magnetosphere in Energetic Neutral Atoms (ENAs). In May 2013, there was an extended period of northward interplanetary magnetic field (IMF) while IBEX was imaging the Earth's magnetotail. During this period, IBEX imaged the development of the cold plasma sheet between about 15 and 20Earth radii (R-E) down the tail from the Earth. The ENA fluxes changed in both amplitude and average energy during this development. In addition, the plasma sheet may have thickened. At the end of the interval, the IMF turned southward and ENA fluxes decreased. The thickening of the plasma sheet suggests that the plasma in this region increases in both density and volume as it develops during extended periods of northward IMF. The decrease in the ENA flux suggests thinning of the plasma sheet and loss of plasma associated with the IMF turning. C1 [Fuselier, S. A.; McComas, D. J.; Valek, P.] Univ Texas San Antonio, Dept Phys & Astron, San Antonio, TX USA. [Funsten, H. O.] Los Alamos Natl Lab, Los Alamos, NM USA. [Petrinec, S. M.] Lockheed Martin Adv Technol Ctr, Palo Alto, CA USA. EM sfuselier@swri.edu OI Funsten, Herbert/0000-0002-6817-1039; Valek, Philip/0000-0002-2318-8750 NR 24 TC 0 Z9 0 U1 0 U2 2 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD OCT 16 PY 2015 VL 42 IS 19 BP 7867 EP 7873 DI 10.1002/2015GL065716 PG 7 WC Geosciences, Multidisciplinary SC Geology GA CU7DF UT WOS:000363695500003 ER PT J AU Wolfe, GM Hanisco, TF Arkinson, HL Bui, TP Crounse, JD Dean-Day, J Goldstein, A Guenther, A Hall, SR Huey, G Jacob, DJ Karl, T Kim, PS Liu, X Marvin, MR Mikoviny, T Misztal, PK Nguyen, TB Peischl, J Pollack, I Ryerson, T St Clair, JM Teng, A Travis, KR Ullmann, K Wennberg, PO Wisthaler, A AF Wolfe, G. M. Hanisco, T. F. Arkinson, H. L. Bui, T. P. Crounse, J. D. Dean-Day, J. Goldstein, A. Guenther, A. Hall, S. R. Huey, G. Jacob, D. J. Karl, T. Kim, P. S. Liu, X. Marvin, M. R. Mikoviny, T. Misztal, P. K. Nguyen, T. B. Peischl, J. Pollack, I. Ryerson, T. St Clair, J. M. Teng, A. Travis, K. R. Ullmann, K. Wennberg, P. O. Wisthaler, A. TI Quantifying sources and sinks of reactive gases in the lower atmosphere using airborne flux observations SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE flux; isoprene; deposition; emission; SEAC4RS; biosphere ID VOLATILE ORGANIC-COMPOUNDS; CHEMISTRY-CLIMATE MODEL; PEROXY NITRATES PAN; BOUNDARY-LAYER; TROPOSPHERIC DEGRADATION; EPOXIDE FORMATION; ISOPRENE VOLCANO; DRY DEPOSITION; AEROSOL; FOREST AB Atmospheric composition is governed by the interplay of emissions, chemistry, deposition, and transport. Substantial questions surround each of these processes, especially in forested environments with strong biogenic emissions. Utilizing aircraft observations acquired over a forest in the southeast U.S., we calculate eddy covariance fluxes for a suite of reactive gases and apply the synergistic information derived from this analysis to quantify emission and deposition fluxes, oxidant concentrations, aerosol uptake coefficients, and other key parameters. Evaluation of results against state-of-the-science models and parameterizations provides insight into our current understanding of this system and frames future observational priorities. As a near-direct measurement of fundamental process rates, airborne fluxes offer a new tool to improve biogenic and anthropogenic emissions inventories, photochemical mechanisms, and deposition parameterizations. C1 [Wolfe, G. M.; Hanisco, T. F.] NASA, Goddard Space Flight Ctr, Atmospher Chem & Dynam Lab, Greenbelt, MD 20771 USA. [Wolfe, G. M.] Univ Maryland Baltimore Cty, Joint Ctr Earth Syst Technol, Baltimore, MD 21228 USA. [Arkinson, H. L.; Marvin, M. R.] Univ Maryland, Dept Ocean & Atmospher Sci, College Pk, MD 20742 USA. [Bui, T. P.; Dean-Day, J.] NASA, Ames Res Ctr, Atmospher Chem & Dynam Branch, Moffett Field, CA 94035 USA. [Crounse, J. D.; Nguyen, T. B.; St Clair, J. M.; Teng, A.; Wennberg, P. O.] CALTECH, Div Geol & Planetary Sci, Pasadena, CA 91125 USA. [Dean-Day, J.] Bay Area Environm Res Inst, Petaluma, CA USA. [Goldstein, A.; Misztal, P. K.] Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. [Guenther, A.] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Hall, S. R.; Ullmann, K.] Natl Ctr Atmospher Res, Div Atmospher Chem, Boulder, CO 80307 USA. [Huey, G.; Liu, X.] Georgia Inst Technol, Sch Earth & Atmospher Sci, Atlanta, GA 30332 USA. [Jacob, D. J.; Kim, P. S.; Travis, K. R.] Harvard Univ, Dept Earth & Planetary Sci, Cambridge, MA 02138 USA. [Jacob, D. J.] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. [Karl, T.] Univ Innsbruck, Inst Meteorol & Geophys, A-6020 Innsbruck, Austria. [Marvin, M. R.] Univ Maryland, Dept Chem, College Pk, MD 20742 USA. [Mikoviny, T.; Wisthaler, A.] Univ Oslo, Dept Chem, Oslo, Norway. [Peischl, J.; Pollack, I.; Ryerson, T.] NOAA, Div Chem Sci, Earth Syst Res Lab, Boulder, CO USA. [Peischl, J.; Pollack, I.] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. [Wennberg, P. O.] CALTECH, Div Engn & Appl Sci, Pasadena, CA 91125 USA. [Wisthaler, A.] Univ Innsbruck, Inst Ion Phys & Appl Phys, A-6020 Innsbruck, Austria. RP Wolfe, GM (reprint author), NASA, Goddard Space Flight Ctr, Atmospher Chem & Dynam Lab, Greenbelt, MD 20771 USA. EM glenn.m.wolfe@nasa.gov RI Karl, Thomas/D-1891-2009; Manager, CSD Publications/B-2789-2015; Misztal, Pawel/B-8371-2009; Wolfe, Glenn/D-5289-2011; Pollack, Ilana/F-9875-2012; Travis, Katherine/G-1417-2016; Peischl, Jeff/E-7454-2010; Crounse, John/C-3700-2014 OI Karl, Thomas/0000-0003-2869-9426; Teng, Alexander/0000-0002-6434-0501; Misztal, Pawel/0000-0003-1060-1750; Travis, Katherine/0000-0003-1628-0353; Peischl, Jeff/0000-0002-9320-7101; Crounse, John/0000-0001-5443-729X FU NASA ROSES SEAC4RS [NNH10ZDA001N, NNX12AC06G]; ACCDAM [NNX14AP48G, NNX14AP46G]; NSF PRF [AGS-1331360]; National Institute of Aerospace (NIA) FX This work was supported by grants from the NASA ROSES SEAC4RS (NNH10ZDA001N and NNX12AC06G) and ACCDAM (NNX14AP48G and NNX14AP46G) programs. T.B.N. acknowledges support from NSF PRF award AGS-1331360. Isoprene measurements were supported by the Austrian Federal Ministry for Transport, Innovation and Technology (bmvit) through the Austrian Space Applications Programme (ASAP) of the Austrian Research Promotion Agency (FFG). A.W. and T.M. received support from the Visiting Scientist Program at the National Institute of Aerospace (NIA). We thank the DC-8 pilots, crew, payload operators, and mission scientists for their hard work and for the opportunity to calibrate the meteorological measurements. We are also grateful to NASA ESPO for mission logistics. We thank the Jimenez, Brock, and Anderson groups for use of aerosol data. We also thank L. Kaser, B. Yuan, S.-W. Kim, and J. Thornton for helpful discussions. All data used in this analysis are publicly available under the SEAC4RS DOI at 10.5067/Aircraft/SEAC4RS/Aerosol-TraceGas-Cloud. NR 51 TC 11 Z9 11 U1 4 U2 38 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD OCT 16 PY 2015 VL 42 IS 19 BP 8231 EP 8240 DI 10.1002/2015GL065839 PG 10 WC Geosciences, Multidisciplinary SC Geology GA CU7DF UT WOS:000363695500047 ER PT J AU Jaing, C Thissen, JB Gardner, S McLoughlin, K Slezak, T Bossart, GD Fair, PA AF Jaing, Crystal Thissen, James B. Gardner, Shea McLoughlin, Kevin Slezak, Tom Bossart, Gregory D. Fair, Patricia A. TI Pathogen surveillance in wild bottlenose dolphins Tursiops truncatus SO DISEASES OF AQUATIC ORGANISMS LA English DT Article DE Diagnostics; Microarray; Microbial community; Molecular detection; Marine diseases; Microbiological culture ID INDIAN RIVER LAGOON; MICROBIAL COMMUNITIES; SOUTH-CAROLINA; ATLANTIC; BACTERIA; IDENTIFICATION; CHARLESTON; MICROARRAY; DIVERSITY; ZOONOSES AB The number and prevalence of diseases is rapidly increasing in the marine ecosystem. Although there is an increase in the number of marine diseases observed world-wide, current understanding of the pathogens associated with marine mammals is limited. An important need exists to develop and apply platforms for rapid detection and characterization of pathogenic agents to assess, prevent and respond to disease outbreaks. In this study, a broad-spectrum molecular detection technology capable of detecting all sequenced microbial organisms, the Lawrence Livermore Microbial Detection Array, was used to assess the microbial agents that could be associated with wild Atlantic dolphins. Blowhole, gastric, and fecal samples from 8 bottlenose dolphins were collected in Charleston, SC, as part of the dolphin assessment effort. The array detected various microbial agents from the dolphin samples. Clostridium perfringens was most prevalent in the samples surveyed using the microarray. This pathogen was also detected using microbiological culture techniques. Additionally, Campylobacter sp., Staphylococcus sp., Erwinia amylovora, Helicobacter pylori, and Frankia sp. were also detected in more than one dolphin using the microarray, but not in culture. This study provides the first survey of pathogens associated with 3 tissue types in dolphins using a broad-spectrum microbial detection microarray and expands insight on the microbial community profile in dolphins. C1 [Jaing, Crystal; Thissen, James B.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94551 USA. [Gardner, Shea; McLoughlin, Kevin; Slezak, Tom] Lawrence Livermore Natl Lab, Computat Directorate, Livermore, CA 94551 USA. [Bossart, Gregory D.] Georgia Aquarium, Nw Atlanta, GA 30313 USA. [Fair, Patricia A.] NOAA Natl Ocean Serv, Ctr Coastal Environm Hlth & Biomol Res, Charleston, SC 29412 USA. RP Jaing, C (reprint author), Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94551 USA. EM jaing2@llnl.gov FU Office of Naval Research Award [N0001411IP20081, N00014110541] FX We thank the numerous researchers who participated in the dolphin capture and release studies in South Carolina. We are especially grateful to B. Joseph, L. Hansen, S. McCulloch, L. Fulford, the NOAA and HBOI staff, the collaborators and veterinarians who provided their expertise, and the many volunteers whose help made the health assessment studies possible. We also thank R. Ober and J. Thompson from Kansas State University for assistance with DNA extraction of some of the dolphin samples during their summer internship at LLNL. This present study was partially supported through Office of Naval Research Award Number N0001411IP20081 and N00014110541. NR 38 TC 0 Z9 0 U1 5 U2 11 PU INTER-RESEARCH PI OLDENDORF LUHE PA NORDBUNTE 23, D-21385 OLDENDORF LUHE, GERMANY SN 0177-5103 EI 1616-1580 J9 DIS AQUAT ORGAN JI Dis. Aquat. Org. PD OCT 16 PY 2015 VL 116 IS 2 BP 83 EP + DI 10.3354/dao02917 PG 22 WC Fisheries; Veterinary Sciences SC Fisheries; Veterinary Sciences GA CU2HD UT WOS:000363343700001 PM 26480911 ER PT J AU Kaleta, J Kaletova, E Cisarova, I Teat, SJ Michl, J AF Kaleta, Jiri Kaletova, Eva Cisarova, Ivana Teat, Simon J. Michl, Josef TI Synthesis of Triptycene-Based Molecular Rotors for Langmuir-Blodgett Monolayers SO JOURNAL OF ORGANIC CHEMISTRY LA English DT Article ID SURFACE INCLUSION; FILMS; ARRAYS; POLYMER; TRIS(O-PHENYLENEDIOXY)CYCLOTRIPHOSPHAZENE; SPECTROSCOPY; ORIENTATION; PAIRS; TPP AB We describe syntheses of six triptycene-containing molecular rotors with several single-crystal X-ray diffraction analyses. These rod-shaped molecules carrying an axial rotator are designed to interleave on an aqueous surface into Langmuir-Blodgett (LB) monolayers containing a two-dimensional trigonal array of dipoles rotatable about an axis normal to the surface. Monolayer formation was verified with the simplest of the rotor structures. On an aqueous subphase containing divalent (c)ations (Mg2+, Ca2+, Zn2+, Sr2+, or Cd2+), the LB isotherm yielded an area of 53 +/- 3 angstrom(2)/molecule (monolayer of type A), compatible with the anticipated triangular packing of axes normal to the surface. On pure water, the area is 30 +/- 3 angstrom(2)/molecule, and it is proposed that in this monolayer (type B), the molecular axes are tilted by 40-45 degrees to a structure similar to those observed in single crystals of related triptycenes. After transfer to a gold surface, ellipsometry and PM IRRAS yield tilt angles of 29 +/- 4 degrees (monolayers of type A) and 38 +/- 4 degrees (type B). A full-scale examination of monolayers from all the rotors on a subphase and after transfer is underway and will be reported separately. C1 [Kaleta, Jiri; Kaletova, Eva; Michl, Josef] Acad Sci Czech Republic, Inst Organ Chem & Biochem, Prague 16610, Czech Republic. [Cisarova, Ivana] Charles Univ Prague, Fac Sci, Dept Inorgan Chem, Prague 12840 2, Czech Republic. [Teat, Simon J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Michl, Josef] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. RP Kaleta, J (reprint author), Acad Sci Czech Republic, Inst Organ Chem & Biochem, Flemingovo Nam 2, Prague 16610, Czech Republic. EM kaleta@uochb.cas.cz RI Michl, Josef/G-9376-2014; Cisarova, Ivana/B-1385-2017 OI Cisarova, Ivana/0000-0002-9612-9831 FU European Research Council under the European Community [227756]; Institute of Organic Chemistry and Biochemistry, Academy of Sciences of the Czech Republic [RVO: 61388963]; National Science Foundation [CHE 1265922]; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the European Research Council under the European Community's Framework Programme (FP7/2007-2013) ERC grant agreement no. 227756, by the Institute of Organic Chemistry and Biochemistry, Academy of Sciences of the Czech Republic (RVO: 61388963) and by the National Science Foundation under grant no. CHE 1265922. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. We are grateful to Dr. Lucie Bednarova for help with IR spectra, Dr. Radek Pohl for help with NMR spectra and Dr. Jakub Chalupsky for help with visualization of calculated transition moments. NR 51 TC 4 Z9 4 U1 5 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0022-3263 J9 J ORG CHEM JI J. Org. Chem. PD OCT 16 PY 2015 VL 80 IS 20 BP 10134 EP 10150 DI 10.1021/acs.joc.5b01753 PG 17 WC Chemistry, Organic SC Chemistry GA CU0QU UT WOS:000363224600035 PM 26382886 ER PT J AU Chan, AH Yi, SW Terwilliger, AL Maresso, AW Jung, ME Clubb, RT AF Chan, Albert H. Yi, Sung Wook Terwilliger, Austen L. Maresso, Anthony W. Jung, Michael E. Clubb, Robert T. TI Structure of the Bacillus anthracis Sortase A Enzyme Bound to Its Sorting Signal A FLEXIBLE AMINO-TERMINAL APPENDAGE MODULATES SUBSTRATE ACCESS SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article ID GRAM-POSITIVE BACTERIA; MAGNETIC-RESONANCE RELAXATION; NMR STRUCTURE DETERMINATION; MODEL-FREE APPROACH; CELL-WALL ENVELOPE; STAPHYLOCOCCUS-AUREUS; DIPOLAR COUPLINGS; SURFACE PROTEIN; ACTIVE-SITE; BIOLOGICAL MACROMOLECULES AB The endospore forming bacterium Bacillus anthracis causes lethal anthrax disease in humans and animals. The ability of this pathogen to replicate within macrophages is dependent upon the display of bacterial surface proteins attached to the cell wall by the B. anthracis Sortase A ((Ba)SrtA) enzyme. Previously, we discovered that the class A (Ba)SrtA sortase contains a unique N-terminal appendage that wraps around the body of the protein to contact the active site of the enzyme. To gain insight into its function, we determined the NMR structure of (Ba)SrtA bound to a LPXTG sorting signal analog. The structure, combined with dynamics, kinetics, and whole cell protein display data suggest that the N terminus modulates substrate access to the enzyme. We propose that it may increase the efficiency of protein display by reducing the unproductive hydrolytic cleavage of enzyme-protein covalent intermediates that form during the cell wall anchoring reaction. Notably, a key active site loop (beta 7/beta 8 loop) undergoes a disordered to ordered transition upon binding the sorting signal, potentially facilitating recognition of lipid II. C1 [Chan, Albert H.; Yi, Sung Wook; Jung, Michael E.] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. [Chan, Albert H.; Clubb, Robert T.] Univ Calif Los Angeles, DOE Inst Genom & Prote, Los Angeles, CA 90095 USA. [Chan, Albert H.; Clubb, Robert T.] Univ Calif Los Angeles, Inst Mol Biol, Los Angeles, CA 90095 USA. [Terwilliger, Austen L.; Maresso, Anthony W.] Baylor Coll Med, Dept Mol Virol & Microbiol, Houston, TX 77030 USA. RP Clubb, RT (reprint author), Univ Calif Los Angeles, Dept Chem & Biochem, 602 Boyer Hall, Los Angeles, CA 90095 USA. EM rclubb@mbi.ucla.edu RI Regan, Clinton/E-6250-2012 FU National Institutes of Health [AI52217, AI097167, AI109465, T32 GM008496]; Department of Energy [DE-FC-03-87ER60615] FX This work was supported, in whole or in part, by National Institutes of Health Grants AI52217 (to R. T. C. and M. E. J.), AI097167 and AI109465 (to A. W. M.), and T32 GM008496 (to A. H. C.) and Department of Energy Grant DE-FC-03-87ER60615. The authors declare that they have no conflicts of interest with the contents of this article. NR 72 TC 2 Z9 2 U1 0 U2 13 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD OCT 16 PY 2015 VL 290 IS 42 BP 25461 EP 25474 DI 10.1074/jbc.M115.670984 PG 14 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CT6ZO UT WOS:000362962800022 PM 26324714 ER PT J AU Basta, LAB Ghosh, A Pan, Y Jakoncic, J Lloyd, EP Townsend, CA Lamichhane, G Bianchet, MA AF Basta, Leighanne A. Brammer Ghosh, Anita Pan, Ying Jakoncic, Jean Lloyd, Evan P. Townsend, Craig A. Lamichhane, Gyanu Bianchet, Mario A. TI Loss of a Functionally and Structurally Distinct LD-Transpeptidase, Ldt(Mt5), Compromises Cell Wall Integrity in Mycobacterium tuberculosis SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article ID PEPTIDOGLYCAN CROSS-LINKING; BETA-LACTAM ANTIBIOTICS; ESCHERICHIA-COLI; CRYSTAL-STRUCTURE; L,D-TRANSPEPTIDASES; MEROPENEM; PROTEIN; RESISTANCE; SYSTEM; IDENTIFICATION AB The final step of peptidoglycan (PG) biosynthesis in bacteria involves cross-linking of peptide side chains. This step in Mycobacterium tuberculosis is catalyzed by LD- and DD-transpeptidases that generate 3 -> 3 and 4 -> 3 transpeptide linkages, respectively. M. tuberculosis PG is predominantly 3 -> 3 cross-linked, and Ldt(Mt2) is the dominant LD-transpeptidase. There are four additional sequence paralogs of Ldt(Mt2) encoded by the genome of this pathogen, and the reason for this apparent redundancy is unknown. Here, we studied one of the paralogs, Ldt(Mt5), and found it to be structurally and functionally distinct. The structures of apo-Ldt(Mt5) and its meropenem adduct presented here demonstrate that, despite overall architectural similarity to Ldt(Mt2), the Ldt(Mt5) active site has marked differences. The presence of a structurally divergent catalytic site and a proline-rich C-terminal subdomain suggest that this protein may have a distinct role in PG metabolism, perhaps involving other cell wall-anchored proteins. Furthermore, M. tuberculosis lacking a functional copy of Ldt(Mt5) displayed aberrant growth and was more susceptible to killing by crystal violet, osmotic shock, and select carbapenem antibiotics. Therefore, we conclude that Ldt(Mt5) is not a functionally redundant LD-transpeptidase, but rather it serves a unique and important role in maintaining the integrity of the M. tuberculosis cell wall. C1 [Basta, Leighanne A. Brammer; Lamichhane, Gyanu] Johns Hopkins Univ, Sch Med, Taskforce Study Resistance Emergence & Antimicrob, Baltimore, MD 21231 USA. [Basta, Leighanne A. Brammer; Lamichhane, Gyanu] Johns Hopkins Univ, Sch Med, Div Infect Dis, Baltimore, MD 21231 USA. [Ghosh, Anita; Pan, Ying; Bianchet, Mario A.] Johns Hopkins Univ, Sch Med, Struct Enzymol & Thermodynam Grp, Dept Biophys & Biophys Chem, Baltimore, MD 21205 USA. [Bianchet, Mario A.] Johns Hopkins Univ, Sch Med, Dept Neurol, Baltimore, MD 21205 USA. [Jakoncic, Jean] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. [Lloyd, Evan P.; Townsend, Craig A.] Johns Hopkins Univ, Dept Chem, Baltimore, MD 21218 USA. RP Lamichhane, G (reprint author), Johns Hopkins Univ, Sch Med, 1503 E Jefferson St, Baltimore, MD 21231 USA. EM lamichhane@jhu.edu; bianchet@jhmi.edu OI Basta, Leighanne/0000-0002-4121-5505; Bianchet, Mario/0000-0001-9032-7549; Lamichhane, Gyanu/0000-0002-2214-0114 FU National Institute of General Medical Sciences, National Institute of Health [GM-0080]; United States Department of Energy [DE-AC02-98CH10886] FX We kindly thank Amit Kaushik for assistance with genetic experiments and Maia Schoonmaker Arnold and Mike Delanoy for assistance with electron microscopy. Research was carried out at X6A beamline funded by the National Institute of General Medical Sciences, National Institute of Health under Agreement GM-0080. The National Synchrotron Light Source, Brookhaven National Laboratory is supported by the United States Department of Energy under Contract DE-AC02-98CH10886. NR 48 TC 2 Z9 2 U1 3 U2 8 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD OCT 16 PY 2015 VL 290 IS 42 BP 25670 EP 25685 DI 10.1074/jbc.M115.660753 PG 16 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CT6ZO UT WOS:000362962800039 ER PT J AU Caro, A Correa, AA Tamm, A Samolyuk, GD Stocks, GM AF Caro, A. Correa, A. A. Tamm, A. Samolyuk, G. D. Stocks, G. M. TI Adequacy of damped dynamics to represent the electron-phonon interaction in solids SO PHYSICAL REVIEW B LA English DT Article ID METAL-SURFACES; DAMAGE; SUPERCONDUCTIVITY; TEMPERATURE; IRRADIATION; VIBRATIONS; CASCADES; EMISSION; SYSTEMS; ATOMS AB Time-dependent density functional theory and Ehrenfest dynamics are used to calculate the electronic excitations produced by a moving Ni ion in a Ni crystal in the case of energetic MeV range (electronic stopping power regime), as well as thermal energy meV range (electron-phonon interaction regime). Results at high energy compare well to experimental databases of stopping power, and at low energy the electron-phonon interaction strength determined in this way is very similar to the linear response calculation and experimental measurements. This approach to electron-phonon interaction as an electronic stopping process provides the basis for a unified framework to perform classical molecular dynamics of ion-solid interaction with ab initio type nonadiabatic terms in a wide range of energies. C1 [Caro, A.; Tamm, A.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Correa, A. A.] Lawrence Livermore Natl Lab, Quantum Simulat Grp, Livermore, CA 94550 USA. [Samolyuk, G. D.; Stocks, G. M.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN USA. RP Caro, A (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. EM caro@lanl.gov RI Stocks, George Malcollm/Q-1251-2016 OI Stocks, George Malcollm/0000-0002-9013-260X FU U.S. Department of Energy [2014ORNL1026]; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX Work was performed at the Energy Dissipation to Defect Evolution Center, an Energy Frontier Research Center funded by the U.S. Department of Energy (Grant No. 2014ORNL1026) at Los Alamos and Oak Ridge National Laboratories. This research used resources provided by the LANL Institutional Computing Program. LANL, an affirmative action/equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. Work by A.A.C. was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 49 TC 5 Z9 5 U1 2 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 16 PY 2015 VL 92 IS 14 AR 144309 DI 10.1103/PhysRevB.92.144309 PG 7 WC Physics, Condensed Matter SC Physics GA CT6BV UT WOS:000362896700004 ER PT J AU Dioguardi, AP Lawson, MM Bush, BT Crocker, J Shirer, KR Nisson, DM Kissikov, T Ran, S Bud'ko, SL Canfield, PC Yuan, S Kuhns, PL Reyes, AP Grafe, HJ Curro, NJ AF Dioguardi, A. P. Lawson, M. M. Bush, B. T. Crocker, J. Shirer, K. R. Nisson, D. M. Kissikov, T. Ran, S. Bud'ko, S. L. Canfield, P. C. Yuan, S. Kuhns, P. L. Reyes, A. P. Grafe, H. -J. Curro, N. J. TI NMR evidence for inhomogeneous glassy behavior driven by nematic fluctuations in iron arsenide superconductors SO PHYSICAL REVIEW B LA English DT Article ID TRANSITION; DISORDER; STATE AB We present As-75 nuclear magnetic resonance spin-lattice and spin-spin relaxation rate data in Ba(Fe1-xCox)(2)As-2 and Ba(Fe1-xCux)(2)As-2 as a function of temperature, doping, and magnetic field. The relaxation curves exhibit a broad distribution of relaxation rates, consistent with inhomogeneous glassy behavior up to 100 K. The doping and temperature response of the width of the dynamical heterogeneity is similar to that of the nematic susceptibility measured by elastoresistance measurements. We argue that quenched random fields which couple to the nematic order give rise to a nematic glass that is reflected in the spin dynamics. C1 [Dioguardi, A. P.; Lawson, M. M.; Bush, B. T.; Crocker, J.; Shirer, K. R.; Nisson, D. M.; Kissikov, T.; Curro, N. J.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Ran, S.; Bud'ko, S. L.; Canfield, P. C.] US DOE, Ames Lab, Ames, IA 50011 USA. [Ran, S.; Bud'ko, S. L.; Canfield, P. C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Yuan, S.; Kuhns, P. L.; Reyes, A. P.] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. [Grafe, H. -J.] IFW Dresden, Inst Solid State Res, D-01171 Dresden, Germany. RP Dioguardi, AP (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM apd@lanl.gov RI Curro, Nicholas/D-3413-2009 OI Curro, Nicholas/0000-0001-7829-0237 FU National Science Foundation [DMR-1005393, DMR-1157490]; Deutsche Forschungsgemeinschaft (DFG) [SPP1458, GR3330/2]; U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering; U.S. Department of Energy [DE-AC02-07CH11358]; State of Florida FX We thank A. Thaler for assistance with initial sample growth, A. Estry for assistance with field calibration studies, as well as A. Benali, I. Fisher, S. Kivelson, E. Carlson, and K. Dahmen for enlightening discussions. Work at UC Davis was supported by the National Science Foundation under Grant No. DMR-1005393. H.-J. G. acknowledges support from the Deutsche Forschungsgemeinschaft (DFG) through SPP1458 (Grant No. GR3330/2). Part of this work performed at the Ames Laboratory (P.C.C., S.L.B., S.R.) was supported by the U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. A portion of this work was performed at the National High Magnetic Field Laboratory, which is supported by National Science Foundation Cooperative Agreement No. DMR-1157490 and the State of Florida. NR 49 TC 8 Z9 8 U1 2 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD OCT 16 PY 2015 VL 92 IS 16 AR 165116 DI 10.1103/PhysRevB.92.165116 PG 8 WC Physics, Condensed Matter SC Physics GA CT6CB UT WOS:000362897500003 ER PT J AU Meisel, Z George, S Ahn, S Bazin, D Brown, BA Browne, J Carpino, JF Chung, H Cole, AL Cyburt, RH Estrade, A Famiano, M Gade, A Langer, C Matos, M Mittig, W Montes, F Morrissey, DJ Pereira, J Schatz, H Schatz, J Scott, M Shapira, D Smith, K Stevens, J Tan, W Tarasov, O Towers, S Wimmer, K Winkelbauer, JR Yurkon, J Zegers, RGT AF Meisel, Z. George, S. Ahn, S. Bazin, D. Brown, B. A. Browne, J. Carpino, J. F. Chung, H. Cole, A. L. Cyburt, R. H. Estrade, A. Famiano, M. Gade, A. Langer, C. Matos, M. Mittig, W. Montes, F. Morrissey, D. J. Pereira, J. Schatz, H. Schatz, J. Scott, M. Shapira, D. Smith, K. Stevens, J. Tan, W. Tarasov, O. Towers, S. Wimmer, K. Winkelbauer, J. R. Yurkon, J. Zegers, R. G. T. TI Mass Measurement of Sc-56 Reveals a Small A=56 Odd-Even Mass Staggering, Implying a Cooler Accreted Neutron Star Crust SO PHYSICAL REVIEW LETTERS LA English DT Article ID GAMMA-RAY BURSTS; ADJUSTMENT PROCEDURES; MAXI J0556-332; INPUT DATA; SUPERBURST; EMISSION; HYDROGEN; DEFORMATIONS; ISOTOPES; NUCLEI AB We present the mass excesses of Sc52-57, obtained from recent time-of-flight nuclear mass measurements at the National Superconducting Cyclotron Laboratory at Michigan State University. The masses of Sc-56 and Sc-57 were determined for the first time with atomic mass excesses of -24.85(59)((+0)(-54)) MeV and -21.0(1.3) MeV, respectively, where the asymmetric uncertainty for Sc-56 was included due to possible contamination from a long-lived isomer. The Sc-56 mass indicates a small odd-even mass staggering in the A = 56 mass chain towards the neutron drip line, significantly deviating from trends predicted by the global FRDM mass model and favoring trends predicted by the UNEDF0 and UNEDF1 density functional calculations. Together with new shell-model calculations of the electron-capture strength function of Sc-56, our results strongly reduce uncertainties in model calculations of the heating and cooling at the Ti-56 electron-capture layer in the outer crust of accreting neutron stars. We find that, in contrast to previous studies, neither strong neutrino cooling nor strong heating occurs in this layer. We conclude that Urca cooling in the outer crusts of accreting neutron stars that exhibit superbursts or high temperature steady-state burning, which are predicted to be rich in A approximate to 56 nuclei, is considerably weaker than predicted. Urca cooling must instead be dominated by electron capture on the small amounts of adjacent odd-A nuclei contained in the superburst and high temperature steady-state burning ashes. This may explain the absence of strong crust Urca cooling inferred from the observed cooling light curve of the transiently accreting x-ray source MAXI J0556-332. C1 [Meisel, Z.; George, S.; Ahn, S.; Bazin, D.; Brown, B. A.; Browne, J.; Cyburt, R. H.; Gade, A.; Langer, C.; Mittig, W.; Montes, F.; Morrissey, D. J.; Pereira, J.; Schatz, H.; Schatz, J.; Scott, M.; Stevens, J.; Tarasov, O.; Wimmer, K.; Winkelbauer, J. R.; Yurkon, J.; Zegers, R. G. T.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Meisel, Z.; Brown, B. A.; Browne, J.; Gade, A.; Mittig, W.; Schatz, H.; Scott, M.; Stevens, J.; Winkelbauer, J. R.; Zegers, R. G. T.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Meisel, Z.; George, S.; Ahn, S.; Browne, J.; Cyburt, R. H.; Langer, C.; Montes, F.; Pereira, J.; Schatz, H.; Smith, K.; Stevens, J.; Zegers, R. G. T.] Michigan State Univ, Joint Inst Nucl Astrophys, E Lansing, MI 48824 USA. [George, S.] Max Planck Inst Kernphys, D-69117 Heidelberg, Germany. [Carpino, J. F.; Chung, H.; Famiano, M.; Towers, S.] Western Michigan Univ, Dept Phys, Kalamazoo, MI 49008 USA. [Cole, A. L.] Kalamazoo Coll, Dept Phys, Kalamazoo, MI 49006 USA. [Estrade, A.] Univ Edinburgh, Sch Phys & Astron, Edinburgh EH8 9YL, Midlothian, Scotland. [Matos, M.] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. [Morrissey, D. J.] Michigan State Univ, Dept Chem, E Lansing, MI 48824 USA. [Shapira, D.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Meisel, Z.; Smith, K.; Tan, W.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. RP Meisel, Z (reprint author), Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. EM zmeisel@nd.edu RI Gade, Alexandra/A-6850-2008; Zegers, Remco/A-6847-2008; Langer, Christoph/L-3422-2016; Tan, Wanpeng/A-4687-2008 OI Gade, Alexandra/0000-0001-8825-0976; Tan, Wanpeng/0000-0002-5930-1823 FU NSF [PHY-0822648, PHY-1102511, PHY-1404442, PHY-1430152]; DFG [GE2183/1-1, GE2183/2-1] FX This project is funded by the NSF through Grants No. PHY-0822648, No. PHY-1102511, No. PHY-1404442, and No. PHY-1430152. S. G. acknowledges support from the DFG under Contracts No. GE2183/1-1 and No. GE2183/2-1. We thank Erik Olsen for providing nuclear binding energies from energy density functional calculations and E. F. Brown and A. T. Deibel for many useful discussions. NR 57 TC 3 Z9 3 U1 1 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 16 PY 2015 VL 115 IS 16 AR 162501 DI 10.1103/PhysRevLett.115.162501 PG 6 WC Physics, Multidisciplinary SC Physics GA CT6FU UT WOS:000362909100006 PM 26550869 ER PT J AU Conradson, SD Gilbertson, SM Daifuku, SL Kehl, JA Durakiewicz, T Andersson, DA Bishop, AR Byler, DD Maldonado, P Oppeneer, PM Valdez, JA Neidig, ML Rodriguez, G AF Conradson, Steven D. Gilbertson, Steven M. Daifuku, Stephanie L. Kehl, Jeffrey A. Durakiewicz, Tomasz Andersson, David A. Bishop, Alan R. Byler, Darrin D. Maldonado, Pablo Oppeneer, Peter M. Valdez, James A. Neidig, Michael L. Rodriguez, George TI Possible Demonstration of a Polaronic Bose-Einstein(-Mott) Condensate in UO2(+x) by Ultrafast THz Spectroscopy and Microwave Dissipation SO SCIENTIFIC REPORTS LA English DT Article ID BOSE-EINSTEIN CONDENSATION; INTERACTING FERMI GAS; NEUTRON-DIFFRACTION; AXIAL OXYGEN; PARAMAGNETIC-RESONANCE; LATTICE INSTABILITIES; ROOM-TEMPERATURE; URANIUM-DIOXIDE; PHASE-DIAGRAM; GROUND-STATE AB Bose-Einstein condensates (BECs) composed of polarons would be an advance because they would combine coherently charge, spin, and a crystal lattice. Following our earlier report of unique structural and spectroscopic properties, we now identify potentially definitive evidence for polaronic BECs in photo-and chemically doped UO2(+x) on the basis of exceptional coherence in the ultrafast time dependent terahertz absorption and microwave spectroscopy results that show collective behavior including dissipation patterns whose precedents are condensate vortex and defect disorder and condensate excitations. That some of these signatures of coherence in an atom-based system extend to ambient temperature suggests a novel mechanism that could be a synchronized, dynamical, disproportionation excitation, possibly via the solid state analog of a Feshbach resonance that promotes the coherence. Such a mechanism would demonstrate that the use of ultra-low temperatures to establish the BEC energy distribution is a convenience rather than a necessity, with the actual requirement for the particles being in the same state that is not necessarily the ground state attainable by other means. A macroscopic quantum object created by chemical doping that can persist to ambient temperature and resides in a bulk solid would be revolutionary in a number of scientific and technological fields. C1 [Conradson, Steven D.] Synchrotron Soleil, Orme Merisiers St Aubin, F-91192 Gif Sur Yvette, France. [Gilbertson, Steven M.; Durakiewicz, Tomasz; Andersson, David A.; Bishop, Alan R.; Byler, Darrin D.; Valdez, James A.; Rodriguez, George] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Daifuku, Stephanie L.; Kehl, Jeffrey A.; Neidig, Michael L.] Univ Rochester, Dept Chem, Rochester, NY 14627 USA. [Maldonado, Pablo; Oppeneer, Peter M.] Uppsala Univ, Dept Phys & Astron, S-75120 Uppsala, Sweden. RP Conradson, SD (reprint author), Synchrotron Soleil, Orme Merisiers St Aubin, F-91192 Gif Sur Yvette, France. EM steven.conradson@synchrotron-soleil.fr RI Rodriguez, George/G-7571-2012; OI Rodriguez, George/0000-0002-6044-9462; Maldonado, Pablo/0000-0002-8524-819X FU National Nuclear Security Administration of U.S. Department of Energy [DEAC52-06NA25396]; Los Alamos LDRD program; U.S. Department of Energy, Office Science, Basic Energy Sciences, Materials Sciences and Engineering and the Chemical Sciences, Biosciences, and Geosciences Divisions; EU [281943]; Synchrotron Soleil FX Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of U.S. Department of Energy under Contract DEAC52-06NA25396. This work was supported by the Los Alamos LDRD program and by the U.S. Department of Energy, Office Science, Basic Energy Sciences, Materials Sciences and Engineering and the Chemical Sciences, Biosciences, and Geosciences Divisions. Portions of this research were carried out at the Stanford Synchrotron Radiation Lightsource, a Directorate of SLAC National Accelerator Laboratory and an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Stanford University. Phonon calculations were supported by EU-FP7 project 'FEMTOSPIN' (grant no. 281943). EPR measurements were supported by the University of Rochester. Preparation of this article was supported by Synchrotron Soleil. Magnetic susceptibility measurements were performed by J. D. Thompson, and we thank H. J. von Bardeleben for useful discussions. NR 94 TC 6 Z9 6 U1 2 U2 21 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 16 PY 2015 VL 5 AR 15278 DI 10.1038/srep15278 PG 14 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CT5XI UT WOS:000362884000001 PM 26472071 ER PT J AU Macklin, C O'Brien, K Hover, D Schwartz, ME Bolkhovsky, V Zhang, X Oliver, WD Siddiqi, I AF Macklin, C. O'Brien, K. Hover, D. Schwartz, M. E. Bolkhovsky, V. Zhang, X. Oliver, W. D. Siddiqi, I. TI A near-quantum-limited Josephson traveling-wave parametric amplifier SO SCIENCE LA English DT Article ID NOISE; AMPLIFICATION; BAND AB Detecting single-photon level signals-carriers of both classical and quantum information-is particularly challenging for low-energy microwave frequency excitations. Here we introduce a superconducting amplifier based on a Josephson junction transmission line. Unlike current standing-wave parametric amplifiers, this traveling wave architecture robustly achieves high gain over a bandwidth of several gigahertz with sufficient dynamic range to read out 20 superconducting qubits. To achieve this performance, we introduce a subwavelength resonant phase-matching technique that enables the creation of nonlinear microwave devices with unique dispersion relations. We benchmark the amplifier with weak measurements, obtaining a high quantum efficiency of 75% (70% including noise added by amplifiers following the Josephson amplifier). With a flexible design based on compact lumped elements, this Josephson amplifier has broad applicability to microwave metrology and quantum optics. C1 [Macklin, C.; Schwartz, M. E.; Siddiqi, I.] Univ Calif Berkeley, Quantum Nanoelect Lab, Berkeley, CA 94720 USA. [Macklin, C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. [O'Brien, K.; Zhang, X.] Univ Calif Berkeley, Nanoscale Sci & Engn Ctr, Berkeley, CA 94720 USA. [Hover, D.; Bolkhovsky, V.; Oliver, W. D.] MIT, Lincoln Lab, Lexington, MA 02420 USA. [Zhang, X.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Zhang, X.] King Abdulaziz Univ, Dept Phys, Jeddah 21589, Saudi Arabia. [Oliver, W. D.] MIT, Elect Res Lab, Cambridge, MA 02139 USA. RP Macklin, C (reprint author), Univ Calif Berkeley, Quantum Nanoelect Lab, Berkeley, CA 94720 USA. EM chris.macklin@berkeley.edu RI Schwartz, Mollie/B-5012-2012; Zhang, Xiang/F-6905-2011 OI Schwartz, Mollie/0000-0003-4406-8974; FU Army Research Office [W911NF-14-1-0078]; Office of the Director of National Intelligence (ODNI); Intelligence Advanced Research Projects Activity (IARPA); MIT Lincoln Laboratory under Air Force Contract [FA8721-05-C-0002]; Multidisciplinary University Research Initiative from the Air Force Office of Scientific Research MURI [FA9550-12-1-0488]; Hertz Foundation Fellowship FX We acknowledge A. Kamal, S. Tolpygo, and G. Fitch for useful discussions and technical assistance. C. M. acknowledges E. Hassell and J. Luke for useful discussions. This research is based on work supported in part by the Army Research Office (under grant no. W911NF-14-1-0078); the Office of the Director of National Intelligence (ODNI), Intelligence Advanced Research Projects Activity (IARPA), via MIT Lincoln Laboratory under Air Force Contract FA8721-05-C-0002; and a Multidisciplinary University Research Initiative from the Air Force Office of Scientific Research MURI grant no. FA9550-12-1-0488. The views and conclusions contained herein are those of the authors and should not be interpreted as necessarily representing the official policies or endorsements, either expressed or implied, of ODNI, IARPA, or the U.S. government. The U.S. government is authorized to reproduce and distribute reprints for governmental purpose notwithstanding any copyright annotation thereon. M. E. S. acknowledges support from a Hertz Foundation Fellowship. NR 33 TC 30 Z9 30 U1 7 U2 39 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD OCT 16 PY 2015 VL 350 IS 6258 BP 307 EP 310 DI 10.1126/science.aaa8525 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CT5HD UT WOS:000362838700037 PM 26338795 ER PT J AU Marcillo, O Arrowsmith, S Blom, P Jones, K AF Marcillo, Omar Arrowsmith, Stephen Blom, Philip Jones, Kyle TI On infrasound generated by wind farms and its propagation in low-altitude tropospheric waveguides SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article AB Infrasound from a 60-turbine wind farm was found to propagate to distances up to 90 km under nighttime atmospheric conditions. Four infrasound sensor arrays were deployed in central New Mexico in February 2014; three of these arrays captured infrasound from a large wind farm. The arrays were in a linear configuration oriented southeast with 13, 54, 90, and 126 km radial distances and azimuths of 166 degrees, 119 degrees, 113 degrees, and 111 degrees from the 60 1.6 MW turbine Red Mesa Wind Farm, Laguna Pueblo, New Mexico, USA. Peaks at a fundamental frequency slightly below 0.9 Hz and its harmonics characterize the spectrum of the detected infrasound. The generation of this signal is linked to the interaction of the blades, flow gradients, and the supporting tower. The production of wind-farm sound, its propagation, and detection at long distances can be related to the characteristics of the atmospheric boundary layer. First, under stable conditions, mostly occurring at night, winds are highly stratified, which enhances the production of thickness sound and the modulation of other higher-frequency wind turbine sounds. Second, nocturnal atmospheric conditions can create low-altitude waveguides (with altitudes on the order of hundreds of meters) allowing long-distance propagation. Third, night and early morning hours are characterized by reduced background atmospheric noise that enhances signal detectability. This work describes the characteristics of the infrasound from a quasi-continuous source with the potential for long-range propagation that could be used to monitor the lower part of the atmospheric boundary layer. C1 [Marcillo, Omar; Blom, Philip] Los Alamos Natl Lab, Earth & Environm Sci, Los Alamos, NM 87544 USA. [Arrowsmith, Stephen; Jones, Kyle] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Marcillo, O (reprint author), Los Alamos Natl Lab, Earth & Environm Sci, Los Alamos, NM 87544 USA. EM omarcillo@lanl.gov FU Los Alamos Laboratory Directed Research and Development program; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Data for arrays LAG, MOT, and LISA are being submitted to IRIS-DMC (http://ds.iris.edu/ds/nodes/dmc/) under the experiment name and number: "Microbaroms" 201363, respectively. The raw waveforms from the SNL array are proprietary of Sandia National Laboratories and not publicly available; however, the results of the f-k analysis for this array can be retrieved from https://github.com/omarmarcillo/SNLarray-f-k-results.git. The radiosonde data are available at the repository of the Department of Atmospheric Science of the University of Wyoming (http://weather.uwyo.edu/upperair/sounding.html). We thank D. Baker and E. Morton for field deployments and R. Whitaker and Y.J. Kim for their comments on different aspects of this work, which helped to strengthen this paper. We thank also D. Beecher from the Environmental Department of Pueblo of Laguna for her support in the deployment of the LAG array. This research was funded by the Los Alamos Laboratory Directed Research and Development program. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 44 TC 3 Z9 3 U1 3 U2 9 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD OCT 16 PY 2015 VL 120 IS 19 BP 9855 EP 9868 DI 10.1002/2014JD022821 PG 14 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA V45WR UT WOS:000209847200002 ER PT J AU Aartsen, MG Abraham, K Ackermann, M Adams, J Aguilar, JA Ahlers, M Ahrens, M Altmann, D Anderson, T Archinger, M Arguelles, C Arlen, TC Auffenberg, J Bai, X Barwick, SW Baum, V Bay, R Beatty, JJ Tjus, JB Becker, KH Beiser, E BenZvi, S Berghaus, P Berley, D Bernardini, E Bernhard, A Besson, DZ Binder, G Bindig, D Bissok, M Blaufuss, E Blumenthal, J Boersma, DJ Bohm, C Borner, M Bos, F Bose, D Boser, S Botner, O Braun, J Brayeur, L Bretz, HP Brown, AM Buzinsky, N Casey, J Casier, M Cheung, E Chirkin, D Christov, A Christy, B Clark, K Classen, L Coenders, S Cowen, DF Silva, AHC Daughhetee, J Davis, JC Day, M de Andre, JPAM De Clercq, C Dembinski, H De Ridder, S Desiati, P de Vries, KD de Wasseige, G de With, M DeYoung, T Diaz-Velez, JC Dumm, JP Dunkman, M Eagan, R Eberhardt, B Ehrhardt, T Eichmann, B Euler, S Evenson, PA Fadiran, O Fahey, S Fazely, AR Fedynitch, A Feintzeig, J Felde, J Filimonov, K Finley, C Fischer-Wasels, T Flis, S Fuchs, T Glagla, M Gaisser, TK Gaior, R Gallagher, J Gerhardt, L Ghorbani, K Gier, D Gladstone, L Glusenkamp, T Goldschmidt, A Golup, G Gonzalez, JG Gora, D Grant, D Gretskov, P Groh, JC Gross, A Ha, C Haack, C Ismail, AH Hallgren, A Halzen, F Hansmann, B Hanson, K Hebecker, D Heereman, D Helbing, K Hellauer, R Hellwig, D Hickford, S Hignight, J Hill, GC Hoffman, KD Hoffmann, R Holzapfel, K Homeier, A Hoshina, K Huang, F Huber, M Huelsnitz, W Hulth, PO Hultqvist, K In, S Ishihara, A Jacobi, E Japaridze, GS Jero, K Jurkovic, M Kaminsky, B Kappes, A Karg, T Karle, A Kauer, M Keivani, A Kelley, JL Kemp, J Kheirandish, A Kiryluk, J Klas, J Klein, SR Kohnen, G Kolanoski, H Konietz, R Koob, A Kopke, L Kopper, C Kopper, S Koskinen, DJ Kowalski, M Krings, K Kroll, G Kroll, M Kunnen, J Kurahashi, N Kuwabara, T Labare, M Lanfranchi, JL Larson, MJ Lesiak-Bzdak, M Leuermann, M Leuner, J Lunemann, J Madsen, J Maggi, G Mahn, KBM Maruyama, R Mase, K Matis, HS Maunu, R McNally, F Meagher, K Medici, M Meli, A Menne, T Merino, G Meures, T Miarecki, S Middell, E Middlemas, E Miller, J Mohrmann, L Montaruli, T Morse, R Nahnhauer, R Naumann, U Niederhausen, H Nowicki, SC Nygren, DR Obertacke, A Olivas, A Omairat, A O'Murchadha, A Palczewski, T Paul, L Pepper, JA de los Heros, CP Pfendner, C Pieloth, D Pinat, E Posselt, J Price, PB Przybylski, GT Putz, J Quinnan, M Radel, L Rameez, M Rawlins, K Redl, P Reimann, R Relich, M Resconi, E Rhode, W Richman, M Richter, S Riedel, B Robertson, S Rongen, M Rott, C Ruhe, T Ruzybayev, B Ryckbosch, D Saba, SM Sabbatini, L Sander, HG Sandrock, A Sandroos, J Sarkar, S Schatto, K Scheriau, F Schimp, M Schmidt, T Schmitz, M Schoenen, S Schoneberg, S Schoenwald, A Schukraft, A Schulte, L Seckel, D Seunarine, S Shanidze, R Smith, MWE Soldin, D Spiczak, GM Spiering, C Stahlberg, M Stamatikos, M Stanev, T Stanisha, NA Stasik, A Stezelberger, T Stokstad, RG Stossl, A Strahler, EA Strom, R Strotjohann, NL Sullivan, GW Sutherland, M Taavola, H Taboada, I Ter-Antonyan, S Terliuk, A Tesic, G Tilav, S Toale, PA Tobin, MN Tosi, D Tselengidou, M Unger, E Usner, M Vallecorsa, S van Eijndhoven, N Vandenbroucke, J van Santen, J Vanheule, S Veenkamp, J Vehring, M Voge, M Vraeghe, M Walck, C Wallraff, M Wandkowsky, N Weaver, C Wendt, C Westerhoff, S Whelan, BJ Whitehorn, N Wichary, C Wiebe, K Wiebusch, CH Wille, L Williams, DR Wissing, H Wolf, M Wood, TR Woschnagg, K Xu, DL Xu, XW Xu, Y Yanez, JP Yodh, G Yoshida, S Zarzhitsky, P Zoll, M AF Aartsen, M. G. Abraham, K. Ackermann, M. Adams, J. Aguilar, J. A. Ahlers, M. Ahrens, M. Altmann, D. Anderson, T. Archinger, M. Arguelles, C. Arlen, T. C. Auffenberg, J. Bai, X. Barwick, S. W. Baum, V. Bay, R. Beatty, J. J. Tjus, J. Becker Becker, K. -H. Beiser, E. BenZvi, S. Berghaus, P. Berley, D. Bernardini, E. Bernhard, A. Besson, D. Z. Binder, G. Bindig, D. Bissok, M. Blaufuss, E. Blumenthal, J. Boersma, D. J. Bohm, C. Boerner, M. Bos, F. Bose, D. Boeser, S. Botner, O. Braun, J. Brayeur, L. Bretz, H. -P. Brown, A. M. Buzinsky, N. Casey, J. Casier, M. Cheung, E. Chirkin, D. Christov, A. Christy, B. Clark, K. Classen, L. Coenders, S. Cowen, D. F. Silva, A. H. Cruz Daughhetee, J. Davis, J. C. Day, M. de Andre, J. P. A. M. De Clercq, C. Dembinski, H. De Ridder, S. Desiati, P. de Vries, K. D. de Wasseige, G. de With, M. DeYoung, T. Diaz-Velez, J. C. Dumm, J. P. Dunkman, M. Eagan, R. Eberhardt, B. Ehrhardt, T. Eichmann, B. Euler, S. Evenson, P. A. Fadiran, O. Fahey, S. Fazely, A. R. Fedynitch, A. Feintzeig, J. Felde, J. Filimonov, K. Finley, C. Fischer-Wasels, T. Flis, S. Fuchs, T. Glagla, M. Gaisser, T. K. Gaior, R. Gallagher, J. Gerhardt, L. Ghorbani, K. Gier, D. Gladstone, L. Gluesenkamp, T. Goldschmidt, A. Golup, G. Gonzalez, J. G. Gora, D. Grant, D. Gretskov, P. Groh, J. C. Gross, A. Ha, C. Haack, C. Ismail, A. Haj Hallgren, A. Halzen, F. Hansmann, B. Hanson, K. Hebecker, D. Heereman, D. Helbing, K. Hellauer, R. Hellwig, D. Hickford, S. Hignight, J. Hill, G. C. Hoffman, K. D. Hoffmann, R. Holzapfel, K. Homeier, A. Hoshina, K. Huang, F. Huber, M. Huelsnitz, W. Hulth, P. O. Hultqvist, K. In, S. Ishihara, A. Jacobi, E. Japaridze, G. S. Jero, K. Jurkovic, M. Kaminsky, B. Kappes, A. Karg, T. Karle, A. Kauer, M. Keivani, A. Kelley, J. L. Kemp, J. Kheirandish, A. Kiryluk, J. Klaes, J. Klein, S. R. Kohnen, G. Kolanoski, H. Konietz, R. Koob, A. Koepke, L. Kopper, C. Kopper, S. Koskinen, D. J. Kowalski, M. Krings, K. Kroll, G. Kroll, M. Kunnen, J. Kurahashi, N. Kuwabara, T. Labare, M. Lanfranchi, J. L. Larson, M. J. Lesiak-Bzdak, M. Leuermann, M. Leuner, J. Luenemann, J. Madsen, J. Maggi, G. Mahn, K. B. M. Maruyama, R. Mase, K. Matis, H. S. Maunu, R. McNally, F. Meagher, K. Medici, M. Meli, A. Menne, T. Merino, G. Meures, T. Miarecki, S. Middell, E. Middlemas, E. Miller, J. Mohrmann, L. Montaruli, T. Morse, R. Nahnhauer, R. Naumann, U. Niederhausen, H. Nowicki, S. C. Nygren, D. R. Obertacke, A. Olivas, A. Omairat, A. O'Murchadha, A. Palczewski, T. Paul, L. Pepper, J. A. de los Heros, C. Perez Pfendner, C. Pieloth, D. Pinat, E. Posselt, J. Price, P. B. Przybylski, G. T. Puetz, J. Quinnan, M. Raedel, L. Rameez, M. Rawlins, K. Redl, P. Reimann, R. Relich, M. Resconi, E. Rhode, W. Richman, M. Richter, S. Riedel, B. Robertson, S. Rongen, M. Rott, C. Ruhe, T. Ruzybayev, B. Ryckbosch, D. Saba, S. M. Sabbatini, L. Sander, H. -G. Sandrock, A. Sandroos, J. Sarkar, S. Schatto, K. Scheriau, F. Schimp, M. Schmidt, T. Schmitz, M. Schoenen, S. Schoeneberg, S. Schoenwald, A. Schukraft, A. Schulte, L. Seckel, D. Seunarine, S. Shanidze, R. Smith, M. W. E. Soldin, D. Spiczak, G. M. Spiering, C. Stahlberg, M. Stamatikos, M. Stanev, T. Stanisha, N. A. Stasik, A. Stezelberger, T. Stokstad, R. G. Stoessl, A. Strahler, E. A. Stroem, R. Strotjohann, N. L. Sullivan, G. W. Sutherland, M. Taavola, H. Taboada, I. Ter-Antonyan, S. Terliuk, A. Tesic, G. Tilav, S. Toale, P. A. Tobin, M. N. Tosi, D. Tselengidou, M. Unger, E. Usner, M. Vallecorsa, S. van Eijndhoven, N. Vandenbroucke, J. van Santen, J. Vanheule, S. Veenkamp, J. Vehring, M. Voge, M. Vraeghe, M. Walck, C. Wallraff, M. Wandkowsky, N. Weaver, Ch. Wendt, C. Westerhoff, S. Whelan, B. J. Whitehorn, N. Wichary, C. Wiebe, K. Wiebusch, C. H. Wille, L. Williams, D. R. Wissing, H. Wolf, M. Wood, T. R. Woschnagg, K. Xu, D. L. Xu, X. W. Xu, Y. Yanez, J. P. Yodh, G. Yoshida, S. Zarzhitsky, P. Zoll, M. TI Search for dark matter annihilation in the Galactic Center with IceCube-79 SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID HALO; GALAXIES; PERFORMANCE; PARTICLES; CLUSTER; DESIGN; SYSTEM; MASS AB The Milky Way is expected to be embedded in a halo of dark matter particles, with the highest density in the central region, and decreasing density with the halo-centric radius. Dark matter might be indirectly detectable at Earth through a flux of stable particles generated in dark matter annihilations and peaked in the direction of the Galactic Center. We present a search for an excess flux of muon (anti-) neutrinos from dark matter annihilation in the Galactic Center using the cubic-kilometer-sized IceCube neutrino detector at the South Pole. There, the Galactic Center is always seen above the horizon. Thus, new and dedicated veto techniques against atmospheric muons are required to make the southern hemisphere accessible for IceCube. We used 319.7 live-days of data from IceCube operating in its 79-string configuration during 2010 and 2011. No neutrino excess was found and the final result is compatible with the background. We present upper limits on the self-annihilation cross-section, < sAv >, for WIMP masses ranging from 30GeV up to 10TeV, assuming cuspy (NFW) and flat-cored (Burkert) dark matter halo profiles, reaching down to similar or equal to 4 . 10(-24) cm(3) s(-1), and similar or equal to 2.6 . 10(-23) cm(3) s(-1) for the nu(nu) over bar channel, respectively. C1 [Auffenberg, J.; Bissok, M.; Blumenthal, J.; Glagla, M.; Gier, D.; Gretskov, P.; Haack, C.; Hansmann, B.; Hellwig, D.; Kemp, J.; Konietz, R.; Koob, A.; Leuermann, M.; Leuner, J.; Paul, L.; Puetz, J.; Raedel, L.; Reimann, R.; Rongen, M.; Schimp, M.; Schoenen, S.; Schukraft, A.; Stahlberg, M.; Vehring, M.; Wallraff, M.; Wichary, C.; Wiebusch, C. H.] Rhein Westfal TH Aachen, Inst Phys 3, D-52056 Aachen, Germany. [Aartsen, M. G.; Hill, G. C.; Robertson, S.; Whelan, B. J.] Univ Adelaide, Sch Chem & Phys, Adelaide, SA 5005, Australia. [Rawlins, K.] Univ Alaska Anchorage, Dept Phys & Astron, Anchorage, AK 99508 USA. [Japaridze, G. S.] Clark Atlanta Univ, CTSPS, Atlanta, GA 30314 USA. [Casey, J.; Daughhetee, J.; Taboada, I.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Casey, J.; Daughhetee, J.; Taboada, I.] Georgia Inst Technol, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Fazely, A. R.; Ter-Antonyan, S.; Xu, X. W.] Southern Univ, Dept Phys, Baton Rouge, LA 70813 USA. [Bay, R.; Binder, G.; Filimonov, K.; Gerhardt, L.; Ha, C.; Klein, S. R.; Miarecki, S.; Price, P. B.; Woschnagg, K.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Binder, G.; Gerhardt, L.; Goldschmidt, A.; Ha, C.; Klein, S. R.; Matis, H. S.; Miarecki, S.; Nygren, D. R.; Przybylski, G. T.; Stezelberger, T.; Stokstad, R. G.] Lawrence Berkeley Natl Lab, Berkeley, CA USA. [de With, M.; Hebecker, D.; Kolanoski, H.; Kowalski, M.] Humboldt Univ, D-12489 Berlin, Germany. [Tjus, J. Becker; Bos, F.; Eichmann, B.; Fedynitch, A.; Kroll, M.; Saba, S. M.; Schoeneberg, S.] Ruhr Univ Bochum, Fak Phys & Astron, D-44780 Bochum, Germany. [Homeier, A.; Schulte, L.; Voge, M.] Univ Bonn, Inst Phys, D-53115 Bonn, Germany. [Aguilar, J. A.; Heereman, D.; Meagher, K.; Meures, T.; O'Murchadha, A.; Pinat, E.] Univ Libre Bruxelles, Fac Sci, B-1050 Brussels, Belgium. [Brayeur, L.; Casier, M.; De Clercq, C.; de Vries, K. D.; de Wasseige, G.; Golup, G.; Kunnen, J.; Maggi, G.; Miller, J.; Strahler, E. A.; van Eijndhoven, N.] Vrije Univ Brussel, Dienst ELEM, Brussels, Belgium. [Gaior, R.; Ishihara, A.; Kuwabara, T.; Mase, K.; Relich, M.; Yoshida, S.] Chiba Univ, Dept Phys, Chiba 2638522, Japan. [Adams, J.; Brown, A. M.] Univ Canterbury, Dept Phys & Astron, Christchurch 1, New Zealand. [Berley, D.; Blaufuss, E.; Cheung, E.; Christy, B.; Felde, J.; Hellauer, R.; Hoffman, K. D.; Huelsnitz, W.; Maunu, R.; Olivas, A.; Redl, P.; Schmidt, T.; Sullivan, G. W.; Wissing, H.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Beatty, J. J.; Davis, J. C.; Pfendner, C.; Stamatikos, M.; Sutherland, M.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Beatty, J. J.; Davis, J. C.; Pfendner, C.; Stamatikos, M.; Sutherland, M.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Beatty, J. J.] Ohio State Univ, Dept Astron, Columbus, OH 43210 USA. [Koskinen, D. J.; Larson, M. J.; Medici, M.; Sandroos, J.; Sarkar, S.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Boerner, M.; Fuchs, T.; Menne, T.; Pieloth, D.; Rhode, W.; Ruhe, T.; Sandrock, A.; Scheriau, F.; Schmitz, M.] TU Dortmund Univ, Dept Phys, D-44221 Dortmund, Germany. [de Andre, J. P. A. M.; DeYoung, T.; Hignight, J.; Mahn, K. B. M.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Buzinsky, N.; Grant, D.; Kopper, C.; Nowicki, S. C.; Riedel, B.; Wood, T. R.] Univ Alberta, Dept Phys, Edmonton, AB T6G 2E1, Canada. [Altmann, D.; Classen, L.; Kappes, A.; Tselengidou, M.] Univ Erlangen Nurnberg, Erlangen Ctr Astroparticle Phys, D-91058 Erlangen, Germany. [Christov, A.; Montaruli, T.; Rameez, M.; Vallecorsa, S.] Univ Geneva, Dept phys nucl & corpusculaire, CH-1211 Geneva, Switzerland. [De Ridder, S.; Ismail, A. Haj; Labare, M.; Meli, A.; Ryckbosch, D.; Vanheule, S.; Vraeghe, M.] Univ Ghent, Dept Phys & Astron, B-9000 Ghent, Belgium. [Barwick, S. W.; Yodh, G.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Besson, D. Z.] Univ Kansas, Dept Phys & Astron, Lawrence, KS 66045 USA. [Gallagher, J.] Univ Wisconsin, Dept Astron, Madison, WI 53706 USA. [Ahlers, M.; Arguelles, C.; Beiser, E.; BenZvi, S.; Braun, J.; Chirkin, D.; Day, M.; Desiati, P.; Diaz-Velez, J. C.; Fadiran, O.; Fahey, S.; Feintzeig, J.; Ghorbani, K.; Gladstone, L.; Halzen, F.; Hanson, K.; Hoshina, K.; Jero, K.; Karle, A.; Kauer, M.; Kelley, J. L.; Kheirandish, A.; McNally, F.; Merino, G.; Middlemas, E.; Morse, R.; Richter, S.; Sabbatini, L.; Tobin, M. N.; Tosi, D.; Vandenbroucke, J.; van Santen, J.; Wandkowsky, N.; Weaver, Ch.; Wendt, C.; Westerhoff, S.; Whitehorn, N.; Wille, L.] Univ Wisconsin, Dept Phys, Wisconsin IceCube Particle Astrophys Ctr, Madison, WI 53706 USA. [Archinger, M.; Baum, V.; Boeser, S.; Eberhardt, B.; Ehrhardt, T.; Koepke, L.; Kroll, G.; Luenemann, J.; Sander, H. -G.; Schatto, K.; Wiebe, K.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55099 Mainz, Germany. [Kohnen, G.] Univ Mons, B-7000 Mons, Belgium. [Abraham, K.; Bernhard, A.; Coenders, S.; Gross, A.; Holzapfel, K.; Huber, M.; Jurkovic, M.; Krings, K.; Resconi, E.; Veenkamp, J.] Tech Univ Munich, D-85748 Garching, Germany. [Dembinski, H.; Evenson, P. A.; Gaisser, T. K.; Gonzalez, J. G.; Ruzybayev, B.; Seckel, D.; Stanev, T.; Tilav, S.] Univ Delaware, Bartol Res Inst, Dept Phys & Astron, Newark, DE 19716 USA. [Kauer, M.; Maruyama, R.] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Sarkar, S.] Univ Oxford, Dept Phys, Oxford OX1 3NP, England. [Kurahashi, N.; Richman, M.] Drexel Univ, Dept Phys, Philadelphia, PA 19104 USA. [Bai, X.] South Dakota Sch Mines & Technol, Dept Phys, Rapid City, SD 57701 USA. [Madsen, J.; Seunarine, S.; Spiczak, G. M.] Univ Wisconsin, Dept Phys, River Falls, WI 54022 USA. [Ahrens, M.; Bohm, C.; Dumm, J. P.; Finley, C.; Flis, S.; Hulth, P. O.; Hultqvist, K.; Walck, C.; Wolf, M.; Zoll, M.] Univ Stockholm, Dept Phys, Oskar Klein Ctr, S-10691 Stockholm, Sweden. [Kiryluk, J.; Lesiak-Bzdak, M.; Niederhausen, H.; Xu, Y.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Bose, D.; In, S.; Rott, C.] Sungkyunkwan Univ, Dept Phys, Suwon 440 746, South Korea. [Clark, K.] Univ Toronto, Dept Phys, Toronto, ON M5S 1A7, Canada. [Palczewski, T.; Pepper, J. A.; Toale, P. A.; Williams, D. R.; Xu, D. L.; Zarzhitsky, P.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA. [Cowen, D. F.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Anderson, T.; Arlen, T. C.; Cowen, D. F.; Dunkman, M.; Eagan, R.; Groh, J. C.; Huang, F.; Keivani, A.; Lanfranchi, J. L.; Quinnan, M.; Smith, M. W. E.; Stanisha, N. A.; Tesic, G.] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Boersma, D. J.; Botner, O.; Euler, S.; Hallgren, A.; de los Heros, C. Perez; Stroem, R.; Taavola, H.; Unger, E.] Uppsala Univ, Dept Phys & Astron, S-75120 Uppsala, Sweden. [Becker, K. -H.; Bindig, D.; Fischer-Wasels, T.; Helbing, K.; Hickford, S.; Hoffmann, R.; Klaes, J.; Kopper, S.; Naumann, U.; Obertacke, A.; Omairat, A.; Posselt, J.; Soldin, D.] Univ Wuppertal, Dept Phys, D-42119 Wuppertal, Germany. [Ackermann, M.; Berghaus, P.; Bernardini, E.; Bretz, H. -P.; Silva, A. H. Cruz; Gluesenkamp, T.; Gora, D.; Jacobi, E.; Kaminsky, B.; Karg, T.; Kopper, S.; Middell, E.; Mohrmann, L.; Nahnhauer, R.; Schoenwald, A.; Shanidze, R.; Spiering, C.; Stasik, A.; Stoessl, A.; Strotjohann, N. L.; Terliuk, A.; Usner, M.; Yanez, J. P.] DESY, D-15735 Zeuthen, Germany. RP Aartsen, MG (reprint author), Univ Adelaide, Sch Chem & Phys, Adelaide, SA 5005, Australia. EM samuel.flis@fysik.su.se RI Tjus, Julia/G-8145-2012; Maruyama, Reina/A-1064-2013; Beatty, James/D-9310-2011; Sarkar, Subir/G-5978-2011; Wiebusch, Christopher/G-6490-2012; Koskinen, David/G-3236-2014 OI Maruyama, Reina/0000-0003-2794-512X; Strotjohann, Nora Linn/0000-0002-4667-6730; Beatty, James/0000-0003-0481-4952; Sarkar, Subir/0000-0002-3542-858X; Wiebusch, Christopher/0000-0002-6418-3008; Koskinen, David/0000-0002-0514-5917 FU U.S. National Science Foundation-Office of Polar Programs; U.S. National Science Foundation-Physics Division, University of Wisconsin Alumni Research Foundation; Grid Laboratory Of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin - Madison; Open Science Grid (OSG) grid infrastructure; U.S. Department of Energy; National Energy Research Scientific Computing Center; Louisiana Optical Network Initiative (LONI); Natural Sciences and Engineering Research Council of Canada; West-Grid and Compute/Calcul Canada; Swedish Research Council, Sweden; Swedish Polar Research Secretariat, Sweden; Swedish National Infrastructure for Computing (SNIC), Sweden; Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF), Germany; Deutsche Forschungsgemeinschaft (DFG), Germany; Helmholtz Alliance for Astroparticle Physics (HAP), Germany; Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO); FWO Odysseus programme; Flanders Institute to encourage scientific and technological research in industry (IWT); Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); Swiss National Science Foundation (SNSF), Switzerland; National Research Foundation of Korea (NRF); Danish National Research Foundation, Denmark (DNRF) FX We acknowledge the support from the following agencies: U.S. National Science Foundation-Office of Polar Programs, U.S. National Science Foundation-Physics Division, University of Wisconsin Alumni Research Foundation, the Grid Laboratory Of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin - Madison, the Open Science Grid (OSG) grid infrastructure; U.S. Department of Energy, and National Energy Research Scientific Computing Center, the Louisiana Optical Network Initiative (LONI) grid computing resources; Natural Sciences and Engineering Research Council of Canada, West-Grid and Compute/Calcul Canada; Swedish Research Council, Swedish Polar Research Secretariat, Swedish National Infrastructure for Computing (SNIC), and Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF), Deutsche Forschungsgemeinschaft (DFG), Helmholtz Alliance for Astroparticle Physics (HAP), Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO), FWO Odysseus programme, Flanders Institute to encourage scientific and technological research in industry (IWT), Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); the Swiss National Science Foundation (SNSF), Switzerland; National Research Foundation of Korea (NRF); Danish National Research Foundation, Denmark (DNRF). NR 51 TC 20 Z9 20 U1 2 U2 6 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD OCT 15 PY 2015 VL 75 IS 10 AR 492 DI 10.1140/epjc/s10052-015-3713-1 PG 12 WC Physics, Particles & Fields SC Physics GA CY3LS UT WOS:000366311800002 ER PT J AU Belmann, P Droge, J Bremges, A McHardy, AC Sczyrba, A Barton, MD AF Belmann, Peter Droege, Johannes Bremges, Andreas McHardy, Alice C. Sczyrba, Alexander Barton, Michael D. TI Bioboxes: standardised containers for interchangeable bioinformatics software SO GIGASCIENCE LA English DT Editorial Material DE Bioinformatics; Software; Docker; Standards; Usability; Reproducibility AB Software is now both central and essential to modern biology, yet lack of availability, difficult installations, and complex user interfaces make software hard to obtain and use. Containerisation, as exemplified by the Docker platform, has the potential to solve the problems associated with sharing software. We propose bioboxes: containers with standardised interfaces to make bioinformatics software interchangeable. C1 [Belmann, Peter; Bremges, Andreas; Sczyrba, Alexander] Univ Bielefeld, Fac Technol, D-33615 Bielefeld, Germany. [Belmann, Peter; Bremges, Andreas; Sczyrba, Alexander] Univ Bielefeld, Ctr Biotechnol, D-33615 Bielefeld, Germany. [Droege, Johannes; Bremges, Andreas; McHardy, Alice C.] Helmholtz Ctr Infect Res, Computat Biol Infect Res, D-38124 Braunschweig, Germany. [Barton, Michael D.] DOE Joint Genome Inst, Walnut Creek, CA 94598 USA. RP Barton, MD (reprint author), DOE Joint Genome Inst, Walnut Creek, CA 94598 USA. EM mail@michaelbarton.me.uk OI Droge, Johannes/0000-0002-6752-2204 NR 6 TC 4 Z9 5 U1 1 U2 4 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND EI 2047-217X J9 GIGASCIENCE JI GigaScience PD OCT 15 PY 2015 VL 4 AR 47 DI 10.1186/s13742-015-0087-0 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CX4KG UT WOS:000365668400001 PM 26473029 ER PT J AU Bi, S Sun, CN Zawodzinski, TA Ren, F Keum, JK Ahn, SK Li, DW Chen, JH AF Bi, Sheng Sun, Che-Nan Zawodzinski, Thomas A., Jr. Ren, Fei Keum, Jong Kahk Ahn, Suk-Kyun Li, Dawen Chen, Jihua TI Reciprocated Suppression of Polymer Crystallization Toward Improved Solid Polymer Electrolytes: Higher Ion Conductivity and Tunable Mechanical Properties SO JOURNAL OF POLYMER SCIENCE PART B-POLYMER PHYSICS LA English DT Article DE blends; crystallization; ion conductivity; polymer crystallization; reciprocated suppression; solid polymer electrolytes; TEM ID POLY(ETHYLENE OXIDE); THERMAL-PROPERTIES; LITHIUM BATTERIES; GEL ELECTROLYTES; SOLAR-CELLS; MORPHOLOGY; CRYSTALLINITY; TRANSPORT; BEHAVIOR; BLENDS AB Solid polymer electrolytes based on lithium bis(trifluoromethanesulfonyl) imide and polymer matrix were extensively studied in the past due to their excellent potential in a broad range of energy related applications. Poly(vinylidene fluoride) (PVDF) and polyethylene oxide (PEO) are among the most examined polymer candidates as solid polymer electrolyte matrix. In this work, we study the effect of reciprocated suppression of polymer crystallization in PVDF/PEO binary matrix on ion transport and mechanical properties of the resultant solid polymer electrolytes. With electron and X-ray diffractions as well as energy filtered transmission electron microscopy, we identify and examine the appropriate blending composition that is responsible for the diminishment of both PVDF and PEO crystallites. A three-fold conductivity enhancement is achieved along with a highly tunable elastic modulus ranging from 20 to 200 MPa, which is expected to contribute toward future designs of solid polymer electrolytes with high room-temperature ion conductivities and mechanical flexibility. (C) 2015 Wiley Periodicals, Inc. C1 [Bi, Sheng; Li, Dawen] Univ Alabama, Dept Elect & Comp Engn, Ctr Mat Informat Technol, Tuscaloosa, AL 35487 USA. [Sun, Che-Nan; Zawodzinski, Thomas A., Jr.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Zawodzinski, Thomas A., Jr.] Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA. [Ren, Fei] Temple Univ, Dept Mech Engn, Philadelphia, PA 19122 USA. [Keum, Jong Kahk] Oak Ridge Natl Lab, Neutron Scattering Sci Div, Oak Ridge, TN 37831 USA. [Keum, Jong Kahk; Ahn, Suk-Kyun; Chen, Jihua] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Ahn, Suk-Kyun] Pusan Natl Univ, Dept Polymer Sci & Engn, Busan 609735, South Korea. RP Chen, JH (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM dawenl@eng.ua.edu; chenj1@ornl.gov RI Chen, Jihua/F-1417-2011; Keum, Jong/N-4412-2015 OI Chen, Jihua/0000-0001-6879-5936; Keum, Jong/0000-0002-5529-1373 FU NSF [ECCS-1151140]; U.S. Department of Energy [DE-AC05-00OR22725] FX This research was conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. J. Chen wish to thank Dr. Kunlun Hong (ORNL) for providing the PEO samples. D. Li acknowledges CNMS user project and financial support from NSF grant #ECCS-1151140. Notice: This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 30 TC 0 Z9 0 U1 4 U2 33 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0887-6266 EI 1099-0488 J9 J POLYM SCI POL PHYS JI J. Polym. Sci. Pt. B-Polym. Phys. PD OCT 15 PY 2015 VL 53 IS 20 BP 1450 EP 1457 DI 10.1002/polb.23793 PG 8 WC Polymer Science SC Polymer Science GA CU9YC UT WOS:000363902000005 ER PT J AU Perticaroli, S Ehlers, G Jalarvo, N Katsaras, J Nickels, JD AF Perticaroli, Stefania Ehlers, Georg Jalarvo, Niina Katsaras, John Nickels, Jonathan D. TI Elasticity and Inverse Temperature Transition in Elastin SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID INELASTIC NEUTRON-SCATTERING; SECONDARY STRUCTURE; BOSON PEAK; BACKBONE CONTRIBUTIONS; HYDROPHOBIC HYDRATION; HUMAN TROPOELASTIN; BOVINE ELASTIN; SIDE-CHAIN; PROTEIN; DYNAMICS AB Elastin is a structural protein and biomaterial that provides elasticity and resilience to a range of tissues. This work provides insights into the elastic properties of elastin and its peculiar inverse temperature transition (ITT). These features are dependent on hydration of elastin and are driven by a similar mechanism of hydrophobic collapse to an entropically favorable state. Using neutron scattering, we quantify the changes in the geometry of molecular motions above and below the transition temperature, showing a reduction in the displacement of water-induced motions upon hydrophobic collapse at the ITT. We also measured the collective vibrations of elastin gels as a function of elongation, revealing no changes in the spectral features associated with local rigidity and secondary structure, in agreement with the entropic origin of elasticity. C1 [Perticaroli, Stefania; Katsaras, John; Nickels, Jonathan D.] Oak Ridge Natl Lab, Joint Inst Neutron Sci, Oak Ridge, TN 37831 USA. [Perticaroli, Stefania] Oak Ridge Natl Lab, Div Chem & Mat Sci, Oak Ridge, TN 37831 USA. [Perticaroli, Stefania] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Ehlers, Georg] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Jalarvo, Niina] Forschungszentrum Julich, Julich Ctr Neutron Sci, D-52425 Julich, Germany. [Jalarvo, Niina] Oak Ridge Natl Lab, Neutron Sci Directorate, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Jalarvo, Niina] Oak Ridge Natl Lab, JCNS Outstn, Spallat Neutron Source, Oak Ridge, TN 37831 USA. [Katsaras, John; Nickels, Jonathan D.] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. [Nickels, Jonathan D.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RP Perticaroli, S (reprint author), Oak Ridge Natl Lab, Joint Inst Neutron Sci, POB 2008,MS-6453, Oak Ridge, TN 37831 USA. EM perticarolis@ornl.gov; nickelsjd@ornl.gov RI Instrument, CNCS/B-4599-2012; Jalarvo, Niina/Q-1320-2015; Nickels, Jonathan/I-1913-2012; Ehlers, Georg/B-5412-2008; OI Jalarvo, Niina/0000-0003-0644-6866; Nickels, Jonathan/0000-0001-8351-7846; Ehlers, Georg/0000-0003-3513-508X; Katsaras, John/0000-0002-8937-4177 FU NSF [DMR-1408811]; Scientific User Facilities Division of the DOE Office of Basic Energy Sciences (BES) [DE-AC05 00OR2275]; Scientific User Facilities Division, Office of Basic Energy Sciences, DOE; UT-Battelle, LLC [DE-AC0500OR22725] FX The authors would like to thank Prof. Alexei P. Sokolov for helpful discussions. S.P. acknowledges partial financial support from NSF Polymer program under Grant DMR-1408811. J.K. and J.D.N. are supported through the Scientific User Facilities Division of the DOE Office of Basic Energy Sciences (BES), under contract no. DE-AC05 00OR2275. Research at Oak Ridge National Laboratory's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, DOE. Oak Ridge National Laboratory facilities are sponsored by UT-Battelle, LLC, for the U.S. Department of Energy under Contract No. DE-AC0500OR22725. NR 63 TC 3 Z9 3 U1 4 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD OCT 15 PY 2015 VL 6 IS 20 BP 4018 EP 4025 DI 10.1021/acs.jpclett.5b01890 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CT8RM UT WOS:000363083900005 PM 26722771 ER PT J AU Savee, JD Selby, TM Welz, O Taatjes, CA Osborn, DL AF Savee, John D. Selby, Talitha M. Welz, Oliver Taatjes, Craig A. Osborn, David L. TI Time- and Isomer-Resolved Measurements of Sequential Addition of Acetylene to the Propargyl Radical SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID SOOT FORMATION; AROMATIC-COMPOUNDS; ALIPHATIC FUELS; CYCLOPENTADIENYL; PHOTOIONIZATION; KINETICS; FLAMES; SYNCHROTRON; MECHANISM; MIXTURES AB Soot formation in combustion is a complex process in which polycyclic aromatic hydrocarbons (PAHs) are believed to play a critical role. Recent works concluded that three consecutive additions of acetylene (C2H2) to propargyl (C3H3) create a facile route to the PAR indene (C9H8). However, the isomeric forms of C5H5 and C7H7 intermediates in this reaction sequence are not known. We directly investigate these intermediates using time- and isomer-resolved experiments. Both the resonance stabilized vinylpropargyl (vp-C5H5) and 2,4-cyclopentadienyl (c-C5H5) radical isomers of C5H5 are produced, with substantially different intensities at 800 K vs 1000 K. In agreement with literature master equation calculations, we find that c-C5H5 + C2H2 produces only the tropyl isomer of C7H7 (tp-C7H7) below 1000 K, and that tp-C7H7 + C2H2 terminates the reaction sequence yielding C9H8 (indene) + H. This work demonstrates a pathway for PAH formation that does not proceed through benzene. C1 [Savee, John D.; Selby, Talitha M.; Welz, Oliver; Taatjes, Craig A.; Osborn, David L.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. RP Osborn, DL (reprint author), Sandia Natl Labs, Combust Res Facil, Mail Stop 9055, Livermore, CA 94551 USA. EM dlosbor@sandia.gov FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; NNSA [DE-AC04-94-AL85000] FX We thank Howard Johnsen and the staff of the Chemical Dynamics Beam line at the Advanced Light Source (ALS) for support of the present experiments. We are also grateful to Dr. Kathrin Fischer and Prof. Ingo Fischer for discussions regarding the tropyl radical. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. Sandia is a multiprogram laboratory operated by the Sandia Corporation, a Lockheed Martin Company, for the NNSA under Contract No. DE-AC04-94-AL85000. This research used resources of the Advanced Light Source of Lawrence Berkeley National Laboratory, which is a DOE Office of Science User Facility. NR 27 TC 8 Z9 8 U1 8 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD OCT 15 PY 2015 VL 6 IS 20 BP 4153 EP 4158 DI 10.1021/acs.jpclett.5b01896 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CT8RM UT WOS:000363083900027 PM 26722791 ER PT J AU Ognibene, TJ Haack, KW Bench, G Brown, TA Turteltaub, KW AF Ognibene, T. J. Haack, K. W. Bench, G. Brown, T. A. Turteltaub, K. W. TI Operation of the "Small" BioAMS spectrometers at CAMS: Past and future prospects SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 13th International Conference on Accelerator Mass Spectrometry (AMS) CY AUG 24-29, 2014 CL Aix en Provence, FRANCE DE Accelerator mass spectrometry; SSAMS; Graphite; Biomedical AMS; C-14 ID ACCELERATOR MASS-SPECTROMETRY; BIOCHEMICAL SAMPLES; ION-SOURCE; C-14; AMS AB A summary of results from the solid samples run on our compact 1 MV AMS system over its 13.5 years of operation is presented. On average 7065 samples per year were measured with that average dropping to 3278 samples per year following the deployment of our liquid sample capability. Although the dynamic range of our spectrometer is 4.5 orders in magnitude, most of the measured graphitic samples had C-14/C concentrations between 0.1 and 1 modern. The measurements of our ANU sucrose standard followed a Gaussian distribution with an average of 1.5082 +/- 0.0134 modern. The LLNL biomedical AMS program supported many different types of experiments, however, the large majority of samples measured were derived from animal model systems. We have transitioned all of our biomedical AMS measurements to the recently installed 250 kV SSAMS instrument with good agreement compared in measured C-14/C isotopic ratios between sample splits. Finally, we present results from replacement of argon stripping gas with helium in the SSAMS with a 22% improvement in ion transmission through the accelerator and high-energy analyzing magnet. (C) 2015 Elsevier B.V. All rights reserved. C1 [Ognibene, T. J.; Haack, K. W.; Bench, G.; Brown, T. A.] Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, Livermore, CA 94551 USA. [Turteltaub, K. W.] Lawrence Livermore Natl Lab, Biol & Biotechnol Div, Livermore, CA 94551 USA. RP Ognibene, TJ (reprint author), Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, 7000 East Ave, Livermore, CA 94551 USA. EM ognibene1@llnl.gov FU U.S. Department of Energy [DE-AC52-07NA27344]; National Institutes of Health (NIH), National Institute of General Medical Sciences (NIGMS), Biomedical Technology Research Resources (BTRR) [8P41GM103483] FX Work performed at the Research Resource for Biomedical AMS, which is operated at LLNL under the auspices of the U.S. Department of Energy under contract DE-AC52-07NA27344, is supported by the National Institutes of Health (NIH), National Institute of General Medical Sciences (NIGMS), Biomedical Technology Research Resources (BTRR) under grant number 8P41GM103483. NR 12 TC 0 Z9 0 U1 1 U2 7 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD OCT 15 PY 2015 VL 361 BP 54 EP 57 DI 10.1016/j.nimb.2015.05.019 PG 4 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CU2HZ UT WOS:000363345900010 PM 26456990 ER PT J AU Ognibene, TJ Thomas, A Daley, PF Bench, G Turteltaub, KW AF Ognibene, T. J. Thomas, At. Daley, P. F. Bench, G. Turteltaub, K. W. TI An interface for the direct coupling of small liquid samples to AMS SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 13th International Conference on Accelerator Mass Spectrometry (AMS) CY AUG 24-29, 2014 CL Aix en Provence, FRANCE DE Accelerator Mass Spectrometry; CO2; HPLC interfaces; C-14 ID ACCELERATOR MASS-SPECTROMETRY; ION-SOURCE; CHROMATOGRAPHY; CARBON; C-14; GAS AB We describe the moving wire interface attached to the 1-MV AMS system at LLNL's Center for Accelerator Mass Spectrometry for the analysis of nonvolatile liquid samples as either discrete drops or from the direct output of biochemical separatory instrumentation, such as high-performance liquid chromatography (HPLC). Discrete samples containing at least a few 10 s of nanograms of carbon and as little as 50 zmol C-14 can be measured with a 3-5% precision in a few minutes. The dynamic range of our system spans approximately 3 orders in magnitude. Sample to sample memory is minimized by the use of fresh targets for each discrete sample or by minimizing the amount of carbon present in a peak generated by an HPLC containing a significant amount of C-14. Liquid sample AMS provides a new technology to expand our biomedical AMS program by enabling the capability to measure low-level biochemicals in extremely small samples that would otherwise be inaccessible. (C) 2015 Elsevier B.V. All rights reserved. C1 [Ognibene, T. J.; Thomas, At.; Daley, P. F.; Bench, G.] Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, Livermore, CA 94551 USA. [Turteltaub, K. W.] Lawrence Livermore Natl Lab, Biol & Biotechnol Div, Livermore, CA 94551 USA. RP Ognibene, TJ (reprint author), Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, 7000 East Ave, Livermore, CA 94551 USA. EM ognibene1@llnl.gov FU U.S. Department of Energy [DE-AC52-07NA27344]; National Institutes of Health (NIH), National Institute of General Medical Sciences (NIGMS), Biomedical Technology Research Resources (BTRR) [8P41GM103483] FX Work performed at the Research Resource for Biomedical AMS, which is operated at LLNL under the auspices of the U.S. Department of Energy under contract DE-AC52-07NA27344, is supported by the National Institutes of Health (NIH), National Institute of General Medical Sciences (NIGMS), Biomedical Technology Research Resources (BTRR) under Grant number 8P41GM103483. NR 13 TC 3 Z9 3 U1 1 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD OCT 15 PY 2015 VL 361 BP 173 EP 177 DI 10.1016/j.nimb.2015.05.018 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CU2HZ UT WOS:000363345900033 PM 26456991 ER PT J AU Liu, Y Batchelder, JC Galindo-Uribarri, A Chu, R Fan, S Romero-Romero, E Stracener, DW AF Liu, Y. Batchelder, J. C. Galindo-Uribarri, A. Chu, R. Fan, S. Romero-Romero, E. Stracener, D. W. TI Ion source development for ultratrace detection of uranium and thorium SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 13th International Conference on Accelerator Mass Spectrometry (AMS) CY AUG 24-29, 2014 CL Aix en Provence, FRANCE DE Ion source; Surface ionization; Laser ionization; Uranium; Thorium ID ENHANCED IONIZATION EFFICIENCY; ACCELERATOR MASS-SPECTROMETRY; CAVITY SOURCE; SEPARATORS; U-236; BEAMS; SAMPLES; HRIBF; TIMS AB Efficient ion sources are needed for detecting ultratrace U and Th impurities in a copper matrix by mass spectrometry techniques such as accelerator mass spectrometry (AMS). Two positive ion sources, a hot-cavity surface ionization source and a resonant ionization laser ion source, are evaluated in terms of ionization efficiencies for generating ion beams of U and Th. The performances of the ion sources are characterized using uranyl nitrate and thorium nitrate sample materials with sample sizes between 20 and 40 mu g of U or Th. For the surface ion source, the dominant ion beams observed are UO+ or ThO+ and ionization efficiencies of 2-4% have been obtained with W and Re cavities. With the laser ion source, three-step resonant photoionization of U atoms has been studied and only atomic U ions are observed. An ionization efficiency of about 9% has been demonstrated. The performances of both ion sources are expected to be further improved. (C) 2015 Elsevier B.V. All rights reserved. C1 [Liu, Y.; Batchelder, J. C.; Galindo-Uribarri, A.; Chu, R.; Fan, S.; Romero-Romero, E.; Stracener, D. W.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Batchelder, J. C.] Oak Ridge Associated Univ, Oak Ridge, TN 37831 USA. [Galindo-Uribarri, A.; Chu, R.; Fan, S.; Romero-Romero, E.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37966 USA. RP Liu, Y (reprint author), Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics; Laboratory Directed Research and Development Program at Oak Ridge National Laboratory FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics and by the Laboratory Directed Research and Development Program at Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy. NR 37 TC 3 Z9 3 U1 2 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD OCT 15 PY 2015 VL 361 BP 267 EP 272 DI 10.1016/j.nimb.2015.04.081 PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CU2HZ UT WOS:000363345900051 ER PT J AU McCartt, AD Ognibene, T Bench, G Turteltaub, K AF McCartt, A. D. Ognibene, T. Bench, G. Turteltaub, K. TI Measurements of carbon-14 with cavity ring-down spectroscopy SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 13th International Conference on Accelerator Mass Spectrometry (AMS) CY AUG 24-29, 2014 CL Aix en Provence, FRANCE DE CRDS; Spectroscopy; Carbon-14 ID INTRACAVITY OPTOGALVANIC SPECTROSCOPY AB Accelerator Mass Spectrometry CAMS) is the most sensitive method for quantitation of C-14 in biological samples. This technology has been used in a variety of low dose, human health related studies over the last 20 years when very high sensitivity was needed. AMS helped pioneer these scientific methods, but its expensive facilities and requirements for highly trained technical staff have limited their proliferation. Quantification of C-14 by cavity ring-down spectroscopy (CRDS) offers an approach that eliminates many of the shortcomings of an accelerator-based system and would supplement the use of AMS in biomedical research. Our initial prototype, using a non-ideal wavelength laser and under suboptimal experimental conditions, has a 3.5-modern, 1-sigma precision for detection of milligram-sized, carbon-14-elevated samples. These results demonstrate proof of principle and provided a starting point for the development of a spectrometer capable of biologically relevant sensitivities. Published by Elsevier B.V. C1 [McCartt, A. D.; Ognibene, T.; Bench, G.] Lawrence Livermore Natl Lab, CAMS, Lawrence, KS USA. [Turteltaub, K.] Lawrence Livermore Natl Lab, Biol & Biotechnol Div, Lawrence, KS USA. RP McCartt, AD (reprint author), Lawrence Livermore Natl Lab, CAMS, Lawrence, KS USA. EM mccartt1@llnl.gov FU NCRR NIH HHS [P41 RR013461]; NIGMS NIH HHS [R21 GM111242, P41 GM103483] NR 14 TC 5 Z9 5 U1 1 U2 14 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD OCT 15 PY 2015 VL 361 BP 277 EP 280 DI 10.1016/j.nimb.2015.05.036 PG 4 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CU2HZ UT WOS:000363345900053 PM 27065506 ER PT J AU Janzen, MS Galindo-Uribarri, A Liu, Y Mills, GD Romero-Romero, E Stracener, DW AF Janzen, Meghan S. Galindo-Uribarri, Alfredo Liu, Yuan Mills, Gerald D. Romero-Romero, Elisa Stracener, Daniel W. TI The use of aluminum nitride to improve Aluminum-26 Accelerator Mass Spectrometry measurements and production of Radioactive Ion Beams SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 13th International Conference on Accelerator Mass Spectrometry (AMS) CY AUG 24-29, 2014 CL Aix en Provence, FRANCE DE AMS; Al-26; Aluminum nitride; Negative ion source ID COSMOGENIC NUCLIDES; TERRESTRIAL; EMISSION; ABOARD; LIMITS; BE-10 AB We present results and discuss the use of aluminum nitride as a promising source material for Accelerator Mass Spectrometry CAMS) and Radioactive Ion Beams (RIBs) science applications of Al-26 isotopes. The measurement of Al-26 in geological samples by AMS is typically conducted on Al2O3 targets. However, Al2O3 is not an ideal source material because it does not form a prolific beam of Al- required for measuring low-levels of Al-26. Multiple samples of aluminum oxide (Al2O3), aluminum nitride (AlN), mixed Al2O3-AlN as well as aluminum fluoride (AlF3) were tested and compared using the ion source test facility and the stable ion beam (SIB) injector platform at the 25-MV tandem electrostatic accelerator at Oak Ridge National Laboratory. Negative ion currents of atomic and molecular aluminum were examined for each source material. It was found that pure AlN targets produced substantially higher beam currents than the other materials and that there was some dependence on the exposure of AlN to air. The applicability of using AlN as a source material for geological samples was explored by preparing quartz samples as Al2O3 and converting them to AlN using a carbothermal reduction technique, which involved reducing the Al2O3 with graphite powder at 1600 degrees C within a nitrogen atmosphere. The quartz material was successfully converted to MN. Thus far, AlN proves to be a promising source material and could lead towards increasing the sensitivity of low-level Al-26 AMS measurements. The potential of using AlN as a source material for nuclear physics is also very promising by placing (AlN)-Al-26 directly into a source to produce more intense radioactive beams of Al-26. (C) 2015 Published by Elsevier B.V. C1 [Janzen, Meghan S.; Galindo-Uribarri, Alfredo; Liu, Yuan; Mills, Gerald D.; Romero-Romero, Elisa; Stracener, Daniel W.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Janzen, Meghan S.; Galindo-Uribarri, Alfredo] Univ Tennessee, Dept Earth & Planetary Sci, Knoxville, TN 37996 USA. [Janzen, Meghan S.; Galindo-Uribarri, Alfredo; Romero-Romero, Elisa] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RP Galindo-Uribarri, A (reprint author), Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. FU Laboratory Directed Research and Development Program at Oak Ridge National Laboratory; U.S. Department of Energy, Office of Science, Office of Nuclear Physics FX Special thanks to Prof. Yingkui Li from University of Tennessee for providing the purified quartz samples for the preparation of AMS targets. This material is based upon work sponsored by the Laboratory Directed Research and Development Program at Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy and is supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics. This research used resources of the Holifield Radioactive Ion Beam Facility of Oak Ridge National Laboratory, which was a DOE Office of Science User Facility. NR 27 TC 0 Z9 0 U1 1 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD OCT 15 PY 2015 VL 361 BP 281 EP 287 DI 10.1016/j.nimb.2015.05.037 PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CU2HZ UT WOS:000363345900054 ER PT J AU Adamic, ML Lister, TE Dufek, EJ Jenson, DD Olson, JE Vockenhuber, C Watrous, MG AF Adamic, M. L. Lister, T. E. Dufek, E. J. Jenson, D. D. Olson, J. E. Vockenhuber, C. Watrous, M. G. TI Electrodeposition as an alternate method for preparation of environmental samples for iodide by AMS SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 13th International Conference on Accelerator Mass Spectrometry (AMS) CY AUG 24-29, 2014 CL Aix en Provence, FRANCE DE Radioiodine; Accelerator mass spectrometry, AMS; Electrodepoition; I-129-AMS sample preparation; I-129 ID ACCELERATOR MASS-SPECTROMETRY; I-129 AB This paper presents an evaluation of an alternate method for preparing environmental samples for I-129 analysis by accelerator mass spectrometry (AMS) at Idaho National Laboratory. The optimal sample preparation method is characterized by ease of preparation, capability of processing very small quantities of iodide, and ease of loading into a cathode. Electrodeposition of iodide on a silver wire was evaluated using these criteria. This study indicates that the electrochemically-formed silver iodide deposits produce ion currents similar to those from precipitated silver iodide for the same sample mass. Precipitated silver iodide samples are usually mixed with niobium or silver powder prior to loading in a cathode. Using electrodeposition, the silver is already mixed with the sample and can simply be picked up with tweezers, placed in the sample die, and pressed into a cathode. The major advantage of this method is that the silver wire/electrodeposited silver iodide is much easier to load into a cathode. (C) 2015 Elsevier B.V. All rights reserved. C1 [Adamic, M. L.; Lister, T. E.; Dufek, E. J.; Jenson, D. D.; Olson, J. E.; Watrous, M. G.] Idaho Natl Lab, Idaho Falls, ID 83402 USA. [Vockenhuber, C.] ETH, Lab Ion Beam Phys, CH-8093 Zurich, Switzerland. RP Adamic, ML (reprint author), Idaho Natl Lab, POB 1625, Idaho Falls, ID 83402 USA. EM Mary.Adamic@inl.gov RI Dufek, Eric/B-8847-2017 OI Dufek, Eric/0000-0003-4802-1997 FU DOE [IN13-AMS255-PD3TE] FX This work was supported by DOE IN13-AMS255-PD3TE. We thank Tammy Trowbridge for performing the scanning electron microscopy, Duane Ball for performing ICP-MS analysis, Gracy Elias and Byron White for performing the ion chromatography analysis. NR 7 TC 0 Z9 0 U1 0 U2 8 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD OCT 15 PY 2015 VL 361 BP 372 EP 375 DI 10.1016/j.nimb.2015.03.015 PG 4 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CU2HZ UT WOS:000363345900070 ER PT J AU Bauder, W Pardo, RC Kondev, FG Kondrashev, S Nair, C Nusair, O Palchan, T Scott, R Seweryniak, D Vondrasek, R Collon, P Paul, M AF Bauder, W. Pardo, R. C. Kondev, F. G. Kondrashev, S. Nair, C. Nusair, O. Palchan, T. Scott, R. Seweryniak, D. Vondrasek, R. Collon, P. Paul, M. TI Developing laser ablation in an electron cyclotron resonance ion source for actinide detection with AMS SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 13th International Conference on Accelerator Mass Spectrometry (AMS) CY AUG 24-29, 2014 CL Aix en Provence, FRANCE DE Accelerator mass spectrometry; Electron cyclotron resonance ion source; Actinides ID MASS-SPECTROMETRY AB A laser ablation material injection system has been developed at the ATLAS electron cyclotron resonance (ECR) ion source for use in accelerator mass spectrometry experiments. Beam production with laser ablation initially suffered from instabilities due to fluctuations in laser energy and cratering on the sample surface by the laser. However, these instabilities were rectified by applying feedback correction for the laser energy and rastering the laser across the sample surface. An initial experiment successfully produced and accelerated low intensity actinide beams with up to 1000 counts per second. With continued development, laser ablation shows promise as an alternative material injection scheme for ECR ion sources and may help substantially reduce cross talk in the source. (C) 2015 Elsevier B.V. All rights reserved. C1 [Bauder, W.; Pardo, R. C.; Kondev, F. G.; Kondrashev, S.; Nair, C.; Nusair, O.; Scott, R.; Seweryniak, D.; Vondrasek, R.] Argonne Natl Lab, Div Phys, Lemont, IL 60439 USA. [Bauder, W.; Collon, P.] Univ Notre Dame, Nucl Sci Lab, Notre Dame, IN 46556 USA. [Palchan, T.; Paul, M.] Hebrew Univ Jerusalem, Racah Inst Phys, IL-91904 Jerusalem, Israel. RP Bauder, W (reprint author), Univ Notre Dame, Nucl Sci Lab, 124 Nieuwland Sci Hall, Notre Dame, IN 46556 USA. FU U.S. Department of Energy Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357] FX This material is based upon work supported by the U.S. Department of Energy Office of Science, Office of Nuclear Physics, under contract number DE-AC02-06CH11357 and work authorization number KB/CH12/9/ARRA-3, FWP #22695. This research used resources of ANL's ATLAS facility, which is a DOE Office of Science User Facility. NR 16 TC 1 Z9 1 U1 2 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD OCT 15 PY 2015 VL 361 BP 465 EP 470 DI 10.1016/j.nimb.2015.04.080 PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CU2HZ UT WOS:000363345900087 ER PT J AU Ostdiek, K Anderson, T Bauder, W Bowers, M Collon, P Dressler, R Greene, J Kutschera, W Lu, W Paul, M Robertson, D Schumann, D Skulski, M Wallner, A AF Ostdiek, K. Anderson, T. Bauder, W. Bowers, M. Collon, P. Dressler, R. Greene, J. Kutschera, W. Lu, W. Paul, M. Robertson, D. Schumann, D. Skulski, M. Wallner, A. TI Towards a measurement of the half-life of Fe-60 for stellar and early Solar System models SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 13th International Conference on Accelerator Mass Spectrometry (AMS) CY AUG 24-29, 2014 CL Aix en Provence, FRANCE DE Accelerator Mass Spectrometry; Half-life; Fe-60; Gamma Ray Spectroscopy AB Radioisotopes, produced in stars and ejected into the Interstellar Medium, are important for constraining stellar and early Solar System (ESS) models. In particular, the half-life of the radioisotope, Fe-60, can have an impact on calculations for the timing for ESS events, the distance to nearby Supernovae, and the brightness of individual, non-steady-state Fe gamma ray sources in the Galaxy. A half-life measurement has been undertaken at the University of Notre Dame and measurements of the Fe-60/Fe-56 concentration of our samples using Accelerator Mass Spectrometry has begun. This result will be coupled with an activity measurement of the isomeric decay in Co-60, which is the decay product of Fe. Preliminary half-life estimates of (2.53 +/- 0.24) x 10(6) years seem to confirm the recent measurement by Rugel et al. (2009). (C) 2015 Elsevier B.V. All rights reserved. C1 [Ostdiek, K.; Anderson, T.; Bauder, W.; Bowers, M.; Collon, P.; Lu, W.; Robertson, D.; Skulski, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Bauder, W.; Greene, J.] Argonne Natl Lab, Lemont, IL 60439 USA. [Dressler, R.; Schumann, D.] Paul Scherrer Inst, Lab Radiochem & Environm Chem, CH-5232 Villigen, Switzerland. [Kutschera, W.] Vienna Environm Res Accelerator Lab, A-1090 Vienna, Austria. [Paul, M.] Hebrew Univ Jerusalem, Racah Inst Phys, IL-91904 Jerusalem, Israel. [Wallner, A.] Australian Natl Univ, Canberra, ACT 0200, Australia. RP Ostdiek, K (reprint author), Univ Notre Dame, Notre Dame, IN 46556 USA. RI Wallner, Anton/G-1480-2011 OI Wallner, Anton/0000-0003-2804-3670 FU National Science Foundation [PHY-1419765] FX We would like to thank the Physics Division of ANL for lending the HPGe detectors and the technical staff at Notre Dame for their expertise with accelerator systems and machining abilities. We would also like to thank the reviewer for their comments and suggestions to improve this paper. This work is supported by the National Science Foundation Grant # PHY-1419765. NR 14 TC 0 Z9 0 U1 3 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD OCT 15 PY 2015 VL 361 BP 638 EP 642 DI 10.1016/j.nimb.2015.05.033 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CU2HZ UT WOS:000363345900119 ER PT J AU Hooper-Bui, LM Kwok, ESC Buchholz, BA Rust, MK Eastmond, DA Vogel, JS AF Hooper-Bui, L. M. Kwok, E. S. C. Buchholz, B. A. Rust, M. K. Eastmond, D. A. Vogel, J. S. TI Insecticide transfer efficiency and lethal load in Argentine ants SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 13th International Conference on Accelerator Mass Spectrometry (AMS) CY AUG 24-29, 2014 CL Aix en Provence, FRANCE DE Argentine ant; Trophallaxis; Hydramethylnon; Fipronil; Accelerator mass spectrometry (AMS) ID IRIDOMYRMEX-HUMILIS MAYR; LABORATORY COLONIES; LINEPITHEMA-HUMILE; FIRE ANT; DELAYED TOXICITY; HYMENOPTERA; FORMICIDAE; BAIT; HYDRAMETHYLNON; DEGRADATION AB Trophallaxis between individual worker ants and the toxicant load in dead and live Argentine ants (Linepithema humile) in colonies exposed to fipronil and hydramethylnon experimental baits were examined using accelerator mass spectrometry (AMS). About 50% of the content of the crop containing trace levels of C-14-sucrose, C-14-hydramethylnon, and C-14-fipronil was shared between single donor and recipient ants. Dead workers and queens contained significantly more hydramethylnon (122.7 and 22.4 amol/mu g ant, respectively) than did live workers and queens (96.3 and 10.4 amol/mu g ant, respectively). Dead workers had significantly more fipronil (420.3 amol/mu g ant) than did live workers (208.5 amol/mu g ant), but dead and live queens had equal fipronil levels (59.5 and 54.3 amol/mu g ant, respectively). The distribution of fipronil differed within the bodies of dead and live queens; the highest amounts of fipronil were recovered in the thorax of dead queens whereas live queens had the highest levels in the head. Resurgence of polygynous ant colonies treated with hydramethylnon baits may be explained by queen survival resulting from sublethal doses due to a slowing of trophallaxis throughout the colony. Bait strategies and dose levels for controlling insect pests need to be based on the specific toxicant properties and trophic strategies for targeting the entire colony. (C) 2015 Elsevier B.V. All rights reserved. C1 [Hooper-Bui, L. M.] Louisiana State Univ, Dept Environm Sci, Baton Rouge, LA 70803 USA. [Hooper-Bui, L. M.; Rust, M. K.] Univ Calif Riverside, Dept Entomol, Riverside, CA 92521 USA. [Kwok, E. S. C.; Eastmond, D. A.] Univ Calif Riverside, Dept Cell Biol & Neurosci, Riverside, CA 92521 USA. [Buchholz, B. A.; Vogel, J. S.] Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, Livermore, CA 94551 USA. [Buchholz, B. A.] Univ Calif Davis, Dept Environm Toxicol, Davis, CA 95616 USA. RP Buchholz, BA (reprint author), Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, Livermore, CA 94551 USA. EM buchholz2@llnl.gov FU University of California Toxic Substances Research and Teaching Program; University of California Campus Laboratory Collaboration Program; Clorox Services Co.; NIH NIGMS [8P41GM103483]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We thank Elizabeth Bartko (University of California, Riverside) for assistance in rearing the ants. The technical and 14C-hydramethylnon were provided by The Clorox Services Co. The technical and 14C-fipronil was provided by Rhone Poulenc Ag Co. This research was supported in part by a grant from the University of California Toxic Substances Research and Teaching Program, the University of California Campus Laboratory Collaboration Program, The Clorox Services Co., and NIH NIGMS 8P41GM103483. This work was partially performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. Paper reviewed and released as LLNL-JRNL-664517. The funders had no part in the design, implementation or data analyses. NR 35 TC 0 Z9 0 U1 3 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD OCT 15 PY 2015 VL 361 BP 665 EP 669 DI 10.1016/j.nimb.2015.06.031 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CU2HZ UT WOS:000363345900124 PM 26504258 ER PT J AU Sekimoto, S Okumura, S Yashima, H Matsushi, Y Matsuzaki, H Matsumura, H Toyoda, A Oishi, K Matsuda, N Kasugai, Y Sakamoto, Y Nakashima, H Boehnlein, D Coleman, R Lauten, G Leveling, A Mokhov, N Ramberg, E Soha, A Vaziri, K Ninomiya, K Omoto, T Shima, T Takahashi, N Shinohara, A Caffee, MW Welten, KC Nishiizumi, K Shibata, S Ohtsuki, T AF Sekimoto, S. Okumura, S. Yashima, H. Matsushi, Y. Matsuzaki, H. Matsumura, H. Toyoda, A. Oishi, K. Matsuda, N. Kasugai, Y. Sakamoto, Y. Nakashima, H. Boehnlein, D. Coleman, R. Lauten, G. Leveling, A. Mokhov, N. Ramberg, E. Soha, A. Vaziri, K. Ninomiya, K. Omoto, T. Shima, T. Takahashi, N. Shinohara, A. Caffee, M. W. Welten, K. C. Nishiizumi, K. Shibata, S. Ohtsuki, T. TI Measurements of production cross sections of Be-10 and Al-26 by 120 GeV and 392 MeV proton bombardment of Y-89, Tb-159, and Cu-nat targets SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article DE Be-10; Al-26; Fragmentation process; Binding energy; 120 GeV proton ID HIGH-ENERGY PROTONS; NUCLIDE PRODUCTION; AMS STANDARDS; ELEMENTS; SPALLATION; RANGE; FE; SI AB The production cross sections of Be-10 and Al-26 were measured by accelerator mass spectrometry using Y-89, Tb-159, and Cu-nat targets bombarded by protons with energies E-p of 120 GeV and 392 MeV. The production cross sections obtained for Be-10 and Al-26 were compared with those previously reported using E-p = 50 MeV-24 GeV and various targets. It was found that the production cross sections of Be-10 monotonically increased with increasing target mass number when the proton energy was greater than a few GeV. On the other hand, it was also found that the production cross sections of Be-10 decreased as the target mass number increased from that of carbon to those near the mass numbers of nickel and zinc when the proton energy was below approximately 1 GeV. They also increased as the target mass number increased from near those of nickel and zinc to that of bismuth, in the same proton energy range. Similar results were observed in the production cross sections of Al-26, though the absolute values were quite different between Be-10 and Al-26. The difference between these production cross sections may depend on the impact parameter (nuclear radius) and/or the target nucleus stiffness. (C) 2015 Elsevier B.V. All rights reserved. C1 [Sekimoto, S.; Okumura, S.; Yashima, H.; Ohtsuki, T.] Kyoto Univ, Inst Res Reactor, Kumatori, Osaka 5900494, Japan. [Matsushi, Y.] Kyoto Univ, Disaster Prevent Res Inst, Uji, Kyoto 6110011, Japan. [Matsuzaki, H.] Univ Tokyo, Sch Engn, Dept Nucl Engn & Management, Bunkyo Ku, Tokyo 1130032, Japan. [Matsumura, H.; Toyoda, A.] High Energy Accelerator Res Org, Tsukuba, Ibaraki 3050801, Japan. [Oishi, K.] Shimizu Corp, Tokyo 1358530, Japan. [Matsuda, N.; Kasugai, Y.; Nakashima, H.] Japan Atom Energy Agcy, Tokai, Ibaraki 3191195, Japan. [Sakamoto, Y.] ATOX Co Ltd, Kashiwa, Chiba 2770861, Japan. [Boehnlein, D.; Coleman, R.; Lauten, G.; Leveling, A.; Mokhov, N.; Ramberg, E.; Soha, A.; Vaziri, K.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Ninomiya, K.; Omoto, T.; Takahashi, N.; Shinohara, A.] Osaka Univ, Grad Sch Sci, Toyonaka, Osaka 5600043, Japan. [Shima, T.] Osaka Univ, Nucl Phys Res Ctr, Suita, Osaka 5670047, Japan. [Caffee, M. W.] Purdue Univ, Dept Phys & Astron, W Lafayette, IN 47907 USA. [Caffee, M. W.] Purdue Univ, Dept Earth Atmospher & Planetary Sci, W Lafayette, IN 47907 USA. [Welten, K. C.; Nishiizumi, K.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Shibata, S.] RIKEN Nishina Ctr Accelerator Based Sci, Wako, Saitama 3510198, Japan. RP Sekimoto, S (reprint author), Kyoto Univ, Inst Res Reactor, Kumatori, Osaka 5900494, Japan. FU Ministry of Education, Science and Culture in Japan [KAKENHI 19360432, 21360473, 23656589, 25790081]; Kyoto University Global COE Program "International Center for integrated Research and Advanced Education in Materials Science"; Kansai Research Foundation for technology promotion; National Science Foundation (NSF); National Aeronautics and Space Administration (NASA); US Department of Energy Laboratory [E-AC02-07CH11359] FX The authors express their gratitude to the RCNP for their generous supports in this experiment (RCNP-E298). This work was supported by a grant-in-aid from the Ministry of Education, Science and Culture (KAKENHI 19360432, 21360473, 23656589, 25790081) in Japan, embryonic research project support in Kyoto University Global COE Program "International Center for integrated Research and Advanced Education in Materials Science", Kansai Research Foundation for technology promotion for SS, National Science Foundation (NSF) and National Aeronautics and Space Administration (NASA) for K.N. and M.W.C. Fermilab is a US Department of Energy Laboratory operated under Contract E-AC02-07CH11359 by the Fermi Research Alliance, LLC. NR 22 TC 1 Z9 1 U1 1 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD OCT 15 PY 2015 VL 361 BP 685 EP 688 DI 10.1016/j.nimb.2015.08.001 PG 4 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CU2HZ UT WOS:000363345900127 ER PT J AU Jiang, Y Huang, XG Liao, JF AF Jiang, Yin Huang, Xu-Guang Liao, Jinfeng TI Chiral vortical wave and induced flavor charge transport in a rotating quark-gluon plasma SO PHYSICAL REVIEW D LA English DT Article ID HEAVY-ION COLLISIONS; AZIMUTHAL CORRELATIONS; PLUS AU; VIOLATION; EVENT; QCD AB We show the existence of a new gapless collective excitation in a rotating fluid system with chiral fermions, named the chiral vortical wave (CVW). The CVW has its microscopic origin at the quantum anomaly and macroscopically arises from interplay between vector and axial charge fluctuations induced by vortical effects. The wave equation is obtained both from hydrodynamic current equations and from chiral kinetic theory, and its solutions show nontrivial CVW-induced charge transport from different initial conditions. Using the rotating quark-gluon plasma in heavy ion collisions as a concrete example, we show the formation of an induced flavor quadrupole in quark-gluon plasma and estimate the elliptic flow splitting effect for. baryons that may be experimentally measured. C1 [Jiang, Yin; Liao, Jinfeng] Indiana Univ, Dept Phys, Bloomington, IN 47408 USA. [Jiang, Yin; Liao, Jinfeng] Indiana Univ, Ctr Explorat Energy & Matter, Bloomington, IN 47408 USA. [Huang, Xu-Guang] Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China. [Huang, Xu-Guang] Fudan Univ, Ctr Particle Phys & Field Theory, Shanghai 200433, Peoples R China. [Liao, Jinfeng] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. RP Jiang, Y (reprint author), Indiana Univ, Dept Phys, 2401 North Milo B Sampson Lane, Bloomington, IN 47408 USA. EM jiangyin@indiana.edu; huangxuguang@fudan.edu.cn; liaoji@indiana.edu RI Huang, Xu-Guang/J-4988-2014 OI Huang, Xu-Guang/0000-0001-6293-4843 FU National Science Foundation [PHY-1352368]; Fudan University [EZH1512519]; Shanghai Natural Science Foundation [14ZR1403000]; RIKEN BNL Research Center FX We thank Shu Lin and Yi Yin for discussions. J. L. is grateful to Aihong Tang and Zhangbu Xu for very helpful discussions on experimental measurements. The research of Y. J. and J. L. is supported by the National Science Foundation (Grant No. PHY-1352368). The research of X.-G. H. is supported by Fudan University (Grant No. EZH1512519) and the Shanghai Natural Science Foundation (Grant No. 14ZR1403000). J. L. also thanks the RIKEN BNL Research Center for partial support. NR 65 TC 13 Z9 13 U1 1 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 15 PY 2015 VL 92 IS 7 AR 071501 DI 10.1103/PhysRevD.92.071501 PG 6 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CT6DI UT WOS:000362901500001 ER PT J AU Mathew, KJ Canaan, RD Hexel, C Giaquinto, J Krichinsky, AM AF Mathew, K. J. Canaan, R. D. Hexel, C. Giaquinto, J. Krichinsky, A. M. TI Qualification and initial characterization of a high-purity U-233 spike for use in uranium analyses SO INTERNATIONAL JOURNAL OF MASS SPECTROMETRY LA English DT Article DE Thermal ionization mass spectrometry; Certified reference materials; Nuclear forensics; Isotope dilution mass spectrometry ID ISOTOPE RATIO MEASUREMENTS; IONIZATION MASS-SPECTROMETRY; UNCERTAINTY; SAMPLES; TIMS AB Several high-purity U-233 items potentially useful as isotope dilution mass spectrometry standards for safeguards, non-proliferation, and nuclear forensics measurements are identified and rescued from downblending. By preserving the supply of U-233 materials of different pedigree for use as source materials for certified reference materials (CRMs), it is ensured that the safeguards community has high quality uranium isotopic standards required for calibration of the analytical instruments. One of the items identified as a source material for a high-purity CRM is characterized for the uranium isotope-amount ratios using thermal ionization mass spectrometry (TIMS). Additional verification measurements on this material using quadrupole inductively coupled plasma mass spectrometry (ICPMS) are also performed. The comparison of the ICPMS uranium isotope-amount ratios with the TIMS data, with much smaller uncertainties, validated the ICPMS measurement practices. ICPMS is proposed for the initial screening of the purity of items in the rescue campaign. Published by Elsevier B.V. C1 [Mathew, K. J.] US DOE, New Brunswick Lab, Argonne, IL 60439 USA. [Canaan, R. D.; Hexel, C.; Giaquinto, J.; Krichinsky, A. M.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Mathew, KJ (reprint author), Savannah River Natl Lab, Area Analyt Labs F H, Bldg 707-F Room 42, Aiken, SC 29808 USA. EM kattathu.mathew@srs.gov RI Hexel, Cole/N-3245-2016 OI Hexel, Cole/0000-0001-8101-2422 NR 17 TC 2 Z9 2 U1 3 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1387-3806 EI 1873-2798 J9 INT J MASS SPECTROM JI Int. J. Mass Spectrom. PD OCT 15 PY 2015 VL 389 BP 47 EP 53 DI 10.1016/j.ijms.2015.08.013 PG 7 WC Physics, Atomic, Molecular & Chemical; Spectroscopy SC Physics; Spectroscopy GA CT6JE UT WOS:000362918500006 ER PT J AU Esbenshade, JL Barile, CJ Fister, TT Bassett, KL Fenter, P Nuzzo, RG Gewirth, AA AF Esbenshade, Jennifer L. Barile, Christopher J. Fister, Timothy T. Bassett, Kimberly L. Fenter, Paul Nuzzo, Ralph G. Gewirth, Andrew A. TI Improving Electrodeposition of Mg through an Open Circuit Potential Hold SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID RECHARGEABLE MAGNESIUM BATTERIES; ELECTROLYTE-SOLUTIONS; SECONDARY BATTERIES; DEPOSITION; DISSOLUTION; CHLORIDE; ELECTROCHEMISTRY; CHALLENGE; SPECTROSCOPY; TECHNOLOGY AB We used in situ X-ray diffraction, XPS, SEM, and electrochemical methods to interrogate the mechanism of Mg electrodeposition from PhMgCl/AlCl3 (APC) and EtMgCl electrolytes. An open circuit potential (OCP) pause following Mg deposition led to retained enhancement of Mg deposition and stripping kinetics along with lowered overpotentials for both. In situ X-ray diffraction demonstrated that the OCP pause led to a more polycrystalline deposit relative to that without the pause, while SEM presented micrographs that showed smaller deposits with an OCP hold. The improvement is attributed to an "enhancement layer" that formed on the electrode during the OCP hold. Analysis of XPS data suggests that the "enhancement layer" consists of Mg and Cl retained on the electrode surface, possibly following electrode depassivation. C1 [Esbenshade, Jennifer L.; Barile, Christopher J.; Bassett, Kimberly L.; Nuzzo, Ralph G.; Gewirth, Andrew A.] Univ Illinois, Dept Chem, Urbana, IL 61801 USA. [Fister, Timothy T.; Fenter, Paul] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Gewirth, AA (reprint author), Univ Illinois, Dept Chem, 505 South Mathews Ave, Urbana, IL 61801 USA. EM agewirth@illinois.edu FU Joint Center for Energy Storage Research, an Energy Innovation Hub - U.S. Department of Energy, Office of Science, Basic Energy Sciences; National Science Foundation [DGE-1144245]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported as part of the Joint Center for Energy Storage Research, an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. J.L.E. acknowledges a National Science Foundation Graduate Research Fellowship under Grant DGE-1144245. C.J.B. acknowledges a Springborn Fellowship. This work was carried out in part in the Frederick Seitz Materials Research Laboratory Central Facilities, University of Illinois. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. NR 38 TC 4 Z9 4 U1 8 U2 47 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 15 PY 2015 VL 119 IS 41 BP 23366 EP 23372 DI 10.1021/acs.jpcc.5b07825 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CT8LP UT WOS:000363068400009 ER PT J AU Fang, ZT Wang, Y Dixon, DA AF Fang, Zongtang Wang, Yong Dixon, David A. TI Computational Study of Ethanol Conversion on Al8O12 as a Model for gamma-Al2O3 SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID GAMMA-ALUMINA; BASIS-SETS; SYNCHRONOUS-TRANSIT; DEFECT SITES; (MO3)(3) M; AB-INITIO; DEHYDRATION; SURFACE; MECHANISM; DENSITY AB Correlated molecular orbital theory at the coupled cluster CCSD(T) level with density functional theory geometries is used to study ethanol dehydration, dehydrogenation, and condensation reactions on an the Al8O12 cluster which is a model for gamma-Al2O3. The Al in the active site on the cluster is a strong Lewis acid. The reactions begin with formation of a very stable Lewis acid-base ethanol-cluster adduct. Dehydration proceeds by beta-H transfer to a bicoordinate oxygen leading to the direct formation of ethylene and two OH groups following an E2 mechanism. Dehydrogenation proceeds directly by alpha-H transfer to the active metal center and a proton transfer to a bicoordinate bridge O to form acetaldehyde plus a metal hydride and a hydroxyl, again an E2 mechanism. After addition of a second ethanol, diethyl ether is generated by an alpha-C transfer from the first to the second ethanol, an acid-driven S(N)2 mechanism. Condensation and dehydration with two alcohols have comparable energy barriers. The addition of a second ethanol or a water molecule raises the energy barriers. Condensation and dehydration are predicted to be more likely than dehydrogenation. The computational results for the mechanism and the energetics agree well with the available experimental data. C1 [Fang, Zongtang; Dixon, David A.] Univ Alabama, Dept Chem, Tuscaloosa, AL 35487 USA. [Wang, Yong] Washington State Univ, Gene & Linda Voiland Sch Chem Engn, Pullman, WA 99164 USA. [Wang, Yong] Washington State Univ, Bioengn Sch, Pullman, WA 99164 USA. [Wang, Yong] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. RP Dixon, DA (reprint author), Univ Alabama, Dept Chem, Shelby Hall,Box 870336, Tuscaloosa, AL 35487 USA. EM dadixon@ua.edu FU Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, U.S. Department of Energy (DOE); Robert Ramsay Chair Fund of The University of Alabama; DOE's Office of Biological and Environmental Research FX This work was supported by the Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, U.S. Department of Energy (DOE) (catalysis center program). D.A.D. also thanks the Robert Ramsay Chair Fund of The University of Alabama for support. Part of this work was performed at the W. R. Wiley Environmental Molecular Sciences Laboratory including the Molecular Sciences Computing Facility, a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory, operated for the DOE by Battelle. PNNL is a multiprogram national laboratory. NR 44 TC 4 Z9 4 U1 8 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 15 PY 2015 VL 119 IS 41 BP 23413 EP 23421 DI 10.1021/acs.jpcc.5b05887 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CT8LP UT WOS:000363068400015 ER PT J AU Yin, XS Cooper, VR Weitering, HH Snijders, PC AF Yin, Xiangshi Cooper, Valentino R. Weitering, Hanno H. Snijders, Paul C. TI Surface Chemical Reactivity of Ultrathin Pd(111) Films on Ru(0001): Importance of Orbital Symmetry in the Application of the d-Band Model SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID TRANSITION-METAL SURFACES; CO CHEMISORPTION; HETEROGENEOUS CATALYSIS; OXYGEN; ADSORPTION; GOLD; STM; PD; DEPENDENCE; STABILITY AB The chemical bonding of adsorbate molecules on transition-metal surfaces is strongly influenced by the hybridization between the molecular orbitals and the metal d-band. The strength of this interaction is often correlated with the location of the metal d-band center relative to the Fermi level. Here, we exploit finite size effects in the electronic structure of ultrathin Pd(111) films grown on Ru(0001) to tune their reactivity by changing the film thickness one atom layer at a time, while keeping all other variables unchanged. Interestingly, while bulk Pd(111) is reactive toward oxygen, Pd(111) films below five monolayers are surprisingly inert. This observation is fully in line with the d-band model prediction when applied to the orbitals involved in the bonding. The shift of the d-band center with film thickness is primarily attributed to shifts in the partial density of states associated with the 4d(xx) 4d(yz) orbitals. This study gives an in-depth look into the orbital specific contributions to the surface chemical reactivity, providing new insights that could be useful in surface catalysis. C1 [Yin, Xiangshi; Weitering, Hanno H.; Snijders, Paul C.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Yin, Xiangshi; Cooper, Valentino R.; Weitering, Hanno H.; Snijders, Paul C.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Weitering, HH (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. EM hanno@utk.edu; snijderspc@ornl.gov RI Cooper, Valentino /A-2070-2012 OI Cooper, Valentino /0000-0001-6714-4410 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; DOE Office of Science [DE-AC02-05CH11231] FX This research was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the DOE Office of Science under Contract No. DE-AC02-05CH11231. NR 39 TC 1 Z9 1 U1 1 U2 7 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 15 PY 2015 VL 119 IS 41 BP 23495 EP 23502 DI 10.1021/acs.jpcc.5606653 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CT8LP UT WOS:000363068400025 ER PT J AU Mu, RT Cantu, DC Glezakou, VA Lyubinetsky, I Rousseau, R Dohnalek, Z AF Mu, Rentao Cantu, David C. Glezakou, Vassiliki-Alexandra Lyubinetsky, Igor Rousseau, Roger Dohnalek, Zdenek TI Deprotonated Water Dimers: The Building Blocks of Segmented Water Chains on Rutile RuO2(110) SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ATOMIC-SCALE INSIGHTS; HETEROGENEOUS CATALYSIS; FUNDAMENTAL-ASPECTS; INITIAL OXIDATION; RUTHENIUM DIOXIDE; ROOM-TEMPERATURE; SOLID-SURFACES; PSEUDOPOTENTIALS; TIO2(110); SPECTRA AB Despite the importance of RuO2 in photocatalytic water splitting and catalysis in general, the interactions of water with even its most stable (110) surface are not well understood. In this study we employ a combination of high-resolution scanning tunneling microscopy imaging with density functional theory based ab initio molecular dynamics, and we follow the formation and binding of linear water clusters on coordinatively unsaturated ruthenium rows. We find that clusters of all sizes (dimers, trirners, tetramers, extended chains) are stabilized by donating one proton per every two water molecules to the surface bridge bonded oxygen sites, in contrast with water monomers that do not show a significant propensity for dissociation. The clusters with odd number of water molecules are less stable than the clusters with even number and are generally not observed under thermal equilibrium. For all clusters with even numbers, the dissociated dimers represent the fundamental building blocks with strong intradimer hydrogen bonds and only very weak interdimer interactions resulting in segmented water chains. C1 [Mu, Rentao; Cantu, David C.; Glezakou, Vassiliki-Alexandra; Rousseau, Roger; Dohnalek, Zdenek] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. [Lyubinetsky, Igor] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Mu, Rentao; Cantu, David C.; Glezakou, Vassiliki-Alexandra; Lyubinetsky, Igor; Rousseau, Roger; Dohnalek, Zdenek] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. RP Rousseau, R (reprint author), Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, POB 999, Richland, WA 99352 USA. EM roger.rousseau@pnnl.gov; zdenek.dohnalek@pnnl.gov RI Rousseau, Roger/C-3703-2014 FU US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences and performed in EMSL; Department of Energy's Office of Biological and Environmental Research; Pacific Northwest National Laboratory (PNNL) FX This work was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences and performed in EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). PNNL is a multiprogram national laboratory operated for DOE by Battelle. The authors also acknowledge Mal-Soon Lee for discussions of the AIMD trajectory analysis and Cortland Johnson for the artistic rendering of the cover image. NR 32 TC 5 Z9 5 U1 4 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 15 PY 2015 VL 119 IS 41 BP 23552 EP 23558 DI 10.1021/acs.jpcc.5b07158 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CT8LP UT WOS:000363068400030 ER PT J AU Wang, FL More, R AF Wang, Feilu More, Richard TI Visible Light Generated By Short X-ray Pulses SO JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN LA English DT Article ID FREE-ELECTRON LASER AB We predict emission of visible or infrared light by ultrashort X-ray pulses moving through a transparent dielectric medium having a visible light index of refraction n(omega(L)) > 1. The emission occurs if the X-ray pulse is collinear and well-focused. We give reasons to expect that this new type of radiation can be observed on X-ray free-electron laser facilities already beginning operation. The emission is coherent and the intensity is proportional to the square of the number of X-ray photons. The emission spectrum is very sensitive to the X-ray pulse length and that sensitivity may offer a useful new method to measure the X-ray pulse length. C1 [Wang, Feilu] Chinese Acad Sci, Key Lab Opt Astron, Natl Astron Observ, Beijing 100012, Peoples R China. [Wang, Feilu; More, Richard] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Wang, FL (reprint author), Chinese Acad Sci, Key Lab Opt Astron, Natl Astron Observ, Beijing 100012, Peoples R China. RI Wang, Feilu/A-9978-2013 FU LLNL-LDRD subcontract [B604796]; NSFC [11173032, 11573040, 11135012]; National Basic Research Program of China (973 Program) [2013 CBA 01503] FX This work was supported in part by LLNL-LDRD subcontract B604796. This work is also partially supported by the NSFC under Grant Nos. 11173032, 11573040, and 11135012, and by the National Basic Research Program of China (973 Program) (Grant No. 2013 CBA 01503). NR 19 TC 0 Z9 0 U1 1 U2 6 PU PHYSICAL SOC JAPAN PI TOKYO PA YUSHIMA URBAN BUILDING 5F, 2-31-22 YUSHIMA, BUNKYO-KU, TOKYO, 113-0034, JAPAN SN 0031-9015 J9 J PHYS SOC JPN JI J. Phys. Soc. Jpn. PD OCT 15 PY 2015 VL 84 IS 10 AR 103301 DI 10.7566/JPSJ.84.103301 PG 4 WC Physics, Multidisciplinary SC Physics GA CT7VU UT WOS:000363023400002 ER PT J AU Drichko, N Hackl, R Schlueter, JA AF Drichko, Natalia Hackl, Rudi Schlueter, John A. TI Antiferromagnetic fluctuations in a quasi-two-dimensional organic superconductor detected by Raman spectroscopy SO PHYSICAL REVIEW B LA English DT Article ID BEDT-TTF; SPIN-LIQUID; NMR; SCATTERING; INSULATOR; SALTS; LIGHT AB Using Raman scattering, the quasi-two-dimensional organic superconductor kappa-(BEDT-TTF)(2)Cu[N(CN)(2)]Br (T-c = 11.8 K) and the related antiferromagnet kappa-(BEDT-TTF)(2)Cu[N(CN)(2)]Cl are studied. Raman scattering provides unique spectroscopic information about magnetic degrees of freedom that has been otherwise unavailable on such organic conductors. Below T = 200 K a broad band at about 500 cm(-1) develops in both compounds. We identify this band with two-magnon excitation. The position and the temperature dependence of the spectral weight are similar in the antiferromagnet and in the metallic Fermi liquid. We conclude that antiferromagnetic correlations are similarly present in the magnetic insulator and the Fermi-liquid state of the superconductor. C1 [Drichko, Natalia] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Hackl, Rudi] Bayer Akademie Wissensch, Walther Meissner Inst, D-85748 Garching, Germany. [Schlueter, John A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Schlueter, John A.] Natl Sci Fdn, Arlington, VA 22230 USA. RP Drichko, N (reprint author), Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. EM drichko@jhu.edu FU Margarete von Wrangell-Habilitationsprogramm; M. Hildred Blewett Fellowship; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Material Sciences and Engineering [DE-FG02-08ER46544]; DFG via the Transregional Collaborative Research Center [TRR 80]; Bavarian Californian Technology Center BaCaTeC [A5 [2012-2]] FX The authors thank R. Valenti, B. Powell, and N. P. Armitage for fruitful discussions. N.D. gratefully acknowledges support via the Margarete von Wrangell-Habilitationsprogramm and an M. Hildred Blewett Fellowship and thanks the Walther-Meissner-Institut and 1. Physikalisches Institut, University of Stuttgart for their hospitality. The work in JHU was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Material Sciences and Engineering under Grant No. DE-FG02-08ER46544. R.H. gratefully acknowledges support by the DFG via the Transregional Collaborative Research Center TRR 80 and the Bavarian Californian Technology Center BaCaTeC (Project No. A5 [2012-2]). NR 39 TC 1 Z9 1 U1 1 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 15 PY 2015 VL 92 IS 16 AR 161112 DI 10.1103/PhysRevB.92.161112 PG 5 WC Physics, Condensed Matter SC Physics GA CT6BO UT WOS:000362895900002 ER PT J AU James, AJA Konik, RM AF James, A. J. A. Konik, R. M. TI Quantum quenches in two spatial dimensions using chain array matrix product states SO PHYSICAL REVIEW B LA English DT Article ID RENORMALIZATION-GROUP; MAGNETIC-FIELD; ISING-MODEL AB We describe a method for simulating the real time evolution of extended quantum systems in two dimensions (2D). The method combines the benefits of integrability and matrix product states in one dimension to avoid several issues that hinder other applications of tensor based methods in 2D. In particular, it can be extended to infinitely long cylinders. As an example application we present results for quantum quenches in the 2D quantum [(2 + 1)-dimensional] Ising model. In quenches that cross a phase boundary we find that the return probability shows nonanalyticities in time. C1 [James, A. J. A.] UCL, London Ctr Nanotechnol, London WC1H 0AH, England. [Konik, R. M.] Brookhaven Natl Lab, CMPMS Dept, Upton, NY 11973 USA. RP James, AJA (reprint author), UCL, London Ctr Nanotechnol, Gordon St, London WC1H 0AH, England. EM andrew.james@ucl.ac.uk RI Konik, Robert/L-8076-2016; OI Konik, Robert/0000-0003-1209-6890; James, Andrew/0000-0001-8454-6219; James, Andrew/0000-0003-3069-4579 FU Engineering and Physical Sciences Research Council [EP/L010623/1]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX We wish to acknowledge enlightening discussions with John Cardy, Fabian Essler, Andrew Goldsborough, Israel Klich, Anatoli Polkonikov, Rudolf Romer, and Steve Simons. This work was supported by the Engineering and Physical Sciences Research Council (Grant No. EP/L010623/1) and the U.S. Department of Energy, Office of Basic Energy Sciences under Contract No. DE-AC02-98CH10886. NR 47 TC 9 Z9 9 U1 0 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 15 PY 2015 VL 92 IS 16 AR 161111 DI 10.1103/PhysRevB.92.161111 PG 5 WC Physics, Condensed Matter SC Physics GA CT6BO UT WOS:000362895900001 ER PT J AU Courtoy, A Baessler, S Gonzalez-Alonso, M Liuti, S AF Courtoy, Aurore Baessler, Stefan Gonzalez-Alonso, Martin Liuti, Simonetta TI Beyond-Standard-Model Tensor Interaction and Hadron Phenomenology SO PHYSICAL REVIEW LETTERS LA English DT Article ID PARTON DISTRIBUTIONS; TRANSVERSITY AB We evaluate the impact of recent developments in hadron phenomenology on extracting possible fundamental tensor interactions beyond the standard model. We show that a novel class of observables, including the chiral-odd generalized parton distributions, and the transversity parton distribution function can contribute to the constraints on this quantity. Experimental extractions of the tensor hadronic matrix elements, if sufficiently precise, will provide a, so far, absent testing ground for lattice QCD calculations. C1 [Courtoy, Aurore] Univ Liege, AGO Dept, IFPA, B-4000 Liege, Belgium. [Courtoy, Aurore] Univ Guanajuato, Div Ciencias & Ingn, Leon 37150, Mexico. [Baessler, Stefan; Liuti, Simonetta] Univ Virginia, Dept Phys, Charlottesville, VA 22904 USA. [Baessler, Stefan] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Gonzalez-Alonso, Martin] Univ Lyon 1, CNRS, IN2P3, IPNL, F-69622 Villeurbanne, France. [Liuti, Simonetta] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Rome, Italy. RP Courtoy, A (reprint author), Univ Liege, AGO Dept, IFPA, Bat B5, B-4000 Liege, Belgium. EM aurore.courtoy@ulg.ac.be; baessler@virginia.edu; mgonzalez@ipnl.in2p3.fr; sl4y@virginia.edu RI Gonzalez-Alonso, Martin/O-1480-2016 OI Gonzalez-Alonso, Martin/0000-0003-0319-8828 FU Belgian Fund F. R. S.-FNRS via the contract of Charge de recherches; DOE [DE-FG02-01ER4120]; NSF [PHY-1205833]; LABEX Lyon Institute of Origins of the Universite de Lyon within the project "Investissements d'Avenir" of the French government [ANR-10-LABX-0066, ANR-11-IDEX-0007] FX We are grateful to H. Avakian, A. Kim, S. Pisano, and J. Zhang for details on the experimental extractions at Jefferson Lab, and to L. Barron Palos, M. Engelhardt, P. Q. Hung, E. Peinado, and D. Pocanic for fruitful discussions. This work was funded by the Belgian Fund F. R. S.-FNRS via the contract of Charge de recherches (A. C.), by DOE Grant No. DE-FG02-01ER4120 (S. L.) and by NSF PHY-1205833 (S. B.). M. G.-A. is grateful to the LABEX Lyon Institute of Origins (ANR-10-LABX-0066) of the Universite de Lyon for its financial support within the project "Investissements d'Avenir" (ANR-11-IDEX-0007) of the French government operated by the National Research Agency (ANR). NR 50 TC 7 Z9 7 U1 1 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 15 PY 2015 VL 115 IS 16 AR 162001 DI 10.1103/PhysRevLett.115.162001 PG 5 WC Physics, Multidisciplinary SC Physics GA CT6FQ UT WOS:000362908700007 PM 26550868 ER PT J AU Knapen, S Robinson, DJ AF Knapen, Simon Robinson, Dean J. TI Disentangling Mass and Mixing Hierarchies SO PHYSICAL REVIEW LETTERS LA English DT Article ID UNIFICATION AB We present a fully perturbative mechanism that naturally generates mass hierarchies for the standard model (SM) fermions in a flavor-blind sector. The dynamics generating the mass hierarchies can therefore be independent from the source of flavor violation, and hence this dynamics may operate at a much lower scale. This mechanism works by dynamically enforcing simultaneous diagonalization-alignment-among a set of flavor-breaking spurions, as well as generating highly singular spectra for them. It also has general applications in model building beyond the SM, wherever alignment between exotic and SM sources of flavor violation is desired. C1 [Knapen, Simon] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. Univ Calif Berkeley, Ernest Orlando Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Knapen, S (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. FU LDRD Program of LBNL under U.S. Department of Energy [DE-AC02-05CH11231]; NSF [PHY-1002399] FX We thank Bob Cahn, Yuval Grossman, Lawrence Hall, Zoltan Ligeti, Aneesh Manohar, Yasunori Nomura, Duccio Pappadopulo, and Michele Papucci for helpful conversations. The work of S. K. was supported by the LDRD Program of LBNL under U.S. Department of Energy Contract No. DE-AC02-05CH11231. D. R. is supported by the NSF under Grant No. PHY-1002399. NR 12 TC 4 Z9 4 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 15 PY 2015 VL 115 IS 16 AR 161803 DI 10.1103/PhysRevLett.115.161803 PG 5 WC Physics, Multidisciplinary SC Physics GA CT6FQ UT WOS:000362908700006 PM 26550867 ER PT J AU Scheinker, A Gessner, S AF Scheinker, Alexander Gessner, Spencer TI Adaptive method for electron bunch profile prediction SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article ID ALGORITHM; OPTIMIZATION; SEEKING AB We report on an experiment performed at the Facility for Advanced Accelerator Experimental Tests (FACET) at SLAC National Accelerator Laboratory, in which a new adaptive control algorithm, one with known, bounded update rates, despite operating on analytically unknown cost functions, was utilized in order to provide quasi-real-time bunch property estimates of the electron beam. Multiple parameters, such as arbitrary rf phase settings and other time-varying accelerator properties, were simultaneously tuned in order to match a simulated bunch energy spectrum with a measured energy spectrum. The simple adaptive scheme was digitally implemented using Matlab and the experimental physics and industrial control system. The main result is a nonintrusive, nondestructive, real-time diagnostic scheme for prediction of bunch profiles, as well as other beam parameters, the precise control of which are important for the plasma wakefield acceleration experiments being explored at FACET. C1 [Scheinker, Alexander] Los Alamos Natl Lab, Los Alamos, NM 87544 USA. [Gessner, Spencer] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. RP Scheinker, A (reprint author), Los Alamos Natl Lab, 1200 Trinity Dr, Los Alamos, NM 87544 USA. EM ascheink@lanl.gov; sgess@slac.stanford.edu FU Los Alamos National Laboratory; SLAC National Laboratory; U.S. Department of Energy [DE-AC02-76SF00515] FX This research was supported by Los Alamos National Laboratory, SLAC National Laboratory, and by the U.S. Department of Energy under Contract No. DE-AC02-76SF00515. NR 24 TC 1 Z9 1 U1 1 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD OCT 15 PY 2015 VL 18 IS 10 AR 102801 DI 10.1103/PhysRevSTAB.18.102801 PG 10 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA CT6HG UT WOS:000362913500001 ER PT J AU Mannige, RV Haxton, TK Proulx, C Robertson, EJ Battigelli, A Butterfoss, GL Zuckermann, RN Whitelam, S AF Mannige, Ranjan V. Haxton, Thomas K. Proulx, Caroline Robertson, Ellen J. Battigelli, Alessia Butterfoss, Glenn L. Zuckermann, Ronald N. Whitelam, Stephen TI Peptoid nanosheets exhibit a new secondary-structure motif SO NATURE LA English DT Article ID ENERGY LANDSCAPE; PROTEINS; SIMULATION; POLYMERS; DYNAMICS; BINDING; FUNNELS; CHARMM AB A promising route to the synthesis of protein-mimetic materials that are capable of complex functions, such as molecular recognition and catalysis, is provided by sequence-defined peptoid polymers(1,2)-structural relatives of biologically occurring polypeptides. Peptoids, which are relatively non-toxic and resistant to degradation3, can fold into defined structures through a combination of sequence-dependent interactions(3-8). However, the range of possible structures that are accessible to peptoids and other biological mimetics is unknown, and our ability to design protein-like architectures from these polymer classes is limited(9). Here we use molecular-dynamics simulations, together with scattering and microscopy data, to determine the atomic-resolution structure of the recently discovered peptoid nanosheet, an ordered supramolecular assembly that extends macroscopically in only two dimensions. Our simulations show that nanosheets are structurally and dynamically heterogeneous, can be formed only from peptoids of certain lengths, and are potentially porous to water and ions. Moreover, their formation is enabled by the peptoids' adoption of a secondary structure that is not seen in the natural world. This structure, a zigzag pattern that we call a Sigma('sigma')-strand, results from the ability of adjacent backbone monomers to adopt opposed rotational states, thereby allowing the backbone to remain linear and untwisted. Linear backbones tiled in a brick-like way form an extended two-dimensional nanostructure, the Sigma-sheet. The binary rotational-statemotif of the Sigma-strand is not seen in regular protein structures, which are usually built from one type of rotational state. We also show that the concept of building regular structures from multiple rotational states can be generalized beyond the peptoid nanosheet system. C1 [Mannige, Ranjan V.; Haxton, Thomas K.; Proulx, Caroline; Robertson, Ellen J.; Battigelli, Alessia; Zuckermann, Ronald N.; Whitelam, Stephen] Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94709 USA. [Butterfoss, Glenn L.] New York Univ Abu Dhabi, Ctr Genom & Syst Biol, Abu Dhabi, U Arab Emirates. RP Mannige, RV (reprint author), Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94709 USA. EM rvmannige@lbl.gov; swhitelam@lbl.gov FU Office of Science, Office of Basic Energy Sciences of the US Department of Energy [DE-AC02-05CH11231]; Defense Threat Reduction Agency [IACRO-B0845281]; Natural Sciences and Engineering Research Council of Canada (NSERC PDF); Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX Portions of this work were done as a User project at the Molecular Foundry at Lawrence Berkeley National Laboratory, supported by the Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under contract no. DE-AC02-05CH11231. R.V.M., T.K.H., C.P., E.J.R., A.B., R.N.Z. and S.W. were supported by the Defense Threat Reduction Agency under contract no. IACRO-B0845281. C.P. was also supported by the Natural Sciences and Engineering Research Council of Canada (NSERC PDF). R.N.Z. and S.W. were also supported by the Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under contract no. DE-AC02-05CH11231. We thank G.K. Olivier for providing the AFM data. This work used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy under contract no. DE-AC02-05CH11231. Quantum-mechanical calculations were carried out on the High Performance Computing resources at New York University Abu Dhabi. NR 36 TC 26 Z9 26 U1 12 U2 78 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD OCT 15 PY 2015 VL 526 IS 7573 BP 415 EP + DI 10.1038/nature15363 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CT3TQ UT WOS:000362730200048 PM 26444241 ER PT J AU Nave, MI Allen, JP Chen-Wiegart, YCK Wang, J Kalidindi, SR Kornev, KG AF Nave, Maryana I. Allen, Jason P. Chen-Wiegart, Yu-chen Karen Wang, Jun Kalidindi, Surya R. Kornev, Konstantin G. TI In situ X-ray nanotomography of metal surfaces during electropolishing SO SCIENTIFIC REPORTS LA English DT Article ID SCANNING-TUNNELING-MICROSCOPY; ENHANCED RAMAN-SPECTROSCOPY; ATOMIC-FORCE MICROSCOPY; ANODIC ALUMINUM-OXIDE; TUNGSTEN TIPS; ELECTROLYTE; FABRICATION; INTERFACE; CAPILLARY; OXIDATION AB A low voltage electropolishing of metal wires is attractive for nanotechnology because it provides centimeter long and micrometer thick probes with the tip radius of tens of nanometers. Using X-ray nanotomography we studied morphological transformations of the surface of tungsten wires in a specially designed electrochemical cell where the wire is vertically submersed into the KOH electrolyte. It is shown that stability and uniformity of the probe span is supported by a porous shell growing at the surface of tungsten oxide and shielding the wire surface from flowing electrolyte. It is discovered that the kinetics of shell growth at the triple line, where meniscus meets the wire, is very different from that of the bulk of electrolyte. Many metals follow similar electrochemical transformations hence the discovered morphological transformations of metal surfaces are expected to play significant role in many natural and technological applications. C1 [Nave, Maryana I.; Kornev, Konstantin G.] Clemson Univ, Dept Mat Sci & Engn, Clemson, SC 29634 USA. [Allen, Jason P.] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA. [Chen-Wiegart, Yu-chen Karen; Wang, Jun] Brookhaven Natl Lab, Photon Sci Directorate, Upton, NY 11973 USA. [Kalidindi, Surya R.] Georgia Inst Technol, Dept Mech Engn, Atlanta, GA 30332 USA. RP Kornev, KG (reprint author), Clemson Univ, Dept Mat Sci & Engn, Clemson, SC 29634 USA. EM kkornev@clemson.edu OI Allen, Jason/0000-0002-3649-7886; Kalidindi, Surya/0000-0001-6909-7507 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886]; National Science Foundation [PoLS 1305338]; AFOSR award [FA9550-12-1-0458]; NSF-IGERT Award [1258425] FX The use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. M.I.N. and K.G.K. were supported by the National Science Foundation through Grant PoLS 1305338. S.R.K. acknowledges support from AFOSR award FA9550-12-1-0458. J.P.A. acknowledges support from NSF-IGERT Award Number 1258425. We would like to thank Dr. Wah-Keat Lee for his help with the X-ray imaging experiments and Ella Marushchenko for drawing Fig. 1. NR 45 TC 1 Z9 1 U1 4 U2 29 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 15 PY 2015 VL 5 AR 15257 DI 10.1038/srep15257 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CT4WO UT WOS:000362808300001 PM 26469184 ER PT J AU Teeguarden, JG Twaddle, NC Churchwell, MI Yang, XX Fisher, JW Seryak, LM Doerge, DR AF Teeguarden, Justin G. Twaddle, Nathan C. Churchwell, Mona I. Yang, Xiaoxia Fisher, Jeffrey W. Seryak, Liesel M. Doerge, Daniel R. TI 24-hour human urine and serum profiles of bisphenol A: Evidence against sublingual absorption following ingestion in soup SO TOXICOLOGY AND APPLIED PHARMACOLOGY LA English DT Article DE Bisphenol A; Pharmacokinetics; Exposure; Oral; Endocrine disruptors; Sublingual ID ROUTE DEPENDENT DOSIMETRY; TANDEM MASS-SPECTROMETRY; SPRAGUE-DAWLEY RATS; LIQUID-CHROMATOGRAPHY; UNITED-STATES; HUMAN BLOOD; EXPOSURE; BPA; SAMPLES; POPULATION AB Extensive first-pass metabolism of ingested bisphenol A (BPA) in the gastro-intestinal tract and liver restricts blood concentrations of bioactive BPA to <1% of total BPA in humans and non-human primates. Absorption of ingested BPA through non-metabolizing tissues of the oral cavity, recently demonstrated in dogs, could lead to the higher serum BPA concentrations reported in some human biomonitoring studies. We hypothesized that the extensive interaction with the oral mucosa by a liquid matrix, like soup, relative to solid food or capsules, might enhance absorption through non-metabolizing oral cavity tissues in humans, producing higher bioavailability and higher serum BPA concentrations. Concurrent serum and urine concentrations of d6-BPA, and its glucuronide and sulfate conjugates, were measured over a 24 hour period in 10 adult male volunteers following ingestion of 30 mu g d6-BPA/kg body weight in soup. Absorption of d6-BPA was rapid (t(1/2) = 0.45 h) and elimination of the administered dose was complete 24 h post-ingestion, evidence against any tissue depot for BPA. The maximum serum d6-BPA concentration was 0.43 nM at 1.6 h after administration and represented <0.3% of total d6-BPA. Pharmacokinetic parameters, pharmacokinetic model simulations, and the significantly faster appearance half-life of d6-BPA-glucuronide compared to d6-BPA (0.29 h vs 0.45 h) were evidence against meaningful absorption of BPA in humans through any non-metabolizing tissue (<1%). This study confirms that typical exposure to BPA in food produces picomolar to subpicomolar serum BPA concentrations in humans, not nM concentrations reported in some biomonitoring studies. Published by Elsevier Inc. C1 [Teeguarden, Justin G.] Pacific NW Natl Lab, Hlth Effects & Exposure Sci, Richland, WA 99352 USA. [Teeguarden, Justin G.] Oregon State Univ, Dept Environm & Mol Toxicol, Corvallis, OR 97331 USA. [Twaddle, Nathan C.; Churchwell, Mona I.; Yang, Xiaoxia; Fisher, Jeffrey W.; Doerge, Daniel R.] US FDA, Div Biochem Toxicol, Natl Ctr Toxicol Res, Jefferson, AR 72079 USA. [Seryak, Liesel M.] Ohio State Univ, Div Epidemiol, Coll Publ Hlth, Columbus, OH 43210 USA. RP Teeguarden, JG (reprint author), Pacific NW Natl Lab, Hlth Effects & Exposure Sci, Richland, WA 99352 USA. EM jt@pnl.gov; nathan.twaddle@fda.hhs.gov; mona.churchwell@fda.hhs.gov; xiaoxia.yang@fda.hhs.gov; jeffrey.fisher@fda.hhs.gov; seryak.2@osu.edu; daniel.doerge@fda.hhs.gov FU American Chemistry Council, Polycarbonate/BPA Global Group [63289]; U.S. Food and Drug Administration; CDC - NIOSH [R21OH010332]; National Center for Advancing Translational Sciences [UL1TR000090] FX Funding for this research was provided by a grant from the American Chemistry Council, Polycarbonate/BPA Global Group (Grant 63289). ACC and member affiliates did not contribute to the study design, data analysis, reporting, or writing and review of the manuscript. The NCTR laboratory activities were supported by U.S. Food and Drug Administration funding. The views expressed in this manuscript do not necessarily reflect those of the U.S. Food and Drug Administration. Research on the material composition of blood collection devices reported in this publication was supported by Grant Number R21OH010332 from CDC - NIOSH and Grant Number UL1TR000090 from the National Center for Advancing Translational Sciences. Its content is solely the responsibility of the authors and does not necessarily represent the official views of CDC - NIOSH or NCATS or the National Institutes of Health. NR 65 TC 10 Z9 10 U1 2 U2 13 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0041-008X EI 1096-0333 J9 TOXICOL APPL PHARM JI Toxicol. Appl. Pharmacol. PD OCT 15 PY 2015 VL 288 IS 2 BP 131 EP 142 DI 10.1016/j.taap.2015.01.009 PG 12 WC Pharmacology & Pharmacy; Toxicology SC Pharmacology & Pharmacy; Toxicology GA CS9DL UT WOS:000362389200001 PM 25620055 ER PT J AU Aidhy, DS Lu, CY Jin, K Bei, HB Zhang, YW Wang, LM Weber, WJ AF Aidhy, Dilpuneet S. Lu, Chenyang Jin, Ke Bei, Hongbin Zhang, Yanwen Wang, Lumin Weber, William J. TI Point defect evolution in Ni, NiFe and NiCr alloys from atomistic simulations and irradiation experiments SO ACTA MATERIALIA LA English DT Article DE Ion irradiation; Single-phase concentrated solid-solution alloys; Molecular dynamics simulations; Dislocation loop; Face-centered cubic crystals ID STACKING-FAULT TETRAHEDRA; HIGH-ENTROPY ALLOY; RADIATION-DAMAGE; MOLECULAR-DYNAMICS; GRAIN-GROWTH; GOLD; FE; CRYSTALS; ELEMENTS; OXIDES AB Using molecular dynamics simulations, we elucidate irradiation-induced point defect evolution in fcc pure Ni, Ni0.5Fe0.5, and Ni0.8Cr0.2 solid solution alloys. We find that irradiation-induced interstitials form dislocation loops that are of 1/3 < 1 1 1 >{1 1 1}-type, consistent with our experimental results. While the loops are formed in all the three materials, the kinetics of formation is considerably slower in NiFe and NiCr than in pure Ni, indicating that defect migration barriers and extended defect formation energies could be higher in the alloys than pure Ni. As a result, while larger size clusters are formed in pure Ni, smaller and more clusters are observed in the alloys. Vacancy diffusion occurs at relatively higher temperatures than interstitials, and their clustering leads to the formation of stacking fault tetrahedra, consistent with our experiments. The results also show that the surviving Frenkel pairs are composition dependent and are largely Ni dominated. (C) 2015 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Aidhy, Dilpuneet S.; Jin, Ke; Bei, Hongbin; Zhang, Yanwen; Weber, William J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Lu, Chenyang; Wang, Lumin] Univ Michigan, Dept Nucl Engn & Radiol Sci, Ann Arbor, MI 48109 USA. [Weber, William J.] Univ Tennessee, Mat Sci & Engn, Knoxville, TN 37996 USA. RP Aidhy, DS (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM aidhyds@ornl.gov RI Weber, William/A-4177-2008; OI Weber, William/0000-0002-9017-7365; Bei, Hongbin/0000-0003-0283-7990 FU Energy Dissipation to Defect Evolution (EDDE), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences; Office of Science, U.S. Department of Energy [DEAC02-05CH11231] FX This work was supported by Energy Dissipation to Defect Evolution (EDDE), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. The computer simulations were performed at the National Energy Research Scientific Computing Center at Lawrence Berkeley National Laboratory, which is supported by the Office of Science, U.S. Department of Energy under Contract No. DEAC02-05CH11231. NR 38 TC 20 Z9 20 U1 12 U2 72 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD OCT 15 PY 2015 VL 99 BP 69 EP 76 DI 10.1016/j.actamat.2015.08.007 PG 8 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA CS5VC UT WOS:000362145400008 ER PT J AU Kirchheim, R Somerday, B Sofronis, P AF Kirchheim, Reiner Somerday, Brian Sofronis, Petros TI Chemomechanical effects on the separation of interfaces occurring during fracture with emphasis on the hydrogen-iron and hydrogen-nickel system SO ACTA MATERIALIA LA English DT Article DE Fracture; Hydrogen embrittlement; Gibbs Adsorption Isotherm; Interface adsorption ID VACANCY FORMATION ENERGIES; REDUCING GRAIN-BOUNDARY; SOLUTE SEGREGATION; NANOCRYSTALLINE NICKEL; DISSOLVED HYDROGEN; DISLOCATION LINE; SURFACE-ENERGY; ADSORPTION; EMBRITTLEMENT; METALS AB During fracture new surfaces are formed by a propagating crack. Depending on the chemical potential of the constituents of a material and their mobility the composition of the newly formed surfaces changes. Thus the surface energy as part of the work to fracture will be affected. This will be treated by combining the work to fracture representing the mechanical aspect and the Gibbs Adsorption Isotherm covering the chemical aspect. Compared to previous studies the present one provides a more generalized but also a simpler insight into chemomechanical effects. In extreme cases separation of lattice planes or separation of two crystals with a common interface occurs without applied external forces. Closed solutions for the work of fracture are derived for brittle fracture and surface segregation of solutes in the limit of a mean field approach. Chemomechanical effects including plastic deformation by dislocation or vacancy generation are discussed qualitatively. (C) 2015 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Kirchheim, Reiner] Univ Gottingen, Inst Mat Phys, D-37073 Gottingen, Germany. [Kirchheim, Reiner] Max Planck Inst Iron Res GmbH, Dusseldorf, Germany. [Kirchheim, Reiner; Somerday, Brian; Sofronis, Petros] Kyushu Univ, Int Inst Carbon Neutral Energy Res WPI I2CNER, Nishi Ku, Fukuoka 8190395, Japan. [Somerday, Brian] Sandia Natl Labs, Livermore, CA 94550 USA. [Sofronis, Petros] Univ Illinois, Urbana, IL 61801 USA. RP Kirchheim, R (reprint author), Univ Gottingen, Inst Mat Phys, D-37073 Gottingen, Germany. EM acta@gwdg.de RI U-ID, Kyushu/C-5291-2016 FU WPI-I2CNER, Japan; Deutsche Forschungsgemeinschaft, Germany [KI-230/34] FX The authors are grateful for the assistance by Prof. Y. Takata from Kyushu University (WPI-12CNER) during the calculation of fugacity of hydrogen. Financial support by WPI-I2CNER, Japan and by the Deutsche Forschungsgemeinschaft, Germany (KI-230/34) is gratefully acknowledged. NR 53 TC 11 Z9 11 U1 8 U2 38 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD OCT 15 PY 2015 VL 99 BP 87 EP 98 DI 10.1016/j.actamat.2015.07.057 PG 12 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA CS5VC UT WOS:000362145400010 ER PT J AU Tamm, A Aabloo, A Klintenberg, M Stocks, M Caro, A AF Tamm, Artur Aabloo, Alvo Klintenberg, Mattias Stocks, Malcolm Caro, Alfredo TI Atomic-scale properties of Ni-based FCC ternary, and quaternary alloys SO ACTA MATERIALIA LA English DT Article DE High entropy alloy; Density functional theory; Monte Carlo; Short-range order; Ni based alloys ID HIGH-ENTROPY ALLOYS; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; SHORT-RANGE ORDER; AB-INITIO; MONTE-CARLO; BASIS-SET; SCATTERING; METALS; SYSTEM AB The aim of this study is to characterize some atomic-scale properties of Ni-based FCC multicomponent alloys. For this purpose, we use Monte Carlo method combined with density functional theory calculations to study short-range order (SRO), atomic displacements, electronic density of states, and magnetic moments in equimolar ternary NiCrCo, and quaternary NiCrCoFe alloys. According to our study, the salient features for the ternary alloy are a negative SRO parameter between Ni-Cr and a positive between Cr-Cr pairs as well as a weakly magnetic state. For the quaternary alloy we predict negative SRO parameter for Ni-Cr and Ni-Fe pairs and positive for Cr-Cr and Fe-Fe pairs. Atomic displacements for both ternary and quaternary alloys are negligible. In contrast to the ternary, the quaternary alloy shows a complex magnetic structure. The electronic structure of the ternary and quaternary alloys shows differences near the Fermi energy between a random solid solution and the predicted structure with SRO. Despite that, the calculated EXAFS spectra does not show enough contrast to discriminate between random and ordered structures. The predicted SRO has an impact on point-defect energetics, electron-phonon coupling and thermodynamic functions and thus, SRO should not be neglected when studying properties of these two alloys. (C) 2015 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved, C1 [Tamm, Artur; Caro, Alfredo] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87544 USA. [Tamm, Artur; Aabloo, Alvo] Univ Tartu, Inst Technol, IMS Lab, EE-50411 Tartu, Estonia. [Klintenberg, Mattias] Uppsala Univ, Dept Phys & Astron, SE-75120 Uppsala, Sweden. [Stocks, Malcolm] Oak Ridge Natl Lab, Oak Ridge, TN 54321 USA. RP Tamm, A (reprint author), Univ Tartu, Inst Technol, IMS Lab, EE-50411 Tartu, Estonia. EM artur.tamm@ut.ee FU Energy Deposition to Defect Evolution (EDDE), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences at Oak Ridge and Los Alamos National Laboratories [2014 ORNL 1026]; European Social Fund's Doctoral Studies and Internationalization Programme DoRa; Foundation Archimedes and Estonian Research Council grant [IUT20-24] FX This work was supported by the Energy Deposition to Defect Evolution (EDDE), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences (Award Number 2014 ORNL 1026) at Oak Ridge and Los Alamos National Laboratories. AT was partially funded by the European Social Fund's Doctoral Studies and Internationalization Programme DoRa, which is carried out by Foundation Archimedes and Estonian Research Council grant IUT20-24. NR 31 TC 6 Z9 6 U1 17 U2 54 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD OCT 15 PY 2015 VL 99 BP 307 EP 312 DI 10.1016/j.actamat.2015.08.015 PG 6 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA CS5VC UT WOS:000362145400032 ER PT J AU Wang, ZL Zheng, P Nie, ZH Ren, Y Wang, YD Mullner, P Dunand, DC AF Wang, Z. L. Zheng, P. Nie, Z. H. Ren, Y. Wang, Y. D. Muellner, P. Dunand, D. C. TI Superelasticity by reversible variants reorientation in a Ni-Mn-Ga microwire with bamboo grains SO ACTA MATERIALIA LA English DT Article DE Ni2MnGa; Size effect; Superelasticity; Shape-memory effect; Twinning; Oligocrystalline materials ID FIELD-INDUCED STRAIN; SHAPE-MEMORY ALLOYS; MARTENSITE; STRESS; CRYSTALS; BEHAVIOR AB The link between microstructure and mechanical properties is investigated for a superelastic Ni-Mn-Ga microwire with 226 mu m diameter, created by solidification via the Taylor method. The wire, which consists of bamboo grains with tetragonal martensite matrix and coarse gamma precipitates, exhibits fully reversible superelastic behavior up to 4% tensile strain. Upon multiple tensile load unload cycles, reproducible stress fluctuations of similar to 3 MPa are measured on the loading superelastic stress plateau of similar to 50 MPa. During cycles at various temperatures spanning similar to 70 to 55 degrees C, the plateau stress decreases from 58 to 48 MPa near linearly with increasing temperature. Based on in situ synchrotron X-ray diffraction measurements, we conclude that this superelastic behavior is due to reversible martensite variants reorientation (i.e., reversible twinning) with lattice rotation of similar to 13 degrees. The reproducible stress plateau fluctuations are assigned to reversible twinning at well-defined locations along the wire. The strain recovery during unloading is attributed to reverse twinning, driven by the internal stress generated on loading between the elastic gamma precipitates and the twinning martensite matrix. The temperature dependence of the twining stress on loading is related to the change in tetragonality of the martensite, as measured by X-ray diffraction. (C) 2015 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Wang, Z. L.; Zheng, P.; Dunand, D. C.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Wang, Z. L.; Nie, Z. H.] Beijing Inst Technol, Sch Mat Sci & Engn, Beijing 100081, Peoples R China. [Ren, Y.] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Wang, Y. D.] Univ Sci & Technol Beijing, State Key Lab Adv Met & Mat, Beijing 100083, Peoples R China. [Muellner, P.] Boise State Univ, Dept Mat Sci & Engn, Boise, ID 83725 USA. RP Dunand, DC (reprint author), Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. EM dunand@northwestern.edu RI wang, yandong/G-9404-2013; Nie, Zhihua/G-9459-2013; Dunand, David/B-7515-2009 OI Nie, Zhihua/0000-0002-2533-933X; FU US National Science Foundation through Northwestern University [DMR-1207282]; National Basic Research Program of China (973 Program) under University of Science and Technology Beijing [2012CB619405]; Fundamental Research Funds for the Central Universities [06111020]; Fundamental Research Fund by State Key Laboratory for Advanced Metals and Materials in China [2014Z-01]; Chinese Scholarship Council (CSC); U.S. Department of Energy, Office of Science, Office of Basic Energy Science [DE-AC02-06CH11357]; US National Science Foundation through Boise State University [DMR-1207192] FX This research was supported by the US National Science Foundation through Grant No. DMR-1207282 at Northwestern University (Z.L.W. and D.C.D.), the National Basic Research Program of China (973 Program) under Contract No. 2012CB619405 (Y.D.W.) at University of Science and Technology Beijing, and by the US National Science Foundation through Grant No. DMR-1207192 at Boise State University (P.M.). Y.D.W. also acknowledges support from the Fundamental Research Funds for the Central Universities (Grant No. 06111020), and the Fundamental Research Fund by State Key Laboratory for Advanced Metals and Materials (Grant No. 2014Z-01) in China. Z. L.W. acknowledges support from the Chinese Scholarship Council (CSC). Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Science, under Contract No. DE-AC02-06CH11357. We thank Dr. Cun Yu at China University of Petroleum for assistance during experiments at APS, Ms. Nikki Kucza at Boise State University for preparing the alloy ingot, and Prof. L.C. Brinson at Northwestern University for use of her dynamical mechanical analysis instrument. NR 41 TC 2 Z9 2 U1 10 U2 50 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD OCT 15 PY 2015 VL 99 BP 373 EP 381 DI 10.1016/j.actamat.2015.08.002 PG 9 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA CS5VC UT WOS:000362145400038 ER PT J AU McLarty, D Brouwer, J Ainscough, C AF McLarty, Dustin Brouwer, Jack Ainscough, Chris TI Development of an open access tool for design, simulated dispatch, and economic assessment of distributed generation technologies SO ENERGY AND BUILDINGS LA English DT Article DE Dispatch control; Economic design; Combined cooling, heating and power (CCHP); Thermal energy storage; Renewable power; Dynamics of distributed generation ID OPTIMIZATION; BUILDINGS; SYSTEMS AB The design and deployment of DG systems requires an integrated assessment of the building and generator dynamics including the time-variant energy costs and emission factors. Static design optimizations are unable to consider the physical generator operating constraints, seasonal variability and non-coincidence in electric, heating, and cooling demands. This paper introduces the Distributed Generation Build-out Economic Assessment Tool (DG-BEAT) which combines building, utilities, and emissions databases with a library of simplified generator and building models in a user-friendly interface. Five control strategies are presented for the dynamic dispatch of distributed generation technologies at commercial buildings. The control approaches stem from the physical limitations of different generator types. Methods are also outlined for the dispatch of complementary technologies (e.g. energy storage) and accommodation of on-site renewables (e.g. solar PV) which could further improve the economic or environmental benefits of distributed generation. This paper details the methodology of sizing and dispatching distributed generation components, outlines eight databases that are employed to capture regional variations in pricing and building dynamics, and discusses the myriad of customizations available to provide a tailored analysis for a single building or national impact studies. (C) 2015 Elsevier B.V. All rights reserved. C1 [McLarty, Dustin] Washington State Univ, Clean Energy Syst Integrat Lab, Pullman, WA 99164 USA. [Brouwer, Jack] Univ Calif Irvine, Natl Fuel Cell Res Ctr, Irvine, CA 92697 USA. [Ainscough, Chris] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP McLarty, D (reprint author), Washington State Univ, Clean Energy Syst Integrat Lab, Pullman, WA 99164 USA. EM dustin.mclarty@wsu.edu OI McLarty, Dustin/0000-0001-8802-2172 FU U.S. Department of Energy FX The authors gratefully acknowledge and recognize the technical contributions of Sam Sprik, Genevieve Saur, Mike Penev and Darlene Steward at the National Renewable Energy Laboratory. We also gratefully acknowledge the funding and technical support from the U.S. Department of Energy and our contract manager Jason Marcinkoski. NR 24 TC 1 Z9 1 U1 5 U2 20 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0378-7788 EI 1872-6178 J9 ENERG BUILDINGS JI Energy Build. PD OCT 15 PY 2015 VL 105 BP 314 EP 325 DI 10.1016/j.enbuild.2015.07.064 PG 12 WC Construction & Building Technology; Energy & Fuels; Engineering, Civil SC Construction & Building Technology; Energy & Fuels; Engineering GA CS5UG UT WOS:000362143200028 ER PT J AU Wang, SJ Liu, XB Gates, S AF Wang, Shaojie Liu, Xiaobing Gates, Steven TI An introduction of new features for conventional and hybrid GSHP simulations in eQUEST 3.7 SO ENERGY AND BUILDINGS LA English DT Article DE Hybrid ground source heat pump; Multi-year simulation; Water-to-water heat pump AB Three new enhancements, newly implemented into eQUEST 3.7 are presented here. These enhancements include: (1) simulation of ground coupled water-to-water heat pump systems; (2) improved multi-year simulations for conventional and hybrid ground source heat pump (GSHP) systems; (3) model of hybrid GSHP (HGSHP) system configurations. The capabilities of each new feature are outlined and some details of the implementation or simulation techniques of each feature area are briefly discussed. Also, the new wizard features are introduced to show how to build the models through the wizard interfaces. (C) 2015 Elsevier B.V. All rights reserved. C1 [Wang, Shaojie] ClimateMaster, Oklahoma City, OK 73179 USA. [Liu, Xiaobing] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Gates, Steven] James Hirsch & Associates, Santa Rosa Valley, CA USA. RP Wang, SJ (reprint author), ClimateMaster, 7300 SW 44th St, Oklahoma City, OK 73179 USA. EM wsjsxn@gmail.com FU U. S. Department of Energy [DE-EE002799] FX This work is based upon work supported by the U. S. Department of Energy under Award No. DE-EE002799. NR 8 TC 1 Z9 1 U1 2 U2 15 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0378-7788 EI 1872-6178 J9 ENERG BUILDINGS JI Energy Build. PD OCT 15 PY 2015 VL 105 BP 368 EP 376 DI 10.1016/j.enbuild.2015.07.041 PG 9 WC Construction & Building Technology; Energy & Fuels; Engineering, Civil SC Construction & Building Technology; Energy & Fuels; Engineering GA CS5UG UT WOS:000362143200033 ER PT J AU Thakur, P Xiong, YL Borkowski, M AF Thakur, Punam Xiong, Yongliang Borkowski, Marian TI An improved thermodynamic model for the complexation of trivalent actinides and lanthanide with oxalic acid valid to high ionic strength SO CHEMICAL GEOLOGY LA English DT Article DE Oxalic acid dissociation constants; Am-Cm-Eu-oxalic acid complexation; Pitzer parameters; Extraction; High ionic strength ID CONCENTRATED SALT-SOLUTIONS; NUCLEAR-WASTE ISOLATION; INTERACTION PITZER PARAMETERS; METAL-LIGAND INTERACTIONS; NATURAL-WATERS; DISSOCIATION-CONSTANTS; MINERAL SOLUBILITIES; STABILITY-CONSTANTS; NACL SOLUTIONS; OXALATE AB The dissociation constants of oxalic acid (Ox), and the stability constants of Am3+, Cm3+ and Eu3+ with Ox(2-) have been determined at 25 degrees C, over a range of concentration varying from 0.1 to 6.60 m NaClO4 using potentiometric titration and extraction techniques, respectively. The experimental data support the formation of complexes, M(Ox)(n)(3) (-) (2n), where (M = Am3+, Cm3+ and Eu3+ and n = 1 and 2). The dissociation constant and the stability constant values measured as a function of NaClO4 concentration were used to estimate the Pitzer parameters for the respective interactions of Am3+, Cm3+ and Eu3+ with Ox. Furthermore, the stability constants data of Am3+ -Ox measured in NaClO4 and in NaCl solutions from the literature were simultaneously fitted in order to refine the existing actinide-oxalate complexation model that can be used universally in the safety assessment of radioactive waste disposal. The thermodynamic stability constant: log beta(0)(101) = 6.30 +/- 0.06 and log beta(0)(102) = 10.84 +/- 0.06 for Am3+ was obtained by simultaneously fitting data in NaCl and NaClO4 media. Additionally, log beta(0)(101) = 6.72 +/- 0.08 and log beta(0)(102) = 11.05 +/- 0.09 for the Cm3+ and log beta(0)(101) = 6.67 +/- 0.08 and log beta(0)(102)= 11.15 +/- 0.09 for the Eu3+ were calculated by extrapolation of data to zero ionic strength in NaClO4 medium only. For all stability constants, the Pitzer model gives an excellent representation of the data using interaction parameters beta((0)), beta((1)), and C-phi determined in this work. The thermodynamic model developed in this work will be useful in accurately modeling the potential solubility of trivalent actinides and early lanthanides to ionic strength of 6.60 m in low temperature environments in the presence of Ox. The work is also applicable to the accurate modeling transport of rare earth elements in various environments under the surface conditions. (C) 2015 Elsevier B.V. All rights reserved. C1 [Thakur, Punam] Florida State Univ, Dept Chem & Biochem, Tallahassee, FL 32306 USA. [Xiong, Yongliang] Sandia Natl Labs, Carlsbad Program Grp, Carlsbad, NM 88220 USA. [Borkowski, Marian] Los Alamos Natl Lab, Carlsbad Operat, Carlsbad, NM 88220 USA. RP Thakur, P (reprint author), Carlsbad Environm Monitoring & Res Ctr, 1400 Univ Dr, Carlsbad, NM 88220 USA. EM pthakur@cemrc.org FU US Department of Energy, Office of Basic Energy Science; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The support of this work by the US Department of Energy, Office of Basic Energy Science, is gratefully acknowledged. The Pitzer calculations were performed at Sandia National Laboratories. Sandia National Laboratories is a multiprogram laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. The authors thank the anonymous reviewers whose comments have helped to improve this manuscript. NR 78 TC 0 Z9 0 U1 7 U2 26 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2541 EI 1878-5999 J9 CHEM GEOL JI Chem. Geol. PD OCT 15 PY 2015 VL 413 BP 7 EP 17 DI 10.1016/j.chemgeo.2015.07.029 PG 11 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CS1RP UT WOS:000361845700002 ER PT J AU Byerly, BL Lassiter, JC AF Byerly, Benjamin L. Lassiter, John C. TI Trace element partitioning and Lu-Hf isotope systematics in spinel peridotites from the Rio Grande Rift and Colorado Plateau: Towards improved age assessment of clinopyroxene Lu/Hf-Hf-176/Hf-177 in SCLM peridotite SO CHEMICAL GEOLOGY LA English DT Article DE Xenolith; SCLM; Lu/Hf; Hf isotopes; Isochron; Melt depletion; Rio Grande Rift; Colorado Plateau; Partition coefficient; Trace element geochemistry; Spinel peridotite; Lithospheric mantle; Metasomatism ID EAST-AFRICAN RIFT; NORTH CHINA CRATON; LITHOSPHERIC MANTLE; ICP-MS; ENRICHMENT PROCESSES; ABYSSAL PERIDOTITES; TEMPORAL EVOLUTION; BASALTIC MELTS; ORTHO-PYROXENE; UNITED-STATES AB Our study of Colorado Plateau and Rio Grande rift spinel peridotite xenoliths determined bulk Lu-Hf budgets and cpx, opx, andwhole rock Hf-176/Hf-177 to evaluate the potential age significance of Lu/Hf-Hf isotope correlations in sub-continental lithospheric mantle (SCLM) derived xenoliths. The samples have fertilities (spinel Cr# range from 0.1 to 0.5), and equilibration temperatures (950-1050 degrees C) that overlap with those of spinel peridotites commonly used in Lu-Hf dating studies. The Lu/Hf of clinopyroxene (cpx) and its associated whole rock (WR) are similar in fertile samples, but cpx has a lower Lu/Hf than that of the WR in refractory samples. Orthopyroxene (opx) has systematically higher Lu/Hf than cpx, but in many samples, the opx and cpx have identical Hf-176/Hf-177, suggesting that the Hf isotope composition of these minerals is supported by the Lu/Hf of the WR rather than that of the individual minerals. Many opx fractions and whole rocks have less radiogenic Hf-176/Hf-177 than their corresponding cpx (but similar to that of the host magma), reflecting contamination. Because the Hf-176/Hf-177 of cpx is supported by the WR Lu/Hf, it is necessary to use the latter rather than the cpx Lu/Hf for isochron dating. However, because the actual WR Lu/Hf values are susceptible to secondary overprinting, we recommend using model WR Lu/Hf values (determined from mineral Lu and Hf concentrations and modal abundances) to construct external cpx isochrons. Model WR and measured cpx Hf-176/Hf-177 are correlated (r(2) = 0.98) in a suite of eastern Colorado Plateau xenoliths and yield an apparent age of 1.2 Ga (versus 1.5 Ga when - incorrectly - using cpx Lu/Hf). Despite the good correlation between Lu/Hf and Hf-176/Hf-177, we do not find correlations between indicators of melt depletion and Lu/Hf or Hf-176/Hf-177. This suggests that Lu/Hf-Hf-176/Hf-177 correlations are not the result of melt depletion. Instead, we propose that Lu/Hf-Hf-176/Hf-177 correlations are the result of mixing between depleted and enriched components (e.g. metasomatism of depleted lithospheric mantle). We emphasize that additional data should be utilized (e.g. whole rock Lu-Hf budget, degree of metasomatism, opx Hf-176/Hf-177) when interpreting apparent Lu-Hf isochrons for age significance. (C) 2015 Elsevier B.V. All rights reserved. C1 [Byerly, Benjamin L.; Lassiter, John C.] Univ Texas Austin, Dept Geol Sci, Jackson Sch Geosci, Austin, TX 78712 USA. [Byerly, Benjamin L.] Los Alamos Natl Lab, Los Alamos, NM USA. RP Byerly, BL (reprint author), Univ Texas Austin, Dept Geol Sci, Jackson Sch Geosci, Austin, TX 78712 USA. EM benbyerly@utexas.edu RI Lassiter, John/P-1892-2015; OI Lassiter, John/0000-0001-5249-168X; Byerly, Benjamin/0000-0003-0165-8122 FU National Science Foundation [EAR-0648409, EAR-0911253]; University of Texas at Austin Jackson School of Geosciences FX This work was supported in part by National Science Foundation grants EAR-0648409 and EAR-0911253, and by the University of Texas at Austin Jackson School of Geosciences. This manuscript benefitted from constructive comments from Erik Scherer and an anonymous reviewer as well as from the editor Catherine Chauvel. NR 60 TC 2 Z9 2 U1 2 U2 19 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2541 EI 1878-5999 J9 CHEM GEOL JI Chem. Geol. PD OCT 15 PY 2015 VL 413 BP 146 EP 158 DI 10.1016/j.chemgeo.2015.08.009 PG 13 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CS1RP UT WOS:000361845700013 ER PT J AU Agarwal, AK Som, S Shukla, PC Goyal, H Longman, D AF Agarwal, Avinash Kumar Som, Sibendu Shukla, Pravesh Chandra Goyal, Harsh Longman, Douglas TI In-nozzle flow and spray characteristics for mineral diesel, Karanja, and Jatropha biodiesels SO APPLIED ENERGY LA English DT Article DE Cavitation; Primary atomization; Injector nozzle hole; Biodiesel; Viscosity ID FUEL ATOMIZATION CHARACTERISTICS; COMBUSTION; CAVITATION; ENGINES; GEOMETRY; PRESSURE; BEHAVIOR; BLENDS; MODEL AB Superior spray behavior of fuels in internal combustion engines lead to improved combustion and emission characteristics therefore it is necessary to investigate fuel spray behavior of new alternative fuels. This study discusses the evolution of the in-nozzle orifice parameters of a numerical simulation and the evolution of spray parameters of fuel spray in a constant-volume spray chamber during an experiment. This study compares mineral diesel, biodiesels (Karanja-and Jatropha-based), and their blends with mineral diesel. The results show that mineral diesel provides superior atomization and evaporation behavior compared to the biodiesel test fuels. Karanja biodiesel provides superior atomization and evaporation characteristics compared to Jatropha biodiesel. The qualitative comparison of simulation and experimental results in tandem shows that nozzle-hole design is a critical parameter for obtaining optimum spray behavior in the engine combustion chamber. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Agarwal, Avinash Kumar; Goyal, Harsh] Indian Inst Technol, Dept Mech Engn, Engine Res Lab, Kanpur 208016, Uttar Pradesh, India. [Som, Sibendu; Longman, Douglas] Argonne Natl Lab, Ctr Transportat Res, Argonne, IL 60439 USA. [Shukla, Pravesh Chandra] Indian Inst Technol, Dept Civil Engn, Engine Res Lab, Kanpur 208016, Uttar Pradesh, India. RP Agarwal, AK (reprint author), Indian Inst Technol, Dept Mech Engn, Engine Res Lab, Kanpur 208016, Uttar Pradesh, India. EM akag@iitk.ac.in FU IIT Kanpur; [DE-AC02-06CH11357] FX The experimental part of the work was carried out at the Engine Research Laboratory, Indian Institute of Technology Kanpur. The help and assistance of Mr. Roshan Lal is gratefully acknowledged. Funding support given by IIT Kanpur for this work is gratefully acknowledged. The CFD simulations were performed at Argonne National Laboratory, Argonne, Illinois, USA.; The submitted manuscript has been created in collaboration with UChicago Argonne, LLC, operator of Argonne National Laboratory (Argonne). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. The U.S. Government retains for itself, and others acting on its behalf, a paid-up, nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. We gratefully acknowledge the computing resources provided on "Fusion," a 320-node computing cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory. NR 34 TC 3 Z9 4 U1 6 U2 22 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD OCT 15 PY 2015 VL 156 BP 138 EP 148 DI 10.1016/j.apenergy.2015.07.003 PG 11 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA CR5VV UT WOS:000361413400008 ER PT J AU Bansal, P AF Bansal, Pradeep TI High efficiency novel window air conditioner SO APPLIED ENERGY LA English DT Article DE Alternative refrigerants; Window air conditioner; Energy efficiency; ECM; GWP ID PERFORMANCE; CONDENSER AB This paper presents the results of an experimental and analytical evaluation of measures to raise the efficiency of window air conditioners (WAC). In order to achieve a higher energy efficiency ratio (EER), the original capacity of a baseline R410A unit was reduced by replacing the original compressor with a lower capacity but higher EER compressor, while all heat exchangers and the chassis from the original unit were retained. Subsequent major modifications included - replacing the alternating current fan motor with a brushless high efficiency electronically commutated motor (ECM) motor, replacing the capillary tube with a needle valve to better control the refrigerant flow and refrigerant set points, and replacing R410A with a 'drop-in' lower global warming potential (GWP) binary mixture of R32/R125 (85/15% molar concentration). All these modifications resulted in significant enhancement in the EER of the baseline WAC. Further, an economic analysis of the new WAC revealed an encouraging payback period. (C) 2015 Elsevier Ltd. All rights reserved. C1 Oak Ridge Natl Lab, Bldg Equipment Grp, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. RP Bansal, P (reprint author), Oak Ridge Natl Lab, Bldg Equipment Grp, Energy & Transportat Sci Div, One Bethel Valley Rd,MS-6070, Oak Ridge, TN 37831 USA. EM bansalpk@ornl.gov FU Building Technologies Office of the US Department of Energy FX The author is thankful to the Building Technologies Office of the US Department of Energy for their financial support and industry partner General Electric Appliances for their in-kind and technical support. Special thanks are due to a number of contributors for their invaluable contributions and support during this project, including Mr. Edward Vineyard, Mr. Van Baxter, Dr. Chris Halford, Dr. Bo Shen, Mr. Brice Bowley, Mr. Charles Smith, Mr. Jiancheng Zong, Mr. Paul Lin, Mr. Mark Hoehne, Dr. Keith Rice, Mr. Randall Linkous, Mr. Neal Durfee, Mr. Geoff Ormston and Mr. Brian Goins. NR 19 TC 1 Z9 1 U1 1 U2 14 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD OCT 15 PY 2015 VL 156 BP 311 EP 320 DI 10.1016/j.apenergy.2015.07.007 PG 10 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA CR5VV UT WOS:000361413400024 ER PT J AU Zhang, J Draxl, C Hopson, T Delle Monache, L Vanvyve, E Hodge, BM AF Zhang, Jie Draxl, Caroline Hopson, Thomas Delle Monache, Luca Vanvyve, Emilie Hodge, Bri-Mathias TI Comparison of numerical weather prediction based deterministic and probabilistic wind resource assessment methods SO APPLIED ENERGY LA English DT Article DE Analog ensemble; Numerical weather prediction; Probabilistic wind resource assessment; Variability; WIND Toolkit; MERRA ID MODEL; PRECIPITATION; SIMULATION; FORECAST; SYSTEMS; SPEED AB Numerical weather prediction (NWP) models have been widely used for wind resource assessment. Model runs with higher spatial resolution are generally more accurate, yet extremely computational expensive. An alternative approach is to use data generated by a low resolution NWP model, in conjunction with statistical methods. In order to analyze the accuracy and computational efficiency of different types of NWP-based wind resource assessment methods, this paper performs a comparison of three deterministic and probabilistic NWP-based wind resource assessment methodologies: (i) a coarse resolution (0.5 degrees x 0.67 degrees) global reanalysis data set, the Modern-Era Retrospective Analysis for Research and Applications (MERRA); (ii) an analog ensemble methodology based on the MERRA, which provides both deterministic and probabilistic predictions; and (iii) a fine resolution (2-km) NWP data set, the Wind Integration National Dataset (WIND) Toolkit, based on the Weather Research and Forecasting model. Results show that: (i) as expected, the analog ensemble and WIND Toolkit perform significantly better than MERRA confirming their ability to downscale coarse estimates; (ii) the analog ensemble provides the best estimate of the multi-year wind distribution at seven of the nine sites, while the WIND Toolkit is the best at one site; (iii) the WIND Toolkit is more accurate in estimating the distribution of hourly wind speed differences, which characterizes the wind variability, at five of the available sites, with the analog ensemble being best at the remaining four locations; and (iv) the analog ensemble computational cost is negligible, whereas the WIND Toolkit requires large computational resources. Future efforts could focus on the combination of the analog ensemble with intermediate resolution (e.g., 10-45 kin) NWP estimates, to considerably reduce the computational burden, while providing accurate deterministic estimates and reliable probabilistic assessments. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Zhang, Jie; Draxl, Caroline; Hodge, Bri-Mathias] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Hopson, Thomas; Delle Monache, Luca; Vanvyve, Emilie] Natl Ctr Atmospher Res, Boulder, CO 80307 USA. [Vanvyve, Emilie] Met Off, Exeter EX1 3PB, Devon, England. RP Hodge, BM (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM bri.mathias.hodge@nrel.gov RI Draxl, Caroline/O-6206-2016 OI Draxl, Caroline/0000-0001-5532-6268 FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory FX This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. NR 44 TC 3 Z9 3 U1 0 U2 15 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD OCT 15 PY 2015 VL 156 BP 528 EP 541 DI 10.1016/j.apenergy.2015.07.059 PG 14 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA CR5VV UT WOS:000361413400042 ER PT J AU Gao, CX Sun, M Shen, B AF Gao, Cuixia Sun, Mei Shen, Bo TI Features and evolution of international fossil energy trade relationships: A weighted multilayer network analysis SO APPLIED ENERGY LA English DT Article DE International fossil energy trade; Multilayer network; Degree distribution; Community; Stability ID GLOBAL OIL TRADE; PERSPECTIVE; PATTERNS; MODEL AB From June 2014 to January 2015, the slumped price of crude oil mainly be caused by the increasing shale gas in the U.S. The market of crude oil was altered by the variation of natural gas trade patterns. It implies that the international fossil energy trade is a multilayer structure, and each layer is a complex system with numerous countries and complicated relations. In this paper, we build the international fossil energy trade multilayer network (ETMN), and study the evolutionary characteristics of networks during 2002-2013. The generalization of several important indicators, including degree distribution, community, stability of communities and the time-varying evolution of main countries' importance were discussed. Our conclusions suggest that: Firstly, the ETMN and three energy-specific networks including coal, oil, and natural gas display the scale-free characteristic in un-weighted and weighted networks. However, it shows that even if a few countries have major trading partners, there are not always a few countries that play critical roles in trade intensity. Secondly, the natural gas network has the largest number of communities and stability compared with networks of coal and oil, and the volatility of stability lagged one year than the other two networks for the specific form of pipeline transportation. Thirdly, studying on the stability of networks shows that geopolitical environment is the most important influenced factor, but the status of renewable and new energy increases with its development obviously. Fourthly, the evolutionary characteristics of three major countries' importance, including United States, China and Japan, are analyzed in detail. At last, some policy suggestions were pointed out according to the results. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Gao, Cuixia; Sun, Mei] Jiangsu Univ, Ctr Energy Dev & Environm Protect, Zhenjiang 212013, Jiangsu, Peoples R China. [Shen, Bo] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Anal & Environm Impact Assessment Dept, China Energy Grp,Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Sun, M (reprint author), Jiangsu Univ, Ctr Energy Dev & Environm Protect, Zhenjiang 212013, Jiangsu, Peoples R China. EM sunm@ujs.edu.cn OI Gao, Cuixia/0000-0002-4345-2934 FU National Nature Science Foundation of China [71273119]; Graduate Innovative Foundation of Jiangsu Province [KYLX15_1076] FX This research was supported by National Nature Science Foundation of China (No. 71273119) and the Graduate Innovative Foundation of Jiangsu Province KYLX15_1076. NR 28 TC 9 Z9 9 U1 18 U2 68 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD OCT 15 PY 2015 VL 156 BP 542 EP 554 DI 10.1016/j.apenergy.2015.07.054 PG 13 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA CR5VV UT WOS:000361413400043 ER PT J AU Craciun, D Socol, G Lambers, E McCumiskey, EJ Taylor, CR Martin, C Argibay, N Tanner, DB Craciun, V AF Craciun, D. Socol, G. Lambers, E. McCumiskey, E. J. Taylor, C. R. Martin, C. Argibay, N. Tanner, D. B. Craciun, V. TI Optical and mechanical properties of nanocrystalline ZrC thin films grown by pulsed laser deposition SO APPLIED SURFACE SCIENCE LA English DT Article; Proceedings Paper CT 10th International Conference on Physics of Advanced Materials (ICPAM) CY SEP 22-28, 2014 CL Iasi, ROMANIA SP Romanian Minist Educ & Res, NanoAndMore, ExpressCredit, Amer Elements, ArcelorMittal Tubular Prod Iasi, Agilrom Sci, Schaefer SE Europe, PIM Copy, Histeresis, ApeLaser, Nitech, Technosteel LBR, Thorlabs GmbH, MaTecK, Sartorom, Antalis, Emfutur, Romanian Phys Soc DE ZrC; Hard coating; Pulsed laser deposition; Infrared optical properties ID GRAZING-INCIDENCE; ZRC/TIN AB Thin ZrC films (<500nm) were grown on (100) Si substrates at a substrate temperature of 500 degrees C by the pulsed laser deposition (PLD) technique using a KrF excimer laser under different CH4 pressures. Glancing incidence X-ray diffraction showed that films were nanocrystalline, while X-ray reflectivity studies found out films were very dense and exhibited a smooth surface morphology. Optical spectroscopy data shows that the films have high reflectivity (>90%) in the infrared region, characteristic of metallic behavior. Nanoindentation results indicated that films deposited under lower CH4 pressures exhibited slightly higher nanohardness and Young modulus values than films deposited under higher pressures. Tribological characterization revealed that these films exhibited relatively high wear resistance and steady-state friction coefficients on the order of mu = 0.4. (C) 2015 Elsevier B.V. All rights reserved. C1 [Craciun, D.; Socol, G.; Craciun, V.] Natl Inst Laser Plasma & Radiat Phys, Laser Dept, Magurele, Romania. [Lambers, E.] Univ Florida, Major Analyt Instrumentat Ctr, Coll Engn, Gainesville, FL 32611 USA. [McCumiskey, E. J.; Taylor, C. R.] Univ Florida, Mech & Aerosp Engn, Gainesville, FL 32611 USA. [Martin, C.] Ramapo Coll, Mahwah, NJ USA. [Argibay, N.] Sandia Natl Labs, Ctr Mat Sci & Engn, Albuquerque, NM 87123 USA. [Tanner, D. B.] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. RP Craciun, D (reprint author), Natl Inst Laser Plasma & Radiat Phys, Laser Dept, Magurele, Romania. EM doina.craciun@inflpr.ro RI Socol, Gabriel/A-5405-2011 OI Socol, Gabriel/0000-0002-1992-7346 NR 20 TC 2 Z9 2 U1 6 U2 27 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0169-4332 EI 1873-5584 J9 APPL SURF SCI JI Appl. Surf. Sci. PD OCT 15 PY 2015 VL 352 BP 28 EP 32 DI 10.1016/j.apsusc.2015.01.026 PG 5 WC Chemistry, Physical; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA CR3EA UT WOS:000361212200007 ER EF