FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Smylie, MP Leroux, M Mishra, V Fang, L Taddei, KM Chmaissem, O Claus, H Kayani, A Snezhko, A Welp, U Kwok, WK AF Smylie, M. P. Leroux, M. Mishra, V. Fang, L. Taddei, K. M. Chmaissem, O. Claus, H. Kayani, A. Snezhko, A. Welp, U. Kwok, W. -K. TI Effect of proton irradiation on superconductivity in optimally doped BaFe2(As1-xPx)(2) single crystals SO PHYSICAL REVIEW B LA English DT Article ID TEMPERATURE PENETRATION DEPTH; UNCONVENTIONAL SUPERCONDUCTORS; IRON PNICTIDES; DEFECTS; YBA2CU3O7-X AB Irradiation with 4 MeV protons was used to systematically introduce defects in single crystals of the iron-arsenide superconductor BaFe2(As1-xPx)(2), x = 0.33. The effect of disorder on the low-temperature behavior of the London penetration depth lambda(T) and transition temperature T-c was investigated. In nearly optimally doped samples with T-c similar to 29 K, signatures of a superconducting gap with nodes were observed. Contrary to previous reports on electron-irradiated crystals, we do not see a disorder-driven lifting of accidental nodes, and we observe that proton-induced defects are weaker pair breakers than electron-induced defects. We attribute our findings to anisotropic electron scattering caused by proton irradiation defects. C1 [Smylie, M. P.; Leroux, M.; Mishra, V.; Fang, L.; Taddei, K. M.; Chmaissem, O.; Claus, H.; Snezhko, A.; Welp, U.; Kwok, W. -K.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Taddei, K. M.; Chmaissem, O.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Kayani, A.] Western Michigan Univ, Dept Phys, Kalamazoo, MI 49008 USA. [Mishra, V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Smylie, MP (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM msmylie@anl.gov RI Leroux, Maxime/E-8703-2016; Taddei, Keith/K-4641-2016 OI Leroux, Maxime/0000-0001-9778-323X; Taddei, Keith/0000-0002-1468-0823 FU US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; Center for Emergent Superconductivity; Center for Emergent Superconductivity, an Energy Frontier Research Center - the US DOE, Office of Science, Office of Basic Energy Sciences FX Tunnel diode oscillator and magnetization measurements were supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. Theoretical work and transport measurements (V.M., M.L.) and synthesis (L.F., K.T.) were supported by the Center for Emergent Superconductivity, an Energy Frontier Research Center funded by the US DOE, Office of Science, Office of Basic Energy Sciences. NR 48 TC 2 Z9 2 U1 7 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 10 PY 2016 VL 93 IS 11 AR 115119 DI 10.1103/PhysRevB.93.115119 PG 5 WC Physics, Condensed Matter SC Physics GA DG0ER UT WOS:000371737400002 ER PT J AU Esbensen, H Montagnoli, G Stefanini, AM AF Esbensen, H. Montagnoli, G. Stefanini, A. M. TI Revised analysis of Ca-40+Zr-96 fusion reactions SO PHYSICAL REVIEW C LA English DT Article ID HEAVY-ION FUSION AB Fusion data for Ca-40+Zr-96 are analyzed by coupled-channels calculations that are based on a standard Woods-Saxon potential and include couplings to multiphonon excitations and transfer channels. The couplings to multiphonon excitations are the same as those used in a previous work. The transfer couplings are calibrated to reproduce the measured neutron transfer data. This type of calculation gives a poor fit to the fusion data. However, by multiplying the transfer couplings with a root 2 one obtains an excellent fit. The scaling of the transfer strengths is supposed to simulate the combined effect of neutron and proton transfer, and the calculated one- and two-nucleon transfer cross sections are indeed in reasonable agreement with the measured cross sections. C1 [Esbensen, H.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Montagnoli, G.] Univ Padua, Dipartimento Fis & Astron, I-35131 Padua, Italy. [Montagnoli, G.] Ist Nazl Fis Nucl, Sez Padova, I-35131 Padua, Italy. [Stefanini, A. M.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Padua, Italy. RP Esbensen, H (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. FU US Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357] FX H.E. was supported by the US Department of Energy, Office of Science, Office of Nuclear Physics, Contract No. DE-AC02-06CH11357. NR 23 TC 1 Z9 1 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 10 PY 2016 VL 93 IS 3 AR 034609 DI 10.1103/PhysRevC.93.034609 PG 8 WC Physics, Nuclear SC Physics GA DG0FS UT WOS:000371741100005 ER PT J AU Karsch, F Morita, K Redlich, K AF Karsch, Frithjof Morita, Kenji Redlich, Krzysztof TI Effects of kinematic cuts on net electric charge fluctuations SO PHYSICAL REVIEW C LA English DT Article ID FREEZE-OUT CONDITIONS; HEAVY-ION COLLISIONS; QCD PHASE-TRANSITION; RESONANCE GAS-MODEL; HADRONIC FLUCTUATIONS; LATTICE QCD; THERMODYNAMICS; LHC AB The effects of kinematic cuts on electric charge fluctuations in a gas of charged particles are discussed. We consider a very transparent example of an ideal pion gas with quantum statistics, which can be viewed as a multicomponent gas of Boltzmann particles with different charges, masses, and degeneracies. Cumulants of net electric charge fluctuations chi(Q)(n) are calculated in a static and expanding medium with flow parameters adjusted to the experimental data. We show that the transverse momentum cut, p(tmin) <= p(t) <= p(tmax), weakens the effects of Bose statistics, i.e., contributions of effectively multicharged states to higher order moments. Consequently, cuts in p(t) modify the experimentally measured cumulants and their ratios. We discuss the influence of kinematic cuts on the ratio of mean and variance of electric charge fluctuations in a hadron resonance gas, in the light of recent data from the STAR and PHENIX Collaborations. We find that the different momentum cuts of p(tmin) = 0.2 GeV (STAR) and p(tmin) = 0.3 GeV (PHENIX) are responsible for more than 30% of the difference between these two data sets. We argue that the p(t) cuts imposed on charged particles will influence the normalized kurtosis kappa(Q) sigma(2)(Q) = chi(Q)(4)/chi(Q)(2) of the electric charge fluctuations. In particular, the reduction of kappa(Q) sigma(2)(Q) with increasing p(tmin) will lead to differences between PHENIX and STAR data of O(6%), which currently are buried under large statistical and systematic errors. We furthermore introduce the relation between momentum cutoff and finite volume effects, which is of relevance for the comparison between experimental data and lattice QCD calculations. C1 [Karsch, Frithjof] Univ Bielefeld, Fak Phys, D-33615 Bielefeld, Germany. [Karsch, Frithjof] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Karsch, Frithjof] Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China. [Karsch, Frithjof] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China. [Morita, Kenji] Kyoto Univ, Yukawa Inst Theoret Phys, Kyoto 6068502, Japan. [Morita, Kenji; Redlich, Krzysztof] Univ Wroclaw, Inst Theoret Phys, PL-50204 Wroclaw, Poland. [Redlich, Krzysztof] ExtreMe Matter Inst EMMI, D-64291 Darmstadt, Germany. [Redlich, Krzysztof] Duke Univ, Dept Phys, Durham, NC 27708 USA. RP Karsch, F (reprint author), Univ Bielefeld, Fak Phys, D-33615 Bielefeld, Germany.; Karsch, F (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA.; Karsch, F (reprint author), Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China.; Karsch, F (reprint author), Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China.; Morita, K (reprint author), Kyoto Univ, Yukawa Inst Theoret Phys, Kyoto 6068502, Japan.; Morita, K; Redlich, K (reprint author), Univ Wroclaw, Inst Theoret Phys, PL-50204 Wroclaw, Poland.; Redlich, K (reprint author), ExtreMe Matter Inst EMMI, D-64291 Darmstadt, Germany.; Redlich, K (reprint author), Duke Univ, Dept Phys, Durham, NC 27708 USA. EM karsch@bnl.gov; kmorita@yukawa.kyoto-u.ac.jp; krzysztof.redlich@ift.uni.wroc.pl RI Morita, Kenji/R-8116-2016 OI Morita, Kenji/0000-0001-6272-1290 FU GSI/EMMI group; MEXT [24105008]; Polish Science Center (NCN) [2013/10/A/ST2/00106]; U.S. Department of Energy [DE-SC0012704, DE-FG02-05ER41367]; Bundesministerium fur Bildung und Forschung (BMBF) [05P15PBCAA] FX K.R. acknowledges stimulating discussions with Peter Braun-Munzinger, Volker Koch, and Nu Xu. We also acknowledge fruitful discussions with Bengt Friman, Swagato Mukherjee, and Chihiro Sasaki. K. M. acknowledges the support of the GSI/EMMI group, where a part of this work was completed. This work was supported by the Grants-in-Aid for Scientific Research on Innovative Areas from MEXT (No. 24105008), the Polish Science Center (NCN) under Maestro Grant No. 2013/10/A/ST2/00106, the U.S. Department of Energy under Contracts No. DE-SC0012704 and No. DE-FG02-05ER41367, as well as the Bundesministerium fur Bildung und Forschung (BMBF) under Grant No. 05P15PBCAA. NR 43 TC 6 Z9 6 U1 1 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 10 PY 2016 VL 93 IS 3 AR 034907 DI 10.1103/PhysRevC.93.034907 PG 9 WC Physics, Nuclear SC Physics GA DG0FS UT WOS:000371741100007 ER PT J AU Li, Y Hu, W Takada, M AF Li, Yin Hu, Wayne Takada, Masahiro TI Separate universe consistency relation and calibration of halo bias SO PHYSICAL REVIEW D LA English DT Article ID LARGE-SCALE BIAS; PEAK-BACKGROUND SPLIT; DARK-MATTER HALOES; MASS FUNCTION; MODEL; COSMOLOGY; SIMULATIONS; OCCUPATION; DEPENDENCE AB The linear halo bias is the response of the dark matter halo number density to a long-wavelength fluctuation in the dark matter density. Using abundance matching between separate universe simulations which absorb the latter into a change in the background, we test the consistency relation between the change in a one-point function, the halo mass function, and a two-point function, the halo-matter cross-correlation in the long-wavelength limit. We find excellent agreement between the two at the 1%-2% level for average halo biases between 1 less than or similar to (h) over bar (1) less than or similar to 4 and no statistically significant deviations at the 4%-5% level out to (h) over bar (1) approximate to 8. The halo bias inferred assuming instead a universal mass function is significantly different and inaccurate at the 10% level or more. The separate universe technique provides a way of calibrating the linear halo bias efficiently for even highly biased rare halos in the. cold dark matter model. Observational violation of the consistency relation would indicate new physics, e.g. in the dark matter, dark energy, or primordial non-Gaussianity sectors. C1 [Li, Yin] Univ Calif Berkeley, Dept Phys, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. [Li, Yin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Li, Yin; Takada, Masahiro] Univ Tokyo, UTIAS, Kavli Inst Phys & Math Universe WPI, Chiba 2778583, Japan. [Hu, Wayne] Univ Chicago, Kavli Inst Cosmol Phys, Enrico Fermi Inst, Dept Astron & Astrophys, Chicago, IL 60637 USA. RP Li, Y (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA.; Li, Y (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.; Li, Y (reprint author), Univ Tokyo, UTIAS, Kavli Inst Phys & Math Universe WPI, Chiba 2778583, Japan. NR 44 TC 6 Z9 6 U1 3 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 10 PY 2016 VL 93 IS 6 AR 063507 DI 10.1103/PhysRevD.93.063507 PG 14 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DG0GS UT WOS:000371743900004 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Abeloos, B Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allen, BW Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Armitage, LJ Arnaez, O Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Artz, S Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Balunas, WK Banas, E Banerjee, S Bannoura, AAE Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Navarro, LB Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, M Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bedognetti, M Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, AS Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Belyaev, NL Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Benitez, J Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Berlendis, S Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertram, IA Bertsche, C Bertsche, D Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Biedermann, D Bielski, R Biesuz, NV Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biondi, S Bjergaard, DM Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Blunier, S Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehler, M Boerner, D Bogaerts, JA Bogavac, D Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Bortfeldt, J Bortoletto, D Bortolotto, V Bos, K Boscherini, D Bosman, M Sola, JDB Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutle, SK Boveia, A Boyd, J Boyko, IR Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Madden, WDB Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Broughton, JH de Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Brunt, B Bruschi, M Bruscino, N Bryant, P Bryngemark, L Buanes, T Buat, Q Buchholz, P Buckley, AG Budagov, IA Buehrer, F Bugge, MK Bulekov, O Bullock, D Burckhart, H Burdin, S Burgard, CD Burghgrave, B Burka, K Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Buzykaev, AR Urban, SC Caforio, D Cairo, VM Cakir, O Calace, N Calafiura, P Calandri, A Calderini, G Calfayan, P Caloba, LP Calvet, D Calvet, S Calvet, TP Toro, RC Camarda, S Camarri, P Cameron, D Armadans, RC Camincher, C Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Carbone, RM Cardarelli, R Cardillo, F Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Casper, DW Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catinaccio, A Catmore, JR Cattai, A Caudron, J Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Alberich, LC Cerio, BC Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chan, SK Chan, YL Chang, P Chapman, JD Charlton, DG Chatterjee, A Chau, CC Barajas, CAC Che, S Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, S Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A Cheremushkina, E El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiarelli, G Chiodini, G Chisholm, AS Chitan, A Chizhov, MV Choi, K Chouridou, S Chow, BKB Christodoulou, V Chromek-Burckhart, D Chudoba, J Chuinard, AJ Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Cinca, D Cindro, V Cioara, IA Ciocio, A Cirotto, F Citron, ZH Ciubancan, M Clark, A Clark, BL Clark, PJ Clarke, RN Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Colasurdo, L Cole, B Cole, S Colijn, AP Collot, J Colombo, T Compostella, G Muino, PC Coniavitis, E Connell, SH Connelly, IA Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cottin, G Cowan, G Cox, BE Cranmer, K Crawley, SJ Cree, G Crepe-Renaudin, S Crescioli, F Cribbs, WA Ortuzar, MC Cristinziani, M Croft, V Crosetti, G Donszelmann, TC Cummings, J Curatolo, M Cuth, J Cuthbert, C Czirr, H Czodrowski, P D'Auria, S D'Onofrio, M De Sousa, MJDS Da Via, C Dabrowski, W Dai, T Dale, O Dallaire, F Dallapiccola, C Dam, M Dandoy, JR Dang, NP Daniells, AC Dann, NS Danninger, M Hoffmann, MD Dao, V Darbo, G Darmora, S Dassoulas, J Dattagupta, A Davey, W David, C Davidek, T Davies, M Davison, P Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Benedetti, A De Castro, S De Cecco, S De Groot, N de Jong, P De la Torre, H De Lorenzi, F De Pedis, D De Salvo, A De Sanctis, U De Santo, A De Regie, JBD Dearnaley, WJ Debbe, R Debenedetti, C Dedovich, DV Deigaard, I Del Peso, J Del Prete, T Delgove, D Deliot, F Delitzsch, CM Deliyergiyev, M Dell'Acqua, A Dell'Asta, L Dell'Orso, M Della Pietra, M della Volpe, D Delmastro, M Delsart, PA Deluca, C DeMarco, DA Demers, S Demichev, M Demilly, A Denisov, SP Denysiuk, D Derendarz, D Derkaoui, JE Derue, F Dervan, P Desch, K Deterre, C Dette, K Deviveiros, PO Dewhurst, A Dhaliwal, S Di Ciaccio, A Di Ciaccio, L Di Clemente, WK Di Domenico, A Di Donato, C Di Girolamo, A Di Girolamo, B Di Mattia, A Di Micco, B Di Nardo, R Di Simone, A Di Sipio, R Di Valentino, D Diaconu, C Diamond, M Dias, FA Diaz, MA Diehl, EB Dietrich, J Diglio, S Dimitrievska, A Dingfelder, J Dita, P Dita, S Dittus, F Djama, F Djobava, T Djuvsland, JI do Vale, MAB Dobos, D Dobre, M Doglioni, C Dohmae, T Dolejsi, J Dolezal, Z Dolgoshein, BA Donadelli, M Donati, S Dondero, P Donini, J Dopke, J Doria, A Dova, MT Doyle, AT Drechsler, E Dris, M Du, Y Duarte-Campderros, J Duchovni, E Duckeck, G Ducu, OA Duda, D Dudarev, A Duflot, L Duguid, L Duhrssen, M Dunford, M Yildiz, HD Duren, M Durglishvili, A Duschinger, D Dutta, B Dyndal, M Eckardt, C Ecker, KM Edgar, RC Edson, W Edwards, NC Eifert, T Eigen, G Einsweiler, K Ekelof, T El Kacimi, M Ellajosyula, V Ellert, M Elles, S Ellinghaus, F Elliot, AA Ellis, N Elmsheuser, J Elsing, M Emeliyanov, D Enari, Y Endner, OC Endo, M Ennis, JS Erdmann, J Ereditato, A Ernis, G Ernst, J Ernst, M Errede, S Ertel, E Escalier, M Esch, H Escobar, C Esposito, B Etienvre, AI Etzion, E Evans, H Ezhilov, A Fabbri, L Facini, G Fakhrutdinov, RM Falciano, S Falla, RJ Faltova, J Fang, Y Fanti, M Farbin, A Farilla, A Farina, C Farooque, T Farrell, S Farrington, SM Farthouat, P Fassi, F Fassnacht, P Fassouliotis, D Giannelli, MF Favareto, A Fayard, L Fedin, OL Fedorko, W Feigl, S Feligioni, L Feng, C Feng, EJ Feng, H Fenyuk, AB Feremenga, L Martinez, PF Perez, SF Ferrando, J Ferrari, A 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Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Measurement of the ZZ Production Cross Section in pp Collisions at root s=13 TeV with the ATLAS Detector SO PHYSICAL REVIEW LETTERS LA English DT Article ID PARTON DISTRIBUTIONS; LHC AB The ZZ production cross section in proton-proton collisions at 13 TeV center-of-mass energy is measured using 3.2 fb(-1) of data recorded with the ATLAS detector at the Large Hadron Collider. The considered Z boson candidates decay to an electron or muon pair of mass 66-116 GeV. The cross section is measured in a fiducial phase space reflecting the detector acceptance. It is also extrapolated to a total phase space for Z bosons in the same mass range and of all decay modes, giving 16.7(-2.0)(+2.2) (stat)(-0.7)(+0.9) (syst)(-0.7)(+1.0) (lumi) pb. The results agree with standard model predictions. C1 [Jackson, P.; Lee, L.; Petridis, A.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Yildiz, H. Duran] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Kuday, S.] Istanbul Aydin Univ, Istanbul, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. 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A.; Jones, S.; Lampl, W.; Lei, X.; Leone, R.; Loch, P.; Nayyar, R.; O'grady, F.; Rutherfoord, J. P.; Shupe, M. A.; Varnes, E. W.; Veatch, J.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Brandt, A.; Bullock, D.; Darmora, S.; De, K.; Farbin, A.; Feremenga, L.; Griffiths, J.; Hadavand, H. K.; Heelan, L.; Kim, H. Y.; Ozturk, N.; Schovancova, J.; Stradling, A. R.; Usai, G.; Vartapetian, A.; White, A.; Yu, J.] Univ Texas Arlington, Dept Phys, POB 19059, Arlington, TX 76019 USA. [Angelidakis, S.; Chouridou, S.; Fassouliotis, D.; Giokaris, N.; Ioannou, P.; Kourkoumelis, C.] Univ Athens, Dept Phys, Athens, Greece. [Alexopoulos, T.; Benekos, N.; Dris, M.; Gazis, E. N.; Karakostas, K.; Karastathis, N.; Karentzos, E.; Leontsinis, S.; Maltezos, S.; Ntekas, K.; St Panagiotopoulou, E.; Papadopoulou, Th. D.; Tsipolitis, G.; Vlachos, S.] Natl Tech Univ Athens, Dept Phys, Zografos, Greece. [Abdinov, O.; Ahmadov, F.; Huseynov, N.; Javadov, N.; Khalil-zada, F.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Anjos, N.; Bosman, M.; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fernandez Perez, S.; Fischer, C.; Fracchia, S.; Gonzalez Parra, G.; Grinstein, S.; Juste Rozas, A.; Korolkov, I.; Lange, J. C.; Le Menedeu, E.; Lopez Paz, I.; Martinez, M.; Mir, L. M.; Pacheco Pages, A.; Padilla Aranda, C.; Riu, I.; Rodriguez Perez, A.; Sorin, V.; Tripiana, M. F.; Tsiskaridze, S.; Valery, L.] Barcelona Inst Sci & Technol, Inst Fis Altes Energies IFAE, Barcelona, Spain. [Agatonovic-Jovin, T.; Bogavac, D.; Dimitrievska, A.; Krstic, J.; Marjanovic, M.; Popovic, D. S.; Sijacki, Dj.; Simic, Lj.; Vranjes, N.; Milosavljevic, M. Vranjes; Zivkovic, L.] Univ Belgrade, Inst Phys, Belgrade, Serbia. [Buanes, T.; Dale, O.; Eigen, G.; Kastanas, A.; Liebig, W.; Lipniacka, A.; Maeland, S.; Latour, B. Martin Dit; Sjursen, T. B.; Smestad, L.; Stugu, B.; Yang, Z.; Zalieckas, J.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Amadio, B. T.; Axen, B.; Barnett, R. M.; Beringer, J.; Bhimji, W.; Brosamer, J.; Calafiura, P.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Einsweiler, K.; Farrell, S.; Gabrielli, A.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Heim, T.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Viel, S.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Amadio, B. T.; Axen, B.; Barnett, R. M.; Beringer, J.; Brosamer, J.; Calafiura, P.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Einsweiler, K.; Farrell, S.; Gabrielli, A.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Heim, T.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W-M.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Biedermann, D.; Dietrich, J.; Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Hristova, I.; Kind, O. M.; Kolanoski, H.; Lacker, H.; Lohse, T.; Mergelmeyer, S.; Nikiforov, A.; Rehnisch, L.; Rieck, P.; Schulz, H.; Sperlich, D.; Stamm, S.; zur Nedden, M.] Humboldt Univ, Dept Phys, Invalidenstr 110, Berlin, Germany. [Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Mullier, G. A.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Mullier, G. A.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allport, P. P.; Bella, L. Aperio; Baca, M. J.; Bracinik, J.; Broughton, J. H.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Gonella, L.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Owen, R. E.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Phys, Gaziantep, Turkey. [Cetin, S. A.] Istanbul Bilgi Univ, Fac Engn & Nat Sci, Istanbul, Turkey. [Beddall, A. J.] Bahcesehir Univ, Fac Engn & Nat Sci, Istanbul, Turkey. [Alberghi, G. L.; Bellagamba, L.; Biondi, S.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, Bologna, Italy. [Alberghi, G. L.; Biondi, S.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Bruscino, N.; Cioara, I. A.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Gaycken, G.; Geich-Gimbel, Ch.; Grefe, C.; Haefner, P.; Hageboeck, S.; Hansen, M. C.; Hohn, D.; Huegging, F.; Janssen, J.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lantzsch, K.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mijovic, L.; Moles-Valls, R.; Obermann, T.; Pohl, D.; Ricken, O.; Sarrazin, B.; Schaepe, S.; Schopf, E.; Schultens, M. J.; Schwindt, T.; Seema, P.; Stillings, J. A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Yuen, S. P. Y.; Zhang, R.] Univ Bonn, Inst Phys, Nussallee 12, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, 590 Commonwealth Ave, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Barone, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Dhaliwal, S.; Loew, K. M.; Sciolla, G.; Venturini, A.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Amaral Coutinho, Y.; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.; Peralva, B. S.] Fed Univ Juiz De Fora UFJF, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao Del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; La Rosa Navarro, J. L.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, CP 20516, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lee, C. A.; Lissauer, D.; Liu, H.; Lynn, D.; Ma, H.; Maeno, T.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Xu, L.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. Transilvania Univ Brasov, Brasov, Romania. [Alexa, C.; Boldea, V.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Sola, J. D. Bossio; Marceca, G.; Otero Y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Brunt, Bh; Carter, J. R.; Chapman, J. D.; Cottin, G.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Potter, C. J.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Gillberg, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Gonzalez, B. Alvarez; Amoroso, S.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beermann, T. A.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Carrillo-Montoya, G. D.; Catinaccio, A.; Cattai, A.; Cerv, M.; Colombo, T.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feng, E. J.; Francis, D.; Fressard-Batraneanu, S. M.; Froidevaux, D.; Gadatsch, S.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Gumpert, C.; Hawkings, R. J.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huelsing, T. A.; Iengo, P.; Jakobsen, S.; Jenni, P.; Klioutchnikova, T.; Krasznahorkay, A.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Berlingen, J. Montejo; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Astigarraga, M. E. Pozo; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Ruthmann, N.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sforza, F.; Sanchez, C. A. Solans; Spigo, G.; Staerz, S.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Andeen, T.; Anderson, K. J.; Bryant, P.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Stark, G. H.; Swiatlowski, M.; Vukotic, I.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Blunier, S.; Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.] Pontificia Univ Catolica Chile, Dept Fis, Alameda 340, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Salazar Loyola, J. E.; Tapia Araya, S.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; da Costa, J. Barreiro Guimaraes; Fang, Y.; Jin, S.; Li, Q.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Geng, C.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y. L.; Liu, Y.; Peng, H.; Song, H. Y.; Zhang, G.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Du, Y.; Feng, C.; Liu, B.; Ma, L. L.; Wang, C.; Zaidan, R.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Shanghai Key Lab Particle Phys & Cosmol, Dept Phys & Astron, Shanghai 200030, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Alkire, S. P.; Angerami, A.; Brooijmans, G.; Carbone, R. M.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, Milan, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Gach, G. P.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Burka, K.; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Kowalewska, A. B.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Bessner, M.; Bloch, I.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Notkestr 85, Hamburg, Germany. [Asbah, N.; Bloch, I.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Zeuthen, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.; Schorlemmer, A. L. S.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Pino, S. A. Olivares; Proissl, M.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Arnold, H.; Bellerive, A.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schnoor, U.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; De Mendizabal, J. Bilbao; Calace, N.; Chatterjee, A.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; March, L.; Mermod, P.; Miucci, A.; Nackenhorst, O.; Nessi, M.; Paolozzi, L.; Ristic, B.; Schramm, S.; Sfyrla, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. 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Moreno; Musheghyan, H.; Nadal, J.; Quadt, A.; Rieger, J.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Berlendis, S.; Camincher, C.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Petit, E.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Chan, S. K.; Clark, B. L.; Franklin, M.; Giromini, P.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Rogan, C. S.; Skottowe, H. P.; Sun, S.; Tolley, E.; Tong, B.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, LV Kirensky Phys Inst, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolb, M.; Lisovyi, M.; Schaetzel, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Castillo, L. R. Flores; Lu, H.; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.; Orlando, N.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Kopeliansky, R.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Benitez, J.; Mallik, U.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Jiang, H.; Krumnack, N.; Pluth, D.; Prell, S.; Yu, J.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gongadze, A.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagai, R.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Unno, Y.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, A.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Bertram, I. A.; Borissov, G.; Bouhova-Thacker, E. V.; Cheatham, S.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Muenstermann, D.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Bachas, K.; Chiodini, G.; Gorini, E.; Longo, L.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Bachas, K.; Gorini, E.; Longo, L.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Armitage, L. J.; Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bell, A. S.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Leney, K. J. C.; Martyniuk, A. C.; McClymont, L. I.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Groh, S.; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Pleskot, V.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schmitz, S.; Schott, M.; Schuh, N.; Simion, S.; Simioni, E.; Simon, M.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Webb, S.; Wolf, A.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Barnes, S. L.; Bielski, R.; Cox, B. E.; Da Via, C.; Dann, N. S.; Forcolin, G. T.; Forti, A.; Ponce, J. M. Iturbe; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Sanchez, F. J. Munoz; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.; Zhang, R.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Hadef, A.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. 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C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hayden, D.; Huston, J.; Martin, B.; Mondragon, M. C.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Manzoni, S.; Mazza, S. M.; Meroni, C.; Monzani, S.; Perini, L.; Ragusa, F.; Ratti, M. G.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Manzoni, S.; Mazza, S. 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A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Heinrich, J. J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; La Rosa, A.; Macchiolo, A.; Maier, A. A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Kawade, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Mc Fadden, N. C.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Konig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Budker Inst Nucl Phys, SB RAS, Novosibirsk, Russia. [Becot, C.; Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Che, S.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Allen, B. W.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Radloff, P.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Abeloos, B.; Ayoub, M. K.; Bassalat, A.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Goudet, C. R.; Grivaz, J. -F.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Maiani, C.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, CNRS, Univ Paris Saclay, IN2P3,LAL, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, M. K.; Cameron, D.; Catmore, J. R.; Feigl, S.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Artoni, G.; Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Bortoletto, D.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Nagai, K.; Nickerson, R. B.; Petrov, M.; Pickering, M. A.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Di Clemente, W. K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Naryshkin, I.; Ryabov, Y. F.; Schegelsky, V. A.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Farina, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Gonalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Seabra, L. F. Oleiro; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Departamento Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Sopczak, A.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Solovyev, V.; Zaitsev, A. M.; Zenin, O.] NRC KI, State Res Ctr, Inst High Energy Phys Protvino, Gatchina, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Di Donato, C.; Falciano, S.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Di Domenico, A.; Di Donato, C.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Denysiuk, D.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Jeanneau, F.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Le Quilleuc, E. P.; Lesage, A. A. J.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Peyaud, A.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [AbouZeid, O. S.; Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Li, Y.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; Mori, T.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Gao, Y. S.; Garelli, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Su, D.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Kar, D.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Ughetto, M.; Santurio, E. Valdes; Wallangen, V.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.; Santurio, E. Valdes; Wallangen, V.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.; Winston, O. J.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Song, H. Y.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.; Zhang, G.] Acad Sinica, Inst Phys, Taipei 115, Taiwan. [Abreu, H.; Di Mattia, A.; Gozani, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Duarte-Campderros, J.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Pascuzzi, V.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Jovicevic, J.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Ito, F.; Kasahara, K.; Kim, S. 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A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Castillo Gimenez, V.; Alberich, L. Cerda; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Jimenez Pena, J.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Castillo Gimenez, V.; Alberich, L. Cerda; Costa, G.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. 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[Vest, A.] Flensburg Univ Appl Sci, Flensburg, Germany. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France.; Aad, G (reprint author), CNRS, IN2P3, Marseille, France. RI Guo, Jun/O-5202-2015; Gorelov, Igor/J-9010-2015; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; Villa, Mauro/C-9883-2009; La Rosa Navarro, Jose Luis/K-4221-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Smirnova, Oxana/A-4401-2013; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Vranjes Milosavljevic, Marija/F-9847-2016; Gladilin, Leonid/B-5226-2011; Chekulaev, Sergey/O-1145-2015; White, Ryan/E-2979-2015; Zhukov, Konstantin/M-6027-2015; SULIN, VLADIMIR/N-2793-2015; Snesarev, Andrey/H-5090-2013; Brooks, William/C-8636-2013; Nechaeva, Polina/N-1148-2015; Mashinistov, Ruslan/M-8356-2015; Vykydal, Zdenek/H-6426-2016; Fedin, Oleg/H-6753-2016; Boyko, Igor/J-3659-2013; Aguilar Saavedra, Juan Antonio/F-1256-2016; Mitsou, Vasiliki/D-1967-2009; Warburton, Andreas/N-8028-2013; Carvalho, Joao/M-4060-2013; Sanchez, Javier/F-5073-2016; Livan, Michele/D-7531-2012; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Tikhomirov, Vladimir/M-6194-2015; Doyle, Anthony/C-5889-2009; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Garcia, Jose /H-6339-2015; Conde Muino, Patricia/F-7696-2011; Stabile, Alberto/L-3419-2016; Coccaro, Andrea/P-5261-2016; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Gavrilenko, Igor/M-8260-2015; Di Domenico, Antonio/G-6301-2011; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017 OI Guo, Jun/0000-0001-8125-9433; Gorelov, Igor/0000-0001-5570-0133; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Villa, Mauro/0000-0002-9181-8048; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Smirnova, Oxana/0000-0003-2517-531X; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Gladilin, Leonid/0000-0001-9422-8636; White, Ryan/0000-0003-3589-5900; SULIN, VLADIMIR/0000-0003-3943-2495; Brooks, William/0000-0001-6161-3570; Mashinistov, Ruslan/0000-0001-7925-4676; Vykydal, Zdenek/0000-0003-2329-0672; Boyko, Igor/0000-0002-3355-4662; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Mitsou, Vasiliki/0000-0002-1533-8886; Warburton, Andreas/0000-0002-2298-7315; Carvalho, Joao/0000-0002-3015-7821; Livan, Michele/0000-0002-5877-0062; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Tikhomirov, Vladimir/0000-0002-9634-0581; Doyle, Anthony/0000-0001-6322-6195; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Pina, Joao /0000-0001-8959-5044; Veneziano, Stefano/0000-0002-2598-2659; Belanger-Champagne, Camille/0000-0003-2368-2617; Belyaev, Nikita/0000-0002-1131-7121; Conde Muino, Patricia/0000-0002-9187-7478; Stabile, Alberto/0000-0002-6868-8329; Coccaro, Andrea/0000-0003-2368-4559; Kukla, Romain/0000-0002-1140-2465; Di Domenico, Antonio/0000-0001-8078-2759; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, China; Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; the Royal Society, and Leverhulme Trust, United Kingdom. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK), and BNL (USA) and in the Tier-2 facilities worldwide. NR 50 TC 5 Z9 5 U1 18 U2 67 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 10 PY 2016 VL 116 IS 10 AR 101801 DI 10.1103/PhysRevLett.116.101801 PG 19 WC Physics, Multidisciplinary SC Physics GA DF9ZX UT WOS:000371722500003 PM 27015473 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T DeWolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Ochesanu, S Rougny, R Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van 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Duric, S. Friis, E. Gomber, B. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Lanaro, A. Levine, A. Long, K. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Ruggles, T. Sarangi, T. Savin, A. Sharma, A. Smith, N. Smith, W. H. Taylor, D. Woods, N. CA CMS Collaboration TI Transverse momentum spectra of inclusive b jets in pPb collisions atv root s(NN)=5.02 TeV SO PHYSICS LETTERS B LA English DT Article DE CMS; Physics; Heavy ions; b-tagging ID QUARK-GLUON PLASMA; COLLABORATION; PERSPECTIVE; DETECTOR AB We present a measurement of b jet transverse momentum (p(T)) spectra in proton-lead (pPb) collisions using a dataset corresponding to about 35nb(-1) collected with the CMS detector at the LHC. Jets from b quark fragmentation are found by exploiting the long lifetime of hadrons containing a b quark through tagging methods using distributions of the secondary vertex mass and displacement. Extracted cross sections for b jets are scaled by the effective number of nucleon-nucleon collisions and are compared to a reference obtained from PYTHIA simulations of pp collisions. The PYTHIA-based estimate of the nuclear modification factor is found to be 1.22 +/- 0.15 (stat + syst pPb) +/- 0.27 (syst PYTHIA) averaged over all jets with p(T) between 55 and 400 GeV/c and with |eta(lab)| < 2. We also compare this result to predictions from models using perturbative calculations in quantum chromodynamics. (C) 2016 CERN for the benefit of the CMS Collaboration. Published by Elsevier B.V. C1 [CMS Collaboration] CERN, CH-1211 Geneva 23, Switzerland. [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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S.; Junkes, A.; Klanner, R.; Kogler, R.; Lapsien, T.; Lenz, T.; Marchesini, I.; Marconi, D.; Meyer, M.; Nowatschin, D.; Ott, J.; Pantaleo, F.; Peiffer, T.; Perieanu, A.; Pietsch, N.; Poehlsen, J.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schwandt, J.; Seidel, M.; Sola, V.; Stadie, H.; Steinbrueck, G.; Tholen, H.; Troendle, D.; Usai, E.; Vanelderen, L.; Vanhoefer, A.; Vormwald, B.] Univ Hamburg, Hamburg, Germany. [Akbiyik, M.; Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Colombo, F.; De Boer, W.; Descroix, A.; Dierlamm, A.; Fink, S.; Frensch, F.; Giffels, M.; Gilbert, A.; Hartmann, F.; Heindl, S. M.; Husemann, U.; Katkov, I.; Kornmayer, A.; Pardo, P. Lobelle; Maier, B.; Mildner, H.; Mozer, M. U.; Mueller, T.; Mueller, Th.; Plagge, M.; Quast, G.; Rabbertz, K.; Roecker, S.; Roscher, F.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weber, M.; Weiler, T.; Woehrmann, C.; Wolf, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Tziaferi, E.] Univ Athens, Athens, Greece. [Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Loukas, N.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hazi, A.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.; Bartok, M.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Bartok, M.; Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Mal, P.; Mandal, K.; Sahoo, N.; Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Bansal, S.; Beri, S. B.; Bhatnagar, V.; Chawla, R.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, A.; Kaur, M.; Kumar, R.; Mehta, A.; Mittal, M.; Singh, J. B.; Walia, G.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Bhardwaj, A.; Choudhary, B. C.; Garg, R. B.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Nishu, N.; Ranjan, K.; Sharma, R.; Sharma, V.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dey, S.; Dutta, S.; Jain, Sa.; Majumdar, N.; Modak, A.; Mondal, K.; Mukherjee, S.; Mukhopadhyay, S.; Roy, A.; Roy, D.; Chowdhury, S. Roy; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Chudasama, R.; Dutta, D.; Jha, V.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Mahakud, B.; Maity, M.; Majumder, G.; Mazumdar, K.; Mitra, S.; Mohanty, G. B.; Parida, B.; Sarkar, T.; Sudhakar, K.; Sur, N.; Sutar, B.; Wickramage, N.] Tata Inst Fundamental Res, Homi Bhabha Rd, Bombay 400005, Maharashtra, India. [Chauhan, S.; Dube, S.; Sharma, S.] Indian Inst Sci Educ & Res, Pune, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Ranieri, A.; Selvaggi, G.; Silvestris, L.; Venditti, R.; Verwilligen, P.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Calabria, C.; Caputo, C.; Cristella, L.; De Palma, M.; Miniello, G.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Battilana, C.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.; Viliani, L.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.; Viliani, L.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.; Primavera, F.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Monge, M. R.; Tosi, S.] Univ Genoa, Genoa, Italy. [Brianza, L.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. 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T.; Passaseo, M.; Pazzini, J.; Pegoraro, M.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.; Kaminskiy, A.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Carlin, R.; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.; Kaminskiy, A.] Univ Padua, Padua, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Montagna, P.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Solestizi, L. Alunni; Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Solestizi, L. Alunni; Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Musich, M.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Daegu, South Korea. [Cifuentes, J. A. Brochero; Kim, H.; Kim, T. J.; Ryu, M. S.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Lee, S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, H.; Kim, J. H.; Lee, J. S. H.; Park, I. 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[Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Leonardo, N.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Bylinkin, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. 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Alcaraz; Calvo, E.; Cerrada, M.; Llatas, M. Chamizo; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; De Castro Manzano, P.; Duarte Campderros, J.; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Merlin, J. A.; Lingemann, J.; Pantaleo, F.; Hartmann, F.; Kornmayer, A.; Mohanty, A. K.; Battilana, C.; Marzocchi, B.; Meola, S.; Paolucci, P.; Azzi, P.; Dall'Osso, M.; Zucchetta, A.; Ciangottini, D.; Donato, S.; D'imperio, G.; Traczyk, P.; Arcidiacono, R.; Finco, L.; Candelise, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Duenser, M.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Zagozdzinska, A.; Zeuner, W. D.; Ulmer, K. A.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Buchmann, M. A.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Kumar, Arun; Bartek, R.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Tali, B.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Albayrak, E. A.; Guelmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-Storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Brew, C.; Brown, R. M.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Thomas, L.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Cripps, N.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Cutts, D.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Sinthuprasith, T.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Justus, C.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Hu, Z.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Kwan, S.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Weber, H. A.; Whitbeck, A.; Yang, F.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Di Giovanni, G. P.; Field, R. D.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Low, J. F.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Rossin, R.; Shchutska, L.; Snowball, M.; Sperka, D.; Terentyev, N.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.] Univ Illinois, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tan, P.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Osherson, M.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Sanders, S.; Stringer, R.; Wang, Q.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Baty, A.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Niu, X.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Trovato, M.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Lynch, S.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Pearson, T.; Planer, M.; Reinsvold, A.; Ruchti, R.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Ji, W.; Kotov, K.; Ling, T. Y.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.] Univ Puerto Rico, Mayaguez, PR USA. [Barnes, V. E.; Benedetti, D.; Bortoletto, D.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Li, W.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; De Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Hindrichs, O.; Khukhunaishvili, A.; Petrillo, G.; Verzetti, M.] Univ Rochester, Rochester, NY 14627 USA. [Demortier, L.] Rockefeller Univ, 1230 York Ave, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Hughes, E.; Kaplan, S.; Elayavalli, R. Kunnawalkam; Lath, A.; Nash, K.; Panwalkar, S.; Park, M.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Foerster, M.; Riley, G.; Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Hernandez, A. Castaneda; Dalchenko, M.; De Mattia, M.; Delgado, A.; Dildick, S.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Krutelyov, V.; Montalvo, R.; Mueller, R.; Osipenkov, I.; Pakhotin, Y.; Patel, R.; Perloff, A.; Roe, J.; Rose, A.; Safonov, A.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kunori, S.; Lamichhane, K.; Lee, S. W.; Libeiro, T.; Undleeb, S.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Janjam, R.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Ni, H.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.; Xu, Q.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Wolfe, E.; Wood, J.; Xia, F.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Christian, A.; Dasu, S.; Dodd, L.; Duric, S.; Friis, E.; Gomber, B.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Levine, A.; Long, K.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Ruggles, T.; Sarangi, T.; Savin, A.; Sharma, A.; Smith, N.; Smith, W. H.; Taylor, D.; Woods, N.] Univ Wisconsin, Madison, WI 53706 USA. [Fruehwirth, R.; Jeitler, M.; Krammer, M.; Schieck, J.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Popov, A.; Zhukov, V.; Katkov, I.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, SP, Brazil. [Moon, C. S.] CNRS, IN2P3, Paris, France. [Finger, M.; Finger, M., Jr.; Tsamalaidze, Z.] Joint Inst Nucl Res, Dubna, Russia. [Abdelalim, A. A.; Mahrous, A.] Helwan Univ, Cairo, Egypt. [Abdelalim, A. A.] Zewail City Sci & Technol, Zewail, Egypt. [Assran, Y.] Suez Univ, Suez, Egypt. [Awad, A.; Radi, A.] Ain Shams Univ, Cairo, Egypt. [Awad, A.; El Sawy, M.; Radi, A.] British Univ Egypt, Cairo, Egypt. [El Sawy, M.] Beni Suef Univ, Bani Suwayf, Egypt. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Hempel, M.; Karacheban, O.; Lohmann, W.; Marfin, I.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Bhowmik, S.; Maity, M.; Sarkar, T.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Plasma Phys Res Ctr, Sci & Res Branch, Tehran, Iran. [Androsov, K.; Ciocci, M. 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RI Puljak, Ivica/D-8917-2017; TUVE', Cristina/P-3933-2015; Flix, Josep/G-5414-2012; Ruiz, Alberto/E-4473-2011; Petrushanko, Sergey/D-6880-2012; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Moraes, Arthur/F-6478-2010; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; ciocci, maria agnese /I-2153-2015; Kirakosyan, Martin/N-2701-2015; Lokhtin, Igor/D-7004-2012; Manganote, Edmilson/K-8251-2013; Calvo Alamillo, Enrique/L-1203-2014; Matorras, Francisco/I-4983-2015; Hernandez Calama, Jose Maria/H-9127-2015; Cerrada, Marcos/J-6934-2014; Andreev, Vladimir/M-8665-2015; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Novaes, Sergio/D-3532-2012; VARDARLI, Fuat Ilkehan/B-6360-2013; Della Ricca, Giuseppe/B-6826-2013; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Colafranceschi, Stefano/M-1807-2016; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Calderon, Alicia/K-3658-2014; Goh, Junghwan/Q-3720-2016; Montanari, Alessandro/J-2420-2012; Azarkin, Maxim/N-2578-2015; Chinellato, Jose Augusto/I-7972-2012; Tomei, Thiago/E-7091-2012; Tinoco Mendes, Andre David/D-4314-2011; Varela, Joao/K-4829-2016; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Stahl, Achim/E-8846-2011 OI TUVE', Cristina/0000-0003-0739-3153; Flix, Josep/0000-0003-2688-8047; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Moraes, Arthur/0000-0002-5157-5686; Ogul, Hasan/0000-0002-5121-2893; ciocci, maria agnese /0000-0003-0002-5462; Calvo Alamillo, Enrique/0000-0002-1100-2963; Matorras, Francisco/0000-0003-4295-5668; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Cerrada, Marcos/0000-0003-0112-1691; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Montanari, Alessandro/0000-0003-2748-6373; Chinellato, Jose Augusto/0000-0002-3240-6270; Tomei, Thiago/0000-0002-1809-5226; Tinoco Mendes, Andre David/0000-0001-5854-7699; Varela, Joao/0000-0003-2613-3146; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Stahl, Achim/0000-0002-8369-7506 FU BMWFW (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN (China); CAS (China); MOST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia); ERC IUT (Estonia); ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP (Republic of Korea); NRF (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie programme; European Research Council and EPLANET (European Union); Leventis Foundation; Alfred P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture(FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS programme of the Foundation for Polish Science; European Union, Regional Development Fund; OPUS programme of the National Science Centre(Poland); Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR (Italy) [20108T4XTM]; Thalis and Aristeia programmes; EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); Welch Foundation [C-1845] FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MOST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP and NRF (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (USA).; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the Alfred P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture(FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS programme of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the OPUS programme of the National Science Centre(Poland); the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); and the Welch Foundation, contract C-1845. NR 43 TC 4 Z9 4 U1 22 U2 59 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD MAR 10 PY 2016 VL 754 BP 59 EP 80 DI 10.1016/j.physletb.2016.01.010 PG 22 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DD0HM UT WOS:000369601000011 ER PT J AU Adam, J Adamova, D Aggarwal, MM Rinella, GA Agnello, M Agrawal, N Ahammed, Z Ahn, SU Aiola, S Akindinov, A Alam, SN Aleksandrov, D Alessandro, B Alexandre, D Molina, RA Alici, A Alkin, A Almaraz, M Alme, J Alt, T Altinpinar, S Altsybeev, I Prado, CAG Andrei, C Andronic, A Anguelov, V Anielski, J Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arcelli, S Arnaldi, R Arnold, OW Arsene, IC Arslandok, M Audurier, B Augustinus, A Averbeck, R Azmi, MD Badala, A Baek, YW Bagnasco, S Bailhache, R Bala, R Baldisseri, A Baral, RC Barbano, AM Barbera, R Barile, F Barnafoeldi, GG Barnby, LS Barret, V Bartalini, P Barth, K Bartke, J Bartsch, E Basile, M Bastid, N Basu, S Bathen, B Batigne, G Camejo, AB Batyunya, B Batzing, PC Bearden, IG Beck, H Bedda, 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CA ALICE Collaboration TI Measurement of electrons from heavy-flavour hadron decays in p-Pb collisions at root s(NN)=5.02 TeV SO PHYSICS LETTERS B LA English DT Article ID QUARK-GLUON PLASMA; CHARGED-PARTICLE PRODUCTION; NUCLEUS-NUCLEUS COLLISIONS; LARGE TRANSVERSE-MOMENTUM; PROTON-PROTON COLLISIONS; PLUS AU COLLISIONS; ROOT-S=7 TEV; ROOT-S-NN=5.02 TEV; MESON PRODUCTION; NEUTRAL PION AB The production of electrons from heavy-flavour hadron decays was measured as a function of transverse momentum (p(T)) in minimum-bias p-Pb collisions at root s(NN) = 5.02 TeV using the ALICE detector at the LHC. The measurement covers the p(T) interval 0.5 < p(T) < 12 GeV/c and the rapidity range -1.065 < y(cms) < 0.135 in the centre-of-mass reference frame. The contribution of electrons from background sources was subtracted using an invariant mass approach. The nuclear modification factor R-pPb was calculated by comparing the p(T)-differential invariant cross section in p-Pb collisions to a pp reference at the same centre-of-mass energy, which was obtained by interpolating measurements at root s = 2.76 TeV and root s= 7 TeV. The R-pPb is consistent with unity within uncertainties of about 25%, which become larger for p(T) below 1 GeV/c. The measurement shows that heavy-flavour production is consistent with binary scaling, so that a suppression in the high-p(T) yield in Pb-Pb collisions has to be attributed to effects induced by the hot medium produced in the final state. The data in p-Pb collisions are described by recent model calculations that include cold nuclear matter effects. (C) 2015 CERN for the benefit of the ALICE Collaboration. Published by Elsevier B.V. C1 [Grigoryan, A.; Papikyan, V.] Yerevan Phys Inst, AI Alikhanyan Natl Sci Lab, Yerevan 375036, Armenia. [Martinez, M. I.; Moreno, L. A. P.; Noris, J. C. 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RI Vechernin, Vladimir/J-5832-2013; De Pasquale, Salvatore/B-9165-2008; Akindinov, Alexander/J-2674-2016; Chinellato, David/D-3092-2012; Takahashi, Jun/B-2946-2012; Pshenichnov, Igor/A-4063-2008; Bregant, Marco/I-7663-2012; Sevcenco, Adrian/C-1832-2012; de Cuveland, Jan/H-6454-2016; Kurepin, Alexey/H-4852-2013; Jena, Deepika/P-2873-2015; Jena, Satyajit/P-2409-2015; Natal da Luz, Hugo/F-6460-2013; Martinez Hernandez, Mario Ivan/F-4083-2010; Ferretti, Alessandro/F-4856-2013; Kovalenko, Vladimir/C-5709-2013; Altsybeev, Igor/K-6687-2013; Vickovic, Linda/F-3517-2017; Fernandez Tellez, Arturo/E-9700-2017; Nattrass, Christine/J-6752-2016; Usai, Gianluca/E-9604-2015; Cosentino, Mauro/L-2418-2014; Suaide, Alexandre/L-6239-2016; Barnby, Lee/G-2135-2010; Peitzmann, Thomas/K-2206-2012; Kondratiev, Valery/J-8574-2013; Vinogradov, Leonid/K-3047-2013; Castillo Castellanos, Javier/G-8915-2013; Ferreiro, Elena/C-3797-2017 OI Vechernin, Vladimir/0000-0003-1458-8055; De Pasquale, Salvatore/0000-0001-9236-0748; Akindinov, Alexander/0000-0002-7388-3022; Chinellato, David/0000-0002-9982-9577; Takahashi, Jun/0000-0002-4091-1779; Pshenichnov, Igor/0000-0003-1752-4524; Sevcenco, Adrian/0000-0002-4151-1056; de Cuveland, Jan/0000-0003-0455-1398; Kurepin, Alexey/0000-0002-1851-4136; Jena, Deepika/0000-0003-2112-0311; Jena, Satyajit/0000-0002-6220-6982; Natal da Luz, Hugo/0000-0003-1177-870X; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Ferretti, Alessandro/0000-0001-9084-5784; Kovalenko, Vladimir/0000-0001-6012-6615; Altsybeev, Igor/0000-0002-8079-7026; Vickovic, Linda/0000-0002-9820-7960; Fernandez Tellez, Arturo/0000-0003-0152-4220; Riggi, Francesco/0000-0002-0030-8377; Scarlassara, Fernando/0000-0002-4663-8216; Nattrass, Christine/0000-0002-8768-6468; Usai, Gianluca/0000-0002-8659-8378; Cosentino, Mauro/0000-0002-7880-8611; Suaide, Alexandre/0000-0003-2847-6556; Barnby, Lee/0000-0001-7357-9904; Peitzmann, Thomas/0000-0002-7116-899X; Kondratiev, Valery/0000-0002-0031-0741; Vinogradov, Leonid/0000-0001-9247-6230; Castillo Castellanos, Javier/0000-0002-5187-2779; Ferreiro, Elena/0000-0002-4449-2356 FU Grid centres; Worldwide LHC Computing Grid (WLCG) Collaboration; ALICE detector: State Committee of Science, Armenia; Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics; Academy of Finland; French CNRS-IN2P3; 'Region Pays de Loire', France; German Bundesministerium fur Bildung, Wissenschaft, Forschung und Technologie (BMBF); Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian Orszagos Tudomanyos Kutatasi Alappgrammok (OTKA); National Office for Research and Technology (NKTH); Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) Italy; MEXT, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT); Direccion General de Asuntos del Personal Academico (DGAPA), Mexico; Amerique Latine Formation academique - European Commission (ALFA-EC); EPLANET Program(European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM); Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics and National Council of Scientific Research in Higher Education(CNCSI-UEFISCDI), Romania; Ministry of Education and Science of Russian Federation; Russian Academy of Sciences; Russian Federal Agency of Atomic Energy; Russian Federal Agency for Science and Innovations; Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, Republic of South Africa, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT); Europe and Latin America (EELA); Ministerio de Economia y Competitividad (MINECO) of Spain; Xunta de Galicia (Conselleria de Educacion); Centro de Aplicaciones Tecnologicas y Desarrollo Nuclear (CEADEN); Cubaenergia, Cuba; IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); United States Department of Energy; United States National Science Foundation; State of Texas; State of Ohio; Ministry of Science, Education and Sports of Croatia and Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India; Pontificia Universidad Catolica del Peru; World Federation of Scientists (WFS), Armenia; Youth of the Czech Republic; 'Region Alsace', France; 'Region Auvergne', France; CEA, France; Centro Fermi - Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy FX `The ALICE Collaboration would like to thank all its engineers and technicians for their invaluable contributions to the construction of the experiment and the CERN accelerator teams for the outstanding performance of the LHC complex. The ALICE Collaboration gratefully acknowledges the resources and support provided by all Grid centres and the Worldwide LHC Computing Grid (WLCG) Collaboration.; The ALICE Collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector: State Committee of Science, World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE) and the Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council, the Carlsberg Foundation and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics and the Academy of Finland; French CNRS-IN2P3, the 'Region Pays de Loire', 'Region Alsace', 'Region Auvergne' and CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung und Technologie (BMBF) and the Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian Orszagos Tudomanyos Kutatasi Alappgrammok (OTKA) and National Office for Research and Technology (NKTH); Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi - Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; MEXT Grant-in-Aid for Specially Promoted Research, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT), Direccion General de Asuntos del Personal Academico (DGAPA), Mexico, Amerique Latine Formation academique - European Commission (ALFA-EC) and the EPLANET Program(European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics and National Council of Scientific Research in Higher Education(CNCSI-UEFISCDI), Romania; Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations and The Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, Republic of South Africa, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT), E-Infrastructure shared between Europe and Latin America (EELA), Ministerio de Economia y Competitividad (MINECO) of Spain, Xunta de Galicia (Conselleria de Educacion), Centro de Aplicaciones Tecnologicas y Desarrollo Nuclear (CEADEN), Cubaenergia, Cuba, and IAEA (International Atomic Energy Agency); Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); The United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio; Ministry of Science, Education and Sports of Croatia and Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India; Pontificia Universidad Catolica del Peru. NR 80 TC 2 Z9 2 U1 8 U2 36 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD MAR 10 PY 2016 VL 754 BP 81 EP 93 DI 10.1016/j.physletb.2015.12.067 PG 13 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DD0HM UT WOS:000369601000012 ER PT J AU Harigaya, K Nomura, Y AF Harigaya, Keisuke Nomura, Yasunori TI Composite models for the 750GeV diphoton excess SO PHYSICS LETTERS B LA English DT Article AB We present composite models explaining the diphoton excess of mass around 750GeV recently reported by the LHC experiments. (C) 2016 The Authors. Published by Elsevier B.V. C1 [Harigaya, Keisuke; Nomura, Yasunori] Univ Calif Berkeley, Dept Phys, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. [Harigaya, Keisuke; Nomura, Yasunori] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. RP Harigaya, K (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. EM keisukeharigaya@berkeley.edu OI Nomura, Yasunori/0000-0002-1497-1479 FU Director, Office of Science, Office of High Energy and Nuclear Physics, of the U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [PHY-1316783, PHY-1521446]; MEXT KAKENHI [15H05895] FX We would like to thank Lawrence Hall, Tongyan Lin, Hou Keong Lou, Michele Papucci, Alex Pomarol, Surjeet Rajendran, and Kathryn Zurek for discussions. This work was supported in part by the Director, Office of Science, Office of High Energy and Nuclear Physics, of the U.S. Department of Energy under Contract DE-AC02-05CH11231, by the National Science Foundation under grants PHY-1316783 and PHY-1521446, and by MEXT KAKENHI Grant Number 15H05895. NR 24 TC 116 Z9 116 U1 2 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD MAR 10 PY 2016 VL 754 BP 151 EP 156 DI 10.1016/j.physletb.2016.01.026 PG 6 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DD0HM UT WOS:000369601000024 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Aring;kesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T 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Wiglesworth, C. Wiik-Fuchs, L. A. M. Wildauer, A. Wilkens, H. G. Williams, H. H. Williams, S. Willis, C. Willocq, S. Wilson, A. Wilson, J. A. Wingerter-Seez, I. Winklmeier, F. Winter, B. T. Wittgen, M. Wittkowski, J. Wollstadt, S. J. Wolter, M. W. Wolters, H. Wosiek, B. K. Wotschack, J. Woudstra, M. J. Wozniak, K. W. Wu, M. Wu, M. Wu, S. L. Wu, X. Wu, Y. Wyatt, T. R. Wynne, B. M. Xella, S. Xu, D. Xu, L. Yabsley, B. Yacoob, S. Yakabe, R. Yamada, M. Yamaguchi, D. Yamaguchi, Y. Yamamoto, A. Yamamoto, S. Yamanaka, T. Yamauchi, K. Yamazaki, Y. Yan, Z. Yang, H. Yang, H. Yang, Y. Yao, W-M. Yap, Y. C. Yasu, Y. Yatsenko, E. Wong, K. H. Yau Ye, J. Ye, S. Yeletskikh, I. Yen, A. L. Yildirim, E. Yorita, K. Yoshida, R. Yoshihara, K. Young, C. Young, C. J. S. Youssef, S. Yu, D. R. Yu, J. Yu, J. M. Yu, J. Yuan, L. Yuen, S. P. Y. Yurkewicz, A. Yusuff, I. Zabinski, B. Zaidan, R. Zaitsev, A. M. Zalieckas, J. Zaman, A. Zambito, S. Zanello, L. Zanzi, D. Zeitnitz, C. Zeman, M. Zemla, A. Zeng, Q. Zengel, K. Zenin, O. Zenis, T. Zerwas, D. Zhang, D. Zhang, F. Zhang, G. Zhang, H. Zhang, J. Zhang, L. Zhang, R. Zhang, X. Zhang, Z. Zhao, X. Zhao, Y. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Dijet production in root s=7 TeV pp collisions with large rapidity gaps at the ATLAS experiment SO PHYSICS LETTERS B LA English DT Article ID DEEP-INELASTIC SCATTERING; CROSS-SECTION; QCD ANALYSIS; HERA; DIFFRACTION; FACTORIZATION; HERWIG AB A 6.8 nb(-1) sample of pp collision data collected under low-luminosity conditions at root s = 7 TeV by the ATLAS detector at the Large Hadron Collider is used to study diffractive dijet production. Events containing at least two jets with p(T) > 20 GeV are selected and analysed in terms of variables which discriminate between diffractive and non-diffractive processes. Cross sections are measured differentially in Delta eta(F), the size of the observable forward region of pseudorapidity which is devoid of hadronic activity, and in an estimator, (xi) over tilde, of the fractional momentum loss of the proton assuming single diffractive dissociation (pp -> pX). Model comparisons indicate a dominant non-diffractive contribution up to moderately large Delta eta(F) and small (xi) over tilde, with a diffractive contribution which is significant at the highest Delta eta(F) and the lowest (xi) over tilde. The rapidity-gap survival probability is estimated from comparisons of the data in this latter region with predictions based on diffractive parton distribution functions. (C) 2016 CERN for the benefit of the ATLAS Collaboration. Published by Elsevier B.V. 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T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Lacey, J.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Schneider, B.; Tarrade, F.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Gonzalez, B. Alvarez; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beermann, T. A.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Carrillo-Montoya, G. D.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Feng, E. J.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Gadatsch, S.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jaekel, M. R.; Jakobsen, S.; Klioutchnikova, T.; Krasznahorkay, A.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Ruthmann, N.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sforza, F.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Toro, R. Camacho; Cheng, Y.; Chisholm, A. S.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Schaffer, A. C.; Schneider, B.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Blunier, S.; Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Alameda 340, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Loyola, J. E. Salazar; Schneider, B.; Araya, S. Tapia; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Schneider, B.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Schneider, B.; Song, H. Y.; Zhang, G.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chisholm, A. S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Schaffer, A. C.; Schneider, B.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Schneider, B.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS IN2P3, Clermont Ferrand, France. [Altheimer, A.; Angerami, A.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Nikiforou, N.; Ochoa, I.; Parsons, J. A.; Schneider, B.; Smith, M. N. K.; Thompson, E. N.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Loevschall-Jensen, A. E.; Monk, J.; Pedersen, L. E.; Pingel, A.; Wiglesworth, C.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] INFN Grp Collegato Cosenza, Lab Nazl Frascati, Arcavacata Di Rende, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Wang, H.; Ye, J.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Notkestr 85, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Schneider, B.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] INFN Lab Nazl Frascati, Frascati, Italy. [Arnold, H.; Betancourt, C.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Di Simone, A.; Herten, G.; Kiss, F.; Kopp, A. K.; Luedtke, C.; Ruehr, F.; Sammel, D.; Schillo, C.; Sundermann, J. E.; Ta, D.; Ungaro, F. C.; von Radziewski, H.; Weiser, C.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Clark, A.; Coccaro, A.; Delitzsch, C. M.; Katre, A.; Miucci, A.; Picazio, A.; Ristic, B.; Tykhonov, A.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] INFN Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Britton, D.; Buckley, A. G.; Buttar, C. M.; Buzatu, A.; Cinca, D.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Knue, A.; Morton, A.; Barrera, C. Oropeza; Pollard, C. S.; Qin, G.; Quilty, D.; Robson, A.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Brandt, G.; Drechsler, E.; Grosse-Knetter, J.; Kawamura, G.; Lemmer, B.; Magradze, E.; Mchedlidze, G.; Musheghyan, H.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Meier, K.; Theenhausen, H. Meyer Zu; Villara, D. I. Narrias; Sahinsoy, M.; Schultz-Coulon, H. -C.; Stamena, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolb, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Castillo, L. R. Flores; Lu, H.; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Jussel, P.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Schneider, B.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] Natl Lab High Energy Phys, KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki 305, Japan. [Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Univ Salento, INFN Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] UPMC, Phys Theor & Hautes Energies Lab, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Ventura, D.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Hu, X.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Tollefson, K.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Univ Milan, INFN Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Bernius, C.; Biebel, O.; Bock, C.; Bortfeldt, J.; Brandt, A.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Univ Naples Federico II, INFN Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartmento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Koenig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Endo, M.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Univ Pavia, INFN Sez Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, INFN Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Amorim, A.; Galhardo, B.; Gomes, A.; Maio, A.; Onofre, A.; Palma, A.; Delgado, A. Tavares] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dep Fis, P-1200 Lisbon, Portugal. Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, P-1200 Lisbon, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] NRC KI, State Res Ctr, Inst High Energy Phys Protvino, Moscow, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapettia, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Sapienza Univ Roma, INFN Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapettia, G.; Di Domenico, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Sapienza Univ Roma, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, INFN Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Univ Rome Tre, INFN Sez Roma Tre, I-00146 Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Techn Nucl, Rabat, Morocco. [El Kacimi, M.; Fassi, F.; Goujdami, D.] Univ Cadi Ayyad, LPHEA, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, IRFU, DSM, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Hance, M.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Plazak, L.; Sykoraa, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urbanb, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Lee, C. A.; Meehan, S.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Kar, D.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Jovicevic, J.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Guest, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] Sez Trieste, INFN Grp Coll Udine, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Cobal, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Gradin, P. O. J.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, IFIC, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, CNM, IMB, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; Gignac, M.; Henkelmann, S.; King, S. B.; Lister, A.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; Le Blanc, M.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Pearce, J.; Sobie, R.; Trovatelli, M.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.; Spangenberg, M.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kaplan, L. S.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Braun, H. M.; Cornelissen, T.; Ellinghaus, F.; Ernis, G.; Fischer, J.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Schneider, B.; Thomsen, L. A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Ctr Calcul Inst Natl Phys Nucl & Phys Particules, Villeurbanne, France. [Acharya, B. 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[Chen, L.; Zhang, R.] CNRS, IN2P3, Marseille, France. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] IPP, Toronto, ON, Canada. [Davies, E.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Barcelona, Spain. [Guo, Y.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Hanagaki, K.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu 30013, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Hsu, P. J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Jenni, P.] CERN, Geneva, Switzerland. [Khubua, J.] GTU, Tbilisi, Rep of Georgia. 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[Toth, J.] Wigner Res Ctr Phys, Inst Nucl & Particle Phys, Budapest, Hungary. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France.; Aad, G (reprint author), CNRS, IN2P3, Marseille, France. RI Vranjes Milosavljevic, Marija/F-9847-2016; Gladilin, Leonid/B-5226-2011; Chekulaev, Sergey/O-1145-2015; White, Ryan/E-2979-2015; Zhukov, Konstantin/M-6027-2015; SULIN, VLADIMIR/N-2793-2015; Snesarev, Andrey/H-5090-2013; Brooks, William/C-8636-2013; Nechaeva, Polina/N-1148-2015; Mashinistov, Ruslan/M-8356-2015; Vykydal, Zdenek/H-6426-2016; Fedin, Oleg/H-6753-2016; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Conde Muino, Patricia/F-7696-2011; Stabile, Alberto/L-3419-2016; Coccaro, Andrea/P-5261-2016; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Di Domenico, Antonio/G-6301-2011; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Carvalho, Joao/M-4060-2013; Guo, Jun/O-5202-2015; Sanchez, Javier/F-5073-2016; Livan, Michele/D-7531-2012; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Tikhomirov, Vladimir/M-6194-2015; Doyle, Anthony/C-5889-2009; Boyko, Igor/J-3659-2013; Aguilar Saavedra, Juan Antonio/F-1256-2016; Warburton, Andreas/N-8028-2013; Mitsou, Vasiliki/D-1967-2009; Gorelov, Igor/J-9010-2015; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; Villa, Mauro/C-9883-2009; BESSON, NATHALIE/L-6250-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Smirnova, Oxana/A-4401-2013; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012 OI Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Gladilin, Leonid/0000-0001-9422-8636; White, Ryan/0000-0003-3589-5900; SULIN, VLADIMIR/0000-0003-3943-2495; Brooks, William/0000-0001-6161-3570; Mashinistov, Ruslan/0000-0001-7925-4676; Vykydal, Zdenek/0000-0003-2329-0672; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; KUBOTA, TAKASHI/0000-0002-1156-5571; Conde Muino, Patricia/0000-0002-9187-7478; Stabile, Alberto/0000-0002-6868-8329; Coccaro, Andrea/0000-0003-2368-4559; Kukla, Romain/0000-0002-1140-2465; Goncalo, Ricardo/0000-0002-3826-3442; Di Domenico, Antonio/0000-0001-8078-2759; Gauzzi, Paolo/0000-0003-4841-5822; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Carvalho, Joao/0000-0002-3015-7821; Guo, Jun/0000-0001-8125-9433; Livan, Michele/0000-0002-5877-0062; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Tikhomirov, Vladimir/0000-0002-9634-0581; Doyle, Anthony/0000-0001-6322-6195; Boyko, Igor/0000-0002-3355-4662; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Warburton, Andreas/0000-0002-2298-7315; Mitsou, Vasiliki/0000-0002-1533-8886; Gorelov, Igor/0000-0001-5570-0133; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Villa, Mauro/0000-0002-9181-8048; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Smirnova, Oxana/0000-0003-2517-531X; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, China; Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF, Canada; Canada Council, Canada; CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET, European Union; ERC, European Union; FP7, European Union; Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, France; ANR, France; Region Auvergne and Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos program; Thales program; Aristeia program; EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. NR 50 TC 5 Z9 5 U1 15 U2 50 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD MAR 10 PY 2016 VL 754 BP 214 EP 234 DI 10.1016/j.physletb.2016.01.028 PG 21 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DD0HM UT WOS:000369601000034 ER PT J AU Adam, J Adamova, D Aggarwal, MM Rinella, GA Agnello, M Agrawal, N Ahammed, Z Ahn, SU Aiola, S Akindinov, A Alam, SN Aleksandrov, D Alessandro, B Alexandre, D Molina, RA Alici, A Alkin, A Almaraz, JRM Alme, J Alt, T Altinpinar, S Altsybeev, I Prado, CAG Andrei, C Andronic, A Anguelov, V Anielski, J Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arcelli, S Arnaldi, R Arnold, OW Arsene, IC Arslandok, M Audurier, B Augustinus, A Averbeck, R Awes, TC Azmi, MD Badala, A Baek, YW Bagnasco, S Bailhache, R Bala, R Baldisseri, A Baral, RC Barbano, AM Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartalini, P Barth, K Bartke, J Bartsch, E Basile, M Bastid, N Basu, S Bathen, B Batigne, G Camejo, AB Batyunya, B Batzing, PC Bearden, IG Beck, H Bedda, C Behera, NK Belikov, I Bellini, F Martinez, HB Bellwied, R Belmont, R Belmont-Moreno, E Belyaev, V Bencedi, G Beole, S Berceanu, I Bercuci, A Berdnikov, Y Berenyi, D Bertens, RA Berzano, D Betev, L Bhasin, A Bhat, IR Bhati, AK Bhattacharjee, B Bhom, J Bianchi, L Bianchi, N Bianchin, C Bielcik, J Bielcikova, J Bilandzic, A Biswas, R Biswas, S Bjelogrlic, S Blair, JT Blau, D Blume, C Bock, F Bogdanov, A Boggild, H Boldizsar, L Bombara, M Book, J Borel, H Borissov, A Borri, M Bossu, F Botta, E Bottger, S Bourjau, C Braun-Munzinger, P Bregant, M Breitner, T Broker, TA Browning, TA Broz, M Brucken, EJ Bruna, E Bruno, GE Budnikov, D Buesching, H Bufalino, S Buncic, P Busch, O Buthelezi, Z Butt, JB Buxton, JT Caffarri, D Cai, X Caines, H Diaz, LC Caliva, A Villar, EC Camerini, P Carena, F Carena, W Carnesecchi, F Castellanos, JC Castro, AJ Casula, EAR Sanchez, CC Cepila, J Cerello, P Cerkala, J Chang, B Chapeland, S Chartier, M Charvet, JL Chattopadhyay, S Chattopadhyay, S Chelnokov, V Cherney, M Cheshkov, C Cheynis, B Barroso, VC Chinellato, DD Cho, S Chochula, P Choi, K Chojnacki, M Choudhury, S Christakoglou, P Christensen, CH Christiansen, P Chujo, T Chung, SU Cicalo, C Cifarelli, L Cindolo, F Cleymans, J Colamaria, F Colella, D Collu, A Colocci, M Balbastre, GC Del Valle, ZC Connors, ME Contreras, JG Cormier, TM Morales, YC Maldonado, IC Cortese, P Cosentino, MR Costa, F Crochet, P Albino, RC Cuautle, E Cunqueiro, L Dahms, T Dainese, A Danu, A Das, D Das, I Das, S Dash, A Dash, S De, S De Caro, A De Cataldo, G De Conti, C De Cuveland, J De Falco, A De Gruttola, D De Marco, N De Pasquale, S Deisting, A Deloff, A Denes, E Deplano, C Dhankher, P Di Bari, D Di Mauro, A Di Nezza, P Corchero, MAD Dietel, T Dillenseger, P Divia, R Djuvsland, O Dobrin, A Gimenez, DD Donigus, B Dordic, O Drozhzhova, T Dubey, AK Dubla, A Ducroux, L Dupieux, P Ehlers, RJ Elia, D Engel, H Epple, E Erazmus, B Erdemir, I Erhardt, F Espagnon, B Estienne, M Esumi, S Eum, J Evans, D Evdokimov, S Eyyubova, G Fabbietti, L Fabris, D Faivre, J Fantoni, A Fasel, M Feldkamp, L Feliciello, A Feofilov, G Ferencei, J Tellez, AF Ferreiro, EG Ferretti, A Festanti, A Feuillard, VJG Figiel, J Figueredo, MAS Filchagin, S Finogeev, D Fionda, FM Fiore, EM Fleck, MG Floris, M Foertsch, S Foka, P Fokin, S Fragiacomo, E Francescon, A Frankenfeld, U Fuchs, U Furget, C Furs, A Girard, MF Gaardhoje, JJ Gagliardi, M Gago, AM Gallio, M Gangadharan, DR Ganoti, P Gao, C Garabatos, C Garcia-Solis, E Gargiulo, C Gasik, P Gauger, EF Germain, M Gheata, A Gheata, M Ghosh, P Ghosh, SK Gianotti, P Giubellino, P Giubilato, P Gladysz-Dziadus, E Glassel, P Coral, DMG Ramirez, AG Gonzalez, V Gonzalez-Zamora, P Gorbunov, S Gorlich, L Gotovac, S Grabski, V Grachov, OA Graczykowski, LK Graham, KL Grelli, A Grigoras, A Grigoras, C Grigoriev, V Grigoryan, A Grigoryan, S Grinyov, B Grion, N Gronefeld, JM Grosse-Oetringhaus, JF Grossiord, JY Grosso, R Guber, F Guernane, R Guerzoni, B Gulbrandsen, K Gunji, T Gupta, A Gupta, R Haake, R Haaland, O Hadjidakis, C Haiduc, M Hamagaki, H Hamar, G Harris, JW Harton, A Hatzifotiadou, D Hayashi, S Heckel, ST Heide, M Helstrup, H Herghelegiu, A Corral, GH Hess, BA Hetland, KF Hillemanns, H Hippolyte, B Hosokawa, R Hristov, P Huang, M Humanic, TJ Hussain, N Hussain, T Hutter, D Hwang, DS Ilkaev, R Inaba, M Ippolitov, M Irfan, M Ivanov, M Ivanov, V Izucheev, V Jacobs, PM Jadhav, MB Jadlovska, S Jadlovsky, J Jahnke, C Jakubowska, MJ Jang, HJ Janik, MA Jayarathna, PHSY Jena, C Jena, S Bustamante, RTJ Jones, PG Jung, H Jusko, A Kalinak, P Kalweit, A Kamin, J Kang, JH Kaplin, V Kar, S Uysal, AK Karavichev, O Karavicheva, T Karayan, L Karpechev, E Kebschull, U Keidel, R Keijdener, DLD Keil, M Khan, MM Khan, P Khan, SA Khanzadeev, A Kharlov, Y Kileng, B Kim, DW Kim, DJ Kim, D Kim, H Kim, JS Kim, M Kim, M Kim, S Kim, T Kirsch, S Kisel, I Kiselev, S Kisiel, A Kiss, G Klay, JL Klein, C Klein, J Klein-Bosing, C Klewin, S Kluge, A Knichel, ML Knospe, AG Kobayashi, T Kobdaj, C Kofarago, M Kollegger, T Kolojvari, A Kondratiev, V Kondratyeva, N Kondratyuk, E Konevskikh, A Kopcik, M Kour, M Kouzinopoulos, C Kovalenko, O Kovalenko, V Kowalski, M Meethaleveedu, GK Kralik, I Kravcakova, A Kretz, M Krivda, M Krizek, F Kryshen, E Krzewicki, M Kubera, AM Kucera, V Kuhn, C Kuijer, PG Kumar, A Kumar, J Kumar, L Kumar, S Kurashvili, P Kurepin, A Kurepin, AB Kuryakin, A Kweon, MJ Kwon, Y LaPointe, SL La Rocca, P De Guevara, PL Fernandes, CL Lakomov, I Langoy, R Lara, C Lardeux, A Lattuca, A Laudi, E Lea, R Leardini, L Lee, GR Lee, S Lehas, F Lemmon, RC Lenti, V Leogrande, E Monzon, IL Vargas, HL Leoncino, M Levai, P Li, S Li, X Lien, J Lietava, R Lindal, S Lindenstruth, V Lippmann, C Lisa, MA Ljunggren, HM Lodato, DF Loenne, PI Loginov, V Loizides, C Lopez, X Torres, EL Lowe, A Luettig, P Lunardon, M Luparello, G Maevskaya, A Mager, M Mahajan, S Mahmood, SM Maire, A Majka, RD Malaev, M Cervantes, IM Malinina, L Mal'Kevich, D Malzacher, P Mamonov, A Manko, V Manso, F Manzari, V Marchisone, M Mares, J Margagliotti, GV Margotti, A Margutti, J Marin, A Markert, C Marquard, M Martin, NA Blanco, JM Martinengo, P Martinez, MI Garcia, GM Pedreira, MM Mas, A Masciocchi, S Masera, M Masoni, A Massacrier, L Mastroserio, A Matyja, A Mayer, C Mazer, J Mazzoni, MA Mcdonald, D Meddi, F Melikyan, Y Menchaca-Rocha, A Meninno, E Perez, JM Meres, M Miake, Y Mieskolainen, MM Mikhaylov, K Milano, L Milosevic, J Minervini, LM Mischke, A Mishra, AN Miskowiec, D Mitra, J Mitu, CM Mohammadi, N Mohanty, B Molnar, L Zetina, LM Montes, E De Godoy, DAM Moreno, LAP Moretto, S Morreale, A Morsch, A Muccifora, V Mudnic, E Muhlheim, D Muhuri, S Mukherjee, M Mulligan, JD Munhoz, MG Munzer, RH Murray, S Musa, L Musinsky, J Naik, B Nair, R Nandi, BK Nania, R Nappi, E Naru, MU Da Luz, HN Nattrass, C Nayak, K Nayak, TK Nazarenko, S Nedosekin, A Nellen, L Ng, F Nicassio, M Niculescu, M Niedziela, J Nielsen, BS Nikolaev, S Nikulin, S Nikulin, V Noferini, F Nomokonov, P Nooren, G Noris, JCC Norman, J Nyanin, A Nystrand, J Oeschler, H Oh, S Oh, SK Ohlson, A Okatan, A Okubo, T Olah, L Oleniacz, J Da Silva, ACO Oliver, MH Onderwaater, J Oppedisano, C Orava, R Velasquez, AO Oskarsson, A Otwinowski, J Oyama, K Ozdemir, M Pachmayer, Y Pagano, P Paic, G Pal, SK Pan, J Pandey, AK Papcun, P Papikyan, V Pappalardo, GS Pareek, P Park, WJ Parmar, S Passfeld, A Paticchio, V Patra, RN Paul, B Peitzmann, T Da Costa, HP De Oliveira, EP Peresunko, D Lara, CEP Lezama, EP Peskov, V Pestov, Y Petracek, V Petrov, V Petrovici, M Petta, C Piano, S Pikna, M Pillot, P Pinazza, O Pinsky, L Piyarathna, DB Ploskon, M Planinic, M Pluta, J Pochybova, S Podesta-Lerma, PLM Poghosyan, MG Polichtchouk, B Poljak, N Poonsawat, W Pop, A Porteboeuf-Houssais, S Porter, J Pospisil, J Prasad, SK Preghenella, R Prino, F Pruneau, CA Pshenichnov, I Puccio, M Puddu, G Pujahari, P Punin, V Putschke, J Qvigstad, H Rachevski, A Raha, S Rajput, S Rak, J Rakotozafindrabe, A Ramello, L Rami, F 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CA ALICE Collaboration TI Direct photon production in Pb-Pb collisions at root s(NN)=2.76 TeV SO PHYSICS LETTERS B LA English DT Article ID QUARK-GLUON PLASMA; NUCLEUS-NUCLEUS COLLISIONS; EQUATION-OF-STATE; TRANSVERSE-MOMENTUM; THERMAL PHOTONS; LEADING ORDER; NEUTRAL PION; FRAGMENTATION; COLLABORATION; PERSPECTIVE AB Direct photon production at mid-rapidity in Pb-Pb collisions at root s(NN) = 2.76 TeV was studied in the transverse momentum range 0.9 < p(T) < 14 GeV/c. Photons were detected with the highly segmented electromagnetic calorimeter PHOS and via conversions in the ALICE detector material with the e(+)e(-) pair reconstructed in the central tracking system. The results of the two methods were combined and direct photon spectra were measured for the 0-20%, 20-40%, and 40-80% centrality classes. For all three classes, agreement was found with perturbative QCD calculations for p(T) greater than or similar to 5 GeV/c. Direct photon spectra down to p(T) approximate to 1 GeV/c could be extracted for the 20-40% and 0-20% centrality classes. The significance of the direct photon signal for 0.9 < p(T) < 2.1 GeV/c is 2.6 sigma for the 0-20% class. The spectrum in this p(T) range and centrality class can be described by an exponential with an inverse slope parameter of (297 +/- 12(stat) +/- 41(syst)) MeV. State-of-the-art models for photon production in heavy-ion collisions agree with the data within uncertainties. (C) 2016 CERN for the benefit of the ALICE Collaboration. Published by Elsevier B.V. C1 [Grigoryan, A.; Papikyan, V.] Yerevan Phys Inst Fdn, AI Alikhanyan Natl Sci Lab, Yerevan, Armenia. [Martinez, H. Bello; Maldonado, I. Cortes; Tellez, A. Fernandez; Martinez, M. I.; Moreno, L. A. P.; Noris, J. C. C.; Cahuantzi, M. Rodriguez; Munoz, G. Tejeda; Vargas, A.; Limon, S. Vergara; Tello, A. Villatoro] Benemerita Univ Autonoma Puebla, Puebla, Mexico. 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[Gunji, T.; Hamagaki, H.; Hayashi, S.; Sekiguchi, Y.; Terasaki, K.; Tsuji, T.; Watanabe, Y.] Univ Tokyo, Tokyo, Japan. [Bhom, J.; Busch, O.; Chujo, T.; Esumi, S.; Hosokawa, R.; Inaba, M.; Kobayashi, T.; Miake, Y.; Sano, M.; Tanaka, N.; Watanabe, D.; Yokoyama, H.] Univ Tsukuba, Tsukuba, Ibaraki, Japan. [Erhardt, F.; Planinic, M.; Poljak, N.; Simatovic, G.; Utrobicic, A.] Univ Zagreb, Zagreb 41000, Croatia. [Cheshkov, C.; Cheynis, B.; Ducroux, L.; Grossiord, J. -Y.; Teyssier, B.; Tieulent, R.; Uras, A.] Univ Lyon 1, CNRS, IN2P3, IPN Lyon, F-69622 Villeurbanne, France. [Altsybeev, I.; Feofilov, G.; Kolojvari, A.; Kondratiev, V.; Kovalenko, V.; Vechernin, V.; Vinogradov, L.; Zarochentsev, A.] St Petersburg State Univ, V Fock Inst Phys, St Petersburg 199034, Russia. [Ahammed, Z.; Alam, S. N.; Basu, S.; Chattopadhyay, S.; Choudhury, S.; Dubey, A. K.; Ghosh, P.; Kar, S.; Khan, S. A.; Mitra, J.; Mohanty, B.; Muhuri, S.; Mukherjee, M.; Nayak, T. K.; Pal, S. K.; Patra, R. 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RI Natal da Luz, Hugo/F-6460-2013; Martinez Hernandez, Mario Ivan/F-4083-2010; Ferretti, Alessandro/F-4856-2013; Kovalenko, Vladimir/C-5709-2013; Altsybeev, Igor/K-6687-2013; Vickovic, Linda/F-3517-2017; Fernandez Tellez, Arturo/E-9700-2017; Nattrass, Christine/J-6752-2016; Usai, Gianluca/E-9604-2015; Cosentino, Mauro/L-2418-2014; Suaide, Alexandre/L-6239-2016; Barnby, Lee/G-2135-2010; Peitzmann, Thomas/K-2206-2012; Kondratiev, Valery/J-8574-2013; Vinogradov, Leonid/K-3047-2013; Castillo Castellanos, Javier/G-8915-2013; Ferreiro, Elena/C-3797-2017; Bregant, Marco/I-7663-2012; Sevcenco, Adrian/C-1832-2012; de Cuveland, Jan/H-6454-2016; Kurepin, Alexey/H-4852-2013; Jena, Deepika/P-2873-2015; Jena, Satyajit/P-2409-2015; Vechernin, Vladimir/J-5832-2013; Akindinov, Alexander/J-2674-2016; Takahashi, Jun/B-2946-2012; De Pasquale, Salvatore/B-9165-2008; Chinellato, David/D-3092-2012; Pshenichnov, Igor/A-4063-2008 OI Natal da Luz, Hugo/0000-0003-1177-870X; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Ferretti, Alessandro/0000-0001-9084-5784; Kovalenko, Vladimir/0000-0001-6012-6615; Altsybeev, Igor/0000-0002-8079-7026; Vickovic, Linda/0000-0002-9820-7960; Fernandez Tellez, Arturo/0000-0003-0152-4220; Riggi, Francesco/0000-0002-0030-8377; Scarlassara, Fernando/0000-0002-4663-8216; Nattrass, Christine/0000-0002-8768-6468; Usai, Gianluca/0000-0002-8659-8378; Cosentino, Mauro/0000-0002-7880-8611; Suaide, Alexandre/0000-0003-2847-6556; Barnby, Lee/0000-0001-7357-9904; Peitzmann, Thomas/0000-0002-7116-899X; Kondratiev, Valery/0000-0002-0031-0741; Vinogradov, Leonid/0000-0001-9247-6230; Castillo Castellanos, Javier/0000-0002-5187-2779; Ferreiro, Elena/0000-0002-4449-2356; Sevcenco, Adrian/0000-0002-4151-1056; de Cuveland, Jan/0000-0003-0455-1398; Kurepin, Alexey/0000-0002-1851-4136; Jena, Deepika/0000-0003-2112-0311; Jena, Satyajit/0000-0002-6220-6982; Vechernin, Vladimir/0000-0003-1458-8055; Akindinov, Alexander/0000-0002-7388-3022; Takahashi, Jun/0000-0002-4091-1779; De Pasquale, Salvatore/0000-0001-9236-0748; Chinellato, David/0000-0002-9982-9577; Pshenichnov, Igor/0000-0003-1752-4524 NR 73 TC 15 Z9 15 U1 6 U2 20 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD MAR 10 PY 2016 VL 754 BP 235 EP 248 DI 10.1016/j.physletb.2016.01.020 PG 14 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DD0HM UT WOS:000369601000035 ER PT J AU Ayangeakaa, AD Janssens, RVF Wu, CY Allmond, JM Wood, JL Zhu, S Albers, M Almaraz-Calderon, S Bucher, B Carpenter, MP Chiara, CJ Cline, D Crawford, HL David, HM Harker, J Hayes, AB Hoffman, CR Kay, BP Kolos, K Korichi, A Lauritsen, T Macchiavelli, AO Richard, A Seweryniak, D Wiens, A AF Ayangeakaa, A. D. Janssens, R. V. F. Wu, C. Y. Allmond, J. M. Wood, J. L. Zhu, S. Albers, M. Almaraz-Calderon, S. Bucher, B. Carpenter, M. P. Chiara, C. J. Cline, D. Crawford, H. L. David, H. M. Harker, J. Hayes, A. B. Hoffman, C. R. Kay, B. P. Kolos, K. Korichi, A. Lauritsen, T. Macchiavelli, A. O. Richard, A. Seweryniak, D. Wiens, A. TI Shape coexistence and the role of axial asymmetry in Ge-72 SO PHYSICS LETTERS B LA English DT Article ID INTERACTING BOSON MODEL; COULOMB-EXCITATION; EXCITED-STATES; ALPHA-DECAY; ATOMIC-NUCLEI; O+ STATES; ISOTOPES; NI-68; TRANSITION; REGION AB The quadrupole collectivity of low-lying states and the anomalous behavior of the 0(2)(+) and 2(3)(+) levels in Ge-72 are investigated via projectile multi-step Coulomb excitation with GRETINA and CHICO-2. Atotal of forty six E2 and M1 matrix elements connecting fourteen low-lying levels were determined using the least-squares search code, GOSIA. Evidence for triaxiality and shape coexistence, based on the model-independent shape invariants deduced from the Kumar-Cline sum rule, is presented. These are interpreted using a simple two-state mixing model as well as multi-state mixing calculations carried out within the framework of the triaxial rotor model. The results represent a significant milestone towards the understanding of the unusual structure of this nucleus. (C) 2016 The Authors. Published by Elsevier B.V. C1 [Ayangeakaa, A. D.; Janssens, R. V. F.; Zhu, S.; Albers, M.; Almaraz-Calderon, S.; Carpenter, M. P.; Chiara, C. J.; David, H. M.; Harker, J.; Hoffman, C. R.; Kay, B. P.; Lauritsen, T.; Seweryniak, D.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Wu, C. Y.; Bucher, B.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Allmond, J. M.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Wood, J. L.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Allmond, J. M.] Univ Maryland, Dept Chem & Biochem, College Pk, MD 20742 USA. [Cline, D.; Hayes, A. B.] Univ Rochester, Dept Phys & Astron, Rochester, NY 14627 USA. [Crawford, H. L.; Richard, A.] Ohio Univ, Dept Phys & Astron, Inst Nucl & Particle Phys, Athens, OH 45701 USA. [Kolos, K.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Korichi, A.] CNRS, CSNSM, IN2P3, F-91405 Orsay, France. [Korichi, A.] Univ Paris 11, F-91405 Orsay, France. [Crawford, H. L.; Macchiavelli, A. O.; Wiens, A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Albers, M.] Ernst & Young GmbH, Mergenthalerallee 3-5, D-65760 Eschborn, Germany. [Almaraz-Calderon, S.] Florida State Univ, Dept Phys, Tallahassee, FL 32306 USA. [Chiara, C. J.] US Army Res Lab, Adelphi, MD 20783 USA. [David, H. M.] Helmholtzzentrum Schwerionenforsch GmbH, GSI, D-64291 Darmstadt, Germany. RP Ayangeakaa, AD (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. EM ayangeakaa@anl.gov RI Kay, Benjamin/F-3291-2011; OI Kay, Benjamin/0000-0002-7438-0208; Ayangeakaa, Akaa D./0000-0003-1679-3175 FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357, DE-AC52-07NA27344, DE-FG02-94ER40834, DE-FG0208ER41556]; National Science Foundation [0969079] FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics under Contract numbers DE-AC02-06CH11357 and DE-AC52-07NA27344, and under Grant Numbers DE-FG02-94ER40834 and DE-FG0208ER41556, and by the National Science Foundation under grant number 0969079. This research used resources of ANL's ATLAS facility, which is a DOE Office of Science User Facility. NR 54 TC 4 Z9 4 U1 5 U2 8 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD MAR 10 PY 2016 VL 754 BP 254 EP 259 DI 10.1016/j.physletb.2016.01.036 PG 6 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DD0HM UT WOS:000369601000037 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Abeloos, B Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaitia, Y Acharyaa, BS Adamczyka, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedraa, JA Ahlen, SP Ahmadov, F Aiellia, G Akerstedta, H Akesson, TPA Akimov, AV Alberghia, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimontia, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allen, BW Allport, PP Aloisioa, A Alonso, A Alkire, SP Allbrooke, BMM Allen, BW Allport, PP Aloisioa, A Alonso, A Alonso, F Alpigiani, C Gonzalez, BA Piqueras, DA Alviggia, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andreia, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arika, M Armbruster, AJ Armitage, LJ Arnaez, O Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Artz, S Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Balunas, WK Banas, E Banerjee, S Bannoura, AAE Barak, L Barberio, EL Barberisa, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Navarro, LB Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Baucea, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, M Beckingham, M Becot, C Beddalle, AJ Beddall, A Bednyakov, VA Bedognetti, M Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, AS Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Benitez, J Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM 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Wotschack, J. Woudstra, M. J. Wozniak, K. W. Wu, M. Wu, M. Wu, S. L. Wu, X. Wu, Y. Wyatt, T. R. Wynne, B. M. Xella, S. Xu, D. Xu, L. Yabsley, B. Yacoob, S. Yakabe, R. Yamaguchi, D. Yamaguchi, Y. Yamamoto, A. Yamamoto, S. Yamanaka, T. Yamauchi, K. Yamazaki, Y. Yan, Z. Yang, H. Yang, H. Yang, Y. Yang, Z. Yao, W-M. Yap, Y. C. Yasu, Y. Yatsenko, E. YauWong, K. H. Ye, J. Ye, S. Yeletskikh, I. Yen, A. L. Yildirim, E. Yorita, K. Yoshida, R. Yoshihara, K. Young, C. Young, C. J. S. Youssef, S. Yu, D. R. Yu, J. Yu, J. M. Yu, J. Yuan, L. Yuen, S. P. Y. Yusuff, I. Zabinski, B. Zaidan, R. Zaitsev, A. M. Zakharchuk, N. Zalieckas, J. Zaman, A. Zambito, S. Zanello, L. Zanzi, D. Zeitnitz, C. Zeman, M. Zemla, A. Zeng, J. C. Zeng, Q. Zengel, K. Zenin, O. Zenis, T. Zerwas, D. Zhang, D. Zhang, F. Zhang, G. Zhang, H. Zhang, J. Zhang, L. Zhang, R. Zhang, R. Zhang, X. Zhang, Z. Zhao, X. Zhao, Y. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. Nedden, M. zur Zurzolo, G. Zwalinski, L. CA Atlas Collaboration TI Search for new phenomena in dijet mass and angular distributions from pp collisions at root s=13 TeV with the ATLAS detector SO PHYSICS LETTERS B LA English DT Article ID QUARK CONTACT INTERACTIONS; BLACK-HOLE PRODUCTION; JET CROSS-SECTIONS; HADRON COLLIDERS; PARTON DISTRIBUTIONS; DIMENSIONS; LHC; COMPUTATION; MILLIMETER; RESONANCES AB This Letter describes a model-agnostic search for pairs of jets (dijets) produced by resonant and non-resonant phenomena beyond the Standard Model in 3.6 fb(-1) of proton-proton collisions with a centre-of-mass energy of root s = 13 TeV recorded by the ATLAS detector at the Large Hadron Collider. The distribution of the invariant mass of the two leading jets is examined for local excesses above a data-derived estimate of the smoothly falling prediction of the Standard Model. The data are also compared to a Monte Carlo simulation of Standard Model angular distributions derived from the rapidity of the two jets. No evidence of anomalous phenomena is observed in the data, which are used to exclude, at 95% CL, quantum black holes with threshold masses below 8.3 TeV, 8.1 TeV, or 5.1 TeV in three different benchmark scenarios; resonance masses below 5.2 TeV for excited quarks, 2.6 TeV in a W' model, a range of masses starting from mZ' = 1.5 TeVand couplings from g(q) = 0.2 in a Z' model; and contact interactions with a compositeness scale below 12.0 TeV and 17.5 TeV respectively for destructive and constructive interference between the new interaction and QCD processes. These results significantly extend the ATLAS limits obtained from 8 TeV data. Gaussian-shaped contributions to the mass distribution are also excluded if the effective cross-section exceeds values ranging from approximately 50-300 fb for masses below 2 TeV to 2-20 fb for masses above 4 TeV. (C) 2016 CERN for the benefit of the ATLAS Collaboration. Published by Elsevier B.V. This is an open access article under the CC BY license. C1 [Jackson, P.; Lee, L.; Petridis, A.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Dassoulas, J.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakira, O.] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Kuday, S.] Istanbul Aydin Univ, Istanbul, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. 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[Blunier, S.; Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.] Pontificia Univ Catolica Chile, Dept Fis, Alameda 340, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Loyola, J. E. Salazar; Araya, S. Tapia; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Barreiro Guimaraes da Costa, J.; Fang, Y.; Jina, S.; Li, Q.; Lou, X.; Ouyanga, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Gengb, C.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y. L.; Liu, Y.; Peng, H.; Song, H. Y.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Dud, Y.; Feng, C.; Liu, B.; Mad, L. L.; Wang, C.; Zaidan, R.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Shanghai Key Lab Particle Phys & Cosmol, Dept Phys & Astron, Shanghai 200030, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Clermont Univ, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Angerami, A.; Brooijmans, G.; Carbone, R. M.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Blegdamsvej 17, DK-2100 Copenhagen, Denmark. [Cairo, V. M.; Capuaa, M.; Crosettia, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Nazl Frascati Lab, INFN Grp Coll Cosenza, Arcavacata Di Rende, Italy. [Cairo, V. M.; Capuaa, M.; Crosettia, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyka, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Gach, G. P.; Grabowska-Bolda, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindura, B.; Przybycien, M.; Zalieckas, J.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Burka, K.; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Phys Nucl, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Bessner, M.; Bloch, I.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Notkestr 85, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Zeuthen, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] INFN Lab Nazl Frascati, Frascati, Italy. [Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schnoor, U.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Mathemat & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; De Mendizabal, J. Bilbao; Calace, N.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; March, L.; Mermod, P.; Nackenhorst, O.; Paolozzi, L.; Ristic, B.; Schramm, S.; Sfyrla, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberisa, D.; Darboa, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Univ Genoa, INFN Sez Genova, Genoa, Italy. [Barberisa, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Via Dodecaneso 33, Genoa, Italy. [Jejelavaa, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Heinz, C.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; Crawley, S. J.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Knue, A.; Mullen, P.; O'Shea, V.; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Denis, R. D. St.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Camincher, C.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Kataoka, Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Petit, E.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Clark, B. L.; Franklin, M.; Giromini, P.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Rogan, C. S.; Skottowe, H. P.; Sun, S.; Tolley, E.; Tong, B.; Tuna, A. N.; Yen, A. L.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andreia, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunforda, M.; Geislera, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E-E.; Lang, V. S.; Meiera, K.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoya, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolbb, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Inforat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Castilloa, L. R. Flores; Lu, H.; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.; Orlando, N.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Kopeliansky, R.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Benitez, J.; Mallik, U.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Jiang, H.; Krumnack, N.; Pluth, D.; Prell, S.; Yu, J.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Casper, D. W.; Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Guest, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gongadze, A.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagai, R.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Cheatham, S.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Muenstermann, D.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Bachas, K.; Chiodini, G.; Gorinia, E.; Longo, L.; Primavera, M.; Spagnolo, S.; Ventura, A.] Univ Salento, INFN Sez Lecce, Lecce, Italy. [Bachas, K.; Gorinia, E.; Longo, L.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Armitage, L. J.; Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bell, A. S.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Phys, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Groh, S.; Heck, T.; Hohlfeld, M.; Huesling, T. A.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Pleskot, V.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schmitz, S.; Schott, M.; Schuh, N.; Simioni, E.; Simon, M.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Bielski, R.; Cox, B. E.; Da Via, C.; Forcolin, G. T.; Forti, A.; Ponce, J. M. Iturbe; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Sanchez, F. J. Munoz; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. 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D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; TicseTorres, R. E.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Picazio, A.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Nuti, F.; Rados, P.; Scutti, F.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Ungaro, F. C.; Urquijo, P.; Volpi, M.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Gengb, C.; Goldfarb, S.; Guan, L.; Guo, Y.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mckee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Martin, B.; Mondragon, M. C.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimontia, G.; Andreazza, A.; Carminati, L.; Cavallia, D.; Costaa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Manzoni, S.; Mazza, S. M.; Meroni, C.; Monzania, S.; Perini, L.; Ragusa, F.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] INFN Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Manzoni, S.; Mazza, S. M.; Monzania, S.; Perini, L.; Ragusa, F.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Hrynevich, A.] Nat Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; ShoalehSaadi, D.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. 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[Barillari, T.; Bethke, S.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; La Rosa, A.; Macchiolo, A.; Maier, A. A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Kawade, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisioa, A.; Alviggia, M. G.; Canalea, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Doria, A.; Izzoa, V.; McCarn, A.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] INFN Sez Napoli, Naples, Italy. [Alviggia, M. G.; Canalea, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Mc Fadden, N. C.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Koenig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Becot, C.; Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Che, S.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Allen, B. W.; Brau, J. E.; Brost, E.; Hard, A. S.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Radloff, P.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Abeloos, B.; Ayoub, M. K.; Bassalat, A.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Goudet, C. R.; Grivaz, J-F.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Maiani, C.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Zeman, M.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris Saclay, Univ Paris Sud, CNRS, IN2P3,LAL, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, M. K.; Cameron, D.; Catmore, J. R.; Feigl, S.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Sandoval, C.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Artoni, G.; Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Bortoletto, D.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Lanza, A.; Livan, M.; Negria, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] INFN Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negria, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Di Clemente, W. K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Naryshkin, I.; Ryabov, Y. F.; Schegelsky, V. A.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Nat Res Ctr Kurchatov Inst, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuza, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orsoa, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] INFN Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuza, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orsoa, M.; Donati, S.; Giannetti, P.; Leone, S.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Farina, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedraa, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalhoa, J.; Castro, N. F.; Muino, P. Conde; Sargedas De Sousaa, M. J. Da Cunha; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maioa, A.; Maneira, J.; Seabra, L. F. Oleiro; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; Sargedas De Sousaa, M. J. Da Cunha; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maioa, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalhoa, J.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maioa, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedraa, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedraa, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Fac Ciencias & Tecnol, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marceca, G.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Sopczak, A.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zanzi, D.; Zenin, O.] NRC KI, State Res Ctr Inst High Energy Phys Protvino, Gatchina, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Baucea, M.; Bini, C.; Ciapetti, G.; Corradi, M.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Di Donato, C.; Falciano, S.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacavaa, F.; Luci, C.; Luminari, L.; Marzano, F.; McCarn, A.; Messina, A.; Nisatia, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; SafaiTehrani, F.; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.] INFN Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Baucea, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Di Domenico, A.; Di Donato, C.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacavaa, F.; Luci, C.; Messina, A.; Vanadia, M.; Verducci, M.] Sapienza Univ Rome, Dipartimento Fis, Rome, Italy. [Aiellia, G.; Camarri, P.; Cardarelli, R.; Di Ciaccioa, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] INFN Sez Roma Tor Vergata, Rome, Italy. [Aiellia, G.; Camarri, P.; Di Ciaccioa, A.; Iuppa, R.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziania, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessaa, M.; Stanescu, C.; Taccini, C.] INFN Sez Roma Tre, Rome, Italy. [Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessaa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummadaa, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdamic, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Mourslie, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Rabat, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J-B.; Boonekamp, M.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Denysiuk, D.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Pinto Firmino Da Costa, J. Goncalves; Guyot, C.; Hanna, R.; Hassani, S.; Jeanneau, F.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Peyaud, A.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, DSM IRFU, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S-C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; SalesDeBruin, P. H.; Pastor, E. Torro; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Li, Y.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Su, D.; Tompkins, L.; Wittgen, M.; Young, C.; Zambito, S.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazeka, T.; Plazak, L.; Sykora, I.; Tokar, S.; Zeitnitz, C.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Brunckob, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Connell, S. H.; Govenderb, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsuc, C.; Kar, D.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaitia, Y.; Akerstedta, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellmana, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossettia, V.; Shaikh, N. W.; Shcherbakova, A.; Silversteina, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.; Wallangen, V.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaitia, Y.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellmana, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossettia, V.; Shaikh, N. W.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.; Wallangen, V.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G-Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Di Mattia, A.; Gozani, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Duarte-Campderros, J.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Pascuzzi, V.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepaa, A.; Chekulaev, S. V.; Gingrich, D. M.; Jovicevic, J.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Navarro, L. Barranco; Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Navarro, L. Barranco; Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Acharyaa, B. S.; Barisonzi, M.; Boldyrev, A. S.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] INFN Grp Coll Udine, Sez Trieste, Udine, Italy. [Acharyaa, B. S.; Barisonzi, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Truong, L.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Boldyrev, A. S.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Gradin, P. O. J.; Isaksson, C.; Maddocks, H. J.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Hooberman, B. H.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.; Zaman, A.; Zeng, J. C.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, IFIC, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, IMB CNM, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; Gignac, M.; Henkelmann, S.; King, S. B.; Lister, A.] Univ British Columbia, Dept Phys, 6224 Agr Rd, Vancouver, BC V6T 1W5, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; McPherson, R. A.; Pearce, J.; Sobie, R.; Trovatelli, M.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Ennis, J. S.; Farrington, S. M.; Harrison, P. F.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.; Spangenberg, M.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Koehler, M. K.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.; Turgeman, D.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kaplan, L. S.; Kashif, L.; Kruse, A.; Ming, Y.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Strohmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fac Phys & Astron, Wurzburg, Germany. [Bannoura, A. A. E.; Boerner, D.; Braun, H. M.; Cornelissen, T.; Ellinghaus, F.; Ernis, G.; Fischer, J.; Flick, T.; Gabizon, O.; Gilles, G.; Hamacher, K.; Harenberg, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Kuechler, J. T.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Vogel, M.; Wagner, W.] Berg Univ Wuppertal, Fachgrp Phys, Fak Mathemat & Naturwissensch, Wuppertal, Germany. [Baker, O. K.; Noccioli, E. Benhar; Cummings, J.; Demers, S.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Hernandez, D. Paredes; Thomsen, L. A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Inst Natl Phys Nucl & Phys Particules IN2P3, Ctr Calcul, Villeurbanne, France. [Acharyaa, B. S.] Kings Coll London, Dept Phys, London, England. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Banerjee, Sw.] Univ Louisville, Dept Phys & Astron, Louisville, KY 40292 USA. [Bawa, H. S.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beck, H. P.] Univ Fribourg, Dept Phys, CH-1700 Fribourg, Switzerland. [Casado, M. P.] Univ Autonoma Barcelona, Dept Fis, E-08193 Barcelona, Spain. [Bawa, H. S.] Univ Porto, Fac Ciencias, Dept Fis Astron, Rua Campo Alegre 823, P-4100 Oporto, Portugal. [Chelkov, G. A.] Tomsk State Univ, Tomsk 634050, Russia. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Inst Catalana Recerca & Estudis Avancats, Barcelona, Spain. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu 30013, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Hsu, P. J.] Illinois State Univ, Inst Theoret Phys, Normal, IL 61761 USA. [Khubua, J.] GTU, Tbilisi, Rep of Georgia. [Kono, T.; Nagai, R.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. 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[Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. [Zhang, R.] Aix Marseille Univ, CPPM, Marseille, France. [Zhang, R.] CNRS, IN2P3, Marseille, France. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France.; Aad, G (reprint author), CNRS, IN2P3, Marseille, France. 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NR 72 TC 44 Z9 44 U1 35 U2 79 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD MAR 10 PY 2016 VL 754 BP 302 EP 322 DI 10.1016/j.physletb.2016.01.032 PG 21 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DD0HM UT WOS:000369601000045 ER PT J AU Adam, J Adamova, D Aggarwal, MM Rinella, GA Agnello, M Agrawal, N Ahammed, Z Ahn, SU Aimo, I Aiola, S Ajaz, M Akindinov, A Alam, SN Aleksandrov, D Alessandro, B Alexandre, D Molina, RA Alici, A Alkin, A Alme, J Alt, T Altinpinar, S Altsybeev, I Prado, CAG Andrei, C Andronic, A Anguelov, V Anielski, J Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arcelli, S Armesto, N Arnaldi, R Arsene, IC Arslandok, M Audurier, B Augustinus, A Averbeck, R Azmi, MD Bach, M Badala, A Baek, YW Bagnasco, S Bailhache, R Bala, R Baldisseri, A Pedrosa, FBDS Baral, RC Barbano, AM Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartalini, P Barth, K Bartke, J Bartsch, E Basile, M Bastid, N Basu, S Bathen, B Batigne, G Camejo, AB Batyunya, B Batzing, PC Bearden, IG Beck, H Bedda, C Behera, NK Belikov, I Bellini, F Martinez, HB Bellwied, R Belmont, R Belmont-Moreno, E Belyaev, V Bencedi, G Beole, S Berceanu, I Bercuci, A Berdnikov, Y Berenyi, D Bertens, RA Berzano, D Betev, L Bhasin, A Bhat, IR Bhati, AK Bhattacharjee, B Bhom, J Bianchi, L Bianchi, N Bianchin, C Bielcik, J Bielcikova, J Bilandzic, A Biswas, R Biswas, S Bjelogrlic, S Blanco, F Blau, D Blume, C Bock, F Bogdanov, A Boggild, H Boldizsar, L Bombara, M Book, J Borel, H Borissov, A Borri, M Bossu, F Botje, M Botta, E Bottger, S Braun-Munzinger, P Bregant, M Breitner, T Broker, TA Browning, TA Broz, M Brucken, EJ Bruna, E Bruno, GE Budnikov, D Buesching, H Bufalino, S Buncic, P Busch, O Buthelezi, Z Buxton, JT Caffarri, D Cai, X Caines, H Diaz, LC Caliva, A Villar, EC Camerini, P Carena, F Carena, W Castellanos, JC Castro, AJ Casula, EAR Cavicchioli, C Sanchez, CC Cepila, J Cerello, P Cerkala, J Chang, B Chapeland, S Chartier, M Charvet, JL Chattopadhyay, S Chattopadhyay, S 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CA ALICE Collaboration TI (3)(Lambda)Hand (3)((Lambda)over-bar)(H)over-bar production in Pb-Pb collisions at root s(NN)=2.76 TeV SO PHYSICS LETTERS B LA English DT Article ID HEAVY-ION COLLISIONS; LIGHT HYPERNUCLEI; MID-RAPIDITY; DECAY-RATE; LIFETIME; MATTER; BARYON; STATE; HYPERTRITON; H-3(LAMBDA) AB The production of the hypertriton nuclei H-3(Lambda) and (3)((Lambda) over bar)(H) over bar has been measured for the first time in Pb-Pb collisions at root s(NN) = 2.76 TeVwith the ALICE experiment at LHC. The p(T)-integrated H-3(Lambda) yield in one unity of rapidity, dN/dy x B.R.((3 Lambda H -> 3He,pi-)) = (3.86 +/- 0.77(stat.) +/- 0.68(syst.)) x 10(-5) in the 0-10% most central collisions, is consistent with the predictions from a statistical thermal model using the same temperature as for the light hadrons. The coalescence parameter B-3 shows a dependence on the transverse momentum, similar to the B-2 of deuterons and the B-3 of He-3 nuclei. The ratio of yields S-3 = H-3(Lambda)/(He-3 x Lambda/p) was measured to be S-3 = 0.60 +/- 0.13(stat.) +/- 0.21(syst.) in 0-10% centrality events; this value is compared to different theoretical models. The measured S-3 is compatible with thermal model predictions. The measured H-3(Lambda) lifetime, tau = 181(-39)(+54)(stat.) +/- 33(syst.) psis in agreement within 1s with the world average value. (C) 2016 CERN for the benefit of the ALICE Collaboration. Published by Elsevier B.V. C1 [Grigoryan, A.; Gulkanyan, H.; Papikyan, V.] Yerevan Phys Inst Fdn, AI Alikhanyan Natl Sci Lab, Yerevan, Armenia. [Martinez, H. Bello; Maldonado, I. Cortes; Tellez, A. Fernandez; Martinez, M. I.; Noris, J. C. C.; Cahuantzi, M. Rodriguez; Munoz, G. Tejeda; Vargas, A.; Limon, S. Vergara] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Alkin, A.; Chelnokov, V.; Grinyov, B.; Martynov, Y.; Shadura, O.; Trubnikov, V.; Yurchenko, V.; Zinovjev, G.] Bogolyubov Inst Theoret Phys, Kiev, Ukraine. 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A.] Univ Santiago de Compostela, IGFAE, Santiago De Compostela, Spain. [Altinpinar, S.; Djuvsland, O.; Haaland, O.; Huang, M.; Loenne, P. I.; Nystrand, J.; Rehman, A.; Rohrich, D.; Ullaland, K.; Velure, A.; Wagner, B.; Zhang, H.; Zhou, Z.; Zhu, H.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Azmi, M. D.; Hussain, T.; Irfan, M.; Khan, M. M.; Tariq, M.] Aligarh Muslim Univ, Dept Phys, Aligarh 202002, Uttar Pradesh, India. [Buxton, J. T.; Humanic, T. J.; Kubera, A. M.; Lisa, M. A.; Salzwedel, J.; Steinpreis, M.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Hwang, D. S.; Kim, S.] Sejong Univ, Dept Phys, Seoul, South Korea. [Arsene, I. C.; Batzing, P. C.; Dordic, O.; Lindal, S.; Mahmood, S. M.; Milosevic, J.; Qvigstad, H.; Richter, M.; Roed, K.; Skaali, T. B.; Tveter, T. S.; Wikne, J.; Zhao, C.] Univ Oslo, Dept Phys, Oslo, Norway. [Minervini, L. M.] Politecn Bari, Dipartimento Elettrotecn & Elettron, Bari, Italy. [Meddi, F.] Univ Roma La Sapienza, Dipartimento Fis, Rome, Italy. [Meddi, F.] Sez INFN Rome, Rome, Italy. [Casula, E. A. R.; Collu, A.; De Falco, A.; Puddu, G.; Terrevoli, C.; Usai, G. L.] Univ Cagliari, Dipartimento Fis, Cagliari, Italy. [Casula, E. A. R.; Collu, A.; De Falco, A.; Puddu, G.; Terrevoli, C.; Usai, G. L.] Sezione Ist Nazl Fis Nucl, Cagliari, Italy. [Camerini, P.; Lea, R.; Luparello, G.; Margagliotti, G. V.; Rui, R.] Univ Trieste, Dipartimento Fis, Trieste, Italy. [Camerini, P.; Lea, R.; Luparello, G.; Margagliotti, G. V.; Rui, R.] Sezione Ist Nazl Fis Nucl, Trieste, Italy. [Beole, S.; Berzano, D.; Botta, E.; Morales, Y. Corrales; Ferretti, A.; Gagliardi, M.; Gallio, M.; Lattuca, A.; Leoncino, M.; Marchisone, M.; Masera, M.; Russo, R.; Shtejer, K.; Vallero, S.; Vercellin, E.] Univ Turin, Dipartimento Fis, Turin, Italy. [Beole, S.; Berzano, D.; Botta, E.; Morales, Y. Corrales; Ferretti, A.; Gagliardi, M.; Gallio, M.; Lattuca, A.; Leoncino, M.; Marchisone, M.; Masera, M.; Russo, R.; Shtejer, K.; Vallero, S.; Vercellin, E.] Sezione Ist Nazl Fis Nucl, Turin, Italy. [Arcelli, S.; Basile, M.; Bellini, F.; Cifarelli, L.; Colocci, M.; Guerzoni, B.; Scioli, G.; Zichichi, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arcelli, S.; Basile, M.; Bellini, F.; Cifarelli, L.; Colocci, M.; Guerzoni, B.; Scioli, G.; Zichichi, A.] Sezione Ist Nazl Fis Nucl, Bologna, Italy. [Barbera, R.; La Rocca, P.; Petta, C.; Riggi, F.; Santagati, G.] Univ Catania, Dipartimento Fis & Astron, Catania, Italy. [Barbera, R.; La Rocca, P.; Petta, C.; Riggi, F.; Santagati, G.] Sezione Ist Nazl Fis Nucl, Catania, Italy. [Festanti, A.; Francescon, A.; Giubilato, P.; Jena, C.; Lunardon, M.; Morando, M.; Moretto, S.; Rossi, A.; Scarlassara, F.; Soramel, F.; Terrevoli, C.; Viesti, G.] Univ Padua, Dipartimento Fis & Astron, Padua, Italy. [Festanti, A.; Francescon, A.; Giubilato, P.; Jena, C.; Lunardon, M.; Morando, M.; Moretto, S.; Rossi, A.; Scarlassara, F.; Soramel, F.; Terrevoli, C.; Viesti, G.] Sezione Ist Nazl Fis Nucl, Padua, Italy. [De Caro, A.; De Gruttola, D.; De Pasquale, S.; Girard, M. Fusco; Meninno, E.; Pagano, P.; Virgili, T.] Univ Salerno, Dipartimento Fis ER Caianiello, I-84100 Salerno, Italy. [De Caro, A.; De Gruttola, D.; De Pasquale, S.; Girard, M. Fusco; Meninno, E.; Pagano, P.; Virgili, T.] Grp Coll INFN, Salerno, Italy. [Cortese, P.; Ramello, L.; Sitta, M.] Univ Piemonte Orientale, Dipartimento Sci & Innovaz Tecnol, Alessandria, Italy. [Cortese, P.; Ramello, L.; Sitta, M.] Grp Coll INFN, Alessandria, Italy. [Barile, F.; Bruno, G. E.; Colamaria, F.; Colella, D.; D'Erasmo, G.; Di Bari, D.; Fiore, E. M.; Mastroserio, A.; Tangaro, M. A.] Dipartimento Interateneo Fis M Merlin, Bari, Italy. [Barile, F.; Bruno, G. E.; Colamaria, F.; Colella, D.; D'Erasmo, G.; Di Bari, D.; Fiore, E. M.; Mastroserio, A.; Tangaro, M. A.] Sezione Ist Nazl Fis Nucl, Bari, Italy. [Christiansen, P.; Ljunggren, H. M.; Oskarsson, A.; Richert, T.; Silvermyr, D.; Sogaard, C.; Stenlund, E.; Vislavicius, V.] Lund Univ, Div Expt High Energy Phys, Lund, Sweden. [Hess, B. A.; Schmidt, H. R.; Wiechula, J.] Univ Tubingen, Tubingen, Germany. [Rinella, G. Aglieri; Akindinov, A.; Augustinus, A.; Pedrosa, F. Baltasar Dos Santos; Barth, K.; Berzano, D.; Betev, L.; Bufalino, S.; Buncic, P.; Caffarri, D.; Carena, F.; Carena, W.; Cavicchioli, C.; Chapeland, S.; Barroso, V. Chibante; Chochula, P.; Costa, F.; Cunqueiro, L.; Di Mauro, A.; Divia, R.; Erazmus, B.; Floris, M.; Francescon, A.; Fuchs, U.; Gargiulo, C.; Gheata, A.; Gheata, M.; Giubellino, P.; Grigoras, A.; Grigoras, C.; Grosse-Oetringhaus, J. F.; Grosso, R.; Hillemanns, H.; Hristov, P.; Ionita, C.; Kluge, A.; Kofarago, M.; Kouzinopoulos, C.; Kryshen, E.; Kugathasan, T.; Lakomov, I.; Laudi, E.; Legrand, I.; Mager, M.; Manzari, V.; Martinengo, P.; Pedreira, M. Martinez; Milano, L.; Morsch, A.; Musa, L.; Niculescu, M.; Niedziela, J.; Ohlson, A.; Pinazza, O.; Preghenella, R.; Reidt, F.; Riedler, P.; Riegler, W.; Rossi, A.; Safarik, K.; Schukraft, J.; Schutz, Y.; Shahoyan, R.; Sielewicz, K. M.; Simonetti, G.; Szczepankiewicz, A.; Tauro, A.; Telesca, A.; Van Hoorne, J. W.; Vyvre, P. Vande; Von Haller, B.; Vranic, D.; Weber, M.; Zimmermann, M. B.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Dahms, T.; Fabbietti, L.; Gasik, P.; Vorobyev, I.] Tech Univ Munich, Excellence Cluster Univ, D-80290 Munich, Germany. [Alme, J.; Helstrup, H.; Hetland, K. F.; Kileng, B.] Bergen Univ Coll, Fac Engn, Bergen, Norway. [Meres, M.; Pikna, M.; Sitar, B.; Strmen, P.; Szabo, A.; Szarka, I.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Adam, J.; Bielcik, J.; Broz, M.; Cepila, J.; Contreras, J. G.; Eyyubova, G.; Krelina, M.; Petracek, V.; Schulc, M.; Spacek, M.] Czech Tech Univ, Fac Nucl Sci & Phys Engn, CR-11519 Prague, Czech Republic. [Bombara, M.; Kravcakova, A.; Vrlakova, J.] Safarik Univ, Fac Sci, Kosice, Slovakia. [Langoy, R.; Lien, J.] Buskerud & Vestfold Univ Coll, Fac Technol, Vestfold, Norway. [Alt, T.; Bach, M.; De Cuveland, J.; Eschweiler, D.; Gorbunov, S.; Hartmann, H.; Hutter, D.; Kirsch, S.; Kisel, I.; Kollegger, T.; Kretz, M.; Krzewicki, M.; Kulakov, I.; Lindenstruth, V.; Rettig, F.; Rohr, D.; Zyzak, M.] Goethe Univ Frankfurt, Frankfurt Inst Adv Studies, D-60054 Frankfurt, Germany. [Baek, Y. W.; Jung, H.; Kim, D. W.; Kim, J. S.; Kim, M.] Gangneung Wonju Natl Univ, Kangnung, South Korea. [Bhattacharjee, B.; Hussain, N.] Gauhati Univ, Dept Phys, Gauhati, India. [Brucken, E. J.; Hilden, T. E.; Mieskolainen, M. M.; Rasanen, S. S.] HIP, Helsinki, Finland. [Okubo, T.; Sekihata, D.; Shigaki, K.; Sugitate, T.; Yano, S.] Hiroshima Univ, Hiroshima, Japan. [Agrawal, N.; Behera, N. K.; Dash, S.; Meethaleveedu, G. Koyithatta; Kumar, J.; Nandi, B. K.; Pandey, A. K.; Pant, D.; Varma, R.] IIT, Mumbai, Maharashtra, India. [Behera, N. K.; Mishra, A. N.; Pareek, P.; Roy, A.; Sahoo, P.; Sahoo, R.] IIT, Indore, Madhya Pradesh, India. [Kweon, M. J.] Inha Univ, Inchon, South Korea. [Del Valle, Z. Conesa; Das, I.; Espagnon, B.; Hadjidakis, C.; Suire, C.; Takaki, J. D. Tapia; Tarhini, M.] Univ Paris 11, CNRS, IPNO, IN2P3, F-91405 Orsay, France. [Arslandok, M.; Blume, C.; Bottger, S.; Breitner, T.; Engel, H.; Ramirez, A. Gomez; Kebschull, U.; Lara, C.; Reichelt, P.] Goethe Univ Frankfurt, Inst Informat, D-60054 Frankfurt, Germany. [Appelshauser, H.; Bailhache, R.; Bartsch, E.; Beck, H.; Book, J.; Broker, T. A.; Buesching, H.; Dillenseger, P.; Donigus, B.; Erdemir, I.; Heckel, S. T.; Kamin, J.; Klein, C.; Luettig, P.; Marquard, M.; Ozdemir, M.; Peskov, V.; Rascanu, B. T.; Renfordt, R.; Sahlmuller, B.; Schuchmann, S.; Peloni, A. Tarantola; Toia, A.] Goethe Univ Frankfurt, Inst Kernphys, Frankfurt, Germany. [Anielski, J.; Bathen, B.; Feldkamp, L.; Haake, R.; Heide, M.; Klein-Bosing, C.; De Godoy, D. A. Moreira; MHlheim, D.; Passfeld, A.; Wessels, J. P.; Westerhoff, U.; Wilde, M.; Zimmermann, M. B.] Univ Munster, Inst Kernphys, D-48149 Munster, Germany. [Belikov, I.; Hippolyte, B.; Kuhn, C.; Maire, A.; Molnar, L.; Roy, C.; Castro, X. Sanchez] Univ Strasbourg, CNRS, IN2P3, IPHC, Strasbourg, France. [Finogeev, D.; Furs, A.; Guber, F.; Karavichev, O.; Karavicheva, T.; Karpechev, E.; Konevskikh, A.; Kurepin, A.; Kurepin, A. B.; Maevskaya, A.; Pshenichnov, I.; Reshetin, A.; Shabanov, A.] Acad Sci, Inst Nucl Res, Moscow, Russia. [Bertens, R. A.; Bianchin, C.; Bjelogrlic, S.; Caliva, A.; Chunhui, Z.; Dobrin, A.; Dubla, A.; Grelli, A.; Keijdener, D. L. D.; Leogrande, E.; Lodato, D. F.; Margutti, J.; Mischke, A.; Mohammadi, N.; Nooren, G.; Peitzmann, T.; Rocco, E.; Snellings, R. J. M.; Van der Maarel, J.; Van Leeuwen, M.; Veen, A. M.; Veldhoen, M.; Wang, H.; Yang, H.; Zhou, Y.] Univ Utrecht, Inst Subat Phys, Utrecht, Netherlands. [Akindinov, A.; Kiselev, S.; Mal'Kevich, D.; Mikhaylov, K.; Nedosekin, A.; Sultanov, R.; Voloshin, K.; Zhigareva, N.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Colella, D.; Kalinak, P.; Kralik, I.; Krivda, M.; Musinsky, J.; Sandor, L.; Vala, M.] Slovak Acad Sci, Inst Expt Phys, Kosice 04353, Slovakia. [Mares, J.; Sharma, N.; Zavada, P.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Baral, R. C.; Sahoo, S.; Sahu, P. K.] Inst Phys, Bhubaneswar 751007, Orissa, India. [Danu, A.; Felea, D.; Gheata, M.; Haiduc, M.; Mitu, C. M.; Niculescu, M.; Ristea, C.; Sevcenco, A.; Stan, I.; Zgura, I. S.] ISS, Bucharest, Romania. [Cuautle, E.; Cervantes, I. Maldonado; Nellen, L.; Velasquez, A. Ortiz; Paic, G.] Univ Nacl Autonoma Mexico, Inst Ciencias Nucl, Mexico City 04510, DF, Mexico. [Molina, R. Alfaro; Belmont-Moreno, E.; Grabski, V.; Menchaca-Rocha, A.; Sandoval, A.; Serradilla, E.] Univ Nacl Autonoma Mexico, Inst Fis, Mexico City, DF, Mexico. [Bossu, F.; Buthelezi, Z.; Foertsch, S.; Murray, S.; Senosi, K.; Steyn, G.] Natl Res Fdn, iThemba LABS, Somerset West, South Africa. [Batyunya, B.; Grigoryan, S.; Malinina, L.; Mikhaylov, K.; Nomokonov, P.; Rogochaya, E.; Vodopyanov, A.; Zaporozhets, S.] JINR, Dubna, Russia. [Oh, S. K.; Seo, J.] Konkuk Univ, Seoul, South Korea. [Ahn, S. U.; Jang, H. J.; Kim, D. W.] Korea Inst Sci & Technol Informat, Daejeon, South Korea. [Ahn, S. U.; Jang, H. J.; Kim, D. W.] Korea Inst Sci & Technol Informat, Daejeon, South Korea. [Uysal, A. Karasu; Okatan, A.] KTO Karatay Univ, Konya, Turkey. [Barret, V.; Bastid, N.; Camejo, A. Batista; Crochet, P.; Dupieux, P.; Feuillard, V. J. G.; Li, S.; Lopez, X.; Manso, F.; Porteboeuf-Houssais, S.; Rosnet, P.; Palomo, L. Valencia; Vulpescu, B.] Univ Clermont Ferrand, Univ Clermont Ferrand 2, CNRS, LPC,IN2P3, Clermont Ferrand, France. [Balbastre, G. Conesa; Faivre, J.; Furget, C.; Guernane, R.; Kox, S.; Real, J. S.; Silvestre, C.; Vauthier, A.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [Bianchi, N.; Diaz, L. Calero; Di Nezza, P.; Fantoni, A.; Gianotti, P.; Muccifora, V.; Reolon, A. R.; Ronchetti, F.; Sakai, S.; Spiriti, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Ricci, R. A.; Venaruzzo, M.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Legnaro, Italy. [Bock, F.; Fasel, M.; Gangadharan, D. R.; Jacobs, P. M.; Loizides, C.; Ploskon, M.; Porter, J.; Symons, T. J. 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[Botje, M.; Christakoglou, P.; Dobrin, A.; Kuijer, P. G.; Lara, C. E. Perez; Manso, A. Rodriguez] NIKHEF H, Natl Inst Subat Phys, NL-1009 DB Amsterdam, Netherlands. [Borri, M.; Lemmon, R. C.] STFC Daresbury Lab, Nucl Phys Grp, Daresbury, England. [Adamova, D.; Bielcikova, J.; Ferencei, J.; Krizek, F.; Kucera, V.; Kushpil, S.; Pospisil, J.; Sumbera, M.; Vajzer, M.; Vanat, T.] Acad Sci Czech Republic, Inst Nucl Phys, CZ-25068 Rez, Czech Republic. [Cormier, T. M.; Silvermyr, D.] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Berdnikov, Y.; Ivanov, V.; Khanzadeev, A.; Malaev, M.; Nikulin, V.; Riabov, V.; Ryabov, Y.; Samsonov, V.; Zhalov, M.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Cherney, M.; Poghosyan, M. G.; Seger, J. E.] Creighton Univ, Dept Phys, Omaha, NE 68178 USA. [Aggarwal, M. M.; Bhati, A. K.; Kumar, L.; Parmar, S.; Rathee, D.] Panjab Univ, Dept Phys, Chandigarh 160014, India. [Ganoti, P.; Roukoutakis, F.; Spyropoulou-Stassinaki, M.; Vasileiou, M.] Univ Athens, Dept Phys, Athens, Greece. [Cleymans, J.; Dietel, T.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Bala, R.; Bhasin, A.; Bhat, I. R.; Gupta, A.; Gupta, R.; Mahajan, S.; Rajput, S.; Sambyal, S.; Sharma, A.] Univ Jammu, Dept Phys, Jammu 180004, India. [Raniwala, R.; Raniwala, S.] Univ Rajasthan, Dept Phys, Jaipur 302004, Rajasthan, India. [Dahms, T.; Fabbietti, L.; Gasik, P.; Vorobyev, I.] Tech Univ Munich, Dept Phys, D-80290 Munich, Germany. [Anguelov, V.; Bock, F.; Busch, O.; Deisting, A.; Fleck, M. G.; Glassel, P.; Klein, J.; Knichel, M. L.; Leardini, L.; Perez, J. Mercado; Oeschler, H.; Oyama, K.; Pachmayer, Y.; Reidt, F.; Reygers, K.; Schicker, R.; Stachel, J.; Stiller, J. H.; Volkl, M. A.; Wang, Y.; Wilkinson, J.; Windelband, B.; Winn, M.; Zimmermann, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Aimo, I.] Politecn Torino, Turin, Italy. [Browning, T. A.; Scharenberg, R. P.; Srivastava, B. K.] Purdue Univ, W Lafayette, IN 47907 USA. [Borissov, A.; Choi, K.; Chung, S. U.; Eum, J.; Seo, J.; Song, J.; Yoo, I. -K.] Pusan Natl Univ, Pusan 609735, South Korea. [Andronic, A.; Averbeck, R.; Braun-Munzinger, P.; Deisting, A.; Foka, P.; Frankenfeld, U.; Garabatos, C.; Ivanov, M.; Bustamante, R. T. Jimenez; Kollegger, T.; Lippmann, C.; Malzacher, P.; Marin, A.; Martin, N. A.; Masciocchi, S.; Miskowiec, D.; Nicassio, M.; Onderwaater, J.; Park, W. J.; Schmidt, C.; Schwarz, K.; Schweda, K.; Selyuzhenkov, I.; Thader, J.; Vranic, D.; Wagner, J.; Weber, S. G.] GSI Helmholtzzentrum Schwerionenforsch, Div Res, Darmstadt, Germany. [Andronic, A.; Averbeck, R.; Braun-Munzinger, P.; Deisting, A.; Foka, P.; Frankenfeld, U.; Garabatos, C.; Ivanov, M.; Bustamante, R. T. Jimenez; Kollegger, T.; Lippmann, C.; Malzacher, P.; Marin, A.; Martin, N. A.; Masciocchi, S.; Miskowiec, D.; Nicassio, M.; Onderwaater, J.; Park, W. J.; Schmidt, C.; Schwarz, K.; Schweda, K.; Selyuzhenkov, I.; Thader, J.; Vranic, D.; Wagner, J.; Weber, S. G.] GSI Helmholtzzentrum Schwerionenforsch, ExtreMe Matter Inst EMMI, Darmstadt, Germany. [Anticic, T.] Rudjer Boskovic Inst, Zagreb, Croatia. [Budnikov, D.; Filchagin, S.; Ilkaev, R.; Kuryakin, A.; Mamonov, A.; Nazarenko, S.; Punin, V.; Tumkin, A.; Vinogradov, Y.; Vyushin, A.; Zaviyalov, N.] Russian Fed Nucl Ctr VNIIEF, Sarov, Russia. [Aleksandrov, D.; Blau, D.; Fokin, S.; Ippolitov, M.; Manko, V.; Nikolaev, S.; Nikulin, S.; Nyanin, A.; Peresunko, D.; Ryabinkin, E.; Sibiriak, Y.; Vasiliev, A.; Vinogradov, A.; Yushmanov, I.] Russian Res Ctr Kurchatov Inst, Moscow, Russia. [Chattopadhyay, S.; Das, D.; Das, I.; Khan, P.; Paul, B.; Roy, P.; Sinha, T.] Saha Inst Nucl Phys, Kolkata, India. [Alexandre, D.; Barnby, L. S.; Evans, D.; Graham, K. L.; Jones, P. G.; Jusko, A.; Krivda, M.; Lee, G. R.; Lietava, R.; Baillie, O. Villalobos; Zardoshti, N.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Villar, E. Calvo; Gago, A. M.] Pontificia Univ Catolica Peru, Dept Ciencias, Secc Fis, Lima, Peru. [De Cataldo, G.; Elia, D.; Fionda, F. M.; Lenti, V.; Manzari, V.; Minervini, L. M.; Nappi, E.; Paticchio, V.] Sezione Ist Nazl Fis Nucl, Bari, Italy. [Alici, A.; Antonioli, P.; Cindolo, F.; Hatzifotiadou, D.; Margotti, A.; Nania, R.; Noferini, F.; Pinazza, O.; Preghenella, R.; Scapparone, E.; Williams, M. C. S.; Zampolli, C.] Sezione Ist Nazl Fis Nucl, Bologna, Italy. [Cicalo, C.; Masoni, A.; Siddhanta, S.] Sezione Ist Nazl Fis Nucl, Cagliari, Italy. [Badala, A.; Pappalardo, G. S.] Sezione Ist Nazl Fis Nucl, Catania, Italy. [Antinori, F.; Dainese, A.; Fabris, D.; Turrisi, R.] Sezione Ist Nazl Fis Nucl, Padua, Italy. [Mazzoni, M. A.] Sezione Ist Nazl Fis Nucl, Rome, Italy. [Fragiacomo, E.; Grion, N.; Piano, S.; Rachevski, A.] Sezione Ist Nazl Fis Nucl, Trieste, Italy. [Agnello, M.; Aimo, I.; Alessandro, B.; Arnaldi, R.; Bagnasco, S.; Barbano, A. M.; Bedda, C.; Bruna, E.; Bufalino, S.; Cerello, P.; De Marco, N.; Feliciello, A.; La Pointe, S. L.; Manceau, L.; Oppedisano, C.; Prino, F.; Puccio, M.; Rivetti, A.; Scomparin, E.; Trogolo, S.] Sezione Ist Nazl Fis Nucl, Turin, Italy. [Evdokimov, S.; Izucheev, V.; Kharlov, Y.; Kondratyuk, E.; Petrov, V.; Polichtchouk, B.; Sadovsky, S.; Shangaraev, A.] NRC Kurchatov Inst, SSC IHEP, Protvino, Russia. [Aphecetche, L.; Audurier, B.; Batigne, G.; Erazmus, B.; Estienne, M.; Germain, M.; Blanco, J. Martin; Garcia, G. Martinez; Massacrier, L.; De Godoy, D. A. Moreira; Morreale, A.; Pillot, P.; Ronflette, L.; Schutz, Y.; Shabetai, A.; Stocco, D.; Wang, M.; Zhu, J.] Univ Nantes, Ecole Mines Nantes, SUBATECH, CNRS,IN2P3, Nantes, France. [Kobdaj, C.; Poonsawat, W.] Suranaree Univ Technol, Nakhon Ratchasima, Thailand. [Cerkala, J.; Jadlovska, S.; Kopcik, M.; Papcun, P.] Tech Univ Kosice, Kosice, Slovakia. [Gotovac, S.; Mudnic, E.; Vickovic, L.] Tech Univ Split FESB, Split, Croatia. [Bartke, J.; Figiel, J.; Gladysz-Dziadus, E.; Gorlich, L.; Kowalski, M.; Matyja, A.; Mayer, C.; Otwinowski, J.; Rybicki, A.; Sputowska, I.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Knospe, A. G.; Markert, C.; Thomas, D.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Monzon, I. Leon; Podesta-Lerma, P. L. M.] Universidad Autonoma Sinaloa, Culiacan, Mexico. [Prado, C. Alves Garcia; Bregant, M.; Cosentino, M. R.; De, S.; Gimenez, D. Domenicis; Jahnke, C.; Fernandes, C. Lagana; Luz, P. H. F. N. D.; Mas, A.; Munhoz, M. G.; Da Silva, A. C. Oliveira; De Oliveira Filho, E. Pereira; Seeder, K. S.; Suaide, A. A. P.; De Toledo, A. Szanto; Zanoli, H. J. C.] Univ Sao Paulo, BR-09500900 Sao Paulo, Brazil. [Chinellato, D. D.; Dash, A.; Takahashi, J.] Univ Estadual Campinas UNICAMP, Campinas, SP, Brazil. [Bellwied, R.; Bianchi, L.; Jayarathna, P. H. S. Y.; Jena, S.; Mcdonald, D.; Ng, F.; Pinsky, L.; Piyarathna, D. B.; Timmins, A. R.] Univ Houston, Houston, TX USA. [Chang, B.; Kim, D. J.; Kral, J.; Rak, J.; Slupecki, M.; Snellman, T. W.; Trzaska, W. H.; Vargyas, M.; Viinikainen, J.] Univ Jyvaskyla, Jyvaskyla, Finland. [Chartier, M.; Figueredo, M. A. S.; Norman, J.; Romita, R.] Univ Liverpool, Liverpool L69 3BX, Merseyside, England. [Castro, A. J.; Hosokawa, R.; Mazer, J.; Nattrass, C.; Read, K. F.; Scott, R.; Sharma, N.; Sorensen, S.] Univ Tennessee, Knoxville, TN USA. [Vilakazi, Z.] Univ Witwatersrand, ZA-2050 Johannesburg, South Africa. [Gunji, T.; Hamagaki, H.; Hayashi, S.; Sekiguchi, Y.; Terasaki, K.; Tsuji, T.; Watanabe, Y.] Univ Tokyo, Tokyo, Japan. [Bhom, J.; Busch, O.; Chujo, T.; Esumi, S.; Inaba, M.; Kobayashi, T.; Masui, H.; Miake, Y.; Sano, M.; Tanaka, N.; Watanabe, D.; Yokoyama, H.] Univ Tsukuba, Tsukuba, Ibaraki, Japan. [Erhardt, F.; Planinic, M.; Poljak, N.; Simatovic, G.; Utrobicic, A.] Univ Zagreb, Zagreb 41000, Croatia. [Cheshkov, C.; Cheynis, B.; Ducroux, L.; Grossiord, J. -Y.; Teyssier, B.; Tieulent, R.; Uras, A.] Univ Lyon 1, CNRS, IN2P3, IPN Lyon, F-69622 Villeurbanne, France. [Altsybeev, I.; Feofilov, G.; Kolojvari, A.; Kondratiev, V.; Kovalenko, V.; Vechernin, V.; Vinogradov, L.; Zarochentsev, A.] St Petersburg State Univ, V Fock Inst Phys, St Petersburg 199034, Russia. [Ahammed, Z.; Alam, S. N.; Basu, S.; Chattopadhyay, S.; Choudhury, S.; Dubey, A. K.; Ghosh, P.; Kar, S.; Khan, S. A.; Mitra, J.; Mohanty, B.; Muhuri, S.; Mukherjee, M.; Nayak, T. K.; Pal, S. K.; Patra, R. N.; Saini, J.; Sarkar, D.; Singaraju, R.; Singha, S.; Singhal, V.; Sinha, B. C.; Viyogi, Y. P.] Ctr Variable Energy Cyclotron, Kolkata, India. [Milosevic, J.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Graczykowski, L. K.; Janik, M. A.; Kisiel, A.; Oleniacz, J.; Pluta, J.; Szymanski, M.; Zaborowska, A.; Zbroszczyk, H.] Warsaw Univ Technol, Warsaw, Poland. [Belmont, R.; Bianchin, C.; Loggins, V. R.; Pan, J.; Pruneau, C. A.; Pujahari, P.; Putschke, J.; Reed, R. J.; Saleh, M. A.; Verweij, M.; Voloshin, S. A.; Yaldo, C. G.] Wayne State Univ, Detroit, MI USA. [Barnafoldi, G. G.; Bencedi, G.; Berenyi, D.; Boldizsar, L.; Denes, E.; Hamar, G.; Keil, M.; Kiss, G.; Levai, P.; Lowe, A.; Olah, L.; Pochybova, S.; Varga, D.; Volpe, G.] Hungarian Acad Sci, Wigner Res Ctr Phys, Budapest, Hungary. [Aiola, S.; Caines, H.; Connors, M. E.; Ehlers, R. J.; Harris, J. W.; Majka, R. D.; Mulligan, J. D.; Oh, S.; Oliver, M. H.; Schuster, T.; Smirnov, N.] Yale Univ, New Haven, CT USA. [Kang, J. H.; Kim, B.; Kim, H.; Kim, M.; Kim, T.; Kwon, Y.; Lee, S.; Song, M.] Yonsei Univ, Seoul 120749, South Korea. [Keidel, R.] ZTT, Fachhsch Worms, Worms, Germany. [Takaki, J. D. Tapia] Univ Kansas, Lawrence, KS 66045 USA. RP Adam, J (reprint author), Czech Tech Univ, Fac Nucl Sci & Phys Engn, CR-11519 Prague, Czech Republic. RI Armesto, Nestor/C-4341-2017; Martinez Hernandez, Mario Ivan/F-4083-2010; Ferretti, Alessandro/F-4856-2013; Kovalenko, Vladimir/C-5709-2013; Altsybeev, Igor/K-6687-2013; Vickovic, Linda/F-3517-2017; Fernandez Tellez, Arturo/E-9700-2017; Takahashi, Jun/B-2946-2012; Nattrass, Christine/J-6752-2016; Usai, Gianluca/E-9604-2015; Cosentino, Mauro/L-2418-2014; Suaide, Alexandre/L-6239-2016; Barnby, Lee/G-2135-2010; Peitzmann, Thomas/K-2206-2012; Kondratiev, Valery/J-8574-2013; Vinogradov, Leonid/K-3047-2013; Castillo Castellanos, Javier/G-8915-2013; Ferreiro, Elena/C-3797-2017; Felea, Daniel/C-1885-2012; Bregant, Marco/I-7663-2012; Sevcenco, Adrian/C-1832-2012; de Cuveland, Jan/H-6454-2016; Kurepin, Alexey/H-4852-2013; Jena, Deepika/P-2873-2015; Jena, Satyajit/P-2409-2015; Vechernin, Vladimir/J-5832-2013; Akindinov, Alexander/J-2674-2016; De Pasquale, Salvatore/B-9165-2008; Chinellato, David/D-3092-2012; Pshenichnov, Igor/A-4063-2008 OI Armesto, Nestor/0000-0003-0940-0783; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Ferretti, Alessandro/0000-0001-9084-5784; Kovalenko, Vladimir/0000-0001-6012-6615; Altsybeev, Igor/0000-0002-8079-7026; Vickovic, Linda/0000-0002-9820-7960; Fernandez Tellez, Arturo/0000-0003-0152-4220; Takahashi, Jun/0000-0002-4091-1779; Nattrass, Christine/0000-0002-8768-6468; Usai, Gianluca/0000-0002-8659-8378; Cosentino, Mauro/0000-0002-7880-8611; Suaide, Alexandre/0000-0003-2847-6556; Barnby, Lee/0000-0001-7357-9904; Peitzmann, Thomas/0000-0002-7116-899X; Kondratiev, Valery/0000-0002-0031-0741; Vinogradov, Leonid/0000-0001-9247-6230; Castillo Castellanos, Javier/0000-0002-5187-2779; Ferreiro, Elena/0000-0002-4449-2356; Felea, Daniel/0000-0002-3734-9439; Sevcenco, Adrian/0000-0002-4151-1056; de Cuveland, Jan/0000-0003-0455-1398; Kurepin, Alexey/0000-0002-1851-4136; Jena, Deepika/0000-0003-2112-0311; Jena, Satyajit/0000-0002-6220-6982; Vechernin, Vladimir/0000-0003-1458-8055; Akindinov, Alexander/0000-0002-7388-3022; De Pasquale, Salvatore/0000-0001-9236-0748; Chinellato, David/0000-0002-9982-9577; Pshenichnov, Igor/0000-0003-1752-4524 FU State Committee of Science, Armenia; World Federation of Scientists (WFS), Armenia; Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics; Academy of Finland; French CNRS-IN2P3, France; 'Region Pays de Loire', France; 'Region Alsace', France; 'Region Auvergne', France; CEA, France; German Bundesministerium fur Bildung; Wissenschaft; Forschung und Technologie (BMBF); Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian Orszagos Tudomanyos Kutatasi Alappgrammok (OTKA); National Office for Research and Technology (NKTH); Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN), Italy; Centro Fermi - Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; MEXT, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT), Mexico; Direccion General de Asuntos del Personal Academico (DGAPA), Mexico; Amerique Latine Formation academique - European Commission (ALFA-EC); EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM), Netherlands; Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics, Romania; National Council of Scientific Research in Higher Education (CNCSI-UEFISCDI), Romania; Ministry of Education and Science of the Russian Federation; Russian Academy of Sciences; Russian Federal Agency of Atomic Energy; Russian Federal Agency for Science and Innovations; Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, Republic of South Africa, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT); Ministerio de Economia y Competitividad (MINECO) of Spain; Xunta de Galicia (Conselleria de Educacion); Centro de Aplicaciones Tecnologicas y Desarrollo Nuclear (CEADEN), Cubaenergia, Cuba; IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut and Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); United States Department of Energy; United States National Science Foundation; State of Texas; State of Ohio; Ministry of Science, Education and Sports of Croatia; Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India FX The ALICE Collaboration would like to thank all its engineers and technicians for their invaluable contributions to the construction of the experiment and the CERN accelerator teams for the outstanding performance of the LHC complex. The ALICE Collaboration gratefully acknowledges the resources and support provided by all Grid centres and the Worldwide LHC Computing Grid (WLCG) Collaboration.; The ALICE Collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector: State Committee of Science, World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia, Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE) and the Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council, the Carlsberg Foundation and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics and the Academy of Finland; French CNRS-IN2P3, the 'Region Pays de Loire', 'Region Alsace', 'Region Auvergne' and CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung und Technologie (BMBF) and the Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian Orszagos Tudomanyos Kutatasi Alappgrammok (OTKA) and National Office for Research and Technology (NKTH); Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi - Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; MEXT Grant-in-Aid for Specially Promoted Research, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT), Direccion General de Asuntos del Personal Academico (DGAPA), Mexico, Amerique Latine Formation academique - European Commission (ALFA-EC) and the EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics and National Council of Scientific Research in Higher Education (CNCSI-UEFISCDI), Romania; Ministry of Education and Science of the Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations and The Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, Republic of South Africa, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT), E-Infrastructure shared between Europe and Latin America (EELA), Ministerio de Economia y Competitividad (MINECO) of Spain, Xunta de Galicia (Conselleria de Educacion), Centro de Aplicaciones Tecnologicas y Desarrollo Nuclear (CEADEN), Cubaenergia, Cuba, and IAEA (International Atomic Energy Agency); Swedish Research Council (VR) and Knut and Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); The United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio; Ministry of Science, Education and Sports of Croatia and Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India. NR 63 TC 9 Z9 9 U1 8 U2 31 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD MAR 10 PY 2016 VL 754 BP 360 EP 372 DI 10.1016/j.physletb.2016.01.040 PG 13 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DD0HM UT WOS:000369601000052 ER PT J AU Adam, J Adamova, D Aggarwal, MM Rinella, GA Agnello, M Agrawal, N Ahammed, Z Ahn, SU Aiola, S Akindinov, A Alam, SN Aleksandrov, D Alessandro, B Alexandre, D Molina, RA Alici, A Alkin, A Almaraz, JRM Alme, J Alt, T Altinpinar, S Altsybeev, I Prado, CAG Andrei, C Andronic, A Anguelov, V Anielski, J Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arcelli, S Arnaldi, R Arnold, OW Arsene, IC Arslandok, M Audurier, B Augustinus, A Averbeck, R Azmi, MD Badala, A Baek, YW Bagnasco, S Bailhache, R Bala, R Baldisseri, A Baral, RC Barbano, AM Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartalini, P Barth, K Bartke, J Bartsch, E Basile, M Bastid, N Basu, S Bathen, B Batigne, G Camejo, AB Batyunya, B Batzing, PC Bearden, IG Beck, H Bedda, C Behera, NK Belikov, I Bellini, F Martinez, HB Bellwied, R Belmont, R Belmont-Moreno, E Belyaev, V Bencedi, G Beole, S Berceanu, I Bercuci, A Berdnikov, Y Berenyi, D Bertens, RA Berzano, D Betev, L Bhasin, A Bhat, IR Bhati, AK Bhattacharjee, B Bhom, J Bianchi, L Bianchi, N Bianchin, C Bielcik, J Bielcikova, J Bilandzic, A Biswas, R Biswas, S Bjelogrlic, S Blair, JT Blau, D Blume, C Bock, F Bogdanov, A Boggild, H Boldizsar, L Bombara, M Book, J Borel, H Borissov, A Borri, M Bossu, F Botta, E Bottger, S Bourjau, C Braun-Munzinger, P Bregant, M Breitner, T Broker, TA Browning, TA Broz, M Brucken, EJ Bruna, E Bruno, GE Budnikov, D Buesching, H Bufalino, S Buncic, P Busch, O Buthelezi, Z Butt, JB Buxton, JT Caffarri, D Cai, X Caines, H Diaz, LC Caliva, A Villar, EC Camerini, P Carena, F Carena, W Carnesecchi, F Castellanos, JC Castro, AJ Casula, EAR Sanchez, CC Cepila, J Cerello, P Cerkala, J Chang, B Chapeland, S Chartier, M Charvet, JL Chattopadhyay, S Chattopadhyay, S Chelnokov, V Cherney, M Cheshkov, C Cheynis, B Barroso, VC Chinellato, DD Cho, S Chochula, P Choi, K Chojnacki, M Choudhury, S Christakoglou, P Christensen, CH Christiansen, P Chujo, T Chung, SU Cicalo, C Cifarelli, L Cindolo, F Cleymans, J Colamaria, F Colella, D Collu, A Colocci, M Balbastre, GC Del Valle, ZC Connors, ME Contreras, JG Cormier, TM Morales, YC Maldonado, IC Cortese, P Cosentino, MR Costa, F Crochet, P Albino, RC Cuautle, E Cunqueiro, L Dahms, T Dainese, A Danu, A Das, D Das, I Das, S Dash, A Dash, S De, S De Caro, A De Cataldo, G De Conti, C De Cuveland, J De Falco, A De Gruttola, D De Marco, N De Pasquale, S Deisting, A Deloff, A Denes, E Deplano, C Dhankher, P Di Bari, D Di Mauro, A Di Nezza, P Corchero, MAD Dietel, T Dillenseger, P Divia, R Djuvsland, O Dobrin, A Gimenez, DD Donigus, B Dordic, O Drozhzhova, T Dubey, AK Dubla, A Ducroux, L Dupieux, P Ehlers, RJ Elia, D Engel, H Epple, E Erazmus, B Erdemir, I Erhardt, F Espagnon, B Estienne, M Esumi, S Eum, J Evans, D Evdokimov, S Eyyubova, G Fabbietti, L Fabris, D Faivre, J Fantoni, A Fasel, M Feldkamp, L Feliciello, A Feofilov, G Ferencei, J Tellez, AF Ferreiro, EG Ferretti, A Festanti, A Feuillard, VJG Figiel, J Figueredo, MAS Filchagin, S Finogeev, D Fionda, FM Fiore, EM Fleck, MG Floris, M Foertsch, S Foka, P Fokin, S Fragiacomo, E Francescon, A Frankenfeld, U Fuchs, U Furget, C Furs, A Girard, MF Gaardhoje, JJ Gagliardi, M Gago, AM Gallio, M Gangadharan, DR Ganoti, P Gao, C Garabatos, C Garcia-Solis, E Gargiulo, C Gasik, P Gauger, EF Germain, M Gheata, A Gheata, M Ghosh, P Ghosh, SK Gianotti, P Giubellino, P Giubilato, P Gladysz-Dziadus, E Glassel, P Coral, DMG Ramirez, AG Gonzalez, V Gonzalez-Zamora, P Gorbunov, S Gorlich, L Gotovac, S Grabski, V Grachov, OA Graczykowski, LK Graham, KL Grelli, A Grigoras, A Grigoras, C Grigoriev, V Grigoryan, A Grigoryan, S Grinyov, B Grion, N Gronefeld, JM Grosse-Oetringhaus, JF Grossiord, JY Grosso, R Guber, F Guernane, R Guerzoni, B Gulbrandsen, K Gunji, T Gupta, A Gupta, R Haake, R Haaland, O Hadjidakis, C Haiduc, M Hamagaki, H Hamar, G Harris, JW Harton, A Hatzifotiadou, D Hayashi, S Heckel, ST Heide, M Helstrup, H Herghelegiu, A Corral, GH Hess, BA Hetland, KF Hillemanns, H Hippolyte, B Hosokawa, R Hristov, P Huang, M Humanic, TJ Hussain, N Hussain, T Hutter, D Hwang, DS Ilkaev, R Inaba, M Ippolitov, M Irfan, M Ivanov, M Ivanov, V Izucheev, V Jacobs, PM Jadhav, MB Jadlovska, S Jadlovsky, J Jahnke, C Jakubowska, MJ Jang, HJ Janik, MA Jayarathna, PHSY Jena, C Jena, S Bustamante, RTJ Jones, PG Jung, H Jusko, A Kalinak, P Kalweit, A Kamin, J Kang, JH Kaplin, V Kar, S Uysal, AK Karavichev, O Karavicheva, T Karayan, L Karpechev, E Kebschull, U Keidel, R Keijdener, DLD Keil, M Khan, MM Khan, P Khan, SA Khanzadeev, A Kharlov, Y Kileng, B Kim, DW Kim, DJ Kim, D Kim, H Kim, JS Kim, M Kim, M Kim, S Kim, T Kirsch, S Kisel, I Kiselev, S Kisiel, A Kiss, G Klay, JL Klein, C Klein, J Klein-Bosing, C Klewin, S Kluge, A Knichel, ML Knospe, AG Kobayashi, T Kobdaj, C Kofarago, M Kollegger, T Kolojvari, A Kondratiev, V Kondratyeva, N Kondratyuk, E Konevskikh, A Kopcik, M Kour, M Kouzinopoulos, C Kovalenko, O Kovalenko, V Kowalski, M Meethaleveedu, GK Kralik, I Kravcakova, A Kretz, M Krivda, M Krizek, F Kryshen, E Krzewicki, M Kubera, AM Kucera, V Kuhn, C Kuijer, PG Kumar, A Kumar, J Kumar, L Kumar, S Kurashvili, P Kurepin, A Kurepin, AB Kuryakin, A Kweon, MJ Kwon, Y La Pointe, SL La Rocca, P De Guevara, PL Fernandes, CL Lakomov, I Langoy, R Lara, C Lardeux, A Lattuca, A Laudi, E Lea, R Leardini, L Lee, GR Lee, S Lehas, F Lemmon, RC Lenti, V Leogrande, E Monzon, IL Vargas, HL Leoncino, M Levai, P Li, S Li, X Lien, J Lietava, R Lindal, S Lindenstruth, V Lippmann, C Lisa, MA Ljunggren, HM Lodato, DF Loenne, PI Loginov, V Loizides, C Lopez, X Torres, EL Lowe, A Luettig, P Lunardon, M Luparello, G Maevskaya, A Mager, M Mahajan, S Mahmood, SM Maire, A Majka, RD Malaev, M Cervantes, IM Iii, LM Mal'Kevich, D Malzacher, P Mamonov, A Manko, V Manso, 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CA ALICE Collaboration TI Centrality evolution of the charged-particle pseudorapidity density over a broad pseudorapidity range in Pb-Pb collisions at root s(NN)=2.76TeV SO PHYSICS LETTERS B LA English DT Article AB The centrality dependence of the charged-particle pseudorapidity density measured with ALICE in Pb-Pb collisions at root s(NN) = 2.76 TeV over a broad pseudorapidity range is presented. This Letter extends the previous results reported by ALICE to more peripheral collisions. No strong change of the overall shape of charged-particle pseudorapidity density distributions with centrality is observed, and when normalised to the number of participating nucleons in the collisions, the evolution over pseudorapidity with centrality is likewise small. The broad pseudorapidity range (-3.5 < eta < 5) allows precise estimates of the total number of produced charged particles which we find to range from 162 +/- 22(syst.) to 17170 +/- 770(syst.) in 80-90% and 0-5% central collisions, respectively. The total charged-particle multiplicity is seen to approximately scale with the number of participating nucleons in the collision. This suggests that hard contributions to the charged-particle multiplicity are limited. The results are compared to models which describe dN(ch)/d(eta) at mid-rapidity in the most central Pb-Pb collisions and it is found that these models do not capture all features of the distributions. (C) 2016 CERN for the benefit of the ALICE Collaboration. Published by Elsevier B.V. C1 [Grigoryan, A.; Papikyan, V.] Yerevan Phys Inst Fdn, AI Alikhanyan Natl Sci Lab, Yerevan, Armenia. [Martinez, H. Bello; Maldonado, I. Cortes; Tellez, A. Fernandez; Martinez, M. I.; Moreno, L. A. P.; Noris, J. C. C.; Cahuantzi, M. 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[Bartke, J.; Figiel, J.; Gladysz-Dziadus, E.; Gorlich, L.; Kowalski, M.; Matyja, A.; Mayer, C.; Otwinowski, J.; Rybicki, A.; Sputowska, I.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Blair, J. T.; Gauger, E. F.; Knospe, A. G.; Markert, C.; Thomas, D.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Almaraz, J. R. M.; Monzon, I. Leon; Podesta-Lerma, P. L. M.] Univ Autonoma Sinaloa, Culiacan, Mexico. [Prado, C. Alves Garcia; Bregant, M.; Cosentino, M. R.; De, S.; De Conti, C.; Gimenez, D. Domenicis; Figueredo, M. A. S.; Jahnke, C.; Fernandes, C. Lagana; Mas, A.; Munhoz, M. G.; Da Luz, H. Natal; Da Silva, A. C. Oliveira; De Oliveira, E. Pereira; Suaide, A. A. P.; De Toledo, A. Szanto; Zanoli, H. J. C.] Univ Sao Paulo, BR-09500900 Sao Paulo, Brazil. [Chinellato, D. D.; Dash, A.; Takahashi, J.] Univ Estadual Campinas UNICAMP, Campinas, SP, Brazil. [Bellwied, R.; Bianchi, L.; Jayarathna, P. H. S. 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[Belmont, R.; Bianchin, C.; Pan, J.; Pruneau, C. A.; Pujahari, P.; Putschke, J.; Reed, R. J.; Saleh, M. A.; Verweij, M.; Voloshin, S. A.; Yaldo, C. G.] Wayne State Univ, Detroit, MI USA. [Barnafoldi, G. G.; Bencedi, G.; Berenyi, D.; Boldizsar, L.; Denes, E.; Hamar, G.; Kiss, G.; Levai, P.; Lowe, A.; Olah, L.; Pochybova, S.; Varga, D.; Volpe, G.] Hungarian Acad Sci, Wigner Res Ctr Phys, Budapest, Hungary. [Aiola, S.; Caines, H.; Connors, M. E.; Ehlers, R. J.; Epple, E.; Grachov, O. A.; Harris, J. W.; Majka, R. D.; Mulligan, J. D.; Oh, S.; Oliver, M. H.; Schuster, T.; Smirnov, N.] Yale Univ, New Haven, CT USA. [Kang, J. H.; Kim, D.; Kim, H.; Kim, M.; Kim, T.; Kwon, Y.; Lee, S.; Song, M.] Yonsei Univ, Seoul 120749, South Korea. [Keidel, R.] ZTT, Fachhsch Worms, Worms, Germany. [Connors, M. E.] Georgia State Univ, Atlanta, GA 30303 USA. [Iii, L. Malinina] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl, Phys, Moscow, Russia. RP Adam, J (reprint author), Czech Tech Univ, Fac Nucl Sci & Phys Engn, CR-11519 Prague, Czech Republic. RI Natal da Luz, Hugo/F-6460-2013; Martinez Hernandez, Mario Ivan/F-4083-2010; Ferretti, Alessandro/F-4856-2013; Kovalenko, Vladimir/C-5709-2013; Altsybeev, Igor/K-6687-2013; Vickovic, Linda/F-3517-2017; Fernandez Tellez, Arturo/E-9700-2017; Nattrass, Christine/J-6752-2016; Usai, Gianluca/E-9604-2015; Cosentino, Mauro/L-2418-2014; Suaide, Alexandre/L-6239-2016; Barnby, Lee/G-2135-2010; Peitzmann, Thomas/K-2206-2012; Kondratiev, Valery/J-8574-2013; Vinogradov, Leonid/K-3047-2013; Castillo Castellanos, Javier/G-8915-2013; Ferreiro, Elena/C-3797-2017; de Cuveland, Jan/H-6454-2016; Kurepin, Alexey/H-4852-2013; Jena, Deepika/P-2873-2015; Jena, Satyajit/P-2409-2015; Vechernin, Vladimir/J-5832-2013; Akindinov, Alexander/J-2674-2016; Takahashi, Jun/B-2946-2012; De Pasquale, Salvatore/B-9165-2008; Chinellato, David/D-3092-2012; Pshenichnov, Igor/A-4063-2008; Bregant, Marco/I-7663-2012; Sevcenco, Adrian/C-1832-2012 OI Natal da Luz, Hugo/0000-0003-1177-870X; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Ferretti, Alessandro/0000-0001-9084-5784; Kovalenko, Vladimir/0000-0001-6012-6615; Altsybeev, Igor/0000-0002-8079-7026; Vickovic, Linda/0000-0002-9820-7960; Fernandez Tellez, Arturo/0000-0003-0152-4220; Nattrass, Christine/0000-0002-8768-6468; Usai, Gianluca/0000-0002-8659-8378; Cosentino, Mauro/0000-0002-7880-8611; Suaide, Alexandre/0000-0003-2847-6556; Barnby, Lee/0000-0001-7357-9904; Peitzmann, Thomas/0000-0002-7116-899X; Kondratiev, Valery/0000-0002-0031-0741; Vinogradov, Leonid/0000-0001-9247-6230; Castillo Castellanos, Javier/0000-0002-5187-2779; Ferreiro, Elena/0000-0002-4449-2356; de Cuveland, Jan/0000-0003-0455-1398; Kurepin, Alexey/0000-0002-1851-4136; Jena, Deepika/0000-0003-2112-0311; Jena, Satyajit/0000-0002-6220-6982; Vechernin, Vladimir/0000-0003-1458-8055; Akindinov, Alexander/0000-0002-7388-3022; Takahashi, Jun/0000-0002-4091-1779; De Pasquale, Salvatore/0000-0001-9236-0748; Chinellato, David/0000-0002-9982-9577; Pshenichnov, Igor/0000-0003-1752-4524; Sevcenco, Adrian/0000-0002-4151-1056 FU State Committee of Science, Armenia; World Federation of Scientists (WFS), Armenia; Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics; Academy of Finland; French CNRS-IN2P3, France; 'Region Pays de Loire', France; 'Region Alsace', France; 'Region Auvergne', France; CEA, France; German Bundesministerium fur Bildung; Wissenschaft; Forschung und Technologie (BMBF); Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; National Research, Development and Innovation Office (NKFIH), Hungary; Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN), Italy; Centro Fermi-Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; Japan Society for the Promotion of Science (JSPS) KAKENHI, Japan; MEXT, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT); Direccion General de Asuntos del Personal Academico (Direccion General Asuntos del Personal Academico, Universidad Nacional Autonoma de Mexico), Mexico; Amerique Latine Formation academique-European Commission (ALFA-EC); EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM), Netherlands; Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics, Romania; National Council of Scientific Research in Higher Education (CNCSI-UEFISCDI), Romania; Ministry of Education and Science of Russian Federation; Russian Academy of Sciences; Russian Federal Agency of Atomic Energy; Russian Federal Agency for Science and Innovations; Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT); Ministerio de Economia y Competitividad (MINECO) of Spain; Xunta de Galicia (Conselleria de Educacion); Centro de Aplicaciones Tecnologicas y Desarrollo Nuclear (CEADEN), Cubaenergia, Cuba; IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut AMP; Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); United States Department of Energy; United States National Science Foundation; State of Texas; State of Ohio; Ministry of Science, Education and Sports of Croatia; Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India; Pontificia Universidad Catolica del Peru FX The ALICE Collaboration would like to thank all its engineers and technicians for their invaluable contributions to the construction of the experiment and the CERN accelerator teams for the outstanding performance of the LHC complex. The ALICE Collaboration gratefully acknowledges the resources and support provided by all Grid centres and the Worldwide LHC Computing Grid (WLCG) Collaboration.; r The ALICE Collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector: State Committee of Science, World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE) and the Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council, the Carlsberg Foundation and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics and the Academy of Finland; French CNRS-IN2P3, the 'Region Pays de Loire', 'Region Alsace', 'Region Auvergne' and CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung und Technologie (BMBF) and the Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; National Research, Development and Innovation Office (NKFIH), Hungary; Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi-Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; Japan Society for the Promotion of Science (JSPS) KAKENHI and MEXT, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT), Direccion General de Asuntos del Personal Academico (Direccion General Asuntos del Personal Academico, Universidad Nacional Autonoma de Mexico), Mexico, Amerique Latine Formation academique-European Commission (ALFA-EC) and the EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics and National Council of Scientific Research in Higher Education (CNCSI-UEFISCDI), Romania; Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations and The Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT), E-Infrastructure shared between Europe and Latin America (EELA), Ministerio de Economia y Competitividad (MINECO) of Spain, Xunta de Galicia (Conselleria de Educacion), Centro de Aplicaciones Tecnologicas y Desarrollo Nuclear (CEADEN), Cubaenergia, Cuba, and IAEA (International Atomic Energy Agency); Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); The United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio; Ministry of Science, Education and Sports of Croatia and Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India; Pontificia Universidad Catolica del Peru. NR 18 TC 3 Z9 3 U1 6 U2 26 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD MAR 10 PY 2016 VL 754 BP 373 EP 385 DI 10.1016/j.physletb.2015.12.082 PG 13 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DD0HM UT WOS:000369601000053 ER PT J AU Craig, N Gu, JY Liu, Z Wang, KC AF Craig, Nathaniel Gu, Jiayin Liu, Zhen Wang, Kechen TI Beyond Higgs couplings: probing the Higgs with angular observables at future e(+)e(-) colliders SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Beyond Standard Model; Effective field theories; Higgs Physics ID BOSON; LHC AB We study angular observables in the e(+)e(-) -> ZH -> l(+)l(-) b (b) over bar channel at future circular e(+)e(-) colliders such as CEPC and FCC-ee. Taking into account the impact of realistic cut acceptance and detector effects, we forecast the precision of six angular asymmetries at CEPC (FCC-ee) with center-of-mass energy root s = 240 GeV and 5 (30) ab(-1) integrated luminosity. We then determine the projected sensitivity to a range of operators relevant for the Higgs-strahlung process in the dimension-6 Higgs EFT. Our results show that angular observables provide complementary sensitivity to rate measurements when constraining various tensor structures arising from new physics. We further find that angular asymmetries provide a novel means of both probing BSM corrections to the HZ gamma coupling and constraining the "blind spot" in indirect limits on supersymmetric scalar top partners. C1 [Craig, Nathaniel] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Gu, Jiayin; Wang, Kechen] Chinese Acad Sci, Inst High Energy Phys, Ctr Future High Energy Phys, Beijing 100049, Peoples R China. [Liu, Zhen] Fermilab Natl Accelerator Lab, Dept Theoret Phys, POB 500, Batavia, IL 60510 USA. RP Craig, N (reprint author), Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA.; Gu, JY; Wang, KC (reprint author), Chinese Acad Sci, Inst High Energy Phys, Ctr Future High Energy Phys, Beijing 100049, Peoples R China.; Liu, Z (reprint author), Fermilab Natl Accelerator Lab, Dept Theoret Phys, POB 500, Batavia, IL 60510 USA. EM ncraig@physics.ucsb.edu; gujy@ihep.ac.cn; zliu2@fnal.gov; kechen@ihep.ac.cn OI Liu, Zhen/0000-0002-3143-1976 FU Department of Energy [DE-SC0014129]; United States Department of Energy [DE-AC02-07CH11359]; CAS Center for Excellence in Particle Physics (CCEPP); Chinese Academy of Science (CAS) International Traveling Award [H95120N1U7] FX We thank Gang Li and Xin Mo for providing us the CEPC pre-CDR simulation events. We thank Nima Arkani-Hamed, Marco Farina, Marat Freytsis, Matthew McCullough, Maxim Perelstein, Matt Reece, and Lian-Tao Wang for useful conversations. KW and JG also thank Cai-Dian Lu for assistance. NC is supported by the Department of Energy under the grant DE-SC0014129. NC and ZL acknowledge the hospitality of the IHEP Center for Future High Energy Physics where this work was initiated. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. KW and JG are supported in part by the CAS Center for Excellence in Particle Physics (CCEPP). JG is also supported in part by the Chinese Academy of Science (CAS) International Traveling Award under Grant H95120N1U7. NR 44 TC 2 Z9 2 U1 1 U2 2 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAR 9 PY 2016 IS 3 AR 050 DI 10.1007/JHEP03(2016)050 PG 28 WC Physics, Particles & Fields SC Physics GA DL0BF UT WOS:000375295500002 ER PT J AU El-Sawy, AM Mosa, IM Su, D Guild, CJ Khalid, S Joesten, R Rusling, JF Suib, SL AF El-Sawy, Abdelhamid M. Mosa, Islam M. Su, Dong Guild, Curtis J. Khalid, Syed Joesten, Raymond Rusling, James F. Suib, Steven L. TI Controlling the Active Sites of Sulfur-Doped Carbon Nanotube-Graphene Nanolobes for Highly Efficient Oxygen Evolution and Reduction Catalysis SO ADVANCED ENERGY MATERIALS LA English DT Article DE bifunctional catalysts; metal-free catalysis; oxygen evolution reaction; oxygen reduction reaction; nanolobes ID WATER OXIDATION; MANGANESE OXIDE; ELECTROCATALYTIC ACTIVITY; BIFUNCTIONAL ELECTROCATALYST; NITROGEN; PERFORMANCE; NANOCRYSTALS; ELECTROLYSIS; NANORIBBONS; PHOTOANODES AB Controlling active sites of metal-free catalysts is an important strategy to enhance activity of the oxygen evolution reaction (OER). Many attempts have been made to develop metal-free catalysts, but the lack of understanding of active-sites at the atomic-level has slowed the design of highly active and stable metal-free catalysts. A sequential two-step strategy to dope sulfur into carbon nanotube-graphene nanolobes is developed. This bidoping strategy introduces stable sulfur-carbon active-sites. Fluorescence emission of the sulfur K-edge by X-ray absorption near edge spectroscopy (XANES) and scanning transmission electron microscopy electron energy loss spectroscopy (STEM-EELS) mapping and spectra confirm that increasing the incorporation of heterocyclic sulfur into the carbon ring of CNTs not only enhances OER activity with an overpotential of 350 mV at a current density of 10 mA cm(-2), but also retains 100% of stability after 75 h. The bidoped sulfur carbon nanotube-graphene nanolobes behave like the state-of-the-art catalysts for OER but outperform those systems in terms of turnover frequency (TOF) which is two orders of magnitude greater than (20% Ir/C) at 400 mV overpotential with very high mass activity 1000 mA cm(-2) at 570 mV. Moreover, the sulfur bidoping strategy shows high catalytic activity for the oxygen reduction reaction (ORR). Stable bifunctional (ORR and OER) catalysts are low cost, and light-weight bidoped sulfur carbon nanotubes are potential candidates for next-generation metal-free regenerative fuel cells. C1 [El-Sawy, Abdelhamid M.; Mosa, Islam M.; Guild, Curtis J.; Joesten, Raymond; Rusling, James F.; Suib, Steven L.] Univ Connecticut, Dept Chem, U-60, Storrs, CT 06269 USA. [El-Sawy, Abdelhamid M.; Rusling, James F.; Suib, Steven L.] Univ Connecticut, Inst Mat Sci, Storrs, CT 06269 USA. [El-Sawy, Abdelhamid M.; Mosa, Islam M.] Tanta Univ, Fac Sci, Dept Chem, Tanta 31527, Egypt. [Su, Dong] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Khalid, Syed] Brookhaven Natl Lab, Photon Sci Directorate, Upton, NY 11973 USA. [Suib, Steven L.] Univ Connecticut, Chem & Biomol Engn, Storrs, CT 06269 USA. RP Suib, SL (reprint author), Univ Connecticut, Dept Chem, U-60, Storrs, CT 06269 USA. EM steven.suib@uconn.edu RI Su, Dong/A-8233-2013 OI Su, Dong/0000-0002-1921-6683 FU Department of Energy, Office of Basic Energy Sciences, Division of Chemical, Geological and Biological Sciences [DE-FGO2-86ER13622.A000]; Ministry of Higher Education in Egypt; [1126100] FX The authors thank the Department of Energy, Office of Basic Energy Sciences, Division of Chemical, Geological and Biological Sciences under Grant No. DE-FGO2-86ER13622.A000 for support of this work. We gratefully acknowledge the assistance of the Bioscience Electron Microscopy Laboratory of the University of Connecticut and Grant No. 1126100 for the purchase of the FEI NovaSEM. A.M.E., and I.M.S. thank the Ministry of Higher Education in Egypt for financial support. NR 46 TC 23 Z9 23 U1 65 U2 220 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD MAR 9 PY 2016 VL 6 IS 5 AR 1501966 DI 10.1002/aenm.201501966 PG 12 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA DH1DV UT WOS:000372525500008 ER PT J AU Lopez, N Yu, KM Tanaka, T Walukiewicz, W AF Lopez, Nair Yu, Kin Man Tanaka, Tooru Walukiewicz, Wladyslaw TI Multicolor Electroluminescence from Intermediate Band Solar Cell Structures SO ADVANCED ENERGY MATERIALS LA English DT Article DE band anticrossing; dilute nitride alloys; photovoltaic devices; solar cells ID ALLOYS; SEMICONDUCTORS; EFFICIENCY AB Intermediate band solar cells are a new generation of photovoltaics that allow for better utilization of the solar spectrum. The key and most challenging requirement for these cells is an efficient optical coupling between the intermediate band and the charge conducting bands. GaNAs based intermediate band solar cells have been used to generate electroluminescence. Two electroluminescence peaks are generated in the structure with electrically blocked intermediate band. The peaks are observed for both forward and reverse bias configuration and are attributed to optical transitions from the conduction to the intermediate band, and from the intermediate band to the valence band. The origin of the electroluminescence is confirmed by the temperature dependence of the electroluminescence peak energies that is consistent with the band anticrossing model of the intermediate band formation in dilute nitride alloys. This is the first direct observation of the optical transitions required for the operation of intermediate band solar cells. The results also demonstrate that properly modified intermediate band solar cell structures could be used as multicolor light emitters. C1 [Lopez, Nair] Univ Autonoma Madrid, Dept Fis Aplicada, C Francisco Tomas & Valiente 7, E-28049 Madrid, Spain. [Yu, Kin Man] City Univ Hong Kong, Dept Phys & Mat Sci, Kowloon, Hong Kong, Peoples R China. [Tanaka, Tooru] Saga Univ, Dept Elect & Elect Engn, Saga 8408502, Japan. [Walukiewicz, Wladyslaw] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Walukiewicz, W (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM w_walukiewicz@lbl.gov OI Tanaka, Tooru/0000-0001-5747-1717; Yu, Kin Man/0000-0003-1350-9642 FU Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division of the U.S. Department of Energy [DE-AC02-05CH11231]; European Commission [PIIF-GA-2012-326579]; LBNL's LDRD fund FX This work was performed at the EMAT, LBNL and was supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. N.L. acknowledges support from the European Commission by Marie Curie International Incoming Fellowship PIIF-GA-2012-326579 and from LBNL's LDRD fund. W.W. and K.M.Y. designed the IBSC structures and provided the interpretation of the experimental results. N.L. fabricated the devices and performed the electroluminescence measurements. All the authors discussed the results and N.L. and W.W. wrote the manuscript. Material growth and device fabrication was partially supported by RoseStreet Labs Energy. NR 23 TC 2 Z9 2 U1 6 U2 22 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD MAR 9 PY 2016 VL 6 IS 5 AR 1501820 DI 10.1002/aenm.201501820 PG 5 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA DH1DV UT WOS:000372525500006 ER PT J AU Sullivan, KT Zhu, C Duoss, EB Gash, AE Kolesky, DB Kuntz, JD Lewis, JA Spadaccini, CM AF Sullivan, Kyle T. Zhu, Cheng Duoss, Eric B. Gash, Alexander E. Kolesky, David B. Kuntz, Joshua D. Lewis, Jennifer A. Spadaccini, Christopher M. TI Controlling Material Reactivity Using Architecture SO ADVANCED MATERIALS LA English DT Article ID NEGATIVE POISSONS RATIO; ENERGETIC COMPOSITES; METAMATERIALS; ULTRALIGHT; BEHAVIOR; AL/MOO3 AB 3D-printing methods are used to generate reactive material architectures. Several geometric parameters are observed to influence the resultant flame propagation velocity, indicating that the architecture can be utilized to control reactivity. Two different architectures, channels and hurdles, are generated, and thin films of thermite are deposited onto the surface. The architecture offers an additional route to control, at will, the energy release rate in reactive composite materials. C1 [Sullivan, Kyle T.; Zhu, Cheng; Duoss, Eric B.; Gash, Alexander E.; Kuntz, Joshua D.; Spadaccini, Christopher M.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Kolesky, David B.; Lewis, Jennifer A.] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. [Kolesky, David B.; Lewis, Jennifer A.] Harvard Univ, Wyss Inst Biol Inspired Engn, Cambridge, MA 02138 USA. RP Sullivan, KT (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM sullivan34@llnl.gov RI ZHU, CHENG/J-4692-2016 FU Laboratory Directed Research and Development Strategic Initiative Program [11-SI-004]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Department of Energy, Energy Frontier Research Center on Light-Material Interactions in Energy Conversion [DE-SC0001293] FX K.T.S. and C.Z. contributed equally to this work. This work was funded by the Laboratory Directed Research and Development Strategic Initiative Program, 11-SI-004, and performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. IM release LLNL-JRNL-678526. D.K. and J.A.L. gratefully acknowledge funding from the Department of Energy, Energy Frontier Research Center on Light-Material Interactions in Energy Conversion under Grant DE-SC0001293. NR 26 TC 3 Z9 3 U1 25 U2 77 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD MAR 9 PY 2016 VL 28 IS 10 BP 1934 EP + DI 10.1002/adma.201504286 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DG8BZ UT WOS:000372308700003 PM 26669517 ER PT J AU Doubek, G Sekol, RC Li, JY Ryu, WH Gittleson, FS Nejati, S Moy, E Reid, C Carmo, M Linardi, M Bordeenithikasem, P Kinser, E Liu, YH Tong, X Osuji, CO Schroers, J Mukherjee, S Taylor, AD AF Doubek, Gustavo Sekol, Ryan C. Li, Jinyang Ryu, Won-Hee Gittleson, Forrest S. Nejati, Siamak Moy, Eric Reid, Candy Carmo, Marcelo Linardi, Marcelo Bordeenithikasem, Punnathat Kinser, Emily Liu, Yanhui Tong, Xiao Osuji, Chinedum O. Schroers, Jan Mukherjee, Sundeep Taylor, Andre D. TI Guided Evolution of Bulk Metallic Glass Nanostructures: A Platform for Designing 3D Electrocatalytic Surfaces SO ADVANCED MATERIALS LA English DT Article ID OXYGEN REDUCTION ELECTROCATALYSTS; FUEL-CELL; METHANOL OXIDATION; CATALYTIC-ACTIVITY; ALLOY NANOPARTICLES; ENHANCED ACTIVITY; LI-O-2 BATTERIES; ALKALINE MEDIA; PLATINUM; RUTHENIUM AB Electrochemical devices such as fuel cells, electrolyzers, lithium-air batteries, and pseudocapacitors are expected to play a major role in energy conversion/storage in the near future. Here, it is demonstrated how desirable bulk metallic glass compositions can be obtained using a combinatorial approach and it is shown that these alloys can serve as a platform technology for a wide variety of electrochemical applications through several surface modification techniques. C1 [Doubek, Gustavo; Sekol, Ryan C.; Li, Jinyang; Ryu, Won-Hee; Gittleson, Forrest S.; Nejati, Siamak; Moy, Eric; Reid, Candy; Carmo, Marcelo; Osuji, Chinedum O.; Taylor, Andre D.] Yale Univ, Dept Chem & Environm Engn, New Haven, CT 06520 USA. [Doubek, Gustavo; Sekol, Ryan C.; Nejati, Siamak; Moy, Eric; Reid, Candy; Carmo, Marcelo; Bordeenithikasem, Punnathat; Kinser, Emily; Liu, Yanhui; Osuji, Chinedum O.; Schroers, Jan; Mukherjee, Sundeep; Taylor, Andre D.] Yale Univ, Ctr Res Interface Struct & Phenomena, New Haven, CT 06520 USA. [Doubek, Gustavo; Linardi, Marcelo] IPEN CNEN SP, Hydrogen & Fuel Cell Ctr, Nucl & Energy Res Inst, Av Prof Lineu Prestes, BR-05508000 Sao Paulo, SP, Brazil. [Bordeenithikasem, Punnathat; Kinser, Emily; Liu, Yanhui; Schroers, Jan] Yale Univ, Dept Mech Engn & Mat Sci, New Haven, CT 06520 USA. [Tong, Xiao] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Doubek, Gustavo] Univ Campinas UNICAMP, Sch Chem Engn, BR-13083852 Campinas, SP, Brazil. [Sekol, Ryan C.] Gen Motors Res & Dev, Warren, MI 48090 USA. [Gittleson, Forrest S.] Sandia Natl Labs, Livermore, CA 94550 USA. [Carmo, Marcelo] Forschungszentrum Julich, IEK 3, D-52428 Julich, Germany. [Mukherjee, Sundeep] Univ N Texas, Dept Mat Sci & Engn, Denton, TX 76203 USA. RP Taylor, AD (reprint author), Yale Univ, Dept Chem & Environm Engn, New Haven, CT 06520 USA.; Taylor, AD (reprint author), Yale Univ, Ctr Res Interface Struct & Phenomena, New Haven, CT 06520 USA. EM andre.taylor@yale.edu RI Linardi, Marcelo/C-9552-2013; Doubek, Gustavo/B-2163-2017; Ryu, Won-Hee/F-8375-2014; OI Doubek, Gustavo/0000-0001-9349-4801; Ryu, Won-Hee/0000-0002-0203-2992; gittleson, forrest/0000-0003-0360-8348; Osuji, Chinedum/0000-0003-0261-3065 FU NSF [MRSEC DMR 1119826]; NSF-PECASE award [CBET-0954985]; Fapesp [2014/09087-4]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX G.D., R.C.S., and J.L. contributed equally to this work. The authors are grateful for support from NSF under Grant No. MRSEC DMR 1119826 (CRISP). G.D. thanks CAPES foundation, Ministry of Education of Brazil. A.D.T. also thanks the AFOSR (FA9550-11-1-0219) and NSF-PECASE award (CBET-0954985). W.-H.R. thanks The NatureNet Program of The Nature Conervancy. G.D. and M.L. acknowledge funding from Fapesp 2014/09087-4. Facilities use was supported by YINQE, NSF MRSEC DMR 1119826 (CRISP). Research was carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 64 TC 5 Z9 5 U1 36 U2 97 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD MAR 9 PY 2016 VL 28 IS 10 BP 1940 EP + DI 10.1002/adma.201504504 PG 11 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DG8BZ UT WOS:000372308700004 PM 26689722 ER PT J AU Bai, F Li, BS Bian, KF Haddad, R Wu, HM Wang, ZW Fan, HY AF Bai, Feng Li, Binsong Bian, Kaifu Haddad, Raid Wu, Huimeng Wang, Zhongwu Fan, Hongyou TI Pressure-Tuned Structure and Property of Optically Active Nanocrystals SO ADVANCED MATERIALS LA English DT Article ID PHASE-TRANSFORMATION; CRYSTALLIZATION; NANOCOMPOSITES; NANOPARTICLES; NANOSHEETS; POLYMERS; CRYSTAL AB Investigations through high-pressure X-ray scattering and spectroscopy in combination with theoretical computations shows that high-pressure compression can systematically tune the optical properties and mechanical stability of the molecular nanocrystals. C1 [Bai, Feng] Henan Univ, Key Lab Special Funct Mat, Minist Educ, Kaifeng 475004, Peoples R China. [Li, Binsong; Bian, Kaifu; Wu, Huimeng; Fan, Hongyou] Sandia Natl Labs, Adv Mat Lab, 1001 Univ Blvd SE, Albuquerque, NM 87106 USA. [Haddad, Raid; Fan, Hongyou] Univ New Mexico, Ctr Microengn Mat, Dept Chem & Biol Engn, Albuquerque, NM 87131 USA. [Wang, Zhongwu] Cornell Univ, Cornell High Energy Synchrotron Source, Ithaca, NY 14853 USA. RP Bai, F (reprint author), Henan Univ, Key Lab Special Funct Mat, Minist Educ, Kaifeng 475004, Peoples R China.; Fan, HY (reprint author), Sandia Natl Labs, Adv Mat Lab, 1001 Univ Blvd SE, Albuquerque, NM 87106 USA.; Fan, HY (reprint author), Univ New Mexico, Ctr Microengn Mat, Dept Chem & Biol Engn, Albuquerque, NM 87131 USA. EM baifengsun@gmail.com; hfan@sandia.gov FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; National Science Foundation; National Institutes of Heath/National Institute of General Medical Sciences under NSF [DMR-0936384]; National Natural Science Foundation of China [21422102, 21171049, 50828302]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX F.B., B.L., and K.B. contributed equally to this work. This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. The Cornell High Energy Synchrotron Source (CHESS) was supported by the National Science Foundation and the National Institutes of Heath/National Institute of General Medical Sciences under NSF award DMR-0936384. F.B. acknowledges the support from the National Natural Science Foundation of China (21422102, 21171049, and 50828302). Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 28 TC 1 Z9 1 U1 16 U2 46 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD MAR 9 PY 2016 VL 28 IS 10 BP 1989 EP + DI 10.1002/adma.201504819 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DG8BZ UT WOS:000372308700011 PM 26755432 ER PT J AU Haynes, BF Shaw, GM Korber, B Kelsoe, G Sodroski, J Hahn, BH Borrow, P McMichael, AJ AF Haynes, Barton F. Shaw, George M. Korber, Bette Kelsoe, Garnett Sodroski, Joseph Hahn, Beatrice H. Borrow, Persephone McMichael, Andrew J. TI HIV-Host Interactions: Implications for Vaccine Design SO CELL HOST & MICROBE LA English DT Review ID BROADLY NEUTRALIZING ANTIBODIES; HIGHLY PATHOGENIC SIV; T-CELL RESPONSES; TEST-OF-CONCEPT; GERMINAL-CENTER; RHESUS-MONKEYS; B-CELLS; IMMUNE-RESPONSES; TRANSMITTED-FOUNDER; PROTECTIVE EFFICACY AB Development of an effective AIDS vaccine is a global priority. However, the extreme diversity of HIV type 1 (HIV-1), which is a consequence of its propensity to mutate to escape immune responses, along with host factors that prevent the elicitation of protective immune responses, continue to hinder vaccine development. Breakthroughs in understanding of the biology of the transmitted virus, the structure and nature of its envelope trimer, vaccine-induced CD8 T cell control in primates, and host control of broadly neutralizing antibody elicitation have given rise to new vaccine strategies. Despite this promise, emerging data from preclinical trials reinforce the need for additional insight into virus-host biology in order to facilitate the development of a successful vaccine. C1 [Haynes, Barton F.] Duke Univ, Dept Med, Durham, NC 27710 USA. [Haynes, Barton F.; Kelsoe, Garnett] Duke Univ, Dept Immunol, Durham, NC 27710 USA. [Haynes, Barton F.; Kelsoe, Garnett] Duke Univ, Human Vaccine Inst, Durham, NC 27710 USA. [Shaw, George M.; Hahn, Beatrice H.] Univ Penn, Dept Med, Perelman Sch Med, Philadelphia, PA 19104 USA. [Shaw, George M.] Univ Penn, Dept Microbiol, Perelman Sch Med, Philadelphia, PA 19104 USA. [Korber, Bette] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87544 USA. [Sodroski, Joseph] Harvard Univ, Dana Farber Canc Inst, Harvard Med Sch, Boston, MA 02215 USA. [Borrow, Persephone; McMichael, Andrew J.] Univ Oxford, Nuffield Dept Clin Med, Oxford OX3 7FZ, England. RP Haynes, BF (reprint author), Duke Univ, Dept Med, Durham, NC 27710 USA.; Haynes, BF (reprint author), Duke Univ, Dept Immunol, Durham, NC 27710 USA.; Haynes, BF (reprint author), Duke Univ, Human Vaccine Inst, Durham, NC 27710 USA. EM barton.haynes@duke.edu OI Korber, Bette/0000-0002-2026-5757 FU Division of AIDS, NIH, NIAID [UM1-AI10064]; Bill and Melinda Gates Foundation FX This work was supported by the Division of AIDS, NIH, NIAID grant UM1-AI10064 for the Duke Center for HIV/AIDS Vaccine Immunology-Immunogen Discovery and Collaboration for AIDS Vaccine Discovery grants from the Bill and Melinda Gates Foundation to B.F.H. We thank Todd Bradley and Kevin Wiehe for Figure 3. The authors thank Kelly Soderberg, Thomas Denny, Cherie Lahti, and Stuart Shapiro for administrative leadership and all of our collaborators in the Duke CHAVI and CHAVI-ID for their invaluable work over the past 10 years. We apologize that due to space limitations we could not fully reference all the fine work of our colleagues in the field. We thank Stephanie Risbon for expert secretarial assistance. NR 115 TC 22 Z9 22 U1 9 U2 11 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 1931-3128 EI 1934-6069 J9 CELL HOST MICROBE JI Cell Host Microbe PD MAR 9 PY 2016 VL 19 IS 3 BP 292 EP 303 DI 10.1016/j.chom.2016.02.002 PG 12 WC Microbiology; Parasitology; Virology SC Microbiology; Parasitology; Virology GA DH0FI UT WOS:000372457500007 PM 26922989 ER PT J AU Knapen, S Redigolo, D Shih, D AF Knapen, Simon Redigolo, Diego Shih, David TI General gauge mediation at the weak scale SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Supersymmetry Phenomenology ID SUPERSYMMETRY BREAKING; HIGGS-BOSON; MASS; MODELS; MSSM; LHC AB We completely characterize General Gauge Mediation (GGM) at the weak scale by solving all IR constraints over the full parameter space. This is made possible through a combination of numerical and analytical methods, based on a set of algebraic relations among the IR soft masses derived from the GGM boundary conditions in the UV. We show how tensions between just a few constraints determine the boundaries of the parameter space: electroweak symmetry breaking (EWSB), the Higgs mass, slepton tachyons, and left-handed stop/sbottom tachyons. While these constraints allow the left-handed squarks to be arbitrarily light, they place strong lower bounds on all of the right-handed squarks. Meanwhile, light EW superpartners are generic throughout much of the parameter space. This is especially the case at lower messenger scales, where a positive threshold correction to m(h) coming from light Higgsinos and winos is essential in order to satisfy the Higgs mass constraint. C1 [Knapen, Simon] Univ Calif Berkeley, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. [Knapen, Simon] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. [Redigolo, Diego] Univ Paris 06, Sorbonne Univ, UMR 7589, LPTHE, F-75005 Paris, France. [Redigolo, Diego] CNRS, UMR 7589, LPTHE, F-75005 Paris, France. [Shih, David] Rutgers State Univ, New High Energy Theory Ctr, Piscataway, NJ 08854 USA. RP Knapen, S (reprint author), Univ Calif Berkeley, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA.; Knapen, S (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA.; Redigolo, D (reprint author), Univ Paris 06, Sorbonne Univ, UMR 7589, LPTHE, F-75005 Paris, France.; Redigolo, D (reprint author), CNRS, UMR 7589, LPTHE, F-75005 Paris, France.; Shih, D (reprint author), Rutgers State Univ, New High Energy Theory Ctr, Piscataway, NJ 08854 USA. EM smknapen@lbl.gov; dredigol@lpthe.jussieu.fr; dshih@physics.rutgers.edu FU LDRD Program of LBNL under U.S. Department of Energy [DE-AC02-05CH11231]; ERC Higgs at LHC; DOE [DE-SC0003883] FX We thank Nathaniel Craig, Patrick Draper, Daniel Egana-Ugrinovic, Alberto Mariotti, David Morrissey, Michele Papucci, Nausheen Shah, Pietro Slavich, Giovanni Villadoro, Hojin Yoo and Kathryn Zurek for interesting discussions. We are also grateful to Alberto Mariotti and Robert Ziegler for comments on the manuscript. The work of SK was supported by the LDRD Program of LBNL under U.S. Department of Energy Contract No. DE-AC02-05CH11231. The work of DR was supported by the ERC Higgs at LHC. The work of DS was supported in part by DOE grant No. DE-SC0003883. NR 54 TC 4 Z9 4 U1 0 U2 2 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAR 9 PY 2016 IS 3 AR 046 DI 10.1007/JHEP03(2016)046 PG 37 WC Physics, Particles & Fields SC Physics GA DG7VC UT WOS:000372290800001 ER PT J AU Maier, S Lechner, BAJ Somorjai, GA Salmeron, M AF Maier, Sabine Lechner, Barbara A. J. Somorjai, Gabor A. Salmeron, Miquel TI Growth and Structure of the First Layers of Ice on Ru(0001) and Pt(111) SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID ATOM SCATTERING; SURFACE; WATER; DISSOCIATION; ADSORPTION; FILMS AB Scanning tunneling microscopy was used to probe the structure and growth of the first few layers of water on Ru(0001) and Pt(111) at the molecular level. The surface bound first layer is composed of a mixture of water molecules forming hexagonal structures, both in registry and out-of registry with the substrate atoms. The hexagons are connected by pentagonal and heptagonal units. At temperatures below 140 K, this layer structure gives rise to the growth of metastable amorphous structures in the second and higher layers. We found that in the transition from amorphous to crystalline ice the structure of the original bottom layer changes to one in perfect local registry with the hexagonal surfaces of Ru(0001) and Pt(111). We further discovered structural defects in the form of extended one-dimensional lines of five- and eight-membered rings that are domain boundaries and stacking faults in the growing ice layers, which lead to the formation of metastable cubic ice. C1 [Maier, Sabine; Lechner, Barbara A. J.; Somorjai, Gabor A.; Salmeron, Miquel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Maier, Sabine] Univ Erlangen Nurnberg, Inst Phys, Erwin Rommel Str 1, D-91058 Erlangen, Germany. [Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Salmeron, Miquel] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Salmeron, M (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Salmeron, M (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. EM mbsalmeron@lbl.gov RI Maier, Sabine/B-5917-2008; Lechner, Barbara/F-4963-2013 OI Maier, Sabine/0000-0001-9589-6855; Lechner, Barbara/0000-0001-9974-1738 FU U.S. Department of Energy [DE-AC02-05CH11231]; Chemical and Mechanical Properties of Surfaces, Interfaces and Nanostructures program [FWP KC3101] FX This work was supported by the Director, Office of Energy Research, Office of Basic Energy Sciences, Materials Science and Engineering Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, through the Chemical and Mechanical Properties of Surfaces, Interfaces and Nanostructures program (FWP KC3101). NR 41 TC 6 Z9 6 U1 9 U2 45 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAR 9 PY 2016 VL 138 IS 9 BP 3145 EP 3151 DI 10.1021/jacs.5b13133 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA DG3BZ UT WOS:000371945800047 PM 26844953 ER PT J AU Li, FX Crooker, SA Sinitsyn, NA AF Li, Fuxiang Crooker, S. A. Sinitsyn, N. A. TI Higher-order spin-noise spectroscopy of atomic spins in fluctuating external fields SO PHYSICAL REVIEW A LA English DT Article ID MAGNETIC-RESONANCE; DYNAMICS AB We discuss the effect of external noisy magnetic fields on mesoscopic spin fluctuations that can be probed in semiconductors and atomic vapors by means of optical spin-noise spectroscopy. We show that conventional arguments of the law of large numbers do not apply to spin correlations induced by external fields, namely, the magnitude of the 4th-order spin cumulant grows as similar to N-2 with the number N of observed spins, i.e., it is not suppressed in comparison to the 2nd-order cumulant. This allows us to design a simple experiment to measure the 4th-order cumulant of spin fluctuations in an atomic system near thermodynamic equilibrium and develop a quantitative theory that explains all observations. C1 [Li, Fuxiang] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Li, Fuxiang; Sinitsyn, N. A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Crooker, S. A.] Los Alamos Natl Lab, Natl High Magnet Field Lab, Los Alamos, NM 87545 USA. RP Li, FX (reprint author), Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA.; Li, FX (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM fuxiangli@lanl.gov RI Li, Fuxiang/O-9132-2015 FU U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; LDRD program at LANL FX The work was carried out under the support of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. The experiments were performed at the National High Magnetic Field Laboratory, which is supported by NSF DMR-1157490 and the State of Florida. Authors also thank the support from LDRD program at LANL. NR 30 TC 0 Z9 0 U1 3 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD MAR 9 PY 2016 VL 93 IS 3 AR 033814 DI 10.1103/PhysRevA.93.033814 PG 8 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA DG0BB UT WOS:000371725700014 ER PT J AU Boyle, PA Christ, NH Garron, N Jung, C Juttner, A Kelly, C Mawhinney, RD McGlynn, G Murphy, DJ Ohta, S Portelli, A Sachrajda, CT AF Boyle, P. A. Christ, N. H. Garron, N. Jung, C. Juettner, A. Kelly, C. Mawhinney, R. D. McGlynn, G. Murphy, D. J. Ohta, S. Portelli, A. Sachrajda, C. T. TI Low energy constants of SU(2) partially quenched chiral perturbation theory from N-f=2+1 domain wall QCD SO PHYSICAL REVIEW D LA English DT Article ID MOBIUS FERMIONS; ORDER P(6); ONE-LOOP; LATTICE; RENORMALIZATION; SCATTERING; MASS AB We have performed fits of the pseudoscalar masses and decay constants, from a variety of the RBC-UKQCD Collaboration's domain wall fermion ensembles, to SU(2) partially quenched chiral perturbation theory at next-to-leading order (NLO) and next-to-next-to-leading order (NNLO). We report values for nine NLO and eight linearly independent combinations of NNLO partially quenched low-energy constants, which we compare to other lattice and phenomenological determinations. We discuss the size of successive terms in the chiral expansion and use our large set of low-energy constants to make predictions for mass splittings due to QCD isospin-breaking effects and the S-wave pi pi scattering lengths. We conclude that, for the range of pseudoscalar masses explored in this work, 115 MeV less than or similar to m(PS) less than or similar to 430 MeV, the NNLO SU(2) expansion is quite robust and can fit lattice data with percent-scale accuracy. C1 [Boyle, P. A.; Portelli, A.] Univ Edinburgh, Sch Phys, SUPA, Edinburgh EH9 3JZ, Midlothian, Scotland. [Christ, N. H.; Mawhinney, R. D.; McGlynn, G.; Murphy, D. J.] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Garron, N.] Univ Plymouth, Ctr Math Sci, Plymouth PL4 8AA, Devon, England. [Jung, C.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Juettner, A.; Portelli, A.; Sachrajda, C. T.] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. [Kelly, C.; Ohta, S.] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Ohta, S.] KEK, Ctr Theory, Tsukuba, Ibaraki 3050801, Japan. [Ohta, S.] SOKENDAI, Dept Particle & Nucl Phys, Hayama, Kanagawa 2400193, Japan. RP Boyle, PA (reprint author), Univ Edinburgh, Sch Phys, SUPA, Edinburgh EH9 3JZ, Midlothian, Scotland. OI Portelli, Antonin/0000-0002-6059-917X; Murphy, David/0000-0002-8538-815X FU USDOE SciDAC program; BAGEL; U.S. Department of Energy (DOE) [DE-SC0011941]; RIKEN foreign postdoctoral research (FPR) grant; UK STFC Grant [ST/L000296/1]; STFC [ST/M006530/1, ST/L000458/1, ST/K005790/1, ST/K005804/1]; DOE [AC-02-98CH10886(BNL)]; Leverhulme Research Grant [RPG-2014-118]; European Research Council under the European Community [279757] FX We thank members of the RBC-UKQCD Collaboration for helpful discussions and support of this work. The 32ID-M1 and 32ID-M2 ensembles were generated using the IBM Blue Gene/Q (BG/Q) "Mira" system at the Argonne Leadership Class Facility (ALCF) and the "Vulcan" BG/Q system at Lawrence Livermore National Laboratory (LLNL). Measurements, on these ensembles as well as older ensembles used in this work, were performed using Vulcan, the "DiRAC" BG/Q system in the Advanced Computing Facility at the University of Edinburgh, and the BG/Q computers of the RIKEN-BNL Research Center and Brookhaven National Lab. The software used includes the CPS QCD code (http://qcdoc.phys.columbia.edu/cps.html) [ 58], supported in part by the USDOE SciDAC program, and the BAGEL (http://www2.ph.ed.ac.uk/paboyle/bagel/Bagel.html) assembler kernel generator for high-performance optimized kernels and fermion solvers [ 59]. Gauge fixing was performed using the "GLU" (gauge link utility) code base (https://github.com/RJhudspith/GLU). Next-to-next-to-leading-order partially quenched SU(2) and SU(3) chiral perturbation theory expressions for the pseudoscalar masses and decay constants were computed using Fortran routines provided by J. Bijnens. Gauge fixing and fitting were performed using the Columbia University CUTH cluster. N. H. C., R. D. M., G. M., and D. J. M. are supported in part by U.S. Department of Energy (DOE) Grant No. DE-SC0011941. C. K. is supported by a RIKEN foreign postdoctoral research (FPR) grant. A. P. and C. T. S. were supported in part by UK STFC Grant No. ST/L000296/1. P. B. has been in part supported by STFC Grants No. ST/M006530/1, No. ST/L000458/1, No. ST/K005790/1, and No. ST/K005804/1. C. J. is supported by DOE Contract No. AC-02-98CH10886(BNL). N. G. is supported by the Leverhulme Research Grant No. RPG-2014-118. A. J. acknowledges funding from the European Research Council under the European Community's Seventh Framework Programme (FP7/2007-2013) ERC Grant Agreement No. 279757. NR 63 TC 0 Z9 0 U1 2 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 9 PY 2016 VL 93 IS 5 AR 054502 DI 10.1103/PhysRevD.93.054502 PG 43 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DG0FZ UT WOS:000371742000011 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rad, N Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S De Klundert, MV Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Van Parijs, I Barria, P Brun, H Caillol, C Clerbaux, B De Lentdecker, G Fang, W Fasanella, G Favart, L Goldouzian, R Grebenyuk, A Karapostoli, G Lenzi, T Leonard, A Maerschalk, T Marinov, A Pernie, L Randle-Conde, A Seva, T Velde, CV Vanlaer, P Yonamine, R Zenoni, F Zhang, F Beernaert, K Benucci, L Cimmino, A Crucy, S Dobur, D Fagot, A Garcia, G Gul, M Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Salva, S Sigamani, M Tytgat, M Van Driessche, W Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bondu, O Brochet, S Bruno, G Caudron, A Ceard, L Delaere, C Favart, D Forthomme, L Giammanco, A Jafari, A Jez, P Komm, M Lemaitre, V Mertens, A Musich, M Nuttens, C Perrini, L Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Beliy, N Hammad, GH Alda, WL Alves, FL Alves, GA Brito, L Martins, MC Hamer, M Hensel, C Moraes, A Pol, ME Teles, PR Das Chagas, EBB Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Guativa, LMH Malbouisson, H Figueiredo, DM Herrera, CM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Ahuja, S Bernardes, CA Santos, AD Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Moon, CS Novaes, SF Padula, SS Abad, DR Vargas, JCR Aleksandrov, A Hadjiiska, R Iaydjiev, P Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Ahmad, M Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Leggat, D Plestina, R Romeo, F Shaheen, SM Spiezia, A Tao, J Wang, C Wang, Z Zhang, H Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Xu, Z Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Puljak, I Cipriano, PMR Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Micanovic, S Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Bodlak, M Finger, M Finger, M Abdelalim, AA Awad, A Mahrous, A Radi, A Calpas, B Kadastik, M Murumaa, M Raidal, M Tiko, A Veelken, C Eerola, P Pekkanen, J Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Peltola, T Tuominiemi, J Tuovinen, E Wendland, L Talvitie, J Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Favaro, C Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Machet, M Malcles, J Rander, J Rosowsky, A Titov, M Zghiche, A Antropov, I Baffioni, S Beaudette, F Busson, P Cadamuro, L Chapon, E Charlot, C Davignon, O Filipovic, N de Cassagnac, RG Jo, M Lisniak, S Mastrolorenzo, L Mine, P Naranjo, IN Nguyen, M Ochando, C Ortona, G Paganini, P Pigard, P Regnard, S Salerno, R Sauvan, JB Sirois, Y Strebler, T Yilmaz, Y Zabi, A Agram, JL Andrea, J Aubin, A Bloch, D Brom, JM Buttignol, M Chabert, EC Chanon, N Collard, C Conte, E Coubez, X Fontaine, JC Gele, D Goerlach, U Goetzmann, C Le Bihan, AC Merlin, JA Skovpen, K Van Hove, P Gadrat, S Beauceron, S Bernet, C Boudoul, G Bouvier, E Montoya, CAC Chierici, R Contardo, D Courbon, B Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Lagarde, F Laktineh, IB Lethuillier, M Mirabito, L Pequegnot, AL Perries, S Alvarez, JDR Sabes, D Sgandurra, L Sordini, V Donckt, MV Verdier, P Viret, S Toriashvili, T Lomidze, D Autermann, C Beranek, S Feld, L Heister, A Kiesel, MK Klein, K Lipinski, M Ostapchuk, A Preuten, M Raupach, F Schael, S Schulte, JF Verlage, T Weber, H Zhukov, V Ata, M Brodski, M Dietz-Laursonn, E Duchardt, D Endres, M Erdmann, M Erdweg, S Esch, T Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Millet, P Mukherjee, S Olschewski, M Padeken, K Papacz, P Pook, T Radziej, M Reithler, H Rieger, M Scheuch, F Sonnenschein, L Teyssier, D Thuer, S Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Hoehle, F Kargoll, B Kress, T Kunsken, A Lingemann, J Nehrkorn, A Nowack, A Nugent, IM Pistone, C Pooth, O Stahl, A Martin, MA Asin, I Bartosik, N Behnke, O Behrens, U Borras, K Burgmeier, A Campbell, A Contreras-Campana, C Costanza, F Pardos, CD Dolinska, G Dooling, S Dorland, T Eckerlin, G Eckstein, D Eichhorn, T Flucke, G Gallo, E Garcia, JG Geiser, A Gizhko, A Gunnellini, P Hauk, J Hempel, M Jung, H Kalogeropoulos, A Karacheban, O Kasemann, M Katsas, P Kieseler, J Kleinwort, C Korol, I Lange, W Leonard, J Lipka, K Lobanov, A Lohmann, W Mankel, R Melzer-Pellmann, IA Meyer, AB Mittag, G Mnich, J Mussgiller, A Naumann-Emme, S Nayak, A Ntomari, E Perrey, H Pitzl, D Placakyte, R Raspereza, A Roland, B Sahin, MO Saxena, P Schoerner-Sadenius, T Seitz, C Spannagel, S Stefaniuk, N Trippkewitz, KD Walsh, R Wissing, C Blobel, V Vignali, MC Draeger, AR Erfle, J Garutti, E Goebel, K Gonzalez, D Gorner, M Haller, J Hoffmann, M Hoing, RS Junkes, A Klanner, R Kogler, R Kovalchuk, N Lapsien, T Lenz, T Marchesini, I Marconi, D Meyer, M Nowatschin, D Ott, J Pantaleo, F Peiffer, T Perieanu, A Pietsch, N Poehlsen, J 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CA CMS Collaboration TI Measurements of t(t)over-bar spin correlations and top quark polarization using dilepton final states in pp collisions at root s=8 TeV SO PHYSICAL REVIEW D LA English DT Article ID DECAY; LHC AB Measurements of the top quark-antiquark (t (t) over bar) spin correlations and the top quark polarization are presented for t (t) over bar pairs produced in pp collisions at root s = 8 TeV. The data correspond to an integrated luminosity of 19.5 fb(-1) collected with the CMS detector at the LHC. The measurements are performed using events with two oppositely charged leptons (electrons or muons) and two or more jets, where at least one of the jets is identified as originating from a bottom quark. The spin correlations and polarization are measured from the angular distributions of the two selected leptons, both inclusively and differentially, with respect to the invariant mass, rapidity, and transverse momentum of the t (t) over bar system. The measurements are unfolded to the parton level and found to be in agreement with predictions of the standard model. A search for new physics in the form of anomalous top quark chromo moments is performed. No evidence of new physics is observed, and exclusion limits on the real part of the chromo-magnetic dipole moment and the imaginary part of the chromo-electric dipole moment are evaluated. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hartl, C.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Knuenz, V.; Koenig, A.; Krammer, M.; Kraetschmer, I.; Liko, D.; Matsushita, T.; Mikulec, I.; Rabady, D.; Rad, N.; Rahbaran, B.; Rohringer, H.; Schieck, J.; Schoefbeck, R.; Strauss, J.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] Inst Hochenergiephys OeAW, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. [Alderweireldt, S.; Cornelis, T.; De Wolf, E. A.; Janssen, X.; Knutsson, A.; Lauwers, J.; Luyckx, S.; De Klundert, M. Van; Van Haevermaet, H.; Van Mechelen, P.; Van Remortel, N.; Van Spilbeeck, A.] Univ Antwerp, B-2020 Antwerp, Belgium. [Abu Zeid, S.; Blekman, F.; D'Hondt, J.; Daci, N.; De Bruyn, I.; Deroover, K.; Heracleous, N.; Keaveney, J.; Lowette, S.; Moreels, L.; Olbrechts, A.; Python, Q.; Strom, D.; Tavernier, S.; Van Doninck, W.; Van Mulders, P.; Van Onsem, G. P.; Van Parijs, I.] Vrije Univ Brussel, Brussels, Belgium. [Barria, P.; Brun, H.; Caillol, C.; Clerbaux, B.; De Lentdecker, G.; Fang, W.; Fasanella, G.; Favart, L.; Goldouzian, R.; Grebenyuk, A.; Karapostoli, G.; Lenzi, T.; Leonard, A.; Maerschalk, T.; Marinov, A.; Pernie, L.; Randle-conde, A.; Seva, T.; Velde, C. Vander; Vanlaer, P.; Yonamine, R.; Zenoni, F.; Zhang, F.] Univ Libre Bruxelles, Brussels, Belgium. [Beernaert, K.; Benucci, L.; Cimmino, A.; Crucy, S.; Dobur, D.; Fagot, A.; Garcia, G.; Gul, M.; Mccartin, J.; Rios, A. A. Ocampo; Poyraz, D.; Ryckbosch, D.; Salva, S.; Sigamani, M.; Tytgat, M.; Van Driessche, W.; Yazgan, E.; Zaganidis, N.] Univ Ghent, B-9000 Ghent, Belgium. [Basegmez, S.; Beluffi, C.; Bondu, O.; Brochet, S.; Bruno, G.; Caudron, A.; Ceard, L.; Delaere, C.; Favart, D.; Forthomme, L.; Giammanco, A.; Jafari, A.; Jez, P.; Komm, M.; Lemaitre, V.; Mertens, A.; Musich, M.; Nuttens, C.; Perrini, L.; Piotrzkowski, K.; Popov, A.; Quertenmont, L.; Selvaggi, M.; Marono, M. Vidal] Catholic Univ Louvain, Louvain La Neuve, Belgium. [Beliy, N.; Hammad, G. H.] Univ Mons, B-7000 Mons, Belgium. [Alda Junior, W. L.; Alves, F. L.; Alves, G. A.; Brito, L.; Correa Martins Junior, M.; Hamer, M.; Hensel, C.; Moraes, A.; Pol, M. E.; Teles, P. Rebello] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. [Belchior Batista Das Chagas, E.; Carvalho, W.; Chinellato, J.; Custodio, A.; Da Costa, E. M.; De Jesus Damiao, D.; De Oliveira Martins, C.; Fonseca De Souza, S.; Huertas Guativa, L. M.; Malbouisson, H.; Matos Figueiredo, D.; Mora Herrera, C.; Mundim, L.; Nogima, H.; Prado Da Silva, W. L.; Santoro, A.; Sznajder, A.; Tonelli Manganote, E. J.; Vilela Pereira, A.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Ahuja, S.; Dogra, S.; Fernandez Perez Tomei, T. R.; Moon, C. S.; Novaes, S. F.; Padula, Sandra S.; Romero Abad, D.; Alvarez, J. D. Ruiz] Univ Estadual Paulista, Sao Paulo, Brazil. [Bernardes, C. A.; De Souza Santos, A.; Gregores, E. M.; Mercadante, P. G.] Univ Fed ABC, Sao Paulo, Brazil. [Aleksandrov, A.; Hadjiiska, R.; Iaydjiev, P.; Rodozov, M.; Stoykova, S.; Sultanov, G.; Vutova, M.] Inst Nucl Energy Res, Sofia, Bulgaria. [Dimitrov, A.; Glushkov, I.; Litov, L.; Pavlov, B.; Petkov, P.] Univ Sofia, BU-1126 Sofia, Bulgaria. [Bian, J. G.; Chen, H. S.; Chen, M.; Cheng, T.; Du, R.; Jiang, C. H.; Leggat, D.; Plestina, R.; Romeo, F.; Shaheen, S. M.; Spiezia, A.; Tao, J.; Wang, C.; Wang, Z.; Zhang, H.; Ahmad, A.] Inst High Energy Phys, Beijing 100039, Peoples R China. [Zhang, F.; Asawatangtrakuldee, C.; Ban, Y.; Li, Q.; Liu, S.; Mao, Y.; Qian, S. J.; Wang, D.; Xu, Z.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Avila, C.; Cabrera, A.; Chaparro Sierra, L. F.; Florez, C.; Gomez, J. P.; Gomez Moreno, B.; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia. [Godinovic, N.; Lelas, D.; Puljak, I.; Cipriano, P. M. Ribeiro] Univ Split, Fac Elect Engn Mech Engn & Naval Architecture, Split, Croatia. [Antunovic, Z.; Kovac, M.] Univ Split, Fac Sci, Split, Croatia. [Brigljevic, V.; Kadija, K.; Luetic, J.; Micanovic, S.; Sudic, L.] Rudjer Boskovic Inst, Zagreb, Croatia. [Attikis, A.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.; Rykaczewski, H.] Univ Cyprus, CY-1678 Nicosia, Cyprus. [Bodlak, M.; Finger, M.] Charles Univ Prague, Prague, Czech Republic. [Abdelalim, A. A.; Awad, A.; Mahrous, A.; Radi, A.] Acad Sci Res & Technol Arab Republ Egypt, Egyptian Network High Energy Phys, Cairo, Egypt. [Giammanco, A.; Calpas, B.; Kadastik, M.; Murumaa, M.; Raidal, M.; Tiko, A.; Veelken, C.] NICPB, Tallinn, Estonia. [Eerola, P.; Pekkanen, J.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Harkonen, J.; Karimaki, V.; Kinnunen, R.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Peltola, T.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Talvitie, J.; Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Couderc, F.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Favaro, C.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Machet, M.; Malcles, J.; Rander, J.; Rosowsky, A.; Titov, M.; Zghiche, A.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Plestina, R.; Antropov, I.; Baffioni, S.; Beaudette, F.; Busson, P.; Cadamuro, L.; Chapon, E.; Charlot, C.; Davignon, O.; Filipovic, N.; de Cassagnac, R. Granier; Jo, M.; Lisniak, S.; Mastrolorenzo, L.; Mine, P.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Ortona, G.; Paganini, P.; Pigard, P.; Regnard, S.; Salerno, R.; Sauvan, J. B.; Sirois, Y.; Strebler, T.; Yilmaz, Y.; Zabi, A.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Beluffi, C.; Agram, J. -L.; Andrea, J.; Aubin, A.; Bloch, D.; Brom, J. -M.; Buttignol, M.; Chabert, E. C.; Chanon, N.; Collard, C.; Conte, E.; Coubez, X.; Fontaine, J. -C.; Gele, D.; Goerlach, U.; Goetzmann, C.; Le Bihan, A. -C.; Merlin, J. A.; Skovpen, K.; Van Hove, P.] Univ Strasbourg, Univ Haute Alsace Mulhouse, CNRS, Inst Pluridisciplinaire Hubert Curien,IN2P3, Strasbourg, France. [Gadrat, S.] CNRS, IN2P3, Ctr Calcul, Villeurbanne, France. [Beauceron, S.; Bernet, C.; Boudoul, G.; Bouvier, E.; Montoya, C. A. Carrillo; Chierici, R.; Contardo, D.; Depasse, P.; El Mamouni, H.; Fan, J.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Lagarde, F.; Laktineh, I. B.; Lethuillier, M.; Mirabito, L.; Pequegnot, A. L.; Perries, S.; Alvarez, J. D. Ruiz; Sabes, D.; Sgandurra, L.; Sordini, V.; Donckt, M. Vander; Verdier, P.; Viret, S.] Univ Lyon 1, CNRS, IN2P3, Inst Phys Nucl Lyon, F-69622 Villeurbanne, France. [Toriashvili, T.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Toriashvili, T.; Lomidze, D.] Tbilisi State Univ, GE-380086 Tbilisi, Rep of Georgia. [Autermann, C.; Beranek, S.; Feld, L.; Heister, A.; Kiesel, M. K.; Klein, K.; Lipinski, M.; Ostapchuk, A.; Preuten, M.; Raupach, F.; Schael, S.; Schulte, J. F.; Verlage, T.; Weber, H.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Ata, M.; Brodski, M.; Dietz-Laursonn, E.; Duchardt, D.; Endres, M.; Erdmann, M.; Erdweg, S.; Esch, T.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Millet, P.; Mukherjee, S.; Olschewski, M.; Padeken, K.; Papacz, P.; Pook, T.; Radziej, M.; Reithler, H.; Rieger, M.; Scheuch, F.; Sonnenschein, L.; Teyssier, D.; Thueer, S.; Borras, K.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Hoehle, F.; Kargoll, B.; Kress, T.; Kuensken, A.; Lingemann, J.; Nehrkorn, A.; Nowack, A.; Nugent, I. M.; Pistone, C.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B 3, Aachen, Germany. [Martin, M. Aldaya; Asin, I.; Bartosik, N.; Behnke, O.; Behrens, U.; Borras, K.; Burgmeier, A.; Campbell, A.; Contreras-Campana, C.; Costanza, F.; Pardos, C. Diez; Dolinska, G.; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Gallo, E.; Garcia, J. Garay; Geiser, A.; Gizhko, A.; Gunnellini, P.; Hauk, J.; Hempel, M.; Jung, H.; Kalogeropoulos, A.; Karacheban, O.; Kasemann, M.; Katsas, P.; Kieseler, J.; Kleinwort, C.; Korol, I.; Lange, W.; Leonard, J.; Lipka, K.; Lobanov, A.; Lohmann, W.; Mankel, R.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mittag, G.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Nayak, A.; Ntomari, E.; Perrey, H.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Roland, B.; Sahin, M. Oe.; Saxena, P.; Schoerner-Sadenius, T.; Seitz, C.; Spannagel, S.; Stefaniuk, N.; Trippkewitz, K. D.; Walsh, R.; Wissing, C.] Deutsch Elekt Synchrotron, Hamburg, Germany. [Gallo, E.; Blobel, V.; Vignali, M. Centis; Draeger, A. R.; Erfle, J.; Garutti, E.; Goebel, K.; Gonzalez, D.; Goerner, M.; Haller, J.; Hoffmann, M.; Hoeing, R. S.; Junkes, A.; Klanner, R.; Kogler, R.; Kovalchuk, N.; Lapsien, T.; Lenz, T.; Marchesini, I.; Marconi, D.; Meyer, M.; Nowatschin, D.; Ott, J.; Pantaleo, F.; Peiffer, T.; Perieanu, A.; Pietsch, N.; Poehlsen, J.; Rathjens, D.; Scharf, C.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schumann, S.; Schwandt, J.; Sola, V.; Stadie, H.; Steinbrueck, G.; Stober, F. M.; Tholen, H.; Troendle, D.; Usai, E.; Vanelderen, L.; Vanhoefer, A.; Vormwald, B.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; Colombo, F.; De Boer, W.; Descroix, A.; Dierlamm, A.; Fink, S.; Frensch, F.; Friese, R.; Giffels, M.; Gilbert, A.; Haitz, D.; Hartmann, F.; Heindl, S. M.; Husemann, U.; Katkov, I.; Kornmayer, A.; Pardo, P. Lobelle; Maier, B.; Mildner, H.; Mueller, T.; Mueller, Th.; Plagge, M.; Quast, G.; Rabbertz, K.; Roecker, S.; Roscher, F.; Schroeder, M.; Sieber, G.; Simonis, H. J.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weber, M.; Weiler, T.; Williamson, S.; Woehrmann, C.; Wolf, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, Inst Nucl & Particle Phys, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Tziaferi, E.; Sphicas, P.] Univ Athens, Athens 11528, Greece. [Evangelou, I.; Flouris, G.; Kokkas, P.; Loukas, N.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hazi, A.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.; Bartok, M.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Bartok, M.; Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Choudhury, S.; Mal, P.; Mandal, K.; Sahoo, N.; Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Bansal, S.; Beri, S. B.; Bhatnagar, V.; Chawla, R.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, A.; Kaur, M.; Kumar, R.; Mehta, A.; Mittal, M.; Singh, J. B.; Walia, G.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Bhardwaj, A.; Choudhary, B. C.; Garg, R. B.; Malhotra, S.; Naimuddin, M.; Nishu, N.; Ranjan, K.; Sharma, R.; Sharma, V.] Univ Delhi, Delhi 110007, India. [Bhattacharya, S.; Chatterjee, K.; Dey, S.; Dutta, S.; Majumdar, N.; Modak, A.; Mondal, K.; Mukhopadhyay, S.; Roy, A.; Roy, D.; Chowdhury, S. Roy; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Chudasama, R.; Dutta, D.; Jha, V.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Jain, Sa.; Kole, G.; Kumar, S.; Mahakud, B.; Maity, M.; Majumder, G.; Mazumdar, K.; Mitra, S.; Mohanty, G. B.; Parida, B.; Sarkar, T.; Sur, N.; Sutar, B.; Wickramage, N.] Tata Inst Fundamental Res, Homi Bhabha Rd, Bombay 400005, Maharashtra, India. [Chauhan, S.; Dube, S.; Kapoor, A.; Kothekar, K.; Sharma, S.] Ind Inst Sci Educ & Res, Pune, Maharashtra, India. [Bakhshiansohi, H.; Etesami, S. M.; Fahim, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.; Benhabib, L.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Ranieri, A.; Selvaggi, G.; Silvestris, L.; Venditti, R.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Calabria, C.; Caputo, C.; Cristella, L.; De Palma, M.; Miniello, G.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Battilana, C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, M.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.] Univ Bologna, Bologna, Italy. [Chiorboli, M.; Costa, S.; Di Mattia, A.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Viliani, L.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gori, V.; Lenzi, P.; Viliani, L.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.; Primavera, F.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Monge, M. R.; Tosi, S.] Univ Genoa, Genoa, Italy. [Brianza, L.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, Via Celoria 16, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Manzoni, R. A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.; Thyssen, F.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Esposito, M.; Iorio, A. O. M.; Sciacca, C.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, I-85100 Potenza, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Dosselli, U.; Fanzago, F.; Gasparini, F.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.] Univ Trento, Trento, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Magnani, A.; Montagna, P.; Ratti, S. P.; Riccardi, C.; Vai, I.; Vitulo, P.] Univ Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Solestizi, L. Alunni; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Solestizi, L. Alunni; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.] Univ Perugia, I-06100 Perugia, Italy. [Aleksandrov, A.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fedi, G.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Donato, S.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Traczyk, P.] Univ Rome, Rome, Italy. [Romeo, F.; Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Romeo, F.; Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. 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[Adzic, P.; Cirkovic, P.; Devetak, D.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Fac Phys, POB 550, YU-11001 Belgrade, Serbia. [Adzic, P.; Cirkovic, P.; Devetak, D.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De la Cruz, B.; Delgado Peris, A.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; De Martino, E. Navarro; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.] CIEMAT, Ctr Invest Energet Medioambientales & Tecnol, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. 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A.; Di Guida, S.; Meola, S.; Paolucci, P.; Azzi, P.; Dall'Osso, M.; Pazzini, J.; Zucchetta, A.; Ciangottini, D.; Azzurri, P.; Donato, S.; D'imperio, G.; Del Re, D.; Traczyk, P.; Arcidiacono, R.; Finco, L.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Castello, R.; Cerminara, G.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Duggan, D.; Duenser, M.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Fulcher, J.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Loureno, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Reis, T.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Seidel, M.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Zagozdzinska, A.; Zeuner, W. D.; Ulmer, K. A.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lecomte, P.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meinhard, M. T.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Schoenenberger, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Wallny, R.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Rauco, G.; Robmann, P.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Pozdnyakov, A.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Kumar, Arun; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. f.; Tzeng, Y. M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Cerci, S.; Damarseckin, S.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Gecit, F. H.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozcan, M.; Ozdemir, K.; Ozturk, S.; Tali, B.; Topakli, H.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, E. A.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cakir, A.; Cankocak, K.; Sen, S.; Vardarli, F. 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[Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Futyan, D.; Hall, G.; Iles, G.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Arcaro, D.; Avetisyan, A.; Bose, T.; Gastler, D.; Rankin, D.; Richardson, C.; Rohlf, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Benelli, G.; Berry, E.; Cutts, D.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Jesus, O.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Chauhan, S.; Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chertok, M.; Conway, R.; Cox, P. T.; Erbacher, R.; Funk, G.; Gardner, M.; Ko, W.; Lander, R.; Mclean, C.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Cousins, R.; Everaerts, P.; Florent, A.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Derdzinski, M.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Padhi, S.; Pieri, M.; Sani, M.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Banerjee, S.; Abdullin, S.; Albrow, M.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hasegawa, S.; Hirschauer, J.; Hu, Z.; Jayatilaka, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kreis, B.; Lammel, S.; Lewis, J.; Linacre, J.; Lincoln, D.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Stoynev, S.; Strobbe, N.; Taylor, L.; Tkaczyk, S.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Wang, M.; Weber, H. A.; Whitbeck, A.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Brinkerhoff, A.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Field, R. D.; Furic, I. K.; Gleyzer, S. V.; Konigsberg, J.; Korytov, A.; Kotov, K.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Rossin, R.; Shchutska, L.; Snowball, M.; Sperka, D.; Terentyev, N.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bein, S.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Colafranceschi, S.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.; Zhang, J.] Univ Illinois, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Eminizer, N.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Osherson, M.; Roskes, J.; Sady, A.; Sarica, U.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Bruner, C.; Majumder, D.; Malek, M.; Mcbrayer, W.; Murray, M.; Sanders, S.; Stringer, R.; Wang, Q.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. 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RI Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Moraes, Arthur/F-6478-2010; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; ciocci, maria agnese /I-2153-2015; Kirakosyan, Martin/N-2701-2015; Puljak, Ivica/D-8917-2017; TUVE', Cristina/P-3933-2015; Montanari, Alessandro/J-2420-2012; Azarkin, Maxim/N-2578-2015; Chinellato, Jose Augusto/I-7972-2012; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Tinoco Mendes, Andre David/D-4314-2011; Varela, Joao/K-4829-2016; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Sznajder, Andre/L-1621-2016; Stahl, Achim/E-8846-2011; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Colafranceschi, Stefano/M-1807-2016; Chadeeva, Marina/C-8789-2016; Danilov, Mikhail/C-5380-2014; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Leonardo, Nuno/M-6940-2016; Calderon, Alicia/K-3658-2014; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Chistov, Ruslan/B-4893-2014; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Novaes, Sergio/D-3532-2012; VARDARLI, Fuat Ilkehan/B-6360-2013; Della Ricca, Giuseppe/B-6826-2013; Dudko, Lev/D-7127-2012; Lokhtin, Igor/D-7004-2012; Manganote, Edmilson/K-8251-2013; Matorras, Francisco/I-4983-2015; Hernandez Calama, Jose Maria/H-9127-2015; Cerrada, Marcos/J-6934-2014; Andreev, Vladimir/M-8665-2015 OI Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Moraes, Arthur/0000-0002-5157-5686; Ogul, Hasan/0000-0002-5121-2893; ciocci, maria agnese /0000-0003-0002-5462; TUVE', Cristina/0000-0003-0739-3153; Montanari, Alessandro/0000-0003-2748-6373; Chinellato, Jose Augusto/0000-0002-3240-6270; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Tinoco Mendes, Andre David/0000-0001-5854-7699; Varela, Joao/0000-0003-2613-3146; Seixas, Joao/0000-0002-7531-0842; Sznajder, Andre/0000-0001-6998-1108; Stahl, Achim/0000-0002-8369-7506; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Chadeeva, Marina/0000-0003-1814-1218; Danilov, Mikhail/0000-0001-9227-5164; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Chistov, Ruslan/0000-0003-1439-8390; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; Dudko, Lev/0000-0002-4462-3192; Matorras, Francisco/0000-0003-4295-5668; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Cerrada, Marcos/0000-0003-0112-1691; FU Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS programme of the Foundation for Polish Science; European Union, Regional Development Fund; National Science Center (Poland); Compagnia di San Paolo (Torino); MIUR (Italy) [20108T4XTM]; Thalis programme - EU-ESF; Aristeia programme - EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Rachadapisek Sompot Fund for Postdoctoral Fellowship; Chulalongkorn University (Thailand); Chulalongkorn Academic into Its 2nd Century Project Advancement Project (Thailand); Welch Foundation [C-1845] FX We would like to thank W. Bernreuther and Z.-G. Si for calculating the theoretical predictions for this paper, and for studies of the effect of anomalous top quark chromo moments on the acceptance of our selection criteria at the parton level. We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses.; Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via IUT23-4 and IUT23-6 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules/CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Ministry of Science, ICT and Future Planning, and National Research Foundation (NRF), Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLPFAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine, and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, UK; the US Department of Energy, and the US National Science Foundation. Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P.; Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS programme of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the OPUS programme of the National Science Center (Poland); the Compagnia di San Paolo (Torino); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); the Chulalongkorn Academic into Its 2nd Century Project Advancement Project (Thailand); and the Welch Foundation, Contract No. C-1845. NR 61 TC 1 Z9 1 U1 16 U2 44 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 9 PY 2016 VL 93 IS 5 AR 052007 DI 10.1103/PhysRevD.93.052007 PG 25 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DG0FZ UT WOS:000371742000002 ER PT J AU Nisar, NK Mohanty, GB Trabelsi, K Aziz, T Abdesselam, A Adachi, I Aihara, H Asner, DM Aulchenko, V Aushev, T Ayad, R Babu, V Badhrees, I Bahinipati, S Barberio, E Behera, P Bhardwaj, V Biswal, J Bobrov, A Bozek, A Bracko, M Breibeck, F Browder, TE Cervenkov, D Chekelian, V Chen, A Cheon, BG Chistov, R Cho, K Chobanova, V Choi, Y Cinabro, D Dalseno, J Dash, N Dolezal, Z Drasal, Z Drutskoy, A Dutta, D Eidelman, S Farhat, H Fast, JE Fulsom, BG Gaur, V Garmash, A Gillard, R Goh, YM Goldenzweig, P Golob, B Greenwald, D Grzymkowska, O Haba, J Hara, T Hayasaka, K Hayashii, H He, XH Hou, WS Inami, K Ishikawa, A Iwasaki, Y Jacobs, WW Jaegle, I Jeon, HB Joffe, D Joo, KK Julius, T Kang, KH Kato, E Kawasaki, T Kiesling, C Kim, DY Kim, HJ Kim, KT Kim, MJ Kim, SH Kinoshita, K Kodys, P Korpar, S Krizan, P Krokovny, P Kuhr, T Kumar, R Kumita, T Kuzmin, A Kwon, YJ Lee, IS Lange, JS Li, H Li, L Gioi, LL Libby, J Liventsev, D Lukin, P Masuda, M Matvienko, D Miyabayashi, K Miyata, H Mizuk, R Mohanty, S Moll, A Moon, HK Mori, T Mussa, R Nakano, E Nakao, M Nanut, T Natkaniec, Z Nayak, M Niiyama, M Nishida, S Ogawa, S Okuno, S Pakhlov, P Pakhlova, G Pal, B Park, CW Park, H Paul, S Pedlar, TK Pesantez, L Pestotnik, R Petric, M Piilonen, LE Prasanth, K Pulvermacher, C Rauch, J Ribezl, E Ritter, M Rostomyan, A Ryu, S Sahoo, H Sakai, Y Sandilya, S Sanuki, T Sato, Y Savinov, V Schluer, T Schneider, O Schnell, G Schwanda, C Schwartz, AJ Seino, Y Senyo, K Seon, O Seong, IS Shebalin, V Shibata, TA Shiu, JG Shwartz, B Simon, F Singh, JB Sohn, YS Solovieva, E Stanic, S Staric, M Stypula, J Sumihama, M Sumiyoshi, T Tamponi, U Teramoto, Y Uchida, M Uglov, T Uno, S Urquijo, P Van Hulse, C Vanhoefer, P Varner, G Varvell, KE Vinokurova, A Vossen, A Wagner, MN Wang, CH Wang, MZ Wang, XL Watanabe, M Watanabe, Y Williams, KM Won, E Yelton, J Yuan, CZ Yusa, Y Zhang, ZP Zhilich, V Zhulanov, V Zupanc, A AF Nisar, N. K. Mohanty, G. B. Trabelsi, K. Aziz, T. Abdesselam, A. Adachi, I. Aihara, H. Asner, D. M. Aulchenko, V. Aushev, T. Ayad, R. Babu, V. Badhrees, I. Bahinipati, S. Barberio, E. Behera, P. Bhardwaj, V. Biswal, J. Bobrov, A. Bozek, A. Bracko, M. Breibeck, F. Browder, T. E. Cervenkov, D. Chekelian, V. Chen, A. Cheon, B. G. Chistov, R. Cho, K. Chobanova, V. Choi, Y. Cinabro, D. Dalseno, J. Dash, N. Dolezal, Z. Drasal, Z. Drutskoy, A. Dutta, D. Eidelman, S. Farhat, H. Fast, J. E. Fulsom, B. G. Gaur, V. Garmash, A. Gillard, R. Goh, Y. M. Goldenzweig, P. Golob, B. Greenwald, D. Grzymkowska, O. Haba, J. Hara, T. Hayasaka, K. Hayashii, H. He, X. H. Hou, W. -S. Inami, K. Ishikawa, A. Iwasaki, Y. Jacobs, W. W. Jaegle, I. Jeon, H. B. Joffe, D. Joo, K. K. Julius, T. Kang, K. H. Kato, E. Kawasaki, T. Kiesling, C. Kim, D. Y. Kim, H. J. Kim, K. T. Kim, M. J. Kim, S. H. Kinoshita, K. Kodys, P. Korpar, S. Krizan, P. Krokovny, P. Kuhr, T. Kumar, R. Kumita, T. Kuzmin, A. Kwon, Y. -J. Lee, I. S. Lange, J. S. Li, H. Li, L. Gioi, L. Li Libby, J. Liventsev, D. Lukin, P. Masuda, M. Matvienko, D. Miyabayashi, K. Miyata, H. Mizuk, R. Mohanty, S. Moll, A. Moon, H. K. Mori, T. Mussa, R. Nakano, E. Nakao, M. Nanut, T. Natkaniec, Z. Nayak, M. Niiyama, M. Nishida, S. Ogawa, S. Okuno, S. Pakhlov, P. Pakhlova, G. Pal, B. Park, C. W. Park, H. Paul, S. Pedlar, T. K. Pesantez, L. Pestotnik, R. Petric, M. Piilonen, L. E. Prasanth, K. Pulvermacher, C. Rauch, J. Ribezl, E. Ritter, M. Rostomyan, A. Ryu, S. Sahoo, H. Sakai, Y. Sandilya, S. Sanuki, T. Sato, Y. Savinov, V. Schlueter, T. Schneider, O. Schnell, G. Schwanda, C. Schwartz, A. J. Seino, Y. Senyo, K. Seon, O. Seong, I. S. Shebalin, V. Shibata, T. -A. Shiu, J. -G. Shwartz, B. Simon, F. Singh, J. B. Sohn, Y. -S. Solovieva, E. Stanic, S. Staric, M. Stypula, J. Sumihama, M. Sumiyoshi, T. Tamponi, U. Teramoto, Y. Uchida, M. Uglov, T. Uno, S. Urquijo, P. Van Hulse, C. Vanhoefer, P. Varner, G. Varvell, K. E. Vinokurova, A. Vossen, A. Wagner, M. N. Wang, C. H. Wang, M. -Z. Wang, X. L. Watanabe, M. Watanabe, Y. Williams, K. M. Won, E. Yelton, J. Yuan, C. Z. Yusa, Y. Zhang, Z. P. Zhilich, V. Zhulanov, V. Zupanc, A. TI Search for the rare decay D-0 -> gamma gamma at Belle SO PHYSICAL REVIEW D LA English DT Article AB We search for the rare radiative decay D-0 -> gamma gamma using a data sample with an integrated luminosity of 832 fb(-1) recorded by the Belle detector at the KEKB e(+)e(-) asymmetric-energy collider. We find no statistically significant signal and set an upper limit on the branching fraction of B(D-0 -> gamma gamma) < 8.5 x 10(-7) at 90% confidence level. This is the most restrictive limit on the decay channel to date. C1 [Nisar, N. K.] Aligarh Muslim Univ, Aligarh 202002, Uttar Pradesh, India. [Schnell, G.; Van Hulse, C.] Univ Basque Country, UPV EHU, Bilbao 48080, Spain. [Pesantez, L.] Univ Bonn, D-53115 Bonn, Germany. [Aulchenko, V.; Bobrov, A.; Eidelman, S.; Garmash, A.; Krokovny, P.; Kuzmin, A.; Lukin, P.; Matvienko, D.; Shebalin, V.; Shwartz, B.; Vinokurova, A.; Zhilich, V.; Zhulanov, V.] Budker Inst Nucl Phys SB RAS, Novosibirsk 630090, Russia. [Cervenkov, D.; Dolezal, Z.; Drasal, Z.; Kodys, P.] Charles Univ Prague, Fac Math & Phys, CR-12116 Prague, Czech Republic. [Joo, K. K.] Chonnam Natl Univ, Kwangju 660701, South Korea. [Kinoshita, K.; Pal, B.; Schwartz, A. J.] Univ Cincinnati, Cincinnati, OH 45221 USA. [Rostomyan, A.] DESY, D-22607 Hamburg, Germany. [Yelton, J.] Univ Florida, Gainesville, FL 32611 USA. [Lange, J. S.; Wagner, M. N.] Univ Giessen, D-35392 Giessen, Germany. [Sumihama, M.] Gifu Univ, Gifu 5011193, Japan. [Trabelsi, K.; Adachi, I.; Haba, J.; Hara, T.; Nakao, M.; Nishida, S.; Sakai, Y.; Uno, S.] SOKENDAI, Hayama 2400193, Japan. [Cheon, B. G.; Goh, Y. M.; Kim, S. H.; Lee, I. S.] Hanyang Univ, Seoul 133791, South Korea. [Browder, T. E.; Jaegle, I.; Sahoo, H.; Seong, I. S.; Varner, G.] Univ Hawaii, Honolulu, HI 96822 USA. [Trabelsi, K.; Adachi, I.; Haba, J.; Hara, T.; Iwasaki, Y.; Liventsev, D.; Nakao, M.; Nishida, S.; Sakai, Y.; Uno, S.] High Energy Accelerator Res Org KEK, Tsukuba, Ibaraki 3050801, Japan. [Schnell, G.] Ikerbasque, Basque Fdn Sci, Bilbao 48013, Spain. [Bahinipati, S.; Dash, N.] Indian Inst Technol bhubaneswar, Satya Nagar 751007, India. [Behera, P.; Libby, J.; Nayak, M.; Prasanth, K.] Indian Inst Technol Madras, Madras 600036, Tamil Nadu, India. [Jacobs, W. W.; Li, H.; Vossen, A.] Indiana Univ, Bloomington, IN 47408 USA. [Yuan, C. Z.] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Breibeck, F.; Schwanda, C.] Inst High Energy Phys, A-1050 Vienna, Austria. [Mussa, R.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Aushev, T.; Chistov, R.; Drutskoy, A.; Mizuk, R.; Pakhlov, P.; Pakhlova, G.; Solovieva, E.; Uglov, T.] Inst Theoret & Expt Phys, Moscow 117218, Russia. [Biswal, J.; Bracko, M.; Golob, B.; Korpar, S.; Krizan, P.; Nanut, T.; Pestotnik, R.; Petric, M.; Ribezl, E.; Staric, M.; Zupanc, A.] J Stefan Inst, Ljubljana 1000, Slovenia. [Okuno, S.; Watanabe, Y.] Kanagawa Univ, Yokohama, Kanagawa 2218686, Japan. [Goldenzweig, P.; Pulvermacher, C.] Karlsruhe Inst Technol, Inst Expt Kernphys, D-76131 Karlsruhe, Germany. [Joffe, D.] Kennesaw State Univ, Kennesaw, GA 30144 USA. [Badhrees, I.] King Abdulaziz City Sci & Technol, Riyadh 11442, Saudi Arabia. [Cho, K.] Korea Inst Sci & Technol Informat, Daejeon 305806, South Korea. [Kim, K. T.; Moon, H. K.; Won, E.] Korea Univ, Seoul 136713, South Korea. [Niiyama, M.] Kyoto Univ, Kyoto 6068502, Japan. [Jeon, H. B.; Kang, K. H.; Kim, H. J.; Kim, M. J.; Park, H.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Schneider, O.] Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland. [Golob, B.; Krizan, P.; Zupanc, A.] Univ Ljubljana, Fac Math & Phys, Ljubljana 1000, Slovenia. [Kuhr, T.; Ritter, M.; Schlueter, T.] Univ Munich, D-80539 Munich, Germany. [Pedlar, T. K.] Luther Coll, Decorah, IA 52101 USA. [Bracko, M.; Korpar, S.] Univ Maribor, SLO-2000 Maribor, Slovenia. [Chekelian, V.; Chobanova, V.; Dalseno, J.; Kiesling, C.; Gioi, L. Li; Moll, A.; Simon, F.; Vanhoefer, P.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Barberio, E.; Julius, T.; Urquijo, P.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Drutskoy, A.; Mizuk, R.; Pakhlov, P.] Moscow Engn Phys Inst, Moscow 115409, Russia. [Aushev, T.; Pakhlova, G.; Uglov, T.] Moscow Inst Phys & Technol, Dolgoprudnyi 141700, Russia. [Inami, K.; Mori, T.; Sato, Y.; Seon, O.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648602, Japan. [Hayasaka, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648602, Japan. [Hayashii, H.; Miyabayashi, K.] Nara Womens Univ, Nara 6308506, Japan. [Chen, A.] Natl Cent Univ, Chungli 32054, Taiwan. [Wang, C. H.] Natl United Univ, Miaoli 36003, Taiwan. [Hou, W. -S.; Shiu, J. -G.; Wang, M. -Z.] Natl Taiwan Univ, Dept Phys, Taipei 10617, Taiwan. [Bozek, A.; Grzymkowska, O.; Natkaniec, Z.; Stypula, J.] H Niewodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. [Kawasaki, T.; Miyata, H.; Seino, Y.; Watanabe, M.; Yusa, Y.] Niigata Univ, Niigata 9502181, Japan. [Stanic, S.] Univ Nova Gor, Nova Gorica 5000, Slovenia. [Aulchenko, V.; Bobrov, A.; Eidelman, S.; Garmash, A.; Krokovny, P.; Kuzmin, A.; Shebalin, V.; Shwartz, B.; Vinokurova, A.; Zhilich, V.; Zhulanov, V.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Nakano, E.; Teramoto, Y.] Osaka City Univ, Osaka 5588585, Japan. [Asner, D. M.; Fast, J. E.; Fulsom, B. G.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [He, X. H.] Peking Univ, Beijing 100871, Peoples R China. [Savinov, V.] Univ Pittsburgh, Pittsburgh, PA 15260 USA. [Kumar, R.] Punjab Agr Univ, Ludhiana 141004, Punjab, India. [Li, L.; Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Ryu, S.] Seoul Natl Univ, Seoul 151742, South Korea. [Kim, D. Y.] Soongsil Univ, Seoul 156743, South Korea. [Bhardwaj, V.] Univ S Carolina, Columbia, SC 29208 USA. [Choi, Y.; Park, C. W.] Sungkyunkwan Univ, Suwon 440746, South Korea. [Varvell, K. E.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdesselam, A.; Ayad, R.; Badhrees, I.] Univ Tabuk, Fac Sci, Dept Phys, Tabuk 71451, Saudi Arabia. [Nisar, N. K.; Mohanty, G. B.; Aziz, T.; Babu, V.; Dutta, D.; Gaur, V.; Mohanty, S.; Sandilya, S.] Tata Inst Fundamental Res, Homi Bhabha Rd, Mumbai 400005, Maharashtra, India. [Dalseno, J.; Moll, A.; Simon, F.] Tech Univ Munich, Excellence Cluster Univ, D-85748 Garching, Germany. [Greenwald, D.; Paul, S.; Rauch, J.] Tech Univ Munich, Dept Phys, D-85748 Garching, Germany. [Ogawa, S.] Toho Univ, Funabashi, Chiba 2748510, Japan. [Ishikawa, A.; Kato, E.; Sanuki, T.] Tohoku Univ, Dept Phys, Sendai, Miyagi 9808578, Japan. [Masuda, M.] Univ Tokyo, Earthquake Res Inst, Tokyo 1130032, Japan. [Aihara, H.] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Shibata, T. -A.; Uchida, M.] Tokyo Inst Technol, Tokyo, Japan. [Kumita, T.; Sumiyoshi, T.] Tokyo Metropolitan Univ, Tokyo 1920397, Japan. [Tamponi, U.] Univ Turin, I-10124 Turin, Italy. [Mohanty, S.] Utkal Univ, Bhubaneswar 751004, Orissa, India. [Liventsev, D.; Piilonen, L. E.; Wang, X. L.; Williams, K. M.] Virginia Polytech Inst & State Univ, CNP, Blacksburg, VA 24061 USA. [Cinabro, D.; Farhat, H.; Gillard, R.] Wayne State Univ, Detroit, MI 48202 USA. [Senyo, K.] Yamagata Univ, Yamagata 9908560, Japan. [Kwon, Y. -J.; Sohn, Y. -S.] Yonsei Univ, Seoul 120749, South Korea. RP Nisar, NK (reprint author), Aligarh Muslim Univ, Aligarh 202002, Uttar Pradesh, India.; Nisar, NK (reprint author), Tata Inst Fundamental Res, Homi Bhabha Rd, Mumbai 400005, Maharashtra, India. RI Mizuk, Roman/B-3751-2014; Pakhlova, Galina/C-5378-2014; Pakhlov, Pavel/K-2158-2013; Cervenkov, Daniel/D-2884-2017; Solovieva, Elena/B-2449-2014; Krokovny, Pavel/G-4421-2016; Aihara, Hiroaki/F-3854-2010; Paul, Stephan/F-7596-2015; Paul, Stephan/K-9237-2016; Uglov, Timofey/B-2406-2014; Chistov, Ruslan/B-4893-2014; Drutskoy, Alexey/C-8833-2016 OI Pakhlova, Galina/0000-0001-7518-3022; Pakhlov, Pavel/0000-0001-7426-4824; Cervenkov, Daniel/0000-0002-1865-741X; Solovieva, Elena/0000-0002-5735-4059; Krokovny, Pavel/0000-0002-1236-4667; Aihara, Hiroaki/0000-0002-1907-5964; Paul, Stephan/0000-0002-8813-0437; Paul, Stephan/0000-0002-8813-0437; Uglov, Timofey/0000-0002-4944-1830; Chistov, Ruslan/0000-0003-1439-8390; Drutskoy, Alexey/0000-0003-4524-0422 FU MEXT (Japan); JSPS (Japan); Nagoya's TLPRC (Japan); ARC (Australia); FWF (Austria); NSFC (China); CCEPP (China); MSMT (Czechia); CZF (Germany); DFG (Germany); VS (Germany); DST (India); INFN (Italy); MOE (Korea); MSIP (Korea); NRF (Korea); BK21Plus (Korea); WCU (Korea); RSRI (Korea); MNiSW (Poland); NCN (Poland); MES (Russia); RFAAE (Russia); ARRS (Slovenia); IKERBASQUE (Spain); UPV/EHU (Spain); SNSF (Switzerland); NSC (Taiwan); MOE (Taiwan); DOE (USA); NSF (USA) FX We thank the KEKB group for excellent operation of the accelerator; the KEK cryogenics group for efficient solenoid operations; and the KEK computer group, the NII, and PNNL/EMSL for valuable computing and SINET4 network support. We acknowledge support from MEXT, JSPS, and Nagoya's TLPRC (Japan); ARC (Australia); FWF (Austria); NSFC and CCEPP (China); MSMT (Czechia); CZF, DFG, and VS (Germany); DST (India); INFN (Italy); MOE, MSIP, NRF, BK21Plus, WCU, and RSRI (Korea); MNiSW and NCN (Poland); MES and RFAAE (Russia); ARRS (Slovenia); IKERBASQUE and UPV/EHU (Spain); SNSF (Switzerland); NSC and MOE (Taiwan); and DOE and NSF (USA). NR 23 TC 1 Z9 1 U1 5 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 9 PY 2016 VL 93 IS 5 AR 051102 DI 10.1103/PhysRevD.93.051102 PG 7 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DG0FZ UT WOS:000371742000001 ER PT J AU Parke, S AF Parke, Stephen TI What is Delta m(ee)(2)? SO PHYSICAL REVIEW D LA English DT Article AB The current short baseline reactor experiments, Daya Bay and RENO (Double Chooz) have measured (or are capable of measuring) an effective Delta m(2) associated with the atmospheric oscillation scale of 0.5 km/MeV in electron antineutrino disappearance. In this paper, I compare and contrast the different definitions of such an effective Delta m(2) and argue that the simple, L/E independent definition given by Delta m(ee)(2) cos(2)theta(12)Delta m(31)(2) + sin(2) theta(12)Delta m(32)(2), i.e. "the nu(e) weighted average of Delta m(31)(2) and Delta m(32)(2)," is superior to all other definitions and is useful for both short baseline experiments mentioned above and for the future medium baseline experiments JUNO and RENO-50. C1 [Parke, Stephen] Fermilab Natl Accelerator Lab, Dept Theoret Phys, POB 500, Batavia, IL 60510 USA. RP Parke, S (reprint author), Fermilab Natl Accelerator Lab, Dept Theoret Phys, POB 500, Batavia, IL 60510 USA. EM parke@fnal.gov FU European Union FP7 ITN INVISIBLES (Marie Curie Actions) [PITN-GA-2011-289442]; U.S. Department of Energy [DE-AC02-07CH11359] FX The author acknowledges discussions with Kam-Biu Luk, Yasuhiro Nakajima, and Daniel Dwyer of the Daya Bay Collaboration; Soo-Bong Kim and Seon-Hee Seo from the RENO Collaboration; and my collaborators Hisakazu Minakata and Peter Denton. The author also acknowledges partial support from the European Union FP7 ITN INVISIBLES (Marie Curie Actions, PITN-GA-2011-289442). Fermilab is operated by the Fermi Research Alliance under Contract No. DE-AC02-07CH11359 with the U.S. Department of Energy. NR 14 TC 3 Z9 3 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 9 PY 2016 VL 93 IS 5 AR 053008 DI 10.1103/PhysRevD.93.053008 PG 9 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DG0FZ UT WOS:000371742000004 ER PT J AU Cigliola, V Populaire, C Pierri, CL Deutsch, S Haefliger, JA Fadista, J Lyssenko, V Groop, L Rueedi, R Thorel, F Herrera, PL Meda, P AF Cigliola, Valentina Populaire, Celine Pierri, Ciro L. Deutsch, Samuel Haefliger, Jacques-Antoine Fadista, Joao Lyssenko, Valeriya Groop, Leif Rueedi, Rico Thorel, Fabrizio Herrera, Pedro Luis Meda, Paolo TI A Variant of GJD2, Encoding for Connexin 36, Alters the Function of Insulin Producing beta-Cells SO PLOS ONE LA English DT Article ID JUVENILE MYOCLONIC EPILEPSY; PANCREATIC-ISLETS; MESSENGER-RNA; GAP-JUNCTIONS; SECONDARY STRUCTURE; GENE; EXPRESSION; SECRETION; ASSOCIATION; MOUSE AB Signalling through gap junctions contributes to control insulin secretion and, thus, blood glucose levels. Gap junctions of the insulin-producing beta-cells are made of connexin 36 (Cx36), which is encoded by the GJD2 gene. Cx36-null mice feature alterations mimicking those observed in type 2 diabetes (T2D). GJD2 is also expressed in neurons, which share a number of common features with pancreatic beta-cells. Given that a synonymous exonic single nucleotide polymorphism of human Cx36 (SNP rs3743123) associates with altered function of central neurons in a subset of epileptic patients, we investigated whether this SNP also caused alterations of beta-cell function. Transfection of rs3743123 cDNA in connexin-lacking HeLa cells resulted in altered formation of gap junction plaques and cell coupling, as compared to those induced by wild type (WT) GJD2 cDNA. Transgenic mice expressing the very same cDNAs under an insulin promoter revealed that SNP rs3743123 expression consistently lead to a post-natal reduction of islet Cx36 levels and beta-cell survival, resulting in hyperglycemia in selected lines. These changes were not observed in sex-and agematched controls expressing WT hCx36. The variant GJD2 only marginally associated to heterogeneous populations of diabetic patients. The data document that a silent polymorphism of GJD2 is associated with altered beta-cell function, presumably contributing to T2D pathogenesis. C1 [Cigliola, Valentina; Thorel, Fabrizio; Herrera, Pedro Luis] Univ Geneva, Fac Med, Dept Genet Med & Dev, Geneva, Switzerland. [Populaire, Celine] Ctr Hosp Reg Univ Besancon, Besancon, France. [Pierri, Ciro L.] Univ Bari, Dept Biosci Biotechnol & Biopharmaceut, Bari, Italy. [Deutsch, Samuel] Joint Genome Inst, Walnut Creek, CA USA. [Haefliger, Jacques-Antoine] CHU Vaudois, Dept Med, Lausanne, Switzerland. [Fadista, Joao; Lyssenko, Valeriya; Groop, Leif] Lund Univ, Dept Clin Sci Diabet & Endocrinol, Malmo, Sweden. [Lyssenko, Valeriya] Steno Diabet Ctr AS, Gentofte, Denmark. [Rueedi, Rico] Univ Lausanne, Dept Computat Biol, Rue Bugnon 27, CH-1011 Lausanne, Switzerland. [Rueedi, Rico] Swiss Inst Bioinformat, CH-1015 Lausanne, Switzerland. [Meda, Paolo] Univ Geneva, Fac Med, Dept Cell Physiol & Metab, Geneva, Switzerland. RP Cigliola, V (reprint author), Univ Geneva, Fac Med, Dept Genet Med & Dev, Geneva, Switzerland.; Meda, P (reprint author), Univ Geneva, Fac Med, Dept Cell Physiol & Metab, Geneva, Switzerland. EM valentina.cigliola@unige.ch; paolo.meda@unige.ch FU Swiss National Science Foundation (SNF) [310030_141162]; Juvenile Diabetes Research Foundation (JDRF) [40-2011-11]; SNF; NIH/NIDDK FX This work was supported by grants from the Swiss National Science Foundation (SNF; 310030_141162) and the Juvenile Diabetes Research Foundation (JDRF; 40-2011-11) to PM, and from the SNF, JDRF and NIH/NIDDK to PLH. NR 59 TC 1 Z9 1 U1 0 U2 1 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 9 PY 2016 VL 11 IS 3 AR e0150880 DI 10.1371/journal.pone.0150880 PG 17 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DG3TF UT WOS:000371992300083 PM 26959991 ER PT J AU Dooraghi, AA Carroll, L Collins, J van Dam, RM Chatziioannou, AF AF Dooraghi, Alex A. Carroll, Lewis Collins, Jeffrey van Dam, R. Michael Chatziioannou, Arion F. TI ARAS: an automated radioactivity aliquoting system for dispensing solutions containing positron-emitting radioisotopes SO EJNMMI RESEARCH LA English DT Article DE Radiation detection; Automation; Aliquot; Dispense; Positron; Beta particle; PET; Positron emission tomography ID DOSE CALIBRATOR SETTINGS; NUCLEAR-MEDICINE AB Background: Automated protocols for measuring and dispensing solutions containing radioisotopes are essential not only for providing a safe environment for radiation workers but also to ensure accuracy of dispensed radioactivity and an efficient workflow. For this purpose, we have designed ARAS, an automated radioactivity aliquoting system for dispensing solutions containing positron-emitting radioisotopes with particular focus on fluorine-18 (F-18). Methods: The key to the system is the combination of a radiation detector measuring radioactivity concentration, in line with a peristaltic pump dispensing known volumes. Results: The combined system demonstrates volume variation to be within 5 % for dispensing volumes of 20 mu L or greater. When considering volumes of 20 mu L or greater, the delivered radioactivity is in agreement with the requested amount as measured independently with a dose calibrator to within 2 % on average. Conclusions: The integration of the detector and pump in an in-line system leads to a flexible and compact approach that can accurately dispense solutions containing radioactivity concentrations ranging from the high values typical of [F-18]fluoride directly produced from a cyclotron (similar to 0.1-1 mCi mu L-1) to the low values typical of batches of [F-18]fluoride-labeled radiotracers intended for preclinical mouse scans (similar to 1-10 mu Ci mu L-1). C1 [Dooraghi, Alex A.; Collins, Jeffrey; van Dam, R. Michael; Chatziioannou, Arion F.] Univ Calif Los Angeles, Crump Inst Mol Imaging, Los Angeles, CA 90095 USA. [Dooraghi, Alex A.; Collins, Jeffrey; van Dam, R. Michael; Chatziioannou, Arion F.] Univ Calif Los Angeles, Dept Mol & Med Pharmacol, Los Angeles, CA 90095 USA. [Dooraghi, Alex A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Carroll, Lewis] Carroll & Ramsey Associates, Albany, CA 94710 USA. RP Dooraghi, AA (reprint author), Univ Calif Los Angeles, Crump Inst Mol Imaging, Los Angeles, CA 90095 USA.; Dooraghi, AA (reprint author), Univ Calif Los Angeles, Dept Mol & Med Pharmacol, Los Angeles, CA 90095 USA.; Dooraghi, AA (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM alexdooraghi@gmail.com FU Department of Energy Office of Biological and Environmental Research [DE-SC0001249]; UCLA Foundation; UCLA Scholars in Oncologic Molecular Imaging program, NIH [R25T CA098010] FX This study was supported in part by the Department of Energy Office of Biological and Environmental Research (DE-SC0001249), the UCLA Foundation from a donation made by Ralph & Marjorie Crump for the UCLA Crump Institute for Molecular Imaging, and the UCLA Scholars in Oncologic Molecular Imaging program, NIH grant R25T CA098010. We thank Saman Sadeghi, Umesh Gangadharmath, and the staff of the UCLA Biomedical Cyclotron for providing the samples of [18F]fluoride and [18F]FDG and for performing sterility tests on samples. Finally, we thank Waldemar Ladno, Mark Lazari, Brandon Maraglia, David Prout, Olga Sergeeva, and David Stout for their input in the design and development of ARAS. NR 8 TC 0 Z9 0 U1 3 U2 18 PU SPRINGER HEIDELBERG PI HEIDELBERG PA TIERGARTENSTRASSE 17, D-69121 HEIDELBERG, GERMANY SN 2191-219X J9 EJNMMI RES JI EJNMMI Res. PD MAR 9 PY 2016 VL 6 AR 22 DI 10.1186/s13550-016-0176-9 PG 10 WC Radiology, Nuclear Medicine & Medical Imaging SC Radiology, Nuclear Medicine & Medical Imaging GA DF9XF UT WOS:000371715100001 PM 26956805 ER PT J AU Stillwell, RL Jenei, Z Weir, ST Vohra, YK Jeffries, JR AF Stillwell, Ryan L. Jenei, Zsolt Weir, Samuel T. Vohra, Yogesh K. Jeffries, Jason R. TI Superconducting Bi2Te: Pressure-induced universality in the (Bi-2)(m)(Bi2Te3)(n) series SO PHYSICAL REVIEW B LA English DT Article ID HGTE QUANTUM-WELLS; TOPOLOGICAL INSULATORS; TRANSITION-TEMPERATURE; PHASE-TRANSITION; SPIN; DEPENDENCE; EQUATION; ELECTRON; SURFACE; SOLIDS AB Using high-pressure magnetotransport techniques we have discovered superconductivity in Bi2Te, a member of the infinitely adaptive (Bi-2)(m)(Bi2Te3)(n) series, whose end members, Bi and Bi2Te3, can be tuned to display topological surface states or superconductivity. Bi2Te has a maximum T-c = 8.6 K at P = 14.5 GPa and goes through multiple high-pressure phase transitions, ultimately collapsing into a bcc structure that suggests a universal behavior across the series. High-pressure magnetoresistance and Hall measurements suggest a semimetal to metal transition near 5.4 GPa, which accompanies the hexagonal to intermediate phase transition seen via x-ray diffraction measurements. In addition, the linearity of H-c2(T) exceeds the Werthamer-Helfand-Hohenberg limit, even in the extreme spin-orbit scattering limit, yet is consistent with other strong spin-orbit materials. Considering these results in combination with similar reports on strong spin-orbit scattering materials seen in the literature, we suggest the need for a new theory that can address the unconventional nature of their superconducting states. C1 [Stillwell, Ryan L.; Jeffries, Jason R.] Lawrence Livermore Natl Lab, Div Mat Sci, Livermore, CA 94550 USA. [Jenei, Zsolt; Weir, Samuel T.] Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94550 USA. [Vohra, Yogesh K.] Univ Alabama Birmingham, Dept Phys, Birmingham, AL 35294 USA. RP Stillwell, RL (reprint author), Lawrence Livermore Natl Lab, Div Mat Sci, Livermore, CA 94550 USA. RI Jenei, Zsolt/B-3475-2011 FU U.S. Department of Energy (DOE) by Lawrence Livermore National Laboratory (LLNL) [DE-AC52-07NA27344]; DOE-NNSA [DE-NA0001974, DE-NA0002014]; DOE-BES [DE-FG02-99ER45775]; NSF; Advanced Photon Source is a U.S. DOE Office of Science User Facility by Argonne National Laboratory [DE-AC02-06CH11357] FX This work was performed under LDRD (Tracking Code No. 14-ERD-041) and under the auspices of the U.S. Department of Energy (DOE) by Lawrence Livermore National Laboratory (LLNL) under Contract No. DE-AC52-07NA27344. Portions of this work were performed at HPCAT (Sector 16), Advanced Photon Source (APS), Argonne National Laboratory. HPCAT operations are supported by the DOE-NNSA under Award No. DE-NA0001974 and the DOE-BES under Award No. DE-FG02-99ER45775 with partial instrumentation funding by the NSF. The Advanced Photon Source is a U.S. DOE Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. Beam time was provided by the Carnegie DOE-Alliance Center (CDAC). Y.K.V. acknowledges support from DOE-NNSA Grant No. DE-NA0002014. NR 56 TC 1 Z9 1 U1 8 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 9 PY 2016 VL 93 IS 9 AR 094511 DI 10.1103/PhysRevB.93.094511 PG 8 WC Physics, Condensed Matter SC Physics GA DG0CF UT WOS:000371729000006 ER PT J AU Bowers, ML Ophus, C Gautam, A Lancon, F Dahmen, U AF Bowers, M. L. Ophus, C. Gautam, A. Lancon, F. Dahmen, U. TI Step Coalescence by Collective Motion at an Incommensurate Grain Boundary SO PHYSICAL REVIEW LETTERS LA English DT Article ID RESOLUTION ELECTRON-MICROSCOPY; THIN-FILMS; MIGRATION; ENERGY; GOLD; DISCONNECTIONS; DISSOCIATION; SIMULATION; INTERFACES; MECHANISM AB Using extended time series scanning transmission electron microscopy, we investigate structural fluctuations at an incommensurate grain boundary in Au. Atomic-resolution imaging reveals the coalescence of two interfacial steps, or disconnections, of different height via coordinated motion of atoms along close-packed directions. Numerical simulations uncover a transition pathway that involves constriction and expansion of a characteristic stacking fault often associated with grain boundaries in face-centered cubic materials. It is found that local atomic fluctuations by enhanced point defect diffusion may play a critical role in initiating this transition. Our results offer new insights into the collective motion of atoms underlying the lateral advance of steps that control the migration of faceted grain boundaries. C1 [Bowers, M. L.; Ophus, C.; Gautam, A.; Dahmen, U.] LBNL, Natl Ctr Elect Microscopy, Mol Foundry, Berkeley, CA 94720 USA. [Lancon, F.] Univ Grenoble Alpes, F-38042 Grenoble, France. [Lancon, F.] CEA, INAC, SP2M, L Sim, F-38054 Grenoble, France. RP Bowers, ML (reprint author), LBNL, Natl Ctr Elect Microscopy, Mol Foundry, Berkeley, CA 94720 USA. FU Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231] FX Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 40 TC 1 Z9 1 U1 5 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 9 PY 2016 VL 116 IS 10 AR 106102 DI 10.1103/PhysRevLett.116.106102 PG 5 WC Physics, Multidisciplinary SC Physics GA DF9ZT UT WOS:000371722000013 PM 27015493 ER PT J AU Bostedt, C Boutet, S Fritz, DM Huang, ZR Lee, HJ Lemke, HT Robert, A Schlotter, WF Turner, JJ Williams, GJ AF Bostedt, Christoph Boutet, Sebastien Fritz, David M. Huang, Zhirong Lee, Hae Ja Lemke, Henrik T. Robert, Aymeric Schlotter, William F. Turner, Joshua J. Williams, Garth J. TI Linac Coherent Light Source: The first five years SO REVIEWS OF MODERN PHYSICS LA English DT Article ID FREE-ELECTRON LASER; RAY FREE-ELECTRON; SOFT-X-RAY; SERIAL FEMTOSECOND CRYSTALLOGRAPHY; AMPLIFIED SPONTANEOUS-EMISSION; LIPIDIC CUBIC PHASE; PROTEIN-STRUCTURE DETERMINATION; SPIN-CROSSOVER DYNAMICS; CHARGE-TRANSFER; ABSORPTION-SPECTROSCOPY AB A new scientific frontier opened in 2009 with the start of operations of the world's first x-ray free-electron laser (FEL), the Linac Coherent Light Source (LCLS), at SLAC National Accelerator Laboratory. LCLS provides femtosecond pulses of x rays (270 eV to 11.2 keV) with very high peak brightness to access new domains of ultrafast x-ray science. This article presents the fundamental FEL physics and outlines the LCLS source characteristics along with the experimental challenges, strategies, and instrumentation that accompany this novel type of x-ray source. The main part of the article reviews the scientific achievements since the inception of LCLS in the five primary areas it serves: atomic, molecular, and optical physics; condensed matter physics; matter in extreme conditions; chemistry and soft matter, and biology. C1 [Bostedt, Christoph; Boutet, Sebastien; Fritz, David M.; Huang, Zhirong; Lee, Hae Ja; Lemke, Henrik T.; Robert, Aymeric; Schlotter, William F.; Turner, Joshua J.; Williams, Garth J.] SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Bostedt, Christoph] Argonne Natl Lab, 9700 S Cass Ave, Lemont, IL 60439 USA. [Bostedt, Christoph] Northwestern Univ, Dept Phys & Astron, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Lemke, Henrik T.] Paul Scherrer Inst, CH-5232 Villigen, Switzerland. [Williams, Garth J.] Brookhaven Natl Lab, POB 5000, Upon, NY 11973 USA. RP Bostedt, C (reprint author), SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. RI Lemke, Henrik Till/N-7419-2016 OI Lemke, Henrik Till/0000-0003-1577-8643 FU LCLS; Stanford University through the Stanford Institute for Materials and Energy Sciences (SIMES); Lawrence Berkeley National Laboratory (LBNL); University of Hamburg through the BMBF priority program [FSP 301]; Center for Free Electron Laser (CFEL); Max Planck Society; Norah Berrah through a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, SISGR Grant [DE-SC0002004]; DOE Office of Science, Office of Fusion Energy Sciences [SF00515]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357, DE-SC0012704, DE-AC02-76SF00515] FX We are especially grateful for the guidance and support of Persis S. Drell in the realization of this manuscript. We express our sincere thanks to the many people at SLAC, Argonne, Lawrence Berkeley, and Lawrence Livermore National Laboratories, Cornell University, and the University of California, Los Angeles, who helped build LCLS, and to the accelerator physicists and the user community across the globe who contributed to making LCLS such a success. We also thank John Arthur, Uwe Bergmann, Mike Dunne, Paul Emma, Michael Forst, Kelly Gaffney, Jerry Hastings, Jerry LaRue, Richard Lee, Ingolf Lindau, Andy MacKinnon, Claudio Pellegrini, Ilme Schlichting, Jochen Schneider, Robert W. Schoenlein, Joachim Stohr, Soichi Wakatsuki, and Linda Young for their valuable feedback at various stages of the manuscript. We thank David Goldgof for his substantial effort assembling the reference list. We thank Terry Anderson and Gregory Stewart for helping with the figures. The SXR instrument at LCLS was funded by a consortium whose membership includes LCLS, Stanford University through the Stanford Institute for Materials and Energy Sciences (SIMES), Lawrence Berkeley National Laboratory (LBNL), the University of Hamburg through the BMBF priority program No. FSP 301, and the Center for Free Electron Laser (CFEL). We acknowledge the Max Planck Society for funding the development and operation of the CAMP instrument within the ASG at CFEL. The LAMP end station at AMO was partially funded by Norah Berrah through a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, SISGR Grant No. DE-SC0002004. The MEC instrument has additional support from the DOE Office of Science, Office of Fusion Energy Sciences under Contract No. SF00515. C. B. and G. J. W. acknowledge support from the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contracts No. DE-AC02-06CH11357 and No. DE-SC0012704, respectively. Use of the Linac Coherent Light Source (LCLS), SLAC National Accelerator Laboratory, is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515. NR 457 TC 31 Z9 31 U1 31 U2 80 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0034-6861 EI 1539-0756 J9 REV MOD PHYS JI Rev. Mod. Phys. PD MAR 9 PY 2016 VL 88 IS 1 AR 015007 DI 10.1103/RevModPhys.88.015007 PG 59 WC Physics, Multidisciplinary SC Physics GA DG0AF UT WOS:000371723300002 ER PT J AU Kelly, LL Racke, DA Schulz, P Li, H Winget, P Kim, H Ndione, P Sigdel, AK Bredas, JL Berry, JJ Graham, S Monti, OLA AF Kelly, Leah L. Racke, David A. Schulz, Philip Li, Hong Winget, Paul Kim, Hyungchul Ndione, Paul Sigdel, Ajaya K. Bredas, Jean-Luc Berry, Joseph J. Graham, Samuel Monti, Oliver L. A. TI Spectroscopy and control of near-surface defects in conductive thin film ZnO SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE gap state; hybrid organic/inorganic interface; two-photon photoemission; ZnO ID ZINC-OXIDE; PHOTOEMISSION; INTERFACES; STATES; CELLS AB The electronic structure of inorganic semiconductor interfaces functionalized with extended pi-conjugated organic molecules can be strongly influenced by localized gap states or point defects, often present at low concentrations and hard to identify spectroscopically. At the same time, in transparent conductive oxides such as ZnO, the presence of these gap states conveys the desirable high conductivity necessary for function as electron-selective interlayer or electron collection electrode in organic optoelectronic devices. Here, we report on the direct spectroscopic detection of a donor state within the band gap of highly conductive zinc oxide by two-photon photoemission spectroscopy. We show that adsorption of the prototypical organic acceptor C-60 quenches this state by ground-state charge transfer, with immediate consequences on the interfacial energy level alignment. Comparison with computational results suggests the identity of the gap state as a near-surface-confined oxygen vacancy. C1 [Kelly, Leah L.; Racke, David A.; Monti, Oliver L. A.] Univ Arizona, Dept Chem & Biochem, 1306 E Univ Blvd, Tucson, AZ 85721 USA. [Schulz, Philip; Ndione, Paul; Sigdel, Ajaya K.; Berry, Joseph J.] Natl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USA. [Schulz, Philip] Princeton Univ, Dept Elect Engn, Princeton, NJ 08544 USA. [Li, Hong; Winget, Paul; Kim, Hyungchul; Graham, Samuel] Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA. [Li, Hong; Winget, Paul; Kim, Hyungchul; Graham, Samuel] Ctr Organ Photon & Elect, Atlanta, GA 30332 USA. [Bredas, Jean-Luc] King Abdullah Univ Sci & Technol, Solar & Photovolta Engn Res Ctr, Div Phys Sci & Engn, Thuwal 239556900, Saudi Arabia. RP Monti, OLA (reprint author), Univ Arizona, Dept Phys, 1118 E Fourth St, Tucson, AZ 85721 USA. EM monti@u.arizona.edu RI Schulz, Philip/N-2295-2015; OI Schulz, Philip/0000-0002-8177-0108; Bredas, Jean-Luc /0000-0001-7278-4471 FU Center for Interface Science: Solar Electric Materials (CISSEM), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0001084] FX This work was supported as part of the Center for Interface Science: Solar Electric Materials (CISSEM), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award Number DE-SC0001084. NR 41 TC 2 Z9 2 U1 4 U2 30 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAR 9 PY 2016 VL 28 IS 9 AR 094007 DI 10.1088/0953-8984/28/9/094007 PG 9 WC Physics, Condensed Matter SC Physics GA DD9WZ UT WOS:000370277700008 PM 26871256 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, M Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Van de Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Van Parijs, I Barria, P Brun, H Caillol, C Clerbaux, B De Lentdecker, G Fasanella, G Favart, L Grebenyuk, A Karapostoli, G Lenzi, T Leonard, A Maerschalk, T Marinov, A Pernie, L Randle-conde, A Reis, T Seva, T Vander Velde, C Vanlaer, P Yonamine, R Zenoni, F Zhang, F Beernaert, K Benucci, L Cimmino, A Crucy, S Dobur, D Fagot, A Garcia, G Gul, M Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Salva, S Sigamani, M Strobbe, N Tytgat, M Van Driessche, W Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bondu, O Brochet, S Bruno, G Caudron, A Ceard, L Da Silveira, GG Delaere, C Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Mertens, A Nuttens, C Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Beliy, N Hammad, GH Alda, WL Alves, FL Alves, GA Brito, L Martins, MC Hamer, M Hensel, C Herrera, CM Moraes, A Pol, ME Teles, PR Das Chagas, EBB Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DDJ Martins, CDO De Souza, SF Guativa, LMH Malbouisson, H Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Ahuja, S Bernardes, CA Santos, ADS Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Moon, CS Novaes, SF Padula, SS Abad, DR Vargas, JCR Aleksandrov, A Hadjiiska, R Iaydjiev, P Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Ahmad, M Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Plestina, R Romeo, F Shaheen, SM Tao, J Wang, C Wang, Z Zhang, H Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Xu, Z Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Puljak, I Cipriano, PMR Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Micanovic, S Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Bodlak, M Finger, M Finger, M Abdelalim, AA Awad, A El Sawy, M Mahrous, A Radi, A Calpas, B Kadastik, M Murumaa, M Raidal, M Tiko, A Veelken, C Eerola, P Pekkanen, J Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Talvitie, J Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Favaro, C Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Machet, M Malcles, J Rander, J Rosowsky, A Titov, M Zghiche, A Antropov, I Baffioni, S Beaudette, F Busson, P Cadamuro, L Chapon, E Charlot, C Dahms, T Davignon, O Filipovic, N Florent, A de Cassagnac, RG Lisniak, S Mastrolorenzo, L Mine, P Naranjo, IN Nguyen, M Ochando, C Ortona, G Paganini, P Pigard, P Regnard, S Salerno, R Sauvan, JB Sirois, Y Strebler, T Yilmaz, Y Zabi, A Agram, JL Andrea, J Aubin, A Bloch, D Brom, JM Buttignol, M Chabert, EC Chanon, N Collard, C Conte, E Coubez, X Fontaine, JC Gelee, D Goerlach, U Goetzmann, C Le Bihan, AC Merlin, JA Skovpen, K Van Hove, P Gadrat, S Beauceron, S Bernet, C Boudoul, G Bouvier, E Montoya, CAC Chierici, R Contardo, D Courbon, B Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Lagarde, F Laktineh, IB Lethuillier, M Mirabito, L Pequegnot, AL Perries, S Alvarez, JDR Sabes, D Sgandurra, L Sordini, V Vander Donckt, M Verdier, P Viret, S Toriashvili, T Tsamalaidze, Z Autermann, C Beranek, S Edelhoff, M Feld, L Heister, A Kiesel, MK Klein, K Lipinski, M Ostapchuk, A Preuten, M Raupach, F Schael, S Schulte, JF Verlage, T Weber, H Wittmer, B Zhukov, V Ata, M Brodski, M Dietz-Laursonn, E Duchardt, D Endres, M Erdmann, M Erdweg, S Esch, T Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Millet, P Olschewski, M Padeken, K Papacz, P Pook, T Radziej, M Reithler, H Rieger, M Scheuch, F Sonnenschein, L Teyssier, D Thuer, S Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Hoehle, F Kargoll, B Kress, T Kuessel, Y Kunsken, A Lingemann, J Nehrkorn, A Nowack, A Nugent, IM Pistone, C Pooth, O Stahl, A Martin, MA Asin, I Bartosik, N Behnke, O Behrens, U Bell, AJ Borras, K Burgmeier, A Cakir, A Calligaris, L Campbell, A Choudhury, S Costanza, F Pardos, CD Dolinska, G Dooling, S Dorland, T Eckerlin, G Eckstein, D Eichhorn, T Flucke, G Gallo, E Garcia, JG Geiser, A Gizhko, A Gunnellini, P Hauk, J Hempel, M Jung, H Kalogeropoulos, A Karacheban, O Kasemann, M Katsas, P Kieseler, J Kleinwort, C Korol, I Lange, W Leonard, J Lipka, K Lobanov, A Lohmann, W Mankel, R Marfin, I Melzer-Pellmann, IA Meyer, AB Mittag, G Mnich, J Mussgiller, A Naumann-Emme, S Nayak, A Ntomari, E Perrey, H Pitzl, D Placakyte, R Raspereza, A Roland, B Sahin, MO Saxena, P Schoerner-Sadenius, T Schroeder, M Seitz, C Spannagel, S Trippkewitz, KD Walsh, R Wissing, C Blobel, V Vignali, MC Draeger, AR Erfle, J Garutti, E Goebel, K Gonzalez, D Gorner, M Haller, J Hoffmann, M Hoing, RS Junkes, A Klanner, R Kogler, R Lapsien, T Lenz, T Marchesini, I Marconi, D 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Lanaro, A. Levine, A. Long, K. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ruggles, T. Sarangi, T. Savin, A. Sharma, A. Smith, N. Smith, W. H. Taylor, D. Woods, N. CA CMS Collaboration TI Measurement of the t(t)over-bar production cross section in the all-jets final state in pp collisions at root s=8TeV SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID TAU LEPTON; TEV; ATLAS; PLUS AB The cross section for tt production in the all-jets final state is measured in pp collisions at a centre-of-mass energy of 8 TeV at the LHC with the CMS detector, in data corresponding to an integrated luminosity of 18.4 fb(-1). The inclusive cross section is found to be 275.6 +/- 6.1 (stat) +/- 37.8 (syst) +/- 7.2 (lumi) pb. The normalized differential cross sections are measured as a function of the top quark transverse momenta, pT, and compared to predictions from quantum chromodynamics. The results are reported at detector, parton, and particle levels. 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T.; Michelotto, M.; Montecassiano, F.; Passaseo, M.; Pazzini, J.; Pegoraro, M.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Carlin, R.; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.] Univ Padua, Padua, Italy. Univ Trent, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Perugia, I-27100 Pavia, Italy. [Montagna, P.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Solestizi, L. Alunni; Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Traczyk, P.] Ist Nazl Fis Nucl, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Musich, M.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. 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[Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Lee, S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, H.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.; Vaitkus, J.] Vilnius State Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan; Yusli, M. N.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De la Cruz-Burelo, E.; Heredia-De la Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Byszuk, A.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Leonardo, N.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Finger, M.; Finger, M., Jr.; Tsamalaidze, Z.; Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Matveev, V.; Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Bylinkin, A.; Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.] PN Lebedev Phys Inst, Leninsky Prospect 53, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Baskakov, A.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Korneeva, N.; Lokhtin, I.; Myagkov, I.; Obraztsov, S.; Perfilov, M.; Savrin, V.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Fac Phys, POB 550, Belgrade 11001, Serbia. [Adzic, P.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De la Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.] Ctr Invest Energet Medioambient & Tecnol CIRMAT, Madrid, Spain. [de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; De Castro Manzano, P.; Duarte Campderros, J.; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Trevisani, N.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Merlin, J. A.; Lingemann, J.; Pantaleo, F.; Hartmann, F.; Kornmayer, A.; Mohanty, A. K.; Silvestris, L.; Battilana, C.; Marzocchi, B.; Di Guida, S.; Paolucci, P.; Azzi, P.; Dall'Osso, M.; Zucchetta, A.; Ciangottini, D.; Donato, S.; D'imperio, G.; Traczyk, P.; Arcidiacono, R.; Candelise, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Castello, R.; Cerminara, G.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; Du Pree, T.; Duenser, M.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Zagozdzinska, A.; Zeuner, W. D.; Ulmer, K. A.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Kumar, Arun; Bartek, R.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Polatoz, A.; Cerci, D. Sunar; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Albayrak, E. A.; Guelmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-Storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Cripps, N.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Vazquez Acosta, M.; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Cutts, D.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Sinthuprasith, T.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Justus, C.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hasegawa, S.; Hirschauer, J.; Hu, Z.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Kwan, S.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Weber, H. A.; Whitbeck, A.; Yang, F.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Jung, A. W.; Taylor, L.; Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Di Giovanni, G. P.; Field, R. D.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Low, J. F.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Rossin, R.; Shchutska, L.; Snowball, M.; Sperka, D.; Terentyev, N.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Colafranceschi, S.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.] Univ Illinois, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Eminizer, N.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Osherson, M.; Roskes, J.; Sady, A.; Sarica, U.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Baty, A.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Niu, X.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Evans, A.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Roozbahani, B.] SUNY Buffalo, Buffalo, NY USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Woo, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Trovato, M.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Lynch, S.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Pearson, T.; Planer, M.; Reinsvold, A.; Ruchti, R.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Ji, W.; Kotov, K.; Ling, T. Y.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. 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P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Hughes, E.; Kaplan, S.; Elayavalli, R. Kunnawalkam; Lath, A.; Nash, K.; Panwalkar, S.; Park, M.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Foerster, M.; Riley, G.; Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Hernandez, A. Castaneda; Dalchenko, M.; De Mattia, M.; Delgado, A.; Dildick, S.; Eusebi, R.; Gilmore, J.; Kamon, T.; Krutelyov, V.; Mueller, R.; Osipenkov, I.; Patel, R.; Perloff, A.; Rose, A.; Safonov, A.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kunori, S.; Lamichhane, K.; Lee, S. W.; Libeiro, T.; Undleeb, S.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Janjam, R.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Ni, H.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.; Xu, Q.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Arenton, M. W.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Sun, X.; Wang, Y.; Wolfe, E.; Wood, J.; Xia, F.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Dodd, L.; Duric, S.; Friis, E.; Gomber, B.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Levine, A.; Long, K.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ruggles, T.; Sarangi, T.; Savin, A.; Sharma, A.; Smith, N.; Smith, W. H.; Taylor, D.; Woods, N.] Univ Wisconsin, Madison, WI 53706 USA. [Fruehwirth, R.; Krammer, M.; Schieck, J.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Zhang, F.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, Brazil. [Moon, C. S.] CNRS IN2P3, Paris, France. [Abdelalim, A. A.; Mahrous, A.] Helwan Univ, Cairo, Egypt. [Abdelalim, A. A.] Zewail City Sci & Technol, Zewail, Egypt. [El Sawy, M.] Beni Suef Univ, Bani Sweif, Egypt. [El Sawy, M.; Radi, A.] British Univ Egypt, Cairo, Egypt. [Radi, A.] Ain Shams Univ, Cairo, Egypt. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Hempel, M.; Karacheban, O.; Marfin, I.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Bhowmik, S.; Maity, M.; Sarkar, T.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.; Squillacioti, P.] Univ Siena, Via Laterina 8, I-53100 Siena, Italy. [Ali, M. A. B. Md] Int Islamic Univ Malaysia, Kuala Lumpur, Malaysia. [Idris, F. Mohamad; Byszuk, A.] Agensi Nuklear Malaysia, MOSTI, Kajang, Malaysia. [Heredia-De la Cruz, I.] Consejo Nacl Ciencia & Technol, Mexico City, DF, Mexico. [Zagozdzinska, A.] Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Orfanelli, S.] Natl Tech Univ Athens, Athens, Greece. [Rolandi, G.] Scuola Normale & Sez INFN, Pisa, Italy. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.] Gaziosmanpasa Univ, Tokat, Turkey. [Kangal, E. 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RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Stahl, Achim/E-8846-2011; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Colafranceschi, Stefano/M-1807-2016; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Andreev, Vladimir/M-8665-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Lokhtin, Igor/D-7004-2012; Della Ricca, Giuseppe/B-6826-2013; Manganote, Edmilson/K-8251-2013; Dubinin, Mikhail/I-3942-2016; TUVE', Cristina/P-3933-2015; VARDARLI, Fuat Ilkehan/B-6360-2013; Tinoco Mendes, Andre David/D-4314-2011; Varela, Joao/K-4829-2016; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Azarkin, Maxim/N-2578-2015; ciocci, maria agnese /I-2153-2015; Kirakosyan, Martin/N-2701-2015; Puljak, Ivica/D-8917-2017; Calderon, Alicia/K-3658-2014; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Ruiz, Alberto/E-4473-2011; Dudko, Lev/D-7127-2012; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Moraes, Arthur/F-6478-2010; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015 OI Stahl, Achim/0000-0002-8369-7506; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Della Ricca, Giuseppe/0000-0003-2831-6982; Dubinin, Mikhail/0000-0002-7766-7175; TUVE', Cristina/0000-0003-0739-3153; Tinoco Mendes, Andre David/0000-0001-5854-7699; Varela, Joao/0000-0003-2613-3146; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; ciocci, maria agnese /0000-0003-0002-5462; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Ruiz, Alberto/0000-0002-3639-0368; Dudko, Lev/0000-0002-4462-3192; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Moraes, Arthur/0000-0002-5157-5686; Ogul, Hasan/0000-0002-5121-2893; FU Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS programme of the Foundation for Polish Science; European Union, Regional Development Fund; OPUS programme of the National Science Center (Poland); Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR project (Italy) [20108T4XTM]; Thalis programme - EU-ESF; Aristeia programme - EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); Welch Foundation [C-1845] FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP and NRF (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (NewZealand); PAEC(Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (UK); DOE and NSF (USA). Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS programme of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the OPUS programme of the National Science Center (Poland); the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); and the Welch Foundation, contract C-1845. NR 56 TC 1 Z9 1 U1 20 U2 38 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD MAR 8 PY 2016 VL 76 IS 3 AR 128 DI 10.1140/epjc/s10052-016-3956-5 PG 26 WC Physics, Particles & Fields SC Physics GA DL0CZ UT WOS:000375300800001 ER PT J AU Pedersen, L Idorn, M Olofsson, GH Lauenborg, B Nookaew, I Hansen, RH Johannesen, HH Becker, JC Pedersen, KS Dethlefsen, C Nielsen, J Gehl, J Pedersen, BK Straten, PT Hojman, P AF Pedersen, Line Idorn, Manja Olofsson, Gitte H. Lauenborg, Britt Nookaew, Intawat Hansen, Rasmus Hvass Johannesen, Helle Hjorth Becker, Jurgen C. Pedersen, Katrine S. Dethlefsen, Christine Nielsen, Jens Gehl, Julie Pedersen, Bente K. Straten, Per Thor Hojman, Pernille TI Voluntary Running Suppresses Tumor Growth through Epinephrine- and IL-6-Dependent NK Cell Mobilization and Redistribution SO CELL METABOLISM LA English DT Article ID MISSING-SELF-RECOGNITION; NATURAL-KILLER-CELLS; PHYSICAL-ACTIVITY; CANCER; EXERCISE; IL-6; MUSCLE; INFLAMMATION; PHENOTYPE; CYTOKINES AB Regular exercise reduces the risk of cancer and disease recurrence. Yet the mechanisms behind this protection remain to be elucidated. In this study, tumor-bearing mice randomized to voluntary wheel running showed over 60% reduction in tumor incidence and growth across five different tumor models. Microarray analysis revealed training-induced up-regulation of pathways associated with immune function. NK cell infiltration was significantly increased in tumors from running mice, whereas depletion of NK cells enhanced tumor growth and blunted the beneficial effects of exercise. Mechanistic analyses showed that NK cells were mobilized by epinephrine, and blockade of beta-adrenergic signaling blunted training-dependent tumor inhibition. Moreover, epinephrine induced a selective mobilization of IL-6-sensitive NK cells, and IL-6-blocking antibodies blunted training-induced tumor suppression, intratumoral NK cell infiltration, and NK cell activation. Together, these results link exercise, epinephrine, and IL-6 to NK cell mobilization and redistribution, and ultimately to control of tumor growth. C1 [Pedersen, Line; Lauenborg, Britt; Pedersen, Katrine S.; Dethlefsen, Christine; Pedersen, Bente K.; Hojman, Pernille] Univ Copenhagen, Rigshosp, Fac Hlth Sci, Ctr Inflammat & Metab, DK-2100 Copenhagen, Denmark. [Pedersen, Line; Lauenborg, Britt; Pedersen, Katrine S.; Dethlefsen, Christine; Pedersen, Bente K.; Hojman, Pernille] Univ Copenhagen, Rigshosp, Fac Hlth Sci, Ctr Phys Act Res, DK-2100 Copenhagen, Denmark. [Idorn, Manja; Olofsson, Gitte H.; Straten, Per Thor] Copenhagen Univ Hosp, Crt Canc Immune Therapy, Dept Hematol, DK-2730 Herlev, Denmark. [Nookaew, Intawat; Nielsen, Jens] Chalmers, Dept Biol & Biol Engn, SE-412 Gothenburg, Sweden. [Nookaew, Intawat] Oak Ridge Natl Lab, Biosci Div, Comparat Genom Grp, Oak Ridge, TN 37831 USA. [Hansen, Rasmus Hvass; Johannesen, Helle Hjorth] Univ Copenhagen Hosp, Dept Radiol, DK-2730 Herlev, Denmark. [Becker, Jurgen C.] Univ Hosp Essen, Westdeutsches Tumorzentrum, German Canc Consortium DKTK, Dept Translat Skin Canc Res TSCR, D-45117 Essen, Germany. [Gehl, Julie; Hojman, Pernille] Copenhagen Univ Hosp, Dept Oncol, DK-2730 Herlev, Denmark. [Straten, Per Thor] Univ Copenhagen, Dept Immunol & Microbiol, DK-2200 Copenhagen, Denmark. RP Hojman, P (reprint author), Univ Copenhagen, Rigshosp, Fac Hlth Sci, Ctr Inflammat & Metab, DK-2100 Copenhagen, Denmark.; Hojman, P (reprint author), Univ Copenhagen, Rigshosp, Fac Hlth Sci, Ctr Phys Act Res, DK-2100 Copenhagen, Denmark.; Hojman, P (reprint author), Copenhagen Univ Hosp, Dept Oncol, DK-2730 Herlev, Denmark. EM phojman@inflammation-metabolism.dk OI Nielsen, Jens/0000-0002-9955-6003; Gehl, Julie/0000-0003-3829-0210; thor Straten, Per/0000-0002-4731-4969 FU Danish National Research Foundation [DNRF55]; TrygFonden; Danish Medical Research Council; Novo Nordic Foundation; Lundbeck Foundation; Danish Cancer Society; Aase og Ejnar Danielsen Foundation FX Anne Boye, Lone Christensen, Lone Peijs, Maria Scheel, and Marianne Fregil are acknowledged for their technical assistance. Centre of Inflammation and Metabolism (CIM) is supported the Danish National Research Foundation (DNRF55). Centre of Physical Activity Research (CFAS) is supported by TrygFonden. This study was further supported by the Danish Medical Research Council, Novo Nordic Foundation, Lundbeck Foundation, Danish Cancer Society, and Aase og Ejnar Danielsen Foundation. NR 33 TC 26 Z9 27 U1 20 U2 46 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 1550-4131 EI 1932-7420 J9 CELL METAB JI Cell Metab. PD MAR 8 PY 2016 VL 23 IS 3 BP 554 EP 562 DI 10.1016/j.cmet.2016.01.011 PG 9 WC Cell Biology; Endocrinology & Metabolism SC Cell Biology; Endocrinology & Metabolism GA DI6MU UT WOS:000373614100022 PM 26895752 ER PT J AU Lee, W Lee, C Yu, H Kim, DJ Wang, C Woo, HY Oh, JH Kim, BJ AF Lee, Wonho Lee, Changyeon Yu, Hojeong Kim, Dong-Jun Wang, Cheng Woo, Han Young Oh, Joon Hak Kim, Bumjoon J. TI Side Chain Optimization of Naphthalenediimide-Bithiophene-Based Polymers to Enhance the Electron Mobility and the Performance in All-Polymer Solar Cells SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article ID POWER CONVERSION EFFICIENCY; THIN-FILM TRANSISTORS; MOLECULAR-ORIENTATION; CONJUGATED POLYMER; BULK HETEROJUNCTIONS; CHARGE-TRANSPORT; BLEND MORPHOLOGY; ADDITIVE-FREE; CRYSTALLINITY; AGGREGATION AB Tuning the side chains of conjugated polymers is a simple, yet effective strategy for modulating their structural and electrical properties, but their impact on n-type conjugated polymers has not been studied extensively, particularly in the area of all-polymer solar cells (all-PSCs). Herein, the effects of side chain engineering of P(NDI2OD-T2) polymer (also known as Polyera Activink N2200) are investigated, which is the most widely used n-type polymer in all-PSCs and organic field-effect transistors (OFETs), on their structural and electronic properties. A series of naphthalenediimide-bithiophene-based copolymers (P(NDIR-T2)) is synthesized, with different side chains (R) of 2-hexyldecyl (2-HD), 2-octyldodecyl (2-OD), and 2-decyltetradecyl (2-DT). The P(NDI2HD-T2) exhibits more noticeable crystalline behaviors than P(NDI2OD-T2) and P(NDI2DT-T2), thereby facilitating superior 3D charge transport. For example, the P(NDI2HD-T2) shows the highest OFET electron mobility (1.90 cm(2) V-1 s(-1)). Also, a series of all-PSCs is produced using different electron donors of PTB7-Th, PTB7, and PPDT2FBT. The P(NDI2HD-T2) based all-PSCs produce much higher power conversion efficiency (PCE) irrespective of the electron donors. In particular, the PTB7-Th: P(NDI2HD-T2) forms highly ordered, strong face-on interchain stackings, and has better intermixed bulk-heterojunction morphology, producing the highest PCE of 6.11% that has been obtained by P(NDIR-T2) based all-PSCs to date. C1 [Lee, Wonho; Lee, Changyeon; Kim, Dong-Jun; Kim, Bumjoon J.] Korea Adv Inst Sci & Technol, Dept Chem & Biomol Engn, Daejeon 305701, South Korea. [Yu, Hojeong; Oh, Joon Hak] Pohang Univ Sci & Technol POSTECH, Dept Chem Engn, Pohang 790784, South Korea. [Yu, Hojeong] UNIST, Sch Energy & Chem Engn, Ulsan 689798, South Korea. [Wang, Cheng] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Woo, Han Young] Korea Univ, Dept Chem, Seoul 136701, South Korea. RP Kim, BJ (reprint author), Korea Adv Inst Sci & Technol, Dept Chem & Biomol Engn, Daejeon 305701, South Korea. EM bumjoonkim@kaist.ac.kr RI Kim, Bumjoon J./C-1714-2011; Oh, Joon Hak/F-1454-2010; Lee, Wonho/K-9246-2016; Wang, Cheng/A-9815-2014 OI Oh, Joon Hak/0000-0003-0481-6069; Lee, Wonho/0000-0003-1323-8184; FU National Research Foundation - Korean Government [2013R1A2A1A03069803]; Global Ph.D. Fellowship Program through the National Research Foundation of Korea - Ministry of Education [2014-1021859] FX This research was supported by the National Research Foundation Grant (2013R1A2A1A03069803), funded by the Korean Government. W.L. acknowledges the Global Ph.D. Fellowship Program through the National Research Foundation of Korea, funded by the Ministry of Education (2014-1021859). NR 68 TC 14 Z9 14 U1 37 U2 104 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD MAR 8 PY 2016 VL 26 IS 10 BP 1543 EP 1553 DI 10.1002/adfm.201504191 PG 11 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DG8CC UT WOS:000372309000005 ER PT J AU Petrie, JR Mitra, C Jeen, H Choi, WS Meyer, TL Reboredo, FA Freeland, JW Eres, G Lee, HN AF Petrie, Jonathan R. Mitra, Chandrima Jeen, Hyoungjeen Choi, Woo Seok Meyer, Tricia L. Reboredo, Fernando A. Freeland, John W. Eres, Gyula Lee, Ho Nyung TI Strain Control of Oxygen Vacancies in Epitaxial Strontium Cobaltite Films SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article ID MINIMUM ENERGY PATHS; ELASTIC BAND METHOD; REDOX REACTIONS; SADDLE-POINTS; DIFFUSION; SRCOO2.5; PHYSICS; OXIDES AB The ability to manipulate oxygen anion defects rather than metal cations in complex oxides can facilitate creating new functionalities critical for emerging energy and device technologies. However, the diffi culty in activating oxygen at reduced temperatures hinders the deliberate control of important defects, oxygen vacancies. Here, strontium cobaltite (SrCoOx) is used to demonstrate that epitaxial strain is a powerful tool for manipulating the oxygen vacancy concentration even under highly oxidizing environments and at annealing temperatures as low as 300 degrees C. By applying a small biaxial tensile strain (2%), the oxygen activation energy barrier decreases by approximate to 30%, resulting in a tunable oxygen defi cient steady-state under conditions that would normally fully oxidize unstrained cobaltite. These strain-induced changes in oxygen stoichiometry drive the cobaltite from a ferromagnetic metal towards an antiferromagnetic insulator. The ability to decouple the oxygen vacancy concentration from its typical dependence on the operational environment is useful for effectively designing oxides materials with a specifi c oxygen stoichiometry. C1 [Petrie, Jonathan R.; Mitra, Chandrima; Jeen, Hyoungjeen; Choi, Woo Seok; Meyer, Tricia L.; Reboredo, Fernando A.; Eres, Gyula; Lee, Ho Nyung] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Freeland, John W.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Lee, HN (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM hnlee@ornl.gov RI Choi, Woo Seok/G-8783-2014; Lee, Ho Nyung/K-2820-2012; Eres, Gyula/C-4656-2017 OI Lee, Ho Nyung/0000-0002-2180-3975; Eres, Gyula/0000-0003-2690-5214 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; U.S. Department of Energy, Office of Science [DE-AC02-06CH11357] FX This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, under Contract No. DE-AC02-06CH11357. NR 47 TC 13 Z9 13 U1 17 U2 58 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD MAR 8 PY 2016 VL 26 IS 10 BP 1564 EP 1570 DI 10.1002/adfm.201504868 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DG8CC UT WOS:000372309000007 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Abeloos, B Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allen, BW Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Armitage, LJ Arnaez, O Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Artz, S Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Balunas, WK Banas, E Banerjee, S Bannoura, AAE Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Navarro, LB Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, M Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bedognetti, M Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, AS Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Belyaev, NL Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Benitez, J Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Berlendis, S Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Biedermann, D Bielski, R Biesuz, NV Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biondi, S Bjergaard, DM Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Blunier, S Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehler, M Boerner, D Bogaerts, JA Bogavac, D Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Bortfeldt, J Bortoletto, D Bortolotto, V Bos, K Boscherini, D Bosman, M Sola, JDB Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutle, SK Boveia, A Boyd, J Boyko, IR Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Madden, WDB Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Broughton, JH De Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Brunt, BH Bruschi, M Bruscino, N Bryant, P Bryngemark, L Buanes, T Buat, Q Buchholz, P Buckley, AG Budagov, IA Buehrer, F Bugge, MK Bulekov, O Bullock, D Burckhart, H Burdin, S Burgard, CD Burghgrave, B Burka, K Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Buzykaev, AR Urban, SC Caforio, D Cairo, VM Cakir, O Calace, N Calafiura, P Calandri, A Calderini, G Calfayan, P Caloba, LP Calvet, D Calvet, S Calvet, TP Toro, RC Camarda, S Camarri, P Cameron, D Armadans, RC Camincher, C Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Carbone, RM Cardarelli, R Cardillo, F Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Casper, DW Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catinaccio, A Catmore, JR Cattai, A Caudron, J Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Alberich, LC Cerio, BC Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chan, YL Chang, P Chapman, JD Charlton, DG Chau, CC Barajas, CAC Che, S Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, S Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A Cheremushkina, E El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiarelli, G Chiodini, G Chisholm, AS Chitan, A Chizhov, MV Choi, K Chouridou, S Chow, BKB Christodoulou, V Chromek-Burckhart, D Chudoba, J Chuinard, AJ Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Cinca, D Cindro, V Cioara, IA Ciocio, A Cirotto, F Citron, ZH Ciubancan, M Clark, A Clark, BL Clark, PJ Clarke, RN Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Colasurdo, L Cole, B Cole, S Colijn, AP Collot, J Colombo, T Compostella, G Muino, PC Coniavitis, E Connell, SH Connelly, IA Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cottin, G Cowan, G Cox, BE Cranmer, K Crawley, SJ Cree, G Crepe-Renaudin, S Crescioli, F Cribbs, WA Ortuzar, MC Cristinziani, M Croft, V Crosetti, G Donszelmann, TC Cummings, J Curatolo, M Cuth, J Cuthbert, C Czirr, H Czodrowski, P D'Auria, S D'Onofrio, M De Sousa, MJDS Da Via, C Dabrowski, W Dai, T Dale, O Dallaire, F Dallapiccola, C Dam, M Dandoy, JR Dang, NP Daniells, AC Dann, NS Danninger, M Hoffmann, MD Dao, V Darbo, G Darmora, S Dassoulas, J Dattagupta, A Davey, W David, C Davidek, T Davies, M Davison, P Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Benedetti, A De Castro, S De Cecco, S De Groot, N de Jong, P De la Torre, H De Lorenzi, F De Pedis, D De Salvo, A De Sanctis, U De Santo, A De Regie, JBDV Dearnaley, WJ Debbe, R Debenedetti, C Dedovich, DV Deigaard, I Del Peso, J Del Prete, T Delgove, D Deliot, F Delitzsch, CM Deliyergiyev, M Dell'Acqua, A Dell'Asta, L Dell'Orso, M Della Pietra, M della Volpe, D Delmastro, M Delsart, PA Deluca, C DeMarco, DA Demers, S Demichev, M Demilly, A Denisov, SP Denysiuk, D Derendarz, D Derkaoui, JE Derue, F Dervan, P Desch, K Deterre, C Dette, K Deviveiros, PO Dewhurst, A Dhaliwal, S Di Ciaccio, A Di Ciaccio, L Di Clemente, WK Di Domenico, A Di Donato, C Di Girolamo, A Di Girolamo, B Di Mattia, A Di Micco, B Di Nardo, R Di Simone, A Di Sipio, R Di Valentino, D Diaconu, C Diamond, M Dias, FA Diaz, MA Diehl, EB Dietrich, J Diglio, S Dimitrievska, A Dingfelder, J Dita, P Dita, S Dittus, F Djama, F Djobava, T Djuvsland, JI do Vale, MAB Dobos, D Dobre, M Doglioni, C Dohmae, T Dolejsi, J Dolezal, Z Dolgoshein, BA Donadelli, M Donati, S Dondero, P Donini, J Dopke, J Doria, A Dova, MT Doyle, AT Drechsler, E Dris, M Du, Y Duarte-Campderros, J Duchovni, E Duckeck, G Ducu, OA Duda, D Dudarev, A Ot, LD Duguid, L Duhrssen, M Dunford, M Yildiz, HD Duren, M Durglishvili, A Duschinger, D Dutta, B Dyndal, M Eckardt, C Ecker, KM Edgar, RC Edson, W Edwards, NC Eifert, T Eigen, G Einsweiler, K Ekelof, T El Kacimi, M Ellajosyula, V Ellert, M Elles, S Ellinghaus, F Elliot, AA Ellis, N Elmsheuser, J Elsing, M Emeliyanov, D Enari, Y Endner, OC Endo, M Ennis, JS Erdmann, J Ereditato, A Ernis, G Ernst, J Ernst, M Errede, S Ertel, E Escalier, M Esch, H Escobar, C Esposito, B Etienvre, AI Etzion, E Evans, H Ezhilov, A Fabbri, L Facini, G Fakhrutdinov, RM Falciano, S Falla, RJ Faltova, J Fang, Y Fanti, M Farbin, A Farilla, A Farina, C Farooque, T Farrell, S Farrington, SM Farthouat, P Fassi, F Fassnacht, P Fassouliotis, D Giannelli, MF Favareto, A Fayard, L Fedin, OL Fedorko, W Feigl, S Feligioni, L Feng, C Feng, EJ Feng, H Fenyuk, AB Feremenga, L Martinez, PF Perez, SF Ferrando, J Ferrari, A Ferrari, P Ferrari, R de Lima, DEF Ferrer, A Ferrere, D Ferretti, C Parodi, AF Fiedler, F Filipcic, A Filipuzzi, M Filthaut, F Fincke-Keeler, M Finelli, KD Fiolhais, MCN Fiorini, L Firan, A Fischer, A Fischer, C Fischer, J Fisher, WC Flaschel, N Fleck, I Fleischmann, P Fletcher, GT Fletcher, G Fletcher, RRM Flick, T Floderus, A Castillo, LRF Flowerdew, MJ Forcolin, GT Formica, A Forti, A Fournier, D Fox, H Fracchia, S Francavilla, P Franchini, M Francis, D Franconi, L Franklin, M Frate, M Fraternali, M Freeborn, D Fressard-Batraneanu, SM Friedrich, F Froidevaux, D Frost, JA Fukunaga, C Torregrosa, EF Fusayasu, T Fuster, J Gabaldon, C Gabizon, O Gabrielli, A Gabrielli, A Gach, GP Gadatsch, S Gadomski, S Gagliardi, G Gagnon, P Galea, C Galhardo, B Gallas, EJ Gallop, BJ Gallus, P Galster, G Gan, KK Gao, J Gao, Y Gao, YS Walls, FMG Garcia, C Navarro, JEG Garcia-Sciveres, M Gardner, RW Garelli, N Garonne, V Bravo, AG Gatti, C Gaudiello, A Gaudio, G Gaur, B Gauthier, L Gavrilenko, IL Gay, C Gaycken, G Gazis, EN Gecse, Z Gee, CNP Geich-Gimbel, C Geisler, MP Gemme, C Genest, MH Geng, C Gentile, S George, S Gerbaudo, D Gershon, A Ghasemi, S Ghazlane, H Giacobbe, B Giagu, S Giannetti, P Gibbard, B Gibson, SM Gignac, M Gilchriese, M Gillam, TPS Gillberg, D Gilles, G Gingrich, DM Giokaris, N Giordani, MP Giorgi, FM Giorgi, FM Giraud, PF Giromini, P Giugni, D Giuliani, C Giulini, M Gjelsten, BK Gkaitatzis, S Gkialas, I Gkougkousis, EL Gladilin, LK Glasman, C Glatzer, J Glaysher, PCF Glazov, A Goblirsch-Kolb, M Godlewski, J Goldfarb, S Golling, T Golubkov, D Gomes, A Goncalo, R Da Costa, JGPF Gonella, L Gongadze, A de la Hoz, SG Parra, GG Gonzalez-Sevilla, S Goossens, L Gorbounov, PA Gordon, HA Gorelov, I Gorini, B Gorini, E Gorisek, A Gornicki, E Goshaw, AT Gossling, C Gostkin, MI Goudet, CR Goujdami, D Goussiou, AG Govender, N Gozani, E 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Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. Nedden, M. zur Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Search for new phenomena with photon plus jet events in proton-proton collisions at TeV with the ATLAS detector SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article ID PARTON DISTRIBUTIONS; HADRON COLLIDERS; DENSITY-FUNCTION; PP COLLISIONS; LHC; DIMENSIONS; MILLIMETER; HIERARCHY; MASS AB A search is performed for the production of high-mass resonances decaying into a photon and a jet in 3.2 fb(-1) of proton-proton collisions at a centre-of-mass energy of TeV collected by the ATLAS detector at the Large Hadron Collider. Selected events have an isolated photon and a jet, each with transverse momentum above 150 GeV. No significant deviation of the gamma+jet invariant mass distribution from the background-only hypothesis is found. Limits are set at 95% confidence level on the cross sections of generic Gaussian-shaped signals and of a few benchmark phenomena beyond the Standard Model: excited quarks with vector-like couplings to the Standard Model particles, and non-thermal quantum black holes in two models of extra spatial dimensions. The minimum excluded visible cross sections for Gaussian-shaped resonances with width-to-mass ratios of 2% decrease from about 6 fb for a mass of 1.5 TeV to about 0.8 fb for a mass of 5 TeV. The minimum excluded visible cross sections for Gaussian-shaped resonances with width-to-mass ratios of 15% decrease from about 50 fb for a mass of 1.5 TeV to about 1.0 fb for a mass of 5 TeV. Excited quarks are excluded below masses of 4.4 TeV, and non-thermal quantum black holes are excluded below masses of 3.8 (6.2) TeV for Randall-Sundrum (Arkani-Hamed-Dimopoulous-Dvali) models with one (six) extra dimensions. C1 [Jackson, P.; Lee, L.; Petridis, A.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Yildiz, H. Duran] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Kuday, S.] Istanbul Aydin Univ, Istanbul, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. 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A.; Jones, S.; Lampl, W.; Leone, R.; Loch, P.; Nayyar, R.; O'grady, F.; Rutherfoord, J. P.; Shupe, M. A.; Varnes, E. W.; Veatch, J.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Brandt, A.; Bullock, D.; Darmora, S.; De, K.; Farbin, A.; Feremenga, L.; Griffiths, J.; Hadavand, H. K.; Heelan, L.; Ozturk, N.; Schovancova, J.; Stradling, A. R.; Usai, G.; Vartapetian, A.; White, A.; Yu, J.] Univ Texas Arlington, Dept Phys, POB 19059, Arlington, TX 76019 USA. [Angelidakis, S.; Chouridou, S.; Fassouliotis, D.; Giokaris, N.; Ioannou, P.; Kourkoumelis, C.; Tsirintanis, N.] Univ Athens, Dept Phys, Athens, Greece. [Alexopoulos, T.; Benekos, N.; Dris, M.; Gazis, E. N.; Karakostas, K.; Karastathis, N.; Karentzos, E.; Leontsinis, S.; Maltezos, S.; Ntekas, K.; Panagiotopoulou, E. St.; Papadopoulou, Th. D.; Tsipolitis, G.; Vlachos, S.] Natl Tech Univ Athens, Dept Phys, Zografos, Greece. [Abdinov, O.; Ahmadov, F.; Huseynov, N.; Javadov, N.; Khalil-zada, F.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Anjos, N.; Bosman, M.; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fernandez Perez, S.; Fisher, W. C.; Gonzalez Parra, G.; Grinstein, S.; Juste Rozas, A.; Korolkov, I.; Lange, J. C.; Le Menedeu, E.; Lopez Paz, I.; Martinez, M.; Mir, L. M.; Pacheco Pages, A.; Padilla Aranda, C.; Riu, I.; Rodriguez Perez, A.; Sorin, V.; Tripiana, M. F.; Tsiskaridze, S.; Valery, L.] Barcelona Inst Sci & Technol, Inst Fis Altes Energies, Barcelona, Spain. [Agatonovic-Jovin, T.; Bogavac, D.; Dimitrievska, A.; Krstic, J.; Marjanovic, M.; Popovic, D. S.; Sijacki, Dj.; Simic, Lj.; Vranjes, N.; Milosavljevic, M. Vranjes; Zivkovic, L.] Univ Belgrade, Inst Phys, Belgrade, Serbia. [Buanes, T.; Dale, O.; Eigen, G.; Kastanas, A.; Liebig, W.; Lipniacka, A.; Maeland, S.; Latour, B. Martin Dit; Sjursen, T. B.; Smestad, L.; Stugu, B.; Yang, Z.; Zalieckas, J.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Amadio, B. T.; Axen, B.; Barnett, R. M.; Beringer, J.; Brosamer, J.; Calafiura, P.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Einsweiler, K.; Farrell, S.; Gabrielli, A.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Heim, T.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Biedermann, D.; Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Hristova, I.; Kind, O. M.; Kolanoski, H.; Lacker, H.; Lohse, T.; Mergelmeyer, S.; Nikiforov, A.; Rehnisch, L.; Rieck, P.; Schulz, H.; Sperlich, D.; Stamm, S.; Nedden, M. zur] Humboldt Univ, Dept Phys, Invalidenstr 110, Berlin, Germany. [Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Mullier, G. A.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Mullier, G. A.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allport, P. P.; Bella, L. Aperio; Baca, M. J.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Gonella, L.; Hawkes, C. M.; Hillier, S. J.; Levy, M.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Owen, R. E.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Cetin, S. A.] Istanbul Bilgi Univ, Fac Engn & Nat Sci, Istanbul, Turkey. [Beddall, A. J.] Bahcesehir Univ, Fac Engn & Nat Sci, Istanbul, Turkey. [Alberghi, G. L.; Bellagamba, L.; Biondi, S.; Boscherini, D.; Bruni, A.; Bruni, G.; De Castro, S.; Fabbri, L.; Franchini, M.; Giacobbe, B.; Giorgi, F. M.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Spighi, R.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Alberghi, G. L.; Biondi, S.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Bruscino, N.; Cioara, I. A.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Gaycken, G.; Geich-Gimbel, Ch.; Grefe, C.; Haefner, P.; Hansen, M. C.; Hohn, D.; Huegging, F.; Jansen, E.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lantzsch, K.; Lenz, T.; Leyko, A. M.; Liebal, J.; Mijovic, L.; Moles-Valls, R.; Obermann, T.; Pohl, D.; Ricken, O.; Sarrazin, B.; Schaepe, S.; Schopf, E.; Schultens, M. J.; Schwindt, T.; Seema, P.; Stillings, J. A.; von Toerne, E.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Yuen, S. P. Y.; Zhang, R.] Univ Bonn, Inst Phys, Nussallee 12, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, 590 Commonwealth Ave, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Barone, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Dhaliwal, S.; Loew, K. M.; Sciolla, G.; Venturini, A.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.; Peralva, B. S.] Fed Univ Juiz De Fora UFJF, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao Del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; La Rosa Navarro, J. L.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, CP 20516, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kravchenko, A.; Lanni, F.; Lee, C. A.; Lissauer, D.; Liu, H.; Lynn, D.; Ma, H.; Maeno, T.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Xu, L.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. Transilvania Univ Brasov, Brasov, Romania. [Alexa, C.; Boldea, V.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Pantea, D.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Bossio Sola, J. D.; Marceca, G.; Otero Y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Brunt, B. H.; Carter, J. R.; Chapman, J. D.; Cottin, G.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Potter, C. J.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Gillberg, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Gonzalez, B. Alvarez; Amoroso, S.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beermann, T. A.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Carrillo-Montoya, G. D.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Colombo, T.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feng, E. J.; Francis, D.; Fressard-Batraneanu, S. M.; Froidevaux, D.; Gadatsch, S.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Gumpert, C.; Hawkings, R. J.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jakobsen, S.; Jenni, P.; Klioutchnikova, T.; Krasznahorkay, A.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Berlingen, J. Montejo; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poulard, G.; Poveda, J.; Astigarraga, M. E. Pozo; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Ruthmann, N.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sforza, F.; Sanchez, C. A. Solans; Spigo, G.; Staerz, S.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wenig, S.; Werner, P.; Wilkens, H. 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Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Geng, C.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y. L.; Liu, Y.; Peng, H.; Song, H. Y.; Zhang, G.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Du, Y.; Feng, C.; Liu, B.; Ma, L. L.; Wang, C.; Zaidan, R.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Shanghai Key Lab Particle Phys & Cosmol, Dept Phys & Astron, Shanghai 200030, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Alkire, S. P.; Angerami, A.; Brooijmans, G.; Carbone, R. M.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Loevschall-Jensen, A. E.; Monk, J.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, Arcavacata Di Rende, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Gach, G. P.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; De Renstrom, P. A. Bruckman; Burka, K.; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Bessner, M.; Bloch, I.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitz, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Notkestr 85, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Zeuthen, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.; Schorlemmer, A. L. S.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Pino, S. A. Olivares; Proissl, M.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schnoor, U.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; De Mendizabal, J. Bilbao; Calace, N.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; March, L.; Mermod, P.; Miucci, A.; Nackenhorst, O.; Nessi, M.; Paolozzi, L.; Ristic, B.; Schramm, S.; Sfyrla, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Heinz, C.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; Crawley, S. J.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Knue, A.; Mullen, P.; O'Shea, V.; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nadal, J.; Quadt, A.; Rieger, J.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Berlendis, S.; Camincher, C.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Petit, E.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subat & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Clark, B. L.; Franklin, M.; Giromini, P.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Rogan, C. S.; Skottowe, H. P.; Sun, S.; Tolley, E.; Tong, B.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolb, M.; Lisovyi, M.; Schaetzel, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Castillo, L. R. Flores; Lu, H.; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.; Orlando, N.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Kopeliansky, R.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Benitez, J.; Mallik, U.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Jiang, H.; Krumnack, N.; Pluth, D.; Prell, S.; Yu, J.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Soloshenko, A.; Yeletskikh, I.; Zhemchugov, A.; Zimine, I.] Joint Inst Nucl Res Dubna, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagai, R.; Nagano, K.; Nakamura, K.; Nozaki, M.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Cheatham, S.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Muenstermann, D.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Bachas, K.; Chiodini, G.; Gorini, E.; Longo, L.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Bachas, K.; Gorini, E.; Longo, L.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Armitage, L. J.; Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Panduro Vazquez, J. G.; Pastore, Fr.; Savage, G.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bell, A. S.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Leney, K. J. C.; Martyniuk, A. C.; McClymont, L. I.; Mcfayden, J. A.; Nurse, E.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] Univ Coll London, Dept Phys & Astron, London, ON, Canada. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Aloisio, A.; Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Groh, S.; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Pleskot, V.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schmitt, C.; Schmitz, S.; Schott, M.; Schuh, N.; Simon, M.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Webb, S.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Barnes, S. L.; Bielski, R.; Cox, B. E.; Da Via, C.; Dann, N. S.; Forcolin, G. T.; Forti, A.; Ponce, J. M. Iturbe; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Sanchez, F. J. Munoz; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.; Zhang, R.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.; Zhang, R.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Picazio, A.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Panduro Vazquez, J. G.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Nuti, F.; Rados, P.; Scutti, F.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Ungaro, F. C.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Geng, C.; Goldfarb, S.; Guan, L.; Guo, Y.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Martin, B.; Mondragon, M. C.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Manzoni, S.; Mazza, S. M.; Meroni, C.; Monzani, S.; Nole, D.; Perini, L.; Ragusa, F.; Ratti, M. G.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Via Celoria 16, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Manzoni, S.; Mazza, S. M.; Monzani, S.; Nole, D.; Perini, L.; Ragusa, F.; Ratti, M. G.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Belyaev, N. L.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ, MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Heinrich, J. J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, S.; Kroha, H.; La Rosa, A.; Macchiolo, A.; Maier, A. A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Kawade, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Mc Fadden, N. C.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Konig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Budker Inst Nucl Phys, SB RAS, Novosibirsk 630090, Russia. [Becot, C.; Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Che, S.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Looper, K. A.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Allen, B. W.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Radloff, P.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Abeloos, B.; Ayoub, M. K.; Bassalat, A.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Goudet, C. R.; Grivaz, J. -F.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Maiani, C.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, CNRS, IN2P3, Univ Paris Saclay,LAL, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, M. K.; Cameron, D.; Catmore, J. R.; Feigl, S.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Artoni, G.; Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Bortoletto, D.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Di Clemente, W. K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Machado Miguens, J.; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Naryshkin, I.; Ryabov, Y. F.; Schegelsky, V. A.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Natl Res Ctr, Kurchatov Inst, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Farina, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Oleiro Seabra, L. F.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Sopczak, A.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] NRC KI, State Res Ctr, Inst High Energy Phys, Moscow, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; Corradi, M.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Di Donato, C.; Falciano, S.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Di Domenico, A.; Di Donato, C.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Denysiuk, D.; Etienvre, A. I.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Jeanneau, F.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Le Quilleuc, E. P.; Lesage, A. A. J.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Peyaud, A.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, Commiss Energie Atom & Energies Alternatives, DSM IRFU, F-91191 Gif Sur Yvette, France. [AbouZeid, O. S.; Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Li, Y.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Su, D.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Kar, D.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Silverstein, S. B.; Sjoelin, J.; Strandberg, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.; Santurio, E. Valdes; Wallangen, V.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.; Santurio, E. Valdes; Wallangen, V.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Song, H. Y.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.; Zhang, G.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Di Mattia, A.; Gozani, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Duarte-Campderros, J.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Pettersson, N. 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[Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellen Open Univ, Patras, Greece. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] State Univ, Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Pinamonti, M.] SISSA, Int Sch Adv Studies, I-34014 Trieste, Italy. Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Shiyakova, M.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy, Sofia, Bulgaria. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Vest, A.] Flensburg Univ Appl Sci, Flensburg, Germany. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France.; Aad, G (reprint author), CNRS, IN2P3, Marseille, France. EM atlas.publications@cern.ch RI Zhukov, Konstantin/M-6027-2015; SULIN, VLADIMIR/N-2793-2015; Warburton, Andreas/N-8028-2013; Snesarev, Andrey/H-5090-2013; Brooks, William/C-8636-2013; Nechaeva, Polina/N-1148-2015; Mashinistov, Ruslan/M-8356-2015; Vykydal, Zdenek/H-6426-2016; Fedin, Oleg/H-6753-2016; Guo, Jun/O-5202-2015; Gorelov, Igor/J-9010-2015; Ventura, Andrea/A-9544-2015; Chekulaev, Sergey/O-1145-2015; Carvalho, Joao/M-4060-2013; Leyton, Michael/G-2214-2016; White, Ryan/E-2979-2015; Livan, Michele/D-7531-2012; Jones, Roger/H-5578-2011; Tikhomirov, Vladimir/M-6194-2015; Doyle, Anthony/C-5889-2009; Boyko, Igor/J-3659-2013; Mitsou, Vasiliki/D-1967-2009; Vranjes Milosavljevic, Marija/F-9847-2016; Gladilin, Leonid/B-5226-2011; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Di Domenico, Antonio/G-6301-2011; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Kantserov, Vadim/M-9761-2015; La Rosa Navarro, Jose Luis/K-4221-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Smirnova, Oxana/A-4401-2013; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Conde Muino, Patricia/F-7696-2011; Stabile, Alberto/L-3419-2016; Villa, Mauro/C-9883-2009; Coccaro, Andrea/P-5261-2016; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Garcia, Jose /H-6339-2015; OI SULIN, VLADIMIR/0000-0003-3943-2495; Warburton, Andreas/0000-0002-2298-7315; Brooks, William/0000-0001-6161-3570; Mashinistov, Ruslan/0000-0001-7925-4676; Vykydal, Zdenek/0000-0003-2329-0672; Guo, Jun/0000-0001-8125-9433; Gorelov, Igor/0000-0001-5570-0133; Ventura, Andrea/0000-0002-3368-3413; Carvalho, Joao/0000-0002-3015-7821; Leyton, Michael/0000-0002-0727-8107; White, Ryan/0000-0003-3589-5900; Livan, Michele/0000-0002-5877-0062; Jones, Roger/0000-0002-6427-3513; Tikhomirov, Vladimir/0000-0002-9634-0581; Doyle, Anthony/0000-0001-6322-6195; Boyko, Igor/0000-0002-3355-4662; Mitsou, Vasiliki/0000-0002-1533-8886; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Gladilin, Leonid/0000-0001-9422-8636; Kukla, Romain/0000-0002-1140-2465; Goncalo, Ricardo/0000-0002-3826-3442; Di Domenico, Antonio/0000-0001-8078-2759; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Smirnova, Oxana/0000-0003-2517-531X; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Conde Muino, Patricia/0000-0002-9187-7478; Stabile, Alberto/0000-0002-6868-8329; Villa, Mauro/0000-0002-9181-8048; Coccaro, Andrea/0000-0003-2368-4559; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Prokofiev, Kirill/0000-0002-2177-6401 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; IN2P3-CNRS, France; CEADSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF; Canada Council; CANARIE; CRC; Compute Canada; FQRNT; Ontario Innovation Trust, Canada; EPLANET; ERC; FP7, Horizon 2020; Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex; Idex; ANR; Region Auvergne; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos programme - EU-ESF; Thales programme - EU-ESF; Aristeia programme - EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; IN2P3-CNRS, CEADSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. NR 56 TC 3 Z9 3 U1 16 U2 54 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAR 8 PY 2016 IS 3 AR 041 DI 10.1007/JHEP03(2016)041 PG 37 WC Physics, Particles & Fields SC Physics GA DG7VI UT WOS:000372291400001 ER PT J AU Zhang, L Wang, ZY Mehio, ND Jin, XB Dai, S AF Zhang, Lin Wang, Zhiyong Mehio, Nada Jin, Xianbo Dai, Sheng TI Thickness- and Particle-Size-Dependent Electrochemical Reduction of Carbon Dioxide on Thin-Layer Porous Silver Electrodes SO CHEMSUSCHEM LA English DT Article DE carbon dioxide chemistry; electrochemistry; heterogeneous catalysis; porous materials; silver ID ELECTROCATALYTIC REDUCTION; SELECTIVE CONVERSION; CO2 REDUCTION; ENHANCED ACTIVITY; AU NANOPARTICLES; IONIC LIQUID; AQUEOUS CO2; IN-SITU; ELECTROREDUCTION; EFFICIENCY AB The electrochemical reduction of CO2 can not only convert it back into fuels, but is also an efficient manner to store forms of renewable energy. Catalysis with silver is a possible technology for CO2 reduction. We report that in the case of monolithic porous silver, the film thickness and primary particle size of the silver particles, which can be controlled by electrochemical growth/reduction of AgCl film on silver substrate, have a strong influence on the electrocatalytic activity towards CO2 reduction. A 6m thick silver film with particle sizes of 30-50nm delivers a CO formation current of 10.5mAcm(-2) and a mass activity of 4.38Ag(Ag)(-1) at an overpotential of 0.39V, comparable to levels achieved with state-of-the-art gold catalysts. C1 [Zhang, Lin; Wang, Zhiyong; Jin, Xianbo] Wuhan Univ, Coll Chem & Mol Sci, Hubei Key Lab Electrochem Power Sources, Wuhan 430072, Peoples R China. [Mehio, Nada; Jin, Xianbo; Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Jin, XB (reprint author), Wuhan Univ, Coll Chem & Mol Sci, Hubei Key Lab Electrochem Power Sources, Wuhan 430072, Peoples R China.; Jin, XB; Dai, S (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA.; Dai, S (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM xbjin@whu.edu.cn; dais@ornl.gov RI Dai, Sheng/K-8411-2015; OI Dai, Sheng/0000-0002-8046-3931; Jin, Xianbo/0000-0002-3095-8979 FU NSFCs [21173161]; MOE Program [NCET-11-0397]; Fundamental Research Funds for the Central Universities of Wuhan University; Fluid Interface Reactions, Structures, and Transport (FIRST) Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX This work is supported by NSFCs (21173161), the MOE Program (NCET-11-0397), and the Fundamental Research Funds for the Central Universities of Wuhan University. N.M. and S.D. were supported by Fluid Interface Reactions, Structures, and Transport (FIRST) Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. NR 35 TC 1 Z9 1 U1 23 U2 112 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1864-5631 EI 1864-564X J9 CHEMSUSCHEM JI ChemSusChem PD MAR 8 PY 2016 VL 9 IS 5 BP 428 EP 432 DI 10.1002/cssc.201501637 PG 5 WC Chemistry, Multidisciplinary; GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY SC Chemistry; Science & Technology - Other Topics GA DG6JX UT WOS:000372191600002 PM 26822587 ER PT J AU Romero-Severson, EO Bulla, I Leitner, T AF Romero-Severson, Ethan O. Bulla, Ingo Leitner, Thomas TI Phylogenetically resolving epidemiologic linkage SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE HIV-1; transmission; paraphyly; coalescent; phylogeny ID HUMAN-IMMUNODEFICIENCY-VIRUS; PRIMARY HIV-1 INFECTION; TRANSMISSION EVENTS; SEXUAL TRANSMISSION; MOLECULAR EVIDENCE; TYPE-1 INFECTION; FLORIDA DENTIST; IN-VIVO; EVOLUTION; DYNAMICS AB Although the use of phylogenetic trees in epidemiological investigations has become commonplace, their epidemiological interpretation has not been systematically evaluated. Here, we use an HIV-1 within-host coalescent model to probabilistically evaluate transmission histories of two epidemiologically linked hosts. Previous critique of phylogenetic reconstruction has claimed that direction of transmission is difficult to infer, and that the existence of unsampled intermediary links or common sources can never be excluded. The phylogenetic relationship between the HIV populations of epidemiologically linked hosts can be classified into six types of trees, based on cladistic relationships and whether the reconstruction is consistent with the true transmission history or not. We show that the direction of transmission and whether unsampled intermediary links or common sources existed make very different predictions about expected phylogenetic relationships: (i) Direction of transmission can often be established when paraphyly exists, (ii) intermediary links can be excluded when multiple lineages were transmitted, and (iii) when the sampled individuals' HIV populations both are monophyletic a common source was likely the origin. Inconsistent results, suggesting the wrong transmission direction, were generally rare. In addition, the expected tree topology also depends on the number of transmitted lineages, the sample size, the time of the sample relative to transmission, and how fast the diversity increases after infection. Typically, 20 or more sequences per subject give robust results. We confirm our theoretical evaluations with analyses of real transmission histories and discuss how our findings should aid in interpreting phylogenetic results. C1 [Romero-Severson, Ethan O.; Bulla, Ingo; Leitner, Thomas] Los Alamos Natl Lab, Theoret Biol & Biophys Grp, POB 1663, Los Alamos, NM 87545 USA. RP Leitner, T (reprint author), Los Alamos Natl Lab, Theoret Biol & Biophys Grp, POB 1663, Los Alamos, NM 87545 USA. EM tkl@lanl.gov FU National Institute of Allergy and Infectious Diseases/National Institutes of Health [R01AI087520]; Deutsche Forschungsgemeinschaft Fellowship [BU 2685/4-1] FX We thank the editor and the reviewers for insightful and constructive comments on an earlier version of this paper. Research reported in this publication was supported by National Institute of Allergy and Infectious Diseases/National Institutes of Health under Grant R01AI087520 and Deutsche Forschungsgemeinschaft Fellowship BU 2685/4-1. NR 55 TC 6 Z9 6 U1 2 U2 3 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAR 8 PY 2016 VL 113 IS 10 BP 2690 EP 2695 DI 10.1073/pnas.1522930113 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DG4AW UT WOS:000372013300042 PM 26903617 ER PT J AU Walker, MA Madduri, R Rodriguez, A Greenstein, JL Winslow, RL AF Walker, Mark A. Madduri, Ravi Rodriguez, Alex Greenstein, Joseph L. Winslow, Raimond L. TI Models and Simulations as a Service: Exploring the Use of Galaxy for Delivering Computational Models SO BIOPHYSICAL JOURNAL LA English DT Article ID CARDIAC MYOCYTES; CALSEQUESTRIN; SOFTWARE; CELLML AB We describe the ways in which Galaxy, a web-based reproducible research platform, can be used for web-based sharing of complex computational models. Galaxy allows users to seamlessly customize and run simulations on cloud computing resources, a concept we refer to as Models and Simulations as a Service (MaSS). To illustrate this application of Galaxy, we have developed a tool suite for simulating a high spatial-resolution model of the cardiac Ca2+ spark that requires supercomputing resources for execution. We also present tools for simulating models encoded in the SBML and CeIIML model description languages, thus demonstrating how Galaxy's reproducible research features can be leveraged by existing technologies. Finally, we demonstrate how the Galaxy workflow editor can be used to compose integrative models from constituent submodules. This work represents an important novel approach, to our knowledge, to making computational simulations more accessible to the broader scientific community. C1 [Walker, Mark A.; Greenstein, Joseph L.; Winslow, Raimond L.] Johns Hopkins Univ, Dept Biomed Engn, Inst Computat Med, Baltimore, MD USA. [Madduri, Ravi; Rodriguez, Alex] Univ Chicago, Argonne Natl Lab, Computat Inst, Chicago, IL 60637 USA. RP Winslow, RL (reprint author), Johns Hopkins Univ, Dept Biomed Engn, Inst Computat Med, Baltimore, MD USA. EM rwinslow@jhu.edu OI Walker, Mark/0000-0001-6613-4560 FU [R24HL085343] FX This work was supported by R24HL085343. NR 25 TC 1 Z9 1 U1 2 U2 4 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD MAR 8 PY 2016 VL 110 IS 5 BP 1038 EP 1043 DI 10.1016/j.bpj.2015.12.041 PG 6 WC Biophysics SC Biophysics GA DG1TI UT WOS:000371850000012 PM 26958881 ER PT J AU Kim, C Pilania, G Ramprasad, R AF Kim, Chiho Pilania, Ghanshyam Ramprasad, Ramamurthy TI From Organized High-Throughput Data to Phenomenological Theory using Machine Learning: The Example of Dielectric Breakdown SO CHEMISTRY OF MATERIALS LA English DT Article ID AUGMENTED-WAVE METHOD; CRYSTAL-STRUCTURE; ELECTRON-GAS; ENERGY; SEMICONDUCTORS; ACCURATE AB Understanding the behavior (and failure) of F.. dielectric insulators experiencing extreme electric fields is critical to the operation of present and emerging electrical and electronic devices. Despite its importance, the development of a predictive theory of dielectric breakdown has remained a challenge, owing to the complex multiscale nature of this process. Here, we focus on the intrinsic dielectric breakdown field of insulators the theoretical limit of. breakdown determined purely by the chemistry of the material, i.e., the elements the material is composed of, the atomic-level structure, and the bonding. Starting from a benchmark data set (generated from laborious first-principles computations) of the intrinsic dielectric breakdown field of a variety of model insulators, simple predictive phenomenological models of dielectric breakdown are distilled using advanced statistical or machine learning schemes, revealing key correlations and analytical relationships between the breakdown field and easily accessible material properties. The models are shown to be general, and can hence guide the screening and systematic identification of high electric field tolerant materials. C1 [Kim, Chiho; Ramprasad, Ramamurthy] Univ Connecticut, Dept Mat Sci & Engn, 97 North Eagleville Rd, Storrs, CT 06269 USA. [Kim, Chiho; Ramprasad, Ramamurthy] Univ Connecticut, Inst Mat Sci, 97 North Eagleville Rd, Storrs, CT 06269 USA. [Pilania, Ghanshyam] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. RP Ramprasad, R (reprint author), Univ Connecticut, Dept Mat Sci & Engn, 97 North Eagleville Rd, Storrs, CT 06269 USA.; Ramprasad, R (reprint author), Univ Connecticut, Inst Mat Sci, 97 North Eagleville Rd, Storrs, CT 06269 USA. EM rampi@uconn.edu OI Pilania, Ghanshyam/0000-0003-4460-1572 FU Office of Naval Research [N00014-10-1-0944, N00014-15-1-2665]; Multidisciplinary University Research Initiative (MURI) grant; U.S. Department of Energy through the LANL/LDRD [20140679PRD3] FX This paper is based on work supported by the Office of Naval Research through grants N00014-10-1-0944 and N00014-15-1-2665, the former being a Multidisciplinary University Research Initiative (MURI) grant. Computational support was provided by the Extreme Science and Engineering Discovery Environment (XSEDE) and the National Energy Research Scientific Computing Center (NERSC). G.P. acknowledges the support of the U.S. Department of Energy through the LANL/LDRD grant (20140679PRD3) as a Director's postdoctoral fellowship. Luca Ghiringhelli, Jan Vybiral and Matthias Scheffler are acknowledged for detailed guidance on using the LASSO-LSF method, and a critical reading of the manuscript. Ying Sun and Clive Bealing are acknowledged for a prior post-Quantum ESPRESSO code development effort to compute the intrinsic dielectric breakdown field. Discussions with Kenny Lipkowitz and Paul Armistead, and a critical reading of the manuscript by Erik Nykwest, Venkatesh Botu, and Huan Tran are also acknowledged. NR 45 TC 7 Z9 7 U1 8 U2 27 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAR 8 PY 2016 VL 28 IS 5 BP 1304 EP 1311 DI 10.1021/acs.chemmater.5b04109 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DG1UC UT WOS:000371852000009 ER PT J AU Arges, CG Kambe, Y Suh, HS Ocola, LE Nealey, PF AF Arges, Christopher G. Kambe, Yu Suh, Hyo Seon Ocola, Leonidas E. Nealey, Paul F. TI Perpendicularly Aligned, Anion Conducting Nanochannels in Block Copolymer Electrolyte Films SO CHEMISTRY OF MATERIALS LA English DT Article ID EXCHANGE MEMBRANES; MICRO-SUPERCAPACITORS; SCALABLE FABRICATION; POLYMER ELECTROLYTES; IONIC-CONDUCTIVITY; ENERGY-STORAGE; TRANSPORT; NAFION; LITHOGRAPHY; DEVICES AB Connecting structure and morphology to bulk transport properties, such as ionic conductivity, in nanostructured polymer electrolyte materials is a difficult proposition because of the challenge to precisely and accurately control order and the orientation of the ionic domains in such polymeric films. In this work, poly(styrene-block-2-vinylpyridine) (PSbP2VP) block copolymers were assembled perpendicularly to a substrate surface over large areas through chemical surface modification at the substrate and utilizing a versatile solvent vapor annealing (SVA) technique. After block copolymer assembly, a novel chemical vapor infiltration reaction (CVIR) technique selectively converted the 2-vinylpyridine block to 2-vinyl n-methylpyridinium (NMP+ X-) groups, which are anion charge carriers. The prepared block copolymer electrolytes maintained their orientation and ordered nanostructure upon the selective introduction of ion moieties into the P2VP block and post ion-exchange to other counterion forms (X- = chloride, hydroxide, etc.). The prepared block copolymer electrolyte films demonstrated high chloride ion conductivities, 45 mS cm(-1) at 20 degrees C in deionized water, the highest chloride ion conductivity for anion conducting polymer electrolyte films. Additionally, straight-line lamellae of block copolymer electrolytes were realized using chemoepitaxy and density multiplication. The devised scheme allowed for precise and accurate control of orientation of ionic domains in nanostructured polymer electrolyte films and enables a platform for future studies that examines the relationship between polymer electrolyte structure and ion transport. C1 [Arges, Christopher G.; Kambe, Yu; Suh, Hyo Seon; Nealey, Paul F.] Univ Chicago, Inst Mol Engn, 5735 South Ellis Ave, Chicago, IL 60637 USA. [Arges, Christopher G.; Kambe, Yu; Suh, Hyo Seon; Nealey, Paul F.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Lemont, IL 60439 USA. [Ocola, Leonidas E.] Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Lemont, IL 60439 USA. [Ocola, Leonidas E.] Univ Chicago, Chicago Mat Res Ctr, MRSEC, 929 East 57th St, Chicago, IL 60637 USA. RP Arges, CG (reprint author), Univ Chicago, Inst Mol Engn, 5735 South Ellis Ave, Chicago, IL 60637 USA.; Arges, CG (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Lemont, IL 60439 USA. RI Arges, Christopher/G-9165-2014; OI Arges, Christopher/0000-0003-1703-8323; Ocola, Leonidas/0000-0003-4990-1064 FU U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; DOE Office of Science [DE-AC02-06CH11357] FX We gratefully acknowledge funding by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. We also wish to acknowledge the following: (i) use of the Center for Nanoscale Materials (user proposal 37900), an Office of Science user facility, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357, (ii) resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357, (iii) the shared instrumentation facilities at the University of Chicago for use of the Asylum MFP3D AFM and Carl Zeiss Merlin SEM, and (iv) the Research Resources Center at the University of Illinois at Chicago for access to the Kratos Axis 165 for XPS experiments. NR 48 TC 4 Z9 4 U1 16 U2 68 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAR 8 PY 2016 VL 28 IS 5 BP 1377 EP 1389 DI 10.1021/acs.chemmater.5b04452 PG 13 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DG1UC UT WOS:000371852000019 ER PT J AU Bo, SH Li, X Toumar, AJ Ceder, G AF Bo, Shou-Hang Li, Xin Toumar, Alexandra J. Ceder, Gerbrand TI Layered-to-Rock-Salt Transformation in Desodiated NaxCrO2 (x 0.4) SO CHEMISTRY OF MATERIALS LA English DT Article ID SODIUM-ION BATTERIES; HIGH-ENERGY; 1ST-PRINCIPLES CALCULATIONS; ELECTROCHEMICAL PROPERTIES; STRUCTURAL EVOLUTION; ELECTRONIC-STRUCTURE; CATHODE MATERIAL; PHASE-STABILITY; COBALT OXIDES; INTERCALATION AB O-3 layered sodium transition metal oxides (i.e., NaMO2, M = Ti, V, Cr, Mn, Fe, Co, Ni) are a promising class of cathode materials for Na-ion battery applications. These materials, however, all suffer from severe capacity decay when the extraction of Na exceeds certain capacity limits. Understanding the causes of this capacity decay is critical to unlocking the potential of these materials for battery applications. In this work, we investigate the structural origins of capacity decay for one of the compounds in this class, NaCrO2. The (de)sodiation processes of NaCrO2 were studied both in situ and ex situ through X-ray and electron diffraction measurements. We demonstrate that NaxCrO2 (0 < x < 1) remains in the layered structural framework without Cr migration up to a composition of Na0.4CrO2. Further removal of Na beyond this composition triggers a layered-to-rock-salt transformation, which converts P'3-Na0.4CrO2 into the rock-salt CrO2 phase. This structural transformation proceeds via the formation of an intermediate O3 Na delta CrO2 phase that contains Cr in both Na and Cr slabs and shares very similar lattice dimensions with those of rock-salt CrO2. It is intriguing to note that intercalation of alkaline ions (i.e., Na and Li) into the rock-salt CrO2 and O3 Na delta CrO2 structures is actually possible, albeit in a limited amount (similar to 0.2 per formula unit). When these results were analyzed under the context of electrochemistry data, it was apparent that preventing the layered-to-rock-salt transformation is crucial to improve the cyclability of NaCrO2. Possible strategies for mitigating this detrimental phase transition are proposed. C1 [Bo, Shou-Hang; Toumar, Alexandra J.; Ceder, Gerbrand] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. [Bo, Shou-Hang; Ceder, Gerbrand] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Li, Xin] Harvard Univ, John A Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USA. [Ceder, Gerbrand] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Ceder, G (reprint author), MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA.; Ceder, G (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Ceder, G (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. EM gceder@mit.edu FU Samsung Advanced Institute of Technology; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by the Samsung Advanced Institute of Technology. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. We thank Jinhyuk Lee, Aziz Abdellahi, Dr. Dong-Hwa Seo, and Dr. Alexander Urban for helpful discussions. NR 60 TC 9 Z9 9 U1 26 U2 82 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAR 8 PY 2016 VL 28 IS 5 BP 1419 EP 1429 DI 10.1021/acs.chemmater.5b04626 PG 11 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DG1UC UT WOS:000371852000023 ER PT J AU Didier, C Guignard, M Suchomel, MR Carlier, D Darriet, J Delmas, C AF Didier, Christophe Guignard, Marie Suchomel, Matthew R. Carlier, Dany Darriet, Jacques Delmas, Claude TI Thermally and Electrochemically Driven Topotactical Transformations in Sodium Layered Oxides NaxVO2 SO CHEMISTRY OF MATERIALS LA English DT Article ID NA-ION BATTERIES; SYSTEM; INTERCALATION; ELECTRODE; NAXCOO2 AB Phase diagrams and structural transformations in the complex NaxVO2 system have been studied using electrochemical (de)intercalation and in situ and operando high resolution synchrotron powder diffraction. Starting from O'3-Na1/2VO2 obtained by sodium electrochemical deintercalation of O'3-NaVO2, the structural details of irreversible and reversible thermally driven transformations to P'3 and P3 type structures are presented. Subsequently, these P'3-NaxVO(2) phases provide a platform for operando studies exploring the NaxVO2 phase diagram as a function of sodium electrochemical (de) intercalation. In this system, three single phase domains have been found: a line phase P'3-Na1/2VO2, one solid solution for 0.53 <= x <= 0.55 characterized by an incommensurate modulated structure, and a second solid solution for 0.63 <= x <= 0.65 with a defective structure resulting from a random stack of O'3 and P'3 layers. With further sodium intercalation (x > 0.65), the structure irreversibly transforms to the starting parent phase O3-NaVO2. This work reveals new details about the diverse structural polymorphs found in sodium layered oxides used as electrode battery materials and the transitional pathways between them as a function of temperature and composition. C1 [Didier, Christophe; Guignard, Marie; Carlier, Dany; Darriet, Jacques; Delmas, Claude] CNRS, 87 Ave Docteur A Schweitzer, F-33608 Pessac, France. [Didier, Christophe; Guignard, Marie; Carlier, Dany; Darriet, Jacques; Delmas, Claude] Univ Bordeaux, ICMCB, 87 Ave Docteur A Schweitzer, F-33608 Pessac, France. [Suchomel, Matthew R.] Argonne Natl Lab, Adv Photon Source, Lemont, IL 60439 USA. [Suchomel, Matthew R.] CNRS, ICMCB, 87 Ave Docteur A Schweitzer, F-33608 Pessac, France. RP Guignard, M (reprint author), CNRS, 87 Ave Docteur A Schweitzer, F-33608 Pessac, France.; Guignard, M (reprint author), Univ Bordeaux, ICMCB, 87 Ave Docteur A Schweitzer, F-33608 Pessac, France. EM marie.guignard@icmcb.cnrs.fr RI CARLIER, Dany/K-2271-2015 OI CARLIER, Dany/0000-0002-5086-4363 FU CNRS; Region Aquitaine FX Financial support was provided by the CNRS and the Region Aquitaine. NR 35 TC 3 Z9 3 U1 7 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAR 8 PY 2016 VL 28 IS 5 BP 1462 EP 1471 DI 10.1021/acs.chemmater.5b04882 PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DG1UC UT WOS:000371852000028 ER PT J AU He, G Huq, A Kan, WH Manthiram, A AF He, Guang Huq, Ashfia Kan, Wang Hay Manthiram, Arumugam TI beta-NaVOPO4 Obtained by a Low-Temperature Synthesis Process: A New 3.3 V Cathode for Sodium-Ion Batteries SO CHEMISTRY OF MATERIALS LA English DT Article ID POSITIVE-ELECTRODE MATERIALS; CARBON-COATED NA3V2(PO4)(3); CRYSTAL-STRUCTURE; LITHIUM BATTERIES; ELECTROCHEMICAL PERFORMANCE; SOLVOTHERMAL SYNTHESIS; INSERTION; EPSILON-VOPO4; LIVOPO4; STORAGE AB Vanadyl phosphates (VOPO4) represent a class of attractive cathodes in lithium-ion batteries. However, the exploration of this type of materials in sodium-ion batteries is rare. Here, we report for the first time the synthesis of orthorhombic beta-NaVOPO4 by first chemically extracting lithium from beta-LiVOPO4 and then inserting sodium into the obtained beta-VOPO4 by a microwave-assisted solvothermal process with NaI, which serves both as a reducing agent and sodium source. Intermediate NaxVOPO4 compositions with x = 0.3, 0.5, and 0.8 have also been obtained by controlling the amount of NaI in the reaction mixture. Joint Rietveld refinement of synchrotron X-ray diffraction (XRD) and neutron diffraction confirms that the fully sodiated beta-NaVOPO4 is isostructural with the lithium counterpart beta-LiVOPO4. Bond valence sum maps suggest that sodium ions possibly diffuse along the [010] direction in the lattice, similar to the ionic conduction pathway in beta-LiVOPO4. Although the initial discharge capacity is low due to the protons in the structure, it steadily increases with cycling with a long plateau at 3.3 V. Ex situ XRD data of cycled beta-VOPO4 and beta-NaVOPO4 electrodes confirm the reversible reaction in sodium cells involving the V4+/V5+ redox couple. C1 [He, Guang; Kan, Wang Hay; Manthiram, Arumugam] Univ Texas Austin, Mat Sci & Engn Program, Austin, TX 78712 USA. [Huq, Ashfia] Univ Texas Austin, Texas Mat Inst, Austin, TX 78712 USA. Oak Ridge Natl Lab, Neutron Scattering Sci Div, Oak Ridge, TN 37831 USA. RP Manthiram, A (reprint author), Univ Texas Austin, Mat Sci & Engn Program, Austin, TX 78712 USA. EM manth@austin.utexas.edu RI Huq, Ashfia/J-8772-2013; He, Guang/B-2967-2017 OI Huq, Ashfia/0000-0002-8445-9649; FU Office of Vehicle Technologies of the U.S. Department of Energy under the Battery Materials Research (BMR) Program [DE-AC02-05CH11231, 7000389]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, Subcontract No. 7000389 under the Battery Materials Research (BMR) Program. Neutron diffraction part of this research at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. We thank Craig A. Bridges for useful discussions on the structural refinements of NaxVOPO4 (x = 0.3, 0.5, and 0.8), and Professor Jianshi Zhou and Dr. Xiang Li for their assistance with collecting the magnetic data. NR 48 TC 3 Z9 3 U1 19 U2 93 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAR 8 PY 2016 VL 28 IS 5 BP 1503 EP 1512 DI 10.1021/acs.chemmater.5b04992 PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DG1UC UT WOS:000371852000033 ER PT J AU Maserati, L Meckler, SM Li, CY Helms, BA AF Maserati, Lorenzo Meckler, Stephen M. Li, Changyi Helms, Brett A. TI Minute-MOFs: Ultrafast Synthesis of M-2(dobpdc) Metal-Organic Frameworks from Divalent Metal Oxide Colloidal Nanocrystals SO CHEMISTRY OF MATERIALS LA English DT Article ID CARBON-DIOXIDE; ELECTRICAL-CONDUCTIVITY; THERMAL-DECOMPOSITION; COORDINATION POLYMERS; ROOM-TEMPERATURE; GROWTH-MECHANISM; CO2 CAPTURE; STORAGE; NANOPARTICLES; MONODISPERSE AB The material demands for metal organic frameworks (MOFs) for next-generation energy-efficient CO2 capture technologies necessitate advances in their expedient and scalable synthesis. Toward that end, the recently discovered expanded MOF-74, or M-2(dobpdc), where M = divalent metal cation and dobpdc = 4,4'-dioxido-3,3'-biphenyldicarboxylate, can now be prepared in minutes via a controlled dissolution crystallization route from divalent metal oxides as precursors. We show that the available surface area of the metal oxide plays a critical role in the precursor dissolution, which was found to be rate-limiting. Based on this understanding of the reaction trajectory, we, pushed the chemical transformation to its fringe kinetic limit by configuring the metal oxide precursors as ligand-free colloidal metal oxide nanocrystals, which allowed MOF formation in less than 1 min. MOFs prepared by this strategy were highly crystalline, with BET surface areas on par with conventional multihour syntheses from metal halide salts. This method was also applied successfully in the synthesis of M-2(dobdc) MOFs, highlighting its generality. Our work challenges the conventional-wisdom that plurality of steps in MOF formation is inherently time-intensive. C1 [Maserati, Lorenzo; Meckler, Stephen M.; Li, Changyi; Helms, Brett A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, One Cyclotron Rd, Berkeley, CA 94720 USA. [Meckler, Stephen M.] Univ Calif Berkeley, Dept Chem, One Cyclotron Rd, Berkeley, CA 94720 USA. [Li, Changyi] Univ Calif Berkeley, Dept Chem & Biomol Engn, One Cyclotron Rd, Berkeley, CA 94720 USA. RP Helms, BA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, One Cyclotron Rd, Berkeley, CA 94720 USA. EM bahelms@lbl.gov OI Maserati, Lorenzo/0000-0002-9938-8935 FU Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences [SC0001015]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy FX We thank W. Queen, D. Sun, D. Britt, J. R. Long, and T. McDonald for helpful discussions, T. E. Williams and M. V. Altoe for assistance with TEM. This work was supported by the Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award #SC0001015. All work was carried out as a User Project at the Molecular Foundry, which is supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. B.A.H. acknowledges support from the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under the same contract. NR 64 TC 3 Z9 3 U1 29 U2 81 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAR 8 PY 2016 VL 28 IS 5 BP 1581 EP 1588 DI 10.1021/acs.chemmater.6b00494 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DG1UC UT WOS:000371852000042 ER PT J AU Barkakaty, B Browning, KL Sumpter, B Uhrig, D Katpisova, I Harman, KW Ivanov, I Hensley, DK Messman, JM Kilbey, SM Lokitz, BS AF Barkakaty, Balaka Browning, Katie L. Sumpter, Bobby Uhrig, David Katpisova, Ivana Harman, Kevin W. Ivanov, Ilia Hensley, Dale K. Messman, Jamie M. Kilbey, S. Michael, II Lokitz, Bradley S. TI Amidine-Functionalized Poly(2-vinyl-4,4-dimethylazlactone) for Selective and Efficient CO2 Fixing SO MACROMOLECULES LA English DT Article ID CARBON-DIOXIDE CAPTURE; POST-POLYMERIZATION MODIFICATION; METAL-ORGANIC FRAMEWORKS; FIXATION-RELEASE SYSTEM; CO2-RESPONSIVE POLYMERS; RADICAL POLYMERIZATION; NANOGEL PARTICLES; SURFACE SCAFFOLDS; ROOM-TEMPERATURE; HIGH-CAPACITY AB Development of novel polymeric materials capable of efficient CO2 capture and separation under ambient conditions is crucial for cost-effective and practical industrial applications. Here we report the facile synthesis of a new CO2-responsive polymer through postpolymerization modification of poly(2-vinyl-4,4-dimethylazlactone) (PVDMA). The reactive pendant azlactone groups of PVDMA are easily modified with 4-(N-methyltetrahydropyrimidine)benzyl alcohol (PBA) without any byproduct formation. FUR and TGA experiments show the new PBA-functionalized polymer powder can reversibly capture CO2 at room temperature and under atmospheric pressure. CO2 capture was selective, showing a high fixing efficiency even with a mixed gas system (20% CO2, 80% N-2) similar to flue gas. CO2 release occurred at room temperature, and release profiles were investigated as a function of temperature. Density functional theory (DFT) calculations coupled with modeling and. simulation reveal the presence of two CO2 binding sites in the PBA-functionalized polymer resulting in a two-step CO2 release at room temperature. The ease of material preparation, high fixing efficiency, and robust release characteristics suggest that postpolymerization modification may be a useful route to designing new materials for CO2 capture. C1 [Barkakaty, Balaka; Lokitz, Bradley S.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, One Bethel Valley Rd, Oak Ridge, TN 37831 USA. [Browning, Katie L.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Kilbey, S. Michael, II] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Katpisova, Ivana] Comenius Univ, Fac Math Phys & Informat, Dept Nucl Phys & Biophys, Bratislava 84248, Slovakia. RP Barkakaty, B; Lokitz, BS (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, One Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM lokitzbs@ornl.gov; barkakatyb@ornl.gov RI Sumpter, Bobby/C-9459-2013; ivanov, ilia/D-3402-2015 OI Sumpter, Bobby/0000-0001-6341-0355; ivanov, ilia/0000-0002-6726-2502 FU European Commission [PIRSES-GA-2010-269182]; CNMS [CNMS2014-033]; Center for Understanding and Control of Acid Gas-Induced Evolution of Materials for Energy (UNCAGE-ME), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences; National Science Foundation [1133320] FX This research was conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. We also thank European Commission under 7 FP (Project No. PIRSES-GA-2010-269182) and CNMS user project (Proposal No. CNMS2014-033) for sponsoring Ivana Karpisova from Comenius University, Slovakia, to contribute to this work. B.G.S. acknowledges partial support from the Center for Understanding and Control of Acid Gas-Induced Evolution of Materials for Energy (UNCAGE-ME), an Energy Frontier Research Center funded by U.S. Department of Energy, Office of Science, Basic Energy Sciences. S.M.K. acknowledges support from the National Science Foundation (Award # 1133320). NR 48 TC 2 Z9 2 U1 18 U2 58 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD MAR 8 PY 2016 VL 49 IS 5 BP 1523 EP 1531 DI 10.1021/acs.macromol.5b02483 PG 9 WC Polymer Science SC Polymer Science GA DG1TT UT WOS:000371851100003 ER PT J AU Mauck, SC Wang, S Ding, WY Rohde, BJ Fortune, CK Yang, GZ Ahn, SK Robertson, ML AF Mauck, Sheli C. Wang, Shu Ding, Wenyue Rohde, Brian J. Fortune, C. Karen Yang, Guozhen Ahn, Suk-Kyun Robertson, Megan L. TI Biorenewable Tough Blends of Polylactide and Acrylated Epoxidized Soybean Oil Compatibilized by a Polylactide Star Polymer SO MACROMOLECULES LA English DT Article ID PLASTICIZED POLY(LACTIC ACID); INDUCED PHASE-SEPARATION; CASTOR-OIL; THERMOSETTING POLYMERS; MORPHOLOGICAL PROPERTIES; RHEOLOGICAL PROPERTIES; MECHANICAL-PROPERTIES; STYRENE REPLACEMENTS; RUBBER BLENDS; PLANT OIL AB Polylactide (PLA), a commercially available thermoplastic derived from plant sugars, finds applications in consumer products, disposable packaging, and textiles, among others. The widespread application of this material is limited by its brittleness, as evidenced by low tensile elongation at break, impact strength, and fracture toughness. Herein, a multifunctional vegetable oil, acrylated epoxidized soybean oil (AESO), was investigated as a biodegradable, renewable additive to improve the toughness of PLA. AESO was found to be a highly reactive oil, providing a dispersed phase with tunable properties in which the acrylate groups underwent cross-linking at the elevated temperatures required for processing the blends. Additionally, the presence of hydroxyl groups on AESO provided two routes for compatibilization of PLA/AESO blends: (1) reactive compatibilization through the transesterification of AESO and PLA and (2) synthesis of a PLA star polymer with an AESO core. The morphological, thermal, and mechanical behaviors of PLA/oil blends were investigated, in which the dispersed oil phase consisted of AESO, soybean oil (SYBO), or a 50/50 mixture of AESO/SYBO. The oil additives were found to toughen the PLA matrix, with significant enhancements in the elongation at break and tensile toughness values, while maintaining the glass transition temperature of neat PLA. In particular, the blend containing PLA, AESO, SYBO, and the PLA star polymer was found to exhibit a uniform oil droplet size distribution with small average droplet size and interparticle distance, resulting in the greatest enhancements of PLA tensile properties with no observable plasticization. C1 [Mauck, Sheli C.; Wang, Shu; Ding, Wenyue; Rohde, Brian J.; Fortune, C. Karen; Yang, Guozhen; Robertson, Megan L.] Univ Houston, Dept Chem & Biomol Engn, Houston, TX 77204 USA. [Ahn, Suk-Kyun] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Ahn, Suk-Kyun] Pusan Natl Univ, Dept Polymer Sci & Engn, Pusan 609735, South Korea. RP Robertson, ML (reprint author), Univ Houston, Dept Chem & Biomol Engn, Houston, TX 77204 USA. EM mlrobertson@uh.edu RI Yang, Guozhen/R-1545-2016 OI Yang, Guozhen/0000-0002-6145-6242 FU National Science Foundation [DMR-1351788, CMMI-1334838, NSF-EEC 1130006]; Norman Hackerman Advanced Research Program of the Texas Higher Education Coordinating Board [003652-0022-2013]; Research Experiences for Teachers program through the Engineering and Computer Science Site at the University of Houston: Innovations in Nanotechnology FX We thank Jeffrey D. Rimer and Jihae Chung for access to and training on the optical microscope and Haleh Ardebili and Mejdi Kammoun for access to and training on the thermogravimetric analysis instrument. We thank John C. Wolfe, Rebecca Kusko, and Apeksha Awale for access to and training on the scanning electron microscope in the University of Houston Cullen College of Engineering Microscopy Center, and Debora F. Rodrigues and Hang N. Nguyen for access to and training on the gold sputterer. We appreciate the assistance of Charles Anderson for access and training in the University of Houston Department of Chemistry Nuclear Magnetic Resonance Facility. We also appreciate the assistance of Kunlun Hong and Vivek Yadav for gel permeation chromatography data analysis. We thank Gila E. Stein, Leonard P. Trombetta, and Kim Mai Le for helpful discussions. A portion of this research was conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. This material is based upon work supported by the National Science Foundation under Grant DMR-1351788 and Grant CMMI-1334838. This work is funded in part by the Norman Hackerman Advanced Research Program of the Texas Higher Education Coordinating Board (003652-0022-2013). C.K.F. acknowledges support from the Research Experiences for Teachers program through the Engineering and Computer Science Site at the University of Houston: Innovations in Nanotechnology, sponsored by the National Science Foundation (NSF-EEC 1130006). NR 69 TC 6 Z9 6 U1 26 U2 67 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD MAR 8 PY 2016 VL 49 IS 5 BP 1605 EP 1615 DI 10.1021/acs.macromol.5b02613 PG 11 WC Polymer Science SC Polymer Science GA DG1TT UT WOS:000371851100012 ER PT J AU Chintapalli, M Le, TNP Venkatesan, NR Mackay, NG Rojas, AA Thelen, JL Chen, XC Devaux, D Balsara, NP AF Chintapalli, Mahati Le, Thao N. P. Venkatesan, Naveen R. Mackay, Nikolaus G. Rojas, Adriana A. Thelen, Jacob L. Chen, X. Chelsea Devaux, Didier Balsara, Nitash P. TI Structure and Ionic Conductivity of Polystyrene-block-poly(ethylene oxide) Electrolytes in the High Salt Concentration Limit SO MACROMOLECULES LA English DT Article ID BLOCK-COPOLYMER ELECTROLYTES; GRAIN-BOUNDARY MORPHOLOGY; RECHARGEABLE LITHIUM BATTERIES; MOLECULAR-WEIGHT; POLYMER ELECTROLYTE; DIBLOCK COPOLYMER; MICROPHASE SEPARATION; LAMELLAR PHASE; THIN-FILMS; TRANSPORT AB We explore the relationship between the morphology and ionic conductivity of block copolymer electrolytes over a wide range of salt concentrations for the system polystyrene-block-poly(ethylene oxide) (PS-b-PEO, SEO) mixed with lithium bis(trifluoromethanesulfonyl)imide salt (LiTFSI). Two SEO polymers were studied, SEO(16-16) and SEO(4.9-5.5), over the salt concentration range r = 0.03-0.55. The numbers x and y in SEO(x-y) are the molecular weights of the blocks in kg mol(-1), and the r value is the molar ratio of salt to ethylene oxide moieties. Small angle X-ray scattering was used to characterize morphology and grain size at 120 degrees C, differential scanning calorimetry was used to study the crystallinity and the glass transition temperature of the PEO-rich microphase, and ac impedance spectroscopy was used to measure ionic conductivity as a function of temperature. The most surprising observation of our study is that ionic conductivity in the concentration regime 0.11 <= r <= 0.21 increases in SEO electrolytes but decreases in PEO electrolytes. The maximum in ionic conductivity with salt concentration occurs at about twice the salt concentration in SEO (r = 0.21) as in PEO (r = 0.11). We propose that these observations are due to the effect of salt concentration on the grain structure in SEO electrolytes. C1 [Chintapalli, Mahati; Venkatesan, Naveen R.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Le, Thao N. P.; Venkatesan, Naveen R.; Mackay, Nikolaus G.; Rojas, Adriana A.; Thelen, Jacob L.; Balsara, Nitash P.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Rojas, Adriana A.; Thelen, Jacob L.; Devaux, Didier; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, JCESR, Berkeley, CA 94720 USA. [Devaux, Didier; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Chintapalli, Mahati; Thelen, Jacob L.; Chen, X. Chelsea; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Venkatesan, Naveen R.] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. RP Balsara, NP (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA.; Balsara, NP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, JCESR, Berkeley, CA 94720 USA.; Balsara, NP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.; Balsara, NP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM nbalsara@berkeley.edu FU National Science Foundation (Division of Materials Research) [1505444]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Soft Matter Electron Microscopy and Scattering program from the Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division of the U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [GE1106400] FX The primary support for this research is by the National Science Foundation (Division of Materials Research), Grant No. 1505444. Small-angle X-ray spectroscopy was performed at beamline 7.3.3 at the Advanced Light Source synchrotron in Berkeley, CA. Beamline 7.3.3 is supported by the Director of the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract DE-AC02-05CH11231. Electron microscopy was supported by the Soft Matter Electron Microscopy and Scattering program from the Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division of the U.S. Department of Energy, under Contract DE-AC02-05CH11231. M.C. was supported by the National Science Foundation Graduate Research Fellowship under Grant GE1106400. NR 82 TC 8 Z9 8 U1 29 U2 74 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD MAR 8 PY 2016 VL 49 IS 5 BP 1770 EP 1780 DI 10.1021/acs.macromol.5b02620 PG 11 WC Polymer Science SC Polymer Science GA DG1TT UT WOS:000371851100029 ER PT J AU Gupta, S Biehl, R Sill, C Allgaier, J Sharp, M Ohl, M Richter, D AF Gupta, Sudipta Biehl, Ralf Sill, Clemens Allgaier, Juergen Sharp, Melissa Ohl, Michael Richter, Dieter TI Protein Entrapment in Polymeric Mesh: Diffusion in Crowded Environment with Fast Process on Short Scales SO MACROMOLECULES LA English DT Article ID POLYSTYRENE LATEX SPHERES; NEUTRON SPIN-ECHO; POLY(ETHYLENE OXIDE); ANOMALOUS DIFFUSION; POLYETHYLENE-GLYCOL; AQUEOUS-SOLUTIONS; SELF-DIFFUSION; DYNAMICS; CRYSTALLIZATION; NANOPARTICLES AB The natural environment of proteins is a crowded environment as in cells, extracellular fluids, or during processing. Semidilute polymer solutions have been a source of rich structural and dynamical properties and mimic a crowded environment, but a proper understanding of protein-dynamics in the crowded environment is far lagging. Such a study not only realizes protein's natural environment in a crowded solution in the cell or during processing but also manifests the underlying protein polymer interaction. By dispersing model globular proteins like alpha-lactalbumin (La) and hemoglobin (Hb), in aqueous solution of poly(ethylene oxide) (PEO) we mimic a crowded environment and use state-of-the-art neutron spin echo (NSE) and small-angle neutron scattering (SANS) techniques to observe the corresponding protein dynamics in semidilute polymer solution. NSE can access the fast diffusion process (D-fast) prior to the slow diffusion process on long times and length scales (D-gamma). The protein dynamics in a crowded environment can be described analogous to the diffusion in a periodic potential. The fast dynamics corresponds to diffusion inside a trap built by the polymer mesh while the slower process is the long time diffusion on macroscopic length scales also observed by other techniques. We observe the onset of fractional diffusion for higher concentrated polymer solutions. C1 [Gupta, Sudipta; Ohl, Michael] JCNS, Outstn SNS, POB 2008,1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. [Gupta, Sudipta; Ohl, Michael] Oak Ridge Natl Lab, Biol & Soft Matter Div, Neutron Sci Directorate, POB 2008,1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. [Biehl, Ralf; Sill, Clemens; Allgaier, Juergen; Richter, Dieter] Forschungszentrum Julich, JCNS, D-52425 Julich, Germany. [Biehl, Ralf; Sill, Clemens; Allgaier, Juergen; Richter, Dieter] Forschungszentrum Julich, ICS, D-52425 Julich, Germany. [Sharp, Melissa] ILL Grenoble, 71 Rue Martyrs, F-38042 Grenoble 9, France. [Sharp, Melissa] ESS, POB 176, SE-22100 Lund, Sweden. RP Gupta, S (reprint author), JCNS, Outstn SNS, POB 2008,1 Bethel Valley Rd, Oak Ridge, TN 37831 USA.; Gupta, S (reprint author), Oak Ridge Natl Lab, Biol & Soft Matter Div, Neutron Sci Directorate, POB 2008,1 Bethel Valley Rd, Oak Ridge, TN 37831 USA.; Biehl, R (reprint author), Forschungszentrum Julich, JCNS, D-52425 Julich, Germany.; Biehl, R (reprint author), Forschungszentrum Julich, ICS, D-52425 Julich, Germany. EM s.gupta@fz-juelich.de; ra.biehl@fz-juelich.de RI Richter, Dieter/H-3701-2013 OI Richter, Dieter/0000-0003-0719-8470 FU Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy FX We thank W. P. Hintzen, A. Wischnewski, and M. Monkenbusch for helpful discussions. We thank S. V. Pingali for helping us with the SANS experiment and G. Kali for helping with NSE measurements. We thank A. Glavic for helping in developing the necessary codes to model the data. Research conducted at Oak Ridge National Laboratory's (ORNL) Spallation Neutron Source (SNS) and High Flux Isotope Reactor (HIFR) was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. NR 63 TC 1 Z9 1 U1 11 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD MAR 8 PY 2016 VL 49 IS 5 BP 1941 EP 1949 DI 10.1021/acs.macromol.5b02281 PG 9 WC Polymer Science SC Polymer Science GA DG1TT UT WOS:000371851100047 ER PT J AU Leuty, GM Tsige, M Grest, GS Rubinstein, M AF Leuty, Gary M. Tsige, Mesfin Grest, Gary S. Rubinstein, Michael TI Tension Amplification in Tethered Layers of Bottle-Brush Polymers SO MACROMOLECULES LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; HUMAN BLOOD-PLASMA; COMPUTER-SIMULATIONS; BRANCHED POLYMERS; BLOCK-COPOLYMERS; MACROMOLECULES; ADSORPTION; SURFACES; POLYELECTROLYTES; LUBRICATION AB Molecular dynamics simulations of a coarse-grained bead spring model have been used to study the effects of molecular crowding on the accumulation of tension in the backbone of bottle-brush polymers tethered to a flat substrate. The number of bottle -brushes per unit surface area, Sigma, as well as the lengths of the bottle-brush backbones N-bb (so <= N-bb <= 200) and side chains N-sc (50 <= N-sc <= 200) were varied to determine how the dimensions and degree of crowding of bottle -brushes give rise to bond tension amplification along the backbone, especially near the substrate. From these simulations, we have identified three separate regimes of tension. For low Sigma, the tension is due solely to intramolecular interactions and is dominated by the side chain repulsion that governs the lateral brush dimensions. With increasing Sigma, the interactions between bottle-brush polymers induce compression of the side chains, transmitting increasing tension to the backbone. For large Sigma, intermolecular side chain repulsion increases, forcing side chain extension and reorientation in the direction normal to the surface and transmitting considerable tension to the backbone. C1 [Leuty, Gary M.; Tsige, Mesfin] Univ Akron, Dept Polymer Sci, Akron, OH 44325 USA. [Grest, Gary S.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Rubinstein, Michael] Univ N Carolina, Dept Chem, Chapel Hill, NC 27599 USA. [Leuty, Gary M.] US Air Force, Res Lab, Mat & Mfg Directorate, Wright Patterson AFB, OH 45433 USA. RP Leuty, GM; Tsige, M (reprint author), Univ Akron, Dept Polymer Sci, Akron, OH 44325 USA.; Leuty, GM (reprint author), US Air Force, Res Lab, Mat & Mfg Directorate, Wright Patterson AFB, OH 45433 USA. EM gary.leuty.ctr@us.af.mil; mtsige@uakron.edu FU National Science Foundation [DMR-1410290, DMR-1309892, DMR-1436201, DMR-1121107]; National Institutes of Health [1-P01-HL108808, 1-UH2-HL123645]; Cystic Fibrosis Foundation; U.S. Department of Energy National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the National Science Foundation (DMR-1410290). M.R acknowledges financial support from the National Science Foundation under Grants DMR-1309892, DMR-1436201, and DMR-1121107, the National Institutes of Health under 1-P01-HL108808 and 1-UH2-HL123645, and the Cystic Fibrosis Foundation. This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 67 TC 1 Z9 1 U1 8 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD MAR 8 PY 2016 VL 49 IS 5 BP 1950 EP 1960 DI 10.1021/acs.macromol.5602305 PG 11 WC Polymer Science SC Polymer Science GA DG1TT UT WOS:000371851100048 PM 27695137 ER PT J AU Huang, L Taufour, V Lamichhane, TN Schrunk, B Bud'ko, SL Canfield, PC Kaminski, A AF Huang, Lunan Taufour, Valentin Lamichhane, T. N. Schrunk, Benjamin Bud'ko, Sergei L. Canfield, P. C. Kaminski, Adam TI Imaging the magnetic nanodomains in Nd2Fe14B SO PHYSICAL REVIEW B LA English DT Article ID SPIN-REORIENTATION TRANSITION; SCANNING-ELECTRON-MICROSCOPY; FORCE MICROSCOPY; SINGLE-CRYSTALS; DOMAIN-STRUCTURE AB We study magnetic domains in Nd2Fe14B single crystals using high resolution magnetic force microscopy (MFM). Previous MFM studies and small angle neutron scattering experiments suggested the presence of nanoscale domains in addition to optically detected micrometer-scale ones. We find, in addition to the elongated, wavy nanodomains reported by a previous MFM study, that the micrometer-sized, star-shaped fractal pattern is constructed of an elongated network of nanodomains similar to 20 nm in width, with resolution-limited domain walls thinner than 2 nm. While the microscopic domains exhibit significant resilience to an external magnetic field, some of the nanodomains are sensitive to the magnetic field of the MFM tip. C1 [Huang, Lunan] US DOE, Div Mat Sci & Engn, Ames Lab, Ames, IA 50011 USA. Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Huang, L (reprint author), US DOE, Div Mat Sci & Engn, Ames Lab, Ames, IA 50011 USA. FU US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; Critical Materials Institute, an Energy Innovation Hub - US Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office; US Department of Energy [DE-AC02-07CH11358] FX This research was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering (data acquisition and analysis). P.C.C., T.N.L., and V.T. acknowledge support from the Critical Materials Institute, an Energy Innovation Hub funded by the US Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office (sample growth). Ames Laboratory is operated for the US Department of Energy by the Iowa State University under Contract No. DE-AC02-07CH11358. NR 17 TC 0 Z9 0 U1 6 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 8 PY 2016 VL 93 IS 9 AR 094408 DI 10.1103/PhysRevB.93.094408 PG 4 WC Physics, Condensed Matter SC Physics GA DG0BV UT WOS:000371727900001 ER PT J AU Carroll, RJ Page, RD Joss, DT O'Donnell, D Uusitalo, J Darby, IG Andgren, K Auranen, K Bonig, S Cederwal, B Doncel, M Drummond, MC Eeckhaudt, S Grahn, T Gray-Jones, C Greenlees, PT Hadinia, B Herzan, A Jakobsson, U Jones, PM Julin, R Juutinen, S Konki, J Kroll, T Leino, M Leppanen, AP McPeake, C Nyman, M Pakarinen, J Partanen, J Peura, P Rahkila, P Revill, J Ruotsalainen, P Sandzelius, M Saren, J Saygi, B Scholey, C Seweryniak, D Simpson, J Sorri, J Stolze, S Taylor, MJ Thornthwaite, A AF Carroll, R. J. Page, R. D. Joss, D. T. O'Donnell, D. Uusitalo, J. Darby, I. G. Andgren, K. Auranen, K. Boenig, S. Cederwal, B. Doncel, M. Drummond, M. C. Eeckhaudt, S. Grahn, T. Gray-Jones, C. Greenlees, P. T. Hadinia, B. Herzan, A. Jakobsson, U. Jones, P. M. Julin, R. Juutinen, S. Konki, J. Kroell, T. Leino, M. Leppanen, A. -P. McPeake, C. Nyman, M. Pakarinen, J. Partanen, J. Peura, P. Rahkila, P. Revill, J. Ruotsalainen, P. Sandzelius, M. Saren, J. Saygi, B. Scholey, C. Seweryniak, D. Simpson, J. Sorri, J. Stolze, S. Taylor, M. J. Thornthwaite, A. TI Excited states in the proton-unbound nuclide Ta-158 SO PHYSICAL REVIEW C LA English DT Article ID NEUTRON-DEFICIENT ISOTOPES; GAMMA-RAY SPECTROSCOPY; TOTAL DATA READOUT; HIGH-SPIN STATES; ROTATIONAL BANDS; DRIP-LINE; DECAY; NUCLEUS; ELEMENTS; ISOMERS AB Excited states in the neutron-deficient odd-odd proton-unbound nuclide Ta-158 have been investigated in two separate experiments. In the first experiment, Ir-166 nuclei were produced in the reactions of 380 MeV Kr-78 ions with an isotopically enriched Mo-92 target. The alpha-decay chain of the 9(+) state in Ir-166 was analyzed. Fine structure in the a decay of the 9(+) state in Re-162 established a 66 keV difference in excitation energy between the lowest-lying 9(+) and 10(+) states in Ta-158. Higher-lying states in Ta-158 were populated in the reactions of 255 MeV Ni-58 ions with an isotopically enriched Pd-102 target. Gamma-ray decay paths that populate, depopulate, and bypass a 19(-) isomeric state have been identified. The general features of the deduced level scheme are discussed and the prospects for observing proton emission branches from excited states are considered. C1 [Carroll, R. J.; Page, R. D.; Joss, D. T.; O'Donnell, D.; Darby, I. G.; Drummond, M. C.; Gray-Jones, C.; McPeake, C.; Revill, J.; Saygi, B.; Thornthwaite, A.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 7ZE, Merseyside, England. [Uusitalo, J.; Auranen, K.; Eeckhaudt, S.; Grahn, T.; Greenlees, P. T.; Herzan, A.; Jakobsson, U.; Jones, P. M.; Julin, R.; Juutinen, S.; Konki, J.; Leino, M.; Leppanen, A. -P.; Nyman, M.; Pakarinen, J.; Partanen, J.; Peura, P.; Rahkila, P.; Ruotsalainen, P.; Sandzelius, M.; Saren, J.; Scholey, C.; Sorri, J.; Stolze, S.] Univ Jyvaskyla, Dept Phys, FI-40014 Jyvaskyla, Finland. [Andgren, K.; Cederwal, B.; Doncel, M.; Hadinia, B.; Jakobsson, U.; Sandzelius, M.] Alba Nova Ctr, Dept Phys, Royal Inst Technol, S-10691 Stockholm, Sweden. [Boenig, S.; Kroell, T.] Tech Univ Darmstadt, Inst Kemphys, Petersenstr 30, D-64289 Darmstadt, Germany. [Seweryniak, D.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Simpson, J.] STFC Daresbury Lab, Warrington WA4 4AD, Cheshire, England. [Taylor, M. J.] Univ Manchester, Schuster Lab, Manchester M13 9PL, Lancs, England. [Carroll, R. J.] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England. [O'Donnell, D.] Univ Glasgow, Dept Phys, Glasgow G12 8QQ, Lanark, Scotland. [Darby, I. G.] IAEA, Dept Nucl Sci & Applicat, A-1400 Vienna, Austria. [Hadinia, B.] Univ Guelph, Dept Phys, Guelph, ON N1G 2W1, Canada. [Jones, P. M.] iThemba Lab Accelerator Based Sci, Dept Nucl Phys, POB 722, ZA-7129 Somerset West, South Africa. [Leppanen, A. -P.] Radiat & Nucl Safety Author, STUK, Helsinki, Finland. [Nyman, M.] IRMM, Retieseweg 111, B-2440 Geel, Belgium. [Peura, P.] Univ Helsinki, Helsinki Inst Phys, FIN-00014 Helsinki, Finland. [Ruotsalainen, P.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. RP Carroll, RJ (reprint author), Univ Liverpool, Oliver Lodge Lab, Liverpool L69 7ZE, Merseyside, England.; Carroll, RJ (reprint author), Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England. RI O'Donnell, David/J-7786-2013; Scholey, Catherine/G-2720-2014 OI O'Donnell, David/0000-0002-4710-3803; Scholey, Catherine/0000-0002-8743-6071 FU UK Science and Technology Facilities Council (S.T.F.C.); Academy of Finland under the Finnish Centre of Excellence Programme [213503]; Finnish Centre of Excellence Programme; Swedish Research Council [2010-3694]; EURONS (European Commission) [RII3-CT-2004-506065]; ENSAR (the European Union Seventh Framework Programme Integrating Activities, Transnational Access) [262010]; U.S. Department of Energy, Office of Nuclear Physics [DEAC02-06CH11357]; Academy of Finland [131665, 111965, 209430] FX This work has been supported through the UK Science and Technology Facilities Council (S.T.F.C.); the Academy of Finland under the Finnish Centre of Excellence Programme 2006-2011 (Nuclear and Accelerator Based Physics Contract No. 213503) and the Finnish Centre of Excellence Programme 2012-2017; Swedish Research Council (Contract No. 2010-3694); EURONS (European Commission Contract No. RII3-CT-2004-506065); ENSAR (the European Union Seventh Framework Programme Integrating Activities, Transnational Access Project No. 262010); and the U.S. Department of Energy, Office of Nuclear Physics, under Contract No. DEAC02-06CH11357. The UK/France (STFC/IN2P3) Loan Pool and GAMMAPOOL network are acknowledged for the EUROGAM detectors of JUROGAM. T.G., P.T.G., and C.S. acknowledge the support of the Academy of Finland, Contracts No. 131665, No. 111965, and No. 209430, respectively. NR 41 TC 1 Z9 1 U1 7 U2 24 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 8 PY 2016 VL 93 IS 3 AR 034307 DI 10.1103/PhysRevC.93.034307 PG 9 WC Physics, Nuclear SC Physics GA DG0FO UT WOS:000371740600002 ER PT J AU Mecca, A Lovato, A Benhar, O Polls, A AF Mecca, Angela Lovato, Alessandro Benhar, Omar Polls, Artur TI Transport properties of the Fermi hard-sphere system SO PHYSICAL REVIEW C LA English DT Article ID NUCLEAR-MATTER; NEUTRON-STARS; DENSE MATTER; TEMPERATURES; EQUATION; FLUIDS; ENERGY; LIQUID; GAS AB The transport properties of neutron star matter play an important role in many astrophysical processes. We report the results of a calculation of the shear viscosity and thermal conductivity coefficients of the hard-sphere fermion system of degeneracy nu = 2, that can be regarded as a model of pure neutron matter. Our approach is based on the effective interaction obtained from the formalism of correlated basis functions and the cluster expansion technique. The resulting transport coefficients show a strong sensitivity to the quasiparticle effective mass, reflecting the effect of second-order contributions to the self-energy that are not taken into account in nuclear matter studies available in the literature. C1 [Mecca, Angela; Benhar, Omar] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Mecca, Angela; Benhar, Omar] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Lovato, Alessandro] Argonne Natl Lab, Argonne Leadership Comp Facil, 9700 S Cass Ave, Argonne, IL 60439 USA. [Lovato, Alessandro] Argonne Natl Lab, Div Phys, 9700 S Cass Ave, Argonne, IL 60439 USA. [Polls, Artur] Dept Estruct & Constituents Mat, E-08028 Barcelona, Spain. [Polls, Artur] Inst Ciencies Cosmos, E-08028 Barcelona, Spain. RP Mecca, A (reprint author), Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. OI Lovato, Alessandro/0000-0002-2194-4954 FU US Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357]; MICINN (Spain) [FI-2014-54672-P]; Generalitat de Catalunya [2014SGR-401]; INFN (Italy) [MANYBODY]; "NewCompStar", COST Action [MP1304] FX This research is supported by the US Department of Energy, Office of Science, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357 (AL), MICINN (Spain), under Grant No. FI-2014-54672-P, and Generalitat de Catalunya, under Grant No. 2014SGR-401 (AP), and INFN (Italy) under Grant No. MANYBODY (AM and OB). AM gratefully acknowledges the hospitality of the Departament d'Estructura i Constituents de la Materia of the University of Barcelona, and support from "NewCompStar", COST Action MP1304. NR 29 TC 0 Z9 0 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 8 PY 2016 VL 93 IS 3 AR 035802 DI 10.1103/PhysRevC.93.035802 PG 10 WC Physics, Nuclear SC Physics GA DG0FO UT WOS:000371740600009 ER PT J AU Ji, XD Schafer, A Yuan, F Zhang, JH Zhao, Y AF Ji, Xiangdong Schaefer, Andreas Yuan, Feng Zhang, Jian-Hui Zhao, Yong TI Spin decomposition of the electron in QED SO PHYSICAL REVIEW D LA English DT Article ID RENORMALIZATION; SCATTERING; NUCLEON AB We perform a systematic study on the spin decomposition of an electron in QED at one-loop order. It is found that the electron orbital angular momentum defined in Jaffe-Manohar and Ji spin sum rules agree with each other, and the so-called potential angular momentum vanishes at this order. The calculations are performed in both dimensional regularization and Pauli-Villars regularization for the ultraviolet divergences, and they lead to consistent results. We further investigate the calculations in terms of light-front wave functions and find a missing contribution from the instantaneous interaction in light- front quantization. This clarifies the confusing issues raised recently in the literature on the spin decomposition of an electron and will help consolidate the spin physics program for nucleons in QCD. C1 [Ji, Xiangdong] Shanghai Jiao Tong Univ, Dept Phys & Astron, INPAC, Shanghai 200240, Peoples R China. [Ji, Xiangdong; Zhao, Yong] Univ Maryland, Maryland Ctr Fundamental Phys, College Pk, MD 20742 USA. [Schaefer, Andreas; Zhang, Jian-Hui] Univ Regensburg, Inst Theoret Phys, D-93040 Regensburg, Germany. [Yuan, Feng; Zhao, Yong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Ji, XD (reprint author), Shanghai Jiao Tong Univ, Dept Phys & Astron, INPAC, Shanghai 200240, Peoples R China.; Ji, XD (reprint author), Univ Maryland, Maryland Ctr Fundamental Phys, College Pk, MD 20742 USA. FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-FG02-93ER-40762, DE-AC02-05CH11231]; Office of Science and Technology in Shanghai Municipal Government [11DZ2260700]; National Science Foundation of China [11175114, 11405104]; DFG [SCHA 458/20-1] FX This work was partially supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics under Grants No. DE-FG02-93ER-40762 and No. DE-AC02-05CH11231, Grant No. 11DZ2260700 from the Office of Science and Technology in Shanghai Municipal Government, Grants No. 11175114 and No. 11405104 from the National Science Foundation of China, and by DFG Grant No. SCHA 458/20-1. NR 32 TC 2 Z9 2 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 8 PY 2016 VL 93 IS 5 AR 054013 DI 10.1103/PhysRevD.93.054013 PG 8 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DG0FW UT WOS:000371741700004 ER PT J AU Mikkelsen, RE Poulsen, T Uggerhoj, UI Klein, SR AF Mikkelsen, R. E. Poulsen, T. Uggerhoj, U. I. Klein, S. R. TI Characteristics of Cherenkov radiation in naturally occurring ice SO PHYSICAL REVIEW D LA English DT Article ID RADIO ARRAY; SOUTH-POLE; DETECTOR; NEUTRINOS; STATION; ARIANNA AB We revisit the theory of Cherenkov radiation in uniaxial crystals. Historically, a number of flawed attempts have been made at explaining this radiation phenomenon, and a consistent error-free description is nowhere available. We apply our calculation to a large modern day telescope-IceCube. Located in Antarctica, this detector makes use of the naturally occurring ice as a medium to generate Cherenkov radiation. However, due to the high pressure at the depth of the detector site, large volumes of hexagonal ice crystals are formed. We calculate how this affects the Cherenkov radiation yield and angular dependence. We conclude that the effect is small, at most about a percent, and would only be relevant in future high-precision instruments like e.g. Precision IceCube Next Generation Upgrade (PINGU). For radio-Cherenkov experiments which use the presence of a clear Cherenkov cone to determine the arrival direction, any variation in emission angle will directly and linearly translate into a change in apparent neutrino direction. In closing, we also describe a simple experiment to test this formalism and calculate the impact of anisotropy on light yields from lead tungstate crystals as used, for example, in the CMS calorimeter at the CERN LHC. C1 [Mikkelsen, R. E.; Poulsen, T.; Uggerhoj, U. I.] Aarhus Univ, Dept Phys & Astron, DK-8000 Aarhus, Denmark. [Klein, S. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Klein, S. R.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RP Mikkelsen, RE (reprint author), Aarhus Univ, Dept Phys & Astron, DK-8000 Aarhus, Denmark. RI Uggerhoj, Ulrik/A-1802-2012 OI Uggerhoj, Ulrik/0000-0002-8229-1512 FU U.S. National Science Foundation [PHY-1307472]; U.S. Department of Energy [DE-AC-76SF00098] FX S. K. acknowledges a useful conversation with Ryan Bay (UC Berkeley). This work was supported in part by the U.S. National Science Foundation under Grant No. PHY-1307472 and the U.S. Department of Energy under Contract No. DE-AC-76SF00098. NR 40 TC 0 Z9 0 U1 1 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 8 PY 2016 VL 93 IS 5 AR 053006 DI 10.1103/PhysRevD.93.053006 PG 9 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DG0FW UT WOS:000371741700001 ER PT J AU Radyushkin, AV AF Radyushkin, A. V. TI Virtuality and transverse momentum dependence of the pion distribution amplitude SO PHYSICAL REVIEW D LA English DT Article ID TRANSITION FORM-FACTORS; CHARMONIUM SUM-RULES; QUANTUM CHROMODYNAMICS; PARTON DISTRIBUTIONS; PSEUDOSCALAR MESONS; EVOLUTION-EQUATIONS; EXCLUSIVE PROCESSES; SPECTRAL PROPERTIES; POWER CORRECTIONS; GAMMA-ASTERISK AB We describe basics of a new approach to transverse momentum dependence in hard exclusive processes. We develop it in application to the transition process gamma*gamma -> pi(0) at the handbag level. Our starting point is coordinate representation for matrix elements of operators [ in the simplest case, bilocal O(0, z)] describing a hadron with momentum p. Treated as functions of (pz) and z(2), they are parametrized through virtuality distribution amplitudes (VDA) Phi(x,sigma), with x being Fourier conjugate to (pz) and sigma Laplace conjugate to z(2). For intervals with z(+) = 0, we introduce the transverse momentum distribution amplitude ( TMDA). Psi(x, k(perpendicular to)), and write it in terms of VDA Phi(x, sigma). The results of covariant calculations, written in terms of Phi(x, sigma), are converted into expressions involving Psi(x, k(perpendicular to)). Starting with scalar toy models, we extend the analysis onto the case of spin-1/2 quarks and QCD. We propose simple models for soft VDAs/TMDAs, and use them for comparison of handbag results with experimental (BABAR and BELLE) data on the pion transition form factor. We also discuss how one can generate high-k(perpendicular to) tails from primordial soft distributions. C1 [Radyushkin, A. V.] Old Dominion Univ, Dept Phys, Norfolk, VA 23529 USA. [Radyushkin, A. V.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. RP Radyushkin, AV (reprint author), Old Dominion Univ, Dept Phys, Norfolk, VA 23529 USA.; Radyushkin, AV (reprint author), Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. FU Jefferson Science Associates, LLC [DE-AC05-06OR23177]; U.S. Department of Energy; U.S. DOE Grant [DE-FG02-97ER41028] FX I thank I. Balitsky, V. M. Braun, G. A. Miller, A. H. Mueller, A. Prokudin, A. Tarasov and C. Weiss for discussions. This work is supported by Jefferson Science Associates, LLC under Contract No. DE-AC05-06OR23177 with the U.S. Department of Energy and by U.S. DOE Grant No. DE-FG02-97ER41028. NR 43 TC 1 Z9 1 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 8 PY 2016 VL 93 IS 5 AR 056002 DI 10.1103/PhysRevD.93.056002 PG 36 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DG0FW UT WOS:000371741700009 ER PT J AU Bennett, MB Wrede, C Brown, BA Liddick, SN Perez-Loureiro, D Bardayan, DW Chen, AA Chipps, KA Fry, C Glassman, BE Langer, C Larson, NR McNeice, EI Meisel, Z Ong, W O'Malley, PD Pain, SD Prokop, CJ Schatz, H Schwartz, SB Suchyta, S Thompson, P Walters, M Xu, X AF Bennett, M. B. Wrede, C. Brown, B. A. Liddick, S. N. Perez-Loureiro, D. Bardayan, D. W. Chen, A. A. Chipps, K. A. Fry, C. Glassman, B. E. Langer, C. Larson, N. R. McNeice, E. I. Meisel, Z. Ong, W. O'Malley, P. D. Pain, S. D. Prokop, C. J. Schatz, H. Schwartz, S. B. Suchyta, S. Thompson, P. Walters, M. Xu, X. TI Isospin Mixing Reveals P-30(p,gamma)S-31 Resonance Influencing Nova Nucleosynthesis SO PHYSICAL REVIEW LETTERS LA English DT Article ID NUCLEAR-DATA SHEETS; FRAGMENT SEPARATOR; MODEL CALCULATIONS; CLASSICAL NOVAE; PRESOLAR GRAINS; REACTION-RATES; METEORITES; GRAPHS; TABLES AB The thermonuclear P-30(p,gamma)S-31 reaction rate is critical for modeling the final elemental and isotopic abundances of ONe nova nucleosynthesis, which affect the calibration of proposed nova thermometers and the identification of presolar nova grains, respectively. Unfortunately, the rate of this reaction is essentially unconstrained experimentally, because the strengths of key S-31 proton capture resonance states are not known, largely due to uncertainties in their spins and parities. Using the beta decay of Cl-31, we have observed the beta-delayed gamma decay of a S-31 state at E-x = 6390.2(7) keV, with a P-30(p,gamma)S-31 resonance energy of E-r = 259.3(8) keV, in the middle of the P-30(p,gamma)S-31 Gamow window for peak nova temperatures. This state exhibits isospin mixing with the nearby isobaric analog state at E-x = 6279.0(6) keV, giving it an unambiguous spin and parity of 3/2(+) and making it an important l = 0 resonance for proton capture on P-30. C1 [Bennett, M. B.; Wrede, C.; Brown, B. A.; Perez-Loureiro, D.; Fry, C.; Glassman, B. E.; Ong, W.; Schatz, H.; Schwartz, S. B.; Xu, X.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Bennett, M. B.; Wrede, C.; Brown, B. A.; Liddick, S. N.; Perez-Loureiro, D.; Fry, C.; Glassman, B. E.; Langer, C.; Larson, N. R.; Ong, W.; Prokop, C. J.; Schatz, H.; Schwartz, S. B.; Suchyta, S.; Xu, X.] Michigan State Univ, Natl Supercond Cyclotron Lab, E Lansing, MI 48824 USA. [Bennett, M. B.; Fry, C.; Langer, C.; Meisel, Z.; Ong, W.; Schatz, H.] Michigan State Univ, Joint Inst Nucl Astrophys, E Lansing, MI 48824 USA. [Liddick, S. N.; Larson, N. R.; Prokop, C. J.; Suchyta, S.] Michigan State Univ, Dept Chem, E Lansing, MI 48824 USA. [Bardayan, D. W.; Meisel, Z.; O'Malley, P. D.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Chen, A. A.; McNeice, E. I.; Walters, M.] McMaster Univ, Dept Phys & Astron, Hamilton, ON L8S 4M1, Canada. [Chipps, K. A.; Pain, S. D.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Chipps, K. A.; Thompson, P.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Schwartz, S. B.] Univ So Indiana, Dept Geol & Phys, 8600 Univ Blvd, Evansville, IN 47712 USA. RP Bennett, MB; Wrede, C (reprint author), Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA.; Bennett, MB; Wrede, C (reprint author), Michigan State Univ, Natl Supercond Cyclotron Lab, E Lansing, MI 48824 USA.; Bennett, MB (reprint author), Michigan State Univ, Joint Inst Nucl Astrophys, E Lansing, MI 48824 USA. EM bennettm@nscl.msu.edu; wrede@nscl.msu.edu RI Pain, Steven/E-1188-2011; Langer, Christoph/L-3422-2016; Larson, Nicole/S-5997-2016 OI Pain, Steven/0000-0003-3081-688X; Larson, Nicole/0000-0003-0292-957X FU U.S. National Science Foundation [PHY-1102511, PHY-1404442, PHY-1419765, PHY-1431052]; U.S. Department of Energy, National Nuclear Security Administration [DE-NA0000979]; Natural Sciences and Engineering Research Council of Canada FX The researchers greatly thank the NSCL operations staff for their support and tireless work to ensure the delivery of multiple very pure beams. This work was supported by the U.S. National Science Foundation under Grants No. PHY-1102511, No. PHY-1404442, No. PHY-1419765, and No. PHY-1431052, the U.S. Department of Energy, National Nuclear Security Administration under Award No. DE-NA0000979, and the Natural Sciences and Engineering Research Council of Canada. NR 44 TC 2 Z9 2 U1 1 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 8 PY 2016 VL 116 IS 10 AR 102502 DI 10.1103/PhysRevLett.116.102502 PG 6 WC Physics, Multidisciplinary SC Physics GA DF9ZP UT WOS:000371721600005 PM 27015475 ER PT J AU Jiang, C Uberuaga, BP AF Jiang, Chao Uberuaga, Bias P. TI Efficient Ab initio Modeling of Random Multicomponent Alloys SO PHYSICAL REVIEW LETTERS LA English DT Article ID HIGH-ENTROPY ALLOYS; QUASI-RANDOM STRUCTURES; 1ST-PRINCIPLES; APPROXIMATION; OPTIMIZATION; STABILITY; DESIGN AB We present in this Letter a novel small set of ordered structures (SSOS) method that allows extremely efficient ab initio modeling of random multicomponent alloys. Using inverse II-III spinel oxides and equiatomic quinary bcc (so-called high entropy) alloys as examples, we demonstrate that a SSOS can achieve the same accuracy as a large supercell or a well-converged cluster expansion, but with significantly reduced computational cost. In particular, because of this efficiency, a large number of quinary alloy compositions can be quickly screened, leading to the identification of several new possible high-entropy alloy chemistries. The SSOS method developed here can be broadly useful for the rapid computational design of multicomponent materials, especially those with a large number of alloying elements, a challenging problem for other approaches. C1 [Jiang, Chao; Uberuaga, Bias P.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. [Jiang, Chao] Idaho Natl Lab, Idaho Falls, ID 83402 USA. RP Jiang, C; Uberuaga, BP (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA.; Jiang, C (reprint author), Idaho Natl Lab, Idaho Falls, ID 83402 USA. EM chao.jiang@inl.gov; bias@lanl.gov RI Jiang, Chao/D-1957-2017 OI Jiang, Chao/0000-0003-0610-6327 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; National Nuclear Security Administration of the (U.S.) Department of Energy [DE-AC52-06NA25396] FX B.P.U. acknowledges support by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the (U.S.) Department of Energy under Contract No. DE-AC52-06NA25396. NR 32 TC 2 Z9 2 U1 14 U2 53 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 8 PY 2016 VL 116 IS 10 AR 105501 DI 10.1103/PhysRevLett.116.105501 PG 5 WC Physics, Multidisciplinary SC Physics GA DF9ZP UT WOS:000371721600008 PM 27015491 ER PT J AU Sangwan, N Xia, FF Gilbert, JA AF Sangwan, Naseer Xia, Fangfang Gilbert, Jack A. TI Recovering complete and draft population genomes from metagenome datasets SO MICROBIOME LA English DT Review DE Metagenomics; Genotype; Assembly; Binning; Curation ID DE-NOVO ASSEMBLER; CODON USAGE BIAS; MICROBIAL GENOMES; PROTEIN FAMILIES; SEQUENCING DATA; BRUIJN GRAPHS; SINGLE-CELL; DATA SETS; COVERAGE; BACTERIAL AB Assembly of metagenomic sequence data into microbial genomes is of fundamental value to improving our understanding of microbial ecology and metabolism by elucidating the functional potential of hard-to-culture microorganisms. Here, we provide a synthesis of available methods to bin metagenomic contigs into species-level groups and highlight how genetic diversity, sequencing depth, and coverage influence binning success. Despite the computational cost on application to deeply sequenced complex metagenomes (e.g., soil), covarying patterns of contig coverage across multiple datasets significantly improves the binning process. We also discuss and compare current genome validation methods and reveal how these methods tackle the problem of chimeric genome bins i.e., sequences from multiple species. Finally, we explore how population genome assembly can be used to uncover biogeographic trends and to characterize the effect of in situ functional constraints on the genome-wide evolution. C1 [Sangwan, Naseer; Gilbert, Jack A.] Argonne Natl Lab, Biosci Div BIO, 9700 South Cass Ave, Argonne, IL 60439 USA. [Xia, Fangfang] Argonne Natl Lab, Comp Environm & Life Sci, 9700 South Cass Ave, Argonne, IL 60439 USA. [Gilbert, Jack A.] Univ Chicago, Dept Ecol & Evolut, 1101 E 57th St, Chicago, IL 60637 USA. [Sangwan, Naseer; Gilbert, Jack A.] Univ Chicago, Dept Surg, 5841 South Maryland Ave,MC 5029, Chicago, IL 60637 USA. [Gilbert, Jack A.] Marine Biol Lab, 7 MBL St, Woods Hole, MA 02543 USA. RP Sangwan, N (reprint author), Univ Chicago, Dept Surg, 5841 South Maryland Ave,MC 5029, Chicago, IL 60637 USA. EM nikki1018sangwan@gmail.com OI Sangwan, Naseer/0000-0002-2407-769X FU US Dept. of Energy [DE-AC02-06CH11357] FX This work was supported by the US Dept. of Energy under Contract DE-AC02-06CH11357. NR 86 TC 10 Z9 10 U1 14 U2 60 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 2049-2618 J9 MICROBIOME JI Microbiome PD MAR 8 PY 2016 VL 4 AR UNSP 8 DI 10.1186/s40168-016-0154-5 PG 11 WC Microbiology SC Microbiology GA DF8EJ UT WOS:000371589700001 PM 26951112 ER PT J AU Bhattacharyya, M Stratton, MM Going, CC McSpadden, ED Huang, Y Susa, AC Elleman, A Cao, YM Pappireddi, N Burkhardt, P Gee, CL Barros, T Schulman, H Williams, ER Kurivan, J AF Bhattacharyya, Moitrayee Stratton, Margaret M. Going, Catherine C. McSpadden, Ethan D. Huang, Yongjian Susa, Anna C. Elleman, Anna Cao, Yumeng Melody Pappireddi, Nishant Burkhardt, Pawel Gee, Christine L. Barros, Tiago Schulman, Howard Williams, Evan R. Kurivan, John TI Molecular mechanism of activation-triggered subunit exchange in Ca2+/ calmodulin-dependent protein kinase II SO ELIFE LA English DT Article ID STRUCTURAL BASIS; ELECTRON-MICROSCOPY; MASS-SPECTROMETRY; CAM KINASE; ASSOCIATION DOMAIN; CRYSTAL-STRUCTURE; GENOME REVEALS; AUTOPHOSPHORYLATION; ALPHA; MEMORY AB Activation triggers the exchange of subunits in Ca2+/calmodulin-dependent protein kinase II (CaMKII), an oligomeric enzyme that is critical for learning, memory, and cardiac function. The mechanism by which subunit exchange occurs remains elusive. We show that the human CaMKII holoenzyme exists in dodecameric and tetradecameric forms, and that the calmodulin (CaM)-binding element of CaMKII can bind to the hub of the holoenzyme and destabilize it to release dimers. The structures of CaMKII from two distantly diverged organisms suggest that the CaM-binding element of activated CaMKII acts as a wedge by docking at intersubunit interfaces in the hub. This converts the hub into a spiral form that can release or gain CaMKII dimers. Our data reveal a three-way competition for the CaM-binding element, whereby phosphorylation biases it towards the hub interface, away from the kinase domain and calmodulin, thus unlocking the ability of activated CaMKII holoenzymes to exchange dimers with unactivated ones. C1 [Bhattacharyya, Moitrayee; Stratton, Margaret M.; McSpadden, Ethan D.; Huang, Yongjian; Elleman, Anna; Cao, Yumeng Melody; Pappireddi, Nishant; Burkhardt, Pawel; Gee, Christine L.; Barros, Tiago; Kurivan, John] Univ Calif Berkeley, Dept Cell & Mol Biol, Berkeley, CA 94720 USA. [Bhattacharyya, Moitrayee; Stratton, Margaret M.; McSpadden, Ethan D.; Huang, Yongjian; Elleman, Anna; Cao, Yumeng Melody; Pappireddi, Nishant; Gee, Christine L.; Barros, Tiago; Kurivan, John] Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. [Bhattacharyya, Moitrayee; Stratton, Margaret M.; McSpadden, Ethan D.; Huang, Yongjian; Elleman, Anna; Cao, Yumeng Melody; Pappireddi, Nishant; Burkhardt, Pawel; Gee, Christine L.; Barros, Tiago; Kurivan, John] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Going, Catherine C.; Susa, Anna C.; Williams, Evan R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Huang, Yongjian; Kurivan, John] Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA. [Schulman, Howard] Allosteros Therapeut, Sunnyvale, CA USA. [Kurivan, John] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Stratton, Margaret M.] Univ Massachusetts, Dept Biochem & Mol Biol, Amherst, MA USA. [Elleman, Anna] Stanford Univ, Dept Chem, Palo Alto, CA 94304 USA. [Cao, Yumeng Melody] Smith Coll, Dept Phys, Northampton, MA 01063 USA. [Burkhardt, Pawel] Marine Biol Assoc UK, Plymouth, Devon, England. RP Kurivan, J (reprint author), Univ Calif Berkeley, Dept Cell & Mol Biol, Berkeley, CA 94720 USA.; Kurivan, J (reprint author), Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA.; Kurivan, J (reprint author), Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA.; Kurivan, J (reprint author), Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA.; Kurivan, J (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM kuriyan@berkeley.edu FU Howard Hughes Medical Institute; National Institutes of Health [RO1GM101277]; Human Frontier Science Program; Jane Coffin Childs Memorial Fund for Medical Research FX Howard Hughes Medical Institute John Kuriyan; National Institutes of Health RO1GM101277 Howard Schulman; Human Frontier Science Program Moitrayee Bhattacharyya; Jane Coffin Childs Memorial Fund for Medical Research Margaret M Stratton NR 107 TC 3 Z9 4 U1 8 U2 13 PU ELIFE SCIENCES PUBLICATIONS LTD PI CAMBRIDGE PA SHERATON HOUSE, CASTLE PARK, CAMBRIDGE, CB3 0AX, ENGLAND SN 2050-084X J9 ELIFE JI eLife PD MAR 7 PY 2016 VL 5 AR e13405 DI 10.7554/eLife.13045 PG 32 WC Biology SC Life Sciences & Biomedicine - Other Topics GA DM3PB UT WOS:000376257400001 ER PT J AU Mineart, KP Al-Mohsin, HA Lee, B Spontak, RJ AF Mineart, Kenneth P. Al-Mohsin, Heba A. Lee, Byeongdu Spontak, Richard J. TI Water-induced nanochannel networks in self-assembled block ionomers SO APPLIED PHYSICS LETTERS LA English DT Article ID SULFONATED PENTABLOCK COPOLYMER; TRIBLOCK COPOLYMER; SOFT MATERIALS; LONG-CHAIN; POLYMERS; MEMBRANES; CELLS; SHAPE AB Block ionomers cast from solution exhibit solvent-templated morphologies that can be altered by solvent-vapor annealing. When cast from a mixed solvent, a midblock-sulfonated pentablock ionomer self-assembles into spherical ionic microdomains that are loosely connected. Upon exposure to liquid water, nanoscale channels irreversibly develop between the microdomains due to swelling and form a continuous mesoscale network. We use electron tomography and real-time X-ray scattering to follow this transformation and show that the resultant morphology provides a highly effective diffusive pathway. (C) 2016 AIP Publishing LLC. C1 [Mineart, Kenneth P.; Spontak, Richard J.] N Carolina State Univ, Dept Chem & Biomol Engn, Raleigh, NC 27695 USA. [Al-Mohsin, Heba A.] N Carolina State Univ, Fiber & Polymer Sci Program, Raleigh, NC 27695 USA. [Lee, Byeongdu] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Spontak, Richard J.] N Carolina State Univ, Dept Mat Sci & Engn, Box 7907, Raleigh, NC 27695 USA. RP Spontak, RJ (reprint author), N Carolina State Univ, Dept Chem & Biomol Engn, Raleigh, NC 27695 USA.; Spontak, RJ (reprint author), N Carolina State Univ, Dept Mat Sci & Engn, Box 7907, Raleigh, NC 27695 USA. EM Rich_Spontak@ncsu.edu OI Lee, Byeongdu/0000-0003-2514-8805 FU NC State Nonwovens Institute; MANN+HUMMEL GmbH; Ministry of Higher Education of Saudi Arabia; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357] FX This work was supported by the NC State Nonwovens Institute and MANN+HUMMEL GmbH (K.P.M.), as well as the Ministry of Higher Education of Saudi Arabia (H.A.A.-M.). In addition, this study used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. We are grateful to Michael Braunfeld and David Rutkowski for technical assistance, and Gregory Parsons for the use of his solar simulator. NR 39 TC 3 Z9 3 U1 9 U2 19 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 7 PY 2016 VL 108 IS 10 AR 101907 DI 10.1063/1.4943505 PG 5 WC Physics, Applied SC Physics GA DH7KV UT WOS:000372973600014 ER PT J AU Miskowiec, A Kirkegaard, MC Herwig, KW Trowbridge, L Mamontov, E Anderson, B AF Miskowiec, A. Kirkegaard, M. C. Herwig, K. W. Trowbridge, L. Mamontov, E. Anderson, B. TI Quasielastic neutron scattering with in situ humidity control: Water dynamics in uranyl fluoride SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID POROUS CARBON AEROGEL; PHASE-TRANSITIONS; CRYSTAL-STRUCTURE; EXCHANGE; SPECTROSCOPY; DIFFRACTION; COMPLEXES; MECHANISM; DIFFUSION; MEMBRANES AB The structural phase diagram of uranyl fluoride (UO2F2), while incomplete, contains at least one anhydrous crystal structure and a second, zeolite-like structure with the formula [(UO2F2)(H2O)](7)center dot(H2O)(4) that can be produced by adding water to the anhydrous structure. While traditional diffraction measurements can easily differentiate these crystals, additional aqueous structures (in general of the form UO2F2+xH2O) have been proposed as well. We present results using a novel sample environment setup to intercalate water during a quasielastic neutron scattering measurement over the course of 86 h. Our sample environment allows low-pressure (< 2 atm) humid air flow across the sample coupled with a system to control the relative humidity of this air flow between 10% and 70%. The water dynamics in UO2F2 and [(UO2F2)(H2O)](7)center dot(H2O)(4) are sufficiently different to distinguish them, with water in the latter executing a restricted diffusion (D = 2.7 x 10(-6) cm(2)/(s)) within the structure's accessible pores (r = 3.17 angstrom) such that the dynamics can be used as a fingerprinting tool. We confirm that water vapor pressure is the driving thermodynamic force for the conversion of the anhydrous structure to [(UO2F2)(H2O)](7) center dot (H2O)(4), and we demonstrate the feasibility of extending this approach to aqueous forms of UO2F2-xH2O. This method has general applicability to systems in which water content itself is a driving variable for structural or dynamical phase transitions. (C) 2016 AIP Publishing LLC. C1 [Miskowiec, A.; Kirkegaard, M. C.; Trowbridge, L.; Anderson, B.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Kirkegaard, M. C.] Univ Tennessee, Knoxville, TN 37996 USA. [Herwig, K. W.; Mamontov, E.] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. RP Miskowiec, A (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM miskowiecaj@ornl.gov RI Mamontov, Eugene/Q-1003-2015; OI Mamontov, Eugene/0000-0002-5684-2675; Anderson, Brian/0000-0002-0675-9750; Miskowiec, Andrew/0000-0002-0361-2614 FU U.S. Department of Energy [DE-AC05-00OR22725] FX This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 33 TC 0 Z9 0 U1 3 U2 8 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAR 7 PY 2016 VL 119 IS 9 AR 094308 DI 10.1063/1.4943164 PG 8 WC Physics, Applied SC Physics GA DG8RS UT WOS:000372351900035 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Abeloos, B Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allen, BW Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Armitage, LJ Arnaez, O Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Artz, S Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Balunas, WK Banas, E Banerjee, S Bannoura, AAE Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Navarro, LB Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, M Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bedognetti, M Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, AS Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Benitez, J Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Biedermann, D Bielski, R Biesuz, NV Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biondi, S Bjergaard, DM Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Blunier, S Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehler, M Boerner, D Bogaerts, JA Bogavac, D Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Bortfeldt, J Bortoletto, D Bortolotto, V Bos, K Boscherini, D Bosman, M Sola, JDB Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutle, SK Boveia, A Boyd, J Boyko, IR Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Madden, WDB Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E de Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Brunt, BH Bruschi, M Bruscino, N Bryant, P Bryngemark, L Buanes, T Buat, Q Buchholz, P Buckley, AG Budagov, IA Buehrer, F Bugge, MK Bulekov, O Bullock, D Burckhart, H Burdin, S Burgard, CD Burghgrave, B Burka, K Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Buzykaev, AR Urban, SC Caforio, D Cairo, VM Cakir, O Calace, N Calafiura, P Calandri, A Calderini, G Calfayan, P Caloba, LP Calvet, D Calvet, S Calvet, TP Toro, RC Camarda, S Camarri, P Cameron, D Armadans, RC Camincher, C Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Carbone, RM Cardarelli, R Cardillo, F Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Casper, DW Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catinaccio, A Catmore, JR Cattai, A Caudron, J Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Alberich, LC Cerio, BC Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chan, YL Chang, P Chapman, JD Charlton, DG Chau, CC Barajas, CAC Che, S Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, S Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A Cheremushkina, E Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiarelli, G Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Choi, K Chouridou, S Chow, BKB Christodoulou, V Chromek-Burckhart, D Chudoba, J Chuinard, AJ Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Cinca, D Cindro, V Cioara, IA Ciocio, A Cirotto, F Citron, ZH Ciubancan, M Clark, A Clark, BL Clark, PJ Clarke, RN Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Colasurdo, L Cole, B Cole, S Colijn, AP Collot, J Colombo, T Compostella, G Muino, PC Coniavitis, E Connell, SH Connelly, IA Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cottin, G Cowan, G Cox, BE Cranmer, K Crawley, SJ Cree, G Crepe-Renaudin, S Crescioli, F Cribbs, WA Ortuzar, MC Cristinziani, M Croft, V Crosetti, G Donszelmann, TC Cummings, J Curatolo, M Cuth, J Cuthbert, C Czirr, H Czodrowski, P D'Auria, S D'Onofrio, M De Sousa, MJDS Da Via, C Dabrowski, W Dai, T Dale, O Dallaire, F Dallapiccola, C Dam, M Dandoy, JR Dang, NP Daniells, AC Danninger, M Hoffmann, MD Dao, V Darbo, G Darmora, S Dassoulas, J Dattagupta, A Davey, W David, C Davidek, T Davies, M Davison, P Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Benedetti, A De Castro, S De Cecco, S De Groot, N de Jong, P De la Torre, H De Lorenzi, F De Pedis, D De Salvo, A De Sanctis, U De Santo, A De Regie, JBD Dearnaley, WJ Debbe, R Debenedetti, C Dedovich, DV Deigaard, I Del Peso, J Del Prete, T Delgove, D Deliot, F Delitzsch, CM Deliyergiyev, M Dell'Acqua, A Dell'Asta, L Dell'Orso, M Della Pietra, M della Volpe, D Delmastro, M Delsart, PA Deluca, C DeMarco, DA Demers, S Demichev, M Demilly, A Denisov, SP Denysiuk, D Derendarz, D Derkaoui, JE Derue, F Dervan, P Desch, K Deterre, C Dette, K Deviveiros, PO Dewhurst, A Dhaliwal, S Di Ciaccio, A Di Ciaccio, L Di Clemente, WK Di Domenico, A Di Donato, C Di Girolamo, A Di Girolamo, B Di Mattia, A Di Micco, B Di Nardo, R Di Simone, A Di Sipio, R Di Valentino, D Diaconu, C Diamond, M Dias, FA Diaz, MA Dickinson, J Diehl, EB Dietrich, J Diglio, S Dimitrievska, A Dingfelder, J Dita, P Dita, S Dittus, F Djama, F Djobava, T Djuvsland, JI do Vale, MAB Dobos, D Dobre, M Doglioni, C Dohmae, T Dolejsi, J Dolezal, Z Dolgoshein, BA Donadelli, M Donati, S Dondero, P Donini, J Dopke, J Doria, A Dova, MT Doyle, AT Drechsler, E Dris, M Du, Y Duarte-Campderros, J Duchovni, E Duckeck, G Ducu, OA Duda, D Dudarev, A Duflot, L Duguid, L Duhrssen, M Dunford, M Yildiz, HD Duren, M Durglishvili, A Duschinger, D Dutta, B Dyndal, M Eckardt, C Ecker, KM Edgar, RC Edson, W Edwards, NC Eifert, T Eigen, G Einsweiler, K Ekelof, T El Kacimi, M Ellajosyula, V Ellert, M Elles, S Ellinghaus, F Elliot, AA Ellis, N Elmsheuser, J Elsing, M Emeliyanov, D Enari, Y Endner, OC Endo, M Ennis, JS Erdmann, J Ereditato, A Ernis, G Ernst, J Ernst, M Errede, S Ertel, E Escalier, M Esch, H Escobar, C Esposito, B Etienvre, AI Etzion, E Evans, H Ezhilov, A Fabbri, L Facini, G Fakhrutdinov, RM Falciano, S Falla, RJ Faltova, J Fang, Y Fanti, M Farbin, A Farilla, A Farina, C Farooque, T Farrell, S Farrington, SM Farthouat, P Fassi, F Fassnacht, P Fassouliotis, D Giannelli, MF Favareto, A Fayard, L Fedin, OL Fedorko, W Feigl, S Feligioni, L Feng, C Feng, EJ Feng, H Fenyuk, AB Feremenga, L Martinez, PF Perez, SF Ferrando, J Ferrari, A Ferrari, P Ferrari, R de Lima, DEF Ferrer, A Ferrere, D Ferretti, C Parodi, AF Fiedler, F Filipcic, A Filipuzzi, M Filthaut, F 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Zivkovic, L. Zobernig, G. Zoccoli, A. Zur Nedden, M. Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Search for strong gravity in multijet final states produced in pp collisions at root s=13 TeV using the ATLAS detector at the LHC SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron scattering ID DISTRIBUTIONS; MILLIMETER; SIGNATURES; DIMENSIONS; HIERARCHY; MASS AB A search is conducted for new physics in multijet final states using 3.6 inverse femtobarns of data from proton-proton collisions at root s = 13TeV taken at the CERN Large Hadron Collider with the ATLAS detector. Events are selected containing at least three jets with scalar sum of jet transverse momenta (H-T) greater than 1TeV. No excess is seen at large H-T and limits are presented on new physics: models which produce final states containing at least three jets and having cross sections larger than 1.6 fb with H-T > 5.8TeV are excluded. 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M.; Beringer, J.; Bhimji, W.; Brosamer, J.; Calafiura, P.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Dickinson, J.; Einsweiler, K.; Farrell, S.; Gabrielli, A.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Heim, T.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Silva, M., Jr.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Amadio, B. T.; Axen, B.; Barnett, R. M.; Beringer, J.; Bhimji, W.; Brosamer, J.; Calafiura, P.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Dickinson, J.; Einsweiler, K.; Farrell, S.; Gabrielli, A.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Heim, T.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Silva, M., Jr.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Biedermann, D.; Dietrich, J.; Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Hristova, I.; Kind, O. M.; Kolanoski, H.; Lacker, H.; Lohse, T.; Mergelmeyer, S.; Nikiforov, A.; Rehnisch, L.; Rieck, P.; Schulz, H.; Sperlich, D.; Stamm, S.; Zur Nedden, M.] Humboldt Univ, Dept Phys, Invalidenstr 110, Berlin, Germany. [Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Mullier, G. A.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Mullier, G. A.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allport, P. P.; Bella, L. Aperio; Baca, M. J.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Owen, R. E.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Cetin, S. A.] Istanbul Bilgi Univ, Fac Engn & Nat Sci, Istanbul, Turkey. [Beddall, A. J.] Bahcesehir Univ, Fac Engn & Nat Sci, Istanbul, Turkey. [Alberghi, G. L.; Bellagamba, L.; Biondi, S.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, INFN Sez Bologna, Bologna, Italy. [Alberghi, G. L.; Biondi, S.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Bruscino, N.; Cioara, I. A.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Grefe, C.; Haefner, P.; Hageboeck, S.; Hansen, M. C.; Hohn, D.; Huegging, F.; Janssen, J.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Kruger, H.; Lantzsch, K.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mijovic, L.; Moles-Valls, R.; Obermann, T.; Pohl, D.; Ricken, O.; Sarrazin, B.; Schaepe, S.; Schopf, E.; Schultens, M. J.; Schwindt, T.; Seema, P.; Stillings, J. A.; Von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Yuen, S. P. Y.; Zhang, R.] Univ Bonn, Inst Phys, Nussallee 12, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, 590 Commonwealth Ave, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Barone, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Dhaliwal, S.; Diaz, M. A.; Loew, K. M.; Sciolla, G.; Venturini, A.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Filho, L. Manhaes de Andrade; Peralva, S.] Univ Fed Juiz de Fora, Elect Circuits Dept, Juiz de Fora, Brazil. [do Vale, M. A. B.] Univ Fed Sao Joao del Rei, Sao Joao del Rei, Brazil. [Donadelli, M.; Navarro, J. L. La Rosa; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, CP 20516, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lee, C. A.; Lissauer, D.; Liu, H.; Lynn, D.; Ma, H.; Maeno, T.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Xu, L.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. Transilvania Univ Brasov, Brasov, Romania. [Alexa, C.; Boldea, V.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Sola, J. D. Bossio; Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Brunt, B. H.; Carter, J. R.; Chapman, J. D.; Cottin, G.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Potter, C. J.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Gillberg, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Asztor, G. P.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Gonzalez, B. Alvarez; Amoroso, S.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beermann, T. A.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Carrillo-Montoya, G. D.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feng, E. J.; Francis, D.; Fressard-Batraneanu, S. M.; Froidevaux, D.; Gadatsch, S.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Gumpert, C.; Hawkings, R. J.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jakobsen, S.; Klioutchnikova, T.; Krasznahorkay, A.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Berlingen, J. Montejo; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Astigarraga, M. E. Pozo; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Ruthmann, N.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sforza, F.; Sanchez, C. A. Solans; Spigo, G.; Staerz, S.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Unal, G.; Van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Andeen, T.; Anderson, K. J.; Bryant, P.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Stark, G. H.; Swiatlowski, M.; Vukotic, I.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Blunier, S.; Carquin, E.; Ochoa-Ricoux, J. P.] Pontificia Univ Catolica Chile, Dept Fis, Alameda 340, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Loyola, J. E. Salazar; Araya, S. Tapia; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; da Costa, J. Barreiro Guimaraes; Fang, Y.; Jin, S.; Li, Q.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Geng, C.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y. L.; Liu, Y.; Peng, H.; Song, H. Y.; Zhang, G.; Zhang, R.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Du, Y.; Feng, C.; Ma, L. L.; Wang, C.; Zaidan, R.; Zhang, X.; Zhao, Y.; Zhao, Z.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Shanghai Key Lab Particle Phys & Cosmol, Dept Phys & Astron, Shanghai 200030, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] PKU CHEP, Beijing, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Gris, Ph; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Gris, Ph; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Gris, Ph; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Alkire, S. P.; Angerami, A.; Brooijmans, G.; Carbone, R. M.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] INFN Grp Collegato Cosenza, Lab Nazl Frascati, Arcavacata Di Rende, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Gach, G. P.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Burka, K.; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75230 USA. [Asbah, N.; Bessner, M.; Bloch, I.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Monig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Notkestr 85, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Monig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Zeuthen, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruhr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schnoor, U.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; De Mendizabal, J. Bilbao; Calace, N.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; March, L.; Mermod, P.; Miucci, A.; Nackenhorst, O.; Paolozzi, L.; Ristic, B.; Schramm, S.; Sfyrla, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. 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S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Camincher, C.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Petit, E.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Clark, B. L.; Franklin, M.; Giromini, P.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Rogan, C. S.; Skottowe, H. P.; Sun, S.; Tolley, E.; Tong, B.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Villar, D. I. 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Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Cheatham, S.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Muenstermann, D.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Bachas, K.; Chiodini, G.; Gorini, E.; Longo, L.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Bachas, K.; Gorini, E.; Longo, L.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Armitage, L. J.; Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bell, A. S.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Haut Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Groh, S.; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Kopke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Pleskot, V.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schafer, U.; Schmitt, C.; Schmitz, S.; Schott, M.; Schuh, N.; Simioni, E.; Simon, M.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Bielski, R.; Cox, B. E.; Da Via, C.; Forcolin, G. T.; Forti, A.; Ponce, J. M. Iturbe; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Sanchez, F. J. Munoz; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. 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C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Martin, B.; Mondragon, M. C.; Pope, G.; Schoenrock, B. D.; Schwienhorst, R.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Manzoni, S.; Mazza, S. M.; Meroni, C.; Monzani, S.; Perini, L.; Ragusa, F.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Via Celoria 16, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Manzoni, S.; Mazza, S. M.; Monzani, S.; Perini, L.; Ragusa, F.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. 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E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; La Rosa, A.; Macchiolo, A.; Maier, A. A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; Von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Kawade, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Mc Fadden, N. C.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Konig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen, Inst Math Astrophys & Particle Phys, Nikhef, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; Van der Geer, R.; Van der Graaf, H.; Van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; Van der Geer, R.; Van der Graaf, H.; Van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Becot, C.; Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Che, S.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Allen, B. W.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Radloff, P.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Abeloos, B.; Ayoub, M. K.; Bassalat, A.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Goudet, C. R.; Grivaz, J. -F.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Maiani, C.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris Saclay, Univ Paris Sud, LAL, CNRS,IN2P3, Orsay, France. [Endo, M.; Nomachi, M.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, M. K.; Cameron, D.; Catmore, J. R.; Feigl, S.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Artoni, G.; Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Bortoletto, D.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Di Clemente, W. K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Naryshkin, I.; Ryabov, Y. F.; Schegelsky, V. A.; Seliverstov, D. M.; Solovyev, V.] Natl Res Ctr Kurchatov Inst, BP Konstantinov Petersburg Nucl Phys Inst, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Farina, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Seabra, L. F. Oleiro; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Saraiva, J. G.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Fac Ciencias & Tecnol, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Sopczak, A.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] NRC KI, State Res Ctr Inst High Energy Phys Protvino, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Di Donato, C.; Falciano, S.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Di Domenico, A.; Di Donato, C.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Piazzale Aldo Moro 5, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Rome, Italy. [Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Haut Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Denysiuk, D.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Jeanneau, F.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Peyaud, A.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, IRFU, DSM, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Li, Y.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Su, D.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Kar, D.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.; Wallangen, V.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.; Wallangen, V.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Di Mattia, A.; Gozani, E.; Rozen, Y.; Tarem, S.; Van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Duarte-Campderros, J.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Pascuzzi, V.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Jovicevic, J.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Taylor, W.; Trigger, I. M.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. 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[Zhang, R.] Aix Marseille Univ, CPPM, Marseille, France. [Zhang, R.] CNRS, IN2P3, Marseille, France. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Zhukov, Konstantin/M-6027-2015; SULIN, VLADIMIR/N-2793-2015; Warburton, Andreas/N-8028-2013; Snesarev, Andrey/H-5090-2013; Brooks, William/C-8636-2013; Nechaeva, Polina/N-1148-2015; Mashinistov, Ruslan/M-8356-2015; Vykydal, Zdenek/H-6426-2016; Fedin, Oleg/H-6753-2016; Guo, Jun/O-5202-2015; Gorelov, Igor/J-9010-2015; Ventura, Andrea/A-9544-2015; White, Ryan/E-2979-2015; Carvalho, Joao/M-4060-2013; Leyton, Michael/G-2214-2016; Livan, Michele/D-7531-2012; Jones, Roger/H-5578-2011; Tikhomirov, Vladimir/M-6194-2015; Doyle, Anthony/C-5889-2009; Boyko, Igor/J-3659-2013; Mitsou, Vasiliki/D-1967-2009; Vranjes Milosavljevic, Marija/F-9847-2016; Gladilin, Leonid/B-5226-2011; Chekulaev, Sergey/O-1145-2015; Kuday, Sinan/C-8528-2014; Gavrilenko, Igor/M-8260-2015; Di Domenico, Antonio/G-6301-2011; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kantserov, Vadim/M-9761-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Smirnova, Oxana/A-4401-2013; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Conde Muino, Patricia/F-7696-2011; Stabile, Alberto/L-3419-2016; Villa, Mauro/C-9883-2009; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016 OI SULIN, VLADIMIR/0000-0003-3943-2495; Warburton, Andreas/0000-0002-2298-7315; Brooks, William/0000-0001-6161-3570; Mashinistov, Ruslan/0000-0001-7925-4676; Vykydal, Zdenek/0000-0003-2329-0672; Guo, Jun/0000-0001-8125-9433; Gorelov, Igor/0000-0001-5570-0133; Ventura, Andrea/0000-0002-3368-3413; White, Ryan/0000-0003-3589-5900; Carvalho, Joao/0000-0002-3015-7821; Leyton, Michael/0000-0002-0727-8107; Livan, Michele/0000-0002-5877-0062; Jones, Roger/0000-0002-6427-3513; Tikhomirov, Vladimir/0000-0002-9634-0581; Doyle, Anthony/0000-0001-6322-6195; Boyko, Igor/0000-0002-3355-4662; Mitsou, Vasiliki/0000-0002-1533-8886; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Gladilin, Leonid/0000-0001-9422-8636; Kuday, Sinan/0000-0002-0116-5494; KUBOTA, TAKASHI/0000-0002-1156-5571; Di Domenico, Antonio/0000-0001-8078-2759; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Smirnova, Oxana/0000-0003-2517-531X; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Conde Muino, Patricia/0000-0002-9187-7478; Stabile, Alberto/0000-0002-6868-8329; Villa, Mauro/0000-0002-9181-8048; Kukla, Romain/0000-0002-1140-2465 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, Italy; I-CORE, Isreael; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF; Canada Council; CANARIE; CRC; Compute Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET; ERC; FP7; Horizon; Marie Sklodowska-Curie Actions; European Union; Investissements d'Avenir Labex and Idex; ANR; Region Auvergne; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos programme; Thales programme; Aristeia programme; EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. NR 32 TC 2 Z9 2 U1 14 U2 46 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAR 7 PY 2016 IS 3 AR 026 DI 10.1007/JHEP03(2016)026 PG 38 WC Physics, Particles & Fields SC Physics GA DG8BL UT WOS:000372307300001 ER PT J AU Choi, EM Kleibeuker, JE Fix, T Xiong, J Kinane, CJ Arena, D Langridge, S Chen, AP Bi, ZX Lee, JH Wang, HY Jia, QX Blamire, MG MacManus-Driscoll, JL AF Choi, Eun-Mi Kleibeuker, Josee E. Fix, Thomas Xiong, Jie Kinane, Christy J. Arena, Dario Langridge, Sean Chen, Aiping Bi, Zhenxing Lee, Joon Hwan Wang, Haiyan Jia, Quanxi Blamire, Mark G. MacManus-Driscoll, Judith L. TI Interface-Coupled BiFeO3/BiMnO3 Superlattices with Magnetic Transition Temperature up to 410 K SO ADVANCED MATERIALS INTERFACES LA English DT Article DE BiFeO3; BiMnO3; magnetism; multilayers; thin films ID THIN-FILMS; DOUBLE PEROVSKITES; EXCHANGE BIAS; FERROELECTRICITY; FERROMAGNETISM; BIFE0.5MN0.5O3; MULTIFERROICS; LA1-XCEXMNO3; COERCIVITY; PHASES C1 [Choi, Eun-Mi; Kleibeuker, Josee E.; Fix, Thomas; Blamire, Mark G.; MacManus-Driscoll, Judith L.] Univ Cambridge, Dept Mat Sci, 27 Charles Babbage Rd, Cambridge CB3 0FS, England. [Xiong, Jie; Chen, Aiping; Bi, Zhenxing; Jia, Quanxi] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Xiong, Jie] Univ Elect Sci & Technol China, State Key Lab Elect Thin Films & Integrated Devic, Chengdu 610054, Peoples R China. [Kinane, Christy J.; Langridge, Sean] Rutherford Appleton Lab, ISIS, Sci & Technol Facil Council, Didcot OX11 0QX, Oxon, England. [Arena, Dario] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. [Arena, Dario] Univ S Florida, Dept Phys, Tampa, FL 33620 USA. [Chen, Aiping; Bi, Zhenxing; Lee, Joon Hwan; Wang, Haiyan] Texas A&M Univ, Dept Elect & Comp Engn, College Stn, TX 77843 USA. RP Choi, EM (reprint author), Univ Cambridge, Dept Mat Sci, 27 Charles Babbage Rd, Cambridge CB3 0FS, England. EM emc63@cam.ac.uk RI Chen, Aiping/F-3212-2011 OI Chen, Aiping/0000-0003-2639-2797 FU Engineering and Physical Sciences Research Council [EP/P50385X/1]; European Research Council [ERC-2009-AdG 247276 NOVOX]; US National Science Foundation [DMR-1401266]; U.S. Department of Energy through the LANL/LDRD program; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This research was funded by the Engineering and Physical Sciences Research Council (EP/P50385X/1) and the European Research Council (ERC-2009-AdG 247276 NOVOX). The work at Texas A&M was funded by the US National Science Foundation (DMR-1401266). The work at Los Alamos was supported by the U.S. Department of Energy through the LANL/LDRD program and was performed, in part, at the Center for Integrated Nanotechnologies, a US Department of Energy, Office of Basic Energy Sciences user facility. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 50 TC 3 Z9 3 U1 18 U2 45 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2196-7350 J9 ADV MATER INTERFACES JI Adv. Mater. Interfaces PD MAR 7 PY 2016 VL 3 IS 5 AR UNSP 1500597 DI 10.1002/admi.201500597 PG 8 WC Chemistry, Multidisciplinary; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DG3YA UT WOS:000372005900004 ER PT J AU Halverson, JD Tkachenko, AV AF Halverson, Jonathan D. Tkachenko, Alexei V. TI Sequential programmable self-assembly: Role of cooperative interactions SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID DNA; COLLOIDS; DESIGN; CRYSTALLIZATION; NANOPARTICLES AB We propose a general strategy of "sequential programmable self-assembly" that enables a bottom-up design of arbitrary multi-particle architectures on nano-and microscales. We show that a naive realization of this scheme, based on the pairwise additive interactions between particles, has fundamental limitations that lead to a relatively high error rate. This can be overcome by using cooperative interparticle binding. The cooperativity is a well known feature of many biochemical processes, responsible, e.g., for signaling and regulations in living systems. Here we propose to utilize a similar strategy for high precision self-assembly, and show that DNA-mediated interactions provide a convenient platform for its implementation. In particular, we outline a specific design of a DNA-based complex which we call "DNA spider," that acts as a smart interparticle linker and provides a built-in cooperativity of binding. We demonstrate versatility of the sequential self-assembly based on spider-functionalized particles by designing several mesostructures of increasing complexity and simulating their assembly process. This includes a number of finite and repeating structures, in particular, the so-called tetrahelix and its several derivatives. Due to its generality, this approach allows one to design and successfully self-assemble virtually any structure made of a "GEOMAG" magnetic construction toy, out of nanoparticles. According to our results, once the binding cooperativity is strong enough, the sequential self-assembly becomes essentially error-free. (C) 2016 AIP Publishing LLC. C1 [Halverson, Jonathan D.; Tkachenko, Alexei V.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Tkachenko, AV (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. EM oleksiyt@bnl.gov RI Tkachenko, Alexei/I-9040-2012 OI Tkachenko, Alexei/0000-0003-1291-243X FU U.S. DOE Office of Science Facility, at Brookhaven National Laboratory [DE-SC0012704] FX This work benefited from discussions with O. Gang, P. Chaikin, and M. Hybertsen. This research used resources of the Center for Functional Nanomaterials, which is a U.S. DOE Office of Science Facility, at Brookhaven National Laboratory under Contract No. DE-SC0012704. NR 24 TC 3 Z9 3 U1 3 U2 11 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAR 7 PY 2016 VL 144 IS 9 AR 094903 DI 10.1063/1.4942615 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DG4EA UT WOS:000372022800031 PM 26957179 ER PT J AU Tretiak, OY Blanchard, JW Budker, D Olshin, PK Smirnov, SN Balabas, MV AF Tretiak, O. Yu. Blanchard, J. W. Budker, D. Olshin, P. K. Smirnov, S. N. Balabas, M. V. TI Raman and nuclear magnetic resonance investigation of alkali metal vapor interaction with alkene-based anti-relaxation coating SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID QUANTUM TELEPORTATION; HYDROCARBONS; OBJECTS; ATOMS; CELLS AB The use of anti-relaxation coatings in alkali vapor cells yields substantial performance improvements compared to a bare glass surface by reducing the probability of spin relaxation in wall collisions by several orders of magnitude. Some of the most effective anti-relaxation coating materials are alpha-olefins,which (as in the case of more traditional paraffin coatings) must undergo a curing period after cell manufacturing in order to achieve the desired behavior. Until now, however, it has been unclear what physicochemical processes occur during cell curing, and how they may affect relevant cell properties. We present the results of nondestructive Raman-spectroscopy and magnetic-resonance investigations of the influence of alkali metal vapor (Cs or K) on an alpha-olefin, 1-nonadecene coating the inner surface of a glass cell. It was found that during the curing process, the alkali metal catalyzes migration of the carbon-carbon double bond, yielding a mixture of cis- and trans-2-nonadecene. (C) 2016 AIP Publishing LLC. C1 [Tretiak, O. Yu.; Balabas, M. V.] St Petersburg State Univ, Fac Phys, 7-9 Univ Nab, St Petersburg 199034, Russia. [Blanchard, J. W.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Blanchard, J. W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Blanchard, J. W.; Budker, D.] Johannes Gutenberg Univ Mainz, Helmholtz Inst Mainz, D-55099 Mainz, Germany. [Budker, D.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Budker, D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Olshin, P. K.] St Petersburg State Univ, Resource Ctr Opt & Laser Methods Mat Res, 7-9 Univ Nab, St Petersburg 199034, Russia. [Smirnov, S. N.] St Petersburg State Univ, Ctr Magnet Resonance, 7-9 Univ Nab, St Petersburg 199034, Russia. RP Tretiak, OY (reprint author), St Petersburg State Univ, Fac Phys, 7-9 Univ Nab, St Petersburg 199034, Russia. EM otretiak@genphys.ru OI Tretiak, Oleg/0000-0002-7667-2933; Blanchard, John/0000-0002-1621-6637; Balabas, Mikhail/0000-0002-5383-7897 FU National Science Foundation [CHE-1308381]; NGA NURI program; DFG DIP Project [FO 703/2-1, SCHM 1049/7-1]; Russian Science Foundation [14-12-00094]; National Science Foundation Graduate Research Fellowship [DGE-1106400] FX We wish to thank Professor A. Vasilyev of the chemical faculty of Saint-Petersburg State University for directing us towards sigmatropic mechanism of isomerization and very helpful discussion of chemical mechanisms of the described processes and interest in our work. Dmitry Budker acknowledges support by the National Science Foundation under Award No. CHE-1308381, by the NGA NURI program, and by the DFG DIP Project Reference No. FO 703/2-1 1 SCHM 1049/7-1. Presentation of the results at the International Conference on Atomic Physics 2014 in Washington DC (USA) was supported by Russian Science Foundation (Grant No. 14-12-00094). J.W.B. was supported by a National Science Foundation Graduate Research Fellowship under Grant No. DGE-1106400. NR 21 TC 0 Z9 0 U1 1 U2 2 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAR 7 PY 2016 VL 144 IS 9 AR 094707 DI 10.1063/1.4943123 PG 5 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DG4EA UT WOS:000372022800028 PM 26957176 ER PT J AU Clark, DL Bursten, BE AF Clark, David L. Bursten, Bruce E. TI Malcolm H. Chisholm (1945-2015) Obituary SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Biographical-Item C1 [Clark, David L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Bursten, Bruce E.] Worcester Polytech Inst, Worcester, MA USA. RP Clark, DL (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA.; Bursten, BE (reprint author), Worcester Polytech Inst, Worcester, MA USA. NR 1 TC 0 Z9 0 U1 1 U2 54 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD MAR 7 PY 2016 VL 55 IS 11 BP 3545 EP 3545 DI 10.1002/anie.201600879 PG 1 WC Chemistry, Multidisciplinary SC Chemistry GA DF7EQ UT WOS:000371521000001 PM 26895411 ER PT J AU Monreal, MJ Seaman, LA Goff, GS Michalczyk, R Morris, DE Scott, BL Kiplinger, JL AF Monreal, Marisa J. Seaman, Lani A. Goff, George S. Michalczyk, Ryszard Morris, David E. Scott, Brian L. Kiplinger, Jaqueline L. TI New Twists and Turns for Actinide Chemistry: Organometallic Infinite Coordination Polymers of Thorium Diazide SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE azides; coordination polymers; nitrogen; Raman spectroscopy; thorium ID TO-END AZIDE; MAGNETIC-BEHAVIOR; CRYSTAL-STRUCTURE; URANIUM AZIDE; STRUCTURAL-CHARACTERIZATION; SUPEROXIDE-DISMUTASE; COMPLEXES; COPPER(II); CHAIN; 1D AB Two organometallic 1D infinite coordination polymers and two organometallic monometallic complexes of thorium diazide have been synthesized and characterized. Steric control of these self-assembled arrays, which are dense in thorium and nitrogen, has also been demonstrated: infinite chains can be circumvented by using steric bulk either at the metallocene or with a donor ligand in the wedge. C1 [Monreal, Marisa J.; Seaman, Lani A.; Goff, George S.; Michalczyk, Ryszard; Morris, David E.; Scott, Brian L.; Kiplinger, Jaqueline L.] Los Alamos Natl Lab, Stop J-514, Los Alamos, NM 87545 USA. RP Kiplinger, JL (reprint author), Los Alamos Natl Lab, Stop J-514, Los Alamos, NM 87545 USA. EM kiplinger@lanl.gov RI Kiplinger, Jaqueline/B-9158-2011; Scott, Brian/D-8995-2017; OI Kiplinger, Jaqueline/0000-0003-0512-7062; Scott, Brian/0000-0003-0468-5396; Monreal, Marisa/0000-0001-6447-932X; Michalczyk, Ryszard/0000-0001-8839-6473 FU U.S. Department of Energy through the LANL LDRD Program; G.T. Seaborg Institute for Transactinium Science (Frederick Reines); Office of Basic Energy Sciences, Heavy Element Chemistry program; National Nuclear Security Administration of U.S. Department of Energy [DE-AC52-06NA25396] FX For financial support of this work, we acknowledge the U.S. Department of Energy through the LANL LDRD Program and G.T. Seaborg Institute for Transactinium Science (Frederick Reines, Director's and G. T. Seaborg PD Fellowships for M.J.M.), and the Office of Basic Energy Sciences, Heavy Element Chemistry program (J.L.K., B.L.S., R.M., materials & supplies). We gratefully acknowledge LANL PADSTE for institutional investment in key NMR equipment. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of U.S. Department of Energy (contract DE-AC52-06NA25396). NR 67 TC 1 Z9 1 U1 7 U2 30 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD MAR 7 PY 2016 VL 55 IS 11 BP 3631 EP 3636 DI 10.1002/anie.201510851 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA DF7EQ UT WOS:000371521000014 PM 26865502 ER PT J AU Bittner, DM Zaleski, DP Tew, DP Walker, NR Legon, AC AF Bittner, Dror M. Zaleski, Daniel P. Tew, David P. Walker, Nicholas R. Legon, Anthony C. TI Highly Unsaturated Platinum and Palladium Carbenes PtC3 and PdC3 Isolated and Characterized in the Gas Phase SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE ab initio calculations; carbenes; palladium; platinum; rotational spectroscopy ID PURE ROTATIONAL SPECTRUM; MICROWAVE-SPECTRUM; TRANSITION-METAL; CARBON CLUSTERS; SPECTROSCOPY; METHANE; ATOMS; (X)OVER-TILDE(2)A(1); MONOCARBIDE; ACTIVATION AB Carbenes of platinum and palladium, PtC3 and PdC3, were generated in the gas phase through laser vaporization of a metal target in the presence of a low concentration of a hydrocarbon precursor undergoing supersonic expansion. Rotational spectroscopy and abinitio calculations confirm that both molecules are linear. The geometry of PtC3 was accurately determined by fitting to the experimental moments of inertia of twenty-six isotopologues. The results are consistent with the proposal of an autogenic isolobal relationship between O, Au+, and Ptatoms. C1 [Bittner, Dror M.; Zaleski, Daniel P.; Walker, Nicholas R.] Newcastle Univ, Sch Chem, Bedson Bldg, Newcastle Upon Tyne NE1 7RU, Tyne & Wear, England. [Tew, David P.; Legon, Anthony C.] Univ Bristol, Sch Chem, Bristol BS8 1TS, Avon, England. [Zaleski, Daniel P.] Argonne Natl Lab, Chem Sci & Engn, 9700 S Cass Ave,Bldg 200, Lemont, IL 60439 USA. RP Walker, NR (reprint author), Newcastle Univ, Sch Chem, Bedson Bldg, Newcastle Upon Tyne NE1 7RU, Tyne & Wear, England.; Legon, AC (reprint author), Univ Bristol, Sch Chem, Bristol BS8 1TS, Avon, England. EM nick.walker@newcastle.ac.uk; a.c.legon@bristol.ac.uk RI Walker, Nicholas /E-6180-2011; Tew, David/E-1458-2011; OI Walker, Nicholas /0000-0002-9450-305X; Tew, David/0000-0002-3220-4177; Zaleski, Daniel/0000-0003-0153-9158 FU European Research Council [CPFTMW-307000]; Engineering and Physical Sciences Research Council (U.K.) [EPK5028931]; University of Bristol; Newcastle University; Royal Society FX The authors thank the European Research Council (CPFTMW-307000) for project funding, the Engineering and Physical Sciences Research Council (U.K.) for the award of a DTA studentship (EPK5028931) to D.M.B., and the EPSRC UK National Service for Computational Chemistry Software (NSCCS) at Imperial College London. A.C.L. thanks the University of Bristol for a Senior Research Fellowship. D.P.Z. thanks Newcastle University for the award of a Faculty of SAgE Research Fellowship. D.P.T. thanks the Royal Society for a University Research Fellowship. NR 39 TC 1 Z9 1 U1 2 U2 11 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD MAR 7 PY 2016 VL 55 IS 11 BP 3768 EP 3771 DI 10.1002/anie.201511646 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DF7EQ UT WOS:000371521000042 PM 26879473 ER PT J AU Brinzari, TV O'Neal, KR Manson, JL Schlueter, JA Litvinchuk, AP Liu, ZX Musfeldt, JL AF Brinzari, Tatiana V. O'Neal, Kenneth R. Manson, Jamie L. Schlueter, John A. Litvinchuk, Alexander P. Liu, Zhenxian Musfeldt, Janice L. TI Local Lattice Distortions in Mn[N(CN)(2)](2) under Pressure SO INORGANIC CHEMISTRY LA English DT Article ID PHASE-TRANSITIONS; ORGANIC METALS; GROUND-STATE; DICYANAMIDE; MAGNETIZATION; TEMPERATURE; MAGNETISM; CROSSOVER; CRYSTAL AB We combined synchrotron-based infrared spectroscopy, Raman scattering, and diamond anvil cell techniques with complementary lattice dynamics calculations to reveal local lattice distortions in Mn[N(CN)(2)](2) under compression. Strikingly, we found a series of transitions involving octahedral counter-rotations, changes in the local Mn environment, and deformations of the superexchange pathway. In addition to reinforcing magnetic property trends, these pressure-induced local lattice distortions may provide an avenue for the development of new functionalities. C1 [Brinzari, Tatiana V.; O'Neal, Kenneth R.; Musfeldt, Janice L.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Manson, Jamie L.] Eastern Washington Univ, Dept Chem & Biochem, Cheney, WA 99004 USA. [Schlueter, John A.] Natl Sci Fdn, Div Mat Res, Arlington, VA 22230 USA. [Schlueter, John A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Litvinchuk, Alexander P.] Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. [Litvinchuk, Alexander P.] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Liu, Zhenxian] Carnegie Inst Sci, Geophys Lab, Washington, DC 20015 USA. RP Brinzari, TV; Musfeldt, JL (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. EM tbrinzar@vols.utk.edu; musfeldt@utk.edu RI Litvinchuk, Alexander/K-6991-2012 OI Litvinchuk, Alexander/0000-0002-5128-5232 FU NSF [DMR-1063880, DMR-1306158]; PRF [52053-ND10]; DOE; State of Texas via the Texas Center for Superconductivity; Independent Research/Development Program at the National Science Foundation; COMPRES under NSF [EAR 06-49658] FX This research was supported by the NSF (DMR-1063880, UT and DMR-1306158, EWU), the PRF (52053-ND10, UT), the DOE (BNL, ANL), and the State of Texas via the Texas Center for Superconductivity (A.P.L., UH). The U2A beamline is supported by COMPRES under NSF Cooperative Agreement EAR 06-49658. J.A.S. acknowledges support from the Independent Research/Development Program while serving at the National Science Foundation. We thank Chunli Ma for assistance with experiments and Mark Meisel for useful discussions. NR 44 TC 2 Z9 2 U1 7 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAR 7 PY 2016 VL 55 IS 5 BP 1956 EP 1961 DI 10.1021/acs.inorgchem.5b01870 PG 6 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DG0KK UT WOS:000371753500002 PM 26863096 ER PT J AU Wang, SC Xie, H Lin, YY Poeppelmeier, KR Li, T Winans, RE Cui, YR Ribeiro, FH Canlas, CP Elam, JW Zhang, HB Marshall, CL AF Wang, Shichao Xie, Hong Lin, Yuyuan Poeppelmeier, Kenneth R. Li, Tao Winans, Randall E. Cui, Yanran Ribeiro, Fabio H. Canlas, Christian P. Elam, Jeffrey W. Zhang, Hongbo Marshall, Christopher L. TI High Thermal Stability of La2O3- and CeO2-Stabilized Tetragonal ZrO2 SO INORGANIC CHEMISTRY LA English DT Article ID WATER-GAS-SHIFT; ATOMIC LAYER DEPOSITION; X-RAY-ABSORPTION; MONOCLINIC PHASE-TRANSFORMATION; SOLID-SOLUTIONS; ZIRCONIA STABILIZATION; HYDROTHERMAL SYNTHESIS; BUTANE ISOMERIZATION; ACTIVE-SITES; MIXED OXIDES AB Catalyst support materials of tetragonal ZrO2, stabilized by either La2O3 (La2O3-ZrO2) or CeO2 (CeO2-ZrO2), were synthesized under hydrothermal conditions at 200 degrees C with NH4OH or tetramethylammonium hydroxide as the mineralizer. From in situ synchrotron powder X-ray diffraction and small-angle X-ray scattering measurements, the calcined La2O3-ZrO2 and CeO2-ZrO2 supports were nonporous nanocrystallites that exhibited rectangular shapes with a thermal stability of up to 1000 degrees C in air. These supports had an average size of similar to 10 nm and a surface area of 59-97 m(2)/g. The catalysts Pt/La2O3-ZrO2 and Pt/CeO2-ZrO2 were prepared by using atomic layer deposition with varying Pt loadings from 6.3 to 12.4 wt %. Monodispersed Pt nanoparticles of similar to 3 nm were obtained for these catalysts. The incorporation of La2O3 and CeO2 into the t-ZrO2 structure did not affect the nature of the active sites for the Pt/ZrO2 catalysts for the water-gas shift reaction. C1 [Wang, Shichao; Xie, Hong; Lin, Yuyuan; Poeppelmeier, Kenneth R.] Northwestern Univ, Dept Chem, Ctr Catalysis & Surface Sci, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Li, Tao; Winans, Randall E.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Cui, Yanran; Ribeiro, Fabio H.] Purdue Univ, Sch Chem Engn, 480 Stadium Mall Dr, W Lafayette, IN 47907 USA. [Canlas, Christian P.; Elam, Jeffrey W.] Argonne Natl Lab, Energy Syst Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Zhang, Hongbo; Marshall, Christopher L.] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Poeppelmeier, KR (reprint author), Northwestern Univ, Dept Chem, Ctr Catalysis & Surface Sci, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM krp@northwestern.edu RI Wang, Shichao/K-1973-2013 OI Wang, Shichao/0000-0003-3632-9193 FU Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, U.S. Department of Energy; Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center - U.S. Department of Energy, Office of Basic Energy Sciences; Institute for Catalysis in Energy Processes (ICEP) - Department of Energy/BES/Chemical Sciences/Catalysis Science [DE-FG02-03ER15457]; DOE Office of Science [DE-AC02-06CH11357] FX The work at Argonne National Laboratory was supported by the Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, U.S. Department of Energy (initial research on metal particle synthesis), and the Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Basic Energy Sciences. The work at Northwestern University was supported by the Institute for Catalysis in Energy Processes (ICEP) (DE-FG02-03ER15457) funded by Department of Energy/BES/Chemical Sciences/Catalysis Science. This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract DE-AC02-06CH11357. NR 57 TC 0 Z9 0 U1 5 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAR 7 PY 2016 VL 55 IS 5 BP 2413 EP 2420 DI 10.1021/acs.inorgchem.5b02810 PG 8 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DG0KK UT WOS:000371753500051 PM 26878202 ER PT J AU Jin, GB AF Jin, Geng Bang TI Three-Dimensional Network of Cation Cation-Bound Neptunyl(V) Squares: Synthesis and in Situ Raman Spectroscopy Studies SO INORGANIC CHEMISTRY LA English DT Article ID MAGNETIC-PROPERTIES; NEPTUNIUM(V) SULFATES; PENTAVALENT ACTINIDES; MOLECULAR-STRUCTURE; CRYSTAL-STRUCTURES; INFRARED-SPECTRA; TRANSURANIUM V; ACID SOLUTION; COMPLEXES; NPO2+ AB Cation-cation interactions (CCIs) are an essential feature of actinyl chemistry, particularly neptunyl(V). To better understand the formation mechanisms of CCIs, the crystallization process of Np(V) CCI compounds has been explored during the evaporation of acidic Np(V) stock solutions using X-ray diffraction and both ex situ and in situ Raman spectroscopy. At least four Np solid products have been isolated from evaporation of the same Np(V) acidic solution. In situ evaporation using a continuous wave laser (532 nm) as a local heat source produced similar solid products to ex situ experiments with matching Raman signatures. The formation of these products is highly dependent on the evaporation conditions. Slower evaporation appears to favor the formation of a new neptunyl(V) compound, (NpO2)Cl(H2O)(2) (1), over other solid products. The structure of 1 features a three-dimensional network of NpO2+ cations, where neighboring Np(V) ions are only connected to each other through CCIs in a square arrangement. The O=Np=O stretching region shows similar Raman bands in both the solids and solution suggesting that CCIs between Np(V) cations exist prior to crystallization. These results provide new insight into the formation mechanism of Np(V) CCI compounds from solutions. C1 [Jin, Geng Bang] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Jin, GB (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM gjin@anl.gov FU United States Department of Energy [DE-AC02-06CH11357]; DOE Office of Basic Energy Sciences, Chemical Sciences, Heavy Elements Chemistry FX This work was performed at Argonne National Laboratory, operated by UChicago Argonne LLC for the United States Department of Energy under contract number DE-AC02-06CH11357 and was supported by a DOE Office of Basic Energy Sciences, Chemical Sciences, Heavy Elements Chemistry. NR 55 TC 0 Z9 0 U1 5 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAR 7 PY 2016 VL 55 IS 5 BP 2612 EP 2619 DI 10.1021/acs.morgchem.5b02955 PG 8 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DG0KK UT WOS:000371753500071 PM 26885939 ER PT J AU Chapman, CAR Ly, S Wang, L Seker, E Matthews, MJ AF Chapman, Christopher A. R. Ly, Sonny Wang, Ling Seker, Erkin Matthews, Manyalibo J. TI Utilizing dynamic laser speckle to probe nanoscale morphology evolution in nanoporous gold thin films SO OPTICS EXPRESS LA English DT Article ID NANOPARTICLES; FABRICATION; SIZE AB This paper demonstrates the use of dynamic laser speckle autocorrelation spectroscopy in conjunction with the photothermal treatment of nanoporous gold (np-Au) thin films to probe nanoscale morphology changes during the photothermal treatment. Utilizing this spectroscopy method, backscattered speckle from the incident laser is tracked during photothermal treatment and both the characteristic feature size and annealing time of the film are determined. These results demonstrate that this method can successfully be used to monitor laser-dbased surface modification processes without the use of ex-situ characterization. (C) 2016 Optical Society of America C1 [Chapman, Christopher A. R.] Univ Calif Davis, Dept Biomed Engn, Davis, CA 95616 USA. [Ly, Sonny; Matthews, Manyalibo J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Wang, Ling; Seker, Erkin] Univ Calif Davis, Dept Elect Engn, Davis, CA 95616 USA. RP Matthews, MJ (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM ibo@llnl.gov OI Seker, Erkin/0000-0003-2401-3562 FU UC Lab Fees Research Program Award [12-LR-237197]; National Science Foundation [CBET-1512745, CBET-DMR-1454426, DGE-1148897]; Laboratory Directed Research and Development grant [15-ERD-037]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Gabe Guss regarding both LabVIEW FX We gratefully acknowledge the help and support of Gabe Guss regarding both LabVIEW and high-speed camera set-up. Additionally, we acknowledge the support from UC Lab Fees Research Program Award (12-LR-237197) and National Science Foundation Awards (CBET-1512745 and CBET-DMR-1454426). C. Chapman was supported by a National Science Foundation Research Fellowship (DGE-1148897). Any opinion, findings, and conclusions or recommendations expressed in the material are those of the author(s) and do not necessarily reflect the views of the National Science Foundation. Work at LLNL was funded through a Laboratory Directed Research and Development grant (15-ERD-037) and performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. NR 25 TC 1 Z9 1 U1 4 U2 9 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD MAR 7 PY 2016 VL 24 IS 5 BP 5323 EP 5333 DI 10.1364/OE.24.005323 PG 11 WC Optics SC Optics GA DF5ZZ UT WOS:000371435000094 ER PT J AU Carbone, C Moras, P Sheverdyaeva, PM Pacile, D Papagno, M Ferrari, L Topwal, D Vescovo, E Bihlmayer, G Freimuth, F Mokrousov, Y Blugel, S AF Carbone, C. Moras, P. Sheverdyaeva, P. M. Pacile, D. Papagno, M. Ferrari, L. Topwal, D. Vescovo, E. Bihlmayer, G. Freimuth, F. Mokrousov, Y. Bluegel, S. TI Asymmetric band gaps in a Rashba film system SO PHYSICAL REVIEW B LA English DT Article ID PLANE-WAVE METHOD; SURFACE; MAGNETIZATION; SYMMETRY AB The joint effect of exchange and Rashba spin-orbit interactions is examined on the surface and quantum well states of Ag2Bi-terminated Ag films grown on ferromagnetic Fe(110). The system displays a particular combination of time-reversal and translational symmetry breaking that strongly influences its electronic structure. Angle-resolved photoemission reveals asymmetric band-gap openings, due to spin-selective hybridization between Rashba-split surface states and exchange-split quantum well states. This results in an unequal number of states along positive and negative reciprocal space directions. We suggest that the peculiar asymmetry of the discovered electronic structure can have significant influence on spin-polarized transport properties. C1 [Carbone, C.; Moras, P.; Sheverdyaeva, P. M.; Pacile, D.; Papagno, M.] CNR, Ist Struttura Mat, I-34149 Trieste, Italy. [Pacile, D.; Papagno, M.] Univ Calabria, Dipartimento Fis, I-87030 Arcavacata Di Rende, Italy. [Ferrari, L.] CNR, Ist Sistemi Complessi, I-00185 Rome, Italy. [Topwal, D.] Abdus Salaam Int Ctr Theoret Phys, I-34151 Trieste, Italy. [Topwal, D.] Inst Phys, Sachivalaya Marg, Bhubaneswar 751005, Orissa, India. [Vescovo, E.] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. [Bihlmayer, G.; Freimuth, F.; Mokrousov, Y.; Bluegel, S.] Forschungszentrum Julich, Peter Grunberg Inst, D-52425 Julich, Germany. [Bihlmayer, G.; Freimuth, F.; Mokrousov, Y.; Bluegel, S.] Forschungszentrum Julich, Inst Adv Simulat, D-52425 Julich, Germany. [Bihlmayer, G.; Freimuth, F.; Mokrousov, Y.; Bluegel, S.] JARA, D-52425 Julich, Germany. RP Carbone, C (reprint author), CNR, Ist Struttura Mat, I-34149 Trieste, Italy. EM carlo.carbone@trieste.ism.cnr.it RI Bihlmayer, Gustav/G-5279-2013 OI Bihlmayer, Gustav/0000-0002-6615-1122 FU Helmholtz Association (HGF) Programme [VH-NG513]; German Research Foundation (DFG) [SPP 1538] FX We gratefully acknowledge computing time at the JUROPA supercomputer from the Julich Supercomputing Centre and financial support from the Helmholtz Association (HGF) Programme VH-NG513 and German Research Foundation (DFG) SPP 1538. We acknowledge the "Progetto Premiale, Materiali e Dispositivi Magnetici e Superconduttivi per Sensoristica e ICT" of the Italian Ministry of Education, University and Research (MIUR). NR 33 TC 1 Z9 1 U1 3 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 7 PY 2016 VL 93 IS 12 AR 125409 DI 10.1103/PhysRevB.93.125409 PG 8 WC Physics, Condensed Matter SC Physics GA DG0EW UT WOS:000371738000004 ER PT J AU Choi, HC Lin, SZ Zhu, JX AF Choi, Hong Chul Lin, Shi-Zeng Zhu, Jian-Xin TI Density functional theory study of skyrmion pinning by atomic defects in MnSi SO PHYSICAL REVIEW B LA English DT Article ID ANISOTROPIC SUPEREXCHANGE INTERACTION; WEAK FERROMAGNETISM; CHIRAL MAGNETS; TEMPERATURE; CRYSTALS; MOTION AB A magnetic skyrmion observed experimentally in chiral magnets is a topologically protected spin texture. For their unique properties, such as high mobility under current drive, skyrmions have a huge potential for applications in next-generation spintronic devices. Defects naturally occurring in magnets have profound effects on the static and dynamical properties of skyrmions. In this work we study the effect of an atomic defect on a skyrmion by performing the first-principles calculations within the density functional theory, taking MnSi as an example. By substituting one site of Mn or Si with different elements, we can tune the pinning energy. The effects of pinning by an atomic defect can be understood qualitatively within a phenomenological model. C1 [Choi, Hong Chul; Lin, Shi-Zeng; Zhu, Jian-Xin] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Zhu, Jian-Xin] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, POB 1663, Los Alamos, NM 87545 USA. RP Choi, HC (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RI Lin, Shi-Zeng/B-2906-2008 OI Lin, Shi-Zeng/0000-0002-4368-5244 FU National Nuclear Security Administration of the US DOE at LANL [DE-AC52-06NA25396]; LANL LDRD-DR Program FX We thank Yuan-Yen Tai for helpful discussions. This work was carried out under the auspices of the National Nuclear Security Administration of the US DOE at LANL under Contract No. DE-AC52-06NA25396 and was supported by the LANL LDRD-DR Program. NR 29 TC 0 Z9 0 U1 6 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 7 PY 2016 VL 93 IS 11 AR 115112 DI 10.1103/PhysRevB.93.115112 PG 6 WC Physics, Condensed Matter SC Physics GA DG0DS UT WOS:000371733800001 ER PT J AU Hallas, AM Gaudet, J Wilson, MN Munsie, TJ Aczel, AA Stone, MB Freitas, RS Arevalo-Lopez, AM Attfield, JP Tachibana, M Wiebe, CR Luke, GM Gaulin, BD AF Hallas, A. M. Gaudet, J. Wilson, M. N. Munsie, T. J. Aczel, A. A. Stone, M. B. Freitas, R. S. Arevalo-Lopez, A. M. Attfield, J. P. Tachibana, M. Wiebe, C. R. Luke, G. M. Gaulin, B. D. TI XY antiferromagnetic ground state in the effective S=1/2 pyrochlore Yb2Ge2O7 SO PHYSICAL REVIEW B LA English DT Article ID MUON-SPIN RELAXATION; CRYSTAL-FIELD; YB2TI2O7; TRANSITION; ER2TI2O7; MAGNETS AB We report neutron scattering and muon spin relaxation measurements (mu SR) on the pyrochlore antiferromagnet Yb2Ge2O7. Inelastic neutron scattering was used to probe the transitions between crystal electric field levels, allowing us to determine the eigenvalues and eigenvectors appropriate to the J = 7/2 Yb3+ ion in this environment. The crystal electric field ground state doublet in Yb2Ge2O7 corresponds primarily to m(J) = +/- 1/2 with local XY anisotropy, consistent with an S-eff = 1/2 description for the Yb moments. mu SR measurements reveal the presence of an ordering transition at T-N = 0.57 K with persistent weak dynamics in the ordered state. Finally, we present neutron diffraction measurements that reveal a clear phase transition to the k = (000) Gamma(5) ground state with an ordered magnetic moment of 0.3(1)mu(B) per Yb ion. We compare and contrast this phenomenology with the low-temperature behavior of Yb2Ti2O7 and Er2Ti2O7, the prototypical S-eff = 1/2 XY pyrochlore magnets. C1 [Hallas, A. M.; Gaudet, J.; Wilson, M. N.; Munsie, T. J.; Luke, G. M.; Gaulin, B. D.] McMaster Univ, Dept Phys & Astron, Hamilton, ON L8S 4M1, Canada. [Aczel, A. A.; Stone, M. B.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Freitas, R. S.] Univ Sao Paulo, Inst Fis, BR-05315970 Sao Paulo, SP, Brazil. [Arevalo-Lopez, A. M.; Attfield, J. P.] Univ Edinburgh, Ctr Sci Extreme Condit, Peter Guthrie Tait Rd,Kings Bldg, Edinburgh EH9 3FD, Midlothian, Scotland. [Arevalo-Lopez, A. M.; Attfield, J. P.] Univ Edinburgh, Sch Chem, Peter Guthrie Tait Rd,Kings Bldg, Edinburgh EH9 3FD, Midlothian, Scotland. [Tachibana, M.] Natl Inst Mat Sci, 1-1 Namiki, Tsukuba, Ibaraki 3050044, Japan. [Wiebe, C. R.] Univ Winnipeg, Dept Chem, Winnipeg, MB R3B 2E9, Canada. [Wiebe, C. R.; Luke, G. M.; Gaulin, B. D.] Canadian Inst Adv Res, 180 Dundas St West, Toronto, ON M5G 1Z7, Canada. [Gaulin, B. D.] Brockhouse Inst Mat Res, Hamilton, ON L8S 4M1, Canada. RP Gaulin, BD (reprint author), McMaster Univ, Dept Phys & Astron, Hamilton, ON L8S 4M1, Canada.; Gaulin, BD (reprint author), Canadian Inst Adv Res, 180 Dundas St West, Toronto, ON M5G 1Z7, Canada.; Gaulin, BD (reprint author), Brockhouse Inst Mat Res, Hamilton, ON L8S 4M1, Canada. EM gaulin@physics.mcmaster.ca RI Stone, Matthew/G-3275-2011; Freitas, Rafael/K-1034-2013; Luke, Graeme/A-9094-2010; Arevalo-Lopez, Angel/C-5597-2013; TACHIBANA, Makoto/H-2794-2011; OI Stone, Matthew/0000-0001-7884-9715; Freitas, Rafael/0000-0002-0225-6195 FU Vanier Canada Graduate Scholarship Program; National Institute for Materials Science (NIMS); Natural Sciences and Engineering Research Council of Canada; Canada Foundation for Innovation; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; EPSRC; Royal Society; CNPq [400278/2012-0] FX We acknowledge useful conversations with M.J.P. Gingras and J. Rau. We appreciate the hospitality of the TRIUMF Centre for Molecular and Materials Science and thank B.S. Hitti, G.D. Morris, and D.J. Arseneau for assistance with the mu SR measurements. A.M.H. acknowledges support from the Vanier Canada Graduate Scholarship Program and thanks the National Institute for Materials Science (NIMS) for their hospitality and support through the NIMS Internship Program. This work was supported by the Natural Sciences and Engineering Research Council of Canada and the Canada Foundation for Innovation. The research at HFIR and SNS, ORNL, was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Work at the University of Edinburgh was supported by EPSRC and the Royal Society. R.S.F. acknowledges support from CNPq (Grant No. 400278/2012-0). NR 63 TC 4 Z9 4 U1 9 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 7 PY 2016 VL 93 IS 10 AR 104405 DI 10.1103/PhysRevB.93.104405 PG 9 WC Physics, Condensed Matter SC Physics GA DG0DF UT WOS:000371732000003 ER PT J AU Heinonen, O Jiang, WJ Somaily, H te Velthuis, SGE Hoffmann, A AF Heinonen, Olle Jiang, Wanjun Somaily, Hamoud te Velthuis, Suzanne G. E. Hoffmann, Axel TI Generation of magnetic skyrmion bubbles by inhomogeneous spin Hall currents SO PHYSICAL REVIEW B LA English DT Article ID WEAK FERROMAGNETISM; DOMAIN-WALLS; TEMPERATURE; FILMS AB Recent experiments have shown that magnetic skyrmion bubbles can be generated and injected at room temperature in thin films [W. Jiang et al., Science 349, 283 (2015)]. Here, we demonstrate, using micromagnetic modeling, that such skyrmions can be generated by an inhomogeneous spin Hall torque in the presence of Dzyaloshinskii-Moriya interactions (DMIs). In the experimental Ta/Co20Fe60B20 thin films, the DMI is rather small; nevertheless, the skyrmion bubbles are stable, or at least metastable on observational time scales. C1 [Heinonen, Olle; Jiang, Wanjun; Somaily, Hamoud; te Velthuis, Suzanne G. E.; Hoffmann, Axel] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. [Heinonen, Olle] Northwestern Argonne Inst Sci & Engn, Evanston, IL 60208 USA. [Somaily, Hamoud] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. RP Heinonen, O (reprint author), Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA.; Heinonen, O (reprint author), Northwestern Argonne Inst Sci & Engn, Evanston, IL 60208 USA. RI te Velthuis, Suzanne/I-6735-2013; Jiang, Wanjun/E-6994-2011; OI te Velthuis, Suzanne/0000-0002-1023-8384; Jiang, Wanjun/0000-0003-0918-3862; Heinonen, Olle/0000-0002-3618-6092 FU Department of Energy, Office of Science, Basic Energy Sciences Materials Science and Engineering Division FX This work was supported by the Department of Energy, Office of Science, Basic Energy Sciences Materials Science and Engineering Division. We gratefully acknowledge the computing resources provided on Blues, a high-performance computing cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory. NR 34 TC 3 Z9 3 U1 9 U2 31 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 7 PY 2016 VL 93 IS 9 AR 094407 DI 10.1103/PhysRevB.93.094407 PG 6 WC Physics, Condensed Matter SC Physics GA DG0BQ UT WOS:000371727300003 ER PT J AU Jeon, I Huang, K Yazici, D Kanchanavatee, N White, BD Ho, PC Jang, S Pouse, N Maple, MB AF Jeon, I. Huang, K. Yazici, D. Kanchanavatee, N. White, B. D. Ho, P. -C. Jang, S. Pouse, N. Maple, M. B. TI Investigation of superconducting and normal-state properties of the filled-skutterudite system PrPt4Ge12-xSbx SO PHYSICAL REVIEW B LA English DT Article ID CORRELATED ELECTRON PHENOMENA; TEMPERATURE; TRANSITION; LA; PR(OS1-XRUX)(4)SB-12; ANTIMONIDES; DEPENDENCE; PRESSURE; BEHAVIOR; CRYSTAL AB We report a study of the superconducting and normal-state properties of the filled-skutterudite system PrPt4Ge12-xSbx. Polycrystalline samples with Sb concentrations up to x = 5 were synthesized and investigated by means of x-ray diffraction, electrical resistivity, magnetic susceptibility, and specific heat measurements. We observed a suppression of superconductivity with increasing Sb substitution up to x = 4, above which no signature of superconductivity was observed down to 140 mK. The Sommerfeld coefficient, gamma, of superconducting specimens decreases with increasing x up to x = 3, suggesting that superconductivity may depend on the density of electronic states in this system. The specific heat for x = 0.5 exhibits an exponential temperature dependence in the superconducting state, reminiscent of a nodeless superconducting energy gap. We observed evidence for a weak "rattling" mode associated with the Pr ions, characterized by an Einstein temperature Theta(E) similar to 60 K for 0 <= x <= 5; however, the rattling mode may not play any role in suppressing superconductivity. C1 [Jeon, I.; Huang, K.; Jang, S.; Maple, M. B.] Univ Calif San Diego, Mat Sci & Engn Program, La Jolla, CA 92093 USA. [Jeon, I.; Huang, K.; Yazici, D.; Kanchanavatee, N.; White, B. D.; Jang, S.; Pouse, N.; Maple, M. B.] Univ Calif San Diego, Ctr Adv Nanosci, La Jolla, CA 92093 USA. [Yazici, D.; Kanchanavatee, N.; White, B. D.; Pouse, N.; Maple, M. B.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Ho, P. -C.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Huang, K.] Fudan Univ, Dept Phys, State Key Lab Surface Phys, Shanghai 200433, Peoples R China. [Yazici, D.] Artvin Coruh Univ, Fac Hlth Sci, TR-08100 Artvin, Turkey. [Kanchanavatee, N.] Chulalongkorn Univ, Dept Phys, Fac Sci, Bangkok 10330, Thailand. [White, B. D.] Cent Washington Univ, Dept Phys, 400 East Univ Way, Ellensburg, WA 98926 USA. [Jang, S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Maple, MB (reprint author), Univ Calif San Diego, Mat Sci & Engn Program, La Jolla, CA 92093 USA.; Maple, MB (reprint author), Univ Calif San Diego, Ctr Adv Nanosci, La Jolla, CA 92093 USA.; Maple, MB (reprint author), Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. EM mbmaple@ucsd.edu FU US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-FG02-04-ER46105]; National Science Foundation [DMR 1206553] FX This work was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under Grant No. DE-FG02-04-ER46105 (characterization and physical properties measurements), and the National Science Foundation under Grant No. DMR 1206553 (low-temperature measurements). Helpful discussions with S. Ran are gratefully acknowledged. NR 64 TC 3 Z9 3 U1 3 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 7 PY 2016 VL 93 IS 10 AR 104507 DI 10.1103/PhysRevB.93.104507 PG 10 WC Physics, Condensed Matter SC Physics GA DG0DF UT WOS:000371732000006 ER PT J AU Mun, E Weickert, F Kim, J Scott, BL Miclea, CF Movshovich, R Wilcox, J Manson, J Zapf, VS AF Mun, Eundeok Weickert, Franziska Kim, Jaewook Scott, Brian L. Miclea, Corneliu Florin Movshovich, Roman Wilcox, Jason Manson, Jamie Zapf, Vivien S. TI Partially disordered antiferromagnetism and multiferroic behavior in a frustrated Ising system CoCl2-2SC(NH2)(2) SO PHYSICAL REVIEW B LA English DT Article ID HIGH-FIELD MAGNETIZATION; NEUTRON-DIFFRACTION; TRIANGULAR LATTICE; DEVILS STAIRCASE; CRYSTAL AB We investigate partially disordered antiferromagnetism in CoCl2-2SC(NH2)(2), in which ab-plane hexagonal layers are staggered along the c axis rather than stacked. A robust 1/3 state forms in applied magnetic fields in which the spins are locked, varying as a function of neither temperature nor field. By contrast, in zero field and applied fields at higher temperatures, partial antiferromagnetic order occurs, in which free spins are available to create a Curie-like magnetic susceptibility. We report measurements of the crystallographic structure and the specific heat, magnetization, and electric polarization down to T = 50 mK and up to mu H-0 = 60 T. The Co2+ S = 3/2 spins are Ising-like and form distorted hexagonal layers. The Ising energy scale is well separated from the magnetic exchange, and both energy scales are accessible to the measurements, allowing us to cleanly parametrize them. In transverse fields, a quantum Ising phase transition can be observed at 2 T. Finally, we find that magnetic exchange striction induces changes in the electric polarization up to 3 mu C/m(2), and single-ion magnetic anisotropy effects induce a much larger electric polarization change of 300 mu C/m(2). C1 [Mun, Eundeok; Kim, Jaewook; Zapf, Vivien S.] Los Alamos Natl Lab, Natl High Magnet Field Lab, Mat Phys & Applicat Condensed Matter & Magnet Sci, POB 1663, Los Alamos, NM 87545 USA. [Weickert, Franziska; Miclea, Corneliu Florin; Movshovich, Roman] Los Alamos Natl Lab, Mat Phys & Applicat Condensed Matter & Magnet Sci, POB 1663, Los Alamos, NM 87545 USA. [Scott, Brian L.] Los Alamos Natl Lab, Mat Phys & Applicat 11, POB 1663, Los Alamos, NM 87545 USA. [Wilcox, Jason; Manson, Jamie] Eastern Washington Univ, Dept Chem & Biochem, Cheney, WA 99004 USA. [Mun, Eundeok] Simon Frazer Univ, Burnaby, BC V5A 1S6, Canada. [Kim, Jaewook] Rutgers Ctr Emergent Mat, Piscataway, NJ 08854 USA. [Miclea, Corneliu Florin] Natl Inst Mat Phys, Bucharest 077125, Romania. RP Mun, E (reprint author), Simon Frazer Univ, Burnaby, BC V5A 1S6, Canada. RI Scott, Brian/D-8995-2017 OI Scott, Brian/0000-0003-0468-5396 FU Laboratory Directed Research and Development program; U.S. National Science Foundation [DMR-1157490, DMR-1306158]; State of Florida; U.S. Department of Energy FX We thank C. D. Batista and R. D. McDonald for valuable discussions. The work at Los Alamos National Lab was supported by the Laboratory Directed Research and Development program. The National High Magnetic Field Laboratory facility is funded by the U.S. National Science Foundation through Cooperative Grant No. DMR-1157490, the State of Florida, and the U.S. Department of Energy. The crystal design and growth at Eastern Washington University was supported by the U.S. National Science Foundation under Grant No. DMR-1306158. NR 44 TC 1 Z9 1 U1 2 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. 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Aidala, C. Ajitanand, N. N. Akiba, Y. Akimoto, R. Alexander, J. Alfred, M. Aoki, K. Apadula, N. Aramaki, Y. Asano, H. Aschenauer, E. C. Atomssa, E. T. Awes, T. C. Azmoun, B. Babintsev, V. Bai, M. Bandara, N. S. Bannier, B. Barish, K. N. Bassalleck, B. Bathe, S. Baublis, V. Baumgart, S. Bazilevsky, A. Beaumier, M. Beckman, S. Belmont, R. Berdnikov, A. Berdnikov, Y. Black, D. Blau, D. S. Bok, J. S. Boyle, K. Brooks, M. L. Bryslawskyj, J. Buesching, H. Bumazhnov, V. Butsyk, S. Campbell, S. Chen, C. -H. Chi, C. Y. Chiu, M. Choi, I. J. Choi, J. B. Choi, S. Choudhury, R. K. Christiansen, P. Chujo, T. Chvala, O. . Cianciolo, V. Citron, Z. Cole, B. A. Connors, M. Cronin, N. Crossette, N. Csanad, M. Csoergo, T. Dairaku, S. Danley, T. W. Datta, A. Daugherity, M. S. David, G. DeBlasio, K. Dehmelt, K. Denisov, A. Deshpande, A. Desmond, E. J. Dietzsch, O. Ding, L. Dion, A. Diss, P. B. Do, J. H. Donadelli, M. D'Orazio, L. Drapier, O. Drees, A. Drees, K. A. Durham, J. M. Durum, A. Edwards, S. 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Moon, H. J. Moon, T. Morrison, D. P. Moskowitz, M. Moukhanova, T. V. Murakami, T. Murata, J. Mwai, A. Nagae, T. Nagamiya, S. Nagashima, K. Nagle, J. L. Nagy, M. I. Nakagawa, I. Nakagomi, H. Nakamiya, Y. Nakamura, K. R. Nakamura, T. Nakano, K. Nattrass, C. Netrakanti, P. K. Nihashi, M. Niida, T. Nishimura, S. Nouicer, R. Novak, T. Novitzky, N. Nukariya, A. Nyanin, A. S. Obayashi, H. O'Brien, E. Ogilvie, C. A. Okada, K. Koop, J. D. Orjuela Osborn, J. D. Oskarsson, A. Ozawa, K. Pak, R. Pantuev, V. Papavassiliou, V. Park, I. H. Park, J. S. Park, S. Park, S. K. Pate, S. F. Patel, L. Patel, M. Pei, H. Peng, J. -C. Perepelitsa, D. V. Perera, G. D. N. Peressounko, D. Yu. Perry, J. Petti, R. Pinkenburg, C. Pinson, R. Pisani, R. P. Purschke, M. L. Qu, H. Rak, J. Ramson, B. J. Ravinovich, I. Read, K. F. Reynolds, D. Riabov, V. Riabov, Y. Richardson, E. Rinn, T. Riveli, N. Roach, D. Roche, G. Rolnick, S. D. Rosati, M. Rowan, Z. Rubin, J. G. Ryu, M. S. Sahlmueller, B. Saito, N. Sakaguchi, T. Sako, H. Samsonov, V. Sarsour, M. Sato, S. Sawada, S. Schaefer, B. Schmoll, B. K. Sedgwick, K. Seidl, R. Sen, A. Seto, R. Sett, P. Sexton, A. Sharma, D. Shein, I. Shibata, T. -A. Shigaki, K. Shimomura, M. Shoji, K. Shukla, P. Sickles, A. Silva, C. L. Silvermyr, D. Sim, K. S. Singh, B. K. Singh, C. P. Singh, V. Skolnik, M. Slunecka, M. Snowball, M. Solano, S. Soltz, R. A. Sondheim, W. E. Sorensen, S. P. Sourikova, I. V. Stankus, P. W. Steinberg, P. Stenlund, E. Stepanov, M. Ster, A. Stoll, S. P. Sugitate, T. Sukhanov, A. Sumita, T. Sun, J. Sziklai, J. Takagui, E. M. Takahara, A. Taketani, A. Tanaka, Y. Taneja, S. Tanida, K. Tannenbaum, M. J. Tarafdar, S. Taranenko, A. Tennant, E. Tieulent, R. Timilsina, A. Todoroki, T. Tomasek, M. Torii, H. Towel, C. L. Towel, R. Towel, R. S. Tserruya, I. Tsuchimoto, Y. Vale, C. van Hecke, H. W. Vargyas, M. Vazquez-Zambrano, E. Veicht, A. Velkovska, J. Vertesi, R. Virius, M. Voas, B. Vrba, V. Vznuzdaev, E. Wang, X. R. Watanabe, D. Watanabe, K. Watanabe, Y. Watanabe, Y. S. Wei, F. Whitaker, S. White, A. S. White, S. N. Winter, D. Wolin, S. Woody, C. L. Wysocki, M. Xia, B. Xue, L. Yalcin, S. Yamaguchi, Y. L. Yanovich, A. Yin, J. Yokkaichi, S. Yoo, J. H. Yoon, I. You, Z. Younus, I. Yu, H. Yushmanov, I. E. Zajc, W. A. Zelenski, A. Zhou, S. Zou, L. TI Single electron yields from semileptonic charm and bottom hadron decays in Au plus Au collisions at root s(NN)=200 GeV SO PHYSICAL REVIEW C LA English DT Article ID NUCLEUS-NUCLEUS COLLISIONS; HEAVY-ION COLLISIONS; QUARK ENERGY-LOSS; QCD MATTER; FLAVOR; COLLABORATION; DETECTOR; FLOW; QGP AB The PHENIX Collaboration at the Relativistic Heavy Ion Collider has measured open heavy flavor production in minimum bias Au + Au collisions at root s(NN) = 200 GeV via the yields of electrons from semileptonic decays of charm and bottom hadrons. Previous heavy flavor electron measurements indicated substantial modification in the momentum distribution of the parent heavy quarks owing to the quark-gluon plasma created in these collisions. For the first time, using the PHENIX silicon vertex detector to measure precision displaced tracking, the relative contributions from charm and bottom hadrons to these electrons as a function of transverse momentum are measured in Au + Au collisions. We compare the fraction of electrons from bottom hadrons to previously published results extracted from electron-hadron correlations in p + p collisions at root s(NN) = 200 GeV and find the fractions to be similar within the large uncertainties on both measurements for p(T) > 4 GeV/c. We use the bottom electron fractions in Au + Au and p + p along with the previously measured heavy flavor electron R-AA to calculate the R-AA for electrons from charm and bottom hadron decays separately. 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R.] Kyoto Univ, Kyoto 6068502, Japan. [Drapier, O.; Fleuret, F.; Gonin, M.; de Cassagnac, R. Granier] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, Route Saclay, F-91128 Palaiseau, France. [Younus, I.] Lahore Univ Management Sci, Dept Phys, Lahore 54792, Pakistan. [Garishvili, I.; Glenn, A.; Levy, L. A. Linden; Soltz, R. A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Aidala, C.; Brooks, M. L.; Durham, J. M.; Jiang, X.; Kapustinsky, J.; Lee, D. M.; Lee, K. B.; Leitch, M. J.; Liu, M. X.; McCumber, M.; McGaughey, P. L.; Silva, C. L.; Snowball, M.; Sondheim, W. E.; van Hecke, H. W.; You, Z.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Roche, G.] Univ Blaise Pascal, LPC, CNRS, IN2P3, F-63177 Aubiere, France. [Christiansen, P.; Oskarsson, A.; Silvermyr, D.; Stenlund, E.] Lund Univ, Dept Phys, Box 118, SE-22100 Lund, Sweden. [Diss, P. B.; D'Orazio, L.; Mignerey, A. C.; Richardson, E.; Sexton, A.] Univ Maryland, College Pk, MD 20742 USA. [Bandara, N. S.; Datta, A.; Kawal, D.; Stepanov, M.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Aidala, C.; Belmont, R.; Osborn, J. D.; Ramson, B. J.; Rubin, J. G.; White, A. S.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Cronin, N.; Crossette, N.; Fadem, B.; Isinhue, A.; Kimelman, B.; Moskowitz, M.; Skolnik, M.; Solano, S.] Muhlenberg Coll, Allentown, PA 18104 USA. [Joo, K. S.; Moon, H. J.] Myongji Univ, Yongin 449728, Kyonggido, South Korea. [Fusayasu, T.; Tanaka, Y.] Nagasaki Inst Appl Sci, Nagasaki shi, Nagasaki 8510193, Japan. [Chvala, O. .; Shimomura, M.] Nara Womens Univ, Kita Uoya Nishi Machi, Nara 6308506, Japan. [Riabov, V.; Samsonov, V.; Taranenko, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst, MEPhI, Moscow 115409, Russia. [Bassalleck, B.; Bok, J. S.; Butsyk, S.; Datta, A.; DeBlasio, K.; Fields, D. E.; Key, J. A.; Younus, I.] Univ New Mexico, Albuquerque, NM 87131 USA. [Bok, J. S.; Kyle, G. S.; Meles, A.; Papavassiliou, V.; Pate, S. F.; Perera, G. D. N.; Tennant, E.; Wang, X. R.; Wei, F.] New Mexico State Univ, Las Cruces, NM 88003 USA. [Danley, T. W.; Frantz, J. E.; Kotchetkov, D.; Riveli, N.; Xia, B.] Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. [Awes, T. C.; Cianciolo, V.; Efremenko, Y. V.; Enokizono, A.; Read, K. F.; Silvermyr, D.; Stankus, P. W.; Wysocki, M.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Jouan, D.] Univ Paris 11, Univ Paris Saclay, IPN Orsay, CNRS IN2P3, BP1, F-91406 Orsay, France. [Yu, H.] Peking Univ, Beijing 100871, Peoples R China. [Baublis, V.; Ivanishchev, D.; Khanzadeev, A.; Komkov, B.; Kotov, D.; Riabov, V.; Riabov, Y.; Samsonov, V.; Vznuzdaev, E.] Petersburg Nucl Phys Inst, St Petersburg 188300, Russia. [Akiba, Y.; Aoki, K.; Aramaki, Y.; Asano, H.; Baumgart, S.; Dairaku, S.; Enokizono, A.; Fukao, Y.; Goto, Y.; Hachiya, T.; Hashimoto, K.; Ichihara, T.; Ikeda, Y.; Imazu, Y.; Karatsu, K.; Kurita, K.; Kurosawa, M.; Miyasaka, S.; Mizuno, S.; Murakami, T.; Murata, J.; Nagamiya, S.; Nakagawa, I.; Nakagomi, H.; Nakamura, T.; Nakano, K.; Nihashi, M.; Seidl, R.; Shibata, T. -A.; Shoji, K.; Sumita, T.; Taketani, A.; Todoroki, T.; Watanabe, K.; Watanabe, Y.; Yokkaichi, S.] RIKEN, Nishina Ctr Accelerator Based Sci, 2-1 Hirosawa, Wako, Saitama 3510198, Japan. [Akiba, Y.; Bathe, S.; Boyle, K.; Chen, C. -H.; Deshpande, A.; Goto, Y.; Ichihara, T.; Koster, J.; Kurosawa, M.; Nakagawa, I.; Nouicer, R.; Okada, K.; Seidl, R.; Taketani, A.; Tanida, K.; Wang, X. R.; Watanabe, Y.; Yokkaichi, S.] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Enokizono, A.; Hashimoto, K.; Kurita, K.; Murata, J.; Watanabe, K.] Rikkyo Univ, Dept Phys, 3-34-1 Nishi Ikebukuro, Tokyo 1718501, Japan. [Berdnikov, A.; Berdnikov, Y.; Kotov, D.; Riabov, Y.] St Petersburg State Polytech Univ, St Petersburg 195251, Russia. [Dietzsch, O.; Donadelli, M.; Leite, M. A. L.; Takagui, E. M.] Univ Sao Paulo, Inst Fis, Caixa Postal 66318, BR-05315970 Sao Paulo, Brazil. [Choi, S.; Kim, M.; Park, J. S.; Park, S.; Tanida, K.; Yoon, I.] Seoul Natl Univ, Dept Phys & Astron, Seoul 151742, South Korea. [Ajitanand, N. N.; Alexander, J.; Gong, X.; Gu, Y.; Jia, J.; Lacey, R.; Mohapatra, S.; Mwai, A.; Reynolds, D.; Taranenko, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Apadula, N.; Atomssa, E. T.; Bannier, B.; Chen, C. -H.; Citron, Z.; Connors, M.; Cronin, N.; Dehmelt, K.; Deshpande, A.; Dion, A.; Drees, A.; Durham, J. M.; Feege, N.; Fields, D. E.; Gal, C.; Ge, H.; Hanks, J.; Hemmick, T. K.; Jacak, B. V.; Kamin, J.; Khachatryan, V.; Kline, P.; Lee, S. H.; Lewis, B.; Manion, A.; Novitzky, N.; Petti, R.; Sahlmueller, B.; Sharma, D.; Sun, J.; Taneja, S.; Yalcin, S.; Yamaguchi, Y. L.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Garishvili, A.; Nattrass, C.; Read, K. F.; Schmoll, B. K.; Sen, A.; Sorensen, S. P.] Univ Tennessee, Knoxville, TN 37996 USA. [Miyasaka, S.; Nakano, K.; Shibata, T. -A.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 1528551, Japan. [Chujo, T.; Esumi, S.; Horaguchi, T.; Ikeda, Y.; Inaba, M.; Miake, Y.; Mizuno, S.; Nakagomi, H.; Niida, T.; Shimomura, M.; Todoroki, T.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki 305, Japan. [Belmont, R.; Greene, S. V.; Huang, S.; Maguire, C. F.; Roach, D.; Schaefer, B.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Citron, Z.; Makek, M.; Milov, A.; Ravinovich, I.; Sharma, D.; Tarafdar, S.; Tserruya, I.] Weizmann Inst Sci, IL-76100 Rehovot, Israel. [Csoergo, T.; Nagy, M. I.; Novak, T.; Ster, A.; Sziklai, J.; Vertesi, R.] Hungarian Acad Sci Wigner RCP RMKI, Wigner Res Ctr Phys, Inst Particle & Nucl Studies, Budapest 114,POB 49, H-1525 Budapest, Hungary. [Do, J. H.; Kang, J. H.; Kwon, Y.; Lee, S.; Lim, S. H.; Moon, T.] Yonsei Univ, IPAP, Seoul 120749, South Korea. [Makek, M.] Univ Zagreb, Fac Sci, Dept Phys, Bijenicka 32, Zagreb HR-10002, Croatia. RP Morrison, DP (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA.; Nagle, JL (reprint author), Univ Colorado, Boulder, CO 80309 USA. EM morrison@bnl.gov; jamie.nagle@colorado.edu RI Durum, Artur/C-3027-2014; Sen, Abhisek/J-1157-2016; Nattrass, Christine/J-6752-2016; Sorensen, Soren /K-1195-2016; Hayano, Ryugo/F-7889-2012; Yokkaichi, Satoshi/C-6215-2017; Taketani, Atsushi/E-1803-2017 OI Sen, Abhisek/0000-0003-1192-3938; Nattrass, Christine/0000-0002-8768-6468; Sorensen, Soren /0000-0002-5595-5643; Hayano, Ryugo/0000-0002-1214-7806; Taketani, Atsushi/0000-0002-4776-2315 FU Office of Nuclear Physics in the Office of Science of the Department of Energy; National Science Foundation; Abilene Christian University Research Council; Research Foundation of SUNY; Ministry of Education, Culture, Sports, Science, and Technology; Japan Society for the Promotion of Science (Japan); Conselho Nacional de Desenvolvimento Cientifico e Tecnologico; Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (Brazil); Natural Science Foundation of China (People's Republic of China); Croatian Science Foundation (Croatia); Ministry of Science, Education, and Sports (Croatia); Ministry of Education, Youth and Sports (Czech Republic); Centre National de la Recherche Scientifique, Commissariat a l'Energie Atomique (France); Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung (Germany); Deutscher Akademischer Austausch Dienst (Germany); Alexander von Humboldt Stiftung (Germany); National Science Fund, OTKA (Hungary); Karoly Robert University College (Hungary); Ch. Simonyi Fund (Hungary); Department of Atomic Energy (India); Department of Science and Technology (India); Israel Science Foundation (Israel); NRF of the Ministry of Education (Korea); Physics Department, Lahore University of Management Sciences (Pakistan); Ministry of Education and Science (Russia); Russian Academy of Sciences (Russia); Federal Agency of Atomic Energy (Russia); VR (Sweden); Wallenberg Foundation (Sweden); U.S. Civilian Research and Development Foundation for the Independent States of the Former Soviet Union; Hungarian American Enterprise Scholarship Fund; US-Israel Binational Science Foundation FX We thank the staff of the Collider-Accelerator and Physics Departments at Brookhaven National Laboratory and the staff of the other PHENIX participating institutions for their vital contributions. We acknowledge support from the Office of Nuclear Physics in the Office of Science of the Department of Energy, the National Science Foundation, Abilene Christian University Research Council, Research Foundation of SUNY, and Dean of the College of Arts and Sciences, Vanderbilt University (U.S.A.); Ministry of Education, Culture, Sports, Science, and Technology and the Japan Society for the Promotion of Science (Japan); Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (Brazil); Natural Science Foundation of China (People's Republic of China); Croatian Science Foundation and Ministry of Science, Education, and Sports (Croatia); Ministry of Education, Youth and Sports (Czech Republic); Centre National de la Recherche Scientifique, Commissariat a l'Energie Atomique, and Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung, Deutscher Akademischer Austausch Dienst, and Alexander von Humboldt Stiftung (Germany); National Science Fund, OTKA, Karoly Robert University College, and the Ch. Simonyi Fund (Hungary); Department of Atomic Energy and Department of Science and Technology (India); Israel Science Foundation (Israel); Basic Science Research Program through NRF of the Ministry of Education (Korea); Physics Department, Lahore University of Management Sciences (Pakistan); Ministry of Education and Science, Russian Academy of Sciences, Federal Agency of Atomic Energy (Russia); VR and Wallenberg Foundation (Sweden); the U.S. Civilian Research and Development Foundation for the Independent States of the Former Soviet Union, the Hungarian American Enterprise Scholarship Fund, and the US-Israel Binational Science Foundation. NR 71 TC 3 Z9 3 U1 9 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 7 PY 2016 VL 93 IS 3 AR 034904 DI 10.1103/PhysRevC.93.034904 PG 29 WC Physics, Nuclear SC Physics GA DG0FM UT WOS:000371740400007 ER PT J AU Sin, M Capote, R Herman, MW Trkov, A AF Sin, M. Capote, R. Herman, M. W. Trkov, A. TI Extended optical model for fission SO PHYSICAL REVIEW C LA English DT Article ID NEUTRON CROSS-SECTIONS; ACTINIDE NUCLEI; SUBTHRESHOLD FISSION; ROTATIONAL BANDS; DATA LIBRARY; 3RD MINIMUM; BARRIER; ENERGY; U-238; APPROXIMATION AB A comprehensive formalism to calculate fission cross sections based on the extension of the optical model for fission is presented. It can be used for description of nuclear reactions on actinides featuring multi-humped fission barriers with partial absorption in the wells and direct transmission through discrete and continuum fission channels. The formalism describes the gross fluctuations observed in the fission probability due to vibrational resonances, and can be easily implemented in existing statistical reaction model codes. The extended optical model for fission is applied for neutron induced fission cross-section calculations on U-234,U-235,U-238 and Pu-239 targets. A triple-humped fission barrier is used for U-234,U-235(n, f), while a double-humped fission barrier is used for U-238(n, f) and Pu-239(n, f) reactions as predicted by theoretical barrier calculations. The impact of partial damping of class-II/III states, and of direct transmission through discrete and continuum fission channels, is shown to be critical for a proper description of the measured fission cross sections for U-234,U-235,U-238(n, f) reactions. The Pu-239(n, f) reaction can be calculated in the complete damping approximation. Calculated cross sections for U-235,U-238(n, f) and Pu-239(n, f) reactions agree within 3% with the corresponding cross sections derived within the Neutron Standards least-squares fit of available experimental data. The extended optical model for fission can be used for both theoretical fission studies and nuclear data evaluation. C1 [Sin, M.] Univ Bucharest, Fac Phys, Bucharest, Romania. [Capote, R.; Trkov, A.] IAEA, NAPC Nucl Data Sect, A-1400 Vienna, Austria. [Herman, M. W.] Brookhaven Natl Lab, Natl Nucl Data Ctr, New York, NY USA. RP Sin, M (reprint author), Univ Bucharest, Fac Phys, Bucharest, Romania.; Capote, R (reprint author), IAEA, NAPC Nucl Data Sect, A-1400 Vienna, Austria. EM mihaela.sin@g.unibuc.ro; r.capotenoy@iaea.org RI Capote Noy, Roberto/M-1245-2014 OI Capote Noy, Roberto/0000-0002-1799-3438 FU European Commission [FP7-249671, FP7-605203] FX The authors acknowledge Vivian Dimitriou for helpful discussions and provision of some 234U(n, f) experimental data. The work of M. S. was partially supported by the European Commission under ANDES (EURATOM Contract No. FP7-249671) and CHANDA (EURATOM Contract No. FP7-605203). NR 73 TC 2 Z9 2 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 7 PY 2016 VL 93 IS 3 AR 034605 DI 10.1103/PhysRevC.93.034605 PG 13 WC Physics, Nuclear SC Physics GA DG0FM UT WOS:000371740400003 ER PT J AU McKenney, JR Sato, N Melnitchouk, W Ji, CR AF McKenney, J. R. Sato, Nobuo Melnitchouk, W. Ji, Chueng-Ryong TI Pion structure function from leading neutron electroproduction and SU(2) flavor asymmetry SO PHYSICAL REVIEW D LA English DT Article ID DEEP-INELASTIC SCATTERING; NUCLEON-NUCLEON INTERACTION; NN FORM-FACTOR; PARTON DISTRIBUTIONS; DRELL-YAN; CHIRAL-SYMMETRY; GOTTFRIED SUM; MODEL; HERA; SEA AB We examine the efficacy of pion exchange models to simultaneously describe leading neutron electroproduction at HERA and the (d) over bar-(u) over bar flavor asymmetry in the proton. A detailed chi(2) analysis of the ZEUS and H1 cross sections, when combined with constraints on the pion flux from Drell-Yan data, allows regions of applicability of one-pion exchange to be delineated. The analysis disfavors several models of the pion flux used in the literature and yields an improved extraction of the pion structure function and its uncertainties at parton momentum fractions in the pion of 4 x 10(-4) less than or similar to x(pi) less than or similar to 0.05 at a scale of Q(2) = 10 GeV2. Based on the fit results, we provide estimates for leading proton structure functions in upcoming tagged deep-inelastic scattering experiments at Jefferson Lab on the deuteron with forward protons. C1 [McKenney, J. R.; Ji, Chueng-Ryong] N Carolina State Univ, Raleigh, NC 27695 USA. [McKenney, J. R.; Sato, Nobuo; Melnitchouk, W.] Jefferson Lab, Newport News, VA 23606 USA. [McKenney, J. R.] Univ N Carolina, Chapel Hill, NC 27599 USA. RP McKenney, JR (reprint author), N Carolina State Univ, Raleigh, NC 27695 USA.; McKenney, JR (reprint author), Jefferson Lab, Newport News, VA 23606 USA.; McKenney, JR (reprint author), Univ N Carolina, Chapel Hill, NC 27599 USA. FU DOE under Jefferson Science Associates, LLC [DE-AC05-06OR23177]; DOE [DE-FG02-03ER41260]; DOE Science Undergraduate Laboratory Internship Program; JSA Initiatives Fund FX We are grateful to T. J. Hobbs for discussions and collaboration on portions of this work. This work was supported by the DOE Contract No. DE-AC05-06OR23177, under which Jefferson Science Associates, LLC, operates Jefferson Lab; DOE Contract No. DE-FG02-03ER41260; the DOE Science Undergraduate Laboratory Internship Program; and the JSA Initiatives Fund. NR 71 TC 2 Z9 2 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 7 PY 2016 VL 93 IS 5 AR 054011 DI 10.1103/PhysRevD.93.054011 PG 20 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DG0FV UT WOS:000371741500003 ER PT J AU Kumah, DP Dogan, M Ngai, JH Qiu, D Zhang, Z Su, D Specht, ED Ismail-Beigi, S Ahn, CH Walker, FJ AF Kumah, D. P. Dogan, M. Ngai, J. H. Qiu, D. Zhang, Z. Su, D. Specht, E. D. Ismail-Beigi, S. Ahn, C. H. Walker, F. J. TI Engineered Unique Elastic Modes at a BaTiO3/(2 x 1)-G(001) Interface SO PHYSICAL REVIEW LETTERS LA English DT Article ID CRYSTALLINE OXIDES; SILICON; CHARGE; HETEROSTRUCTURES; SURFACE; GROWTH; ORDER; FILMS AB The strong interaction at an interface between a substrate and thin film leads to epitaxy and provides a means of inducing structural changes in the epitaxial film. These induced material phases often exhibit technologically relevant electronic, magnetic, and functional properties. The 2 x 1 surface of a Ge(001) substrate applies a unique type of epitaxial constraint on thin films of the perovskite oxide BaTiO3 where a change in bonding and symmetry at the interface leads to a non-bulk-like crystal structure of the BaTiO3. While the complex crystal structure is predicted using first-principles theory, it is further shown that the details of the structure are a consequence of hidden phases found in the bulk elastic response of the BaTiO3 induced by the symmetry of forces exerted by the germanium substrate. C1 [Kumah, D. P.; Dogan, M.; Ngai, J. H.; Qiu, D.; Ismail-Beigi, S.; Ahn, C. H.; Walker, F. J.] Yale Univ, Ctr Res Interface Struct & Phenomena, New Haven, CT 06520 USA. [Zhang, Z.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Su, D.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Specht, E. D.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Kumah, DP; Walker, FJ (reprint author), Yale Univ, Ctr Res Interface Struct & Phenomena, New Haven, CT 06520 USA. EM dpkumah@ncsu.edu; fred.walker@yale.edu RI Zhang, Zhan/A-9830-2008; Su, Dong/A-8233-2013; Kumah, Divine/A-7031-2011 OI Zhang, Zhan/0000-0002-7618-6134; Su, Dong/0000-0002-1921-6683; Kumah, Divine/0000-0003-0715-1285 FU NSF [MRSEC DMR-1119826, DMR-1309868, CNS 08-21132, TG-MCA08X007]; DOE, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; U.S. Department of Energy, Office of Basic Energy Science [DE-AC02-98CH10886] FX The authors acknowledge support from the NSF under Grants No. MRSEC DMR-1119826 (CRISP) and No. DMR-1309868. Work at the Advanced Photon Source was supported by the DOE, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. Work at Brookhaven was supported by the U.S. Department of Energy, Office of Basic Energy Science, under Contract No. DE-AC02-98CH10886. Computational facilities are supported by NSF Grant No. CNS 08-21132 and by the facilities and staff of the Yale University Faculty of Arts and Sciences High Performance Computing Center. Additional computations are carried out via the NSF TeraGrid and XSEDE resources through Grant No. TG-MCA08X007. NR 46 TC 0 Z9 0 U1 5 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 7 PY 2016 VL 116 IS 10 AR 106101 DI 10.1103/PhysRevLett.116.106101 PG 6 WC Physics, Multidisciplinary SC Physics GA DF9ZM UT WOS:000371721200003 PM 27015492 ER PT J AU Smith, MD Petridis, L Cheng, XL Mostofian, B Smith, JC AF Smith, Micholas Dean Petridis, Loukas Cheng, Xiaolin Mostofian, Barmak Smith, Jeremy C. TI Enhanced sampling simulation analysis of the structure of lignin in the THF-water miscibility gap SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID MOLECULAR-DYNAMICS METHOD; HISTOGRAM ANALYSIS METHOD; LINEAR CONSTRAINT SOLVER; REPLICA-EXCHANGE; LIGNOCELLULOSIC BIOMASS; PHASE-EQUILIBRIA; GROMACS 4.5; TRANSITION; DEPENDENCE; GLOBULE AB Using temperature replica-exchange molecular dynamics, we characterize a globule-to-coil transition for a softwood-like lignin biopolymer in a tetrahydrofuran (THF)-water cosolvent system at temperatures at which the cosolvent undergoes a de-mixing transition. The lignin is found to be in a coil state, similar to that in the high-temperature miscible region. Analysis of the transition kinetics indicates that THF acts in a surfactant-like fashion. The present study thus suggests that THF-water based pretreatments may efficiently remove lignin from biomass even at relatively low (non-water boiling) temperatures. C1 [Smith, Micholas Dean; Petridis, Loukas; Cheng, Xiaolin; Mostofian, Barmak; Smith, Jeremy C.] Univ Tennessee, Oak Ridge Natl Lab, Ctr Biophys Mol, Oak Ridge, TN 37830 USA. [Smith, Micholas Dean; Smith, Jeremy C.] Univ Tennessee, Dept Biochem & Cellular & Mol Biol, M407 Walters Life Sci,1414 Cumberland Ave, Knoxville, TN 37996 USA. [Smith, Micholas Dean; Petridis, Loukas; Cheng, Xiaolin; Mostofian, Barmak; Smith, Jeremy C.] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37830 USA. [Mostofian, Barmak] Univ Tennessee, Oak Ridge Natl Lab, Joint Inst Biol Sci, Oak Ridge, TN 37830 USA. RP Smith, JC (reprint author), Univ Tennessee, Oak Ridge Natl Lab, Ctr Biophys Mol, Oak Ridge, TN 37830 USA.; Smith, JC (reprint author), Univ Tennessee, Dept Biochem & Cellular & Mol Biol, M407 Walters Life Sci,1414 Cumberland Ave, Knoxville, TN 37996 USA.; Smith, JC (reprint author), Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37830 USA. EM smithjc@ornl.gov RI Petridis, Loukas/B-3457-2009; smith, jeremy/B-7287-2012; OI Petridis, Loukas/0000-0001-8569-060X; smith, jeremy/0000-0002-2978-3227; Smith, Micholas/0000-0002-0777-7539 FU BioEnergy Science Center, a U.S. Department of Energy (DOE) Bioenergy Research Center - Office of Biological and Environmental Research in the DOE Office of Science; Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725] FX This work was supported by the BioEnergy Science Center, a U.S. Department of Energy (DOE) Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science. This research used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. This research also used the computing resources provided by the U.S. Department of Energy's National Energy Research Scientific Computing Center. NR 39 TC 1 Z9 1 U1 10 U2 32 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD MAR 7 PY 2016 VL 18 IS 9 BP 6394 EP 6398 DI 10.1039/c5cp07088k PG 5 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DF1ZR UT WOS:000371139400003 PM 26862597 ER PT J AU Ding, Y Wang, ZX Feng, W Marnay, C Zhou, N AF Ding, Yan Wang, Zhaoxia Feng, Wei Marnay, Chris Zhou, Nan TI Influence of occupancy-oriented interior cooling load on building cooling load design SO APPLIED THERMAL ENGINEERING LA English DT Article DE Cooling load; Part load ratio; Occupancy rate; Correction coefficient; Assurance rate ID USER BEHAVIOR; ENERGY; MODEL; SYSTEMS; PERFORMANCE; VENTILATION; RETROFIT; DEMAND AB In the traditional mechanical design of new buildings, the occupancy number is usually over-estimated and results in over-predicted cooling loads and oversized chillers. When building occupancy is low relative to the design phase assumptions, those oversized chillers run inefficiently. To further explore the influence of occupancy on building cooling load design, the occupancy rate of office building is proposed in this paper and investigated with questionnaires. In a case study for an office building in Tianjin, the interior heat gain from occupants, lighting and equipment accounts for 66.6% of the total cooling load, while the part load ratio (PLR) of the chiller is only 30%. A Markov transition matrix is established based on the survey results. This paper describes the occupancy pattern of the building by using a stationary distribution of a one-step transition probability. A correction coefficient is proposed for the design phase cooling load calculation, which results in a 35.9% cooling load reduction for the building case study. The simulated cooling load is validated by consistency check according to the real cooling load. Assurance analysis is also conducted to calculate the design error and predicted operation error between simulated and actual cooling loads. With above analysis, interior disturbances resulting from occupant behavior are proved to be the most important uncertainty for building cooling load design. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Ding, Yan; Wang, Zhaoxia] Tianjin Univ, Tianjin Key Lab Indoor Air Environm Qual Control, Sch Environm Sci & Engn, Tianjin 300072, Peoples R China. [Feng, Wei; Marnay, Chris; Zhou, Nan] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Ding, Y (reprint author), Tianjin Univ, Tianjin Key Lab Indoor Air Environm Qual Control, Sch Environm Sci & Engn, Tianjin 300072, Peoples R China. EM jensxing@126.com FU National Nature Science Foundation of China (NSFC) [51308383] FX Project (51308383) supported by the National Nature Science Foundation of China (NSFC). NR 26 TC 4 Z9 4 U1 1 U2 4 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-4311 J9 APPL THERM ENG JI Appl. Therm. Eng. PD MAR 5 PY 2016 VL 96 BP 411 EP 420 DI 10.1016/j.applthermaleng.2015.11.096 PG 10 WC Thermodynamics; Energy & Fuels; Engineering, Mechanical; Mechanics SC Thermodynamics; Energy & Fuels; Engineering; Mechanics GA DJ0AI UT WOS:000373863400043 ER PT J AU Tian, B Wu, WT Yang, ZQ Zhou, YX AF Tian, Bo Wu, Wenting Yang, Zhaoqing Zhou, Yunxuan TI Drivers, trends, and potential impacts of long-term coastal reclamation in China from 1985 to 2010 SO ESTUARINE COASTAL AND SHELF SCIENCE LA English DT Article DE Coastal reclamation; Urbanization; Coastal economy; Remote sensing; China ID SEA-LEVEL RISE; SHORELINE CHANGES; LAND RECLAMATION; RESTORATION; MANAGEMENT; SHANGHAI; WETLANDS; FACE AB The reclamation of coastal land for agricultural, industrial, and urban land use-a common worldwide practice-has occurred extensively in the coastal region of China. In recent decades, all coastal provinces and metropolises in China have experienced severe coastal reclamation related to land scarcity caused by rapid economic growth and urbanization. However, the value of coastal wetlands and ecosystems has not been well understood and appreciated until recent development of advantageous methods of restoring reclaimed land to coastal wetlands in many developed countries. The overall objective of this study is to provide detailed spatial and temporal distributions of coastal reclamation; analyze drivers such as coastal economy, population growth, and urbanization; and understand the relationships among the drivers and land reclamation. We used long-term Landsat image time series from 1985 to 2010 in 5-year intervals, in combination with remotely sensed image interpretation and spatial analysis, to map the reclamation status and changes across the coastal region of China. The Landsat images time-series analysis was also conducted to evaluate the effects of the economy, population, and urbanization drivers on coastal reclamation. The analysis results indicated that 754,697 ha of coastal wetlands have been reclaimed across all coastal provinces and metropolises from 1985 to 2010, and the trend increased sharply after 2005. High-intensity coastal reclamation was mainly driven by the booming economy, especially after 2000, associated with urbanization and industrial development in China's coastal region; this was closely correlated with the gross domestic product (GDP) per capita. The continuous large-scale coastal reclamation of its coastal region now means China is facing a great challenge, including the enormous loss of vegetated coastal wetlands, negative environmental effects, and potential disaster risks related to coastal flooding under future change climate conditions. Long-term ecosystem-based coastal protection and management are critical to support sustainable coastal ecosystems in China in the future. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Tian, Bo; Wu, Wenting; Zhou, Yunxuan] E China Normal Univ, State Key Lab Estuarine & Coastal Res, Shanghai 200062, Peoples R China. [Yang, Zhaoqing] Pacific NW Natl Lab, Seattle, WA USA. RP Tian, B (reprint author), E China Normal Univ, State Key Lab Estuarine & Coastal Res, Shanghai 200062, Peoples R China. EM btian@sklec.ecnu.edu.cn FU National Natural Science Foundation of China (NSFC) [41371112, 41476151] FX This work was funded by the National Natural Science Foundation of China (NSFC) (41371112, 41476151). We would like to thank Qing Yuan, Xiuzhen Li, Qing He of East China Normal University, China, and Heida L. Diefenderfer, Ronald M. Thom of Pacific Northwest National Laboratory, USA, for providing invaluable assistance over the course of this work and useful suggestions and comments on the original draft of the manuscript. NR 41 TC 8 Z9 9 U1 19 U2 46 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0272-7714 EI 1096-0015 J9 ESTUAR COAST SHELF S JI Estuar. Coast. Shelf Sci. PD MAR 5 PY 2016 VL 170 BP 83 EP 90 DI 10.1016/j.ecss.2016.01.006 PG 8 WC Marine & Freshwater Biology; Oceanography SC Marine & Freshwater Biology; Oceanography GA DG9CH UT WOS:000372379900008 ER PT J AU Lv, C Aitchison, EW Wu, DS Zheng, LQ Cheng, XL Yang, W AF Lv, Chao Aitchison, Erick W. Wu, Dongsheng Zheng, Lianqing Cheng, Xiaolin Yang, Wei TI Comparative Exploration of Hydrogen Sulfide and Water Transmembrane Free Energy Surfaces via Orthogonal Space Tempering Free Energy Sampling SO JOURNAL OF COMPUTATIONAL CHEMISTRY LA English DT Article DE free energy calculation; enhanced sampling; membrane permeation ID MOLECULAR-DYNAMICS SIMULATION; LIPID-BILAYER-MEMBRANES; COMPUTER-SIMULATIONS; RANDOM-WALK; CHARMM; PERMEABILITY; PERMEATION; EFFICIENT; PROGRAM; SYSTEMS AB Hydrogen sulfide (H2S), a commonly known toxic gas compound, possesses unique chemical features that allow this small solute molecule to quickly diffuse through cell membranes. Taking advantage of the recent orthogonal space tempering (OST) method, we comparatively mapped the transmembrane free energy landscapes of H2S and its structural analogue, water (H2O), seeking to decipher the molecular determinants that govern their drastically different permeabilities. As revealed by our OST sampling results, in contrast to the highly polar water solute, hydrogen sulfide is evidently amphipathic, and thus inside membrane is favorably localized at the interfacial region, that is, the interface between the polar head-group and nonpolar acyl chain regions. Because the membrane binding affinity of H2S is mainly governed by its small hydrophobic moiety and the barrier height inbetween the interfacial region and the membrane center is largely determined by its moderate polarity, the transmembrane free energy barriers to encounter by this toxic molecule are very small. Moreover when H2S diffuses from the bulk solution to the membrane center, the above two effects nearly cancel each other, so as to lead to a negligible free energy difference. This study not only explains why H2S can quickly pass through cell membranes but also provides a practical illustration on how to use the OST free energy sampling method to conveniently analyze complex molecular processes. (C) 2015 Wiley Periodicals, Inc. C1 [Lv, Chao; Yang, Wei] Florida State Univ, Dept Chem & Biochem, Tallahassee, FL 32306 USA. [Aitchison, Erick W.; Wu, Dongsheng; Zheng, Lianqing; Yang, Wei] Florida State Univ, Inst Mol Biophys, Tallahassee, FL 32306 USA. [Cheng, Xiaolin] Oak Ridge Natl Lab, UT ORNL Ctr Mol Biophys, Oak Ridge, TN 37830 USA. [Cheng, Xiaolin] Univ Tennessee, Dept Biochem Cellular & Mol Biol, Knoxville, TN 37996 USA. [Lv, Chao] Washington Univ, Campus Box 1134,One Brookings Dr, St Louis, MO 63130 USA. RP Yang, W (reprint author), Florida State Univ, Dept Chem & Biochem, Tallahassee, FL 32306 USA.; Yang, W (reprint author), Florida State Univ, Inst Mol Biophys, Tallahassee, FL 32306 USA. EM yyang2@fsu.edu FU National Science Foundation [MCB1158284] FX Contract grant sponsor: National Science Foundation; Contract grant number: MCB1158284 NR 31 TC 6 Z9 6 U1 4 U2 14 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0192-8651 EI 1096-987X J9 J COMPUT CHEM JI J. Comput. Chem. PD MAR 5 PY 2016 VL 37 IS 6 SI SI BP 567 EP 574 DI 10.1002/jcc.23982 PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA DD9OF UT WOS:000370254600004 PM 26119423 ER PT J AU Helmich, KE Pereira, JH Gall, DL Heins, RA McAndrew, RP Bingman, C Deng, K Holland, KC Noguera, DR Simmons, BA Sale, KL Ralph, J Donohue, TJ Adams, PD Phillips, GN AF Helmich, Kate E. Pereira, Jose Henrique Gall, Daniel L. Heins, Richard A. McAndrew, Ryan P. Bingman, Craig Deng, Kai Holland, Keefe C. Noguera, Daniel R. Simmons, Blake A. Sale, Kenneth L. Ralph, John Donohue, Timothy J. Adams, Paul D. Phillips, George N., Jr. TI Structural Basis of Stereospecificity in the Bacterial Enzymatic Cleavage of beta-Aryl Ether Bonds in Lignin SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article DE enzyme catalysis; enzyme mechanism; enzyme structure; lignin degradation; plant cell wall; protein structure; stereoselectivity; X-ray crystallography; structural enzymology ID GLUTATHIONE-S-TRANSFERASE; SMALL-ANGLE SCATTERING; SP STRAIN SYK-6; 3-DIMENSIONAL STRUCTURE; CRYSTAL-STRUCTURE; EADOCK DSS; PROTEIN; DEGRADATION; REFINEMENT; EVOLUTION AB Lignin is a combinatorial polymer comprising monoaromatic units that are linked via covalent bonds. Although lignin is a potential source of valuable aromatic chemicals, its recalcitrance to chemical or biological digestion presents major obstacles to both the production of second-generation biofuels and the generation of valuable coproducts from lignin's monoaromatic units. Degradation of lignin has been relatively well characterized in fungi, but it is less well understood in bacteria. A catabolic pathway for the enzymatic breakdown of aromatic oligomers linked via -aryl ether bonds typically found in lignin has been reported in the bacterium Sphingobium sp. SYK-6. Here, we present x-ray crystal structures and biochemical characterization of the glutathione-dependent -etherases, LigE and LigF, from this pathway. The crystal structures show that both enzymes belong to the canonical two-domain fold and glutathione binding site architecture of the glutathione S-transferase family. Mutagenesis of the conserved active site serine in both LigE and LigF shows that, whereas the enzymatic activity is reduced, this amino acid side chain is not absolutely essential for catalysis. The results include descriptions of cofactor binding sites, substrate binding sites, and catalytic mechanisms. Because -aryl ether bonds account for 50-70% of all interunit linkages in lignin, understanding the mechanism of enzymatic -aryl ether cleavage has significant potential for informing ongoing studies on the valorization of lignin. C1 [Helmich, Kate E.; Bingman, Craig; Ralph, John] Univ Wisconsin, Dept Chem, 1101 Univ Ave, Madison, WI 53706 USA. [Helmich, Kate E.; Gall, Daniel L.; Noguera, Daniel R.; Ralph, John; Donohue, Timothy J.] Univ Wisconsin, Wisconsin Energy Inst, United States Dept Energy, Great Lakes Bioenergy Res Ctr, Madison, WI 53726 USA. [Pereira, Jose Henrique; Heins, Richard A.; McAndrew, Ryan P.; Deng, Kai; Holland, Keefe C.; Simmons, Blake A.; Sale, Kenneth L.; Adams, Paul D.] Joint BioEnergy Inst, Emeryville, CA 94608 USA. [Pereira, Jose Henrique; McAndrew, Ryan P.; Adams, Paul D.] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Gall, Daniel L.; Noguera, Daniel R.] Univ Wisconsin, Dept Civil & Environm Engn, Madison, WI 53706 USA. [Donohue, Timothy J.] Univ Wisconsin, Dept Bacteriol, Madison, WI 53706 USA. [Heins, Richard A.; Deng, Kai; Holland, Keefe C.; Simmons, Blake A.; Sale, Kenneth L.] Sandia Natl Labs, Biol & Engn Sci Ctr, Livermore, CA 94551 USA. [Adams, Paul D.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Phillips, George N., Jr.] Rice Univ, Dept Biochem & Cell Biol, Houston, TX 77251 USA. RP Donohue, TJ (reprint author), Univ Wisconsin, Wisconsin Energy Inst, United States Dept Energy, Great Lakes Bioenergy Res Ctr, Madison, WI 53726 USA.; Adams, PD (reprint author), Joint BioEnergy Inst, Emeryville, CA 94608 USA.; Adams, PD (reprint author), Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA.; Donohue, TJ (reprint author), Univ Wisconsin, Dept Bacteriol, Madison, WI 53706 USA.; Adams, PD (reprint author), Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA.; Phillips, GN (reprint author), Rice Univ, Dept Biochem & Cell Biol, Houston, TX 77251 USA. EM tdonohue@bact.wisc.edu; pdadams@lbl.gov; georgep@rice.edu FU NIGMS, National Institutes of Health (NIH); Office of Science, Office of Basic Energy Sciences, of the United States Department of Energy [DE-AC02-05CH11231]; United States Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231]; NIH; United States Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Michigan Economic Development Corporation; Michigan Technology Tri-Corridor [085P1000817]; NCI; NIH [ACB-12002, AGM-12006, P41GM103399, S10RR027000]; NIGMS; University of Wisconsin (Madison, WI) FX We are grateful to the staff of the Berkeley Center for Structural Biology at the Advanced Light Source of Lawrence Berkeley National Laboratory. The Berkeley Center for Structural Biology is supported in part by NIGMS, National Institutes of Health (NIH). The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the United States Department of Energy under Contract DE-AC02-05CH11231. The Joint Bio-Energy Institute is supported by the United States Department of Energy, Office of Science, Office of Biological and Environmental Research, through Grant DE-AC02-05CH11231. We thank Dr. Brian G. Fox and Dr. Christopher M. Bianchetti for helpful discussion and the NIH-funded Center for Eukaryotic Structural Genomics for general access to computers and equipment for the structural work. Use of the Advanced Photon Source was supported by the United States Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. Use of Life Sciences Collaborative Access Team Sector 21 was supported by the Michigan Economic Development Corporation and by Michigan Technology Tri-Corridor Grant 085P1000817. Use of GM/CA@APS Sector 23 was supported by Federal funds NCI, NIH, Grant ACB-12002 and NIGMS, NIH, Grant AGM-12006. This study made use of the National Magnetic Resonance Facility at Madison, which is supported by NIGMS, NIH, Grant P41GM103399. Small angle x-ray scattering studies were supported by funds from NIH Shared Instrumentation Grant S10RR027000 and the University of Wisconsin (Madison, WI). NR 70 TC 1 Z9 1 U1 7 U2 23 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD MAR 4 PY 2016 VL 291 IS 10 BP 5234 EP 5246 DI 10.1074/jbc.M115.694307 PG 13 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DF8WF UT WOS:000371640600034 PM 26637355 ER PT J AU Park, CM Johnson, BA Duan, JC Park, JJ Day, JJ Gang, D Qian, WJ Xian, M AF Park, Chung-Min Johnson, Brett A. Duan, Jicheng Park, Jeong-Jin Day, Jacob J. Gang, David Qian, Wei-Jun Xian, Ming TI 9-Fluorenylmethyl (Fm) Disulfides: Biomimetic Precursors for Persulfides SO ORGANIC LETTERS LA English DT Article ID PROTEIN S-SULFHYDRATION; HYDROGEN-SULFIDE; CHEMICAL BIOLOGY; CHEMISTRY; H2S; BIOCHEMISTRY; MOLECULE; STRESS; CARBON AB The development of a functional disulfide, FmSSPy-A (Fm = 9-fluorenylmethyl; Py = pyridinyl), is reported. It can effectively convert small molecule and protein thiols (-SH) to form -S-SFm adducts under mild conditions. This method allows for a H2S-free and biomimetic protocol to generate highly reactive persulfides (in their anionic forms). The high nucleophilicity of persulfides toward a number of thiol-blocking reagents is also demonstrated. The method holds promise for further understanding the chemical biology of persulfides and S-sulfhydration. C1 [Park, Chung-Min; Johnson, Brett A.; Day, Jacob J.; Xian, Ming] Washington State Univ, Dept Chem, Pullman, WA 99164 USA. [Duan, Jicheng; Qian, Wei-Jun] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. [Park, Jeong-Jin; Gang, David] Washington State Univ, Tissue Imaging & Prote Lab, Pullman, WA 99164 USA. RP Xian, M (reprint author), Washington State Univ, Dept Chem, Pullman, WA 99164 USA. EM mxian@wsu.edu FU NIH [R01HL116571, P41 GM103493]; DOE [DE-AC05-76RL01830] FX This work was supported by the NIH (R01HL116571 and P41 GM103493). Part of the mass spectromtery analyses was performed in the Environmental Molecular Sciences Laboratory, a DOE national scientific user facility located at Pacific Northwest National Laboratory, which is operated by Battelle Memorial Institute for the DOE under Contract DE-AC05-76RL01830. NR 25 TC 2 Z9 2 U1 7 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1523-7060 EI 1523-7052 J9 ORG LETT JI Org. Lett. PD MAR 4 PY 2016 VL 18 IS 5 BP 904 EP 907 DI 10.1021/acs.orglett.5b03557 PG 4 WC Chemistry, Organic SC Chemistry GA DG0KP UT WOS:000371754000005 PM 26870874 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Aring;kesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Antrim, DJ Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Aring;sman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Aurousseau, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Balunas, WK Banas, E Banerjee, S Bannoura, AAE Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, M Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Biedermann, D Bieniek, SP Biesuz, NV Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biondi, S Bjergaard, DM Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Blunier, S Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehler, M Bogaerts, JA Bogavac, D Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutle, SK Boveia, A Boyd, J Boyko, IR Bozic, I Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Madden, WDB Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E de Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Bruschi, M Bruscino, N Bryngemark, L Buanes, T Buat, Q Buchholz, P Buckley, AG Buda, SI Budagov, IA Buehrer, F Bugge, L Bugge, MK Bulekov, O Bullock, D Burckhart, H Burdin, S Burgard, CD Burghgrave, B Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Buzykaev, AR Urban, SC Caforio, D Cairo, VM Cakir, O Calace, N Calafiura, P Calandri, A Calderini, G Calfayan, P Caloba, LP Calvet, D Calvet, S Toro, RC Camarda, S Camarri, P Cameron, D Armadans, RC Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Carbone, RM Cardarelli, R Cardillo, F Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Caudron, J Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, BC Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chan, YL Chang, P Chapman, JD Charlton, DG Chau, CC Barajas, CAC Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, S Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A Cheremushkina, E El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiarelli, G Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Choi, K Chouridou, S Chow, BKB Christodoulou, V Chromek-Burckhart, D Chudoba, J Chuinard, AJ Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Cinca, D Cindro, V Cioara, IA Ciocio, A Cirotto, F Citron, ZH Ciubancan, M Clark, A Clark, BL Clark, PJ Clarke, RN Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Cogan, JG Colasurdo, L Cole, B Cole, S Colijn, AP Collot, J Colombo, T Compostella, G Muino, PC Coniavitis, E Connell, SH Connelly, IA Consorti, V Constantinescu, S Conta, C Conti, G 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Zhang, D. Zhang, F. Zhang, G. Zhang, H. Zhang, J. Zhang, L. Zhang, R. Zhang, X. Zhang, Z. Zhao, X. Zhao, Y. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Search for the electroweak production of supersymmetric particles in root s=8 TeV pp collisions with the ATLAS detector SO PHYSICAL REVIEW D LA English DT Article ID DYNAMICAL SYMMETRY-BREAKING; NONUNIVERSAL HIGGS MASSES; HADRON COLLIDERS; SUPERGAUGE TRANSFORMATIONS; E(+)E(-) COLLISIONS; MODEL; ENERGY; MSSM; NEUTRALINOS; EXTENSION AB The ATLAS experiment has performed extensive searches for the electroweak production of charginos, neutralinos, and staus. This article summarizes and extends the search for electroweak supersymmetry with new analyses targeting scenarios not covered by previously published searches. New searches use vector-boson fusion production, initial-state radiation jets, and low-momentum lepton final states, as well as multivariate analysis techniques to improve the sensitivity to scenarios with small mass splittings and low-production cross sections. Results are based on 20 fb(-1) of proton-proton collision data at root s = 8 TeV recorded with the ATLAS experiment at the Large Hadron Collider. No significant excess beyond Standard Model expectations is observed. The new and existing searches are combined and interpreted in terms of 95% confidence-level exclusion limits in simplified models, where a single production process and decay mode is assumed, as well as within phenomenological supersymmetric models. C1 [Jackson, P.; Lee, L.; Petridis, A.; Soni, N.; White, M. 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West Univ Timisoara, Timisoara, Romania. [Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Gonzalez, B. Alvarez; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beermann, T. A.; Beltramello, O.; Bianco, M.; Bogaerts, J. 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G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Shanghai Key Lab Particle Phys & Cosmol, Dept Phys & Astron, Shanghai 200030, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Carbone, R. M.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Collegato Cosenza, Lab Nazl Frascati, Milan, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Phys Dept, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Phys Dept, Richardson, TX 75083 USA. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Notkestr 85, Hamburg, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Calace, N.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Paolozzi, L.; Picazio, A.; Ristic, B.; Schramm, S.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, Lab Phys Subatom & Cosmol, CNRS IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolb, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Castillo, L. R. Flores; Lu, H.; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN USA. [Jansky, R.; Jussel, P.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Span, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Aloisio, A.; Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] CNRS IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjrnmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fys Inst, Lund, Sweden. [Barreiro, F.; Cantero, J.; Cuth, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Nagai, Y.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Aloisio, A.; Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Hu, X.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Tollefson, K.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Besana, M. I.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Stabile, A.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Tartarelli, G. F.; Taylor, F. E.; Troncon, C.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu; Smirnov, Y.; Soldatov, E. Yu; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Koenig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen, Inst Math Astrophys & Particle Phys, Nikhef, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] NIKHEF H, Natl Inst Subat Phys, NL-1009 DB Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.; Yurkewicz, A.] Univ Illinois, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu A.] SB RAS, Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS IN2P3, Orsay, France. [Endo, M.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Machado Miguens, J.; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph; Schwemling, Ph; Schwindling, J.] CEA Saclay, DSM IRFU, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Hance, M.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Aloisio, A.; Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnuclear Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Lee, C. A.; Meehan, S.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Kar, D.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Univ Stockholm, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Aloisio, A.; Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Aloisio, A.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Jovicevic, J.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Antrim, D. J.; Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Guest, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Aloisio, A.; Barisonzi, M.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] Ist Nazl Fis Nucl, Sez Trieste, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Aloisio, A.; Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Gradin, P. O. J.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Piqueras, D. Alvarez; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Snchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Piqueras, D. Alvarez; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Snchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Piqueras, D. Alvarez; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Snchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingen Elect, Valencia, Spain. [Piqueras, D. Alvarez; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Snchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, IMB, CNM, Valencia, Spain. [Piqueras, D. Alvarez; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Snchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; Gignac, M.; Henkelmann, S.; King, S. B.; Lister, A.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Pearce, J.; Sobie, R.; Trovatelli, M.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.; Spangenberg, M.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. 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A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] IN2P3, Ctr Calcul, Villeurbanne, France. Kings Coll London, Dept Phys, London WC2R 2LS, England. [Ahmadov, F.; Huseynov, N.; Javadov, N.; Liu, B.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Anisenkov, A. V.; Baldin, E. M.; Bawa, H. S.; Bobrovnikov, V. S.; Bortolotto, V.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Myagkov, A. G.; Nikolaenko, V.; Peleganchuk, S. V.; Prokofiev, K.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu A.; Zaitsev, A. M.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Azuelos, G.; Gingrich, D. M.; Oakham, F. G.; Savard, P.; Vetterli, M. C.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Gao, Y. S.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beck, H. 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E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Jenni, P.] CERN, Geneva, Switzerland. [Khubua, J.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellen Open Univ, Patras, Greece. [Li, B.; Song, H. Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Li, Y.] Univ Paris 11, LAL, Orsay, France. [Li, Y.] CNRS IN2P3, Orsay, France. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Liu, B.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys, Dolgoprudnyi, Russia. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Technol State Univ, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tompkins, L.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France.; Aad, G (reprint author), CNRS IN2P3, Marseille, France. RI Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Garcia, Jose /H-6339-2015; Gorelov, Igor/J-9010-2015; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; BESSON, NATHALIE/L-6250-2015; La Rosa Navarro, Jose Luis/K-4221-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Smirnova, Oxana/A-4401-2013; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Conde Muino, Patricia/F-7696-2011; Vranjes Milosavljevic, Marija/F-9847-2016; Gladilin, Leonid/B-5226-2011; Chekulaev, Sergey/O-1145-2015; White, Ryan/E-2979-2015; Zhukov, Konstantin/M-6027-2015; SULIN, VLADIMIR/N-2793-2015; Snesarev, Andrey/H-5090-2013; Brooks, William/C-8636-2013; Nechaeva, Polina/N-1148-2015; Mashinistov, Ruslan/M-8356-2015; Vykydal, Zdenek/H-6426-2016; Fedin, Oleg/H-6753-2016; Aguilar Saavedra, Juan Antonio/F-1256-2016; Warburton, Andreas/N-8028-2013; Carvalho, Joao/M-4060-2013; Tikhomirov, Vladimir/M-6194-2015; Doyle, Anthony/C-5889-2009; Boyko, Igor/J-3659-2013; Mitsou, Vasiliki/D-1967-2009; Guo, Jun/O-5202-2015; Sanchez, Javier/F-5073-2016; Livan, Michele/D-7531-2012; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Stabile, Alberto/L-3419-2016; Villa, Mauro/C-9883-2009; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Gavrilenko, Igor/M-8260-2015; Di Domenico, Antonio/G-6301-2011; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Peleganchuk, Sergey/J-6722-2014 OI Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; KUBOTA, TAKASHI/0000-0002-1156-5571; Gorelov, Igor/0000-0001-5570-0133; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Smirnova, Oxana/0000-0003-2517-531X; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Conde Muino, Patricia/0000-0002-9187-7478; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Gladilin, Leonid/0000-0001-9422-8636; White, Ryan/0000-0003-3589-5900; SULIN, VLADIMIR/0000-0003-3943-2495; Brooks, William/0000-0001-6161-3570; Mashinistov, Ruslan/0000-0001-7925-4676; Vykydal, Zdenek/0000-0003-2329-0672; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Warburton, Andreas/0000-0002-2298-7315; Carvalho, Joao/0000-0002-3015-7821; Tikhomirov, Vladimir/0000-0002-9634-0581; Doyle, Anthony/0000-0001-6322-6195; Boyko, Igor/0000-0002-3355-4662; Mitsou, Vasiliki/0000-0002-1533-8886; Guo, Jun/0000-0001-8125-9433; Livan, Michele/0000-0002-5877-0062; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Stabile, Alberto/0000-0002-6868-8329; Villa, Mauro/0000-0002-9181-8048; Kukla, Romain/0000-0002-1140-2465; Di Domenico, Antonio/0000-0001-8078-2759; Gauzzi, Paolo/0000-0003-4841-5822; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Peleganchuk, Sergey/0000-0003-0907-7592 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; RGC, Hong Kong SAR, China; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; NSC, Taiwan; TAEK, Turkey; DOE, United States of America; NSF, United States of America; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We thank Sabine Kraml for her advice while preparing the model files of the NUHM2 grid. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC, and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST, and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR, and VSC CR, Czech Republic; DNRF, DNSRC, and Lundbeck Foundation, Denmark; EPLANET, ERC, and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG, and AvH Foundation, Germany; GSRT and NSRF, Greece; RGC, Hong Kong SAR, China; ISF, MINERVA, GIF, I-CORE, and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF, and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK), and BNL (USA) and in the Tier-2 facilities worldwide. NR 119 TC 9 Z9 9 U1 20 U2 53 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 4 PY 2016 VL 93 IS 5 AR 052002 DI 10.1103/PhysRevD.93.052002 PG 50 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DF5TA UT WOS:000371414200001 ER PT J AU Cho, JH Paik, SY AF Cho, Jun Ho Paik, Samuel Y. TI Association between Electronic Cigarette Use and Asthma among High School Students in South Korea SO PLOS ONE LA English DT Article ID FIBERS IN-VITRO; SMOKING; MACROPHAGES; NICOTINE; ALVEOLAR; RAT AB Objectives Little is known about health outcomes related to electronic cigarette (EC) use, despite its growing popularity. The aim of this study is to investigate the association between EC use and asthma. Methods The study design is a cross-sectional study. A total of 35,904 high school students were included as the final study population. The presence of asthma was based on a student's self-reported doctor diagnosis of asthma in the past 12 months. Results Prevalence rates of asthmatics in 'current EC users' (n = 2,513), 'former EC users' (n = 2,078), and 'never EC users' (n = 31,313), were 3.9% (n = 98), 2.2% (n = 46) and 1.7% (n = 530), respectively. Comparing 'current EC' users with 'never EC' users, the unadjusted OR for asthma was 2.36 (95% CI: 1.89-2.94). In order to control for the effect of conventional cigarette (CC) smoking, after stratifying the subjects by the three CC smoking categories (never CC, former CC, and current CC), within the 'never CC' category, the unadjusted OR for asthma for 'current EC' users was 3.41 (95% CI: 1.79-6.49), and the adjusted OR was 2.74 (95% CI: 1.30-5.78). Severe asthma was reflected by the number of days absent from school due to asthma symptoms; current EC users had the highest adjusted OR for severe asthma compared to 'never EC' users. Conclusions When compared to a reference population of high school students in South Korea, EC users have an increased association with asthma and are more likely to have had days absent from school due to severe asthma symptoms. In conclusion, the results indicate that EC use may be a risk factor for asthma. The results may be useful in developing a scientific basis for the evaluation of a potential health hazard by EC. C1 [Cho, Jun Ho] Hanyang Womens Univ, Dept Publ Hlth Adm, 17 Haeng Dong Sungdong Ku, Seoul 133793, South Korea. [Paik, Samuel Y.] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. RP Cho, JH (reprint author), Hanyang Womens Univ, Dept Publ Hlth Adm, 17 Haeng Dong Sungdong Ku, Seoul 133793, South Korea. EM cjhjunho@hywoman.ac.kr FU 2nd semester Hanyang Women's University Research Fund FX The study was supported by the 2014-2nd semester Hanyang Women's University Research Fund. NR 27 TC 5 Z9 5 U1 1 U2 11 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 4 PY 2016 VL 11 IS 3 AR e0151022 DI 10.1371/journal.pone.0151022 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DG0FG UT WOS:000371739400072 PM 26942764 ER PT J AU Johnson, JL Haardt, F AF Johnson, Jarrett L. Haardt, Francesco TI The Early Growth of the First Black Holes SO PUBLICATIONS OF THE ASTRONOMICAL SOCIETY OF AUSTRALIA LA English DT Review DE accretion, accretion disks; radiation: dynamics; black hole physics; quasars: general; cosmology: theory ID ATOMIC COOLING HALOES; BARYONIC STREAMING VELOCITIES; HIGH-REDSHIFT FORMATION; SLIM ACCRETION DISCS; DARK-MATTER HALOES; DIRECT COLLAPSE; GALAXY MERGERS; EARLY UNIVERSE; SUPERMASSIVE STARS; ANGULAR-MOMENTUM AB With detections of quasars powered by increasingly massive black holes at increasingly early times in cosmic history over the past decade, there has been correspondingly rapid progress made on the theory of early black hole formation and growth. Here, we review the emerging picture of how the first massive black holes formed from the primordial gas and then grew to supermassive scales. We discuss the initial conditions for the formation of the progenitors of these seed black holes, the factors dictating the initial masses with which they form, and their initial stages of growth via accretion, which may occur at super-Eddington rates. Finally, we briefly discuss how these results connect to large-scale simulations of the growth of supermassive black holes in the first billion years after the Big Bang. C1 [Johnson, Jarrett L.] Los Alamos Natl Lab, X Theoret Design, POB 1663, Los Alamos, NM 87545 USA. [Haardt, Francesco] Univ Insubria, DiSAT, Via Valleggio 11, I-22100 Como, Italy. RP Johnson, JL (reprint author), Los Alamos Natl Lab, X Theoret Design, POB 1663, Los Alamos, NM 87545 USA. EM jlj@lanl.gov FU National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396] FX The authors would like to thank Rosa Valiante, Rafaella Schneider, and Marta Volonteri for the opportunity to contribute this review. Work at LANL was done under the auspices of the National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. NR 179 TC 6 Z9 6 U1 2 U2 12 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 1323-3580 EI 1448-6083 J9 PUBL ASTRON SOC AUST JI Publ. Astron. Soc. Aust. PD MAR 4 PY 2016 VL 33 AR e007 DI 10.1017/pasa.2016.4 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DF9XS UT WOS:000371716500001 ER PT J AU Stanislavchuk, TN Wang, YZ Janssen, Y Carr, GL Cheong, SW Sirenko, AA AF Stanislavchuk, T. N. Wang, Yazhong Janssen, Y. Carr, G. L. Cheong, S. -W. Sirenko, A. A. TI Magnon and electromagnon excitations in multiferroic DyFeO3 SO PHYSICAL REVIEW B LA English DT Article ID RARE-EARTH ORTHOFERRITES; ORTHO-FERRITES; MAGNETIC EXCITATIONS; SPIN-WAVES; SCATTERING; TEMPERATURE; PARALLEL AB Optical properties of orthorhombic DyFeO3 single crystals have been studied in the far-infrared spectral range of 11-120 cm(-1) at temperatures between 1.5 and 50 K and in magnetic fields up to 7 T. The temperature and magnetic-field dependencies of the antiferromagnetic (AFM) resonance spectra have been measured below and above the AFM ordering temperature of Dy3+ moments with T-N(Dy) = 4.2 K. Hardening of the quasiferromagnetic mode frequency of the AFM resonance due to ordering of Dy3+ moments is observed. Below T-N(Dy) two electric dipole-active magnetic excitations, or electromagnons, appear in the spectra at similar to 20 and similar to 50 cm(-1). The electromagnons vanish with the application of a strong magnetic field along the a or b axis which changes the magnetic structures of Fe3+ and Dy3+ moments into the ones compatible with the spatial inversion symmetry. We show that the electromagnon at similar to 20 cm(-1) provides a significant contribution to the static electric permittivity epsilon. The energies of the electromagnons as well as static electric permittivity manifest a strong hysteresis upon cycling of an external magnetic field at T < T-N(Dy). C1 [Stanislavchuk, T. N.; Sirenko, A. A.] New Jersey Inst Technol, Dept Phys, Newark, NJ 07102 USA. [Wang, Yazhong; Cheong, S. -W.] Rutgers State Univ, Dept Phys & Astron, Rutgers Ctr Emergent Mat, POB 849, Piscataway, NJ 08854 USA. [Janssen, Y.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Carr, G. L.] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. RP Stanislavchuk, TN (reprint author), New Jersey Inst Technol, Dept Phys, Newark, NJ 07102 USA. EM stantar@njit.edu FU U.S. Department of Energy [DE-FG02-07ER46382, DE-AC02-98CH10886] FX The authors are grateful to R. Basistyy for help with modeling of experimental data and to S. Artyukhin for interest and useful discussions. Work at the New Jersey Institute of Technology and Rutgers University was supported by the U.S. Department of Energy under Contract No. DE-FG02-07ER46382. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the U.S. Department of Energy under Contract No. DE-AC02-98CH10886. NR 42 TC 2 Z9 2 U1 10 U2 34 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 4 PY 2016 VL 93 IS 9 AR 094403 DI 10.1103/PhysRevB.93.094403 PG 12 WC Physics, Condensed Matter SC Physics GA DF5OQ UT WOS:000371401900002 ER PT J AU Simon, A Guttormsen, M Larsen, AC Beausang, CW Humby, P Burke, JT Casperson, RJ Hughes, RO Ross, TJ Allmond, JM Chyzh, R Dag, M Koglin, J McCleskey, E McCleskey, M Ota, S Saastamoinen, A AF Simon, A. Guttormsen, M. Larsen, A. C. Beausang, C. W. Humby, P. Burke, J. T. Casperson, R. J. Hughes, R. O. Ross, T. J. Allmond, J. M. Chyzh, R. Dag, M. Koglin, J. McCleskey, E. McCleskey, M. Ota, S. Saastamoinen, A. TI First observation of low-energy gamma-ray enhancement in the rare-earth region SO PHYSICAL REVIEW C LA English DT Article ID STRENGTH; NUCLEI AB The gamma-ray strength function and level density in the quasi-continuum of Sm-151,Sm-153 have been measured using bismuth germanate shielded Ge clover detectors of the STARLiTeR system. The Compton shields allow an extraction of the. strength down to unprecedentedly low. energies of approximate to 500 keV. For the first time an enhanced low-energy gamma-ray strength has been observed in the rare-earth region. In addition, for the first time both the upbend and the well-known scissors resonance have been observed simultaneously for the same nucleus. Hauser-Feshbach calculations show that this strength enhancement at low. energies could have an impact of 2-3 orders of magnitude on the (n,gamma)reaction rates for gamma-process nucleosynthesis. C1 [Simon, A.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Guttormsen, M.; Larsen, A. C.; Beausang, C. W.] Univ Oslo, Dept Phys, N-0316 Oslo, Norway. [Humby, P.] Univ Richmond, Dept Phys, Richmond, VA 23171 USA. [Humby, P.] Univ Surrey, Dept Phys, Surrey GU2 7XH, England. [Burke, J. T.; Casperson, R. J.; Hughes, R. O.; Koglin, J.; Ota, S.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Ross, T. J.] Univ Kentucky, Dept Chem, Lexington, KY 40506 USA. [Allmond, J. M.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Chyzh, R.; Dag, M.; McCleskey, E.; McCleskey, M.; Saastamoinen, A.] Texas A&M Univ, Inst Cyclotron, College Stn, TX 77843 USA. [Ota, S.] Rutgers State Univ, Dept Phys & Astron, New Brunswick, NJ 08903 USA. RP Simon, A (reprint author), Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA.; Guttormsen, M; Larsen, AC (reprint author), Univ Oslo, Dept Phys, N-0316 Oslo, Norway. EM anna.simon@nd.edu; magne.guttormsen@fys.uio.no; a.c.larsen@fys.uio.no RI Larsen, Ann-Cecilie/C-8742-2014 OI Larsen, Ann-Cecilie/0000-0002-2188-3709 FU US Department of Energy [DE-NA0001801, DE-FG02-05ER41379, DE-AC52-07NA27344]; Research Council of Norway (NFR); National Science Foundation [PHY-1430152]; Research Council of Norway [205528]; ERC-STG [637686] FX The authors would like to thank ORNL for providing one of the clover detectors for the STARLiTeR setup. This work was supported by the US Department of Energy under Grants No. DE-NA0001801, No. DE-FG02-05ER41379, and No. DE-AC52-07NA27344; the Research Council of Norway (NFR); and the National Science Foundation under Grant No. PHY-1430152 (JINA-CEE). A.C.L. acknowledges financial support from the Research Council of Norway, Grant No. 205528, and funding from the ERC-STG-2014 under Grant Agreement No. 637686. NR 50 TC 5 Z9 5 U1 6 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 4 PY 2016 VL 93 IS 3 AR 034303 DI 10.1103/PhysRevC.93.034303 PG 7 WC Physics, Nuclear SC Physics GA DF5RK UT WOS:000371409600002 ER PT J AU Ferrie, C Blume-Kohout, R AF Ferrie, Christopher Blume-Kohout, Robin TI Minimax Quantum Tomography: Estimators and Relative Entropy Bounds SO PHYSICAL REVIEW LETTERS LA English DT Article AB A minimax estimator has the minimum possible error ("risk") in the worst case. We construct the first minimax estimators for quantum state tomography with relative entropy risk. The minimax risk of nonadaptive tomography scales as O(1/root N)-in contrast to that of classical probability estimation, which is O(1/N)-where N is the number of copies of the quantum state used. We trace this deficiency to sampling mismatch: future observations that determine risk may come from a different sample space than the past data that determine the estimate. This makes minimax estimators very biased, and we propose a computationally tractable alternative with similar behavior in the worst case, but superior accuracy on most states. C1 [Ferrie, Christopher] Univ New Mexico, Ctr Quantum Informat & Control, Albuquerque, NM 87131 USA. [Ferrie, Christopher] Univ Sydney, Sch Phys, Ctr Engn Quantum Syst, Sydney, NSW 2006, Australia. [Blume-Kohout, Robin] Sandia Natl Labs, Ctr Comp Res, POB 5800, Albuquerque, NM 87185 USA. RP Ferrie, C (reprint author), Univ New Mexico, Ctr Quantum Informat & Control, Albuquerque, NM 87131 USA.; Ferrie, C (reprint author), Univ Sydney, Sch Phys, Ctr Engn Quantum Syst, Sydney, NSW 2006, Australia. OI Ferrie, Christopher/0000-0003-2736-9943 FU National Science Foundation [PHY-1212445]; Canadian Government through the NSERC PDF program; IARPA MQCO program; ARC, via EQuS [CE11001013]; U.S. Army Research Office [W911NF-14-1-0098, W911NF-14-1-0103]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX C. F. was supported by National Science Foundation Grant No. PHY-1212445; by the Canadian Government through the NSERC PDF program, the IARPA MQCO program, and the ARC, via EQuS Project No. CE11001013; and by U.S. Army Research Office Grants No. W911NF-14-1-0098 and No. W911NF-14-1-0103. Sandia National Laboratories is a multiprogram laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration, under Contract No. DE-AC04-94AL85000. NR 22 TC 1 Z9 1 U1 2 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 4 PY 2016 VL 116 IS 9 AR 090407 DI 10.1103/PhysRevLett.116.090407 PG 5 WC Physics, Multidisciplinary SC Physics GA DF5VM UT WOS:000371420600003 PM 26991163 ER PT J AU Bennett, SP Wong, AT Glavic, A Herklotz, A Urban, C Valmianski, I Biegalski, MD Christen, HM Ward, TZ Lauter, V AF Bennett, S. P. Wong, A. T. Glavic, A. Herklotz, A. Urban, C. Valmianski, I. Biegalski, M. D. Christen, H. M. Ward, T. Z. Lauter, V. TI Giant Controllable Magnetization Changes Induced by Structural Phase Transitions in a Metamagnetic Artificial Multiferroic SO SCIENTIFIC REPORTS LA English DT Article ID FERH THIN-FILMS; ROOM-TEMPERATURE; ALLOY; REFLECTOMETER; ORDER AB The realization of a controllable metamagnetic transition from AFM to FM ordering would open the door to a plethora of new spintronics based devices that, rather than reorienting spins in a ferromagnet, harness direct control of a materials intrinsic magnetic ordering. In this study FeRh films with drastically reduced transition temperatures and a large magneto-thermal hysteresis were produced for magnetocaloric and spintronics applications. Remarkably, giant controllable magnetization changes (measured to be as high has similar to 25%) are realized by manipulating the strain transfer from the external lattice when subjected to two structural phase transitions of BaTiO3 (001) single crystal substrate. These magnetization changes are the largest seen to date to be controllably induced in the FeRh system. Using polarized neutron reflectometry we reveal how just a slight in plane surface strain change at similar to 290C results in a massive magnetic transformation in the bottom half of the film clearly demonstrating a strong lattice-spin coupling in FeRh. By means of these substrate induced strain changes we show a way to reproducibly explore the effects of temperature and strain on the relative stabilities of the FM and AFM phases in multi-domain metamagnetic systems. This study also demonstrates for the first time the depth dependent nature of a controllable magnetic order using strain in an artificial multiferroic heterostructure. C1 [Bennett, S. P.; Glavic, A.; Lauter, V.] Oak Ridge Natl Lab, Neutron Sci Directorate, Quantum Condensed Matter Div, Oak Ridge, TN 37830 USA. [Wong, A. T.; Herklotz, A.; Ward, T. Z.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37830 USA. [Glavic, A.] Paul Scherrer Inst, Lab Neutron Scattering & Imaging, CH-5232 Villigen, Switzerland. [Wong, A. T.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Biegalski, M. D.; Christen, H. M.] Oak Ridge Natl Lab, Ctr Nanoscale Mat Sci, Oak Ridge, TN 37830 USA. [Urban, C.; Valmianski, I.] Univ Calif San Diego, Dept Phys, San Diego, CA 92110 USA. RP Bennett, SP; Lauter, V (reprint author), Oak Ridge Natl Lab, Neutron Sci Directorate, Quantum Condensed Matter Div, Oak Ridge, TN 37830 USA. EM bennettsp@ornl.gov; lauterv@ornl.gov RI Glavic, Artur/B-3453-2015; Ward, Thomas/I-6636-2016; Christen, Hans/H-6551-2013; OI Glavic, Artur/0000-0003-4951-235X; Ward, Thomas/0000-0002-1027-9186; Christen, Hans/0000-0001-8187-7469; Bennett, Steven/0000-0003-2615-6321 FU Scientific User Facilities Division, the Office of Basic Energy Sciences (BES), US Department of Energy (DOE); US Department of Energy (DOE), Office of Basic Energy Sciences (BES), Materials Sciences and Engineering Division; US DOE [DE-SC0002136]; Department of Energy's Office of Basic Energy Science [DE FG02 87ER-45332] FX This work was supported by the Scientific User Facilities Division, the Office of Basic Energy Sciences (BES), US Department of Energy (DOE), (S.B., V.L., A.G. & H.C.). This effort was also supported in part by the US Department of Energy (DOE), Office of Basic Energy Sciences (BES), Materials Sciences and Engineering Division, (T.Z.W. and A.H.) and under US DOE grant DE-SC0002136 (A.W.). And grant DE FG02 87ER-45332, DMS funded by the Department of Energy's Office of Basic Energy Science, (C.U. & I.V.). NR 38 TC 4 Z9 4 U1 10 U2 57 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 4 PY 2016 VL 6 AR 22708 DI 10.1038/srep22708 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DF5WD UT WOS:000371422400001 PM 26940159 ER PT J AU Panuwet, P Hunter, RE D'Souza, PE Chen, XY Radford, SA Cohen, JR Marder, ME Kartavenka, K Ryan, PB Barr, DB AF Panuwet, Parinya Hunter, Ronald E., Jr. D'Souza, Priya E. Chen, Xianyu Radford, Samantha A. Cohen, Jordan R. Marder, M. Elizabeth Kartavenka, Kostya Ryan, P. Barry Barr, Dana Boyd TI Biological Matrix Effects in Quantitative Tandem Mass Spectrometry-Based Analytical Methods: Advancing Biomonitoring SO CRITICAL REVIEWS IN ANALYTICAL CHEMISTRY LA English DT Review DE tandem mass-spectrometry; Analytical method development; matrix effects; biomonitoring; biological analysis ID HUMAN URINE; ION SUPPRESSION; ELECTROSPRAY-IONIZATION; GAS-CHROMATOGRAPHY; ORGANOPHOSPHORUS PESTICIDES; SIGNAL SUPPRESSION; SAMPLE PREPARATION; VALIDATION; QUANTIFICATION; BIOANALYSIS AB The ability to quantify levels of target analytes in biological samples accurately and precisely in biomonitoring involves the use of highly sensitive and selective instrumentation such as tandem mass spectrometers and a thorough understanding of highly variable matrix effects. Typically, matrix effects are caused by co-eluting matrix components that alter the ionization of target analytes as well as the chromatographic response of target analytes, leading to reduced or increased sensitivity of the analysis. Thus, before the desired accuracy and precision standards of laboratory data are achieved, these effects must be characterized and controlled. Here we present our review and observations of matrix effects encountered during the validation and implementation of tandem mass spectrometry-based analytical methods. We also provide systematic, comprehensive laboratory strategies needed to control challenges posed by matrix effects in order to ensure delivery of the most accurate data for biomonitoring studies assessing exposure to environmental toxicants. C1 [Panuwet, Parinya; Hunter, Ronald E., Jr.; D'Souza, Priya E.; Chen, Xianyu; Radford, Samantha A.; Cohen, Jordan R.; Marder, M. Elizabeth; Kartavenka, Kostya; Ryan, P. Barry; Barr, Dana Boyd] Emory Univ, Rollins Sch Publ Hlth, Dept Environm Hlth, 201 Dowman Dr, Atlanta, GA 30322 USA. [Chen, Xianyu; Radford, Samantha A.; Ryan, P. Barry] Emory Univ, Dept Chem, 1515 Pierce Dr, Atlanta, GA 30322 USA. [Hunter, Ronald E., Jr.] Ctr Dis Control & Prevent, ORISE, Atlanta, GA USA. RP Panuwet, P (reprint author), Emory Univ, Rollins Sch Publ Hlth, Dept Environm Hlth, 201 Dowman Dr, Atlanta, GA 30322 USA. EM ppanuwe@emory.edu FU American Recovery and Reinvestment Act under NIH [5RC1ES01829902]; National Children's Study [HHSN267200700007C]; PBDE Body Burdens, House Dust Concentrations, and Associations with Thyroid Hormones under NIH [1R21ES019697-01]; Emory Parkinson's disease Collaborative Environmental Research Center under NIEHS [P01 ES016731]; HERCULES: Health and Exposome Research Center at Emory University under NIEHS [1P30ES019776-01A1]; Graduate and Postdoctoral Training in Toxicology NIH grant [T32 ES012870] FX This work was supported in part by the American Recovery and Reinvestment Act of 2009 under NIH grant 5RC1ES01829902, the National Children's Study under contract number HHSN267200700007C, PBDE Body Burdens, House Dust Concentrations, and Associations with Thyroid Hormones under NIH grant 1R21ES019697-01, the Emory Parkinson's disease Collaborative Environmental Research Center under NIEHS grant P01 ES016731, and HERCULES: Health and Exposome Research Center at Emory University under NIEHS grant 1P30ES019776-01A1. Samantha A. Radford was supported by Graduate and Postdoctoral Training in Toxicology NIH grant T32 ES012870. NR 57 TC 5 Z9 6 U1 9 U2 25 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 1040-8347 EI 1547-6510 J9 CRIT REV ANAL CHEM JI Crit. Rev. Anal. Chem. PD MAR 3 PY 2016 VL 46 IS 2 BP 93 EP 105 DI 10.1080/10408347.2014.980775 PG 13 WC Chemistry, Analytical SC Chemistry GA DG8VL UT WOS:000372361600002 PM 25562585 ER PT J AU Tanner-Smith, EE Risser, MD AF Tanner-Smith, Emily E. Risser, Mark D. TI A meta-analysis of brief alcohol interventions for adolescents and young adults: variability in effects across alcohol measures SO AMERICAN JOURNAL OF DRUG AND ALCOHOL ABUSE LA English DT Article DE systematic review; alcohol use; Adolescents; meta-analysis; brief alcohol intervention; youth ID COLLEGE-STUDENT DRINKING; DEPENDENT EFFECT SIZES; COST-EFFECTIVENESS; EMERGENCY-DEPARTMENT; 3-LEVEL METAANALYSIS; BINGE DRINKING; CONSUMPTION; FREQUENCY; QUANTITY; ISSUES AB Background: Brief alcohol interventions are one approach for reducing drinking among youth, but may vary in effectiveness depending on the type of alcohol assessments used to measure effects. Objectives: To conduct a meta-analysis that examined the effectiveness of brief alcohol interventions for adolescents and young adults, with particular emphasis on exploring variability in effects across outcome measurement characteristics. Method: Eligible studies were those using an experimental or quasi-experimental design to examine the effects of a brief alcohol intervention on a post-intervention alcohol use measure for youth aged 11-30. A comprehensive literature review identified 190 unique samples that were included in the meta-analysis. Taking a Bayesian approach, we used random-effects multilevel models to estimate the average effect and model variability across outcome measurement types. Results: Brief alcohol interventions led to significant reductions in self-reported alcohol use among adolescents ( [GRAPHICS] = 0.25, 95% credible interval [CrI 0.13, 0.37]) and young adults ( [GRAPHICS] = 0.15, 95% CrI [0.12, 0.18]). These results were consistent across outcomes with varying reference periods, but varied across outcome construct type and assessment instruments. Among adolescents, effects were larger when measured using the Timeline Followback; among young adults, effects were smaller when measured using the Alcohol Use Disorders Identification Test. Conclusion: The strength of the beneficial effects of brief alcohol interventions on youth's alcohol use may vary depending upon the outcome measure utilized. Nevertheless, significant effects were observed across measures. Although effects were modest in size, they were clinically significant and show promise for interrupting problematic alcohol use trajectories among youth. C1 [Tanner-Smith, Emily E.] Vanderbilt Univ, Peabody Res Inst, Dept Human & Org Dev, Box 0181 GPC, Nashville, TN 37203 USA. [Risser, Mark D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Tanner-Smith, EE (reprint author), Vanderbilt Univ, Peabody Res Inst, Dept Human & Org Dev, Box 0181 GPC, Nashville, TN 37203 USA. EM e.tanner-smith@vanderbilt.edu RI Risser, Mark/J-5801-2015 OI Risser, Mark/0000-0003-1956-1783 FU National Institute on Alcohol Abuse and Alcoholism [R01AA020286] FX This work was supported by Award Number R01AA020286 from the National Institute on Alcohol Abuse and Alcoholism. The content is solely the responsibility of the authors and does not necessarily represent the official views of the National Institute on Alcohol Abuse and Alcoholism or the National Institutes of Health. NR 43 TC 0 Z9 0 U1 5 U2 8 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 0095-2990 EI 1097-9891 J9 AM J DRUG ALCOHOL AB JI Am. J. Drug Alcohol Abuse PD MAR 3 PY 2016 VL 42 IS 2 BP 140 EP 151 DI 10.3109/00952990.2015.1136638 PG 12 WC Psychology, Clinical; Substance Abuse SC Psychology; Substance Abuse GA DG9SC UT WOS:000372423100004 PM 26905387 ER PT J AU Niezgoda, JS Rosenthal, SJ AF Niezgoda, J. Scott Rosenthal, Sandra J. TI Synthetic Strategies for Semiconductor Nanocrystals Expressing Localized Surface Plasmon Resonance SO CHEMPHYSCHEM LA English DT Review DE doping; nanocrystals; semiconductors; surface plasmon resonance; quantum dots ID UP-CONVERSION SPECTROSCOPY; DOPED SILICON NANOCRYSTALS; CUXINYS2 QUANTUM DOTS; SOLAR-CELLS; COPPER SULFIDE; COLLOIDAL SEMICONDUCTOR; ABSORPTION ENHANCEMENT; CONTROLLABLE SYNTHESIS; SELENIDE NANOCRYSTALS; CU2-XSE NANOCRYSTALS AB The field of semiconductor plasmonics has grown rapidly since its outset, only roughly six years ago, and now includes many crystalline substances ranging from GeTe to wide-bandgap transition-metal oxides. One byproduct of this proliferation is the sea of differing synthetic methods to realize localized surface plasmon resonances (LSPRs) based on the studied material. Strategies vary widely from material to material, but all have the common goal of introducing extremely high carrier densities to the semiconductor system. This doping results in tunable, size-quantized, and on/off-switchable LSPR modes, which are a complete departure from traditional metal-nanoparticle-based plasmon resonances. This Minireview will provide an overview of the current state of nanocrystal and quantum-dot plasmonics and the physical basis thereof, however its main purpose is to summarize the methods for realizing LSPRs in the various syntheses and systems that have been reported to date. C1 [Niezgoda, J. Scott; Rosenthal, Sandra J.] Vanderbilt Univ, Dept Chem, Box 1583, Nashville, TN 37235 USA. [Niezgoda, J. Scott; Rosenthal, Sandra J.] Vanderbilt Univ, Vanderbilt Inst Nanoscale Sci, 221 Kirkland Hall, Nashville, TN 37235 USA. [Rosenthal, Sandra J.] Vanderbilt Univ, Dept Interdisciplinary Mat Sci, Dept Phys & Astron, Dept Chem & Biomol Engn, 221 Kirkland Hall, Nashville, TN 37235 USA. [Rosenthal, Sandra J.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Rosenthal, SJ (reprint author), Vanderbilt Univ, Dept Chem, Box 1583, Nashville, TN 37235 USA.; Rosenthal, SJ (reprint author), Vanderbilt Univ, Vanderbilt Inst Nanoscale Sci, 221 Kirkland Hall, Nashville, TN 37235 USA.; Rosenthal, SJ (reprint author), Vanderbilt Univ, Dept Interdisciplinary Mat Sci, Dept Phys & Astron, Dept Chem & Biomol Engn, 221 Kirkland Hall, Nashville, TN 37235 USA.; Rosenthal, SJ (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM sandra.j.rosenthal@vanderbilt.edu NR 96 TC 1 Z9 1 U1 27 U2 69 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1439-4235 EI 1439-7641 J9 CHEMPHYSCHEM JI ChemPhysChem PD MAR 3 PY 2016 VL 17 IS 5 BP 645 EP 653 DI 10.1002/cphc.201500758 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DG6JR UT WOS:000372190900007 PM 26530667 ER PT J AU Caliandro, R Sibillano, T Belviso, BD Scarfiello, R Hanson, JC Dooryhee, E Manca, M Cozzoli, PD Giannini, C AF Caliandro, Rocco Sibillano, Teresa Belviso, B. Danilo Scarfiello, Riccardo Hanson, Jonathan C. Dooryhee, Eric Manca, Michele Cozzoli, P. Davide Giannini, Cinzia TI Static and Dynamical Structural Investigations of Metal-Oxide Nanocrystals by Powder X-ray Diffraction: Colloidal Tungsten Oxide as a Case Study SO CHEMPHYSCHEM LA English DT Article DE colloids; nanoparticles; oxides; pair distribution function; X-ray diffraction ID MODULATION-ENHANCED DIFFRACTION; PAIR DISTRIBUTION-FUNCTIONS; MULTIVARIATE-ANALYSIS; TRANSITION-METAL; SIZE; SELECTIVITY; SOFTWARE; GROWTH; SHAPE AB We have developed a general X-ray powder diffraction (XPD) methodology for the simultaneous structural and compositional characterization of inorganic nanomaterials. The approach is validated on colloidal tungsten oxide nanocrystals (WO3-x NCs), as a model polymorphic nanoscale material system. Rod-shaped WO3-x NCs with different crystal structure and stoichiometry are comparatively investigated under an inert atmosphere and after prolonged air exposure. An initial structural model for the as-synthesized NCs is preliminarily identified by means of Rietveld analysis against several reference crystal phases, followed by atomic pair distribution function (PDF) refinement of the best-matching candidates (static analysis). Subtle stoichiometry deviations from the corresponding bulk standards are revealed. NCs exposed to air at room temperature are monitored by XPD measurements at scheduled time intervals. The static PDF analysis is complemented with an investigation into the evolution of the WO3-x NC structure, performed by applying the modulation enhanced diffraction technique to the whole time series of XPD profiles (dynamical analysis). Prolonged contact with ambient air is found to cause an appreciable increase in the static disorder of the O atoms in the WO3-x NC lattice, rather than a variation in stoichiometry. The time behavior of such structural change is identified on the basis of multivariate analysis. C1 [Caliandro, Rocco; Sibillano, Teresa; Belviso, B. Danilo; Giannini, Cinzia] CNR, Inst Crystallog, Via Amendola 122-o, I-70126 Bari, Italy. [Scarfiello, Riccardo; Cozzoli, P. Davide] Univ Salento, Dipartimento Matemat & Fis E De Giorgi, Via Arnesano, I-73100 Lecce, Italy. [Scarfiello, Riccardo; Manca, Michele] Ist Italiano Tecnol, Ctr Biomol Nanotechnol UNILE, Via Barsanti, I-73010 Arnesano, LE, Italy. [Hanson, Jonathan C.] Brookhaven Natl Lab, Dept Chem, POB 5000, Upton, NY USA. [Dooryhee, Eric] Brookhaven Natl Lab, Photon Sci, POB 5000, Upton, NY USA. [Scarfiello, Riccardo; Cozzoli, P. Davide] Univ Salento, CNR, NANOTEC, Inst Nanotechnol, C Campus Ecotekne,Via Monteroni, I-73100 Lecce, Italy. RP Caliandro, R; Giannini, C (reprint author), CNR, Inst Crystallog, Via Amendola 122-o, I-70126 Bari, Italy. EM rocco.caliandro@ic.cnr.it; cinzia.giannini@ic.cnr.it RI Manca, Michele/O-8468-2015; caliandro, rocco/A-2686-2013; OI Manca, Michele/0000-0002-6903-2954; caliandro, rocco/0000-0002-0368-4925; Cozzoli, Pantaleo Davide/0000-0001-8037-6937 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886]; CNR program; project RINAME [RBAP114AMK_006]; project MAAT [PON02_00563_3316357] FX Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. This research has been partially supported by the short-term mobility CNR program, by the project RINAME (contract no. RBAP114AMK_006) and by the project MAAT (contract no. PON02_00563_3316357). Goknur Tutuncu and Milinda Abeykoon are acknowledged for their support at X17A, Rocco Lassandro and Lucrezia Cassano for technical and administrative support. NR 44 TC 2 Z9 2 U1 10 U2 24 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1439-4235 EI 1439-7641 J9 CHEMPHYSCHEM JI ChemPhysChem PD MAR 3 PY 2016 VL 17 IS 5 BP 699 EP 709 DI 10.1002/cphc.201501175 PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DG6JR UT WOS:000372190900016 PM 26756645 ER PT J AU Williamson, CHD Sahl, JW Smith, TJ Xie, G Foley, BT Smith, LA Fernandez, RA Lindstrom, M Korkeala, H Keim, P Foster, J Hill, K AF Williamson, Charles H. D. Sahl, Jason W. Smith, Theresa J. Xie, Gary Foley, Brian T. Smith, Leonard A. Fernandez, Rafael A. Lindstrom, Miia Korkeala, Hannu Keim, Paul Foster, Jeffrey Hill, Karen TI Comparative genomic analyses reveal broad diversity in botulinum-toxin-producing Clostridia SO BMC GENOMICS LA English DT Article DE Clostridium botulinum; Botulinum neurotoxin; Whole genome sequence; Comparative genomics ID FRAGMENT LENGTH POLYMORPHISM; FIELD GEL-ELECTROPHORESIS; NEUROTOXIN COMPLEX GENES; DNA-SEQUENCING DATA; GROUP-I; INFANT BOTULISM; E STRAINS; PHYLOGENETIC ANALYSIS; HIGH-THROUGHPUT; FOOD AB Background: Clostridium botulinum is a diverse group of bacteria characterized by the production of botulinum neurotoxin. Botulinum neurotoxins are classified into serotypes (BoNT/A-G), which are produced by six species/Groups of Clostridia, but the genetic background of the bacteria remains poorly understood. The purpose of this study was to use comparative genomics to provide insights into the genetic diversity and evolutionary history of bacteria that produce the potent botulinum neurotoxin. Results: Comparative genomic analyses of over 170 Clostridia genomes, including our draft genome assemblies for 59 newly sequenced Clostridia strains from six continents and publicly available genomic data, provided in-depth insights into the diversity and distribution of BoNT-producing bacteria. These newly sequenced strains included Group I and II strains that express BoNT/A,/B,/E, or/F as well as bivalent strains. BoNT-producing Clostridia and closely related Clostridia species were delineated with a variety of methods including 16S rRNA gene, concatenated marker genes, core genome and concatenated multi-locus sequencing typing (MLST) gene phylogenies that related whole genome sequenced strains to publicly available strains and sequence types. These analyses illustrated the phylogenetic diversity in each Group and the diversity of genomic backgrounds that express the same toxin type or subtype. Comparisons of the botulinum neurotoxin genes did not identify novel toxin types or variants. Conclusions: This study represents one of the most comprehensive analyses of whole genome sequence data for Group I and II BoNT-producing strains. Read data and draft genome assemblies generated for 59 isolates will be a resource to the research community. Core genome phylogenies proved to be a powerful tool for differentiating BoNT-producing strains and can provide a framework for the study of these bacteria. Comparative genomic analyses of Clostridia species illustrate the diversity of botulinum-neurotoxin-producing strains and the plasticity of the genomic backgrounds in which bont genes are found. C1 [Williamson, Charles H. D.; Sahl, Jason W.; Keim, Paul; Foster, Jeffrey] Univ Arizona, Ctr Microbial Genet & Genom, Flagstaff, AZ 86011 USA. [Smith, Theresa J.] US Army, Med Res Inst Infect Dis, Mol & Translat Sci Div, Ft Detrick, MD 21702 USA. [Xie, Gary; Hill, Karen] Los Alamos Natl Lab, Biosci Div, POB 1663, Los Alamos, NM 87545 USA. [Foley, Brian T.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM USA. [Smith, Leonard A.] US Army, Med Res & Mat Command, Med Countermeasures Technol, Med Res Inst Infect Dis, Ft Detrick, MD 21702 USA. [Fernandez, Rafael A.] Univ Nacl Cuyo, Fac Ciencias Med, Dept Patol, Area Microbiol,Ctr Univ, RA-5500 Mendoza, Argentina. [Lindstrom, Miia; Korkeala, Hannu] Univ Helsinki, Dept Food Hyg & Environm Hlth, Helsinki, Finland. [Foster, Jeffrey] Univ New Hampshire, Dept Mol Cellular & Biomed Sci, Durham, NH 03824 USA. RP Keim, P; Foster, J (reprint author), Univ Arizona, Ctr Microbial Genet & Genom, Flagstaff, AZ 86011 USA.; Hill, K (reprint author), Los Alamos Natl Lab, Biosci Div, POB 1663, Los Alamos, NM 87545 USA.; Foster, J (reprint author), Univ New Hampshire, Dept Mol Cellular & Biomed Sci, Durham, NH 03824 USA. EM Paul.Keim@nau.edu; Jeff.Foster@unh.edu; khill@lanl.gov OI Foster, Jeffrey/0000-0001-8235-8564; xie, gary/0000-0002-9176-924X FU U.S. Department of Homeland Security Science and Technology [HSHQDC 10 C 00139, DHS-2010-ST-108-000019]; Arizona's Technology Research Initiative Fund; Arizona's Technology and Research Initiative Fund FX The work was supported by the U.S. Department of Homeland Security Science and Technology Directorate via awards HSHQDC 10 C 00139 and DHS-2010-ST-108-000019. CHDW was supported by funding from Arizona's Technology Research Initiative Fund. Some of the computational analyses were run on Northern Arizona University's Monsoon computing cluster, also funded by Arizona's Technology and Research Initiative Fund. The authors would like to thank Dr. C. Shone of Public Health England, Salisbury, UK for his kind gift of DNA from the Mauritius bont/A2 strain, and Dr. J. Rood of Monash University, Melbourne, Australia for providing C. botulinum strains for analyses. Opinions, interpretations, conclusions and recommendations are those of the authors and not necessarily endorsed by the U.S. Army. NR 104 TC 5 Z9 5 U1 7 U2 22 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2164 J9 BMC GENOMICS JI BMC Genomics PD MAR 3 PY 2016 VL 17 AR 180 DI 10.1186/s12864-016-2502-z PG 20 WC Biotechnology & Applied Microbiology; Genetics & Heredity SC Biotechnology & Applied Microbiology; Genetics & Heredity GA DF8GI UT WOS:000371595000006 PM 26939550 ER PT J AU Jager, HI Parsley, MJ Cech, JJ McLaughlin, RL Forsythe, PS Elliott, RF Pracheil, BM AF Jager, Henriette I. Parsley, Michael J. Cech, Joseph J., Jr. McLaughlin, Robert L. Forsythe, Patrick S. Elliott, Robert F. Pracheil, Brenda M. TI Reconnecting Fragmented Sturgeon Populations in North American Rivers SO FISHERIES LA English DT Article ID ADULT WHITE STURGEON; SHORTNOSE STURGEON; LAKE STURGEON; SWIMMING PERFORMANCE; UPSTREAM PASSAGE; COLUMBIA RIVER; STREAM FISHES; DAM; CONSERVATION; MANAGEMENT AB The majority of large North American rivers are fragmented by dams that interrupt migrations of wide-ranging fishes like sturgeons. Reconnecting habitat is viewed as an important means of protecting sturgeon species in U.S. rivers because these species have lost between 5% and 60% of their historical ranges. Unfortunately, facilities designed to pass other fishes have rarely worked well for sturgeons. The most successful passage facilities were sized appropriately for sturgeons and accommodated bottom-oriented species. For upstream passage, facilities with large entrances, full-depth guidance systems, large lifts, or wide fishways without obstructions or tight turns worked well. However, facilitating upstream migration is only half the battle. Broader recovery for linked sturgeon populations requires safe "round-trip" passage involving multiple dams. The most successful downstream passage facilities included nature-like fishways, large canal bypasses, and bottom-draw sluice gates. We outline an adaptive approach to implementing passage that begins with temporary programs and structures and monitors success both at the scale of individual fish at individual dams and the scale of metapopulations in a river basin. The challenge will be to learn from past efforts and reconnect North American sturgeon populations in a way that promotes range expansion and facilitates population recovery. C1 [Jager, Henriette I.; Pracheil, Brenda M.] Oak Ridge Natl Lab, Div Environm Sci, Mail Stop 6036,POB 2008, Oak Ridge, TN 37831 USA. [Parsley, Michael J.] US Geol Survey, Columbia River Res Lab, Western Fisheries Res Ctr, Cook, WA USA. [Cech, Joseph J., Jr.] Univ Calif Davis, Dept Wildlife Fish & Conservat Biol, Davis, CA 95616 USA. [McLaughlin, Robert L.] Univ Guelph, Dept Integrat Biol, Guelph, ON N1G 2W1, Canada. [Forsythe, Patrick S.] Univ Wisconsin, Dept Nat & Appl Sci, Green Bay, WI 54302 USA. [Elliott, Robert F.] US Fish & Wildlife Serv, Green Bay Fish & Wildlife Conservat Off, New Franken, WI USA. RP Jager, HI (reprint author), Oak Ridge Natl Lab, Div Environm Sci, Mail Stop 6036,POB 2008, Oak Ridge, TN 37831 USA. EM jagerhi@ornl.gov OI Jager, Henriette/0000-0003-4253-533X FU University of California, Davis; U.S. Geological Survey; U.S. Fish and Wildlife Service; Great Lakes Fishery Commission; Fisheries and Oceans Canada; University of Wisconsin, Green Bay; DOE Energy Efficiency and Renewable Energy Office, Wind and Water Power Technologies Program FX J.C. was supported by the University of California, Davis. M.P. was supported by the U.S. Geological Survey. R.E. was supported by the U.S. Fish and Wildlife Service. R.M. was supported by the Great Lakes Fishery Commission and Fisheries and Oceans Canada. P.F. was supported by University of Wisconsin, Green Bay. H.J. and B.P. were partially funded by the DOE Energy Efficiency and Renewable Energy Office, Wind and Water Power Technologies Program. NR 44 TC 1 Z9 1 U1 12 U2 26 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 0363-2415 EI 1548-8446 J9 FISHERIES JI Fisheries PD MAR 3 PY 2016 VL 41 IS 3 BP 140 EP 148 DI 10.1080/03632415.2015.1132705 PG 9 WC Fisheries SC Fisheries GA DF7GL UT WOS:000371525900001 ER PT J AU Castillo, H Schoderbek, D Dulal, S Escobar, G Wood, J Nelson, R Smith, G AF Castillo, Hugo Schoderbek, Donald Dulal, Santosh Escobar, Gabriela Wood, Jeffrey Nelson, Roger Smith, Geoffrey TI Immune responses of a wall lizard to whole-body exposure to radiofrequency electromagnetic radiation Response SO INTERNATIONAL JOURNAL OF RADIATION BIOLOGY LA English DT Letter C1 [Castillo, Hugo; Escobar, Gabriela; Smith, Geoffrey] New Mexico State Univ, Dept Biol, Las Cruces, NM 88003 USA. [Schoderbek, Donald] Univ Alberta, Dept Agr Food & Nutr Sci, Edmonton, AB, Canada. [Dulal, Santosh] Univ N Carolina, Sch Med, Chapel Hill, NC USA. [Wood, Jeffrey; Nelson, Roger] US DOE, Carlsbad Field Off, Carlsbad, NM USA. RP Smith, G (reprint author), New Mexico State Univ, Dept Biol, Las Cruces, NM 88003 USA. EM gsmith@nmsu.edu NR 3 TC 0 Z9 0 U1 0 U2 0 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 0955-3002 EI 1362-3095 J9 INT J RADIAT BIOL JI Int. J. Radiat. Biol. PD MAR 3 PY 2016 VL 92 IS 3 BP 169 EP 170 PG 2 WC Biology; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging SC Life Sciences & Biomedicine - Other Topics; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging GA DG1AG UT WOS:000371796800008 PM 27340716 ER PT J AU Coloma, P AF Coloma, Pilar TI Non-standard interactions in propagationat the Deep Underground Neutrino Experiment SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Beyond Standard Model; Neutrino Physics; CP violation ID LINE-EXPERIMENT-SIMULATOR; OSCILLATION EXPERIMENTS; STANDARD MODEL; VIOLATION; MATTER; T2K AB We study the sensitivity of current and future long-baseline neutrino oscillation experiments to the effects of dimension six operators affecting neutrino propagation through Earth, commonly referred to as Non-Standard Interactions (NSI). All relevant parameters entering the oscillation probabilities (standard and non-standard) are considered at once, in order to take into account possible cancellations and degeneracies between them. We find that the Deep Underground Neutrino Experiment will significantly improve over current constraints for most NSI parameters. Most notably, it will be able to rule out the so-called LMA-dark solution, still compatible with current oscillation data, and will be sensitive to off-diagonal NSI parameters at the level of epsilon similar to O (0.05 - 0.5). We also identify two degeneracies among standard and non-standard parameters, which could be partially resolved by combining T2HK and DUNE data. C1 [Coloma, Pilar] Fermilab Natl Accelerator Lab, Dept Theoret Phys, POB 500, Batavia, IL 60510 USA. RP Coloma, P (reprint author), Fermilab Natl Accelerator Lab, Dept Theoret Phys, POB 500, Batavia, IL 60510 USA. EM pcoloma@fnal.gov FU European Union [PITN-GA-2011-289442-INVISIBLES]; U.S. Department of Energy [DE-AC02-07CH11359] FX I am especially grateful to Enrique Fernandez-Martinez for support regarding the use of the MonteCUBES software as well as for useful discussions and comments on the manuscript. I would like to thank Jacobo Lopez-Pavon and Stephen Parke for useful comments on the manuscript, and Alexander Friedland, Andre de Gouvea and Thomas Schwetz for useful discussions. I would also like to thank David Vanegas Forero for his help in writing the T2K files with the 2013 fluxes, and Michele Maltoni for useful communications regarding the prior constraints on NSI coming from current oscillation data. I acknowledge partial support by the European Union through the ITN INVISIBLES (Marie Curie Actions, PITN-GA-2011-289442-INVISIBLES). Fermilab is operated by the Fermi Research Alliance under contract DE-AC02-07CH11359 with the U.S. Department of Energy. NR 93 TC 21 Z9 21 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAR 3 PY 2016 IS 3 AR 016 DI 10.1007/JHEP03(2016)016 PG 27 WC Physics, Particles & Fields SC Physics GA DF6AF UT WOS:000371435800003 ER PT J AU Fischer, SA Ueltschi, TW El-Khoury, PZ Mifflin, AL Hess, WP Wang, HF Cramer, CJ Govind, N AF Fischer, Sean A. Ueltschi, Tyler W. El-Khoury, Patrick Z. Mifflin, Amanda L. Hess, Wayne P. Wang, Hong-Fei Cramer, Christopher J. Govind, Niranjan TI Infrared and Raman Spectroscopy from Ab Initio Molecular Dynamics and Static Normal Mode Analysis: The C-H Region of DMSO as a Case Study SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID DENSITY-FUNCTIONAL THEORY; GENERATION VIBRATIONAL SPECTROSCOPY; SELF-CONSISTENT-FIELD; BASIS-SET; ANHARMONIC CALCULATIONS; SCATTERING MICROSCOPY; DIMETHYL-SULFOXIDE; PROTON-TRANSFER; WAVE-FUNCTIONS; SCALE FACTORS AB Carbon-hydrogen (C-H) vibration modes serve as key probes in the chemical identification of hydrocarbons and in vibrational sum-frequency generation spectroscopy of hydrocarbons at the liquid/gas interface. Their assignments pose a challenge from a theoretical viewpoint. In this work, we present a detailed study of the C-H stretching region of dimethyl sulfoxide using a new ab initio molecular dynamics (AIMD) module that we have implemented in NWChem. Through a combination of AIMD simulations and static normal mode analysis, we interpret experimental infrared and Raman spectra and explore the role of anharmonic effects in this system. Comprehensive anharmonic normal mode analysis of the C-H stretching region casts doubt upon previous experimental assignments of the shoulder on the symmetric C-H stretching peak. In addition, our AIMD simulations also show significant broadening of the in-phase symmetric C-H stretching resonance, which suggests that the experimentally observed shoulder is due to thermal broadening of the symmetric stretching resonance. C1 [Fischer, Sean A.; Wang, Hong-Fei; Govind, Niranjan] Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, POB 999, Richland, WA 99352 USA. [Ueltschi, Tyler W.; Mifflin, Amanda L.] Univ Puget Sound, Dept Chem, 1500 North Warner St, Tacoma, WA 98416 USA. [El-Khoury, Patrick Z.; Hess, Wayne P.] Pacific NW Natl Lab, Div Phys Sci, POB 999, Richland, WA 99352 USA. [Cramer, Christopher J.] Univ Minnesota, Inst Supercomp, Dept Chem, 207 Pleasant St South East, Minneapolis, MN 55455 USA. [Cramer, Christopher J.] Univ Minnesota, Chem Theory Ctr, 207 Pleasant St South East, Minneapolis, MN 55455 USA. RP Govind, N (reprint author), Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, POB 999, Richland, WA 99352 USA.; El-Khoury, PZ (reprint author), Pacific NW Natl Lab, Div Phys Sci, POB 999, Richland, WA 99352 USA. EM patrick.elkhoury@pnnl.gov; niri.govind@pnnl.gov RI Wang, Hongfei/B-1263-2010; Cramer, Christopher/B-6179-2011 OI Wang, Hongfei/0000-0001-8238-1641; Cramer, Christopher/0000-0001-5048-1859 FU U.S. Department of Energy (DOE), Office of Science, Office of Advanced Scientific Computing Research, Scientific Discovery through Advanced Computing (SciDAC) program [DE-SCO008666, KC030102062653]; Laboratory Directed Research and Development Program through a Linus Pauling Fellowship at Pacific Northwest National Laboratory (PNNL); U.S. DOE, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences [KC030102016248]; U.S. DOE, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Visiting Faculty Program (VFP); Office of Biological and Environmental Research and located at PNNL; United States Department of Energy under DOE [DE-AC05-76RL1830] FX This material is based on work supported by the U.S. Department of Energy (DOE), Office of Science, Office of Advanced Scientific Computing Research, Scientific Discovery through Advanced Computing (SciDAC) program under Award Numbers DE-SCO008666 (C.J.C.) and KC030102062653 (S.A.F, N.G.). P.Z.E. acknowledges support from the Laboratory Directed Research and Development Program through a Linus Pauling Fellowship at Pacific Northwest National Laboratory (PNNL) and an allocation of computing time from the National Science Foundation (TG-CHE130003). W.P.H. acknowledges support from the U.S. DOE, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences under Award Number KC030102016248. T.W.U. and A.L.M. were supported in part by the U.S. DOE, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Visiting Faculty Program (VFP). This work also benefitted from resources provided by PNNL Institutional Computing. This research was performed using EMSL, a DOE Office of Science User Facility sponsored by the Office of Biological and Environmental Research and located at PNNL. PNNL is operated by Battelle Memorial Institute for the United States Department of Energy under DOE contract number DE-AC05-76RL1830. NR 67 TC 6 Z9 6 U1 4 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAR 3 PY 2016 VL 120 IS 8 BP 1429 EP 1436 DI 10.1021/acs.jpcb.5b03323 PG 8 WC Chemistry, Physical SC Chemistry GA DF7UI UT WOS:000371562700005 PM 26222601 ER PT J AU Roy, S Dang, LX AF Roy, Santanu Dang, Liem X. TI Computer Simulation of Methanol Exchange Dynamics around Cations and Anions SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID INITIO MOLECULAR-DYNAMICS; GRADIENT DIFFUSION MEASUREMENTS; LIQUID METHANOL; NEUTRON-DIFFRACTION; ION-PAIR; WATER-MOLECULES; SOLVATION; INTERFACE; CHLORIDE; CONSTANTS AB In this paper, we present the first computer simulation of methanol exchange dynamics between the first and second solvation shells around different cations and anions. After water, methanol is the most frequently used solvent for ions. Methanol has different structural and dynamical properties than water, so its ion solvation process is different. To this end, we performed molecular dynamics simulations using polarizable potential models to describe methanol methanol and ion-methanol interactions. In particular, we computed methanol exchange rates by employing the transition state theory, the Impey-Madden-McDonald method, the reactive flux approach, and the Grote-Hynes theory. We observed that methanol exchange occurs at a nanosecond time scale for Na+ and at a picosecond time scale for Cs+, Cl-, and I-. We also observed a trend in which, for like charges, the exchange rate is slower for smaller ions because they are more strongly bound to methanol. C1 [Roy, Santanu; Dang, Liem X.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP Dang, LX (reprint author), Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. EM liem.dang@pnnl.gov RI Roy, Santanu/D-6215-2012 OI Roy, Santanu/0000-0001-6991-8205 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences FX This work was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences. The calculations were carried out using computer resources provided by the Office of Basic Energy Sciences. NR 36 TC 2 Z9 2 U1 0 U2 13 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAR 3 PY 2016 VL 120 IS 8 BP 1440 EP 1445 DI 10.1021/acs.jpcb.5b04174 PG 6 WC Chemistry, Physical SC Chemistry GA DF7UI UT WOS:000371562700007 PM 26086242 ER PT J AU Valiev, M Deng, SHM Wang, XB AF Valiev, Marat Deng, Shihu H. M. Wang, Xue-Bin TI How Anion Chaotrope Changes the Local Structure of Water: Insights from Photoelectron Spectroscopy and Theoretical Modeling of SCN- Water Clusters SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID MOLECULAR-ORBITAL METHODS; DOUBLY-CHARGED ANION; HOFMEISTER SERIES; AIR/WATER INTERFACE; IONS; SIMULATIONS; HYDRATION; DYNAMICS; MACROMOLECULES; MICROSOLVATION AB The behavior of charged solute molecules in aqueous solutions is often classified using the concept of kosmotropes ("structure makers") and chaotropes ("structure breakers"). There is a growing consensus that the key to kosmotropic/chaotropic behaviors lies in the local solvent region, but the exact microscopic basis for such differentiation is not well-understood. This issue is examined in this work by analyzing size selective solvation of a well-known chaotrope, a negatively charged SCN- molecule. Combining experimental photoelectron spectroscopy measurements with theoretical modeling, we examine evolution of solvation structure up to eight waters. We observe that SCN- indeed fits the description of weakly hydrated ion, and its solvation is heavily driven by stabilization of water-water interaction network. However, the impact on water structure is more subtle than that associated with "structure breaker". In particular, we observe that the solvation structure of SCN- preserves the "packing" structure of the water network but changes local directionality of hydrogen bonds in the local solvent region. The resulting effect is closer to that of "structure weakener", where solute can be readily accommodated into the native water network, at the cost of compromising its stability due to constraints on hydrogen bonding directionality. C1 [Valiev, Marat] Pacific NW Natl Lab, Environm Mol Sci Lab, POB 999, Richland, WA 99352 USA. [Deng, Shihu H. M.; Wang, Xue-Bin] Pacific NW Natl Lab, Div Phys Sci, 902 Battelle Blvd,POB 999,MS K8-88, Richland, WA 99352 USA. RP Valiev, M (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, POB 999, Richland, WA 99352 USA.; Wang, XB (reprint author), Pacific NW Natl Lab, Div Phys Sci, 902 Battelle Blvd,POB 999,MS K8-88, Richland, WA 99352 USA. EM marat.valiev@pnnl.gov; xuebin.wang@pnnl.gov FU U.S. Department of Energy (DOE); Office of Science; Office of Basic Energy Sciences; Division of Chemical Sciences; Geosciences and Biosciences; EMSL; DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory FX This work was supported by U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences, and performed using EMSL, a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory, which is operated by Battelle Memorial Institute for the DOE. NR 48 TC 1 Z9 1 U1 7 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAR 3 PY 2016 VL 120 IS 8 BP 1518 EP 1525 DI 10.1021/acs.jpcb.5b07257 PG 8 WC Chemistry, Physical SC Chemistry GA DF7UI UT WOS:000371562700015 PM 26352899 ER PT J AU Fu, L Chen, SL Wang, HF AF Fu, Li Chen, Shun-Li Wang, Hong-Fei TI Validation of Spectra and Phase in Sub-1 cm(-1) Resolution Sum-Frequency Generation Vibrational Spectroscopy through Internal Heterodyne Phase-Resolved Measurement SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID ABSOLUTE MOLECULAR-ORIENTATION; MAXIMUM-ENTROPY METHOD; AIR/WATER INTERFACE; SFG-VS; UNIFIED TREATMENT; NONLINEAR OPTICS; ALPHA-QUARTZ; SURFACE; POLARIZATION; CHIRALITY AB Reliable determination of the spectral features and their phases in sum frequency generation vibrational spectroscopy (SFG-VS) for surfaces with closely overlapping peaks has been a standing issue. Here we present two approaches toward resolving such issue. The first utilizes the high-resolution and accurate line shape from the recently developed subwavenumber high-resolution broadband SFG-VS (HR-BB-SFG-VS), from which the detail spectral parameters, including relative spectral phases, of overlapping peaks can be determined through reliable spectral fitting. These results are further Validated by using the second method that utilizes the azimuthal angle phase dependence of the z-cut a-quartz crystal, a common phase standard, through the spectral interference between the SFG fields of the quartz surface, as the internal phase reference, and the adsorbed' molecular layer. Even though this approach is limited to molecular layers that can be transferred or deposited onto the quartz surface, it is simple and straightforward, as it requires only an internal phase standard with a single measurement that is free of phase drifts. More importantly, it provides unambiguous SFG spectral phase information on such surfaces. Using this method, the absolute phase of the molecular susceptibility tensors of the CH3, CH2, and chiral C-H groups different Langmuir-Blodgett (LB) molecular monolayers and drop-cast peptide films are determined. These two approaches are fully consistent with and complement to each other, making both easily applicable tools in SFG-VS studies. More importantly, because the HR-BB-SFG-VS technique can be easily applied to various surfaces and interfaces, such validation of the spectral and phase information from HR-BB-SFG-VS measurement demonstrates it as one of the most promising tools for interrogating the detailed structure and interactions of complex molecular interfaces. C1 [Fu, Li; Chen, Shun-Li; Wang, Hong-Fei] Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, 902 Battelle Blvd,POB 999, Richland, WA 99352 USA. RP Wang, HF (reprint author), Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, 902 Battelle Blvd,POB 999, Richland, WA 99352 USA. EM hongfei.wang@pnnl.gov RI Wang, Hongfei/B-1263-2010 OI Wang, Hongfei/0000-0001-8238-1641 FU U.S. Department of Energy's (DOE) Office of Biological and Environmental Research (BER) FX H.-F.W. thanks Chuanshan Tian for discussion on eq 1. H.-F.W. also thanks Franz Geiger for suggestions in revising the manuscript. This work was conducted at the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility located at the Pacific Northwest National Laboratory (PNNL) and sponsored by the U.S. Department of Energy's (DOE) Office of Biological and Environmental Research (BER). L.F. is the William R. Wiley postdoc fellow at EMSL. S.-L.C., who is an assistant professor at the Xinjiang Technical Institute of Physics & Chemistry of the Chinese Academy of Sciences, is an Alternate Sponsored Fellow at PNNL working in EMSL. NR 56 TC 9 Z9 9 U1 12 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAR 3 PY 2016 VL 120 IS 8 BP 1579 EP 1589 DI 10.1021/acs.jpcb.5b07780 PG 11 WC Chemistry, Physical SC Chemistry GA DF7UI UT WOS:000371562700021 PM 26509581 ER PT J AU Cox, RM Armentrout, PB de Jong, WA AF Cox, Richard M. Armentrout, P. B. de Jong, Wibe A. TI Reactions of Th+ + H-2, D-2, and HD Studied by Guided Ion Beam Tandem Mass Spectrometry and Quantum Chemical Calculations SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID GUIDED-ION-BEAM; COLLISION-INDUCED DISSOCIATION; GAS-PHASE CHEMISTRY; TRANSLATIONAL ENERGY-DEPENDENCE; TRANSITION-METAL HYDRIDES; X=0-3 BOND-ENERGIES; 30 EV CM; ELECTRONIC-ENERGY; PERIODIC TRENDS; ACTINIDE CHEMISTRY AB Kinetic energy dependent reactions of Th+ with H-2, D-2, and HD were studied using a guided ion beam tandem mass spectrometer. Formation of ThH+ and ThD+ is endothermic in all cases with similar thresholds. Branching ratio results for the reaction with HD indicate that Th+ reacts via a statistical mechanism, similar to Hf+. The kinetic energy dependent cross sections for formation of ThH+ and ThD+ were evaluated to determine a 0 K bond dissociation energy (BDE) of D-0(Th+-H) = 2.45 +/- 0.07 eV. This value is in good agreement with a previous result obtained from analysis of the Th+ + CH4 reaction. D-0(Th+-H) is observed to be larger than its transition metal congeners, TiH+, ZrH+, and HfH+, believed to be a result of lanthanide contraction. The reactions with H-2 were also explored using quantum chemical calculations that include a semiempirical estimation and explicit calculation of spin-orbit contributions. These calculations agree nicely and indicate that ThH+ most likely has a (3)Delta(1) ground level with a low-lying (1)Sigma(+) excited state. Theory also provides the reaction potential energy surfaces and BDEs that are in reasonable agreement with experiment. C1 [Cox, Richard M.; Armentrout, P. B.] Univ Utah, Dept Chem, Salt Lake City, UT 84112 USA. [de Jong, Wibe A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, One Cyclotron Rd, Berkeley, CA 94720 USA. RP Armentrout, PB (reprint author), Univ Utah, Dept Chem, Salt Lake City, UT 84112 USA. EM armentrout@chem.utah.edu RI DE JONG, WIBE/A-5443-2008; Cox, Richard /C-5001-2017 OI DE JONG, WIBE/0000-0002-7114-8315; Cox, Richard /0000-0003-1812-3431 FU Heavy Element Chemistry Program, Office of Basic Energy Sciences, U.S. Department of Energy [DE-SC0012249]; DOE Office of Science User Facility [DE-AC05-00OR22725] FX This work is supported by the Heavy Element Chemistry Program, Office of Basic Energy Sciences, U.S. Department of Energy, Grant No. DE-SC0012249. We thank the Center for High Performance Computing at the University of Utah for the generous allocation of computer time. This research used resources of the Oak Ridge Leadership Computing Facility, which is a DOE Office of Science User Facility supported under Contract DE-AC05-00OR22725. An award of computer time was provided by the Innovative and Novel Computational Impact on Theory and Experiment (INCITE) program. NR 115 TC 1 Z9 1 U1 3 U2 9 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAR 3 PY 2016 VL 120 IS 8 BP 1601 EP 1614 DI 10.1021/acs.jpcb.5b08008 PG 14 WC Chemistry, Physical SC Chemistry GA DF7UI UT WOS:000371562700023 PM 26414691 ER PT J AU Batista, APD Zahariev, F Slowing, II Braga, AAC Ornellas, FR Gordon, MS AF de Lima Batista, Ana P. Zahariev, Federico Slowing, Igor I. Braga, Ataualpa A. C. Ornellas, Fernando R. Gordon, Mark S. TI Silanol-Assisted Carbinolamine Formation in an Amine-Functionalized Mesoporous Silica Surface: Theoretical Investigation by Fragmentation Methods SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID MOLECULAR-ORBITAL METHOD; SI(100)-2 X-1 SURFACE; MM3 FORCE-FIELD; COOPERATIVE CATALYSIS; ALDOL REACTION; MECHANICS; SYSTEMS; BASE; EFFICIENT; ACID AB The aldol reaction catalyzed by an amine-substituted mesoporous silica nanoparticle (amine-MSN) surface was investigated using a large molecular cluster model (Si392O958C6NH361) combined with the surface integrated molecular orbital/molecular mechanics (SIMOMM) and fragment molecular orbital (FMO) methods. Three distinct pathways for the carbinolamine formation, the first step of the amine-catalyzed aldol reaction, are proposed and investigated in order to elucidate the role of the silanol environment on the catalytic capability of the amine-MSN material. The computational study reveals that the most likely mechanism involves the silanol groups actively participating in the reaction, forming and breaking covalent bonds in the carbinolamine step. Therefore, the active participation of MSN silanol groups in the reaction mechanism leads to a significant reduction in the overall energy barrier for the carbinolamine formation. In addition, a comparison between the findings using a minimal cluster model and the Si392O958C6NH361 cluster suggests that the use of larger models is important when heterogeneous catalysis problems are the target. C1 [de Lima Batista, Ana P.; Braga, Ataualpa A. C.; Ornellas, Fernando R.] Inst Quim, Dept Quim Fundamental, BR-05508000 Sao Paulo, SP, Brazil. [Zahariev, Federico; Slowing, Igor I.; Gordon, Mark S.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Zahariev, Federico; Slowing, Igor I.; Gordon, Mark S.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. RP Gordon, MS (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA.; Gordon, MS (reprint author), Iowa State Univ, Dept Chem, Ames, IA 50011 USA. EM mark@si.msg.chem.iastate.edu RI Institute of Chemistry - USP, Dept. of Chemistry/B-8988-2012; Braga, Ataualpa/G-3757-2012; de Lima Batista, Ana Paula/K-8719-2013; OI Braga, Ataualpa/0000-0001-7392-3701; de Lima Batista, Ana Paula/0000-0002-9675-6106; Slowing, Igor/0000-0002-9319-8639 FU Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq) of Brazil; CNPq [236761/2012-9]; Sao Paulo Research Foundation (FAPESP) [2013/22235-0]; Computation Center of the University of Sao Paulo (LCCA-USP)/Rice University (National Science Foundation) [OCI-0959097]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; U.S. Department of Energy by Iowa State University [DE-AC02-07CH11358] FX F.R.O. acknowledges the Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq) of Brazil for academic support. A.P.d.L.B. gratefully acknowledges Grant #236761/2012-9 CNPq, Grant #2013/22235-0 Sao Paulo Research Foundation (FAPESP), and the support of the Computation Center of the University of Sao Paulo (LCCA-USP)/Rice University (National Science Foundation Grant OCI-0959097). I.I.S., F.Z., and M.S.G. were supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, through the Ames Laboratory Catalysis Science and Chemical Physics programs, respectively. The Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract DE-AC02-07CH11358. NR 68 TC 0 Z9 0 U1 3 U2 10 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAR 3 PY 2016 VL 120 IS 8 BP 1660 EP 1669 DI 10.1021/acs.jpcb.5b08446 PG 10 WC Chemistry, Physical SC Chemistry GA DF7UI UT WOS:000371562700029 ER PT J AU Pluharova, E Baer, MD Schenter, GK Jungwirth, P Mundy, CJ AF Pluharova, Eva Baer, Marcel D. Schenter, Gregory K. Jungwirth, Pavel Mundy, Christopher J. TI Dependence of the Rate of LiF Ion-Pairing on the Description of Molecular Interaction SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID TRANSITION-STATE THEORY; ACTIVATED CHEMICAL-REACTIONS; NONEQUILIBRIUM SOLVATION; RATE-CONSTANT; HYDRATION STRUCTURE; POLARIZABLE WATER; DYNAMICS; SOLVENT; NUCLEATION; FRICTION AB We present an analysis of the dynamics of ion-pairing of lithium fluoride (LiF) in aqueous solvent using both detailed molecular simulation as well as reduced models within a generalized Langevin equation (GLE) framework. We explored the sensitivity of the ion-pairing phenomena to the details of descriptions of molecular interaction, comparing two empirical potentials to explicit quantum based density functional theory. We find quantitative differences in the potentials of mean force for ion pairing as well as time dependent frictions that lead to variations in the rate constant and reactive flux correlation functions. These details reflect differences in solvent response to ion-pairing between different representations of molecular interaction and influence anharmonicity of the dynamic response. We find that the short-time anharmonic response is recovered with a GLE parametrization. Recovery of the details of long time response may require extensions to the reduced model. We show that the utility of using a reduced model leads to a straightforward application of variational transition state theory concepts to the condensed phase system. The significance of this is reflected in the analysis of committor distributions and the variation of planar hypersurfaces, leading to an improved understanding of factors that determine the rate of LiF ion-pairing. C1 [Pluharova, Eva; Jungwirth, Pavel] Acad Sci Czech Republic, Inst Organ Chem & Biochem, Flemingovo Nam 2, CR-16610 Prague 6, Czech Republic. Univ Paris 06, Ecole Normale Super PSL Res Univ, Dept Chem, CNRS UMR 8640,Sorbonne Univ, 24 Rue Lhomond, F-75005 Paris, France. [Baer, Marcel D.; Schenter, Gregory K.; Mundy, Christopher J.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP Schenter, GK (reprint author), Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. EM greg.schenter@pnnl.gov RI Pluharova, Eva/B-1092-2012; Jungwirth, Pavel/D-9290-2011 OI Jungwirth, Pavel/0000-0002-6892-3288 FU U.S. Department of Energy's (DOE) Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences; Laboratory Directed Research and Development under PNNL's Laboratory Initiative Materials Synthesis and Simulation across Scales (MS3); PNNL's Alternate Sponsored Fellowship program; IMPRS Dresden; Czech Science Foundation [P208/12/G016]; Academy of Sciences (Praemium Academie award); Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX C.J.M. and G.K.S. are supported by the U.S. Department of Energy's (DOE) Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences. Pacific Northwest National Laboratory (PNNL) is operated for the Department of Energy by Battelle. M.D.B. is grateful for the support of Laboratory Directed Research and Development funding under the auspices of PNNL's Laboratory Initiative Materials Synthesis and Simulation across Scales (MS3). Additional computing resources were generously allocated by PNNL's Institutional Computing program. E.P. acknowledges support from PNNL's Alternate Sponsored Fellowship program and IMPRS Dresden. Support to P.J. from the Czech Science Foundation (Grant P208/12/G016) and the Academy of Sciences (Praemium Academie award) is gratefully acknowledged. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 58 TC 6 Z9 6 U1 4 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAR 3 PY 2016 VL 120 IS 8 BP 1749 EP 1758 DI 10.1021/acs.jpcb.5b09344 PG 10 WC Chemistry, Physical SC Chemistry GA DF7UI UT WOS:000371562700039 PM 26501355 ER PT J AU Walker, JA Mezyk, SP Roduner, E Bartels, DM AF Walker, J. A. Mezyk, S. P. Roduner, E. Bartels, D. M. TI Isotope Dependence and Quantum Effects on Atomic Hydrogen Diffusion in Liquid Water SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID ELECTRON-SPIN EXCHANGE; AQUEOUS-SOLUTION; DEUTERIUM ATOMS; RATE-CONSTANT; FREE-RADICALS; H-ATOMS; MUONIUM; POLARIZATION; TEMPERATURE; RADIOLYSIS AB Relative diffusion coefficients were determined in water for the D, H, and Mu isotopes of atomic hydrogen by measuring their diffusion-limited' spin-exchange rate constants with Ni2+ as a function of temperature. H and D atoms were generated by pulse radiolysis of water and measured by time-resolved pulsed EPR. Mu atoms are detected by muonium spin resonance. To isolate the atomic mass effect from solvent isotope effect, we measured all three spin-exchange rates in 90% D2O. The diffusion depends on the atomic mass, demonstrating breakdown of Stokes-Einstein behavior. The diffusion can be understood using a combination of water "cavity diffusion" and "hopping" mechanisms, as has been proposed in the literature. The H/D isotope effect agrees with previous modeling using ring polymer molecular dynamics. The "quantum swelling" effect on muonium due to its larger de Broglie wavelength does not seem to slow its "hopping" diffusion as much as predicted in previous work. Quantum effects of both the atom mass and the water librations have been modeled using RPMD and a qTIP4P/f quantized flexible water model. These results suggest that the muonium diffusion is very sensitive to the Mu versus water potential used. C1 [Walker, J. A.; Bartels, D. M.] Notre Dame Univ, Radiat Lab, Notre Dame, IN 46556 USA. [Walker, J. A.; Bartels, D. M.] Notre Dame Univ, Dept Chem & Biochem, Notre Dame, IN 46556 USA. [Bartels, D. M.] Argonne Natl Lab, Div Chem, 9700 S Cass Ave, Argonne, IL 60439 USA. [Mezyk, S. P.] Calif State Univ Long Beach, Dept Chem & Biochem, 1250 Bellflower Blvd, Long Beach, CA 90840 USA. [Roduner, E.] Univ Stuttgart, Inst Phys Chem, Pfaffenwaldring 55, D-70569 Stuttgart, Germany. [Roduner, E.] Univ Pretoria, Dept Chem, ZA-0002 Pretoria, South Africa. RP Bartels, DM (reprint author), Notre Dame Univ, Radiat Lab, Notre Dame, IN 46556 USA.; Bartels, DM (reprint author), Notre Dame Univ, Dept Chem & Biochem, Notre Dame, IN 46556 USA.; Bartels, DM (reprint author), Argonne Natl Lab, Div Chem, 9700 S Cass Ave, Argonne, IL 60439 USA. EM bartels.5@nd.edu FU Office of Science, Division of Chemical Science, US-DOE [W-31-109-ENG-38]; Paul Scherrer Institute in Villigen, Switzerland; Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-FC02-04ER15533] FX Work at Argonne National Laboratory was performed under the auspices of the Office of Science, Division of Chemical Science, US-DOE under contract number W-31-109-ENG-38. Muon work was conducted at and supported by the Paul Scherrer Institute in Villigen, Switzerland. Work at Notre Dame was supported by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy through award DE-FC02-04ER15533. This is manuscript number 5088 of the Notre Dame Radiation Laboratory. NR 46 TC 0 Z9 0 U1 10 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAR 3 PY 2016 VL 120 IS 8 BP 1771 EP 1779 DI 10.1021/acs.jpcb.5b09375 PG 9 WC Chemistry, Physical SC Chemistry GA DF7UI UT WOS:000371562700041 PM 26623663 ER PT J AU You, XL Chaudhari, MI Rempe, SB Pratt, LR AF You, Xinli Chaudhari, Mangesh I. Rempe, Susan B. Pratt, Lawrence R. TI Dielectric Relaxation of Ethylene Carbonate and Propylene Carbonate from Molecular Dynamics Simulations SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID DIFFUSION; PHASE AB Ethylene carbonate (EC) and propylene carbonate (PC) are widely used solvents in lithium (Li)-ion batteries and supercapacitors. Ion dissolution and diffusion in those media are correlated with solvent dielectric responses. Here, we use all-atom molecular dynamics simulations of the pure solvents to calculate dielectric constants and relaxation times, and molecular mobilities. The computed results are compared with limited available experiments to assist more exhaustive studies of these important characteristics. The observed agreement is encouraging and provides guidance for further validation of force-field simulation models for EC and PC solvents. C1 [You, Xinli; Pratt, Lawrence R.] Tulane Univ, Dept Biomol & Chem Engn, New Orleans, LA 70118 USA. [Chaudhari, Mangesh I.; Rempe, Susan B.] Sandia Natl Labs, Ctr Biol & Engn Sci, POB 5800, Albuquerque, NM 87185 USA. RP Rempe, SB (reprint author), Sandia Natl Labs, Ctr Biol & Engn Sci, POB 5800, Albuquerque, NM 87185 USA. EM slrempe@sandia.gov FU U.S. Department of Energy's (DOE) National Nuclear Security Administration [DE-AC04-94AL85000]; Sandia's LDRD program, DOE; Battery Materials Research Program of the Office of Energy Efficiency & Renewable Energy, Office of Vehicle Technologies, Department of Energy; National Science Foundation under the NSF EPSCoR [EPS-1003897]; Louisiana Board of Regents; U.S DOE's Office of Science by Los Alamos National Laboratory [DE-AC52-06NA25396] FX Sandia National Laboratories (SNL) is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's (DOE) National Nuclear Security Administration under Contract DE-AC04-94AL85000. This work was supported by Sandia's LDRD program, DOE, and the Battery Materials Research Program of the Office of Energy Efficiency & Renewable Energy, Office of Vehicle Technologies, Department of Energy (MIC and SBR). We acknowledge the National Science Foundation under the NSF EPSCoR Cooperative Agreement No. EPS-1003897, with additional support from the Louisiana Board of Regents (X.Y. and L.R.P.). This work was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S DOE's Office of Science by Los Alamos National Laboratory (Contract DE-AC52-06NA25396) and SNL. NR 21 TC 5 Z9 5 U1 7 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAR 3 PY 2016 VL 120 IS 8 BP 1849 EP 1853 DI 10.1021/acs.jpcb.5b09561 PG 5 WC Chemistry, Physical SC Chemistry GA DF7UI UT WOS:000371562700050 PM 26599721 ER PT J AU Chaudhari, MI Rempe, SB Asthagiri, D Tan, L Pratt, LR AF Chaudhari, Mangesh I. Rempe, Susan B. Asthagiri, D. Tan, L. Pratt, L. R. TI Molecular Theory and the Effects of Solute Attractive Forces on Hydrophobic Interactions SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID SCALED-PARTICLE THEORY; INVERSE TEMPERATURE TRANSITION; ELASTIN-LIKE POLYPEPTIDE; AQUEOUS-SOLUTIONS; NONPOLAR GASES; LCST BEHAVIOR; FREE-ENERGY; WATER; HYDRATION; DYNAMICS AB The role of solute attractive forces on hydrophobic interactions is studied by coordinated development of theory and simulation results for Ar atoms in water. We present a concise derivation of the local molecular field (LMF) theory for the effects of solute attractive forces on hydrophobic interactions, a derivation that clarifies the close relation of LMF theory to the EXP approximation applied to this problem long ago. The simulation results show that change from purely repulsive atomic solute interactions to include realistic attractive interactions diminishes the strength of hydrophobic bonds. For the Ar-Ar rdfs considered pointwise, the numerical results for the effects of solute attractive forces on hydrophobic interactions are opposite in sign and larger in magnitude than predicted by LMF theory. That comparison is discussed from the point of view of quasichemical theory, and it is suggested that the first reason for this difference is the incomplete evaluation within LMF theory of the hydration energy of the Ar pair. With a recent suggestion for the system-size extrapolation of the required correlation function integrals, the Ar-Ar rdfs permit evaluation of osmotic second virial coefficients B-2. Those B-2's also show that incorporation of attractive interactions leads to more positive (repulsive) values. With attractive interactions in play, B-2, can change from positive to negative values with increasing temperatures. This is consistent with the puzzling suggestions of decades ago that B-2 approximate to 0 for intermediate cases of temperature or solute size. In all cases here, B-2 becomes more attractive with increasing temperature. C1 [Chaudhari, Mangesh I.; Rempe, Susan B.] Sandia Natl Labs, Ctr Biol & Mat Sci, POB 5800, Albuquerque, NM 87185 USA. [Asthagiri, D.] Rice Univ, Dept Biomol & Chem Engn, Houston, TX 77005 USA. [Tan, L.; Pratt, L. R.] Tulane Univ, Dept Biomol & Chem Engn, New Orleans, LA 70118 USA. RP Pratt, LR (reprint author), Tulane Univ, Dept Biomol & Chem Engn, New Orleans, LA 70118 USA. EM lpratt@tulane.edu RI Asthagiri, Dilipkumar/P-9450-2016 OI Asthagiri, Dilipkumar/0000-0001-5869-0807 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL8500]; Sandia's LDRD program; Gulf of Mexico Research Initiative [SA 12-05/GoMRI-002] FX We thank J. D. Weeks (University of Maryland) for helpful discussions. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL8500. The financial support of Sandia's LDRD program and the Gulf of Mexico Research Initiative (Consortium for Ocean Leadership Grant SA 12-05/GoMRI-002) is gratefully acknowledged. NR 74 TC 3 Z9 3 U1 5 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAR 3 PY 2016 VL 120 IS 8 BP 1864 EP 1870 DI 10.1021/acs.jpcb.5b09552 PG 7 WC Chemistry, Physical SC Chemistry GA DF7UI UT WOS:000371562700052 PM 26694688 ER PT J AU Baer, MD Mundy, CJ AF Baer, Marcel D. Mundy, Christopher J. TI Local Aqueous Solvation Structure Around Ca2+ During Ca2+center dot center dot center dot Cl- Pair Formation SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID MOLECULAR-DYNAMICS SIMULATION; DENSITY-FUNCTIONAL THEORY; X-RAY-DIFFRACTION; QUASI-CHEMICAL THEORY; HYDRATED CALCIUM-ION; AB-INITIO; ACCURATE DESCRIPTION; DIVALENT-CATIONS; FREE-ENERGIES; WATER AB The molecular details of single ion solvation around Ca2+ and ion-pairing of Ca2+center dot center dot center dot Cl- are investigated using ab initio molecular dynamics. The use of empirical dispersion corrections to the BLYP functional are investigated by comparison to experimentally available extended X-ray absorption fine structure (EXAFS) measurements that probe the first solvation shell in great detail. Besides finding differences in the free-energy for both ion-pairing and the coordination number of ion solvation between the quantum and classical descriptions of interaction, there were important differences found between dispersion corrected and uncorrected density functional theory (DFT). Specifically, we show significantly different free-energy landscapes for both coordination number of Ca2+ and its ion-pairing with Cl- depending on the DFT simulation protocol. Our findings produce a self-consistent treatment of short-range solvent response to the ion and the intermediate to long-range collective response of the electrostatics of the ion-ion interaction to produce a detailed picture of ion-pairing that is consistent with experiment. C1 [Baer, Marcel D.; Mundy, Christopher J.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99354 USA. RP Baer, MD; Mundy, CJ (reprint author), Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99354 USA. EM marcel.baer@pnnl.gov; chris.mundy@pnnl.gov FU MS3 (Materials Synthesis and Simulation Across Scales) Initiative at Pacific Northwest National Laboratory; US Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX M.D.B. is supported by MS3 (Materials Synthesis and Simulation Across Scales) Initiative at Pacific Northwest National Laboratory. It was conducted under the Laboratory Directed Research and Development Program at PNNL, a multiprogram national laboratory operated by Battelle for the U.S. Department of Energy. C.J.M. acknowledges support from US Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Additional computing resources were generously allocated by PNNL's Institutional Computing program. The authors thank Tom Beck for discussions regarding QCT, and John Fulton, Tim Duignan, Greg Schenter, and Shawn Kathmann for insightful comments. NR 73 TC 4 Z9 4 U1 5 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAR 3 PY 2016 VL 120 IS 8 BP 1885 EP 1893 DI 10.1021/acs.jpcb.5b09579 PG 9 WC Chemistry, Physical SC Chemistry GA DF7UI UT WOS:000371562700054 PM 26788746 ER PT J AU Smith, RS May, RA Kay, BD AF Smith, R. Scott May, R. Alan Kay, Bruce D. TI Desorption Kinetics of Ar, Kr, Xe, N-2, O-2, CO, Methane, Ethane, and Propane from Graphene and Amorphous Solid Water Surfaces SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID TEMPERATURE-PROGRAMMED DESORPTION; MOLECULAR-HYDROGEN FORMATION; INCIDENT COLLISION ENERGY; THERMAL-DESORPTION; INTERSTELLAR ICES; DISPLACEMENT KINETICS; N-ALKANES; ADSORPTION; FILMS; MORPHOLOGY AB The desorption kinetics for Ar, Kr, Xe, N-2, O-2, CO, methane, ethane, and propane from graphene-covered Pt(111) and amorphous solid water (ASW) surfaces are investigated using temperature-programmed desorption (TPD). The TPD spectra for all of the adsorbates from graphene have well-resolved first, second, third, and multilayer desorption peaks. The alignment of the leading edges is consistent the zero-order desorption for all of the adsorbates. An Arrhenius analysis is used to obtain desorption energies and prefactors for desorption from graphene for all of the adsorbates. In contrast, the leading desorption edges for the adsorbates from ASW do not align (for coverages < 2 ML). The nonalignment of TPD leading edges suggests that there are multiple desorption binding sites on the ASW surface. Inversion analysis is used to obtain the coverage dependent desorption energies and prefactors for desorption from ASW for all of the adsorbates. C1 [Smith, R. Scott; May, R. Alan; Kay, Bruce D.] Pacific NW Natl Lab, Phys & Computat Sci Directorate, Richland, WA 99352 USA. RP Smith, RS; Kay, BD (reprint author), Pacific NW Natl Lab, Phys & Computat Sci Directorate, Richland, WA 99352 USA. EM scott.smith@pnnl.gov; bruce.kay@pnnl.gov RI Smith, Scott/G-2310-2015 OI Smith, Scott/0000-0002-7145-1963 FU U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory; DOE [DE-AC05-76RL01830] FX This work was supported by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences. The research was performed using EMSL, a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory, which is operated by Battelle for the DOE under Contract No. DE-AC05-76RL01830. NR 47 TC 5 Z9 5 U1 6 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAR 3 PY 2016 VL 120 IS 8 BP 1979 EP 1987 DI 10.1021/acs.jpcb.5b10033 PG 9 WC Chemistry, Physical SC Chemistry GA DF7UI UT WOS:000371562700063 PM 26595145 ER PT J AU Pandit, B Jackson, NE Zheng, TY Fauvell, TJ Manley, EF Orr, M Brown-Xu, S Yu, LP Chen, LX AF Pandit, Bill Jackson, Nicholas E. Zheng, Tianyue Fauvell, Thomas J. Manley, Eric F. Orr, Meghan Brown-Xu, Samantha Yu, Luping Chen, Lin X. TI Molecular Structure Controlled Transitions between Free-Charge Generation and Trap Formation in a Conjugated Copolymer Series SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID POLYMER SOLAR-CELLS; DONOR-ACCEPTOR COPOLYMERS; ORGANIC PHOTOVOLTAICS; EFFICIENT TANDEM; RATIONAL DESIGN; TRANSFER STATE; DYNAMICS; TRANSPORT; DEVICES; MODELS AB Rational design strategies for controlling the energetics of conjugated "donor-acceptor" copolymers are ubiquitous in the literature, as they allow for simple energy-level tuning strategies to be employed for photovoltaic and transistor applications. Utilizing the recently reported PTRn series of conjugated polymers closely related to the widely implemented material PTB7, we investigate the effect of local copolymer block energetics on the generation of transient excitonic and charge carrier species. It is clearly demonstrated that local copolymer block energetics play a much larger role than is apparent from simple energy-level tuning arguments, and drastically affect the ultrafast generation of free-charge carrier and trap state populations. Specifically, we observe an almost complete reversal in the efficient generation of free-charge in PTB7 to the ultrafast creation of a high percentage of trapped pseudo charge-transfer states. The implications of this secondary effect of "donor-acceptor" energy level tuning are discussed, along with strategies for avoiding the generation of trap states in "donor-acceptor" copolymers. C1 [Pandit, Bill; Jackson, Nicholas E.; Fauvell, Thomas J.; Manley, Eric F.; Orr, Meghan; Brown-Xu, Samantha; Chen, Lin X.] Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Pandit, Bill; Jackson, Nicholas E.; Fauvell, Thomas J.; Manley, Eric F.; Orr, Meghan; Brown-Xu, Samantha; Chen, Lin X.] Northwestern Univ, Argonne Northwestern Solar Energy Res Ctr, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Zheng, Tianyue; Yu, Luping] Univ Chicago, Dept Chem, 929 East 57th St, Chicago, IL 60637 USA. [Zheng, Tianyue; Yu, Luping] Univ Chicago, James Franck Inst, 929 East 57th St, Chicago, IL 60637 USA. [Jackson, Nicholas E.; Fauvell, Thomas J.; Manley, Eric F.; Chen, Lin X.] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Lemont, IL 60439 USA. RP Chen, LX (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA.; Chen, LX (reprint author), Northwestern Univ, Argonne Northwestern Solar Energy Res Ctr, 2145 Sheridan Rd, Evanston, IL 60208 USA.; Yu, LP (reprint author), Univ Chicago, Dept Chem, 929 East 57th St, Chicago, IL 60637 USA.; Yu, LP (reprint author), Univ Chicago, James Franck Inst, 929 East 57th St, Chicago, IL 60637 USA.; Chen, LX (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Lemont, IL 60439 USA. EM lupingyu@uchicago.edu; l-chen@northwestern.edu RI Zheng, Tianyue/P-2674-2016 FU Sustainable Energy Pathways Program of the National Science Foundation [DMR-1230217, DMR-1263006]; NIST CHiMAD program; Northwestern Presidential Fellowship; ANSER Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001059] FX This work is support by the Sustainable Energy Pathways Program of the National Science Foundation (Grant number DMR-1230217 for L.X.C. and DMR-1263006 for L.Y.). L.Y. also would like to acknowledge the support from the NIST CHiMAD program. N.E.J. would like to thank the Northwestern Presidential Fellowship for funding. T.J.F. and E.F.M. are supported by ANSER Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award number DE-SC0001059. NR 51 TC 1 Z9 1 U1 5 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 3 PY 2016 VL 120 IS 8 BP 4189 EP 4198 DI 10.1021/acs.jpcc.5b10291 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DF7UB UT WOS:000371562000004 ER PT J AU Young, JL Doscher, H Turner, JA Deutsch, TG AF Young, James L. Doescher, Henning Turner, John A. Deutsch, Todd G. TI Reversible GaInP2 Surface Passivation by Water Adsorption: A Model System for Ambient-Dependent Photoluminescence SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID HYDROGEN-PRODUCTION; SOLAR-CELLS; INTERFACE AB The photoluminescence (PL) intensity of semiconductors can be modulated by their ambient. We show GaInP2 to respond reversibly to water vapor, irreversibly to oxygen, and with a time dependence to air. We characterize the reversible PL response to water vapor in a set of steady-state measurements that reveal a systematic dependence on pressure. We derive a model for this behavior based on Langmuir adsorption and Shockley-Read-Hall recombination principles to describe how partial pressure controls luminescence. The expression for the GaInP2/water vapor system shows excellent agreement to measurements. Combined, the PL monitoring technique and model demonstrate a quantitative approach for probing gas/surface defect interactions of semiconductor processing steps, luminescence-based sensors, and photocatalytic surfaces. C1 [Young, James L.; Doescher, Henning; Turner, John A.; Deutsch, Todd G.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Young, James L.] Univ Colorado, Mat Sci & Engn Program, Boulder, CO 80309 USA. [Doescher, Henning] Univ Marburg, D-35032 Marburg, Germany. RP Deutsch, TG (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM todd.deutsch@nrel.gov FU National Science Foundation Graduate Research Fellowship Program [DGE 1144083]; EU Marie Curie fellowship [300971]; NREL [DE-AC36-08GO28308] FX J.L.Y. acknowledges support from the National Science Foundation Graduate Research Fellowship Program Award No. DGE 1144083 and acknowledges Steven George for advice and use of the ALD reactor modified for PL measurements. H.D. appreciates financial support by an EU Marie Curie fellowship (IOF No. 300971). This work was supported by the U.S. Department of Energy (DOE) Fuel Cell Technology Office under Contract No. DE-AC36-08GO28308 with NREL. NR 32 TC 1 Z9 1 U1 0 U2 9 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 3 PY 2016 VL 120 IS 8 BP 4418 EP 4422 DI 10.1021/acs.jpcc.5b12498 PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DF7UB UT WOS:000371562000029 ER PT J AU Shi, R Xu, JZ Liu, GK Zhang, XJ Zhou, WJ Pan, FJ Huang, Y Tao, Y Liang, HB AF Shi, Rui Xu, Jinzhong Liu, Guokui Zhang, Xuejie Zhou, Weijie Pan, Fengjuan Huang, Yan Tao, Ye Liang, Hongbin TI Spectroscopy and Luminescence Dynamics of Ce3+ and Sm3+ in LiYSiO4 SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ORBIT-LATTICE RELAXATION; RARE-EARTH IONS; ENERGY-TRANSFER; OPTICAL-PROPERTIES; VIBRONIC TRANSITIONS; CROSS-RELAXATION; CRYSTAL-GROWTH; EXCITATION; PHOSPHORS; GLASSES AB The lithium yttrium silicate series of LiY1-x-Ln(x)SiO(4) exhibits superb chemical and optical properties, and with Ln = Ce3+, Sm3+, its spectroscopic characteristics and luminescence dynamics are investigated in the present work. Energy transfer and nonradiative relaxation dramatically influence the Ln(3+) luminescence spectra and decay dynamics, especially in the Ce3+ Sm3+ codoped phosphors. It is shown that thermal-quenching of the blue Ce3+ luminescence is primarily due to thermal ionization in the 5d excited states rather than multiphonon relaxation, whereas cross-relaxation arising from electric dipole dipole interaction between adjacent Sm3+ ions is the leading mechanism that quenches the red Sm3+ luminescence. In the codoped systems, Ce3+-Sm3+ energy transfer in competing with the thermal quenching enhance the emission from Sm3+. The combined influences of concentration quenching, thermal ionization, and energy transfer including cross-relaxation on the luminescence intensity of single-center and codoped phosphors are analyzed based on the theories of ion-ion and ion-lattice interactions. C1 [Shi, Rui; Xu, Jinzhong; Zhang, Xuejie; Zhou, Weijie; Pan, Fengjuan; Liang, Hongbin] Sun Yat Sen Univ, Sch Chem & Chem Engn, KLGHEI Environm & Energy Chem, MOE Key Lab Bioinorgan & Synthet Chem, Guangzhou 510275, Guangdong, Peoples R China. [Liu, Guokui] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Huang, Yan; Tao, Ye] Chinese Acad Sci, Inst High Energy Phys, Beijing Synchrotron Radiat Facil, Beijing 100039, Peoples R China. RP Liang, HB (reprint author), Sun Yat Sen Univ, Sch Chem & Chem Engn, KLGHEI Environm & Energy Chem, MOE Key Lab Bioinorgan & Synthet Chem, Guangzhou 510275, Guangdong, Peoples R China.; Liu, GK (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. EM gkliu@anl.gov; cesbin@mail.sysu.edu.cn OI Zhou, Weijie/0000-0001-5199-9836 FU National Natural Science Foundation of China [21171176, U1232108, U1432249]; Natural Science Foundation of Guangdong Province [S2013030012842]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-AC02-06CH11357] FX This work is financially supported by the National Natural Science Foundation of China (21171176, U1232108, and U1432249), and the Natural Science Foundation of Guangdong Province (S2013030012842). G.L. acknowledges the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences through Grant DE-AC02-06CH11357 for funding the work on heavy elements chemistry, and travel support from the CAS/SAFEA International Partnership Program for Creative Research Teams. NR 52 TC 12 Z9 12 U1 14 U2 41 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 3 PY 2016 VL 120 IS 8 BP 4529 EP 4537 DI 10.1021/acs.jpcc.5b12501 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DF7UB UT WOS:000371562000042 ER PT J AU Li, J Liu, CH Ye, YF Zhu, JF Wang, SD Guo, JH Sham, TK AF Li, Jun Liu, Changhai Ye, Yifan Zhu, Junfa Wang, Suidong Guo, Jinghua Sham, Tsun-Kong TI Tracking the Local Effect of Fluorine Self-Doping in Anodic TiO2 Nanotubes SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID POLARIZATION DEPENDENCE; PHOTOCATALYTIC ACTIVITY; NANOCRYSTALLINE TIO2; HYDROGEN GENERATION; TITANIA NANOTUBES; SOLAR ABSORPTION; ARRAYS; SPECTROSCOPY; ANATASE; MORPHOLOGY AB We report herein a study in which we reveal the role of F- incorporated in the very anodic TiO2 nanotubes prepared electrochemically from a Ti foil using a fluoride based electrolyte. X-ray absorption near edge structure (XANES), resonant X-ray emission spectroscopy (RXES), and X-ray photoelectron spectroscopy (XPS) have been used to examine the as-prepared and the annealed TiO2 nanotubes. It is found that the additional electron resulting from the substitution of O-2(-) by self-doped F- in the TiO2 lattice is localized in the t(2g) state. Consequently, a localized Ti3+ state can be tracked by a d-d energy loss peak with a constant energy of 1.6 eV in the RXES, in contrast to TiO2 nanostructures where this peak is hardly noticeable when F- is driven out of the lattice upon annealing. C1 [Li, Jun; Sham, Tsun-Kong] Univ Western Ontario, Dept Chem, 1151 Richmond St, London, ON N6A 5B7, Canada. [Liu, Changhai; Wang, Suidong; Sham, Tsun-Kong] Soochow Univ, Inst Funct Nano & Soft Mat FUNSOM, Soochow Univ Western Univ Joint Ctr Synchrotron R, Suzhou 215123, Jiangsu, Peoples R China. [Ye, Yifan; Zhu, Junfa] Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230029, Anhui, Peoples R China. [Ye, Yifan; Zhu, Junfa] Univ Sci & Technol China, Collaborat Innovat Ctr Suzhou Nano Sci & Technol, Hefei 230029, Anhui, Peoples R China. [Ye, Yifan; Guo, Jinghua] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Guo, Jinghua] Univ Calif Santa Cruz, Dept Chem & Biochem, Santa Cruz, CA 95064 USA. RP Sham, TK (reprint author), Univ Western Ontario, Dept Chem, 1151 Richmond St, London, ON N6A 5B7, Canada.; Sham, TK (reprint author), Soochow Univ, Inst Funct Nano & Soft Mat FUNSOM, Soochow Univ Western Univ Joint Ctr Synchrotron R, Suzhou 215123, Jiangsu, Peoples R China. EM tsham@uwo.ca RI Zhu, Junfa/E-4020-2010; 刘, 长海/F-9445-2013; Li, Jun/I-8384-2012 OI Zhu, Junfa/0000-0003-0888-4261; 刘, 长海/0000-0001-6774-5216; Li, Jun/0000-0002-1958-5665 FU Natural Science and Engineering Research Council of Canada (NSERC); Canada Research Chair (CRC) Program; Canada Foundation for Innovation (CFI); Interdisciplinary Initiative (IDI) grant of the University of Western Ontario (UWO); CFI; NSERC; National Research Council (NRC); Canadian Institute for Health Research (CIHR); University of Saskatchewan; Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; CLS Graduate Student Travel Support Program; National Natural Science Foundation of China [U1232102, 21473178] FX Research at the University of Western Ontario is supported by the Discovery grant of the Natural Science and Engineering Research Council of Canada (NSERC), the Canada Research Chair (CRC) Program, the Canada Foundation for Innovation (CFI), and the Interdisciplinary Initiative (IDI) grant of the University of Western Ontario (UWO). The work at the Canadian Light Source (CLS) is supported by CFI, NSERC, National Research Council (NRC), Canadian Institute for Health Research (CIHR), and the University of Saskatchewan. The work at Advanced Light Source is supported by the Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We would like to thank Dr. T. Regier for technical support at the SGM beamline at CLS. J.L. acknowledges the receipt of support from the CLS Graduate Student Travel Support Program. J.Z. thanks the National Natural Science Foundation of China (U1232102 and 21473178) for financial support. NR 40 TC 3 Z9 3 U1 12 U2 42 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 3 PY 2016 VL 120 IS 8 BP 4623 EP 4628 DI 10.1021/acs.jpcc.5b11445 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DF7UB UT WOS:000371562000053 ER PT J AU Jiang, XK Liu, Y Qiao, R AF Jiang, Xikai Liu, Ying Qiao, Rui TI Current Rectification for Transport of Room-Temperature Ionic Liquids through Conical Nanopores SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID CONE-SHAPED NANOPORE; CONCENTRATION POLARIZATION; NANOFLUIDIC DIODE; ACCESS RESISTANCE; SLIT NANOPORE; CAPACITANCE; DYNAMICS; CONDUCTIVITY; PROPAGATION; INTERFACE AB We studied the transport of room-temperature ionic liquids (RTILs) through charged conical nanopores using a Landau-Ginzburg-type continuum model (Bazant et al. Phys. Rev. Lett 2011, 106, 046102) that takes steric effect and strong ion-ion correlations into account. When the surface charge is uniform on the pore wall, weak current rectification is observed. When the charge density near the pore base is removed, the ionic current is greatly suppressed under negative bias voltage while nearly unchanged under positive bias voltage, thereby leading to enhanced current rectification. These predictions agree qualitatively with prior experimental observations, and we elucidated them by analyzing the different components of the ionic current and the structural changes of electrical double layers (EDLs) at the pore tip under different bias voltages and surface charge patterns. These analyses reveal that the different modifications of the EDL structure near the pore tip by the positive and negative bias voltages cause the current rectification and the observed dependence on the distribution of surface charge on the pore wall. The fact that the current rectification phenomena are captured qualitatively by the simple model originally developed for describing EDLs at equilibrium conditions suggests that this model may be promising for understanding the ionic transport under nonequilibrium conditions when the EDL structure is strongly perturbed by external fields. C1 [Jiang, Xikai] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. [Liu, Ying; Qiao, Rui] Virginia Tech, Dept Mech Engn, Blacksburg, VA 24061 USA. RP Jiang, XK (reprint author), Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA.; Qiao, R (reprint author), Virginia Tech, Dept Mech Engn, Blacksburg, VA 24061 USA. EM xikai@anl.gov; ruiqiao@vt.edu RI Qiao, Rui/B-2350-2009 OI Qiao, Rui/0000-0001-5219-5530 FU U.S. DOE, Office of Science [DE-AC02-06CH11357]; NSF [CBET-1264578] FX The authors thank the ARC at Virginia Tech for generous allocation of computer time. The authors thank Dr. Olle Heinonen at Argonne National Laboratory for careful reading and suggestions on the manuscript. X.J. acknowledges support from U.S. DOE, Office of Science under Contract No. DE-AC02-06CH11357. Y.L. and RQ, acknowledge support from the NSF under Grant No. CBET-1264578. NR 57 TC 2 Z9 2 U1 8 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 3 PY 2016 VL 120 IS 8 BP 4629 EP 4637 DI 10.1021/acs.jpcc.5b11522 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DF7UB UT WOS:000371562000054 ER PT J AU Lewis, NHC Fleming, GR AF Lewis, Nicholas H. C. Fleming, Graham R. TI Two-Dimensional Electronic-Vibrational Spectroscopy of Chlorophyll a and b SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID RESONANCE RAMAN-SPECTROSCOPY; LIGHT-HARVESTING COMPLEX; ENERGY-TRANSFER; RELAXATION; SPECTRA; INVITRO; TIME AB We present two-dimensional electronic-vibrational (2DEV) spectra of isolated chlorophyll a and b in deuterated ethanol. We excite the Q-band electronic transitions and measure the effects on the carbonyl and C=C double-bond stretch region of the infrared spectrum. With the aid of density functional theory calculations, we provide assignments for the major features of the spectrum. We show how the 2DEV spectra can be used to readily distinguish different solvation states of the chlorophyll, with features corresponding to the minority pentacoordinate magnesium (Mg) species being resolved along each dimension of the 2DEV spectra from the dominant hexacoordinate Mg species. These assignments represent a crucial first step toward the application of 2DEV spectroscopy to chlorophyll-containing pigment-protein complexes. C1 [Lewis, Nicholas H. C.; Fleming, Graham R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Lewis, Nicholas H. C.; Fleming, Graham R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA. [Lewis, Nicholas H. C.; Fleming, Graham R.] Kavli Energy Nanosci Inst Berkeley, Berkeley, CA 94720 USA. RP Fleming, GR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Fleming, GR (reprint author), Kavli Energy Nanosci Inst Berkeley, Berkeley, CA 94720 USA. EM grfleming@lbl.gov FU Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC02-05CH11231]; Division of Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences [DE-AC03-76F000098]; NSF [CHE-0840505] FX We thank Tom Oliver for helpful discussions. This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy under Contract DE-AC02-05CH11231 and the Division of Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences through Grant DE-AC03-76F000098 (at Lawrence Berkeley National Laboratory and University of California, Berkeley). The DFT calculations were performed using the computation resources at the College of Chemistry Molecular Graphics facility, which is funded by NSF under Contract CHE-0840505. NR 31 TC 2 Z9 2 U1 7 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAR 3 PY 2016 VL 7 IS 5 BP 831 EP 837 DI 10.1021/acs.jpclett.6b00037 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DF7US UT WOS:000371563700018 PM 26894783 ER PT J AU Chen, B Yang, MJ Priya, S Zhu, K AF Chen, Bo Yang, Mengjin Priya, Shashank Zhu, Kai TI Origin of J-V Hysteresis in Perovskite Solar Cells SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID METHYLAMMONIUM LEAD IODIDE; ORGANOMETAL HALIDE PEROVSKITES; CH3NH3PBI3 PEROVSKITE; HIGH-EFFICIENCY; LOW-TEMPERATURE; HIGH-PERFORMANCE; FERROELECTRIC POLARIZATION; THIN-FILMS; ANOMALOUS HYSTERESIS; CARRIER SEPARATION AB High-performance perovskite solar cells (PSCs) based on organometal halide perovskite have emerged in the past five years as excellent devices for harvesting solar energy. Some remaining challenges should be resolved to continue the momentum in their development. The photocurrent density-voltage (J-V) responses of the PSCs demonstrate anomalous dependence on the voltage scan direction/rate/range, voltage conditioning history, and device configuration. The hysteretic J-V behavior presents a challenge for determining the accurate power conversion efficiency of the PSCs. Here, we review the recent progress on the investigation of the origin(s) of J-V hysteresis behavior in PSCs. We discuss the impact of slow transient capacitive current, trapping and detrapping process, ion migrations, and ferroelectric polarization on the hysteresis behavior. The remaining issues and future research required toward the understanding of J-V hysteresis in PSCs will also be discussed. C1 [Chen, Bo; Priya, Shashank] Virginia Tech, Ctr Energy Harvesting Mat & Syst, Blacksburg, VA 24061 USA. [Yang, Mengjin; Zhu, Kai] Natl Renewable Energy Lab, Chem & Nanosci Ctr, Golden, CO 80401 USA. RP Chen, B (reprint author), Virginia Tech, Ctr Energy Harvesting Mat & Syst, Blacksburg, VA 24061 USA.; Zhu, K (reprint author), Natl Renewable Energy Lab, Chem & Nanosci Ctr, Golden, CO 80401 USA. EM bochen09@vt.edu; kai.zhu@nrel.gov OI Yang, Mengjin/0000-0003-2019-4298 FU Office of Naval Research (ONR); National Renewable Energy Laboratory by the U.S. Department of Energy SunShot Initiative under the Next Generation Photovoltaics 3 program [DE-FOA-0000990, DE-AC36-08-GO28308] FX S.P. acknowledges the financial support from Office of Naval Research (ONR). KZ. acknowledges the support at the National Renewable Energy Laboratory by the U.S. Department of Energy SunShot Initiative under the Next Generation Photovoltaics 3 program (DE-FOA-0000990) under Contract No. DE-AC36-08-GO28308. NR 91 TC 50 Z9 50 U1 38 U2 150 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAR 3 PY 2016 VL 7 IS 5 BP 905 EP 917 DI 10.1021/acs.jpclett.6b00215 PG 13 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DF7US UT WOS:000371563700027 PM 26886052 ER PT J AU Adare, A Aidala, C Ajitanand, NN Akiba, Y Akimoto, R Alexander, J Alfred, M Aoki, K Apadula, N Asano, H Atomssa, ET Awes, TC Azmoun, B Babintsev, V Bai, M Bai, X Bandara, NS Bannier, B Barish, KN Bathe, S Baublis, V Baumann, C Baumgart, S Bazilevsky, A Beaumier, M Beckman, S Belmont, R Berdnikov, A Berdnikov, Y Black, D Blau, DS Bok, JS Boyle, K Brooks, ML Bryslawskyj, J Buesching, H Bumazhnov, V Butsyk, S Campbell, S Chen, CH Chi, CY Chiu, M Choi, IJ Choi, JB Choi, S Christiansen, P Chujo, T Cianciolo, V Citron, Z Cole, BA Cronin, N Crossette, N Csanad, M Csorgo, T Danley, TW Datta, A Daugherity, MS David, G DeBlasio, K Dehmelt, K Denisov, A Deshpande, A Desmond, EJ Ding, L Dion, A Diss, PB Do, JH D'Orazio, L Drapier, O Drees, A Drees, KA Durham, JM Durum, A Engelmore, T Enokizono, A Esumi, S Eyser, KO Fadem, B Feege, N Fields, DE Finger, M Finger, M Fleuret, F Fokin, SL Frantz, JE Franz, A Frawley, AD Fukao, Y Fusayasu, T Gainey, K Gal, C Gallus, P Garg, P Garishvili, A Garishvili, I Ge, H Giordano, F Glenn, A Gong, X Gonin, M Goto, Y de Cassagnac, RG Grau, N Greene, SV Perdekamp, MG Gu, Y Gunji, T Guragain, H Hachiya, T Haggerty, JS Hahn, KI Hamagaki, H Hamilton, HF Han, SY Hanks, J Hasegawa, S Haseler, TOS Hashimoto, K Hayano, R He, X Hemmick, TK Hester, T Hill, JC Hollis, RS Homma, K Hong, B Hoshino, T Hotvedt, N Huang, J Huang, S Ichihara, T Ikeda, Y Imai, K Imazu, Y Inaba, M Iordanova, A Isenhower, D Isinhue, A Ivanishchev, D Jacak, BV Jeon, SJ Jezghani, M Jia, J Jiang, X Johnson, BM Joo, KS Jouan, D Jumper, DS Kamin, J Kanda, S Kang, BH Kang, JH Kang, JS Kapustinsky, J Kawall, D Kazantsev, AV Key, JA Khachatryan, V Khandai, PK Khanzadeev, A Kijima, KM Kim, C Kim, DJ Kim, EJ Kim, GW Kim, M Kim, YJ Kim, YK Kimelman, B Kistenev, E Kitamura, R Klatsky, J Kleinjan, D Kline, P Koblesky, T Kofarago, M Komkov, B Koster, J Kotchetkov, D Kotov, D Krizek, F Kurita, K Kurosawa, M Kwon, Y Lacey, R Lai, YS Lajoie, JG Lebedev, A Lee, DM Lee, GH Lee, J Lee, KB Lee, KS Lee, S Lee, SH Leitch, MJ Leitgab, M Lewis, B Li, X Lim, SH Liu, MX Lynch, D Maguire, CF Makdisi, YI Makek, M Manion, A Manko, VI Mannel, E Maruyama, T McCumber, M McGaughey, PL McGlinchey, D McKinney, C Meles, A Mendoza, M Meredith, B Miake, Y Mibe, T Mignerey, AC Milov, A Mishra, DK Mitchell, JT Miyasaka, S Mizuno, S Mohanty, AK Mohapatra, S Montuenga, P Moon, T Morrison, DP Moskowitz, M Moukhanova, TV Murakami, T Murata, J Mwai, A Nagae, T Nagamiya, S Nagashima, K Nagle, JL Nagy, MI Nakagawa, I Nakagomi, H Nakamiya, Y Nakamura, KR Nakamura, T Nakano, K Nattrass, C Netrakanti, PK Nihashi, M Niida, T Nishimura, S Nouicer, R Novak, T Novitzky, N Nyanin, AS O'Brien, E Ogilvie, CA Oide, H Okada, K Koop, JDO Osborn, JD Oskarsson, A Ozawa, K Pak, R Pantuev, V Papavassiliou, V Park, IH Park, JS Park, S Park, SK Pate, SF Patel, L Patel, M Peng, JC Perepelitsa, DV Perera, GDN Peressounko, DY Perry, J Petti, R Pinkenburg, C Pinson, R Pisani, RP Purschke, ML Qu, H Rak, J Ramson, BJ Ravinovich, I Read, KF Reynolds, D Riabov, V Riabov, Y Richardson, E Rinn, T Riveli, N Roach, D Rolnick, SD Rosati, M Rowan, Z Rubin, JG Ryu, MS Sahlmueller, B Saito, N Sakaguchi, T Sako, H Samsonov, V Sarsour, M Sato, S Sawada, S Schaefer, B Schmoll, BK Sedgwick, K Seele, J Seidl, R Sekiguchi, Y Sen, A Seto, R Sett, P Sexton, A Sharma, D Shaver, A Shein, I Shibata, TA Shigaki, K Shimomura, M Shoji, K Shukla, P Sickles, A Silva, CL Silvermyr, D Singh, BK Singh, CP Singh, V Skolnik, M Slunecka, M Snowball, M Solano, S Soltz, RA Sondheim, WE Sorensen, SP Sourikova, IV Stankus, PW Steinberg, P Stenlund, E Stepanov, M Ster, A Stoll, SP Stone, MR Sugitate, T Sukhanov, A Sumita, T Sun, J Sziklai, J Takahara, A Taketani, A Tanaka, Y Tanida, K Tannenbaum, MJ Tarafdar, S Taranenko, A Tennant, E Tieulent, R Timilsina, A Todoroki, T Tomasek, M Torii, H Towell, CL Towell, R Towell, RS Tserruya, I van Hecke, HW Vargyas, M Vazquez-Zambrano, E Veicht, A Velkovska, J Vertesi, R Virius, M Vrba, V Vznuzdaev, E Wang, XR Watanabe, D Watanabe, K Watanabe, Y Watanabe, YS Wei, F Whitaker, S White, AS Wolin, S Woody, CL Wysocki, M Xia, B Xue, L Yalcin, S Yamaguchi, YL Yanovich, A Yokkaichi, S Yoo, JH Yoon, I You, Z Younus, I Yu, H Yushmanov, IE Zajc, WA Zelenski, A Zhou, S Zou, L AF Adare, A. Aidala, C. Ajitanand, N. N. Akiba, Y. Akimoto, R. Alexander, J. Alfred, M. Aoki, K. Apadula, N. Asano, H. Atomssa, E. T. Awes, T. C. Azmoun, B. Babintsev, V. Bai, M. Bai, X. Bandara, N. S. Bannier, B. Barish, K. N. Bathe, S. Baublis, V. Baumann, C. Baumgart, S. Bazilevsky, A. Beaumier, M. Beckman, S. Belmont, R. Berdnikov, A. Berdnikov, Y. Black, D. Blau, D. S. Bok, J. S. Boyle, K. Brooks, M. L. Bryslawskyj, J. Buesching, H. Bumazhnov, V. Butsyk, S. Campbell, S. Chen, C. -H. Chi, C. Y. Chiu, M. Choi, I. J. Choi, J. B. Choi, S. Christiansen, P. Chujo, T. Cianciolo, V. Citron, Z. Cole, B. A. Cronin, N. Crossette, N. Csanad, M. Csoergo, T. Danley, T. W. Datta, A. Daugherity, M. S. David, G. DeBlasio, K. Dehmelt, K. Denisov, A. Deshpande, A. Desmond, E. J. Ding, L. Dion, A. Diss, P. B. Do, J. H. D'Orazio, L. Drapier, O. Drees, A. Drees, K. A. Durham, J. M. Durum, A. Engelmore, T. Enokizono, A. Esumi, S. Eyser, K. O. Fadem, B. Feege, N. Fields, D. E. Finger, M. Finger, M., Jr. Fleuret, F. Fokin, S. L. Frantz, J. E. Franz, A. Frawley, A. D. Fukao, Y. Fusayasu, T. Gainey, K. Gal, C. Gallus, P. Garg, P. Garishvili, A. Garishvili, I. Ge, H. Giordano, F. Glenn, A. Gong, X. Gonin, M. Goto, Y. de Cassagnac, R. Granier Grau, N. Greene, S. V. Perdekamp, M. Grosse Gu, Y. Gunji, T. Guragain, H. Hachiya, T. Haggerty, J. S. Hahn, K. I. Hamagaki, H. Hamilton, H. F. Han, S. Y. Hanks, J. Hasegawa, S. Haseler, T. O. S. Hashimoto, K. Hayano, R. He, X. Hemmick, T. K. Hester, T. Hill, J. C. Hollis, R. S. Homma, K. Hong, B. Hoshino, T. Hotvedt, N. Huang, J. Huang, S. Ichihara, T. Ikeda, Y. Imai, K. Imazu, Y. Inaba, M. Iordanova, A. Isenhower, D. Isinhue, A. Ivanishchev, D. Jacak, B. V. Jeon, S. J. Jezghani, M. Jia, J. Jiang, X. Johnson, B. M. Joo, K. S. Jouan, D. Jumper, D. S. Kamin, J. Kanda, S. Kang, B. H. Kang, J. H. Kang, J. S. Kapustinsky, J. Kawall, D. Kazantsev, A. V. Key, J. A. Khachatryan, V. Khandai, P. K. Khanzadeev, A. Kijima, K. M. Kim, C. Kim, D. J. Kim, E. -J. Kim, G. W. Kim, M. Kim, Y. -J. Kim, Y. K. Kimelman, B. Kistenev, E. Kitamura, R. Klatsky, J. Kleinjan, D. Kline, P. Koblesky, T. Kofarago, M. Komkov, B. Koster, J. Kotchetkov, D. Kotov, D. Krizek, F. Kurita, K. Kurosawa, M. Kwon, Y. Lacey, R. Lai, Y. S. Lajoie, J. G. Lebedev, A. Lee, D. M. Lee, G. H. Lee, J. Lee, K. B. Lee, K. S. Lee, S. Lee, S. H. Leitch, M. J. Leitgab, M. Lewis, B. Li, X. Lim, S. H. Liu, M. X. Lynch, D. Maguire, C. F. Makdisi, Y. I. Makek, M. Manion, A. Manko, V. I. Mannel, E. Maruyama, T. McCumber, M. McGaughey, P. L. McGlinchey, D. McKinney, C. Meles, A. Mendoza, M. Meredith, B. Miake, Y. Mibe, T. Mignerey, A. C. Milov, A. Mishra, D. K. Mitchell, J. T. Miyasaka, S. Mizuno, S. Mohanty, A. K. Mohapatra, S. Montuenga, P. Moon, T. Morrison, D. P. Moskowitz, M. Moukhanova, T. V. Murakami, T. Murata, J. Mwai, A. Nagae, T. Nagamiya, S. Nagashima, K. Nagle, J. L. Nagy, M. I. Nakagawa, I. Nakagomi, H. Nakamiya, Y. Nakamura, K. R. Nakamura, T. Nakano, K. Nattrass, C. Netrakanti, P. K. Nihashi, M. Niida, T. Nishimura, S. Nouicer, R. Novak, T. Novitzky, N. Nyanin, A. S. O'Brien, E. Ogilvie, C. A. Oide, H. Okada, K. Koop, J. D. Orjuela Osborn, J. D. Oskarsson, A. Ozawa, K. Pak, R. Pantuev, V. Papavassiliou, V. Park, I. H. Park, J. S. Park, S. Park, S. K. Pate, S. F. Patel, L. Patel, M. Peng, J. -C. Perepelitsa, D. V. Perera, G. D. N. Peressounko, D. Yu. Perry, J. Petti, R. Pinkenburg, C. Pinson, R. Pisani, R. P. Purschke, M. L. Qu, H. Rak, J. Ramson, B. J. Ravinovich, I. Read, K. F. Reynolds, D. Riabov, V. Riabov, Y. Richardson, E. Rinn, T. Riveli, N. Roach, D. Rolnick, S. D. Rosati, M. Rowan, Z. Rubin, J. G. Ryu, M. S. Sahlmueller, B. Saito, N. Sakaguchi, T. Sako, H. Samsonov, V. Sarsour, M. Sato, S. Sawada, S. Schaefer, B. Schmoll, B. K. Sedgwick, K. Seele, J. Seidl, R. Sekiguchi, Y. Sen, A. Seto, R. Sett, P. Sexton, A. Sharma, D. Shaver, A. Shein, I. Shibata, T. -A. Shigaki, K. Shimomura, M. Shoji, K. Shukla, P. Sickles, A. Silva, C. L. Silvermyr, D. Singh, B. K. Singh, C. P. Singh, V. Skolnik, M. Slunecka, M. Snowball, M. Solano, S. Soltz, R. A. Sondheim, W. E. Sorensen, S. P. Sourikova, I. V. Stankus, P. W. Steinberg, P. Stenlund, E. Stepanov, M. Ster, A. Stoll, S. P. Stone, M. R. Sugitate, T. Sukhanov, A. Sumita, T. Sun, J. Sziklai, J. Takahara, A. Taketani, A. Tanaka, Y. Tanida, K. Tannenbaum, M. J. Tarafdar, S. Taranenko, A. Tennant, E. Tieulent, R. Timilsina, A. Todoroki, T. Tomasek, M. Torii, H. Towell, C. L. Towell, R. Towell, R. S. Tserruya, I. van Hecke, H. W. Vargyas, M. Vazquez-Zambrano, E. Veicht, A. Velkovska, J. Vertesi, R. Virius, M. Vrba, V. Vznuzdaev, E. Wang, X. R. Watanabe, D. Watanabe, K. Watanabe, Y. Watanabe, Y. S. Wei, F. Whitaker, S. White, A. S. Wolin, S. Woody, C. L. Wysocki, M. Xia, B. Xue, L. Yalcin, S. Yamaguchi, Y. L. Yanovich, A. Yokkaichi, S. Yoo, J. H. Yoon, I. You, Z. Younus, I. Yu, H. Yushmanov, I. E. Zajc, W. A. Zelenski, A. Zhou, S. Zou, L. CA Collaboration, P TI Forward J/psi production in U plus U collisions at root S-NN=193 GeV SO PHYSICAL REVIEW C LA English DT Article ID PB-PB COLLISIONS; SUPPRESSION; NUCLEI AB The invariant yields, dN/dy, for J/psi production at forward rapidity (1.2 < vertical bar y vertical bar < 2.2) in U + U collisions at root S-NN = 193 GeV have been measured as a function of collision centrality. The invariant yields and nuclear-modification factor R-AA are presented and compared with those from Au + Au collisions in the same rapidity range. Additionally, the direct ratio of the invariant yields from U + U and Au + Au collisions within the same centrality class is presented, and used to investigate the role of c (c) over bar coalescence. Two different parametrizations of the deformed Woods-Saxon distribution were used in Glauber calculations to determine the values of the number of nucleon-nucleon collisions in each centrality class, N-coll, and these were found to give significantly different Ncoll values. Results using N-coll values from both deformed Woods-Saxon distributions are presented. The measured ratios show that the J/psi suppression, relative to binary collision scaling, is similar in U + U and Au + Au for peripheral and midcentral collisions, but that J/psi show less suppression for the most central U + U collisions. The results are consistent with a picture in which, for central collisions, increase in the J/psi yield due to c (c) over bar coalescence becomes more important than the decrease in yield due to increased energy density. 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[Csoergo, T.; Novak, T.; Ster, A.; Sziklai, J.; Vertesi, R.] RMKI, Inst Particle & Nucl Phys, Hungarian Acad Sci Wigner RCP, Wigner Res Ctr Phys, POB 49, H-1525 Budapest 114, Hungary. [Do, J. H.; Kang, J. H.; Kwon, Y.; Lee, S.; Lim, S. H.; Moon, T.] Yonsei Univ, IPAP, Seoul 120749, South Korea. [Makek, M.] Univ Zagreb, Fac Sci, Dept Phys, Bijenicka 32, HR-10002 Zagreb, Croatia. RP Morrison, DP (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA.; Nagle, JL (reprint author), Univ Colorado, Boulder, CO 80309 USA. EM morrison@bnl.gov; jamie.nagle@colorado.edu RI Durum, Artur/C-3027-2014; Sen, Abhisek/J-1157-2016; Nattrass, Christine/J-6752-2016; Sorensen, Soren /K-1195-2016; Hayano, Ryugo/F-7889-2012; Yokkaichi, Satoshi/C-6215-2017 OI Sen, Abhisek/0000-0003-1192-3938; Nattrass, Christine/0000-0002-8768-6468; Sorensen, Soren /0000-0002-5595-5643; Hayano, Ryugo/0000-0002-1214-7806; FU Office of Nuclear Physics in the Office of Science of the Department of Energy; National Science Foundation; Abilene Christian University Research Council; Research Foundation of SUNY; College of Arts and Sciences, Vanderbilt University (U.S.A.); Ministry of Education, Culture, Sports, Science, and Technology; Japan Society for the Promotion of Science (Japan); Conselho Nacional de Desenvolvimento Cientifico e Tecnologico; Natural Science Foundation of China (People's Republic of China); Croatian Science Foundation and Ministry of Science, Education, and Sports (Croatia); Ministry of Education, Youth and Sports (Czech Republic); Centre National de la Recherche Scientifique; Commissariat a l'Energie Atomique; Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung; Deutscher Akademischer Austauschdienst; Alexander von Humboldt Stiftung (Germany); National Science Fund; OTKA; Karoly Robert University College (Hungary) Department of Atomic Energy; Department of Science and Technology (India); Israel Science Foundation (Israel); Basic Science Research Program through NRF of the Ministry of Education (Korea); Physics Department, Lahore University of Management Sciences (Pakistan); Ministry of Education and Science; Russian Academy of Sciences; Federal Agency of Atomic Energy (Russia); VR; Wallenberg Foundation (Sweden); U.S. Civilian Research and Development Foundation for the Independent States of the Former Soviet Union; Hungarian American Enterprise Scholarship Fund; US-Israel Binational Science Foundation; Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (Brazil) FX We thank the staff of the Collider-Accelerator and Physics Departments at Brookhaven National Laboratory and the staff of the other PHENIX participating institutions for their vital contributions. We acknowledge support from the Office of Nuclear Physics in the Office of Science of the Department of Energy, the National Science Foundation, Abilene Christian University Research Council, Research Foundation of SUNY, and Dean of the College of Arts and Sciences, Vanderbilt University (U.S.A.), Ministry of Education, Culture, Sports, Science, and Technology and the Japan Society for the Promotion of Science (Japan), Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (Brazil), Natural Science Foundation of China (People's Republic of China), Croatian Science Foundation and Ministry of Science, Education, and Sports (Croatia), Ministry of Education, Youth and Sports (Czech Republic), Centre National de la Recherche Scientifique, Commissariat a l'Energie Atomique, and Institut National de Physique Nucleaire et de Physique des Particules (France), Bundesministerium fur Bildung und Forschung, Deutscher Akademischer Austauschdienst, and Alexander von Humboldt Stiftung (Germany), National Science Fund, OTKA, Karoly Robert University College (Hungary) Department of Atomic Energy and Department of Science and Technology (India), Israel Science Foundation (Israel), Basic Science Research Program through NRF of the Ministry of Education (Korea), Physics Department, Lahore University of Management Sciences (Pakistan), Ministry of Education and Science, Russian Academy of Sciences, Federal Agency of Atomic Energy (Russia), VR and Wallenberg Foundation (Sweden), the U.S. Civilian Research and Development Foundation for the Independent States of the Former Soviet Union, the Hungarian American Enterprise Scholarship Fund, and the US-Israel Binational Science Foundation. NR 35 TC 0 Z9 0 U1 11 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 3 PY 2016 VL 93 IS 3 AR 034903 DI 10.1103/PhysRevC.93.034903 PG 12 WC Physics, Nuclear SC Physics GA DF5RE UT WOS:000371409000007 ER PT J AU Chipps, KA AF Chipps, K. A. TI Resonances above the proton threshold in Si-26 SO PHYSICAL REVIEW C LA English DT Article ID REACTION-RATES; MASSIVE STARS; AL-26; GALAXY; STATES AB Al-26 remains an intriguing target for observational gamma-ray astronomy, thanks to its characteristic decay. The Al-25( p,gamma) Si-26 reaction is the crucial link in a sequence that bypasses the production of the observable Al-26(g) in favor of the short-lived isomeric state; determining its astrophysical reaction rate across a range of stellar environments has been the focus of many studies. A reanalysis of previous work, utilizing recent improvements in excitation energies and ground state masses, is presented to reduce the ambiguities in the literature and provide focus to future measurements. C1 [Chipps, K. A.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Chipps, K. A.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RP Chipps, KA (reprint author), Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA.; Chipps, KA (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. OI Chipps, Kelly/0000-0003-3050-1298 FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics FX The author wishes to thank those whose data were reanalyzed in this work for providing the nuclear properties needed to understand stellar nucleosynthesis, and in particular A. M. Hurst, C. Wrede, A. A. Chen, and M. S. Smith for useful discussions. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics. NR 46 TC 1 Z9 1 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 3 PY 2016 VL 93 IS 3 AR 035801 DI 10.1103/PhysRevC.93.035801 PG 8 WC Physics, Nuclear SC Physics GA DF5RE UT WOS:000371409000008 ER PT J AU Roig, O Jandel, M Meot, V Bond, EM Bredeweg, TA Couture, AJ Haight, RC Keksis, AL Rundberg, RS Ullmann, JL Vieira, DJ AF Roig, O. Jandel, M. Meot, V. Bond, E. M. Bredeweg, T. A. Couture, A. J. Haight, R. C. Keksis, A. L. Rundberg, R. S. Ullmann, J. L. Vieira, D. J. TI Radiative neutron capture cross sections on Lu-176 at DANCE SO PHYSICAL REVIEW C LA English DT Article ID STELLAR INTERIORS; COSMIC CLOCK; DECAY; NUCLEOSYNTHESIS; ENDF/B-VII.1; ABUNDANCES; DETECTOR; STARS; RATES; SOLAR AB The cross section of the neutron capture reaction Lu-176(n,gamma) has been measured for a wide incident neutron energy range with the Detector for Advanced Neutron Capture Experiments at the Los Alamos Neutron Science Center. The thermal neutron capture cross section was determined to be (1912 +/- 132) b for one of the Lu natural isotopes, Lu-176. The resonance part was measured and compared to the Mughabghab's atlas using the R-matrix code, SAMMY. At higher neutron energies the measured cross sections are compared to ENDF/B-VII.1, JEFF-3.2, and BRC evaluated nuclear data. The Maxwellian averaged cross sections in a stellar plasma for thermal energies between 5 keV and 100 keV were extracted using these data. C1 [Roig, O.; Meot, V.] CEA, DAM, DIF, F-91297 Arpajon, France. [Jandel, M.; Bond, E. M.; Bredeweg, T. A.; Couture, A. J.; Haight, R. C.; Keksis, A. L.; Rundberg, R. S.; Ullmann, J. L.; Vieira, D. J.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Roig, O (reprint author), CEA, DAM, DIF, F-91297 Arpajon, France. EM olivier.roig@cea.fr FU US Department of Energy, National Nuclear Security Administration [DE-AC52-06NA25396] FX The authors would like to thank P. Romain and B. Morillon from CEA, DAM, DIF for providing us their data evaluation. We would like to thank D. Le Du from CSNSM for the production of the target and R. S. Rundberg from LANL and Ph. Hubert from CENBG (Bordeaux), independently, for their precise measurement of the low activity of our target. This work has benefited from the use of the LANSCE facility at the Los Alamos National Laboratory, and was performed under the auspices of the US Department of Energy, National Nuclear Security Administration, by Los Alamos National Security, LLC, under Contract No. DE-AC52-06NA25396. One of us (O.R.) is grateful to the Los Alamos National Laboratory and the Commissariat a l'Energie Atomique et aux energies alternatives for support during his extended stay in Los Alamos and to the C-NR team and the DANCE collaboration for their warm hospitality. NR 51 TC 1 Z9 1 U1 6 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 3 PY 2016 VL 93 IS 3 AR 034602 DI 10.1103/PhysRevC.93.034602 PG 12 WC Physics, Nuclear SC Physics GA DF5RE UT WOS:000371409000005 ER PT J AU Davoudiasl, H Zhang, C AF Davoudiasl, Hooman Zhang, Cen TI 750 GeV messenger of dark conformal symmetry breaking SO PHYSICAL REVIEW D LA English DT Article ID RANDALL-SUNDRUM MODEL; PP COLLISIONS; ROOT-S=8 TEV; PHENOMENOLOGY; RESONANCES; HIERARCHY; SEARCH; FIELDS; MATTER AB The tentative hints for a diphoton resonance at a mass of similar to 750 GeV from the ATLAS and CMS experiments at the LHC may be interpreted as first contact with a "dark" sector with a spontaneously broken conformal symmetry. The implied TeV scale of the dark sector may be motivated by the interaction strength required to accommodate a viable thermal relic dark matter (DM) candidate. We model the conformal dynamics using a Randall-Sundrum-type five-dimensional geometry whose IR boundary is identified with the dynamics of the composite dark sector, while the Standard Model (SM) matter content resides on the UV boundary, corresponding to "elementary" fields. We allow the gauge fields to reside in the five-dimensional bulk, which can be minimally chosen to be SU(3)(c) x U(1)(Y). The "dark" radion is identified as the putative 750 GeV resonance. Heavy vectorlike fermions, often invoked to explain the diphoton excess, are not explicitly present in our model and are not predicted to appear in the spectrum of TeV scale states. Our minimal setup favors scalar DM of O(TeV) mass. A generic expectation in this scenario, suggested by DM considerations, is the appearance of vector bosons at similar to few TeV, corresponding to the gluon and hypercharge Kaluza-Klein (KK) modes that couple to UV boundary states with strengths that are suppressed uniformly compared to their SM values. Our analysis suggests that these KK modes could be within the reach of the LHC in the coming years. C1 [Davoudiasl, Hooman; Zhang, Cen] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Davoudiasl, H; Zhang, C (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. EM hooman@bnl.gov; cenzhang@bnl.gov FU United States Department of Energy [DE-SC0012704] FX H. D. thanks K. Agashe for discussions. C. Z. thanks M. Backovic for help on MADDM. This work is supported in part by the United States Department of Energy under Grant No. DE-SC0012704. NR 70 TC 33 Z9 33 U1 2 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 3 PY 2016 VL 93 IS 5 AR 055006 DI 10.1103/PhysRevD.93.055006 PG 5 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DF5SW UT WOS:000371413800009 ER PT J AU Liu, ZQ Li, L Gai, Z Clarkson, JD Hsu, SL Wong, AT Fan, LS Lin, MW Rouleau, CM Ward, TZ Lee, HN Sefat, AS Christen, HM Ramesh, R AF Liu, Z. Q. Li, L. Gai, Z. Clarkson, J. D. Hsu, S. L. Wong, A. T. Fan, L. S. Lin, M-W Rouleau, C. M. Ward, T. Z. Lee, H. N. Sefat, A. S. Christen, H. M. Ramesh, R. TI Full Electroresistance Modulation in a Mixed-Phase Metallic Alloy SO PHYSICAL REVIEW LETTERS LA English DT Article ID ELECTRIC-FIELD CONTROL; ROOM-TEMPERATURE; VALENT MANGANITES; MAGNETIC ORDER; FERH; TRANSITION; SEPARATION; MAGNETORESISTANCE; RESISTIVITY; FILMS AB We report a giant, similar to 22%, electroresistance modulation for a metallic alloy above room temperature. It is achieved by a small electric field of 2 kV/cm via piezoelectric strain-mediated magnetoelectric coupling and the resulting magnetic phase transition in epitaxial FeRh/BaTiO3 heterostructures. This work presents detailed experimental evidence for an isothermal magnetic phase transition driven by tetragonality modulation in FeRh thin films, which is in contrast to the large volume expansion in the conventional temperature-driven magnetic phase transition in FeRh. Moreover, all the experimental results in this work illustrate FeRh as a mixed-phase model system well similar to phase-separated colossal magnetoresistance systems with phase instability therein. C1 [Liu, Z. Q.; Gai, Z.; Lin, M-W; Rouleau, C. M.; Christen, H. M.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Liu, Z. Q.; Clarkson, J. D.; Hsu, S. L.; Ramesh, R.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Li, L.; Wong, A. T.; Fan, L. S.; Ward, T. Z.; Lee, H. N.; Sefat, A. S.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Wong, A. T.] Univ Tennessee, Mat Sci & Engn, Knoxville, TN 37996 USA. [Ramesh, R.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Ramesh, R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Ramesh, R.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Liu, ZQ; Christen, HM (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.; Liu, ZQ; Ramesh, R (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.; Ramesh, R (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.; Ramesh, R (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Ramesh, R (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM liuzhiqi@berkeley.edu; christenhm@ornl.gov; rramesh@berkeley.edu RI Gai, Zheng/B-5327-2012; Li, Li/G-6406-2013; Ward, Thomas/I-6636-2016; Christen, Hans/H-6551-2013; Lee, Ho Nyung/K-2820-2012; Sefat, Athena/R-5457-2016 OI Gai, Zheng/0000-0002-6099-4559; Li, Li/0000-0003-1683-8118; Ward, Thomas/0000-0002-1027-9186; Christen, Hans/0000-0001-8187-7469; Lee, Ho Nyung/0000-0002-2180-3975; Sefat, Athena/0000-0002-5596-3504 FU FAME, one of six centers of STARnet, a Semiconductor Research Corporation program - MARCO; Laboratory Directed Research and Development (LDRD) Programs of ORNL; U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; U.S. DOE [DE-SC0002136]; DARPA FX The work at Berkeley was supported in part by FAME, one of six centers of STARnet, a Semiconductor Research Corporation program sponsored by MARCO and DARPA. The work at ORNL was sponsored by the Laboratory Directed Research and Development (LDRD) Programs of ORNL managed by UT-Battelle, LLC (Z. Q. L. and L. L.); by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division (A. S. S., L. S. F., T. Z. W., and H. N. L.); and under U.S. DOE Grant No. DE-SC0002136 (A. T. W.). Part of the work was performed at ORNL's Center for Nanophase Materials Sciences, which is DOE Office of Science User Facility. We thank Dr. J. M. Black and Dr. N. Balke in CNMS-ORNL for their help on setting up MFM measurements. NR 52 TC 6 Z9 6 U1 20 U2 56 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 3 PY 2016 VL 116 IS 9 AR 097203 DI 10.1103/PhysRevLett.116.097203 PG 6 WC Physics, Multidisciplinary SC Physics GA DF5VC UT WOS:000371419600014 PM 26991197 ER PT J AU Wu, SM Zhang, W Amit, KC Borisov, P Pearson, JE Jiang, JS Lederman, D Hoffmann, A Bhattacharya, A AF Wu, Stephen M. Zhang, Wei Amit, K. C. Borisov, Pavel Pearson, John E. Jiang, J. Samuel Lederman, David Hoffmann, Axel Bhattacharya, Anand TI Antiferromagnetic Spin Seebeck Effect SO PHYSICAL REVIEW LETTERS LA English DT Article ID CRYSTAL-STRUCTURE; MNF2; RESONANCE; COF2; DIFFRACTION; DISPERSION; TRANSPORT; FLUORIDE; FIELDS; PHASE AB We report on the observation of the spin Seebeck effect in antiferromagnetic MnF2. A device scale on-chip heater is deposited on a bilayer of MnF2 (110) (30 nm)= Pt (4 nm) grown by molecular beam epitaxy on a MgF2 (110) substrate. Using Pt as a spin detector layer, it is possible to measure the thermally generated spin current from MnF2 through the inverse spin Hall effect. The low temperature (2-80 K) and high magnetic field (up to 140 kOe) regime is explored. A clear spin-flop transition corresponding to the sudden rotation of antiferromagnetic spins out of the easy axis is observed in the spin Seebeck signal when large magnetic fields (> 9 T) are applied parallel to the easy axis of the MnF2 thin film. When the magnetic field is applied perpendicular to the easy axis, the spin-flop transition is absent, as expected. C1 [Wu, Stephen M.; Zhang, Wei; Pearson, John E.; Jiang, J. Samuel; Hoffmann, Axel; Bhattacharya, Anand] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Amit, K. C.; Borisov, Pavel; Lederman, David] W Virginia Univ, Dept Phys & Astron, Morgantown, WV 26506 USA. RP Wu, SM (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM swu@anl.gov RI Borisov, Pavel/A-6218-2015; Bhattacharya, Anand/G-1645-2011 OI Borisov, Pavel/0000-0003-1464-6999; Bhattacharya, Anand/0000-0002-6839-6860 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; U.S. Department of Energy, Basic Energy Sciences [DE-AC02-06CH11357]; West Virginia Higher Education Policy Commission [HEPC.DSR.12.29]; National Science Foundation [DMR-1434897]; WVU Shared Research Facilities FX All work at Argonne was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. The use of facilities at the Center for Nanoscale Materials, an Office of Science user facility, was supported by the U.S. Department of Energy, Basic Energy Sciences under Contract No. DE-AC02-06CH11357. The work at WVU was supported by a Research Challenge Grant from the West Virginia Higher Education Policy Commission (Grant No. HEPC.DSR.12.29), a grant from the National Science Foundation (Grant No. DMR-1434897), and the WVU Shared Research Facilities. We thank S. M. Rezende for bringing the historical spin-flop boundary information to our attention and sharing his unpublished work with us. NR 45 TC 17 Z9 17 U1 20 U2 52 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 3 PY 2016 VL 116 IS 9 AR 097204 DI 10.1103/PhysRevLett.116.097204 PG 5 WC Physics, Multidisciplinary SC Physics GA DF5VC UT WOS:000371419600015 PM 26991198 ER PT J AU Casella, AM Loyalka, SK AF Casella, Andrew M. Loyalka, Sudarshan K. TI Monte Carlo N-particle tracking of ultrafine particle flow in bent microtubes SO AEROSOL SCIENCE AND TECHNOLOGY LA English DT Article ID LAMINAR-FLOW; PENETRATION EFFICIENCY; CURVED PIPES; DEPOSITION; FLUID; BEHAVIOR AB The problem of large pressure-differential-driven laminar convective-diffusive ultrafine aerosol flow through bent microtubes is of interest in several contemporary research areas including; release of contents from pressurized containment vessels, aerosol sampling equipment, advanced scientific instruments, gas-phase microheat exchangers, and microfluidic devices. In each of these areas, the predominant problem is the determination of the fraction of particles entering the microtube that is deposited within the tube and the fraction that is transmitted through. Due to the extensive parameter restrictions of this class of problems, a Lagrangian particle tracking method making use of the coupling of the analytical stream line solutions of Dean for convective motion and a sampling of a Gaussian distribution for diffusive motion is a useful tool in problem characterization. This method is a direct analog to the Monte Carlo N-Particle method of particle transport extensively used in nuclear physics and engineering. In this work, 10-nm-diameter particles with a density of 1g/cm(3) are tracked within microtubes with toroidal bends with pressure differentials ranging between 0.2175 and 0.87 atmospheres. The tubes have radii of 25 microns or 50 microns and the radius of curvature is either 1m or 0.3183cm. The carrier gas is helium, and temperatures of 298K and 558K are considered. Numerical convergence is considered as a function of time step size and of the number of particles per simulation. Particle transmission rates and deposition patterns within the bent microtubes are calculated.Copyright (c) 2016 American Association for Aerosol Research C1 [Casella, Andrew M.] Pacific NW Natl Lab, Nucl Engn & Anal Grp, Richland, WA 99352 USA. [Loyalka, Sudarshan K.] Univ Missouri, Nucl Sci & Engn Inst, Columbia, MO USA. [Loyalka, Sudarshan K.] Univ Missouri, Particulate Syst Res Ctr, Columbia, MO USA. RP Casella, AM (reprint author), Pacific NW Natl Lab, Nucl Engn & Anal Grp, Natl Secur Directorate, 902 Battelle Blvd,POB 999,MSIN K8-34, Richland, WA 99352 USA. EM andrew.casella@pnnl.gov NR 38 TC 0 Z9 0 U1 2 U2 4 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 0278-6826 EI 1521-7388 J9 AEROSOL SCI TECH JI Aerosol Sci. Technol. PD MAR 3 PY 2016 VL 50 IS 3 BP 272 EP 283 DI 10.1080/02786826.2016.1143548 PG 12 WC Engineering, Chemical; Engineering, Mechanical; Environmental Sciences; Meteorology & Atmospheric Sciences SC Engineering; Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA DE9NN UT WOS:000370964700003 ER PT J AU Mosier, AC Miller, CS Frischkorn, KR Ohm, RA Li, Z LaButti, K Lapidus, A Lipzen, A Chen, C Johnson, J Lindquist, EA Pan, CL Hettich, RL Grigoriev, IV Singer, SW Banfield, JF AF Mosier, Annika C. Miller, Christopher S. Frischkorn, Kyle R. Ohm, Robin A. Li, Zhou LaButti, Kurt Lapidus, Alla Lipzen, Anna Chen, Cindy Johnson, Jenifer Lindquist, Erika A. Pan, Chongle Hettich, Robert L. Grigoriev, Igor V. Singer, Steven W. Banfield, Jillian F. TI Fungi Contribute Critical but Spatially Varying Roles in Nitrogen and Carbon Cycling in Acid Mine Drainage SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE fungi; metagenomics; transcriptomics; proteomics; carbon; nitrogen; biofilm ID IN-SITU DETECTION; PHYLOGENETIC IDENTIFICATION; BIOFILM COMMUNITIES; FUSARIUM-OXYSPORUM; PROTEOMIC ANALYSIS; PROTEIN FAMILIES; ANALYSIS REVEALS; GENOMES; DENITRIFICATION; DATABASE AB The ecosystem roles of fungi have been extensively studied by targeting one organism and/or biological process at a time, but the full metabolic potential of fungi has rarely been captured in an environmental context. We hypothesized that fungal genome sequences could be assembled directly from the environment using metagenomics and that transcriptomics and proteomics could simultaneously reveal metabolic differentiation across habitats. We reconstructed the near-complete 27 Mbp genome of a filamentous fungus, Acidomyces richrnondensis, and evaluated transcript and protein expression in floating and streamer biofilms from an acid mine drainage (AMD) system. A. richmondensis transcripts involved in denitrification and in the degradation of complex carbon sources (including cellulose) were up regulated in floating biofilms, whereas central carbon metabolism and stress-related transcripts were significantly up-regulated in streamer biofilms. These findings suggest that the biofilm niches are distinguished by distinct carbon and nitrogen resource utilization, oxygen availability, and environmental challenges. An isolated A. richmondensis strain from this environment was used to validate the metagenomics-derived genome and confirm nitrous oxide production at pH 1. Overall, our analyses defined mechanisms of fungal adaptation and identified a functional shift related to different roles in carbon and nitrogen turnover for the same species of fungi growing in closely located but distinct biofilm niches. C1 [Mosier, Annika C.; Miller, Christopher S.; Frischkorn, Kyle R.; Banfield, Jillian F.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Ohm, Robin A.; LaButti, Kurt; Lapidus, Alla; Lipzen, Anna; Chen, Cindy; Johnson, Jenifer; Lindquist, Erika A.; Grigoriev, Igor V.] US DOE, Joint Genome Inst, Walnut Creek, CA USA. [Li, Zhou; Pan, Chongle; Hettich, Robert L.] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Li, Zhou] Univ Tennessee, Oak Ridge Natl Lab, Grad Sch Genome Sci & Technol, Knoxville, TN USA. [Singer, Steven W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Banfield, Jillian F.] Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. [Mosier, Annika C.; Miller, Christopher S.] Univ Colorado, Dept Integrat Biol, Denver, CO 80202 USA. [Frischkorn, Kyle R.] Columbia Univ, Dept Earth & Environm Sci, Lamont Doherty Earth Observ, Palisades, NY USA. [Lapidus, Alla] St Petersburg State Univ, Ctr Algorithm Biotechnol, St Petersburg 199034, Russia. RP Mosier, AC; Banfield, JF (reprint author), Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA.; Banfield, JF (reprint author), Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA.; Mosier, AC (reprint author), Univ Colorado, Dept Integrat Biol, Denver, CO 80202 USA. EM annika.mosier@gmail.com; jbanfield@berkeley.edu RI Ohm, Robin/I-6689-2016; Hettich, Robert/N-1458-2016; Li, Zhou/L-7976-2015; Lapidus, Alla/I-4348-2013; OI Hettich, Robert/0000-0001-7708-786X; Lapidus, Alla/0000-0003-0427-8731; Miller, Christopher/0000-0002-9448-8144 FU U.S. Department of Energy [DE-FG02-10ER64996, DE-SC0004918]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX T.W. Arman (President, Iron Mountain Mines) is thanked for providing site access to the RiChmond Mine and R. Carver and M. Jones for on-site assistance. We thank Susan Spaulding for laboratory assistance. Funding was provided by the U.S. Department of Energy, through the Carbon-Cycling (DE-FG02-10ER64996) and Knowledgebase (DE-SC0004918 for ggKbase funding) programs. The work conducted by the U.S. Department of Energy Joint Genome institute is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 98 TC 2 Z9 2 U1 12 U2 37 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD MAR 3 PY 2016 VL 7 AR 238 DI 10.3389/fmicb.2016.00238 PG 18 WC Microbiology SC Microbiology GA DF2XD UT WOS:000371206800001 PM 26973616 ER PT J AU Rodriguez, S Denby, CM Van Vu, T Baidoo, EEK Wang, G Keasling, JD AF Rodriguez, Sarah Denby, Charles M. Van Vu, T. Baidoo, Edward E. K. Wang, George Keasling, Jay D. TI ATP citrate lyase mediated cytosolic acetyl-CoA biosynthesis increases mevalonate production in Saccharomyces cerevisiae SO MICROBIAL CELL FACTORIES LA English DT Article DE ATP citrate lyase; Mevalonate pathway; Saccharomyces cerevisiae; Acetyl Coenzyme A; Metabolic engineering; Isoprenoid synthesis ID NON-OLEAGINOUS YEASTS; ISOPRENOID PRODUCTION; LIPID-ACCUMULATION; MICROORGANISMS; SYNTHASE; PROTEIN; DEHYDROGENASE; MITOCHONDRIAL; CONSTRUCTION; METABOLISM AB Background: With increasing concern about the environmental impact of a petroleum based economy, focus has shifted towards greener production strategies including metabolic engineering of microbes for the conversion of plant-based feedstocks to second generation biofuels and industrial chemicals. Saccharomyces cerevisiae is an attractive host for this purpose as it has been extensively engineered for production of various fuels and chemicals. Many of the target molecules are derived from the central metabolite and molecular building block, acetyl-CoA. To date, it has been difficult to engineer S. cerevisiae to continuously convert sugars present in biomass-based feedstocks to acetylCoA derived products due to intrinsic physiological constraints-in respiring cells, the precursor pyruvate is directed away from the endogenous cytosolic acetyl-CoA biosynthesis pathway towards the mitochondria, and in fermenting cells pyruvate is directed towards the by product ethanol. In this study we incorporated an alternative mode of acetylCoA biosynthesis mediated by ATP citrate lyase (ACL) that may obviate such constraints. Results: We characterized the activity of several heterologously expressed ACLs in crude cell lysates, and found that ACL from Aspergillus nidulans demonstrated the highest activity. We employed a push/pull strategy to shunt citrate towards ACL by deletion of the mitochondrial NAD+-dependent isocitrate dehydrogenase (IDH1) and engineering higher flux through the upper mevalonate pathway. We demonstrated that combining the two modifications increases accumulation of mevalonate pathway intermediates, and that both modifications are required to substantially increase production. Finally, we incorporated a block strategy by replacing the native ERG12 (mevalonate kinase) promoter with the copper-repressible CTR3 promoter to maximize accumulation of the commercially important molecule mevalonate. Conclusion: By combining the push/pull/block strategies, we significantly improved mevalonate production. We anticipate that this strategy can be used to improve the efficiency with which industrial strains of S. cerevisiae convert feedstocks to acetyl-CoA derived fuels and chemicals. C1 [Rodriguez, Sarah; Denby, Charles M.; Van Vu, T.; Baidoo, Edward E. K.; Wang, George; Keasling, Jay D.] Joint BioEnergy Inst, Emeryville, CA USA. [Rodriguez, Sarah; Baidoo, Edward E. K.; Wang, George; Keasling, Jay D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Denby, Charles M.; Keasling, Jay D.] Univ Calif Berkeley, Calif Inst Quantitat Biosci QB3, Berkeley, CA 94720 USA. [Van Vu, T.; Keasling, Jay D.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Biomol & Chem Engn, Berkeley, CA 94720 USA. RP Keasling, JD (reprint author), Joint BioEnergy Inst, Emeryville, CA USA. EM JDKeasling@lbl.gov FU National Science Foundation [MCB-1330914]; Joint BioEnergy Institute - US Department of Energy, Office of Science, Office of Biological and Environmental Research [DEAC02-05CH11231] FX This work was funded by a grant from the National Science Foundation (MCB-1330914) and by the Joint BioEnergy Institute, which is funded by the US Department of Energy, Office of Science, Office of Biological and Environmental Research, under Contract DEAC02-05CH11231. The authors would like to acknowledge the work of Samuel Deutsch and Matthew Hamilton of the Joint Genome Institute for synthesis of ACL constructs. NR 44 TC 4 Z9 5 U1 6 U2 40 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1475-2859 J9 MICROB CELL FACT JI Microb. Cell. Fact. PD MAR 3 PY 2016 VL 15 AR 48 DI 10.1186/s12934-016-0447-1 PG 12 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA DF8EG UT WOS:000371589400001 PM 26939608 ER PT J AU Jia, Y Chopdekar, RV Arenholz, E Liu, ZQ Biegalski, MD Porter, ZD Mehta, A Takamura, Y AF Jia, Yue Chopdekar, Rajesh V. Arenholz, Elke Liu, Zhiqi Biegalski, Michael D. Porter, Zachary D. Mehta, Apurva Takamura, Yayoi TI Thickness dependence of exchange coupling in (111)-oriented perovskite oxide superlattices SO PHYSICAL REVIEW B LA English DT Article ID X-RAY-ABSORPTION; THIN-FILMS; MAGNETIC-ANISOTROPY; LAYER FORMATION; BIAS; LA1-XSRXMNO3; TRANSITION; BILAYERS; MAGNETORESISTANCE; HETEROINTERFACE AB Epitaxial La0.7Sr0.3MnO3 (LSMO)/La0.7Sr0.3FeO3 (LSFO) superlattices on (111)-oriented SrTiO3 substrates with sublayer thicknesses ranging from 3 to 60 unit cells (u.c.) were synthesized and characterized. Detailed analysis of their structural, electronic, and magnetic properties were performed to explore the effect of sublayer thickness on the magnetic structure and exchange coupling at (111)-oriented perovskite oxide interfaces. In the ultrathin limit (3-6 u.c.), we find that the antiferromagnetic (AF) properties of the LSFO sublayers are preserved with an out-of-plane canting of the AF spin axis, while the ferromagnetic (FM) properties of the LSMO sublayers are significantly depressed. For thicker LSFO layers (>9 u.c.), the out-of-plane canting of the AF spin axis is only present in superlattices with thick LSMO sublayers. As a result, exchange coupling in the form of spin-flop coupling exists only in superlattices which display both robust ferromagnetism and out-of-plane canting of the AF spin axis. C1 [Jia, Yue; Chopdekar, Rajesh V.; Takamura, Yayoi] Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA. [Arenholz, Elke] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Liu, Zhiqi; Biegalski, Michael D.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Porter, Zachary D.; Mehta, Apurva] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. RP Jia, Y (reprint author), Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA. RI Chopdekar, Rajesh/D-2067-2009 OI Chopdekar, Rajesh/0000-0001-6727-6501 FU Semiconductor Research Corporation [2309.001]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515] FX This work was supported by the Semiconductor Research Corporation under Task No. 2309.001. The Advanced Light Source, Lawrence Berkeley Laboratory, is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Use of the Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-76SF00515. Part of the sample fabrication of this research was conducted at the Center for Nanophase Materials Sciences, a U.S. DOE Office of Science User Facility. NR 54 TC 2 Z9 2 U1 9 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 3 PY 2016 VL 93 IS 10 AR 104403 DI 10.1103/PhysRevB.93.104403 PG 9 WC Physics, Condensed Matter SC Physics GA DF5NZ UT WOS:000371400100003 ER PT J AU Terashima, T Kikugawa, N Kiswandhi, A Graf, D Choi, ES Brooks, JS Kasahara, S Watashige, T Matsuda, Y Shibauchi, T Wolf, T Bohmer, AE Hardy, F Meingast, C Lohneysen, HV Uji, S AF Terashima, Taichi Kikugawa, Naoki Kiswandhi, Andhika Graf, David Choi, Eun-Sang Brooks, James S. Kasahara, Shigeru Watashige, Tatsuya Matsuda, Yuji Shibauchi, Takasada Wolf, Thomas Boehmer, Anna E. Hardy, Frederic Meingast, Christoph Loehneysen, Hilbert V. Uji, Shinya TI Fermi surface reconstruction in FeSe under high pressure SO PHYSICAL REVIEW B LA English DT Article ID MAGNETIC-FIELD; SUPERCONDUCTIVITY; NEMATICITY; PHASE AB We report Shubnikov-de Haas (SdH) oscillation measurements on FeSe under high pressure up to P = 16.1 kbar. We find a sudden change in SdH oscillations at the onset of the pressure-induced antiferromagnetism at P similar to 8 kbar. We argue that this change can be attributed to a reconstruction of the Fermi surface by the antiferromagnetic order. The negative dT(c)/dP observed in a range between P similar to 8 and 12 kbar may be explained by the reduction in the density of states due to the reconstruction. The ratio of the transition temperature to the effective Fermi energy remains high under high pressure: k(B)T(c)/E-F similar to 0.1 even at P = 16.1 kbar. C1 [Terashima, Taichi; Kikugawa, Naoki; Uji, Shinya] Natl Inst Mat Sci, Tsukuba, Ibaraki 3050003, Japan. [Kiswandhi, Andhika; Graf, David; Choi, Eun-Sang; Brooks, James S.] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. [Kasahara, Shigeru; Watashige, Tatsuya; Matsuda, Yuji] Kyoto Univ, Dept Phys, Kyoto 6068502, Japan. [Shibauchi, Takasada] Univ Tokyo, Dept Adv Mat Sci, Chiba 2778561, Japan. [Wolf, Thomas; Boehmer, Anna E.; Hardy, Frederic; Meingast, Christoph; Loehneysen, Hilbert V.] Karlsruhe Inst Technol, Inst Solid State Phys IFP, D-76021 Karlsruhe, Germany. [Kiswandhi, Andhika] Univ Texas Dallas, Dept Phys, Richardson, TX 75080 USA. [Boehmer, Anna E.] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. RP Terashima, T (reprint author), Natl Inst Mat Sci, Tsukuba, Ibaraki 3050003, Japan. RI Shibauchi, Takasada/B-9349-2008; Kasahara, Shigeru/H-3064-2014 OI Shibauchi, Takasada/0000-0001-5831-4924; Kasahara, Shigeru/0000-0002-6007-9617 FU KAKENHI Grant [15H05852]; DAAD [56393598]; JSPS KAKENHI [26400373]; NSF [DMR-1157490]; State of Florida; Japan-Germany Research Cooperative Program, KAKENHI from JSPS FX This work has been supported by a Grant-in-Aid for Scientific Research on Innovative Areas "Topological Materials Science" (KAKENHI Grant No. 15H05852), Japan-Germany Research Cooperative Program, KAKENHI from JSPS and Project No. 56393598 from DAAD, and JSPS KAKENHI Grant Number 26400373. A portion of this work was performed at the National High Magnetic Field Laboratory, which is supported by NSF Cooperative Agreement No. DMR-1157490 and the State of Florida. T.T. thanks Ola Kenji Forslund for technical assistance. NR 67 TC 6 Z9 6 U1 10 U2 36 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 3 PY 2016 VL 93 IS 9 AR 094505 DI 10.1103/PhysRevB.93.094505 PG 10 WC Physics, Condensed Matter SC Physics GA DF5OO UT WOS:000371401700003 ER PT J AU Bezrukov, F Gorbunov, D AF Bezrukov, Fedor Gorbunov, Dmitry TI Applicability of approximations used in calculations of the spectrum of dark matter particles produced in particle decays SO PHYSICAL REVIEW D LA English DT Article ID STERILE NEUTRINOS AB For the warm dark matter (WDM) candidates the momentum distribution of particles becomes important, since it can be probed with observations of Lyman-alpha forest structures and confronted with coarse grained phase space density in galaxy clusters. We recall the calculation [M. Kaplinghat, Phys. Rev. D 72, 063510 (2005)] of the spectrum in the case of dark matter nonthermal production in decays of heavy particles emphasizing the inherent applicability conditions, which are rather restrictive and sometimes ignored in literature. The cold part of the spectrum requires special care when WDM is considered. C1 [Bezrukov, Fedor] CERN, CH-1211 Geneva 23, Switzerland. [Bezrukov, Fedor] Univ Connecticut, Dept Phys, Storrs, CT 06269 USA. [Bezrukov, Fedor] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Gorbunov, Dmitry] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Gorbunov, Dmitry] Moscow Inst Phys & Technol, Dolgoprudnyi 141700, Russia. RP Bezrukov, F (reprint author), CERN, CH-1211 Geneva 23, Switzerland.; Bezrukov, F (reprint author), Univ Connecticut, Dept Phys, Storrs, CT 06269 USA.; Bezrukov, F (reprint author), Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA.; Gorbunov, D (reprint author), Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia.; Gorbunov, D (reprint author), Moscow Inst Phys & Technol, Dolgoprudnyi 141700, Russia. EM fedor.bezrukov@uconn.edu; gorby@ms2.inr.ac.ru FU RSF [1412-01430] FX The work was supported by the RSF Grant No. 1412-01430. NR 23 TC 2 Z9 2 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 3 PY 2016 VL 93 IS 6 AR 063502 DI 10.1103/PhysRevD.93.063502 PG 6 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DF5SY UT WOS:000371414000002 ER PT J AU Neupane, M Ishida, Y Sankar, R Zhu, JX Sanchez, DS Belopolski, I Xu, SY Alidoust, N Hosen, MM Shin, S Chou, FC Hasan, MZ Durakiewicz, T AF Neupane, Madhab Ishida, Yukiaki Sankar, Raman Zhu, Jian-Xin Sanchez, Daniel S. Belopolski, Ilya Xu, Su-Yang Alidoust, Nasser Hosen, M. Mofazzel Shin, Shik Chou, Fangcheng Hasan, M. Zahid Durakiewicz, Tomasz TI Electronic structure and relaxation dynamics in a superconducting topological material SO SCIENTIFIC REPORTS LA English DT Article ID AUGMENTED-WAVE METHOD; INSULATOR; SURFACE; COEXISTENCE; BI2SE3; BI2TE3; ORDER; GAS AB Topological superconductors host new states of quantum matter which show a pairing gap in the bulk and gapless surface states providing a platform to realize Majorana fermions. Recently, alkaline-earth metal Sr intercalated Bi2Se3 has been reported to show superconductivity with a T-c similar to 3 K and a large shielding fraction. Here we report systematic normal state electronic structure studies of Sr0.06Bi2Se3 (T-c similar to 2.5 K) by performing photoemission spectroscopy. Using angle-resolved photoemission spectroscopy (ARPES), we observe a quantum well confined two-dimensional (2D) state coexisting with a topological surface state in Sr0.06Bi2Se3. Furthermore, our time-resolved ARPES reveals the relaxation dynamics showing different decay mechanism between the excited topological surface states and the two-dimensional states. Our experimental observation is understood by considering the intra-band scattering for topological surface states and an additional electron phonon scattering for the 2D states, which is responsible for the superconductivity. Our first-principles calculations agree with the more effective scattering and a shorter lifetime of the 2D states. Our results will be helpful in understanding low temperature superconducting states of these topological materials. C1 [Neupane, Madhab; Durakiewicz, Tomasz] Los Alamos Natl Lab, Condensed Matter & Magnet Sci Grp, POB 1663, Los Alamos, NM 87545 USA. [Neupane, Madhab; Hosen, M. Mofazzel] Univ Cent Florida, Dept Phys, Orlando, FL 32816 USA. [Ishida, Yukiaki; Shin, Shik] Univ Tokyo, ISSP, Kashiwa, Chiba 2778581, Japan. [Sankar, Raman; Chou, Fangcheng] Natl Taiwan Univ, Ctr Condensed Matter Sci, Taipei 10617, Taiwan. [Zhu, Jian-Xin] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Sanchez, Daniel S.; Belopolski, Ilya; Xu, Su-Yang; Alidoust, Nasser; Hasan, M. Zahid] Princeton Univ, Joseph Henry Lab, Princeton, NJ 08544 USA. [Sanchez, Daniel S.; Belopolski, Ilya; Xu, Su-Yang; Alidoust, Nasser; Hasan, M. Zahid] Princeton Univ, Dept Phys, Princeton, NJ 08544 USA. RP Neupane, M (reprint author), Los Alamos Natl Lab, Condensed Matter & Magnet Sci Grp, POB 1663, Los Alamos, NM 87545 USA.; Neupane, M (reprint author), Univ Cent Florida, Dept Phys, Orlando, FL 32816 USA. EM Madhab.Neupane@ucf.edu RI ISHIDA, Yukiaki/D-4261-2016 FU LANL LDRD Program; University of Central Florida; NSF IR/D program; Office of Basic Energy Sciences, US Department of Energy [DE-FG-02-05ER46200, AC03-76SF00098, DE-FG02-07ER46352]; KAKENHI [26800165]; MEXT, Photon and Quantum Basic Research Coordinated Development Program; Center for Integrated Nanotechnologies, a DOE Office of Basic Energy Sciences user facility FX Acknowledgements M.N. is supported by LANL LDRD Program and start-up fund from University of Central Florida. T.D. was supported by NSF IR/D program. The work at Princeton and synchrotron X-ray-based measurements are supported by the Office of Basic Energy Sciences, US Department of Energy (grants DE-FG-02-05ER46200, AC03-76SF00098 and DE-FG02-07ER46352). Y.I. acknowledges support from KAKENHI No. 26800165. S.S. acknowledges support from MEXT, Photon and Quantum Basic Research Coordinated Development Program. J.-X. Zhu is supported by the Center for Integrated Nanotechnologies, a DOE Office of Basic Energy Sciences user facility. M.N. acknowledges A.V. Balatsky at LANL for fruitful discussion. We thank Plumb Nicholas Clark for beamline assistance at the SLS, PSI. NR 44 TC 4 Z9 4 U1 16 U2 59 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 3 PY 2016 VL 6 AR 22557 DI 10.1038/srep22557 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DF2XH UT WOS:000371207200001 PM 26936229 ER PT J AU Bienfait, A Pla, JJ Kubo, Y Zhou, X Stern, M Lo, CC Weis, CD Schenkel, T Vion, D Esteve, D Morton, JJL Bertet, P AF Bienfait, A. Pla, J. J. Kubo, Y. Zhou, X. Stern, M. Lo, C. C. Weis, C. D. Schenkel, T. Vion, D. Esteve, D. Morton, J. J. L. Bertet, P. TI Controlling spin relaxation with a cavity SO NATURE LA English DT Article ID SPONTANEOUS EMISSION; RESONANCE EXPERIMENTS; SILICON; POLARIZATION; MICROCAVITY; DONORS AB Spontaneous emission of radiation is one of the fundamental mechanisms by which an excited quantum system returns to equilibrium. For spins, however, spontaneous emission is generally negligible compared to other non-radiative relaxation processes because of the weak coupling between the magnetic dipole and the electromagnetic field. In 1946, Purcell realized(1) that the rate of spontaneous emission can be greatly enhanced by placing the quantum system in a resonant cavity. This effect has since been used extensively to control the lifetime of atoms and semiconducting heterostructures coupled to microwave(2) or optical(3,4) cavities, and is essential for the realization of high-efficiency single-photon sources(5). Here we report the application of this idea to spins in solids. By coupling donor spins in silicon to a superconducting microwave cavity with a high quality factor and a small mode volume, we reach the regime in which spontaneous emission constitutes the dominant mechanism of spin relaxation. The relaxation rate is increased by three orders of magnitude as the spins are tuned to the cavity resonance, demonstrating that energy relaxation can be controlled on demand. Our results provide a general way to initialize spin systems into their ground state and therefore have applications in magnetic resonance and quantum information processing(6). They also demonstrate that the coupling between the magnetic dipole of a spin and the electromagnetic field can be enhanced up to the point at which quantum fluctuations have a marked effect on the spin dynamics; as such, they represent an important step towards the coherent magnetic coupling of individual spins to microwave photons. C1 [Bienfait, A.; Kubo, Y.; Zhou, X.; Stern, M.; Vion, D.; Esteve, D.; Bertet, P.] Univ Paris Saclay, CEA Saclay, CNRS, Quantron Grp,SPEC,CEA, F-91191 Gif Sur Yvette, France. [Pla, J. J.; Lo, C. C.; Morton, J. J. L.] UCL, London Ctr Nanotechnol, London WC1H 0AH, England. [Zhou, X.] CNRS, UMR 8520, ISEN Dept, Inst Elect Microelect & Nanotechnol, Ave Poincare,CS 60069, F-59652 Villeneuve Dascq, France. [Stern, M.] Bar Ilan Univ, BINA, Quantum Nanoelect Lab, Ramat Gan, Israel. [Weis, C. D.; Schenkel, T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Accelerator Technol & Appl Phys Div, Berkeley, CA 94720 USA. [Pla, J. J.] Univ New S Wales, Sch Elect Engn & Telecommun, Sydney, NSW 2052, Australia. [Kubo, Y.] Okinawa Inst Sci & Technol, Grad Univ, Onna, Okinawa 9040495, Japan. RP Bertet, P (reprint author), Univ Paris Saclay, CEA Saclay, CNRS, Quantron Grp,SPEC,CEA, F-91191 Gif Sur Yvette, France. EM patrice.bertet@cea.fr RI Kubo, Yuimaru/I-6546-2013; Morton, John/I-3515-2013 OI Kubo, Yuimaru/0000-0001-5803-4287; FU European Research Council under the European Community [615767, 279781, 630070]; C'Nano IdF project QUANTROCRYO; Royal Society; Royal Commission; US Department of Energy [DE-AC02-05CH11231] FX We acknowledge technical support from P. Senat, D. Duet, J.-C. Tack, P. Pari and P. Forget, as well as discussions within the Quantronics group. We acknowledge support of the European Research Council under the European Community's Seventh Framework Programme (FP7/2007-2013) through grant agreements No. 615767 (CIRQUSS), 279781 (ASCENT) and 630070 (quRAM), and of the C'Nano IdF project QUANTROCRYO. J.J.L.M. is supported by the Royal Society. C.C.L. is supported by the Royal Commission for the Exhibition of 1851. T.S. and C.D.W. were supported by the US Department of Energy under contract DE-AC02-05CH11231. NR 40 TC 10 Z9 10 U1 17 U2 48 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD MAR 3 PY 2016 VL 531 IS 7592 BP 74 EP + DI 10.1038/nature16944 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DF2YW UT WOS:000371211900042 PM 26878235 ER PT J AU Robertson, M Wei, SC Beer, L Adedinsewo, D Stockwell, S Dombrowski, JC Johnson, C Skarbinski, J AF Robertson, McKaylee Wei, Stanley C. Beer, Linda Adedinsewo, Demilade Stockwell, Sandra Dombrowski, Julia C. Johnson, Christopher Skarbinski, Jacek TI Delayed entry into HIV medical care in a nationally representative sample of HIV-infected adults receiving medical care in the USA SO AIDS CARE-PSYCHOLOGICAL AND SOCIO-MEDICAL ASPECTS OF AIDS/HIV LA English DT Article DE initiation of care; HIV testing; HIV/AIDS; HIV care continuum; Linkage to care ID HUMAN-IMMUNODEFICIENCY-VIRUS; ANTIRETROVIRAL THERAPY; UNITED-STATES; EARLY RETENTION; RISK-FACTORS; VIRAL LOAD; DIAGNOSIS; LINKAGE; TRANSMISSION; PREVENTION AB Before widespread antiretroviral therapy (ART), an estimated 17% of people delayed HIV care. We report national estimates of the prevalence and factors associated with delayed care entry in the contemporary ART era. We used Medical Monitoring Project data collected from June 2009 through May 2011 for 1425 persons diagnosed with HIV from May 2004 to April 2009 who initiated care within 12 months. We defined delayed care as entry >three months from diagnosis. Adjusted prevalence ratios (aPRs) were calculated to identify risk factors associated with delayed care. In this nationally representative sample of HIV-infected adults receiving medical care, 7.0% (95% confidence interval [CI]: 5.3-8.8) delayed care after diagnosis. Black race was associated with a lower likelihood of delay than white race (aPR 0.38). Men who have sex with women versus women who have sex with men (aPR 1.86) and persons required to take an HIV test versus recommended by a provider (aPR 2.52) were more likely to delay. Among those who delayed 48% reported a personal factor as the primary reason. Among persons initially diagnosed with HIV (non-AIDS), those who delayed care were twice as likely (aPR 2.08) to develop AIDS as of May 2011. Compared to the pre-ART era, there was a nearly 60% reduction in delayed care entry. Although relatively few HIV patients delayed care entry, certain groups may have an increased risk. Focus on linkage to care among persons who are required to take an HIV test may further reduce delayed care entry. C1 [Robertson, McKaylee; Adedinsewo, Demilade] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. [Robertson, McKaylee; Wei, Stanley C.; Beer, Linda; Adedinsewo, Demilade; Stockwell, Sandra; Johnson, Christopher; Skarbinski, Jacek] Ctr Dis Control & Prevent, Div HIV AIDS Prevent, Atlanta, GA USA. [Wei, Stanley C.] US PHS, Atlanta, GA USA. [Dombrowski, Julia C.] Univ Washington, Dept Med, Seattle, WA USA. [Dombrowski, Julia C.] Publ Hlth Seattle & King Cty HIV STD Program, Seattle, WA USA. RP Robertson, M (reprint author), Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA.; Robertson, M (reprint author), Ctr Dis Control & Prevent, Div HIV AIDS Prevent, Atlanta, GA USA. EM mr1472@hunter.cuny.edu OI Adedinsewo, Demilade/0000-0002-8629-2029 FU Centers for Disease Control and Prevention [PS09-937] FX This research was supported in part by an appointment to the Research Participation Program at the Centers for Disease Control and Prevention administered by the Oak Ridge Institute for Science and Education through an agreement between the US Department of Energy and CDC. Funding for the Medical Monitoring Project is provided by a cooperative agreement (PS09-937) from the Centers for Disease Control and Prevention. NR 32 TC 1 Z9 1 U1 3 U2 5 PU ROUTLEDGE JOURNALS, TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXFORDSHIRE, ENGLAND SN 0954-0121 EI 1360-0451 J9 AIDS CARE JI Aids Care-Psychol. Socio-Med. Asp. Aids-Hiv PD MAR 3 PY 2016 VL 28 IS 3 BP 325 EP 333 DI 10.1080/09540121.2015.1096891 PG 9 WC Health Policy & Services; Public, Environmental & Occupational Health; Psychology, Multidisciplinary; Respiratory System; Social Sciences, Biomedical SC Health Care Sciences & Services; Public, Environmental & Occupational Health; Psychology; Respiratory System; Biomedical Social Sciences GA DE5PD UT WOS:000370682600009 PM 26493721 ER PT J AU Miyamoto, H Schnupf, U Crowley, MF Brady, JW AF Miyamoto, Hitomi Schnupf, Udo Crowley, Michael F. Brady, John W. TI Comparison of the simulations of cellulosic crystals with three carbohydrate force fields SO CARBOHYDRATE RESEARCH LA English DT Article DE Molecular mechanics calculations; Molecular dynamics simulations; Carbohydrate force fields; Conformational energy calculations ID MOLECULAR-DYNAMICS; COMPUTER-SIMULATION; BETA; METHYL; WATER; DIFFRACTION; ALGORITHMS; METHANOL; PROGRAM; GLUCOSE AB Three independently developed molecular mechanics force fields for carbohydrates have been used to simulate a suite of small molecule analogs of cellulose for which crystal structures have been reported, as a test to determine which might be best for simulations of cellulose itself. Such evaluation is necessary since the reported cellulose crystal structure is not stable in molecular dynamics simulations with any available force field. The present simulations found that all three resulted in small deviations from the reported crystal structures, but that all were reasonably accurate and none was clearly superior to the others for the entire suite of structures examined. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Miyamoto, Hitomi] Technion Israel Inst Technol, Dept Chem Engn, IL-32000 Haifa, Israel. [Miyamoto, Hitomi; Brady, John W.] Cornell Univ, Dept Food Sci, Ithaca, NY 14853 USA. [Schnupf, Udo] Bradley Univ, Dept Chem & Biochem, Peoria, IL 61625 USA. [Crowley, Michael F.] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA. [Crowley, Michael F.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. RP Brady, JW (reprint author), Cornell Univ, Dept Food Sci, Ithaca, NY 14853 USA. EM jwb7@cornell.edu RI Schnupf, Udo/H-4703-2016 OI Schnupf, Udo/0000-0002-1457-1985 FU Office of Advanced Scientific Computing Research; JSPS Postdoctoral Fellowships FX The U.S. Department of Energy, Office of Biological and Environmental Research, and the Office of Advanced Scientific Computing Research supported this work under the SciDAC Program. H.M. thanks the JSPS Postdoctoral Fellowships for Research Abroad. NR 41 TC 1 Z9 1 U1 5 U2 14 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0008-6215 EI 1873-426X J9 CARBOHYD RES JI Carbohydr. Res. PD MAR 3 PY 2016 VL 422 BP 17 EP 23 DI 10.1016/j.carres.2016.01.001 PG 7 WC Biochemistry & Molecular Biology; Chemistry, Applied; Chemistry, Organic SC Biochemistry & Molecular Biology; Chemistry GA DD8FP UT WOS:000370161200004 PM 26845704 ER PT J AU Amorim, B Cortijo, A de Juan, F Grushine, AG Guinea, F Gutierrez-Rubio, A Ochoa, H Parente, V Roldan, R San-Jose, P Schiefele, J Sturla, M Vozmediano, MAH AF Amorim, B. Cortijo, A. de Juan, F. Grushine, A. G. Guinea, F. Gutierrez-Rubio, A. Ochoa, H. Parente, V. Roldan, R. San-Jose, P. Schiefele, J. Sturla, M. Vozmediano, M. A. H. TI Novel effects of strains in graphene and other two dimensional materials SO PHYSICS REPORTS-REVIEW SECTION OF PHYSICS LETTERS LA English DT Review DE Graphene; 2D materials; Strain; Elasticity theory ID SCANNING-TUNNELING-MICROSCOPY; HEXAGONAL BORON-NITRIDE; TRANSITION-METAL DICHALCOGENIDES; CHEMICAL-VAPOR-DEPOSITION; BILAYER MOLYBDENUM-DISULFIDE; FRENKEL-KONTOROVA MODEL; PSEUDO-MAGNETIC FIELDS; SELF-CONSISTENT THEORY; FERMI-LIQUID BEHAVIOR; POLYMERIZED MEMBRANES AB The analysis of the electronic properties of strained or lattice deformed graphene combines ideas from classical condensed matter physics, soft matter, and geometrical aspects of quantum field theory (QFT) in curved spaces. Recent theoretical and experimental work shows the influence of strains in many properties of graphene not considered before, such as electronic transport, spin orbit coupling, the formation of Moire patterns and optics. There is also significant evidence of anharmonic effects, which can modify the structural properties of graphene. These phenomena are not restricted to graphene, and they are being intensively studied in other two dimensional materials, such as the transition metal dichalcogenides. We review here recent developments related to the role of strains in the structural and electronic properties of graphene and other two dimensional compounds. (C) 2016 Elsevier B.V. All rights reserved. C1 [Amorim, B.; Cortijo, A.; Gutierrez-Rubio, A.; Ochoa, H.; Parente, V.; Roldan, R.; San-Jose, P.; Schiefele, J.; Vozmediano, M. A. H.] CSIC, Inst Ciencia Mat Madrid, Plaza Murillo 2, E-28049 Madrid, Spain. [Amorim, B.] Univ Minho, Dept Phys, P-4710057 Braga, Portugal. [Amorim, B.] Univ Minho, Ctr Phys, P-4710057 Braga, Portugal. [de Juan, F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [de Juan, F.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Grushine, A. G.] Max Planck Inst Phys Komplexer Syst, D-01187 Dresden, Germany. [Guinea, F.] Univ Manchester, Sch Phys & Astron, Oxford Rd, Manchester M13 9PL, Lancs, England. [Guinea, F.; Parente, V.] IMDEA Nanociencia, Calle Faraday 9, Madrid 28049, Spain. [Guinea, F.; Ochoa, H.] DIPC, San Sebastian 20018, Spain. [Sturla, M.] Univ Nacl La Plata, Dept Fis, IFLP CONICET, RA-1900 La Plata, Buenos Aires, Argentina. RP Amorim, B (reprint author), CSIC, Inst Ciencia Mat Madrid, Plaza Murillo 2, E-28049 Madrid, Spain. EM amorim.bac@icmm.csic.es RI Roldan, Rafael/A-9075-2011; San-Jose, Pablo/A-4795-2010; DONOSTIA INTERNATIONAL PHYSICS CTR., DIPC/C-3171-2014; Ochoa, Hector/K-1504-2015; Guinea, Francisco/A-7122-2008; Amorim, Bruno/J-5018-2015; Cortijo Fernandez, Alberto/K-5808-2013; de Juan, Fernando/B-9392-2008; OI Roldan, Rafael/0000-0002-9316-464X; San-Jose, Pablo/0000-0002-7920-5273; Guinea, Francisco/0000-0001-5915-5427; Amorim, Bruno/0000-0001-8566-0718; Cortijo Fernandez, Alberto/0000-0002-6689-3871; de Juan, Fernando/0000-0001-6852-1484; Schiefele, Jurgen/0000-0002-6422-0200 FU Fundacao para a Ciencia e a Tecnologia, Portugal [SFRI-I/BD/78987/2011]; European Union through ESF funded-JAE doc program; JAE-Pre (CSIC, Spain); Juan de la Cierva Program (MINECO, Spain); FCT-Portugal [EXPL/FIS-NAN/1728/2013]; ERC Advanced Grant [290846]; Spanish Ministry of Economy (MINECO) [FIS2011-23713, FIS2014-58445-JIN]; CONICET [PIP 0747]; ANPCyT [PICT 2012-1724]; Spanish MECD grant [PIB2010BZ-00512]; European Union Seventh Framework Programme [604391] FX We acknowledge the financial support of the following institutions: Fundacao para a Ciencia e a Tecnologia, Portugal, through Grant No. SFRI-I/BD/78987/2011 (BA); European Union through ESF funded-JAE doc program (AC); JAE-Pre (CSIC, Spain) (AGR); Juan de la Cierva Program (MINECO, Spain) and FCT-Portugal through Grant No. EXPL/FIS-NAN/1728/2013 (RR); ERC Advanced Grant 290846 (FG, VP); Spanish Ministry of Economy (MINECO) through Grant Nos. FIS2011-23713 (PSJ) and FIS2014-58445-JIN (RR); CONICET (PIP 0747) and ANPCyT (PICT 2012-1724) (MS); Spanish MECD grant PIB2010BZ-00512, and the European Union Seventh Framework Programme under Grant Agreement No. 604391 Graphene Flagship (MV, JS). NR 430 TC 27 Z9 27 U1 88 U2 226 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-1573 EI 1873-6270 J9 PHYS REP JI Phys. Rep.-Rev. Sec. Phys. Lett. PD MAR 3 PY 2016 VL 617 BP 1 EP 54 DI 10.1016/j.physrep.2015.12.006 PG 54 WC Physics, Multidisciplinary SC Physics GA DE2KG UT WOS:000370455600001 ER PT J AU Sha, SJ Khazenzon, AM Ghosh, PM Rankin, KP Pribadi, M Coppola, G Geschwind, DH Rabinovici, GD Miller, BL Lee, SE AF Sha, Sharon J. Khazenzon, Anna M. Ghosh, Pia M. Rankin, Katherine P. Pribadi, Mochtar Coppola, Giovanni Geschwind, Daniel H. Rabinovici, Gil D. Miller, Bruce L. Lee, Suzee E. TI Early-onset Alzheimer's disease versus frontotemporal dementia: resolution with genetic diagnoses? SO NEUROCASE LA English DT Article DE Frontotemporal dementia; Alzheimer's disease ID HEXANUCLEOTIDE REPEAT EXPANSION; AMYOTROPHIC-LATERAL-SCLEROSIS; TRAUMATIC BRAIN-INJURY; BEHAVIORAL VARIANT; C9ORF72 MUTATIONS; TEMPORAL-LOBE; HEAD TRAUMA; ATROPHY; TAU; DEGENERATION AB We report a diagnostically challenging case of a 64-year-old man with a history of remote head trauma who developed mild behavioral changes and dyscalculia. He was diagnosed with clinical Alzheimer's disease (AD), with additional features consistent with behavioral variant frontotemporal dementia. Structural magnetic resonance imaging revealed atrophy in bilateral frontal and parietal cortices and hippocampi on visual inspection and left frontal pole and bilateral anterior temporal encephalomalacia, suspected to be due to head trauma. Consistent with the diagnosis of Alzheimer's pathology, positron emission tomography (PET) with Pittsburgh compound B suggested the presence of beta-amyloid. Fluorodeoxyglucose PET demonstrated hypometabolism in bilateral frontal and temporoparietal cortices. Voxel-based morphometry showed atrophy predominant in ventral frontal regions (bilateral orbitofrontal cortex, pregenual anterior cingulate/medial superior frontal gyrus), bilateral mid cingulate, bilateral lateral temporal cortex, and posterior insula. Bilateral caudate, thalamus, hippocampi, and cerebellum were prominently atrophied. Unexpectedly, a pathologic hexanucleotide repeat expansion in C9ORF72 was identified in this patient. This report underscores the clinical variability in C9ORF72 expansion carriers and the need to consider mixed pathologies, particularly when imaging studies are inconsistent with a single syndrome or pathology. C1 [Sha, Sharon J.] Stanford Univ, Dept Neurol & Neurol Sci, Stanford, CA 94305 USA. [Khazenzon, Anna M.; Ghosh, Pia M.; Rankin, Katherine P.; Rabinovici, Gil D.; Miller, Bruce L.; Lee, Suzee E.] Univ Calif San Francisco, Dept Neurol, Memory & Aging Ctr, San Francisco, CA USA. [Ghosh, Pia M.; Rabinovici, Gil D.] Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA. [Pribadi, Mochtar; Coppola, Giovanni; Geschwind, Daniel H.] Univ Calif Los Angeles, Semel Inst Neurosci & Human Behav, Dept Psychiat, Los Angeles, CA 90024 USA. [Pribadi, Mochtar; Coppola, Giovanni; Geschwind, Daniel H.] Univ Calif Los Angeles, Semel Inst Neurosci & Human Behav, Dept Neurol, Los Angeles, CA 90024 USA. [Rabinovici, Gil D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Radiol, Berkeley, CA 94720 USA. RP Lee, SE (reprint author), Univ Calif San Francisco, Dept Neurol, Memory & Aging Ctr, San Francisco, CA USA. EM suzeelee@memory.ucsf.edu FU National Institute on Aging [R01 AG029577, P50 AG023501, P01 AG019724, K23 AG039414]; John Douglas French Alzheimer's Foundation; Tau Consortium FX Dr. Rankin is supported by the National Institute on Aging under Grant R01 AG029577. Dr. Coppola is supported by the John Douglas French Alzheimer's Foundation and the Tau Consortium. Dr. Miller is supported by the National Institute on Aging under Grant P50 AG023501; under grant P01 AG019724. Dr. Geschwind is also supported by P01 AG019724, Miller, PI and the Tau Consortium. Dr. Lee is supported by the National Institute on Aging under grant K23 AG039414. NR 37 TC 0 Z9 0 U1 0 U2 21 PU ROUTLEDGE JOURNALS, TAYLOR & FRANCIS LTD PI ABINGDON PA 2-4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 1355-4794 EI 1465-3656 J9 NEUROCASE JI Neurocase PD MAR 3 PY 2016 VL 22 IS 2 BP 161 EP 167 DI 10.1080/13554794.2015.1080283 PG 7 WC Clinical Neurology; Psychiatry; Psychology SC Neurosciences & Neurology; Psychiatry; Psychology GA DD2RR UT WOS:000369770400005 PM 26304661 ER PT J AU Amonette, JE Matyas, J AF Amonette, J. E. Matyas, J. TI Determination of ferrous and total iron in refractory spinels SO ANALYTICA CHIMICA ACTA LA English DT Article DE Ferrous iron; Spinel; 1,10-Phenanthroline; Nickel; Hydrofluoric acid; Silver; Potentiometry; Ferrous ethylenediammonium sulfate; Ferrous ammonium sulfate; Potassium bromide ID ELEMENTAL CONCENTRATION DATA; QUANTITATIVE ASSAY; PHOTOCHEMICAL METHOD; SILICATE MINERALS; FERRIC IRON; ROCKS; 1,10-PHENANTHROLINE; OXIDE; COMPILATION; FE AB Accurate and precise determination of the redox state of iron (Fe) in spinels presents a significant challenge due to their refractory nature. The resultant extreme conditions needed to obtain complete dissolution generally oxidize some of the Fe(II) initially present and thus prevent the use of colorimetric methods for Fe(II) measurements. To overcome this challenge we developed a hybrid oxidimetric/colorimetric approach, using Ag(I) as the oxidimetric reagent for determination of Fe(II) and 1,10-phenanthroline as the colorimetric reagent for determination of total Fe. This approach, which allows determination of Fe(II) and total Fe on the same sample, was tested on a series of four geochemical reference materials and then applied to the analysis of Fe(Ni) spinel crystals isolated from simulated high-level-waste (HLW) glass and of several reagent magnetites. Results for the reference materials were in excellent agreement with recommended values, with the exception of USGS BIR-1, for which higher Fe(II) values and lower total Fe values were obtained. The Fe(Ni) spinels showed Fe(II) values at the detection limit (ca. 0.03 wt% Fe) and total Fe values higher than obtained by ICP-AES analysis after decomposition by lithium metaborate/tetraborate fusion. For the magnetite samples, total Fe values were in agreement with reference results, but a wide range in Fe(II) values was obtained indicating various degrees of conversion to maghemite. Formal comparisons of accuracy and precision were made with 13 existing methods. Accuracy for Fe(II) and total Fe was at or near the top of the group. Precision varied with the parameter used to measure it but was generally in the middle to upper part of the group for Fe(II) while that for total Fe ranged from the bottom of the group to near the top. (C) 2016 Elsevier B.V. All rights reserved. C1 [Amonette, J. E.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. [Matyas, J.] Pacific NW Natl Lab, Dept Mat Sci, Richland, WA 99352 USA. RP Amonette, JE (reprint author), Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. FU U.S. Department of Energy's Waste Treatment and Immobilization Plant Federal Project Office; U.S. Department of Energy [DE-AC05-76RL01830] FX This project has been supported by the U.S. Department of Energy's Waste Treatment and Immobilization Plant Federal Project Office under the direction of Dr. Albert A. Kruger. Pacific Northwest National Laboratory is operated by Battelle for the U.S. Department of Energy under Contract DE-AC05-76RL01830. We thank Odeta Qafoku for preparing and providing samples of the in-house-synthesized magnetite analyzed. NR 33 TC 1 Z9 1 U1 12 U2 38 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0003-2670 EI 1873-4324 J9 ANAL CHIM ACTA JI Anal. Chim. Acta PD MAR 3 PY 2016 VL 910 BP 25 EP 35 DI 10.1016/j.aca.2015.12.024 PG 11 WC Chemistry, Analytical SC Chemistry GA DD0VE UT WOS:000369637600003 PM 26873465 ER PT J AU Scholl, M Lockhart, SN Schonhaut, DR O'Neil, JP Janabi, M Ossenkoppele, R Baker, SL Vogel, JW Faria, J Schwimmer, HD Rabinovici, GD Jagust, WJ AF Schoell, Michael Lockhart, Samuel N. Schonhaut, Daniel R. O'Neil, James P. Janabi, Mustafa Ossenkoppele, Rik Baker, Suzanne L. Vogel, Jacob W. Faria, Jamie Schwimmer, Henry D. Rabinovici, Gil D. Jagust, William J. TI PET Imaging of Tau Deposition in the Aging Human Brain SO NEURON LA English DT Article ID MILD COGNITIVE IMPAIRMENT; ALZHEIMERS-DISEASE; NEUROFIBRILLARY TANGLES; EPISODIC MEMORY; CEREBROSPINAL-FLUID; NATIONAL INSTITUTE; AGE CATEGORIES; SENILE PLAQUES; AMYLOID-BETA; A-BETA AB Tau pathology is a hallmark of Alzheimer's disease (AD) but also occurs in normal cognitive aging. Using the tau PET agent F-18-AV-1451, we examined retention patterns in cognitively normal older people in relation to young controls and AD patients. Age and beta-amyloid (measured using PiB PET) were differentially associated with tau tracer retention in healthy aging. Older age was related to increased tracer retention in regions of the medial temporal lobe, which predicted worse episodic memory performance. PET detection of tau in other isocortical regions required the presence of cortical b-amyloid and was associated with decline in global cognition. Furthermore, patterns of tracer retention corresponded well with Braak staging of neurofibrillary tau pathology. The present study defined patterns of tau tracer retention in normal aging in relation to age, cognition, and beta-amyloid deposition. C1 [Schoell, Michael; Lockhart, Samuel N.; Ossenkoppele, Rik; Vogel, Jacob W.; Schwimmer, Henry D.; Rabinovici, Gil D.; Jagust, William J.] Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA. [Schoell, Michael] MedTech West, S-41345 Gothenburg, Sweden. [Schoell, Michael] Univ Gothenburg, Dept Clin Neurosci & Rehabil, S-41345 Gothenburg, Sweden. [Schonhaut, Daniel R.; Ossenkoppele, Rik; Rabinovici, Gil D.] Univ Calif San Francisco, Dept Neurol, Memory & Aging Ctr, San Francisco, CA 94158 USA. [O'Neil, James P.; Janabi, Mustafa; Baker, Suzanne L.; Faria, Jamie; Rabinovici, Gil D.; Jagust, William J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Ossenkoppele, Rik] Vrije Univ Amsterdam, Med Ctr, Dept Neurol & Alzheimer Ctr, Neurosci Campus Amsterdam, NL-1081 HV Amsterdam, Netherlands. RP Jagust, WJ (reprint author), Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA.; Jagust, WJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM jagust@berkeley.edu RI Scholl, Michael/A-4184-2014; OI Scholl, Michael/0000-0001-7800-1781; Schwimmer, Henry/0000-0002-6055-6401 FU UCSF Alzheimer's Disease Research Center (NIH) [P50-AG23501]; NIH [P50-AG23501, AG034570, R01-AG045611]; Swedish Medical Association; Tau Consortium; Blanceflor Foundation; John Douglas French Alzheimer's Foundation; Marie Curie FP7 International Outgoing Fellowship [628812]; BrightFocus Foundation; Avid Radiopharmaceuticals FX We thank Philip Insel for statistical analyses support, and Dr. Bruce Miller and the UCSF Alzheimer's Disease Research Center (NIH grant P50-AG23501) for AD patient evaluations and referrals. This research was supported by NIH grants AG034570 (W.J.J.), R01-AG045611 (G.D.R.), and P50-AG23501 (Dr. Bruce L. Miller, G.D.R.), the Swedish Medical Association (M.S.), Tau Consortium (W.J.J., G.D.R.), the Blanceflor Foundation (M.S.), John Douglas French Alzheimer's Foundation (G.D.R.), the Marie Curie FP7 International Outgoing Fellowship (628812) (R.O.), and the donors of (Alzheimer's Disease Research), a program of BrightFocus Foundation (R.O.). Avid Radiopharmaceuticals enabled use of the 18F-AV-1451 tracer but did not provide direct funding and were not involved in data analysis or interpretation. G.D.R. receives research support from Avid Radiopharmaceuticals, which owns the rights to the 18F-AV-1451 compound. W.J.J. has served as a consultant to Bioclinica, Genentech, and Novartis pharmaceuticals. NR 52 TC 44 Z9 44 U1 16 U2 30 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0896-6273 EI 1097-4199 J9 NEURON JI Neuron PD MAR 2 PY 2016 VL 89 IS 5 BP 971 EP 982 DI 10.1016/j.neuron.2016.01.028 PG 12 WC Neurosciences SC Neurosciences & Neurology GA DI5UG UT WOS:000373565400011 PM 26938442 ER PT J AU Park, KH Oh, DY Choi, YE Nam, YJ Han, LL Kim, JY Xin, HL Lin, F Oh, SM Jung, YS AF Park, Kern Ho Oh, Dae Yang Choi, Young Eun Nam, Young Jin Han, Lili Kim, Ju-Young Xin, Huolin Lin, Feng Oh, Seung M. Jung, Yoon Seok TI Solution-Processable Glass LiI-Li4SnS4 Superionic Conductors for All-Solid-State Li-Ion Batteries SO ADVANCED MATERIALS LA English DT Article ID LITHIUM SECONDARY BATTERIES; THIO-LISICON; RECHARGEABLE BATTERIES; ELECTRODE MATERIALS; CONDUCTIVITY; CHALLENGES; SYSTEMS; STORAGE; LICOO2; FILM C1 [Park, Kern Ho; Oh, Dae Yang; Choi, Young Eun; Nam, Young Jin; Jung, Yoon Seok] UNIST, Dept Energy Engn, Sch Energy & Chem Engn, Ulsan 689798, South Korea. [Park, Kern Ho; Oh, Seung M.] Seoul Natl Univ, Sch Chem & Biol Engn, 599 Gwanangno, Seoul 151742, South Korea. [Han, Lili; Xin, Huolin] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Kim, Ju-Young] UNIST, Mat Sci & Engn, Ulsan 689798, South Korea. [Lin, Feng] Lawrence Berkeley Natl Lab, Energy Storage & Distributed Resources Div, Berkeley, CA 94720 USA. RP Jung, YS (reprint author), UNIST, Dept Energy Engn, Sch Energy & Chem Engn, Ulsan 689798, South Korea.; Oh, SM (reprint author), Seoul Natl Univ, Sch Chem & Biol Engn, 599 Gwanangno, Seoul 151742, South Korea. EM seungoh@snu.ac.kr; ysjung@unist.ac.kr RI Xin, Huolin/E-2747-2010; Jung, Yoon Seok/B-8512-2011 OI Xin, Huolin/0000-0002-6521-868X; Jung, Yoon Seok/0000-0003-0357-9508 FU Basic Science Research Program through the National Research Foundation of Korea (NRF) - Ministry of Education [NRF-2014R1A1A2058760]; Energy Efficiency & Resources Core Technology Program of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) - Korea government Ministry of Trade, Industry Energy [20152010103470]; MSIP; POSTECH; U.S. DOE Office of Science Facility, at Brookhaven National Laboratory [DE-SC0012704] FX This work was supported by Basic Science Research Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Education (No. NRF-2014R1A1A2058760), and by the Energy Efficiency & Resources Core Technology Program of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant funded by the Korea government Ministry of Trade, Industry & Energy (No. 20152010103470). Experiments at PLS were supported in part by MSIP and POSTECH. This research used the EM facility of the Center for Functional Nanomaterials, which is a U.S. DOE Office of Science Facility, at Brookhaven National Laboratory under Contract No. DE-SC0012704. NR 51 TC 9 Z9 9 U1 47 U2 116 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD MAR 2 PY 2016 VL 28 IS 9 BP 1874 EP 1883 DI 10.1002/adma.201505008 PG 10 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DG6EV UT WOS:000372176200021 PM 26690558 ER PT J AU Semelsberger, TA Veenstra, M Dixon, C AF Semelsberger, Troy A. Veenstra, Mike Dixon, Craig TI Room temperature thermal conductivity measurements of neat MOF-5 compacts with high pressure hydrogen and helium SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Thermal conductivity; MOF-5; High pressure; Hydrogen; Heat capacity; Hydrogen storage ID STORAGE AB Metal-organic frameworks (MOFs) are a highly porous crystalline material with potential in various applications including on-board vehicle hydrogen storage for fuel cell vehicles. The thermal conductivity of MOFs is an important parameter in the design and ultimate performance of an on-board hydrogen storage system. However, in-situ thermal conductivity measurements have not been previously reported. The present study reports room temperature thermal conductivity and thermal diffusivity measurements performed on neat MOF-5 cylindrical compacts (rho = 0.4 g/mL) as a function of pressure (0.27-90 bar) and gas type (hydrogen and helium). The transient plane source technique was used to measure both the non-directional thermal properties (isotropic method) and the directional thermal properties (anisotropic method). High pressure measurements were made using our in-house built low temperature, high pressure thermal conductivity sample cell. The intrinsic thermal properties of neat MOF-5 measured under vacuum were-Isotropic: k(isotropic) = 0.1319 W/m K, alpha(isotropic) = 0.4165 mm(2)/s; Anisotropic: k(axial) = 0.1477 W/m K, k(radial) = 0.1218 W/m K, alpha(axial) = 0.5096 mm(2)/s, and alpha(radial) = 0.4232 mm(2)/s. The apparent thermal properties of neat MOF-5 increased with increasing hydrogen and helium pressure, with the largest increase occurring in the narrow pressure range of 0-10 bar and then monotonically asymptoting with increasing pressures up to around 90 bar. On average, a greater than two-fold enhancement in the apparent thermal properties was observed with neat MOF-5 in the presence of helium and hydrogen compared to the intrinsic values of neat MOF-5 measured under vacuum. The apparent thermal properties of neat MOF-5 measured with hydrogen were higher than those measured with helium, which were directly related to the gas-specific thermal properties of helium and hydrogen. Neat MOF-5 exhibited a small degree of anisotropy under all conditions measured with thermal conductivities and diffusivities in the axial direction being higher than those in the radial direction. The low temperature specific heat capacities of neat MOF-5 were also measured and reported for the temperature range of 93-313 K (-180-40 degrees C). Copyright (c) 2016, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Semelsberger, Troy A.] Los Alamos Natl Lab, Mat Phys & Applicat Div, POB 1663,Mail Stop K763, Los Alamos, NM 87545 USA. [Veenstra, Mike] Ford Motor Co, Res & Adv Engn, Dearborn, MI 48121 USA. [Dixon, Craig] ThermTest Inc, 34 Melissa St,Unit 1, Fredericton, NB E3A 6W1, Canada. RP Semelsberger, TA (reprint author), Los Alamos Natl Lab, Mat Phys & Applicat Div, POB 1663,Mail Stop K763, Los Alamos, NM 87545 USA. EM troy@lanl.gov FU United States Department of Energy, Office of Energy Efficiency and Renewable Energy, Fuel Cell Technologies Office [DE-PS36-08GO98006] FX This work was funded by the United States Department of Energy, Office of Energy Efficiency and Renewable Energy, Fuel Cell Technologies Office (DE-PS36-08GO98006). The authors gratefully acknowledge our DOE program managers Dr. Ned Stetson (Hydrogen Storage Team Lead) and Mr. Jesse Adams (DOE Golden Field Office). The authors also acknowledge the Hydrogen Storage Engineering Center of Excellence Partners for productive discussions and their dedication to hydrogen storage. NR 11 TC 1 Z9 1 U1 6 U2 23 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 EI 1879-3487 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD MAR 2 PY 2016 VL 41 IS 8 BP 4690 EP 4702 DI 10.1016/j.ijhydene.2015.12.059 PG 13 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA DH1RQ UT WOS:000372563000017 ER PT J AU Karuppagounder, SS Alim, I Khim, SJ Bourassa, MW Sleiman, SF John, R Thinnes, CC Yeh, TL Demetriades, M Neitemeier, S Cruz, D Gazaryan, I Killilea, DW Morgenstern, L Xi, GH Keep, RF Schallert, T Tappero, RV Zhong, J Cho, S Maxfield, FR Holman, TR Culmsee, C Fong, GH Su, YJ Ming, GL Song, HJ Cave, JW Schofield, CJ Colbourne, F Coppola, G Ratan, RR AF Karuppagounder, Saravanan S. Alim, Ishraq Khim, Soah J. Bourassa, Megan W. Sleiman, Sama F. John, Roseleen Thinnes, Cyrille C. Yeh, Tzu-Lan Demetriades, Marina Neitemeier, Sandra Cruz, Dana Gazaryan, Irina Killilea, David W. Morgenstern, Lewis Xi, Guohua Keep, Richard F. Schallert, Timothy Tappero, Ryan V. Zhong, Jian Cho, Sunghee Maxfield, Frederick R. Holman, Theodore R. Culmsee, Carsten Fong, Guo-Hua Su, Yijing Ming, Guo-li Song, Hongjun Cave, John W. Schofield, Christopher J. Colbourne, Frederick Coppola, Giovanni Ratan, Rajiv R. TI Therapeutic targeting of oxygen-sensing prolyl hydroxylases abrogates ATF4-dependent neuronal death and improves outcomes after brain hemorrhage in several rodent models SO SCIENCE TRANSLATIONAL MEDICINE LA English DT Article ID INDUCED INTRACEREBRAL HEMORRHAGE; FOCAL CEREBRAL-ISCHEMIA; CENTRAL-NERVOUS-SYSTEM; MOUSE MODEL; TRANSCRIPTION FACTOR; ALZHEIMERS-DISEASE; OXIDATIVE STRESS; IN-VIVO; HYPOXIA; INJURY AB Disability or death due to intracerebral hemorrhage (ICH) is attributed to blood lysis, liberation of iron, and consequent oxidative stress. Iron chelators bind to free iron and prevent neuronal death induced by oxidative stress and disability due to ICH, but the mechanisms for this effect remain unclear. We show that the hypoxia-inducible factor prolyl hydroxylase domain (HIF-PHD) family of iron-dependent, oxygen-sensing enzymes are effectors of iron chelation. Molecular reduction of the three HIF-PHD enzyme isoforms in the mouse striatum improved functional recovery after ICH. A low-molecular-weight hydroxyquinoline inhibitor of the HIF-PHD enzymes, adaptaquin, reduced neuronal death and behavioral deficits after ICH in several rodent models without affecting total iron or zinc distribution in the brain. Unexpectedly, protection fromo xidative death invitroor from ICH in vivo by adaptaquin was associated with suppression of activity of the prodeath factor ATF4 rather than activation of an HIF-dependent prosurvival pathway. Together, these findings demonstrate that brain-specific inactivation of the HIF-PHD metalloenzymes with the blood-brain barrier-permeable inhibitor adaptaquin can improve functional outcomes after ICH in several rodent models. C1 [Karuppagounder, Saravanan S.; Alim, Ishraq; Khim, Soah J.; Bourassa, Megan W.; Sleiman, Sama F.; Gazaryan, Irina; Zhong, Jian; Cho, Sunghee; Cave, John W.; Ratan, Rajiv R.] Cornell Univ, Coll Med, Burke Med Res Inst, Sperling Ctr Hemorrhag Stroke Recovery, White Plains, NY 10605 USA. [Karuppagounder, Saravanan S.; Alim, Ishraq; Khim, Soah J.; Bourassa, Megan W.; Sleiman, Sama F.; Gazaryan, Irina; Zhong, Jian; Cho, Sunghee; Cave, John W.; Ratan, Rajiv R.] Cornell Univ, Weill Med Coll, Feil Family Brain & Mind Res Inst, New York, NY 10065 USA. [John, Roseleen; Colbourne, Frederick] Univ Alberta, Dept Psychol, Edmonton, AB T6G 2E9, Canada. [Thinnes, Cyrille C.; Yeh, Tzu-Lan; Demetriades, Marina; Schofield, Christopher J.] Univ Oxford, Dept Chem, Oxford OX1 3TA, England. [Neitemeier, Sandra; Culmsee, Carsten] Univ Marburg, Inst Pharmakol & Klin Pharm, D-35032 Marburg, Germany. [Cruz, Dana; Maxfield, Frederick R.] Cornell Univ, Weill Med Coll, Dept Biochem, New York, NY 10065 USA. [Killilea, David W.] Childrens Hosp Oakland, Oakland, CA 94609 USA. [Morgenstern, Lewis] Univ Michigan, Dept Neurol, Ann Arbor, MI 48109 USA. [Xi, Guohua; Keep, Richard F.] Univ Michigan, Dept Neurosurg, Ann Arbor, MI 48109 USA. [Schallert, Timothy] Univ Texas Austin, Dept Psychol, Austin, TX 78712 USA. [Tappero, Ryan V.] Brookhaven Natl Lab, Photon Sci Directorate, Upton, NY 11973 USA. [Zhong, Jian; Holman, Theodore R.] Univ Calif Santa Cruz, Chem & Biochem, Santa Cruz, CA 95064 USA. [Fong, Guo-Hua] Univ Connecticut, Ctr Hlth, Ctr Vasc Biol, Farmington, CT 06030 USA. [Su, Yijing; Ming, Guo-li; Song, Hongjun] Johns Hopkins Univ, Sch Med, Inst Cell Engn, Baltimore, MD 21205 USA. [Coppola, Giovanni] Univ Calif Los Angeles, Dept Psychiat, Los Angeles, CA 90095 USA. RP Ratan, RR (reprint author), Cornell Univ, Coll Med, Burke Med Res Inst, Sperling Ctr Hemorrhag Stroke Recovery, White Plains, NY 10605 USA.; Ratan, RR (reprint author), Cornell Univ, Weill Med Coll, Feil Family Brain & Mind Res Inst, New York, NY 10065 USA. EM rrr2001@med.cornell.edu OI Cruz, Dana/0000-0003-4793-7696; Schofield, Christopher/0000-0002-0290-6565 FU Dr. Miriam and Sheldon G. Adelson Medical Research Foundation; Burke Foundation; New York State Department of Health Center for Research Excellence in Spinal Cord Injury [DOHC019772]; NIH [P01 NIA AG014930]; Welcome Trust; British Heart Foundation; National Institute of Neurological Disorders and Stroke Informatics Center for Neurogenetics and Neurogenomics [P30 NS062691]; Sperling Center for Hemorrhagic Stroke Recovery at the Burke Medical Research Institute FX This work was funded with support from the Dr. Miriam and Sheldon G. Adelson Medical Research Foundation, the Burke Foundation, the Sperling Center for Hemorrhagic Stroke Recovery at the Burke Medical Research Institute, New York State Department of Health Center for Research Excellence in Spinal Cord Injury (grant DOHC019772), NIH (grant P01 NIA AG014930, project 1, to R.R.R.). G.C. thanks the National Institute of Neurological Disorders and Stroke Informatics Center for Neurogenetics and Neurogenomics (P30 NS062691). C.J.S. thanks the Welcome Trust and the British Heart Foundation for funding Cancer Research, UK. C.C. thanks the Neuroscience PhD program of the University of Marburg. NR 52 TC 3 Z9 3 U1 5 U2 8 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 1946-6234 EI 1946-6242 J9 SCI TRANSL MED JI Sci. Transl. Med. PD MAR 2 PY 2016 VL 8 IS 328 AR 328ra29 DI 10.1126/scitranslmed.aac6008 PG 17 WC Cell Biology; Medicine, Research & Experimental SC Cell Biology; Research & Experimental Medicine GA DG4YL UT WOS:000372079000003 PM 26936506 ER PT J AU Kim, YY Semsarilar, M Carloni, JD Cho, KR Kulak, AN Polishchuk, I Hendley, CT Smeets, PJM Fielding, LA Pokroy, B Tang, CC Estroff, LA Baker, SP Armes, SP Meldrum, FC AF Kim, Yi-Yeoun Semsarilar, Mona Carloni, Joseph D. Cho, Kang Rae Kulak, Alexander N. Polishchuk, Iryna Hendley, Coit T. Smeets, Paul J. M. Fielding, Lee A. Pokroy, Boaz Tang, Chiu C. Estroff, Lara A. Baker, Shefford P. Armes, Steven P. Meldrum, Fiona C. TI Structure and Properties of Nanocomposites Formed by the Occlusion of Block Copolymer Worms and Vesicles Within Calcite Crystals SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article ID RAFT DISPERSION POLYMERIZATION; BIOGENIC CALCITE; AMINO-ACIDS; NANOCRYSTAL SUPERLATTICES; INORGANIC NANOPARTICLES; MECHANICAL-PROPERTIES; ORGANIC-MOLECULES; NONPOLAR-SOLVENTS; SINGLE-CRYSTALS; NANO-OBJECTS AB This article describes an experimentally versatile strategy for producing inorganic/organic nanocomposites, with control over the microstructure at the nano-and mesoscales. Taking inspiration from biominerals, CaCO3 is coprecipitated with anionic diblock copolymer worms or vesicles to produce single crystals of calcite occluding a high density of the organic component. This approach can also be extended to generate complex structures in which the crystals are internally patterned with nano-objects of differing morphologies. Extensive characterization of the nanocomposite crystals using high resolution synchrotron powder X-ray diffraction and vibrational spectroscopy demonstrates how the occlusions affect the short and long-range order of the crystal lattice. By comparison with nanocomposite crystals containing latex particles and copolymer micelles, it is shown that the effect of these occlusions on the crystal lattice is dominated by the interface between the inorganic crystal and the organic nano-objects, rather than the occlusion size. This is supported by in situ atomic force microscopy studies of worm occlusion in calcite, which reveal flattening of the copolymer worms on the crystal surface, followed by burial and void formation. Finally, the mechanical properties of the nanocomposite crystals are determined using nanoindentation techniques, which reveal that they have hardnesses approaching those of biogenic calcites. C1 [Kim, Yi-Yeoun; Kulak, Alexander N.; Meldrum, Fiona C.] Univ Leeds, Sch Chem, Leeds LS2 9JT, W Yorkshire, England. [Semsarilar, Mona; Fielding, Lee A.; Armes, Steven P.] Univ Sheffield, Dept Chem, Sheffield S3 7HF, S Yorkshire, England. [Carloni, Joseph D.; Hendley, Coit T.; Estroff, Lara A.; Baker, Shefford P.] Cornell Univ, Dept Mat Sci & Engn, Ithaca, NY 14853 USA. [Carloni, Joseph D.; Hendley, Coit T.; Fielding, Lee A.; Baker, Shefford P.] Cornell Univ, Kavli Inst Nanoscale Sci Phys Sci Bldg, Ithaca, NY 14853 USA. [Cho, Kang Rae; Smeets, Paul J. M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Polishchuk, Iryna; Pokroy, Boaz] Technion Israel Inst Technol, Dept Mat Sci & Engn, IL-32000 Haifa, Israel. [Polishchuk, Iryna; Pokroy, Boaz] Technion Israel Inst Technol, Russell Berrie Nanotechnol Inst, IL-32000 Haifa, Israel. [Tang, Chiu C.] Diamond Light Source, Harwell Sci & Innovat Campus, Didcot OX11 0DE, Oxon, England. [Armes, Steven P.] Univ Manchester, Sch Mat, Oxford Rd, Manchester M13 9PL, Lancs, England. RP Kim, YY; Meldrum, FC (reprint author), Univ Leeds, Sch Chem, Leeds LS2 9JT, W Yorkshire, England. EM Y.Y.Kim@leeds.ac.uk; F.Meldrum@leeds.ac.uk RI Fielding, Lee/B-8440-2011; Semsarilar, Mona/P-1939-2016; OI Fielding, Lee/0000-0002-4958-1155; Semsarilar, Mona/0000-0002-1544-1824; Smeets, Paul/0000-0002-7281-0120 FU US National Science Foundation (Materials Word Network) [DMR 1210304]; Engineering and Physical Sciences Research Council (EPSRC) [EP/H005374/1]; EPSRC [EP/J018589/1, EP/K006304/1]; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; Hysitron Inc, (Edina, MN, USA) FX This project was supported by a grant from the US National Science Foundation (Materials Word Network Award DMR 1210304,), an Engineering and Physical Sciences Research Council (EPSRC) Leadership Fellowship (F.C.M. and YYK, EP/H005374/1), and EPSRC grants EP/J018589/1 (Materials World Network, F.C.M. and Y.Y.K.) and EP/K006304/1 (F.C.M. and A.N.K.). Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The work was further supported by Hysitron Inc, (Edina, MN, USA). The authors acknowledge Diamond Light Source for time on beamline I11 under commissioning time and proposal EE10137. The authors would also like to thank Prof. Jim De Yoreo for providing access to AFM facilities and for giving useful advice, and Andre H. Groschel for providing the copolymer schematics. NR 53 TC 10 Z9 10 U1 23 U2 82 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD MAR 2 PY 2016 VL 26 IS 9 BP 1382 EP 1392 DI 10.1002/adfm.201504292 PG 11 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DG6FR UT WOS:000372179100009 ER PT J AU Khabibullin, A Bhangaonkar, K Mahoney, C Lu, Z Schmitt, M Sekizkardes, AK Bockstaller, MR Matyjaszewski, K AF Khabibullin, Amir Bhangaonkar, Karan Mahoney, Clare Lu, Zhao Schmitt, Michael Sekizkardes, Ali Kemal Bockstaller, Michael R. Matyjaszewski, Krzysztof TI Grafting PMMA Brushes from alpha-Alumina Nanoparticles via SI-ATRP SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE SI-ATRP; hybrid materials; alpha-alumina; polymer brushes; poly(methyl methacrylate); grafting density ID TRANSFER RADICAL POLYMERIZATION; HYBRID MATERIALS; NANOCOMPOSITES; SURFACES; COMPOSITES; MEMBRANES; BEHAVIOR AB Alumina nanoparticles are widely used as nano fillers for polymer nanocomposites. Among several different polymorphs of alumina, alpha-alumina has the most desirable combination of physical properties. Hence, the attachment of polymer chains to alpha-alumina to enhance compatibility in polymeric matrixes is an important goal. However, the chemical inertness and low concentration of surface hydroxyl groups have rendered polymer modification of alpha-alumina a long-standing challenge. Herein, we report that activation of a-alumina in concentrated or molten NaOH as well as in molten K2S2O7 increased polymer graft density up to 50%, thereby facilitating the synthesis of alpha-alumina brush particles with uniform grafting density of 0.05 nm(-2) that are readily miscible or dispersible in organic solvents or in chemically compatible polymeric hosts. C1 [Khabibullin, Amir; Bhangaonkar, Karan; Matyjaszewski, Krzysztof] Carnegie Mellon Univ, Dept Chem, 4400 Fifth Ave, Pittsburgh, PA 15213 USA. [Mahoney, Clare; Lu, Zhao; Schmitt, Michael; Bockstaller, Michael R.] Carnegie Mellon Univ, Dept Mat Sci & Engn, 5000 Forbes Ave, Pittsburgh, PA 15213 USA. [Sekizkardes, Ali Kemal] US DOE, NETL, 626 Cochrans Mill Rd, Pittsburgh, PA 15129 USA. RP Matyjaszewski, K (reprint author), Carnegie Mellon Univ, Dept Chem, 4400 Fifth Ave, Pittsburgh, PA 15213 USA. EM km3b@andrew.cmu.edu RI Bockstaller, Michael/A-9124-2011; Matyjaszewski, Krzysztof/A-2508-2008 OI Bockstaller, Michael/0000-0001-9046-9539; Matyjaszewski, Krzysztof/0000-0003-1960-3402 FU National Science Foundation [NSF DMR-1501324]; U.S. Department of Energy [DoE EE0006702] FX The authors acknowledge financial support from the National Science Foundation (NSF DMR-1501324) and the U.S. Department of Energy (DoE EE0006702). NR 39 TC 3 Z9 3 U1 18 U2 48 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD MAR 2 PY 2016 VL 8 IS 8 BP 5458 EP 5465 DI 10.1021/acsami.5b12311 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DF6GJ UT WOS:000371453600048 PM 26901494 ER PT J AU Zheng, JM Yan, PF Cao, RG Xiang, HF Engelhard, MH Polzin, BJ Wang, CM Zhang, JG Xu, W AF Zheng, Jianming Yan, Pengfei Cao, Ruiguo Xiang, Hongfa Engelhard, Mark H. Polzin, Bryant J. Wang, Chongmin Zhang, Ji-Guang Xu, Wu TI Effects of Propylene Carbonate Content in CsPF6-Containing Electrolytes on the Enhanced Performances of Graphite Electrode for Lithium-Ion Batteries SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE propylene carbonate; cesium cation; solid electrolyte interphase; graphite exfoliation; lithium-ion battery ID INTERPHASIAL CHEMISTRY; NONAQUEOUS ELECTROLYTES; ENERGY-STORAGE; ANODE; CELLS; INTERCALATION; LNTERPHASE AB The effects Of propylene carbonate (PC) content in CsPF6-containing electrolytes on the performances of graphite electrode in lithium half cells and in graphite parallel to LiNi0.80Co0.15Al0.05O2 (NCA) full cells are investigated. It is found that the performance of graphite electrode is significantly-affected by PC content in the CsPF6-containing electrolytes. An optimal PC content of 20% by weight in the solvent mixtures is identified. The enhanced electrochemical performance of graphite electrode can be attributed to the synergistic effects of the PC solvent and the Cs+ additive. The synergistic effects of Cs+ additive and appropriate amount of PC enable the formation of a robust, ultrathin, and compact solid electrolyte interphase (SEI) layer on the surface of graphite electrode, which is only permeable for desolvated Li+ ions and allows fast Li+ ion transport through it. Therefore, this SEI layer effectively suppresses the PC cointercalation and largely alleviates the Li dendrite formation on graphite electrode during lithiation even at relatively high current densities. The presence of low-melting-point PC solvent improves the sustainable operation of graphite parallel to NCA full cells under a wide temperature range. The fundamental findings also shed light On the importance of manipulating/maintaining the electrode/electrolyte interphasial stability in various energy-storage devices. C1 [Zheng, Jianming; Cao, Ruiguo; Xiang, Hongfa; Zhang, Ji-Guang; Xu, Wu] Pacific NW Natl Lab, Energy & Environm Directorate, 902 Battelle Blvd, Richland, WA 99354 USA. [Yan, Pengfei; Engelhard, Mark H.; Wang, Chongmin] Pacific NW Natl Lab, Environm Mol Sci Lab, 902 Battelle Blvd, Richland, WA 99354 USA. [Xiang, Hongfa] Hefei Univ Technol, Sch Mat Sci & Engn, Hefei 230009, Anhui, Peoples R China. [Polzin, Bryant J.] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Zhang, JG; Xu, W (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, 902 Battelle Blvd, Richland, WA 99354 USA. EM jiguang.zhang@pnnl.gov; wu.xu@pnnl.gov RI Zheng, Jianming/F-2517-2014; yan, pengfei/E-4784-2016; Cao, Ruiguo/O-7354-2016; Xiang, Hongfa/I-5126-2012; OI Zheng, Jianming/0000-0002-4928-8194; yan, pengfei/0000-0001-6387-7502; Xiang, Hongfa/0000-0002-6182-1932; Engelhard, Mark/0000-0002-5543-0812 FU Advanced Battery Materials Research (BMR) programs of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231, 18769]; DOE's Office of Biological and Environmental Research; National Science Foundation of China [21006033, 51372060]; Fundamental Research Funds for the Central Universities [2013HGCH0002]; DOE [DE-AC05-76RLO1830] FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, the Advanced Battery Materials Research (BMR) programs of the U.S. Department of Energy (DOE) under contract no. DE-AC02-05CH11231, subcontract no. 18769. The SEM/TEM observations and XPS analysis were conducted in the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). H.X. acknowledges financial support from National Science Foundation of China (Grant Nos. 21006033 and 51372060) and Fundamental Research Funds for the Central Universities (2013HGCH0002). Pacific Northwest National Laboratory is operated by Battelle for the DOE under Contract DE-AC05-76RLO1830. NR 27 TC 2 Z9 2 U1 21 U2 55 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD MAR 2 PY 2016 VL 8 IS 8 BP 5715 EP 5722 DI 10.1021/acsami.5b12517 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DF6GJ UT WOS:000371453600077 PM 26862677 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Aurousseau, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Balunas, WK Banas, E Banerjee, S Bannoura, AAE Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, M Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Biedermann, D Bieniek, SP Biesuz, NV Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biondi, S Bjergaard, DM Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Blunier, S Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehler, M Bogaerts, JA Bogavac, D Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutle, SK Boveia, A Boyd, J Boyko, IR Bozic, I Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Madden, WDB Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, K Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E de Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Bruschi, M Bruscino, N Bryngemark, L Buanes, T Buat, Q Buchholz, P Buckley, AG Buda, SI Budagov, IA Buehrer, F Bugge, L Bugge, MK Bulekov, O Bullock, D Burckhart, H Burdin, S Burgard, CD Burghgrave, B Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Buzykaev, AR Urban, SC Caforio, D Cairo, VM Cakir, O Calace, N Calafiura, P Calandri, A Calderini, G Calfayan, P Caloba, LP Calvet, D Calvet, S Toro, RC Camarda, S Camarri, P Cameron, D Armadans, RC Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Carbone, RM Cardarelli, R Cardillo, F Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Caudron, J Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, BC Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chang, P Chapman, JD Charlton, DG Chau, CC Barajas, CAC Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, S Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A Cheremushkina, E El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiarelli, G Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Choi, K Chouridou, S Chow, BKB Christodoulou, V Chromek-Burckhart, D Chudoba, J Chuinard, AJ Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Cinca, D Cindro, V Cioara, IA Ciocio, A Cirotto, F Citron, ZH Ciubancan, M Clark, A Clark, BL Clark, PJ Clarke, RN Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Cogan, JG Colasurdo, L Cole, B Cole, S Colijn, AP Collot, J Colombo, T Compostella, G Muino, PC Coniavitis, E Connell, SH Connelly, IA Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cote, D Cottin, G Cowan, G Cox, BE Cranmer, K Cree, G Crepe-Renaudin, S Crescioli, F Cribbs, WA Ortuzar, MC Cristinziani, M Croft, V Crosetti, G Donszelmann, TC Cummings, J Curatolo, M Cuth, J Cuthbert, C Czirr, H Czodrowski, P D'Auria, S D'Onofrio, M De Sousa, MJDS Da Via, C Dabrowski, W Dafinca, A Dai, T Dale, O Dallaire, F Dallapiccola, C Dam, M Dandoy, JR Dang, NP Daniells, AC Danninger, M Hoffmann, MD Dao, V Darbo, G Darmora, S Dassoulas, J Dattagupta, A Davey, W David, C Davidek, T Davies, E Davies, M Davison, P Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Benedetti, A De Castro, S De Cecco, S De Groot, N de Jong, P De la Torre, H De Lorenzi, F De Pedis, D De Salvo, A De Sanctis, U De Santo, A De Regie, JBDV 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Zhang, F. Zhang, G. Zhang, H. Zhang, J. Zhang, L. Zhang, R. Zhang, X. Zhang, Z. Zhao, X. Zhao, Y. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Measurement of jet charge in dijet events from root s=8 TeV pp collisions with the ATLAS detector SO PHYSICAL REVIEW D LA English DT Article ID GAUGE-BOSON COUPLINGS; B-QUARK PRODUCTION; PARTON DISTRIBUTIONS; GLUON JETS; NET CHARGE; ASYMMETRY; DECAYS; FRAGMENTATION; Z0; SCATTERING AB The momentum-weighted sum of the charges of tracks associated to a jet is sensitive to the charge of the initiating quark or gluon. This paper presents a measurement of the distribution of momentum-weighted sums, called jet charge, in dijet events using 20.3 fb(-1) of data recorded with the ATLAS detector at root s = 8 TeV in pp collisions at the LHC. The jet charge distribution is unfolded to remove distortions from detector effects and the resulting particle-level distribution is compared with several models. The p(T) dependence of the jet charge distribution average and standard deviation are compared to predictions obtained with several leading-order and next-to-leading-order parton distribution functions. The data are also compared to different Monte Carlo simulations of QCD dijet production using various settings of the free parameters within these models. The chosen value of the strong coupling constant used to calculate gluon radiation is found to have a significant impact on the predicted jet charge. There is evidence for a pT dependence of the jet charge distribution for a given jet flavor. In agreement with perturbative QCD predictions, the data show that the average jet charge of quark-initiated jets decreases in magnitude as the energy of the jet increases. C1 [Jackson, P.; Lee, L.; Petridis, A.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Yildiz, H. Duran] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Kuday, S.] Istanbul Aydin Univ, Istanbul, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. 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M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] INFN Grp Collegato Cosenza, Lab Nazl Frascati, Cosenza, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. 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S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Notkestr 85, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] INFN Lab Nazl Frascati, Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Calace, N.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Paolozzi, L.; Picazio, A.; Ristic, B.; Schramm, S.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] INFN Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Schott, M.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Schwartz, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolb, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Bortolotto, V.; Castillo, L. R. Flores; Salvucci, A.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores; Salvucci, A.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Jussel, P.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] INFN Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Aad, G.; Alio, L.; Barbero, M.; Beau, T.; Bomben, M.; Calderini, G.; Coadou, Y.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Francavilla, P.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Le Guirriec, E.; Lefebvre, G.; Liu, J.; Liu, K.; Madaffari, D.; Malaescu, B.; Marchiori, G.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Pralavorio, P.; Ridel, M.; Roos, L.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Trincaz-Duvoid, S.; Vacavant, L.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fys Inst, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Hu, X.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Tollefson, K.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] INFN Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. 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Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] INFN Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Konig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.; Slawinska, M.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] INFN Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Machado Miguens, J.; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] INFN Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] INFN Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] INFN Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] INFN Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, DSM IRFU Inst Rech Lois Fondament Uniers, Commissariat Energie Atom & Energies Alternat, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Hance, M.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. 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Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. 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D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. 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[Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Jovicevic, J.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] INFN Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Giordani, M. P.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Cobal, M.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Gradin, P. O. J.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. 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A.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; Gignac, M.; Henkelmann, S.; King, S. B.; Lister, A.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; Marino, C. 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C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Braun, H. M.; Cornelissen, T.; Ellinghaus, F.; Ernis, G.; Fischer, J.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Thomsen, L. A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Inst Natl Phys Nucl & Phys Particules IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London WC2R 2LS, England. 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RI Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Garcia, Jose /H-6339-2015; Stabile, Alberto/L-3419-2016; Villa, Mauro/C-9883-2009; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Gavrilenko, Igor/M-8260-2015; Di Domenico, Antonio/G-6301-2011; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Vranjes Milosavljevic, Marija/F-9847-2016; Gladilin, Leonid/B-5226-2011; Chekulaev, Sergey/O-1145-2015; White, Ryan/E-2979-2015; Zhukov, Konstantin/M-6027-2015; SULIN, VLADIMIR/N-2793-2015; Snesarev, Andrey/H-5090-2013; Brooks, William/C-8636-2013; Nechaeva, Polina/N-1148-2015; Mashinistov, Ruslan/M-8356-2015; Fedin, Oleg/H-6753-2016; Vykydal, Zdenek/H-6426-2016; Aguilar Saavedra, Juan Antonio/F-1256-2016; Livan, Michele/D-7531-2012; Warburton, Andreas/N-8028-2013; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Tikhomirov, Vladimir/M-6194-2015; Doyle, Anthony/C-5889-2009; Carvalho, Joao/M-4060-2013; Boyko, Igor/J-3659-2013; Mitsou, Vasiliki/D-1967-2009; Guo, Jun/O-5202-2015; Sanchez, Javier/F-5073-2016; Gorelov, Igor/J-9010-2015; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; BESSON, NATHALIE/L-6250-2015; La Rosa Navarro, Jose Luis/K-4221-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Smirnova, Oxana/A-4401-2013; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Conde Muino, Patricia/F-7696-2011 OI Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; KUBOTA, TAKASHI/0000-0002-1156-5571; Stabile, Alberto/0000-0002-6868-8329; Villa, Mauro/0000-0002-9181-8048; Kukla, Romain/0000-0002-1140-2465; Di Domenico, Antonio/0000-0001-8078-2759; Gauzzi, Paolo/0000-0003-4841-5822; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Gladilin, Leonid/0000-0001-9422-8636; White, Ryan/0000-0003-3589-5900; SULIN, VLADIMIR/0000-0003-3943-2495; Brooks, William/0000-0001-6161-3570; Mashinistov, Ruslan/0000-0001-7925-4676; Vykydal, Zdenek/0000-0003-2329-0672; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Livan, Michele/0000-0002-5877-0062; Warburton, Andreas/0000-0002-2298-7315; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Tikhomirov, Vladimir/0000-0002-9634-0581; Doyle, Anthony/0000-0001-6322-6195; Carvalho, Joao/0000-0002-3015-7821; Boyko, Igor/0000-0002-3355-4662; Mitsou, Vasiliki/0000-0002-1533-8886; Guo, Jun/0000-0001-8125-9433; Gorelov, Igor/0000-0001-5570-0133; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Smirnova, Oxana/0000-0003-2517-531X; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Conde Muino, Patricia/0000-0002-9187-7478 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF, Canada; Canada Council, Canada; CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET, European Union; ERC, European Union; FP7, European Union; Horizon, European Union; Marie Sk?odowska-Curie Actions, European Union; Investissements d'Avenir Labex, France; Investissements d'Avenir Idex, France; ANR, France; Region Auvergne, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos programme - EU-ESF; Thales programme - EU-ESF; Aristeia programme - EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sk?odowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 80 TC 0 Z9 0 U1 19 U2 50 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 2 PY 2016 VL 93 IS 5 AR 052003 DI 10.1103/PhysRevD.93.052003 PG 35 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DF5SH UT WOS:000371412100001 ER PT J AU Bond-Lamberty, B Bolton, H Fansler, S Heredia-Langner, A Liu, CX McCue, LA Smith, J Bailey, V AF Bond-Lamberty, Ben Bolton, Harvey Fansler, Sarah Heredia-Langner, Alejandro Liu, Chongxuan McCue, Lee Ann Smith, Jeffrey Bailey, Vanessa TI Soil Respiration and Bacterial Structure and Function after 17 Years of a Reciprocal Soil Transplant Experiment SO PLOS ONE LA English DT Article ID ORGANIC-MATTER DECOMPOSITION; SHRUB-STEPPE ECOSYSTEM; CLIMATE-CHANGE; MICROBIAL COMMUNITIES; TEMPERATURE SENSITIVITY; TERRESTRIAL ECOSYSTEMS; SEMIARID ECOSYSTEMS; NORTH-AMERICA; FOREST SOIL; GAS FLUXES AB The effects of climate change on soil organic matter-its structure, microbial community, carbon storage, and respiration response-remain uncertain and widely debated. In addition, the effects of climate changes on ecosystem structure and function are often modulated or delayed, meaning that short-term experiments are not sufficient to characterize ecosystem responses. This study capitalized on a long-term reciprocal soil transplant experiment to examine the response of dryland soils to climate change. The two transplant sites were separated by 500 m of elevation on the same mountain slope in eastern Washington state, USA, and had similar plant species and soil types. We resampled the original 1994 soil transplants and controls, measuring CO2 production, temperature response, enzyme activity, and bacterial community structure after 17 years. Over a laboratory incubation of 100 days, reciprocally transplanted soils respired roughly equal cumulative amounts of carbon as non-transplanted controls from the same site. Soils transplanted from the hot, dry, lower site to the cooler and wetter (difference of -5 degrees C monthly maximum air temperature, +50 mm yr(-1) precipitation) upper site exhibited almost no respiratory response to temperature (Q(10) of 1.1), but soils originally from the upper, cooler site had generally higher respiration rates. The bacterial community structure of transplants did not differ significantly from that of untransplanted controls, however. Slight differences in local climate between the upper and lower Rattlesnake locations, simulated with environmental control chambers during the incubation, thus prompted significant differences in microbial activity, with no observed change to bacterial structure. These results support the idea that environmental shifts can influence soil C through metabolic changes, and suggest that microbial populations responsible for soil heterotrophic respiration may be constrained in surprising ways, even as shorter-and longer-term soil microbial dynamics may be significantly different under changing climate. C1 [Bond-Lamberty, Ben] Univ Maryland, Pacific NW Natl Lab, Joint Global Change Res Inst, 5825 Univ Res Court 3500, College Pk, MD 20740 USA. [Bolton, Harvey; Fansler, Sarah; Heredia-Langner, Alejandro; Liu, Chongxuan; McCue, Lee Ann; Bailey, Vanessa] Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99352 USA. [Smith, Jeffrey] Washington State Univ, USDA ARS, 215 Johnson Hall, Pullman, WA 99164 USA. RP Bond-Lamberty, B (reprint author), Univ Maryland, Pacific NW Natl Lab, Joint Global Change Res Inst, 5825 Univ Res Court 3500, College Pk, MD 20740 USA. EM bondlamberty@pnnl.gov RI Bond-Lamberty, Ben/C-6058-2008; Liu, Chongxuan/C-5580-2009; OI Bond-Lamberty, Ben/0000-0001-9525-4633; Bailey, Vanessa/0000-0002-2248-8890; McCue, Lee Ann/0000-0003-4456-517X FU U.S. Department of Energy, Office of Science, Biological and Environmental Research (BER) as part of the Terrestrial Ecosystem Sciences Program; Signature Discovery Initiative at the Pacific Northwest National Laboratory (PNNL); BER; DOE [DE-AC05-76RL01830] FX This research was supported by the U.S. Department of Energy, Office of Science, Biological and Environmental Research (BER) as part of the Terrestrial Ecosystem Sciences Program and the Signature Discovery Initiative at the Pacific Northwest National Laboratory (PNNL). Carbon analyses were performed at the Environmental Molecular Sciences Laboratory, a DOE Office of Science user facility sponsored by the BER and located at PNNL. PNNL is operated for DOE by Battelle Memorial Institute under contract DE-AC05-76RL01830. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript.; This research was supported by the U.S. Department of Energy, Office of Science, Biological and Environmental Research (BER) as part of the Terrestrial Ecosystem Sciences Program and the Signature Discovery Initiative at the Pacific Northwest National Laboratory (PNNL). Carbon analyses were performed at the Environmental Molecular Sciences Laboratory, a DOE Office of Science user facility sponsored by the BER and located at PNNL. PNNL is operated for DOE by Battelle Memorial Institute under contract DE-AC05-76RL01830. This paper is dedicated to the memory of Jeff Smith. NR 64 TC 3 Z9 3 U1 7 U2 39 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 2 PY 2016 VL 11 IS 3 AR e0150599 DI 10.1371/journal.pone.0150599 PG 16 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DG0AN UT WOS:000371724200105 PM 26934712 ER PT J AU Montella, S Balan, V Sousa, LD Gunawan, C Giacobbe, S Pepe, O Faraco, V AF Montella, Salvatore Balan, Venkatesh Sousa, Leonardo da Costa Gunawan, Christa Giacobbe, Simona Pepe, Olimpia Faraco, Vincenza TI Saccharification of newspaper waste after ammonia fiber expansion or extractive ammonia SO AMB EXPRESS LA English DT Article DE AFEX pretreatment; Arabinofuranosidase; Biorefining; Cellulase; EA pretreatment; Hemicellulase; Municipal solid waste; Newspaper waste ID ENZYMATIC-HYDROLYSIS; FERMENTABLE SUGARS; PLATFORM CHEMICALS; ETHANOL-PRODUCTION; EXPLOSION AFEX; CONVERSION; LIGNOCELLULOSE; PRETREATMENT; BIOREFINERY; OPPORTUNITIES AB The lignocellulosic fractions of municipal solid waste (MSW) can be used as renewable resources due to the widespread availability, predictable and low pricing and suitability for most conversion technologies. In particular, after the typical paper recycling loop, the newspaper waste (NW) could be further valorized as feedstock in biorefinering industry since it still contains up to 70 % polysaccharides. In this study, two different physicochemical methods-ammonia fiber expansion (AFEX) and extractive ammonia (EA) were tested for the pretraetment of NW. Furthermore, based on the previously demonstrated ability of the recombinant enzymes endocellulase rCelStrep, alpha-L-arabinofuranosidase rPoAbf and its evolved variant rPoAbf F435Y/Y446F to improve the saccharification of different lignocellulosic pretreated biomasses (such as corn stover and Arundo donax), in this study these enzymes were tested for the hydrolysis of pretreated NW, with the aim of valorizing the lignocellulosic fractions of the MSW. In particular, a mixture of purified enzymes containing cellulases, xylanases and accessory hemicellulases, was chosen as reference mix and rCelStrep and rPoAbf or its variant were replaced to EGI and Larb. The results showed that these enzymatic mixes are not suitable for the hydrolysis of NW after AFEX or EA pretreatment. On the other hand, when the enzymes rCelStrep, rPoAbf and rPoAbf F435Y/Y446F were tested for their effect in hydrolysis of pretreated NW by addition to a commercial enzyme mixture, it was shown that the total polysaccharides conversion yield reached 37.32 % for AFEX pretreated NW by adding rPoAbf to the mix whilst the maximum sugars conversion yield for EA pretreated NW was achieved 40.80 % by adding rCelStrep. The maximum glucan conversion yield obtained (45.61 % for EA pretreated NW by adding rCelStrep to the commercial mix) is higher than or comparable to those reported in recent manuscripts adopting hydrolysis conditions similar to those used in this study. C1 [Montella, Salvatore; Giacobbe, Simona; Faraco, Vincenza] Univ Naples Federico II, Complesso Univ Monte S Angelo, Dept Chem Sci, Via Cintia 4, I-80126 Naples, Italy. [Balan, Venkatesh; Sousa, Leonardo da Costa; Gunawan, Christa] Michigan State Univ, DOE Great Lakes Bioenergy Res Ctr, Dept Chem Engn & Mat Sci, E Lansing, MI 48823 USA. [Pepe, Olimpia] Univ Naples Federico II, Dept Agr, Via Cintia 4, I-80126 Naples, Italy. RP Faraco, V (reprint author), Univ Naples Federico II, Complesso Univ Monte S Angelo, Dept Chem Sci, Via Cintia 4, I-80126 Naples, Italy. EM vfaraco@unina.it FU European Community [318931]; office of Biological and Environmental Research in the DOE Office of Science through the Great Lakes Bioenergy Research Centre (GLBRC) [DE-FC02-07ER64494] FX This research was supported by a Marie Curie International Research Staff Exchange Scheme Fellowship within the 7th European Community Framework Programme: 'Improvement of technologies and tools, e.g., biosystems and biocatalysts, for waste conversion to develop an assortment of high added value eco-friendly and cost-effective bio-products' BIOASSORT (grant number 318931). We gratefully acknowledge support given to VB by the office of Biological and Environmental Research in the DOE Office of Science through the Great Lakes Bioenergy Research Centre (GLBRC) (Grant DE-FC02-07ER64494). We also thank Lucigen Enzyme Company for supplying the research enzymes and Novozyme for supplying the enzyme solutions Cellic (R) CTec3 and the Cellic (R) HTec3 for this work. NR 38 TC 2 Z9 2 U1 4 U2 31 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 2191-0855 J9 AMB EXPRESS JI AMB Express PD MAR 2 PY 2016 VL 6 AR 18 DI 10.1186/s13568-016-0189-9 PG 10 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA DF5IT UT WOS:000371385800001 PM 26936848 ER PT J AU Roy, S Skoff, D Perroni, DV Mondal, J Yethiraj, A Mahanthappa, MK Zanni, MT Skinner, JL AF Roy, Santanu Skoff, David Perroni, Dominic V. Mondal, Jagannath Yethiraj, Arun Mahanthappa, Mahesh K. Zanni, Martin T. Skinner, James L. TI Water Dynamics in Gyroid Phases of Self-Assembled Gemini Surfactants SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID FUEL-CELL MEMBRANES; SPECTRAL DIFFUSION; REVERSE MICELLES; SPECTROSCOPY; INTERFACE; NAFION; CONFINEMENT; NETWORK; SCALES AB Water-mediated ion transport through functional nanoporous materials depends on the dynamics of water-confined within a given nanostructured morphology. Here, we investigate H-bonding dynamics of interfacial water within a "normal" (Type I) lyotropic gyroid phase formed by a gemini dicarboxylate surfactant self-assembly using a combination of 2DIR spectroscopy and molecular dynamics simulations. Experiments and :simulations demonstrate that water dynamics in the normal gyroid phase is 1 order of magnitude slower than that in bulk water, due to specific interactions between water, the ionic surfactant headgroups, and counterions. Yet, the dynamics of water in the normal gyroid phase are faster than those of water confined in a reverse spherical micelle of a sulfonate surfactant, given that the water pool in the reverse micelle and the water, pore in the gyroid phase have roughly the same diameters. This difference in confined water dynamics likely arises from the significantly reduced curvature-induced frustration at the convex interfaces of the normal gyroid, as compared to the concave interfaces of a reverse spherical micelle. These detailed insights into confined water dynamics may guide the future design of artificial membranes that rapidly transport protons and other ions. C1 [Roy, Santanu; Skoff, David; Perroni, Dominic V.; Mondal, Jagannath; Yethiraj, Arun; Mahanthappa, Mahesh K.; Zanni, Martin T.; Skinner, James L.] Univ Wisconsin, Dept Chem, 1101 Univ Ave, Madison, WI 53706 USA. [Roy, Santanu] Pacific NW Natl Lab, Richland, WA 99352 USA. [Mondal, Jagannath] TIFR Ctr Interdisciplinary Sci, Hyderabad, Telangana, India. [Mahanthappa, Mahesh K.] Univ Minnesota, Dept Chem Engn & Mat Sci, 421 Washington Ave SE, Minneapolis, MN 55455 USA. RP Roy, S; Skinner, JL (reprint author), Univ Wisconsin, Dept Chem, 1101 Univ Ave, Madison, WI 53706 USA.; Roy, S (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM santanu.roy@pnnl.gov; skinner@chem.wisc.edu RI Roy, Santanu/D-6215-2012; OI Roy, Santanu/0000-0001-6991-8205; Mahanthappa, Mahesh/0000-0002-9871-804X FU U.S. Department of Energy (DOE) [DE-FG02-09ER16110, DE-SC0010328]; National Science Foundation Grant [CHE-084049] FX This work was primarily supported by U.S. Department of Energy (DOE) Grant No. DE-FG02-09ER16110 (S.R. and J.L.S.), and in part by U.S. DOE Grant No. DE-SC0010328 (D.V.P., A.Y., and M.K.M.), and National Science Foundation Grant CHE-0840494 (supporting the computer cluster PHOENIX at Department of Chemistry, UW-Madison, Wisconsin). NR 38 TC 5 Z9 5 U1 12 U2 64 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAR 2 PY 2016 VL 138 IS 8 BP 2472 EP 2475 DI 10.1021/jacs.5b12370 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DF6GK UT WOS:000371453700003 PM 26875689 ER PT J AU Petrie, JR Cooper, VR Freeland, JW Meyer, TL Zhang, ZY Lutterman, DA Lee, HN AF Petrie, Jonathan R. Cooper, Valentino R. Freeland, John W. Meyer, Tricia L. Zhang, Zhiyong Lutterman, Daniel A. Lee, Ho Nyung TI Enhanced Bifunctional Oxygen Catalysis in Strained LaNiO3 Perovskites SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID FUEL-CELLS; REDUCTION ACTIVITY; EVOLUTION REACTION; OXIDE CATALYSTS; ELECTROCATALYSIS; SURFACES; DESIGN; ALLOY; PRINCIPLES; BATTERIES AB Strain is known to greatly influence low temperature oxygen electro catalysis on noble metal films, leading to significant enhancements in bifunctional activity essential for fuel cells and Metal-air batteries. However, its catalytic impact on transition-metal oxide thin films, such as perovskites, is not widely understood. Here, we epitaxially strain the conducting perovskite LaNiO3 to systematically determine its influence on both the oxygen reduction and oxygen evolution reaction. Uniquely, we found that compressive strain could significantly enhance both reactions, yielding a bifunctional catalyst that surpasses the performance of noble metals' such as Pt. We attribute the improved bifunctionality to strain induced splitting of the e(g) Orbitals, which can customize orbital asymmetry at the surface. Analogous to strain induced shifts in the d-band center of noble metals relative to the Fermi level, :such splitting can dramatically affect catalytic activity in this perovskite and other potentially more active Oxides. C1 [Petrie, Jonathan R.; Cooper, Valentino R.; Meyer, Tricia L.; Lee, Ho Nyung] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Zhang, Zhiyong; Lutterman, Daniel A.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Freeland, John W.] Argonne Natl Lab, Adv Photon Source, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Lee, HN (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM hnlee@ornl.gov RI Cooper, Valentino /A-2070-2012; Zhang, Zhiyong/H-5611-2012; Lee, Ho Nyung/K-2820-2012 OI Cooper, Valentino /0000-0001-6714-4410; Zhang, Zhiyong/0000-0001-7936-9510; Lee, Ho Nyung/0000-0002-2180-3975 FU U.S. Department of Energy (DOE); Office of Science (OS); Basic Energy Sciences (BES); Materials Science and Engineering Division (synthesis, physical property characterization, and XAS data analysis; Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; Scientific User Facilities Division, BES; Fluid Interface Reactions, Structures, and Transport (FIRST) Center, an Energy Frontier Research Center - U.S. DOE, OS, BES [06CH113.57]; BES FX We acknowledge S. Okamoto for theoretical insight. This work was supported by the U.S. Department of Energy (DOE), Office of Science (OS), Basic Energy Sciences (BES), Materials Science and Engineering Division (synthesis, physical property characterization, and XAS data analysis) and by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. DOE (electrochemical characterization and theory). Reference electrode preparation was performed as a user project at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, BES, U.S. DOE. Use of electrochemical testing system was supported by the Fluid Interface Reactions, Structures, and Transport (FIRST) Center, an Energy Frontier Research Center funded by the U.S. DOE, OS, BES. Use of the Advanced Photon Source for XAS was supported by the U.S. DOE, OS, under contract no. DE-AC02-06CH113.57. NR 40 TC 12 Z9 12 U1 43 U2 159 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAR 2 PY 2016 VL 138 IS 8 BP 2488 EP 2491 DI 10.1021/jacs.5b11713 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DF6GK UT WOS:000371453700007 PM 26866808 ER PT J AU Yin, PC Wu, B Mamontov, E Daemen, LL Cheng, YQ Lo, T Seifert, S Hong, KL Bonnesen, PV Keum, JK Ramirez-Cuesta, AJ AF Yin, Panchao Wu, Bin Mamontov, Eugene Daemen, Luke L. Cheng, Yonqiang Lo, Tao Seifert, Soenke Hong, Kunlun Bonnesen, Peter V. Keum, Jong Kahk Ramirez-Cuesta, Anibal J. TI X-ray and Neutron Scattering Study of the Formation of Core-Shell-Type Polyoxometalates SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID BUILDING-BLOCKS; BIOLOGICAL MACROMOLECULES; SUPRAMOLECULAR CHEMISTRY; MASS-SPECTROMETRY; POROUS CAPSULES; ORGANIC HYBRID; ACTIVE-SITES; CLUSTERS; ION; ASSEMBLIES AB A typical type of core-shell polyoxometalates can be obtained through the Keggin-type polyoxometalate-templated growth of a layer of spherical shell structure of {Mo72Fe30}. Small-angle X-ray scattering is used to study the structural features and stability of the core-shell structures in aqueous solutions. Time-resolved small-angle X-ray scattering is applied to monitor the synthetic reactions, and a three-stage formation mechanism is proposed to describe the synthesis of the core-shell polyoxometalates based on the monitoring results. New protocols have been developed by fitting the X-ray data with custom physical models, which provide more convincing, objective, and completed data interpretation. Quasi-elastic and inelastic neutron scattering are used to probe the dynamics of water molecules in the core-shell structures, and two different types of water molecules, the confined and structured water, are observed. These water molecules play an important role in bridging core and shell structures and stabilizing the cluster structures. C1 [Yin, Panchao; Mamontov, Eugene; Daemen, Luke L.; Cheng, Yonqiang; Ramirez-Cuesta, Anibal J.] Oak Ridge Natl Lab, Neutron Sci Directorate, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Wu, Bin] Univ Tennessee, Joint Inst Neutron Sci, Dept Phys & Astron, Knoxville, TN 37996 USA. [Lo, Tao; Seifert, Soenke] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Hong, Kunlun; Bonnesen, Peter V.; Keum, Jong Kahk] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Yin, PC (reprint author), Oak Ridge Natl Lab, Neutron Sci Directorate, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. EM yinp@ornl.gov RI Mamontov, Eugene/Q-1003-2015; Ramirez-Cuesta, Timmy/A-4296-2010; Yin, Panchao/J-3322-2013; Hong, Kunlun/E-9787-2015; Keum, Jong/N-4412-2015 OI Mamontov, Eugene/0000-0002-5684-2675; Ramirez-Cuesta, Timmy/0000-0003-1231-0068; Yin, Panchao/0000-0003-2902-8376; Hong, Kunlun/0000-0002-2852-5111; Keum, Jong/0000-0002-5529-1373 FU Neutron Sciences Directorate of Oak Ridge National Laboratory; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; Office of Science of the US Department of Energy [DE-AC05-00OR22725]; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357] FX P.Y. is grateful to the support of Clifford G. Shull Fellowship from Neutron Sciences Directorate of Oak Ridge National Laboratory. The research performed in BL-2 (BASIS) and BL-16B (VISION) at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. The sample preparation and initial SAXS study in the X-ray lab were conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. Oak Ridge National Laboratory is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC05-00OR22725. The synchrotron-based SAXS study carried out in 12-ID-B and 12-ID-C used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 52 TC 4 Z9 5 U1 14 U2 64 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAR 2 PY 2016 VL 138 IS 8 BP 2638 EP 2643 DI 10.1021/jacs.5b11465 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA DF6GK UT WOS:000371453700035 PM 26848596 ER PT J AU Giordani, V Tozier, D Tan, HJ Burke, CM Gallant, BM Uddin, J Greer, JR McCloskey, BD Chase, GV Addison, D AF Giordani, Vincent Tozier, Dylan Tan, Hongjin Burke, Colin M. Gallant, Betar M. Uddin, Jasim Greer, Julia R. McCloskey, Bryan D. Chase, Gregory V. Addison, Dan TI A Molten Salt Lithium-Oxygen Battery SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID NONAQUEOUS LI-O-2 BATTERIES; DIMETHYL-SULFOXIDE; AIR BATTERIES; ELECTROLYTE; REDUCTION; REACTIVITY; STABILITY AB Despite the promise of extremely high theoretical capacity (2Li + 02 Li2O2, 1675 mAh per gram of oxygen), many challenges currently impede development of Li/O-2 battery technology. Finding suitable electrode and electrolyte materials remains the most elusive challenge to date. A radical new approach is to replace volatile, unstable and air -intolerant organic electrolytes common to prior research in the field with alkali metal nitrate molten salt electrolytes and operate the battery above the liquidus temperature (>80 degrees C). Here we demonstrate an intermediate temperature Li/O-2, battery using a lithium anode, a molten nitrate -based electrolyte (e.g., LiNO3-KNO3 eutectic) and a porous carbon 02 cathode with high energy efficiency (similar to 95%) and improved rate capability because the discharge product, lithium peroxide, is stable and moderately soluble in the molten salt electrolyte. The results, supported by essential state-of--the-art electrochemical, and analytical techniques such as in situ pressure and gas analyses, scanning electron microscopy, rotating disk electrode voltammetry, demonstrate that Li2O2 electro-chemically forms and decomposes upon cycling with discharge/charge overpotentials as low as life of such batteries is limited only by carbon reactivity and by the uncontrolled precipitation of Li2O2, which eventually becomes electrically disconnected from the O-2 electrode. C1 [Giordani, Vincent; Tan, Hongjin; Uddin, Jasim; Chase, Gregory V.; Addison, Dan] Liox Power Inc, 129 N Hill Ave, Pasadena, CA 91106 USA. [Tozier, Dylan; Greer, Julia R.] CALTECH, Div Engn & Appl Sci, Pasadena, CA 91125 USA. [Gallant, Betar M.] CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA. [Burke, Colin M.; McCloskey, Bryan D.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Burke, Colin M.; McCloskey, Bryan D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Storage & Distributed Resources Div, Berkeley, CA 94720 USA. RP Giordani, V; Addison, D (reprint author), Liox Power Inc, 129 N Hill Ave, Pasadena, CA 91106 USA. EM vincent@liox.com; dan@liox.com FU FY Vehicle Technologies Program Wide Funding Opportunity Announcement, by U.S. Department of Energy (DOE) [DE-FOA-0000991 (0991-1872)]; National Energy Technology Laboratory (NETL) on behalf of the Office of Energy Efficiency and Renewable Energy (EERE) FX This work is financially supported as part of the FY 2014 Vehicle Technologies Program Wide Funding Opportunity Announcement, under Award Number DE-FOA-0000991 (0991-1872), by the U.S. Department of Energy (DOE) and National Energy Technology Laboratory (NETL) on behalf of the Office of Energy Efficiency and Renewable Energy (EERE). NR 26 TC 10 Z9 10 U1 32 U2 147 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAR 2 PY 2016 VL 138 IS 8 BP 2656 EP 2663 DI 10.1021/jacs.5b11744 PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA DF6GK UT WOS:000371453700038 PM 26871485 ER PT J AU Tan, XY Fabbris, G Haskel, D Yaroslavtsev, AA Cao, HB Thompson, CM Kovnir, K Menushenkov, AP Chernikov, RV Garlea, VO Shatruk, M AF Tan, Xiaoyan Fabbris, Gilberto Haskel, Daniel Yaroslavtsev, Alexander A. Cao, Huibo Thompson, Corey M. Kovnir, Kirill Menushenkov, Alexey P. Chernikov, Roman V. Garlea, V. Ovidiu Shatruk, Michael TI A Transition from Localized to Strongly Correlated Electron Behavior and Mixed Valence Driven by Physical or Chemical Pressure in ACo(2)As(2) (A = Eu and Ca) SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID MAGNETIC-STRUCTURE; SUPERCONDUCTIVITY; DIFFRACTION; PHOSPHIDES; EUCO2P2; IRON AB We demonstrate that the action of physical pressure, chemical compression, or aliovalent substitution in ACo(2)As(2) (A = Eu and Ca) has a general consequence of causing these antiferromagnetic materials to become ferromagnets. In all cases, the mixed valence triggered at the electropositive A site results in the increase of the Co 3d density of states at the Fermi level. Remarkably, the dramatic alteration of magnetic behavior results from the very minor (<0.15 eleetron) change in the population of the 3d orbitals. The mixed valence state of En observed in the high-pressure (HP) form of EuCo2As2 exhibits a remarkable stability, achieving the average oxidation state of +2.25 at 12.6 GPa. In the case of CaCo2As2, substituting even 10% of Eu or La into the Ca site causes ferromagnetic ordering of Co moments. Similar to HP-EuCo2As2, the itinerant 3d ferromagnetism emerges from electronic doping into the Co layer because of chemical compression of Eu sites in Ca0.9Eu0.1Co1.91As2 or direct electron doping in Ca0.85La0.15Co1.89As2. The results reported herein demonstrate the general possibility of amplifying minor localized electronic effects to achieve major changes in material's properties via involvement of strongly correlated electrons. C1 [Tan, Xiaoyan; Thompson, Corey M.; Kovnir, Kirill; Shatruk, Michael] Florida State Univ, Dept Chem & Biochem, Tallahassee, FL 32306 USA. [Fabbris, Gilberto; Haskel, Daniel] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Fabbris, Gilberto] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Yaroslavtsev, Alexander A.; Menushenkov, Alexey P.] Natl Res Nucl Univ MEPhI, Moscow Engn Phys Inst, Moscow 115409, Russia. [Yaroslavtsev, Alexander A.] European XFEL GmbH, D-22761 Hamburg, Germany. [Cao, Huibo; Garlea, V. Ovidiu] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Chernikov, Roman V.] DESY Photon Sci, D-22603 Hamburg, Germany. [Thompson, Corey M.] Purdue Univ, Dept Chem, 560 Oval Dr, W Lafayette, IN 47907 USA. [Kovnir, Kirill] Univ Calif Davis, Dept Chem, One Shields Ave, Davis, CA 95616 USA. RP Shatruk, M (reprint author), Florida State Univ, Dept Chem & Biochem, Tallahassee, FL 32306 USA. EM shatruk@chem.fsu.edu RI Fabbris, Gilberto/F-3244-2011 OI Fabbris, Gilberto/0000-0001-8278-4985 FU National Science Foundation [DMR-1507233]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (DOE); U.S. DOE [DEAC02-06CH11357]; Russian Scientific Foundation [14-22-00098] FX This work was supported by the National Science Foundation (Award DMR-1507233 to M.S.). The work at the Oak Ridge National Laboratory was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (DOE). The use of the Advanced Photon Source at Argonne National Laboratory was supported by U.S. DOE under Contract No. DEAC02-06CH11357. A.P.M. and A.A.Y. thank the Russian Scientific Foundation (project 14-22-00098) for support. NR 35 TC 10 Z9 10 U1 15 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAR 2 PY 2016 VL 138 IS 8 BP 2724 EP 2731 DI 10.1021/jacs.5b12659 PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA DF6GK UT WOS:000371453700045 PM 26840063 ER PT J AU Malonzo, CD Shaker, SM Ren, LM Prinslow, SD Platero-Prats, AE Gallington, LC Borycz, J Thompson, AB Wang, TC Farha, OK Hupp, JT Lu, CC Chapman, KW Myers, JC Penn, RL Gagliardi, L Tsapatsis, M Stein, A AF Malonzo, Camille D. Shaker, Sammy M. Ren, Limin Prinslow, Steven D. Platero-Prats, Ana E. Gallington, Leighanne C. Borycz, Joshua Thompson, Anthony B. Wang, Timothy C. Farha, Omar K. Hupp, Joseph T. Lu, Connie C. Chapman, Karena W. Myers, Jason C. Penn, R. Lee Gagliardi, Laura Tsapatsis, Michael Stein, Andreas TI Thermal Stabilization of Metal-Organic Framework-Derived Single Site Catalytic Clusters through Nanocasting SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID ATOMIC LAYER DEPOSITION; HETEROGENEOUS CATALYSTS; RATIONAL DESIGN; THIN-FILM; STABILITY; PYRIDINE; OXIDES; DEHYDROGENATION; ISOMERIZATION; PALLADIUM AB Metal-organic frameworks (MOFs) provide convenient systems for organizing high concentrations of single catalytic sites derived from metallic or oxo-metallic nodes. However, high-temperature processes cause agglomeration of these nodes, so that the single-site character and catalytic activity are lost. In this work, we present a simple nanocasting approach to provide a thermally stable secondary scaffold for MOP-based catalytic single sites, preventing their aggregation even after exposure to air at 600 degrees C. We describe the nanocasting of NU-1000, a MOP with 3 nm channels and Lewis-acidic oxozirconium clusters, with silica. By condensing tetramethylorthosilicate within the NU-1000 pores via a vapor-phase HCl treatment, a silica layer is created on the inner walls of NU-1000. This silica layer provides anchoring sites for the oxozirconium clusters in NU-1000 after the organic linkers are removed at high temperatures. Differential pair distribution functions obtained from synchrotron X-ray scattering confirmed that isolated oxozirconium clusters are maintained in the heated nanocast materials. Pyridine adsorption experiments and a glucose isomerization reaction demonstrate that the clusters remain accessible to reagents and maintain their acidic character and catalytic activity even after the nanocast materials have been heated to 500-600 degrees C in air. Density functional theory calculations show a correlation between the Lewis acidity of the oxozirconium clusters and their catalytic activity. The ability to produce MOF-derived materials that retain their catalytic properties after exposure to high temperatures makes nanocasting a useful technique for obtaining single-site catalysts suitable for high-temperature reactions. C1 [Malonzo, Camille D.; Shaker, Sammy M.; Prinslow, Steven D.; Borycz, Joshua; Thompson, Anthony B.; Lu, Connie C.; Penn, R. Lee; Gagliardi, Laura; Stein, Andreas] Univ Minnesota, Dept Chem, 207 Pleasant St SE, Minneapolis, MN 55455 USA. [Ren, Limin; Tsapatsis, Michael] Univ Minnesota, Dept Chem Engn & Mat Sci, 421 Washington Ave SE, Minneapolis, MN 55455 USA. [Prinslow, Steven D.] Austin Coll, Dept Chem, 900 North Grand Ave, Sherman, TX 75090 USA. [Platero-Prats, Ana E.; Gallington, Leighanne C.; Chapman, Karena W.] Argonne Natl Lab, Xray Sci Div, Adv Photon Source, 9700 S Cass Ave, Argonne, IL 60439 USA. [Wang, Timothy C.; Farha, Omar K.; Hupp, Joseph T.] Northwestern Univ, Dept Chem & Chem & Biol Engn, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Farha, Omar K.] King Abdulaziz Univ, Fac Sci, Dept Chem, Jeddah 21413, Saudi Arabia. [Myers, Jason C.] Univ Minnesota, Coll Sci & Engn Characterizat Facil, 100 Union St SE, Minneapolis, MN 55455 USA. RP Stein, A (reprint author), Univ Minnesota, Dept Chem, 207 Pleasant St SE, Minneapolis, MN 55455 USA. EM a-stein@umn.edu RI Gallington, Leighanne/G-9341-2011; Lu , Connie/A-2281-2010; Platero-Prats, Ana Eva/B-2870-2017; Faculty of, Sciences, KAU/E-7305-2017 OI Gallington, Leighanne/0000-0002-0383-7522; Platero-Prats, Ana Eva/0000-0002-2248-2739; FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences [DE-SC-0012702]; NSF through MRSEC program; NSF through ERC program; NSF through MRI program; NSF through NNIN program; Catalysis Center for Energy Innovation, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0001004]; Ministry of Economy and Knowledge (Catalan Government) [BP-DGR 2014]; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357] FX This research was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences under Award DE-SC-0012702, except for the parts listed below. Parts of this work were carried out in the University of Minnesota Characterization Facility, which receives partial support from the NSF through the MRSEC, ERC, MRI and NNIN programs. The sugar isomerization work was supported as part of the Catalysis Center for Energy Innovation, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award DE-SC0001004. Work done at Argonne was performed using the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. A.E.P.P. acknowledges a Beatriu de Pinos fellowship (BP-DGR 2014) from the Ministry of Economy and Knowledge (Catalan Government). We thank Dr. Stephen Rudisill for obtaining SAED patterns. NR 60 TC 5 Z9 5 U1 45 U2 184 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAR 2 PY 2016 VL 138 IS 8 BP 2739 EP 2748 DI 10.1021/jacs.5b12688 PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA DF6GK UT WOS:000371453700047 PM 26848741 ER PT J AU Li, LS Jacobs, R Gao, P Gan, LY Wang, F Morgan, D Jin, S AF Li, Linsen Jacobs, Ryan Gao, Peng Gan, Liyang Wang, Feng Morgan, Dane Jin, Song TI Origins of Large Voltage Hysteresis in High-Energy-Density Metal Fluoride Lithium-Ion Battery Conversion Electrodes SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID RECHARGEABLE LI BATTERIES; HIGH-CAPACITY; X-RAY; IRON FLUORIDE; SPECTROSCOPY; CATHODES; STORAGE; NANOCOMPOSITES; CHALLENGES; TRANSPORT AB Metal fluorides and oxides can store multiple lithium ions through conversion chemistry to enable high-energy -density lithium-ion batteries. However, their practical applications have been hindered by an unusually large voltage hysteresis between charge and discharge voltage profiles and the consequent low-energy efficiency (<80%). The physical origins of such, hysteresis are rarely studied and poorly understood. Here we employ in situ X-ray absorption spectroscopy, transmission electron microscopy, density functional theory calculations, and galvanostatic intermittent titration technique to first correlate the voltage profile of iron fluoride (FeF3), a representative conversion electrode material, With evolution and spatial distribution of intermediate phases in the electrode: The results reveal that, contrary to conventional belief, the phase evolution in the electrode is symmetrical during discharge and charge. However, the spatial evolution of the electrochemically active phases, which is controlled by reaction kinetics, is different. We further propose that the voltage hysteresis in the FeF3 electrode is kinetic in nature. It is the result of ohmic voltage drop, reaction overpotential, and different spatial distributions of electrochemically active phases (i.e., compositional inliomogeneity). Therefore, the large hysteresis Can be expected to be mitigated by rational design and optimization of material microstructure and electrode architecture to improve the energy efficiency of lithium-ion batteries based on conversion chemistry. C1 [Li, Linsen; Gan, Liyang; Jin, Song] Univ Wisconsin, Dept Chem, Madison, WI 53705 USA. [Jacobs, Ryan; Morgan, Dane] Univ Wisconsin, Dept Mat Sci & Engn, Madison, WI 53706 USA. [Gao, Peng; Wang, Feng] Brookhaven Natl Lab, Sustainable Energy Technol Div, New York, NY 11973 USA. [Li, Linsen] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. [Gao, Peng] Peking Univ, Sch Phys, Beijing 100871, Peoples R China. RP Jin, S (reprint author), Univ Wisconsin, Dept Chem, Madison, WI 53705 USA.; Morgan, D (reprint author), Univ Wisconsin, Dept Mat Sci & Engn, Madison, WI 53706 USA. EM ddmorgan@wisc.edu; jin@chem.wisc.edu RI Jin, Song/B-4300-2008; Gao, Peng/B-4675-2012 FU NSF [DMR-1106184, DMR-1508558]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]; NSF Software Infrastructure for Sustained Innovation (SI2) [1148011]; Laboratory Directed Research and Development (LDRD) program at Brookhaven National Laboratory; Vilas Research Travel Awards FX This research is supported by NSF grant DMR-1106184 and DMR-1508558 for the synthesis and structural characterization of the materials, and a UW-Madison WEI Seed Grant and Research Corporation SciaLog Award for the electrochemical and theoretical studies. The in situ X-ray absorption spectroscopy experiments were performed at beamline X18A, National Synchrotron Light Source, Brookhaven National Laboratory, which are supported by the U.S. Department of Energy, Office of Basic Energy Sciences under contract no. DE-AC02-98CH10886. R.J. and D.M. were supported by the NSF Software Infrastructure for Sustained Innovation (SI2) award no. 1148011. P.G. and F.W. were supported by the Laboratory Directed Research and Development (LDRD) program at Brookhaven National Laboratory. L.L. also thanks Vilas Research Travel Awards for partially supporting the travel cost to the synchrotron facilities. NR 50 TC 10 Z9 10 U1 35 U2 126 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAR 2 PY 2016 VL 138 IS 8 BP 2838 EP 2848 DI 10.1021/jacs.6b00061 PG 11 WC Chemistry, Multidisciplinary SC Chemistry GA DF6GK UT WOS:000371453700059 PM 26847657 ER PT J AU Jungfleisch, MB Zhang, W Iacocca, E Sklenar, J Ding, J Jiang, W Zhang, S Pearson, JE Novosad, V Ketterson, JB Heinonen, O Hoffmann, A AF Jungfleisch, M. B. Zhang, W. Iacocca, E. Sklenar, J. Ding, J. Jiang, W. Zhang, S. Pearson, J. E. Novosad, V. Ketterson, J. B. Heinonen, O. Hoffmann, A. TI Dynamic response of an artificial square spin ice SO PHYSICAL REVIEW B LA English DT Article ID FRUSTRATION AB Magnetization dynamics in an artificial square spin-ice lattice made of Ni80Fe20 with magnetic field applied in the lattice plane is investigated by broadband ferromagnetic resonance spectroscopy. The experimentally observed dispersion shows a rich spectrum of modes corresponding to different magnetization states. These magnetization states are determined by exchange and dipolar interaction between individual islands, as is confirmed by a semianalytical model. In the low field regime below 400 Oe a hysteretic behavior in the mode spectrum is found. Micromagnetic simulations reveal that the origin of the observed spectra is due to the initialization of different magnetization states of individual nanomagnets. Our results indicate that it might be possible to determine the spin-ice state by resonance experiments and are a first step towards the understanding of artificial geometrically frustrated magnetic systems in the high-frequency regime. C1 [Jungfleisch, M. B.; Zhang, W.; Sklenar, J.; Ding, J.; Jiang, W.; Zhang, S.; Pearson, J. E.; Novosad, V.; Heinonen, O.; Hoffmann, A.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Iacocca, E.] Univ Colorado, Dept Appl Math, Boulder, CO 80309 USA. [Iacocca, E.] Chalmers, Dept Appl Phys, Div Condensed Matter Theory, S-41296 Gothenburg, Sweden. [Sklenar, J.; Ketterson, J. B.] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [Heinonen, O.] Northwestern Univ, Northwestern Argonne Inst Sci & Engn, Evanston, IL 60208 USA. RP Jungfleisch, MB (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM jungfleisch@anl.gov RI Jungfleisch, Matthias Benjamin/G-1069-2015; Jiang, Wanjun/E-6994-2011; DING, Junjia/K-2277-2013; Novosad, V /J-4843-2015; OI Jungfleisch, Matthias Benjamin/0000-0001-8204-3677; Jiang, Wanjun/0000-0003-0918-3862; DING, Junjia/0000-0002-9917-9156; Heinonen, Olle/0000-0002-3618-6092; Iacocca, Ezio/0000-0002-8870-5106 FU US Department of Energy, Office of Science, Materials Science and Engineering Division; DOE, Office of Science, Basic Energy Science [DE-AC02-06CH11357]; Swedish Research Council [637-2014-6863] FX We thank Vitali Metlushko and Ralu Divan for assistance with the electron beam lithography. The work at Argonne was supported by the US Department of Energy, Office of Science, Materials Science and Engineering Division. Lithography was carried out at the Center for Nanoscale Materials, an Office of Science user facility, which is supported by DOE, Office of Science, Basic Energy Science under Contract No. DE-AC02-06CH11357. E. Iacocca acknowledges support from the Swedish Research Council, Reg. No. 637-2014-6863. We gratefully acknowledge the computing resources provided on Blues, a high-performance computing cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory. NR 30 TC 6 Z9 6 U1 5 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 2 PY 2016 VL 93 IS 10 AR 100401 DI 10.1103/PhysRevB.93.100401 PG 5 WC Physics, Condensed Matter SC Physics GA DF5NT UT WOS:000371399500001 ER PT J AU Martins, ML Ignazzi, R Eckert, J Watts, B Kaneno, R Zambuzzi, WF Daemen, L Saeki, MJ Bordallo, HN AF Martins, Murillo L. Ignazzi, Rosanna Eckert, Juergen Watts, Benjamin Kaneno, Ramon Zambuzzi, Willian F. Daemen, Luke Saeki, Margarida J. Bordallo, Heloisa N. TI Restricted mobility of specific functional groups reduces anti-cancer drug activity in healthy cells SO SCIENTIFIC REPORTS LA English DT Article ID INELASTIC NEUTRON-SCATTERING; CANCER-CELLS; BREAST-CANCER; HYDROXYAPATITE NANOPARTICLES; IN-VIVO; DELIVERY-SYSTEM; LUNG-CANCER; PACLITAXEL; CHITOSAN; TAXOL AB The most common cancer treatments currently available are radio- and chemo-therapy. These therapies have, however, drawbacks, such as, the reduction in quality of life and the low efficiency of radiotherapy in cases of multiple metastases. To lessen these effects, we have encapsulated an anti-cancer drug into a biocompatible matrix. In-vitro assays indicate that this bio-nanocomposite is able to interact and cause morphological changes in cancer cells. Meanwhile, no alterations were observed in monocytes and fibroblasts, indicating that this system might carry the drug in living organisms with reduced clearance rate and toxicity. X-rays and neutrons were used to investigate the carrier structure, as well as to assess the drug mobility within the bio-nanocomposite. From these unique data we show that partial mobility restriction of active groups of the drug molecule suggests why this carrier design is potentially safer to healthy cells. C1 [Martins, Murillo L.; Ignazzi, Rosanna; Bordallo, Heloisa N.] Univ Copenhagen, Niels Bohr Inst, Blegdamsvej 17, DK-2100 Copenhagen, Denmark. [Martins, Murillo L.; Kaneno, Ramon; Zambuzzi, Willian F.; Saeki, Margarida J.] Univ Estadual Paulista, Inst Biociencias, BR-18618970 Botucatu, SP, Brazil. [Eckert, Juergen] Univ S Florida, Dept Chem, 4202 E Fowler Ave, Tampa, FL 33620 USA. [Eckert, Juergen; Daemen, Luke] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. [Watts, Benjamin] Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland. [Bordallo, Heloisa N.] European Spallat Source ESS AB, POB 176, SE-22100 Lund, Sweden. RP Bordallo, HN (reprint author), Univ Copenhagen, Niels Bohr Inst, Blegdamsvej 17, DK-2100 Copenhagen, Denmark.; Bordallo, HN (reprint author), European Spallat Source ESS AB, POB 176, SE-22100 Lund, Sweden. EM bordallo@nbi.ku.dk RI Bordallo, Heloisa/I-6836-2012 OI Bordallo, Heloisa/0000-0003-0750-0553 FU Department of Energy's Office of Basic Energy Sciences; DOE [DE-AC52-06NA25396]; German Minister fur Bildung und Forschung (BMBF) [05KS4WE1/6, 05KS7WE1]; FAPESP; CNPq; DANSCATT FX This work has benefited from the use of the Manuel Lujan, Jr. Neutron Scattering Center at Los Alamos National Laboratory and funding from the Department of Energy's Office of Basic Energy Sciences. Los Alamos National Laboratory (LANL) is operated by Los Alamos National Security LLC under DOE contract DE-AC52-06NA25396. MLM and RI thank the Swiss Light Source for beamtime at PolLux, which is financed by the German Minister fur Bildung und Forschung (BMBF) through contracts 05KS4WE1/6 and 05KS7WE1. The authors thank FAPESP, CNPq and DANSCATT for the financial support. JE would like to thank the Physics and Chemistry of Materials Group (T-1) at LANL for making computing resources available, and Dr. Jernej Stare for performing some calculations at the National Institute of Chemistry, Ljubljana, Slovenia. Dr. Walter Kalceff (UTS, Australia) is also gratefully acknowledged for critical review and discussions of this work. NR 54 TC 0 Z9 0 U1 6 U2 16 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 2 PY 2016 VL 6 AR 22478 DI 10.1038/srep22478 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DF2KQ UT WOS:000371172300001 PM 26932808 ER PT J AU Huang, YX Huang, L Wang, CZ Kramer, MJ Ho, KM AF Huang, Yuxiang Huang, Li Wang, C. Z. Kramer, M. J. Ho, K. M. TI Ab initio molecular dynamics simulations of short-range order in Zr50Cu45Al5 and Cu50Zr45Al5 metallic glasses SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE metallic glass; ab initio molecular dynamics; x-ray diffraction ID ZR-CU-AL; MECHANICAL-PROPERTIES; FORMING ABILITY; THERMAL-STABILITY; AMORPHOUS-ALLOYS; DENSITY; PACKING; MICROSTRUCTURE; FORMABILITY; PLASTICITY AB Comparative analysis between Zr-rich Zr50Cu45Al5 and Cu-rich Cu50Zr45Al5 metallic glasses (MGs) is extensively performed to locate the key structural motifs accounting for their difference of glass forming ability. Here we adopt ab initio molecular dynamics simulations to investigate the local atomic structures of Zr50Cu45Al5 and Cu50Zr45Al5 MGs. A high content of icosahedral-related (full and distorted) orders was found in both samples, while in the Zr-rich MG full icosahedrons < 0, 0, 12, 0 > is dominant, and in the Cu-rich one the distorted icosahedral orders, especially < 0, 2, 8, 2 > and < 0, 2, 8, 1 >, are prominent. And the < 0, 2, 8, 2 > polyhedra in Cu50Zr45Al5 MG mainly originate from Al-centered clusters, while the < 0, 0, 12, 0 > in Zr50Cu45Al5 derives from both Cu-centered clusters and Al-centered clusters. These difference may be ascribed to the atomic size difference and chemical property between Cu and Zr atoms. The relatively large size of Zr and large negative heat of mixing between Zr and Al atoms, enhancing the packing density and stability of metallic glass system, may be responsible for the higher glass forming ability of Zr50Cu45Al5. C1 [Huang, Yuxiang; Huang, Li] South Univ Sci & Technol, Dept Phys, Shenzhen 518055, Guangdong, Peoples R China. [Huang, Li; Wang, C. Z.; Kramer, M. J.; Ho, K. M.] US DOE, Ames Lab, Ames, IA 50011 USA. [Wang, C. Z.; Kramer, M. J.; Ho, K. M.] Iowa State Univ, Dept Phys, Ames, IA 50011 USA. RP Huang, L (reprint author), South Univ Sci & Technol, Dept Phys, Shenzhen 518055, Guangdong, Peoples R China.; Huang, L (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. EM huangl@sustc.edu.cn FU startup of South University of Science and Technology of China; NSFC [11404160]; US Department of Energy, Office of Basic Energy Sciences, Materials Science and Engineering Division [DE-AC02-06CH11357]; [DE-AC02-07CH11358] FX YX Huang and L Huang acknowledge the support by the startup of South University of Science and Technology of China and the NSFC under Grant No. 11404160. Work at Ames Laboratory (analysis, samples and HEXRD) was supported by the US Department of Energy, Office of Basic Energy Sciences, Materials Science and Engineering Division, synchrotron studies were performed at the Advanced Photon Source, Argonne National Laboratory, under Grant No. DE-AC02-06CH11357, a grant of computer time at the National Energy Research Supercomputing Center (NERSC) in Berkeley, under Contract No. DE-AC02-07CH11358. NR 38 TC 2 Z9 2 U1 9 U2 42 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAR 2 PY 2016 VL 28 IS 8 AR 085102 DI 10.1088/0953-8984/28/8/085102 PG 7 WC Physics, Condensed Matter SC Physics GA DC8OP UT WOS:000369479200007 PM 26828778 ER PT J AU Baltazar, LM Nakayasu, ES Sobreira, TJP Choi, H Casadevall, A Nimrichter, L Nosanchuk, JD AF Baltazar, Ludmila Matos Nakayasu, Ernesto S. Sobreira, Tiago J. P. Choi, Hyungwon Casadevall, Arturo Nimrichter, Leonardo Nosanchuk, Joshua D. TI Antibody Binding Alters the Characteristics and Contents of Extracellular Vesicles Released by Histoplasma capsulatum SO MSPHERE LA English DT Article DE H. capsulatum; Hsp60; monoclonal antibodies; vesicles ID CRYPTOCOCCUS-NEOFORMANS; GENE-EXPRESSION; CELL-WALL; PATHOGENESIS; MECHANISMS; TRANSPORT; VIRULENCE; PROTEINS; EXPORT AB Histoplasma capsulatum produces extracellular vesicles containing virulence-associated molecules capable of modulating host machinery, benefiting the pathogen. Treatment of H. capsulatum cells with monoclonal antibodies (MAbs) can change the outcome of infection in mice. We evaluated the sizes, enzymatic contents, and proteomic profiles of the vesicles released by fungal cells treated with either protective MAb 6B7 (IgG1) or nonprotective MAb 7B6 (IgG2b), both of which bind H. capsulatum heat shock protein 60 (Hsp60). Our results showed that treatment with either MAb was associated with changes in size and vesicle loading. MAb treatments reduced vesicle phosphatase and catalase activities compared to those of vesicles from untreated controls. We identified 1,125 proteins in vesicles, and 250 of these manifested differences in abundance relative to that of proteins in vesicles isolated from yeast cells exposed to Hsp60-binding MAbs, indicating that surface binding of fungal cells by MAbs modified protein loading in the vesicles. The abundance of upregulated proteins in vesicles upon MAb 7B6 treatment was 44.8% of the protein quantities in vesicles from fungal cells treated with MAb 6B7. Analysis of orthologous proteins previously identified in vesicles from other fungi showed that different ascomycete fungi have similar proteins in their extracellular milieu, many of which are associated with virulence. Our results demonstrate that antibody binding can modulate fungal cell responses, resulting in differential loading of vesicles, which could alter fungal cell susceptibility to host defenses. This finding provides additional evidence that antibody binding modulates microbial physiology and suggests a new function for specific immunoglobulins through alterations of fungal secretion. IMPORTANCE Diverse fungal species release extracellular vesicles, indicating that this is a common pathway for the delivery of molecules to the extracellular space. However, there has been no study reporting the impact of antibody binding to the fungal cell on extracellular vesicle release. In the present work, we observed that treatment of H. capsulatum cells with Hsp60-binding MAbs significantly changed the size and cargo of extracellular vesicles, as well as the enzymatic activity of certain virulence factors, such as laccase and phosphatase. Furthermore, this finding demonstrates that antibody binding can directly impact protein loading in vesicles and fungal metabolism. Hence, this work presents a new role for antibodies in the modification of fungal physiology. C1 [Baltazar, Ludmila Matos; Nosanchuk, Joshua D.] Albert Einstein Coll Med, Dept Microbiol & Immunol, Bronx, NY 10467 USA. [Baltazar, Ludmila Matos; Nosanchuk, Joshua D.] Albert Einstein Coll Med, Dept Med, Div Infect Dis, Bronx, NY 10467 USA. [Nakayasu, Ernesto S.] Pacific Northwest Natl Lab, Div Biol Sci, Richland, WA USA. [Nakayasu, Ernesto S.; Sobreira, Tiago J. P.] Purdue Univ, Bindley Biosci Ctr, W Lafayette, IN 47907 USA. [Choi, Hyungwon] Natl Univ Singapore, Saw Swee Hock Sch Publ Hlth, Singapore, Singapore. [Casadevall, Arturo] Johns Hopkins Univ, Dept Mol Microbiol & Immunol, Johns Hopkins Bloomberg Sch Publ Hlth, Baltimore, MD USA. [Nimrichter, Leonardo] Univ Fed Rio de Janeiro, Inst Microbiol Paulo de Goes, Rio De Janeiro, Brazil. [Baltazar, Ludmila Matos] Univ Fed Minas Gerais, Belo Horizonte, MG, Brazil. RP Baltazar, LM (reprint author), Albert Einstein Coll Med, Dept Microbiol & Immunol, Bronx, NY 10467 USA.; Baltazar, LM (reprint author), Albert Einstein Coll Med, Dept Med, Div Infect Dis, Bronx, NY 10467 USA. EM ludmilabaltazar@gmail.com FU HHS \ National Institutes of Health (NIH) [3R37AI033142-21S1, R21 AI124797-01]; Coordenacao de Aperfeicoamento de Pessoal de Nivel Superior (CAPES) [3226-13-1] FX This work, including the efforts of Arturo Casadevall, was funded by HHS vertical bar National Institutes of Health (NIH) (3R37AI033142-21S1). This work, including the efforts of Joshua D. Nosanchuk, was funded by HHS vertical bar National Institutes of Health (NIH) (3R37AI033142-21S1). This work, including the efforts of Ernesto S. Nakayasu, was funded by HHS vertical bar National Institutes of Health (NIH) (R21 AI124797-01). This work, including the efforts of Joshua D. Nosanchuk, was funded by HHS vertical bar National Institutes of Health (NIH) (R21 AI124797-01). This work, including the efforts of Ludmila Matos Baltazar, was funded by Coordenacao de Aperfeicoamento de Pessoal de Nivel Superior (CAPES) (3226-13-1). NR 37 TC 1 Z9 1 U1 0 U2 0 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2379-5042 J9 MSPHERE JI mSphere PD MAR-APR PY 2016 VL 1 IS 2 AR UNSP e00085-15 DI 10.1128/mSphere.00085-15 PG 17 WC Microbiology SC Microbiology GA EI6DH UT WOS:000392584700025 ER PT J AU Huan, TD Mannodi-Kanakkithodi, A Kim, C Sharma, V Pilania, G Ramprasad, R AF Tran Doan Huan Mannodi-Kanakkithodi, Arun Kim, Chiho Sharma, Vinit Pilania, Ghanshyam Ramprasad, Rampi TI A polymer dataset for accelerated property prediction and design SO SCIENTIFIC DATA LA English DT Article ID FUNCTIONAL PERTURBATION-THEORY; TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; CRYSTAL-STRUCTURE; X-RAY; RATIONAL DESIGN; FORCE-FIELD; DIELECTRIC-PROPERTIES; POLYPROPYLENE; DIFFRACTION AB Emerging computation-and data-driven approaches are particularly useful for rationally designing materials with targeted properties. Generally, these approaches rely on identifying structure-property relationships by learning from a dataset of sufficiently large number of relevant materials. The learned information can then be used to predict the properties of materials not already in the dataset, thus accelerating the materials design. Herein, we develop a dataset of 1,073 polymers and related materials and make it available at http://khazana.uconn.edu/. This dataset is uniformly prepared using first-principles calculations with structures obtained either from other sources or by using structure search methods. Because the immediate target of this work is to assist the design of high dielectric constant polymers, it is initially designed to include the optimized structures, atomization energies, band gaps, and dielectric constants. It will be progressively expanded by accumulating new materials and including additional properties calculated for the optimized structures provided. C1 [Tran Doan Huan; Mannodi-Kanakkithodi, Arun; Kim, Chiho; Sharma, Vinit; Ramprasad, Rampi] Univ Connecticut, Inst Mat Sci, 97 North Eagleville Rd,Unit 3136, Storrs, CT 06269 USA. [Pilania, Ghanshyam] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. [Sharma, Vinit] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Ramprasad, R (reprint author), Univ Connecticut, Inst Mat Sci, 97 North Eagleville Rd,Unit 3136, Storrs, CT 06269 USA. EM rampi.ramprasad@uconn.edu OI Tran, Huan/0000-0002-8093-9426; Pilania, Ghanshyam/0000-0003-4460-1572 FU Multidisciplinary University Research Initiative (MURI) grant from the Office of Naval Research [N00014-10-1-0944]; U.S. Department of Energy through the LANL/LDRD Program's Director's postdoctoral fellowship FX The present work was supported by Multidisciplinary University Research Initiative (MURI) grant from the Office of Naval Research under Award No. N00014-10-1-0944. G.P. acknowledges the support provided by U.S. Department of Energy through the LANL/LDRD Program's Director's postdoctoral fellowship. A.M.K. would like to thank Turab Lookman at Los Alamos National Laboratory for providing access to computational resources. Computational work was made possible through XSEDE computational resource allocation number TG-DMR080058N59. NR 84 TC 4 Z9 4 U1 4 U2 4 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2052-4463 J9 SCI DATA JI Sci. Data PD MAR 1 PY 2016 VL 3 AR UNSP 160012 DI 10.1038/sdata.2016.12 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA EF3GR UT WOS:000390213300001 ER PT J AU Zhou, J AF Zhou, Jia TI Novel hetero-bilayered materials for photovoltaics SO APPLIED MATERIALS TODAY LA English DT Article DE GaS; MoSe2; Density functional theory; Two dimensional hetero-structures; Optical absorbance ID HEXAGONAL BORON-NITRIDE; LAYERED MATERIALS; BAND-GAPS; GRAPHENE; NANOSHEETS; GAS; HETEROBILAYERS; ELECTRONICS; POINTS; FILMS AB The recently synthesized GaS and MoSe2 nanosheets have been used as appropriate substrates for other layered materials, e.g. silicene/GaS heterosheets akin to graphene/BN systems. Here, we have performed a comprehensive first-principles study of the electronic and optical properties of two-dimensional (2D) GaS/MoSe2 hetero-bilayers based on density functional theory (DFT). We found almost all proposed GaS/MoSe2 hetero-bilayers in the current study have an indirect band gap from the F point to the K point, except for one with a direct band gap at the K point. Tunable band gaps GaS/MoSe2 hetero-bilayers can be controlled by strain modulation. State-of-the-art GW-Bethe-Salpeter method, accounting for electron electron and electron-hole interactions, has been employed to compute accurate absorbance spectra for layered materials. Compared with its composing GaS and MoSe2 monolayers, GaS/MoSe2 heterobilayers show superior behavior on optical absorbance, indicating a stronger visible-light absorption and applications in solar energy harvesting. We foresee that the novel GaS/MoSe2 hetero-bilayers would stimulate the fabrication of materials with unprecedented optical and physico-chemical properties that may apply in nanodevices and photovoltaic cells. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Zhou, Jia] Harbin Inst Technol, Dept Chem, Harbin 150001, Peoples R China. [Zhou, Jia] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Bethel Valley Rd, Oak Ridge, TN 37831 USA. RP Zhou, J (reprint author), Harbin Inst Technol, Dept Chem, Harbin 150001, Peoples R China. EM jiazhou@hit.edu.cn FU Fundamental Research Funds for the Central Universities of China [AUGA5710013115]; Office of Science of the U.S. Department of Energy [DE-AC05-00OR22750, DE-AC02-05CH11231]; Center for Nanophase Materials Sciences - Scientific User Facilities Division, U.S. Department of Energy at ORNL FX This research is supported by the Fundamental Research Funds for the Central Universities of China (Grant No. AUGA5710013115). This work used computational resources of the Oak Ridge Leadership Computing Facility at Oak Ridge National laboratory and of the National Energy Research Scientific Computing Center, which are supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22750 and DE-AC02-05CH11231, respectively. We acknowledge the support from the Center for Nanophase Materials Sciences, which is sponsored at ORNL by the Scientific User Facilities Division, U.S. Department of Energy. The author also thanks Dr. Jingsong Huang (ORNL, US) and Prof. Xiaoming Cao (ECUST, China) for the assistance on the computations. NR 54 TC 7 Z9 7 U1 6 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2352-9407 J9 APPL MATER TODAY JI Appl. Mater. Today PD MAR PY 2016 VL 2 BP 24 EP 31 DI 10.1016/j.apmt.2015.12.001 PG 8 WC Materials Science, Multidisciplinary SC Materials Science GA EC9LF UT WOS:000388465400004 ER PT J AU Fitzsimmons, J Nayak, T Cutler, C Atcher, R AF Fitzsimmons, Jonathan Nayak, Tapan Cutler, Cathy Atcher, Robert TI Synthesis and Preliminary Biological Evaluations of Fluorescent or (149)Promethium Labeled Trastuzumab-Polyethylenimine SO BIOMEDICINES LA English DT Article DE Promethium-149; Trastuzumab; polyethylenimine; radiotherapy; targeted therapy; Actinium-225 ID HUMAN-BREAST-CANCER; GENE DELIVERY; HERCEPTIN FAB; ANTIBODY; AC-225; HER2; RADIOTHERAPY; EXPRESSION; HER-2/NEU; TUMORS AB Background: Radioimmunotherapy utilize a targeting antibody coupled to a therapeutic isotope to target and treat a tumor or disease. In this study we examine the synthesis and cell binding of a polymer scaffold containing a radiotherapeutic isotope and a targeting antibody. Methods: The multistep synthesis of a fluorescent or (149)Promethium-labeled Trastuzumab-polyethyleneimine (PEI), Trastuzumab, or PEI is described. In vitro uptake, internalization and/or the binding affinity to the Her2/neu expressing human breast adenocarcinoma SKBr3 cells was investigated with the labeled compounds. Results: Fluorescent-labeled Trastuzumab-PEI was internalized more into cells at 2 and 18 h than fluorescent-labeled Trastuzumab or PEI. The fluorescent-labeled Trastuzumab was concentrated on the cell surface at 2 and 18 h and the labeled PEI had minimal uptake. DOTA-PEI was prepared and contained an average of 16 chelates per PEI; the compound was radio-labeled with (149)Promethium and conjugated to Trastuzumab. The purified Pm-149-DOTA-PEI-Trastuzumab had a radiochemical purity of 96.7% and a specific activity of 0.118 TBq/g. The compound demonstrated a dissociation constant for the Her2/neu receptor of 20.30 +/- 6.91 nM. Conclusion: The results indicate the DOTA-PEI-Trastuzumab compound has potential as a targeted therapeutic carrier, and future in vivo studies should be performed. C1 [Fitzsimmons, Jonathan; Atcher, Robert] Los Alamos Natl Lab, Chem Life & Earth Sci Directorate, Los Alamos, NM 87545 USA. [Nayak, Tapan] Univ New Mexico, Hlth Sci Ctr, Sch Med, Dept Cell Biol & Physiol, Albuquerque, NM 87131 USA. [Nayak, Tapan; Atcher, Robert] Univ New Mexico, Hlth Sci Ctr, Coll Pharm, Radiopharmaceut Sci Program, Albuquerque, NM 87131 USA. [Cutler, Cathy] Univ Missouri Columbia, MURR, Columbia, MO 65211 USA. [Fitzsimmons, Jonathan; Cutler, Cathy] Brookhaven Natl Lab, Bldg 801, Upton, NY 11973 USA. [Nayak, Tapan] F Hoffmann La Roche, CH-4070 Basel, Switzerland. RP Fitzsimmons, J (reprint author), Los Alamos Natl Lab, Chem Life & Earth Sci Directorate, Los Alamos, NM 87545 USA. EM jfitzsimmons@bnl.gov; tapann@gmail.com; ccutler@bnl.gov; ratcher@lanl.gov OI Atcher, Robert/0000-0003-4656-2247 NR 31 TC 0 Z9 0 U1 1 U2 1 PU MDPI AG PI BASEL PA ST ALBAN-ANLAGE 66, CH-4052 BASEL, SWITZERLAND SN 2227-9059 J9 BIOMEDICINES JI Biomedicines PD MAR PY 2016 VL 4 IS 1 AR 1 DI 10.3390/biomedicines4010001 PG 11 WC Pharmacology & Pharmacy SC Pharmacology & Pharmacy GA DZ2GL UT WOS:000385660200001 ER PT J AU Francis, S AF Francis, Sybil TI Big Science: Ernest Lawrence, the Cyclotron, and the Birth of the Military-Industrial Complex SO ISSUES IN SCIENCE AND TECHNOLOGY LA English DT Book Review C1 [Francis, Sybil] Arizona State Univ, Sch Future Innovat Soc, Tempe, AZ 85287 USA. [Francis, Sybil] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Francis, S (reprint author), Arizona State Univ, Sch Future Innovat Soc, Tempe, AZ 85287 USA.; Francis, S (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. NR 1 TC 0 Z9 0 U1 2 U2 2 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0748-5492 EI 1938-1557 J9 ISSUES SCI TECHNOL JI Issues Sci. Technol. PD SPR PY 2016 VL 32 IS 3 BP 94 EP 95 PG 2 WC Engineering, Multidisciplinary; Engineering, Industrial; Multidisciplinary Sciences; Social Issues SC Engineering; Science & Technology - Other Topics; Social Issues GA DX9IM UT WOS:000384706800036 ER PT J AU Ghim, YS Won, SR Choi, Y Chang, YS Jin, HC Kim, YP Kang, CH AF Ghim, Young Sung Won, Soo Ran Choi, Yongjoo Chang, Young-Soo Jin, Hyoun Cher Kim, Yong Pyo Kang, Chang-Hee TI Concentration Variations in Primary and Secondary Particulate Matter near a Major Road in Korea SO ASIAN JOURNAL OF ATMOSPHERIC ENVIRONMENT LA English DT Article DE Vehicle emissions; Biomass burning; Open burning; Fugitive dust; Secondary formation ID ULTRAFINE PARTICLES; HIGHWAY AB Particle-phase concentrations were measured at 10, 80, and 200 m from the roadside of a national highway near Seoul in January and May 2008. The high-way has two lanes each way, with an average hourly traffic volume of 1,070 vehicles. In January 2008, PM10 concentrations decreased from 10 to 80 m but increased at 200 m. Black carbon (BC) decreased only slightly with distance due to the influence of biomass burning and open burning from the surrounding areas. In May 2008, the effect of secondary formation on both PM10 and PM2.5 was significant due to high temperatures compared with January. Because on-road emissions had little effect on secondary formation for a short time, variations in PM10 concentrations became smaller, and PM2.5 concentrations increased with distance. The effects of fugitive dust on PM concentrations were greater in May than in January when the mean temperature was below freezing. In the composition variations, the amounts of primary ions, organic carbon (OC), and BC were larger in January, while those of secondary ions and others were larger in PM10, as well as PM2.5 in May. C1 [Ghim, Young Sung; Won, Soo Ran; Choi, Yongjoo] Hankuk Univ Foreign Studies, Dept Environm Sci, Yongin 17035, Gyeonggi, South Korea. [Chang, Young-Soo] Argonne Natl Lab, Div Environm Sci, 9700 South Cass Ave, Argonne, IL 60439 USA. [Jin, Hyoun Cher] Korea Inst Sci & Technol, Ctr Environm Hlth & Welf Res, Seoul 02792, South Korea. [Kim, Yong Pyo] Ewha Womans Univ, Dept Environm Sci & Engn, Seoul 03760, South Korea. [Kang, Chang-Hee] Jeju Natl Univ, Dept Chem, Jeju 63243, Jeju, South Korea. [Won, Soo Ran] Natl Inst Environm Res, Indoor Environm & Noise Res Div, Inchon 22689, South Korea. RP Ghim, YS (reprint author), Hankuk Univ Foreign Studies, Dept Environm Sci, Yongin 17035, Gyeonggi, South Korea. EM ysghim@hufs.ac.kr NR 21 TC 0 Z9 0 U1 1 U2 1 PU JAPAN SOC ATMOSPHERIC ENVIRONMENT PI SEOUL PA JAPAN SOC ATMOSPHERIC ENVIRONMENT, SEOUL, 00000, SOUTH KOREA SN 1976-6912 EI 2287-1160 J9 ASIAN J ATMOS ENVIRO JI Asian J. Atmos. Environ. PD MAR PY 2016 VL 10 IS 1 BP 32 EP 41 DI 10.5572/ajae.2016.10.1.032 PG 10 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DV5JT UT WOS:000382964000004 ER PT J AU Finnell, J AF Finnell, Joshua TI The Grand Tour: The Life and Music of George Jones SO LIBRARY JOURNAL LA English DT Book Review C1 [Finnell, Joshua] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Finnell, J (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. NR 1 TC 0 Z9 0 U1 0 U2 0 PU REED BUSINESS INFORMATION PI NEW YORK PA 360 PARK AVENUE SOUTH, NEW YORK, NY 10010 USA SN 0363-0277 J9 LIBR J JI Libr. J. PD MAR 1 PY 2016 VL 141 IS 4 BP 100 EP 101 PG 2 WC Information Science & Library Science SC Information Science & Library Science GA DF1NB UT WOS:000371105400124 ER PT J AU Le Pape, Y Giorla, A Sanahuja, J AF Le Pape, Yann Giorla, Alain Sanahuja, Julien TI Combined Effects of Temperature and Irradiation on Concrete Damage SO JOURNAL OF ADVANCED CONCRETE TECHNOLOGY LA English DT Article ID ALKALI-SILICA REACTION; NUCLEAR-POWER-PLANTS; THERMAL-EXPANSION; PROPERTY CHANGES; VITREOUS SILICA; FAST-NEUTRONS; CEMENT PASTE; QUARTZ; KINETICS; STRESS AB Aggregate radiation-induced volumetric expansion (RIVE) is a predominant mechanism in the formation of mechanical damage in the hardened cement paste (hcp) of irradiated concrete under fast-neutron flux (Giorla et al. 2015). Among the operating conditions difference between test reactors and light water reactors (LWRs), the difference of irradiation flux and temperature is significant. While a temperature increase is quite generally associated with a direct, or indirect (e.g., by dehydration) loss of mechanical properties (Maruyama et al. 2014), it causes a partial annealing of irradiation amorphization of alpha-quartz, hence, reducing RIVE rate. Based on data collected by Bykov et al. (1981), an incremental RIVE model coupling neutron fluence and temperature is developed. The elastic properties and coefficient of thermal expansion (CTE) of irradiated polycrystalline quartz are interpreted through analytical homogenization of experimental data on irradiated alpha-quartz published by Mayer and Lecomte (1960). The proposed model, implemented in the meso-scale simulation code AMIE, is compared to experimental data obtained on ordinary concrete made of quartz/quartzite aggregate (Dubrovskii et al. 1967). Substantial discrepancy, in terms of damage and volumetric expansion developments, is found when comparing irradiation scenarios assuming constant flux and temperature, as opposed to more realistic test reactor operation conditions. C1 [Le Pape, Yann; Giorla, Alain] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Sanahuja, Julien] EDF Lab, F-77818 Moret Sur Loing, France. RP Le Pape, Y (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM lepapeym@ornl.gov FU U.S. Department of Energy (DOE) Light Water Reactor Sustainability Program; U.S. Department of Energy [DE-AC05-00OR22725] FX This research is sponsored by the U.S. Department of Energy (DOE) Light Water Reactor Sustainability Program. This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan, (http://energy.gov/downloads/doe-public-access-plan). NR 59 TC 3 Z9 3 U1 5 U2 5 PU JAPAN CONCRETE INST PI CHIYODA-KU PA SOGO HANZOMON BLDG 12F, NO 7, KOJIMACHI 1-CHOME, CHIYODA-KU, TOKYO 102-0083, JAPAN SN 1346-8014 EI 1347-3913 J9 J ADV CONCR TECHNOL JI J. Adv. Concr. Technol. PD MAR PY 2016 VL 14 IS 3 BP 70 EP 86 DI 10.3151/jact.14.70 PG 17 WC Construction & Building Technology; Engineering, Civil; Materials Science, Multidisciplinary SC Construction & Building Technology; Engineering; Materials Science GA DT4TD UT WOS:000381473000002 ER PT J AU Hong, JM Lambson, B Dhuey, S Bokor, J AF Hong, Jeongmin Lambson, Brian Dhuey, Scott Bokor, Jeffrey TI Experimental test of Landauer's principle in single-bit operations on nanomagnetic memory bits SO SCIENCE ADVANCES LA English DT Article ID THERMODYNAMICS; COMPUTATION; LOGIC AB Minimizing energy dissipation has emerged as the key challenge in continuing to scale the performance of digital computers. The question of whether there exists a fundamental lower limit to the energy required for digital operations is therefore of great interest. A well-known theoretical result put forward by Landauer states that any irreversible single-bit operation on a physical memory element in contact with a heat bath at a temperature T requires at least k(B)T ln(2) of heat be dissipated from the memory into the environment, where k(B) is the Boltzmann constant. We report an experimental investigation of the intrinsic energy loss of an adiabatic single-bit reset operation using nanoscale magnetic memory bits, by far the most ubiquitous digital storage technology in use today. Through sensitive, high-precision magnetometry measurements, we observed that the amount of dissipated energy in this process is consistent (within 2 SDs of experimental uncertainty) with the Landauer limit. This result reinforces the connection between "information thermodynamics" and physical systems and also provides a foundation for the development of practical information processing technologies that approach the fundamental limit of energy dissipation. The significance of the result includes insightful direction for future development of information technology. C1 [Hong, Jeongmin; Bokor, Jeffrey] Univ Calif Berkeley, Elect Engn & Comp Sci, Berkeley, CA 94720 USA. [Lambson, Brian] Haynes & Boone LLP, 525 Univ Ave, Palo Alto, CA 94301 USA. [Dhuey, Scott] Lawrence Berkeley Natl Lab, Mol Foundry, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Bokor, J (reprint author), Univ Calif Berkeley, Elect Engn & Comp Sci, Berkeley, CA 94720 USA. EM jbokor@eecs.berkeley.edu RI Bokor, Jeffrey/A-2683-2011 NR 16 TC 6 Z9 6 U1 2 U2 2 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 2375-2548 J9 SCI ADV JI Sci. Adv. PD MAR PY 2016 VL 2 IS 3 AR e1501492 DI 10.1126/sciadv.1501492 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DR0TQ UT WOS:000379620200030 PM 26998519 ER PT J AU Martinez, U Dumont, JH Holby, EF Artyushkova, K Purdy, GM Singh, A Mack, NH Atanassov, P Cullen, DA More, KL Chhowalla, M Zelenay, P Dattelbaum, AM Mohite, AD Gupta, G AF Martinez, Ulises Dumont, Joseph H. Holby, Edward F. Artyushkova, Kateryna Purdy, Geraldine M. Singh, Akhilesh Mack, Nathan H. Atanassov, Plamen Cullen, David A. More, Karren L. Chhowalla, Manish Zelenay, Piotr Dattelbaum, Andrew M. Mohite, Aditya D. Gupta, Gautam TI Critical role of intercalated water for electrocatalytically active nitrogen-doped graphitic systems SO SCIENCE ADVANCES LA English DT Article ID ELECTROCHEMICAL ENERGY-CONVERSION; GRAPHENE OXIDE; FUEL-CELLS; INITIAL CONFIGURATIONS; MOLECULAR-DYNAMICS; CATALYSTS; CARBON; MEMBRANE; STORAGE; IRON AB Graphitic materials are essential in energy conversion and storage because of their excellent chemical and electrical properties. The strategy for obtaining functional graphitic materials involves graphite oxidation and subsequent dissolution in aqueous media, forming graphene-oxide nanosheets (GNs). Restacked GNs contain substantial intercalated water that can react with heteroatom dopants or the graphene lattice during reduction. We demonstrate that removal of intercalated water using simple solvent treatments causes significant structural reorganization, substantially affecting the oxygen reduction reaction (ORR) activity and stability of nitrogen-doped graphitic systems. Amid contrasting reports describing the ORR activity of GN- based catalysts in alkaline electrolytes, we demonstrate superior activity in an acidic electrolyte with an onset potential of similar to 0.9 V, a half-wave potential (E-1/2) of 0.71 V, and a selectivity for four-electron reduction of >95%. Further, durability testing showed E-1/2 retention >95% in N-2- and O-2- saturated solutions after 2000 cycles, demonstrating the highest ORR activity and stability reported to date for GN- based electrocatalysts in acidic media. C1 [Martinez, Ulises; Dumont, Joseph H.; Purdy, Geraldine M.; Singh, Akhilesh; Zelenay, Piotr; Dattelbaum, Andrew M.; Mohite, Aditya D.; Gupta, Gautam] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. [Dumont, Joseph H.; Artyushkova, Kateryna; Atanassov, Plamen] Univ New Mexico, Dept Chem & Biol Engn, Albuquerque, NM 87131 USA. [Holby, Edward F.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. [Mack, Nathan H.] Los Alamos Natl Lab, Chem Div, Los Alamos, NM 87545 USA. [Cullen, David A.; More, Karren L.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Chhowalla, Manish] Rutgers State Univ, Sci & Engn, 607 Taylor Rd, Piscataway, NJ 08854 USA. RP Gupta, G (reprint author), Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA.; Chhowalla, M (reprint author), Rutgers State Univ, Sci & Engn, 607 Taylor Rd, Piscataway, NJ 08854 USA. EM manish1@rci.rutgers.edu; gautam@lanl.gov RI Cullen, David/A-2918-2015 OI Cullen, David/0000-0002-2593-7866 NR 38 TC 5 Z9 5 U1 14 U2 16 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 2375-2548 J9 SCI ADV JI Sci. Adv. PD MAR PY 2016 VL 2 IS 3 AR e1501178 DI 10.1126/sciadv.1501178 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DR0TQ UT WOS:000379620200009 PM 27034981 ER PT J AU Gao, YF AF Gao, Yanfei TI Deformation fields near a steady fatigue crack with anisotropic plasticity SO EXTREME MECHANICS LETTERS LA English DT Article DE Fatigue; Cohesive interface simulations; Anisotropic plasticity ID COHESIVE ZONE MODEL; BRITTLE MATERIALS; FAR-FIELDS; GROWTH; FRACTURE; SIMULATIONS; NUCLEATION; EXTRACTION; PROJECTION; BEHAVIOR AB In this work, from finite element simulations based on an irreversible, hysteretic cohesive interface model, a steady fatigue crack can be realized if the crack extension exceeds about twice the plastic zone size, and both the crack increment per loading cycle and the crack bridging zone size are smaller than the plastic zone size. The corresponding deformation fields develop a plastic wake behind the crack tip and a compressive residual stress field ahead of the crack tip. In addition, the Hill's plasticity model is used to study the role of plastic anisotropy on the retardation of fatigue crack growth and the elastic strain fields. It is found that for Mode-I cyclic loading, an enhanced yield stress in directions that are inclined from the crack plane will lead to slower crack growth rate, but this retardation is insignificant for typical degrees of plastic anisotropy. These results provide key inputs for future comparisons to neutron and synchrotron diffraction measurements that provide full-field lattice strain mapping near fracture and fatigue crack tips, especially in textured materials such as wrought or rolled Mg alloys. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Gao, Yanfei] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Gao, Yanfei] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Gao, YF (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. EM ygao7@utk.edu RI Gao, Yanfei/F-9034-2010 OI Gao, Yanfei/0000-0003-2082-857X NR 23 TC 1 Z9 1 U1 2 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2352-4316 J9 EXTREME MECH LETT JI EXTREME MECH. LETT. PD MAR PY 2016 VL 6 BP 45 EP 51 DI 10.1016/j.eml.2015.11.006 PG 7 WC Engineering, Mechanical SC Engineering GA DQ5OH UT WOS:000379254200006 ER PT J AU Shepherd, HJ Tonge, G Hatcher, LE Bryant, MJ Knichal, JV Raithby, PR Halcrow, MA Kulmaczewski, R Gagnon, KJ Teat, SJ AF Shepherd, Helena J. Tonge, George Hatcher, Lauren E. Bryant, Mathew J. Knichal, Jane V. Raithby, Paul R. Halcrow, Malcolm A. Kulmaczewski, Rafal Gagnon, Kevin J. Teat, Simon J. TI A High Pressure Investigation of the Order-Disorder Phase Transition and Accompanying Spin Crossover in [FeL1(2)](ClO4)(2) (L1 = 2,6-bis{3-methylpyrazol-1-yl}-pyrazine) SO MAGNETOCHEMISTRY LA English DT Article DE spin-crossover; molecular materials; high pressure; order-disorder phenomena ID SYSTEMS; POLYMORPHISM AB A high pressure single crystal X-ray diffraction and Raman spectroscopy study has revealed a similar mechanism for both thermal and pressure-induced spin crossover in [FeL1(2)](ClO4)(2) (L1 = 2,6-bisI3-methylpyrazol-1-yll-pyrazine) and the concomitant anion order-disorder transition. C1 [Shepherd, Helena J.; Tonge, George] Univ Kent, Sch Phys Sci, Canterbury CT2 7NH, Kent, England. [Hatcher, Lauren E.; Bryant, Mathew J.; Knichal, Jane V.; Raithby, Paul R.] Univ Bath, Dept Chem, Claverton Down, Bath BA2 7AY, Avon, England. [Halcrow, Malcolm A.; Kulmaczewski, Rafal] Univ Leeds, Sch Chem, Woodhouse Lane, Leeds LS2 9JT, W Yorkshire, England. [Gagnon, Kevin J.; Teat, Simon J.] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Shepherd, HJ (reprint author), Univ Kent, Sch Phys Sci, Canterbury CT2 7NH, Kent, England. EM h.j.shepherd@kent.ac.uk; gt88@kent.ac.uk; l.e.hatcher@bath.ac.uk; m.bryant@bath.ac.uk; j.v.knichal@bath.ac.uk; p.r.raithby@bath.ac.uk; m.a.halcrow@leeds.ac.uk; r.kulmaczewski@leeds.ac.uk; kjgagnon@lbl.gov; sjteat@lbl.gov RI Shepherd, Helena/M-4621-2015; Bryant, Mathew/J-2307-2016; OI Shepherd, Helena/0000-0003-0832-4475; Bryant, Mathew/0000-0001-8714-9761; Halcrow, Malcolm/0000-0001-7491-9034; Kulmaczewski, Rafal/0000-0002-3855-4530; Raithby, Paul/0000-0002-2944-0662 NR 26 TC 1 Z9 1 U1 4 U2 7 PU MDPI AG PI BASEL PA POSTFACH, CH-4005 BASEL, SWITZERLAND SN 2312-7481 J9 MAGNETOCHEMISTRY JI Magnetochemistry PD MAR PY 2016 VL 2 IS 1 AR 9 DI 10.3390/magnetochemistry2010009 PG 9 WC Chemistry, Physical SC Chemistry GA DQ4ZJ UT WOS:000379213400009 ER PT J AU O'Briant, SA Gupta, SB Vasu, SS AF O'Briant, Steven A. Gupta, Sreenath B. Vasu, Subith S. TI Review: laser ignition for aerospace propulsion SO PROPULSION AND POWER RESEARCH LA English DT Review DE Laser ignition; Ignition limit; Scramjet; Gas turbines; Rocket; Plasma ignition; Propulsion ID PLASMA-ASSISTED IGNITION; INDUCED SPARK-IGNITION; SOLID-PROPELLANTS; COMBUSTION; FUEL; FLAMES; SCRAMJETS; ABLATION; PARTICLES; INJECTOR AB Renewed interest in the use of high-speed ramjets and scramjets and more efficient lean burning engines has led to many subsequent developments in the field of laser ignition for aerospace use and application. Demands for newer, more advanced forms of ignition, are increasing as individuals strive to meet regulations that seek to reduce the level of pollutants in the atmosphere, such as CHx, NOx, and SO2. Many aviation gas turbine manufacturers are interested in increasing combustion efficiency in engines, all the while reducing the aforementioned pollutants. There is also a desire for a new generation of aircraft and spacecraft, utilizing technologies such as scramjet propulsion, which will never realize their fullest potential without the use of advanced ignition processes. These scenarios are all limited by the use of conventional spark ignition methods, thus leading to the desire to find new, alternative methods of ignition. This paper aims to provide the reader an overview of advanced ignition methods, with an emphasis on laser ignition and its applications to aerospace propulsion. A comprehensive review of advanced ignition systems in aerospace applications is performed. This includes studies on gas turbine applications, ramjet and scramjet systems, and space and rocket applications. A brief overview of ignition and laser ignition phenomena is also provided in earlier sections of the report. Throughout the reading, research papers, which were presented at the 2nd Laser Ignition Conference in April 2014, are mentioned to indicate the vast array of projects that are currently being pursued. (C) 2016 National Laboratory for Aeronautics and Astronautics. Production and hosting by Elsevier B.V. This is an open access article under the CC BY-NC-ND license (http//creativecommons.org/by-nc-nd/4.0/). C1 [O'Briant, Steven A.; Vasu, Subith S.] Univ Cent Florida, Ctr Adv Turbomachinery & Energy Res, Dept Mech & Aerosp Engn, Orlando, FL 32816 USA. [Gupta, Sreenath B.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Vasu, SS (reprint author), Univ Cent Florida, Ctr Adv Turbomachinery & Energy Res, Dept Mech & Aerosp Engn, Orlando, FL 32816 USA. EM subith@ucf.edu NR 93 TC 1 Z9 1 U1 8 U2 20 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 2212-540X J9 PROPULS POWER RES JI Propuls. Power Res. PD MAR PY 2016 VL 5 IS 1 BP 1 EP 21 DI 10.1016/j.jppr.2016.01.004 PG 21 WC Engineering, Aerospace SC Engineering GA DQ5PB UT WOS:000379256200001 ER PT J AU Phan-Lai, V AF Vy Phan-Lai TI Adoptive immunotherapy via CD4+ versus CD8+ T cells SO BIOMEDICAL RESEARCH AND THERAPY LA English DT Review DE Adoptive T cell therapy; immunotherapy; CD4+ T cells; CD8+ T cells; Th1; Th17; cytokines; TILs ID CANCER-IMMUNOTHERAPY; METASTATIC MELANOMA; PANCREATIC-CANCER; VACCINE DESIGN; HELPER-CELLS; TH17 CELLS; TUMOR; THERAPY; ANTIGEN; CD4(+) AB The goal of cancer immunotherapy is to induce specific and durable antitumor immunity. Adoptive T cell therapy (ACT) has garnered wide interest, particularly in regard to strategies to improve T cell efficacy in trials. There are many types of T cells (and subsets) which can be selected for use in ACT. CD4+ T cells are critical for the regulation, activation and aid of host defense mechanisms and, importantly, for enhancing the function of tumor-specific CD8+ T cells. To date, much research in cancer immunotherapy has focused on CD8+ T cells, in melanoma and other cancers. Both CD4+ T cells and CD8+ T cells have been evaluated as ACT in mice and humans, and both are effective at eliciting antitumor responses. IL-17 producing CD4+ T cells are a new subset of CD4+ T cells to be evaluated in ACT models. This review discusses the benefits of adoptive immunotherapy mediated by CD8+ and CD4+ cells. It also discusses the various type of T cells, source of T cells, and ex vivo cytokine growth factors for augmenting clinical efficacy of ACT. C1 [Vy Phan-Lai] Univ Calif Los Angeles, Ctr Global Mentoring, UCLA DOE Inst, Los Angeles, CA 90024 USA. [Vy Phan-Lai] Vietnam Natl Univ, Univ Sci, Ho Chi Minh City, Vietnam. RP Phan-Lai, V (reprint author), Univ Calif Los Angeles, Ctr Global Mentoring, UCLA DOE Inst, Los Angeles, CA 90024 USA.; Phan-Lai, V (reprint author), Vietnam Natl Univ, Univ Sci, Ho Chi Minh City, Vietnam. EM vyphanlai@mbi.ucla.edu NR 52 TC 0 Z9 0 U1 5 U2 6 PU BIOMEDPRESS PI HO CHI MINH PA BIOMEDPRESS, HO CHI MINH, 00000, VIETNAM SN 2198-4093 J9 BIOMED RES THER JI Biomed. Res. Ther. PD MAR PY 2016 VL 3 IS 4 BP 588 EP 595 DI 10.7603/s40730-016-0016-6 PG 8 WC Medicine, Research & Experimental SC Research & Experimental Medicine GA DP1CX UT WOS:000378229200002 ER PT J AU Wenk, ES Callaham, MA O'Brien, JJ Hanson, PJ AF Wenk, Evelyn S. Callaham, Mac A., Jr. O'Brien, Joseph J. Hanson, Paul J. TI Soil Macroinvertebrate Communities across a Productivity Gradient in Deciduous Forests of Eastern North America SO NORTHEASTERN NATURALIST LA English DT Article ID EXOTIC EARTHWORM INVASION; LITTER DECOMPOSITION; BIOLOGICAL INVASIONS; BOREAL FORESTS; PINE FORESTS; 1ST RECORDS; OLD-GROWTH; MILLIPEDES; MACROFAUNA; TEMPERATE AB Within the temperate, deciduous forests of the eastern US, diverse soil-fauna communities are structured by a combination of environmental gradients and interactions with other biota. The introduction of non-native soil taxa has altered communities and soil processes, and adds another degree of variability to these systems. We sampled soil macroinvertebrate abundance from forested sites in Missouri (MO), Michigan (MI), Massachusetts (MA), and New Hampshire (NH), with the objective of comparing community assemblages and evaluating the role of invasive earthworms along the temperature-productivity gradient represented by the sites. The primary detritivores encountered were earthworms and millipedes. Earthworms were collected only in MO and MI, and at much greater density in MO. Millipedes were found at every site except in MO, and at their highest mean density in NH. Warmer temperatures, higher litter productivity, and low Oa horizon depth (as found in MO) were correlated with high earthworm activity. Oa horizon depth was the greatest in NH, where the macroinvertebrate community was dominated (in terms of abundance) by predators and herbivores, not detritivores. Our results are suggestive of, and congruent with, the concept of earthworms as ecosystem engineers, as we found that the presence of non-native earthworm species was associated with significant differences in soil characteristics such as apparent rapid decomposition rates and reduced carbon storage in the Oa horizon. C1 [Wenk, Evelyn S.; Callaham, Mac A., Jr.; O'Brien, Joseph J.] US Forest Serv, Ctr Forest Disturbance Sci, USDA, So Res Stn, 320 Green St, Athens, GA 30602 USA. [Hanson, Paul J.] Oak Ridge Natl Lab, Environm Sci Div, POB 2008, Oak Ridge, TN 37831 USA. RP Callaham, MA (reprint author), US Forest Serv, Ctr Forest Disturbance Sci, USDA, So Res Stn, 320 Green St, Athens, GA 30602 USA. EM mcallaham@fs.fed.us RI Hanson, Paul J./D-8069-2011 OI Hanson, Paul J./0000-0001-7293-3561 FU US Department of Energy, Office of Science, Office of Biological and Environmental Research through Oak Ridge National Laboratory; US Department of Energy [DE-AC05-00OR22725] FX Greta Langhenry, David Combs, Jim Le Moine, and Jasmine Crumsey assisted with field sampling. This material is based upon work supported by the US Department of Energy, Office of Science, Office of Biological and Environmental Research through a contract with Oak Ridge National Laboratory, which is managed by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725 with the US Department of Energy. NR 74 TC 1 Z9 1 U1 9 U2 19 PU HUMBOLDT FIELD RESEARCH INST PI STEUBEN PA PO BOX 9, STEUBEN, ME 04680-0009 USA SN 1092-6194 EI 1938-5307 J9 NORTHEAST NAT JI Northeast. Nat PD MAR PY 2016 VL 23 IS 1 BP 25 EP 44 PG 20 WC Biodiversity Conservation; Ecology SC Biodiversity & Conservation; Environmental Sciences & Ecology GA DP0FG UT WOS:000378163600005 ER PT J AU Eddy, EN Roman, CT AF Eddy, Elizabeth N. Roman, Charles T. TI Relationship Between Epibenthic Invertebrate Species Assemblages and Environmental Variables in Boston Harbor's Intertidal Habitat SO NORTHEASTERN NATURALIST LA English DT Article ID GRAIN-SIZE DISTRIBUTION; ORGANIC-MATTER; WAVE EXPOSURE; ROCKY SHORES; COMMUNITY STRUCTURE; MARINE HABITATS; TIDAL COMMUNITY; SURFACE-AREA; COBSCOOK BAY; PATTERNS AB The Boston Harbor Islands National Recreation Area has an extensive intertidal zone, with 47% of the area composed of mixed-coarse substrate. Given anticipated climate-change impacts such as sea-level rise and ocean warming, and other stressors associated with the urban environment, the critical ecosystem functions (i.e., species habitat, food-web support) provided by this dominant mixed-coarse habitat of Boston Harbor, and elsewhere throughout the Northeast, have been and will likely be further altered. To evaluate the present-day epibenthic invertebrate communities and to determine what environmental factors of the mixed-coarse substrate affect community structure, we used a stratified random design to sample epibenthic macroinvertebrates along with various physical and environmental variables from the intertidal zone. Epibenthic macroinvertebrate species assemblages and diversity differed significantly between wave-exposed and wave-protected sites, with higher diversity present at protected sites. We also found that environmental variables collectively explained up to 67% of the variation in species assemblages, with elevation, organic content, water content, and sediment type individually explaining up to 56%, 30%, 42%, and 33% of the variation, respectively. This study provides a baseline for long-term monitoring aimed at understanding the response of cobble and mixed-coarse intertidal communities to multiple disturbances, and a foundation to support habitat restoration or other management actions. C1 [Eddy, Elizabeth N.] Univ Rhode Isl, Grad Sch Oceanog, Narragansett, RI 02882 USA. [Roman, Charles T.] Univ Rhode Isl, Natl Pk Serv, Narragansett, RI 02882 USA. RP Eddy, EN (reprint author), US EPA, ORISE Res Participat Program, Washington, DC 20460 USA. EM eeddy@my.uri.edu FU National Park Service FX Funding for this research was provided by the National Park Service, with funds administered through the North Atlantic Coast Cooperative Ecosystem Studies Unit at the University of Rhode Island. We thank Penelope Pooler Eisenbies for contributions to the study design; Sarah Waterworth, Annie Kreider, and the Green Ambassadors for their field assistance; Sheldon Pratt and Sebastian Kvist for taxonomic guidance; John King and Danielle Cares for sediment and grain-size analysis assistance; and Candace Oviatt, Carol Thornber, Mary-Jane James, and Marc Albert for their support throughout the study. NR 76 TC 0 Z9 0 U1 17 U2 24 PU HUMBOLDT FIELD RESEARCH INST PI STEUBEN PA PO BOX 9, STEUBEN, ME 04680-0009 USA SN 1092-6194 EI 1938-5307 J9 NORTHEAST NAT JI Northeast. Nat PD MAR PY 2016 VL 23 IS 1 BP 45 EP 66 PG 22 WC Biodiversity Conservation; Ecology SC Biodiversity & Conservation; Environmental Sciences & Ecology GA DP0FG UT WOS:000378163600006 ER PT J AU Armstrong, JC Favorite, JA AF Armstrong, Jerawan C. Favorite, Jeffrey A. TI Using a derivative-free optimization method for multiple solutions of inverse transport problems SO OPTIMIZATION AND ENGINEERING LA English DT Article DE Inverse transport problem; Derivative-free optimization; Stochastic global optimization; Multilevel single linkage; Mesh adaptive direct search ID ADAPTIVE DIRECT SEARCH; CONSTRAINED GLOBAL OPTIMIZATION; ALGORITHMS; CONVERGENCE AB Identifying unknown components of an object that emits radiation is an important problem for national and global security. Radiation signatures measured from an object of interest can be used to infer object parameter values that are not known. This problem is called an inverse transport problem. An inverse transport problem may have multiple solutions and the most widely used approach for its solution is an iterative optimization method. This paper proposes a stochastic derivative-free global optimization algorithm to find multiple solutions of inverse transport problems. The algorithm is an extension of a multilevel single linkage (MLSL) method where a mesh adaptive direct search (MADS) algorithm is incorporated into the local phase. Numerical test cases using uncollided fluxes of discrete gamma-ray lines are presented to show the performance of this new algorithm. C1 [Armstrong, Jerawan C.; Favorite, Jeffrey A.] Los Alamos Natl Lab, XCP Monte Carlo Methods Codes & Applicat Grp 3, Computat Phys Div, MS F663, Los Alamos, NM 87545 USA. RP Armstrong, JC (reprint author), Los Alamos Natl Lab, XCP Monte Carlo Methods Codes & Applicat Grp 3, Computat Phys Div, MS F663, Los Alamos, NM 87545 USA. EM jerawan@lanl.gov; fave@lanl.gov NR 34 TC 0 Z9 0 U1 1 U2 1 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 1389-4420 EI 1573-2924 J9 OPTIM ENG JI Optim. Eng. PD MAR PY 2016 VL 17 IS 1 SI SI BP 105 EP 125 DI 10.1007/s11081-015-9306-x PG 21 WC Engineering, Multidisciplinary; Operations Research & Management Science; Mathematics, Interdisciplinary Applications SC Engineering; Operations Research & Management Science; Mathematics GA DP1GP UT WOS:000378238800006 ER PT J AU Muller, J AF Mueller, Juliane TI MISO: mixed-integer surrogate optimization framework SO OPTIMIZATION AND ENGINEERING LA English DT Article DE Mixed-integer optimization; Surrogate models; Black-box optimization; Radial basis functions; Derivative-free; Global optimization ID BOX GLOBAL OPTIMIZATION; DERIVATIVE-FREE OPTIMIZATION; EXPENSIVE FUNCTIONS; ALGORITHMS; DESIGN; MODELS; MANAGEMENT; ENSEMBLE; SEARCH AB We introduce MISO, the mixed-integer surrogate optimization framework. MISO aims at solving computationally expensive black-box optimization problems with mixed-integer variables. This type of optimization problem is encountered in many applications for which time consuming simulation codes must be run in order to obtain an objective function value. Examples include optimal reliability design and structural optimization. A single objective function evaluation may take from several minutes to hours or even days. Thus, only very few objective function evaluations are allowable during the optimization. The development of algorithms for this type of optimization problems has, however, rarely been addressed in the literature. Because the objective function is black-box, derivatives are not available and numerically approximating the derivatives requires a prohibitively large number of function evaluations. Therefore, we use computationally cheap surrogate models to approximate the expensive objective function and to decide at which points in the variable domain the expensive objective function should be evaluated. We develop a general surrogate model framework and show how sampling strategies of well-known surrogate model algorithms for continuous optimization can be modified for mixed-integer variables. We introduce two new algorithms that combine different sampling strategies and local search to obtain high-accuracy solutions. We compare MISO in numerical experiments to a genetic algorithm, NOMAD version 3.6.2, and SO-MI. The results show that MISO is in general more efficient than NOMAD and the genetic algorithm with respect to finding improved solutions within a limited budget of allowable evaluations. The performance of MISO depends on the chosen sampling strategy. The MISO algorithm that combines a coordinate perturbation search with a target value strategy and a local search performs best among all algorithms. C1 [Mueller, Juliane] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Computat Sci & Engn, Berkeley, CA 94720 USA. RP Muller, J (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Computat Sci & Engn, Berkeley, CA 94720 USA. EM juliane.mueller2901@gmail.com FU U.S. Department of Energy, Office of Science, Office of Advanced Scientific Computing Research, Applied Mathematics program [DE-AC02005CH11231]; NSF CISE [1116298] FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Advanced Scientific Computing Research, Applied Mathematics program under contract number DE-AC02005CH11231. Partial support was also provided by NSF CISE 1116298 to Prof. Shoemaker at Cornell University, School of Civil and Environmental Engineering. NR 36 TC 0 Z9 0 U1 1 U2 2 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 1389-4420 EI 1573-2924 J9 OPTIM ENG JI Optim. Eng. PD MAR PY 2016 VL 17 IS 1 SI SI BP 177 EP 203 DI 10.1007/s11081-015-9281-2 PG 27 WC Engineering, Multidisciplinary; Operations Research & Management Science; Mathematics, Interdisciplinary Applications SC Engineering; Operations Research & Management Science; Mathematics GA DP1GP UT WOS:000378238800009 ER PT J AU Larson, J Wild, SM AF Larson, Jeffrey Wild, Stefan M. TI A batch, derivative-free algorithm for finding multiple local minima SO OPTIMIZATION AND ENGINEERING LA English DT Article DE Derivative-free optimization; Multistart; Parallel algorithms; Global optimization ID GLOBAL OPTIMIZATION METHODS; DIRECT SEARCH ALGORITHM; SOFTWARE AB We propose a derivative-free algorithm for finding high-quality local minima for functions that require significant computational resources to evaluate. Our algorithm efficiently utilizes the computational resources allocated to it and also has strong theoretical results, almost surely starting a finite number of local optimization runs and identifying all local minima. We propose metrics for measuring how efficiently an algorithm finds local minima, and we benchmark our algorithm on synthetic problems (with known local minima) and two real-world applications. C1 [Larson, Jeffrey; Wild, Stefan M.] Argonne Natl Lab, 9700 S Cass Ave,Bldg 240, Argonne, IL 60439 USA. RP Larson, J (reprint author), Argonne Natl Lab, 9700 S Cass Ave,Bldg 240, Argonne, IL 60439 USA. EM jmlarson@anl.gov; wild@anl.gov RI Wild, Stefan/P-4907-2016 OI Wild, Stefan/0000-0002-6099-2772 FU U.S. Department of Energy, Office of Science, Office of Advanced Scientific Computing Research [DE-AC02-06CH11357] FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Advanced Scientific Computing Research, SciDAC and applied mathematics programs under Contract DE-AC02-06CH11357. NR 22 TC 1 Z9 1 U1 2 U2 2 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 1389-4420 EI 1573-2924 J9 OPTIM ENG JI Optim. Eng. PD MAR PY 2016 VL 17 IS 1 SI SI BP 205 EP 228 DI 10.1007/s11081-015-9289-7 PG 24 WC Engineering, Multidisciplinary; Operations Research & Management Science; Mathematics, Interdisciplinary Applications SC Engineering; Operations Research & Management Science; Mathematics GA DP1GP UT WOS:000378238800010 ER PT J AU Stelpflug, SC Sekhon, RS Vaillancourt, B Hirsch, CN Buell, CR de Leon, N Kaeppler, SM AF Stelpflug, Scott C. Sekhon, Rajandeep S. Vaillancourt, Brieanne Hirsch, Candice N. Buell, C. Robin de Leon, Natalia Kaeppler, Shawn M. TI An Expanded Maize Gene Expression Atlas based on RNA Sequencing and its Use to Explore Root Development SO PLANT GENOME LA English DT Article ID F-BOX PROTEINS; CELL-GROWTH; ARABIDOPSIS-THALIANA; INFLORESCENCE ARCHITECTURE; TRANSCRIPTOME ATLAS; SPECIALIZED ZONES; ANALYSIS TOOLKIT; DATA SETS; ETHYLENE; GENOMICS AB Comprehensive and systematic transcriptome profiling provides valuable insight into biological and developmental processes that occur throughout the life cycle of a plant. We have enhanced our previously published microarray-based gene atlas of maize (Zea mays L.) inbred B73 to now include 79 distinct replicated samples that have been interrogated using RNA sequencing (RNA-seq). The current version of the atlas includes 50 original array-based gene atlas samples, a time-course of 12 stalk and leaf samples postflowering, and an additional set of 17 samples from the maize seedling and adult root system. The entire dataset contains 4.6 billion mapped reads, with an average of 20.5 million mapped reads per biological replicate, allowing for detection of genes with lower transcript abundance. As the new root samples represent key additions to the previously examined tissues, we highlight insights into the root transcriptome, which is represented by 28,894 (73.2%) annotated genes in maize. Additionally, we observed remarkable expression differences across both the longitudinal (four zones) and radial gradients (cortical parenchyma and stele) of the primary root supported by fourfold differential expression of 9353 and 4728 genes, respectively. Among the latter were 1110 genes that encode transcription factors, some of which are orthologs of previously characterized transcription factors known to regulate root development in Arabidopsis thaliana (L.) Heynh., while most are novel, and represent attractive targets for reverse genetics approaches to determine their roles in this important organ. This comprehensive transcriptome dataset is a powerful tool toward understanding maize development, physiology, and phenotypic diversity. C1 [Stelpflug, Scott C.; de Leon, Natalia; Kaeppler, Shawn M.] Univ Wisconsin, Dept Agron, 1575 Linden Dr, Madison, WI 53706 USA. [Sekhon, Rajandeep S.] Clemson Univ, Dept Genet & Biochem, Clemson, SC USA. [Vaillancourt, Brieanne; Buell, C. Robin] Michigan State Univ, Dept Plant Biol, E Lansing, MI 48824 USA. [Buell, C. Robin; de Leon, Natalia; Kaeppler, Shawn M.] DOE Great Lakes Bioenergy Res Ctr, E Lansing, MI USA. [Hirsch, Candice N.] Univ Minnesota, Dept Agron & Plant Genet, St Paul, MN 55108 USA. RP Kaeppler, SM (reprint author), Univ Wisconsin, Dept Agron, 1575 Linden Dr, Madison, WI 53706 USA.; Kaeppler, SM (reprint author), DOE Great Lakes Bioenergy Res Ctr, E Lansing, MI USA. EM smkaeppl@wisc.edu OI Kaeppler, Shawn/0000-0002-5964-1668 FU Department of Energy Great Lakes Bioenergy Research Center (Department of Energy Office of Biological and Environmental Research) [DE-FC02-07ER64494]; National Science Foundation's (NSF) Basic Research to Enable Agricultural Development (BREAD) program [0965480]; Agriculture and Food Research Initiative of the U.S. Department of Agriculture National Institute of Food and Agriculture [2014-67013-2157]; National Institute of Food and Agriculture, USDA Hatch funding [WIS01645] FX This work was funded by the Department of Energy Great Lakes Bioenergy Research Center (Department of Energy Office of Biological and Environmental Research grant number DE-FC02-07ER64494), the National Science Foundation's (NSF) Basic Research to Enable Agricultural Development (BREAD) program (0965480), and Agriculture and Food Research Initiative of the U.S. Department of Agriculture National Institute of Food and Agriculture (grant no. 2014-67013-2157). The authors thank the MaizeGDB team of Jack Gardiner, Mary Schaeffer, Carson Andorf, and John Portwood for making this resource easily visualized and utilized by the plant community. S.C.S was supported in part by the National Institute of Food and Agriculture, USDA Hatch funding (WIS01645). The authors declare no conflict of interest. NR 83 TC 3 Z9 3 U1 6 U2 9 PU CROP SCIENCE SOC AMER PI MADISON PA 677 S SEGOE ROAD, MADISON, WI 53711 USA SN 1940-3372 J9 PLANT GENOME-US JI Plant Genome PD MAR PY 2016 VL 9 IS 1 DI 10.3835/plantgenome2015.04.0025 PG 16 WC Plant Sciences; Genetics & Heredity SC Plant Sciences; Genetics & Heredity GA DO9ZM UT WOS:000378146900004 ER PT J AU Wagh, K Bhattacharya, T Williamson, C Robles, A Bayne, M Garrity, J Rist, M Rademeyer, C Yoon, H Lapedes, A Gao, HM Greene, K Louder, MK Kong, R Karim, SA Burton, DR Barouch, DH Nussenzweig, MC Mascola, JR Morris, L Montefiori, DC Korber, B Seaman, MS AF Wagh, Kshitij Bhattacharya, Tanmoy Williamson, Carolyn Robles, Alex Bayne, Madeleine Garrity, Jetta Rist, Michael Rademeyer, Cecilia Yoon, Hyejin Lapedes, Alan Gao, Hongmei Greene, Kelli Louder, Mark K. Kong, Rui Karim, Salim Abdool Burton, Dennis R. Barouch, Dan H. Nussenzweig, Michel C. Mascola, John R. Morris, Lynn Montefiori, David C. Korber, Bette Seaman, Michael S. TI Optimal Combinations of Broadly Neutralizing Antibodies for Prevention and Treatment of HIV-1 Clade C SO PLOS PATHOGENS LA English DT Article ID IMMUNODEFICIENCY-VIRUS TYPE-1; HUMAN MONOCLONAL-ANTIBODY; MUCOSAL SHIV CHALLENGE; N-GLYCAN RECOGNITION; POTENT NEUTRALIZATION; HUMANIZED MICE; IN-VITRO; GP41-GP120 INTERFACE; IMPROVES PROTECTION; VACCINE DEVELOPMENT AB The identification of a new generation of potent broadly neutralizing HIV-1 antibodies (bnAbs) has generated substantial interest in their potential use for the prevention and/or treatment of HIV-1 infection. While combinations of bnAbs targeting distinct epitopes on the viral envelope (Env) will likely be required to overcome the extraordinary diversity of HIV-1, a key outstanding question is which bnAbs, and how many, will be needed to achieve optimal clinical benefit. We assessed the neutralizing activity of 15 bnAbs targeting four distinct epitopes of Env, including the CD4-binding site (CD4bs), the V1/V2-glycan region, the V3-glycan region, and the gp41 membrane proximal external region (MPER), against a panel of 200 acute/early clade C HIV-1 Env pseudoviruses. A mathematical model was developed that predicted neutralization by a subset of experimentally evaluated bnAb combinations with high accuracy. Using this model, we performed a comprehensive and systematic comparison of the predicted neutralizing activity of over 1,600 possible double, triple, and quadruple bnAb combinations. The most promising bnAb combinations were identified based not only on breadth and potency of neutralization, but also other relevant measures, such as the extent of complete neutralization and instantaneous inhibitory potential (IIP). By this set of criteria, triple and quadruple combinations of bnAbs were identified that were significantly more effective than the best double combinations, and further improved the probability of having multiple bnAbs simultaneously active against a given virus, a requirement that may be critical for countering escape in vivo. These results provide a rationale for advancing bnAb combinations with the best in vitro predictors of success into clinical trials for both the prevention and treatment of HIV-1 infection. C1 [Wagh, Kshitij; Bhattacharya, Tanmoy; Yoon, Hyejin; Lapedes, Alan; Korber, Bette] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM USA. [Bhattacharya, Tanmoy] Santa Fe Inst, Santa Fe, NM 87501 USA. [Williamson, Carolyn; Rademeyer, Cecilia] Univ Cape Town, Inst Infect Dis & Mol Med, Div Med Virol, ZA-7925 Cape Town, South Africa. [Williamson, Carolyn; Rademeyer, Cecilia] NHLS, Cape Town, South Africa. [Robles, Alex; Bayne, Madeleine; Garrity, Jetta; Rist, Michael; Seaman, Michael S.] Beth Israel Deaconess Med Ctr, Ctr Virol & Vaccine Res, Boston, MA 02215 USA. [Gao, Hongmei; Greene, Kelli; Montefiori, David C.] Duke Univ, Med Ctr, Dept Surg, Durham, NC 27710 USA. [Louder, Mark K.; Kong, Rui; Mascola, John R.] NIAID, Vaccine Res Ctr, NIH, 9000 Rockville Pike, Bethesda, MD 20892 USA. [Karim, Salim Abdool] Univ KwaZulu Natal, Durban Dept Immunol & Microbial Sci, Durban, South Africa. [Karim, Salim Abdool; Morris, Lynn] Univ KwaZulu Natal, Ctr AIDS Programme Res S Africa CAPRISA, Durban, South Africa. [Burton, Dennis R.] Scripps Res Inst, La Jolla, CA 92037 USA. [Nussenzweig, Michel C.] Rockefeller Univ, Lab Mol Immunol, 1230 York Ave, New York, NY 10021 USA. [Morris, Lynn] Univ Witwatersrand, Natl Inst Communicable Dis, NHLS, Johannesburg 2050, South Africa. RP Seaman, MS (reprint author), Beth Israel Deaconess Med Ctr, Ctr Virol & Vaccine Res, Boston, MA 02215 USA. EM mseaman@bidmc.harvard.edu FU Bill and Melinda Gates Foundation Collaboration for AIDS Vaccine Discovery (CAVD) grant [1032144]; intramural research program of the Vaccine Research Center (VRC), NIAID, NIH; Center for Nonlinear Studies (CNLS) at Los Alamos National Laboratory FX This work was supported by the Bill and Melinda Gates Foundation Collaboration for AIDS Vaccine Discovery (CAVD) grant #1032144, and in part from the intramural research program of the Vaccine Research Center (VRC), NIAID, NIH. KW was supported by the Center for Nonlinear Studies (CNLS) at Los Alamos National Laboratory. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 87 TC 16 Z9 16 U1 1 U2 4 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1553-7366 EI 1553-7374 J9 PLOS PATHOG JI PLoS Pathog. PD MAR PY 2016 VL 12 IS 3 AR e1005520 DI 10.1371/journal.ppat.1005520 PG 27 WC Microbiology; Parasitology; Virology SC Microbiology; Parasitology; Virology GA DP0CH UT WOS:000378154800037 PM 27028935 ER PT J AU Chen, CT Liao, JC AF Chen, Chang-Ting Liao, James C. TI Frontiers in microbial 1-butanol and isobutanol production SO FEMS MICROBIOLOGY LETTERS LA English DT Review DE butanol; metabolic engineering; synthetic biology; ABE fermentation; isobutanol ID CLOSTRIDIUM-BEIJERINCKII BA101; ACETOBUTYLICUM ATCC 824; BUTANOL PRODUCTION; ESCHERICHIA-COLI; GENOME SEQUENCE; SACCHAROMYCES-CEREVISIAE; TRANSCRIPTIONAL PROGRAM; RECOMBINANT STRAINS; BIOFUEL PRODUCTION; BACILLUS-SUBTILIS AB The heavy dependence on petroleum-derived fuel has raised concerns about energy sustainability and climate change, which have prompted researchers to explore fuel production from renewable sources. 1-Butanol and isobutanol are promising biofuels that have favorable properties and can also serve as solvents or chemical feedstocks. Microbial production of these alcohols provides great opportunities to access a wide spectrum of renewable resources. In recent years, research has improved the native 1-butanol production and has engineered isobutanol production in various organisms to explore metabolic diversity and a broad range of substrates. This review focuses on progress in metabolic engineering for the production of these two compounds using various resources. C1 [Chen, Chang-Ting; Liao, James C.] Univ Calif Los Angeles, Dept Chem & Biomol Engn, 420 Westwood Plaza, Los Angeles, CA 90095 USA. [Liao, James C.] Univ Calif Los Angeles, UCLA DOE Inst Genom & Prote, 420 Westwood Plaza, Los Angeles, CA 90095 USA. RP Liao, JC (reprint author), Univ Calif Los Angeles, Dept Chem & Biomol Engn, 420 Westwood Plaza, Los Angeles, CA 90095 USA. EM liaoj@ucla.edu FU US Department of Energy BioEnergy Science Center; US National Science Foundation [MCB-1139318]; Department of Energy [DE-SC0012384] FX The authors are supported in part by the US Department of Energy BioEnergy Science Center, and grants from the US National Science Foundation (MCB-1139318) and Department of Energy (DE-SC0012384). NR 86 TC 1 Z9 1 U1 15 U2 29 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0378-1097 EI 1574-6968 J9 FEMS MICROBIOL LETT JI FEMS Microbiol. Lett. PD MAR PY 2016 VL 363 IS 5 AR fnw020 DI 10.1093/femsle/fnw020 PG 13 WC Microbiology SC Microbiology GA DO7ML UT WOS:000377966600003 PM 26832641 ER PT J AU Lahiri, D Choi, Y Yusuf, SM Kumar, A Ramanan, N Chattopadhyay, S Haskel, D Sharma, SM AF Lahiri, Debdutta Choi, Yongseong Yusuf, S. M. Kumar, Amit Ramanan, Nitya Chattopadhyay, Soma Haskel, Daniel Sharma, Surinder M. TI Understanding temperature and magnetic-field actuated magnetization polarity reversal in the Prussian blue analogue Cu0.73Mn0.77[Fe(CN)(6)]center dot zH(2)O, using XMCD SO MATERIALS RESEARCH EXPRESS LA English DT Article DE XMCD; negative magnetization; magnetic switch; Prussian blue analog; molecular magnet ID SPIN REORIENTATION TRANSITION; CIRCULAR-DICHROISM; NEUTRON-DIFFRACTION; COMPENSATION; REFRIGERATOR; ND2FE14B; PROBE AB We have investigated the microscopic origin of temperature and magnetic-field actuated magnetization reversal in Cu0.73Mn0.77[Fe(CN)(6)]center dot zH(2)O, using XMCD. Our results show a fair deviation from the mean-field-theory in the form of different ordering temperatures of Fe and Mn sublattices. A preferential sign reversal of Mn spin under magnetic field and different spin cant angles for the two sublattices have also been observed. An antiferromagnetic coupling between the Fe and Mn sublattices along with different ordering temperatures (sublattice decoupling) for these sublattices explain the temperature-dependent magnetization reversal. Whereas, Mn spin reversal alone (under external magnetic field) is responsible for the observed field-dependent magnetization reversal. The dissimilar magnetic behavior of Fe and Mn sublattices in this cubic 3d-orbital system has been understood by invoking disparity and competition among inter-sublattice magnetic control parameters, viz. magnetic Zeeman energy, exchange coupling constant and magnetic anisotropy constant. Our results have significant design implications for future magnetic switches, by optimizing the competition among these magnetic control parameters. C1 [Lahiri, Debdutta; Ramanan, Nitya; Sharma, Surinder M.] Bhabha Atom Res Ctr, High Pressure& Synchrotron Radiat Phys Div, Bombay 400085, Maharashtra, India. [Choi, Yongseong; Chattopadhyay, Soma; Haskel, Daniel] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Yusuf, S. M.; Kumar, Amit] Bhabha Atom Res Ctr, Div Solid State Phys, Bombay 400085, Maharashtra, India. [Chattopadhyay, Soma] Elgin Community Coll, Dept Phys Sci, 1700 Spartan Dr, Elgin, IL 60123 USA. RP Lahiri, D (reprint author), Bhabha Atom Res Ctr, High Pressure& Synchrotron Radiat Phys Div, Bombay 400085, Maharashtra, India. EM dlahiri@barc.gov.in; smyusuf@barc.gov.in FU U.S. Department of Energy, Office of Science [DE-AC02-06CH11357] FX Work at Argonne was supported by the U.S. Department of Energy, Office of Science, under Contract No. DE-AC02-06CH11357. NR 37 TC 1 Z9 1 U1 4 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2053-1591 J9 MATER RES EXPRESS JI Mater. Res. Express PD MAR PY 2016 VL 3 IS 3 AR UNSP 036101 DI 10.1088/2053-1591/3/3/036101 PG 7 WC Materials Science, Multidisciplinary SC Materials Science GA DO5GH UT WOS:000377811100030 ER PT J AU Engel, P Kwong, WK McFrederick, Q Anderson, KE Barribeau, SM Chandler, JA Cornman, RS Dainat, J de Miranda, JR Doublet, V Emery, O Evans, JD Farinelli, L Flenniken, ML Granberg, F Grasis, JA Gauthier, L Hayer, J Koch, H Kocher, S Martinson, VG Moran, N Munoz-Torres, M Newton, I Paxton, RJ Powell, E Sadd, BM Schmid-Hempel, P Schmid-Hempel, R Song, SJ Schwarz, RS Vanengelsdorp, D Dainat, B AF Engel, Philipp Kwong, Waldan K. McFrederick, Quinn Anderson, Kirk E. Barribeau, Seth Michael Chandler, James Angus Cornman, R. Scott Dainat, Jacques de Miranda, Joachim R. Doublet, Vincent Emery, Olivier Evans, Jay D. Farinelli, Laurent Flenniken, Michelle L. Granberg, Fredrik Grasis, Juris A. Gauthier, Laurent Hayer, Juliette Koch, Hauke Kocher, Sarah Martinson, Vincent G. Moran, Nancy Munoz-Torres, Monica Newton, Irene Paxton, Robert J. Powell, Eli Sadd, Ben M. Schmid-Hempel, Paul Schmid-Hempel, Regula Song, Se Jin Schwarz, Ryan S. vanengelsdorp, Dennis Dainat, Benjamin TI The Bee Microbiome: Impact on Bee Health and Model for Evolution and Ecology of Host-Microbe Interactions SO MBIO LA English DT Review ID HONEYBEE APIS-MELLIFERA; DEFORMED-WING-VIRUS; PATHOGENS NOSEMA-CERANAE; COLONY COLLAPSE DISORDER; GUT MICROBIOTA; BUMBLE BEES; DROSOPHILA-MELANOGASTER; DEFENSE-MECHANISMS; DIVERSITY; INFECTION AB As pollinators, bees are cornerstones for terrestrial ecosystem stability and key components in agricultural productivity. All animals, including bees, are associated with a diverse community of microbes, commonly referred to as the micro biome. The bee micro biome is likely to be a crucial factor affecting host health. However, with the exception of a few pathogens, the impacts of most members of the bee microbiome on host health are poorly understood. Further, the evolutionary and ecological forces that shape and change the microbiome are unclear. Here, we discuss recent progress in our understanding of the bee microbiome, and we present challenges associated with its investigation. We conclude that global coordination of research efforts is needed to fully understand the complex and highly dynamic nature of the interplay between the bee micro biome, its host, and the environment. High-throughput sequencing technologies are ideal for exploring complex biological systems, including host-microbe interactions. To maximize their value and to improve assessment of the factors affecting bee health, sequence data should be archived, curated, and analyzed in ways that promote the synthesis of different studies. To this end, the BeeBiome consortium aims to develop an online database which would provide reference sequences, archive metadata, and host analytical resources. The goal would be to support applied and fundamental research on bees and their associated microbes and to provide a collaborative framework for sharing primary data from different research programs, thus furthering our understanding of the bee microbiome and its impact on pollinator health. C1 [Engel, Philipp; Emery, Olivier; Gauthier, Laurent; Dainat, Benjamin] Univ Lausanne, Dept Fundamental Microbiol, Lausanne, Switzerland. [Kwong, Waldan K.; Gauthier, Laurent] Yale Univ, Ecol & Evolutionary Biol, New Haven, CT USA. [Kwong, Waldan K.; Koch, Hauke; Moran, Nancy; Powell, Eli] Univ Texas Austin, Dept Integrat Biol, Austin, TX 78712 USA. [McFrederick, Quinn] Univ Calif Riverside, Dept Entomol, Riverside, CA 92521 USA. [Anderson, Kirk E.] USDA, Carl Hayden Bee Res Ctr, Tucson, AZ USA. [Barribeau, Seth Michael] E Carolina Univ, Dept Biol, Greenville, NC USA. [Chandler, James Angus] Calif Acad Sci, Dept Microbiol, San Francisco, CA 94118 USA. [Cornman, R. Scott] US Geol Survey, Ft Collins Sci Ctr, Ft Collins, CO USA. [Dainat, Jacques] Linkopings Univ Victoria Westling, BILS, Linkoping, Sweden. [Dainat, Jacques] Uppsala Univ, Dept Med Biochem & Microbiol, Uppsala, Sweden. [de Miranda, Joachim R.] Swedish Univ Agr Sci, Dept Ecol, Uppsala, Sweden. [Doublet, Vincent; Paxton, Robert J.] Univ Halle Wittenberg, Inst Biol, D-06108 Halle, Germany. [Doublet, Vincent; Paxton, Robert J.] German Ctr Integrat Biodivers Res iDiv, Leipzig, Germany. [Evans, Jay D.; Schwarz, Ryan S.] ARS, USDA, Bee Res Lab, Beltsville, MD USA. [Farinelli, Laurent] Fasteris SA, Plan Les Ouates, Switzerland. [Flenniken, Michelle L.] Montana State Univ, Dept Plant Sci & Plant Pathol, Bozeman, MT 59717 USA. [Granberg, Fredrik] BVF, SLU, Uppsala, Sweden. [Grasis, Juris A.] San Diego State Univ, Dept Biol, North Life Sci, San Diego, CA 92182 USA. [Hayer, Juliette] SLU, Inst Husdjursgenet, Uppsala, Sweden. [Koch, Hauke] Royal Bot Gardens, Richmond, Surrey, England. [Kocher, Sarah] Harvard Univ, Dept Organism & Evolutionary Biol, Museum Comparat Zool, Cambridge, MA 02138 USA. [Martinson, Vincent G.] Univ Rochester, Dept Biol, Rochester, NY 14627 USA. [Munoz-Torres, Monica] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Genom & Syst Biol Div, Berkeley, CA 94720 USA. [Newton, Irene] Indiana Univ, Dept Biol, Bloomington, IN USA. [Sadd, Ben M.] Illinois State Univ, Sch Biol Sci, Normal, IL 61761 USA. [Schmid-Hempel, Paul; Schmid-Hempel, Regula] ETHZ Inst Integrat Biol, Zurich, Switzerland. [Song, Se Jin] Univ Colorado, Boulder, CO 80309 USA. [vanengelsdorp, Dennis] Univ Maryland, Dept Entomol, College Pk, MD 20742 USA. [Dainat, Benjamin] Swiss Bee Resegman Ctr, Bern, Switzerland. [Dainat, Benjamin] Apiservice, Bee Hlth Extens Serv, Bern, Switzerland. [Chandler, James Angus; Dainat, Benjamin] Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. RP Engel, P (reprint author), Univ Lausanne, Dept Fundamental Microbiol, Lausanne, Switzerland.; Dainat, B (reprint author), Apiservice, Bee Hlth Extens Serv, Bern, Switzerland.; Dainat, B (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. EM philipp.engel@unil.ch; benjamin.dainat@agroscope.admin.ch RI Paxton, Robert/D-7082-2015; Doublet, Vincent/D-8050-2015; Granberg, Fredrik/F-2325-2014; OI Paxton, Robert/0000-0003-2517-1351; Doublet, Vincent/0000-0002-6313-1222; Granberg, Fredrik/0000-0001-5497-9611; Evans, Jay/0000-0002-0036-4651; Grasis, Juris/0000-0002-3945-0135; Rodrigues de Miranda, Joachim/0000-0002-0335-0386; Sadd, Ben/0000-0003-3136-5144 FU National Evolutionary Synthesis Center (NESCent), NSF [EF-0905606] FX This manuscript arose from the discussions by the Bee Microbiome consortium at the National Evolutionary Synthesis Center (NESCent) workshop "BeeBiome:Omic approaches for understanding bee microbe relationships" held in Durham, NC, USA from 20 to 24th October 2014. The workshop was supported by the National Evolutionary Synthesis Center (NESCent), grant NSF #EF-0905606 to B.D., P.E., J.R.M., J.D.E., and L.G. NR 100 TC 9 Z9 9 U1 27 U2 57 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD MAR-APR PY 2016 VL 7 IS 2 AR e02164 DI 10.1128/mBio.02164-15 PG 9 WC Microbiology SC Microbiology GA DO4QT UT WOS:000377768700029 PM 27118586 ER PT J AU Hemme, CL Green, SJ Rishishwar, L Prakash, O Pettenato, A Chakraborty, R Deutschbauer, AM Van Nostrand, JD Wu, LY He, ZL Jordan, IK Hazen, TC Arkin, AP Kostka, JE Zhou, JZ AF Hemme, Christopher L. Green, Stefan J. Rishishwar, Lavanya Prakash, Om Pettenato, Angelica Chakraborty, Romy Deutschbauer, Adam M. Van Nostrand, Joy D. Wu, Liyou He, Zhili Jordan, I. King Hazen, Terry C. Arkin, Adam P. Kostka, Joel E. Zhou, Jizhong TI Lateral Gene Transfer in a Heavy Metal-Contaminated-Groundwater Microbial Community SO MBIO LA English DT Article ID IN-SITU BIOREMEDIATION; HORIZONTAL TRANSFERS; SUBSURFACE SEDIMENTS; REDUCING BACTERIA; ANALYSIS SYSTEM; LOW-PH; NITRATE; GENERATION; EVOLUTION; ALIGNMENT AB Unraveling the drivers controlling the response and adaptation of biological communities to environmental change, especially anthropogenic activities, is a central but poorly understood issue in ecology and evolution. Comparative genomics studies suggest that lateral gene transfer (LGT) is a major force driving microbial genome evolution, but its role in the evolution of microbial communities remains elusive. To delineate the importance of LGT in mediating the response of a groundwater microbial community to heavy metal contamination, representative Rhodanobacter reference genomes were sequenced and compared to shotgun metagenome sequences. 16S rRNA gene-based amplicon sequence analysis indicated that Rhodanobacter populations were highly abundant in contaminated wells with low pHs and high levels of nitrate and heavy metals but remained rare in the uncontaminated wells. Sequence comparisons revealed that multiple geochemically important genes, including genes encoding Fe2+/Pb2+ permeases, most denitrification enzymes, and cytochrome c(553), were native to Rhodanobacter and not subjected to LGT. In contrast, the Rhodanobacter pangenome contained a recombinational hot spot in which numerous metal resistance genes were subjected to LGT and/or duplication. In particular, Co2+/Zn2+/Cd2+ efflux and mercuric resistance operon genes appeared to be highly mobile within Rhodanobacter populations. Evidence of multiple duplications of a mercuric resistance operon common to most Rhodanobacter strains was also observed. Collectively, our analyses indicated the importance of LGT during the evolution of groundwater microbial communities in response to heavy metal contamination, and a conceptual model was developed to display such adaptive evolutionary processes for explaining the extreme dominance of Rhodanobacter populations in the contaminated groundwater microbiome. IMPORTANCE Lateral gene transfer (LGT), along with positive selection and gene duplication, are the three main mechanisms that drive adaptive evolution of microbial genomes and communities, but their relative importance is unclear. Some recent studies suggested that LGT is a major adaptive mechanism for microbial populations in response to changing environments, and hence, it could also be critical in shaping microbial community structure. However, direct evidence of LGT and its rates in extant natural microbial communities in response to changing environments is still lacking. Our results presented in this study provide explicit evidence that LGT played a crucial role in driving the evolution of a groundwater microbial community in response to extreme heavy metal contamination. It appears that acquisition of genes critical for survival, growth, and reproduction via LGT is the most rapid and effective way to enable microorganisms and associated microbial communities to quickly adapt to abrupt harsh environmental stresses. C1 [Hemme, Christopher L.; Van Nostrand, Joy D.; Wu, Liyou; He, Zhili; Zhou, Jizhong] Univ Oklahoma, Dept Microbiol & Plant Sci, Inst Environm Genom, Norman, OK 73019 USA. [Hemme, Christopher L.] Univ So Calif, Ostrow Sch Dent, Los Angeles, CA USA. [Green, Stefan J.] Univ Illinois, Dept Biol Sci, Chicago, IL 60680 USA. [Green, Stefan J.] Univ Illinois, DNA Serv Facil, Chicago, IL USA. [Rishishwar, Lavanya; Jordan, I. King; Kostka, Joel E.] Georgia Inst Technol, Sch Biol & Earth & Atmospher Sci, Atlanta, GA 30332 USA. [Prakash, Om] Natl Ctr Cell Sci, Pune, Maharashtra, India. [Pettenato, Angelica; Chakraborty, Romy; Zhou, Jizhong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Deutschbauer, Adam M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Jordan, I. King] PanAmer Bioinformat Inst, Santa Marta, Magdalena, Colombia. [Hazen, Terry C.] Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN USA. [Hazen, Terry C.] Univ Tennessee, Dept Earth & Planetary Sci, Knoxville, TN USA. [Hazen, Terry C.] Univ Tennessee, Dept Microbiol, Knoxville, TN 37996 USA. [Hazen, Terry C.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. [Arkin, Adam P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Bioengn, Berkeley, CA 94720 USA. [Zhou, Jizhong] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China. [Hemme, Christopher L.] Univ Rhode Isl, Christopher L Hemme Dept Biomed & Pharmaceut Sci, Kingston, RI 02881 USA. RP Zhou, JZ (reprint author), Univ Oklahoma, Dept Microbiol & Plant Sci, Inst Environm Genom, Norman, OK 73019 USA.; Zhou, JZ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA.; Zhou, JZ (reprint author), Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China. EM jzhou@ou.edu RI Hazen, Terry/C-1076-2012; Chakraborty, Romy/D-9230-2015; OI Hazen, Terry/0000-0002-2536-9993; Chakraborty, Romy/0000-0001-9326-554X; Arkin, Adam/0000-0002-4999-2931 FU U.S. Department of Energy (DOE) [DE-AC02-05CH11231, DE-FG02-07ER64398] FX This work, including the efforts of Terry C. Hazen and Adam P. Arkin, was funded by U.S. Department of Energy (DOE) (DE-AC02-05CH11231 and DE-FG02-07ER64398). NR 71 TC 1 Z9 1 U1 20 U2 33 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD MAR-APR PY 2016 VL 7 IS 2 AR e02234-15 DI 10.1128/mBio.02234-15 PG 14 WC Microbiology SC Microbiology GA DO4QT UT WOS:000377768700041 PM 27048805 ER PT J AU Bellum, JC Field, ES Winstone, TB Kletecka, DE AF Bellum, John C. Field, Ella S. Winstone, Trevor B. Kletecka, Damon E. TI Low Group Delay Dispersion Optical Coating for Broad Bandwidth High Reflection at 45 degrees Incidence, P Polarization of Femtosecond Pulses with 900 nm Center Wavelength SO COATINGS LA English DT Article DE optical coatings; broad bandwidth high reflection; low group delay dispersion; high laser-induced damage thresholds AB We describe an optical coating design suitable for broad bandwidth high reflection (BBHR) at 45 degrees angle of incidence (AOI), P polarization (Ppol) of femtosecond (fs) laser pulses whose wavelengths range from 800 to 1000 nm. Our design process is guided by quarter-wave HR coating properties. The design must afford low group delay dispersion (GDD) for reflected light over the broad, 200 nm bandwidth in order to minimize temporal broadening of the fs pulses due to dispersive alteration of relative phases between their frequency components. The design should also be favorable to high laser-induced damage threshold (LIDT). We base the coating on TiO2/SiO2 layer pairs produced by means of e-beam evaporation with ion-assisted deposition, and use OptiLayer Thin Film Software to explore designs starting with TiO2/SiO2 layers having thicknesses in a reverse chirped arrangement. This approach led to a design with R > 99% from 800 to 1000 nm and GDD < 20 fs(2) from 843 to 949 nm (45 degrees AOI, Ppol). The design's GDD behaves in a smooth way, suitable for GDD compensation techniques, and its electric field intensities show promise for high LIDTs. Reflectivity and GDD measurements for the initial test coating indicate good performance of the BBHR design. Subsequent coating runs with improved process calibration produced two coatings whose HR bands satisfactorily meet the design goals. For the sake of completeness, we summarize our previously reported transmission spectra and LIDT test results with 800 ps, 8 ps and 675 fs pulses for these two coatings, and present a table of the LIDT results we have for all of our TiO2/SiO2 BBHR coatings, showing the trends with test laser pulse duration from the ns to sub-ps regimes. C1 [Bellum, John C.; Field, Ella S.; Kletecka, Damon E.] Sandia Natl Labs, POB 5800,MS 1197, Albuquerque, NM 87185 USA. [Winstone, Trevor B.] Rutherford Appleton Lab, STFC, Didcot OX11 0QX, Oxon, England. RP Bellum, JC (reprint author), Sandia Natl Labs, POB 5800,MS 1197, Albuquerque, NM 87185 USA. EM jcbellu@sandia.gov; efield@sandia.gov; trevor.winstone@stfc.ac.uk; dkletec@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. This paper is based on invited presentations by one of us (JCB) at the 3rd Frontiers of Optical Coatings International Conference on Optical Thin Film and Coating Technology held at Tongji University in Shanghai, China 20-24 October 2014, and at the Pacific Rim Laser Damage 2015: Optical Materials for High-Power Lasers Conference held in Jiading, Shanghai, China 17-20 May 2015. We thank James Oliver and Christopher Smith of University of Rochester in the United States for providing the GDD measurements, and Laurent Lamaignere and Martin Sozet of CEA/CESTA in France for providing the LIDT measurements with 675 fs pulses at 1053 nm. NR 21 TC 3 Z9 3 U1 7 U2 8 PU MDPI AG PI BASEL PA POSTFACH, CH-4005 BASEL, SWITZERLAND SN 2079-6412 J9 COATINGS JI Coatings PD MAR PY 2016 VL 6 IS 1 AR 11 DI 10.3390/coatings6010011 PG 17 WC Materials Science, Coatings & Films SC Materials Science GA DN7KH UT WOS:000377253800010 ER PT J AU Haugan, HJ Brown, GJ Olson, BV Kadlec, EA Kim, JK Shaner, EA AF Haugan, Heather J. Brown, Gail J. Olson, Benjamin V. Kadlec, Emil A. Kim, Jin K. Shaner, Eric A. TI Minority carrier lifetimes in very long-wave infrared InAs/GaInSb superlattices SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B LA English DT Article ID II SUPERLATTICES; DETECTORS AB Significantly improved carrier lifetimes in very-long wave infrared InAs/GaInSb superlattice (SL) absorbers are demonstrated by using time-resolved microwave reflectance (TMR) measurements. A nominal 47.0 angstrom InAs/21.5 angstrom Ga0.75In0.25Sb SL structure that produces an approximately 25 mu m response at 10 K has a minority carrier lifetime of 140 +/- 20 ns at 18 K, which is markedly long for SL absorber with such a narrow bandgap. This improvement is attributed to the strain-engineered ternary design. Such SL employs a shorter period with reduced gallium in order to achieve good optical absorption and epitaxial advantages, which ultimately leads to the improvements in the minority carrier lifetime by reducing Shockley-Read-Hall (SRH) defects. By analyzing the temperature-dependence of TMR decay data, the recombination mechanisms and trap states that currently limit the performance of this SL absorber have been identified. The results show a general decrease in the long-decay lifetime component, which is dominated by the SRH recombination at temperature below similar to 30 K, and by Auger recombination at temperatures above similar to 45 K. (C) 2016 American Vacuum Society. C1 [Haugan, Heather J.; Brown, Gail J.] Air Force Res Lab, Mat & Mfg Directorate, Wright Patterson AFB, OH 45433 USA. [Olson, Benjamin V.; Kadlec, Emil A.; Kim, Jin K.; Shaner, Eric A.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Haugan, HJ (reprint author), Air Force Res Lab, Mat & Mfg Directorate, Wright Patterson AFB, OH 45433 USA. EM heather.haugan.ctr@us.af.mil NR 22 TC 2 Z9 2 U1 6 U2 7 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 1071-1023 J9 J VAC SCI TECHNOL B JI J. Vac. Sci. Technol. B PD MAR PY 2016 VL 34 IS 2 AR 02L104 DI 10.1116/1.4941132 PG 4 WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology; Physics, Applied SC Engineering; Science & Technology - Other Topics; Physics GA DN0UU UT WOS:000376782200012 ER PT J AU Theisen, MK Rivera, JGL Liao, JC AF Theisen, Matthew K. Rivera, Jimmy G. Lafontaine Liao, James C. TI Stability of Ensemble Models Predicts Productivity of Enzymatic Systems SO PLOS COMPUTATIONAL BIOLOGY LA English DT Article ID METABOLIC SYSTEMS; PHOSPHOFRUCTOKINASE; THERMODYNAMICS; INHIBITION; HEXOKINASE; GLYCOLYSIS; NETWORKS; PATHWAYS AB Stability in a metabolic system may not be obtained if incorrect amounts of enzymes are used. Without stability, some metabolites may accumulate or deplete leading to the irreversible loss of the desired operating point. Even if initial enzyme amounts achieve a stable steady state, changes in enzyme amount due to stochastic variations or environmental changes may move the system to the unstable region and lose the steady-state or quasi-steady-state flux. This situation is distinct from the phenomenon characterized by typical sensitivity analysis, which focuses on the smooth change before loss of stability. Here we show that metabolic networks differ significantly in their intrinsic ability to attain stability due to the network structure and kinetic forms, and that after achieving stability, some enzymes are prone to cause instability upon changes in enzyme amounts. We use Ensemble Modelling for Robustness Analysis (EMRA) to analyze stability in four cell-free enzymatic systems when enzyme amounts are changed. Loss of stability in continuous systems can lead to lower production even when the system is tested experimentally in batch experiments. The predictions of instability by EMRA are supported by the lower productivity in batch experimental tests. The EMRA method incorporates properties of network structure, including stoichiometry and kinetic form, but does not require specific parameter values of the enzymes. C1 [Theisen, Matthew K.; Liao, James C.] Univ Calif Los Angeles, Dept Bioengn, Los Angeles, CA USA. [Theisen, Matthew K.; Rivera, Jimmy G. Lafontaine; Liao, James C.] Univ Calif Los Angeles, Dept Chem & Biomol Engn, Los Angeles, CA USA. [Liao, James C.] Univ Calif Los Angeles, UCLA DOE Inst, Los Angeles, CA USA. RP Liao, JC (reprint author), Univ Calif Los Angeles, Dept Bioengn, Los Angeles, CA USA.; Liao, JC (reprint author), Univ Calif Los Angeles, Dept Chem & Biomol Engn, Los Angeles, CA USA.; Liao, JC (reprint author), Univ Calif Los Angeles, UCLA DOE Inst, Los Angeles, CA USA. EM liaoj@ucla.edu FU National Science Foundation [MCB-1139318]; UCLA-DOE Institute for Genomics and Proteomics; U.S. Department of Energy Office of Science Biological and Environmental Research Program [DE-SC0012384, DE-SC0001060, DE-SC0008744] FX This work was supported by National Science Foundation (MCB-1139318) (www.nsf.gov), UCLA-DOE Institute for Genomics and Proteomics (http://www.doe-mbi.ucla.edu/), and the U.S. Department of Energy Office of Science Biological and Environmental Research Program (http://science.energy.gov/ber/)), (DE-SC0012384, DE-SC0001060 and DE-SC0008744). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 34 TC 1 Z9 1 U1 3 U2 4 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1553-734X EI 1553-7358 J9 PLOS COMPUT BIOL JI PLoS Comput. Biol. PD MAR PY 2016 VL 12 IS 3 AR e1004800 DI 10.1371/journal.pcbi.1004800 PG 18 WC Biochemical Research Methods; Mathematical & Computational Biology SC Biochemistry & Molecular Biology; Mathematical & Computational Biology GA DM8AU UT WOS:000376583800043 PM 26963521 ER PT J AU Shuryak, I Sun, YP Balajee, AS AF Shuryak, Igor Sun, Youping Balajee, Adayabalam S. TI Advantages of Binomial Likelihood Maximization for Analyzing and Modeling Cell Survival Curves SO RADIATION RESEARCH LA English DT Article ID RADIATION SENSITIVITY; HISTONE H2AX; V79 CELLS; PARAMETERS; INDUCTION; OXYGEN; DAMAGE; ASSAY AB Mathematical analysis of cell survival allows parameter estimation for radiobiological models and selection of an appropriate model. To our knowledge, no rigorous comparisons on the accuracy of various methods used for such analysis have been performed. In this study we compared three methods: 1. maximization of binomial log-likelihood (BLL); 2. minimization of sum of squares (SS); and 3. method 2 using log-transformed data (SS log). Analysis of Monte Carlo simulated data (A) generated from the linear-quadratic (LQ) model showed that model parameter estimates from the BLL method were more accurate and less affected by "noise" than those from other methods. Analysis of actual breast cancer cell data showed substantial differences among LQ parameters estimated by the three methods (B). To select among radiobiological models, we used: 1. Sample size-corrected Akaike information criterion (AICc), calculated from BLL method-generated log-likelihood values; and 2. Adjusted coefficient of determination (R-2), calculated from SS/SSlog method-generated SS values. Analysis of data simulated from the repair-misrepair (RMR) formalism (C) showed that the first approach outperformed the second approach at identifying the true data-generating model. Examples of how the first approach discriminates between several models were explored using actual mouse (H2AX-proficient and -deficient) and human [DNA-dependent protein kinase (DNA-PK)-proficient and -deficient] cell data (D). Based on this work, we concluded that BLL maximization combined with AICc-based model selection constitutes an effective method for analyzing cell survival data. (C) 2016 by Radiation Research Society C1 [Shuryak, Igor] Columbia Univ, Ctr Radiol Res, 630 West 168th St,VC-11-234-5, New York, NY 10032 USA. [Sun, Youping] Columbia Univ, Med Ctr, Dept Radiat Oncol, New York, NY 10032 USA. [Balajee, Adayabalam S.] Oak Ridge Inst Sci & Educ, Cytogenet Biodosimetry Lab, Radiat Emergency Assistance Ctr & Training Site, Oak Ridge, TN USA. RP Shuryak, I (reprint author), Columbia Univ, Ctr Radiol Res, 630 West 168th St,VC-11-234-5, New York, NY 10032 USA. EM is144@cumc.columbia.edu NR 29 TC 1 Z9 1 U1 0 U2 0 PU RADIATION RESEARCH SOC PI LAWRENCE PA 810 E TENTH STREET, LAWRENCE, KS 66044 USA SN 0033-7587 EI 1938-5404 J9 RADIAT RES JI Radiat. Res. PD MAR PY 2016 VL 185 IS 3 BP 246 EP 256 DI 10.1667/RR14195.1 PG 11 WC Biology; Biophysics; Radiology, Nuclear Medicine & Medical Imaging SC Life Sciences & Biomedicine - Other Topics; Biophysics; Radiology, Nuclear Medicine & Medical Imaging GA DN0KY UT WOS:000376754000004 PM 26930380 ER PT J AU Britten, RA Jewell, JS Miller, VD Davis, LK Hadley, MM Wyrobek, AJ AF Britten, Richard A. Jewell, Jessica S. Miller, Vania D. Davis, Leslie K. Hadley, Melissa M. Wyrobek, Andrew J. TI Impaired Spatial Memory Performance in Adult Wistar Rats Exposed to Low (5-20 cGy) Doses of 1 GeV/n Fe-56 Particles SO RADIATION RESEARCH LA English DT Article ID MOUSE HIPPOCAMPUS; OXIDATIVE STRESS; RADIATION; LIPOPOLYSACCHARIDE; IRRADIATION; DEFICITS AB Prolonged deep space missions to planets and asteroids will expose astronauts to galactic cosmic radiation, comprised of low-linear energy transfer (LET) ionizing radiations, high-energy protons and high-Z and energy (HZE) particles, such as Fe-56 nuclei. In prior studies with rodents exposed to HZE particle radiation at doses likely to be encountered during deep space missions (<20 cGy) investigators reported impaired hippocampal-dependent neurocognitive performance and further observed substantial variation among the irradiated animals in neurocognitive impairment, ranging from no observable effects to severe impairment. These findings point to the importance of incorporating quantitative measures of interindividual variations into next generation risk assessment models of radiation risks on neurocognition. In this study, 269 male proven breeder Wistar rats were exposed to 1 GeV/n Fe-56 at doses of 0, 5, 10, 15 and 20 cGy, and tested for spatial memory performance on the Barnes maze at three months after exposure. The radiation response data were compared using changes in mean cohort performance and by the proportion of poor responders using the performance benchmark of two standard deviations below the mean value among the sham-irradiated cohort. Acute exposures to mission-relevant doses of 1 GeV/n Fe-56 reduced the mean spatial memory performance at three months after exposure (P < 0.002) and increased the proportions of poor performers, 2- to 3-fold. However, a substantial fraction of animals in all exposure cohorts showed no detectable change in performance, compared to the distribution of sham-irradiated animals. Our findings suggest that individualized metrics of susceptibility or resistance to radiation-induce changes in neurocognitive performance will be advantageous to the development of probabilistic risk assessment models for HZE-induced neurocognitive impairment. (C) 2016 by Radiation Research Society C1 [Britten, Richard A.; Jewell, Jessica S.; Miller, Vania D.; Davis, Leslie K.; Hadley, Melissa M.] Eastern Virginia Med Sch, Dept Radiat Oncol, 700 W Olney Rd,Lewis Hall, Norfolk, VA 23507 USA. [Britten, Richard A.] Eastern Virginia Med Sch, Dept Microbiol, Norfolk, VA 23507 USA. [Britten, Richard A.] Eastern Virginia Med Sch, Leroy T Canoles Jr Canc Ctr, Norfolk, VA 23507 USA. [Wyrobek, Andrew J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Syst & Engn Div, Berkeley, CA 94720 USA. RP Britten, RA (reprint author), Eastern Virginia Med Sch, Dept Radiat Oncol, 700 W Olney Rd,Lewis Hall, Norfolk, VA 23507 USA. EM brittera@evms.edu FU National Aeronautics and Space Administration (NASA) [NNJ06HD89D, NNX11AC56G, NNX14AE73G]; NASA [NNJ14HP06I] FX This work was funded by the National Aeronautics and Space Administration (NASA grant nos. NNJ06HD89D, NNX11AC56G and NNX14AE73G). The authors are indebted to Dr. Adam Rusek for his help with the rat irradiations at Brookhaven National Laboratories, this study would not have been possible without his help. We also thank Jian-Hua Mao of the Lawrence Berkeley National Laboratory for statistical discussions. The contribution of AJW to this work was supported by NASA grant no. NNJ14HP06I. NR 18 TC 5 Z9 5 U1 1 U2 2 PU RADIATION RESEARCH SOC PI LAWRENCE PA 810 E TENTH STREET, LAWRENCE, KS 66044 USA SN 0033-7587 EI 1938-5404 J9 RADIAT RES JI Radiat. Res. PD MAR PY 2016 VL 185 IS 3 BP 332 EP 337 DI 10.1667/RR14120.1 PG 6 WC Biology; Biophysics; Radiology, Nuclear Medicine & Medical Imaging SC Life Sciences & Biomedicine - Other Topics; Biophysics; Radiology, Nuclear Medicine & Medical Imaging GA DN0KY UT WOS:000376754000011 PM 26943453 ER PT J AU Basmanov, OL Kiryukhin, AV Maguskin, MA Dvigalo, VN Rutqvist, J AF Basmanov, O. L. Kiryukhin, A. V. Maguskin, M. A. Dvigalo, V. N. Rutqvist, J. TI Thermo-hydrogeomechanical modeling of vertical ground deformation during the operation of the Mutnovskii Geothermal Field SO JOURNAL OF VOLCANOLOGY AND SEISMOLOGY LA English DT Article ID KAMCHATKA AB Vertical ground displacements at the Mutnovskii Geothermal Field were measured annually during the 2004-2013 period using a network of borehole markers. Three areas have been identified where the vertical displacements were different in character. Positive vertical deformation (2-5 mm/yr) was recorded in the middle of the Dachnyi Area in 2005-2006, giving way to a later stabilization. The North Test Area where the exhaust heat carrier was reinjected did not show any substantial deformation during the 2003-2006 period. This was followed by an uplift in 2006-2008 (6-7 mm/yr) and then by a subsidence (5-8 mm/yr) in 2009-2013. No vertical deformation worth mentioning was recorded in the Verkhne-Mutnovskii Area prior to 2008, but a rapid subsidence began at a rate of 6-18 mm/yr after 2008. We used the TOUGH-FLAC software to analyze vertical ground deformation. This program is used to perform thermo-hydrogeomechanical (THM) modeling based on the previous TOUGH2 model. THM modeling can explain relative vertical deformation during the exploitation of the Mutnovskii Geothermal Field by separating the geothermal field into two compartments by the Osnovnoi fault, as the two have different tectonic settings and petrophysical properties. C1 [Basmanov, O. L.] OAO Geoterm, Ul Ak Koroleva 60, Petropavlovsk Kamchatski 683009, Russia. [Kiryukhin, A. V.; Maguskin, M. A.; Dvigalo, V. N.] Russian Acad Sci, Far East Branch, Inst Volcanol & Seismol, Bulvar Piipa 9, Petropavlovsk Kamchatski 683006, Russia. [Rutqvist, J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Kiryukhin, AV (reprint author), Russian Acad Sci, Far East Branch, Inst Volcanol & Seismol, Bulvar Piipa 9, Petropavlovsk Kamchatski 683006, Russia. EM AVKiryukhin2@mail.ru RI Rutqvist, Jonny/F-4957-2015; Kiryukhin, Alexey/Q-3615-2016 OI Rutqvist, Jonny/0000-0002-7949-9785; FU Russian Foundation for Basic Research [12-05-00125]; Far East Branch of the Russian Academy of Sciences [12-III-A-08-170, 12-I-P27-04] FX This work was supported by the Russian Foundation for Basic Research, project no. 12-05-00125 and by the Far East Branch of the Russian Academy of Sciences, project nos. 12-III-A-08-170 and 12-I-P27-04. NR 21 TC 0 Z9 0 U1 3 U2 3 PU MAIK NAUKA/INTERPERIODICA/SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013-1578 USA SN 0742-0463 EI 1819-7108 J9 J VOLCANOL SEISMOL+ JI J. Volcanol. Seismol. PD MAR PY 2016 VL 10 IS 2 BP 138 EP 149 DI 10.1134/S0742046316020032 PG 12 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DM5XN UT WOS:000376424000006 ER PT J AU Long, W Jung, KW Yang, ZQ Copping, A Deng, ZD AF Long, Wen Jung, Ki Won Yang, Zhaoqing Copping, Andrea Deng, Z. Daniel TI Coupled Modeling of Hydrodynamics and Sound in Coastal Ocean for Renewable Ocean Energy Development SO MARINE TECHNOLOGY SOCIETY JOURNAL LA English DT Article; Proceedings Paper CT OCEANS MTS/IEEE Conference CY OCT 19-22, 2015 CL Washington, DC SP MTS, IEEE DE Sound; coastal ocean; ranewable; ocean coupling; Helmholtz; equation ID NONSYMMETRIC LINEAR-SYSTEMS; UNDERWATER NOISE; PROPAGATION; EQUATION AB The rapid growth of renewable offshore energy development has raised concerns that underwater noise from construction and operation of offshore devices may interfere with communication of marine animals. An underwater sound model was developed to simulate sound propagation from marine and hydrokinetic energy (MHK) devices or offshore wind (OSW) energy platforms. Finite difference methods were developed to solve the 3-D Helmholtz equation for sound propagation in the coastal environment. A 3-D sparse matrix solver with complex coefficients was formed for solving the resulting acoustic pressure field. The complex shifted Laplacian preconditioner (CSLP) method was applied to solve the matrix system iteratively with Message Passing Interface (MPI) parallelization using a high-performance cluster. The sound model was then coupled with the Finite Volume Community Ocean Model (FVCOM) for simulating sound propagation generated by human activities, such as construction of OSW turbines or tidal stream turbine operations, in a range-dependent setting. As a proof of concept, the validation of the solver is tested with an ideal case against two other methods, and its application is then presented for two coastal wedge problems. This sound model can be useful for evaluating impacts on marine mammals due to deployment of MHK devices and OSW energy platforms. C1 [Long, Wen; Jung, Ki Won; Yang, Zhaoqing; Copping, Andrea; Deng, Z. Daniel] Pacific NW Natl Lab, POB 999, Richland, WA 99352 USA. RP Jung, KW (reprint author), Pacific NW Natl Lab, POB 999, Richland, WA 99352 USA. EM KiWon.Jung@pnnl.gov RI Deng, Daniel/A-9536-2011; OI Deng, Daniel/0000-0002-8300-8766; Jung, Ki Won/0000-0001-9847-3532 NR 27 TC 0 Z9 0 U1 3 U2 7 PU MARINE TECHNOLOGY SOC INC PI COLUMBIA PA 5565 STERRETT PLACE, STE 108, COLUMBIA, MD 21044 USA SN 0025-3324 EI 1948-1209 J9 MAR TECHNOL SOC J JI Mar. Technol. Soc. J. PD MAR-APR PY 2016 VL 50 IS 2 BP 27 EP 36 PG 10 WC Engineering, Ocean; Oceanography SC Engineering; Oceanography GA DL8MS UT WOS:000375896700004 ER PT J AU Albright, BJ Yin, L Bowers, KJ Bergen, B AF Albright, B. J. Yin, L. Bowers, K. J. Bergen, B. TI Multi-dimensional dynamics of stimulated Brillouin scattering in a laser speckle: Ion acoustic wave bowing, breakup, and laser-seeded two-ion-wave decay SO PHYSICS OF PLASMAS LA English DT Article ID PLASMA; BACKSCATTER; SUPPRESSION; BEAMS AB Two- and three-dimensional particle-in-cell simulations of stimulated Brillouin scattering (SBS) in laser speckle geometry have been analyzed to evaluate the relative importance of competing nonlinear processes in the evolution and saturation of SBS. It is found that ion-trapping-induced wavefront bowing and breakup of ion acoustic waves (IAW) and the associated side-loss of trapped ions dominate electron-trapping-induced IAW wavefront bowing and breakup, as well as the two-ion-wave decay instability over a range of ZT(e)/T-i conditions and incident laser intensities. In the simulations, the latter instability does not govern the nonlinear saturation of SBS; however, evidence of two-ion-wave decay is seen, appearing as a modulation of the ion acoustic wavefronts. This modulation is periodic in the laser polarization plane, anti-symmetric across the speckle axis, and of a wavenumber matching that of the incident laser pulse. A simple analytic model is provided for how spatial "imprinting" from a high frequency inhomogeneity (in this case, the density modulation from the laser) in an unstable system with continuum eigenmodes can selectively amplify modes with wavenumbers that match that of the inhomogeneity. (C) 2016 Author(s). C1 [Albright, B. J.; Yin, L.; Bowers, K. J.; Bergen, B.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Albright, BJ (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. OI Albright, Brian/0000-0002-7789-6525; Yin, Lin/0000-0002-8978-5320 FU U.S. Department of Energy by the Los Alamos National Security, LLC Los Alamos National Laboratory [DE-AC52-06NA25396]; U.S. Department of Energy Office of Science, Fusion Energy Sciences project FX Work performed under the auspices of the U.S. Department of Energy by the Los Alamos National Security, LLC Los Alamos National Laboratory under contract DE-AC52-06NA25396. This work was supported by a U.S. Department of Energy Office of Science, Fusion Energy Sciences project. Computing time on the Cielo machine was provided by Capability Class Computing. The authors wish to acknowledge useful discussions with Richard Berger, Thomas Chapman, and David S. Montgomery. NR 30 TC 2 Z9 2 U1 2 U2 3 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAR PY 2016 VL 23 IS 3 AR 032703 DI 10.1063/1.4943102 PG 9 WC Physics, Fluids & Plasmas SC Physics GA DL7XY UT WOS:000375854900054 ER PT J AU Andriyash, IA Lehe, R Lifschitz, A AF Andriyash, Igor A. Lehe, Remi Lifschitz, Agustin TI Laser-plasma interactions with a Fourier-Bessel particle-in-cell method SO PHYSICS OF PLASMAS LA English DT Article ID SIMULATIONS; IMPLEMENTATION; ACCELERATION; PROPAGATION; COMPUTATION; WAKEFIELD; ALGORITHM; SCHEME AB A new spectral particle-in-cell (PIC) method for plasma modeling is presented and discussed. In the proposed scheme, the Fourier-Bessel transform is used to translate the Maxwell equations to the quasi-cylindrical spectral domain. In this domain, the equations are solved analytically in time, and the spatial derivatives are approximated with high accuracy. In contrast to the finite-difference time domain (FDTD) methods, that are used commonly in PIC, the developed method does not produce numerical dispersion and does not involve grid staggering for the electric and magnetic fields. These features are especially valuable in modeling the wakefield acceleration of particles in plasmas. The proposed algorithm is implemented in the code PLARES-PIC, and the test simulations of laser plasma interactions are compared to the ones done with the quasi-cylindrical FDTD PIC code CALDER-CIRC. (C) 2016 AIP Publishing LLC. C1 [Andriyash, Igor A.] Synchrotron SOLEIL, Lorme Merisiers, F-91192 Gif Sur Yvette, France. [Andriyash, Igor A.; Lifschitz, Agustin] Univ Paris Saclay, Ecole polytech, CNRS, LOA,ENSTA ParisTech, 828 Bd Marechaux, F-91762 Palaiseau, France. [Lehe, Remi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Andriyash, IA (reprint author), Synchrotron SOLEIL, Lorme Merisiers, F-91192 Gif Sur Yvette, France.; Andriyash, IA (reprint author), Univ Paris Saclay, Ecole polytech, CNRS, LOA,ENSTA ParisTech, 828 Bd Marechaux, F-91762 Palaiseau, France. EM igor.andriyash@gmail.com FU ERC [339128, 340015] FX One of the authors (I. A. A.) acknowledges the support of Victor Malka and Marie-Emmanuelle Couprie and partial funding from their ERC programs X-Five (Contract No. 339128) and COXINEL (Contract No. 340015). NR 35 TC 1 Z9 1 U1 3 U2 4 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAR PY 2016 VL 23 IS 3 AR 033110 DI 10.1063/1.4943281 PG 8 WC Physics, Fluids & Plasmas SC Physics GA DL7XY UT WOS:000375854900069 ER PT J AU Banks, JW Brunner, S Berger, RL Tran, TM AF Banks, J. W. Brunner, S. Berger, R. L. Tran, T. M. TI Vlasov simulations of electron-ion collision effects on damping of electron plasma waves SO PHYSICS OF PLASMAS LA English DT Article ID HEAT-TRANSPORT; COULOMB COLLISIONS; ACOUSTIC-WAVES; MODEL; DISTRIBUTIONS; OSCILLATIONS; FREQUENCY; EQUATIONS; ECHOES AB Collisional effects can play an essential role in the dynamics of plasma waves by setting a minimum damping rate and by interfering with wave-particle resonances. Kinetic simulations of the effects of electron-ion pitch angle scattering on Electron Plasma Waves (EPWs) are presented here. In particular, the effects of such collisions on the frequency and damping of small-amplitude EPWs for a range of collision rates and wave phase velocities are computed and compared with theory. Both the Vlasov simulations and linear kinetic theory find the direct contribution of electron-ion collisions to wave damping significantly reduced from that obtained through linearized fluid theory. To our knowledge, this simple result has not been published before. Simulations have been carried out using a grid-based (Vlasov) approach, based on a high-order conservative finite difference method for discretizing the Fokker-Planck equation describing the evolution of the electron distribution function. Details of the implementation of the collision operator within this framework are presented. Such a grid-based approach, which is not subject to numerical noise, is of particular interest for the accurate measurements of the wave damping rates. (C) 2016 AIP Publishing LLC. C1 [Banks, J. W.] Rensselaer Polytech Inst, Dept Math Sci, Troy, NY 12180 USA. [Brunner, S.; Tran, T. M.] Ecole Polytech Fed Lausanne, Swiss Plasma Ctr, CH-1015 Lausanne, Switzerland. [Berger, R. L.] Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94551 USA. RP Banks, JW (reprint author), Rensselaer Polytech Inst, Dept Math Sci, Troy, NY 12180 USA. EM banksj3@rpi.edu RI Banks, Jeffrey/A-9718-2012 FU Laboratory Research and Development Program at LLNL [12-ERD-061, 15-ERD-038]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We are pleased to acknowledge valuable discussions with T. Chapman and B. I. Cohen. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344 and funded by the Laboratory Research and Development Program at LLNL under Project Tracking Code Nos. 12-ERD-061 and 15-ERD-038. Computing support for this work came from the Lawrence Livermore National Laboratory (LLNL) Institutional Computing Grand Challenge program. NR 43 TC 0 Z9 0 U1 5 U2 11 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAR PY 2016 VL 23 IS 3 AR 032108 DI 10.1063/1.4943194 PG 18 WC Physics, Fluids & Plasmas SC Physics GA DL7XY UT WOS:000375854900010 ER PT J AU Comisso, L Grasso, D AF Comisso, Luca Grasso, Daniela TI Visco-resistive plasmoid instability SO PHYSICS OF PLASMAS LA English DT Article ID TEARING MODE; MAGNETIC RECONNECTION; CURRENT SHEETS; NONLINEAR GROWTH; TRANSITION; FIELDS; PINCH AB The plasmoid instability in visco-resistive current sheets is analyzed in both the linear and nonlinear regimes. The linear growth rate and the wavenumber are found to scale as S-1/4(1 + P-m)(-5/8) and S-3/8(1 + P-m)(-3/16) with respect to the Lundquist number S and the magnetic Prandtl number P-m. Furthermore, the linear layer width is shown to scale as S-1/8(1 + P-m)(1/16). The growth of the plasmoids slows down from an exponential growth to an algebraic growth when they enter into the nonlinear regime. In particular, the time-scale of the nonlinear growth of the plasmoids is found to be tau(NL) similar to S-3/16(1 + P-m)(19/32) tau(A,L). The nonlinear growth of the plasmoids is radically different from the linear one, and it is shown to be essential to understand the global current sheet disruption. It is also discussed how the plasmoid instability enables fast magnetic reconnection in viscoresistive plasmas. In particular, it is shown that the recursive plasmoid formation can trigger a collisionless reconnection regime if S greater than or similar to L-cs(epsilon(c)l(k))(-1) (1 + P-m)(1/2), where L-cs is the half-length of the global current sheet and l(k) is the relevant kinetic length scale. On the other hand, if the current sheet remains in the collisional regime, the global ( time-averaged) reconnection rate is shown to be < d psi/dt vertical bar(X)> approximate to epsilon(c)v(A,u)B(u)(1 + P-m)(-1/2), where epsilon(c) is the critical inverse aspect ratio of the current sheet, while v(A,u) and Bu are the Alfven speed and the magnetic field upstream of the global reconnection layer. (C) 2016 AIP Publishing LLC. C1 [Comisso, Luca] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA. [Comisso, Luca] Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08544 USA. [Comisso, Luca; Grasso, Daniela] Politecn Torino, Ist Sistemi Complessi CNR, I-10129 Turin, Italy. [Comisso, Luca; Grasso, Daniela] Politecn Torino, Dipartimento Energia, I-10129 Turin, Italy. RP Comisso, L (reprint author), Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA.; Comisso, L (reprint author), Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08544 USA.; Comisso, L (reprint author), Politecn Torino, Ist Sistemi Complessi CNR, I-10129 Turin, Italy.; Comisso, L (reprint author), Politecn Torino, Dipartimento Energia, I-10129 Turin, Italy. EM lcomisso@princeton.edu OI Comisso, Luca/0000-0001-8822-8031; grasso, daniela/0000-0001-7522-3805 FU Euratom; ENEA FX We benefited from stimulating discussions with Amitava Bhattacharjee, Yi-Min Huang, Manasvi Lingam, Nuno F. Loureiro, and Francois L. Waelbroeck. We acknowledge financial support from the European Community under the contracts of Association between Euratom and ENEA. NR 69 TC 4 Z9 4 U1 4 U2 4 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAR PY 2016 VL 23 IS 3 AR 032111 DI 10.1063/1.4942940 PG 9 WC Physics, Fluids & Plasmas SC Physics GA DL7XY UT WOS:000375854900013 ER PT J AU Daligault, J AF Daligault, Jerome TI On the quantum Landau collision operator and electron collisions in dense plasmas SO PHYSICS OF PLASMAS LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; FOKKER-PLANCK EQUATION; PARTICLE SIMULATION; THERMAL CONDUCTION; KINETIC-EQUATION; TRANSPORT; SCHEME AB The quantum Landau collision operator, which extends the widely used Landau/Fokker-Planck collision operator to include quantum statistical effects, is discussed. The quantum extension can serve as a reference model for including electron collisions in non-equilibrium dense plasmas, in which the quantum nature of electrons cannot be neglected. In this paper, the properties of the Landau collision operator that have been useful in traditional plasma kinetic theory and plasma transport theory are extended to the quantum case. We outline basic properties in connection with the conservation laws, the H-theorem, and the global and local equilibrium distributions. We discuss the Fokker-Planck form of the operator in terms of three potentials that extend the usual two Rosenbluth potentials. We establish practical closed-form expressions for these potentials under local thermal equilibrium conditions in terms of Fermi-Dirac and Bose-Einstein integrals. We study the properties of linearized quantum Landau operator, and extend two popular approximations used in plasma physics to include collisions in kinetic simulations. We apply the quantum Landau operator to the classic test-particle problem to illustrate the physical effects embodied in the quantum extension. We present useful closed-form expressions for the electron-ion momentum and energy transfer rates. Throughout the paper, similarities and differences between the quantum and classical Landau collision operators are emphasized. (C) 2016 AIP Publishing LLC. C1 [Daligault, Jerome] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Daligault, J (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM daligaul@lanl.gov FU United States Department of Energy [DE-AC52-06NA25396]; DOE Office of Fusion Energy Sciences; LDRD grant at Los Alamos National Laboratory FX This work was performed under the auspices of the United States Department of Energy under Contract No. DE-AC52-06NA25396. This research was supported by the DOE Office of Fusion Energy Sciences, and by an LDRD grant at Los Alamos National Laboratory. NR 43 TC 1 Z9 1 U1 3 U2 4 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAR PY 2016 VL 23 IS 3 AR 032706 DI 10.1063/1.4944392 PG 22 WC Physics, Fluids & Plasmas SC Physics GA DL7XY UT WOS:000375854900057 ER PT J AU Fu, XR Cowee, MM Gary, SP Winske, D AF Fu, Xiangrong Cowee, Misa M. Gary, S. Peter Winske, Dan TI On the generation of double layers from ion- and electron-acoustic instabilities SO PHYSICS OF PLASMAS LA English DT Article ID WEAK DOUBLE-LAYERS; FIELD STRUCTURES; AURORAL CAVITY; SIMULATION; EVOLUTION; REGION; EARTHS; WAVES AB A plasma double layer (DL) is a nonlinear electrostatic structure that carries a uni-polar electric field parallel to the background magnetic field due to local charge separation. Past studies showed that DLs observed in space plasmas are mostly associated with the ion acoustic instability. Recent Van Allen Probes observations of parallel electric field structures traveling much faster than the ion acoustic speed have motivated a computational study to test the hypothesis that a new type of DLs-electron acoustic DLs-generated from the electron acoustic instability are responsible for these electric fields. Nonlinear particle-in-cell simulations yield negative results, i.e., the hypothetical electron acoustic DLs cannot be formed in a way similar to ion acoustic DLs. Linear theory analysis and the simulations show that the frequencies of electron acoustic waves are too high for ions to respond and maintain charge separation required by DLs. However, our results do show that local density perturbations in a two-electron-component plasma can result in unipolar-like electric field structures that propagate at the electron thermal speed, suggesting another potential explanation for the observations. (C) 2016 AIP Publishing LLC. C1 [Fu, Xiangrong; Cowee, Misa M.; Winske, Dan] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. [Gary, S. Peter] Space Sci Inst, Boulder, CO 80301 USA. RP Fu, XR (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM xrfu@lanl.gov FU U.S. Department of Energy - LANL IGPPS mini-grant; U.S. Department of Energy National Nuclear Security Administration [DE-AC52-06NA25396]; National Science Foundation [1303300] FX The Los Alamos portion of this research was performed under the auspices of the U.S. Department of Energy, supported by LANL IGPPS mini-grant. This research used resources provided by the Los Alamos National Laboratory Institutional Computing Program, which was supported by the U.S. Department of Energy National Nuclear Security Administration under Contract No. DE-AC52-06NA25396. S.P.G.'s contribution to this research was supported by the National Science Foundation GEM project 1303300. NR 32 TC 0 Z9 0 U1 1 U2 1 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAR PY 2016 VL 23 IS 3 AR 032308 DI 10.1063/1.4943881 PG 8 WC Physics, Fluids & Plasmas SC Physics GA DL7XY UT WOS:000375854900038 ER PT J AU Gueroult, R Fisch, NJ AF Gueroult, Renaud Fisch, Nathaniel J. TI Practicality of magnetic compression for plasma density control SO PHYSICS OF PLASMAS LA English DT Article ID MAGNETOSONIC SHOCK-WAVE; RESONANT ION-ACCELERATION; COLLISION-FREE PLASMA; LARGE-AMPLITUDE; HYDROMAGNETIC WAVES; THETA-PINCH; OSCILLATIONS; FIELD; MODEL AB Plasma densification through magnetic compression has been suggested for time-resolved control of the wave properties in plasma-based accelerators [P. F. Schmit and N. J. Fisch, Phys. Rev. Lett. 109, 255003 (2012)]. Using particle in cell simulations with real mass ratio, the practicality of large magnetic compression on timescales shorter than the ion gyro-period is investigated. For compression times shorter than the transit time of a compressional Alfven wave across the plasma slab, results show the formation of two counter-propagating shock waves, leading to a highly non-uniform plasma density profile. Furthermore, the plasma slab displays large hydromagnetic like oscillations after the driving field has reached steady state. Peak compression is obtained when the two shocks collide in the mid-plane. At this instant, very large plasma heating is observed, and the plasma beta is estimated to be about 1. Although these results point out a densification mechanism quite different and more complex than initially envisioned, these features still might be advantageous in particle accelerators. (C) 2016 AIP Publishing LLC. C1 [Gueroult, Renaud; Fisch, Nathaniel J.] Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. RP Gueroult, R (reprint author), Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. OI Fisch, Nathaniel/0000-0002-0301-7380 FU DTRA [HDTRA1-11-1-0037]; DOE [67350-9960, DOE DE-NA0001836] FX This work was supported by DTRA Grant No. HDTRA1-11-1-0037 and DOE Grant No. 67350-9960 (Prime No. DOE DE-NA0001836). NR 28 TC 2 Z9 2 U1 0 U2 1 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAR PY 2016 VL 23 IS 3 AR 032113 DI 10.1063/1.4943877 PG 8 WC Physics, Fluids & Plasmas SC Physics GA DL7XY UT WOS:000375854900015 ER PT J AU Hu, D Qin, H AF Hu, Di Qin, Hong TI On the inward drift of runaway electrons during the plateau phase of runaway current SO PHYSICS OF PLASMAS LA English DT Article ID MOMENTUM-SPACE; DISRUPTIONS; GENERATION; AVALANCHE; TRANSPORT; JET AB The well observed inward drift of current carrying runaway electrons during runaway plateau phase after disruption is studied by considering the phase space dynamic of runaways in a large aspect ratio toroidal system. We consider the case where the toroidal field is unperturbed and the toroidal symmetry of the system is preserved. The balance between the change in canonical angular momentum and the input of mechanical angular momentum in such a system requires runaways to drift horizontally in configuration space for any given change in momentum space. The dynamic of this drift can be obtained by integrating the modified Euler-Lagrange equation over one bounce time. It is then found that runaway electrons will always drift inward as long as they are decelerating. This drift motion is essentially non-linear, since the current is carried by runaways themselves, and any runaway drift relative to the magnetic axis will cause further displacement of the axis itself. A simplified analytical model is constructed to describe such inward drift both in the ideal wall case and no wall case, and the runaway current center displacement as a function of parallel momentum variation is obtained. The time scale of such displacement is estimated by considering effective radiation drag, which shows reasonable agreement with the observed displacement time scale. This indicates that the phase space dynamic studied here plays a major role in the horizontal displacement of runaway electrons during plateau phase. (C) 2016 AIP Publishing LLC. C1 [Hu, Di] Peking Univ, Sch Phys, Beijing 100871, Peoples R China. [Qin, Hong] Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08540 USA. [Qin, Hong] Univ Sci & Technol China, Sch Nucl Sci & Technol, Hefei 230026, Peoples R China. [Qin, Hong] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Peoples R China. RP Hu, D (reprint author), Peking Univ, Sch Phys, Beijing 100871, Peoples R China.; Hu, D (reprint author), PPPL, Princeton, NJ 08540 USA. EM hudi_2@pku.edu.cn FU National Magnetic Confinement Fusion Energy Research Project [2015GB111003]; National Natural Science Foundation of China [1126114032, 11575185, 11575186, 11305171]; JSPS-NRF-NSFC [11261140328]; China Scholarship Council; U.S. DoE [AC02-09-CH11466] FX The authors thank C. Liu, X.-G. Wang, and A. Bhattacharjee for fruitful discussion. The authors also thank an anonymous referee for constructive comments. This work was partially supported by National Magnetic Confinement Fusion Energy Research Project under Grant No. 2015GB111003, National Natural Science Foundation of China under Grant Nos. 1126114032, 11575185, 11575186, and 11305171, JSPS-NRF-NSFC A3 Foresight Program under Grant No. 11261140328, the China Scholarship Council, and U.S. DoE Contract No. AC02-09-CH11466. NR 27 TC 0 Z9 0 U1 4 U2 5 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAR PY 2016 VL 23 IS 3 AR 032510 DI 10.1063/1.4944934 PG 11 WC Physics, Fluids & Plasmas SC Physics GA DL7XY UT WOS:000375854900050 ER PT J AU Koliner, JJ Cianciosa, MR Boguski, J Anderson, JK Hanson, JD Chapman, BE Brower, DL Den Hartog, DJ Ding, WX Duff, JR Goetz, JA McGarry, M Morton, LA Parke, E AF Koliner, J. J. Cianciosa, M. R. Boguski, J. Anderson, J. K. Hanson, J. D. Chapman, B. E. Brower, D. L. Den Hartog, D. J. Ding, W. X. Duff, J. R. Goetz, J. A. McGarry, M. Morton, L. A. Parke, E. TI Three dimensional equilibrium solutions for a current-carrying reversed-field pinch plasma with a close-fitting conducting shell SO PHYSICS OF PLASMAS LA English DT Article ID MADISON SYMMETRIC TORUS; SINGLE HELICITY; INJECTION; PARADIGM; PELLET AB In order to characterize the Madison Symmetric Torus (MST) reversed-field pinch (RFP) plasmas that bifurcate to a helical equilibrium, the V3FIT equilibrium reconstruction code was modified to include a conducting boundary. RFP plasmas become helical at a high plasma current, which induces large eddy currents in MST's thick aluminum shell. The V3FIT conducting boundary accounts for the contribution from these eddy currents to external magnetic diagnostic coil signals. This implementation of V3FIT was benchmarked against MSTFit, a 2D Grad-Shafranov solver, for axisymmetric plasmas. The two codes both fit B-theta measurement loops around the plasma minor diameter with qualitative agreement between each other and the measured field. Fits in the 3D case converge well, with q-profile and plasma shape agreement between two distinct toroidal locking phases. Greater than 60% of the measured n = 5 component of B-theta at r = a is due to eddy currents in the shell, as calculated by the conducting boundary model. (C) 2016 AIP Publishing LLC. C1 [Koliner, J. J.; Boguski, J.; Anderson, J. K.; Chapman, B. E.; Den Hartog, D. J.; Duff, J. R.; Goetz, J. A.; McGarry, M.; Morton, L. A.; Parke, E.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Cianciosa, M. R.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Hanson, J. D.] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. [Brower, D. L.; Ding, W. X.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. RP Boguski, J (reprint author), Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. EM boguski@wisc.edu FU U.S. Department of Energy Office of Science, Office of Fusion Energy Sciences program [DE-FC02-05ER54814] FX We would like to thank K. J. McCollam and M. D. Nornberg for their careful review of the manuscript. MST data shown in this paper can be obtained in digital format (supplementary material).37 This material is based upon work supported by the U.S. Department of Energy Office of Science, Office of Fusion Energy Sciences program under Award No. DE-FC02-05ER54814. NR 36 TC 0 Z9 0 U1 0 U2 0 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAR PY 2016 VL 23 IS 3 AR 032508 DI 10.1063/1.4944670 PG 8 WC Physics, Fluids & Plasmas SC Physics GA DL7XY UT WOS:000375854900048 ER PT J AU Le, A Daughton, W Karimabadi, H Egedal, J AF Le, A. Daughton, W. Karimabadi, H. Egedal, J. TI Hybrid simulations of magnetic reconnection with kinetic ions and fluid electron pressure anisotropy SO PHYSICS OF PLASMAS LA English DT Article ID COLLISIONLESS RECONNECTION; MAGNETOTAIL RECONNECTION; LINE AB We present the first hybrid simulations with kinetic ions and recently developed equations of state for the electron fluid appropriate for reconnection with a guide field. The equations of state account for the main anisotropy of the electron pressure tensor. Magnetic reconnection is studied in two systems, an initially force-free current sheet and a Harris sheet. The hybrid model with the equations of state is compared to two other models, hybrid simulations with isothermal electrons and fully kinetic simulations. Including the anisotropic equations of state in the hybrid model provides a better match to the fully kinetic model. In agreement with fully kinetic results, the main feature captured is the formation of an electron current sheet that extends several ion inertial lengths. This electron current sheet modifies the Hall magnetic field structure near the X-line, and it is not observed in the standard hybrid model with isotropic electrons. The saturated reconnection rate in this regime nevertheless remains similar in all three models. Implications for global modeling are discussed. (C) 2016 AIP Publishing LLC. C1 [Le, A.; Daughton, W.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Karimabadi, H.] CureMetrix, La Jolla, CA 92037 USA. [Egedal, J.] Univ Wisconsin, Madison, WI 53706 USA. RP Le, A (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RI Daughton, William/L-9661-2013 FU LDRD office at LANL; NASA's Heliophysics Theory Program; NSF GEM award [1405166]; NASA grant [NNX14AC68G] FX A.L. received support from the LDRD office at LANL. W.D.'s work was supported by NASA's Heliophysics Theory Program. J.E. acknowledges the support through NSF GEM award 1405166 and NASA grant NNX14AC68G. Simulations were performed on Pleiades provided by NASA's HEC Program, with LANL Institutional Computing resources, and on Mira provided by the ALCF at ANL. NR 38 TC 3 Z9 4 U1 2 U2 7 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAR PY 2016 VL 23 IS 3 AR 032114 DI 10.1063/1.4943893 PG 7 WC Physics, Fluids & Plasmas SC Physics GA DL7XY UT WOS:000375854900016 ER PT J AU Milovich, JL Dewald, EL Pak, A Michel, P Town, RPJ Bradley, DK Landen, O Edwards, MJ AF Milovich, J. L. Dewald, E. L. Pak, A. Michel, P. Town, R. P. J. Bradley, D. K. Landen, O. Edwards, M. J. TI Early-time radiation flux symmetry optimization and its effect on gas-filled hohlraum ignition targets on the National Ignition Facility SO PHYSICS OF PLASMAS LA English DT Article ID INERTIAL CONFINEMENT FUSION; DENSE-PLASMAS; PHYSICS BASIS; GAIN; BALL; SIMULATION; ASYMMETRY AB Achieving ignition on the National Ignition Facility (NIF) is tied to our ability to control and minimize deviations from sphericity of the capsule implosion. Low-mode asymmetries of the hot spot result from the combined effect of radiation drive asymmetries throughout the laser pulse and initial roughness on the capsule surface. In this paper, we report on simulations and experiments designed to assess, measure, and correct the drive asymmetries produced by the early-time (approximate to first 2 ns or "picket") period of the laser pulse. The drive asymmetry during the picket is commonly thought to introduce distortions in the hot-spot shape at ignition time. However, a more subtle effect not previously considered is that it also leads to an asymmetry in shock velocity and timing, thereby increasing the fuel adiabat and reducing the margin for ignition. It is shown via hydrodynamic simulations that minimizing this effect requires that the early-time asymmetry be kept below 7.5% in the second Legendre mode (P-2), thus keeping the loss of performance margin below approximate to 10% for a layered implosion. Asymmetries during the picket of the laser pulse are measured using the instantaneous self-emission of a high-Z re-emission sphere in place of an ignition capsule in a hohlraum with large azimuthal diagnostic windows. Three dimensional simulations using the code HYDRA (to capture the effect of non-azimuthal hohlraum features) coupled to a cross-beam energy transfer model [Michel et al., Phys. Plasmas 17, 056305 (2010)] are used to establish the surrogacy of the re-emit target and to assess the early-time drive symmetry. Calculations using this model exhibit the same sensitivity to variations in the relative input powers between the different cones of NIF beams as measured for the "Rev5" CH target [Haan et al., Phys Plasmas 18, 051001 (2011)] and reported by Dewald et al. [Phys. Rev. Lett. 111, 235001 (2013)]. The same methodology applied to recently improved implosions using different hohlraum geometries and picket powers show good agreement with experimental data. (C) 2016 AIP Publishing LLC. C1 [Milovich, J. L.; Dewald, E. L.; Pak, A.; Michel, P.; Town, R. P. J.; Bradley, D. K.; Landen, O.; Edwards, M. J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Milovich, JL (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM milovich1@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-A52-07NA27344] FX We are especially grateful to B. Chang for many insightful discussions. We also thank the NIF shape team for continued support and dedication to keep the diagnostic calibrated: R. Benedetti, N. Izumi, S. Glenn. We are especially indebted to the NIF operations, cryogenics, and targets teams for their efforts and long hours in preparing, fielding, and instrumenting all of the shots discussed here. Very special thanks go to P. Amendt and H. F. Robey for the careful reading of this manuscript. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-A52-07NA27344. NR 53 TC 0 Z9 0 U1 3 U2 5 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAR PY 2016 VL 23 IS 3 AR 032701 DI 10.1063/1.4941979 PG 15 WC Physics, Fluids & Plasmas SC Physics GA DL7XY UT WOS:000375854900052 ER PT J AU Seguin, FH Li, CK DeCiantis, JL Frenje, JA Rygg, JR Petrasso, RD Marshall, FJ Smalyuk, V Glebov, VY Knauer, JP Sangster, TC Kilkenny, JD Nikroo, A AF Seguin, F. H. Li, C. K. DeCiantis, J. L. Frenje, J. A. Rygg, J. R. Petrasso, R. D. Marshall, F. J. Smalyuk, V. Glebov, V. Yu. Knauer, J. P. Sangster, T. C. Kilkenny, J. D. Nikroo, A. TI Effects of fuel-capsule shimming and drive asymmetry on inertial-confinement-fusion symmetry and yield SO PHYSICS OF PLASMAS LA English DT Article ID OMEGA LASER SYSTEM; IMPLOSIONS; NOVA AB Three orthogonal proton emission imaging cameras were used to study the 3D effects of low-mode drive asymmetries and target asymmetries on nuclear burn symmetry and yield in direct-drive, inertial-confinement-fusion experiments. The fusion yield decreased quickly as the burn region became asymmetric due to either drive or capsule asymmetry. Measurements and analytic scaling are used to predict how intentionally asymmetric capsule shells could improve performance by compensating for drive asymmetry when it cannot be avoided (such as with indirect drive or with polar direct drive). (C) 2016 AIP Publishing LLC. C1 [Seguin, F. H.; Li, C. K.; DeCiantis, J. L.; Frenje, J. A.; Rygg, J. R.; Petrasso, R. D.] MIT, Plasma Sci & Fus Ctr, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Marshall, F. J.; Smalyuk, V.; Glebov, V. Yu.; Knauer, J. P.; Sangster, T. C.] Univ Rochester, Laser Energet Lab, 250 E River Rd, Rochester, NY 14623 USA. [Kilkenny, J. D.; Nikroo, A.] Gen Atom Co, San Diego, CA 92121 USA. [DeCiantis, J. L.] AREVA Inc, Lynchburg, VA 24503 USA. [Rygg, J. R.; Smalyuk, V.; Nikroo, A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Seguin, FH (reprint author), MIT, Plasma Sci & Fus Ctr, 77 Massachusetts Ave, Cambridge, MA 02139 USA. FU U.S. DOE [DE-NA0002726, DE-NA0002949] FX We thank the OMEGA staff for their help in making these experiments possible. The work described here was supported in part by U.S. DOE Grants Nos. DE-NA0002726 and DE-NA0002949. NR 24 TC 3 Z9 3 U1 1 U2 6 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAR PY 2016 VL 23 IS 3 AR 032705 DI 10.1063/1.4943883 PG 6 WC Physics, Fluids & Plasmas SC Physics GA DL7XY UT WOS:000375854900056 ER PT J AU Simakov, AN Molvig, K AF Simakov, Andrei N. Molvig, Kim TI Hydrodynamic description of an unmagnetized plasma with multiple ion species. I. General formulation SO PHYSICS OF PLASMAS LA English DT Article AB A generalization of the Braginskii ion fluid description [S. I. Braginskii, Sov. Phys. - JETP 6, 358 (1958)] to the case of an unmagnetized collisional plasma with multiple ion species is presented. An asymptotic expansion in the ion Knudsen number is used to derive the individual ion species continuity, as well as the total ion mass density, momentum, and energy evolution equations accurate through the second order. Expressions for the individual ion species drift velocities with respect to the center of mass reference frame, as well as for the total ion heat flux and viscosity, which are required to close the fluid equations, are evaluated in terms of the first-order corrections to the lowest order Maxwellian ion velocity distribution functions. A variational formulation for evaluating such corrections and its relation to the plasma entropy are presented. Employing trial functions for the corrections, written in terms of expansions in generalized Laguerre polynomials, and maximizing the resulting functionals produce two systems of linear equations (for "vector" and "tensor" portions of the corrections) for the expansion coefficients. A general matrix formulation of the linear systems as well as expressions for the resulting transport fluxes are presented in forms convenient for numerical implementation. The general formulation is employed in Paper II [A. N. Simakov and K. Molvig, Phys. Plasmas 23, 032116 (2016)] to evaluate the individual ion drift velocities and the total ion heat flux and viscosity for specific cases of two and three ion species plasmas. (C) 2016 AIP Publishing LLC. C1 [Simakov, Andrei N.; Molvig, Kim] Los Alamos Natl Lab, Computat Phys Div, Los Alamos, NM 87545 USA. RP Simakov, AN (reprint author), Los Alamos Natl Lab, Computat Phys Div, Los Alamos, NM 87545 USA. EM simakov@lanl.gov OI Simakov, Andrei/0000-0001-7064-9153 FU Thermonuclear Burn Initiative of the NNSA Advanced Scientific and Computing ASC) Program at Los Alamos National Laboratory; U.S. Department of Energy [DE-AC52-06NA25396] FX Work supported by the Thermonuclear Burn Initiative of the NNSA Advanced Scientific and Computing ASC) Program at Los Alamos National Laboratory, operated by Los Alamos National Security, LLC for the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. NR 24 TC 2 Z9 2 U1 0 U2 0 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAR PY 2016 VL 23 IS 3 AR 032115 DI 10.1063/1.4943894 PG 16 WC Physics, Fluids & Plasmas SC Physics GA DL7XY UT WOS:000375854900017 ER PT J AU Simakov, AN Molvig, K AF Simakov, Andrei N. Molvig, Kim TI Hydrodynamic description of an unmagnetized plasma with multiple ion species. II. Two and three ion species plasmas SO PHYSICS OF PLASMAS LA English DT Article AB Paper I [A. N. Simakov and K. Molvig, Phys. Plasmas 23, 032115 (2016)] obtained a fluid description for an unmagnetized collisional plasma with multiple ion species. To evaluate collisional plasma transport fluxes, required for such a description, two linear systems of equations need to be solved to obtain corresponding transport coefficients. In general, this should be done numerically. Herein, the general formalism is used to obtain analytical expressions for such fluxes for several specific cases of interest: a deuterium-tritium plasma; a plasma containing two ion species with strongly disparate masses, which agrees with previously obtained results; and a three ion species plasma made of deuterium, tritium, and gold. These results can be used for understanding the behavior of the aforementioned plasmas, or for verifying a code implementation of the general multi-ion formalism. (C) 2016 AIP Publishing LLC. C1 [Simakov, Andrei N.; Molvig, Kim] Los Alamos Natl Lab, Computat Phys Div, Los Alamos, NM 87545 USA. RP Simakov, AN (reprint author), Los Alamos Natl Lab, Computat Phys Div, Los Alamos, NM 87545 USA. EM simakov@lanl.gov OI Simakov, Andrei/0000-0001-7064-9153 FU Thermonuclear Burn Initiative of the NNSA Advanced Scientific and Computing (ASC) Program at Los Alamos National Laboratory; U.S. Department of Energy [DE-AC52-06NA25396] FX This work was supported by the Thermonuclear Burn Initiative of the NNSA Advanced Scientific and Computing (ASC) Program at Los Alamos National Laboratory, operated by Los Alamos National Security, LLC for the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. NR 6 TC 1 Z9 1 U1 0 U2 1 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAR PY 2016 VL 23 IS 3 AR 032116 DI 10.1063/1.4943895 PG 12 WC Physics, Fluids & Plasmas SC Physics GA DL7XY UT WOS:000375854900018 ER PT J AU Tang, TF Xu, XQ Ma, CH Bass, EM Holland, C Candy, J AF Tang, T. F. Xu, X. Q. Ma, C. H. Bass, E. M. Holland, C. Candy, J. TI Benchmark studies of the gyro-Landau-fluid code and gyro-kinetic codes on kinetic ballooning modes SO PHYSICS OF PLASMAS LA English DT Article ID ASPECT-RATIO; SIMULATIONS; MICROTURBULENCE; STABILIZATION; TOKAMAKS; GEOMETRY AB A Gyro-Landau-Fluid (GLF) 3 + 1 model has been recently implemented in BOUT++ framework, which contains full Finite-Larmor-Radius effects, Landau damping, and toroidal resonance [Ma et al., Phys. Plasmas 22, 055903 (2015)]. A linear global beta scan has been conducted using the JET-like circular equilibria (cbm18 series), showing that the unstable modes are kinetic ballooning modes (KBMs). In this work, we use the GYRO code, which is a gyrokinetic continuum code widely used for simulation of the plasma microturbulence, to benchmark with GLF 3+1 code on KBMs. To verify our code on the KBM case, we first perform the beta scan based on "Cyclone base case parameter set." We find that the growth rate is almost the same for two codes, and the KBM mode is further destabilized as beta increases. For JET-like global circular equilibria, as the modes localize in peak pressure gradient region, a linear local beta scan using the same set of equilibria has been performed at this position for comparison. With the drift kinetic electron module in the GYRO code by including small electron-electron collision to damp electron modes, GYRO generated mode structures and parity suggest that they are kinetic ballooning modes, and the growth rate is comparable to the GLF results. However, a radial scan of the pedestal for a particular set of cbm18 equilibria, using GYRO code, shows different trends for the low-n and high-n modes. The low-n modes show that the linear growth rate peaks at peak pressure gradient position as GLF results. However, for high-n modes, the growth rate of the most unstable mode shifts outward to the bottom of pedestal and the real frequency of what was originally the KBMs in ion diamagnetic drift direction steadily approaches and crosses over to the electron diamagnetic drift direction. (C) 2016 AIP Publishing LLC. C1 [Tang, T. F.] Dalian Univ Technol, Dalian 116024, Peoples R China. [Tang, T. F.; Xu, X. Q.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Ma, C. H.] Peking Univ, Sch Phys, Fus Simulat Ctr, Beijing 100871, Peoples R China. [Bass, E. M.; Candy, J.] Gen Atom Co, POB 85608, San Diego, CA 92186 USA. [Holland, C.] Univ Calif San Diego, La Jolla, CA 92093 USA. RP Tang, TF (reprint author), Dalian Univ Technol, Dalian 116024, Peoples R China.; Tang, TF (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. OI Tang, Tengfei/0000-0002-8698-9985 FU CSC [201406060053]; Ministry of Science and Technology of the People's Republic of China [2013GB107003, 2013GB109001]; National Natural Science Foundation of China [11575039] FX The authors wish to acknowledge Professor Dezhen Wang and Professor Jizhong Sun for useful discussions. This work was performed under the auspices of the CSC (No. 201406060053) and supported by Ministry of Science and Technology of the People's Republic of China under National Magnetic Confinement Fusion Science Program Contract Nos. 2013GB107003 and 2013GB109001, and National Natural Science Foundation of China under Grant No. 11575039. NR 25 TC 2 Z9 2 U1 5 U2 6 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAR PY 2016 VL 23 IS 3 AR 032119 DI 10.1063/1.4944391 PG 7 WC Physics, Fluids & Plasmas SC Physics GA DL7XY UT WOS:000375854900021 ER PT J AU Umansky, MV Ryutov, DD AF Umansky, M. V. Ryutov, D. D. TI Toroidally symmetric plasma vortex at tokamak divertor null point SO PHYSICS OF PLASMAS LA English DT Article AB Reduced MHD equations are used for studying toroidally symmetric plasma dynamics near the divertor null point. Numerical solution of these equations exhibits a plasma vortex localized at the null point with the time-evolution defined by interplay of the curvature drive, magnetic restoring force, and dissipation. Convective motion is easier to achieve for a second-order null (snowflake) divertor than for a regular x-point configuration, and the size of the convection zone in a snowflake configuration grows with plasma pressure at the null point. The trends in simulations are consistent with tokamak experiments which indicate the presence of enhanced transport at the null point. C1 [Umansky, M. V.; Ryutov, D. D.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Umansky, MV (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM umansky1@llnl.gov FU U.S. Department of Energy [DE-AC52-07NA27344] FX The authors are grateful to colleagues I. Joseph and L. LoDestro for helpful comments. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Security, LLC, Lawrence Livermore National Laboratory, under Contract No. DE-AC52-07NA27344. NR 16 TC 1 Z9 1 U1 0 U2 1 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAR PY 2016 VL 23 IS 3 AR 030701 DI 10.1063/1.4943101 PG 5 WC Physics, Fluids & Plasmas SC Physics GA DL7XY UT WOS:000375854900001 ER PT J AU Zhang, GB Chen, M Schroeder, CB Luo, J Zeng, M Li, FY Yu, LL Weng, SM Ma, YY Yu, TP Sheng, ZM Esarey, E AF Zhang, Guo-Bo Chen, Min Schroeder, C. B. Luo, Ji Zeng, Ming Li, Fei-Yu Yu, Lu-Le Weng, Su-Ming Ma, Yan-Yun Yu, Tong-Pu Sheng, Zheng-Ming Esarey, E. TI Acceleration and evolution of a hollow electron beam in wakefields driven by a Laguerre-Gaussian laser pulse SO PHYSICS OF PLASMAS LA English DT Article ID IONIZATION; INJECTION AB We show that a ring-shaped hollow electron beam can be injected and accelerated by using a Laguerre-Gaussian laser pulse and ionization-induced injection in a laser wakefield accelerator. The acceleration and evolution of such a hollow, relativistic electron beam are investigated through three-dimensional particle-in-cell simulations. We find that both the ring size and the beam thickness oscillate during the acceleration. The beam azimuthal shape is angularly dependent and evolves during the acceleration. The beam ellipticity changes resulting from the electron angular momenta obtained from the drive laser pulse and the focusing forces from the wakefield. The dependence of beam ring radius on the laser-plasma parameters (e.g., laser intensity, focal size, and plasma density) is studied. Such a hollow electron beam may have potential applications for accelerating and collimating positively charged particles. (C) 2016 AIP Publishing LLC. C1 [Zhang, Guo-Bo; Chen, Min; Luo, Ji; Zeng, Ming; Yu, Lu-Le; Weng, Su-Ming; Sheng, Zheng-Ming] Shanghai Jiao Tong Univ, Key Lab Laser Plasmas MOE, Shanghai 200240, Peoples R China. [Zhang, Guo-Bo; Chen, Min; Luo, Ji; Zeng, Ming; Yu, Lu-Le; Weng, Su-Ming; Sheng, Zheng-Ming] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai 200240, Peoples R China. [Zhang, Guo-Bo; Ma, Yan-Yun; Yu, Tong-Pu] Natl Univ Def Technol, Coll Sci, Changsha 410073, Hunan, Peoples R China. [Schroeder, C. B.; Esarey, E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Li, Fei-Yu; Sheng, Zheng-Ming] Univ Strathclyde, Dept Phys, SUPA, Glasgow G4 0NG, Lanark, Scotland. RP Chen, M (reprint author), Shanghai Jiao Tong Univ, Key Lab Laser Plasmas MOE, Shanghai 200240, Peoples R China.; Chen, M (reprint author), Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai 200240, Peoples R China.; Ma, YY (reprint author), Natl Univ Def Technol, Coll Sci, Changsha 410073, Hunan, Peoples R China. EM minchen@sjtu.edu.cn; yanyunma@126.com RI Yu, Tong-Pu/A-2360-2011; Chen, Min/A-9955-2010; Weng, Su-Ming/F-8076-2011; Sheng, Zheng-Ming/H-5371-2012 OI Chen, Min/0000-0002-4290-9330; Weng, Su-Ming/0000-0001-7746-9462; FU National Basic Research Program of China [2013CBA01504]; National Science Foundation of China [11374209, 11374210, 11475260, 11375265]; Leverhulme Trust Research Project Grant; U.S. Department of Energy [DE-AC02-05CH11231]; National 1000 Youth Talent Project of China; EPSRC [EP/L000237/1] FX This work was supported by the National Basic Research Program of China (Grant No. 2013CBA01504), the National Science Foundation of China (Grant Nos. 11374209, 11374210, 11475260, 11375265), a Leverhulme Trust Research Project Grant, the U.S. Department of Energy under Contract Nos. DE-AC02-05CH11231. M.C. appreciates the support from National 1000 Youth Talent Project of China. F.Y.L. and Z.M.S. acknowledge access to the ARCHER computing service through the Plasma HEC Consortium EPSRC grant number EP/L000237/1. Simulations were performed on the P supercomputer at Shanghai Jiao Tong University and Tianhe II supercomputer at Guangzhou. NR 28 TC 2 Z9 2 U1 9 U2 19 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD MAR PY 2016 VL 23 IS 3 AR 033114 DI 10.1063/1.4943892 PG 7 WC Physics, Fluids & Plasmas SC Physics GA DL7XY UT WOS:000375854900073 ER PT J AU Bower, WR Pearce, CI Smith, AD Pimblott, SM Mosselmans, JFW Haigh, SJ McKinley, JP Pattrick, RAD AF Bower, William R. Pearce, Carolyn I. Smith, Andrew D. Pimblott, Simon M. Mosselmans, J. Frederick W. Haigh, Sarah J. McKinley, James P. Pattrick, Richard A. D. TI Radiation damage in biotite mica by accelerated alpha-particles: A synchrotron microfocus X-ray diffraction and X-ray absorption spectroscopy study SO AMERICAN MINERALOGIST LA English DT Article DE Radiation damage; phyllosilicates; biotite; alpha-particle; pelletron; irradiation; synchrotron; microfocus; X-ray diffraction; X-ray absorption; EXAFS; infrared; spectroscopy; geodisposal; nuclear waste ID IRRADIATION; OXIDATION; AMORPHIZATION; REDUCTION; MUSCOVITE; MINERALS; CHLORITE; SORPTION; SILICA AB A critical radiation damage assessment of the materials that will be present in a Geological Disposal Facility (GDF) for radioactive waste is a priority for building a safety case. Detailed analysis of the effects of high-energy alpha-particle damage in phyllosilicates such as mica is a necessity, as these are model structures for both the clay-based backfill material and the highly sorbent components of a crystalline host rock. The alpha-radiation stability of biotite mica [general formula: K(Mg,Fe)(3)(Al,Si3O10) (F,OH)(2)] has been investigated using the 5 MV tandem pelletron at the University of Manchester's Dalton Cumbrian Facility (DCF) and both the microfocus spectroscopy (I18) and core X-ray absorption spectroscopy (B18) beamlines at Diamond Light Source (U.K.). Microfocus X-ray diffraction mapping has demonstrated extensive structural aberrations in the mica resulting from controlled exposure to the focused He-4(2+) ion (alpha-particle) beam. Delivered doses were comparable to alpha-particle fluences expected in the highly active, near-field of a GDF. At doses up to 6.77 displacements per atom (dpa) in the region of highest particle fluence, biotite mica displays a heterogeneous structural response to irradiation on a micrometer scale, with sequential dilation and contraction of regions of the structure perpendicular to the sheets, as well as a general overall contraction of the phyllosilicate layer spacing. At the peak of ion fluence, the structure collapses under a high point defect density and amorphous areas are pervasive among altered domains of the original lattice. Such structural alterations are likely to affect the material's capacity to sorb and retain escaped radionuclides over long timescales; increased edge site availability may favor increased sorption while interlayer uptake will likely be reduced due to collapse. Radiation-induced reduction of structural iron at the region of highest structural damage across an alpha-particle's track has been demonstrated by Fe K-edge X-ray absorption near edge spectroscopy (XANES) and local structural disorder has been confirmed by analysis of both potassium K-edge XANES and Fe K-edge extended X-ray absorption fine structure analysis. An infrared absorption study of deformations in the OH- stretching region, along with electron probe microanalysis complements the synchrotron data presented here. C1 [Bower, William R.; Pattrick, Richard A. D.] Univ Manchester, Sch Earth Atmospher & Environm Sci, Res Ctr Radwaste Disposal, Oxford Rd, Manchester M13 9PL, Lancs, England. [Bower, William R.; Pattrick, Richard A. D.] Univ Manchester, Sch Earth, Williamson Res Ctr, Oxford Rd, Manchester M13 9PL, Lancs, England. [Pearce, Carolyn I.] Univ Manchester, Dalton Nucl Inst, Oxford Rd, Manchester M13 9PL, Lancs, England. [Pearce, Carolyn I.] Univ Manchester, Sch Chem, Oxford Rd, Manchester M13 9PL, Lancs, England. [Smith, Andrew D.; Pimblott, Simon M.] Dalton Cumbrian Facil, Dalton Nucl Inst, Westlakes Sci Pk, Moor Row CA24 3HA, Cumbria, England. [Mosselmans, J. Frederick W.] Diamond Light Source, Harwell Campus, Didcot OX11 0DE, Oxon, England. [Haigh, Sarah J.] Univ Manchester, Sch Mat, Oxford Rd, Manchester M13 9PL, Lancs, England. [McKinley, James P.] Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99354 USA. RP Bower, WR (reprint author), Univ Manchester, Sch Earth Atmospher & Environm Sci, Res Ctr Radwaste Disposal, Oxford Rd, Manchester M13 9PL, Lancs, England.; Bower, WR (reprint author), Univ Manchester, Sch Earth, Williamson Res Ctr, Oxford Rd, Manchester M13 9PL, Lancs, England. EM william.bower@manchester.ac.uk RI mosselmans, j fred/H-4985-2013 FU NERC [NE/K500859/1]; Diamond Light Source, U.K. [SP9044, SP9647, SP9598]; U.K. Nuclear Decommissioning Authority; University of Manchester; Geochemistry Group at Pacific Northwest National Laboratory FX The authors are extremely grateful for the high-quality sample sectioning and preparation throughout the project performed by Stephen Stockley, University of Manchester, and the technical expertise and precision fabrication provided by Barry Gale and Lee Paul, University of Manchester. W.R.B. acknowledges NERC for funding under the DTA grant scheme awarded to the University of Manchester (code NE/K500859/1). The authors are also grateful to the Diamond Light Source, U.K., for analysis time on beamlines I18 and B18 (Beamtime award nos: SP9044, SP9647, SP9598) and invaluable project assistance. The Dalton Cumbrian Facility is a joint endeavor by the U.K. Nuclear Decommissioning Authority and the University of Manchester and its construction and commissioning was supported by both bodies. Spotlight 400 FTIR and Bruker D8 XRD data were collected in the University of Manchester's Williamson Research Centre and the authors acknowledge John Waters for assistance with XRD data collection. The authors gratefully acknowledge Steve Heald (Advanced Photon Source, Argonne National Lab) for providing the wustite and hematite Fe K-edge XANES data. J.P. McKinley acknowledges support for the EPMA analyses from the Geochemistry Group at Pacific Northwest National Laboratory. NR 58 TC 0 Z9 0 U1 3 U2 9 PU MINERALOGICAL SOC AMER PI CHANTILLY PA 3635 CONCORDE PKWY STE 500, CHANTILLY, VA 20151-1125 USA SN 0003-004X EI 1945-3027 J9 AM MINERAL JI Am. Miner. PD MAR-APR PY 2016 VL 101 IS 3-4 BP 928 EP 942 DI 10.2138/am-2016-5280CCBYNCND PG 15 WC Geochemistry & Geophysics; Mineralogy SC Geochemistry & Geophysics; Mineralogy GA DK0TW UT WOS:000374626100034 ER PT J AU Fan, ZS Neff, JC Wieder, WR AF Fan, Zhaosheng Neff, Jason C. Wieder, William R. TI Model-based analysis of environmental controls over ecosystem primary production in an alpine tundra dry meadow SO BIOGEOCHEMISTRY LA English DT Article DE Carbon; Nitrogen; Phosphorus; Plant productivity; Ecosystem model; Climate change ID SOIL MICROBIAL COMMUNITIES; COLORADO FRONT RANGE; CONSTRAINED EVOLUTIONARY OPTIMIZATION; DISSOLVED ORGANIC-CARBON; GROSS PRIMARY PRODUCTION; CLIMATE-CHANGE; PARAMETER-ESTIMATION; AMERICAN CORDILLERA; NITROGEN DEPOSITION; STOCHASTIC RANKING AB We investigated several key limiting factors that control alpine tundra productivity by developing an ecosystem biogeochemistry model. The model simulates the coupled cycling of carbon (C), nitrogen (N), and phosphorus (P) and their interactions with gross primary production (GPP). It was parameterized with field observations from an alpine dry meadow ecosystem using a global optimization strategy to estimate the unknown parameters. The model, along with the estimated parameters, was first validated against independent data and then used to examine the environmental controls over plant productivity. Our results show that air temperature is the strongest limiting factor to GPP in the early growing season, N availability becomes important during the middle portion of the growing season, and soil moisture is the strongest limiting factors by late in the growing season. Overall, the controls over GPP during the growing season, from strongest to weakest, are soil moisture content, air temperature, N availability, and P availability. This simulation provides testable predictions of the shifting nature of physical and nutrient limitations on plant growth. The model also indicates that changing environmental conditions in the alpine will likely lead to changes in productivity. For example, warming eliminates the control of P availability on GPP and makes N availability surpass air temperature to become the second strongest limiting factor. In contrast, an increase in atmospheric nutrient deposition eliminates the control of N availability and enhances the importance of P availability. These analyses provide a quantitative and conceptual framework that can be used to test predictions and refine ecological analyses at this long-term ecological research site. C1 [Fan, Zhaosheng] Argonne Natl Lab, Div Environm Sci, Argonne, IL 60439 USA. [Neff, Jason C.] Univ Colorado, Dept Geol Sci, Boulder, CO 80309 USA. [Wieder, William R.] Univ Colorado, Inst Arctic & Alpine Res, Boulder, CO 80309 USA. [Wieder, William R.] Natl Ctr Atmospher Res, Boulder, CO 80307 USA. RP Fan, ZS (reprint author), Argonne Natl Lab, Div Environm Sci, Argonne, IL 60439 USA. EM zfan@anl.gov OI WIEDER, WILLIAM/0000-0001-7116-1985 FU U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, Climate and Environmental Science Division [DE-AC02-06CH11357]; Niwot Ridge Long-Term Ecological Research Program - U.S. National Science Foundation [DEB1027341] FX This work was supported by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, Climate and Environmental Science Division under contract DE-AC02-06CH11357 and by the Niwot Ridge Long-Term Ecological Research Program that is funded by the U.S. National Science Foundation (#DEB1027341). NR 73 TC 0 Z9 0 U1 8 U2 16 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0168-2563 EI 1573-515X J9 BIOGEOCHEMISTRY JI Biogeochemistry PD MAR PY 2016 VL 128 IS 1-2 BP 35 EP 49 DI 10.1007/s10533-016-0193-9 PG 15 WC Environmental Sciences; Geosciences, Multidisciplinary SC Environmental Sciences & Ecology; Geology GA DJ9UB UT WOS:000374557300003 ER PT J AU Huang, EL Piehowski, PD Orton, DJ Moore, RJ Qian, WJ Casey, CP Sun, XF Dey, SK Burnum-Johnson, KE Smith, RD AF Huang, Eric L. Piehowski, Paul D. Orton, Daniel J. Moore, Ronald J. Qian, Wei-Jun Casey, Cameron P. Sun, Xiaofei Dey, Sudhansu K. Burnum-Johnson, Kristin E. Smith, Richard D. TI SNaPP: Simplified Nanoproteomics Platform for Reproducible Global Proteomic Analysis of Nanogram Protein Quantities SO ENDOCRINOLOGY LA English DT Article ID SAMPLE PREPARATION; MASS-SPECTROMETRY; ZONA-PELLUCIDA; MOUSE; BLASTOCYSTS; OOCYTE; MICE; UBIQUITINATION; IDENTIFICATION; LOCALIZATION AB Global proteomic analyses of complex protein samples in nanogram quantities require a fastidious approach to achieve in-depth protein coverage and quantitative reproducibility. Biological samples are often severely mass limited and can preclude the application of more robust bulk sample processing workflows. In this study, we present a system that minimizes sample handling by using online immobilized trypsin digestion and solid phase extraction to create a simple, sensitive, robust, and reproducible platform for the analysis of nanogram-size proteomic samples. To demonstrate the effectiveness of our simplified nanoproteomics platform, we used the system to analyze preimplantation blastocysts collected on day 4 of pregnancy by flushing the uterine horns with saline. For each of our three sample groups, blastocysts were pooled from three mice resulting in 22, 22, and 25 blastocysts, respectively. The resulting proteomic data provide novel insight into mouse blastocyst protein expression on day 4 of normal pregnancy because we characterized 348 proteins that were identified in at least two sample groups, including 59 enzymes and blastocyst specific proteins (eg, zona pellucida proteins). This technology represents an important advance in which future studies could perform global proteomic analyses of blastocysts obtained from an individual mouse, thereby enabling researchers to investigate interindividual variation as well as increase the statistical power without increasing animal numbers. This approach is also easily adaptable to other mass-limited sample types. C1 [Huang, Eric L.; Piehowski, Paul D.; Orton, Daniel J.; Moore, Ronald J.; Qian, Wei-Jun; Casey, Cameron P.; Burnum-Johnson, Kristin E.; Smith, Richard D.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Sun, Xiaofei; Dey, Sudhansu K.] Cincinnati Childrens Hosp Med Ctr, Cincinnati, OH 45229 USA. RP Burnum-Johnson, KE; Smith, RD (reprint author), Pacific NW Natl Lab, MSIN, POB 999,K8-98, Richland, WA 99352 USA. EM kristin.burnum-johnson@pnnl.gov; dick.smith@pnnl.gov RI Smith, Richard/J-3664-2012; OI Smith, Richard/0000-0002-2381-2349; Casey, Cameron/0000-0001-6790-2170; Piehowski, Paul/0000-0001-5108-2227 FU Department of Energy; Laboratory Directed Research and Development Program at the Pacific Northwest National Laboratory; National Institutes of Health [P41GM103493]; National Institutes of Health/Eunice Kennedy Shriver National Institute of Child Health and Human Development [R01HD068524]; March of Dimes; Department of Energy [DE-AC05-76RL0 1830] FX Portions of the experimental work described herein were performed in the Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the Department of Energy and located at the Pacific Northwest National Laboratory, which is operated by Battelle Memorial Institute for the Department of Energy.; This work was supported in part by the Laboratory Directed Research and Development Program at the Pacific Northwest National Laboratory, National Institutes of Health Grant P41GM103493 (to R.D.S.) and Grant R01HD068524 from the National Institutes of Health/Eunice Kennedy Shriver National Institute of Child Health and Human Development and March of Dimes (to S.K.D.). The Pacific Northwest National Laboratory is operated by Battelle Memorial Institute for the Department of Energy under Contract DE-AC05-76RL0 1830. NR 41 TC 2 Z9 2 U1 4 U2 5 PU ENDOCRINE SOC PI WASHINGTON PA 2055 L ST NW, SUITE 600, WASHINGTON, DC 20036 USA SN 0013-7227 EI 1945-7170 J9 ENDOCRINOLOGY JI Endocrinology PD MAR PY 2016 VL 157 IS 3 BP 1307 EP 1314 DI 10.1210/en.2015-1821 PG 8 WC Endocrinology & Metabolism SC Endocrinology & Metabolism GA DK0CC UT WOS:000374579000030 PM 26745641 ER PT J AU Cieplak, AM Slosar, A AF Cieplak, Agnieszka M. Slosar, Anze TI Towards physics responsible for large-scale Lyman-alpha forest bias parameters SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS LA English DT Article DE cosmological parameters from LSS; Lyman alpha forest; cosmological simulations ID BARYON ACOUSTIC-OSCILLATIONS; POWER SPECTRUM; INTERGALACTIC MEDIUM; FLUCTUATIONS; QUASARS AB Using a series of carefully constructed numerical experiments based on hydrodynamic cosmological SPH simulations, we attempt to build an intuition for the relevant physics behind the large scale density (b(delta)) and velocity gradient (b(eta)) biases of the Lyman-alpha forest. Starting with the fluctuating Gunn-Peterson approximation applied to the smoothed total density field in real-space, and progressing through redshift-space with no thermal broadening, redshift-space with thermal broadening and hydrodynamically simulated baryon fields, we investigate how approximations found in the literature fare. We find that Seljak's 2012 analytical formulae for these bias parameters work surprisingly well in the limit of no thermal broadening and linear redshift-space distortions. We also show that his b(eta) formula is exact in the limit of no thermal broadening. Since introduction of thermal broadening significantly affects its value, we speculate that a combination of large-scale measurements of b(eta) and the small scale flux PDF might be a sensitive probe of the thermal state of the IGM. We find that large-scale biases derived from the smoothed total matter field are within 10-20% to those based on hydrodynamical quantities, in line with other measurements in the literature. C1 [Cieplak, Agnieszka M.; Slosar, Anze] Brookhaven Natl Lab, Bldg 510A, Upton, NY 11973 USA. RP Cieplak, AM; Slosar, A (reprint author), Brookhaven Natl Lab, Bldg 510A, Upton, NY 11973 USA. EM acieplak@bnl.gov; anze@bnl.gov NR 31 TC 2 Z9 2 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1475-7516 J9 J COSMOL ASTROPART P JI J. Cosmol. Astropart. Phys. PD MAR PY 2016 IS 3 AR 016 DI 10.1088/1475-7516/2016/03/016 PG 21 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DL4LO UT WOS:000375608200018 ER PT J AU Egorov, AE Gaskins, JM Pierpaoli, E Pietrobon, D AF Egorov, Andrey E. Gaskins, Jennifer M. Pierpaoli, Elena Pietrobon, Davide TI Dark matter implications of the WMAP-Planck Haze SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS LA English DT Article DE dark matter theory; cosmic ray theory; absorption and radiation processes ID GAMMA-RAY HAZE; GALACTIC-CENTER; MICROWAVE HAZE; FERMI BUBBLES; MILKY-WAY; EMISSION; RADIO; WIND; CONSTRAINTS; PROPAGATION AB Gamma rays and microwave observations of the Galactic Center and surrounding areas indicate the presence of anomalous emission, whose origin remains ambiguous. The possibility of dark matter annihilation explaining both signals through prompt emission at gamma rays and secondary emission at microwave frequencies from interactions of high-energy electrons produced in annihilation with the Galactic magnetic fields has attracted much interest in recent years. We investigate the dark matter interpretation of the Galactic Center gamma-ray excess by searching for the associated synchrotron emission in the WMAP and Planck microwave data. Considering various magnetic field and cosmic-ray propagation models, we predict the synchrotron emission due to dark matter annihilation in our Galaxy, and compare it with the WMAP and Planck data at 23-70 GHz. In addition to standard microwave foregrounds, we separately model the microwave counterpart to the Fermi Bubbles and the signal due to dark matter annihilation, and use component separation techniques to extract the signal associated with each template from the total emission. We confirm the presence of the Haze at the level of approximate to 7% of the total sky intensity at 23 GHz in our chosen region of interest, with a harder spectrum (I similar to nu(-0.8)) than the synchrotron from regular cosmic-ray electrons. The data do not show a strong preference towards fitting the Haze by either the Bubbles or dark matter emission only. Inclusion of both components provides a better fit with a dark matter contribution to the Haze emission of approximate to 20% at 23 GHz, however, due to significant uncertainties in foreground modeling, we do not consider this a clear detection of a dark matter signal. We set robust upper limits on the annihilation cross section by ignoring foregrounds, and also report best-fit dark matter annihilation parameters obtained from a complete template analysis. We conclude that the WMAP and Planck data are consistent with a dark matter interpretation of the gamma-ray excess. C1 [Egorov, Andrey E.; Pierpaoli, Elena] Univ So Calif, 3620 McClintock Ave,SGM 408, Los Angeles, CA 90089 USA. [Gaskins, Jennifer M.] CALTECH, 1200 E Calif Blvd, Pasadena, CA 91125 USA. [Gaskins, Jennifer M.] Univ Amsterdam, GRAPPA, Sci Pk 904, NL-1098 XH Amsterdam, Netherlands. [Pietrobon, Davide] Univ Calif Berkeley, Space Sci Lab, 7 Gauss Rd, Berkeley, CA 94720 USA. [Pietrobon, Davide] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Pietrobon, Davide] HERE, 2075 Allston Way, Berkeley, CA 94704 USA. RP Egorov, AE; Pierpaoli, E (reprint author), Univ So Calif, 3620 McClintock Ave,SGM 408, Los Angeles, CA 90089 USA.; Gaskins, JM (reprint author), CALTECH, 1200 E Calif Blvd, Pasadena, CA 91125 USA.; Gaskins, JM (reprint author), Univ Amsterdam, GRAPPA, Sci Pk 904, NL-1098 XH Amsterdam, Netherlands.; Pietrobon, D (reprint author), Univ Calif Berkeley, Space Sci Lab, 7 Gauss Rd, Berkeley, CA 94720 USA.; Pietrobon, D (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA.; Pietrobon, D (reprint author), HERE, 2075 Allston Way, Berkeley, CA 94704 USA. EM egorov@usc.edu; jgaskins@uva.nl; pierpaol@usc.edu; daddeptr@gmail.com RI Egorov, Andrey/K-4009-2016; OI Pierpaoli, Elena/0000-0002-7957-8993 FU NASA [NNX13AP25G, NAS8-03060]; NASA - Chandra X-ray Center [PF1-120089]; Marie Curie International Incoming Fellowship in the project "IGMultiWave - ADD" [PIIF-GA-2013-628997]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX It is a pleasure to thank Loris Colombo for extensive help with the CMB emission modeling and Planck data interpretation, Andrew Strong for valuable consultations on GALPROP, and Antony Lewis for assistance with GetDist. AE and EP acknowledge the support of NASA grant NNX13AP25G and the usage of the computers at the USC High Performance Computing Center. JG acknowledges support from NASA through Einstein Postdoctoral Fellowship grant PF1-120089 awarded by the Chandra X-ray Center, which is operated by the Smithsonian Astrophysical Observatory for NASA under contract NAS8-03060, and from a Marie Curie International Incoming Fellowship in the project "IGMultiWave (PIIF-GA-2013-628997) - ADD". We also acknowledge the use of the LevelScheme package for Mathematica developed by Mark Caprio [76], it greatly helped in preparation of high-quality plots. In addition, this research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Some of the results in this paper have been derived using the HEALPix [58] package. NR 70 TC 2 Z9 2 U1 1 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1475-7516 J9 J COSMOL ASTROPART P JI J. Cosmol. Astropart. Phys. PD MAR PY 2016 IS 3 AR 060 DI 10.1088/1475-7516/2016/03/060 PG 35 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DL4LO UT WOS:000375608200062 ER PT J AU Errard, J Feeney, SM Peiris, HV Jaffe, AH AF Errard, Josquin Feeney, Stephen M. Peiris, Hiranya V. Jaffe, Andrew H. TI Robust forecasts on fundamental physics from the foreground-obscured, gravitationally-lensed CMB polarization SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS LA English DT Article DE CMBR experiments; CMBR polarisation; cosmological parameters from CMBR; gravitational waves and CMBR polarization ID MICROWAVE BACKGROUND ANISOTROPY; B-MODE POLARIZATION; PARAMETRIC COMPONENT SEPARATION; LARGE-SCALE STRUCTURE; MAXIMUM-LIKELIHOOD; GRAVITY-WAVES; INFLATION; EMISSION; CONSTRAINTS; DUST AB Recent results from the BICEP, Keck Array and Planck Collaborations demonstrate that Galactic foregrounds are an unavoidable obstacle in the search for evidence of inflationary gravitational waves in the cosmic microwave background (CMB) polarization. Beyond the foregrounds, the effect of lensing by intervening large-scale structure further obscures all but the strongest inflationary signals permitted by current data. With a plethora of ongoing and upcoming experiments aiming to measure these signatures, careful and self-consistent consideration of experiments' foreground- and lensing-removal capabilities is critical in obtaining credible forecasts of their performance. We investigate the capabilities of instruments such as Advanced ACTPo1, BICEP3 and Keck Array, CLASS, EBEX10K, PIPER, Simons Array, SPT-3G and SPIDER, and projects as COrE+, LiteBIRD-ext, PIXIE and Stage IV, to clean contamination due to polarized synchrotron and dust from raw multi-frequency data, and remove lensing from the resulting co-added CMB maps (either using iterative CMB-only techniques or through cross-correlation with external data). Incorporating these effects, we present forecasts for the constraining power of these experiments in terms of inflationary physics, the neutrino sector, and dark energy parameters. Made publicly available through an online interface, this tool enables the next generation of CMB experiments to foreground proof their designs, optimize their frequency coverage to maximize scientific output, and determine where cross-experimental collaboration would be most beneficial. We find that analyzing data from ground, balloon and space instruments in complementary combinations can significantly improve component separation performance, delensing, and cosmological constraints over individual datasets. In particular, we find that a combination of post-2020 ground- and space-based experiments could achieve constraints such as sigma (r) similar to 1.3 x 10(-4), sigma(n(t)) similar to 0.03, sigma(ns) similar to 1.8 x 10(-3), sigma(alpha(s)) similar to 1.7 x 10(-3), alpha(M-nu) similar to 31 meV, sigma(w) similar to 0.09, sigma(w(0)) similar to 0.25, sigma(w(a)) similar to 0.50, sigma(N-eff) similar to 0.024 and sigma(Omega(k)) similar to 1.5 x 10(-3), after component separation and iterative delensing. C1 [Errard, Josquin] Sorbonne Univ, ILP, 98 Bis Blvd Arago, F-75014 Paris, France. [Errard, Josquin] CNRS, IN2P3, LPNHE, 4 Pl Jussieu, F-75252 Paris 05, France. [Errard, Josquin] Univ Paris 06, 4 Pl Jussieu, F-75252 Paris 05, France. [Errard, Josquin] Univ Paris 07, 4 Pl Jussieu, F-75252 Paris 05, France. [Errard, Josquin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Computat Cosmol Ctr, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Errard, Josquin] Univ Calif Berkeley, Space Sci Lab, 7 Gauss Way, Berkeley, CA 94720 USA. [Feeney, Stephen M.; Jaffe, Andrew H.] Univ London Imperial Coll Sci Technol & Med, Blackett Lab, Dept Phys, Prince Consort Rd, London SW7 2AZ, England. [Peiris, Hiranya V.] UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. RP Errard, J (reprint author), Sorbonne Univ, ILP, 98 Bis Blvd Arago, F-75014 Paris, France.; Errard, J (reprint author), CNRS, IN2P3, LPNHE, 4 Pl Jussieu, F-75252 Paris 05, France.; Errard, J (reprint author), Univ Paris 06, 4 Pl Jussieu, F-75252 Paris 05, France.; Errard, J (reprint author), Univ Paris 07, 4 Pl Jussieu, F-75252 Paris 05, France.; Errard, J (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Computat Cosmol Ctr, 1 Cyclotron Rd, Berkeley, CA 94720 USA.; Errard, J (reprint author), Univ Calif Berkeley, Space Sci Lab, 7 Gauss Way, Berkeley, CA 94720 USA.; Feeney, SM; Jaffe, AH (reprint author), Univ London Imperial Coll Sci Technol & Med, Blackett Lab, Dept Phys, Prince Consort Rd, London SW7 2AZ, England.; Peiris, HV (reprint author), UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. EM josquin.errarad@lpnhe.in2p3.fr; s.feeney@imperial.ac.uk; h.peiris@ucl.ac.uk; a.jaffe@imperial.ac.uk FU Agence Nationale de la Recherche [ANR-11-IDEX-0004-02]; Science and Technology Facilities Council in the U.K.; New Frontiers in Astronomy and Cosmology [37426]; National Science Foundation [PHYS-1066293]; European Research Council under the European Community [306478-CosmicDawn] FX This work was partially completed within the Labex ILP (reference ANR-10-LABX-63) part of the Idex SUPER, and received financial state aid managed by the Agence Nationale de la Recherche, as part of the programme Investissements d'avenir under the reference ANR-11-IDEX-0004-02. SMF is supported by the Science and Technology Facilities Council in the U.K.. This work was also partially supported by a New Frontiers in Astronomy and Cosmology grant #37426, as well as by National Science Foundation Grant No. PHYS-1066293 and the hospitality of the Aspen Center for Physics. HVP was partially supported by the European Research Council under the European Community's Seventh Framework Programme (FP7/2007- 2013) / ERC grant agreement no 306478-CosmicDawn. NR 108 TC 15 Z9 15 U1 5 U2 8 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1475-7516 J9 J COSMOL ASTROPART P JI J. Cosmol. Astropart. Phys. PD MAR PY 2016 IS 3 AR 052 DI 10.1088/1475-7516/2016/03/052 PG 59 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DL4LO UT WOS:000375608200054 ER PT J AU Hooper, D Mohlabeng, G AF Hooper, Dan Mohlabeng, Gopolang TI The gamma-ray luminosity function of millisecond pulsars and implications for the GeV excess SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS LA English DT Article DE millisecond pulsars; gamma ray theory ID GLOBULAR-CLUSTER 47-TUCANAE; LARGE-AREA TELESCOPE; GALACTIC-CENTER; RADIO PULSARS; DARK-MATTER; POPULATION; EMISSION; BINARY; EVOLUTION; CATALOG AB It has been proposed that a large population of unresolved millisecond pulsars (MSPs) could potentially account for the excess of GeV-scale gamma-rays observed from the region surrounding the Galactic Center. The viability of this scenario depends critically on the gamma-ray luminosity function of this source population, which determines how many MSPs Fermi should have already detected as resolved point sources. In this paper, we revisit the gamma-ray luminosity function of MSPs, without relying on uncertain distance measurements. Our determination, based on a comparison of models with the observed characteristics of the MSP population, suggests that Fermi should have already detected a significant number of sources associated with such a hypothesized Inner Galaxy population. We cannot rule out a scenario in which the MSPs residing near the Galactic Center are systematically less luminous than those present in the Galactic Plane or within globular clusters. C1 [Hooper, Dan; Mohlabeng, Gopolang] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, POB 500, Batavia, IL 60510 USA. [Hooper, Dan] Univ Chicago, Dept Astron & Astrophys, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Mohlabeng, Gopolang] Univ Kansas, Dept Phys & Astron, Lawrence, KS 66045 USA. RP Hooper, D; Mohlabeng, G (reprint author), Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, POB 500, Batavia, IL 60510 USA.; Hooper, D (reprint author), Univ Chicago, Dept Astron & Astrophys, 5640 S Ellis Ave, Chicago, IL 60637 USA.; Mohlabeng, G (reprint author), Univ Kansas, Dept Phys & Astron, Lawrence, KS 66045 USA. EM dhooper@fnal.gov; gopolang.mohlabeng@ku.edu FU Fermilab Graduate Student Research Program in Theoretical Physics; National Research Foundation of South Africa [88614]; US Department of Energy FX We would like to thank Tim Linden, Christoph Weniger, Richard Bartels, Alex Drlica-Wagner, and Timothy Brandt for valuable discussions. GM is supported by the Fermilab Graduate Student Research Program in Theoretical Physics and in part by the National Research Foundation of South Africa, Grant No. 88614. This work has been supported by the US Department of Energy. NR 72 TC 4 Z9 4 U1 8 U2 9 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1475-7516 J9 J COSMOL ASTROPART P JI J. Cosmol. Astropart. Phys. PD MAR PY 2016 IS 3 AR 049 DI 10.1088/1475-7516/2016/03/049 PG 17 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DL4LO UT WOS:000375608200051 ER PT J AU Vlah, Z Seljak, U Chu, MY Feng, Y AF Vlah, Zvonimir Seljak, Uros Chu, Man Yat Feng, Yu TI Perturbation theory, effective field theory, and oscillations in the power spectrum SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS LA English DT Article DE cosmological perturbation theory; dark matter simulations; power spectrum ID LARGE-SCALE STRUCTURE; ANALYTIC MODEL; GALAXY; HALO AB We explore the relationship between the nonlinear matter power spectrum and the various Lagrangian and Standard Perturbation Theories (LPT and SPT). We first look at it in the context of one dimensional (1-d) dynamics, where 1LPT is exact at the perturbative level and one can exactly resum the SPT series into the 1LPT power spectrum. Shell crossings lead to non-perturbative effects, and the PT ignorance can be quantified in terms of their ratio, which is also the transfer function squared in the absence of stochasticity. At the order of PT we work, this parametrization is equivalent to the results of effective field theory (EFT), and can thus be expanded in terms of the same parameters. We find that its radius of convergence is larger than the SPT loop expansion. The same EFT parametrization applies to all SPT loop terms and if stochasticity can be ignored, to all N-point correlators. In 3-d, the LPT structure is considerably more complicated, and we find that LPT models with parametrization motivated by the EFT exhibit running with k and that SPT is generally a better choice. Since these transfer function expansions contain free parameters that change with cosmological model their usefulness for broadband power is unclear. For this reason we test the predictions of these models on baryonic acoustic oscillations (BAO) and other primordial oscillations, including string monodromy models, for which we ran a series of simulations with and without oscillations. Most models are successful in predicting oscillations beyond their corresponding PT versions, confirming the basic validity of the model. We show that if primordial oscillations are localized to a scale q, the wiggles in power spectrum are approximately suppressed as exp[-k(2)Sigma(2)(q)/2], where Sigma(q) is rms displacement of particles separated by q, which saturates on large scales, and decreases as q is reduced. No oscillatory features survive past k similar to 0.5h/Mpc at z = 0. C1 [Vlah, Zvonimir] Stanford Univ, Stanford Inst Theoret Phys, Stanford, CA 94306 USA. [Vlah, Zvonimir] Stanford Univ, Dept Phys, Stanford, CA 94306 USA. [Vlah, Zvonimir] SLAC, Kavli Inst Particle Astrophys & Cosmol, Menlo Pk, CA 94025 USA. [Vlah, Zvonimir] Stanford Univ, Menlo Pk, CA 94025 USA. [Seljak, Uros] Univ Calif Berkeley, Dept Astron, Phys, 601 Campbell Hall, Berkeley, CA 94720 USA. [Seljak, Uros] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Seljak, Uros; Chu, Man Yat; Feng, Yu] Univ Calif Berkeley, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. RP Vlah, Z (reprint author), Stanford Univ, Stanford Inst Theoret Phys, Stanford, CA 94306 USA.; Vlah, Z (reprint author), Stanford Univ, Dept Phys, Stanford, CA 94306 USA.; Vlah, Z (reprint author), SLAC, Kavli Inst Particle Astrophys & Cosmol, Menlo Pk, CA 94025 USA.; Vlah, Z (reprint author), Stanford Univ, Menlo Pk, CA 94025 USA.; Seljak, U (reprint author), Univ Calif Berkeley, Dept Astron, Phys, 601 Campbell Hall, Berkeley, CA 94720 USA.; Seljak, U (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.; Seljak, U; Chu, MY; Feng, Y (reprint author), Univ Calif Berkeley, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. EM zvlah@stanford.edu; useljak@berkeley.edu; jack_chu@berkeley.edu; yfeng1@berkeley.edu FU U.S. Department of Energy [DE-AC02-76SF00515]; NASA ATP [NNX12AG71G] FX We thank Tobias Baldauf, Leonardo Senatore, Martin White and Matias Zaldarriaga for useful disussions. We thank Matt McQuinn and Martin White for 1-d simulation and theory data. Z.V. is supported in part by the U.S. Department of Energy contract to SLAC no. DE-AC02-76SF00515. U.S. is supported in part by the NASA ATP grant NNX12AG71G. NR 35 TC 2 Z9 2 U1 2 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1475-7516 J9 J COSMOL ASTROPART P JI J. Cosmol. Astropart. Phys. PD MAR PY 2016 IS 3 AR 057 DI 10.1088/1475-7516/2016/03/057 PG 28 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DL4LO UT WOS:000375608200059 ER PT J AU Winslow, DM Fisher, AT Stauffer, PH Gable, CW Zyvoloski, GA AF Winslow, D. M. Fisher, A. T. Stauffer, P. H. Gable, C. W. Zyvoloski, G. A. TI Three-dimensional modeling of outcrop-to-outcrop hydrothermal circulation on the eastern flank of the Juan de Fuca Ridge SO JOURNAL OF GEOPHYSICAL RESEARCH-SOLID EARTH LA English DT Article DE hydrothermal circulation; fluid flow; heat flow; permeability; modeling; three-dimensional ID YOUNG OCEANIC-CRUST; HEAT-FLOW; CASCADIA BASIN; BABY BARE; SEA-FLOOR; BASALTIC BASEMENT; FLUXES; FLUID; PERMEABILITY; CONSTRAINTS AB We present three-dimensional simulations of coupled fluid and heat transport in the ocean crust, to explore patterns and controls on ridge-flank hydrothermal circulation on the eastern flank of the Juan de Fuca Ridge. Field studies have shown that there is large-scale fluid flow in the volcanic ocean crust in this region, including local convection and circulation between two basement outcrops separated by similar to 50km. New simulations include an assessment of crustal permeability and aquifer thickness, outcrop permeability, the potential influence of multiple discharging outcrops, and a comparison between two-dimensional (profile) and three-dimensional representations of the natural system. Field observations that help to constrain new simulations include a modest range of flow rates between recharging and discharging outcrops, secondary convection adjacent to the recharging outcrop, crustal permeability determinations made in boreholes, and the lack of a regional seafloor heat flux anomaly as a consequence of advective heat loss from the crust. Three-dimensional simulations are most consistent with field observations when models use a crustal permeability of 3x10(-13) to 2x10(-12)m(2), and the crustal aquifer is 300m thick, values consistent with borehole observations. We find fluid flow rates and crustal cooling efficiencies that are an order of magnitude greater in three-dimensional simulations than in two-dimensional simulations using equivalent properties. Simulations including discharge from an additional outcrop can also replicate field observations but tend to increase the overall rate of recharge and reduce the flow rate at the primary discharge site. C1 [Winslow, D. M.; Fisher, A. T.] Univ Calif Santa Cruz, Dept Earth & Planetary Sci, Santa Cruz, CA 95064 USA. [Stauffer, P. H.; Gable, C. W.; Zyvoloski, G. A.] Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. RP Fisher, AT (reprint author), Univ Calif Santa Cruz, Dept Earth & Planetary Sci, Santa Cruz, CA 95064 USA. EM afisher@ucsc.edu OI Stauffer, Philip/0000-0002-6976-221X FU National Science Foundation [OIA-0939564, OCE-1031808, OCE-1260408]; Consortium for Ocean Leadership Projects [T327A7, T327B7] FX This research used data provided by the Ocean Drilling Program (ODP) and the Integrated Ocean Drilling Program (IODP) and was supported by National Science Foundation grants OIA-0939564, OCE-1031808, and OCE-1260408, and Consortium for Ocean Leadership Projects T327A7 and T327B7 (A.T.F.). We thank L. Coogan and two anonymous reviewers for their helpful suggestions that improved this paper. This is C-DEBI contribution 316. NR 61 TC 0 Z9 0 U1 2 U2 8 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9313 EI 2169-9356 J9 J GEOPHYS RES-SOL EA JI J. Geophys. Res.-Solid Earth PD MAR PY 2016 VL 121 IS 3 BP 1365 EP 1382 DI 10.1002/2015JB012606 PG 18 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DK1ST UT WOS:000374695200007 ER PT J AU Frederick, JM Buffett, BA AF Frederick, Jennifer M. Buffett, Bruce A. TI Submarine groundwater discharge as a possible formation mechanism for permafrost-associated gas hydrate on the circum-Arctic continental shelf SO JOURNAL OF GEOPHYSICAL RESEARCH-SOLID EARTH LA English DT Article DE gas hydrate; submarine permafrost; Arctic; numerical model; submarine groundwater discharge; methane gas ID METHANE RELEASE; BLAKE RIDGE; HEAT-FLOW; SEA-FLOOR; MICROBIAL METHANE; MARINE-SEDIMENTS; NUMERICAL-MODEL; FLUID-FLOW; MARGIN; STABILITY AB Submarine groundwater discharge (SGD) is a large-scale, buoyancy-driven, offshore flow of terrestrial groundwater. If SGD occurs within the permafrost-bearing sediments of the circum-Arctic shelf, such fluid circulation may transport large amounts of dissolved methane to the circum-Arctic shelf, aiding the formation of permafrost-associated gas hydrate. We investigate the feasibility of this new permafrost-associated gas hydrate formation mechanism with a 2-D, multiphase fluid flow model, using the Canadian Beaufort Shelf as an example. The numerical model includes freeze/thaw permafrost processes and predicts the unsteady, 2-D methane solubility field for hydrate inventory calculations. Model results show that widespread, low-saturation hydrate deposits accumulate within and below submarine permafrost, even if offshore-flowing groundwater is undersaturated in methane gas. While intrapermafrost hydrate inventory varies widely depending on permafrost extent, subpermafrost hydrate stability remains largely intact across consecutive glacial cycles, allowing widespread subpermafrost accumulation over time. Methane gas escape to the sediment surface (atmosphere) is predicted along the seaward permafrost boundary during the early to middle years of each glacial epoch; however, if free gas is trapped within the forming permafrost layer instead, venting may be delayed until ocean transgression deepens the permafrost table during interglacial periods, and may be related to the spatial distribution of observed pingo-like features (PLFs) on the Canadian Beaufort Shelf. Shallow, gas-charged sediments are predicted above the gas hydrate stability zone at the midshelf to shelf edge and the upper slope, where a gap in hydrate stability allows free gas to accumulate and numerous PLFs have been observed. C1 [Frederick, Jennifer M.] Univ Nevada, Desert Res Inst, Div Hydrol Sci, Reno, NV 89506 USA. [Frederick, Jennifer M.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Buffett, Bruce A.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. RP Frederick, JM (reprint author), Univ Nevada, Desert Res Inst, Div Hydrol Sci, Reno, NV 89506 USA.; Frederick, JM (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM jmfrede@sandia.gov FU National Research Council Methane Hydrate Fellowship; National Academies of Sciences FX This study is supported by funding from the National Research Council Methane Hydrate Fellowship administered by the Department of Energy and the National Academies of Sciences. The authors thank Dale Issler for his help in providing us with insight to the local geological setting, and comments from the peer reviewers which helped improve the quality of this manuscript. For data supporting this numerical study, contact the corresponding author, Jennifer M. Frederick, jenn@eps.berkeley.edu. NR 93 TC 0 Z9 0 U1 9 U2 12 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9313 EI 2169-9356 J9 J GEOPHYS RES-SOL EA JI J. Geophys. Res.-Solid Earth PD MAR PY 2016 VL 121 IS 3 BP 1383 EP 1404 DI 10.1002/2015JB012627 PG 22 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DK1ST UT WOS:000374695200008 ER PT J AU Zoccarato, C Bau, D Ferronato, M Gambolati, G Alzraiee, A Teatini, P AF Zoccarato, C. Bau, D. Ferronato, M. Gambolati, G. Alzraiee, A. Teatini, P. TI Data assimilation of surface displacements to improve geomechanical parameters of gas storage reservoirs SO JOURNAL OF GEOPHYSICAL RESEARCH-SOLID EARTH LA English DT Article DE Reservoir geomechanics; Transverse isotropy; PSI measurements; Data Assimilation; Land displacements ID ENSEMBLE KALMAN FILTER; PO RIVER-BASIN; RADAR INTERFEROMETRY; LAND SUBSIDENCE; STATE VARIABLES; MODEL; COMPRESSIBILITY; INVERSION; FIELD; OIL AB Although the beginning of reservoir geomechanics dates back to the late 1960s, only recently stochastical geomechanical modelling has been introduced into the general framework of reservoir operational planning. In this study, the ensemble smoother (ES) algorithm, i.e., an ensemble-based data assimilation method, is employed to reduce the uncertainty of the constitutive parameters characterizing the geomechanical model of an underground gas storage (UGS) field situated in the upper Adriatic sedimentary basin (Italy), the Lombardia UGS. The model is based on a nonlinear transversely isotropic stress-strain constitutive law and is solved by 3-D finite elements. The Lombardia UGS experiences seasonal pore pressure change caused by fluid extraction/injection leading to land settlement/upheaval. The available observations consist of vertical and horizontal time-lapse displacements accurately measured by persistent scatterer interferometry (PSI) on RADARSAT scenes acquired between 2003 and 2008. The positive outcome of preliminary tests on simplified cases has supported the use of the ES to jointly assimilate vertical and horizontal displacements. The ES approach is shown to effectively reduce the spread of the uncertain parameters, i.e., the Poisson's ratio, the ratio between the horizontal and vertical Young and shear moduli, and the ratio between the virgin loading (I cycle) and unloading/reloading (II cycle) compressibility. The outcomes of the numerical simulations point out that the updated parameters depend on the assimilated measurement locations as well as the error associated to the PSI measurements. The parameter estimation may be improved by taking into account possible model and/or observation biases along with the use of an assimilation approach, e.g., the Iterative ensemble smoother, more appropriate for nonlinear problems. C1 [Zoccarato, C.; Ferronato, M.; Gambolati, G.; Teatini, P.] Univ Padua, Dept Civil Environm & Architectural Engn, I-35100 Padua, Italy. [Bau, D.] Univ Sheffield, Dept Civil & Struct Engn, Sheffield, S Yorkshire, England. [Alzraiee, A.] Sandia Natl Labs, Carlsbad, NM USA. RP Zoccarato, C (reprint author), Univ Padua, Dept Civil Environm & Architectural Engn, I-35100 Padua, Italy. EM claudia.zoccarato@dicea.unipd.it FU eni S.p.A. FX This work was funded by eni S.p.A. within the DAG (data assimilation in geomechanics) project. The PSI data are available upon specific request to the authors. The authors are much indebted to the Associated Editor, Peter Fokker, and another anonymous reviewer whose comments and suggestions helped improve greatly the quality of the paper. NR 45 TC 2 Z9 2 U1 2 U2 3 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9313 EI 2169-9356 J9 J GEOPHYS RES-SOL EA JI J. Geophys. Res.-Solid Earth PD MAR PY 2016 VL 121 IS 3 BP 1441 EP 1461 DI 10.1002/2015JB012090 PG 21 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DK1ST UT WOS:000374695200011 ER PT J AU Lieou, CKC Elbanna, AE Carlson, JM AF Lieou, Charles K. C. Elbanna, Ahmed E. Carlson, Jean M. TI Dynamic friction in sheared fault gouge: Implications of acoustic vibration on triggering and slow slip SO JOURNAL OF GEOPHYSICAL RESEARCH-SOLID EARTH LA English DT Article DE earthquake triggering; triggered slip; slow slip; fault gouge; granular; stick slip ID STICK-SLIP; SUBDUCTION ZONE; SOUTHWEST JAPAN; SILENT SLIP; EARTHQUAKES; DEFORMATION; TREMOR AB Friction and deformation in granular fault gouge are among various dynamic interactions associated with seismic phenomena that have important implications for slip mechanisms on earthquake faults. To this end, we propose a mechanistic model of granular fault gouge subject to acoustic vibrations and shear deformation. The grain-scale dynamics is described by the Shear-Transformation-Zone theory of granular flow, which accounts for irreversible plastic deformation in terms of flow defects whose density is governed by an effective temperature. Our model accounts for stick-slip instabilities observed at seismic slip rates. In addition, as the vibration intensity increases, we observe an increase in the temporal advancement of large slip events, followed by a plateau and gradual decrease. Furthermore, slip becomes progressively slower upon increasing the vibration intensity. The results shed important light on the physical mechanisms of earthquake triggering and slow slip and provide essential elements for the multiscale modeling of earthquake ruptures. In particular, the results suggest that slow slip may be triggered by tremors. C1 [Lieou, Charles K. C.; Carlson, Jean M.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Lieou, Charles K. C.] Los Alamos Natl Lab, Solid Earth Geophys Grp, Los Alamos, NM USA. [Lieou, Charles K. C.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Elbanna, Ahmed E.] Univ Illinois, Dept Civil & Environm Engn, Urbana, IL USA. RP Lieou, CKC (reprint author), Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA.; Lieou, CKC (reprint author), Los Alamos Natl Lab, Solid Earth Geophys Grp, Los Alamos, NM USA.; Lieou, CKC (reprint author), Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. EM clieou@lanl.gov RI Lieou, Charles/G-4244-2016 OI Lieou, Charles/0000-0003-2514-7335 FU NSF [DMR0606092, EAR-1345108, EAR-0529922]; NSF/USGS Southern California Earthquake Center; USGS [07HQAG0008]; David and Lucile Packard Foundation FX We thank Jean-Paul Ampuero and Ralph Archuleta for instructive discussions. This work was supported by NSF grants DMR0606092 and EAR-1345108, and the NSF/USGS Southern California Earthquake Center, funded by NSF Cooperative Agreement EAR-0529922 and USGS Cooperative Agreement 07HQAG0008, and the David and Lucile Packard Foundation. The data and codes for this paper are available by contacting the corresponding author. NR 46 TC 1 Z9 1 U1 2 U2 6 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9313 EI 2169-9356 J9 J GEOPHYS RES-SOL EA JI J. Geophys. Res.-Solid Earth PD MAR PY 2016 VL 121 IS 3 BP 1483 EP 1496 DI 10.1002/2015JB012741 PG 14 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DK1ST UT WOS:000374695200013 ER PT J AU Sigsbee, K Kletzing, CA Smith, CW MacDowall, R Spence, H Reeves, G Blake, JB Baker, DN Green, JC Singer, HJ Carr, C Santolik, O AF Sigsbee, K. Kletzing, C. A. Smith, C. W. MacDowall, R. Spence, H. Reeves, G. Blake, J. B. Baker, D. N. Green, J. C. Singer, H. J. Carr, C. Santolik, O. TI Van Allen Probes, THEMIS, GOES, and Cluster observations of EMIC waves, ULF pulsations, and an electron flux dropout SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article ID ION-CYCLOTRON WAVES; RADIATION BELT ELECTRONS; 1-2 MAGNETIC PULSATIONS; RING CURRENT; EQUATORIAL MAGNETOSPHERE; RELATIVISTIC ELECTRONS; PLASMASPHERIC PLUME; GEOMAGNETIC STORMS; SYNCHRONOUS ORBIT; MAGNETOPAUSE AB We examined an electron flux dropout during the 12-14 November 2012 geomagnetic storm using observations from seven spacecraft: the two Van Allen Probes, Time History of Events and Macroscale Interactions during Substorms (THEMIS)-A (P5), Cluster 2, and Geostationary Operational Environmental Satellites (GOES) 13, 14, and 15. The electron fluxes for energies greater than 2.0 MeV observed by GOES 13, 14, and 15 at geosynchronous orbit and by the Van Allen Probes remained at or near instrumental background levels for more than 24 h from 12 to 14 November. For energies of 0.8 MeV, the GOES satellites observed two shorter intervals of reduced electron fluxes. The first interval of reduced 0.8 MeV electron fluxes on 12-13 November was associated with an interplanetary shock and a sudden impulse. Cluster, THEMIS, and GOES observed intense He+ electromagnetic ion cyclotron (EMIC) waves from just inside geosynchronous orbit out to the magnetopause across the dayside to the dusk flank. The second interval of reduced 0.8 MeV electron fluxes on 13-14 November was associated with a solar sector boundary crossing and development of a geomagnetic storm with Dst <- 100nT. At the start of the recovery phase, both the 0.8 and 2.0 MeV electron fluxes finally returned to near prestorm values, possibly in response to strong ultralow frequency (ULF) waves observed by the Van Allen Probes near dawn. A combination of adiabatic effects, losses to the magnetopause, scattering by EMIC waves, and acceleration by ULF waves can explain the observed electron behavior. C1 [Sigsbee, K.; Kletzing, C. A.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Smith, C. W.; Spence, H.] Univ New Hampshire, Inst Earth Oceans & Space, Durham, NH 03824 USA. [MacDowall, R.] NASA, Goddard Space Flight Ctr, Planetary Magnetospheres Lab, Greenbelt, MD USA. [Reeves, G.] Los Alamos Natl Lab, Space & Atmospher Sci, NIS 1, Los Alamos, NM USA. [Blake, J. B.] Aerosp Corp, El Segundo, CA 90245 USA. [Baker, D. N.] Univ Colorado, Atmospher & Space Phys Lab, Campus Box 392, Boulder, CO 80309 USA. [Green, J. C.] Space Hazards Applicat, Golden, CO USA. [Singer, H. J.] NOAA, Space Weather Predict Ctr, Boulder, CO USA. [Carr, C.] Univ London Imperial Coll Sci Technol & Med, Dept Phys, London, England. [Santolik, O.] Inst Atmospher Phys AS CR, Prague, Czech Republic. [Santolik, O.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. RP Sigsbee, K (reprint author), Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. EM kristine-sigsbee@uiowa.edu RI Santolik, Ondrej/F-7766-2014; OI Kletzing, Craig/0000-0002-4136-3348; Sigsbee, Kristine/0000-0001-8727-380X; Reeves, Geoffrey/0000-0002-7985-8098 FU JHU/APL under NASA prime contract [921647, 967399, NAS5-01072]; Czech Academy of Sciences through the Praemium Academiae award; NASA [NAS5-02099]; German Ministry for Economy and Technology; German Center for Aviation and Space (DLR) [50 OC 0302]; [LH14010] FX This work was performed under JHU/APL contract 921647 under NASA prime contract NAS5-01072. We acknowledge William Kurth for providing density calculations from the EMFISIS data. RBSP-ECT funding was provided by JHU/APL contract 967399 under NASA prime contract NAS5-01072. O. Santolik acknowledges funding from the Czech Academy of Sciences through the Praemium Academiae award and from the LH14010 grant. We acknowledge NASA contract NAS5-02099 and V. Angelopoulos for use of data from the THEMIS Mission. Specifically, K.H. Glassmeier, U. Auster, and W. Baumjohann provided THEMIS FGM data under the lead of the Technical University of Braunschweig and with financial support through the German Ministry for Economy and Technology and the German Center for Aviation and Space (DLR) under contract 50 OC 0302. Data from the Van Allen Probes can be obtained through the Van Allen Probes Science Gateway (http://rbspgway.jhuapl.edu/). GOES data are available from the NOAA National Geophysical Data Center, and the Preliminary Reports and Forecasts of Solar Geophysical Data are available from the NOAA Space Weather Prediction Center. THEMIS data are publicly available through the University of California Berkeley (http://themis.ssl.berkeley.edu). Cluster data are available from the Cluster Science Archive. Solar wind data and geomagnetic indexes are available online from NASA OMNIWeb. Wind and ACE data are available online through CDAWeb. NR 62 TC 1 Z9 1 U1 0 U2 7 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD MAR PY 2016 VL 121 IS 3 BP 1990 EP 2008 DI 10.1002/2014JA020877 PG 19 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DK2FV UT WOS:000374730900013 ER PT J AU Hao, Y Lembege, B Lu, Q Guo, F AF Hao, Y. Lembege, B. Lu, Q. Guo, F. TI Formation of downstream high-speed jets by a rippled nonstationary quasi-parallel shock: 2-D hybrid simulations SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article ID AMPLITUDE MAGNETIC-STRUCTURES; PERPENDICULAR BOW SHOCKS; 2-DIMENSIONAL SIMULATIONS; COLLISIONLESS SHOCKS; ION DISTRIBUTIONS; UPSTREAM WAVES; RE-FORMATION; ANISOTROPY INSTABILITIES; SUBSOLAR MAGNETOSHEATH; PARTICLE-ACCELERATION AB Experimental observations from space missions (including more recently Cluster and Time History of Events and Macroscale Interactions during Substorms data) have clearly revealed the existence of high-speed jets (HSJs) in the downstream region of the quasi-parallel terrestrial bow shock. Presently, two-dimensional hybrid simulations are performed in order to investigate the formation of such HSJs through a rippled quasi-parallel shock front. The simulation results show that (i) such shock fronts are strongly nonstationary along the shock normal, and (ii) ripples are evidenced along the shock front as the upstream ULF waves (excited by interaction between incident and reflected ions) are convected back to the front by the solar wind and contribute to the rippling formation. Then, these ripples are inherent structures of a quasi-parallel shock. As a consequence, new incident solar wind ions interact differently at different locations along the shock surface, and the ion bulk velocity strongly differs locally as ions are transmitted downstream. Preliminary results show that (i) local bursty patterns of turbulent magnetic field may form within the rippled front and play the role of local secondary shock; (ii) some incident ion flows penetrate the front, suffer some deflection (instead of being decelerated) at the locations of these secondary shocks, and are at the origin of well-structured (filamentary) HSJs downstream; and (iii) the spatial scales of HSJs are in a good agreement with experimental observations. Such downstream HSJs are shown to be generated by local curvature effects (front rippling) and the nonstationarity of the shock front itself. C1 [Hao, Y.; Lembege, B.] CNRS, LATMOS, IPSL, UVSQ, Guyancourt, France. [Hao, Y.; Lu, Q.] Univ Sci & Technol China, Dept Geophys & Planetary Sci, CAS Key Lab Geospace Environm, Hefei 230026, Peoples R China. [Hao, Y.; Lu, Q.] Collaborat Innovat Ctr Astronaut Sci & Technol, Hefei, Peoples R China. [Guo, F.] Los Alamos Natl Lab, Los Alamos, NM USA. RP Lembege, B (reprint author), CNRS, LATMOS, IPSL, UVSQ, Guyancourt, France. EM bertrand.lembege@latmos.ipsl.fr FU National Science Foundation of China [41331067, 11235009, 41274144, 41121003]; 973 Program [2012CB825602, 2013CBA01503]; CAS Key Research Program [KZZD-EW-01-4]; China Scholarship Council (CSC) FX This work is supported by the National Science Foundation of China (grants 41331067, 11235009, 41274144, and 41121003), 973 Program (2012CB825602 and 2013CBA01503), and CAS Key Research Program KZZD-EW-01-4. Computer resources were provided by the National Supercomputer Center of China in Tianjin and Alabama Supercomputer Center. The authors also thank D.W. Swift for his help and discussions in the code development. The numerical data can be obtained by contacting the corresponding author via email. One of the authors (Y.H.) thanks the China Scholarship Council (CSC) for attributing a fellowship for a 1 year stay in LATMOS laboratory (Guyancourt, France) which is warmly thanked for its welcome and hospitality. The authors thank the referees for their detailed and helpful comments. NR 73 TC 2 Z9 2 U1 5 U2 8 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD MAR PY 2016 VL 121 IS 3 BP 2080 EP 2094 DI 10.1002/2015JA021419 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DK2FV UT WOS:000374730900018 ER PT J AU Russell, CT Wei, HY Cowee, MM Neubauer, FM Dougherty, MK AF Russell, C. T. Wei, H. Y. Cowee, M. M. Neubauer, F. M. Dougherty, M. K. TI Ion cyclotron waves at Titan SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article AB During the interaction of Titan's thick atmosphere with the ambient plasma, it was expected that ion cyclotron waves would be generated by the free energy of the highly anisotropic velocity distribution of the freshly ionized atmospheric particles created in the interaction. However, ion cyclotron waves are rarely observed near Titan, due to the long growth times of waves associated with the major ion species from Titan's ionosphere, such as CH4+ and N-2(+). In the over 100 Titan flybys obtained by Cassini to date, there are only two wave events, for just a few minutes during T63 flyby and for tens of minutes during T98 flyby. These waves occur near the gyrofrequencies of proton and singly ionized molecular hydrogen. They are left-handed, elliptically polarized, and propagate nearly parallel to the field lines. Hybrid simulations are performed to understand the wave growth under various conditions in the Titan environment. The simulations using the plasma and field conditions during T63 show that pickup protons with densities ranging from 0.01 cm(-3) to 0.02 cm(-3) and singly ionized molecular hydrogens with densities ranging from 0.015 cm(-3) to 0.25 cm(-3) can drive ion cyclotron waves with amplitudes of similar to 0.02nT and of similar to 0.04nT within appropriate growth times at Titan, respectively. Since the T98 waves were seen farther upstream than the T63 waves, it is possible that the instability was stronger and grew faster on T98 than T63. C1 [Russell, C. T.; Wei, H. Y.] Univ Calif Los Angeles, Earth Planetary & Space Sci, Los Angeles, CA 90095 USA. [Russell, C. T.; Wei, H. Y.] Univ Calif Los Angeles, Inst Geophys & Planetary Phys, Los Angeles, CA USA. [Cowee, M. M.] Los Alamos Natl Lab, Los Alamos, NM USA. [Neubauer, F. M.] Univ Cologne, Inst Geophys & Meteorol, Cologne, Germany. [Dougherty, M. K.] Univ London Imperial Coll Sci Technol & Med, Blackett Lab, Space & Atmospher Phys Grp, London, England. RP Wei, HY (reprint author), Univ Calif Los Angeles, Earth Planetary & Space Sci, Los Angeles, CA 90095 USA.; Wei, HY (reprint author), Univ Calif Los Angeles, Inst Geophys & Planetary Phys, Los Angeles, CA USA. EM hwei@igpp.ucla.edu FU NASA's Cassini project through a subcontract with the Jet Propulsion Laboratory; NASA [NNH15AZ13I] FX Work at UCLA was supported by NASA's Cassini project through a subcontract with the Jet Propulsion Laboratory. Work at Los Alamos was supported by NASA grant NNH15AZ13I. Work at Cologne University was supported by internal funds. The Cassini data used in the manuscript are publicly accessible on the Planetary Data System (http://ppi.pds.nasa.gov/search/view/?f=yes&id=pds://PPI/CO-E_SW_J_S-MAG -4-SUMM-1SECAVG-V1.0). NR 18 TC 1 Z9 1 U1 2 U2 2 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD MAR PY 2016 VL 121 IS 3 BP 2095 EP 2103 DI 10.1002/2015JA022293 PG 9 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DK2FV UT WOS:000374730900019 ER PT J AU Krall, J Huba, JD Jordanova, VK Denton, RE Carranza, T Moldwin, MB AF Krall, J. Huba, J. D. Jordanova, V. K. Denton, R. E. Carranza, T. Moldwin, M. B. TI Measurement and modeling of the refilling plasmasphere during 2001 SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE plasmasphere; refilling; dynamics; thermosphere; exosphere ID INTERNATIONAL REFERENCE IONOSPHERE; INNER MAGNETOSPHERE; EARTHS PLASMASPHERE; FIELD LINES; THERMOSPHERE; SIMULATION; HE+; SPACECRAFT; PLASMAPAUSE; FREQUENCIES AB The Naval Research Laboratory SAMI3 (Sami3 is Also a Model of the Ionosphere) and the RAM-CPL (Ring current Atmosphere interaction Model-Cold PLasma) codes are used to model observed plasmasphere dynamics during 25 November 2001 to 1 December 2001 and 1-5 February 2001. Model results compare well to plasmasphere observations of electron and mass densities. Comparison of model results to refilling data and to each other shows good agreement, generally within a factor of 2. We find that SAMI3 plasmaspheric refilling rates and ion densities are sensitive to the composition and temperature of the thermosphere and exosphere, and to photoelectron heating. Results also support our previous finding that the wind-driven dynamo significantly impacts both refilling rates and plasmasphere dynamics during quiet periods. C1 [Krall, J.; Huba, J. D.] Naval Res Lab, Plasma Phys Div, Washington, DC 20375 USA. [Jordanova, V. K.] Los Alamos Natl Lab, Los Alamos, NM USA. [Denton, R. E.] Dartmouth Coll, Dept Phys & Astron, Hanover, NH 03755 USA. [Carranza, T.; Moldwin, M. B.] Univ Michigan, Dept Climate & Space Sci & Engn, Ann Arbor, MI 48109 USA. RP Krall, J (reprint author), Naval Res Lab, Plasma Phys Div, Washington, DC 20375 USA. EM jonathan.krall@nrl.navy.mil OI Jordanova, Vania/0000-0003-0475-8743 FU NRL Base Funds; NASA LWS Program; NASA [NNX10AQ60G]; NSF [AGS-1105790]; U.S. Department of Energy; LDRD; NASA/LWS; NSF Graduate Fellowship; [NSFAGS-1265651] FX This research was supported by NRL Base Funds and the NASA LWS Program. Work at Dartmouth College was supported by NASA grant NNX10AQ60G (Living with a Star Targeted Research Plasmasphere focused science topic) and NSF grant AGS-1105790. Work at LANL was performed under the auspices of the U.S. Department of Energy with partial support from the LDRD and NASA/LWS programs. M.B.M. was partially supported by NSFAGS-1265651 and T.C. was supported by a NSF Graduate Fellowship. We thank Joel Fedder of Icarus Research, John Emmert of NRL, and Hanbyul Lee of the Korea Polar Research Institute for helpful discussions. We similarly thank the LWS Plasmasphere Team, led by Pontus Brandt of the Johns Hopkins University Applied Physics Laboratory. We thank Yongli Wang of Goddard Space Flight Center for assistance with the IMAGE/RPI data. Data and models were obtained from the following sources: Solar wind (OMNI data set), EUV indices, and geomagnetic indices were obtained from the Coordinated Data Analysis Web (CDAWeb, http://cdaweb.gsfc.nasa.gov/istp_public/). IMAGE/RPI electron densities [see Denton et al., 2012] are available at CDAWeb; data used here can be obtained by contacting J.K. Refilling values can be derived from the IMAGE/RPI electron density data as described above. These values are provided in figures; the exact values can be obtained by contacting J.K. Magnetometer data are available at http://supermag.jhuapl.edu/ for MEASURE; the inferred mass densities were provided by the MEASURE team; these values are shown in figures; the exact values can be obtained by contacting J.K. SAMI3 electron and ion densities are numerical information provided in figures; these are produced by solving the SAMI3 equations [Huba and Krall, 2013; Huba et al., 2000]. RAM-CPL electron densities are numerical information provided in figures; these are produced by solving the RAM equations [Jordanova et al., 2006; Rasmussen et al., 1993]. Refilling rates for SAMI3 and RAM-CPL are obtained by analyzing SAMI3 and RAM-CPL electron densities and are provided in figures; exact values can be obtained by contacting J.K. NR 62 TC 2 Z9 2 U1 3 U2 6 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD MAR PY 2016 VL 121 IS 3 BP 2226 EP 2248 DI 10.1002/2015JA022126 PG 23 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DK2FV UT WOS:000374730900027 ER PT J AU Adams, D Alekou, A Apollonio, M Asfandiyarov, R Barber, G Barclay, P de Bari, A Bayes, R Bayliss, V Bertoni, R Blackmore, VJ Blondel, A Blot, S Bogomilov, M Bonesini, M Booth, CN Bowring, D Boyd, S Brashaw, TW Bravar, U Bross, AD Capponi, M Carlisle, T Cecchet, G Charnley, C Chignoli, F Cline, D Cobb, JH Colling, G Collomb, N Coney, L Cooke, P Courthold, M Cremaldi, LM DeMello, A Dick, A Dobbs, A Dornan, P Drews, M Drielsma, F Filthaut, F Fitzpatrick, T Franchini, P Francis, V Fry, L Gallagher, A Gamet, R Gardener, R Gourlay, S Grant, A Greis, JR Griffiths, S Hanlet, P Hansen, OM Hanson, GG Hart, TL Hartnett, T Hayler, T Heidt, C Hills, M Hodgson, P Hunt, C Iaciofano, A Ishimoto, S Kafka, G Kaplan, DM Karadzhov, Y Kim, YK Kuno, Y Kyberd, P Lagrange, JB Langlands, J Lau, W Leonova, M Li, D Lintern, A Littlefield, M Long, K Luo, T Macwaters, C Martlew, B Martyniak, J Mazza, R Middleton, S Moretti, A Moss, A Muir, A Mullacrane, I Nebrensky, JJ Neuffer, D Nichols, A Nicholson, R Nugent, JC Oates, A Onel, Y Orestano, D Overton, E Owens, P Palladino, V Pasternak, J Pastore, F Pidcott, C Popovic, M Preece, R Prestemon, S Rajaram, D Ramberger, S Rayner, MA Ricciardi, S Roberts, TJ Robinson, M Rogers, C Ronald, K Rubinov, P Rucinski, P Sakamato, H Sanders, DA Santos, E Savidge, T Smith, PJ Snopok, P Soler, FJP Speirs, D Stanley, T Stokes, G Summers, DJ Tarrant, J Taylor, I Tortora, L Torun, Y Tsenov, R Tunnell, CD Uchida, MA Vankova-Kirilova, G Virostek, S Vretenar, M Warburton, P Watson, S White, C Whyte, CG Wilson, A Winter, M Yang, X Young, A Zisman, M AF Adams, D. Alekou, A. Apollonio, M. Asfandiyarov, R. Barber, G. Barclay, P. de Bari, A. Bayes, R. Bayliss, V. Bertoni, R. Blackmore, V. J. Blondel, A. Blot, S. Bogomilov, M. Bonesini, M. Booth, C. N. Bowring, D. Boyd, S. Brashaw, T. W. Bravar, U. Bross, A. D. Capponi, M. Carlisle, T. Cecchet, G. Charnley, C. Chignoli, F. Cline, D. Cobb, J. H. Colling, G. Collomb, N. Coney, L. Cooke, P. Courthold, M. Cremaldi, L. M. DeMello, A. Dick, A. Dobbs, A. Dornan, P. Drews, M. Drielsma, F. Filthaut, F. Fitzpatrick, T. Franchini, P. Francis, V. Fry, L. Gallagher, A. Gamet, R. Gardener, R. Gourlay, S. Grant, A. Greis, J. R. Griffiths, S. Hanlet, P. Hansen, O. M. Hanson, G. G. Hart, T. L. Hartnett, T. Hayler, T. Heidt, C. Hills, M. Hodgson, P. Hunt, C. Iaciofano, A. Ishimoto, S. Kafka, G. Kaplan, D. M. Karadzhov, Y. Kim, Y. K. Kuno, Y. Kyberd, P. Lagrange, J. -B. Langlands, J. Lau, W. Leonova, M. Li, D. Lintern, A. Littlefield, M. Long, K. Luo, T. Macwaters, C. Martlew, B. Martyniak, J. Mazza, R. Middleton, S. Moretti, A. Moss, A. Muir, A. Mullacrane, I. Nebrensky, J. J. Neuffer, D. Nichols, A. Nicholson, R. Nugent, J. C. Oates, A. Onel, Y. Orestano, D. Overton, E. Owens, P. Palladino, V. Pasternak, J. Pastore, F. Pidcott, C. Popovic, M. Preece, R. Prestemon, S. Rajaram, D. Ramberger, S. Rayner, M. A. Ricciardi, S. Roberts, T. J. Robinson, M. Rogers, C. Ronald, K. Rubinov, P. Rucinski, P. Sakamato, H. Sanders, D. A. Santos, E. Savidge, T. Smith, P. J. Snopok, P. Soler, F. J. P. Speirs, D. Stanley, T. Stokes, G. Summers, D. J. Tarrant, J. Taylor, I. Tortora, L. Torun, Y. Tsenov, R. Tunnell, C. D. Uchida, M. A. Vankova-Kirilova, G. Virostek, S. Vretenar, M. Warburton, P. Watson, S. White, C. Whyte, C. G. Wilson, A. Winter, M. Yang, X. Young, A. Zisman, M. CA MICE Collaboration TI Pion contamination in the MICE muon beam SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Instrumentation for particle accelerators and storage rings - low energy (linear accelerators, cyclotrons, electrostatic accelerators); Beam-line instrumentation (beam position and profile; monitors; beam-intensity monitors; bunch length monitors) ID DESIGN; CONSTRUCTION AB The international Muon Ionization Cooling Experiment (MICE) will perform a systematic investigation of ionization cooling with muon beams of momentum between 140 and 240 MeV/c at the Rutherford Appleton Laboratory ISIS facility. The measurement of ionization cooling in MICE relies on the selection of a pure sample of muons that traverse the experiment. To make this selection, the MICE Muon Beam is designed to deliver a beam of muons with less than similar to 1% contamination. To make the final muon selection, MICE employs a particle-identification (PID) system upstream and downstream of the cooling cell. The PID system includes time-of-flight hodoscopes, threshold-Cherenkov counters and calorimetry. The upper limit for the pion contamination measured in this paper is f(pi) < 1 : 4% at 90% C.L., including systematic uncertainties. Therefore, the MICE Muon Beam is able to meet the stringent pion-contamination requirements of the study of ionization cooling. C1 [Bogomilov, M.; Tsenov, R.; Vankova-Kirilova, G.] Sofia Univ St Kliment Ohridski, Dept Atom Phys, Sofia, Bulgaria. [Bertoni, R.; Bonesini, M.; Chignoli, F.; Mazza, R.] Sez INFN Milano Bicocca, Dipartimento Fis G Occhialini, Milan, Italy. [Palladino, V.] Univ Naples Federico II, Complesso Univ Monte S Angelo, Sez INFN Napoli, Naples, Italy. [Palladino, V.] Univ Naples Federico II, Complesso Univ Monte S Angelo, Dipartimento Fis, Naples, Italy. [de Bari, A.; Cecchet, G.] Sez INFN Pavia, Pavia, Italy. [de Bari, A.; Cecchet, G.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Capponi, M.; Iaciofano, A.; Orestano, D.; Pastore, F.; Tortora, L.] Sez INFN Roma Tre, Rome, Italy. [Capponi, M.; Iaciofano, A.; Orestano, D.; Pastore, F.; Tortora, L.] Dipartimento Fis, Rome, Italy. [Kuno, Y.; Sakamato, H.] Osaka Univ, Dept Phys, Grad Sch Sci, Toyonaka, Osaka 560, Japan. [Ishimoto, S.] High Energy Accelerator Res Org, KEK, Inst Particle & Nucl Studies, Tsukuba, Ibaraki, Japan. [Filthaut, F.] Nikhef, Amsterdam, Netherlands. [Hansen, O. M.; Ramberger, S.; Vretenar, M.] CERN, Geneva, Switzerland. [Asfandiyarov, R.; Blondel, A.; Drielsma, F.; Karadzhov, Y.] Univ Geneva, DPNC, Sect Phys, CH-1211 Geneva, Switzerland. [Charnley, C.; Collomb, N.; Gallagher, A.; Grant, A.; Griffiths, S.; Hartnett, T.; Martlew, B.; Moss, A.; Mullacrane, I.; Oates, A.; Owens, P.; Stokes, G.; Warburton, P.; White, C.] STFC Daresbury Lab, Daresbury, Cheshire, England. [Adams, D.; Barclay, P.; Bayliss, V.; Brashaw, T. W.; Courthold, M.; Francis, V.; Fry, L.; Hayler, T.; Hills, M.; Lintern, A.; Macwaters, C.; Nichols, A.; Preece, R.; Ricciardi, S.; Rogers, C.; Stanley, T.; Tarrant, J.; Watson, S.; Wilson, A.] Harwell Oxford, STFC Rutherford Appleton Lab, Didcot, Oxon, England. [Bayes, R.; Nugent, J. C.; Soler, F. J. P.] Univ Glasgow, Sch Phys & Astron, Kelvin Bldg, Glasgow, Lanark, Scotland. [Cooke, P.; Gamet, R.] Univ Liverpool, Dept Phys, Liverpool L69 3BX, Merseyside, England. [Alekou, A.; Apollonio, M.; Barber, G.; Blackmore, V. J.; Colling, G.; Dobbs, A.; Dornan, P.; Hunt, C.; Lagrange, J. -B.; Long, K.; Martyniak, J.; Middleton, S.; Pasternak, J.; Santos, E.; Savidge, T.; Uchida, M. A.] Univ London Imperial Coll Sci Technol & Med, Dept Phys, Blackett Lab, London, England. [Blackmore, V. J.; Carlisle, T.; Cobb, J. H.; Lau, W.; Rayner, M. A.; Tunnell, C. D.] Univ Oxford, Dept Phys, Denys Wilkinson Bldg, Oxford, England. [Booth, C. N.; Hodgson, P.; Langlands, J.; Nicholson, R.; Overton, E.; Robinson, M.; Smith, P. J.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Dick, A.; Ronald, K.; Speirs, D.; Whyte, C. G.; Young, A.] Univ Strathclyde, Dept Phys, Glasgow, Lanark, Scotland. [Boyd, S.; Franchini, P.; Greis, J. R.; Pidcott, C.; Taylor, I.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Gardener, R.; Kyberd, P.; Littlefield, M.; Nebrensky, J. J.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Bross, A. D.; Fitzpatrick, T.; Leonova, M.; Moretti, A.; Neuffer, D.; Popovic, M.; Rubinov, P.; Rucinski, P.] Fermilab Natl Accelerator Lab, Batavia, IL USA. [Roberts, T. J.] Muons Inc, Batavia, IL USA. [Bowring, D.; DeMello, A.; Gourlay, S.; Li, D.; Prestemon, S.; Virostek, S.; Zisman, M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Drews, M.; Hanlet, P.; Kafka, G.; Kaplan, D. M.; Rajaram, D.; Snopok, P.; Torun, Y.; Winter, M.] IIT, Chicago, IL 60616 USA. [Blot, S.; Kim, Y. K.; Nichols, A.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Bravar, U.] Univ New Hampshire, Durham, NH 03824 USA. [Onel, Y.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Cremaldi, L. M.; Hart, T. L.; Luo, T.; Sanders, D. A.; Summers, D. J.] Univ Mississippi, Oxford, MS USA. [Cline, D.; Yang, X.] Univ Calif Los Angeles, Los Angeles, CA USA. [Coney, L.; Hanson, G. G.; Heidt, C.] Univ Calif Riverside, Riverside, CA 92521 USA. [Filthaut, F.] Radboud Univ Nijmegen, NL-6525 ED Nijmegen, Netherlands. RP Soler, FJP (reprint author), Univ Glasgow, Sch Phys & Astron, Kelvin Bldg, Glasgow, Lanark, Scotland. EM paul.soler@glasgow.ac.uk RI Soler, Paul/E-8464-2011; Asfandiyarov, Ruslan/B-5407-2017; OI Soler, Paul/0000-0002-4893-3729; Asfandiyarov, Ruslan/0000-0002-6631-9220; Nebrensky, Jindrich/0000-0002-8412-4259; Torun, Yagmur/0000-0003-2336-6585 FU Department of Energy and National Science Foundation (U.S.A.); Instituto Nazionale di Fisica Nucleare (Italy); Science and Technology Facilities Council (U.K.); European Community under the European Commission Framework Programme 7 (AIDA project) [262025]; European Community under the European Commission Framework Programme 7 (TIARA project) [261905]; European Community under the European Commission Framework Programme 7 (EuCARD); Japan Society for the Promotion of Science; Swiss National Science Foundation FX The work described here was made possible by grants from Department of Energy and National Science Foundation (U.S.A.), the Instituto Nazionale di Fisica Nucleare (Italy), the Science and Technology Facilities Council (U.K.), the European Community under the European Commission Framework Programme 7 (AIDA project, grant agreement no. 262025, TIARA project, grant agreement no. 261905, and EuCARD), the Japan Society for the Promotion of Science and the Swiss National Science Foundation, in the framework of the SCOPES programme. We gratefully acknowledge all sources of support. NR 39 TC 0 Z9 0 U1 2 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD MAR PY 2016 VL 11 AR P03001 DI 10.1088/1748-0221/11/03/P03001 PG 15 WC Instruments & Instrumentation SC Instruments & Instrumentation GA DL6JT UT WOS:000375746200064 ER PT J AU Agnes, P Agostino, L Albuquerque, IFM Alexandere, T Alton, AK Arisaka, K Back, HO Baldin, B Biery, K Bonfini, G Bossa, M Bottino, B Brigatti, A Brodsky, J Budano, F Bussino, S Cadeddu, M Cadonati, L Cadoni, M Calaprice, F Canci, N Candela, A Cao, H Cariello, M Carlini, M Catalanotti, S Cavalcante, P Chepurnov, A Cocco, AG Covone, G Crippa, L D'Angelo, D D'Incecco, M Davini, S De Cecco, S De Deo, M De Vincenzi, M Derbin, A Devoto, A Di Eusanio, F Di Pietro, G Edkins, E Empl, A Fan, A Fiorillo, G Fomenko, K Foster, G Franco, D Gabriele, F Galbiati, C Giganti, C Goretti, AM Granato, F Grandi, L Gromov, M Guan, M Guardincerri, Y Hackett, BR Herner, KR Hungerford, EV Ianni, A Ianni, A James, I Johnson, T Jollet, C Keeter, K Kendziora, CL Kobychev, V Koh, G Korablev, D Korga, G Kubankin, A Li, X Lissia, M Lombardi, P Luitz, S Ma, Y Machulin, IN Mandarano, A Mari, SM Maricic, J Marini, L Martoff, CJ Meregaglia, A Meyers, PD Miletic, T Milincic, R Montanari, D Monte, A Montuschi, M Monzani, ME Mosteiro, P Mount, BJ Muratova, VN Musico, P Napolitano, J Nelson, A Odrowski, S Orsini, M Ortica, F Pagani, L Pallavicini, M Pantic, E Parmeggiano, S Pelczar, K Pelliccia, N Perasso, S Pocar, A Pordes, S Pugachev, DA Qian, H Randle, K Ranucci, G Razeto, A Reinhold, B Renshaw, AL Romani, A Rossi, B Rossi, N Rountree, SD Sablone, D Saggese, P Saldanha, R Sands, W Sangiorgio, S Savarese, C Segreto, E Semenov, DA Shields, E Singh, PN Skorokhvatov, MD Smirnov, O Sotnikov, A Stanford, C Suvorov, Y Tartaglia, R Tatarowicz, J Testera, G Tonazzo, A Trinchese, P Unzhakov, EV Vishneva, A Vogelaar, RB Wada, M Walker, S Wang, H Wang, Y Watson, AW Westerdale, S Wilhelmi, J Wojcik, MM Xiang, X Xu, J Yang, C Yoo, J Zavatarelli, S Zec, A Zhong, W Zhu, C Zuzel, G AF Agnes, P. Agostino, L. Albuquerque, I. F. M. Alexandere, T. Alton, A. K. Arisaka, K. Back, H. O. Baldin, B. Biery, K. Bonfini, G. Bossa, M. Bottino, B. Brigatti, A. Brodsky, J. Budano, F. Bussino, S. Cadeddu, M. Cadonati, L. Cadoni, M. Calaprice, F. Canci, N. Candela, A. Cao, H. Cariello, M. Carlini, M. Catalanotti, S. Cavalcante, P. Chepurnov, A. Cocco, A. G. Covone, G. Crippa, L. D'Angelo, D. D'Incecco, M. Davini, S. De Cecco, S. De Deo, M. De Vincenzi, M. Derbin, A. Devoto, A. Di Eusanio, F. Di Pietro, G. Edkins, E. Empl, A. Fan, A. Fiorillo, G. Fomenko, K. Foster, G. Franco, D. Gabriele, F. Galbiati, C. Giganti, C. Goretti, A. M. Granato, F. Grandi, L. Gromov, M. Guan, M. Guardincerri, Y. Hackett, B. R. Herner, K. R. Hungerford, E. V. Ianni, Aldo Ianni, Andrea James, I. Johnson, T. Jollet, C. Keeter, K. Kendziora, C. L. Kobychev, V. Koh, G. Korablev, D. Korga, G. Kubankin, A. Li, X. Lissia, M. Lombardi, P. Luitz, S. Ma, Y. Machulin, I. N. Mandarano, A. Mari, S. M. Maricic, J. Marini, L. Martoff, C. J. Meregaglia, A. Meyers, P. D. Miletic, T. Milincic, R. Montanari, D. Monte, A. Montuschi, M. Monzani, M. E. Mosteiro, P. Mount, B. J. Muratova, V. N. Musico, P. Napolitano, J. Nelson, A. Odrowski, S. Orsini, M. Ortica, F. Pagani, L. Pallavicini, M. Pantic, E. Parmeggiano, S. Pelczar, K. Pelliccia, N. Perasso, S. Pocar, A. Pordes, S. Pugachev, D. A. Qian, H. Randle, K. Ranucci, G. Razeto, A. Reinhold, B. Renshaw, A. L. Romani, A. Rossi, B. Rossi, N. Rountree, S. D. Sablone, D. Saggese, P. Saldanha, R. Sands, W. Sangiorgio, S. Savarese, C. Segreto, E. Semenov, D. A. Shields, E. Singh, P. N. Skorokhvatov, M. D. Smirnov, O. Sotnikov, A. Stanford, C. Suvorov, Y. Tartaglia, R. Tatarowicz, J. Testera, G. Tonazzo, A. Trinchese, P. Unzhakov, E. V. Vishneva, A. Vogelaar, R. B. Wada, M. Walker, S. Wang, H. Wang, Y. Watson, A. W. Westerdale, S. Wilhelmi, J. Wojcik, M. M. Xiang, X. Xu, J. Yang, C. Yoo, J. Zavatarelli, S. Zec, A. Zhong, W. Zhu, C. Zuzel, G. TI The veto system of the DarkSide-50 experiment SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Neutron detectors (cold, thermal, fast neutrons); Scintillators, scintillation and light emission processes (solid, gas and liquid scintillators); Dark Matter detectors (WIMPs, axions, etc.); Cherenkov and transition radiation ID DEL GRAN SASSO; LIQUID SCINTILLATOR; BOREXINO DETECTOR; CALIBRATION; FACILITY; LNGS AB Nuclear recoil events produced by neutron scatters form one of the most important classes of background in WIMP direct detection experiments, as they may produce nuclear recoils that look exactly like WIMP interactions. In DarkSide-50, we both actively suppress and measure the rate of neutron-induced background events using our neutron veto, composed of a boron-loaded liquid scintillator detector within a water Cherenkov detector. This paper is devoted to the description of the neutron veto system of DarkSide-50, including the detector structure, the fundamentals of event reconstruction and data analysis, and basic performance parameters. C1 [Agnes, P.; Franco, D.; Perasso, S.; Tonazzo, A.] Univ Paris Diderot, APC, CNRS IN2P3, CEA Irfu,Obs Paris,Sorbonne Paris Cite, F-75205 Paris, France. [Agostino, L.; De Cecco, S.; Giganti, C.] Univ Paris 06, Univ Paris Diderot, CNRS IN2P3, LPNHE Paris, F-75252 Paris, France. [Albuquerque, I. F. M.; Back, H. O.; Brigatti, A.; Brodsky, J.; Calaprice, F.; Candela, A.; Cao, H.; Di Eusanio, F.; Galbiati, C.; Ianni, Andrea; Koh, G.; Li, X.; Meyers, P. D.; Mosteiro, P.; Nelson, A.; Pocar, A.; Qian, H.; Razeto, A.; Rossi, B.; Sands, W.; Shields, E.; Stanford, C.; Wada, M.; Westerdale, S.; Xiang, X.; Xu, J.; Zhu, C.] Princeton Univ, Dept Phys, Princeton, NJ 08544 USA. [Albuquerque, I. F. M.] Univ Sao Paulo, Inst Fis, BR-05508090 Sao Paulo, Brazil. [Alexandere, T.; Cadonati, L.; Foster, G.; Monte, A.; Pocar, A.; Randle, K.; Zec, A.] Univ Massachusetts, Amherst Ctr Fundamental Interact, Amherst, MA 01003 USA. [Alexandere, T.; Cadonati, L.; Foster, G.; Monte, A.; Pocar, A.; Randle, K.; Zec, A.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Alexandere, T.; Baldin, B.; Biery, K.; Foster, G.; Guardincerri, Y.; Herner, K. R.; Kendziora, C. L.; Montanari, D.; Pordes, S.; Yoo, J.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Alton, A. K.] Augustana Univ, Dept Phys, Sioux Falls, SD 57197 USA. [Arisaka, K.; Fan, A.; Renshaw, A. L.; Suvorov, Y.; Wang, H.; Wang, Y.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Back, H. O.] Pacific NW Natl Lab, Richland, WA 99354 USA. [Bonfini, G.; Canci, N.; Candela, A.; Carlini, M.; Cavalcante, P.; D'Incecco, M.; Davini, S.; De Deo, M.; Di Pietro, G.; Gabriele, F.; Goretti, A. M.; Ianni, Aldo; Korga, G.; Mandarano, A.; Montuschi, M.; Odrowski, S.; Orsini, M.; Razeto, A.; Rossi, N.; Sablone, D.; Savarese, C.; Suvorov, Y.; Tartaglia, R.] Lab Nazl Gran Sasso, I-67010 Assergi, AQ, Italy. [Bossa, M.; Davini, S.; Mandarano, A.; Savarese, C.] Gran Sasso Sci Inst, I-67100 Laquila, Italy. [Bottino, B.; Marini, L.; Pagani, L.; Pallavicini, M.] Univ Genoa, Dept Phys, I-16146 Genoa, Italy. [Bottino, B.; Brigatti, A.; Cariello, M.; Marini, L.; Musico, P.; Pagani, L.; Pallavicini, M.; Testera, G.; Zavatarelli, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Brigatti, A.; Crippa, L.; D'Angelo, D.; Di Pietro, G.; Galbiati, C.; Lombardi, P.; Parmeggiano, S.; Ranucci, G.; Saggese, P.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Brigatti, A.; Budano, F.; Bussino, S.; De Vincenzi, M.; James, I.; Mari, S. M.] Ist Nazl Fis Nucl, Sez Roma Tre, I-00146 Rome, Italy. [Budano, F.; Bussino, S.; De Vincenzi, M.; James, I.; Mari, S. M.] Univ Rome Tre, Dept Math & Phys, I-00146 Rome, Italy. [Cadeddu, M.; Cadoni, M.; Devoto, A.] Univ Cagliari, Dept Phys, I-09042 Cagliari, Italy. [Cadeddu, M.; Cadoni, M.; Devoto, A.; Lissia, M.] Ist Nazl Fis Nucl, Sez Cagliari, I-09042 Cagliari, Italy. [Canci, N.; Empl, A.; Hungerford, E. V.; Korga, G.; Renshaw, A. L.; Singh, P. N.] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Catalanotti, S.; Cocco, A. G.; Covone, G.; Fiorillo, G.; Rossi, B.; Walker, S.] Ist Nazl Fis Nucl, Sez Napoli, I-80126 Naples, Italy. [Catalanotti, S.; Covone, G.; Fiorillo, G.; Trinchese, P.; Walker, S.] Univ Naples Federico II, Dept Phys, I-80126 Naples, Italy. [Cavalcante, P.; Rountree, S. D.; Vogelaar, R. B.] Virginia Tech, Dept Phys, Blacksburg, VA 24061 USA. [Chepurnov, A.; Gromov, M.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow 119991, Russia. [Crippa, L.; D'Angelo, D.] Univ Milan, Dept Phys, I-20133 Milan, Italy. [Derbin, A.; Muratova, V. N.; Semenov, D. A.; Unzhakov, E. V.] St Petersburg Nucl Phys Inst, NRC Kurchatov Inst, Gatchina 188350, Russia. [Edkins, E.; Hackett, B. R.; Maricic, J.; Milincic, R.; Reinhold, B.] Univ Hawaii, Dept Phys & Astron, Honolulu, HI 96822 USA. [Fomenko, K.; Korablev, D.; Smirnov, O.; Sotnikov, A.; Vishneva, A.] Joint Inst Nucl Res, Dubna 141980, Russia. [Granato, F.; Martoff, C. J.; Miletic, T.; Napolitano, J.; Tatarowicz, J.; Watson, A. W.; Wilhelmi, J.] Temple Univ, Dept Phys, Philadelphia, PA 19122 USA. [Grandi, L.; Saldanha, R.] Univ Chicago, Enrico Fermi Inst, Kavli Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Grandi, L.; Saldanha, R.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Guan, M.; Ma, Y.; Wang, Y.; Yang, C.; Zhong, W.] Inst High Energy Phys, Beijing 100049, Peoples R China. [Ianni, Aldo] Canfranc Estn, Lab Subterraneo Canfranc, E-22880 Barcelona, Spain. [Jollet, C.; Meregaglia, A.] Univ Strasbourg, CNRS IN2P3, IPHC 19, F-67037 Strasbourg, France. [Keeter, K.; Mount, B. J.] Black Hills State Univ, Sch Nat Sci, Spearfish, SD 57799 USA. [Kobychev, V.] Natl Acad Sci Ukraine, Inst Natl Res, UA-03680 Kiev, Ukraine. [Kubankin, A.] Belgorod Natl Res Univ, Radiat Phys Lab, Belgorod 308007, Russia. [Monzani, M. E.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Machulin, I. N.; Pugachev, D. A.; Skorokhvatov, M. D.; Suvorov, Y.] Natl Res Ctr Kurchatov Inst, Moscow 123182, Russia. [Machulin, I. N.; Pugachev, D. A.; Skorokhvatov, M. D.] Natl Res Nucl Univ MEPhI, Moscow 115409, Russia. [Ortica, F.; Pelliccia, N.; Romani, A.] Univ Perugia, Dept Chem Biol & Biotechnol, I-06123 Perugia, Italy. [Ortica, F.; Pelliccia, N.; Romani, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06123 Perugia, Italy. [Johnson, T.; Pantic, E.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Pelczar, K.; Wojcik, M. M.; Zuzel, G.] Jagiellonian Univ, Smoluchowski Inst Phys, PL-30059 Krakow, Poland. [Sangiorgio, S.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Segreto, E.] Univ Estadual Campinas, Inst Phys Gleb Wataghin, BR-13083859 Sao Paulo, Brazil. [Wang, Y.] Univ Chinese Acad Sci, Sch Phys, Beijing 100049, Peoples R China. RP Westerdale, S (reprint author), Princeton Univ, Dept Phys, Princeton, NJ 08544 USA.; Davini, S (reprint author), Lab Nazl Gran Sasso, I-67010 Assergi, AQ, Italy.; Davini, S (reprint author), Gran Sasso Sci Inst, I-67100 Laquila, Italy. RI Romani, Aldo/G-8103-2012; Ortica, Fausto/C-1001-2013; Kubankin, Alexander/A-8745-2014; Fiorillo, Giuliana/A-2248-2012; DAngelo, Davide/K-9164-2013; Machulin, Igor/R-9711-2016; Skorokhvatov, Mikhail/R-9735-2016; Canci, Nicola/E-7498-2017; Covone, Giovanni/J-6040-2012; OI Romani, Aldo/0000-0002-7338-0097; Xu, Jingke/0000-0001-8084-5609; Ortica, Fausto/0000-0001-8276-452X; Fiorillo, Giuliana/0000-0002-6916-6776; DAngelo, Davide/0000-0001-9857-8107; Canci, Nicola/0000-0002-4797-4297; Catalanotti, Sergio/0000-0002-2337-4246; Covone, Giovanni/0000-0002-2553-096X; Brodsky, Jason/0000-0002-7498-6461; Franco, Davide/0000-0001-5604-2531; Unzhakov, Evgeniy/0000-0003-2952-6412; Rossi, Nicola/0000-0002-7046-528X; Wang, Yi/0000-0002-7351-6978 FU US NSF [PHY-0919363, PHY-1004072, PHY-1004054, PHY-1242585, PHY-1314483, PHY-1314507, PHY-1211308, PHY-1455351]; Italian Istituto Nazionale di Fisica Nucleare (INFN); US DOE [DE-FG02-91ER40671, DE-AC02-07CH11359]; Polish NCN [UMO-2012/05/E/ST2/02333]; UnivEarthS Labex program of Sorbonne Paris Cite [ANR-10-LABX-0023, ANR-11-IDEX-0005-02]; Sao Paulo Research Foundation (FAPESP) FX The DarkSide-50 Collaboration would like to thank LNGS laboratory and its staff for invaluable technical and logistical support. This report is based upon work supported by the US NSF (Grants PHY-0919363, PHY-1004072, PHY-1004054, PHY-1242585, PHY-1314483, PHY-1314507 and associated collaborative grants; grants PHY-1211308 and PHY-1455351), the Italian Istituto Nazionale di Fisica Nucleare (INFN), the US DOE (Contract Nos. DE-FG02-91ER40671 and DE-AC02-07CH11359), and the Polish NCN (Grant UMO-2012/05/E/ST2/02333). We thank the staff of the Fermilab Particle Physics, Scientific and Core Computing Divisions for their support. We acknowledge the financial support from the UnivEarthS Labex program of Sorbonne Paris Cite (ANR-10-LABX-0023 and ANR-11-IDEX-0005-02) and from the Sao Paulo Research Foundation (FAPESP). NR 47 TC 4 Z9 4 U1 10 U2 16 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD MAR PY 2016 VL 11 AR P03016 DI 10.1088/1748-0221/11/03/P03016 PG 41 WC Instruments & Instrumentation SC Instruments & Instrumentation GA DL6JT UT WOS:000375746200079 ER PT J AU Alexander, T Escobar, CO Lippincott, WH Rubinov, P AF Alexander, T. Escobar, C. O. Lippincott, W. H. Rubinov, P. TI Near-infrared scintillation of liquid argon SO JOURNAL OF INSTRUMENTATION LA English DT Article; Proceedings Paper CT Conference on Light Detection in Noble Elements (LIDINE) CY AUG 28-30, 2015 CL Albany, NY DE Scintillators, scintillation and light emission processes (solid, gas and liquid scintillators); Noble liquid detectors (scintillation, ionization, double-phase) ID EMISSION; KRYPTON; SPECTRA; XE; AR AB Since the 1970s it has been known that noble gases scintillate in the near infrared (NIR) region of the spectrum (0.7 mu m < lambda < 1.5 mu m). More controversial has been the question of the NIR light yield for condensed noble gases. We first present the motivation for using the NIR scintillation in liquid argon detectors, then briefly review early as well as more recent efforts and finally show encouraging preliminary results of a test performed at Fermilab. C1 [Alexander, T.; Escobar, C. O.; Lippincott, W. H.; Rubinov, P.] Fermilab Natl Accelerator Lab, Kirk Rd & Pine St, Batavia, IL 60510 USA. [Escobar, C. O.] Univ Estadual Campinas, Inst Fis, Rua Sergio Buarque de Holanda 777, BR-1308859 Campinas, SP, Brazil. RP Escobar, CO (reprint author), Fermilab Natl Accelerator Lab, Kirk Rd & Pine St, Batavia, IL 60510 USA.; Escobar, CO (reprint author), Univ Estadual Campinas, Inst Fis, Rua Sergio Buarque de Holanda 777, BR-1308859 Campinas, SP, Brazil. EM escobar@fnal.gov NR 25 TC 0 Z9 0 U1 3 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD MAR PY 2016 VL 11 AR C03010 DI 10.1088/1748-0221/11/03/C03010 PG 9 WC Instruments & Instrumentation SC Instruments & Instrumentation GA DL6JT UT WOS:000375746200011 ER PT J AU Fisher-Levine, M Nomerotski, A AF Fisher-Levine, M. Nomerotski, A. TI TimepixCam: a fast optical imager with time-stamping SO JOURNAL OF INSTRUMENTATION LA English DT Article; Proceedings Paper CT 17th International Workshop on Radiation Imaging Detectors CY JUN 28-JUL 02, 2015 CL DESY, Hamburg, GERMANY HO DESY DE Imaging spectroscopy; Mass spectrometers; Instrumentation and methods for time-of-flight (TOF) spectroscopy AB We describe a novel fast optical imager, TimepixCam, based on an optimized silicon pixel sensor with a thin entrance window, read out by a Timepix ASIC. TimepixCam is able to record and time-stamp light flashes in excess of 1,000 photons with high quantum efficiency in the 400-1000nm wavelength range with 20ns timing resolution, corresponding to an effective rate of 50 Megaframes per second. The camera was used for imaging ions impinging on a microchannel plate followed by a phosphor screen. Possible applications include spatial and velocity map imaging of ions in time-of-flight mass spectroscopy; coincidence imaging of ions and electrons, and other time-resolved types of imaging spectroscopy. C1 [Fisher-Levine, M.; Nomerotski, A.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Fisher-Levine, M (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM merlin.fisherlevine@gmail.com NR 12 TC 4 Z9 4 U1 2 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD MAR PY 2016 VL 11 AR C03016 DI 10.1088/1748-0221/11/03/C03016 PG 10 WC Instruments & Instrumentation SC Instruments & Instrumentation GA DL6JT UT WOS:000375746200017 ER PT J AU Ilieva, Y Allison, L Cao, T Kalicy, G Nadel-Turonski, P Park, K Schwarz, C Schwiening, J Zorn, C AF Ilieva, Y. Allison, L. Cao, T. Kalicy, G. Nadel-Turonski, P. Park, K. Schwarz, C. Schwiening, J. Zorn, C. TI MCP-PMT studies at the High-B test facility at Jefferson Lab SO JOURNAL OF INSTRUMENTATION LA English DT Article; Proceedings Paper CT International Workshop on Fast Cherenkov Detectors - Photon Detection, DIRC Design and DAQ CY NOV 11-13, 2015 CL Giessen, GERMANY DE Cherenkov detectors; Photon detectors for UV, visible and IR photons (solid-state); Photon detectors for UV, visible and IR photons (solid-state) (PIN diodes, APDs, Si-PMTs, G-APDs, CCDs, EBCCDs, EMCCDs etc) ID MICROCHANNEL PLATE PMTS; MAGNETIC-FIELDS; PERFORMANCE AB Here we present preliminary results for the gain performance of commercially available 3-mu m and 6-mu m pore-size single-anode microchannel-plate photomultipliers (MCP PMTs) in magnetic fields up to 5 T and for various orientations of the sensor relative to the field direction. The measurements were performed at Thomas Jefferson National Accelerator Facility in Newport News, VA. Our results show that smaller-pore-size PMTs have better gain performance in magnetic fields. At various angles, the shape of the gain dependence on the strength of the magnetic field strongly depends on the type of the sensor. Also, for each sensor, the azimuthal dependence is strongly correlated with the polar angle. Overall, the sensors exhibit a reasonable performance up to 2 T, although that upper limit depends on the sensor, the applied high voltage, and the orientation of the sensor relative to the field. To optimize the operational and design parameters of MCP PMTs for performance in high magnetic fields, further measurements and simulation studies will be pursued. Our studies are part of an R&D for development of a Detector of Internally Reflected Cherenkov Light for the central detector of a future U.S. Electron Ion Collider. C1 [Ilieva, Y.; Cao, T.] Univ S Carolina, 712 Main St, Columbia, SC 29208 USA. [Allison, L.; Kalicy, G.; Park, K.] Old Dominion Univ, 4600 Elkhorn Ave, Norfolk, VA 23529 USA. [Nadel-Turonski, P.; Zorn, C.] Thomas Jefferson Natl Accelerator Facil, 12000 Jefferson Ave, Newport News, VA 23606 USA. [Schwarz, C.; Schwiening, J.] GSI Helmholtzzentrum Schwerionenforsch GmbH, Planckstr 1, D-64291 Darmstadt, Germany. RP Ilieva, Y (reprint author), Univ S Carolina, 712 Main St, Columbia, SC 29208 USA. EM ilieva@sc.edu NR 14 TC 0 Z9 0 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD MAR PY 2016 VL 11 AR C03061 DI 10.1088/1748-0221/11/03/C03061 PG 10 WC Instruments & Instrumentation SC Instruments & Instrumentation GA DL6JT UT WOS:000375746200062 ER PT J AU Kadel, RW AF Kadel, R. W. TI On the analytic estimation of radioactive contamination from degraded alphas SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Dark Matter detectors (WIMPs, axions, etc.); Double-beta decay detectors; dE/dx detectors; Radiation calculations AB The high energy spectrum of alpha particles emitted from a single isotope uniformly contaminating a bulk solid has a flat energy spectrum with a high end cutoff energy equal to the maximal alpha kinetic energy (T-alpha) of the decay. In this flat region of the spectrum, we show the surface rate r(b) (Bq keV(-1) cm(-2)) arising from a bulk alpha contamination rho(b) (Bq cm(-3)) from a single isotope is given by r(b) = rho(b)Delta R/4 Delta E, where Delta E = E-1 - E-2 > 0 is the energy interval considered (keV) in the flat region of the spectrum and Delta R = R-2 - R-1 , where R-2 (R-1) is the amount of the bulk material (cm) necessary to degrade the energy of the alpha from T-alpha to E-2 (E-1). We compare our calculation to a rate measurement of alphas from Sm-147, (15.32 +/- 0.03% of Sm(nat) and half life of (1.06 +/- 0.01) x 10(11) yr [1]), and find good agreement, with the ratio between prediction to measurement of 100.2% +/- 1.6% (stat) +/- 2.1% (sys). We derive the condition for the flat spectrum, and also calculate the relationship between the decay rate measured at the surface for a [near] surface contamination with an exponential dependence on depth and a second case of an alpha source with a thin overcoat. While there is excellent agreement between our implementation of the sophisticated Monte Carlo program SRIM [2] and our intuitive model in all cases, both fail to describe the measured energy distribution of a Gd-148 alpha source with a thin (similar to 200 mu g cm(-2)) Au overcoat. We discuss possible origins of the disagreement and suggest avenues for future study. C1 [Kadel, R. W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM rwkadel@lbl.gov FU Office of Science, Office of High Energy Physics, of the U.S. Department of Energy [DE-AC02-05CH11231]; Richard W. Kadel Living Trust FX This work was supported by the Director, Office of Science, Office of High Energy Physics, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 and The Richard W. Kadel Living Trust. NR 13 TC 0 Z9 0 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD MAR PY 2016 VL 11 AR T03004 DI 10.1088/1748-0221/11/03/T03004 PG 19 WC Instruments & Instrumentation SC Instruments & Instrumentation GA DL6JT UT WOS:000375746200097 ER PT J AU Kazkaz, K Joshi, TH AF Kazkaz, K. Joshi, T. H. TI A model for the secondary scintillation pulse shape from a gas proportional scintillation counter SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Scintillators, scintillation and light emission processes (solid, gas and liquid scintillators); Detector modelling and simulations II (electric fields, charge transport, multiplication and; induction, pulse formation, electron emission, etc); Time projection Chambers (TPC); Gaseous detectors ID MONTE-CARLO-SIMULATION; ELECTRON-DRIFT; ARGON; KRYPTON; XENON; EFFICIENCIES; IONIZATION; ENERGY AB Proportional scintillation counters (PSCs), both single-and dual-phase, can measure the scintillation (S1) and ionization (S2) channels from particle interactions within the detector volume. The signal obtained from these detectors depends first on the physics of the medium (the initial scintillation and ionization), and second how the physics of the detector manipulates the resulting photons and liberated electrons. In this paper we develop a model of the detector physics that incorporates event topology, detector geometry, electric field configuration, purity, optical properties of components, and wavelength shifters. We present an analytic form of the model, which allows for general study of detector design and operation, and a Monte Carlo model which enables a more detailed exploration of S2 events. This model may be used to study systematic effects in current detectors such as energy and position reconstruction, pulse shape discrimination, event topology, dead time calculations, purity, and electric field uniformity. We present a comparison of this model with experimental data collected with an argon gas proportional scintillation counter (GPSC), operated at 20 C and 1 bar, and irradiated with an internal, collimated Fe-55 source. Additionally we discuss how the model may be incorporated in Monte Carlo simulations of both GPSCs and dual-phase detectors, increasing the reliability of the simulation results and allowing for tests of the experimental data analysis algorithms. C1 [Kazkaz, K.; Joshi, T. H.] Lawrence Livermore Natl Lab, Rare Event Detect Grp, 7000 East Ave, Livermore, CA USA. [Joshi, T. H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Kazkaz, K (reprint author), Lawrence Livermore Natl Lab, Rare Event Detect Grp, 7000 East Ave, Livermore, CA USA. EM kareem@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Lab-wide LDRD; Department of Homeland Security ARI FX We would like to thank M. Szydagis, S. Sangiorgio, and B. Lenardo for helpful discussions. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. Funded by Lab-wide LDRD and the Department of Homeland Security ARI. LLNL-JRNL-680202. NR 32 TC 1 Z9 1 U1 3 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD MAR PY 2016 VL 11 AR P03002 DI 10.1088/1748-0221/11/03/P03002 PG 15 WC Instruments & Instrumentation SC Instruments & Instrumentation GA DL6JT UT WOS:000375746200065 ER PT J AU Levy, C Fallon, S Genovesi, J Khaitan, D Klimov, K Mock, J Szydagis, M AF Levy, C. Fallon, S. Genovesi, J. Khaitan, D. Klimov, K. Mock, J. Szydagis, M. TI Xenon bubble chambers for direct dark matter detection SO JOURNAL OF INSTRUMENTATION LA English DT Article; Proceedings Paper CT Conference on Light Detection in Noble Elements (LIDINE) CY AUG 28-30, 2015 CL Albany, NY DE dE/dx detectors; Hybrid detectors; Dark Matter detectors (WIMPs, axions, etc.); Time projection chambers ID LIQUID XENON AB The search for dark matter is one of today's most exciting fields. As bigger detectors are being built to increase their sensitivity, background reduction is an ever more challenging issue. To this end, a new type of dark matter detector is proposed, a xenon bubble chamber, which would combine the strengths of liquid xenon TPCs, namely event by event energy resolution, with those of a bubble chamber, namely insensitivity to electronic recoils. In addition, it would be the first time ever that a dark matter detector is active on all three detection channels, ionization and scintillation characteristic of xenon detectors, and heat through bubble formation in superheated fluids. Preliminary simulations show that, depending on threshold, a discrimination of 99.99% to 99.9999+% can be achieved, which is on par or better than many current experiments. A prototype is being built at the University at Albany, SUNY. The prototype is currently undergoing seals, thermal, and compression testing. C1 [Levy, C.; Fallon, S.; Genovesi, J.; Mock, J.; Szydagis, M.] SUNY Albany, 1400 Washington Ave, Albany, NY 12222 USA. [Khaitan, D.] Univ Rochester, Rochester, NY 14627 USA. [Mock, J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Klimov, K.] SUNY Stony Brook, Stony Brook, NY 11794 USA. RP Levy, C (reprint author), SUNY Albany, 1400 Washington Ave, Albany, NY 12222 USA. EM clevy@albany.edu NR 26 TC 0 Z9 0 U1 3 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD MAR PY 2016 VL 11 AR C03003 DI 10.1088/1748-0221/11/03/C03003 PG 11 WC Instruments & Instrumentation SC Instruments & Instrumentation GA DL6JT UT WOS:000375746200005 ER PT J AU Lockwitz, S Jostlein, H AF Lockwitz, S. Jostlein, H. TI A study of dielectric breakdown along insulators surrounding conductors in liquid argon SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Time projection chambers; Neutrino detectors; Cryogenic detectors AB High voltage breakdown in liquid argon is an important concern in the design of liquid argon time projection chambers, which are often used as neutrino and dark matter detectors. We have made systematic measurements of breakdown voltages in liquid argon along insulators surrounding negative rod electrodes where the breakdown is initiated at the anode. The measurements were performed in an open cryostat filled with commercial grade liquid argon exposed to air, and not the ultra-pure argon required for electron drift. While not addressing all high voltage concerns in liquid argon, these measurements have direct relevance to the design of high voltage feedthroughs especially for averting the common problem of flash-over breakdown. The purpose of these tests is to understand the effects of materials, of breakdown path length, and of surface topology for this geometry and setup. We have found that the only material-specific effects are those due to their permittivity. We have found that the breakdown voltage has no dependence on the length of the exposed insulator. A model for the breakdown mechanism is presented that can help inform future designs. C1 [Lockwitz, S.; Jostlein, H.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. RP Lockwitz, S (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM lockwitz@fnal.gov FU United States Department of Energy [De-AC02-07 CH11359] FX Fermilab is operated by Fermi Research Alliance, LLC under Contract No. De-AC02-07 CH11359 with the United States Department of Energy. NR 13 TC 0 Z9 0 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD MAR PY 2016 VL 11 AR P03026 DI 10.1088/1748-0221/11/03/P03026 PG 14 WC Instruments & Instrumentation SC Instruments & Instrumentation GA DL6JT UT WOS:000375746200088 ER PT J AU Nakajima, Y Goldschmidt, A Matis, HS Miller, T Nygren, DR Oliveira, CAB Renner, J AF Nakajima, Y. Goldschmidt, A. Matis, H. S. Miller, T. Nygren, D. R. Oliveira, C. A. B. Renner, J. TI Measurement of scintillation and ionization yield with high-pressure gaseous mixtures of Xe and TMA for improved neutrinoless double beta decay and dark matter searches SO JOURNAL OF INSTRUMENTATION LA English DT Article; Proceedings Paper CT Conference on Light Detection in Noble Elements (LIDINE) CY AUG 28-30, 2015 CL Albany, NY DE Scintillators, scintillation and light emission processes (solid, gas and liquid scintillators); Double-beta decay detectors; Charge transport and multiplication in gas; Dark Matter detectors (WIMPs, axions, etc.) AB The gaseous Xenon(Xe) time projection chamber (TPC) is an attractive detector technique for neutrinoless double beta decay and WIMP dark matter searches. While it is less dense compared to Liquid Xe detectors, it has intrinsic advantages in tracking capability and better energy resolution. The performance of gaseous Xe can be further improved by molecular additives such as trimethylamine(TMA), which is expected to (1) cool down the ionization electrons, (2) convert Xe excitation energy to TMA ionizations through Penning transfer, and (3) produce scintillation and electroluminescence light in a more easily detectable wavelength (300 nm). In order to test the feasibility of the performance improvements with TMA, we made the first direct measurement of Penning and fluorescence transfer efficiency with gaseous mixtures of Xe and TMA. While we observed a Penning transfer efficiency up to similar to 35%, we found strong suppression of primary scintillation light with TMA. We also found that the primary scintillation light with Xe and TMA mixture can be well characterized by similar to 3% fluorescence transfer from Xe to TMA, with further suppression due to TMA self-quenching. No evidence of the scintillation light produced by recombination of TMA ions was found. This strong suppression of scintillation light makes dark matter searches quite challenging, while the possibility of improved neutrinoless double beta decay searches remains open. This work has been carried out within the context of the NEXT collaboration. C1 [Nakajima, Y.; Goldschmidt, A.; Matis, H. S.; Miller, T.; Nygren, D. R.; Oliveira, C. A. B.; Renner, J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Nygren, D. R.] Univ Texas Arlington, 701 S Nedderman Dr, Arlington, TX 76019 USA. RP Nakajima, Y (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM YNakajima@lbl.gov NR 10 TC 0 Z9 0 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD MAR PY 2016 VL 11 AR C03041 DI 10.1088/1748-0221/11/03/C03041 PG 8 WC Instruments & Instrumentation SC Instruments & Instrumentation GA DL6JT UT WOS:000375746200042 ER PT J AU Stolp, D Dalager, O Dhaliwal, N Godfrey, B Irving, M Kazkaz, K Manalaysay, A Neher, C Stephenson, S Tripathi, M AF Stolp, D. Dalager, O. Dhaliwal, N. Godfrey, B. Irving, M. Kazkaz, K. Manalaysay, A. Neher, C. Stephenson, S. Tripathi, M. TI An estimation of photon scattering length in tetraphenyl-butadiene SO JOURNAL OF INSTRUMENTATION LA English DT Article; Proceedings Paper CT Conference on Light Detection in Noble Elements (LIDINE) CY AUG 28-30, 2015 CL Albany, NY DE Photoemission; Optical detector readout concepts; Noble liquid detectors (scintillation, ionization, double-phase); Dark Matter detectors (WIMPs, axions, etc.) AB Tetraphenyl-butadiene (TPB) is a wavelength shifting material that can absorb ultraviolet photons and emit blue photons. It is used in the detection of vacuum ultraviolet (VUV) photons, for which typical photo-sensors, such as most photomultiplier tubes (PMT) and silicon photomultipliers (SiPM), do not have any quantum efficiency. The secondary blue light is emitted isotropically, however, due to scattering within the material, its angular distribution upon exiting the material can not be easily predicted. Here we describe a procedure for estimating the scattering length of blue light in TPB, by measuring and modeling the angular distribution as a function of layer thickness. The experiment consists of shining 254nm light at various thicknesses of TPB deposited on fused silica, and measuring the intensity of blue light using SiPMs on either side of the sample. We simulate light propagation within the sample to estimate the light yield and compare that to the data, which allows us to estimate mean scattering length for photons in TPB to be in the range 2-3 mu m, with some preference for a central value of 2.75 mu m. C1 [Stolp, D.; Dalager, O.; Dhaliwal, N.; Godfrey, B.; Irving, M.; Manalaysay, A.; Neher, C.; Stephenson, S.; Tripathi, M.] Univ Calif Davis, One Shields Ave, Davis, CA 95616 USA. [Kazkaz, K.] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA USA. RP Stolp, D (reprint author), Univ Calif Davis, One Shields Ave, Davis, CA 95616 USA. EM dostolp@ucdavis.com NR 4 TC 0 Z9 0 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD MAR PY 2016 VL 11 AR C03025 DI 10.1088/1748-0221/11/03/C03025 PG 12 WC Instruments & Instrumentation SC Instruments & Instrumentation GA DL6JT UT WOS:000375746200026 ER PT J AU Dongarra, J Heroux, MA Luszczek, P AF Dongarra, Jack Heroux, Michael A. Luszczek, Piotr TI A new metric for ranking high-performance computing systems SO NATIONAL SCIENCE REVIEW LA English DT Editorial Material C1 [Dongarra, Jack; Luszczek, Piotr] Univ Tennessee, Dept EECS, Innovat Comp Lab, Knoxville, TN 37996 USA. [Heroux, Michael A.] Sandia Natl Labs, Scalable Algorithms Dept, St Paul, MN USA. RP Dongarra, J (reprint author), Univ Tennessee, Dept EECS, Innovat Comp Lab, Knoxville, TN 37996 USA. EM dongarra@icl.utk.edu NR 10 TC 1 Z9 1 U1 1 U2 1 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 2095-5138 EI 2053-714X J9 NATL SCI REV JI Natl. Sci. Rev. PD MAR PY 2016 VL 3 IS 1 BP 30 EP 35 DI 10.1093/nsr/nwv084 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DJ4NT UT WOS:000374183700013 ER PT J AU Eudes, A Pereira, JH Yogiswara, S Wang, G Benites, VT Baidoo, EEK Lee, TS Adams, PD Keasling, JD Loque, D AF Eudes, Aymerick Pereira, Jose H. Yogiswara, Sasha Wang, George Benites, Veronica Teixeira Baidoo, Edward E. K. Lee, Taek Soon Adams, Paul D. Keasling, Jay D. Loque, Dominique TI Exploiting the Substrate Promiscuity of Hydroxycinnamoyl-CoA:Shikimate Hydroxycinnamoyl Transferase to Reduce Lignin SO PLANT AND CELL PHYSIOLOGY LA English DT Article DE Arabidopsis; Bioenergy; Cell wall; HCT; Lignin; Saccharification ID ESCHERICHIA-COLI; SHIKIMATE HYDROXYCINNAMOYLTRANSFERASE; PHENYLPROPANOID METABOLISM; SECONDARY METABOLISM; POPULUS-TRICHOCARPA; ACID BIOSYNTHESIS; CHLOROGENIC ACID; UBIC GENE; ARABIDOPSIS; PLANTS AB Lignin poses a major challenge in the processing of plant biomass for agro-industrial applications. For bioengineering purposes, there is a pressing interest in identifying and characterizing the enzymes responsible for the biosynthesis of lignin. Hydroxycinnamoyl-CoA:shikimate hydroxycinnamoyl transferase (HCT; EC 2.3.1.133) is a key metabolic entry point for the synthesis of the most important lignin monomers: coniferyl and sinapyl alcohols. In this study, we investigated the substrate promiscuity of HCT from a bryophyte (Physcomitrella) and from five representatives of vascular plants (Arabidopsis, poplar, switchgrass, pine and Selaginella) using a yeast expression system. We demonstrate for these HCTs a conserved capacity to acylate with p-coumaroyl-CoA several phenolic compounds in addition to the canonical acceptor shikimate normally used during lignin biosynthesis. Using either recombinant HCT from switchgrass (PvHCT2a) or an Arabidopsis stem protein extract, we show evidence of the inhibitory effect of these phenolics on the synthesis of p-coumaroyl shikimate in vitro, which presumably occurs via a mechanism of competitive inhibition. A structural study of PvHCT2a confirmed the binding of a non-canonical acceptor in a similar manner to shikimate in the active site of the enzyme. Finally, we exploited in Arabidopsis the substrate flexibility of HCT to reduce lignin content and improve biomass saccharification by engineering transgenic lines that overproduce one of the HCT non-canonical acceptors. Our results demonstrate conservation of HCT substrate promiscuity and provide support for a new strategy for lignin reduction in the effort to improve the quality of plant biomass for forage and cellulosic biofuels. C1 [Eudes, Aymerick; Pereira, Jose H.; Yogiswara, Sasha; Wang, George; Benites, Veronica Teixeira; Baidoo, Edward E. K.; Lee, Taek Soon; Adams, Paul D.; Keasling, Jay D.; Loque, Dominique] EmeryStn East, Joint BioEnergy Inst, 5885 Hollis St,4th Floor, Emeryville, CA 94608 USA. [Eudes, Aymerick; Yogiswara, Sasha; Wang, George; Benites, Veronica Teixeira; Baidoo, Edward E. K.; Lee, Taek Soon; Keasling, Jay D.; Loque, Dominique] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Syst & Engn Div, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Pereira, Jose H.; Adams, Paul D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Divg, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Yogiswara, Sasha; Keasling, Jay D.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Yogiswara, Sasha; Keasling, Jay D.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Benites, Veronica Teixeira] San Francisco State Univ, Grad Program, San Francisco, CA 94132 USA. RP Loque, D (reprint author), EmeryStn East, Joint BioEnergy Inst, 5885 Hollis St,4th Floor, Emeryville, CA 94608 USA.; Loque, D (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Syst & Engn Div, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM dloque@lbl.gov FU U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231]; National Institutes of Health, National Institute of General Medical Sciences; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was part of the DOE Joint BioEnergy Institute (http://www.jbei.org) supported by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, through contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the U.S. Department of Energy. The Berkeley Center for Structural Biology is supported in part by the National Institutes of Health, National Institute of General Medical Sciences. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 62 TC 5 Z9 5 U1 7 U2 21 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0032-0781 EI 1471-9053 J9 PLANT CELL PHYSIOL JI Plant Cell Physiol. PD MAR PY 2016 VL 57 IS 3 BP 568 EP 579 DI 10.1093/pcp/pcw016 PG 12 WC Plant Sciences; Cell Biology SC Plant Sciences; Cell Biology GA DJ9ZP UT WOS:000374572400011 PM 26858288 ER PT J AU Golub, M Lott, D Garamus, VM Laipple, D Stoermer, M Watkins, EB Schreyer, A Willumeit-Romer, R AF Golub, Maksym Lott, Dieter Garamus, Vasil M. Laipple, Daniel Stoermer, Michael Watkins, Erik B. Schreyer, Andreas Willumeit-Roemer, Regine TI Neutron study of phospholipids 1-palmitoyl-2-oleoyl-sn-glycero-3-phospho-ethanolamine spray coating on titanium implants SO BIOINTERPHASES LA English DT Article ID HUMAN-SERUM-ALBUMIN; LIPID-MEMBRANES; REFLECTIVITY; FLUCTUATIONS; MECHANISMS; INTERFACE; RAY AB Permanent implants made from titanium are widely used and successfully implemented in medicine to address problems related to orthopedic and oral disorders. However, implants that interact in all cases optimally and durably with bone tissue have yet to be developed. Here, the authors suggest a phospholipids 1-palmitoyl-2-oleoyl-sn-glycero-3-phospho-ethanolamine (POPE) lipid coating to partially mimic the biological cell membrane. To improve the homogeneity of the POPE distribution on the metal surface, the lipids are applied by spray coating. It is shown that the spray coating leads to two types of multilamellar POPE structures. Our experimental results demonstrate that these coatings are stable in a liquid environment in the range of physiological temperatures due to the unique interbilayer interaction of POPE lipids. Additionally, the interaction of the POPE multilayer structure with human serum albumin is considered. A simultaneous analysis of the specular and off-specular data provides structural information necessary to assess the quality of the coating for future applications. (C) 2015 American Vacuum Society. C1 [Golub, Maksym] Univ Grenoble 1, Inst Biol Struct, 71 Ave Martyrs, F-38000 Grenoble, France. [Lott, Dieter; Garamus, Vasil M.; Laipple, Daniel; Stoermer, Michael; Schreyer, Andreas; Willumeit-Roemer, Regine] Helmholtz Zentrum Geesthacht, Zentrum Mat & Kustenforsch HZG, Inst Mat Res, Max Plank Str 1, D-21502 Geesthacht, Germany. [Watkins, Erik B.] Los Alamos Natl Lab, Mat Phys & Applicat Div, Mat Synth & Integrated Devices Grp MPA 11, POB 1663,Mail Stop K763, Los Alamos, NM 87545 USA. RP Golub, M (reprint author), Univ Grenoble 1, Inst Biol Struct, 71 Ave Martyrs, F-38000 Grenoble, France. EM maksym.golub@hotmail.com NR 35 TC 0 Z9 0 U1 1 U2 3 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1934-8630 EI 1559-4106 J9 BIOINTERPHASES JI Biointerphases PD MAR PY 2016 VL 11 IS 1 AR 011002 DI 10.1116/1.4938556 PG 8 WC Biophysics; Materials Science, Biomaterials SC Biophysics; Materials Science GA DK5TB UT WOS:000374982200002 PM 26714450 ER PT J AU Troia, MJ Denk, MA Gido, KB AF Troia, Matthew J. Denk, Michael A. Gido, Keith B. TI Temperature-dependent performance as a driver of warm-water fish species replacement along the river continuum SO CANADIAN JOURNAL OF FISHERIES AND AQUATIC SCIENCES LA English DT Article ID STREAM FISHES; CLIMATE-CHANGE; COMPETITIVE INTERACTIONS; LIMITING FACTORS; COLORADO RIVER; ECOLOGY; ASSEMBLAGES; GRADIENTS; PATTERNS; MODEL AB Replacement of fish species by their congeners along gradients of stream size is common in warm-water streams, but the causative environmental factors driving this turnover are not fully understood. We used laboratory experiments to test for differences in temperature-dependent egg hatch success and age-0 food ration size for three congeneric cyprinids that differ in abundance along temperature-stream size gradients. Headwater species (Pimephales promelas and Pimephales notatus) had lower thermal optima and narrower thermal breadths for hatch success compared with a river mainstem species (Pimephales vigilax). Temperature sensitivity of ration size was lowest for P. promelas, intermediate for P. notatus, and highest for P. vigilax. Using an empirical stream temperature model, we predicted water temperatures and projected hatch success and ration size for 7974 stream segments in Kansas, USA. Projected hatch success from May to July and ration size from July to September generally matched abundance-stream size patterns, suggesting that increasing temperature along the river continuum may drive replacements among Pimephales species. Our findings combined with evaluations of timing and duration of spawning seasons will improve mechanistic understanding of species replacements along the river continuum. C1 [Troia, Matthew J.; Denk, Michael A.; Gido, Keith B.] Kansas State Univ, Div Biol, 116 Ackert Hall, Manhattan, KS 66506 USA. [Troia, Matthew J.] Oak Ridge Natl Lab, Div Environm Sci, POB 2008 MS6038, Oak Ridge, TN 37830 USA. RP Troia, MJ (reprint author), Kansas State Univ, Div Biol, 116 Ackert Hall, Manhattan, KS 66506 USA.; Troia, MJ (reprint author), Oak Ridge Natl Lab, Div Environm Sci, POB 2008 MS6038, Oak Ridge, TN 37830 USA. EM troiamj@gmail.com FU National Science Foundation (DEB) [1311183]; Southwestern Association of Naturalists; Prairie Biotic Research Inc.; Kansas Academy of Science FX The authors thank Nate Cathcart, Sky Hedden, Emily Johnson, Kevin Kirkbride, Josh Perkin, Dustin Shaw, Trevor Starks, Allison Veach, James Whitney, and Rebecca Zheng for field and laboratory assistance, as well as the Tallgrass Prairie National Preserve, Kansas Department of Wildlife Parks and Tourism, Joe and Alison Gerken, and many other private land owners for providing access to streams. The authors also thank Jake Schaefer for advice on experimental design and data analysis, as well as John Blair for use of equipment and laboratory facilities. This research was funded by the National Science Foundation (DEB No. 1311183), the Southwestern Association of Naturalists, Prairie Biotic Research Inc., and the Kansas Academy of Science. Brood stocks were collected under the permission of the Kansas Department of Wildlife Parks and Tourism (permit No. SC-089-2014) and housed and spawned under the permission of the Kansas State University Institutional Animal Care and Use Committee (permit No. 2996). This is publication 16-086-J from the Kansas Agricultural Experiment Station. The authors have no conflicts of interest to declare. NR 77 TC 1 Z9 1 U1 4 U2 9 PU CANADIAN SCIENCE PUBLISHING, NRC RESEARCH PRESS PI OTTAWA PA 65 AURIGA DR, SUITE 203, OTTAWA, ON K2E 7W6, CANADA SN 0706-652X EI 1205-7533 J9 CAN J FISH AQUAT SCI JI Can. J. Fish. Aquat. Sci. PD MAR PY 2016 VL 73 IS 3 BP 394 EP 405 DI 10.1139/cjfas-2015-0094 PG 12 WC Fisheries; Marine & Freshwater Biology SC Fisheries; Marine & Freshwater Biology GA DL1WM UT WOS:000375423600007 ER PT J AU Buizer, JL Dow, K Black, ME Jacobs, KL Waple, A Moss, RH Moser, S Luers, A Gustafson, DI Richmond, TC Hays, SL Field, CB AF Buizer, James L. Dow, Kirstin Black, Mary E. Jacobs, Katharine L. Waple, Anne Moss, Richard H. Moser, Susanne Luers, Amy Gustafson, David I. Richmond, T. C. Hays, Sharon L. Field, Christopher B. TI Building a sustained climate assessment process SO CLIMATIC CHANGE LA English DT Article AB The leaders and authors of the Third US National Climate Assessment (NCA3) developed new modes of engaging academia, the private sector, government agencies and civil society to support their needs for usable, rigorous, and timely information and better connect science and decision-making. A strategic vision for assessment activities into the future was built during the NCA3 process, including recommendations on how to establish a sustained assessment process that would integrate evolving scientific understanding into decision making to manage the risks of climate change over time. This vision includes a collaborative assessment process that involves partnerships across a diverse and widely distributed set of non-governmental and governmental entities. The new approach to assessments would produce timely, scientifically sound climate information products and processes, rather than focusing on the production of single quadrennial synthesis reports. If properly implemented, a sustained assessment would be more efficient and cost-effective, avoiding the painful and time-consuming process of beginning the assessment process anew every 4 years. This ongoing assessment would also encourage scientific and social innovations and explore new insights and opportunities, building the capacity to advance the development and delivery of climate information to meet societal requirements and benefit from scientific opportunities. C1 [Buizer, James L.; Black, Mary E.; Jacobs, Katharine L.] Univ Arizona, Tucson, AZ USA. [Dow, Kirstin] Univ S Carolina, Columbia, SC 29208 USA. [Waple, Anne] Second Nat, Boston, MA USA. [Moss, Richard H.] Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD USA. [Moss, Richard H.] Univ Maryland, College Pk, MD 20742 USA. [Moser, Susanne] Susanne Moser Res & Consulting, Santa Cruz, CA USA. [Luers, Amy] Skoll Global Threats Fund, San Francisco, CA USA. [Gustafson, David I.] ILSI Res Fdn, Washington, DC USA. [Richmond, T. C.] Van Ness Feldman LLP, Seattle, WA USA. [Hays, Sharon L.] Comp Sci Corp, Falls Church, VA USA. [Field, Christopher B.] Carnegie Inst Sci, Palo Alto, CA USA. RP Buizer, JL (reprint author), Univ Arizona, Tucson, AZ USA. EM buizer@email.arizona.edu NR 13 TC 7 Z9 7 U1 1 U2 3 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0165-0009 EI 1573-1480 J9 CLIMATIC CHANGE JI Clim. Change PD MAR PY 2016 VL 135 IS 1 BP 23 EP 37 DI 10.1007/s10584-015-1501-4 PG 15 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA DL2LG UT WOS:000375465700003 ER PT J AU Moss, RH AF Moss, Richard H. TI Assessing decision support systems and levels of confidence to narrow the climate information "usability gap" SO CLIMATIC CHANGE LA English DT Article ID CHANGE ADAPTATION; BARRIERS AB This article focuses on the implications for the US National Climate Assessment (NCA) of diversifying information needs to support climate change risk management. It describes how the Third US National Climate Assessment (NCA3) evolved to begin to narrow the gap between information from climate and impact scientists and "intermediaries" (individuals who have expertise in climate science, communication, and decision-support processes)-who are sometimes collectively described as "producers" in this article-and the decision-making needs of a wide range of "users" (individuals involved in advising or making a wide range of policy and management decisions). One step in the evolution of the NCA3 included adding a chapter to assess decision-support tools and systems being used in climate-related decisions. Another involved efforts to improve characterization of the level of confidence of NCA3 authors in their findings to help decision-makers and their advisors differentiate well-established and more preliminary conclusions. This paper lays out an argument for increasing the role of the NCA in assessing decision-support systems in the Fourth Assessment (NCA4) and the Sustained Assessment. It also briefly reviews approaches and potential next steps related to characterizing uncertainty and communicating confidence intended to improve application of assessment findings by decision-makers. C1 [Moss, Richard H.] Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD USA. [Moss, Richard H.] Univ Maryland, College Pk, MD 20742 USA. RP Moss, RH (reprint author), Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD USA.; Moss, RH (reprint author), Univ Maryland, College Pk, MD 20742 USA. EM rhm@pnnl.gov FU DOE by Battelle Memorial Institute [DE-AC05-76RL01830]; University of Arizona, Center for Climate Adaptation Science and Solutions FX The Joint Global Change Research Institute is part of the Pacific Northwest National Laboratory, which is operated for DOE by Battelle Memorial Institute under contract DE-AC05-76RL01830, and the University of Maryland. The author gratefully acknowledges the University of Arizona, Center for Climate Adaptation Science and Solutions, for providing intellectual and financial support during a period of residence as a visiting scholar when the first draft of this article was prepared. NR 31 TC 4 Z9 4 U1 4 U2 8 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0165-0009 EI 1573-1480 J9 CLIMATIC CHANGE JI Clim. Change PD MAR PY 2016 VL 135 IS 1 BP 143 EP 155 DI 10.1007/s10584-015-1549-1 PG 13 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA DL2LG UT WOS:000375465700011 ER PT J AU Moser, SC Melillo, JM Jacobs, KL Moss, RH Buizer, JL AF Moser, Susanne C. Melillo, Jerry M. Jacobs, Katharine L. Moss, Richard H. Buizer, James L. TI Aspirations and common tensions: larger lessons from the third US national climate assessment SO CLIMATIC CHANGE LA English DT Article ID CHANGE IMPACTS AB The Third US National Climate Assessment (NCA3) was produced by experts in response to the US Global Change Research Act of 1990. Based on lessons learned from previous domestic and international assessments, the NCA3 was designed to speak to a broad public and inform the concerns of policy-and decision-makers at different scales. The NCA3 was also intended to be the first step in an ongoing assessment process that would build the nation's capacity to respond to climate change. This concluding paper draws larger lessons from the insights gained throughout the assessment process that are of significance to future US and international assessment designers. We bring attention to process and products delivered, communication and engagement efforts, and how they contributed to the sustained assessment. Based on areas where expectations were exceeded or not fully met, we address four common tensions that all assessment designers must confront and manage: between (1) core assessment ingredients (knowledge base, institutional set-up, principled process, and the people involved), (2) national scope and subnational adaptive management information needs, (3) scope, complexity, and manageability, and (4) deliberate evaluation and ongoing learning approaches. Managing these tensions, amidst the social and political contexts in which assessments are conducted, is critical to ensure that assessments are feasible and productive, while its outcomes are perceived as credible, salient, and legitimate. C1 [Moser, Susanne C.] Stanford Univ, Susanne Moser Res & Consulting, Santa Cruz, CA USA. [Melillo, Jerry M.] Marine Biol Lab, Woods Hole, MA 02543 USA. [Jacobs, Katharine L.] Univ Arizona, Ctr Climate Adaptat Sci & Solut, Tucson, AZ USA. [Moss, Richard H.] Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD USA. [Buizer, James L.] Univ Arizona, Inst Environm, Climate Adaptat & Dev, Tucson, AZ USA. [Moser, Susanne C.] Stanford Univ, Woods Inst Environm, Palo Alto, CA 94304 USA. [Jacobs, Katharine L.] Univ Arizona, Dept Soil Water & Environm Sci, Tucson, AZ USA. [Buizer, James L.] Univ Arizona, Sch Nat Resources & Environm, Tucson, AZ USA. RP Moser, SC (reprint author), Stanford Univ, Susanne Moser Res & Consulting, Santa Cruz, CA USA.; Moser, SC (reprint author), Stanford Univ, Woods Inst Environm, Palo Alto, CA 94304 USA. EM promundi@susannemoser.com NR 13 TC 3 Z9 3 U1 2 U2 4 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0165-0009 EI 1573-1480 J9 CLIMATIC CHANGE JI Clim. Change PD MAR PY 2016 VL 135 IS 1 BP 187 EP 201 DI 10.1007/s10584-015-1530-z PG 15 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA DL2LG UT WOS:000375465700014 ER PT J AU Dharmarajan, G Beasley, JC Beatty, WS Olson, ZH Fike, JA Rhodes, OE AF Dharmarajan, Guha Beasley, James C. Beatty, William S. Olson, Zachary H. Fike, Jennifer A. Rhodes, Olin E., Jr. TI Genetic co-structuring in host-parasite systems: Empirical data from raccoons and raccoon ticks SO ECOSPHERE LA English DT Article DE animal movement; disease ecology; ectoparasite; kin structure; mesocarnivore; microsatellite; parasite; spatial structure; Upper Wabash River Basin ID COMPARATIVE POPULATION-GENETICS; PROCYON-LOTOR; DIFFERENTIATION MEASURE; TRANSMISSION DYNAMICS; FRAGMENTED LANDSCAPE; SPATIAL-ORGANIZATION; BOVINE TUBERCULOSIS; SCHISTOSOMA-MANSONI; MICROSATELLITE LOCI; ACARI IXODIDAE AB Many aspects of parasite biology critically depend on their hosts, and understanding how host-parasite populations are co-structured can help improve our understanding of the ecology of parasites, their hosts, and host-parasite interactions. This study utilized genetic data collected from raccoons (Procyon lotor), and a specialist parasite, the raccoon tick (Ixodes texanus), to test for genetic co-structuring of host-parasite populations at both landscape and host scales. At the landscape scale, our analyses revealed a significant correlation between genetic and geographic distance matrices (i.e., isolation by distance) in ticks, but not their hosts. While there are several mechanisms that could lead to a stronger pattern of isolation by distance in tick vs. raccoon datasets, our analyses suggest that at least one reason for the above pattern is the substantial increase in statistical power (due to the approximate to 8-fold increase in sample size) afforded by sampling parasites. Host-scale analyses indicated higher relatedness between ticks sampled from related vs. unrelated raccoons trapped within the same habitat patch, a pattern likely driven by increased contact rates between related hosts. By utilizing fine-scale genetic data from both parasites and hosts, our analyses help improve our understanding of epidemiology and host ecology. C1 [Dharmarajan, Guha; Beasley, James C.; Beatty, William S.; Olson, Zachary H.; Fike, Jennifer A.; Rhodes, Olin E., Jr.] Purdue Univ, Dept Forestry & Nat Resources, W Lafayette, IN 47907 USA. [Dharmarajan, Guha] Indian Inst Sci Educ & Res Kolkata, Dept Biol Sci, Mohanpur 741246, W Bengal, India. [Beasley, James C.] Univ Georgia, Savannah River Ecol Lab, Warnell Sch Forestry & Nat Resources, Aiken, SC 29802 USA. [Beatty, William S.] US Geol Survey, Alaska Sci Ctr, Anchorage, AK 99508 USA. [Olson, Zachary H.] Univ New England, Biddeford, ME 04005 USA. [Fike, Jennifer A.] Ft Collins Sci Ctr, Ft Collins, CO 80526 USA. [Rhodes, Olin E., Jr.] Univ Georgia, Savannah River Ecol Lab, Odum Sch Ecol, Aiken, SC 29802 USA. RP Rhodes, OE (reprint author), Purdue Univ, Dept Forestry & Nat Resources, W Lafayette, IN 47907 USA.; Rhodes, OE (reprint author), Univ Georgia, Savannah River Ecol Lab, Odum Sch Ecol, Aiken, SC 29802 USA. EM rhodes@srel.uga.edu OI Beatty, William/0000-0003-0013-3113 FU Purdue University; Department of Energy Office of Environmental Management [DE-FC09-07SR22506]; Department of Science and Technology, Government of India FX We thank the numerous landowners, who permitted us access to their land, for their cooperation. We also thank colleagues in the genetics laboratory at the Department of Forestry and Natural Resources and the numerous field assistants. Funding for this research was provided by Purdue University. This material is based on work supported by the Department of Energy Office of Environmental Management under award number DE-FC09-07SR22506. GD is supported through a Ramanujan Fellowship Grant from the Department of Science and Technology, Government of India. Any use of trade names is for descriptive purposes only and does not represent endorsement by the U.S. federal government. NR 98 TC 0 Z9 0 U1 9 U2 20 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2150-8925 J9 ECOSPHERE JI Ecosphere PD MAR PY 2016 VL 7 IS 3 AR e01269 DI 10.1002/ecs2.1269 PG 15 WC Ecology SC Environmental Sciences & Ecology GA DK4OB UT WOS:000374896800028 ER PT J AU Diefenderfer, HL Johnson, GE Thom, RM Buenau, KE Weitkamp, LA Woodley, CM Borde, AB Kropp, RK AF Diefenderfer, Heida L. Johnson, Gary E. Thom, Ronald M. Buenau, Kate E. Weitkamp, Laurie A. Woodley, Christa M. Borde, Amy B. Kropp, Roy K. TI Evidence-based evaluation of the cumulative effects of ecosystem restoration SO ECOSPHERE LA English DT Article DE causal criteria; critical thinking; cumulative effects; evidence-based medicine; fisheries; floodplain food web; habitat connectivity; hydropower mitigation; large-scale ecosystem restoration; salmon recovery; sustainability science; systematic review; tidal wetlands ID JUVENILE CHINOOK SALMON; LOWER COLUMBIA RIVER; RESTORED ESTUARINE WETLAND; DIEL FEEDING CHRONOLOGY; ONCORHYNCHUS-KISUTCH; COHO SALMON; FOOD WEBS; SEASONAL FLOODPLAIN; ADAPTIVE MANAGEMENT; GASTRIC EVACUATION AB This study adapts and applies the evidence-based approach for causal inference, a medical standard, to the restoration and sustainable management of large-scale aquatic ecosystems. Despite long-term investments in restoring aquatic ecosystems, it has proven difficult to adequately synthesize and evaluate program outcomes, and no standard method has been adopted. Complex linkages between restorative actions and ecosystem responses at a landscape scale make evaluations problematic and most programs focus on monitoring and analysis. Herein, we demonstrate a new transdisciplinary approach integrating techniques from evidence-based medicine, critical thinking, and cumulative effects assessment. Tiered hypotheses about the effects of landscape-scale restorative actions are identified using an ecosystem conceptual model. The systematic literature review, a health sciences standard since the 1960s, becomes just one of seven lines of evidence assessed collectively, using critical thinking strategies, causal criteria, and cumulative effects categories. As a demonstration, we analyzed data from 166 locations on the Columbia River and estuary representing 12 indicators of habitat and fish response to floodplain restoration actions intended to benefit culturally and economically important, threatened and endangered salmon. Synthesis of the lines of evidence demonstrated that hydrologic reconnection promoted macrodetritis export, prey availability, and juvenile fish access and feeding. Upon evaluation, the evidence was sufficient to infer cross-boundary, indirect, compounding, and delayed cumulative effects, and suggestive of nonlinear, landscape-scale, and spatial density effects. Therefore, on the basis of causal inferences regarding food-web functions, we concluded that the restoration program is having a cumulative beneficial effect on juvenile salmon. The lines of evidence developed are transferable to other ecosystems: modeling of cumulative net ecosystem improvement, physical modeling of ecosystem controlling factors, meta-analysis of restoration action effectiveness, analysis of data on target species, research on critical ecological uncertainties, evidence-based review of the literature, and change analysis on the landscape setting. As with medicine, the science of ecological restoration needs scientific approaches to management decisions, particularly because the consequences affect species extinctions and the availability of ecosystem services. This evidence-based approach will enable restoration in complex coastal, riverine, and tidal-fluvial ecosystems like the lower Columbia River to be evaluated when data have accumulated without sufficient synthesis. C1 [Diefenderfer, Heida L.; Johnson, Gary E.; Thom, Ronald M.; Buenau, Kate E.; Woodley, Christa M.; Borde, Amy B.; Kropp, Roy K.] Pacific NW Natl Lab, Marine Sci Lab, 1529 West Sequim Bay Rd, Sequim, WA 98382 USA. [Weitkamp, Laurie A.] NOAA, NW Fisheries Sci Ctr, Newport, OR 97365 USA. [Woodley, Christa M.] US Army Engineer Res & Dev Ctr, Vicksburg, MS 39180 USA. RP Diefenderfer, HL (reprint author), Pacific NW Natl Lab, Marine Sci Lab, 1529 West Sequim Bay Rd, Sequim, WA 98382 USA. EM heida.diefenderfer@pnnl.gov OI Buenau, Kate/0000-0003-2156-7260 FU U.S. Army Corps of Engineers, Portland District; NOAA Fisheries; Northwest Fisheries Science Center; U.S. Army Corps of Engineers, Walla Walla District FX We appreciate the financial support of the U.S. Army Corps of Engineers, Portland District. We are grateful to biologists B Ebberts, C Studebaker, and C Roegner for their leadership. Data collection by L Weitkamp was funded by the NOAA Fisheries, Northwest Fisheries Science Center and collection by C Woodley was funded by U.S. Army Corps of Engineers, Portland District and Walla Walla District. We thank A Cameron, A Coleman, V Cullinan, E Dawley, B Ebberts, M Hudson, J Johnson, L Johnson, K MacNeale, K Marcoe, R McNatt, D Putman, M Russell, N Sather, J Skalski, K Sobocinski, and A Uber for their contributions and others for help in the field and laboratory. HLD thanks B. Brehm, D. Qualley, and P. Steinberger for guidance on critical reasoning and judgment. NR 136 TC 3 Z9 3 U1 25 U2 54 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2150-8925 J9 ECOSPHERE JI Ecosphere PD MAR PY 2016 VL 7 IS 3 AR e01242 DI 10.1002/ecs2.1242 PG 33 WC Ecology SC Environmental Sciences & Ecology GA DK4OB UT WOS:000374896800014 ER PT J AU Pepin, KM Davis, AJ Beasley, J Boughton, R Campbell, T Cooper, SM Gaston, W Hartley, S Kilgo, JC Wisely, SM Wyckoff, C VerCauteren, KC AF Pepin, Kim M. Davis, Amy J. Beasley, James Boughton, Raoul Campbell, Tyler Cooper, Susan M. Gaston, Wes Hartley, Steve Kilgo, John C. Wisely, Samantha M. Wyckoff, Christy VerCauteren, Kurt C. TI Contact heterogeneities in feral swine: implications for disease management and future research SO ECOSPHERE LA English DT Article DE contact; disease transmission; feral swine; GPS; meta-analysis; network; social structure; Sus scrofa ID WILD BOARS; EPIDEMIOLOGY; TRANSMISSION; NETWORKS; PATTERNS; CATTLE; MODELS; VIRUS; TEXAS; PIGS AB Contact rates vary widely among individuals in socially structured wildlife populations. Understanding the interplay of factors responsible for this variation is essential for planning effective disease management. Feral swine (Sus scrofa) are a socially structured species which pose an increasing threat to livestock and human health, and little is known about contact structure. We analyzed 11 GPS data sets from across the United States to understand the interplay of ecological and demographic factors on variation in co-location rates, a proxy for contact rates. Between-sounder contact rates strongly depended on the distance among home ranges (less contact among sounders separated by >2 km; negligible between sounders separated by >6 km), but other factors causing high clustering between groups of sounders also seemed apparent. Our results provide spatial parameters for targeted management actions, identify data gaps that could lead to improved management and provide insight on experimental design for quantitating contact rates and structure. C1 [Pepin, Kim M.; Davis, Amy J.; VerCauteren, Kurt C.] USDA, Natl Wildlife Res Ctr, 4101 Laporte Ave, Ft Collins, CO 80526 USA. [Beasley, James] Univ Georgia, Savannah River Ecol Lab, Warnell Sch Forestry & Nat Resources, PO Drawer E, Aiken, SC 29802 USA. [Boughton, Raoul] Univ Florida, Wildlife Ecol & Conservat, Range Cattle Res & Educ Ctr, 3401 Expt Stn, Ona, FL 33865 USA. [Campbell, Tyler] East Fdn, 200 Concord Plaza Dr,Suite 410, San Antonio, TX 78216 USA. [Cooper, Susan M.] Texas A&M AgriLife Res, 1619 Garner Field Rd, Uvalde, TX 78801 USA. [Gaston, Wes] USDA APHIS Wildlife Serv, Auburn, AL 36849 USA. [Hartley, Steve] US Geol Survey, Natl Wetlands Res Ctr, 700 Cajundome Blvd, Lafayette, LA 70506 USA. [Kilgo, John C.] US Forest Serv, Southern Res Stn, USDA, POB 700, New Ellenton, SC 29809 USA. [Wisely, Samantha M.] Univ Florida, Dept Wildlife Ecol & Conservat, Gainesville, FL 32611 USA. [Wyckoff, Christy] Santa Lucia Conservancy, 26700 Rancho San Carlos Rd, Carmel, CA 93923 USA. [Wyckoff, Christy] Texas A&M Univ Kingsville, Caesar Kleberg Wildlife Res Inst, 955 Univ Blvd, Kingsville, TX 78363 USA. RP Pepin, KM (reprint author), USDA, Natl Wildlife Res Ctr, 4101 Laporte Ave, Ft Collins, CO 80526 USA. EM kim.m.pepin@aphis.usda.gov FU U.S. Department of Agriculture National Wildlife Research Center; U.S. Department of Energy [DE-FC09-07SR22506, DE-AI09-00SR22188]; U.S. Department of Agriculture Forest Service Savannah River; USDA NWRC [1274120896CA] FX We thank two anonymous reviewers for their careful, insightful reviews of an earlier version of this manuscript. Funding was provided by the U.S. Department of Agriculture National Wildlife Research Center and the U.S. Department of Energy under Award Number DE-FC09-07SR22506 to the University of Georgia Research Foundation and under Interagency Agreement No. DE-AI09-00SR22188 with the U.S. Department of Agriculture Forest Service Savannah River. USDA NWRC provided funding to University of Florida under USDA APHIS Cooperative Agreement 1274120896CA. NR 26 TC 2 Z9 2 U1 7 U2 13 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2150-8925 J9 ECOSPHERE JI Ecosphere PD MAR PY 2016 VL 7 IS 3 AR e01230 DI 10.1002/ecs2.1230 PG 11 WC Ecology SC Environmental Sciences & Ecology GA DK4OB UT WOS:000374896800009 ER PT J AU Boman, EG Deweese, K Gilbert, JR AF Boman, Erik G. Deweese, Kevin Gilbert, John R. TI Evaluating the Dual Randomized Kaczmarz Laplacian Linear Solver SO INFORMATICA-JOURNAL OF COMPUTING AND INFORMATICS LA English DT Article DE Laplacian solver; randomized Kaczmarz; cycle basis ID PRECONDITIONERS AB A new method for solving Laplacian linear systems proposed by Kelner et al. involves the random sampling and update of fundamental cycles in a graph. Kelner et al. proved asymptotic bounds on the complexity of this method but did not report experimental results. We seek to both evaluate the performance of this approach and to explore improvements to it in practice. We compare the performance of this method to other Laplacian solvers on a variety of real world graphs. We consider different ways to improve the performance of this method by exploring different ways of choosing the set of cycles and the sequence of updates, with the goal of providing more flexibility and potential parallelism. We propose a parallel model of the Kelner et al. method, for evaluating potential parallelism in terms of the span of edges updated at each iteration. We provide experimental results comparing the potential parallelism of the fundamental cycle basis and our extended cycle set. Our preliminary experiments show that choosing a non-fundamental set of cycles can save significant work compared to a fundamental cycle basis. C1 [Boman, Erik G.] Sandia Natl Labs, Ctr Res Comp, Livermore, CA 94550 USA. [Deweese, Kevin; Gilbert, John R.] UC Santa Barbara, Dept Comp Sci, Santa Barbara, CA USA. RP Boman, EG (reprint author), Sandia Natl Labs, Ctr Res Comp, Livermore, CA 94550 USA.; Deweese, K; Gilbert, JR (reprint author), UC Santa Barbara, Dept Comp Sci, Santa Barbara, CA USA. EM egboman@sandia.gov; kdeweese@cs.ucsb.edu; gilbert@cs.ucsb.edu NR 27 TC 1 Z9 1 U1 0 U2 0 PU SLOVENSKO DRUSTVO INFORMATIKA PI LJUBLJANA PA VOZARSKI POT 12, LJUBLJANA, 1000, SLOVENIA SN 0350-5596 J9 INFORM-J COMPUT INFO JI Inform.-J. Comput. Inform. PD MAR PY 2016 VL 40 IS 1 BP 95 EP 107 PG 13 WC Computer Science, Software Engineering SC Computer Science GA DK7SD UT WOS:000375125100009 ER PT J AU Kim, W Braun, JE AF Kim, Woohyun Braun, James E. TI Development and evaluation of virtual refrigerant mass flow sensors for fault detection and diagnostics SO INTERNATIONAL JOURNAL OF REFRIGERATION-REVUE INTERNATIONALE DU FROID LA English DT Article DE Virtual sensor; Refrigerant mass flow rate; Fault detection and diagnostics; Compressor; Expansion device; Performance monitoring ID EXPANSION VALVES; SPEED; PERFORMANCE; SYSTEMS AB Refrigerant mass flow rate is an important measurement for monitoring equipment performance and enabling fault detection and diagnostics. This paper presents and evaluates three different virtual refrigerant mass flow (VRMF) sensors that use mathematical models to estimate flow rate using low cost measurements. The first model uses a compressor map that relates refrigerant flow rate to measurements of condensing and evaporating saturation temperature, and to compressor inlet temperature measurements. The second model uses an energy-balance method on the compressor that uses the compressor power consumption. The third model is developed using an empirical correlation for an electronic expansion valve (EEV) based on an orifice equation. The three VRMFs are shown to work well in estimating refrigerant mass flow rate for various systems under fault-free conditions with less than 5% RMS error. The combination of the three VRMFs can be utilized to detect and diagnose when the compressor and/or expansion device is not providing the expected flow. (C) 2016 Elsevier Ltd and International Institute of Refrigeration. All rights reserved. C1 [Kim, Woohyun] Pacific NW Natl Lab, Richland, WA 99352 USA. [Braun, James E.] Purdue Univ, Herrick Lab Mech Engn, W Lafayette, IN 47906 USA. RP Kim, W (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM Woohyun.Kim@pnnl.gov FU Department of Energy through the Consortium for Building Energy Innovation FX This work was supported by the Department of Energy through the Consortium for Building Energy Innovation (formerly the Energy Efficient Buildings Hub). NR 23 TC 0 Z9 0 U1 3 U2 5 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0140-7007 EI 1879-2081 J9 INT J REFRIG JI Int. J. Refrig.-Rev. Int. Froid PD MAR PY 2016 VL 63 BP 184 EP 198 DI 10.1016/j.ijrefrig.2015.11.005 PG 15 WC Thermodynamics; Engineering, Mechanical SC Thermodynamics; Engineering GA DK5ZT UT WOS:000375000600017 ER PT J AU Romps, DM AF Romps, David M. TI The Stochastic Parcel Model: A deterministic parameterization of stochastically entraining convection SO JOURNAL OF ADVANCES IN MODELING EARTH SYSTEMS LA English DT Article DE Stochastic Parcel Model; convective parameterization ID HIGH-RESOLUTION SIMULATION; GENERAL-CIRCULATION MODEL; DEEP CUMULUS CONVECTION; LARGE-SCALE MODELS; MASS-FLUX SCHEME; CLIMATE SENSITIVITY; COLD POOLS; QUASI-EQUILIBRIUM; ARAKAWA-SCHUBERT; CLOUD ENSEMBLE AB Convective entrainment is a process that is poorly represented in existing convective parameterizations. By many estimates, convective entrainment is the leading source of error in global climate models. As a potential remedy, an Eulerian implementation of the Stochastic Parcel Model (SPM) is presented here as a convective parameterization that treats entrainment in a physically realistic and computationally efficient way. Drawing on evidence that convecting clouds comprise air parcels subject to Poisson-process entrainment events, the SPM calculates the deterministic limit of an infinite number of such parcels. For computational efficiency, the SPM groups parcels at each height by their purity, which is a measure of their total entrainment up to that height. This reduces the calculation of convective fluxes to a sequence of matrix multiplications. The SPM is implemented in a single-column model and compared with a large-eddy simulation of deep convection. C1 [Romps, David M.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Romps, David M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Climate & Ecosyst Sci Div, Berkeley, CA 94720 USA. RP Romps, DM (reprint author), Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA.; Romps, DM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Climate & Ecosyst Sci Div, Berkeley, CA 94720 USA. EM romps@berkeley.edu FU Scientific Discovery through Advanced Computing (SciDAC) program - U.S. Department of Energy Office of Advanced Scientific Computing Research [DE-AC02-05CH11231]; Scientific Discovery through Advanced Computing (SciDAC) program - U.S. Department of Energy Office of Biological and Environmental Research [DE-AC02-05CH11231] FX This work was supported by the Scientific Discovery through Advanced Computing (SciDAC) program funded by the U.S. Department of Energy Office of Advanced Scientific Computing Research and Office of Biological and Environmental Research under contract DE-AC02-05CH11231. We note that there are no data sharing issues since all of the numerical information is provided in the figures. NR 56 TC 3 Z9 3 U1 3 U2 5 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 1942-2466 J9 J ADV MODEL EARTH SY JI J. Adv. Model. Earth Syst. PD MAR PY 2016 VL 8 IS 1 BP 319 EP 344 DI 10.1002/2015MS000537 PG 26 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DK2UP UT WOS:000374770200016 ER PT J AU Lasue, J Clegg, SM Forni, O Cousin, A Wiens, RC Lanza, N Mangold, N Le Deit, L Gasnault, O Maurice, S Berger, JA Stack, K Blaney, D Fabre, C Goetz, W Johnson, J Le Mouelic, S Nachon, M Payre, V Rapin, W Sumner, DY AF Lasue, J. Clegg, S. M. Forni, O. Cousin, A. Wiens, R. C. Lanza, N. Mangold, N. Le Deit, L. Gasnault, O. Maurice, S. Berger, J. A. Stack, K. Blaney, D. Fabre, C. Goetz, W. Johnson, J. Le Mouelic, S. Nachon, M. Payre, V. Rapin, W. Sumner, D. Y. TI Observation of > 5wt % zinc at the Kimberley outcrop, Gale crater, Mars SO JOURNAL OF GEOPHYSICAL RESEARCH-PLANETS LA English DT Article DE Mars; data reduction technique; laser-induced breakdown spectroscopy (LIBS) ID SCIENCE LABORATORY MISSION; CHEMCAM INSTRUMENT SUITE; CONTINENTAL-CRUST; MINERALOGY; ROCKS; ROVER; GEOCHEMISTRY; EVOLUTION; DEPOSIT; ORIGIN AB Zinc-enriched targets have been detected at the Kimberley formation, Gale crater, Mars, using the Chemistry Camera (ChemCam) instrument. The Zn content is analyzed with a univariate calibration based on the 481.2nm emission line. The limit of quantification for ZnO is 3wt % (at 95% confidence level) and 1wt % (at 68% confidence level). The limit of detection is shown to be around 0.5wt %. As of sol 950, 12 targets on Mars present high ZnO content ranging from 1.0wt % to 8.4wt % (Yarrada, sol 628). Those Zn-enriched targets are almost entirely located at the Dillinger member of the Kimberley formation, where high Mn and alkali contents were also detected, probably in different phases. Zn enrichment does not depend on the textures of the rocks (coarse-grained sandstones, pebbly conglomerates, and resistant fins). The lack of sulfur enhancement suggests that Zn is not present in the sphalerite phase. Zn appears somewhat correlated with Na2O and the ChemCam hydration index, suggesting that it could be in an amorphous clay phase (such as sauconite). On Earth, such an enrichment would be consistent with a supergene alteration of a sphalerite gossan cap in a primary siliciclastic bedrock or a possible hypogene nonsulfide zinc deposition where Zn, Fe, Mn would have been transported in a reduced sulfur-poor fluid and precipitated rapidly in the form of oxides. C1 [Lasue, J.; Forni, O.; Cousin, A.; Gasnault, O.; Maurice, S.; Rapin, W.] CNRS, OMP, IRAP, Toulouse, France. [Lasue, J.; Forni, O.; Cousin, A.; Gasnault, O.; Maurice, S.; Rapin, W.] UPS, OMP, IRAP, Toulouse, France. [Clegg, S. M.] Los Alamos Natl Lab, C PCS, MS J565, Los Alamos, NM USA. [Wiens, R. C.; Lanza, N.; Le Mouelic, S.; Nachon, M.] Los Alamos Natl Lab, ISR, MS D466, Los Alamos, NM USA. [Mangold, N.; Le Deit, L.; Le Mouelic, S.; Nachon, M.] Los Alamos Natl Lab, CNRS UMR 6112, LPGNantes, Lab Planetol & Geodynam, POB 1663, Los Alamos, NM USA. [Berger, J. A.; Payre, V.] Univ Western Ontario, Dept Earth Sci, London, ON, Canada. [Stack, K.; Blaney, D.; Sumner, D. Y.] CALTECH, Jet Prop Lab, Pasadena, CA 91125 USA. [Fabre, C.] Lorraine Univ, CNRS, GeoRessources, Vandoeuvre Les Nancy, France. [Goetz, W.] Max Planck Inst Stromungsforsch, Bunsenstr 10, D-37073 Gottingen, Germany. [Johnson, J.] Johns Hopkins Univ, Appl Phys Lab, Laurel, MD USA. RP Lasue, J (reprint author), CNRS, OMP, IRAP, Toulouse, France.; Lasue, J (reprint author), UPS, OMP, IRAP, Toulouse, France. EM jlasue@irap.omp.eu RI Gasnault, Olivier/F-4327-2010; OI Gasnault, Olivier/0000-0002-6979-9012; Clegg, Sam/0000-0002-0338-0948 FU NASA Mars Exploration Program; CNES; CNRS FX The authors acknowledge fruitful discussions with Ralf Gellert. We are grateful to C.A. Johnson, P. Giesting, and M. Boni for very constructive and useful comments which helped significantly improve the manuscript. Funding for MSL and ChemCam operations and science in the U.S. was provided by the NASA Mars Exploration Program. Funding for ChemCam operations in France was provided by CNES; science funding in France was provided by CNRS. The authors gratefully acknowledge the support of all of the people at JPL involved in making MSL a successful mission. The data used in this study were generated by the ChemCam and the Mars Science Laboratory teams and are freely available at the Planetary Data Systemof NASA (https://pds.jpl.nasa.gov/). All data described in the text are indicated together with the spacecraft clock and three letters that describe the type of data used, which singly identify the data in PDS. NR 62 TC 5 Z9 5 U1 4 U2 11 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9097 EI 2169-9100 J9 J GEOPHYS RES-PLANET JI J. Geophys. Res.-Planets PD MAR PY 2016 VL 121 IS 3 BP 338 EP 352 DI 10.1002/2015JE004946 PG 15 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DJ6VY UT WOS:000374352500005 ER PT J AU Mangold, N Thompson, LM Forni, O Williams, AJ Fabre, C Le Deit, L Wiens, RC Williams, R Anderson, RB Blaney, DL Calef, F Cousin, A Clegg, SM Dromart, G Dietrich, WE Edgett, KS Fisk, MR Gasnault, O Gellert, R Grotzinger, JP Kah, L Le Mouelic, S McLennan, SM Maurice, S Meslin, PY Newsom, HE Palucis, MC Rapin, W Sautter, V Siebach, KL Stack, K Sumner, D Yingst, A AF Mangold, N. Thompson, L. M. Forni, O. Williams, A. J. Fabre, C. Le Deit, L. Wiens, R. C. Williams, R. Anderson, R. B. Blaney, D. L. Calef, F. Cousin, A. Clegg, S. M. Dromart, G. Dietrich, W. E. Edgett, K. S. Fisk, M. R. Gasnault, O. Gellert, R. Grotzinger, J. P. Kah, L. Le Mouelic, S. McLennan, S. M. Maurice, S. Meslin, P-Y. Newsom, H. E. Palucis, M. C. Rapin, W. Sautter, V. Siebach, K. L. Stack, K. Sumner, D. Yingst, A. TI Composition of conglomerates analyzed by the Curiosity rover: Implications for Gale Crater crust and sediment sources SO JOURNAL OF GEOPHYSICAL RESEARCH-PLANETS LA English DT Article DE Mars; fluvial; sedimentary rocks; Gale Crater ID CHEMCAM INSTRUMENT SUITE; CONTINENTAL-CRUST; YELLOWKNIFE BAY; MARTIAN CRUST; GRAIN-SIZE; MARS; EVOLUTION; DIVERSITY; METEORITE; OLIVINE AB The Curiosity rover has analyzed various detrital sedimentary rocks at Gale Crater, among which fluvial and lacustrine rocks are predominant. Conglomerates correspond both to the coarsest sediments analyzed and the least modified by chemical alteration, enabling us to link their chemistry to that of source rocks on the Gale Crater rims. In this study, we report the results of six conglomerate targets analyzed by Alpha-Particle X-ray Spectrometer and 40 analyzed by ChemCam. The bulk chemistry derived by both instruments suggests two distinct end-members for the conglomerate compositions. The first group (Darwin type) is typical of conglomerates analyzed before sol 540; it has a felsic alkali-rich composition, with a Na2O/K2O>5. The second group (Kimberley type) is typical of conglomerates analyzed between sols 540 and 670 in the vicinity of the Kimberley waypoint; it has an alkali-rich potassic composition with Na2O/K2O<2. The variety of chemistry and igneous textures (when identifiable) of individual clasts suggest that each conglomerate type is a mixture of multiple source rocks. Conglomerate compositions are in agreement with most of the felsic alkali-rich float rock compositions analyzed in the hummocky plains. The average composition of conglomerates can be taken as a proxy of the average igneous crust composition at Gale Crater. Differences between the composition of conglomerates and that of finer-grained detrital sediments analyzed by the rover suggest modifications by diagenetic processes (especially for Mg enrichments in fine-grained rocks), physical sorting, and mixing with finer-grained material of different composition. C1 [Mangold, N.; Le Deit, L.; Le Mouelic, S.] Univ Nantes, CNRS, Lab Planetol & Geodynam Nantes, UMR 6112, Nantes, France. [Thompson, L. M.] Univ New Brunswick, Dept Earth Sci, Planetary & Space Sci Ctr, Fredericton, NB, Canada. [Forni, O.; Cousin, A.; Gasnault, O.; Maurice, S.; Meslin, P-Y.; Rapin, W.] Univ Toulouse, UPS OMP, CNRS, Inst Rech Astrophys & Planetol, Toulouse, France. [Williams, A. J.] Towson Univ, Dept Phys Astron & Geosci, Towson, MD USA. [Fabre, C.] Univ Lorraine, GeoRessources, Nancy, France. [Wiens, R. C.; Clegg, S. M.] Los Alamos Natl Lab, Los Alamos, NM USA. [Williams, R.; Yingst, A.] Planetary Sci Inst, Tucson, AZ USA. [Anderson, R. B.] USGS, Flagstaff, AZ USA. [Blaney, D. L.; Calef, F.; Stack, K.] CALTECH, Jet Prop Lab, Pasadena, CA USA. [Dromart, G.] Univ Lyon, Lab Geol Lyon, Lyon, France. [Dietrich, W. E.; Palucis, M. C.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Edgett, K. S.] Malin Space Sci Syst, San Diego, CA USA. [Fisk, M. R.] Oregon State Univ, Coll Earth Ocean & Atmospher Sci, Corvallis, OR USA. [Gellert, R.] Univ Guelph, Dept Phys, Guelph, ON N1G 2W1, Canada. [Grotzinger, J. P.; Siebach, K. L.] CALTECH, Div Geol & Planetary Sci, Pasadena, CA 91125 USA. [Kah, L.] Univ Tennessee, Dept Earth & Planetary Sci, Knoxville, TN USA. [McLennan, S. M.] SUNY Stony Brook, Dept Geosci, Stony Brook, NY 11794 USA. [Newsom, H. E.] Univ New Mexico, Inst Meteorit, Dept Earth & Planetary Sci, Albuquerque, NM 87131 USA. [Sautter, V.] Museum Natl Hist Nat, IMPMC, F-75231 Paris, France. [Sumner, D.] Univ Calif Davis, Dept Earth & Planetary Sci, Davis, CA 95616 USA. RP Mangold, N (reprint author), Univ Nantes, CNRS, Lab Planetol & Geodynam Nantes, UMR 6112, Nantes, France. EM nicolas.mangold@univ-nantes.fr RI Gasnault, Olivier/F-4327-2010; OI Gasnault, Olivier/0000-0002-6979-9012; Siebach, Kirsten/0000-0002-6628-6297; Clegg, Sam/0000-0002-0338-0948 FU French space agency, Centre National d'Etudes Spatiales (CNES); Canadian Space Agency (CSA) FX We are grateful to Marjorie Chan and two anonymous reviewers for their insightful comments. Development and operation of the ChemCam instrument was supported in France by funds from the French space agency, Centre National d'Etudes Spatiales (CNES). Support for development and operation in the U.S. was provided by NASA to the Mars Exploration Program and specifically to the MSL team. The APXS is managed and financed by the Canadian Space Agency (CSA). Imaging and chemical data presented here are available in the NASA Planetary Data System (PDS) http://pds-geosciences.wustl.edu/missions/msl. We are grateful to the MSL engineering and management teams (and especially the Jet Propulsion Laboratory, California Institute of Technology, under contract with NASA) for making the mission and this scientific investigation possible and to science team members who contributed to mission operations. NR 96 TC 4 Z9 4 U1 8 U2 21 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9097 EI 2169-9100 J9 J GEOPHYS RES-PLANET JI J. Geophys. Res.-Planets PD MAR PY 2016 VL 121 IS 3 BP 353 EP 387 DI 10.1002/2015JE004977 PG 35 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DJ6VY UT WOS:000374352500006 ER PT J AU Schmoll, M Dattenbock, C Carreras-Villasenor, N Mendoza-Mendoza, A Tisch, D Aleman, MI Baker, SE Brown, C Cervantes-Badillo, MG Cetz-Chel, J Cristobal-Mondragon, GR Delaye, L Esquivel-Naranjo, EU Frischmann, A Gallardo-Negrete, JD Garca-Esquivel, M Gomez-Rodriguez, EY Greenwood, DR Hernandez-Onate, M Kruszewska, JS Lawry, R Mora-Montes, HM Munoz-Centeno, T Nieto-Jacobo, MF Lopez, GN Olmedo-Monfil, V Osorio-Concepcion, M Pilsyk, S Pomraning, KR Rodriguez-Iglesias, A Rosales-Saavedra, MT Sanchez-Arreguin, JA Seidl-Seiboth, V Stewart, A Uresti-Rivera, EE Wang, CL Wang, TF Zeilinger, S Casas-Flores, S Herrera-Estrella, A AF Schmoll, Monika Dattenboeck, Christoph Carreras-Villasenor, Nohem Mendoza-Mendoza, Artemio Tisch, Doris Ivan Aleman, Mario Baker, Scott E. Brown, Christopher Guadalupe Cervantes-Badillo, Mayte Cetz-Chel, Jose Rosa Cristobal-Mondragon, Gema Delaye, Luis Ulises Esquivel-Naranjo, Edgardo Frischmann, Alexa de Jesus Gallardo-Negrete, Jose Garca-Esquivel, Monica Yazmin Gomez-Rodriguez, Elida Greenwood, David R. Hernandez-Onate, Miguel Kruszewska, Joanna S. Lawry, Robert Mora-Montes, Hector M. Munoz-Centeno, Tania Nieto-Jacobo, Maria Fernanda Lopez, Guillermo Nogueira Olmedo-Monfil, Vianey Osorio-Concepcion, Macario Pilsyk, Sebastian Pomraning, Kyle R. Rodriguez-Iglesias, Aroa Teresa Rosales-Saavedra, Maria Alejandro Sanchez-Arreguin, J. Seidl-Seiboth, Verena Stewart, Alison Elena Uresti-Rivera, Edith Wang, Chih-Li Wang, Ting-Fang Zeilinger, Susanne Casas-Flores, Sergio Herrera-Estrella, Alfredo TI The Genomes of Three Uneven Siblings: Footprints of the Lifestyles of Three Trichoderma Species SO MICROBIOLOGY AND MOLECULAR BIOLOGY REVIEWS LA English DT Review ID HEAT-SHOCK-PROTEIN; YEAST SACCHAROMYCES-CEREVISIAE; CELL-CYCLE PROGRESSION; RICE-BLAST FUNGUS; DNA-REPAIR GENES; CARBON CATABOLITE REPRESSOR; NUCLEOTIDE EXCISION-REPAIR; HISTONE H3 PHOSPHORYLATION; NEUROSPORA CIRCADIAN CLOCK; PLANT-PATHOGENIC FUNGUS AB The genus Trichoderma contains fungi with high relevance for humans, with applications in enzyme production for plant cell wall degradation and use in biocontrol. Here, we provide a broad, comprehensive overview of the genomic content of these species for "hot topic" research aspects, including CAZymes, transport, transcription factors, and development, along with a detailed analysis and annotation of less-studied topics, such as signal transduction, genome integrity, chromatin, photobiology, or lipid, sulfur, and nitrogen metabolism in T. reesei, T. atroviride, and T. virens, and we open up new perspectives to those topics discussed previously. In total, we covered more than 2,000 of the predicted 9,000 to 11,000 genes of each Trichoderma species discussed, which is >20% of the respective gene content. Additionally, we considered available transcriptome data for the annotated genes. Highlights of our analyses include overall carbohydrate cleavage preferences due to the different genomic contents and regulation of the respective genes. We found light regulation of many sulfur metabolic genes. Additionally, a new Golgi 1,2-mannosidase likely involved in N-linked glycosylation was detected, as were indications for the ability of Trichoderma spp. to generate hybrid galactose-containing N-linked glycans. The genomic inventory of effector proteins revealed numerous compounds unique to Trichoderma, and these warrant further investigation. We found interesting expansions in the Trichoderma genus in several signaling pathways, such as G-protein-coupled receptors, RAS GTPases, and casein kinases. A particularly interesting feature absolutely unique to T. atroviride is the duplication of the alternative sulfur amino acid synthesis pathway. C1 [Schmoll, Monika; Dattenboeck, Christoph; Rodriguez-Iglesias, Aroa] Austrian Inst Technol, Dept Hlth & Environm, Bioresources Unit, Tulln, Austria. [Carreras-Villasenor, Nohem; Cetz-Chel, Jose; Ulises Esquivel-Naranjo, Edgardo; Garca-Esquivel, Monica; Hernandez-Onate, Miguel; Alejandro Sanchez-Arreguin, J.; Herrera-Estrella, Alfredo] Cinvestav Irapuato, Natl Lab Genom Biodivers, LANGEBIO, Guanajuato, Mexico. [Mendoza-Mendoza, Artemio; Lawry, Robert; Nieto-Jacobo, Maria Fernanda; Lopez, Guillermo Nogueira] Lincoln Univ, Bioprotect Res Ctr, Canterbury, New Zealand. [Tisch, Doris; Frischmann, Alexa; Seidl-Seiboth, Verena; Zeilinger, Susanne] TU Wien, Inst Chem Engn, Res Div Biotechnol & Microbiol, Vienna, Austria. [Ivan Aleman, Mario; Delaye, Luis] CINVESTAV, Dept Genet Engn, Irapuato, Guanajuato, Mexico. [Baker, Scott E.; Pomraning, Kyle R.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Brown, Christopher] Univ Otago, Dept Biochem & Genet, Dunedin, New Zealand. [Guadalupe Cervantes-Badillo, Mayte; Rosa Cristobal-Mondragon, Gema; de Jesus Gallardo-Negrete, Jose; Yazmin Gomez-Rodriguez, Elida; Munoz-Centeno, Tania; Osorio-Concepcion, Macario; Teresa Rosales-Saavedra, Maria; Elena Uresti-Rivera, Edith; Casas-Flores, Sergio] IPICYT, Div Mol Biol, San Luis Potosi, Mexico. [Greenwood, David R.] Univ Auckland, Sch Biol Sci, Auckland 1, New Zealand. [Kruszewska, Joanna S.; Pilsyk, Sebastian] Polish Acad Sci, Inst Biochem & Biophys, Lab Fungal Glycobiol, Warsaw, Poland. [Mora-Montes, Hector M.; Olmedo-Monfil, Vianey] Univ Guanajuato, Dept Biol, Guanajuato, Guanajuato, Mexico. [Stewart, Alison] Marrone Bio Innovat, Davis, CA USA. [Wang, Chih-Li] Natl Chung Hsing Univ, Dept Plant Pathol, Taichung 40227, Taiwan. [Wang, Ting-Fang] Acad Sinica, Inst Mol Biol, Taipei, Taiwan. [Zeilinger, Susanne] Univ Innsbruck, Inst Microbiol, A-6020 Innsbruck, Austria. [Ulises Esquivel-Naranjo, Edgardo] Autonomous Univ Queretaro, Fac Nat Sci, Unit Basic & Appl Microbiol, Queretaro, Mexico. [Hernandez-Onate, Miguel] Res Ctr Food & Dev, Coordinat Food Technol Plant Origin, Hermosillo, Sonora, Mexico. RP Schmoll, M (reprint author), Austrian Inst Technol, Dept Hlth & Environm, Bioresources Unit, Tulln, Austria.; Herrera-Estrella, A (reprint author), Cinvestav Irapuato, Natl Lab Genom Biodivers, LANGEBIO, Guanajuato, Mexico. EM monika.schmoll@ait.ac.at; aherrera@langebio.cinvestav.mx RI Schmoll, Monika/I-6541-2016; Greenwood, David/D-2375-2016; Herrera-Estrella, Alfredo/F-3185-2011; OI Schmoll, Monika/0000-0003-3918-0574; Greenwood, David/0000-0001-5280-042X; Herrera-Estrella, Alfredo/0000-0002-4589-6870; Pomraning, Kyle/0000-0003-2324-2881 FU Austrian Science Fund FWF [V152-B20, P22511, P24350, V139-B20]; CONACyT, Mexico [FORDECYT-2012-02-93512, CB2011-166860, CB-2011-169045]; Vienna Science and Technology Fund WWTF [LS09-036, LS13-086]; FWF Austrian Science Fund [V263-B20]; Academia Sinica; National Science Council, Taiwan; Operational Programme, Innovative Economy, Poland [UDA-POIG.01.03.01-14-038/09]; Marsden Fund; Bio-Protection Research Centre, a New Zealand Centre of Research Excellence; Lincoln University Research Fund, and Massey-Lincoln Agriculture and Life Sciences Partnership for Excellence; Meadow Mushrooms scholarship; SEP-CONACYT [CB-2013-01-220791]; CONACyT, Mexico FX The work of M.S., D.T., A.R.-I., and C.D. was supported by the Austrian Science Fund FWF, grants V152-B20, P22511, and P24350 to M.S. The work of A.H.-E., M.H.-O., N.C.-V., J.A.S.-A., and J.C.-C. was supported by grant FORDECYT-2012-02-93512 from CONACyT, Mexico, to A.H.-E. The work of S.Z. was supported by the Austrian Science Fund FWF (grant V139-B20) to S.Z. and the Vienna Science and Technology Fund WWTF (grants LS09-036 and LS13-086) to S.Z. The work of V.S.-S. was supported by the FWF Austrian Science Fund (V263-B20). This work was supported by grants to T.-F.W. from Academia Sinica and the National Science Council, Taiwan. C.-L.W. was supported by postdoctoral fellowship grants to T.-F.W. J.S.K. is supported by Operational Programme, Innovative Economy, Poland (grant UDA-POIG.01.03.01-14-038/09). H.M.M.-M. is supported by CONACyT, Mexico (grant number CB2011-166860). The work of A.M.-M, M.F.N.-J., R.L., G.N.L., and A.S. was supported by the Marsden Fund; The Bio-Protection Research Centre, a New Zealand Centre of Research Excellence; Lincoln University Research Fund, and Massey-Lincoln Agriculture and Life Sciences Partnership for Excellence to A. M.-M. G.N.L. was supported by CONACyT, Mexico, and a Meadow Mushrooms scholarship for his Ph.D. studies. The work of S.C.-F., M.O.-C., M.G.C.-B., E.Y.G.-R., E.E.U.-R., T.M.-C, M.T.R.-S., J.D.J.G.-N., and G.R.C.-M. was supported by grant SEP-CONACYT CB-2013-01-220791. E.U.E.-N. is supported by CONACyT, Mexico (grant number CB-2011-169045). NR 1307 TC 6 Z9 6 U1 9 U2 28 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 1092-2172 EI 1098-5557 J9 MICROBIOL MOL BIOL R JI Microbiol. Mol. Biol. Rev. PD MAR PY 2016 VL 80 IS 1 BP 205 EP 327 DI 10.1128/MMBR.00040-15 PG 123 WC Microbiology SC Microbiology GA DK6UK UT WOS:000375060700008 PM 26864432 ER PT J AU Sechet, J Frey, A Effroy-Cuzzi, D Berger, A Perreau, F Cueff, G Charif, D Rajjou, L Mouille, G North, HM Marion-Poll, A AF Sechet, Julien Frey, Anne Effroy-Cuzzi, Delphine Berger, Adeline Perreau, Francois Cueff, Gwendal Charif, Delphine Rajjou, Loic Mouille, Gregory North, Helen M. Marion-Poll, Annie TI Xyloglucan Metabolism Differentially Impacts the Cell Wall Characteristics of the Endosperm and Embryo during Arabidopsis Seed Germination SO PLANT PHYSIOLOGY LA English DT Article ID ABSCISIC-ACID; MONOCLONAL-ANTIBODIES; ABA ACCUMULATION; GENE-EXPRESSION; GROWTH DEFECTS; THALIANA SEEDS; MESSENGER-RNA; DORMANCY; MUTANT; DEFICIENT AB Cell wall remodeling is an essential mechanism for the regulation of plant growth and architecture, and xyloglucans (XyGs), the major hemicellulose, are often considered as spacers of cellulose microfibrils during growth. In the seed, the activity of cell wall enzymes plays a critical role in germination by enabling embryo cell expansion leading to radicle protrusion, as well as endosperm weakening prior to its rupture. A screen for Arabidopsis (Arabidopsis thaliana) mutants affected in the hormonal control of germination identified a mutant, xyl1, able to germinate on paclobutrazol, an inhibitor of gibberellin biosynthesis. This mutant also exhibited reduced dormancy and increased resistance to high temperature. The XYL1 locus encodes an a-xylosidase required for XyG maturation through the trimming of Xyl. The xyl1 mutant phenotypes were associated with modifications to endosperm cell wall composition that likely impact on its resistance, as further demonstrated by the restoration of normal germination characteristics by endosperm-specific XYL1 expression. The absence of phenotypes in mutants defective for other glycosidases, which trim Gal or Fuc, suggests that XYL1 plays the major role in this process. Finally, the decreased XyG abundance in hypocotyl longitudinal cell walls of germinating embryos indicates a potential role in cell wall loosening and anisotropic growth together with pectin de-methylesterification. C1 [Sechet, Julien; Frey, Anne; Effroy-Cuzzi, Delphine; Berger, Adeline; Perreau, Francois; Cueff, Gwendal; Charif, Delphine; Rajjou, Loic; Mouille, Gregory; North, Helen M.; Marion-Poll, Annie] Univ Paris Saclay, CNRS, AgroParisTech, INRA,Inst Jean Pierre Bourgin,RD10, F-78026 Versailles, France. [Sechet, Julien] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, Berkeley, CA 94720 USA. [Sechet, Julien] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Marion-Poll, A (reprint author), Univ Paris Saclay, CNRS, AgroParisTech, INRA,Inst Jean Pierre Bourgin,RD10, F-78026 Versailles, France. EM annie.marion-poll@versailles.inra.fr FU National Research Agency [ANR-2010-BLAN-1233-01, ANR-11-BSV5-0007] FX This work was supported by the National Research Agency (projects ABSIG ANR-2010-BLAN-1233-01 and AuxiWall ANR-11-BSV5-0007). NR 55 TC 2 Z9 2 U1 8 U2 34 PU AMER SOC PLANT BIOLOGISTS PI ROCKVILLE PA 15501 MONONA DRIVE, ROCKVILLE, MD 20855 USA SN 0032-0889 EI 1532-2548 J9 PLANT PHYSIOL JI Plant Physiol. PD MAR PY 2016 VL 170 IS 3 BP 1367 EP 1380 DI 10.1104/pp.15.01312 PG 14 WC Plant Sciences SC Plant Sciences GA DL1VI UT WOS:000375420300016 PM 26826221 ER PT J AU Cai, F Bernstein, SL Wilson, SC Kerfeld, CA AF Cai, Fei Bernstein, Susan L. Wilson, Steven C. Kerfeld, Cheryl A. TI Production and Characterization of Synthetic Carboxysome Shells with Incorporated Luminal Proteins SO PLANT PHYSIOLOGY LA English DT Article ID BACTERIAL MICROCOMPARTMENT SHELLS; THIOBACILLUS-NEAPOLITANUS; ELECTRON CRYOTOMOGRAPHY; POLYHEDRAL BODIES; SYNECHOCOCCUS; ORGANELLE; PHOTOSYNTHESIS; CONSTRUCTION; CO2; CYANOBACTERIA AB Spatial segregation of metabolism, such as cellular-localized CO2 fixation in C4 plants or in the cyanobacterial carboxysome, enhances the activity of inefficient enzymes by selectively concentrating them with their substrates. The carboxysome and other bacterial microcompartments (BMCs) have drawn particular attention for bioengineering of nanoreactors because they are selfassembling proteinaceous organelles. All BMCs share an architecturally similar, selectively permeable shell that encapsulates enzymes. Fundamental to engineering carboxysomes and other BMCs for applications in plant synthetic biology and metabolic engineering is understanding the structural determinants of cargo packaging and shell permeability. Here we describe the expression of a synthetic operon in Escherichia coli that produces carboxysome shells. Protein domains native to the carboxysome core were used to encapsulate foreign cargo into the synthetic shells. These synthetic shells can be purified to homogeneity with or without luminal proteins. Our results not only further the understanding of protein-protein interactions governing carboxysome assembly, but also establish a platform to study shell permeability and the structural basis of the function of intact BMC shells both in vivo and in vitro. This system will be especially useful for developing synthetic carboxysomes for plant engineering. C1 [Cai, Fei; Bernstein, Susan L.; Wilson, Steven C.; Kerfeld, Cheryl A.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Cai, Fei; Bernstein, Susan L.; Wilson, Steven C.; Kerfeld, Cheryl A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA. [Kerfeld, Cheryl A.] Michigan State Univ, MSU DOE Plant Res Lab, E Lansing, MI 48824 USA. [Kerfeld, Cheryl A.] Michigan State Univ, Dept Biochem & Mol Biol, E Lansing, MI 48824 USA. RP Kerfeld, CA (reprint author), Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA.; Kerfeld, CA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA.; Kerfeld, CA (reprint author), Michigan State Univ, MSU DOE Plant Res Lab, E Lansing, MI 48824 USA.; Kerfeld, CA (reprint author), Michigan State Univ, Dept Biochem & Mol Biol, E Lansing, MI 48824 USA. EM ckerfeld@lbl.gov FU National Science Foundation Emerging Frontiers Program [EF1105897]; Basic Energy Sciences, US Department of Energy [DE-FG02-91ER20021] FX This work was supported by the National Science Foundation Emerging Frontiers Program (no. EF1105897) and Basic Energy Sciences, US Department of Energy (no. DE-FG02-91ER20021) with infrastructure support from MSU AgBioResearch. NR 54 TC 3 Z9 3 U1 9 U2 15 PU AMER SOC PLANT BIOLOGISTS PI ROCKVILLE PA 15501 MONONA DRIVE, ROCKVILLE, MD 20855 USA SN 0032-0889 EI 1532-2548 J9 PLANT PHYSIOL JI Plant Physiol. PD MAR PY 2016 VL 170 IS 3 BP 1868 EP 1877 DI 10.1104/pp.15.01822 PG 10 WC Plant Sciences SC Plant Sciences GA DL1VI UT WOS:000375420300049 PM 26792123 ER PT J AU Voetsch, K Sequeira, S Chavez, AH AF Voetsch, Karen Sequeira, Sonia Chavez, Amy Holmes TI A Customizable Model for Chronic Disease Coordination: Lessons Learned From the Coordinated Chronic Disease Program SO PREVENTING CHRONIC DISEASE LA English DT Article ID PUBLIC-HEALTH AB In 2012, the Centers for Disease Control and Prevention provided funding and technical assistance to all states and territories to implement the Coordinated Chronic Disease Program, marking the first time that all state health departments had federal resources to coordinate chronic disease prevention and control programs. This article describes lessons learned from this initiative and identifies key elements of a coordinated approach. We analyzed 80 programmatic documents from 21 states and conducted semistructured interviews with 7 chronic disease directors. Six overarching themes emerged: 1) focused agenda, 2) identification of functions, 3) comprehensive planning, 4) collaborative leadership and expertise, 5) managed resources, and 6) relationship building. These elements supported 4 essential activities: 1) evidence-based interventions, 2) strategic use of staff, 3) consistent communication, and 4) strong program infrastructure. On the basis of these elements and activities, we propose a conceptual model that frames overarching concepts, skills, and strategies needed to coordinate state chronic disease prevention and control programs. C1 [Voetsch, Karen] Ctr Dis Control & Prevent, 4770 Buford Hwy, Atlanta, GA 30341 USA. [Sequeira, Sonia; Chavez, Amy Holmes] Ctr Dis Control & Prevent, Natl Ctr Chron Dis Prevent & Hlth Promot, Atlanta, GA 30341 USA. [Sequeira, Sonia; Chavez, Amy Holmes] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. RP Voetsch, K (reprint author), Ctr Dis Control & Prevent, 4770 Buford Hwy, Atlanta, GA 30341 USA. EM kmp9@cdc.gov FU NCCDPHP, CDC FX We thank Fran Butterfoss, Renee Lavinghouze, and Debra Wigand for input on the conceptual framework, Patrick Brady for graphic design, Natasha Underwood and Jeanne Alongi for technical assistance, and the Connecticut, Montana, and Ohio state health departments for the use of graphics. This project was supported in part by an appointment to the Research Participation Program at the NCCDPHP, CDC, administered by the Oak Ridge Institute for Science and Education through an interagency agreement between the US Department of Energy and CDC. The findings and conclusions in this report are those of the authors and do not necessarily represent the official position of the CDC.. NR 12 TC 0 Z9 0 U1 0 U2 2 PU CENTERS DISEASE CONTROL PI ATLANTA PA 1600 CLIFTON RD, ATLANTA, GA 30333 USA SN 1545-1151 J9 PREV CHRONIC DIS JI Prev. Chronic Dis. PD MAR PY 2016 VL 13 AR 150509 DI 10.5888/pcd13.150509 PG 8 WC Public, Environmental & Occupational Health SC Public, Environmental & Occupational Health GA DK8UG UT WOS:000375203200014 ER PT J AU Zachara, JM Chen, XY Murray, C Hammond, G AF Zachara, John M. Chen, Xingyuan Murray, Chris Hammond, Glenn TI River stage influences on uranium transport in a hydrologically dynamic groundwater-surface water transition zone SO WATER RESOURCES RESEARCH LA English DT Article DE groundwater-surface water interaction; uranium groundwater plume; reactive transport modeling ID HANFORD 300 AREA; AQUIFER CHARACTERIZATION; CONTAMINATED SEDIMENTS; ADSORPTION; DESORPTION; KINETICS; EXCHANGE; CLIMATE; MODEL; SCALE AB A well-field within a uranium (U) plume in the groundwater-surface water transition zone was monitored for a 3 year period for water table elevation and dissolved solutes. The plume discharges to the Columbia River, which displays a dramatic spring stage surge resulting from snowmelt. Groundwater exhibits a low hydrologic gradient and chemical differences with river water. River water intrudes the site in spring. Specific aims were to assess the impacts of river intrusion on dissolved uranium (U-aq), specific conductance (SpC), and other solutes, and to discriminate between transport, geochemical, and source term heterogeneity effects. Time series trends for U-aq and SpC were complex and displayed large temporal and well-to-well variability as a result of water table elevation fluctuations, river water intrusion, and changes in groundwater flow directions. The wells were clustered into subsets exhibiting common behaviors resulting from the intrusion dynamics of river water and the location of source terms. Hot-spots in U-aq varied in location with increasing water table elevation through the combined effects of advection and source term location. Heuristic reactive transport modeling with PFLOTRAN demonstrated that mobilized U-aq was transported between wells and source terms in complex trajectories, and was diluted as river water entered and exited the groundwater system. While U-aq time-series concentration trends varied significantly from year-to-year as a result of climate-caused differences in the spring hydrograph, common and partly predictable response patterns were observed that were driven by water table elevation, and the extent and duration of river water intrusion. C1 [Zachara, John M.; Chen, Xingyuan; Murray, Chris] Pacific NW Natl Lab, Richland, WA 99352 USA. [Hammond, Glenn] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Zachara, JM (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM john.zachara@pnnl.gov FU U. S. Department of Energy (USDOE), Biological and Environmental Research Division (BER) as part of BER's Subsurface Biogeochemical Research Program (SBR); Pacific Northwest National Laboratory (PNNL), Subsurface Biogeochemical Research (SBR) Scientific Focus Area (SFA) FX The research described in this publication was supported by the U. S. Department of Energy (USDOE), Biological and Environmental Research Division (BER), as part of BER's Subsurface Biogeochemical Research Program (SBR). Groundwater sampling and analysis was performed by Jim McKinley, Tom Resch, and Rachael Lund as part of the monitoring program of the Hanford Integrated Field Research Challenge Project (IFRC). Statistical analyses, groundwater flow modeling, reactive transport modeling, and manuscript preparation were supported by the Pacific Northwest National Laboratory (PNNL), Subsurface Biogeochemical Research (SBR) Scientific Focus Area (SFA). The helpful comments of three anonymous reviewers are appreciated. PNNL is operated for the DOE by Battelle. The data used in this publication are available upon request by contacting the corresponding author at john.zachara@pnnl.gov. NR 64 TC 0 Z9 0 U1 11 U2 16 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0043-1397 EI 1944-7973 J9 WATER RESOUR RES JI Water Resour. Res. PD MAR PY 2016 VL 52 IS 3 BP 1568 EP 1590 DI 10.1002/2015WR018009 PG 23 WC Environmental Sciences; Limnology; Water Resources SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water Resources GA DK1WR UT WOS:000374706300002 ER PT J AU Sjoberg, Y Coon, E Sannel, ABK Pannetier, R Harp, D Frampton, A Painter, SL Lyon, SW AF Sjoberg, Ylva Coon, Ethan Sannel, A. Britta K. Pannetier, Romain Harp, Dylan Frampton, Andrew Painter, Scott L. Lyon, Steve W. TI Thermal effects of groundwater flow through subarctic fens: A case study based on field observations and numerical modeling SO WATER RESOURCES RESEARCH LA English DT Article DE permafrost; groundwater; numerical modeling; advective heat transfer ID POLAR YEAR 2007-2009; CLIMATE-CHANGE; NORTHERN SWEDEN; PERMAFROST; PALSA; HEAT; REGIONS; VULNERABILITY; CONDUCTIVITY; TEMPERATURES AB Modeling and observation of ground temperature dynamics are the main tools for understanding current permafrost thermal regimes and projecting future thaw. Until recently, most studies on permafrost have focused on vertical ground heat fluxes. Groundwater can transport heat in both lateral and vertical directions but its influence on ground temperatures at local scales in permafrost environments is not well understood. In this study we combine field observations from a subarctic fen in the sporadic permafrost zone with numerical simulations of coupled water and thermal fluxes. At the Tavvavuoma study site in northern Sweden, ground temperature profiles and groundwater levels were observed in boreholes. These observations were used to set up one- and two-dimensional simulations down to 2 m depth across a gradient of permafrost conditions within and surrounding the fen. Two-dimensional scenarios representing the fen under various hydraulic gradients were developed to quantify the influence of groundwater flow on ground temperature. Our observations suggest that lateral groundwater flow significantly affects ground temperatures. This is corroborated by modeling results that show seasonal ground ice melts 1 month earlier when a lateral groundwater flux is present. Further, although the thermal regime may be dominated by vertically conducted heat fluxes during most of the year, isolated high groundwater flow rate events such as the spring freshet are potentially important for ground temperatures. As sporadic permafrost environments often contain substantial portions of unfrozen ground with active groundwater flow paths, knowledge of this heat transport mechanism is important for understanding permafrost dynamics in these environments. C1 [Sjoberg, Ylva; Sannel, A. Britta K.; Pannetier, Romain; Frampton, Andrew; Lyon, Steve W.] Stockholm Univ, Bolin Ctr Climate Res, Dept Phys Geog, S-10691 Stockholm, Sweden. [Coon, Ethan; Harp, Dylan] Los Alamos Natl Lab, Computat Earth Sci, Los Alamos, NM USA. [Painter, Scott L.] Oak Ridge Natl Lab, Climate Change Sci Inst, Oak Ridge, TN USA. [Painter, Scott L.] Oak Ridge Natl Lab, Div Environm Sci, POB 2008, Oak Ridge, TN 37831 USA. RP Sjoberg, Y (reprint author), Stockholm Univ, Bolin Ctr Climate Res, Dept Phys Geog, S-10691 Stockholm, Sweden. EM ylva.sjoberg@natgeo.su.se RI Painter, Scott/C-2586-2016; OI Painter, Scott/0000-0002-0901-6987; Harp, Dylan/0000-0001-9777-8000; Frampton, Andrew/0000-0002-4587-6706 FU Swedish Geological Survey (SGU) [60-1626/2009, 362-1593/2013]; Helge Ax:son Johnsons Stiftelse; Goran Gustafssons Stiftelse; Bolin Center for Climate Research; Swedish Society for Anthropology and Geography; LANL Laboratory Directed Research and Development Project [LDRD201200068DR]; Next-Generation Ecosystem Experiments (NGEE Arctic) project; Office of Biological and Environmental Research in the DOE Office of Science; Bolin Centre for Climate Research; Goran Gustafsson Foundation for Nature and Environment in Lapland; Foundation Lars Hiertas Minne; Ahlmann Foundation; Foundation Kungstenen; Lagrelius Foundation; Albert and Maria Bergstrom Foundation; Sandstrom Foundation; Foundation Rhodins Minne; Swedish Research Council for Environment, Agricultural Sciences and Spatial Planning [214 - 2014-562] FX The data used to generate the results in this paper can be made available upon request from the authors. Financial support was provided by the Swedish Geological Survey (SGU) projects #60-1626/2009 and #362-1593/2013, Helge Ax:son Johnsons Stiftelse, Goran Gustafssons Stiftelse, the Bolin Center for Climate Research, and the Swedish Society for Anthropology and Geography. Financial support for coauthors EC, DH, and SP was provided by LANL Laboratory Directed Research and Development Project LDRD201200068DR and by the The Next-Generation Ecosystem Experiments (NGEE Arctic) project. NGEE-Arctic is supported by the Office of Biological and Environmental Research in the DOE Office of Science. Coauthor BS has received financial support for monitoring of meteorological parameters and ground temperatures in the peat plateau in Tavvavuoma from the Bolin Centre for Climate Research, Goran Gustafsson Foundation for Nature and Environment in Lapland, Foundation Lars Hiertas Minne, Helge Ax:son Johnson Foundation, Swedish Society for Anthropology and Geography, Ahlmann Foundation, Foundation Kungstenen, Lagrelius Foundation, Albert and Maria Bergstrom Foundation, A Sandstrom Foundation and Foundation Rhodins Minne, and for data analysis from the Swedish Research Council for Environment, Agricultural Sciences and Spatial Planning (project #214 - 2014-562). Benjamin Kjellson and Elin Magnusson at Stockholm University helped with statistical consulting. Fredrik Palm, Joakim Lannek, Jenny Sundkvist, and Lars Labba provided much needed support during fieldwork. NR 51 TC 4 Z9 4 U1 7 U2 14 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0043-1397 EI 1944-7973 J9 WATER RESOUR RES JI Water Resour. Res. PD MAR PY 2016 VL 52 IS 3 BP 1591 EP 1606 DI 10.1002/2015WR017571 PG 16 WC Environmental Sciences; Limnology; Water Resources SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water Resources GA DK1WR UT WOS:000374706300003 ER PT J AU Chen, JS Hubbard, SS Williams, KH Ficklin, DL AF Chen, Jinsong Hubbard, Susan S. Williams, Kenneth H. Ficklin, Darren L. TI Estimating groundwater dynamics at a Colorado River floodplain site using historical hydrological data and climate information SO WATER RESOURCES RESEARCH LA English DT Article DE groundwater dynamics; Bayesian integration; climate change; streamflow; time series; Monte Carlo sampling ID URANIUM-CONTAMINATED AQUIFER; PARAMETER-ESTIMATION; BIOREMEDIATION; SEDIMENT; MODELS AB Long-term prediction of groundwater dynamics is important for assessing water resources and their impacts on biogeochemical cycling. However, estimating future groundwater dynamics is challenging due to the wide range of spatiotemporal scales in hydrological processes and uncertainty in future climate conditions. In this study, we develop a Bayesian model to combine small-scale historical hydrological data with large-scale climate information to estimate groundwater dynamics at a floodplain site in Rifle, Colorado. Although we have only a few years of groundwater elevation measurements, we have 47 years of streamflow data from a gaging station approximately 43 km upstream and long-term climate prediction on the Upper Colorado River Basin. To estimate future daily groundwater dynamics, we first develop a time series model to downscale the monthly streamflow derived from climate information to daily streamflow, and then transform the daily streamflow to groundwater dynamics at the downstream floodplain site. We use Monte Carlo methods to estimate future groundwater dynamics at the site through sampling from the joint posterior probability distribution. The results suggest that although future groundwater levels are expected to be similar to the current levels, the timing of the high groundwater levels is predicted to occur about 1 month earlier. The developed framework is extendable to other sites to estimate future groundwater dynamics given disparate data sets and climate projections. Additionally, the obtained estimates are being used as input to a site-specific watershed reactive transport models to predict how climate-induced changes will influence future biogeochemical cycling relevant to a variety of ecosystem services. C1 [Chen, Jinsong; Hubbard, Susan S.; Williams, Kenneth H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Earth & Environm Sci Area, Berkeley, CA 94720 USA. [Ficklin, Darren L.] Indiana Univ, Dept Geog, Bloomington, IN 47405 USA. RP Chen, JS (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Earth & Environm Sci Area, Berkeley, CA 94720 USA. EM jchen@lbl.gov RI Chen, Jinsong/A-1374-2009; Hubbard, Susan/E-9508-2010; Williams, Kenneth/O-5181-2014 OI Williams, Kenneth/0000-0002-3568-1155 FU Sustainable Systems Scientific Focus Area by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231] FX This material is based upon work supported as part of the Sustainable Systems Scientific Focus Area funded by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research under award DE-AC02-05CH11231. Data sets are available upon request by contacting the corresponding author (Jinsong Chen at jchen@lbl.gov). NR 35 TC 0 Z9 0 U1 6 U2 12 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0043-1397 EI 1944-7973 J9 WATER RESOUR RES JI Water Resour. Res. PD MAR PY 2016 VL 52 IS 3 BP 1881 EP 1898 DI 10.1002/2015WR017777 PG 18 WC Environmental Sciences; Limnology; Water Resources SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water Resources GA DK1WR UT WOS:000374706300019 ER PT J AU James, GA Zhao, AG Usui, M Underwood, RA Nguyen, H Beyenal, H Pulcini, ED Hunt, AA Bernstein, HC Fleckman, P Olerud, J Williamson, KS Franklin, MJ Stewart, PS AF James, Garth A. Zhao, Alice Ge Usui, Marcia Underwood, Robert A. Nguyen, Hung Beyenal, Haluk Pulcini, Elinor deLancey Hunt, Alessandra Agostinho Bernstein, Hans C. Fleckman, Philip Olerud, John Williamson, Kerry S. Franklin, Michael J. Stewart, Philip S. TI Microsensor and transcriptomic signatures of oxygen depletion in biofilms associated with chronic wounds SO WOUND REPAIR AND REGENERATION LA English DT Article ID PSEUDOMONAS-AERUGINOSA BIOFILMS; INFLAMMATORY RESPONSE; MICROARRAY ANALYSIS; STRESS-RESPONSE; GROWTH; MODEL; TENSION; GENES; IDENTIFICATION; EXPRESSION AB Biofilms have been implicated in delayed wound healing, although the mechanisms by which biofilms impair wound healing are poorly understood. Many species of bacteria produce exotoxins and exoenzymes that may inhibit healing. In addition, oxygen consumption by biofilms and by the responding leukocytes, may impede wound healing by depleting the oxygen that is required for healing. In this study, oxygen microsensors to measure oxygen transects through in vitro cultured biofilms, biofilms formed in vivo within scabs from a diabetic (db/db) mouse wound model, and ex vivo human chronic wound specimens was used. The results showed that oxygen levels within mouse scabs had steep gradients that reached minima ranging from 17 to 72 mmHg on live mice and from 6.4 to 1.1 mmHg on euthanized mice. The oxygen gradients in the mouse scabs were similar to those observed for clinical isolates cultured in vitro and for human ex vivo specimens. To characterize the metabolic activities of the bacteria in the mouse scabs, transcriptomics analyses of Pseudomonas aeruginosa biofilms associated with the db/db mice wounds was performed. The results demonstrated that the bacteria expressed genes for metabolic activities associated with cell growth. Interestingly, the transcriptome results also indicated that the bacteria within the wounds experienced oxygen-limitation stress. Among the bacterial genes that were expressed in vivo were genes associated with the Anr-mediated hypoxia-stress response. Other bacterial stress response genes highly expressed in vivo were genes associated with stationary-phase growth, osmotic stress, and RpoH-mediated heat shock stress. Overall, the results supported the hypothesis that bacterial biofilms in chronic wounds promote chronicity by contributing to the maintenance of localized low oxygen tensions, through their metabolic activities and through their recruitment of cells that consume oxygen for host defensive processes. C1 [James, Garth A.; Pulcini, Elinor deLancey; Williamson, Kerry S.; Franklin, Michael J.; Stewart, Philip S.] Montana State Univ, Ctr Biofilm Engn, Bozeman, MT 59717 USA. [Zhao, Alice Ge; Usui, Marcia; Underwood, Robert A.; Fleckman, Philip; Olerud, John] Univ Washington, Dept Med, Div Dermatol, Seattle, WA USA. [Nguyen, Hung; Beyenal, Haluk] Washington State Univ, Gene & Linda Voiland Sch Chem Engn & Bioengn, Pullman, WA 99164 USA. [Hunt, Alessandra Agostinho] Michigan State Univ, Dept Microbiol & Mol Genet, 5180 Biomed & Phys Sci, E Lansing, MI 48824 USA. [Bernstein, Hans C.] Pacific NW Natl Lab, Chem & Biol Signature Sci, Richland, WA 99352 USA. RP James, GA (reprint author), Montana State Univ, Ctr Biofilm Engn, Bozeman, MT 59717 USA. EM gjames@biofilm.montana.edu OI Bernstein, Hans/0000-0003-2913-7708 FU National Institutes of Health (NIH) [1P20GM078445-01, R21AI094268, RO1GM109452, T32AR056969]; George F. Odland Endowed Research Fund FX The authors thank James Marshall MHS, CWS, PA-C, Wound Clinic, Bozeman Health, for collecting the human wound debridement specimens. This research was supported in part by grant numbers 1P20GM078445-01, R21AI094268, RO1GM109452, and T32AR056969 from the National Institutes of Health (NIH) and the George F. Odland Endowed Research Fund. The contents of this report are solely the responsibility of the authors and do not necessarily represent the official views of the NIH. NR 39 TC 7 Z9 7 U1 2 U2 7 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1067-1927 EI 1524-475X J9 WOUND REPAIR REGEN JI Wound Repair Regen. PD MAR-APR PY 2016 VL 24 IS 2 BP 373 EP 383 DI 10.1111/wrr.12401 PG 11 WC Cell Biology; Dermatology; Medicine, Research & Experimental; Surgery SC Cell Biology; Dermatology; Research & Experimental Medicine; Surgery GA DK8DP UT WOS:000375157700147 PM 26748963 ER PT J AU Berryman, JG Kwon, TH Dou, S Ajo-Franklin, JB Hubbard, SS AF Berryman, J. G. Kwon, T. -H. Dou, S. Ajo-Franklin, J. B. Hubbard, S. S. TI Analysis of laboratory data on ultrasonic monitoring of permeability reduction due to biopolymer formation in unconsolidated granular media SO GEOPHYSICAL PROSPECTING LA English DT Article DE Permeability reduction ID COMPLEX DIELECTRIC-CONSTANT; 2-COMPONENT COMPOSITE-MATERIAL; 2-POINT CORRELATION-FUNCTIONS; SATURATED POROUS-MEDIA; BIOT SLOW-WAVE; DYNAMIC PERMEABILITY; CHARACTERIZE MICROGEOMETRY; COMPRESSIONAL WAVE; FLUID PERMEABILITY; RIGOROUS BOUNDS AB We show how to estimate the fluid permeability changes due to accumulated biopolymer within the pore space of a granular material using laboratory measurements of overall permeability, together with various well-known quantitative measures (e.g., porosity, specific surface area, and formation factor) of the granular medium microstructure. The main focus of the paper is on mutual validation of existing theory and a synthesis of new experimental results. We find that the theory and data are in good agreement within normal experimental uncertainties. We also establish quantitative empirical relationships between seismic and/or acoustic attenuation and overall permeability for these same systems. C1 [Berryman, J. G.; Dou, S.; Ajo-Franklin, J. B.; Hubbard, S. S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Kwon, T. -H.] Korea Adv Inst Sci & Technol, Dept Civil & Environm Engn, Daejeon 305338, South Korea. RP Berryman, JG (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. EM jgberryman@lbl.gov RI Hubbard, Susan/E-9508-2010; Ajo-Franklin, Jonathan/G-7169-2015; Kwon, Tae-Hyuk/F-2183-2013; Dou, Shan/H-5085-2016; OI Dou, Shan/0000-0001-5420-8489; Ajo-Franklin, Jonathan/0000-0002-6666-4702 FU U.S. Department of Energy (DOE) at the Lawrence Berkeley National Laboratory (LBNL), University of California, Berkeley; Office of Biological and Environmental Research, Office of Science, U.S. DOE [DE-AC02-05CH1131]; Energy Biosciences Institute; Geosciences Research Program of the DOE Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences FX Work is performed under the auspices of the U.S. Department of Energy (DOE) at the Lawrence Berkeley National Laboratory (LBNL), University of California, Berkeley. This material is based upon work funded by the Office of Biological and Environmental Research, Office of Science, U.S. DOE, under Contract DE-AC02-05CH1131. The authors would like to thank R. Chakraborty (LBNL) for assistance in culturing and microbial analysis and B. P. Bonner (LBNL) for suggestions during the data analysis phase. Primary support for the research was funded by the Energy Biosciences Institute. Some additional support was provided by the Geosciences Research Program of the DOE Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences during the completion, review, and publication phases of the work. All support of this research is hereby gratefully acknowledged. NR 45 TC 0 Z9 0 U1 2 U2 5 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0016-8025 EI 1365-2478 J9 GEOPHYS PROSPECT JI Geophys. Prospect. PD MAR PY 2016 VL 64 IS 2 BP 445 EP 455 DI 10.1111/1365-2478.12295 PG 11 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DJ6UG UT WOS:000374348100013 ER PT J AU Maddi, B Panisko, E Albrecht, K Howe, D AF Maddi, Balakrishna Panisko, Ellen Albrecht, Karl Howe, Daniel TI Qualitative Characterization of the Aqueous Fraction from Hydrothermal Liquefaction of Algae Using 2D Gas Chromatography with Time-of-flight Mass Spectrometry SO JOVE-JOURNAL OF VISUALIZED EXPERIMENTS LA English DT Article DE Bioengineering; Issue 109; Bio-crude; bio-oil; bio-fuel; aqueous product; hydrothermal liquefaction; microalgae; biomass; aquatic biomass; GC x GC - TOF-MS; catalytic fast pyrolysis; pyridine; pyrazine; organic acids; succinimide ID BIO-OILS; PYROLYSIS; FEEDSTOCKS; BIOMASS; FUELS; CRUDE; SEPARATION; PRODUCTS; SOLVENT; PHASE AB Two-dimensional gas chromatography coupled with time-of-flight mass spectrometry is a powerful tool for identifying and quantifying chemical components in complex mixtures. It is often used to analyze gasoline, jet fuel, diesel, bio-diesel and the organic fraction of bio-crude/bio-oil. In most of those analyses, the first dimension of separation is non-polar, followed by a polar separation. The aqueous fractions of bio-crude and other aqueous samples from biofuels production have been examined with similar column combinations. However, sample preparation techniques such as derivatization, solvent extraction, and solid-phase extraction were necessary prior to analysis. In this study, aqueous fractions obtained from the hydrothermal liquefaction of algae were characterized by two-dimensional gas chromatography coupled with time-of-flight mass spectrometry without prior sample preparation techniques using a polar separation in the first dimension followed by a non-polar separation in the second. Two-dimensional plots from this analysis were compared with those obtained from the more traditional column configuration. Results from qualitative characterization of the aqueous fractions of algal bio-crude are discussed in detail. The advantages of using a polar separation followed by a non-polar separation for characterization of organics in aqueous samples by two-dimensional gas chromatography coupled with time-of-flight mass spectrometry are highlighted. C1 [Maddi, Balakrishna; Panisko, Ellen; Albrecht, Karl; Howe, Daniel] Pacific NW Natl Lab, Chem & Biol Proc Dev, Richland, WA 99352 USA. RP Howe, D (reprint author), Pacific NW Natl Lab, Chem & Biol Proc Dev, Richland, WA 99352 USA. EM Daniel.Howe@pnnl.gov FU U.S. Department of Energy [DE-AC05-76RL01830] FX This manuscript has been authored by Battelle Memorial Institute under Contract No. DE-AC05-76RL01830 with the U.S. Department of Energy. The U.S Government retains and the publisher, by accepting the article for publication, acknowledges that the U.S. Government retains a non-exclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for U.S. Government purposes. NR 47 TC 1 Z9 1 U1 4 U2 9 PU JOURNAL OF VISUALIZED EXPERIMENTS PI CAMBRIDGE PA 1 ALEWIFE CENTER, STE 200, CAMBRIDGE, MA 02140 USA SN 1940-087X J9 JOVE-J VIS EXP JI J. Vis. Exp. PD MAR PY 2016 IS 109 AR e53634 DI 10.3791/53634 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DK0XR UT WOS:000374636300034 ER PT J AU Blake, JB Mauk, BH Baker, DN Carranza, P Clemmons, JH Craft, J Crain, WR Crew, A Dotan, Y Fennell, JF Friedel, RH Friesen, LM Fuentes, F Galvan, R Ibscher, C Jaynes, A Katz, N Lalic, M Lin, AY Mabry, DM Nguyen, T Pancratz, C Redding, M Reeves, GD Smith, S Spence, HE Westlake, J AF Blake, J. B. Mauk, B. H. Baker, D. N. Carranza, P. Clemmons, J. H. Craft, J. Crain, W. R., Jr. Crew, A. Dotan, Y. Fennell, J. F. Friedel, R. H. Friesen, L. M. Fuentes, F. Galvan, R. Ibscher, C. Jaynes, A. Katz, N. Lalic, M. Lin, A. Y. Mabry, D. M. Nguyen, T. Pancratz, C. Redding, M. Reeves, G. D. Smith, S. Spence, H. E. Westlake, J. TI The Fly's Eye Energetic Particle Spectrometer (FEEPS) Sensors for the Magnetospheric Multiscale (MMS) Mission SO SPACE SCIENCE REVIEWS LA English DT Review DE Magnetospheric Multiscale mission; Energetic electrons and protons; Fly's Eye Electron Proton Spectrometer (FEEPS) AB The Energetic Particle Detector (EPD) Investigation is one of five particles and fields investigations on the Magnetospheric Multiscale (MMS) mission. This mission consists of four satellites operating in close proximity in elliptical, low-inclination orbits, and is focused upon the fundamental physics of magnetic reconnection. The Energetic Particle Detector (EPD) investigation aboard the four MMS spacecraft consists of two instrument designs, the EIS (Energetic Ion Spectrometer) and the FEEPS (Fly's Eye Electron Proton Spectrometer). This present paper describes FEEPS from an instrument physics and engineering point of view, and provides some test and calibration data to facilitate effective analysis and use of the flight data for scientific purposes. A FEEPS consists of six Heads, each composed of two Eyes. Each eye is a particle telescope with a single silicon detector; there are nine electron eyes and three ion eyes per FEEPS. The energy coverage is from 25 keV to 650 keV for electrons and 45 keV to 650 keV for ions. Each eye has sixteen energy channels, the spacing of which can be modified by command. The fields of view and pointing of each eye are designed to provide a broad, instantaneous field of view for the twelve eyes per FEEPS. There are two FEEPS per MMS spacecraft mounted such that the pair along with the single EIS provide more than -sr instantaneous solid-angle coverage and complete coverage in the equatorial region. A twenty-second spacecraft rotation period is divided into sixty-four sectors to provide detailed temporal and spatial sampling. Data are acquired in three modes: Burst Mode, the primary science mode; Fast Survey Mode; and Slow Survey Mode. C1 [Blake, J. B.; Carranza, P.; Clemmons, J. H.; Crain, W. R., Jr.; Dotan, Y.; Fennell, J. F.; Friesen, L. M.; Fuentes, F.; Galvan, R.; Ibscher, C.; Katz, N.; Lalic, M.; Lin, A. Y.; Mabry, D. M.; Nguyen, T.; Redding, M.] Aerosp Corp, Space Sci Applicat Lab, El Segundo, CA 90245 USA. [Mauk, B. H.; Westlake, J.] Johns Hopkins Univ, Appl Phys Lab, 11100 Johns Hopkins Rd, Laurel, MD 20723 USA. [Baker, D. N.; Craft, J.; Jaynes, A.; Pancratz, C.] Atmospher & Space Phys Lab, 3665 Discovery Dr, Boulder, CO 80303 USA. [Crew, A.; Smith, S.; Spence, H. E.] Univ New Hampshire, Ctr Earth Oceans & Space, Durham, NH 03824 USA. [Friedel, R. H.; Reeves, G. D.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Blake, JB (reprint author), Aerosp Corp, Space Sci Applicat Lab, El Segundo, CA 90245 USA. EM jbernard.blake@aero.org RI NASA MMS, Science Team/J-5393-2013; Mauk, Barry/E-8420-2017; OI NASA MMS, Science Team/0000-0002-9504-5214; Mauk, Barry/0000-0001-9789-3797; Clemmons, James/0000-0002-5298-5222; Reeves, Geoffrey/0000-0002-7985-8098 FU Johns Hopkins Applied Physics Laboratory [792084N/E99017JD] FX This work was supported by the Johns Hopkins Applied Physics Laboratory under Contract 792084N/E99017JD. NR 5 TC 10 Z9 10 U1 0 U2 0 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0038-6308 EI 1572-9672 J9 SPACE SCI REV JI Space Sci. Rev. PD MAR PY 2016 VL 199 IS 1-4 BP 309 EP 329 DI 10.1007/s11214-015-0163-x PG 21 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DJ6DI UT WOS:000374299800012 ER PT J AU Pollock, C Moore, T Jacques, A Burch, J Gliese, U Saito, Y Omoto, T Avanov, L Barrie, A Coffey, V Dorelli, J Gershman, D Giles, B Rosnack, T Salo, C Yokota, S Adrian, M Aoustin, C Auletti, C Aung, S Bigio, V Cao, N Chandler, M Chornay, D Christian, K Clark, G Collinson, G Corris, T De Los Santos, A Devlin, R Diaz, T Dickerson, T Dickson, C Diekmann, A Diggs, F Duncan, C Figueroa-Vinas, A Firman, C Freeman, M Galassi, N Garcia, K Goodhart, G Guererro, D Hageman, J Hanley, J Hemminger, E Holland, M Hutchins, M James, T Jones, W Kreisler, S Kujawski, J Lavu, V Lobell, J LeCompte, E Lukemire, A MacDonald, E Mariano, A Mukai, T Narayanan, K Nguyan, Q Onizuka, M Paterson, W Persyn, S Piepgrass, B Cheney, F Rager, A Raghuram, T Ramil, A Reichenthal, L Rodriguez, H Rouzaud, J Rucker, A Saito, Y Samara, M Sauvaud, JA Schuster, D Shappirio, M Shelton, K Sher, D Smith, D Smith, K Smith, S Steinfeld, D Szymkiewicz, R Tanimoto, K Taylor, J Tucker, C Tull, K Uhl, A Vloet, J Walpole, P Weidner, S White, D Winkert, G Yeh, PS Zeuch, M AF Pollock, C. Moore, T. Jacques, A. Burch, J. Gliese, U. Saito, Y. Omoto, T. Avanov, L. Barrie, A. Coffey, V. Dorelli, J. Gershman, D. Giles, B. Rosnack, T. Salo, C. Yokota, S. Adrian, M. Aoustin, C. Auletti, C. Aung, S. Bigio, V. Cao, N. Chandler, M. Chornay, D. Christian, K. Clark, G. Collinson, G. Corris, T. De Los Santos, A. Devlin, R. Diaz, T. Dickerson, T. Dickson, C. Diekmann, A. Diggs, F. Duncan, C. Figueroa-Vinas, A. Firman, C. Freeman, M. Galassi, N. Garcia, K. Goodhart, G. Guererro, D. Hageman, J. Hanley, J. Hemminger, E. Holland, M. Hutchins, M. James, T. Jones, W. Kreisler, S. Kujawski, J. Lavu, V. Lobell, J. LeCompte, E. Lukemire, A. MacDonald, E. Mariano, A. Mukai, T. Narayanan, K. Nguyan, Q. Onizuka, M. Paterson, W. Persyn, S. Piepgrass, B. Cheney, F. Rager, A. Raghuram, T. Ramil, A. Reichenthal, L. Rodriguez, H. Rouzaud, J. Rucker, A. Saito, Y. Samara, M. Sauvaud, J. -A. Schuster, D. Shappirio, M. Shelton, K. Sher, D. Smith, D. Smith, K. Smith, S. Steinfeld, D. Szymkiewicz, R. Tanimoto, K. Taylor, J. Tucker, C. Tull, K. Uhl, A. Vloet, J. Walpole, P. Weidner, S. White, D. Winkert, G. Yeh, P. -S. Zeuch, M. TI Fast Plasma Investigation for Magnetospheric Multiscale SO SPACE SCIENCE REVIEWS LA English DT Review DE Magnetospheric Multiscale; Magnetic reconnection; Particle instrumentation; Electron spectrometer; Ion spectrometer; Instrument characterization and calibration ID MICROCHANNEL PLATE; ION DETECTION; ELECTRON; SPACECRAFT; EFFICIENCY; ANALYZER AB The Fast Plasma Investigation (FPI) was developed for flight on the Magnetospheric Multiscale (MMS) mission to measure the differential directional flux of magnetospheric electrons and ions with unprecedented time resolution to resolve kinetic-scale plasma dynamics. This increased resolution has been accomplished by placing four dual 180-degree top hat spectrometers for electrons and four dual 180-degree top hat spectrometers for ions around the periphery of each of four MMS spacecraft. Using electrostatic field-of-view deflection, the eight spectrometers for each species together provide 4pi-sr field-of-view with, at worst, 11.25-degree sample spacing. Energy/charge sampling is provided by swept electrostatic energy/charge selection over the range from 10 eV/q to 30000 eV/q. The eight dual spectrometers on each spacecraft are controlled and interrogated by a single block redundant Instrument Data Processing Unit, which in turn interfaces to the observatory's Instrument Suite Central Instrument Data Processor. This paper describes the design of FPI, its ground and in-flight calibration, its operational concept, and its data products. C1 [Pollock, C.; Moore, T.; Jacques, A.; Gliese, U.; Avanov, L.; Barrie, A.; Dorelli, J.; Gershman, D.; Giles, B.; Rosnack, T.; Salo, C.; Adrian, M.; Auletti, C.; Aung, S.; Bigio, V.; Cao, N.; Chornay, D.; Christian, K.; Clark, G.; Collinson, G.; Corris, T.; Devlin, R.; Dickerson, T.; Dickson, C.; Diggs, F.; Duncan, C.; Figueroa-Vinas, A.; Firman, C.; Galassi, N.; Garcia, K.; Hageman, J.; Hemminger, E.; Holland, M.; James, T.; Jones, W.; Kreisler, S.; Kujawski, J.; Lavu, V.; Lobell, J.; MacDonald, E.; Mariano, A.; Narayanan, K.; Nguyan, Q.; Onizuka, M.; Paterson, W.; Cheney, F.; Rager, A.; Raghuram, T.; Ramil, A.; Reichenthal, L.; Rucker, A.; Samara, M.; Schuster, D.; Shappirio, M.; Shelton, K.; Sher, D.; Smith, D.; Smith, S.; Steinfeld, D.; Szymkiewicz, R.; Tucker, C.; Tull, K.; Uhl, A.; Walpole, P.; Winkert, G.; Yeh, P. -S.; Zeuch, M.] NASA, Goddard Space Flight Ctr, Greenbelt, MD USA. [Burch, J.; De Los Santos, A.; Diaz, T.; Freeman, M.; Goodhart, G.; Guererro, D.; Hanley, J.; Hutchins, M.; Persyn, S.; Piepgrass, B.; Rodriguez, H.; Smith, K.; Taylor, J.; Vloet, J.; Walpole, P.; Weidner, S.; White, D.] SW Res Inst, San Antonio, TX USA. [Gliese, U.; Corris, T.; Devlin, R.; Galassi, N.; Uhl, A.] SGT Inc, Greenbelt, MD USA. [Saito, Y.; Yokota, S.; Mukai, T.] Inst Space & Astronaut Sci, 3-1-1 Yoshinodai, Sagamihara, Kanagawa 229, Japan. [Omoto, T.; Tanimoto, K.] Meisei Elect Co Ltd, Isesaki, Japan. [Avanov, L.; Gershman, D.; Chornay, D.] Univ Maryland, College Pk, MD 20742 USA. [Barrie, A.] Millenium Engn, Arlington, VA USA. [Coffey, V.; Chandler, M.; Diekmann, A.] NASA, Marshall Space Flight Ctr, Huntsville, AL USA. [Gershman, D.] Oak Ridge Associated Univ, Oak Ridge, TN USA. [Rosnack, T.; Aung, S.; Lavu, V.; Smith, D.] Orbital Sci Corp, Beltsville, MD USA. [Salo, C.] Stellar Solut Inc, Chantilly, VA USA. [Aoustin, C.; LeCompte, E.; Rouzaud, J.; Sauvaud, J. -A.] Inst Res Astrophys & Planetol, Toulouse, France. [Auletti, C.; Dickson, C.; Diggs, F.; Rucker, A.; Zeuch, M.] Northrup Grumman, Hyattsville, MD USA. [Auletti, C.] Florez Engn LLC, Laurel, MD USA. [Cao, N.] MEI Technol, Houston, TX USA. [Christian, K.] Global Programming Solut, Fairfax, VA USA. [Clark, G.; Collinson, G.; Rager, A.; Smith, S.] Catholic Univ Amer, Washington, DC 20064 USA. [Clark, G.] Johns Hopkins Appl Phys Lab, Laurel, MD USA. [Dickerson, T.; Raghuram, T.; Shelton, K.] ASRC AS & D Inc, Beltsville, MD USA. [Diekmann, A.] Jacobs ESSSA Grp, Huntsville, AL USA. [Firman, C.] Prototype Prod Inc, Ashburn, VA USA. [Hemminger, E.] Ares Tech Serv Corp, Greenbelt, MD USA. [Jones, W.] Bandwidth Solut Inc, Mclean, VA USA. [Kreisler, S.] Hammers Co, Greenbelt, MD USA. [Kujawski, J.] Siena Coll, Loudonville, NY USA. [Lukemire, A.] Space Power Elect Inc, Kathleen, GA USA. [Onizuka, M.] Teledyne Brown Engn Inc, Huntsville, AL 35807 USA. [Paterson, W.] NASA Headquarders, Washington, DC USA. [Saito, Y.] YS Design, Tokyo, Japan. [Schuster, D.] Vantage Syst Inc, Lanham, MD USA. [Sher, D.] Design Amer Inc, College Pk, MD USA. [Tucker, C.] Global Sci & Technol Inc, Greenbelt, MD USA. [Tull, K.] Jackson & Tull, Greenbelt, MD USA. RP Pollock, C (reprint author), NASA, Goddard Space Flight Ctr, Greenbelt, MD USA. EM craig@denaliscientific.org RI NASA MMS, Science Team/J-5393-2013 OI NASA MMS, Science Team/0000-0002-9504-5214 NR 27 TC 66 Z9 66 U1 5 U2 12 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0038-6308 EI 1572-9672 J9 SPACE SCI REV JI Space Sci. Rev. PD MAR PY 2016 VL 199 IS 1-4 BP 331 EP 406 DI 10.1007/s11214-016-0245-4 PG 76 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DJ6DI UT WOS:000374299800013 ER PT J AU Mauk, BH Blake, JB Baker, DN Clemmons, JH Reeves, GD Spence, HE Jaskulek, SE Schlemm, CE Brown, LE Cooper, SA Craft, JV Fennell, JF Gurnee, RS Hammock, CM Hayes, JR Hill, PA Ho, GC Hutcheson, JC Jacques, AD Kerem, S Mitchell, DG Nelson, KS Paschalidis, NP Rossano, E Stokes, MR Westlake, JH AF Mauk, B. H. Blake, J. B. Baker, D. N. Clemmons, J. H. Reeves, G. D. Spence, H. E. Jaskulek, S. E. Schlemm, C. E. Brown, L. E. Cooper, S. A. Craft, J. V. Fennell, J. F. Gurnee, R. S. Hammock, C. M. Hayes, J. R. Hill, P. A. Ho, G. C. Hutcheson, J. C. Jacques, A. D. Kerem, S. Mitchell, D. G. Nelson, K. S. Paschalidis, N. P. Rossano, E. Stokes, M. R. Westlake, J. H. TI The Energetic Particle Detector (EPD) Investigation and the Energetic Ion Spectrometer (EIS) for the Magnetospheric Multiscale (MMS) Mission SO SPACE SCIENCE REVIEWS LA English DT Review DE NASA mission; Magnetospheric multiscale; Magnetosphere; Magnetic reconnection; Space plasma; Particle acceleration ID PLASMA SHEET ION; MAGNETIC RECONNECTION; MAGNETOTAIL RECONNECTION; ELECTRON ACCELERATION; FIELD; DISTRIBUTIONS; ENERGIZATION; INSTRUMENT; SPACECRAFT; MECHANISM AB The Energetic Particle Detector (EPD) Investigation is one of 5 fields-and-particles investigations on the Magnetospheric Multiscale (MMS) mission. MMS comprises 4 spacecraft flying in close formation in highly elliptical, near-Earth-equatorial orbits targeting understanding of the fundamental physics of the important physical process called magnetic reconnection using Earth's magnetosphere as a plasma laboratory. EPD comprises two sensor types, the Energetic Ion Spectrometer (EIS) with one instrument on each of the 4 spacecraft, and the Fly's Eye Energetic Particle Spectrometer (FEEPS) with 2 instruments on each of the 4 spacecraft. EIS measures energetic ion energy, angle and elemental compositional distributions from a required low energy limit of 20 keV for protons and 45 keV for oxygen ions, up to > 0.5 MeV (with capabilities to measure up to > 1 MeV). FEEPS measures instantaneous all sky images of energetic electrons from 25 keV to > 0.5 MeV, and also measures total ion energy distributions from 45 keV to > 0.5 MeV to be used in conjunction with EIS to measure all sky ion distributions. In this report we describe the EPD investigation and the details of the EIS sensor. Specifically we describe EPD-level science objectives, the science and measurement requirements, and the challenges that the EPD team had in meeting these requirements. Here we also describe the design and operation of the EIS instruments, their calibrated performances, and the EIS in-flight and ground operations. Blake et al. (The Flys Eye Energetic Particle Spectrometer (FEEPS) contribution to the Energetic Particle Detector (EPD) investigation of the Magnetospheric Magnetoscale (MMS) Mission, this issue) describe the design and operation of the FEEPS instruments, their calibrated performances, and the FEEPS in-flight and ground operations. The MMS spacecraft will launch in early 2015, and over its 2-year mission will provide comprehensive measurements of magnetic reconnection at Earth's magnetopause during the 18 months that comprise orbital phase 1, and magnetic reconnection within Earth's magnetotail during the about 6 months that comprise orbital phase 2. C1 [Mauk, B. H.; Jaskulek, S. E.; Schlemm, C. E.; Brown, L. E.; Cooper, S. A.; Gurnee, R. S.; Hayes, J. R.; Hill, P. A.; Ho, G. C.; Hutcheson, J. C.; Kerem, S.; Mitchell, D. G.; Nelson, K. S.; Stokes, M. R.; Westlake, J. H.] Johns Hopkins Univ, Appl Phys Lab, Laurel, MD USA. [Blake, J. B.; Clemmons, J. H.; Fennell, J. F.] Aerosp Corp, El Segundo, CA 90245 USA. [Baker, D. N.; Craft, J. V.] Univ Colorado, LASP, Boulder, CO 80309 USA. [Spence, H. E.] Univ New Hampshire, Durham, NH 03824 USA. [Reeves, G. D.] Los Alamos Natl Lab, Los Alamos, NM USA. [Jacques, A. D.; Paschalidis, N. P.; Rossano, E.] NASA, Goddard Space Flight Ctr, Greenbelt, MD USA. [Hammock, C. M.] NASA, Johnson Space Ctr, Houston, TX USA. RP Mauk, BH (reprint author), Johns Hopkins Univ, Appl Phys Lab, Laurel, MD USA. EM barry.mauk@jhuapl.edu RI NASA MMS, Science Team/J-5393-2013; Mauk, Barry/E-8420-2017; OI NASA MMS, Science Team/0000-0002-9504-5214; Mauk, Barry/0000-0001-9789-3797; Clemmons, James/0000-0002-5298-5222; Reeves, Geoffrey/0000-0002-7985-8098 NR 46 TC 23 Z9 23 U1 0 U2 2 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0038-6308 EI 1572-9672 J9 SPACE SCI REV JI Space Sci. Rev. PD MAR PY 2016 VL 199 IS 1-4 BP 471 EP 514 DI 10.1007/s11214-014-0055-5 PG 44 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DJ6DI UT WOS:000374299800015 ER PT J AU Austin, KG Farina, EK Lieberman, HR AF Austin, Krista G. Farina, Emily K. Lieberman, Harris R. TI Self-reported side-effects associated with use of dietary supplements in an armed forces population SO DRUG TESTING AND ANALYSIS LA English DT Article DE protein supplements; combination products; body mass index; physical fitness ID MILITARY PERSONNEL; SAFETY; SOLDIERS AB Approximately 60-70% of Armed Forces personnel consume a dietary supplement (DS) at least once a week and there have been numerous reports of severe adverse events among DS users. This study assessed patterns of DS use and self-reported side-effects among 4400 Armed Forces personnel using a paper-and-pencil survey. Multivariable logistic regression was used to examine associations between patterns of DS use and self-reported side-effects. Sixty-nine percent of personnel surveyed reported using a DS. Seven percent of DS users reported experiencing abnormal heart beats, 6% tremors, 5% stomach pain, 3% dizziness, and 3% numbness/tingling and they believed these symptoms were associated with the use of DS. After adjustment for use of other DS classes, total supplement use, and demographic characteristics, protein supplement users were more likely than non-users to report numbness/tingling; combination product users were more likely to report experiencing abnormal heart beats, stomach pain, dizziness, tremors, and numbness/tingling; and users of purported steroid analogues were more likely to report dizziness. Use of more than one DS per week was associated with an increased likelihood of reporting side-effects. Respondents with a higher body mass index were more likely to report side-effects. Further research is necessary to determine whether self-reported side-effects associated with multiple DS use and some DS classes impact the long-term health or performance of service members. Surveillance of military populations using surveys like this one may provide a method for detecting adverse health events of DS before they are apparent in the civilian population. Copyright (c) 2015 John Wiley & Sons, Ltd. C1 [Austin, Krista G.; Farina, Emily K.; Lieberman, Harris R.] US Army, Mil Nutr Div, Environm Med Res Inst, Kansas St,Bldg 42, Natick, MA 01760 USA. [Austin, Krista G.; Farina, Emily K.] Oak Ridge Inst Sci & Educ, Belcamp, MD 21017 USA. RP Lieberman, HR (reprint author), US Army, Mil Nutr Div, Environm Med Res Inst, Kansas St,Bldg 42, Natick, MA 01760 USA. EM harris.r.lieberman.civ@mail.mil FU US Army Medical Research and Materiel Command; Department of Defense Center Alliance for Nutrition and Dietary Supplements Research FX US Army Medical Research and Materiel Command; Department of Defense Center Alliance for Nutrition and Dietary Supplements Research NR 23 TC 1 Z9 1 U1 1 U2 2 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1942-7603 EI 1942-7611 J9 DRUG TEST ANAL JI Drug Test. Anal. PD MAR-APR PY 2016 VL 8 IS 3-4 SI SI BP 287 EP 295 DI 10.1002/dta.1905 PG 9 WC Biochemical Research Methods; Chemistry, Analytical; Pharmacology & Pharmacy SC Biochemistry & Molecular Biology; Chemistry; Pharmacology & Pharmacy GA DJ5NP UT WOS:000374255900003 PM 26526399 ER PT J AU Mohamed, W Miller, B Porter, D Murty, K AF Mohamed, Walid Miller, Brandon Porter, Douglas Murty, Korukonda TI The Role of Grain Size on Neutron Irradiation Response of Nanocrystalline Copper SO MATERIALS LA English DT Article DE copper; nanocrystalline; neutron irradiation; grain growth; radiation hardening; thermal stability ID MECHANICAL-PROPERTIES; NANOSTRUCTURED MATERIALS; MATERIALS CHALLENGES; STRUCTURAL-MATERIALS; MICROSTRUCTURE; ALLOYS; GROWTH; STEEL; RESISTANCE; TOLERANCE AB The role of grain size on the developed microstructure and mechanical properties of neutron irradiated nanocrystalline copper was investigated by comparing the radiation response of material to the conventional micrograined counterpart. Nanocrystalline (nc) and micrograined (MG) copper samples were subjected to a range of neutron exposure levels from 0.0034 to 2 dpa. At all damage levels, the response of MG-copper was governed by radiation hardening manifested by an increase in strength with accompanying ductility loss. Conversely, the response of nc-copper to neutron irradiation exhibited a dependence on the damage level. At low damage levels, grain growth was the primary response, with radiation hardening and embrittlement becoming the dominant responses with increasing damage levels. Annealing experiments revealed that grain growth in nc-copper is composed of both thermally-activated and irradiation-induced components. Tensile tests revealed minimal change in the source hardening component of the yield stress in MG-copper, while the source hardening component was found to decrease with increasing radiation exposure in nc-copper. C1 [Mohamed, Walid; Murty, Korukonda] N Carolina State Univ, Dept Nucl Engn, Raleigh, NC 27695 USA. [Miller, Brandon; Porter, Douglas] Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. [Mohamed, Walid] Argonne Natl Lab, Nucl Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Mohamed, W (reprint author), N Carolina State Univ, Dept Nucl Engn, Raleigh, NC 27695 USA.; Mohamed, W (reprint author), Argonne Natl Lab, Nucl Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM wmohamed@anl.gov; brandon.miller@inl.gov; douglas.porter@inl.gov; murty@ncsu.edu FU NSUF-ATR through the US Department of Energy (DOE), Office of Nuclear Energy under DOE Idaho Operations Office [DE-AC07-051D14517] FX This work is supported by the NSUF-ATR through the US Department of Energy (DOE), Office of Nuclear Energy under DOE Idaho Operations Office Contract DE-AC07-051D14517. The authors wish to thank Joseph W. Nielsen for reactor environment and material damage calculations and Paul E. Murray for the thermal (Abaqus) calculations. NR 47 TC 1 Z9 1 U1 7 U2 16 PU MDPI AG PI BASEL PA POSTFACH, CH-4005 BASEL, SWITZERLAND SN 1996-1944 J9 MATERIALS JI Materials PD MAR PY 2016 VL 9 IS 3 AR UNSP 144 DI 10.3390/ma9030144 PG 23 WC Materials Science, Multidisciplinary SC Materials Science GA DI9ER UT WOS:000373805400026 ER PT J AU Machida, S Kelliher, DJ Edmonds, CS Kirkman, IW Berg, JS Jones, JK Muratori, BD Garland, JM AF Machida, S. Kelliher, D. J. Edmonds, C. S. Kirkman, I. W. Berg, J. S. Jones, J. K. Muratori, B. D. Garland, J. M. TI Amplitude-dependent orbital period in alternating gradient accelerators SO PROGRESS OF THEORETICAL AND EXPERIMENTAL PHYSICS LA English DT Article ID STORAGE-RING LASER; FFAG; EMMA AB Orbital period in a ring accelerator and time of flight in a linear accelerator depend on the amplitude of betatron oscillations. The variation is negligible in ordinary particle accelerators with relatively small beam emittance. In an accelerator for large emittance beams like muons and unstable nuclei, however, this effect cannot be ignored. We measured orbital period in a linear non-scaling fixed-field alternating-gradient accelerator, which is a candidate for muon acceleration, and compared it with the theoretical prediction. The good agreement between them gives important ground for the design of particle accelerators for a new generation of particle and nuclear physics experiments. C1 [Machida, S.; Kelliher, D. J.] STFC Rutherford Appleton Lab, ASTeC, Didcot OX11 0QX, Oxon, England. [Edmonds, C. S.; Kirkman, I. W.] Univ Liverpool, Liverpool L69 7ZE, Merseyside, England. [Berg, J. S.] Brookhaven Natl Lab, Bldg 901A,POB 5000, Upton, NY 11973 USA. [Jones, J. K.; Muratori, B. D.] STFC Daresbury Lab, ASTeC, Warrington WA4 4AD, Cheshire, England. [Garland, J. M.] Univ Manchester, Manchester M13 9PL, Lancs, England. [Edmonds, C. S.; Kirkman, I. W.; Jones, J. K.; Muratori, B. D.; Garland, J. M.] Cockcroft Inst Accelerator Sci & Technol, Warrington WA4 4AD, Cheshire, England. RP Machida, S (reprint author), STFC Rutherford Appleton Lab, ASTeC, Didcot OX11 0QX, Oxon, England. EM shinji.machida@stfc.ac.uk FU BASROC/CONFORM project under the EPSRC grant [EP/E032869]; US Department of Energy [DE-AC02-98CH10886, DE-SC0012704, DE-AC02-07CH11359]; STFC FX The work is supported by the BASROC/CONFORM project under the EPSRC grant No. EP/E032869, the US Department of Energy under contract Nos. DE-AC02-98CH10886, DE-SC0012704, and DE-AC02-07CH11359, and STFC. We would like to thank the entire ALICE/EMMA team. We would also like to thank Drs M. W. Poole, C. R. Prior, S. L. Smith, and A. Wolski for their encouragement. NR 27 TC 0 Z9 0 U1 3 U2 3 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 2050-3911 J9 PROG THEOR EXP PHYS JI Prog. Theor. Exp. Phys. PD MAR PY 2016 IS 3 AR 033G01 DI 10.1093/ptep/ptw006 PG 8 WC Physics, Multidisciplinary; Physics, Particles & Fields SC Physics GA DJ5BY UT WOS:000374223000003 ER PT J AU Dutheil, JY Mannhaupt, G Schweizer, G Sieber, CMK Munsterkotter, M Guldener, U Schirawski, J Kahmann, R AF Dutheil, Julien Y. Mannhaupt, Gertrud Schweizer, Gabriel Sieber, Christian M. K. Munsterkoetter, Martin Gueldener, Ulrich Schirawski, Jan Kahmann, Regine TI A Tale of Genome Compartmentalization: The Evolution of Virulence Clusters in Smut Fungi SO GENOME BIOLOGY AND EVOLUTION LA English DT Article DE genome architecture; effector proteins; gene duplication; repeat sequences; selection interference; gene cluster ID PATHOGEN USTILAGO-MAYDIS; INDUCED POINT MUTATIONS; TRANSPOSABLE ELEMENTS; SPORISORIUM-SCITAMINEUM; PHYLOGENETIC ANALYSIS; POPULATION GENOMICS; PLANT-PATHOGENS; OPEN SOFTWARE; SEQUENCES; ALIGNMENT AB Smut fungi are plant pathogens mostly parasitizing wild species of grasses as well as domesticated cereal crops. Genome analysis of several smut fungi including Ustilago maydis revealed a singular clustered organization of genes encoding secreted effectors. In U. maydis, many of these clusters have a role in virulence. Reconstructing the evolutionary history of clusters of effector genes is difficult because of their intrinsically fast evolution, which erodes the phylogenetic signal and homology relationships. Here, we describe the use of comparative evolutionary analyses of quality draft assemblies of genomes to study the mechanisms of this evolution. We report the genome sequence of a South African isolate of Sporisorium scitamineum, a smut fungus parasitizing sugar cane with a phylogenetic position intermediate to the two previously sequenced species U. maydis and Sporisorium reilianum. We show that the genome of S. scitamineum contains more and larger gene clusters encoding secreted effectors than any previously described species in this group. We trace back the origin of the clusters and find that their evolution is mainly driven by tandem gene duplication. In addition, transposable elements play a major role in the evolution of the clustered genes. Transposable elements are significantly associated with clusters of genes encoding fast evolving secreted effectors. This suggests that such clusters represent a case of genome compartmentalization that restrains the activity of transposable elements on genes under diversifying selection for which this activity is potentially beneficial, while protecting the rest of the genome from its deleterious effect. C1 [Dutheil, Julien Y.; Mannhaupt, Gertrud; Schweizer, Gabriel; Schirawski, Jan; Kahmann, Regine] Max Planck Inst Terr Microbiol, Dept Organism Interact, D-35043 Marburg, Germany. [Mannhaupt, Gertrud; Sieber, Christian M. K.; Munsterkoetter, Martin; Gueldener, Ulrich] German Res Ctr Environm Hlth GmbH, Helmholtz Zentrum Munchen, Inst Bioinformat & Syst Biol, Neuherberg, Germany. [Dutheil, Julien Y.] Max Planck Inst Evolutionary Biol, Dept Evolutionary Genet, Plon, Germany. [Sieber, Christian M. K.] DOE Joint Genome Inst, Walnut Creek, CA USA. [Schirawski, Jan] Rhein Westfal TH Aachen, Microbial Genet, Inst Appl Microbiol Aachen Biol & Biotechnol, Aachen, Germany. RP Dutheil, JY; Kahmann, R (reprint author), Max Planck Inst Terr Microbiol, Dept Organism Interact, D-35043 Marburg, Germany.; Dutheil, JY (reprint author), Max Planck Inst Evolutionary Biol, Dept Evolutionary Genet, Plon, Germany. EM dutheil@evolbio.mpg.de; kahmann@mpi-marburg.mpg.de RI Dutheil, Julien/K-5479-2016; OI Dutheil, Julien/0000-0001-7753-4121; Guldener, Ulrich/0000-0001-5052-8610 FU LOEWE program of the state of Hesse through SYNMIKRO; LOEWE program of the state of Hesse through Max Planck Society FX Our work was supported through the LOEWE program of the state of Hesse through SYNMIKRO and through the Max Planck Society. J.Y.D. would like to thank Eva H. Stukenbrock for her comments on a previous version of this manuscript. NR 86 TC 9 Z9 9 U1 16 U2 26 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 1759-6653 J9 GENOME BIOL EVOL JI Genome Biol. Evol. PD MAR PY 2016 VL 8 IS 3 BP 681 EP 704 DI 10.1093/gbe/evw026 PG 24 WC Evolutionary Biology; Genetics & Heredity SC Evolutionary Biology; Genetics & Heredity GA DI9RD UT WOS:000373839200018 PM 26872771 ER PT J AU Carmichael, JD Nemzek, R Arrowsmith, S Sentz, K AF Carmichael, Joshua D. Nemzek, Robert Arrowsmith, Stephen Sentz, Kari TI Fusing geophysical signatures of locally recorded surface explosions to improve blast detection SO GEOPHYSICAL JOURNAL INTERNATIONAL LA English DT Article DE Probability distributions; Electromagnetic theory; Controlled source seismology; Statistical seismology; Wave propagation; Acoustic properties ID FILTER AB We recorded acoustic, seismic and radio-frequency signatures of 70 solid charge (similar to 2-12 kg) surface explosions (shots) at local distances (0.1-1.5 km) to determine if such signals could be fused for blast monitoring. We observed that each geophysical signature was sufficiently repeatable between similar shots to be identifiable with multichannel correlation detectors. Using template signals from a large explosion, we then processed heavily contaminated data recording a smaller shot with these detectors, and missed or marginally detected the resultant target signals. By then fusing the p-values of these statistics through Fisher's combined probability test, we clearly identified the same explosion signals at thresholds consistent with the false alarm on noise rates of the correlation detectors. This resulting Fisher test thereby provided high-probability detections, zero false alarms and higher theoretical detection capability. C1 [Carmichael, Joshua D.; Nemzek, Robert; Arrowsmith, Stephen; Sentz, Kari] Los Alamos Natl Lab, Bikini Atoll Rd,SM 30, Los Alamos, NM 87544 USA. RP Carmichael, JD (reprint author), Los Alamos Natl Lab, Bikini Atoll Rd,SM 30, Los Alamos, NM 87544 USA. EM josh.carmichael@gmail.com FU DOE Office of Defense Nuclear Non-proliferation Research and Development; Defense Threat Reduction Agency [HD-TRA1411431] FX The DOE Office of Defense Nuclear Non-proliferation Research and Development funded data collection. The Defense Threat Reduction Agency supported work under Interagency Agreement HD-TRA1411431. Amanda Ziemann improved writing clarity. Rick Picard provided helpful feedback on statistics. NR 10 TC 2 Z9 2 U1 2 U2 3 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0956-540X EI 1365-246X J9 GEOPHYS J INT JI Geophys. J. Int. PD MAR PY 2016 VL 204 IS 3 BP 1838 EP 1842 DI 10.1093/gji/ggw006 PG 5 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DI7YY UT WOS:000373719100030 ER PT J AU Amer, BR Macdonald, R Jacobitz, AW Liauw, B Clubb, RT AF Amer, Brendan R. Macdonald, Ramsay Jacobitz, Alex W. Liauw, Brandon Clubb, Robert T. TI Rapid addition of unlabeled silent solubility tags to proteins using a new substrate-fused sortase reagent SO JOURNAL OF BIOMOLECULAR NMR LA English DT Article DE Silent solubility tag; Sortase; Protein ligation; SUMO ID STAPHYLOCOCCUS-AUREUS SORTASE; SUMO FUSION TECHNOLOGY; ESCHERICHIA-COLI; CELL-WALL; MYCOBACTERIUM-TUBERCULOSIS; RECOMBINANT PROTEINS; MEDIATED LIGATION; SURFACE-PROTEINS; IN-VIVO; EXPRESSION AB Many proteins can't be studied using solution NMR methods because they have limited solubility. To overcome this problem, recalcitrant proteins can be fused to a more soluble protein that functions as a solubility tag. However, signals arising from the solubility tag hinder data analysis because they increase spectral complexity. We report a new method to rapidly and efficiently add a non-isotopically labeled Small Ubiquitin-like Modifier protein (SUMO) solubility tag to an isotopically labeled protein. The method makes use of a newly developed SUMO-Sortase tagging reagent in which SUMO and the Sortase A (SrtA) enzyme are present within the same polypeptide. The SUMO-Sortase reagent rapidly attaches SUMO to any protein that contains the sequence LPXTG at its C-terminus. It modifies proteins at least 15-times faster than previously described approaches, and does not require active dialysis or centrifugation during the reaction to increase product yields. In addition, silently tagged proteins are readily purified using the well-established SUMO expression and purification system. The utility of the SUMO-Sortase tagging reagent is demonstrated using PhoP and green fluorescent proteins, which are similar to 90 % modified with SUMO at room temperature within four hours. SrtA is widely used as a tool to construct bioconjugates. Significant rate enhancements in these procedures may also be achieved by fusing the sortase enzyme to its nucleophile substrate. C1 [Amer, Brendan R.; Macdonald, Ramsay; Jacobitz, Alex W.; Liauw, Brandon; Clubb, Robert T.] Univ Calif Los Angeles, Dept Chem & Biochem, 602 Boyer Hall, Los Angeles, CA 90095 USA. [Amer, Brendan R.; Macdonald, Ramsay; Jacobitz, Alex W.; Liauw, Brandon; Clubb, Robert T.] Univ Calif Los Angeles, UCLA DOE, Inst Genom & Prote, 611 Charles Young Dr East, Los Angeles, CA 90095 USA. [Clubb, Robert T.] Univ Calif Los Angeles, Inst Mol Biol, 611 Charles Young Dr East, Los Angeles, CA 90095 USA. RP Clubb, RT (reprint author), Univ Calif Los Angeles, Dept Chem & Biochem, 602 Boyer Hall, Los Angeles, CA 90095 USA.; Clubb, RT (reprint author), Univ Calif Los Angeles, UCLA DOE, Inst Genom & Prote, 611 Charles Young Dr East, Los Angeles, CA 90095 USA.; Clubb, RT (reprint author), Univ Calif Los Angeles, Inst Mol Biol, 611 Charles Young Dr East, Los Angeles, CA 90095 USA. EM rclubb@mbi.ucla.edu FU UCLA Molecular Biology Institute; Cellular and Molecular Biology Training Grant (Ruth L. Kirschstein National Research Service Award) [GM007185]; National Institutes of Health [AI52217]; US Department of Energy Office of Science, Office of Biological and Environmental Research program [DE-FC02-02ER63421] FX We would like to thank Dibyendu Sakar (Institute of Microbial Technology, India) for the plasmid encoding PhoP and members of the Clubb group for useful discussion. B.R.A was supported by a Whitcome Pre-doctoral training grant from the UCLA Molecular Biology Institute, and R.M. was supported by a Cellular and Molecular Biology Training Grant (Ruth L. Kirschstein National Research Service Award GM007185). This work was supported by the National Institutes of Health grant AI52217 to RTC. As well as support through the US Department of Energy Office of Science, Office of Biological and Environmental Research program under Award Number DE-FC02-02ER63421. NR 35 TC 2 Z9 2 U1 1 U2 4 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0925-2738 EI 1573-5001 J9 J BIOMOL NMR JI J. Biomol. NMR PD MAR PY 2016 VL 64 IS 3 BP 197 EP 205 DI 10.1007/s10858-016-0019-z PG 9 WC Biochemistry & Molecular Biology; Spectroscopy SC Biochemistry & Molecular Biology; Spectroscopy GA DI9YZ UT WOS:000373859900002 PM 26852413 ER PT J AU Feng, H Qian, Y Gallagher, FJ Zhang, WG Yu, LZ Liu, CJ Jones, KW Tappero, R AF Feng, Huan Qian, Yu Gallagher, Frank J. Zhang, Weiguo Yu, Lizhong Liu, Changjun Jones, Keith W. Tappero, Ryan TI Synchrotron micro-scale measurement of metal distributions in Phragmites australis and Typha latifolia root tissue from an urban brownfield site SO JOURNAL OF ENVIRONMENTAL SCIENCES LA English DT Article DE Phragmites australis; Typha latifolia; Trace metals; Synchrotron radiation technique; Brownfield ID X-RAY-FLUORESCENCE; RIVER INTERTIDAL ZONE; HEAVY-METAL; IRON PLAQUE; CADMIUM ACCUMULATION; ASTER-TRIPOLIUM; AQUATIC PLANTS; ZINC; LEAD; FE AB Liberty State Park in New Jersey, USA, is a "brownfield" site containing various levels of contaminants. To investigate metal uptake and distributions in plants on the brownfield site, Phragmites australis and Typha latifolia were collected in Liberty State Park during the growing season (May-September) in 2011 at two sites with the high and low metal loads, respectively. The objective of this study was to understand the metal (Fe, Mn, Cu, Pb and Zn) concentration and spatial distributions in P. australis and T. latifolia root systems with micro-meter scale resolution using synchrotron X-ray microfluorescence (mu XRF) and synchrotron X-ray computed microtomography (mu CMT) techniques. The root structure measurement by synchrotron mu CMT showed that high X-ray attenuation substance appeared in the epidermis. Synchrotron mu XRF measurement showed that metal concentrations and distributions in the root cross-section between epidermis and vascular tissue were statistically different. Significant correlations were found between metals (Cu, Mn, Pb and Zn) and Fe in the epidermis, implying that metals were scavenged by Fe oxides. The results from this study suggest that the expression of metal transport and accumulation within the root systems may be element specific. The information derived from this study can improve our current knowledge of the wetland plant ecological function in brownfield remediation. (C) 2015 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V. C1 [Feng, Huan; Qian, Yu] Montclair State Univ, Dept Earth & Environm Studies, Montclair, NJ 07043 USA. [Gallagher, Frank J.] Rutgers State Univ, Urban Forestry Program, Dept Ecol Evolut & Nat Resources, New Brunswick, NJ 08901 USA. [Zhang, Weiguo; Yu, Lizhong] E China Normal Univ, State Key Lab Estuarine & Coastal Res, Shanghai 200062, Peoples R China. [Liu, Changjun; Jones, Keith W.] Brookhaven Natl Lab, Biol Environm & Climate Sci Dept, Upton, NY 11973 USA. [Tappero, Ryan] Brookhaven Natl Lab, Photon Sci Directorate, Upton, NY 11973 USA. RP Feng, H (reprint author), Montclair State Univ, Dept Earth & Environm Studies, Montclair, NJ 07043 USA. EM fengh@mail.montclair.edu FU Margaret and Herman Sokol Foundation; China Scholarship Council; State Key Laboratory of Estuarine and Coastal Research Open Research Fund [SKLEC-KF201304]; U.S. Department of Energy, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Visiting Faculty Program (VFP); Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the US Department of Energy [DEAC0298CH10886]; National Science Foundation [MCB-1051675]; U.S. Department of Energy-Geosciences [DE-FG02-92ER14244]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work was supported in part by the Margaret and Herman Sokol Foundation (HF), China Scholarship Council (YQ) and the State Key Laboratory of Estuarine and Coastal Research Open Research Fund (Ref #: SKLEC-KF201304) (HF, WZ, LY, YQ). This project was also supported in part by the U.S. Department of Energy, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Visiting Faculty Program (VFP) (HF). Portions of this work were performed at Beamline X27A, National Synchrotron Light Source (NSLS), and Biosciences Department, Brookhaven National Laboratory. Work in Bioscience Department, BNL, was partially supported by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the US Department of Energy through Grant DEAC0298CH10886 and the National Science Foundation through grant MCB-1051675 (CJL). X27A is supported in part by the U.S. Department of Energy-Geosciences (DE-FG02-92ER14244 to The University of Chicago - CARS). Use of the NSLS was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. We are also grateful to two anonymous reviewers who offered constructive comments and suggestions on an earlier draft of this paper. NR 54 TC 3 Z9 3 U1 9 U2 26 PU SCIENCE PRESS PI BEIJING PA 16 DONGHUANGCHENGGEN NORTH ST, BEIJING 100717, PEOPLES R CHINA SN 1001-0742 EI 1878-7320 J9 J ENVIRON SCI-CHINA JI J. Environ. Sci. PD MAR 1 PY 2016 VL 41 BP 172 EP 182 DI 10.1016/j.jes.2015.07.015 PG 11 WC Environmental Sciences SC Environmental Sciences & Ecology GA DI1BQ UT WOS:000373231400020 PM 26969063 ER PT J AU Hiatt, JR Rivard, MJ Hughes, HG AF Hiatt, Jessica R. Rivard, Mark J. Hughes, H. Grady TI Simulation evaluation of NIST air-kerma rate calibration standard for electronic brachytherapy SO MEDICAL PHYSICS LA English DT Article DE electronic brachytherapy; calibration; MCNP6 ID MONTE-CARLO; LOW-ENERGY; DOSIMETRY; FORMALISM; WATER AB Purpose: Dosimetry for the model S700 50 kV electronic brachytherapy (eBT) source (Xoft, Inc., a subsidiary of iCAD, San Jose, CA) was simulated using Monte Carlo (MC) methods by Rivard et al. ["Calculated and measured brachytherapy dosimetry parameters in water for the Xoft Axxent x-ray source: An electronic brachytherapy source," Med. Phys. 33, 4020-4032 (2006)] and recently by Hiatt et al. ["A revised dosimetric characterization of the model S700 electronic brachytherapy source containing an anode-centering plastic insert and other components not included in the 2006 model," Med. Phys. 42, 2764-2776 (2015)] with improved geometric characterization. While these studies examined the dose distribution in water, there have not previously been reports of the eBT source calibration methods beyond that recently reported by Seltzer et al. ["New national air-kerma standard for low-energy electronic brachytherapy sources," J. Res. Natl. Inst. Stand. Technol. 119, 554-574 (2014)]. Therefore, the motivation for the current study was to provide an independent determination of air-kerma rate at 50 cm in air. (K)over dot(air)(d = 50 cm) using MC methods for the model S700 eBT source. Methods: Using CAD information provided by the vendor and disassembled sources, an MC model was created for the S700 eBT source. Simulations were run using the MCNP6 radiation transport code for the NIST Lamperti air ionization chamber according to specifications by Boutillon et al. ["Comparison of exposure standards in the 10-50 kV x-ray region," Metrologia 5, 1-11 (1969)], in air without the Lamperti chamber, and in vacuum without the Lamperti chamber. (K)over dot(air)(d = 50 cm) was determined using the *F4 tally with NIST values for the mass energy-absorption coefficients for air. Photon spectra were evaluated over 2 pi azimuthal sampling for polar angles of 0 degrees <= theta <= 180 degrees every 1 degrees. Volume averaging was averted through tight radial binning. Photon energy spectra were determined over all polar angles in both air and vacuum using the *F4 tally with 0.1 keV resolution. A total of 1011 simulated histories were run for the Lamperti chamber geometry (statistical uncertainty of 0.14%), with 1010 histories for the in-air and in-vacuum simulations (statistical uncertainty of 0.04%). The total standard uncertainty in the calculated air-kerma rate determination amounted to 6.8%. Results: MC simulations determined the air-kerma rate at 50 cm from the source with the modeled Lamperti chamber to be (1.850 +/- 0.126) x10(-4) Gy/s, which was within the range of (K)over dot(air)(d = 50 cm) values (1.67-2.11) x10-4 Gy/s measured by NIST. The ratio of the photon spectra in air and in vacuum were in good agreement above 13 keV, and for theta < 150 degrees where the influence of the Kovar sleeve and the Ag epoxy components caused increased scatter in air. Below 13 keV, the ratio of the photon spectra in air to vacuum exhibited a decrease that was attributed to increased attenuation of the photons in air. Across most of the energy range on the source transverse plane, there was good agreement between the authors' simulated spectra and that measured by NIST. Discrepancies were observed above 40 keV where the NIST spectrum had a steeper fall-off towards 50 keV. Conclusions: Through MC simulations of radiation transport, this study provided an independent validation of the measured air-kerma rate at 50 cm in air at NIST for the model S700 eBT source, with mean results in agreement within 3.3%. This difference was smaller than the range (i. e., 23%) of the measured values. (C) 2016 American Association of Physicists in Medicine. C1 [Hiatt, Jessica R.] Univ Massachusetts, Biomed Engn & Biotechnol, Lowell, MA 01854 USA. [Rivard, Mark J.] Tufts Univ, Sch Med, Dept Radiat Oncol, Boston, MA 02111 USA. [Hughes, H. Grady] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Rivard, MJ (reprint author), Tufts Univ, Sch Med, Dept Radiat Oncol, Boston, MA 02111 USA. EM mark.j.rivard@gmail.com NR 30 TC 1 Z9 1 U1 0 U2 1 PU AMER ASSOC PHYSICISTS MEDICINE AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 0094-2405 J9 MED PHYS JI Med. Phys. PD MAR PY 2016 VL 43 IS 3 BP 1119 EP 1129 DI 10.1118/1.4940791 PG 11 WC Radiology, Nuclear Medicine & Medical Imaging SC Radiology, Nuclear Medicine & Medical Imaging GA DI7UI UT WOS:000373707100010 PM 26936699 ER PT J AU Cavender-Bares, J Meireles, JE Couture, JJ Kaproth, MA Kingdon, CC Singh, A Serbin, SP Center, A Zuniga, E Pilz, G Townsend, PA AF Cavender-Bares, Jeannine Meireles, Jose Eduardo Couture, John J. Kaproth, Matthew A. Kingdon, Clayton C. Singh, Aditya Serbin, Shawn P. Center, Alyson Zuniga, Esau Pilz, George Townsend, Philip A. TI Associations of Leaf Spectra with Genetic and Phylogenetic Variation in Oaks: Prospects for Remote Detection of Biodiversity SO REMOTE SENSING LA English DT Article DE evolution; leaf functional traits; hyperspectral data; optical classification; tree of life; PLS-DA; genetic variation; hierarchical organization of plant diversity; phylogenetic signal; populations ID MULTIVARIATE IMAGE-ANALYSIS; CLIMATIC-NICHE EVOLUTION; QUERCUS SERIES VIRENTES; ECONOMICS SPECTRUM; CANOPY DIVERSITY; PLANT DIVERSITY; PLS-DA; SPECTROSCOPY; TRAITS; FOREST AB Species and phylogenetic lineages have evolved to differ in the way that they acquire and deploy resources, with consequences for their physiological, chemical and structural attributes, many of which can be detected using spectral reflectance form leaves. Recent technological advances for assessing optical properties of plants offer opportunities to detect functional traits of organisms and differentiate levels of biological organization across the tree of life. Here, we connect leaf-level full range spectral data (400-2400 nm) of leaves to the hierarchical organization of plant diversity within the oak genus (Quercus) using field and greenhouse experiments in which environmental factors and plant age are controlled. We show that spectral data significantly differentiate populations within a species and that spectral similarity is significantly associated with phylogenetic similarity among species. We further show that hyperspectral information allows more accurate classification of taxa than spectrally-derived traits, which by definition are of lower dimensionality. Finally, model accuracy increases at higher levels in the hierarchical organization of plant diversity, such that we are able to better distinguish clades than species or populations. This pattern supports an evolutionary explanation for the degree of optical differentiation among plants and demonstrates potential for remote detection of genetic and phylogenetic diversity. C1 [Cavender-Bares, Jeannine; Meireles, Jose Eduardo; Kaproth, Matthew A.; Center, Alyson] Univ Minnesota, Dept Ecol Evolut & Behav, St Paul, MN 55108 USA. [Couture, John J.; Kingdon, Clayton C.; Singh, Aditya; Serbin, Shawn P.; Townsend, Philip A.] Univ Wisconsin, Dept Forest & Wildlife Ecol, Madison, WI 53706 USA. [Serbin, Shawn P.] Brookhaven Natl Lab, Environm & Climate Sci Dept, Upton, NY 11973 USA. [Center, Alyson] St Olaf Coll, Dept Biol, Northfield, MN 55057 USA. [Zuniga, Esau; Pilz, George] Univ Zamorano, Dept Ingn Ambiente & Desarrollo, Zamorano, Honduras. RP Cavender-Bares, J; Meireles, JE (reprint author), Univ Minnesota, Dept Ecol Evolut & Behav, St Paul, MN 55108 USA. EM cavender@umn.edu; meireles@umn.edu; jjcouture@wisc.edu; mkaproth@umn.edu; kingdon@wisc.edu; singh22@wisc.edu; sserbin@bnl.gov; center1@stolaf.edu; esaunico@gmail.com; gpilz@zamorano.edu; ptownsend@wisc.edu RI Singh, Aditya/I-3628-2013; Serbin, Shawn/B-6392-2009; Townsend, Philip/B-5741-2008 OI Singh, Aditya/0000-0001-5559-9151; Serbin, Shawn/0000-0003-4136-8971; Townsend, Philip/0000-0001-7003-8774 FU National Science Foundation [IOS 0843665, DEB 1146380, DEB 1342872]; National Aeronautic and Space Agency (NASA) [NNX12AQ28G] FX We thank Susan Ustin for the invitation to submit the manuscript; John McVay, Andrew Hipp, Paul Manos and Antonio Gonzalez-Rodriguez for use of unpublished phylogenetic information on an ongoing collaborative project on the Oaks of the Americas. The project was funded by the National Science Foundation IOS 0843665, DEB 1146380 (Jeannine Cavender-Bares) and DEB 1342872 (Jeannine Cavender-Bares and Philip A. Townsend), co-funded by the National Aeronautic and Space Agency (NASA) through the Dimensions of Biodiversity program and from the HyspIRI program grant NNX12AQ28G (Philip A. Townsend). We thank Timothy Longwell for managing Experiment 1 in an early phase of the project. NR 63 TC 2 Z9 2 U1 8 U2 18 PU MDPI AG PI BASEL PA POSTFACH, CH-4005 BASEL, SWITZERLAND SN 2072-4292 J9 REMOTE SENS-BASEL JI Remote Sens. PD MAR PY 2016 VL 8 IS 3 DI 10.3390/rs8030221 PG 17 WC Remote Sensing SC Remote Sensing GA DI6RJ UT WOS:000373627400043 ER PT J AU Rafique, R Zhao, F de Jong, R Zeng, N Asrar, GR AF Rafique, Rashid Zhao, Fang de Jong, Rogier Zeng, Ning Asrar, Ghassem R. TI Global and Regional Variability and Change in Terrestrial Ecosystems Net Primary Production and NDVI: A Model-Data Comparison SO REMOTE SENSING LA English DT Article DE spatial trends; carbon cycle; TRENDY models; NPP; NDVI; ecosystems; temporal trends ID EARTH SYSTEM MODELS; LEAF-AREA INDEX; VEGETATION INDEX; CARBON-CYCLE; FUTURE-DIRECTIONS; CLIMATE-CHANGE; TIME-SERIES; TRENDS; SOIL; NPP AB The net primary productivity (NPP) is commonly used for understanding the dynamics of terrestrial ecosystems and their role in carbon cycle. We used a combination of the most recent NDVI and model-based NPP estimates (from five models of the TRENDY project) for the period 1982-2012, to study the role of terrestrial ecosystems in carbon cycle under the prevailing climate conditions. We found that 80% and 67% of the global land area showed positive NPP and NDVI values, respectively, for this period. The global NPP was estimated to be about 63 Pg C center dot y(-1), with an increase of 0.214 Pg C center dot y(-1)center dot y(-1). Similarly, the global mean NDVI was estimated to be 0.33, with an increasing trend of 0.00041 y(-1). The spatial patterns of NPP and NDVI demonstrated substantial variability, especially at the regional level, for most part of the globe. However, on temporal scale, both global NPP and NDVI showed a corresponding pattern of increase (decrease) for the duration of this study except for few years (e.g., 1990 and 1995-1998). Generally, the Northern Hemisphere showed stronger NDVI and NPP increasing trends over time compared to the Southern Hemisphere; however, NDVI showed larger trends in Temperate regions while NPP showed larger trends in Boreal regions. Among the five models, the maximum and minimum NPP were produced by JULES (72.4 Pg C center dot y(-1)) and LPJ (53.72 Pg C center dot y(-1)) models, respectively. At latitudinal level, the NDVI and NPP ranges were similar to 0.035 y(-1) to similar to-0.016 y(-1) and similar to 0.10 Pg C center dot y(-1)center dot y(-1) to similar to-0.047 Pg C center dot y(-1)center dot y(-1), respectively. Overall, the results of this study suggest that the modeled NPP generally correspond to the NDVI trends in the temporal dimension. The significant variability in spatial patterns of NPP and NDVI trends points to a need for research to understand the causes of these discrepancies between molded and observed ecosystem dynamics, and the carbon cycle. C1 [Rafique, Rashid; Asrar, Ghassem R.] Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD 20740 USA. [Zhao, Fang; Zeng, Ning] Univ Maryland, Dept Atmospher & Ocean Sci, College Pk, MD 20740 USA. [Zhao, Fang] Potsdam Inst Climate Impact Res, D-14412 Potsdam, Germany. [de Jong, Rogier] Univ Zurich, Dept Geog, Remote Sensing Labs, Winterthurerstr 190, CH-8057 Zurich, Switzerland. RP Rafique, R (reprint author), Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD 20740 USA. EM rashidbao@gmail.com; fangzhao@pik-potsdam.de; rogier.dejong@geo.uzh.ch; zeng@umd.edu; Ghassem.Asrar@pnnl.gov RI Zeng, Ning/A-3130-2008; OI Zeng, Ning/0000-0002-7489-7629; Rafique, Rashid/0000-0001-9591-6588 FU Laboratory Directed Research and Development project - Pacific Northwest National Laboratory of the U.S. Department of Energy FX This study was funded primarily by a Laboratory Directed Research and Development project sponsored by the Pacific Northwest National Laboratory of the U.S. Department of Energy. We acknowledge the contribution of by the TRENDY project teams for allowing us to use their simulated NPP data. We thank three anonymous reviewers for their valuable comments that led to further improvement of the manuscript. NR 49 TC 2 Z9 2 U1 9 U2 21 PU MDPI AG PI BASEL PA POSTFACH, CH-4005 BASEL, SWITZERLAND SN 2072-4292 J9 REMOTE SENS-BASEL JI Remote Sens. PD MAR PY 2016 VL 8 IS 3 DI 10.3390/rs8030177 PG 16 WC Remote Sensing SC Remote Sensing GA DI6RJ UT WOS:000373627400038 ER PT J AU Wang, R Gamon, JA Emmerton, CA Li, HT Nestola, E Pastorello, GZ Menzer, O AF Wang, Ran Gamon, John A. Emmerton, Craig A. Li, Haitao Nestola, Enrica Pastorello, Gilberto Z. Menzer, Olaf TI Integrated Analysis of Productivity and Biodiversity in a Southern Alberta Prairie SO REMOTE SENSING LA English DT Article DE biomass; eddy covariance; remote sensing; grassland; biodiversity ID USE EFFICIENCY MODEL; FUNCTIONAL DIVERSITY; SPECIES RICHNESS; GRASSLAND; VEGETATION; RADIATION; EVENNESS; NDVI; FLUX; CLASSIFICATION AB Grasslands play important roles in ecosystem production and support a large farming and grazing industry. An accurate and efficient way is needed to estimate grassland health and production for monitoring and adjusting management to get sustainable products and other ecosystem services. Previous studies of grasslands have shown varying relationships between productivity and biodiversity, with most showing either a positive or a hump-shaped relationship where productivity peaks at intermediate diversity. In this study, we used airborne imaging spectrometry combined with ground sampling and eddy covariance measurements to estimate the spatial pattern of production and biodiversity for two sites of contrasting productivity in a southern Alberta prairie ecosystem. Resulting patterns revealed that more diverse sites generally had greater productivity, supporting the hypothesis of a positive relationship between production and biodiversity for this site. We showed that the addition of evenness to richness (using the Shannon Index of dominant species instead of the number of dominant species alone) improved the correlation with optical diversity, an optically derived metric of biodiversity based on the coefficient of variation in spectral reflectance across space. Similarly, the Shannon Index was better correlated with productivity (estimated via NDVI (Normalized Difference Vegetation Index)) than the number of dominant species alone. Optical diversity provided a potent proxy for other more traditional biodiversity metrics (richness and Shannon index). Coupling field measurements and imaging spectrometry provides a method for assessing grassland productivity and biodiversity at a larger scale than can be sampled from the ground, and allows the integrated analysis of the productivity-biodiversity relationship over large areas. C1 [Wang, Ran; Gamon, John A.] Univ Alberta, Dept Earth & Atmospher Sci, Edmonton, AB T6G 2E3, Canada. [Gamon, John A.; Emmerton, Craig A.] Univ Alberta, Dept Biol Sci, Edmonton, AB T6G 2E9, Canada. [Li, Haitao] Univ Alberta, Dept Renewable Resources, Edmonton, AB T6G 2H1, Canada. [Nestola, Enrica] CNR, Inst Agroenvironm & Forest Biol IBAF, I-05010 Porano, Italy. [Pastorello, Gilberto Z.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. [Menzer, Olaf] Univ Calif Santa Barbara, Dept Geog, Santa Barbara, CA 93106 USA. RP Wang, R; Gamon, JA (reprint author), Univ Alberta, Dept Earth & Atmospher Sci, Edmonton, AB T6G 2E3, Canada.; Gamon, JA (reprint author), Univ Alberta, Dept Biol Sci, Edmonton, AB T6G 2E9, Canada. EM rw6@ualberta.ca; jgamon@gmail.com; emmerton@ualberta.ca; haitao2@ualberta.ca; enrica.nestola@ibaf.cnr.it; gzpastorello@lbl.gov; menzer@umail.ucsb.edu FU iCORE; AITF; Rangeland Research Institute; CFI; NSERC; China Scholarship Council fellowship FX We thank David Stonehouse and Verimap for help with the airborne acquisition, Adrienne Tastad, Ellen Macdonald and Lori Schroeder for providing information regarding the Mattheis Research Ranch land cover and soil map, and Ed Bork for information on grazing and management regimes. Evan Delancey provided help in using geo-referencing code for airborne data. Chris Wong, Shayna Harris, Saulo Castro, and Kyle Springer provided field assistance. This work was supported by iCORE, AITF, Rangeland Research Institute, CFI, and NSERC funding to J.A.G., and China Scholarship Council fellowship to R.W. We are grateful to Edwin and Ruth Mattheis for providing the University of Alberta with the Mattheis Ranch to support long-term research. NR 60 TC 3 Z9 3 U1 6 U2 18 PU MDPI AG PI BASEL PA POSTFACH, CH-4005 BASEL, SWITZERLAND SN 2072-4292 J9 REMOTE SENS-BASEL JI Remote Sens. PD MAR PY 2016 VL 8 IS 3 DI 10.3390/rs8030214 PG 20 WC Remote Sensing SC Remote Sensing GA DI6RJ UT WOS:000373627400071 ER PT J AU Zeng, HC Lu, T Jenkins, H Negron-Juarez, RI Xu, JC AF Zeng, Hongcheng Lu, Tao Jenkins, Hillary Negron-Juarez, Robinson I. Xu, Jiceng TI Assessing Earthquake-Induced Tree Mortality in Temperate Forest Ecosystems: A Case Study from Wenchuan, China SO REMOTE SENSING LA English DT Article DE biomass carbon loss; synthetic approach; remote sensing; earthquake; forest mortality ID VEGETATION RECOVERY; TIBETAN PLATEAU; BOREAL FORESTS; RIVER-BASIN; LANDSLIDES; BIOMASS; DAMAGE; DISTURBANCE; LANDSAT; MODEL AB Earthquakes can produce significant tree mortality, and consequently affect regional carbon dynamics. Unfortunately, detailed studies quantifying the influence of earthquake on forest mortality are currently rare. The committed forest biomass carbon loss associated with the 2008 Wenchuan earthquake in China is assessed by a synthetic approach in this study that integrated field investigation, remote sensing analysis, empirical models and Monte Carlo simulation. The newly developed approach significantly improved the forest disturbance evaluation by quantitatively defining the earthquake impact boundary and detailed field survey to validate the mortality models. Based on our approach, a total biomass carbon of 10.9 Tg center dot C was lost in Wenchuan earthquake, which offset 0.23% of the living biomass carbon stock in Chinese forests. Tree mortality was highly clustered at epicenter, and declined rapidly with distance away from the fault zone. It is suggested that earthquakes represent a significant driver to forest carbon dynamics, and the earthquake-induced biomass carbon loss should be included in estimating forest carbon budgets. C1 [Zeng, Hongcheng; Lu, Tao; Xu, Jiceng] Chinese Acad Sci, Chengdu Inst Biol, Chengdu 610041, Peoples R China. [Zeng, Hongcheng; Lu, Tao; Xu, Jiceng] Chinese Acad Sci, Key Lab Mt Ecol Restorat & Bioresource Utilizat &, Key Lab Sichuan Prov, Chengdu 610041, Peoples R China. [Zeng, Hongcheng] Univ Toronto, Fac Forestry, Toronto, ON M5S 3B3, Canada. [Jenkins, Hillary] Univ Redlands, Dept Environm Studies, Redlands, CA 92373 USA. [Negron-Juarez, Robinson I.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Lu, T (reprint author), Chinese Acad Sci, Chengdu Inst Biol, Chengdu 610041, Peoples R China.; Lu, T (reprint author), Chinese Acad Sci, Key Lab Mt Ecol Restorat & Bioresource Utilizat &, Key Lab Sichuan Prov, Chengdu 610041, Peoples R China. EM zenghch@gmail.com; lutao@cib.ac.cn; hillarysandfordjenkins@gmail.com; robinson.inj@lbl.gov; Jicengxu@gmail.com RI Negron-Juarez, Robinson/I-6289-2016 FU Strategic Priority Research Program of the Chinese Academy of Sciences [XDA05050407]; National Natural Science Foundation of China [41371126]; Office of Science, Office of Biological and Environmental Research of the US Department of Energy as part of Next-Generation Ecosystems Experiments (NGEE Tropics) [DE-AC02-05CH11231]; Regional and Global Climate Modeling (RGCM) FX The study was funded jointly by the Strategic Priority Research Program of the Chinese Academy of Sciences (#XDA05050407) and the National Natural Science Foundation of China (#41371126). R.N-J. was supported by the Director, Office of Science, Office of Biological and Environmental Research of the US Department of Energy under Contract No. DE-AC02-05CH11231 as part of Next-Generation Ecosystems Experiments (NGEE Tropics) and the Regional and Global Climate Modeling (RGCM) and Programs. NR 40 TC 0 Z9 0 U1 3 U2 8 PU MDPI AG PI BASEL PA POSTFACH, CH-4005 BASEL, SWITZERLAND SN 2072-4292 J9 REMOTE SENS-BASEL JI Remote Sens. PD MAR PY 2016 VL 8 IS 3 DI 10.3390/rs8030252 PG 17 WC Remote Sensing SC Remote Sensing GA DI6RJ UT WOS:000373627400033 ER PT J AU Martel, I Bontoiu, C Orduz, AK Acosta, L Barrios, E Carrasco, R Duenas, JA Gordo-Yanez, D Peregrin, A Pinto-Gomez, AR Prieto-Thomas, JA Ruiz-Pomares, MJ Junquera, T Sanchez-Segovia, J Ostroumov, PN Villari, ACC Harakeh, MN Acosta, LA AF Martel, I. Bontoiu, C. Orduz, A. K. Acosta, L. Barrios, E. Carrasco, R. Duenas, J. A. Gordo-Yanez, D. Peregrin, A. Pinto-Gomez, A. R. Prieto-Thomas, J. A. Ruiz-Pomares, M. J. Junquera, T. Sanchez-Segovia, J. Ostroumov, P. N. Villari, A. C. C. Harakeh, M. N. Acosta, L. A. TI ECOS-LINCE: A HIGH-INTENSITY HEAVY-ION FACILITY FOR NUCLEAR STRUCTURE AND REACTIONS SO ACTA PHYSICA POLONICA B LA English DT Article AB During the last years, the ECOS working group has been considering the construction of a new high-intensity accelerator of stable ion beams for the next Long-Range Plan of the nuclear physics community in Europe. The new facility (LINCE) will be a multi-user facility dedicated to ECOS science: fundamental physics, astrophysics, nuclear structure and reaction dynamics. In this paper, we summarize preliminary design studies of the low-energy part of this facility based on the use of a multi-ion superconducting linac. C1 [Martel, I.; Bontoiu, C.; Orduz, A. K.; Acosta, L.; Barrios, E.; Carrasco, R.; Duenas, J. A.; Gordo-Yanez, D.; Peregrin, A.; Pinto-Gomez, A. R.; Prieto-Thomas, J. A.; Ruiz-Pomares, M. J.] Univ Huelva, Huelva 21071, Spain. [Junquera, T.] ACS, 86 Rue Paris, F-91400 Orsay, France. [Sanchez-Segovia, J.] Hosp Juan Ramon Jimenez, Huelva 21001, Spain. [Ostroumov, P. N.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Villari, A. C. C.] FRIB, E Lansing, MI USA. [Harakeh, M. N.] Univ Groningen, KVI CART, NL-9747 AA Groningen, Netherlands. [Acosta, L. A.] Univ Nacl Autonoma Mexico, Inst Fis, Apartado Postal 20-364, Mexico City 01000, DF, Mexico. RP Martel, I (reprint author), Univ Huelva, Huelva 21071, Spain. RI Acosta, Luis/M-1838-2014; OI Acosta, Luis/0000-0001-9136-1909; Martel, Ismael/0000-0002-4895-2305 FU Spanish Government under the grant Feder-Interconnecta "Aceltec" [ITC-20111070]; Alter Technology-Tuv; Avs; Cibernos; Elitt Energy; Faysol; Idom; Tti Norte FX Work partially supported by the Spanish Government under the grant Feder-Interconnecta "Aceltec" ITC-20111070. The authors are also grateful to the companies Alter Technology-Tuv, Avs, Cibernos, Elitt Energy, Faysol, Idom, and Tti Norte for partial funding of this work and active participation in the design and prototyping carried-out in this study. NR 16 TC 0 Z9 0 U1 2 U2 3 PU JAGIELLONIAN UNIV PRESS PI KRAKOW PA UL MICHALOWSKIEGO 9-2, KRAKOW, 31126, POLAND SN 0587-4254 EI 1509-5770 J9 ACTA PHYS POL B JI Acta Phys. Pol. B PD MAR PY 2016 VL 47 IS 3 BP 607 EP 618 DI 10.5506/APhysPolB.47.607 PG 12 WC Physics, Multidisciplinary SC Physics GA DI4US UT WOS:000373495500002 ER PT J AU Hix, WR Lentz, EJ Bruenn, SW Mezzacappa, A Messer, OEB Endeve, E Blondin, JM Harris, JA Marronetti, P Yakunin, KN AF Hix, W. R. Lentz, E. J. Bruenn, S. W. Mezzacappa, A. Messer, O. E. B. Endeve, E. Blondin, J. M. Harris, J. A. Marronetti, P. Yakunin, K. N. TI THE MULTI-DIMENSIONAL CHARACTER OF CORE-COLLAPSE SUPERNOVAE SO ACTA PHYSICA POLONICA B LA English DT Article ID NEUTRINO-HYDRODYNAMICS SIMULATIONS; ACCRETION-SHOCK INSTABILITY; CIRCLE-DOT STARS; MASSIVE STARS; 3 DIMENSIONS; SASI ACTIVITY; INFALL EPOCH; EXPLOSIONS; NUCLEOSYNTHESIS; CONVECTION AB Core-collapse supernovae, the culmination of massive stellar evolution, are spectacular astronomical events and the principle actors in the story of our elemental origins. Our understanding of these events, while still incomplete, centers around a neutrino-driven central engine that is highly hydrodynamically unstable. Increasingly sophisticated simulations reveal a shock that stalls for hundreds of milliseconds before reviving. Though brought back to life by neutrino heating, the development of the supernova explosion is inextricably linked to multi-dimensional fluid flows. In this paper, the outcomes of three-dimensional simulations that include sophisticated nuclear physics and spectral neutrino transport are juxtaposed to learn about the nature of the three-dimensional fluid flow that shapes the explosion. Comparison is also made between the results of simulations in spherical symmetry from several groups, to give ourselves confidence in the understanding derived from this juxtaposition. C1 [Hix, W. R.; Lentz, E. J.; Messer, O. E. B.; Yakunin, K. N.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Hix, W. R.; Lentz, E. J.; Mezzacappa, A.; Messer, O. E. B.; Endeve, E.; Harris, J. A.; Yakunin, K. N.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Bruenn, S. W.] Florida Atlantic Univ, Dept Phys, Boca Raton, FL 33431 USA. [Mezzacappa, A.; Endeve, E.; Yakunin, K. N.] Oak Ridge Natl Lab, Joint Inst Computat Sci, Oak Ridge, TN 37831 USA. [Messer, O. E. B.] Oak Ridge Natl Lab, Natl Ctr Computat Sci, Oak Ridge, TN 37831 USA. [Endeve, E.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Blondin, J. M.] N Carolina State Univ, Dept Phys, Raleigh, NC 27695 USA. [Harris, J. A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Marronetti, P.] Natl Sci Fdn, Div Phys, Arlington, VA 22207 USA. RP Hix, WR (reprint author), Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. RI Messer, Bronson/G-1848-2012; Lentz, Eric/M-7173-2015; Mezzacappa, Anthony/B-3163-2017; OI Messer, Bronson/0000-0002-5358-5415; Lentz, Eric/0000-0002-5231-0532; Mezzacappa, Anthony/0000-0001-9816-9741; Harris, J. Austin/0000-0003-3023-7140; Hix, William/0000-0002-9481-9126 FU U.S. Department of Energy Office of Nuclear Physics; NASA Astrophysics Theory Program [NNH11AQ72I]; National Science Foundation; National Institute for Computational Sciences [TG-MCA08X010]; U.S. DOE Office of Science [DE-AC02-05CH11231, DE-AC05-00OR22725]; INCITE program at the Oak Ridge Leadership Computing Facility FX We thank M. Liebendorfer and E. O'Connor for making data from [46] and [50] publicly available, and B. Muller for providing the data from [49]. This research was supported by the U.S. Department of Energy Office of Nuclear Physics and the NASA Astrophysics Theory Program (NNH11AQ72I). P.M. is supported by the National Science Foundation through its employee IR/D program. The opinions and conclusions expressed herein are those of the authors and do not represent the National Science Foundation. The simulations here were performed using NSF TeraGrid resources provided by the National Institute for Computational Sciences under grant number TG-MCA08X010; resources of the National Energy Research Scientific Computing Center, supported by the U.S. DOE Office of Science under Contract No. DE-AC02-05CH11231; and an award of computer time from the INCITE program at the Oak Ridge Leadership Computing Facility, supported by the U.S. DOE Office of Science under Contract No. DE-AC05-00OR22725. NR 53 TC 2 Z9 2 U1 0 U2 2 PU JAGIELLONIAN UNIV PRESS PI KRAKOW PA UL MICHALOWSKIEGO 9-2, KRAKOW, 31126, POLAND SN 0587-4254 EI 1509-5770 J9 ACTA PHYS POL B JI Acta Phys. Pol. B PD MAR PY 2016 VL 47 IS 3 BP 645 EP 657 DI 10.5506/APhysPolB.47.645 PG 13 WC Physics, Multidisciplinary SC Physics GA DI4US UT WOS:000373495500006 ER PT J AU Surman, R Mumpower, M Aprahamian, A AF Surman, Rebecca Mumpower, Matthew Aprahamian, Ani TI UNCORRELATED NUCLEAR MASS UNCERTAINTIES AND r-PROCESS ABUNDANCE PREDICTIONS SO ACTA PHYSICA POLONICA B LA English DT Article ID NUCLEOSYNTHESIS AB Nuclear masses have long been recognized as key nuclear physics inputs for calculations of rapid neutron capture, or r-process, nucleosynthesis. Here, we investigate how uncorrelated uncertainties in nuclear masses translate into uncertainties in the final abundance pattern produced in r-process simulations. These uncertainties can obscure details of the abundance pattern that, in principle, could be used to diagnose the r-process astrophysical site. We additionally examine the impact of reductions of mass uncertainties that will come with new experiments. C1 [Surman, Rebecca; Mumpower, Matthew; Aprahamian, Ani] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Mumpower, Matthew] Los Alamos Natl Lab, Div Theoret, POB 1663, Los Alamos, NM 87544 USA. RP Surman, R (reprint author), Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. FU National Science Foundation through the Joint Institute for Nuclear Astrophysics [PHY0822648, PHY1419765]; U.S. Department of Energy [DE-SC0013039]; National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396] FX This work was supported in part by the National Science Foundation through the Joint Institute for Nuclear Astrophysics Grant Nos. PHY0822648 and PHY1419765, and the U.S. Department of Energy under Contract No. DE-SC0013039 (R.S.). A portion of this work was carried out under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396 (M.M.). NR 12 TC 0 Z9 0 U1 2 U2 3 PU JAGIELLONIAN UNIV PRESS PI KRAKOW PA UL MICHALOWSKIEGO 9-2, KRAKOW, 31126, POLAND SN 0587-4254 EI 1509-5770 J9 ACTA PHYS POL B JI Acta Phys. Pol. B PD MAR PY 2016 VL 47 IS 3 BP 673 EP 679 DI 10.5506/APhysPolB.47.673 PG 7 WC Physics, Multidisciplinary SC Physics GA DI4US UT WOS:000373495500008 ER PT J AU Briz, JA Zakari-Issoufou, AA Fallot, M Porta, A Algora, A Tain, JL Valencia, E Rice, S Guadilla, V Agramunt, J Aysto, J Bowry, M Bui, VM Caballero-Folch, R Cano-Ott, D Cormon, S Cucoanes, A Eloma, V Eronen, T Estevez, E Estienne, M Farrelly, GF Fraile, LM Ganioglu, E Garcia, A Gelletly, W Gomez-Hornillos, MB Gorlychev, V Hakala, J Jokinen, A Jordan, MD Kankainen, A Kondev, FG Lebois, M Martinez, T Mendoza, E Molina, F Montaner, A Moore, I Nacher, E Orrigo, S Penttila, H Perez, AB Podolyak, Z Regan, PH Rissanen, J Rubio, B Shiba, T Sonzogni, A Vedia, V Weber, C Wilson, J AF Briz, J. A. Zakari-Issoufou, A-A Fallot, M. Porta, A. Algora, A. Tain, J. L. Valencia, E. Rice, S. Guadilla, V. Agramunt, J. Aysto, J. Bowry, M. Bui, V. M. Caballero-Folch, R. Cano-Ott, D. Cormon, S. Cucoanes, A. Eloma, V. Eronen, T. Estevez, E. Estienne, M. Farrelly, G. F. Fraile, L. M. Ganioglu, E. Garcia, A. Gelletly, W. Gomez-Hornillos, M. B. Gorlychev, V. Hakala, J. Jokinen, A. Jordan, M. D. Kankainen, A. Kondev, F. G. Lebois, M. Martinez, T. Mendoza, E. Molina, F. Montaner, A. Moore, I. Nacher, E. Orrigo, S. Penttila, H. Perez, A. B. Podolyak, Zs. Regan, P. H. Rissanen, J. Rubio, B. Shiba, T. Sonzogni, A. Vedia, V. Weber, C. Wilson, J. CA IGISOL Collaboration TI TOTAL ABSORPTION SPECTROSCOPY OF FISSION FRAGMENTS RELEVANT FOR REACTOR ANTINEUTRINO SPECTRA DETERMINATION SO ACTA PHYSICA POLONICA B LA English DT Article ID PRODUCTS; DECAY; PU-239 AB The contribution of each fission fragment to the reactor antineutrino spectra was determined using the summation method based on the existing information on fission yields and decay data contained in nuclear databases and the reactor evolution code MURE. The beta decay of some of the main contributors has been studied using the Total Absorption Spectroscopy (TAS) technique during two experimental campaigns at the IGISOL facility, in Jyvaskyla (Finland). Results on the decay of Rb-92, the most important contributor in the 4-8 MeV energy region are reported. The status of the analysis of the second experiment is presented as well. C1 [Briz, J. A.; Zakari-Issoufou, A-A; Fallot, M.; Porta, A.; Bui, V. M.; Cormon, S.; Cucoanes, A.; Estienne, M.; Shiba, T.] Univ Nantes, Ecole Mines Nantes, SUBATECH, CNRS,IN2P3, Nantes, France. [Algora, A.; Tain, J. L.; Valencia, E.; Guadilla, V.; Agramunt, J.; Estevez, E.; Jordan, M. D.; Molina, F.; Montaner, A.; Orrigo, S.; Perez, A. B.; Rubio, B.] Univ Valencia, CSIC, IFIC, Valencia, Spain. [Algora, A.] MTA ATOMKI, Debrecen, Hungary. [Rice, S.; Bowry, M.; Farrelly, G. F.; Gelletly, W.; Podolyak, Zs.; Regan, P. H.] Univ Surrey, Guildford GU2 5XH, Surrey, England. [Aysto, J.; Eloma, V.; Eronen, T.; Hakala, J.; Jokinen, A.; Kankainen, A.; Moore, I.; Penttila, H.; Rissanen, J.; Weber, C.; IGISOL Collaboration] Univ Jyvaskyla, IGISOL, Jyvaskyla, Finland. [Caballero-Folch, R.; Gomez-Hornillos, M. B.; Gorlychev, V.] Univ Politecn Cataluna, Barcelona, Spain. [Cano-Ott, D.; Garcia, A.; Martinez, T.; Mendoza, E.] CIEMAT, E-28040 Madrid, Spain. [Fraile, L. M.; Vedia, V.] Univ Complutense Madrid, Madrid, Spain. [Ganioglu, E.] Istanbul Univ, Dept Phys, Istanbul, Turkey. [Kondev, F. G.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Lebois, M.; Wilson, J.] Inst Phys Nucl, BP 1, F-91406 Orsay, France. [Nacher, E.] CSIC, Inst Estruct Mat, Serrano 119, E-28006 Madrid, Spain. [Sonzogni, A.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Sonzogni, A.] Natl Phys Lab, Teddington TW11 0LW, Middx, England. RP Briz, JA (reprint author), Univ Nantes, Ecole Mines Nantes, SUBATECH, CNRS,IN2P3, Nantes, France. RI Mendoza Cembranos, Emilio/K-5789-2014; Molina, Francisco/D-5319-2014; Kankainen, Anu/K-3448-2014; Jokinen, Ari/C-2477-2017; Martinez, Trinitario/K-6785-2014; OI Mendoza Cembranos, Emilio/0000-0002-2843-1801; Molina, Francisco/0000-0002-9459-1336; Kankainen, Anu/0000-0003-1082-7602; Jokinen, Ari/0000-0002-0451-125X; Martinez, Trinitario/0000-0002-0683-5506; Fraile, Luis M/0000-0002-6281-3635; Garcia Rios, Aczel Regino/0000-0002-7955-1475 NR 23 TC 0 Z9 0 U1 9 U2 19 PU JAGIELLONIAN UNIV PRESS PI KRAKOW PA UL MICHALOWSKIEGO 9-2, KRAKOW, 31126, POLAND SN 0587-4254 EI 1509-5770 J9 ACTA PHYS POL B JI Acta Phys. Pol. B PD MAR PY 2016 VL 47 IS 3 BP 755 EP 762 DI 10.5506/APhysPolB.47.755 PG 8 WC Physics, Multidisciplinary SC Physics GA DI4US UT WOS:000373495500018 ER PT J AU Asakura, D Hosono, E Nanba, Y Zhou, HS Okabayashi, J Ban, CM Glans, PA Guo, JH Mizokawa, T Chen, G Achkar, AJ Hawthron, DG Regier, TZ Wadati, H AF Asakura, Daisuke Hosono, Eiji Nanba, Yusuke Zhou, Haoshen Okabayashi, Jun Ban, Chunmei Glans, Per-Anders Guo, Jinghua Mizokawa, Takashi Chen, Gang Achkar, Andrew J. Hawthron, David G. Regier, Thomas Z. Wadati, Hiroki TI Material/element-dependent fluorescence-yield modes on soft X-ray absorption spectroscopy of cathode materials for Li-ion batteries SO AIP ADVANCES LA English DT Article ID DARK CHANNEL FLUORESCENCE; CHARGE-TRANSFER; LIXFEPO4; PEAKS; DIPS AB We evaluate the utilities of fluorescence-yield (FY) modes in soft X-ray absorption spectroscopy (XAS) of several cathode materials for Li-ion batteries. In the case of total-FY (TFY) XAS for LiNi0.5Mn1.5O4, the line shape of the Mn L-3-edge XAS was largely distorted by the self-absorption and saturation effects, while the distortions were less pronounced at the Ni L-3 edge. The distortions were suppressed for the inverse-partial-FY (IPFY) spectra. We found that, in the cathode materials, the IPFY XAS is highly effective for the Cr, Mn, and Fe L edges and the TFY and PFY modes are useful enough for the Ni L edge which is far from the O K edge. (C) 2016 Author(s). C1 [Asakura, Daisuke; Hosono, Eiji; Nanba, Yusuke; Zhou, Haoshen] Natl Inst Adv Ind Sci & Technol, Energy Technol Res Inst, Tsukuba, Ibaraki 3058568, Japan. [Okabayashi, Jun] Univ Tokyo, Res Ctr Spectrochem, Bunkyo Ku, Tokyo 1130033, Japan. [Ban, Chunmei] Natl Renewable Energy Lab, Chem & Mat Sci Ctr, Golden, CO 80401 USA. [Glans, Per-Anders; Guo, Jinghua] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Guo, Jinghua] Univ Calif Santa Cruz, Dept Chem & Biochem, Santa Cruz, CA 95064 USA. [Mizokawa, Takashi] Univ Tokyo, Dept Complex Sci & Engn, Kashiwa, Chiba 2778561, Japan. [Chen, Gang] Jilin Univ, State Key Lab Superhard Mat, Coll Phys, Changchun 130012, Peoples R China. [Achkar, Andrew J.; Hawthron, David G.] Univ Waterloo, Dept Phys & Astron, Waterloo, ON N2L 3G1, Canada. [Regier, Thomas Z.] Univ Saskatchewan, Canadian Light Source, Saskatoon, SK S7N 0X4, Canada. [Wadati, Hiroki] Univ Tokyo, Solar Energy Res Inst, Kashiwa, Chiba 2778581, Japan. [Nanba, Yusuke] Kyushu Univ, Inamori Frontier Res Ctr, Fukuoka 8190395, Japan. [Mizokawa, Takashi] Waseda Univ, Dept Appl Phys, Tokyo 1698555, Japan. RP Asakura, D (reprint author), Natl Inst Adv Ind Sci & Technol, Energy Technol Res Inst, Tsukuba, Ibaraki 3058568, Japan. EM daisuke-asakura@aist.go.jp RI Glans, Per-Anders/G-8674-2016; Hosono, Eiji/M-8402-2013 FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; CFI; NSERC; University of Saskatchewan; Government of Saskatchewan; WD; NRC; CIHR; NREL LDRD Program FX This work was performed under the approvals of the Photon Factory Program Advisory Committee (Proposal Nos. 2012G107, 2013G169 and 2014G100) and the Advanced Light Source (Proposal No. 04907R). The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Research described in this paper was partly performed at the Canadian Light Source, which is supported by CFI, NSERC, the University of Saskatchewan, the Government of Saskatchewan, WD, NRC, and CIHR. The synthesis work at NREL was supported by the NREL LDRD Program. This work was also conducted based on the Japan-U.S. cooperation project for research and standardization of Clean Energy Technologies. NR 33 TC 0 Z9 0 U1 11 U2 22 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 2158-3226 J9 AIP ADV JI AIP Adv. PD MAR PY 2016 VL 6 IS 3 AR 035105 DI 10.1063/1.4943673 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA DI7MG UT WOS:000373684200033 ER PT J AU Appel, AA Larson, JC Jiang, B Zhong, Z Anastasio, MA Brey, EM AF Appel, Alyssa A. Larson, Jeffery C. Jiang, Bin Zhong, Zhong Anastasio, Mark A. Brey, Eric M. TI X-ray Phase Contrast Allows Three Dimensional, Quantitative Imaging of Hydrogel Implants SO ANNALS OF BIOMEDICAL ENGINEERING LA English DT Article DE X-ray phase contrast; Imaging; Hydrogels; Tissue engineering; Micro-computed tomography ID OPTICAL COHERENCE TOMOGRAPHY; TISSUE-ENGINEERED SKIN; IN-VIVO; ARTICULAR-CARTILAGE; SOFT-TISSUE; DIFFRACTION; BIOMATERIALS; RADIOGRAPHY; SCAFFOLDS; COLLAGEN AB Three dimensional imaging techniques are needed for the evaluation and assessment of biomaterials used for tissue engineering and drug delivery applications. Hydrogels are a particularly popular class of materials for medical applications but are difficult to image in tissue using most available imaging modalities. Imaging techniques based on X-ray Phase Contrast (XPC) have shown promise for tissue engineering applications due to their ability to provide image contrast based on multiple X-ray properties. In this manuscript, we investigate the use of XPC for imaging a model hydrogel and soft tissue structure. Porous fibrin loaded poly(ethylene glycol) hydrogels were synthesized and implanted in a rodent subcutaneous model. Samples were explanted and imaged with an analyzer-based XPC technique and processed and stained for histology for comparison. Both hydrogel and soft tissues structures could be identified in XPC images. Structure in skeletal muscle adjacent could be visualized and invading fibrovascular tissue could be quantified. There were no differences between invading tissue measurements from XPC and the gold-standard histology. These results provide evidence of the significant potential of techniques based on XPC for 3D imaging of hydrogel structure and local tissue response. C1 [Appel, Alyssa A.; Larson, Jeffery C.; Jiang, Bin; Brey, Eric M.] IIT, Dept Biomed Engn, 3255 South Dearborn St, Chicago, IL 60616 USA. [Appel, Alyssa A.; Larson, Jeffery C.; Jiang, Bin] Edward Hines Jr VA Hosp, Res Serv, Hines, IL USA. [Zhong, Zhong] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. [Anastasio, Mark A.] Washington Univ, Dept Biomed Engn, St Louis, MO USA. RP Brey, EM (reprint author), IIT, Dept Biomed Engn, 3255 South Dearborn St, Chicago, IL 60616 USA. EM brey@iit.edu OI Jiang, Bin/0000-0003-2390-4312 FU Veterans Administration; National Science Foundation [IIS-1125412, CBET-1263994]; National Institute of Health [R01EB009715] FX The authors would like to thank Banu Akar and Frederick Doe for staining the samples. This work was supported by grants from the Veterans Administration, National Science Foundation (IIS-1125412, CBET-1263994) and the National Institute of Health (R01EB009715). NR 50 TC 1 Z9 1 U1 1 U2 7 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0090-6964 EI 1573-9686 J9 ANN BIOMED ENG JI Ann. Biomed. Eng. PD MAR PY 2016 VL 44 IS 3 BP 773 EP 781 DI 10.1007/s10439-015-1482-5 PG 9 WC Engineering, Biomedical SC Engineering GA DI8HK UT WOS:000373741900012 PM 26487123 ER PT J AU Yang, Y Beekman, C Siemons, W Schleputz, CM Senabulya, N Clarke, R Christen, HM AF Yang, Yongsoo Beekman, Christianne Siemons, Wolter Schlepuetz, Christian M. Senabulya, Nancy Clarke, Roy Christen, Hans M. TI Origin of thickness dependence of structural phase transition temperatures in highly strained BiFeO3 thin films SO APL MATERIALS LA English DT Article ID LANDAU THEORY; FERROELECTRICS; HETEROSTRUCTURES; SURFACE AB Two structural phase transitions are investigated in highly strained BiFeO3 thin films as a function of film thickness and temperature via synchrotron x-ray diffraction. Both transition temperatures (upon heating: monoclinic MC to monoclinic MA to tetragonal) decrease as the film becomes thinner. A film-substrate interface layer, evidenced by half-order peaks, contributes to this behavior, but at larger thicknesses (above a few nanometers), the temperature dependence results from electrostatic considerations akin to size effects in ferroelectric phase transitions, but observed here for structural phase transitions within the ferroelectric phase. For ultra-thin films, the tetragonal structure is stable to low temperatures. (C) 2016 Author(s). C1 [Yang, Yongsoo; Senabulya, Nancy; Clarke, Roy] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Beekman, Christianne; Siemons, Wolter] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Schlepuetz, Christian M.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Christen, Hans M.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Yang, Yongsoo] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Beekman, Christianne] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. [Siemons, Wolter] ASML, De Run 6501, NL-5504 DR Veldhoven, Netherlands. [Schlepuetz, Christian M.] Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland. RP Yang, Y (reprint author), Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. RI Christen, Hans/H-6551-2013; Yang, Yongsoo/P-7716-2014; Schleputz, Christian/C-4696-2008; OI Christen, Hans/0000-0001-8187-7469; Yang, Yongsoo/0000-0001-8654-302X; Schleputz, Christian/0000-0002-0485-2708; Senabulya, Nancy/0000-0002-3394-5452 FU U. S. Department of Energy (DOE), Basic Energy Sciences (BES), Materials Science and Engineering Division; DOE [DE-FG02-06ER46273]; U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX Research at ORNL was supported by the U. S. Department of Energy (DOE), Basic Energy Sciences (BES), Materials Science and Engineering Division (H.M.C., W.S., and C.B.). Research at Michigan was supported by DOE Contract No. DE-FG02-06ER46273 (PI: R.C.). Synchrotron x-ray experiments were performed at Sectors 33-BM-C and 33-ID-D at the APS. Excellent beamline support by Z. Zhang, E. Karapetrova, and the staff of the APS is gratefully acknowledged. The use of the APS was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 43 TC 0 Z9 0 U1 7 U2 22 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 2166-532X J9 APL MATER JI APL Mater. PD MAR PY 2016 VL 4 IS 3 AR 036106 DI 10.1063/1.4944749 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA DI7MO UT WOS:000373685100019 ER PT J AU Zhang, W Sklenar, J Hsu, B Jiang, WJ Jungfleisch, MB Xiao, J Fradin, FY Liu, YH Pearson, JE Ketterson, JB Yang, Z Hoffmann, A AF Zhang, Wei Sklenar, Joseph Hsu, Bo Jiang, Wanjun Jungfleisch, Matthias B. Xiao, Jiao Fradin, Frank Y. Liu, Yaohua Pearson, John E. Ketterson, John B. Yang, Zheng Hoffmann, Axel TI Research Update: Spin transfer torques in permalloy on monolayer MoS2 SO APL MATERIALS LA English DT Article ID TOPOLOGICAL INSULATOR; HETEROSTRUCTURE; MAGNETIZATION; RESONANCE; FIELD AB We observe current induced spin transfer torque resonance in permalloy (Py) grown on monolayer MoS2. By passing rf current through the Py/MoS2 bilayer, field-like and damping-like torques are induced which excite the ferromagnetic resonance of Py. The signals are detected via a homodyne voltage from anisotropic magnetoresistance of Py. In comparison to other bilayer systems with strong spin-orbit torques, the monolayer MoS2 cannot provide bulk spin Hall effects and thus indicates the purely interfacial nature of the spin transfer torques. Therefore our results indicate the potential of two-dimensional transition-metal dichalcogenide for the use of interfacial spin-orbitronics applications. (C) 2016 Author(s). C1 [Zhang, Wei; Sklenar, Joseph; Jiang, Wanjun; Jungfleisch, Matthias B.; Fradin, Frank Y.; Pearson, John E.; Hoffmann, Axel] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Sklenar, Joseph; Ketterson, John B.] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [Hsu, Bo; Xiao, Jiao; Yang, Zheng] Univ Illinois, Dept Elect & Comp Engn, Chicago, IL 60607 USA. [Liu, Yaohua] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP Hoffmann, A (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA.; Yang, Z (reprint author), Univ Illinois, Dept Elect & Comp Engn, Chicago, IL 60607 USA. EM yangzhen@uic.edu; hoffmann@anl.gov RI Liu, Yaohua/B-2529-2009; Jiang, Wanjun/E-6994-2011; Yang, Zheng/A-1028-2011; Jungfleisch, Matthias Benjamin/G-1069-2015 OI Liu, Yaohua/0000-0002-5867-5065; Jiang, Wanjun/0000-0003-0918-3862; Yang, Zheng/0000-0002-4620-4223; Jungfleisch, Matthias Benjamin/0000-0001-8204-3677 FU Department of Electrical and Computer Engineering and College of Engineering at University of Illinois at Chicago; IGNITE Award; Discovery Award for the CVD growth of the MoS2 and optical characterizations; U.S. Department of Energy, Office of Science, Materials Science and Engineering Division; U.S. Department of Energy, Office of Science, and Basic Energy Sciences [DE-AC02-06CH11357]; Division of Scientific User Facilities of the Office of Basic Energy Sciences, U.S. Department of Energy FX Z.Y. acknowledges the financial support from the Department of Electrical and Computer Engineering and College of Engineering at University of Illinois at Chicago, IGNITE Award, and Discovery Award for the CVD growth of the MoS2 and optical characterizations. Work at Argonne, including device fabrication and magnetic and transport measurements, was supported by the U.S. Department of Energy, Office of Science, Materials Science and Engineering Division. Use of the Center for Nanoscale Materials for lithographic patterning was supported by the U.S. Department of Energy, Office of Science, and Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. Work at ORNL is supported by the Division of Scientific User Facilities of the Office of Basic Energy Sciences, U.S. Department of Energy. NR 38 TC 6 Z9 6 U1 10 U2 35 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 2166-532X J9 APL MATER JI APL Mater. PD MAR PY 2016 VL 4 IS 3 AR 032302 DI 10.1063/1.4943076 PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA DI7MO UT WOS:000373685100005 ER PT J AU Tom, N Lawson, M Yu, YH Wright, A AF Tom, Nathan Lawson, Michael Yu, Yi-Hsiang Wright, Alan TI Spectral modeling of an oscillating surge wave energy converter with control surfaces SO APPLIED OCEAN RESEARCH LA English DT Article DE Oscillating surge wave energy converter; Variable structures; Irregular wave; Nonlinear optimization; Viscous linearization; Fatigue damage ID IRREGULAR WAVES; ABSORBER AB The aim of this research is to use spectral techniques in evaluating the irregular wave performance of a novel wave energy converter concept that combines an oscillating surge wave energy converter with control surfaces. The control surfaces allow the wave energy converter to have a time-varying geometry that enables the hydrodynamic exciting and radiation coefficients to be altered. In the current state of development the device geometry is controlled on a sea state-to-sea state time scale and combined with control of the power take-off (PTO) on a wave-to-wave time scale to maximize power capture, increase capacity factor, and reduce design loads. Analysis begins with the application of linear hydrodynamic theory to evaluate the device performance in terms of absorbed power, foundation loads, and accumulation of fatigue damage on the PTO. To determine the linear PTO damping coefficient that maximizes the time-averaged absorbed power for a given sea state, an optimization problem was constructed while incorporating a motion constraint on the maximum pitch amplitude of motion. The inclusion of the motion constraint prevents linear scaling of the performance results with the significant wave height. Previous studies on the modeling of oscillating surge wave energy converter designs have included nonlinear hydrodynamics. Therefore, a quadratic viscous drag moment was added to the system dynamics through use of a quasi-linear viscous damping coefficient. The same performance quantities were calculated for both the linear and nonlinear models while assuming an irregular wave surface elevation described by a Bretscheider spectrum. One major effect of including the viscous drag moment was flattening of the capture width and structural load curves with respect to the wave spectrum peak frequency while reducing the sensitivity with respect to the significant wave height compared to the linear analysis. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Tom, Nathan; Lawson, Michael; Yu, Yi-Hsiang; Wright, Alan] Natl Renewable Energy Lab, MS 3811,15013 Denver West Pkwy, Golden, CO 80401 USA. RP Tom, N (reprint author), Natl Renewable Energy Lab, MS 3811,15013 Denver West Pkwy, Golden, CO 80401 USA. EM nathan.tom@nrel.gov; Michael.Lawson@nrel.gov; Yi-Hsiang.Yu@nrel.gov; Alan.Wright@nrel.gov FU U.S. Department of Energy [DE-AC36-08GO28308]; National Renewable Energy Laboratory; DOE Office of Energy Efficiency and Renewable Energy, Wind and Water Power Technologies Office FX This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08GO28308 with the National Renewable Energy Laboratory. Funding for the work was provided by the DOE Office of Energy Efficiency and Renewable Energy, Wind and Water Power Technologies Office. NR 33 TC 1 Z9 1 U1 2 U2 6 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0141-1187 EI 1879-1549 J9 APPL OCEAN RES JI Appl. Ocean Res. PD MAR PY 2016 VL 56 BP 143 EP 156 DI 10.1016/j.apor.2016.01.006 PG 14 WC Engineering, Ocean; Oceanography SC Engineering; Oceanography GA DI5QD UT WOS:000373552800011 ER PT J AU Scheunert, G Heinonen, O Hardeman, R Lapicki, A Gubbins, M Bowman, RM AF Scheunert, G. Heinonen, O. Hardeman, R. Lapicki, A. Gubbins, M. Bowman, R. M. TI A review of high magnetic moment thin films for microscale and nanotechnology applications SO APPLIED PHYSICS REVIEWS LA English DT Review ID FE-N FILMS; MOLECULAR-BEAM EPITAXY; SINGLE-CRYSTAL FILMS; IRON NITRIDE FILMS; RARE-EARTH-METALS; GENERALIZED GRADIENT APPROXIMATION; GADOLINIUM TUNGSTEN MULTILAYERS; PERPENDICULAR WRITE HEAD; PULSED-LASER DEPOSITION; ATOMIC LAYER DEPOSITION AB The creation of large magnetic fields is a necessary component in many technologies, ranging from magnetic resonance imaging, electric motors and generators, and magnetic hard disk drives in information storage. This is typically done by inserting a ferromagnetic pole piece with a large magnetisation density MS in a solenoid. In addition to large MS, it is usually required or desired that the ferromagnet is magnetically soft and has a Curie temperature well above the operating temperature of the device. A variety of ferromagnetic materials are currently in use, ranging from FeCo alloys in, for example, hard disk drives, to rare earth metals operating at cryogenic temperatures in superconducting solenoids. These latter can exceed the limit on MS for transition metal alloys given by the Slater-Pauling curve. This article reviews different materials and concepts in use or proposed for technological applications that require a large MS, with an emphasis on nanoscale material systems, such as thin and ultra-thin films. Attention is also paid to other requirements or properties, such as the Curie temperature and magnetic softness. In a final summary, we evaluate the actual applicability of the discussed materials for use as pole tips in electromagnets, in particular, in nanoscale magnetic hard disk drive read-write heads; the technological advancement of the latter has been a very strong driving force in the development of the field of nanomagnetism. (C) 2016 AIP Publishing LLC. C1 [Scheunert, G.] Weizmann Inst Sci, Dept Phys Complex Syst, IL-76100 Rehovot, Israel. [Scheunert, G.; Bowman, R. M.] Queens Univ Belfast, Sch Math & Phys, Ctr Nanostruct Media, Belfast BT7 1NN, Antrim, North Ireland. [Heinonen, O.] Argonne Natl Lab, Div Mat Sci, 9700 South Cass Ave, Lemont, IL 60439 USA. [Heinonen, O.] Northwestern Argonne Inst Sci & Technol, Evanston, IL 60208 USA. [Hardeman, R.; Lapicki, A.; Gubbins, M.] Seagate Technol Ireland, Springtown Ind Estate,1 Disc Dr, Derry BT48 0BF, North Ireland. RP Scheunert, G (reprint author), Weizmann Inst Sci, Dept Phys Complex Syst, IL-76100 Rehovot, Israel.; Scheunert, G (reprint author), Queens Univ Belfast, Sch Math & Phys, Ctr Nanostruct Media, Belfast BT7 1NN, Antrim, North Ireland. EM gunther.scheunert@weizmann.ac.il OI Bowman, Robert/0000-0002-4855-2387; Scheunert, Gunther/0000-0002-9406-8094; Heinonen, Olle/0000-0002-3618-6092 FU Seagate Technology (Ireland); Department of Energy, Office of Science, Materials Science and Engineering Division FX The authors would like to thank M. Coey (Trinity College, Dublin) and R. Chantrell (University of York) for helpful discussions and D. Oron (Weizmann Institute of Science) for his ongoing support in publishing this review. Special thanks go to A. Freeman (Northwestern University) for first-principle work on the RE-IE-TM system, which helped identifying GdMnP as a possible high-moment candidate. We would also like to thank Seagate Technology (Ireland) for financial support to establish ANSIN (www.ansin.eu). The work by O. Heinonen was supported by the Department of Energy, Office of Science, Materials Science and Engineering Division. NR 456 TC 9 Z9 9 U1 33 U2 85 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1931-9401 J9 APPL PHYS REV JI Appl. Phys. Rev. PD MAR PY 2016 VL 3 IS 1 AR 011301 DI 10.1063/1.4941311 PG 44 WC Physics, Applied SC Physics GA DI7MY UT WOS:000373686200007 ER PT J AU Cunsolo, A AF Cunsolo, Alessandro TI The Spectrum of Density Fluctuations of Noble Gases Probed by THz Neutron and X-ray Spectroscopy SO APPLIED SCIENCES-BASEL LA English DT Review DE liquid and supercritical systems; inelastic X-ray scattering; relaxation phenomena; inelastic neutron scattering; noble gases ID TIME-CORRELATION-FUNCTIONS; DYNAMIC STRUCTURE FACTOR; HIGH-FREQUENCY DYNAMICS; WAVELENGTH SOUND MODES; BRILLOUIN-SCATTERING; LIQUID ARGON; SUPERCOOLED WATER; STRUCTURAL RELAXATION; INELASTIC-SCATTERING; COLLECTIVE DYNAMICS AB Approximately 50 years of inelastic scattering studies of noble gases are reviewed to illustrate the main advances achieved in the understanding of the THz dynamics of simple systems. The gradual departure of the spectral shape from the hydrodynamic regime is discussed with an emphasis on the phenomenology of fast (sub-ps) relaxation processes. This review shows that relaxation phenomena in noble gases have an essentially collisional origin, which is also revealed by the parallelism between their characteristic timescale and the interatomic collision time. Additionally, recent THz spectroscopy results on noble gases at extreme thermodynamic conditions are discussed to illustrate the need for a revision of our current understanding of the supercritical phase. C1 [Cunsolo, Alessandro] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. RP Cunsolo, A (reprint author), Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. EM acunsolo@bnl.gov FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0012704] FX I wish to thank Tawandra Rowell-Cunsolo for the help in the manuscript preparation. Work performed at the National Synchrotron Light Source II, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-SC0012704. NR 118 TC 1 Z9 1 U1 1 U2 5 PU MDPI AG PI BASEL PA POSTFACH, CH-4005 BASEL, SWITZERLAND SN 2076-3417 J9 APPL SCI-BASEL JI Appl. Sci.-Basel PD MAR PY 2016 VL 6 IS 3 DI 10.3390/app6030064 PG 31 WC Chemistry, Multidisciplinary; Materials Science, Multidisciplinary; Physics, Applied SC Chemistry; Materials Science; Physics GA DI5HY UT WOS:000373530700012 ER PT J AU Bhat, P Brandenburg, A AF Bhat, P. Brandenburg, A. TI Hydraulic effects in a radiative atmosphere with ionization SO ASTRONOMY & ASTROPHYSICS LA English DT Article DE radiative transfer; hydrodynamics; Sun: atmosphere; sunspots ID TURBULENT COMPRESSIBLE CONVECTION; SOLAR PHOTOSPHERE; NUMERICAL SIMULATIONS; MAGNETIC-FIELDS; DEEP ATMOSPHERE; MHD SIMULATIONS; FLUX TUBES; STABILITY; SURFACE AB Context. In his 1978 paper, Eugene Parker postulated the need for hydraulic downward motion to explain magnetic flux concentrations at the solar surface. A similar process has also recently been seen in simplified (e.g., isothermal) models of flux concentrations from the negative effective magnetic pressure instability (NEMPI). Aims. We study the effects of partial ionization near the radiative surface on the formation of these magnetic flux concentrations. Methods. We first obtain one-dimensional (1D) equilibrium solutions using either a Kramers-like opacity or the H-opacity. The resulting atmospheres are then used as initial conditions in two-dimensional (2D) models where flows are driven by an imposed gradient force that resembles a localized negative pressure in the form of a blob. To isolate the effects of partial ionization and radiation, we ignore turbulence and convection. Results. Because of partial ionization, an unstable stratification always forms near the surface. We show that the extrema in the specific entropy profiles correspond to the extrema in the degree of ionization. In the 2D models without partial ionization, strong flux concentrations form just above the height where the blob is placed. Interestingly, in models with partial ionization, such flux concentrations always form at the surface well above the blob. This is due to the corresponding negative gradient in specific entropy. Owing to the absence of turbulence, the downflows reach transonic speeds. Conclusions. We demonstrate that, together with density stratification, the imposed source of negative pressure drives the formation of flux concentrations. We find that the inclusion of partial ionization affects the entropy profile dramatically, causing strong flux concentrations to form closer to the surface. We speculate that turbulence effects are needed to limit the strength of flux concentrations and homogenize the specific entropy to a stratification that is close to marginal. C1 [Bhat, P.; Brandenburg, A.] KTH Royal Inst Technol, NORDITA, Roslagstullsbacken 23, S-10691 Stockholm, Sweden. [Bhat, P.; Brandenburg, A.] Stockholm Univ, Roslagstullsbacken 23, S-10691 Stockholm, Sweden. [Bhat, P.] Inter Univ, Ctr Astron & Astrophys, Post Bag 4,Pune Univ Campus, Pune 411007, Maharashtra, India. [Bhat, P.] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08540 USA. [Bhat, P.] Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08540 USA. [Brandenburg, A.] Stockholm Univ, AlbaNova Univ Ctr, Dept Astron, S-10691 Stockholm, Sweden. [Brandenburg, A.] Univ Colorado, JILA, Boulder, CO 80303 USA. [Brandenburg, A.] Univ Colorado, Dept Astrophys & Planetary Sci, Boulder, CO 80303 USA. [Brandenburg, A.] Univ Colorado, Lab Atmospher & Space Phys, Boulder, CO 80303 USA. RP Bhat, P (reprint author), KTH Royal Inst Technol, NORDITA, Roslagstullsbacken 23, S-10691 Stockholm, Sweden.; Bhat, P (reprint author), Stockholm Univ, Roslagstullsbacken 23, S-10691 Stockholm, Sweden.; Bhat, P (reprint author), Inter Univ, Ctr Astron & Astrophys, Post Bag 4,Pune Univ Campus, Pune 411007, Maharashtra, India.; Bhat, P (reprint author), Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08540 USA.; Bhat, P (reprint author), Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08540 USA. EM palvi@iucaa.ernet.in RI Brandenburg, Axel/I-6668-2013 OI Brandenburg, Axel/0000-0002-7304-021X FU CSIR in India; European Research Council [227952]; Swedish Research Council [621-2011-5076, 2012-5797]; Nordita FX We are grateful to the referee for making a number of useful suggestions. PB thanks Nordita for support and warm hospitality while work on this paper was being carried out. She also acknowledges support from CSIR in India and use of high performance facility at IUCAA, India. This work was supported in part by the European Research Council under the AstroDyn Research Project No. 227952, and by the Swedish Research Council under the project grants 621-2011-5076 and 2012-5797. We acknowledge the allocation of computing resources provided by the Swedish National Allocations Committee at the Center for Parallel Computers at the Royal Institute of Technology in Stockholm and the National Supercomputer Centers in Linkoping, the High Performance Computing Center North in Umea, and the Nordic High Performance Computing Center in Reykjavik. NR 27 TC 0 Z9 0 U1 1 U2 2 PU EDP SCIENCES S A PI LES ULIS CEDEX A PA 17, AVE DU HOGGAR, PA COURTABOEUF, BP 112, F-91944 LES ULIS CEDEX A, FRANCE SN 1432-0746 J9 ASTRON ASTROPHYS JI Astron. Astrophys. PD MAR PY 2016 VL 587 AR A90 DI 10.1051/0004-6361/201425396 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DF8EK UT WOS:000371589800101 ER PT J AU Palanque-Delabrouille, N Magneville, C Yeche, C Paris, I Petitjean, P Burtin, E Dawson, K McGreer, I Myers, AD Rossi, G Schlegel, D Schneider, D Streblyanska, A Tinker, J AF Palanque-Delabrouille, N. Magneville, Ch. Yeche, Ch Paris, I. Petitjean, P. Burtin, E. Dawson, K. McGreer, I. Myers, A. D. Rossi, G. Schlegel, D. Schneider, D. Streblyanska, A. Tinker, J. TI The extended Baryon Oscillation Spectroscopic Survey: Variability selection and quasar luminosity function SO ASTRONOMY & ASTROPHYSICS LA English DT Article DE quasars: general; large-scale structure of Universe; surveys ID DIGITAL-SKY-SURVEY; QSO REDSHIFT SURVEY; 9TH DATA RELEASE; SDSS STRIPE 82; STELLAR OBJECTS; ACOUSTIC-OSCILLATIONS; TARGET SELECTION; 2DF-SDSS LRG; EVOLUTION; CATALOG AB The extended Baryon Oscillation Spectroscopic Survey of the Sloan Digital Sky Survey (SDSS-IV/eBOSS) has an extensive quasar program that combines several selection methods. Among these, the photometric variability technique provides highly uniform samples, which are unaffected by the redshift bias of traditional optical-color selections, when z = 2.7-3.5 quasars cross the stellar locus or when host galaxy light affects quasar colors at z < 0.9. We present the variability selection of quasars in eBOSS, focusing on a specific program that led to a sample of 13876 quasars to g(dered) = 22.5 over a 94.5 deg(2) region in Stripe 82, which has an areal density 1.5 times higher than over the rest of the eBOSS footprint. We use these variability-selected data to provide a new measurement of the quasar luminosity function ((AT) in the redshift range of 0.68 < z < 4.0. Our sample is denser and reaches more deeply than those used in previous studies of the QLF, and it is among the largest ones. At the faint end, our QLF extends to M-g(z = 2) = -21.80 at low redshift and to M-g(z = 2) = -26.20 at z similar to 4. We fit the QLF using two independent double-power-law models with ten free parameters each. The first model is a pure luminosity-function evolution (PLE) with bright-end and faint-end slopes allowed to he different on either side of z = 2.2. The other is a simple PLE at z < 2.2, combined with a model that comprises both luminosity and density evolution (LEDE) at z > 2.2. Both models are constrained to be continuous at z = 2.2. They present a flattening of the bright-end slope at high redshift. The LEDE model indicates a reduction of the break density' with increasing redshift, but the evolution of the break magnitude depends on the parameterization. The models are in excellent accord, predicting quasar counts that agree within 0.3% (resp., 1.1%) to g < 22.5 (resp., g < 23). The models are also in good agreement over the entire redshift range with models from previous studies. C1 [Palanque-Delabrouille, N.; Magneville, Ch.; Yeche, Ch; Burtin, E.] CEA, Ctr Saclay, Irfu SPP, F-91191 Gif Sur Yvette, France. [Paris, I.] INAF Osservatorio Astron Trieste, Via GB Tiepolo 11, I-34131 Trieste, Italy. [Petitjean, P.] UPMC, CNRS, UMR7095, Inst Astrophys Paris, F-75014 Paris, France. [Dawson, K.] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. [McGreer, I.] Univ Arizona, Steward Observ, 933 North Cherry Ave, Tucson, AZ 85721 USA. [Myers, A. D.] Univ Wyoming, Dept Phys & Astron, Laramie, WY 82071 USA. [Rossi, G.] Sejong Univ, Dept Astron & Space Sci, Seoul 143747, South Korea. [Schlegel, D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Schneider, D.] Penn State Univ, Dept Astron & Astrophys, 525 Davey Lab, University Pk, PA 16802 USA. [Schneider, D.] Penn State Univ, Inst Gravitat & Cosmos, University Pk, PA 16802 USA. [Streblyanska, A.] Inst Astrofis Canarias, Tenerife 38200, Spain. [Streblyanska, A.] Univ La Laguna, Dept Astrofis, E-38206 Tenerife, Spain. [Tinker, J.] NYU, 550 1St Ave, New York, NY 10003 USA. RP Palanque-Delabrouille, N (reprint author), CEA, Ctr Saclay, Irfu SPP, F-91191 Gif Sur Yvette, France. EM nathalie.palanque-delabrouille@cea.fr FU Alfred P. Sloan Foundation; U.S. Department of Energy Office of Science; Participating Institutions; Center for High-Performance Computing at the University of Utah FX Funding for the Sloan Digital Sky Survey IV has been provided by the Alfred P. Sloan Foundation, the U.S. Department of Energy Office of Science, and the Participating Institutions. SDSS-IV acknowledges support and resources from the Center for High-Performance Computing at the University of Utah. The SDSS web site is www.sdss.org.SDSS-IV is managed by the Astrophysical Research Consortium for the Participating Institutions of the SDSS Collaboration including the Brazilian Participation Group, the Carnegie Institution for Science, Carnegie Mellon University, the Chilean Participation Group, the French Participation Group, Harvard-Smithsonian Center for Astrophysics, Institute de Astroffsica de Canarias, The Johns Hopkins University, Kavli Institute for the Physics and Mathematics of the Universe (IPMU)/University of Tokyo, Lawrence Berkeley National Laboratory, Leibniz Institut fur Astrophysik Potsdam (AIP), Max-Planck-Institut fur Astronomic (MPIA Heidelberg), Max-Planck-Institut fur Astrophysik (MPA Garching), Max-Planck-institut fur Extraterrestrische Physik (MPE), National Astronomical Observatory of China, New Mexico State University, New York University, University of Notre Dame, Observatario Nacional/MCTI, The Ohio State University, Pennsylvania State University, Shanghai Astronomical Observatory, United Kingdom Participation Group, Universidad Nacional Autonoma de Mexico, University of Arizona, University of Colorado Boulder, University of Portsmouth, University of Utah, University of Virginia, University of Washington, University of Wisconsin, Vanderbilt University, and Yale University. We acknowledge D. Vilanova for his help in the selection of the quasar targets with the variability algorithm. NR 51 TC 5 Z9 5 U1 2 U2 3 PU EDP SCIENCES S A PI LES ULIS CEDEX A PA 17, AVE DU HOGGAR, PA COURTABOEUF, BP 112, F-91944 LES ULIS CEDEX A, FRANCE SN 1432-0746 J9 ASTRON ASTROPHYS JI Astron. Astrophys. PD MAR PY 2016 VL 587 AR A41 DI 10.1051/0004-6361/201527392 PG 14 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DF8EK UT WOS:000371589800052 ER PT J AU Taddia, F Moquist, P Sollerman, J Rubin, A Leloudas, G Gal-Yam, A Arcavi, I Cao, Y Filippenko, AV Graham, ML Mazzali, PA Nugent, PE Pan, YC Silverman, JM Xu, D Yaron, O AF Taddia, F. Moquist, P. Sollerman, J. Rubin, A. Leloudas, G. Gal-Yam, A. Arcavi, I. Cao, Y. Filippenko, A. V. Graham, M. L. Mazzali, P. A. Nugent, P. E. Pan, Y. -C. Silverman, J. M. Xu, D. Yaron, O. TI Metallicity from Type II supernovae from the (i)PTF SO ASTRONOMY & ASTROPHYSICS LA English DT Article DE supernovae: general; Galaxy: abundances ID CORE-COLLAPSE SUPERNOVAE; DIGITAL SKY SURVEY; GALAXIES; SPECTRA; PROGENITOR; ABUNDANCE AB Type IIP supernovae (SNe IIP) have recently been proposed as metallicity (Z) probes. The spectral models of Dessart et al. (2014, MNRAS, 440, 1856) showed that the pseudo-equivalent width of Fe lambda 5018 (pEW(5018)) during the plateau phase depends on the primordial Z, but there was a paucity of SNe IIP exhibiting pEW(5018) that were compatible with Z < 0.4 Z(circle dot). This lack might be due to some physical property of the SN II population or to the fact that those SNe have been discovered in luminous, metal-rich targeted galaxies. Here we use SN II observations from the untargeted (intermediate) Palomar Transient Factory [(i)PTF] survey, aiming to investigate the pEW5018 distribution of this SN population and, in particular, to look for the presence of SNe II at lower Z. We perform pEW(5018) measurements on the spectra of a sample of 39 (i) PTF SNe II, selected to have well-constrained explosion epochs and light-curve properties. Based on the comparison with the pEW(5018) spectral models, we subgrouped our SNe into four Z bins from Z approximate to 0.1 Z(circle dot) up to Z approximate to 2 Z(circle dot). We also independently investigated the Z of the hosts by using their absolute magnitudes and colors and, in a few cases, using strong-line diagnostics from spectra. We searched for possible correlations between SN observables, such as their peak magnitudes and the Z inferred from pEW(5018). We found 11 events with pEW(5018) that were small enough to indicate Z approximate to 0.1 Z(circle dot). The trend of pEW(5018) with Z matches the Z estimates obtained from the host-galaxy photometry, although the significance of the correlation is weak. We also found that SNe with brighter peak magnitudes have smaller pEW(5018) and occur at lower Z. C1 [Taddia, F.; Moquist, P.; Sollerman, J.] Stockholm Univ, AlbaNova, Dept Astron, Oskar Klein Ctr, S-10691 Stockholm, Sweden. [Rubin, A.; Leloudas, G.; Gal-Yam, A.; Yaron, O.] Weizmann Inst Sci, Dept Particle Phys & Astrophys, IL-76100 Rehovot, Israel. [Leloudas, G.] Univ Copenhagen, Niels Bohr Inst, Dark Cosmol Ctr, Juliane Maries Vej 30, DK-2100 Copenhagen, Denmark. [Arcavi, I.] Las Cumbres Observ Global Telescope, 6740 Cortona Dr,Suite 102, Goleta, CA 93117 USA. [Arcavi, I.] Univ Calif Santa Barbara, Kavli Inst Theoret Phys, Santa Barbara, CA 93106 USA. [Cao, Y.] CALTECH, Dept Astron, Pasadena, CA 91125 USA. [Filippenko, A. V.; Graham, M. L.; Nugent, P. E.] Univ Calif Berkeley, Dept Astron, 601 Campbell Hall, Berkeley, CA 94720 USA. [Mazzali, P. A.] Liverpool John Moores Univ, Astrophys Res Inst, 146 Brownlow Hill, Liverpool L3 5RF, Merseyside, England. [Mazzali, P. A.] Max Planck Inst Astrophys, Karl Schwarzschild Str 1, D-85748 Garching, Germany. [Nugent, P. E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Pan, Y. -C.] Univ Illinois, Dept Astron, 1002 W Green St, Urbana, IL 61801 USA. [Silverman, J. M.] Univ Texas Austin, Dept Astron, RLM 15308, Austin, TX 78712 USA. [Xu, D.] Chinese Acad Sci, Natl Astron Observ, Key Lab Space Astron & Technol, 20A Datun Rd, Beijing 100012, Peoples R China. RP Taddia, F (reprint author), Stockholm Univ, AlbaNova, Dept Astron, Oskar Klein Ctr, S-10691 Stockholm, Sweden. EM ftadd@astro.su.se OI Sollerman, Jesper/0000-0003-1546-6615 FU Knut and Alice Wallenberg Foundation; Swedish Research Council; EU/FP7 via ERC grant [307260]; Israeli Committee for Planning and Budgeting; ISF; Minerva grant; ISF grant; Weizmann-UK "making connections" program; Kimmel award; ARCHES award; Christopher R. Redlich Fund; TABASGO Foundation; NSF grant [AST-1211916]; Google; W. M. Keck Foundation; Office of Science of the US Department of Energy [DE-AC02-05CH11231]; NSF Astronomy and Astrophysics Postdoctoral Fellowship [AST-1302771]; National Astronomical Observatories, Chinese Academy of Sciences FX We gratefully acknowledge the support from the Knut and Alice Wallenberg Foundation. The Oskar Klein Centre is funded by the Swedish Research Council. A.G.-Y. is supported by the EU/FP7 via ERC grant No. 307260, the Quantum Universe I-Core program by the Israeli Committee for Planning and Budgeting and the ISF; by Minerva and ISF grants; by the Weizmann-UK "making connections" program; and by Kimmel and ARCHES awards. A.V.F.'s research is supported by the Christopher R. Redlich Fund, the TABASGO Foundation, and NSF grant AST-1211916. We are grateful to the staffs at the many observatories where data for this study were collected (Palomar, Lick, Keck, etc.). We thank R. Foley, J. Bloom, Green, N. Cucchiara, A. Horesh, K. I. Clubb, M. T. Kandrashoff, K. Maguire, A. De Cia, S. Tang, B. Zackay, B. Sesar, A. Waszczak, I. Shivvers, who helped with some of the observations and data reduction. Research at Lick Observatory is partially supported by a generous gift from Google. Some of the data presented herein were obtained at the W. M. Keck Observatory, which is operated as a scientific partnership among the California Institute of Technology, the University of California, and NASA; the observatory was made possible by the generous financial support of the W. M. Keck Foundation. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. J.M.S. is supported by an NSF Astronomy and Astrophysics Postdoctoral Fellowship under award AST-1302771. D.X. acknowledges the support of the One-Hundred-Talent Program from the National Astronomical Observatories, Chinese Academy of Sciences. This work is partly based on the Bachelor thesis by P. Moquist. NR 25 TC 1 Z9 1 U1 1 U2 2 PU EDP SCIENCES S A PI LES ULIS CEDEX A PA 17, AVE DU HOGGAR, PA COURTABOEUF, BP 112, F-91944 LES ULIS CEDEX A, FRANCE SN 1432-0746 J9 ASTRON ASTROPHYS JI Astron. Astrophys. PD MAR PY 2016 VL 587 AR L7 DI 10.1051/0004-6361/201527983 PG 6 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DF8EK UT WOS:000371589800010 ER PT J AU Son, S Chen, L Kang, QJ Derome, D Carmeliet, J AF Son, Soyoun Chen, Li Kang, Qinjun Derome, Dominique Carmeliet, Jan TI Contact Angle Effects on Pore and Corner Arc Menisci in Polygonal Capillary Tubes Studied with the Pseudopotential Multiphase Lattice Boltzmann Model SO COMPUTATION LA English DT Article DE curvature; polygonal tube; wettability; corner arc; saturation; single component multiphase lattice Boltzmann method; capillary rise; menisci ID FLUID VOF METHOD; PARALLEL CYLINDERS; CURVED BOUNDARY; RISE DYNAMICS; LIQUID-GAS; FLOWS; SIMULATIONS; ASSEMBLIES; EQUATIONS; SCALE AB In porous media, pore geometry and wettability are determinant factors for capillary flow in drainage or imbibition. Pores are often considered as cylindrical tubes in analytical or computational studies. Such simplification prevents the capture of phenomena occurring in pore corners. Considering the corners of pores is crucial to realistically study capillary flow and to accurately estimate liquid distribution, degree of saturation and dynamic liquid behavior in pores and in porous media. In this study, capillary flow in polygonal tubes is studied with the Shan-Chen pseudopotential multiphase lattice Boltzmann model (LBM). The LB model is first validated through a contact angle test and a capillary intrusion test. Then capillary rise in square and triangular tubes is simulated and the pore meniscus height is investigated as a function of contact angle theta. Also, the occurrence of fluid in the tube corners, referred to as corner arc menisci, is studied in terms of curvature versus degree of saturation. In polygonal capillary tubes, the number of sides leads to a critical contact angle theta(c) which is known as a key parameter for the existence of the two configurations. LBM succeeds in simulating the formation of a pore meniscus at theta > theta(c) or the occurrence of corner arc menisci at theta < theta(c). The curvature of corner arc menisci is known to decrease with increasing saturation and decreasing contact angle as described by the Mayer and Stoewe-Princen (MS-P) theory. We obtain simulation results that are in good qualitative and quantitative agreement with the analytical solutions in terms of height of pore meniscus versus contact angle and curvature of corner arc menisci versus saturation degree. LBM is a suitable and promising tool for a better understanding of the complicated phenomena of multiphase flow in porous media. C1 [Son, Soyoun; Derome, Dominique; Carmeliet, Jan] EMPA, Swiss Fed Labs Mat Sci & Technol, Lab Multiscale Studies Bldg Phys, CH-8600 Dubendorf, Switzerland. [Son, Soyoun; Carmeliet, Jan] ETH, Chair Bldg Phys, Swiss Fed Inst Technol Zurich, CH-8093 Zurich, Switzerland. [Chen, Li; Kang, Qinjun] Los Alamos Natl Lab, Earth & Environm Sci Div EES 16, Los Alamos, NM 87545 USA. [Chen, Li] Xi An Jiao Tong Univ, Sch Energy & Power Engn, Key Lab Thermofluid Sci & Engn MOE, Xian 710049, Peoples R China. RP Son, S (reprint author), EMPA, Swiss Fed Labs Mat Sci & Technol, Lab Multiscale Studies Bldg Phys, CH-8600 Dubendorf, Switzerland.; Son, S (reprint author), ETH, Chair Bldg Phys, Swiss Fed Inst Technol Zurich, CH-8093 Zurich, Switzerland. EM soyoun.son@empa.ch; lichenmt@lanl.gov; qkang@lanl.gov; dominique.derome@empa.ch; carmeliet@arch.ethz.ch RI Chen, Li/P-4886-2014 OI Chen, Li/0000-0001-7956-3532 NR 46 TC 0 Z9 0 U1 4 U2 6 PU MDPI AG PI BASEL PA POSTFACH, CH-4005 BASEL, SWITZERLAND SN 2079-3197 J9 COMPUTATION JI Computation PD MAR PY 2016 VL 4 IS 1 DI 10.3390/computation4010012 PG 18 WC Mathematics, Interdisciplinary Applications SC Mathematics GA DI6KF UT WOS:000373607000006 ER PT J AU Castillo-Villar, KK Minor-Popocatl, H Webb, E AF Castillo-Villar, Krystel K. Minor-Popocatl, Hertwin Webb, Erin TI Quantifying the Impact of Feedstock Quality on the Design of Bioenergy Supply Chain Networks SO ENERGIES LA English DT Article DE bioenergy; optimization; logging residues; quality costing; biomass; logistics; supply chain network design; bioethanol ID COST-OF-QUALITY; OPTIMIZATION MODEL; BIOMASS; LOGISTICS; FUEL AB Logging residues, which refer to the unused portions of trees cut during logging, are important sources of biomass for the emerging biofuel industry and are critical feedstocks for the first-type biofuel facilities (e.g., corn-ethanol facilities). Logging residues are under-utilized sources of biomass for energetic purposes. To support the scaling-up of the bioenergy industry, it is essential to design cost-effective biofuel supply chains that not only minimize costs, but also consider the biomass quality characteristics. The biomass quality is heavily dependent upon the moisture and the ash contents. Ignoring the biomass quality characteristics and its intrinsic costs may yield substantial economic losses that will only be discovered after operations at a biorefinery have begun. This paper proposes a novel bioenergy supply chain network design model that minimizes operational costs and includes the biomass quality-related costs. The proposed model is unique in the sense that it supports decisions where quality is not unrealistically assumed to be perfect. The effectiveness of the proposed methodology is proven by assessing a case study in the state of Tennessee, USA. The results demonstrate that the ash and moisture contents of logging residues affect the performance of the supply chain (in monetary terms). Higher-than-target moisture and ash contents incur in additional quality-related costs. The quality-related costs in the optimal solution (with final ash content of 1% and final moisture of 50%) account for 27% of overall supply chain cost. Based on the numeral experimentation, the total supply chain cost increased 7%, on average, for each additional percent in the final ash content. C1 [Castillo-Villar, Krystel K.] Univ Texas San Antonio, Dept Mech Engn, One UTSA Circle, San Antonio, TX 78249 USA. [Minor-Popocatl, Hertwin] Polytech Univ Tulancingo, Dept Engn, Calle Ingn 100, Col Huapalcalco 43629, Hidalgo, Mexico. [Webb, Erin] Oak Ridge Natl Lab, Div Environm Sci, One Bethel Valley Rd, Oak Ridge, TN 37831 USA. RP Castillo-Villar, KK (reprint author), Univ Texas San Antonio, Dept Mech Engn, One UTSA Circle, San Antonio, TX 78249 USA. EM Krystel.Castillo@utsa.edu; hertwin.minor@upt.edu.mx; webbeg@ornl.gov OI Webb, Erin/0000-0002-1501-8647 FU U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Bioenergy Technologies Office [4000142556]; U.S. Department of Agriculture/National Institute of Food and Agriculture [2015-38422-24064] FX This material is based upon work supported by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Bioenergy Technologies Office (4000142556) and U.S. Department of Agriculture/National Institute of Food and Agriculture (2015-38422-24064). The support provided by the administration of the Polytechnic University of Tulancingo and the comments from the faculty of Applied Mathematics are appreciated. NR 40 TC 0 Z9 0 U1 3 U2 11 PU MDPI AG PI BASEL PA POSTFACH, CH-4005 BASEL, SWITZERLAND SN 1996-1073 J9 ENERGIES JI Energies PD MAR PY 2016 VL 9 IS 3 DI 10.3390/en9030203 PG 23 WC Energy & Fuels SC Energy & Fuels GA DI6QR UT WOS:000373625500035 ER PT J AU Abbott, BW Jones, JB Schuur, EAG Chapin, FS Bowden, WB Bret-Harte, MS Epstein, HE Flannigan, MD Harms, TK Hollingsworth, TN Mack, MC McGuire, AD Natali, SM Rocha, AV Tank, SE Turetsky, MR Vonk, JE Wickland, KP Aiken, GR Alexander, HD Amon, RMW Benscoter, BW Bergeron, Y Bishop, K Blarquez, O Bond-Lamberty, B Breen, AL Buffam, I Cai, YH Carcaillet, C Carey, SK Chen, JM Chen, HYH Christensen, TR Cooper, LW Cornelissen, JHC de Groot, WJ DeLuca, TH Dorrepaal, E Fetcher, N Finlay, JC Forbes, BC French, NHF Gauthier, S Girardin, MP Goetz, SJ Goldammer, JG Gough, L Grogan, P Guo, LD Higuera, PE Hinzman, L Hu, FS Hugelius, G Jafarov, EE Jandt, R Johnstone, JF Karlsson, J Kasischke, ES Kattner, G Kelly, R Keuper, F Kling, GW Kortelainen, P Kouki, J Kuhry, P Laudon, H Laurion, I Macdonald, RW Mann, PJ Martikainen, PJ McClelland, JW Molau, U Oberbauer, SF Olefeldt, D Pare, D Parisien, MA Payette, S Peng, CH Pokrovsky, OS Rastetter, EB Raymond, PA Raynolds, MK Rein, G Reynolds, JF Robards, M Rogers, BM Schadel, C Schaefer, K Schmidt, IK Shvidenko, A Sky, J Spencer, RGM Starr, G Striegl, RG Teisserenc, R Tranvik, LJ Virtanen, T Welker, JM Zimov, S AF Abbott, Benjamin W. Jones, Jeremy B. Schuur, Edward A. G. Chapin, F. Stuart, III Bowden, William B. Bret-Harte, M. Syndonia Epstein, Howard E. Flannigan, Michael D. Harms, Tamara K. Hollingsworth, Teresa N. Mack, Michelle C. McGuire, A. David Natali, Susan M. Rocha, Adrian V. Tank, Suzanne E. Turetsky, Merritt R. Vonk, Jorien E. Wickland, Kimberly P. Aiken, George R. Alexander, Heather D. Amon, Rainer M. W. Benscoter, Brian W. Bergeron, Yves Bishop, Kevin Blarquez, Olivier Bond-Lamberty, Ben Breen, Amy L. Buffam, Ishi Cai, Yihua Carcaillet, Christopher Carey, Sean K. Chen, Jing M. Chen, Han Y. H. Christensen, Torben R. Cooper, Lee W. Cornelissen, J. Hans C. de Groot, William J. DeLuca, Thomas H. Dorrepaal, Ellen Fetcher, Ned Finlay, Jacques C. Forbes, Bruce C. French, Nancy H. F. Gauthier, Sylvie Girardin, Martin P. Goetz, Scott J. Goldammer, Johann G. Gough, Laura Grogan, Paul Guo, Laodong Higuera, Philip E. Hinzman, Larry Hu, Feng Sheng Hugelius, Gustaf Jafarov, Elchin E. Jandt, Randi Johnstone, Jill F. Karlsson, Jan Kasischke, Eric S. Kattner, Gerhard Kelly, Ryan Keuper, Frida Kling, George W. Kortelainen, Pirkko Kouki, Jari Kuhry, Peter Laudon, Hjalmar Laurion, Isabelle Macdonald, Robie W. Mann, Paul J. Martikainen, Pertti J. McClelland, James W. Molau, Ulf Oberbauer, Steven F. Olefeldt, David Pare, David Parisien, Marc-Andre Payette, Serge Peng, Changhui Pokrovsky, Oleg S. Rastetter, Edward B. Raymond, Peter A. Raynolds, Martha K. Rein, Guillermo Reynolds, James F. Robards, Martin Rogers, Brendan M. Schaedel, Christina Schaefer, Kevin Schmidt, Inger K. Shvidenko, Anatoly Sky, Jasper Spencer, Robert G. M. Starr, Gregory Striegl, Robert G. Teisserenc, Roman Tranvik, Lars J. Virtanen, Tarmo Welker, Jeffrey M. Zimov, Sergei TI Biomass offsets little or none of permafrost carbon release from soils, streams, and wildfire: an expert assessment SO ENVIRONMENTAL RESEARCH LETTERS LA English DT Article DE permafrost carbon; Arctic; boreal; wildfire; dissolved organic carbon; particulate organic carbon; coastal erosion ID CLIMATE-CHANGE; BOREAL FOREST; NITROGEN DEPOSITION; INTERIOR ALASKA; ARCTIC TUNDRA; FIRE; SEQUESTRATION; VULNERABILITY; ECOSYSTEMS; STORAGE AB As the permafrost region warms, its large organic carbon pool will be increasingly vulnerable to decomposition, combustion, and hydrologic export. Models predict that some portion of this release will be offset by increased production of Arctic and boreal biomass; however, the lack of robust estimates of net carbon balance increases the risk of further overshooting international emissions targets. Precise empirical or model-based assessments of the critical factors driving carbon balance are unlikely in the near future, so to address this gap, we present estimates from 98 permafrost-region experts of the response of biomass, wildfire, and hydrologic carbon flux to climate change. Results suggest that contrary to model projections, total permafrost-region biomass could decrease due to water stress and disturbance, factors that are not adequately incorporated in current models. Assessments indicate that end-of-the-century organic carbon release from Arctic rivers and collapsing coastlines could increase by 75% while carbon loss via burning could increase four-fold. Experts identified water balance, shifts in vegetation community, and permafrost degradation as the key sources of uncertainty in predicting future system response. In combination with previous findings, results suggest the permafrost region will become a carbon source to the atmosphere by 2100 regardless of warming scenario but that 65%-85% of permafrost carbon release can still be avoided if human emissions are actively reduced. C1 [Abbott, Benjamin W.] Univ Rennes 1, OSUR, CNRS, UMR ECOBIO 6553, F-35014 Rennes, France. [Abbott, Benjamin W.; Jones, Jeremy B.; Chapin, F. Stuart, III; Bret-Harte, M. Syndonia; Harms, Tamara K.] Univ Alaska Fairbanks, Inst Arctic Biol, Fairbanks, AK USA. [Abbott, Benjamin W.; Jones, Jeremy B.; Chapin, F. Stuart, III; Bret-Harte, M. Syndonia; Harms, Tamara K.] Univ Alaska Fairbanks, Dept Biology& Wildlife, Fairbanks, AK USA. [Schuur, Edward A. G.; Mack, Michelle C.; Schaedel, Christina] No Arizona Univ, Ctr Ecosyst Sci & Soc, Flagstaff, AZ 86011 USA. [Bowden, William B.] Univ Vermont, Rubenstein Sch Environm & Nat Resources, Burlington, VT 05405 USA. [Epstein, Howard E.] Univ Virginia, Dept Environm Sci, Charlottesville, VA 22903 USA. [Flannigan, Michael D.] Univ Alberta, Dept Renewable Resources, Edmonton, AB T6G 2M7, Canada. [Hollingsworth, Teresa N.] Univ Alaska Fairbanks, PNW Res Stn, USDA Forest Serv, Fairbanks, AK USA. [McGuire, A. David] Univ Alaska Fairbanks, Alaska Cooperat Fish & Wildlife Res Unit, US Geol Survey, Anchorage, AK USA. [Natali, Susan M.; Goetz, Scott J.; Rogers, Brendan M.] Woods Hole Res Ctr, Woods Hole, MA USA. [Rocha, Adrian V.] Univ Notre Dame, Dept Biol Sci, Notre Dame, IN 46556 USA. [Rocha, Adrian V.] Univ Notre Dame, Environm Change Initiat, Notre Dame, IN 46556 USA. [Tank, Suzanne E.] Univ Alberta, Dept Biol Sci, Edmonton, AB T6G 2M7, Canada. [Turetsky, Merritt R.] Univ Guelph, Dept Integrat Biol, Guelph, ON N1G 2W1, Canada. [Vonk, Jorien E.] Vrije Univ Amsterdam, Dept Earth Sci, Amsterdam, Netherlands. [Wickland, Kimberly P.; Aiken, George R.; Striegl, Robert G.] US Geol Survey, Natl Res Program, Boulder, CO USA. [Alexander, Heather D.] Mississippi State Univ, Forest & Wildlife Res Ctr, Mississippi State, MS 39762 USA. [Amon, Rainer M. W.] Texas A&M Univ, Galveston, TX USA. [Benscoter, Brian W.] Florida Atlantic Univ, Boca Raton, FL 33431 USA. [Bergeron, Yves] Univ Quebec Abitibi Temiscamingue, Forest Res Inst, Rouyn Noranda, PQ, Canada. [Bishop, Kevin] Uppsala Univ, Dept Earth Sci, Uppsala, Sweden. [Bishop, Kevin] Swedish Univ Agr Sci, Dept Aquat Sci & Assessment, S-90183 Umea, Sweden. [Blarquez, Olivier] Univ Montreal, Dept Geog, Montreal, PQ H3C 3J7, Canada. [Bond-Lamberty, Ben] Pacific NW Natl Lab, Richland, WA 99352 USA. [Breen, Amy L.] Univ Alaska Fairbanks, Int Arctic Res Ctr, Scenarios Network Alaska & Arctic Planning, Fairbanks, AK USA. [Buffam, Ishi] Univ Cincinnati, Cincinnati, OH 45221 USA. [Cai, Yihua] Xiamen Univ, State Key Lab Marine Environm Sci, Xiamen, Peoples R China. [Carcaillet, Christopher] Ecole Prat Hautes Etud, UMR5023, CNRS Lyon 1, Lyon, France. [Carey, Sean K.] McMaster Univ, Hamilton, ON L8S 4L8, Canada. [Chen, Jing M.] Univ Toronto, Toronto, ON M5S 1A1, Canada. [Chen, Han Y. H.] Lakehead Univ, Fac Nat Resources Management, Thunder Bay, ON P7B 5E1, Canada. [Christensen, Torben R.] Lund Univ, Arctic Res Ctr, S-22100 Lund, Sweden. [Christensen, Torben R.] Aarhus Univ, DK-8000 Aarhus C, Denmark. [Cooper, Lee W.] Univ Maryland, Ctr Environm Sci, Bethesda, MD USA. [Cornelissen, J. Hans C.] Vrije Univ Amsterdam, Syst Ecol, Amsterdam, Netherlands. [de Groot, William J.] Nat Resources Canada, Canadian Forest Serv, Toronto, ON, Canada. [DeLuca, Thomas H.] Univ Washington, Sch Environm & Forest Sci, Seattle, WA 98195 USA. [Dorrepaal, Ellen; Karlsson, Jan; Keuper, Frida] Umea Univ, Dept Ecol & Environm Sci, Climate Impacts Res Ctr, S-90187 Umea, Sweden. [Fetcher, Ned] Wilkes Univ, Inst Environm Sci & Sustainabil, Wilkes Barre, PA 18766 USA. [Finlay, Jacques C.] Univ Minnesota, Dept Ecol Evolut & Behav, Minneapolis, MN 55455 USA. [Forbes, Bruce C.] Univ Lapland, Arctic Ctr, Rovaniemi, Finland. [French, Nancy H. F.] Michigan Technol Univ, Michigan Tech Res Inst, Houghton, MI 49931 USA. [Gauthier, Sylvie; Girardin, Martin P.; Pare, David] Nat Resources Canada, Canadian Forest Serv, Laurentian Forestry Ctr, Toronto, ON, Canada. [Goldammer, Johann G.] Max Planck Inst Chem, Global Fire Monitoring Ctr, Berlin, Germany. [Gough, Laura] Towson Univ, Dept Biol Sci, Towson, MD USA. [Grogan, Paul] Queens Univ, Dept Biol, Kingston, ON K7L 3N6, Canada. [Guo, Laodong] Univ Wisconsin Milwaukee, Sch Freshwater Sci, Milwaukee, WI USA. [Higuera, Philip E.] Univ Montana, Dept Ecosyst & Conservat Sci, Missoula, MT 59812 USA. [Hinzman, Larry] Univ Alaska Fairbanks, Fairbanks, AK USA. [Hu, Feng Sheng] Univ Illinois, Dept Plant Biol, Chicago, IL 60680 USA. [Hu, Feng Sheng] Univ Illinois, Dept Geol, Chicago, IL 60680 USA. [Hugelius, Gustaf] Stockholm Univ, Dept Phys Geog, Stockholm, Sweden. [Jafarov, Elchin E.] Univ Colorado Boulder, Inst Arctic & Alpine Res, Boulder, CO USA. [Jandt, Randi] Univ Alaska Fairbanks, Alaska Fire Sci Consortium, Fairbanks, AK USA. [Johnstone, Jill F.] Univ Saskatchewan, Dept Biol, Saskatoon, SK S7N 0W0, Canada. [Kasischke, Eric S.] Univ Maryland, Dept Geog Sci, Bethesda, MD USA. [Kattner, Gerhard] Helmholtz Ctr Polar & Marine Res, Alfred Wegener Inst, Berlin, Germany. [Kelly, Ryan] Neptune & Co Inc, North Wales, PA USA. [Keuper, Frida] INRA, AgroImpact UPR1158, New York, NY USA. [Kling, George W.] Univ Michigan, Ann Arbor, MI 48109 USA. [Kortelainen, Pirkko] Finnish Environm Inst, Helsinki, Finland. [Kouki, Jari] Univ Eastern Finland, Sch Forest Sci, Joensuu, Finland. [Kuhry, Peter] Stockholm Univ, Dept Phys Geog, Stockholm, Sweden. [Laudon, Hjalmar] Swedish Univ Agr Sci, Dept Forest Ecol & Management, S-90183 Umea, Sweden. [Laurion, Isabelle] Inst Natl Rech Sci, Ctr Eau Terre Environm, Toronto, ON, Canada. [Macdonald, Robie W.] Inst Ocean Sci, Dept Fisheries & Oceans, Toronto, ON, Canada. [Mann, Paul J.] Northumbria Univ, Dept Geog, Newcastle Upon Tyne NE1 8ST, Tyne & Wear, England. [Martikainen, Pertti J.] Univ Eastern Finland, Dept Environm & Biol Sci, Joensuu, Finland. [McClelland, James W.] Univ Texas Austin, Inst Marine Sci, Austin, TX 78712 USA. [Molau, Ulf] Univ Gothenburg, Dept Biol & Environm Sci, Gothenburg, Sweden. [Oberbauer, Steven F.] Florida Int Univ, Dept Biol Sci, Miami, FL 33199 USA. [Olefeldt, David] Univ Alberta, Dept Revewable Resources, Edmonton, AB T6G 2M7, Canada. [Parisien, Marc-Andre] Nat Resources Canada, Canadian Forest Serv, No Forestry Ctr, Toronto, ON, Canada. [Payette, Serge] Univ Laval, Ctr Etud Nord, Quebec City, PQ G1K 7P4, Canada. [Peng, Changhui] Univ Quebec, Ctr CEF, ESCER, Montreal, PQ H3C 3P8, Canada. [Peng, Changhui] Northwest A&F Univ, Coll Forestry, State Key Lab Soil Eros & Dryland Farming Loess P, Xian, Peoples R China. [Pokrovsky, Oleg S.] CNRS, Georesources & Environm, Toulouse, France. [Pokrovsky, Oleg S.] Tomsk State Univ, BIO GEO CLIM Lab, Tomsk, Russia. [Rastetter, Edward B.] Marine Biol Lab, Ctr Ecosyst, Woods Hole, MA 02543 USA. [Raymond, Peter A.] Yale Univ, Sch Forestry & Environm Studies, New Haven, CT 06520 USA. [Raynolds, Martha K.] Univ Alaska Fairbanks, Inst Arctic Biol, Fairbanks, AK USA. [Rein, Guillermo] Univ London Imperial Coll Sci Technol & Med, Dept Mech Engn, London SW7 2AZ, England. [Reynolds, James F.] Lanzhou Univ, Sch Life Sci, Lanzhou 730000, Peoples R China. [Reynolds, James F.] Duke Univ, Nicholas Sch Environm, Durham, NC 27706 USA. [Robards, Martin] Arctic Beringia Program, Wildlife Conservat Soc, New York, NY USA. [Schaefer, Kevin] Univ Colorado Boulder, Cooperat Inst Res Environm Sci, Natl Snow & Ice Data Ctr, Boulder, CO USA. [Schmidt, Inger K.] Univ Copenhagen, Dept Geosci & Nat Resource Management, DK-1168 Copenhagen, Denmark. [Shvidenko, Anatoly] Int Inst Appl Syst Anal, A-2361 Laxenburg, Austria. [Shvidenko, Anatoly] Sukachev Inst Forest, Moscow, Russia. [Sky, Jasper] Cambridge Ctr Climate Change Res, Cambridge, England. [Spencer, Robert G. M.] Florida State Univ, Dept Earth Ocean & Atmospher Sci, Tallahassee, FL 32306 USA. [Starr, Gregory] Univ Alabama, Dept Biol Sci, Tuscaloosa, AL 35487 USA. [Teisserenc, Roman] Univ Toulouse, CNRS, INPT, ECOLAB,UPS, Toulouse, France. [Tranvik, Lars J.] Uppsala Univ, Dept Ecol & Genet, Limnol, Uppsala, Sweden. [Virtanen, Tarmo] Univ Helsinki, Dept Environm Sci, FIN-00014 Helsinki, Finland. [Welker, Jeffrey M.] Univ Alaska Anchorage, Anchorage, AK USA. [Zimov, Sergei] Russian Acad Sci, Northeast Sci Stn, Moscow 117901, Russia. RP Abbott, BW (reprint author), Univ Rennes 1, OSUR, CNRS, UMR ECOBIO 6553, F-35014 Rennes, France.; Abbott, BW (reprint author), Univ Alaska Fairbanks, Inst Arctic Biol, Fairbanks, AK USA.; Abbott, BW (reprint author), Univ Alaska Fairbanks, Dept Biology& Wildlife, Fairbanks, AK USA. EM benabbo@gmail.com RI Chen, Han/A-1359-2008; Vonk, Jorien/H-5422-2011; Tank, Suzanne/I-4816-2012; Olefeldt, David/E-8835-2013; Carcaillet, Christopher/G-1218-2011; Cooper, Lee/E-5251-2012; Shvidenko, Anatoly/I-1505-2016; Finlay, Jacques/B-6081-2011; Benscoter, Brian/K-8105-2016; Bond-Lamberty, Ben/C-6058-2008; Raymond, Peter/C-4087-2009; Forbes, Bruce/L-4431-2013; McClelland, James/C-5396-2008; Macdonald, Robie/A-7896-2012; Higuera, Philip/B-1330-2010 OI Johnstone, Jill/0000-0001-6131-9339; Pare, David/0000-0003-0177-6428; Chen, Han/0000-0001-9477-5541; Buffam, Ishi/0000-0002-2625-6640; JAFAROV, ELCHIN/0000-0002-8310-3261; Rastetter, Edward/0000-0002-8620-5431; Rein, Guillermo/0000-0001-7207-2685; Wickland, Kimberly/0000-0002-6400-0590; Abbott, Benjamin/0000-0001-5861-3481; Tank, Suzanne/0000-0002-5371-6577; Olefeldt, David/0000-0002-5976-1475; Carcaillet, Christopher/0000-0002-6632-1507; Cooper, Lee/0000-0001-7734-8388; Shvidenko, Anatoly/0000-0001-7640-2151; Finlay, Jacques/0000-0002-7968-7030; Benscoter, Brian/0000-0002-2706-4667; Bond-Lamberty, Ben/0000-0001-9525-4633; Raymond, Peter/0000-0002-8564-7860; Forbes, Bruce/0000-0002-4593-5083; McClelland, James/0000-0001-9619-8194; Macdonald, Robie/0000-0002-1141-8520; Higuera, Philip/0000-0001-5396-9956 FU National Science Foundation ARCSS program and Vulnerability of Permafrost Carbon Research Coordination Network [OPP-0806465, OPP-0806394, 955713]; SITES (Swedish Science Foundation); Future Forest (Mistra); Marie Curie International Reintegration Grant within the 7th European Community Framework Programme. [277059] FX Peter J Fix provided valuable input on the methods and manuscript. This work was supported by the National Science Foundation ARCSS program and Vulnerability of Permafrost Carbon Research Coordination Network (grants OPP-0806465, OPP-0806394, and 955713) with additional funding from SITES (Swedish Science Foundation), Future Forest (Mistra), and a Marie Curie International Reintegration Grant (TOMCAR-Permafrost #277059) within the 7th European Community Framework Programme. This work complies with the US HHS Policy for Protection of Human Research Subjects. Any use of trade, firm, or product names is for descriptive purposes only and does not imply endorsement by the US Government. NR 86 TC 8 Z9 8 U1 50 U2 104 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-9326 J9 ENVIRON RES LETT JI Environ. Res. Lett. PD MAR PY 2016 VL 11 IS 3 AR 034014 DI 10.1088/1748-9326/11/3/034014 PG 13 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA DI3LY UT WOS:000373401400017 ER PT J AU Paudel, R Mahowald, NM Hess, PGM Meng, L Riley, WJ AF Paudel, Rajendra Mahowald, Natalie M. Hess, Peter G. M. Meng, Lei Riley, William J. TI Attribution of changes in global wetland methane emissions from pre-industrial to present using CLM4.5-BGC SO ENVIRONMENTAL RESEARCH LETTERS LA English DT Article DE wetland; methane emissions; attribution; Community Land Model; climate; environmental factors; simulations ID LAST GLACIAL MAXIMUM; NATURAL WETLANDS; ATMOSPHERIC CO2; CARBON-DIOXIDE; CLIMATE-CHANGE; SYSTEM MODEL; WOOD-HARVEST; VARIABILITY; SENSITIVITY; DEPOSITION AB An understanding of potential factors controlling methane emissions from natural wetlands is important to accurately project future atmospheric methane concentrations. Here, we examine the relative contributions of climatic and environmental factors, such as precipitation, temperature, atmospheric CO2 concentration, nitrogen deposition, wetland inundation extent, and land-use and land-cover change, on changes in wetland methane emissions from pre-industrial to present day (i.e., 1850-2005). We apply a mechanistic methane biogeochemical model integrated in the Community Land Model version 4.5 (CLM4.5), the land component of the Community Earth System Model. The methane model explicitly simulates methane production, oxidation, ebullition, transport through aerenchyma of plants, and aqueous and gaseous diffusion. We conduct a suite of model simulations from 1850 to 2005, with all changes in environmental factors included, and sensitivity studies isolating each factor. Globally, we estimate that preindustrial methane emissions were higher by 10% than present-day emissions from natural wetlands, with emissions changes from preindustrial to the present of +15%, -41%, and -11% for the high latitudes, temperate regions, and tropics, respectively. The most important change is due to the estimated change in wetland extent, due to the conversion of wetland areas to drylands by humans. This effect alone leads to higher preindustrial global methane fluxes by 33% relative to the present, with the largest change in temperate regions (+80%). These increases were partially offset by lower preindustrial emissions due to lower CO2 levels (10%), shifts in precipitation (7%), lower nitrogen deposition (3%), and changes in land-use and land-cover (2%). Cooler temperatures in the preindustrial regions resulted in our simulations in an increase in global methane emissions of 6% relative to present day. Much of the sensitivity to these perturbations is mediated in the model by changes in methane substrate production and the areal extent of wetlands. The detrended interannual variability of high-latitude methane emissions is explained by the variation in substrate production and wetland inundation extent, whereas the tropical emission variability is explained by both of those variables and precipitation. C1 [Paudel, Rajendra; Mahowald, Natalie M.] Cornell Univ, Dept Earth & Atmospher Sci, Ithaca, NY 14850 USA. [Paudel, Rajendra] Everglades Fdn, Palmetto Bay, FL 33157 USA. [Hess, Peter G. M.] Cornell Univ, Dept Biol & Environm Engn, Ithaca, NY 14850 USA. [Meng, Lei] Western Michigan Univ, Dept Geog, Kalamazoo, MI 49008 USA. [Meng, Lei] Western Michigan Univ, Environm & Sustainabil Studies Program, Kalamazoo, MI 49008 USA. [Riley, William J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Paudel, R (reprint author), Cornell Univ, Dept Earth & Atmospher Sci, Ithaca, NY 14850 USA.; Paudel, R (reprint author), Everglades Fdn, Palmetto Bay, FL 33157 USA. EM rpaudel@evergladesfoundation.org RI Riley, William/D-3345-2015 OI Riley, William/0000-0002-4615-2304 FU NSF [1049033]; Office of Science, Office of Biological and Environmental Research of the US Department of Energy, Regional and Global Climate Modeling (RGCM) program [DE-AC02-05CH11231]; [DE-SC0006791] FX The authors wish to acknowledge the assistance of Drs Sean Swenson and David Lawrence from National Center for Atmospheric Research for some code modifications in CLM4.5. We would also like to thank Dr Catherine Prigent for providing multi-satellite observations of wetland inundation fraction. This research was supported by the DE-SC0006791, NSF 1049033, and the Director, Office of Science, Office of Biological and Environmental Research of the US Department of Energy under Contract No. DE-AC02-05CH11231 as part of the Regional and Global Climate Modeling (RGCM) program. Any opinions, findings and conclusions or recommendations expressed in this material are those of the author(s) and do not necessarily reflect the views of the Everglades Foundation. NR 66 TC 0 Z9 0 U1 6 U2 17 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-9326 J9 ENVIRON RES LETT JI Environ. Res. Lett. PD MAR PY 2016 VL 11 IS 3 AR 034020 DI 10.1088/1748-9326/11/3/034020 PG 12 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA DI3LY UT WOS:000373401400023 ER PT J AU Edwards, RA McNair, K Faust, K Raes, J Dutilh, BE AF Edwards, Robert A. McNair, Katelyn Faust, Karoline Raes, Jeroen Dutilh, Bas E. TI Computational approaches to predict bacteriophage-host relationships SO FEMS MICROBIOLOGY REVIEWS LA English DT Review DE phages; viruses of microbes; metagenomics; co-occurrence; CRISPR; oligonucleotide usage ID NATURAL MICROBIAL COMMUNITIES; HUMAN GUT VIROME; SUPERINFECTION EXCLUSION; P22 PROPHAGE; SALMONELLA-TYPHIMURIUM; LEVEL DECONVOLUTION; PALINDROMIC REPEATS; SERINE RECOMBINASES; ACQUIRED-RESISTANCE; VIRAL METAGENOMICS AB Metagenomics has changed the face of virus discovery by enabling the accurate identification of viral genome sequences without requiring isolation of the viruses. As a result, metagenomic virus discovery leaves the first and most fundamental question about any novel virus unanswered: What host does the virus infect? The diversity of the global virosphere and the volumes of data obtained in metagenomic sequencing projects demand computational tools for virus-host prediction. We focus on bacteriophages (phages, viruses that infect bacteria), the most abundant and diverse group of viruses found in environmental metagenomes. By analyzing 820 phages with annotated hosts, we review and assess the predictive power of in silico phage-host signals. Sequence homology approaches are the most effective at identifying known phage-host pairs. Compositional and abundance-based methods contain significant signal for phage-host classification, providing opportunities for analyzing the unknowns in viral metagenomes. Together, these computational approaches further our knowledge of the interactions between phages and their hosts. Importantly, we find that all reviewed signals significantly link phages to their hosts, illustrating how current knowledge and insights about the interaction mechanisms and ecology of coevolving phages and bacteria can be exploited to predict phage-host relationships, with potential relevance for medical and industrial applications.New viruses infecting bacteria are increasingly being discovered in many environments through sequence-based explorations. To understand their role in microbial ecosystems, computational tools are indispensable to prioritize and guide experimental efforts. This review assesses and discusses a range of bioinformatic approaches to predict bacteriophage-host relationships when all that is known is their genome sequence.New viruses infecting bacteria are increasingly being discovered in many environments through sequence-based explorations. To understand their role in microbial ecosystems, computational tools are indispensable to prioritize and guide experimental efforts. This review assesses and discusses a range of bioinformatic approaches to predict bacteriophage-host relationships when all that is known is their genome sequence. C1 [Edwards, Robert A.; McNair, Katelyn] San Diego State Univ, Dept Comp Sci, 5500 Campanile Dr, San Diego, CA 92182 USA. [Edwards, Robert A.; Dutilh, Bas E.] Univ Fed Rio de Janeiro, Inst Biol, Dept Marine Biol, BR-21941902 Rio De Janeiro, Brazil. [Edwards, Robert A.] Argonne Natl Lab, Div Math & Comp Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Faust, Karoline; Raes, Jeroen] Katholieke Univ Leuven, Rega Inst, Dept Microbiol & Immunol, Herestr 49, B-3000 Leuven, Belgium. [Faust, Karoline; Raes, Jeroen] VIB, Ctr Biol Dis, Herestr 49, B-3000 Leuven, Belgium. [Faust, Karoline; Raes, Jeroen] Vrije Univ Brussel, Microbiol Lab, Pleinlaan 2, B-1050 Brussels, Belgium. [Dutilh, Bas E.] Univ Utrecht, Theoret Biol & Bioinformat, Padualaan 8, NL-3584 CH Utrecht, Netherlands. [Dutilh, Bas E.] Radboud Univ Nijmegen, Med Ctr, Ctr Mol & Biomol Informat, Radboud Inst Mol Life Sci, Geert Grooteplein 28, NL-6525 GA Nijmegen, Netherlands. RP Dutilh, BE (reprint author), Univ Utrecht, Theoret Biol & Bioinformat, Padualaan 8, NL-3584 CH Utrecht, Netherlands. EM bedutilh@gmail.com OI Dutilh, Bas E./0000-0003-2329-7890 FU National Science Foundation [CNS-1305112, MCB-1330800]; Netherlands Organization for Scientific Research (NWO) Vidi grant [864.14.004]; CAPES/BRASIL FX This work was supported by the National Science Foundation [CNS-1305112 and MCB-1330800 to RAE]. BED was supported by the Netherlands Organization for Scientific Research (NWO) Vidi grant 864.14.004 and CAPES/BRASIL. NR 120 TC 15 Z9 15 U1 15 U2 39 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0168-6445 EI 1574-6976 J9 FEMS MICROBIOL REV JI Fems Microbiol. Rev. PD MAR PY 2016 VL 40 IS 2 BP 258 EP 272 AR fuv048 DI 10.1093/femsre/fuv048 PG 15 WC Microbiology SC Microbiology GA DI7YP UT WOS:000373718200005 PM 26657537 ER PT J AU Lichtscheidl, AG Pagano, JK Scott, BL Nelson, AT Kiplinger, JL AF Lichtscheidl, Alejandro G. Pagano, Justin K. Scott, Brian L. Nelson, Andrew T. Kiplinger, Jaqueline L. TI Expanding the Chemistry of Actinide Metallocene Bromides. Synthesis, Properties and Molecular Structures of the Tetravalent and Trivalent Uranium Bromide Complexes: (C5Me4R)(2)UBr2, (C5Me4R)(2)U(O-2,6-(Pr2C6H3)-Pr-i)(Br), and [K(THF)][(C5Me4R)(2)UBr2] (R = Me, Et) SO INORGANICS LA English DT Article DE trivalent and tetravalent uranium; bromide; organometallic ID FUNCTIONAL THEORY ANALYSIS; ORGANO-METALLIC COMPOUNDS; NEUTRAL OXYGEN DONOR); CRYSTAL-STRUCTURES; LANTHANIDE(III)/ACTINIDE(III) DIFFERENTIATION; HALIDE-COMPLEXES; ORGANOMETALLIC CHEMISTRY; TRIPHENYLPHOSPHINE OXIDE; SPECTROSCOPIC PROPERTIES; CHEMICAL-REDUCTION AB The organometallic uranium species (C5Me4R)(2)UBr2 (R = Me, Et) were obtained by treating their chloride analogues (C5Me4R)(2)UCl2 (R = Me, Et) with Me3SiBr. Treatment of (C5Me4R)(2)UCl2 and (C5Me4R)(2)UBr2 (R = Me, Et) with K(O-2,6-(Pr2C6H3)-Pr-i) afforded the halide aryloxide mixed-ligand complexes (C5Me4R)(2)U(O-2,6-(Pr2C6H3)-Pr-i)(X) (R = Me, Et; X = Cl, Br). Complexes (C5Me4R)(2)U(O-2,6-(Pr2C6H3)-Pr-i)(Br) (R = Me, Et) can also be synthesized by treating (C5Me4R)(2)U(O-2,6-(Pr2C6H3)-Pr-i)(Cl) (R = Me, Et) withMe3SiBr, respectively. Reduction of (C5Me4R)(2)UCl2 and (C5Me4R)(2)UBr2 (R = Me, Et) with KC8 led to isolation of uranium(III) "ate" species [K(THF)][(C5Me5)(2)UX2] (X = Cl, Br) and [K(THF)(0.5)][(C5Me4Et)(2)UX2] (X = Cl, Br), which can be converted to the neutral complexes (C5Me4R)(2)U[N(SiMe3)(2)] (R = Me, Et). Analyses by nuclear magnetic resonance spectroscopy, X-ray crystallography, and elemental analysis are also presented. C1 [Lichtscheidl, Alejandro G.; Pagano, Justin K.; Kiplinger, Jaqueline L.] Los Alamos Natl Lab, Div Chem, Mail Stop J-514, Los Alamos, NM 87545 USA. [Scott, Brian L.] Los Alamos Natl Lab, Mat Phys & Applicat Div, Mail Stop J-514, Los Alamos, NM 87545 USA. [Nelson, Andrew T.] Los Alamos Natl Lab, Div Mat Sci & Technol, Mail Stop E-549, Los Alamos, NM 87545 USA. RP Kiplinger, JL (reprint author), Los Alamos Natl Lab, Div Chem, Mail Stop J-514, Los Alamos, NM 87545 USA.; Nelson, AT (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, Mail Stop E-549, Los Alamos, NM 87545 USA. EM agl@lanl.gov; pagano@lanl.gov; bscott@lanl.gov; atnelson@lanl.gov; kiplinger@lanl.gov RI Kiplinger, Jaqueline/B-9158-2011 OI Kiplinger, Jaqueline/0000-0003-0512-7062 NR 89 TC 1 Z9 1 U1 5 U2 8 PU MDPI AG PI BASEL PA POSTFACH, CH-4005 BASEL, SWITZERLAND SN 2304-6740 J9 Inorganics JI Inorganics PD MAR PY 2016 VL 4 IS 1 AR 1 DI 10.3390/inorganics4010001 PG 17 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DI2SV UT WOS:000373349900001 ER PT J AU Vannan, S Beaty, TW Cook, RB Wright, DM Devarakonda, R Wei, YX Hook, LA McMurry, BF AF Vannan, Suresh Beaty, Tammy W. Cook, Robert B. Wright, Daine M. Devarakonda, Ranjeet Wei, Yaxing Hook, Les A. McMurry, Benjamin F. TI A Semi-Automated Workflow Solution for Data Set Publication SO ISPRS INTERNATIONAL JOURNAL OF GEO-INFORMATION LA English DT Article DE data ingest; publication workflow; data deluge; terrestrial ecology; automation; aeospatial AB To address the need for published data, considerable effort has gone into formalizing the process of data publication. From funding agencies to publishers, data publication has rapidly become a requirement. Digital Object Identifiers (DOI) and data citations have enhanced the integration and availability of data. The challenge facing data publishers now is to deal with the increased number of publishable data products and most importantly the difficulties of publishing diverse data products into an online archive. The Oak Ridge National Laboratory Distributed Active Archive Center (ORNL DAAC), a NASA-funded data center, faces these challenges as it deals with data products created by individual investigators. This paper summarizes the challenges of curating data and provides a summary of a workflow solution that ORNL DAAC researcher and technical staffs have created to deal with publication of the diverse data products. The workflow solution presented here is generic and can be applied to data from any scientific domain and data located at any data center. C1 [Vannan, Suresh; Beaty, Tammy W.; Cook, Robert B.; Wright, Daine M.; Devarakonda, Ranjeet; Wei, Yaxing; Hook, Les A.; McMurry, Benjamin F.] Oak Ridge Natl Lab, Div Environm Sci, Climate Change Sci Inst, POB 2008, Oak Ridge, TN 37831 USA. RP Vannan, S (reprint author), Oak Ridge Natl Lab, Div Environm Sci, Climate Change Sci Inst, POB 2008, Oak Ridge, TN 37831 USA. EM santhanavans@ornl.gov; beatytw@ornl.gov; cookrb@ornl.gov; wrightdm@ornl.gov; devarakondar@ornl.gov; weiy@ornl.gov; hookla@ornl.gov; mcmurrybf@ornl.gov OI Wright, Daine/0000-0002-8108-0027; Cook, Robert/0000-0001-7393-7302 FU Earth Observing System Data and Information System (EOSDIS) [NNG14HH39I]; U.S. Department of Energy [DE-AC05-00OR22725] FX The authors would like to thank Earth Observing System Data and Information System (EOSDIS) for its support, NASA Interagency Agreement No. NNG14HH39I, and all members of the ORNL DAAC data archive for their contributions to the development of the Semi-Automated Ingest System. Oak Ridge National Laboratory is operated by UT-Battelle, LLC for the U.S. Department of Energy, under contract DE-AC05-00OR22725. NR 12 TC 1 Z9 1 U1 2 U2 2 PU MDPI AG PI BASEL PA POSTFACH, CH-4005 BASEL, SWITZERLAND SN 2220-9964 J9 ISPRS INT J GEO-INF JI ISPRS Int. Geo-Inf. PD MAR PY 2016 VL 5 IS 3 AR 30 DI 10.3390/ijgi5030030 PG 17 WC Geography, Physical; Remote Sensing SC Physical Geography; Remote Sensing GA DI2ZH UT WOS:000373367400009 ER PT J AU He, HS Wang, DL Xu, Y Tan, JD AF He, Hongsheng Wang, Dali Xu, Yang Tan, Jindong TI Data synthesis in the Community Land Model for ecosystem simulation SO JOURNAL OF COMPUTATIONAL SCIENCE LA English DT Article DE Data synthesis; Data analysis; Machine learning; Affinity Propagation; ARIMA model ID TIME-SERIES; DATA ASSIMILATION AB Though many ecosystem states are physically observable, the number of measured variables is limited owning to the constraints of practical environments and onsite sensors. It is therefore beneficial to only measure fundamental variables that determine the behavior of the whole ecosystem, and to simulate other variables with the measured ones. This paper proposes an approach to extract fundamental variables from simulated or observed ecosystem data, and to synthesize the other variables using the fundamental variables. Because the relation of variables in the ecosystem depends on sampling time and frequencies, a region of interest (ROI) is determined using a sliding window on time series with a predefined sampling point and frequency. Within each ROI, system variables are clustered in accordance with a group of selective features by a combination of Affinity Propagation and k-Nearest-Neighbor. In each cluster, the unobserved variables are synthesized from selected fundamental variables using a linear fitting model with ARIMA errors. In the experiment, we studied the performance of variable clustering and data synthesis under a community-land-model based simulation platform. The performance of data synthesis is evaluated by data fitting errors in prediction and forecasting, and the change of system dynamics when synthesized data are in the loop. The experiment proves the high accuracy of the proposed approach in time-series analysis and synthesis for ecosystem simulation. (C) 2016 Elsevier B.V. All rights reserved. C1 [He, Hongsheng] Univ Tennessee, Dept Mech Aerosp & Biomed Engn, Knoxville, TN 37996 USA. [Wang, Dali] Oak Ridge Natl Lab, Div Environm Sci, POB 2008, Oak Ridge, TN 37831 USA. [Xu, Yang] Univ Tennessee, Dept Geog, Knoxville, TN 37996 USA. RP Wang, DL (reprint author), Oak Ridge Natl Lab, Div Environm Sci, POB 2008, Oak Ridge, TN 37831 USA. EM he@utk.edu; wangd@ornl.gov; tan@utk.edu OI Tan, Jindong/0000-0003-0339-8811; Xu, Yang/0000-0003-3898-022X FU NSFC [61305114]; Terrestrial Ecosystem Science (TES) project; Accelerated Climate Modeling for Energy (ACME) project - Biological and Environmental Research (BER), Office of Science, Department of Energy (DOE); Department of Energy [DE-AC05-00OR22725] FX The work was supported in part by NSFC Grant 61305114. The authors also would like to acknowledge the supports from Terrestrial Ecosystem Science (TES) project and Accelerated Climate Modeling for Energy (ACME) project funded by Biological and Environmental Research (BER), Office of Science, Department of Energy (DOE). This research also used computing resources at Oak Ridge National Laboratory (ORNL), which is managed by UT-Battelle LLC for the Department of Energy under contract DE-AC05-00OR22725. NR 23 TC 0 Z9 0 U1 1 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1877-7503 J9 J COMPUT SCI-NETH JI J. Comput. Sci. PD MAR PY 2016 VL 13 BP 83 EP 95 DI 10.1016/j.jocs.2016.01.005 PG 13 WC Computer Science, Interdisciplinary Applications; Computer Science, Theory & Methods SC Computer Science GA DI5LZ UT WOS:000373541900007 ER PT J AU He, F Yin, YF Wang, JH Yang, YN AF He, Fang Yin, Yafeng Wang, Jianhui Yang, Yanni TI Sustainability SI: Optimal Prices of Electricity at Public Charging Stations for Plug-in Electric Vehicles SO NETWORKS & SPATIAL ECONOMICS LA English DT Article DE Plug-in electric vehicle; Price of electricity; Public charging station; Power distribution gird; Real power loss; Travel time ID DISTRIBUTION NETWORKS; POWER-FLOW; COMPLEMENTARITY CONSTRAINTS; MATHEMATICAL PROGRAMS; DISTRIBUTION-SYSTEM; DIRECT SEARCH; MODELS; IMPACT AB With an increasing deployment of plug-in electric vehicles, evaluating and mitigating the impacts of additional electrical loads created by these vehicles on power distribution grids become more important. This paper explores the use of prices of electricity at public charging stations as an instrument, in couple of road pricing, to better manage both power distribution and urban transportation networks. More specifically, a multi-class combined distribution and assignment model is formulated to capture the spatial distribution of plug-in electric vehicles across the transportation network and estimate the electrical loads they impose on the power distribution network. Power flow equations are subsequently solved to estimate real power losses. Prices of electricity at public charging stations and road tolls are then optimized to minimize both real power losses in the distribution grid and total travel time in the urban transportation network. The pricing model is formulated as a mathematical program with complementarity constraints and solved by a manifold suboptimization algorithm and a pattern search method. Numerical examples are presented to demonstrate the proposed model and solution algorithms. C1 [He, Fang; Yin, Yafeng; Yang, Yanni] Univ Florida, Dept Civil & Coastal Engn, Gainesville, FL 32611 USA. [Wang, Jianhui] Argonne Natl Lab, Decis & Informat Sci Div, Argonne, IL 60439 USA. RP Yin, YF (reprint author), Univ Florida, Dept Civil & Coastal Engn, Gainesville, FL 32611 USA. EM yafeng@ce.ufl.edu FU National Science Foundation [CNS-1239364]; National Natural Science Foundation of China [71228101] FX This research was partly funded by National Science Foundation (CNS-1239364) and National Natural Science Foundation of China (71228101). We thank three anonymous reviewers for their helpful comments. NR 46 TC 6 Z9 6 U1 5 U2 14 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 1566-113X EI 1572-9427 J9 NETW SPAT ECON JI Netw Spat. Econ. PD MAR PY 2016 VL 16 IS 1 BP 131 EP 154 DI 10.1007/s11067-013-9212-8 PG 24 WC Operations Research & Management Science; Transportation Science & Technology SC Operations Research & Management Science; Transportation GA DI6RM UT WOS:000373627700007 ER PT J AU Creely, AJ White, AE Edlund, EM Howard, NT Hubbard, AE AF Creely, A. J. White, A. E. Edlund, E. M. Howard, N. T. Hubbard, A. E. TI Perturbative thermal diffusivity from partial sawtooth crashes in Alcator C-Mod SO NUCLEAR FUSION LA English DT Article DE perturbative transport; thermal diffusivity; sawtooth ID HEAT-PULSE-PROPAGATION; ELECTRON-TRANSPORT; FOURIER-ANALYSIS; FUSION PLASMAS; TOKAMAK; TFTR; JET; CONFINEMENT; DISCHARGES; TURBULENCE AB Perturbative thermal diffusivity has been measured on Alcator C-Mod via the use of the extended-time-to-peak method on heat pulses generated by partial sawtooth crashes. Perturbative thermal diffusivity governs the propagation of heat pulses through a plasma. It differs from power balance thermal diffusivity, which governs steady state thermal transport. Heat pulses generated by sawtooth crashes have been used extensively in the past to study heat pulse thermal diffusivity (Lopes Cardozo 1995 Plasma Phys. Control. Fusion 37 799), but the details of the sawtooth event typically lead to non-diffusive 'ballistic' transport, making them an unreliable measure of perturbative diffusivity on many tokamaks (Fredrickson et al 2000 Phys. Plasmas 7 5051). Partial sawteeth are common on numerous tokamaks, and generate a heat pulse without the 'ballistic' transport that often accompanies full sawteeth (Fredrickson et al 2000 Phys. Plasmas 7 5051). This is the first application of the extended-time-to-peak method of diffusivity calculation (Tubbing et al 1987 Nucl. Fusion 27 1843) to partial sawtooth crashes. This analysis was applied to over 50 C-Mod shots containing both L-and I-Mode. Results indicate correlations between perturbative diffusivity and confinement regime (L-versus I-mode), as well as correlations with local temperature, density, the associated gradients, and gradient scale lengths (a/LTe and a/L-n). In addition, diffusivities calculated from partial sawteeth are compared to perturbative diffusivities calculated with the nonlinear gyrokinetic code GYRO. We find that standard ion-scale simulations (ITG/TEM turbulence) under-predict the perturbative thermal diffusivity, but new multi-scale (ITG/TEM coupled with ETG) simulations can match the experimental perturbative diffusivity within error bars for an Alcator C-Mod L-mode plasma. Perturbative diffusivities extracted from heat pulses due to partial sawteeth provide a new constraint that can be used to validate gyrokinetic simulations. C1 [Creely, A. J.; White, A. E.; Hubbard, A. E.] MIT Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA. [Edlund, E. M.] Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. [Howard, N. T.] Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37831 USA. RP Creely, AJ (reprint author), MIT Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA. EM acreely@mit.edu FU US DOE [DE-SC0006419, DEFC02-99ER54512-CMOD] FX This work is supported by the US DOE under grants DE-SC0006419 and DEFC02-99ER54512-CMOD. NR 51 TC 1 Z9 1 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD MAR PY 2016 VL 56 IS 3 AR 036003 DI 10.1088/0029-5515/56/3/036003 PG 12 WC Physics, Fluids & Plasmas SC Physics GA DI3DK UT WOS:000373378200004 ER PT J AU Goumiri, IR Rowley, CW Sabbagh, SA Gates, DA Gerhardt, SP Boyer, MD Andre, R Kolemen, E Taira, K AF Goumiri, I. R. Rowley, C. W. Sabbagh, S. A. Gates, D. A. Gerhardt, S. P. Boyer, M. D. Andre, R. Kolemen, E. Taira, K. TI Modeling and control of plasma rotation for NSTX using neoclassical toroidal viscosity and neutral beam injection SO NUCLEAR FUSION LA English DT Article DE magnetic confinement; feedback control; rotation Control; neutral beam injection; neoclassical toroidal viscosity; NSTX ID FUSION-REACTORS; FACILITY; TURBULENCE; TRANSPORT; TOKAMAK AB A model-based feedback system is presented to control plasma rotation in a magnetically confined toroidal fusion device, to maintain plasma stability for long-pulse operation. This research uses experimental measurements from the National Spherical Torus Experiment (NSTX) and is aimed at controlling plasma rotation using two different types of actuation: momentum from injected neutral beams and neoclassical toroidal viscosity generated by three-dimensional applied magnetic fields. Based on the data-driven model obtained, a feedback controller is designed, and predictive simulations using the TRANSP plasma transport code show that the controller is able to attain desired plasma rotation profiles given practical constraints on the actuators and the available measurements of rotation. C1 [Goumiri, I. R.; Rowley, C. W.] Princeton Univ, Dept Mech & Aerosp Engn, Princeton, NJ 08544 USA. [Sabbagh, S. A.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. [Gates, D. A.; Gerhardt, S. P.; Boyer, M. D.; Andre, R.; Kolemen, E.] Princeton Plasma Phys Lab, Princeton, NJ 08544 USA. [Taira, K.] Florida State Univ, Dept Mech Engn, Tallahassee, FL 32310 USA. RP Goumiri, IR (reprint author), Princeton Univ, Dept Mech & Aerosp Engn, Princeton, NJ 08544 USA. EM igoumiri@princeton.edu FU US Department of Energy [DE-AC02-09CH11466, DE-FG02-99ER54524] FX This work was supported by the US Department of Energy under contract No. DE-AC02-09CH11466 (PPPL) and US Department of Energy grant number DE-FG02-99ER54524 (Columbia University). NR 49 TC 1 Z9 1 U1 4 U2 8 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD MAR PY 2016 VL 56 IS 3 AR 036023 DI 10.1088/0029-5515/56/3/036023 PG 14 WC Physics, Fluids & Plasmas SC Physics GA DI3DK UT WOS:000373378200024 ER PT J AU Logan, NC Park, JK Paz-Soldan, C Lanctot, MJ Smith, SP Burrell, KH AF Logan, N. C. Park, J. -K. Paz-Soldan, C. Lanctot, M. J. Smith, S. P. Burrell, K. H. TI Dependence of neoclassical toroidal viscosity on the poloidal spectrum of applied nonaxisymmetric fields SO NUCLEAR FUSION LA English DT Article DE tokamaks; magnetohydrodynamics; transport properties ID NO MOMENTUM INPUT; DIII-D TOKAMAK; C-MOD PLASMAS; TRANSPORT; ROTATION; CONFINEMENT; DISSIPATION AB This paper presents a single mode model that accurately predicts the coupling of applied nonaxisymmetric fields to the plasma response that induces neoclassical toroidal viscosity (NTV) torque in DIII-D H-mode plasmas. The torque is measured and modeled to have a sinusoidal dependence on the relative phase of multiple nonaxisymmetric field sources, including a minimum in which large amounts of nonaxisymmetric drive is decoupled from the NTV torque. This corresponds to the coupling and decoupling of the applied field to a NTV-driving mode spectrum. Modeling using the perturbed equilibrium nonambipolar transport (PENT) code confirms an effective single mode coupling between the applied field and the resultant torque, despite its inherent nonlinearity. The coupling to the NTV mode is shown to have a similar dependence on the relative phasing as that of the IPEC dominant mode, providing a physical basis for the efficacy of this linear metric in predicting error field correction optima in NTV dominated regimes. C1 [Logan, N. C.; Park, J. -K.] Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. [Paz-Soldan, C.; Lanctot, M. J.; Smith, S. P.; Burrell, K. H.] Gen Atom Co, POB 85608, San Diego, CA 92186 USA. RP Logan, NC (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. EM nlogan@pppl.gov RI Lanctot, Matthew J/O-4979-2016 OI Lanctot, Matthew J/0000-0002-7396-3372 FU U.S. Department of Energy Office of Science Office of Fusion Energy Sciences, a DOE Office of Science user facility [DE-FC02-04ER54698, DE-AC02-09CH11466] FX This work was supported by the U.S. Department of Energy Office of Science Office of Fusion Energy Sciences using the DIII-D National Fusion Facility, a DOE Office of Science user facility, under Awards DE-FC02-04ER54698 and DE-AC02-09CH11466. The authors are grateful for the hard work of the entire DIII-D team, and of the Princeton collaboration headed by R. Nazikian that provided support for this work. NR 52 TC 1 Z9 1 U1 1 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD MAR PY 2016 VL 56 IS 3 AR 036008 DI 10.1088/0029-5515/56/3/036008 PG 11 WC Physics, Fluids & Plasmas SC Physics GA DI3DK UT WOS:000373378200009 ER PT J AU Munro, DH AF Munro, David H. TI Interpreting inertial fusion neutron spectra SO NUCLEAR FUSION LA English DT Article DE neutron spectrum; burn temperature; neutron peak shape AB A burning laser fusion plasma produces a neutron spectrum first described by Brysk (1973 Plasma Phys. Control. Fusion 15 611). This and more recent work deals with the spectrum produced by a single fluid element. The distribution of temperatures and velocities in multiple fluid elements combine in any real spectrum; we derive formulas for how the neutron spectrum averages these contributions. The single element momentum spectrum is accurately Gaussian, but the multi-element spectrum exhibits higher moments. In particular, the skew and kurtosis are likely to be large enough to measure. Even the single fluid element spectrum may exhibit measurable directional anisotropy, so that instruments with different lines of sight should see different yields, mean velocities, mean temperatures, and higher moments. Finally, we briefly discuss how scattering in the imploded core modifies the neutron spectrum by changing the relative weighting of fuel regions with different temperatures and velocities. C1 [Munro, David H.] Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94551 USA. RP Munro, DH (reprint author), Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94551 USA. EM munro1@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 17 TC 4 Z9 4 U1 6 U2 14 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD MAR PY 2016 VL 56 IS 3 AR 036001 DI 10.1088/0029-5515/56/3/036001 PG 15 WC Physics, Fluids & Plasmas SC Physics GA DI3DK UT WOS:000373378200002 ER PT J AU Orlov, DM Moyer, RA Evans, TE Paz-Soldan, C Ferraro, NM Nazikian, R deGrassie, JS Grierson, BA Eldon, D Fenstermacher, ME King, JD Logan, NC Lanctot, MJ Maingi, R Snyder, PB Strait, EJ Wingen, A AF Orlov, D. M. Moyer, R. A. Evans, T. E. Paz-Soldan, C. Ferraro, N. M. Nazikian, R. deGrassie, J. S. Grierson, B. A. Eldon, D. Fenstermacher, M. E. King, J. D. Logan, N. C. Lanctot, M. J. Maingi, R. Snyder, P. B. Strait, E. J. Wingen, A. TI Suppression of type-I ELMs with reduced RMP coil set on DIII-D SO NUCLEAR FUSION LA English DT Article DE macroinstabilities; magnetic confinement; tokamaks; kinetic modes; plasma simulation ID EDGE; MODES AB Recent experiments on DIII-D have demonstrated that having a toroidally-monochromatic spectral content of edge-resonant magnetic perturbations (RMPs) is not a necessary condition for suppression of edge localized modes (ELMs). Robust ELM suppression has been reproducibly obtained on DIII-D during experiments in which various non-axisymmetric coil loops were turned off pseudo-randomly producing a variety of n = 1, n = 2, and n = 3 spectral contributions. It was shown that RMP ELM suppression could be achieved with as few as 5 out of 12 internal coil loops (I-coils) on DIII-D at similar coil currents and with good plasma confinement. Linear MHD plasma response (M3DCI, IPEC, mars) and vacuum (SURFMN, TRIP3D) modelling have been performed in order to understand the effects of the perturbation spectrum on the plasma response and ELM suppression. The results suggest that reduction of the dominant n = 3 perturbation field is compensated by increased n = 2 field in the plasma that may lead to RMP ELM suppression at lower levels of n = 3 perturbative magnetic flux from the I-coils. These results provide additional confidence that ITER may be capable of RMP ELM suppression in the event of multiple internal coil failures. C1 [Orlov, D. M.; Moyer, R. A.; Eldon, D.] Univ Calif San Diego, Energy Res Ctr, La Jolla, CA 92093 USA. [Evans, T. E.; Paz-Soldan, C.; Ferraro, N. M.; deGrassie, J. S.; King, J. D.; Lanctot, M. J.; Snyder, P. B.; Strait, E. J.] Gen Atom Co, POB 85608, San Diego, CA 92186 USA. [Nazikian, R.; Grierson, B. A.; Logan, N. C.; Maingi, R.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Fenstermacher, M. E.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Wingen, A.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Orlov, DM (reprint author), Univ Calif San Diego, Energy Res Ctr, La Jolla, CA 92093 USA. EM orlov@fusion.gat.com RI Orlov, Dmitriy/D-2406-2016; Lanctot, Matthew J/O-4979-2016 OI Orlov, Dmitriy/0000-0002-2230-457X; Lanctot, Matthew J/0000-0002-7396-3372 FU US Department of Energy, Office of Science, Office of Fusion Energy Sciences [DE-FG02-05ER54809, DE-FC02-04ER54698, DE-AC01-09CH11466, DE-AC52-07NA27344] FX The authors would like to thank A. Loarte (ITER Organization) and C.M. Greenfield (US BPO, US ITER Project Office) for their support of the experiments, and D. Campbell (ITER Organization) for nominating this work for an invited talk at the APS DPP meeting. The authors also acknowledge beneficial discussions with J.D. Callen (University of Wisconsin, Madison) and F. Waelbroeck (University of Texas, Austin) while preparing this manuscript. This material is based upon work supported by the US Department of Energy, Office of Science, Office of Fusion Energy Sciences under Award Number DE-FG02-05ER54809, under contract numbers DE-FC02-04ER54698, DE-AC01-09CH11466, and DE-AC52-07NA27344, using the DIII-D National Fusion Facility, a DOE Office of Science user facility. DIII-D data shown in this paper can be obtained in digital format by following the links at https://fusion.gat.com/global/D3D_DMP. NR 31 TC 1 Z9 1 U1 5 U2 16 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD MAR PY 2016 VL 56 IS 3 AR 036020 DI 10.1088/0029-5515/56/3/036020 PG 17 WC Physics, Fluids & Plasmas SC Physics GA DI3DK UT WOS:000373378200021 ER PT J AU Rice, JE Gao, C Mumgaard, R Parker, RR Scott, SD Shiraiwa, S Wallace, GM Bonoli, PT Delgado-Aparicio, L Fenzi, C Granetz, RS Greenwald, MJ Hubbard, AE Hughes, JW Irby, JH Lee, JP Marmar, ES Reinke, ML Wolfe, SM AF Rice, J. E. Gao, C. Mumgaard, R. Parker, R. R. Scott, S. D. Shiraiwa, S. Wallace, G. M. Bonoli, P. T. Delgado-Aparicio, L. Fenzi, C. Granetz, R. S. Greenwald, M. J. Hubbard, A. E. Hughes, J. W. Irby, J. H. Lee, J. P. Marmar, E. S. Reinke, M. L. Wolfe, S. M. TI Effects of the q profile on toroidal rotation in Alcator C-Mod LHCD plasmas SO NUCLEAR FUSION LA English DT Article DE rotation; q profile; lower hybrid current drive; tokamak ID JET; CYCLOTRON AB Changes in the core toroidal rotation profiles following injection of lower hybrid (LH) waves have been documented in Alcator C-Mod plasmas. Shot by shot scans of LH input power have been performed at fixed magnetic field and electron density for several plasma currents. For sawtoothing target plasmas, if the input power is low enough that the central safety factor q(0) remains below 1, the change in the core rotation is in the counter-current direction, consistent in sign, magnitude and LH power scaling with direct momentum input from the LH waves. If the power level is high enough that there are significant changes to the q profile, including the termination of sawtooth oscillations, the change in the toroidal rotation is in the co-current direction, consistent with changes in the momentum flux through its dependence on the current density profile. The direction of the rotation changes depends on whether q(0) is below or above unity, and seemingly not on the magnetic shear, nor the Ohmic confinement regime of the target plasma. C1 [Rice, J. E.; Gao, C.; Mumgaard, R.; Parker, R. R.; Shiraiwa, S.; Wallace, G. M.; Bonoli, P. T.; Granetz, R. S.; Greenwald, M. J.; Hubbard, A. E.; Hughes, J. W.; Irby, J. H.; Lee, J. P.; Marmar, E. S.; Wolfe, S. M.] MIT, PSFC, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Scott, S. D.; Delgado-Aparicio, L.] PPPL, Princeton, NJ 08543 USA. [Fenzi, C.] CEA, IRFM, F-13108 St Paul Les Durance, France. [Reinke, M. L.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Rice, JE (reprint author), MIT, PSFC, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM rice@psfc.mit.edu FU DoE [DE-FC02-99ER54512] FX The authors thank the Alcator C-Mod operations and LH groups for expert running of the tokamak. Work supported at MIT by DoE Contract No. DE-FC02-99ER54512. NR 36 TC 1 Z9 1 U1 5 U2 19 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD MAR PY 2016 VL 56 IS 3 AR 036015 DI 10.1088/0029-5515/56/3/036015 PG 7 WC Physics, Fluids & Plasmas SC Physics GA DI3DK UT WOS:000373378200016 ER PT J AU Wilcox, RS Talmadge, JN Anderson, DT Anderson, FSB Lore, JD AF Wilcox, R. S. Talmadge, J. N. Anderson, D. T. Anderson, F. S. B. Lore, J. D. TI Intrinsic plasma rotation and Reynolds stress at the plasma edge in the HSX stellarator SO NUCLEAR FUSION LA English DT Article DE quasi-symmetric stellarators; plasma rotation; Reynolds stress; Langmuir probes ID NONAXISYMMETRIC TOROIDAL PLASMAS; RADIAL ELECTRIC-FIELD; TRANSPORT-COEFFICIENTS; NEOCLASSICAL TRANSPORT; CONFINEMENT SYSTEMS; PFIRSCH-SCHLUTER; PLATEAU REGIME; FLOW; GENERATION; TOKAMAKS AB Using multi-tipped Langmuir probes in the edge of the HSX stellarator, the radial electric field and parallel flows are found to deviate from the values calculated by the neoclassical transport code PENTA for the optimized quasi-helically symmetric (QHS) configuration. To understand whether Reynolds stress might explain the discrepancy, fluctuating floating potential measurements are made at two locations in the torus corresponding to the low field and high field sides of the device. The measurements at the two locations show clear evidence of a gradient in the Reynolds stress. However, the resulting flow due to the gradient in the stress is found to be large and in opposite directions for the two locations. This makes an estimation of the flux surface average using a small number of measurement locations impractical from an experimental perspective. These results neither confirm nor rule out whether Reynolds stress plays an important role for the QHS configuration. Measurements made in configurations with the quasi-symmetry degraded show even larger flows and greater deviations from the neoclassically calculated velocity profiles than the QHS configuration while the fluctuation magnitudes are reduced. Therefore, for these configurations in particular, the Reynolds stress is most likely not responsible for the additional momentum. C1 [Wilcox, R. S.; Lore, J. D.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Wilcox, R. S.; Talmadge, J. N.; Anderson, D. T.; Anderson, F. S. B.] Univ Wisconsin, Dept Elect & Comp Engn, 1415 Johnson Dr, Madison, WI 53706 USA. [Wilcox, R. S.] Gen Atom Co, San Diego, CA USA. RP Wilcox, RS (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.; Wilcox, RS (reprint author), Univ Wisconsin, Dept Elect & Comp Engn, 1415 Johnson Dr, Madison, WI 53706 USA.; Wilcox, RS (reprint author), Gen Atom Co, San Diego, CA USA. EM wilcoxr@fusion.gat.com OI Wilcox, Robert/0000-0003-1369-1739 FU US DOE Grant [DE-FG02-93ER54222] FX The authors would like to thank L Stephey, C Deng, K Likin, S Kumar and M Frankowski for their assistance over the course of this work. This work is supported by US DOE Grant DE-FG02-93ER54222. Data relevant to all figures and tables is available for access from the HSX website at www.hsx.wisc.edu/HSX_Publication_Data.shtml. NR 46 TC 1 Z9 1 U1 2 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD MAR PY 2016 VL 56 IS 3 AR 036002 DI 10.1088/0029-5515/56/3/036002 PG 14 WC Physics, Fluids & Plasmas SC Physics GA DI3DK UT WOS:000373378200003 ER PT J AU Roland, BP Zeccola, AM Larsen, SB Amrich, CG Talsma, AD Stuchul, KA Heroux, A Levitan, ES VanDemark, AP Palladino, MJ AF Roland, Bartholomew P. Zeccola, Alison M. Larsen, Samantha B. Amrich, Christopher G. Talsma, Aaron D. Stuchul, Kimberly A. Heroux, Annie Levitan, Edwin S. VanDemark, Andrew P. Palladino, Michael J. TI Structural and Genetic Studies Demonstrate Neurologic Dysfunction in Triosephosphate Isomerase Deficiency Is Associated with Impaired Synaptic Vesicle Dynamics SO PLOS GENETICS LA English DT Article ID TRIOSE-PHOSPHATE ISOMERASE; SENSITIVE PARALYTIC MUTANTS; DROSOPHILA NEUROMUSCULAR-JUNCTION; HEREDITARY HEMOLYTIC-ANEMIA; CRYSTAL-STRUCTURE; NEURODEGENERATIVE DISEASES; MITOCHONDRIAL DYSFUNCTION; POINT-MUTATION; TPI DEFICIENCY; ACTIVE-SITE AB Triosephosphate isomerase (TPI) deficiency is a poorly understood disease characterized by hemolytic anemia, cardiomyopathy, neurologic dysfunction, and early death. TPI deficiency is one of a group of diseases known as glycolytic enzymopathies, but is unique for its severe patient neuropathology and early mortality. The disease is caused by missense mutations and dysfunction in the glycolytic enzyme, TPI. Previous studies have detailed structural and catalytic changes elicited by disease-associated TPI substitutions, and samples of patient erythrocytes have yielded insight into patient hemolytic anemia; however, the neuropathophysiology of this disease remains a mystery. This study combines structural, biochemical, and genetic approaches to demonstrate that perturbations of the TPI dimer interface are sufficient to elicit TPI deficiency neuropathogenesis. The present study demonstrates that neurologic dysfunction resulting from TPI deficiency is characterized by synaptic vesicle dysfunction, and can be attenuated with catalytically inactive TPI. Collectively, our findings are the first to identify, to our knowledge, a functional synaptic defect in TPI deficiency derived from molecular changes in the TPI dimer interface. C1 [Roland, Bartholomew P.; Zeccola, Alison M.; Larsen, Samantha B.; Talsma, Aaron D.; Stuchul, Kimberly A.; Levitan, Edwin S.; Palladino, Michael J.] Univ Pittsburgh, Sch Med, Dept Pharmacol & Chem Biol, Pittsburgh, PA USA. [Roland, Bartholomew P.; Zeccola, Alison M.; Larsen, Samantha B.; Talsma, Aaron D.; Stuchul, Kimberly A.; Palladino, Michael J.] Univ Pittsburgh, Sch Med, Pittsburgh Inst Neurodegenerat Dis, Pittsburgh, PA USA. [Amrich, Christopher G.; VanDemark, Andrew P.] Univ Pittsburgh, Dept Biol Sci, Pittsburgh, PA 15260 USA. [Heroux, Annie] Brookhaven Natl Lab, Energy Sci Directorate, Photon Sci Div, Upton, NY 11973 USA. [Roland, Bartholomew P.] Vanderbilt Univ, Dept Biol Sci, 221 Kirkland Hall, Nashville, TN 37235 USA. RP Palladino, MJ (reprint author), Univ Pittsburgh, Sch Med, Dept Pharmacol & Chem Biol, Pittsburgh, PA USA.; Palladino, MJ (reprint author), Univ Pittsburgh, Sch Med, Pittsburgh Inst Neurodegenerat Dis, Pittsburgh, PA USA. EM mjp44@pitt.edu OI Roland, Bartholomew/0000-0002-9033-9942 FU Achievement Rewards for College Scientists: Pittsburgh Chapter; DOE/BER [FWP BO-70]; National Institutes of Health [R01 GM103369, R01 GM108073, R01 GM097204, R01 NS32385, 8P41GM103473-16, T32 GM8424-17]; U.S. Department of Energy Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work was supported by a fellowship from Achievement Rewards for College Scientists: Pittsburgh Chapter [BPR]; DOE/BER grant FWP BO-70 (AH); and the National Institutes of Health [grant numbers R01 GM103369 & R01 GM108073 (MJP), R01 GM097204 (APV), R01 NS32385 (ESL), 8P41GM103473-16 (AH), and T32 GM8424-17 (BPR)]. Data was collected at beamline X25 of the National Synchrotron Light Source (NSLS), which was supported under Contract No. DE-AC02-98CH10886 of U.S. Department of Energy Office of Basic Energy Sciences. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 97 TC 0 Z9 0 U1 12 U2 13 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1553-7404 J9 PLOS GENET JI PLoS Genet. PD MAR PY 2016 VL 12 IS 3 AR e1005941 DI 10.1371/journal.pgen.1005941 PG 30 WC Genetics & Heredity SC Genetics & Heredity GA DI1PV UT WOS:000373268900046 PM 27031109 ER PT J AU Erskine, DJ Eggert, JH Celliers, PM Hicks, DG AF Erskine, David J. Eggert, J. H. Celliers, P. M. Hicks, D. G. TI Ghost fringe removal techniques using Lissajous data presentation SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID INTERFEROMETER AB A VISAR (Velocity Interferometer System for Any Reflector) is a Doppler velocity interferometer which is an important optical diagnostic in shockwave experiments at the national laboratories, used to measure equation of state (EOS) of materials under extreme conditions. Unwanted reflection of laser light from target windows can produce an additional component to the VISAR fringe record that can distort and obscure the true velocity signal. Accurately removing this so-called ghost artifact component is essential for achieving high accuracy EOS measurements, especially when the true light signal is only weakly reflected from the shock front. Independent of the choice of algorithm for processing the raw data into a complex fringe signal, we have found it beneficial to plot this signal as a Lissajous and seek the proper center of this path, even under time varying intensity which can shift the perceived center. The ghost contribution is then solved by a simple translation in the complex plane that recenters the Lissajous path. For continuous velocity histories, we find that plotting the fringe magnitude vs nonfringing intensity and optimizing linearity is an invaluable tool for determining accurate ghost offsets. For discontinuous velocity histories, we have developed graphically inspired methods which relate the results of two VISARs having different velocity per fringe proportionalities or assumptions of constant fringe magnitude to find the ghost offset. The technique can also remove window reflection artifacts in generic interferometers, such as in the metrology of surfaces. (C) 2016 AIP Publishing LLC. C1 [Erskine, David J.; Eggert, J. H.; Celliers, P. M.] Lawrence Livermore Natl Lab, L-487, Livermore, CA 94551 USA. [Hicks, D. G.] Swinburne Univ Technol, Ctr Microphoton, Hawthorn, Vic 3122, Australia. RP Erskine, DJ (reprint author), Lawrence Livermore Natl Lab, L-487, Livermore, CA 94551 USA. EM erskine1@llnl.gov OI Hicks, Damien/0000-0001-8322-9983 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. Thanks to Amy Lazicki for data taking at the Omega laser facility. NR 9 TC 0 Z9 0 U1 5 U2 11 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0034-6748 EI 1089-7623 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD MAR PY 2016 VL 87 IS 3 AR 033106 DI 10.1063/1.4943563 PG 9 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA DI7WS UT WOS:000373713300007 PM 27036757 ER PT J AU Higley, DJ Hirsch, K Dakovski, GL Jal, E Yuan, E Liu, TM Lutman, AA MacArthur, JP Arenholz, E Chen, Z Coslovich, G Denes, P Granitzka, PW Hart, P Hoffmann, MC Joseph, J Le Guyader, L Mitra, A Moeller, S Ohldag, H Seaberg, M Shafer, P Stohr, J Tsukamoto, A Nuhn, HD Reid, AH Durr, HA Schlotter, WF AF Higley, Daniel J. Hirsch, Konstantin Dakovski, Georgi L. Jal, Emmanuelle Yuan, Edwin Liu, Tianmin Lutman, Alberto A. MacArthur, James P. Arenholz, Elke Chen, Zhao Coslovich, Giacomo Denes, Peter Granitzka, Patrick W. Hart, Philip Hoffmann, Matthias C. Joseph, John Le Guyader, Loic Mitra, Ankush Moeller, Stefan Ohldag, Hendrik Seaberg, Matthew Shafer, Padraic Stoehr, Joachim Tsukamoto, Arata Nuhn, Heinz-Dieter Reid, Alex H. Duerr, Hermann A. Schlotter, William F. TI Femtosecond X-ray magnetic circular dichroism absorption spectroscopy at an X-ray free electron laser SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID ANGULAR-MOMENTUM TRANSFER; LIGHT-SOURCE; TRANSITION; REVERSAL AB X-ray magnetic circular dichroism spectroscopy using an X-ray free electron laser is demonstrated with spectra over the Fe L-3,L-2-edges. The high brightness of the X-ray free electron laser combined with high accuracy detection of incident and transmitted X-rays enables ultrafast X-ray magnetic circular dichroism studies of unprecedented sensitivity. This new capability is applied to a study of all-optical magnetic switching dynamics of Fe and Gd magnetic sublattices in a GdFeCo thin film above its magnetization compensation temperature. (c) 2016 AIP Publishing LLC. C1 [Higley, Daniel J.; Hirsch, Konstantin; Dakovski, Georgi L.; Jal, Emmanuelle; Yuan, Edwin; Liu, Tianmin; Lutman, Alberto A.; MacArthur, James P.; Chen, Zhao; Coslovich, Giacomo; Granitzka, Patrick W.; Hart, Philip; Hoffmann, Matthias C.; Le Guyader, Loic; Mitra, Ankush; Moeller, Stefan; Ohldag, Hendrik; Seaberg, Matthew; Stoehr, Joachim; Nuhn, Heinz-Dieter; Reid, Alex H.; Duerr, Hermann A.; Schlotter, William F.] SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Higley, Daniel J.; Yuan, Edwin] Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA. [Liu, Tianmin; MacArthur, James P.; Chen, Zhao] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Arenholz, Elke; Denes, Peter; Joseph, John; Shafer, Padraic] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Granitzka, Patrick W.] Univ Amsterdam, Van der Waals Zeeman Inst, Kruislaan 403, NL-1018 XE Amsterdam, Netherlands. [Le Guyader, Loic] Radboud Univ Nijmegen, IMM, Heyendaalseweg 135, NL-6525 AJ Nijmegen, Netherlands. [Le Guyader, Loic] European XFEL GmbH, Albert Einstein Ring 19, D-22761 Hamburg, Germany. [Tsukamoto, Arata] Nihon Univ, Dept Elect & Comp Sci, 7-24-1 Narashino Dai Funabashi, Chiba 2748501, Japan. RP Higley, DJ (reprint author), SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.; Higley, DJ (reprint author), Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA. EM dhigley@stanford.edu RI Hoffmann, Matthias/B-3893-2009; Durr, Hermann/F-6205-2012; OI Hirsch, Konstantin/0000-0001-5050-3026; Hoffmann, Matthias/0000-0002-3596-9853; Jal, Emmanuelle/0000-0001-5297-9124 FU Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division [DE-AC02-76SF00515]; European Research Council [339813 EXCHANGE]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Feodor-Lynen program; Volkswagen-Stiftung FX We would like to thank J. Aldrich, S. Carron, C. Ford, G. McCracken, and C. P. O'Grady for technical assistance. This work is supported by the Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division, under Contract No. DE-AC02-76SF00515, and the European Research Council (Grant No. 339813 EXCHANGE). Use of the linac coherent light source, SLAC National Accelerator Laboratory, is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Use of the Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515. K. H. thanks the AvH foundation for financial support through the Feodor-Lynen program. L. L. G. thanks the Volkswagen-Stiftung for financial support through the Peter-Paul-Ewald Fellowship. NR 34 TC 3 Z9 3 U1 10 U2 28 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0034-6748 EI 1089-7623 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD MAR PY 2016 VL 87 IS 3 AR 033110 DI 10.1063/1.4944410 PG 5 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA DI7WS UT WOS:000373713300011 PM 27036761 ER PT J AU Kim, D Rho, HS Jambovane, S Shin, S Hong, JW AF Kim, Duckjong Rho, Hoon Suk Jambovane, Sachin Shin, Soojeong Hong, Jong Wook TI Evaluation of peristaltic micromixers for highly integrated microfluidic systems SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID CHIP; MICROPUMPS; VALVES; PUMP AB Microfluidic devices based on the multilayer soft lithography allow accurate manipulation of liquids, handling reagents at the sub-nanoliter level, and performing multiple reactions in parallel processors by adapting micromixers. Here, we have experimentally evaluated and compared several designs of micromixers and operating conditions to find design guidelines for the micromixers. We tested circular, triangular, and rectangular mixing loops and measured mixing performance according to the position and the width of the valves that drive nanoliters of fluids in the micrometer scale mixing loop. We found that the rectangular mixer is best for the applications of highly integrated microfluidic platforms in terms of the mixing performance and the space utilization. This study provides an improved understanding of the flow behaviors inside micromixers and design guidelines for micromixers that are critical to build higher order fluidic systems for the complicated parallel bio/ chemical processes on a chip. (C) 2016 AIP Publishing LLC. C1 [Kim, Duckjong; Rho, Hoon Suk; Jambovane, Sachin; Hong, Jong Wook] Auburn Univ, Dept Mech Engn, Mat Res & Educ Ctr, Auburn, AL 36849 USA. [Kim, Duckjong] Korea Inst Machinery & Mat, Dept Nano Mech, Daejeon 34103, South Korea. [Rho, Hoon Suk] Univ Twente, MESA Inst Nanotechnol, Mesoscale Chem Syst Grp, POB 217, NL-7500 AE Enschede, Netherlands. [Jambovane, Sachin] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Shin, Soojeong; Hong, Jong Wook] Hanyang Univ, Dept Bionano Engn, Ansan 15588, South Korea. [Hong, Jong Wook] Hanyang Univ, Grad Sch, Dept Bionano Technol, Seoul 04763, South Korea. RP Hong, JW (reprint author), Auburn Univ, Dept Mech Engn, Mat Res & Educ Ctr, Auburn, AL 36849 USA.; Hong, JW (reprint author), Hanyang Univ, Dept Bionano Engn, Ansan 15588, South Korea.; Hong, JW (reprint author), Hanyang Univ, Grad Sch, Dept Bionano Technol, Seoul 04763, South Korea. EM jwh@hanyang.ac.kr RI Jambovane, Sachin/G-2865-2016 OI Jambovane, Sachin/0000-0002-5063-6969 FU US Department of Agriculture through the National Institute of Food and Agriculture [2009-35603-05051]; US National Institutes of Health (NIH) [R01 008392]; US National Science Foundation (NSF CBET) [1063536]; Global Frontier Project Grant [2014M3A6A4062860]; Small Grant Exploratory Research and Engineering Research Center of the National Research Foundation - Ministry of Science, ICT and Future Planning of Korea [2008-0061891, 2014R1A1A2A16055291] FX This research was supported by the US Department of Agriculture through the National Institute of Food and Agriculture (No. 2009-35603-05051), the US National Institutes of Health (NIH Grant No. R01 008392), and the US National Science Foundation (NSF CBET Grant No. 1063536). Also, partial supports were provided by the Global Frontier Project Grant (No. 2014M3A6A4062860), Small Grant Exploratory Research (No. 2014R1A1A2A16055291), and Engineering Research Center (No. 2008-0061891) of the National Research Foundation funded by the Ministry of Science, ICT and Future Planning of Korea. NR 24 TC 0 Z9 0 U1 3 U2 7 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0034-6748 EI 1089-7623 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD MAR PY 2016 VL 87 IS 3 AR 035003 DI 10.1063/1.4940927 PG 8 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA DI7WS UT WOS:000373713300059 PM 27036809 ER PT J AU Wang, GM Shaftan, T Cheng, WX Guo, W Ilinsky, P Li, Y Podobedov, B Willeke, F AF Wang, G. M. Shaftan, T. Cheng, W. X. Guo, W. Ilinsky, P. Li, Y. Podobedov, B. Willeke, F. TI Emittance and lifetime measurement with damping wigglers SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article AB National Synchrotron Light Source II (NSLS-II) is a new third-generation storage ring light source at Brookhaven National Laboratory. The storage ring design calls for small horizontal emittance (< 1 nm-rad) and diffraction-limited vertical emittance at 12 keV (8 pm-rad). Achieving low value of the beam size will enable novel user experiments with nm-range spatial and meV-energy resolution. The high-brightness NSLS-II lattice has been realized by implementing 30-cell double bend achromatic cells producing the horizontal emittance of 2 nm rad and then halving it further by using several Damping Wigglers (DWs). This paper is focused on characterization of the DW effects in the storage ring performance, namely, on reduction of the beam emittance, and corresponding changes in the energy spread and beam lifetime. The relevant beam parameters have been measured by the X-ray pinhole camera, beam position monitors, beam filling pattern monitor, and current transformers. In this paper, we compare the measured results of the beam performance with analytic estimates for the complement of the 3 DWs installed at the NSLS-II. (C) 2016 AIP Publishing LLC. C1 [Wang, G. M.; Shaftan, T.; Cheng, W. X.; Guo, W.; Ilinsky, P.; Li, Y.; Podobedov, B.; Willeke, F.] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11793 USA. RP Shaftan, T (reprint author), Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11793 USA. EM shaftan@bnl.gov FU DOE [DE-SC00112704] FX This work was supported by DOE, Contract No. DE-SC00112704. NR 15 TC 0 Z9 0 U1 1 U2 2 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0034-6748 EI 1089-7623 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD MAR PY 2016 VL 87 IS 3 AR 033301 DI 10.1063/1.4942903 PG 5 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA DI7WS UT WOS:000373713300016 PM 27036766 ER PT J AU Wang, T Parnell, SR Hamilton, WA Li, F Washington, AL Baxter, DV Pynn, R AF Wang, T. Parnell, S. R. Hamilton, W. A. Li, F. Washington, A. L. Baxter, D. V. Pynn, R. TI Compact spherical neutron polarimeter using high-T-c YBCO films SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID POLARIZATION ANALYSIS; SPIN-ECHO; INELASTIC-SCATTERING; FLIPPER; PERFORMANCE; CHROMIUM; DESIGN; FILTER AB We describe a simple, compact device for spherical neutron polarimetry measurements at small neutron scattering angles. The device consists of a sample chamber with very low (<0.01 G) magnetic field flanked by regions within which the neutron polarization can be manipulated in a controlled manner. This allows any selected initial and final polarization direction of the neutrons to be obtained. We have constructed a prototype device using high-Tc superconducting films and mu-metal to isolate regions with different magnetic fields and tested device performance in transmission geometry. Finite-element methods were used to simulate the device's field profile and these have been verified by experiment using a small solenoid as a test sample. Measurements are reported using both monochromatic and polychromatic neutron sources. The results show that the device is capable of extracting sample information and distinguishing small angular variations of the sample magnetic field. As a more realistic test, we present results on the characterization of a 10 mu m thick Permalloy film in zero magnetic field, as well as its response to an external magnetic field. (C) 2016 AIP Publishing LLC. C1 [Wang, T.; Parnell, S. R.; Li, F.; Baxter, D. V.; Pynn, R.] Indiana Univ, Ctr Explorat Energy & Matter, Bloomington, IN 47408 USA. [Parnell, S. R.] Delft Univ Technol, Fac Appl Sci, Mekelweg 15, NL-2629 JB Delft, Netherlands. [Hamilton, W. A.; Pynn, R.] Oak Ridge Natl Lab, Neutron Sci Directorate, Oak Ridge, TN 37381 USA. [Washington, A. L.] Univ Sheffield, Dept Phys & Astron, Sheffield S10 2TN, S Yorkshire, England. RP Wang, T (reprint author), Indiana Univ, Ctr Explorat Energy & Matter, Bloomington, IN 47408 USA. RI Baxter, David /D-3769-2013; OI Baxter, David /0000-0003-2812-0904; Washington, Adam/0000-0002-3243-1556; Pynn, Roger/0000-0002-0867-7505 FU National Science Foundation [DMR-0956741, DMR-0220560, DMR-0320627]; 21st Century Science and Technology fund of Indiana, Indiana University; Department of Defence; Office of the Vice Provost for Research at Indiana University; U.S. Department of Energy [DE-AC05-00OR22725] FX The design and construction of the device were supported by the National Science Foundation through Grant No. DMR-0956741. Construction of LENS was supported by the National Science Foundation Grant Nos. DMR-0220560 and DMR-0320627, the 21st Century Science and Technology fund of Indiana, Indiana University, and the Department of Defence. Operations of LENS are supported by the Office of the Vice Provost for Research at Indiana University. Measurement time on the HB-2D beamline at the HFIR at Oak Ridge National Laboratory (ORNL) is managed by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. NR 38 TC 1 Z9 1 U1 1 U2 9 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0034-6748 EI 1089-7623 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD MAR PY 2016 VL 87 IS 3 AR 033901 DI 10.1063/1.4943254 PG 11 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA DI7WS UT WOS:000373713300035 PM 27036785 ER PT J AU Nunez, JK Harrington, LB Doudna, JA AF Nunez, James K. Harrington, Lucas B. Doudna, Jennifer A. TI Chemical and Biophysical Modulation of Cas9 for Tunable Genome Engineering SO ACS CHEMICAL BIOLOGY LA English DT Review ID SEQUENCE-SPECIFIC CONTROL; PLURIPOTENT STEM-CELLS; OPTICAL CONTROL; EDITING SPECIFICITY; MEDIATED DELIVERY; CRYSTAL-STRUCTURE; MAMMALIAN-CELLS; GENE-EXPRESSION; GUIDE RNAS; IN-VIVO AB The application of the CRISPR Cas9 system for genome engineering has revolutionized the ability to interrogate genomes of mammalian cells. Programming the Cas9 endonuclease to induce DNA breaks at specified sites is achieved by simply modifying the sequence of its cognate guide RNA. Although Cas9-mediated genome editing has been shown to be highly specific, cleavage events at off-target sites have also been reported. Minimizing, and eventually abolishing, unwanted off-target cleavage remains a major goal of the CRISPR Cas9 technology before its implementation for therapeutic use. Recent efforts have turned to chemical biology and biophysical approaches to engineer inducible genome editing systems for controlling Cas9 activity at the transcriptional and protein levels. Here, we review recent advancements to modulate Cas9-mediated genome editing by engineering split-Cas9 constructs, inteins, small molecules, protein-based dimerizing domains, and light-inducible systems. C1 [Nunez, James K.; Harrington, Lucas B.; Doudna, Jennifer A.] Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Howard Hughes Med Inst, Innovat Genom Inst, Dept Chem,Ctr RNA Syst Biol, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Doudna, JA (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA.; Doudna, JA (reprint author), Univ Calif Berkeley, Howard Hughes Med Inst, Innovat Genom Inst, Dept Chem,Ctr RNA Syst Biol, Berkeley, CA 94720 USA.; Doudna, JA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. EM doudna@berkeley.edu FU National Science Foundation [1244557]; U.S. National Science Foundation Graduate Research Fellowships; UC Berkeley Chancellor's Graduate Fellowship FX We acknowledge support from National Science Foundation grant No. 1244557 to J.A.D. J.K.N. and L.B.H. are supported by U.S. National Science Foundation Graduate Research Fellowships and J.K.N. by a UC Berkeley Chancellor's Graduate Fellowship. J.A.D. is an Investigator of the Howard Hughes Medical Institute. NR 62 TC 9 Z9 9 U1 12 U2 22 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1554-8929 EI 1554-8937 J9 ACS CHEM BIOL JI ACS Chem. Biol. PD MAR PY 2016 VL 11 IS 3 BP 681 EP 688 DI 10.1021/acschembio.5b01019 PG 8 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DH3CJ UT WOS:000372664800014 PM 26857072 ER PT J AU McCreary, A Ghosh, R Amani, M Wang, J Duerloo, KAN Sharma, A Jarvis, K Reed, EJ Dongare, AM Banerjee, SK Terrones, M Namburu, RR Dubey, M AF McCreary, Amber Ghosh, Rudresh Amani, Matin Wang, Jin Duerloo, Karel-Alexander N. Sharma, Ankit Jarvis, Karalee Reed, Evan J. Dongare, Avinash M. Banerjee, Sanjay K. Terrones, Mauricio Namburu, Raju R. Dubey, Madan TI Effects of Uniaxial and Biaxial Strain on Few-Layered Terrace Structures of MoS2 Grown by Vapor Transport SO ACS NANO LA English DT Article DE molybdenum disulfide; strain engineering; Raman; photoluminescence; interlayer sliding; CVD; few-layer ID TRANSITION-METAL DICHALCOGENIDES; MONOLAYER MOLYBDENUM-DISULFIDE; FIELD-EFFECT TRANSISTORS; AUGMENTED-WAVE METHOD; RAMAN-SPECTROSCOPY; ATOMIC LAYERS; ELECTRONIC-PROPERTIES; MULTILAYER MOS2; ULTRATHIN MOS2; BILAYER MOS2 AB One of the most fascinating properties of molybdenum disulfide (MoS2) is its ability to be subjected to large amounts of strain without experiencing degradation. The potential of MoS2 mono- and few-layers in electronics, opto electronics, and flexible devices requires the fundamental understanding of their properties as a function of strain. While previous reports have studied mechanically exfoliated flakes, tensile strain experiments on chemical vapor deposition (CVD)-grown few-layered MoS2 have not been examined hitherto, although CVD is a state of the art synthesis technique with clear potential for scale-up processes. In this report, we used CVD-grown terrace MoS2 layers to study how the number and size of the layers affected the physical properties under uniaxial and biaxial tensile strain. Interestingly, we observed significant shifts in both the Raman in-plane mode (as high as -5.2 cm(-1)) and photoluminescence (PL) energy (as high as -88 meV) for the few-layered MoS2 under similar to 1.5% applied uniaxial tensile strain when compared to monolayers and few-layers of MoS2 studied previously. We also observed slippage between the layers which resulted in a hysteresis of the Raman and PL spectra during further applications of strain. Through DFT calculations, we contended that this random layer slippage was due to defects present in CVD-grown materials. This work demonstrates that CVD-grown few-layered MoS2 is a realistic, exciting material for tuning its properties under tensile strain. C1 [McCreary, Amber; Amani, Matin; Dubey, Madan] US Army, Res Lab, Sensors & Elect Devices Directorate, Adelphi, MD 20783 USA. [McCreary, Amber; Namburu, Raju R.] US Army, Res Lab, Computat & Informat Sci Directorate, Aberdeen Proving Ground, MD 21005 USA. [McCreary, Amber; Terrones, Mauricio] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [McCreary, Amber; Terrones, Mauricio] Penn State Univ, Ctr Dimens & Layered Mat 2, University Pk, PA 16802 USA. [Terrones, Mauricio] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Terrones, Mauricio] Penn State Univ, Dept Chem, University Pk, PA 16802 USA. [Ghosh, Rudresh; Sharma, Ankit] Univ Texas Austin, Microelect Res Ctr, Austin, TX 78758 USA. [Jarvis, Karalee] Univ Texas Austin, Texas Mat Inst, Austin, TX 78758 USA. [Wang, Jin; Dongare, Avinash M.] Univ Connecticut, Dept Mat Sci & Engn, Storrs, CT 06269 USA. [Wang, Jin; Dongare, Avinash M.] Univ Connecticut, Inst Mat Sci, Storrs, CT 06269 USA. [Duerloo, Karel-Alexander N.; Reed, Evan J.] Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA. [Amani, Matin] Univ Calif Berkeley, Elect Engn & Comp Sci, Berkeley, CA 94720 USA. [Amani, Matin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Dubey, M (reprint author), US Army, Res Lab, Sensors & Elect Devices Directorate, Adelphi, MD 20783 USA.; Terrones, M (reprint author), Penn State Univ, Dept Phys, University Pk, PA 16802 USA.; Terrones, M (reprint author), Penn State Univ, Ctr Dimens & Layered Mat 2, University Pk, PA 16802 USA.; Terrones, M (reprint author), Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA.; Terrones, M (reprint author), Penn State Univ, Dept Chem, University Pk, PA 16802 USA. EM mut11@psu.edu; madan.dubey.civ@mail.mil FU Army Research Laboratory [W911NF-14-2-0059]; U.S. Army Research Laboratory (ARL) Director's Strategic Initiative (DSI) program on interfaces in stacked 2D atomic layered materials; U.S. Army Research Office MURI [W911NF-11-1-0362]; Army Research Office under STTR [W911NF-14-P-0030] FX This research was sponsored by the Army Research Laboratory. A.M., MA, RN., and M.D. acknowledge the support of the U.S. Army Research Laboratory (ARL) Director's Strategic Initiative (DSI) program on interfaces in stacked 2D atomic layered materials. A.M. and M.T. acknowledge the support of the U.S. Army Research Office MURI (Grant No. W911NF-11-1-0362). R.G. and S.KB. thank the Army Research Office for partial support of this work under STTR Award No. W911NF-14-P-0030. J.W. and A.D. acknowledge that this research was accomplished under Cooperative Agreement No. W911NF-14-2-0059 with the Army Research Laboratory. A.M. thanks Zefang Wang from the Physics Department at The Pennsylvania State University for her help with the differential reflectance measurements. J.W. and A.D. acknowledge Professor Douglas E. Spearot for giving us the implemented parameters of Mo-S in LAMMPS. The views and conclusions contained in this document are those of the authors and should not be interpreted as representing the official policies, either expressed or implied, of the Army Research Laboratory or the U.S. Government. The U.S. Government is authorized to reproduce and distribute reprints for Government purposes notwithstanding any copyright notation herein. NR 72 TC 6 Z9 6 U1 21 U2 66 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD MAR PY 2016 VL 10 IS 3 BP 3186 EP 3197 DI 10.1021/acsnano.5b04550 PG 12 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DH5TR UT WOS:000372855400019 PM 26881920 ER PT J AU Zhou, YL Marson, RL van Anders, G Zhu, J Ma, GX Ercius, P Sun, K Yeom, B Glotzer, SC Kotov, NA AF Zhou, Yunlong Marson, Ryan L. van Anders, Greg Zhu, Jian Ma, Guanxiang Ercius, Peter Sun, Kai Yeom, Bongjun Glotzer, Sharon C. Kotov, Nicholas A. TI Biomimetic Hierarchical Assembly of Helical Supraparticles from Chiral Nanoparticles SO ACS NANO LA English DT Article DE biomimetic nanoparticles; self-assembly; chirality; supraparticles; helices; virus-like nanostructures ID CORE/SHELL QUANTUM DOTS; SEMICONDUCTOR NANOPARTICLES; CIRCULAR-DICHROISM; GOLD NANOPARTICLE; OPTICAL-ACTIVITY; NANOWIRES; NANOCRYSTALS; ORGANIZATION; BIOMOLECULES; RIBBONS AB Chiroptical materials found in butterflies, beetles, stomatopod crustaceans, and other creatures are attributed to biocomposites with helical motifs and multiscale hierarchical organization. These structurally sophisticated materials self-assemble from primitive nanoscale building blocks, a process that is simpler and more energy efficient than many top-down methods currently used to produce similarly sized three-dimensional materials. Here, we report that molecular-scale chirality of a CdTe nanoparticle surface can be translated to nanoscale helical assemblies, leading to chiroptical activity in the visible electromagnetic range. Chiral CdTe nanoparticles coated with cysteine self organize around Te cores to produce helical supraparticles. D-/L-Form of the amino acid determines the dominant left/right helicity of the supraparticles. Coarse-grained molecular dynamics simulations with a helical pair-potential confirm the assembly mechanism and the origin of its enantioselectivity, providing a framework for engineering three-dimensional chiral materials by self-assembly. The helical supraparticles further self-organize into lamellar crystals with liquid crystalline order, demonstrating the possibility of hierarchical organization and with multiple structural motifs and length scales determined by molecular-scale asymmetry of nanoparticle interactions. C1 [Zhou, Yunlong; van Anders, Greg; Zhu, Jian; Ma, Guanxiang; Yeom, Bongjun; Glotzer, Sharon C.; Kotov, Nicholas A.] Univ Michigan, Dept Chem Engn, Ann Arbor, MI 48109 USA. [Marson, Ryan L.; van Anders, Greg; Glotzer, Sharon C.; Kotov, Nicholas A.] Univ Michigan, Biointerfaces Inst, Ann Arbor, MI 48109 USA. [Marson, Ryan L.; Sun, Kai; Glotzer, Sharon C.; Kotov, Nicholas A.] Univ Michigan, Dept Mat Sci & Engn, Ann Arbor, MI 48109 USA. [Kotov, Nicholas A.] Univ Michigan, Dept Biomed Engn, Ann Arbor, MI 48109 USA. [Zhou, Yunlong] Wenzhou Med Univ, CNITECH CAS, Wenzhou Inst Biomat & Engn, Wenzhou 325011, Zhejiang, Peoples R China. [Ercius, Peter] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Natl Ctr Electron Microscopy Mol Foundry, Berkeley, CA 94720 USA. [Yeom, Bongjun] Myongji Univ, Dept Chem Engn, Yongin 17058, Gyeonggido, South Korea. RP Glotzer, SC; Kotov, NA (reprint author), Univ Michigan, Dept Chem Engn, Ann Arbor, MI 48109 USA.; Glotzer, SC; Kotov, NA (reprint author), Univ Michigan, Biointerfaces Inst, Ann Arbor, MI 48109 USA.; Glotzer, SC; Kotov, NA (reprint author), Univ Michigan, Dept Mat Sci & Engn, Ann Arbor, MI 48109 USA.; Kotov, NA (reprint author), Univ Michigan, Dept Biomed Engn, Ann Arbor, MI 48109 USA. EM sglotzer@umich.edu; kotov@umich.edu OI Yeom, Bongjun/0000-0001-8914-0947 FU U.S. Army Research Office [ARO MURI W911NF-10-1-0518]; National Natural Science Foundation of China [NSFC-21573162]; National Science Foundation, Division of Materials Research Award [DMR 1120923]; NSF [ECS-0601345, CBET 0933384, CBET 0932823, CBET 1036672]; U.S. Department of Energy [DE-AC02-05CH11231]; University of Michigan's Electron Microscopy and Analysis Laboratory (EMAL) [DMR-0320740, DMR-9871177]; [WIBEZD2014001-02] FX This material is based upon work supported by the U.S. Army Research Office under Grant Award No. ARO MURI W911NF-10-1-0518. Y.L.Z. acknowledges support from National Natural Science Foundation of China (NSFC-21573162) and WIBEZD2014001-02. R.L.M. and N.A.K. were supported in part by the National Science Foundation, Division of Materials Research Award # DMR 1120923. N.A.K also wishes to acknowledge support from NSF under grants ECS-0601345; CBET 0933384; CBET 0932823; and CBET 1036672. We thank the University of Michigan's Electron Microscopy and Analysis Laboratory (EMAL) for its assistance with electron microscopy and for NSF grants (numbers DMR-0320740 and DMR-9871177), for funding the FEI Nova Nanolab Dualbeam focused ion beam workstation and scanning electron microscope and the JEM-2010F analytical electron microscope used in this work. Y.L.Z. thanks Jinyan Chen and Hailin Qiu for the assistance with the PL lifetime experiment. R.L.M. is grateful to Matthew Spellings for numerous fruitful discussions. Simulations were carried out using computational resources and services supported by Advanced Research Computing at the University of Michigan, Ann Arbor. The experiments performed at the Molecular Foundry, Lawrence Berkeley National Laboratory were supported by the U.S. Department of Energy under contract no. DE-AC02-05CH11231. We also thank EMAL and the College of Engineering for assistance with the Bruker NanoStar small-angle X-ray scattering. The experiments performed at the Molecular Foundry, Lawrence Berkeley National Laboratory were supported by the U.S. Department of Energy under contract #DE-AC02-05CH11231. NR 56 TC 12 Z9 12 U1 68 U2 159 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD MAR PY 2016 VL 10 IS 3 BP 3248 EP 3256 DI 10.1021/acsnano.5b05983 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DH5TR UT WOS:000372855400026 PM 26900920 ER PT J AU Ryu, WH Wilson, H Sohn, S Li, JY Tong, X Shaulsky, E Schroers, J Elimelech, M Taylor, AD AF Ryu, Won-Hee Wilson, Hope Sohn, Sungwoo Li, Jinyang Tong, Xiao Shaulsky, Evyatar Schroers, Jan Elimelech, Menachem Taylor, Andre D. TI Heterogeneous WSX/WO3 Thorn-Bush Nanofiber Electrodes for Sodium-Ion Batteries SO ACS NANO LA English DT Article DE sodium-ion batteries; electrospinning tungsten sulfide; nanofiber; heterogeneous structure ID OXYSULFIDE THIN-FILMS; RECHARGEABLE LITHIUM BATTERIES; PERFORMANCE ANODE MATERIALS; CARBON NANOFIBERS; HIGH-CAPACITY; CONVERSION REACTIONS; TUNGSTEN DISULFIDE; ENERGY-STORAGE; AMORPHOUS MOS3; GRAPHENE AB Heterogeneous electrode materials with hierarchical architectures promise to enable considerable improvement in future energy storage devices. In this study, we report on a tailored synthetic strategy used to create heterogeneous tungsten sulfide/oxide core shell nanofiber materials with vertically and randomly aligned thorn-bush features, and we evaluate them as potential anode materials for high-performance Na-ion batteries. The WSx (2 <= x <= 3, amorphous WS3 and crystalline WS2) nanofiber is successfully prepared by electrospinning and subsequent calcination in a reducing atmosphere. To prevent capacity degradation of the WSx anodes originating from sulfur dissolution, a facile post-thermal treatment in air is applied to form an oxide passivation surface. Interestingly, WO3 thorn bundles are randomly grown on the nanofiber stem, resulting from the surface conversion. We elucidate the evolving morphological and structural features of the nanofibers during post-thermal treatment. The heterogeneous thorn-bush nanofiber electrodes deliver a high second discharge capacity of 791 mAh g(-1) and improved cycle performance for 100 cycles compared to the pristine WSx nanofiber. We show that this hierarchical design is effective in reducing sulfur dissolution, as shown by cycling analysis with counter Na electrodes. C1 [Ryu, Won-Hee; Wilson, Hope; Li, Jinyang; Shaulsky, Evyatar; Elimelech, Menachem; Taylor, Andre D.] Yale Univ, Dept Chem & Environm Engn, 9 Hillhouse Ave, New Haven, CT 06511 USA. [Sohn, Sungwoo; Schroers, Jan] Yale Univ, Dept Mech Engn & Mat Sci, Prospect St, New Haven, CT 06511 USA. [Tong, Xiao] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Taylor, AD (reprint author), Yale Univ, Dept Chem & Environm Engn, 9 Hillhouse Ave, New Haven, CT 06511 USA. EM andre.taylor@yale.edu RI Ryu, Won-Hee/F-8375-2014 OI Ryu, Won-Hee/0000-0002-0203-2992 FU NatureNet Program of the Nature Conservancy; National Science Foundation [NSF-CBET-0954985]; MRSEC DMR [1119826]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX W.-H.R. acknowledges support from The NatureNet Program of the Nature Conservancy. The National Science Foundation NSF-CBET-0954985 PECASE Award and MRSEC DMR 1119826 (CRISP) provided partial support of this work. The Yale Institute for Nanoscience and Quantum Engineering (YINQE) and NSF MRSEC DMR 1119826 (CRISP) provided facility support. Research was carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract DE-AC02-98CH10886. NR 60 TC 11 Z9 11 U1 60 U2 185 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD MAR PY 2016 VL 10 IS 3 BP 3257 EP 3266 DI 10.1021/acsnano.5b06538 PG 10 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DH5TR UT WOS:000372855400027 PM 26808095 ER PT J AU Miller, EM Kroupa, DM Zhang, JB Schulz, P Marshall, AR Kahn, A Lany, S Luther, JM Beard, MC Perkins, CL van de Lagemaat, J AF Miller, Elisa M. Kroupa, Daniel M. Zhang, Jianbing Schulz, Philip Marshall, Ashley R. Kahn, Antoine Lany, Stephan Luther, Joseph M. Beard, Matthew C. Perkins, Craig L. van de Lagemaat, Jao TI Revisiting the Valence and Conduction Band Size Dependence of PbS Quantum Dot Thin Films SO ACS NANO LA English DT Article DE PbS quantum dot films; valence band maximum; photoelectron spectroscopy; energy alignment ID SOLAR-CELLS; SEMICONDUCTOR NANOCRYSTALS; PHOTOEMISSION SPECTRA; LIGAND-EXCHANGE; POST-SYNTHESIS; ENERGY; PERFORMANCE; SPECTROSCOPY; GENERATION; SURFACE AB We use a high signal-to-noise X-ray photoelectron spectrum of bulk PbS, GW calculations, and a model assuming parabolic bands to unravel the various X-ray and ultraviolet photoelectron spectral features of bulk PbS as well as determine how to best analyze the valence band region of PbS quantum dot (QD) films. X-ray and ultraviolet photoelectron spectroscopy (XPS and UPS) are commonly used to probe the difference between the Fermi level and valence band maximum (VBM) for crystalline and thin-film semiconductors. However, we find that when the standard XPS/UPS analysis is used for PbS, the results are often unrealistic due to the low density of states at the VBM. Instead, a parabolic band model is used to determine the VBM for the PbS QD films, which is based on the bulk PbS experimental spectrum and bulk GW calculations. Our analysis highlights the breakdown of the Brillioun zone representation of the band diagram for large band gap, highly quantum confined PbS QDs. We have also determined that in 1,2-ethanedithiol-treated PbS QD films the Fermi level position is dependent on the QD size; specifically, the smallest band gap QD films have the Fermi level near the conduction band minimum and the Fermi level moves away from the conduction band for larger band gap PbS QD films. This change in the Fermi level within the QD band gap could be due to changes in the Pb:S ratio. In addition, we use inverse photoelectron spectroscopy to measure the conduction band region, which has similar challenges in the analysis of PbS QD films due to a low density of states near the conduction band minimum. C1 [Miller, Elisa M.; Kroupa, Daniel M.; Zhang, Jianbing; Schulz, Philip; Marshall, Ashley R.; Lany, Stephan; Luther, Joseph M.; Beard, Matthew C.; Perkins, Craig L.; van de Lagemaat, Jao] Natl Renewable Energy Lab, Chem & Mat Sci Ctr, Golden, CO 80401 USA. [Kroupa, Daniel M.; Marshall, Ashley R.] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. [Schulz, Philip; Kahn, Antoine] Princeton Univ, Dept Elect Engn, Princeton, NJ 08544 USA. [Zhang, Jianbing] Huazhong Univ Sci & Technol, Sch Opt & Elect Informat, 1037 Luoyu Rd, Wuhan 430074, Peoples R China. RP van de Lagemaat, J (reprint author), Natl Renewable Energy Lab, Chem & Mat Sci Ctr, Golden, CO 80401 USA. EM Jao.vandeLagemaat@nrel.gov RI Schulz, Philip/N-2295-2015; OI Schulz, Philip/0000-0002-8177-0108; Lany, Stephan/0000-0002-8127-8885; BEARD, MATTHEW/0000-0002-2711-1355 FU NREL; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; U.S. Department of Energy Office of Science, Office of Basic Energy Sciences Energy Frontier Research Centers Program within the Center for Advanced Solar Photophysics; Energy Frontier Research Center "Center for Next Generation of Materials by Design"; DOE [DE-AC36-08GO28308]; National Science Foundation [DMR-1005892] FX E.M.M. and C.L.P. thank the NREL Director's Fellowship for funding. J.v.L., D.M.K., and M.C.B. were supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences. J.Z., A.R.M., and J.M.L. are supported by the U.S. Department of Energy Office of Science, Office of Basic Energy Sciences Energy Frontier Research Centers Program within the Center for Advanced Solar Photophysics. S.L. was supported by the Energy Frontier Research Center "Center for Next Generation of Materials by Design". All DOE funding to NREL is through contract DE-AC36-08GO28308. The National Science Foundation (DMR-1005892) supported work performed at Princeton by A.K. and P.S. The authors are indebted to G. Teeter and G. Herman for helpful discussions. Also, we thank S. Kim for synthesizing the smallest PbS QD size and J. Endres as well as X. Lin for additional help with the IPES experiments. The authors appreciate help from R. Crisp with regards to the FET measurements. Finally, we thank J. Blackburn for the Seebeck coefficient measurements and helpful discussions. NR 61 TC 8 Z9 8 U1 25 U2 62 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD MAR PY 2016 VL 10 IS 3 BP 3302 EP 3311 DI 10.1021/acsnano.5b06833 PG 10 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DH5TR UT WOS:000372855400031 PM 26895310 ER PT J AU Qiu, Y Vlassiouk, I Hinkle, P Toimil-Molares, ME Levine, AJ Siwy, ZS AF Qiu, Yinghua Vlassiouk, Ivan Hinkle, Preston Toimil-Molares, Maria Eugenia Levine, Alex J. Siwy, Zuzanna S. TI Role of Particle Focusing in Resistive-Pulse Technique: Direction-Dependent Velocity in Micropores SO ACS NANO LA English DT Article DE resistive pulse; particle focusing; micropore; asymmetric transport ID INDIVIDUAL NANOPARTICLES; CHARGED-PARTICLES; BROWNIAN MOTORS; TRANSPORT; PORES; NANOPORE; CHANNEL; SIZE; DNA; DIFFUSION AB Passage time through single micropores is an important parameter used to quantify the surface charge and zeta potential of particles. In the resistive-pulse technique, the measured time of pressure- or electric field-induced translocation is assumed to be direction independent. This assumption is supported by the low velocities of the particles and the supporting fluid such that the transport reversibility known for Stokes flow is expected to apply. In this article, we present examples of micropores in which passage time of similar to 400 nm diameter particles becomes direction-dependent; that is, the particles' trans location times from left to right and right to left are different. These pores are characterized by an undulating inner diameter such that at least one wider zone called a cavity separates two narrower regions of different lengths. We propose that the observed direction-dependence of the translocation velocity is caused by an asymmetric efficiency of particle focusing toward the pore axis, which leads to a direction-dependent set of particle trajectories. The reported pores present the simplest system in which time-broken symmetry has been observed. The results are of importance for sensing of particles and molecules by the resistive-pulse technique since pores used for detection are often characterized by finite roughness or noncylindrical shape. This article also points to the role of particle focusing in the magnitude and distribution of the translocation times. C1 [Qiu, Yinghua; Hinkle, Preston; Siwy, Zuzanna S.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Qiu, Yinghua] Southeast Univ, Sch Mech Engn, Nanjing 211189, Jiangsu, Peoples R China. [Qiu, Yinghua] Southeast Univ, Jiangsu Key Lab Design & Mfg Micronano Biomed Ins, Nanjing 211189, Jiangsu, Peoples R China. [Vlassiouk, Ivan] Oak Ridge Natl Lab, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. [Toimil-Molares, Maria Eugenia] GSI Helmholtz Ctr Heavy Ion Res, Dept Mat Sci, Darmstadt, Germany. [Levine, Alex J.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Levine, Alex J.] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. [Levine, Alex J.] Univ Calif Los Angeles, Dept Biomath, Los Angeles, CA 90095 USA. RP Siwy, ZS (reprint author), Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. EM zsiwy@uic.edu RI Qiu, Yinghua/N-6497-2014; Vlassiouk, Ivan/F-9587-2010 OI Qiu, Yinghua/0000-0003-2489-0784; Vlassiouk, Ivan/0000-0002-5494-0386 FU National Science Foundation [CHE 1306058]; China Scholarship Council [CSC 201406090034]; [NSF-DMR-1301988] FX This research was supported by the National Science Foundation (CHE 1306058). Y.Q, acknowledges financial support from the China Scholarship Council (CSC 201406090034). A.J.L. acknowledges support from NSF-DMR-1301988. We are grateful to Prof. Miguel Rubi from the University of Barcelona for discussions and guidance. NR 56 TC 4 Z9 4 U1 9 U2 28 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD MAR PY 2016 VL 10 IS 3 BP 3509 EP 3517 DI 10.1021/acsnano.5b07709 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DH5TR UT WOS:000372855400053 PM 26901283 ER PT J AU Tselev, A Velmurugan, J Ievlev, AV Kalinin, SV Kolmakov, A AF Tselev, Alexander Velmurugan, Jeyavel Ievlev, Anton V. Kalinin, Sergei V. Kolmakov, Andrei TI Seeing through Walls at the Nanoscale: Microwave Microscopy of Enclosed Objects and Processes in Liquids SO ACS NANO LA English DT Article DE in situ imaging; radiolysis-free in-liquid imaging; encapsulation; near-field microwave microscopy ID SCANNING-ELECTRON-MICROSCOPY; X-RAY MICROSCOPY; AQUEOUS-SOLUTIONS; FORCE MICROSCOPY; BREAST-CANCER; CELLS; SILVER; SPECTROSCOPY; RESOLUTION; SAMPLES AB Noninvasive in situ nanoscale imaging in liquid environments is a current imperative in the analysis of delicate biomedical objects and electrochemical processes at reactive liquid solid interfaces. Microwaves of a few gigahertz frequencies offer photons with energies of approximate to 10 mu eV, which can affect neither electronic states nor chemical bonds in condensed matter. Here, we describe an implementation of scanning near-field microwave microscopy for imaging in liquids using ultrathin molecular impermeable membranes separating scanning probes from samples enclosed in environmental cells. We imaged a model electroplating reaction as well as individual live cells. Through a side-by-side comparison of the microwave imaging with scanning electron microscopy, we demonstrate the advantage of microwaves for artifact-free imaging. C1 [Tselev, Alexander; Ievlev, Anton V.; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Tselev, Alexander; Kalinin, Sergei V.] Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA. [Velmurugan, Jeyavel; Kolmakov, Andrei] NIST, Ctr Nanoscale Sci & Technol, Gaithersburg, MD 20899 USA. [Velmurugan, Jeyavel] Univ Maryland, Maryland NanoCtr, College Pk, MD 20742 USA. RP Tselev, A (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.; Tselev, A (reprint author), Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA.; Kolmakov, A (reprint author), NIST, Ctr Nanoscale Sci & Technol, Gaithersburg, MD 20899 USA. EM atselev@utk.edu; andrei.kolmakov@nist.gov RI Ievlev, Anton/H-3678-2012; Kolmakov, Andrei/B-1460-2017 OI Ievlev, Anton/0000-0003-3645-0508; Kolmakov, Andrei/0000-0001-5299-4121 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; U.S. Civilian Research and Development Foundation; NIST-CNST/UMD-IREAP Cooperative Agreement FX Microwave imaging was conducted at the Center for Nanoscale Science and Technology, NIST, and at the Center for Nanophase Materials Sciences, ORNL, which also provided support (AT., A.V.I., S.V.K.) and which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. A.T. acknowledges support by U.S. Civilian Research and Development Foundation. J.V. work was supported by a NIST-CNST/UMD-IREAP Cooperative Agreement. Authors are thankful to Dr. K. Siebein for the experimental support, and to Dr. T. Moffat, Dr. M. Stiles, and Dr. N. Zhitenev (all at NIST) for their valuable discussions. NR 40 TC 4 Z9 4 U1 10 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD MAR PY 2016 VL 10 IS 3 BP 3562 EP 3570 DI 10.1021/acsnano.5b07919 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DH5TR UT WOS:000372855400059 PM 26866377 ER PT J AU Chen, K Chai, ZG Li, C Shi, LR Liu, MX Xie, Q Zhang, YF Xu, DS Manivannan, A Liu, ZF AF Chen, Ke Chai, Zhigang Li, Cong Shi, Liurong Liu, Mengxi Xie, Qin Zhang, Yanfeng Xu, Dongsheng Manivannan, Ayyakkannu Liu, Zhongfan TI Catalyst-Free Growth of Three-Dimensional Graphene Flakes and Graphene/g-C3N4 Composite for Hydrocarbon Oxidation SO ACS NANO LA English DT Article DE graphene; chemical vapor deposition; three-dimensional; powder; g-C3N4 ID CHEMICAL-VAPOR-DEPOSITION; CARBON NITRIDE NANOSHEETS; METAL-FREE CATALYSTS; FEW-LAYER GRAPHENE; GRAPHITE OXIDE; REDUCTION; CYCLOHEXANE; SUPERCAPACITORS; ACTIVATION; NANOTUBES AB Mass production of high-quality graphene flakes is important for commercial applications. Graphene microsheets have been produced on an industrial scale by chemical and liquid -phase exfoliation of graphite. However, strong-interaction-induced interlayer aggregation usually leads to the degradation of their intrinsic properties. Moreover, the crystallinity or layer -thickness controllability is not so perfect to fulfill the requirement for advanced technologies. Herein, we report a quartz-powder-derived chemical vapor deposition growth of three-dimensional (3D) high-quality graphene flakes and demonstrate the fabrication and application of graphene/g-C3N4 composites. The graphene flakes obtained after the removal of growth substrates exhibit the 3D curved microstructure, controllable layer thickness, good crystallinity, as well as weak interlayer interactions suitable for preventing the interlayer stacking. Benefiting from this, we achieved the direct synthesis of g-C3N4 on purified graphene flakes to form the uniform graphene/g-C3N4 composite, which provides efficient electron transfer interfaces to boost its catalytic oxidation activity of cycloalkane with relatively high yield, good selectivity, and reliable stability. C1 [Chen, Ke; Chai, Zhigang; Li, Cong; Shi, Liurong; Liu, Mengxi; Xie, Qin; Zhang, Yanfeng; Xu, Dongsheng; Liu, Zhongfan] Peking Univ, Coll Chem & Mol Engn, Ctr Nanochem CNC, Beijing Natl Lab Mol Sci State,Key Lab Struct Che, Beijing 100871, Peoples R China. [Li, Cong; Zhang, Yanfeng] Peking Univ, Coll Engn, Dept Mat Sci & Engn, Beijing 100871, Peoples R China. [Chen, Ke] Henan Univ, Key Lab Special Funct Mat, Minist Educ, Kaifeng 475004, Peoples R China. [Manivannan, Ayyakkannu] W Virginia Univ, Dept Aerosp & Mech Engn, Morgantown, WV 26507 USA. [Manivannan, Ayyakkannu] US DOE, NETL, Morgantown, WV 26507 USA. [Liu, Mengxi] Natl Ctr Nanosci & Technol, CAS Key Lab Standardizat & Measurement Nanotechno, Beijing 100190, Peoples R China. RP Zhang, YF; Liu, ZF (reprint author), Peking Univ, Coll Chem & Mol Engn, Ctr Nanochem CNC, Beijing Natl Lab Mol Sci State,Key Lab Struct Che, Beijing 100871, Peoples R China.; Zhang, YF (reprint author), Peking Univ, Coll Engn, Dept Mat Sci & Engn, Beijing 100871, Peoples R China. EM yanfengzhang@pku.edu.cn; zfliu@pku.edu.cn RI Liu, Zhong/P-2974-2014; Chen, Ke/F-8985-2014; Chai, Zhigang/D-4291-2016 OI Liu, Zhong/0000-0001-5554-1902; Chen, Ke/0000-0003-2384-8437; Chai, Zhigang/0000-0002-5536-734X FU National Basic Research Program of China [2013CB932603, 2012CB933404, 2012CB921404, 2013CB934600]; National Natural Science Foundation of China [51432002, 51121091, 51520105003, 51290272, 51222201, 51502077]; Specialized Research Fund for the Doctoral Program of Higher Education of China [20120001130010]; Beijing Municipal Science and Technology Planning Project [Z151100003315013] FX This work was financially supported by the National Basic Research Program of China (Nos. 2013CB932603, 2012CB933404, 2012CB921404, and 2013CB934600), the National Natural Science Foundation of China (Nos. 51432002, 51121091, 51520105003, 51290272, 51222201, and 51502077), the Specialized Research Fund for the Doctoral Program of Higher Education of China (No. 20120001130010), and the Beijing Municipal Science and Technology Planning Project (No. Z151100003315013). NR 46 TC 3 Z9 3 U1 71 U2 223 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD MAR PY 2016 VL 10 IS 3 BP 3665 EP 3673 DI 10.1021/acsnano.6b00113 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DH5TR UT WOS:000372855400071 PM 26918323 ER PT J AU Wu, YMA Li, L Li, Z Kinaci, A Chan, MKY Sun, YG Guest, JR McNulty, I Rajh, T Liu, YZ AF Wu, Yimin A. Li, Liang Li, Zheng Kinaci, Alper Chan, Maria K. Y. Sun, Yugang Guest, Jeffrey R. McNulty, Ian Rajh, Tijana Liu, Yuzi TI Visualizing Redox Dynamics of a Single Ag/AgCl Heterogeneous Nanocatalyst at Atomic Resolution SO ACS NANO LA English DT Article DE environmental TEM; in situ TEM; Ag/AgCl heterogeneous nanocatalyst; density functional theory ID AG-AT-AGCL; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; IN-SITU; VISIBLE-LIGHT; PLASMONIC PHOTOCATALYST; ELECTRON-MICROSCOPY; CATALYST NANOPARTICLES; PHASE-TRANSITIONS; BASIS-SET AB Operando characterization of gas solid reactions at the atomic scale is of great importance for determining the mechanism of catalysis. This is especially true in the study of heterostructures because of structural correlation between the different parts. However, such experiments are challenging and have rarely been accomplished. In this work, atomic scale redox dynamics of Ag/AgCl heterostructures have been studied using in situ environmental transmission electron microscopy (ETEM) in combination with density function theory (DFT) calculations. The reduction of Ag/AgCl to Ag is likely a result of the formation of Cl vacancies while Ag+ ions accept electrons. The oxidation process of Ag/AgCl has been observed: rather than direct replacement of Cl by O, the Ag/AgCl nanocatalyst was first reduced to Ag, and then Ag was oxidized to different phases of silver oxide under different O-2 partial pressures. Ag2O formed at low O-2 partial pressure, whereas AgO formed at atmospheric pressure. By combining in situ ETEM observation and DFT calculations, this structural evolution is characterized in a distinct nanoscale environment. C1 [Wu, Yimin A.; Li, Liang; Li, Zheng; Kinaci, Alper; Chan, Maria K. Y.; Sun, Yugang; Guest, Jeffrey R.; McNulty, Ian; Rajh, Tijana; Liu, Yuzi] Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. [Sun, Yugang] Temple Univ, Dept Chem, 1901 N 13th St, Philadelphia, PA 19122 USA. RP Liu, YZ (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. EM yuziliu@anl.gov RI Liu, Yuzi/C-6849-2011; Guest, Jeffrey/B-2715-2009; Sun, Yugang /A-3683-2010; Li, Zheng/L-1355-2016; OI Guest, Jeffrey/0000-0002-9756-8801; Sun, Yugang /0000-0001-6351-6977; Li, Zheng/0000-0001-5281-8101; Wu, Yimin A./0000-0002-3807-8431; Kinaci, Alper/0000-0003-2167-3776 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; National Science Foundation [ACI-1053575] FX Use of the Center for Nanoscale Materials, an Office of Science user facility, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. This work used the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by National Science Foundation grant number ACI-1053575.64 NR 64 TC 5 Z9 5 U1 22 U2 62 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD MAR PY 2016 VL 10 IS 3 BP 3738 EP 3746 DI 10.1021/acsnano.6b00355 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DH5TR UT WOS:000372855400078 PM 26937679 ER PT J AU Durniak, MT Bross, AS Elsaesser, D Chaudhuri, A Smith, ML Allerman, AA Lee, SC Brueck, SRJ Wetzel, C AF Durniak, Mark T. Bross, Adam S. Elsaesser, David Chaudhuri, Anabil Smith, Michael L. Allerman, Andrew A. Lee, Seung C. Brueck, Steven R. J. Wetzel, Christian TI Green Emitting Cubic GaInN/GaN Quantum Well Stripes on Micropatterned Si(001) and Their Strain Analysis SO ADVANCED ELECTRONIC MATERIALS LA English DT Article ID GAN; EPITAXY; GAAS; ZINCBLENDE; SUBSTRATE; GROWTH; FIELDS AB GaInN/GaN heterostructures in the cubic lattice variant have the potential to overcome the limitations of wurtzite structures as commonly used for light emitting and laser diodes. Wurtzite GaInN (0001), suffers from large internal polarization fields, which force design compromises toward ultranarrow quantum wells and reduce recombination volume and efficiency, particularly in the green, yellow, and red visible spectral regions. Cubic GaInN microstripes on micropatterned Si(001), with {111} V-grooves oriented along Si 01 (1) over bar, offer a system free of internal polarization fields, wider quantum wells, and a smaller bandgap energy. 6 and 9 nm Ga1-xInxN/GaN single quantum well structures are prepared and their emission spectra found to be dominated by the recombination in the cubic wells. The peak wavelength ranges from 520 to 570 nm with a polarization predominately perpendicular to the grooves. These values are about 26 nm longer in wavelength than the equivalent wurtzite (1 (1) over bar 01) sample portions and 40 nm longer than the wurtzite (0001) oriented portions. An alloy composition range of 0.2 < x < 0.3 has been estimated in those cubic portions and quantum efficiency comparable to planar wurtzite structures. The stripe geometry and photon polarization may be suitable for optical mode confinement and reduced threshold stimulated emission. C1 [Durniak, Mark T.; Bross, Adam S.; Wetzel, Christian] Rensselaer Polytech Inst, Dept Mat Sci & Engn, 110 8th St, Troy, NY 12180 USA. [Elsaesser, David; Wetzel, Christian] Rensselaer Polytech Inst, Dept Phys Appl Phys & Astron, 110 8th St, Troy, NY 12180 USA. [Chaudhuri, Anabil; Lee, Seung C.; Brueck, Steven R. J.] Ctr High Technol Mat, 1313 Goddard St SE, Albuquerque, NM 87106 USA. [Smith, Michael L.; Allerman, Andrew A.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Wetzel, C (reprint author), Rensselaer Polytech Inst, Dept Mat Sci & Engn, 110 8th St, Troy, NY 12180 USA.; Wetzel, C (reprint author), Rensselaer Polytech Inst, Dept Phys Appl Phys & Astron, 110 8th St, Troy, NY 12180 USA. EM wetzel@ieee.org RI Wetzel, Christian/O-4017-2014 OI Wetzel, Christian/0000-0002-6055-0990 FU Engineering Research Centers Program (ERC) of the National Science Foundation under NSF [EEC-0812056]; New York State under NYSTAR [C130145]; Sandia National Laboratories Campus Executive Fellowship for Laboratory Directed Research and Development FX This work was supported primarily by the Engineering Research Centers Program (ERC) of the National Science Foundation under NSF Cooperative Agreement No. EEC-0812056, in part by New York State under NYSTAR Contract No. C130145, and in part by the Sandia National Laboratories Campus Executive Fellowship for Laboratory Directed Research and Development. NR 33 TC 3 Z9 3 U1 10 U2 19 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2199-160X J9 ADV ELECTRON MATER JI Adv. Electron. Mater. PD MAR PY 2016 VL 2 IS 3 AR 1500327 DI 10.1002/aelm.201500327 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA DH6SV UT WOS:000372922800010 ER PT J AU Sun, KY Hong, TZ Taylor-Lange, SC Piette, MA AF Sun, Kaiyu Hong, Tianzhen Taylor-Lange, Sarah C. Piette, Mary Ann TI A pattern-based automated approach to building energy model calibration SO APPLIED ENERGY LA English DT Article DE Building simulation; Energy use pattern; EnergyPlus; Model calibration; Pattern recognition ID HIGH-PERFORMANCE BUILDINGS; SIMULATION PROGRAMS; GRAPHICAL INDEXES; OFFICE BUILDINGS; RETROFIT; METHODOLOGY; OCCUPANCY; RP-1051; DEMAND; MATCH AB Building model calibration is critical in bringing simulated energy use closer to the actual consumption. This paper presents a novel, automated model calibration approach that uses logic linking parameter tuning with bias pattern recognition to overcome some of the disadvantages associated with traditional calibration processes. The pattern-based process contains four key steps: (1) running the original pre-calibrated energy model to obtain monthly simulated electricity and gas use; (2) establishing a pattern bias, either Universal or Seasonal Bias, by comparing load shape patterns of simulated and actual monthly energy use; (3) using programmed logic to select which parameter to tune first based on bias pattern, weather and input parameter interactions; and (4) automatically tuning the calibration parameters and checking the progress using pattern-fit criteria. The automated calibration algorithm was implemented in the Commercial Building Energy Saver, a web-based building energy retrofit analysis toolkit. The proof of success of the methodology was demonstrated using a case study of an office building located in San Francisco. The case study inputs included the monthly electricity bill, monthly gas bill, original building model and weather data with outputs resulting in a calibrated model that more closely matched that of the actual building energy use profile. The novelty of the developed calibration methodology lies in linking parameter tuning with the underlying logic associated with bias pattern identification. Although there are some limitations to this approach, the pattern-based automated calibration methodology can be universally adopted as an alternative to manual or hierarchical calibration approaches. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Sun, Kaiyu; Hong, Tianzhen; Taylor-Lange, Sarah C.; Piette, Mary Ann] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Bldg Technol & Urban Syst Div, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Hong, TZ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Bldg Technol & Urban Syst Div, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM thong@LBL.gov OI Hong, Tianzhen/0000-0003-1886-9137 FU California Energy Commission under the Public Interest Energy Research (PIER) Program [PIR-12-031]; U.S. Department of Energy [DE-AC02-05CH11231] FX This study was funded by California Energy Commission under the Public Interest Energy Research (PIER) Program Award No. PIR-12-031. This work was also supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Authors appreciated help from project team members Yixing Chen and Rongpeng Zhang. NR 54 TC 4 Z9 4 U1 1 U2 2 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD MAR 1 PY 2016 VL 165 BP 214 EP 224 DI 10.1016/j.apenergy.2015.12.026 PG 11 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DH3GV UT WOS:000372676400016 ER PT J AU Peng, JQ Curcija, DC Lu, L Selkowitz, SE Yang, HX Zhang, WL AF Peng, Jinqing Curcija, Dragan C. Lu, Lin Selkowitz, Stephen E. Yang, Hongxing Zhang, Weilong TI Numerical investigation of the energy saving potential of a semi-transparent photovoltaic double-skin facade in a cool-summer Mediterranean climate SO APPLIED ENERGY LA English DT Article DE Building-integrated photovoltaic (BIPV); Energy saving potential; Building energy use; Double-skin facade; Semi-transparent thin-film photovoltaic (STPV) ID HONG-KONG; THERMAL PERFORMANCE; OFFICE BUILDINGS; SOLAR-CELLS; PV MODULES; BIPV WINDOW; INTEGRATION; ELEMENTS; INDOOR; BEHAVIOR AB This paper presents the annual overall energy performance and energy-saving potential of a ventilated photovoltaic double-skin facade (PV-DSF) in a cool-summer Mediterranean climate zone. A numerical simulation model based on EnergyPlus was utilized to simulate the PV-DSF overall energy performance, simultaneously taking into account thermal power and daylight. Based on numerical model, sensitivity analyses about air gap width and ventilation modes have been lead in Berkeley (California) with the aim to optimize unit's structure design and operational strategy of PV-DSF. Via simulation, the overall energy performance including thermal, power and daylighting of the optimized PV-DSF was evaluated using the typical meteorological year (TMY) weather data. It was found that per unit area of the proposed PV-DSF was able to generate about 65 kW h electricity yearly. If high efficiency cadmium telluride (CdTe) semi-transparent PV modules are adopted, the annual energy output could be even doubled. The PV-DSF studied, also featured good thermal and daylighting performances. The PV-DSF can effectively block solar radiation while still providing considerable daylighting illuminance. Due simply to excellent overall energy performance, a PV-DSF at Berkeley can reduce net electricity use by about 50% compared with other commonly used glazing systems. Efficiency improvements of semi-transparent PV modules would further increase the energy saving potential of a PV-DSF and thus making this technology more promising. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Peng, Jinqing] Hunan Univ, Coll Civil Engn, Changsha 410082, Hunan, Peoples R China. [Peng, Jinqing; Lu, Lin; Yang, Hongxing; Zhang, Weilong] Hong Kong Polytech Univ, Dept Bldg Serv Engn, RERG, Hong Kong, Hong Kong, Peoples R China. [Curcija, Dragan C.; Selkowitz, Stephen E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Bldg Technol & Urban Syst Div, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Lu, L (reprint author), Hong Kong Polytech Univ, Dept Bldg Serv Engn, RERG, Hong Kong, Hong Kong, Peoples R China. EM Jallenpeng@gmail.com; bellu@polyu.edu.hk RI Lu, Lin/D-6919-2013; Yang, Hongxing/E-5737-2014; OI Lu, Lin/0000-0002-4114-3468; Yang, Hongxing/0000-0001-5117-5394; Zhang, Weilong/0000-0002-8847-650X; Selkowitz, Stephen/0000-0002-5274-6635; Peng, Jinqing (Jallen)/0000-0003-4455-5908 FU Public Policy Research (PPR) of the Hong Kong Special Administrative Region (HKSAR) [2013.A6.010.13A]; Hong Kong Construction Industry Council Research Fund (CIC Project) [K-ZJK1]; Fundamental Research Funds for the Central Universities (Hunan University); Hong Kong Housing Authority Research Fund [K-ZJHE] FX The authors appreciate the financial supports provided by the Public Policy Research (PPR) Funding Scheme 2013/14 (PPR Project: 2013.A6.010.13A) of the Hong Kong Special Administrative Region (HKSAR), the Hong Kong Construction Industry Council Research Fund (CIC Project: K-ZJK1), the Fundamental Research Funds for the Central Universities (Hunan University), as well as the Hong Kong Housing Authority Research Fund (Project no. K-ZJHE). NR 43 TC 6 Z9 6 U1 8 U2 18 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD MAR 1 PY 2016 VL 165 BP 345 EP 356 DI 10.1016/j.apenergy.2015.12.074 PG 12 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DH3GV UT WOS:000372676400028 ER PT J AU Ravi, S Macknick, J Lobell, D Field, C Ganesan, K Jain, R Elchinger, M Stoltenberg, B AF Ravi, Sujith Macknick, Jordan Lobell, David Field, Christopher Ganesan, Karthik Jain, Rishabh Elchinger, Michael Stoltenberg, Blaise TI Colocation opportunities for large solar infrastructures and agriculture in drylands SO APPLIED ENERGY LA English DT Article DE Renewable energy; Life cycle assessment; Water use efficiency; Land use; Food-energy-water nexus ID ENERGY USE PATTERN; ENVIRONMENTAL IMPACTS; PV SYSTEMS; INDIA; PERFORMANCE; WATER; RECOMMENDATIONS; CHALLENGES; RAJASTHAN; DESERTS AB Solar energy installations in arid and semi-arid regions are rapidly increasing due to technological advances and policy support. Although solar energy provides several benefits such as reduction of greenhouse gases, reclamation of degraded land, and improved quality of life in developing countries, the deployment of large-scale renewable energy infrastructure may negatively impact land and water resources. Meeting the ever-expanding energy demand with limited land and water resources in the context of increasing demand for alternative uses such as agricultural and domestic consumption is a major challenge. The goal of this study was to explore opportunities to colocate solar infrastructures and agricultural crops to maximize the efficiency of land and water use. We investigated the energy inputs/outputs, water use, greenhouse gas emissions, and economics of solar installations in northwestern India in comparison to aloe vera cultivation, another widely promoted and economically important land use in these systems. The life cycle analyses show that the colocated systems are economically viable in some rural areas and may provide opportunities for rural electrification and stimulate economic growth. The water inputs for cleaning solar panels are similar to amounts required for annual aloe productivity, suggesting the possibility of integrating the two systems to maximize land and water use efficiency. A life cycle analysis of a hypothetical colocation indicated higher returns per m(3) of water used than either system alone. The northwestern region of India has experienced high population growth in the past decade, creating additional demand for land and water resources. In these water-limited areas, coupled solar infrastructure and agriculture could be established in marginal lands with low water use, thus minimizing the socioeconomic and environmental issues resulting from cultivation of economically important non-food crops (e.g., aloe) in prime agricultural lands. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Ravi, Sujith] Temple Univ, Dept Earth & Environm Sci, 1901 N 13th St, Philadelphia, PA 19122 USA. [Macknick, Jordan; Elchinger, Michael; Stoltenberg, Blaise] Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. [Lobell, David; Field, Christopher] Stanford Univ, Dept Environm Earth Syst Sci, 473 Via Ortega, Stanford, CA 94305 USA. [Field, Christopher] Carnegie Inst Sci, Dept Global Ecol, Stanford, CA 94301 USA. [Ganesan, Karthik; Jain, Rishabh] Council Energy Environm & Water, New Delhi 110001, India. [Jain, Rishabh] Natl Univ Singapore, Lee Kuan Yew Sch Publ Policy, Singapore 119077, Singapore. RP Ravi, S (reprint author), Temple Univ, Dept Earth & Environm Sci, 1901 N 13th St, Philadelphia, PA 19122 USA. EM sravi@temple.edu RI Ravi, Sujith/C-3586-2008 OI Ravi, Sujith/0000-0002-0425-9373 FU Joint Institute for Strategic Energy Analysis (JISEA) FX The Joint Institute of Strategic Energy Analysis (JISEA - IRAAP), TomKat Center for Sustainable Energy at Stanford University, Council on Environment, Energy & Water (CEEW). This work was supported by the Joint Institute for Strategic Energy Analysis (JISEA). JISEA is operated by the Alliance for Sustainable Energy, LLC, on behalf of the U.S. Department of Energy's National Renewable Energy Laboratory, the University of Colorado-Boulder, the Colorado School of Mines, the Colorado State University, the Massachusetts Institute of Technology, and Stanford University. The U.S. Government retains and the publisher, by accepting the article for publication, acknowledges that the U.S. Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this work, or allow others to do so, for U.S. Government purposes. Some symbols used in the graphical abstract are courtesy of the Integration and Application Network (ian.umces.edu/symbols). NR 61 TC 1 Z9 1 U1 5 U2 25 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD MAR 1 PY 2016 VL 165 BP 383 EP 392 DI 10.1016/j.apenergy.2015.12.078 PG 10 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DH3GV UT WOS:000372676400031 ER PT J AU Jafari-Marandi, R Hu, MQ Omitaomu, OA AF Jafari-Marandi, Ruholla Hu, Mengqi Omitaomu, OluFemi A. TI A distributed decision framework for building clusters with different heterogeneity settings SO APPLIED ENERGY LA English DT Article DE Distributed decision making; Electricity consumption behavior; Self-organizing map; Genetic algorithm ID DEMAND-SIDE MANAGEMENT; THERMAL MASS; PREDICTIVE CONTROL; ENERGY MANAGEMENT; OPERATION; SYSTEM; LOAD; UNCERTAINTY; OPTIMIZATION; MODEL AB In the past few decades, extensive research has been conducted to develop operation and control strategy for smart buildings with the purpose of reducing energy consumption. Besides studying on single building, it is envisioned that the next generation buildings can freely connect with one another to share energy and exchange information in the context of smart grid. It was demonstrated that a network of connected buildings (aka building clusters) can significantly reduce primary energy consumption, improve environmental sustainability and building's resilience capability. However, an analytic tool to determine which type of buildings should form a cluster and what is the impact of building clusters' heterogeneity based on energy profile to the energy performance of building clusters is missing. To bridge these research gaps, we propose a self-organizing map clustering algorithm to divide multiple buildings to different clusters based on their energy profiles, and a homogeneity index to evaluate the heterogeneity of different building clusters configurations. In addition, a bi-level distributed decision model is developed to study the energy sharing in the building clusters. To demonstrate the effectiveness of the proposed clustering algorithm and decision model, we employ a dataset including monthly energy. consumption data for 30 buildings where the data is collected every 15 min. It is demonstrated that the proposed decision model can achieve at least 13% cost savings for building clusters. The results show that the heterogeneity of energy profile is an important factor to select battery and renewable energy source for building clusters, and the shared battery and renewable energy are preferred for more heterogeneous building clusters. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Jafari-Marandi, Ruholla] Mississippi State Univ, Dept Ind & Syst Engn, 260 McCain Engn Bldg, Mississippi State, MS 39762 USA. [Hu, Mengqi] Univ Illinois, Dept Mech & Ind Engn, 842 W Taylor St,3023 ERF, Chicago, IL 60607 USA. [Omitaomu, OluFemi A.] Oak Ridge Natl Lab, Computat Sci & Engn Div, Oak Ridge, TN 37831 USA. [Omitaomu, OluFemi A.] Univ Tennessee, Dept Ind & Syst Engn, Knoxville, TN 37996 USA. RP Hu, MQ (reprint author), Univ Illinois, Dept Mech & Ind Engn, 842 W Taylor St,3023 ERF, Chicago, IL 60607 USA. EM mhu@uic.edu OI Omitaomu, OluFemi/0000-0002-3078-7196 NR 46 TC 3 Z9 3 U1 4 U2 9 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD MAR 1 PY 2016 VL 165 BP 393 EP 404 DI 10.1016/j.apenergy.2015.12.088 PG 12 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DH3GV UT WOS:000372676400032 ER PT J AU Zaccaria, V Tucker, D Traverso, A AF Zaccaria, V. Tucker, D. Traverso, A. TI Transfer function development for SOFC/GT hybrid systems control using cold air bypass SO APPLIED ENERGY LA English DT Article DE SOFC; Cyber-physical simulation; Transfer functions; Cathode airflow ID OXIDE FUEL-CELL; TEMPERATURE DISTRIBUTION; TEST RIG; STACK; MODEL AB Fuel cell gas turbine hybrids present significant challenges in terms of system control because of the coupling of different time-scale phenomena. Hence, the importance of studying the integrated system dynamics is critical. With the aim of safe operability and efficiency optimization, the cold air bypass valve was considered an important actuator since it affects several key parameters and can be very effective in controlling compressor surge. Two different tests were conducted using a cyber-physical approach. The Hybrid Performance (HyPer) facility couples gas turbine equipment with a cyber physical solid oxide fuel cell in which the hardware is driven by a numerical fuel cell model operating in real time. The tests were performed moving the cold air valve from the nominal position of 40% with a step of 15% up and down, while the system was in open loop, i.e. no control on turbine speed or inlet temperature. The effect of the valve change on the system was analyzed and transfer functions were developed for several important variables such as cathode mass flow, total pressure drop and surge margin. Transfer functions can show the response time of different system variables, and are used to characterize the dynamic response of the integrated system. Opening the valve resulted in an immediate positive impact on pressure drop and surge margin. A valve change also significantly affected fuel cell temperature, demonstrating that the cold air bypass can be used for thermal management of the cell. Published by Elsevier Ltd. C1 [Zaccaria, V.; Tucker, D.] US DOE, NETL, 3610 Collins Ferry Rd, Morgantown, WV 26507 USA. [Traverso, A.] Univ Genoa, Thermochem Power Grp, Via Montallegro 1, I-16145 Genoa, Italy. RP Zaccaria, V (reprint author), 3610 Collins Ferry Rd, Morgantown, WV 26507 USA. EM valentina.zaccaria@contr.netl.doe.gov FU U.S. Department of Energy, Crosscutting Research program FX This work was funded through the U.S. Department of Energy, Crosscutting Research program implemented through the Strategic Center for Coal in the Office of Fossil Energy. The authors also would like to thank Professor Larry Banta from West Virginia University, Dr. Paolo. Pezzini from Ames Laboratory and Nor Farida Harun from MacMaster University for their support. NR 35 TC 3 Z9 3 U1 3 U2 5 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD MAR 1 PY 2016 VL 165 BP 695 EP 706 DI 10.1016/j.apenergy.2015.12.094 PG 12 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DH3GV UT WOS:000372676400056 ER PT J AU Reddy, HK Muppaneni, T Ponnusamy, S Sudasinghe, N Pegallapati, A Selvaratnam, T Seger, M Dungan, B Nirmalakhandan, N Schaub, T Holguin, FO Lammers, P Voorhies, W Deng, SG AF Reddy, Harvind Kumar Muppaneni, Tapaswy Ponnusamy, Sundaravadivelnathan Sudasinghe, Nilusha Pegallapati, Ambica Selvaratnam, Thinesh Seger, Mark Dungan, Barry Nirmalakhandan, Nagamany Schaub, Tanner Holguin, F. Omar Lammers, Peter Voorhies, Wayne Deng, Shuguang TI Temperature effect on hydrothermal liquefaction of Nannochloropsis gaditana and Chlorella sp. SO APPLIED ENERGY LA English DT Article DE Hydrothermal liquefaction; Wet algae; Sequential extraction and liquefaction; Energy recovery; Nutrients; By-products ID SUBCRITICAL WATER EXTRACTION; SUPERCRITICAL WATER; BIO-OIL; BIODIESEL PRODUCTION; NUTRIENT REMOVAL; MICROALGAE; ALGAE; BIOFUELS; BIOMASS; TECHNOLOGIES AB Temperature effect on hydrothermal liquefaction (HTL) of Nannochloropsis gaditana and Chlorella sp. was investigated with 10% biomass loading at HTL temperatures of 180-330 degrees C, and reaction time of 30 min. Maximum yields of 47.5% for Nannochloropsis sp. and 32.5% biocrude oil yields for Chlorella sp. were obtained at 300 degrees C. The higher heating values of biocrude oils produced in this work ranged between 34 and 39 MJ/kg. 79% of energy in the Nannochloropsis sp. was recovered at 300 degrees C and 62% of energy recovery from Chlorella sp. was achieved at 200 degrees C. Valuable nutrients (NH3-N and PO43-) produced during the HTL process were quantified, from the aqueous phase for both strains of biomass. The aqueous phase samples obtained at all temperatures were also analyzed for amino acids and carbohydrates. The suitable temperatures for extraction of lipids, amino acids and carbohydrates have been identified. Sequential HTL experiments conducted have shown the prospect of recovering nutrients and other valuable byproducts along with biocrude oil. The experimental results and analysis indicate that sustainable biofuel production requires the development of strain based strategies for the hydrothermal liquefaction process. (C) 2016 Published by Elsevier Ltd. C1 [Reddy, Harvind Kumar; Muppaneni, Tapaswy; Ponnusamy, Sundaravadivelnathan; Deng, Shuguang] New Mexico State Univ, Dept Chem Engn, Las Cruces, NM 88003 USA. [Sudasinghe, Nilusha; Schaub, Tanner] New Mexico State Univ, Chem Anal & Instrumentat Lab, Las Cruces, NM 88003 USA. [Selvaratnam, Thinesh; Nirmalakhandan, Nagamany] New Mexico State Univ, Civil & Geol Engn, Las Cruces, NM 88003 USA. [Seger, Mark; Lammers, Peter] New Mexico State Univ, Energy Res Lab, Las Cruces, NM 88003 USA. [Voorhies, Wayne] New Mexico State Univ, Mol Biol, Las Cruces, NM 88003 USA. [Dungan, Barry; Holguin, F. Omar] New Mexico State Univ, Plant & Environm Sci, Las Cruces, NM 88003 USA. [Pegallapati, Ambica] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Deng, SG (reprint author), New Mexico State Univ, Dept Chem Engn, Las Cruces, NM 88003 USA. EM sdeng@nmsu.edu RI Deng, Shuguang/G-5926-2011 OI Deng, Shuguang/0000-0003-2892-3504 FU U.S. Department of Energy [DE-EE0003046, DE-EE0006316]; National Science Foundation [EEC-1028968, IIA-1301346] FX This project was partially supported by U.S. Department of Energy (DE-EE0003046, DE-EE0006316) and National Science Foundation (EEC-1028968, IIA-1301346). NR 39 TC 5 Z9 5 U1 13 U2 38 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD MAR 1 PY 2016 VL 165 BP 943 EP 951 DI 10.1016/j.apenergy.2015.11.067 PG 9 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DH3GV UT WOS:000372676400076 ER PT J AU Siriwardane, R Riley, J Tian, HJ Richards, G AF Siriwardane, Ranjani Riley, Jarrett Tian, Hanjing Richards, George TI Chemical looping coal gasification with calcium ferrite and barium ferrite via solid-solid reactions SO APPLIED ENERGY LA English DT Article DE Chemical looping coal gasification; Oxygen carriers for coal gasification; Steam gasification of coal with oxygen carriers ID SYNTHESIS GAS GENERATION; OXIDE OXYGEN CARRIERS; BIOMASS GASIFICATION; STEAM GASIFICATION; SYNGAS PRODUCTION; NATURAL HEMATITE; CO2 CAPTURE; COMBUSTION; HYDROGEN; METHANE AB Coal gasification to produce synthesis gas by chemical looping was investigated with two oxygen carriers, barium ferrite (BaFe2O4) and calcium ferrite (CaFe2O4). Thermo-gravimetric analysis (TGA) and fixed-bed flow reactor data indicated that a solid-solid interaction occurred between oxygen carriers and coal to produce synthesis gas. Both thermodynamic analysis and experimental data indicated that BaFe2O4 and CaFe2O4 have high reactivity with coal but have a low reactivity with synthesis gas, which makes them very attractive for the coal gasification process. Adding steam increased the production of hydrogen (H-2) and carbon monoxide (CO), but carbon dioxide (CO2) remained low because these oxygen carriers have minimal reactivity with H-2 and CO. Therefore, the combined steam-oxygen carrier produced the highest quantity of synthesis gas. It appeared that neither the water-gas shift reaction nor the water splitting reaction promoted additional H-2 formation with the oxygen carriers when steam was present. Wyodak coal, which is a sub-bituminous coal, had the best gasification yield with oxygen carrier-steam while Illinois #6 coal had the lowest. The rate of gasification and selectivity for synthesis gas production was significantly higher when these oxygen carriers were present during steam gasification of coal. The rates and synthesis gas yields during the temperature ramps of coal-steam with oxygen carriers were better than with gaseous oxygen. Published by Elsevier Ltd. C1 [Siriwardane, Ranjani; Riley, Jarrett; Tian, Hanjing; Richards, George] US DOE, Natl Energy Technol Lab, 3610 Collins Ferry Rd,POB 880, Morgantown, WV 26507 USA. [Riley, Jarrett; Tian, Hanjing] W Virginia Univ, Dept Chem Engn, Morgantown, WV 26505 USA. RP Siriwardane, R (reprint author), US DOE, Natl Energy Technol Lab, 3610 Collins Ferry Rd,POB 880, Morgantown, WV 26507 USA. EM ranjani.siriwardane@netl.doe.gov NR 60 TC 5 Z9 5 U1 11 U2 43 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD MAR 1 PY 2016 VL 165 BP 952 EP 966 DI 10.1016/j.apenergy.2015.12.085 PG 15 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DH3GV UT WOS:000372676400077 ER PT J AU Gohla, H Auer, M Cassette, P Hague, RK Lechermann, M Nadalut, B AF Gohla, H. Auer, M. Cassette, Ph. Hague, R. K. Lechermann, M. Nadalut, B. TI Radioxenon standards used in laboratory inter-comparisons SO APPLIED RADIATION AND ISOTOPES LA English DT Article; Proceedings Paper CT 20th International Conference on Radionuclide Metrology and its Applications (ICRM) CY JUN 08-12, 2015 CL TU Wien, Vienna, AUSTRIA SP Austrian Bundesamt Eich & Vermessungswesen, European Commiss, Joint Res Ctr Enlargement & Integrat Act, Univ Bodenkultur HO TU Wien DE Comprehensive Nuclear-Test-Ban Treaty (CTBT); International Monitoring System (IMS); Noble gas; Radioxenon standards; QA/QC program; Environmental monitoring; Xe-131m; Xe-133; Xe-133m; Xe-135; Xe-127 ID RADIOACTIVE XENON; XE-127 AB Preparation methods for Xe-133 standards of activity concentration and the results of the 2014 Xe-133 laboratory inter-comparison exercise are described. One element of the quality assurance/quality control (QA/QC) program for laboratories of the International Monitoring System (IMS) will be regular inter comparison exercises. However, until recently, no activity concentration standards for benchmarking were available. Therefore, two Xe-133 activity concentration reference standards were produced independently by Idaho National Laboratory and Seibersdorf Laboratories and used for the 2014 laboratory inter-comparison exercise. The preparation of a complementary Xe-127 activity concentration standard as well as a Xe-127 laboratory inter-comparison exercise suggests Xe-127 as a suitable isotope for QA/QC of remote IMS noble gas stations. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Gohla, H.; Auer, M.; Nadalut, B.] CIBTO Preparatory Commiss, Vienna, Austria. [Cassette, Ph.] Lab Natl Henri Becquerel, Lyon, France. [Hague, R. K.] Idaho Natl Lab, Idaho Falls, ID USA. [Lechermann, M.] Seibersdorf Labs, Seibersdorf, Austria. RP Gohla, H (reprint author), CIBTO Preparatory Commiss, Vienna, Austria. EM herbert.gohla@ctbto.org OI Cassette, Philippe/0000-0001-5254-9183 NR 19 TC 0 Z9 0 U1 0 U2 1 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0969-8043 J9 APPL RADIAT ISOTOPES JI Appl. Radiat. Isot. PD MAR PY 2016 VL 109 BP 24 EP 29 DI 10.1016/j.apradiso.2015.11.044 PG 6 WC Chemistry, Inorganic & Nuclear; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging SC Chemistry; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging GA DH3GX UT WOS:000372676600006 PM 26682890 ER PT J AU Williams, RM Aalseth, CE Bowyer, TW Day, AR Fuller, ES Haas, DA Hayes, JC Hoppe, EW Humble, PH Keillor, ME LaFerriere, BD Mace, EK McIntyre, JI Miley, HS Myers, AW Orrell, JL Overman, CT Panisko, ME Seifert, A AF Williams, R. M. Aalseth, C. E. Bowyer, T. W. Day, A. R. Fuller, E. S. Haas, D. A. Hayes, J. C. Hoppe, E. W. Humble, P. H. Keillor, M. E. LaFerriere, B. D. Mace, E. K. McIntyre, J. I. Miley, H. S. Myers, A. W. Orrell, J. L. Overman, C. T. Panisko, M. E. Seifert, A. TI Development of a low-level Ar-37 calibration standard SO APPLIED RADIATION AND ISOTOPES LA English DT Article; Proceedings Paper CT 20th International Conference on Radionuclide Metrology and its Applications (ICRM) CY JUN 08-12, 2015 CL TU Wien, Vienna, AUSTRIA SP Austrian Bundesamt Eich & Vermessungswesen, European Commiss, Joint Res Ctr Enlargement & Integrat Act, Univ Bodenkultur HO TU Wien DE Absolute radiation measurement; Length compensated proportional counting; Ultra low-background; Electroformed copper; Uncertainty analysis ID INITIAL-CHARACTERIZATION; GAS; SYSTEM AB Argon-37 is an environmental signature of an underground nuclear explosion. Producing and quantifying low-level Ar-37 standards is an important step in the development of sensitive field measurement instruments. This paper describes progress at Pacific Northwest National Laboratory in developing a process to generate and quantify low-level Ar-37 standards, which can be used to calibrate sensitive field systems at activities consistent with soil background levels. This paper presents a discussion of the measurement analysis, along with assumptions and uncertainty estimates. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Williams, R. M.; Aalseth, C. E.; Bowyer, T. W.; Day, A. R.; Fuller, E. S.; Haas, D. A.; Hayes, J. C.; Hoppe, E. W.; Humble, P. H.; Keillor, M. E.; LaFerriere, B. D.; Mace, E. K.; McIntyre, J. I.; Miley, H. S.; Myers, A. W.; Orrell, J. L.; Overman, C. T.; Panisko, M. E.; Seifert, A.] Pacific NW Natl Lab, POB 999, Richland, WA 99352 USA. RP Williams, RM (reprint author), Pacific NW Natl Lab, POB 999, Richland, WA 99352 USA. EM Richard.Williams@pnnl.gov RI McIntyre, Justin/P-1346-2014; Humble, Paul/K-1961-2012; Orrell, John/E-9313-2015 OI McIntyre, Justin/0000-0002-3706-4310; Humble, Paul/0000-0002-2632-6557; Orrell, John/0000-0001-7968-4051 NR 16 TC 1 Z9 1 U1 0 U2 4 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0969-8043 J9 APPL RADIAT ISOTOPES JI Appl. Radiat. Isot. PD MAR PY 2016 VL 109 BP 430 EP 434 DI 10.1016/j.apradiso.2015.12.027 PG 5 WC Chemistry, Inorganic & Nuclear; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging SC Chemistry; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging GA DH3GX UT WOS:000372676600091 PM 26701655 ER PT J AU van Weeren, RJ Williams, WL Hardcastle, MJ Shimwell, TW Rafferty, DA Sabater, J Heald, G Sridhar, SS Dijkema, TJ Brunetti, G Bruggen, M Andrade-Santos, F Ogrean, GA Rottgering, HJA Dawson, WA Forman, WR de Gasperin, F Jones, C Miley, UK Rudnick, L Sarazin, CL Bonafede, A Best, PN Birzan, L Cassano, R Chyzy, KT Croston, JH Ensslin, T Ferrari, C Hoeft, M Horellou, C Jarvis, MJ Kraft, RP Mevius, M Intema, HT Murray, SS Orru, E Pizzo, R Simionescu, A Stroe, A van der Tol, S White, GJ AF van Weeren, R. J. Williams, W. L. Hardcastle, M. J. Shimwell, T. W. Rafferty, D. A. Sabater, J. Heald, G. Sridhar, S. S. Dijkema, T. J. Brunetti, G. Brueggen, M. Andrade-Santos, F. Ogrean, G. A. Roettgering, H. J. A. Dawson, W. A. Forman, W. R. de Gasperin, F. Jones, C. Miley, U. K. Rudnick, L. Sarazin, C. L. Bonafede, A. Best, P. N. Birzan, L. Cassano, R. Chyzy, K. T. Croston, J. H. Ensslin, T. Ferrari, C. Hoeft, M. Horellou, C. Jarvis, M. J. Kraft, R. P. Mevius, M. Intema, H. T. Murray, S. S. Orru, E. Pizzo, R. Simionescu, A. Stroe, A. van der Tol, S. White, G. J. TI LOFAR FACET CALIBRATION SO ASTROPHYSICAL JOURNAL SUPPLEMENT SERIES LA English DT Article DE techniques: interferometric ID RADIO INTERFEROMETRIC CALIBRATION; WIDE-FIELD; GAIN CALIBRATION; SELF-CALIBRATION; W-PROJECTION; SKY SURVEY; ALGORITHM; I.; ASTRONOMY; SYSTEM AB LOFAR, the Low-Frequency Array, is a powerful new radio telescope operating between 10 and 240 MHz. LOFAR allows detailed sensitive high-resolution studies of the low-frequency radio sky. At the same time LOFAR also provides excellent short baseline coverage to map diffuse extended emission. However, producing highquality deep images is challenging due to the presence of direction-dependent calibration errors, caused by imperfect knowledge of the station beam shapes and the ionosphere. Furthermore, the large data volume and presence of station clock errors present additional difficulties. In this paper we present a new calibration scheme, which we name facet calibration, to obtain deep high-resolution LOFAR High Band Antenna images using the Dutch part of the array. This scheme solves and corrects the direction-dependent errors in a number of facets that cover the observed field of view. Facet calibration provides close to thermal noise limited images for a typical 8 hr observing run at similar to 5. resolution, meeting the specifications of the LOFAR Tier-1 northern survey. C1 [van Weeren, R. J.; Andrade-Santos, F.; Ogrean, G. A.; Forman, W. R.; Jones, C.; Kraft, R. P.; Murray, S. S.] Harvard Smithsonian Ctr Astrophys, 60 Garden St, Cambridge, MA 02138 USA. [Williams, W. L.; Shimwell, T. W.; Roettgering, H. J. A.; de Gasperin, F.; Miley, U. K.; Stroe, A.] Leiden Univ, Leiden Observ, POB 9513, NL-2300 RA Leiden, Netherlands. [Williams, W. L.; Heald, G.; Sridhar, S. S.; Dijkema, T. J.; Mevius, M.; Orru, E.; Pizzo, R.; van der Tol, S.] Netherlands Inst Radio Astron, ASTRON, Postbus 2, NL-7990 AA Dwingeloo, Netherlands. [Williams, W. L.; Hardcastle, M. J.] Univ Hertfordshire, Sch Phys Astron & Math, Coll Lane, Hatfield AL10 9AB, Herts, England. [Rafferty, D. A.; Brueggen, M.; de Gasperin, F.; Bonafede, A.; Birzan, L.] Hamburger Sternwarte, Gojenbergsweg 112, D-21029 Hamburg, Germany. [Sabater, J.; Best, P. N.] Royal Observ, Univ Edinburgh, Inst Astron, Blackford Hill, Edinburgh EH9 3HJ, Midlothian, Scotland. [Heald, G.; Sridhar, S. S.] Univ Groningen, Kapteyn Astron Inst, POB 800, NL-9700 AV Groningen, Netherlands. [Brunetti, G.; Cassano, R.] INAF, Ist Radioastron, Via Gobetti 101, I-40129 Bologna, Italy. [Dawson, W. A.] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. [Rudnick, L.] Univ Minnesota, Minnesota Inst Astrophys, 116 Church St SE, Minneapolis, MN 55455 USA. [Sarazin, C. L.] Univ Virginia, Dept Astron, Charlottesville, VA 22904 USA. [Chyzy, K. T.] Jagiellonian Univ, Astron Observ, Ul Orla 171, PL-30244 Krakow, Poland. [Croston, J. H.] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. [Ensslin, T.] Max Planck Inst Astrophys, Karl Schwarzschildstr 1, D-85741 Garching, Germany. [Ferrari, C.] Univ Cote Azur, Observ Cote Azur, CNRS, Lab Lagrange, Blvd Observ,CS 34229, F-06304 Nice 4, France. [Hoeft, M.] Thuringer Landessternwarte Tautenburg, Sternwarte 5, D-07778 Tautenburg, Germany. [Horellou, C.] Chalmers, Onsala Space Observ, Dept Earth & Space Sci, SE-43992 Onsala, Sweden. [Jarvis, M. J.] Oxford Astrophys, Dept Phys, Keble Rd, Oxford OX1 3RH, England. [Jarvis, M. J.] Univ Western Cape, ZA-7535 Bellville, South Africa. [Intema, H. T.] Natl Radio Astron Observ, 1003 Lopezville Rd, Socorro, NM 87801 USA. [Murray, S. S.] Johns Hopkins Univ, Dept Phys & Astron, 3400 North Charles St, Baltimore, MD 21218 USA. [Simionescu, A.] JAXA, ISAS, Chuo Ku, 3-1-1 Yoshinodai, Sagamihara, Kanagawa 2525210, Japan. [White, G. J.] Open Univ, Dept Phys Sci, Walton Hall, Milton Keynes MK7 6AA, Bucks, England. [White, G. J.] Rutherford Appleton Lab, RALSpace, Didcot OX11 0NL, Oxon, England. RP van Weeren, RJ (reprint author), Harvard Smithsonian Ctr Astrophys, 60 Garden St, Cambridge, MA 02138 USA. EM rvanweeren@cfa.harvard.edu RI Intema, Huib/D-1438-2012; OI Intema, Huib/0000-0002-5880-2730; Seethapuram Sridhar, Sarrvesh/0000-0002-7587-4779; Hardcastle, Martin/0000-0003-4223-1117; Sabater, Jose/0000-0003-1149-6294; van Weeren, Reinout/0000-0002-0587-1660 FU NASA through the Einstein Postdoctoral grant [PF2-130104]; NASA [NAS8-03060, NAS5-26555]; National Aeronautics and Space Administration through Chandra Award [GO3-14138X]; National Aeronautics Space Administration [NAS8-03060]; NASA through a Hubble Fellowship - Space Telescope Science Institute [HST-HF2-51345.001-A]; Alexander von Humboldt Foundation; PRIN-INAF; Smithsonian Institution; Agence Nationale pour la Recherche, MAGEL-LAN project [ANR-14-CE23-0004-01]; NSF [AST-1211595]; U.S. DOE by LLNL [DE-AC52-07NA27344]; [G03-14131X] FX We would like to thank the anonymous referee for useful comments. R.J.W. was supported by NASA through the Einstein Postdoctoral grant number PF2-130104 awarded by the Chandra X-ray Center, which is operated by the Smithsonian Astrophysical Observatory for NASA under contract NAS8-03060. Support for this work was provided by the National Aeronautics and Space Administration through Chandra Award Number GO3-14138X, issued by the Chandra X-ray Observatory Center, which is operated by the Smithsonian Astrophysical Observatory for and on behalf of the National Aeronautics Space Administration under contract NAS8-03060. G.A.O. acknowledges support by NASA through a Hubble Fellowship grant HST-HF2-51345.001-A awarded by the Space Telescope Science Institute, which is operated by the Association of Universities for Research in Astronomy, Incorporated, under NASA contract NAS5-26555. G.B. acknowledges support from the Alexander von Humboldt Foundation. G. B. and R.C. acknowledge support from PRIN-INAF 2014. W.R.F., C.J., and F.A.-S. acknowledge support from the Smithsonian Institution. F.A.-S. acknowledges support from Chandra grant G03-14131X. C.F. acknowledges support by the Agence Nationale pour la Recherche, MAGEL-LAN project, ANR-14-CE23-0004-01. Partial support for L.R. is provided by NSF Grant AST-1211595 to the University of Minnesota. Part of this work performed under the auspices of the U.S. DOE by LLNL under Contract DE-AC52-07NA27344. LOFAR, the Low Frequency Array designed and constructed by ASTRON, has facilities in several countries that are owned by various parties (each with their own funding sources), and that are collectively operated by the International LOFAR Telescope (ILT) foundation under a joint scientific policy. We thank the staff of the GMRT that made these observations possible. GMRT is run by the National Centre for Radio Astrophysics of the Tata Institute of Fundamental Research. The Open University is incorporated by Royal Charter (RC 000391), an exempt charity in England & Wales and a charity registered in Scotland (SC 038302). The Open University is authorized and regulated by the Financial Conduct Authority. NR 45 TC 8 Z9 8 U1 2 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0067-0049 EI 1538-4365 J9 ASTROPHYS J SUPPL S JI Astrophys. J. Suppl. Ser. PD MAR PY 2016 VL 223 IS 1 AR 2 DI 10.3847/0067-0049/223/1/2 PG 16 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DI0TB UT WOS:000373208900002 ER PT J AU Reed, S Lau, G Delattre, B Lopez, DD Tomsia, AP Wu, BM AF Reed, Stephanie Lau, Grace Delattre, Benjamin Lopez, David Don Tomsia, Antoni P. Wu, Benjamin M. TI Macro- and micro-designed chitosan-alginate scaffold architecture by three-dimensional printing and directional freezing SO BIOFABRICATION LA English DT Article DE 3D printing; directional freezing; cartilage regeneration; acellular scaffold; channeled architecture; native cell uptake; zonal cartilage ID TISSUE-ENGINEERING SCAFFOLDS; MESENCHYMAL STEM-CELLS; ARTICULAR-CARTILAGE; PORE-SIZE; OSTEOCHONDRAL DEFECTS; BIPHASIC SCAFFOLD; RABBIT MODEL; REPAIR; REGENERATION; CHONDROGENESIS AB While many tissue-engineered constructs aim to treat cartilage defects, most involve chondrocyte or stem cell seeding on scaffolds. The clinical application of cell-based techniques is limited due to the cost of maintaining cellular constructs on the shelf, potential immune response to allogeneic cell lines, and autologous chondrocyte sources requiring biopsy from already diseased or injured, scarce tissue. An acellular scaffold that can induce endogenous influx and homogeneous distribution of native stem cells from bone marrow holds great promise for cartilage regeneration. This study aims to develop such an acellular scaffold using designed, channeled architecture that simultaneously models the native zones of articular cartilage and subchondral bone. Highly porous, hydrophilic chitosan-alginate (Ch-Al) scaffolds were fabricated in three-dimensionally printed (3DP) molds designed to create millimeter scale macro-channels. Different polymer preform casting techniques were employed to produce scaffolds from both negative and positive 3DP molds. Macro-channeled scaffolds improved cell suspension distribution and uptake overly randomly porous scaffolds, with a wicking volumetric flow rate of 445.6 +/- 30.3 mm(3) s(-1) for aqueous solutions and 177 +/- 16 mm(3) s(-1) for blood. Additionally, directional freezing was applied to Ch-Al scaffolds, resulting in lamellar pores measuring 300 mu m and 50 mu m the long and short axes, thus creating micrometer scale micro- channels. After directionally freezing Ch-Al solution cast in 3DP molds, the combined macro-and micro-channeled scaffold architecture enhanced cell suspension uptake beyond either macro- or micro-channels alone, reaching a volumetric flow rate of 1782.1 +/- 48 mm(3) s(-1) for aqueous solutions and 440.9 +/- 0.5 mm(3) s(-1) for blood. By combining 3DP and directional freezing, we can control the micro-and macro-architecture of Ch-Al to drastically improve cell influx into and distribution within the scaffold, while achieving porous zones that mimic articular cartilage zonal architecture. In future applications, precisely controlled micro-and macro-channels have the potential to assist immediate endogenous bone marrow uptake, stimulate chondrogenesis, and encourage vascularization of bone in an osteochondral scaffold. C1 [Reed, Stephanie; Wu, Benjamin M.] Univ Calif Los Angeles, Dept Bioengn, Los Angeles, CA USA. [Lau, Grace; Delattre, Benjamin; Lopez, David Don; Tomsia, Antoni P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Wu, Benjamin M.] Univ Calif Los Angeles, Div Adv Prosthodont, Los Angeles, CA USA. RP Wu, BM (reprint author), Univ Calif Los Angeles, Dept Bioengn, Los Angeles, CA USA.; Wu, BM (reprint author), Univ Calif Los Angeles, Div Adv Prosthodont, Los Angeles, CA USA. EM benwu@ucla.edu NR 66 TC 1 Z9 1 U1 20 U2 61 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1758-5082 EI 1758-5090 J9 BIOFABRICATION JI Biofabrication PD MAR PY 2016 VL 8 IS 1 AR 015003 DI 10.1088/1758-5090/8/1/015003 PG 16 WC Engineering, Biomedical; Materials Science, Biomaterials SC Engineering; Materials Science GA DI1WZ UT WOS:000373289000007 PM 26741113 ER PT J AU Gorczynska, I Migacz, JV Zawadzki, RJ Capps, AG Werner, JS AF Gorczynska, Iwona Migacz, Justin V. Zawadzki, Robert J. Capps, Arlie G. Werner, John S. TI Comparison of amplitude-decorrelation, speckle-variance and phase-variance OCT angiography methods for imaging the human retina and choroid SO BIOMEDICAL OPTICS EXPRESS LA English DT Article ID OPTICAL COHERENCE TOMOGRAPHY; LIVING HUMAN EYE; SWEPT-SOURCE; BLOOD-FLOW; MOTION-CORRECTION; HIGH-SPEED; TRACKING SLO; 1060 NM; DOPPLER; MICROVASCULATURE AB We compared the performance of three OCT angiography (OCTA) methods: speckle variance, amplitude decorrelation and phase variance for imaging of the human retina and choroid. Two averaging methods, split spectrum and volume averaging, were compared to assess the quality of the OCTA vascular images. All data were acquired using a swept-source OCT system at 1040 nm central wavelength, operating at 100,000 A-scans/s. We performed a quantitative comparison using a contrast-to-noise (CNR) metric to assess the capability of the three methods to visualize the choriocapillaris layer. For evaluation of the static tissue noise suppression in OCTA images we proposed to calculate CNR between the photoreceptor/RPE complex and the choriocapillaris layer. Finally, we demonstrated that implementation of intensity-based OCT imaging and OCT angiography methods allows for visualization of retinal and choroidal vascular layers known from anatomic studies in retinal preparations. OCT projection imaging of data flattened to selected retinal layers was implemented to visualize retinal and choroidal vasculature. User guided vessel tracing was applied to segment the retinal vasculature. The results were visualized in a form of a skeletonized 3D model. (C) 2016 Optical Society of America C1 [Gorczynska, Iwona; Migacz, Justin V.; Zawadzki, Robert J.; Capps, Arlie G.; Werner, John S.] Univ Calif Davis, Dept Ophthalmol & Vis Sci, Sacramento, CA 95817 USA. [Gorczynska, Iwona] Nicholas Copernicus Univ, Fac Phys Astron & Informat, PL-87100 Torun, Poland. [Capps, Arlie G.] Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94550 USA. RP Gorczynska, I (reprint author), Univ Calif Davis, Dept Ophthalmol & Vis Sci, Sacramento, CA 95817 USA.; Gorczynska, I (reprint author), Nicholas Copernicus Univ, Fac Phys Astron & Informat, PL-87100 Torun, Poland. EM imgorczynska@ucdavis.edu RI Gorczynska, Iwona/P-9367-2015; OI Gorczynska, Iwona/0000-0002-6120-8791; Zawadzki, Robert/0000-0002-9574-156X FU National Institutes of Health, National Eye Institute [R01 EY024239, EY012576]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344, LLNL-JRNL-680059] FX This work was supported by grants from the National Institutes of Health, National Eye Institute R01 EY024239 and EY012576. This work was performed, in part, under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. LLNL-JRNL-680059. We gratefully acknowledge UC Davis VSRI laboratory members: Ravi Jonnal and Kyle Mc Dermott for valuable discussions during the work on this study, and Susan Garcia for help with subject recruitment and testing. NR 92 TC 15 Z9 15 U1 9 U2 14 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 2156-7085 J9 BIOMED OPT EXPRESS JI Biomed. Opt. Express PD MAR 1 PY 2016 VL 7 IS 3 BP 911 EP 942 DI 10.1364/BOE.7.000911 PG 32 WC Biochemical Research Methods; Optics; Radiology, Nuclear Medicine & Medical Imaging SC Biochemistry & Molecular Biology; Optics; Radiology, Nuclear Medicine & Medical Imaging GA DG4JR UT WOS:000372039000016 PM 27231598 ER PT J AU Ou, LW Li, BY Dang, Q Jones, S Brown, R Wright, MM AF Ou, Longwen Li, Boyan Dang, Qi Jones, Susanne Brown, Robert Wright, Mark M. TI Understanding Uncertainties in the Economic Feasibility of Transportation Fuel Production using Biomass Gasification and Mixed Alcohol Synthesis SO ENERGY TECHNOLOGY LA English DT Article DE biomass; ethanol; fuels; techno-economic analysis; uncertainty analysis ID CELLULOSIC BIOFUEL PATHWAYS; TECHNOECONOMIC ANALYSIS; CATALYTIC PYROLYSIS; HYDROTHERMAL LIQUEFACTION; LIGNOCELLULOSIC BIOMASS; MICROALGAE; ETHANOL; TECHNOLOGIES; HYBRID; ENERGY AB This study evaluates uncertainties in the techno-economic analysis of transportation fuel production from biomass gasification and mixed alcohol synthesis. Two scenarios are considered: a state-of-technology scenario and a target scenario with projected technological advances. Uncertainties of more than 10parameters are investigated. The probability distributions of these parameters are estimated based on historical price data and experimental data. Data samples generated from the corresponding distribution are then utilized to run a MonteCarlo simulation. The results yield minimum fuel-selling prices of $1.85L(-1) with a standard deviation of 0.13 for the state-of-technology scenario and $1.14L(-1) with a standard deviation of 0.11 for the target scenario, respectively. The feedstock price and internal rate of return (IRR) have significant impacts on the minimum fuel-selling price in both scenarios. These findings are indicative of the reduction in biofuel cost and uncertainty achievable with increasing technology maturity. C1 [Ou, Longwen; Li, Boyan; Dang, Qi; Brown, Robert; Wright, Mark M.] Iowa State Univ, Dept Mech Engn, Ames, IA 50010 USA. [Dang, Qi; Brown, Robert; Wright, Mark M.] Iowa State Univ, Bioecon Inst, Ames, IA 50012 USA. [Jones, Susanne] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Wright, MM (reprint author), Iowa State Univ, Dept Mech Engn, Ames, IA 50010 USA.; Wright, MM (reprint author), Iowa State Univ, Bioecon Inst, Ames, IA 50012 USA. EM markmw@iastate.edu FU U.S. Department of Energy through Bioenergy Technologies Office (BETO) [4042514] FX The authors acknowledge the support for this research provided by the U.S. Department of Energy through its Bioenergy Technologies Office (BETO) (Grant Number 4042514). NR 35 TC 2 Z9 2 U1 4 U2 11 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 2194-4288 EI 2194-4296 J9 ENERGY TECHNOL-GER JI Energy Technol. PD MAR PY 2016 VL 4 IS 3 BP 441 EP 448 DI 10.1002/ente.201500367 PG 8 WC Energy & Fuels SC Energy & Fuels GA DH9IR UT WOS:000373110300012 ER PT J AU Studt, L Janevska, S Niehaus, EM Burkhardt, I Arndt, B Sieber, CMK Humpf, HU Dickschat, JS Tudzynski, B AF Studt, Lena Janevska, Slavica Niehaus, Eva-Maria Burkhardt, Immo Arndt, Birgit Sieber, Christian M. K. Humpf, Hans-Ulrich Dickschat, Jeroen S. Tudzynski, Bettina TI Two separate key enzymes and two pathway-specific transcription factors are involved in fusaric acid biosynthesis in Fusarium fujikuroi SO ENVIRONMENTAL MICROBIOLOGY LA English DT Article ID NONRIBOSOMAL PEPTIDE-SYNTHESIS; CYTOCHROME P450 REDUCTASE; F-SP VASINFECTUM; GIBBERELLA-FUJIKUROI; GENE-CLUSTER; ASPERGILLUS-FUMIGATUS; SECONDARY METABOLISM; SACCHAROMYCES-CEREVISIAE; MASS-SPECTROMETRY; TRANSPORTER GENE AB Fusaric acid (FSA) is a mycotoxin produced by several fusaria, including the rice pathogen Fusarium fujikuroi. Genes involved in FSA biosynthesis were previously identified as a cluster containing a polyketide synthase (PKS)-encoding (FUB1) and four additional genes (FUB2-FUB5). However, the biosynthetic steps leading to FSA as well as the origin of the nitrogen atom, which is incorporated into the polyketide backbone, remained unknown. In this study, seven additional cluster genes (FUB6-FUB12) were identified via manipulation of the global regulator FfSge1. The extended FUB gene cluster encodes two Zn(II)(2)Cys(6) transcription factors: Fub10 positively regulates expression of all FUB genes, whereas Fub12 is involved in the formation of the two FSA derivatives, i.e. dehydrofusaric acid and fusarinolic acid, serving as a detoxification mechanism. The major facilitator superfamily transporter Fub11 functions in the export of FSA out of the cell and is essential when FSA levels become critical. Next to Fub1, a second key enzyme was identified, the non-canonical non-ribosomal peptide synthetase Fub8. Chemical analyses of generated mutant strains allowed for the identification of a triketide as PKS product and the proposition of an FSA biosynthetic pathway, thereby unravelling the unique formation of a hybrid metabolite consisting of this triketide and an amino acid moiety. C1 [Studt, Lena; Janevska, Slavica; Niehaus, Eva-Maria; Tudzynski, Bettina] Univ Munster, Inst Plant Biol & Biotechnol, Schlosspl 8, D-48143 Munster, Germany. [Burkhardt, Immo; Dickschat, Jeroen S.] Univ Bonn, Kekule Inst Organ Chem & Biochem, D-53121 Bonn, Germany. [Arndt, Birgit; Humpf, Hans-Ulrich] Univ Munster, Inst Food Chem, Corrensstr 45, D-48149 Munster, Germany. [Sieber, Christian M. K.] Lawrence Berkeley Natl Lab, DOE Joint Genome Inst, 2800 Mitchell Dr, Walnut Creek, CA 94598 USA. [Studt, Lena] BOKU Univ Nat Resources & Life Sci, Dept Appl Genet & Cell Biol, Fungal Genet & Genom Unit, Campus Tulln, A-3430 Tulln, Austria. RP Tudzynski, B (reprint author), Univ Munster, Inst Plant Biol & Biotechnol, Schlosspl 8, D-48143 Munster, Germany. EM bettina.tudzynski@uni-muenster.de FU German Research Foundation [TU101/16-2, HU 730/9-3] FX We thank Kathleen Huss for excellent technical assistance. We are particularly grateful to Brian Williamson for critical reading of this manuscript. The project was funded by the German Research Foundation (project numbers TU101/16-2 and HU 730/9-3). We declare that no conflict of interest exists. NR 73 TC 8 Z9 8 U1 16 U2 26 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1462-2912 EI 1462-2920 J9 ENVIRON MICROBIOL JI Environ. Microbiol. PD MAR PY 2016 VL 18 IS 3 SI SI BP 936 EP 956 DI 10.1111/1462-2920.13150 PG 21 WC Microbiology SC Microbiology GA DH7HV UT WOS:000372964800015 PM 26662839 ER PT J AU Lai, Y Veser, G AF Lai, Yungchieh Veser, Goetz TI Zn-HZSM-5 catalysts for methane dehydroaromatization SO ENVIRONMENTAL PROGRESS & SUSTAINABLE ENERGY LA English DT Article DE methane dehydroaromatization; non-oxidative aromatization; ZSM-5; zeolites; zinc ID PROMOTED H-ZSM-5 CATALYSTS; ZSM-5 ZEOLITES; ACID SITES; W/HZSM-5-BASED CATALYSTS; PROPANE AROMATIZATION; CONVERSION; BENZENE; ZN; DEHYDROGENATION; AROMATICS AB The nature of the active species in Zn-containing HZSM-5 catalysts was investigated by preparing Zn-HZSM-5 via three different synthetic approaches: wet ion exchange, wet impregnation, and core-shell synthesis. By investigating the impact of the preparation methods on the distribution of Zn species, and studying the catalytic performance of the resulting materials in methane dehydroaromatization (DHA), it was shown that metallic Zn-0 nanoclusters inside the zeolite micropore constituted the most active species for DHA, but get irreversible loss from the catalyst via evaporation at the high-temperature conditions of DHA. In contrast, Zn2+ anchored at the exchange sites of the zeolite were the most stable species, but provided little to no aromatization activity. As a result, and counter to previous reports in the literature, it was concluded that Zn/HZSM-5 was not a suitable catalyst for non-oxidative methane dehydroaromatization. Nonetheless, the study confirmed that well-dispersed metal species inside the zeolitic micropores were critical for aromatization activity of zeolite-based catalysts. (c) 2016 American Institute of Chemical Engineers Environ Prog, 35: 334-344, 2016 C1 [Lai, Yungchieh; Veser, Goetz] US DOE, Natl Energy Technol Lab, Pittsburgh, PA USA. [Lai, Yungchieh; Veser, Goetz] Univ Pittsburgh, Dept Chem Engn, Swanson Sch Engn, Pittsburgh, PA 15261 USA. [Lai, Yungchieh; Veser, Goetz] Univ Pittsburgh, Ctr Energy, Pittsburgh, PA USA. RP Veser, G (reprint author), US DOE, Natl Energy Technol Lab, Pittsburgh, PA USA.; Veser, G (reprint author), Univ Pittsburgh, Dept Chem Engn, Swanson Sch Engn, Pittsburgh, PA 15261 USA.; Veser, G (reprint author), Univ Pittsburgh, Ctr Energy, Pittsburgh, PA USA. EM gveser@pitt.edu FU U.S. Department of Energy's National Energy Technology Laboratory under the RDS [DE-AC26-04NT41817]; University of Pittsburgh's Center for Energy FX This technical effort was in parts performed in support of the U.S. Department of Energy's National Energy Technology Laboratory under the RDS contract DE-AC26-04NT41817. Furthermore, financial support by the University of Pittsburgh's Center for Energy through a R. K. Mellon fellowship (YL) is gratefully acknowledged. Finally, the authors would like to thank Drs D. Shekhawat, S. Natesakhawat, and V. Abdel-Sayed for their assistance with micropore and NH3-TPD analysis. NR 32 TC 1 Z9 1 U1 22 U2 60 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1944-7442 EI 1944-7450 J9 ENVIRON PROG SUSTAIN JI Environ. Prog. Sustain. Energy PD MAR-APR PY 2016 VL 35 IS 2 BP 334 EP 344 DI 10.1002/ep.12322 PG 11 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Engineering, Environmental; Engineering, Chemical; Engineering, Industrial; Environmental Sciences SC Science & Technology - Other Topics; Engineering; Environmental Sciences & Ecology GA DH7KP UT WOS:000372972900003 ER PT J AU Escuer, A Cordero, B Font-Bardia, M Teat, SJ Roubeau, O AF Escuer, Albert Cordero, Beatriz Font-Bardia, Merce Teat, Simon J. Roubeau, Olivier TI Manganese-Salicyloximate Clusters Starting from [Mn-II(hfacac)(2)]: From Mn-4 to Mn-12 SO EUROPEAN JOURNAL OF INORGANIC CHEMISTRY LA English DT Article DE Cluster compounds; Magnetic properties; Manganese; N; O ligands ID SINGLE-MOLECULE MAGNETS; TARGETED STRUCTURAL DISTORTION; CARBOXYLATO COMPLEXES; ENERGY BARRIER; SMM PROPERTIES; HEXANUCLEAR; FAMILY; ANISOTROPY; SALICYLALDOXIME; METALLACROWNS AB The systematic exploration of the reactivity of [Mn(hfacac)(2)] with R-salicyloximes (R-saloxH(2): R = H, Me, Et) yielded a family of clusters with nuclearities ranging from Mn-4 to Mn-12. The compounds with formula [Mn-6(O)(2)(salox)(6)(CF3COO)(2)(EtOH)(4)] (1) and [Mn-12(salox)(12)(O)(4)(N-3)(4)(H2O)(2)(MeOH)(6)] (4) show two or four linked {Mn(mu(3)-O)(salox)(3)}(+) triangular subunits. Magnetic measurements revealed spin ground states of S = 4 for 1 and S = 8 for 4, as well as single-molecule magnet responses and magnetic hysteresis above 2 K. The cubic [Mn-4(Mesalox)(4)(MesaloxH)(4)] (2), the hexanuclear [Mn-6(Etsalox)(6)(O)(2)(MeO)(4)(MeOH)(2)] (3) and the octanuclear [Mn-8(Mesalox)(6)(O)(2)(N-3)(6)(MeOH)(8)] (5) are polymorphs of previously reported systems. Small structural changes allows an S = 11 ground state for 3. C1 [Escuer, Albert; Cordero, Beatriz] Univ Barcelona, Dept Quim Inorgan, Av Diagonal 645, E-08028 Barcelona, Spain. [Escuer, Albert; Cordero, Beatriz] Univ Barcelona, Inst Nanociencia & Nanotecnol IN2UB, Av Diagonal 645, E-08028 Barcelona, Spain. [Font-Bardia, Merce] Univ Barcelona, Dept Cristallog Mineral & Diposits Minerals, Marti Franques S-N, E-08028 Barcelona, Spain. [Teat, Simon J.] Berkeley Lab, Adv Light Source, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Roubeau, Olivier] Univ Zaragoza, CSIC, ICMA, Pl San Francisco S-N, E-50009 Zaragoza, Spain. RP Escuer, A (reprint author), Univ Barcelona, Dept Quim Inorgan, Av Diagonal 645, E-08028 Barcelona, Spain.; Escuer, A (reprint author), Univ Barcelona, Inst Nanociencia & Nanotecnol IN2UB, Av Diagonal 645, E-08028 Barcelona, Spain. EM albert.escuer@ub.edu RI Roubeau, Olivier/A-6839-2010; Escuer, Albert/L-4706-2014 OI Roubeau, Olivier/0000-0003-2095-5843; Escuer, Albert/0000-0002-6274-6866 FU Centro de Investigacion Cientifica y Tecnologica (CICYT) [CTQ2015-63614-P]; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Centro de Investigacion Cientifica y Tecnologica (CICYT) (project number CTQ2015-63614-P). The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy (contract number DE-AC02-05CH11231). NR 67 TC 3 Z9 3 U1 3 U2 7 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1434-1948 EI 1099-0682 J9 EUR J INORG CHEM JI Eur. J. Inorg. Chem. PD MAR PY 2016 IS 8 BP 1232 EP 1241 DI 10.1002/ejic.201501372 PG 10 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DH2ZZ UT WOS:000372657700012 ER PT J AU Egbert, JD Labios, LA Darmon, JM Piro, NA Kassel, WS Mock, MT AF Egbert, Jonathan D. Labios, Liezel A. Darmon, Jonathan M. Piro, Nicholas A. Kassel, W. Scott Mock, Michael T. TI Synthesis and Structure of Vanadium Halide Complexes Containing Diphosphine Ligands with Pendant Amines SO EUROPEAN JOURNAL OF INORGANIC CHEMISTRY LA English DT Article DE Vanadium; Phosphane ligands; Cyclopentadienyl ligands; Amines; Proton transport ID ELECTROCATALYTIC OXIDATION; MOLECULAR ELECTROCATALYST; HETEROLYTIC CLEAVAGE; COORDINATION SPHERE; PHOSPHINE COMPLEXES; HYDROGEN; MOLYBDENUM; BASE; H-2 AB A series of vanadium(III) diiodide complexes of the formula CpV((PNPR)-N-R-P-R)I-2 [Cp = (5)-C5H5; (PNPR)-N-R-P-R = (R2PCH2)(2)N(R); R = Et, R = Me (1a); R = Et, R = Ph (1b); R = Ph, R = Me (1c)] is reported. The corresponding vanadium(II) monoiodide complexes of the formula CpV((PNPR)-N-R-P-R)I [R = Et, R = Me (2a); R = Et, R = Ph (2b); R = Ph, R = Me (2c)] were prepared in THF by reduction of 1a-c with Zn powder. We report the preparation of the vanadium(II) complexes CpV((P2N2Ph)-N-Ph)I (3) ((P2N2Ph)-N-Ph = 1,3,5,7-tetraphenyl-1,5-diaza-3,7-diphosphacyclooctane) as well as trans-[VCl2((PNPEt)-N-Et-P-Me)(2)] (4a) and trans-[VCl2((PNPEt)-N-Et-P-Ph)(2)] (4b). These paramagnetic complexes are characterized by elemental analysis, H-1 NMR spectroscopy, and cyclic voltammetry for 2a, 2b, 3 and 4b. Complexes 1c, 2a-c, 3, and 4b were also characterized by single-crystal X-ray crystallography. These complexes represent initial examples for the coordination chemistry of vanadium with (PNPR)-N-R-P-R and (P2N2Ph)-N-Ph diphosphine ligands, which contain a pendant amino groups in the second coordination sphere. C1 [Egbert, Jonathan D.; Labios, Liezel A.; Darmon, Jonathan M.; Mock, Michael T.] Pacific NW Natl Lab, Ctr Mol Electrocatalysis, Div Phys Sci, Richland, WA 99352 USA. [Piro, Nicholas A.; Kassel, W. Scott] Villanova Univ, Dept Chem, Villanova, PA 19085 USA. RP Mock, MT (reprint author), Pacific NW Natl Lab, Ctr Mol Electrocatalysis, Div Phys Sci, Richland, WA 99352 USA. EM michael.mock@pnnl.gov FU Center for Molecular Electrocatalysis, an Energy Frontier Research Center - U.S. Department of Energy (U.S. DOE), Office of Science, Office of Basic Energy Sciences FX This work was supported as part of the Center for Molecular Electrocatalysis, an Energy Frontier Research Center funded by the U.S. Department of Energy (U.S. DOE), Office of Science, Office of Basic Energy Sciences. Pacific Northwest National Laboratory is operated by Battelle for the U.S. DOE. NR 35 TC 1 Z9 1 U1 2 U2 6 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1434-1948 EI 1099-0682 J9 EUR J INORG CHEM JI Eur. J. Inorg. Chem. PD MAR PY 2016 IS 8 BP 1293 EP 1299 DI 10.1002/ejic.201501477 PG 7 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DH2ZZ UT WOS:000372657700019 ER PT J AU Marrocchi, A Adriaensens, P Bartollini, E Barkakaty, B Carleer, R Chen, JH Hensley, DK Petrucci, C Tassi, M Vaccaro, L AF Marrocchi, Assunta Adriaensens, Peter Bartollini, Elena Barkakaty, Balaka Carleer, Robert Chen, Jihua Hensley, Dale K. Petrucci, Chiara Tassi, Marco Vaccaro, Luigi TI Novel cross-linked polystyrenes with large space network as tailor-made catalyst supports for sustainable media (vol 73, pg 391, 2015) SO EUROPEAN POLYMER JOURNAL LA English DT Correction C1 [Marrocchi, Assunta; Bartollini, Elena; Petrucci, Chiara; Vaccaro, Luigi] Univ Perugia, Lab Green Synthet Organ Chem, CEMIN Dipartimento Chim Biol & Biotecnol, Via Elce di Sotto 8, I-06123 Perugia, Italy. [Adriaensens, Peter; Carleer, Robert; Tassi, Marco] Hasselt Univ Appl & Analyt Chem, Agoralaan Bldg D, BE-3590 Diepenbeek, Belgium. [Barkakaty, Balaka; Chen, Jihua; Hensley, Dale K.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Marrocchi, A; Vaccaro, L (reprint author), Univ Perugia, Lab Green Synthet Organ Chem, CEMIN Dipartimento Chim Biol & Biotecnol, Via Elce di Sotto 8, I-06123 Perugia, Italy. EM assunta.marrocchi@unipg.it; luigi.vaccaro@unipg.it RI Vaccaro, Luigi/K-1043-2013; marrocchi, assunta/B-7583-2014; Chen, Jihua/F-1417-2011; Adriaensens, Peter/F-3877-2017 OI Vaccaro, Luigi/0000-0003-4168-2303; Chen, Jihua/0000-0001-6879-5936; Adriaensens, Peter/0000-0003-4183-0150 NR 1 TC 0 Z9 0 U1 3 U2 7 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0014-3057 EI 1873-1945 J9 EUR POLYM J JI Eur. Polym. J. PD MAR PY 2016 VL 76 BP 1 EP 1 DI 10.1016/j.eurpolymj.2016.01.023 PG 1 WC Polymer Science SC Polymer Science GA DH3HE UT WOS:000372677300001 ER PT J AU Hill, MC Kavetski, D Clark, M Ye, M Arabi, M Lu, D Foglia, L Mehl, S AF Hill, Mary C. Kavetski, Dmitri Clark, Martyn Ye, Ming Arabi, Mazdak Lu, Dan Foglia, Laura Mehl, Steffen TI Practical Use of Computationally Frugal Model Analysis Methods SO GROUNDWATER LA English DT Article ID EVALUATING PARAMETER IDENTIFIABILITY; SENSITIVITY-ANALYSIS; ERROR REDUCTION; 2 STATISTICS; UNCERTAINTY; SYSTEM; IDENTIFICATION; VALIDATION; TRANSPORT; POLICY AB Three challenges compromise the utility of mathematical models of groundwater and other environmental systems: (1) a dizzying array of model analysis methods and metrics make it difficult to compare evaluations of model adequacy, sensitivity, and uncertainty; (2) the high computational demands of many popular model analysis methods (requiring 1000's, 10,000s, or more model runs) make them difficult to apply to complex models; and (3) many models are plagued by unrealistic nonlinearities arising from the numerical model formulation and implementation. This study proposes a strategy to address these challenges through a careful combination of model analysis and implementation methods. In this strategy, computationally frugal model analysis methods (often requiring a few dozen parallelizable model runs) play a major role, and computationally demanding methods are used for problems where (relatively) inexpensive diagnostics suggest the frugal methods are unreliable. We also argue in favor of detecting and, where possible, eliminating unrealistic model nonlinearitiesthis increases the realism of the model itself and facilitates the application of frugal methods. Literature examples are used to demonstrate the use of frugal methods and associated diagnostics. We suggest that the strategy proposed in this paper would allow the environmental sciences community to achieve greater transparency and falsifiability of environmental models, and obtain greater scientific insight from ongoing and future modeling efforts. C1 [Hill, Mary C.] Univ Kansas, Dept Geol, 1475 Jayhawk Blvd, Lawrence, KS 66049 USA. [Hill, Mary C.] US Geol Survey, Boulder, CO USA. [Kavetski, Dmitri] Univ Adelaide, Adelaide, SA, Australia. [Clark, Martyn] Natl Ctr Atmospher Res, POB 3000, Boulder, CO 80307 USA. [Ye, Ming] Florida State Univ, Tallahassee, FL 32306 USA. [Arabi, Mazdak] Colorado State Univ, Ft Collins, CO 80523 USA. [Lu, Dan] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Foglia, Laura] Univ Darmstadt, Darmstadt, Germany. [Mehl, Steffen] Calif State Univ Chico, Chico, CA 95929 USA. RP Hill, MC (reprint author), Univ Kansas, Dept Geol, 1475 Jayhawk Blvd, Lawrence, KS 66049 USA.; Hill, MC (reprint author), US Geol Survey, Boulder, CO USA. EM mchill@ku.edu; dmitri.kavetski@adelaide.edu.au; mclark@ucar.edu; mye@fsu.edu; marabi@engr.colostate.edu; lud1@ornl.gov; foglia@geo.tu-darmstadt.de; smehl@csuchico.edu RI Ye, Ming/A-5964-2008 FU U.S. Geological Survey programs National Water Quality Assessment (NAWQA); Groundwater Resources Program (GWRP); National Research Program (NRP); NSF-EAR [0911074]; DOE [DE-SC0008272]; Swiss National Science Foundation (SNF) [21-66885] FX Mary Hill and Steffen Mehl were funded by the U.S. Geological Survey programs National Water Quality Assessment (NAWQA), Groundwater Resources Program (GWRP), and National Research Program (NRP). Ming Ye and Dan Lu were funded by NSF-EAR grant 0911074 and the DOE Early Career Award DE-SC0008272. Laura Foglia was funded by Swiss National Science Foundation (SNF) grant number 21-66885. We thank George Kuczera (University of Newcastle) and Sujay Kumar (NASA) for comments on early versions of the manuscript. We are also grateful to the editors of Ground Water and three anonymous reviewers. NR 68 TC 4 Z9 4 U1 7 U2 15 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0017-467X EI 1745-6584 J9 GROUNDWATER JI Groundwater PD MAR-APR PY 2016 VL 54 IS 2 BP 159 EP 170 DI 10.1111/gwat.12330 PG 12 WC Geosciences, Multidisciplinary; Water Resources SC Geology; Water Resources GA DI0TW UT WOS:000373211200006 PM 25810333 ER PT J AU Robinson, J Slater, L Johnson, T Shapiro, A Tiedeman, C Ntarlagiannis, D Johnson, C Day-Lewis, F Lacombe, P Imbrigiotta, T Lane, J AF Robinson, Judith Slater, Lee Johnson, Timothy Shapiro, Allen Tiedeman, Claire Ntarlagiannis, Dimitrios Johnson, Carole Day-Lewis, Frederick Lacombe, Pierre Imbrigiotta, Thomas Lane, John TI Imaging Pathways in Fractured Rock Using Three-Dimensional Electrical Resistivity Tomography SO GROUNDWATER LA English DT Article ID SENSITIVITY-ANALYSIS; DC RESISTIVITY; MASS-TRANSFER; RIVER-WATER; INVERSION; TRANSPORT; SURFACE; GROUNDWATER; AQUIFER; ERT AB Major challenges exist in delineating bedrock fracture zones because these cause abrupt changes in geological and hydrogeological properties over small distances. Borehole observations cannot sufficiently capture heterogeneity in these systems. Geophysical techniques offer the potential to image properties and processes in between boreholes. We used three-dimensional cross borehole electrical resistivity tomography (ERT) in a 9m (diameter)x15m well field to capture high-resolution flow and transport processes in a fractured mudstone contaminated by chlorinated solvents, primarily trichloroethylene. Conductive (sodium bromide) and resistive (deionized water) injections were monitored in seven boreholes. Electrode arrays with isolation packers and fluid sampling ports were designed to enable acquisition of ERT measurements during pulsed tracer injections. Fracture zone locations and hydraulic pathways inferred from hydraulic head drawdown data were compared with electrical conductivity distributions from ERT measurements. Static ERT imaging has limited resolution to decipher individual fractures; however, these images showed alternating conductive and resistive zones, consistent with alternating laminated and massive mudstone units at the site. Tracer evolution and migration was clearly revealed in time-lapse ERT images and supported by in situ borehole vertical apparent conductivity profiles collected during the pulsed tracer test. While water samples provided important local information at the extraction borehole, ERT delineated tracer migration over spatial scales capturing the primary hydrogeological heterogeneity controlling flow and transport. The fate of these tracer injections at this scale could not have been quantified using borehole logging and/or borehole sampling methods alone. C1 [Robinson, Judith; Slater, Lee; Ntarlagiannis, Dimitrios] Rutgers State Univ, Dept Earth & Environm Sci, 101 Warren St,Smith Hall Rm 135, Newark, NJ 07102 USA. [Johnson, Timothy] Pacific NW Natl Lab, Richland, WA 99352 USA. [Shapiro, Allen] US Geol Survey, 959 Natl Ctr, Reston, VA 22092 USA. [Tiedeman, Claire] US Geol Survey, 345 Middlefield Rd, Menlo Pk, CA 94025 USA. [Johnson, Carole; Day-Lewis, Frederick; Lane, John] US Geol Survey, Storrs, CT USA. [Lacombe, Pierre; Imbrigiotta, Thomas] US Geol Survey, Lawrenceville, NJ USA. RP Robinson, J (reprint author), Rutgers State Univ, Dept Earth & Environm Sci, 101 Warren St,Smith Hall Rm 135, Newark, NJ 07102 USA. EM judy.robinson@rutgers.edu; lslater@andromeda.rutgers.edu; TJ@pnnl.gov; ashapiro@usgs.gov; tiedeman@usgs.gov; cjohnson@usgs.gov; placombe@usgs.gov OI Day-Lewis, Frederick/0000-0003-3526-886X FU U. S. Department of Defense (DOD) under the Environmental Security Technology Certification Program [ER 201118] FX Funding for this project was provided by the U. S. Department of Defense (DOD) under the Environmental Security Technology Certification Program ER 201118 (L. Slater, PI). Inverse computations were performed on the Pacific Northwest National Laboratory Institutional Computing System (http://pic.pnnl.gov). We thank Daniel Goode for his contributions to this project. We are grateful for the field and laboratory support provided by Sundeep Sharma, Jeff Heenan, Jay Nolan, and USGS summer interns Alex Fiore, Carla Valdes, and Chris Leach. Additional support for this work came from the U.S. Geological Survey Toxic Substances Hydrology Program. Any use of trade, firm, or product names is for descriptive purposes only and does not imply endorsement by the U. S. Government. We thank three anonymous reviewers and Ryan Swanson for improving this manuscript. NR 56 TC 0 Z9 0 U1 5 U2 16 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0017-467X EI 1745-6584 J9 GROUNDWATER JI Groundwater PD MAR-APR PY 2016 VL 54 IS 2 BP 186 EP 201 DI 10.1111/gwat.12356 PG 16 WC Geosciences, Multidisciplinary; Water Resources SC Geology; Water Resources GA DI0TW UT WOS:000373211200008 PM 26172032 ER PT J AU Fritz, BG Mackley, RD Arntzen, EV AF Fritz, Bradley G. Mackley, Rob D. Arntzen, Evan V. TI Conducting Slug Tests in Mini-Piezometers SO GROUNDWATER LA English DT Article ID PARTIALLY PENETRATING WELLS; HYDRAULIC CONDUCTIVITY; HYPORHEIC ZONE; RIVER; EXCHANGE AB Slug tests performed using mini-piezometers with internal diameters as small as 0.43 cm can provide a cost effective tool for hydraulic characterization. We evaluated the hydraulic properties of the apparatus in a laboratory environment and compared those results with field tests of mini-piezometers installed into locations with varying hydraulic properties. Based on our evaluation, slug tests conducted in mini-piezometers using the fabrication and installation approach described here are effective within formations where the hydraulic conductivity is less than 1 x 10(-3) cm/s. While these constraints limit the potential application of this method, the benefits to this approach are that the installation, measurement, and analysis is cost effective, and the installation can be completed in areas where other (larger diameter) methods might not be possible. Additionally, this methodology could be applied to existing mini-piezometers previously installed for other purposes. Such analysis of existing installations could be beneficial in interpreting previously collected data (e.g., water-quality data or hydraulic head data). C1 [Fritz, Bradley G.; Mackley, Rob D.; Arntzen, Evan V.] Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99354 USA. RP Fritz, BG (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99354 USA. EM Bradley.Fritz@pnnl.gov NR 26 TC 0 Z9 0 U1 0 U2 4 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0017-467X EI 1745-6584 J9 GROUNDWATER JI Groundwater PD MAR-APR PY 2016 VL 54 IS 2 BP 291 EP 295 DI 10.1111/gwat.12335 PG 5 WC Geosciences, Multidisciplinary; Water Resources SC Geology; Water Resources GA DI0TW UT WOS:000373211200017 PM 25818983 ER PT J AU Almeida, SF Mireles, J Garcia, EJ Zubia, D AF Almeida, Sergio F. Mireles, Jose, Jr. Garcia, Ernest J. Zubia, David TI MEMS Closed-Loop Control Incorporating a Memristor as Feedback Sensing Element SO IEEE TRANSACTIONS ON CIRCUITS AND SYSTEMS II-EXPRESS BRIEFS LA English DT Article DE Circuit simulation; closed-loop control; feedback; memristor; microelectromechanical systems (MEMS); micromechanical devices ID PARALLEL-PLATE; OSCILLATORS; ACTUATOR AB In this brief, the integration of a memristor with a microelectromechanical systems (MEMS) parallel plate capacitor coupled by an amplification stage is simulated. It is shown that the MEMS upper plate position can be controlled up to 95% of the total gap. Due to its common operation principle, the change in the MEMS plate position can be interpreted by the change in the memristor resistance or memristance. A memristance modulation of similar to 1 k Omega was observed. A polynomial expression representing the MEMS upper plate displacement as a function of the memristance is presented. Thereafter, a simple design for a voltage closed-loop control is presented, showing that the MEMS upper plate can be stabilized up to 95% of the total gap by using the memristor as a feedback sensing element. The memristor can play important dual roles in overcoming the limited operation range of MEMS parallel plate capacitors and in simplifying read-out circuits of those devices by representing the motion of the upper plate in the form of resistance change instead of capacitance change. C1 [Almeida, Sergio F.; Zubia, David] Univ Texas El Paso, Dept Elect & Comp Engn, El Paso, TX 79968 USA. [Mireles, Jose, Jr.] Univ Autonoma Ciudad Juarez, Juarez 32310, Mexico. [Garcia, Ernest J.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Almeida, SF; Zubia, D (reprint author), Univ Texas El Paso, Dept Elect & Comp Engn, El Paso, TX 79968 USA.; Mireles, J (reprint author), Univ Autonoma Ciudad Juarez, Juarez 32310, Mexico.; Garcia, EJ (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM sfalmeida@utep.edu; jmireles@uacj.mx; ejgarci@sandia.gov; dzubia@utep.edu FU Sandia National Laboratories [1156850]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by Sandia National Laboratories under contract 1156850. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 25 TC 2 Z9 2 U1 0 U2 8 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1549-7747 EI 1558-3791 J9 IEEE T CIRCUITS-II JI IEEE Trans. Circuits Syst. II-Express Briefs PD MAR PY 2016 VL 63 IS 3 BP 294 EP 298 DI 10.1109/TCSII.2015.2504258 PG 5 WC Engineering, Electrical & Electronic SC Engineering GA DH9SN UT WOS:000373136200014 ER PT J AU Mondal, A Illindala, MS Khalsa, AS Klapp, DA Eto, JH AF Mondal, Abrez Illindala, Mahesh S. Khalsa, Amrit S. Klapp, David A. Eto, Joseph H. TI Design and Operation of Smart Loads to Prevent Stalling in a Microgrid SO IEEE TRANSACTIONS ON INDUSTRY APPLICATIONS LA English DT Article DE Distributed power generation; generators; industrial power systems; load management; microgrids; power system reliability; smart grids; underfrequency load shedding ID SYSTEM AB This paper investigates the benefits of smart loads in an iXndustrial microgrid. Such smart loads offer the microgrid greater flexibility to regulate frequency for large fluctuating load scenarios, commonly encountered in industrial plants. A case study of stone-crushing facility is analyzed when it is fed by natural gas engine driven generator sets (also known as "gensets"). The problem of genset stalling is addressed in this work, and a solution of deploying smart loads is presented. Furthermore, smart load algorithms are proposed to restore the services at an industrial site in a timely manner. C1 [Mondal, Abrez; Illindala, Mahesh S.] Ohio State Univ, Dept Elect & Comp Engn, Columbus, OH 43210 USA. [Khalsa, Amrit S.] Amer Elect Power Co, Dolan Technol Ctr, Groveport, OH 43125 USA. [Klapp, David A.] Adv Microgrid Syst, Westerville, OH 43081 USA. [Eto, Joseph H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Mondal, A; Illindala, MS (reprint author), Ohio State Univ, Dept Elect & Comp Engn, Columbus, OH 43210 USA.; Khalsa, AS (reprint author), Amer Elect Power Co, Dolan Technol Ctr, Groveport, OH 43125 USA.; Klapp, DA (reprint author), Adv Microgrid Syst, Westerville, OH 43081 USA.; Eto, JH (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM mondal.14@osu.edu; millindala@ieee.org; askhalsa@aep.com; microgrids@outlook.com; jheto@lbl.gov RI Illindala, Mahesh/B-2822-2013 OI Illindala, Mahesh/0000-0002-2015-1338 FU Office of Electricity Delivery and Energy Reliability, Transmission Reliability Program of the U.S. Department of Energy [7004227]; Ohio State University FX This work was supported by the Office of Electricity Delivery and Energy Reliability, Transmission Reliability Program of the U.S. Department of Energy under Subcontract 7004227 with The Ohio State University administered by the Lawrence Berkeley National Laboratory. NR 24 TC 1 Z9 1 U1 4 U2 10 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0093-9994 EI 1939-9367 J9 IEEE T IND APPL JI IEEE Trans. Ind. Appl. PD MAR-APR PY 2016 VL 52 IS 2 BP 1184 EP 1192 DI 10.1109/TIA.2015.2483579 PG 9 WC Engineering, Multidisciplinary; Engineering, Electrical & Electronic SC Engineering GA DH7PP UT WOS:000372986600007 ER PT J AU Chen, C Wang, JH Qiu, F Zhao, DB AF Chen, Chen Wang, Jianhui Qiu, Feng Zhao, Dongbo TI Resilient Distribution System by Microgrids Formation After Natural Disasters SO IEEE TRANSACTIONS ON SMART GRID LA English DT Article DE Distribution system; microgrids; mixed-integer linear program (MILP); multiagent coordination; resilience ID SERVICE RESTORATION; EXPERT-SYSTEM; CONSENSUS; SEARCH AB Microgrids with distributed generation (DG) provide a resilient solution in the case of major faults in a distribution system due to natural disasters. This paper proposes a novel distribution system operational approach by forming multiple microgrids energized by DG from the radial distribution system in real-time operations to restore critical loads from the power outage. Specifically, a mixed-integer linear program is formulated to maximize the critical loads to be picked up while satisfying the self-adequacy and operation constraints for the microgrids formation problem by controlling the ON/OFF status of the remotely controlled switch devices and DG. A distributed multiagent coordination scheme is designed via local communications for the global information discovery as inputs of the optimization, which is suitable for autonomous communication requirements after the disastrous event. The formed microgrids can be further utilized for power quality control and can be connected to a larger microgrid before the restoration of the main grids is complete. Numerical results based on modified IEEE distribution test systems validate the effectiveness of our proposed scheme. C1 [Chen, Chen; Wang, Jianhui; Qiu, Feng] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. [Zhao, Dongbo] Eaton Corp, Eden Prairie, MN 55344 USA. RP Chen, C; Wang, JH; Qiu, F (reprint author), Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA.; Zhao, DB (reprint author), Eaton Corp, Eden Prairie, MN 55344 USA. EM morningchen@anl.gov; jianhui.wang@anl.gov; fqiu@anl.gov; dongbozhao@eaton.com FU U.S. Department of Energy Office of Electricity Delivery and Energy Reliability FX This work was supported by the U.S. Department of Energy Office of Electricity Delivery and Energy Reliability. Paper no. TSG-00064-2015. NR 32 TC 5 Z9 5 U1 5 U2 8 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1949-3053 EI 1949-3061 J9 IEEE T SMART GRID JI IEEE Trans. Smart Grid PD MAR PY 2016 VL 7 IS 2 SI SI BP 958 EP 966 DI 10.1109/TSG.2015.2429653 PG 9 WC Engineering, Electrical & Electronic SC Engineering GA DG4BK UT WOS:000372014900040 ER PT J AU Sun, HB Zhang, BM Wang, JH Sun, D Tong, JZ Moslehi, K Li, FX Strunz, K Li, FR AF Sun, Hongbin Zhang, Boming Wang, Jianhui Sun, David Tong, Jianzhong Moslehi, Khosrow Li, Fangxing Strunz, Kai Li, Furong TI Distributed Energy Management Systems SO IEEE TRANSACTIONS ON SMART GRID LA English DT Editorial Material C1 [Sun, Hongbin; Zhang, Boming] Tsinghua Univ, Beijing 100084, Peoples R China. [Wang, Jianhui] Argonne Natl Lab, Lemont, IL USA. [Sun, David] Alstom, Redmond, WA USA. [Tong, Jianzhong] PJM Interconnect LLC, Valley Forge, PA USA. [Moslehi, Khosrow] ABB, Santa Clara, CA USA. [Li, Fangxing] Univ Tennessee, Knoxville, TN USA. [Strunz, Kai] Berlin TU, Berlin, Germany. [Li, Furong] Univ Bath, Bath BA2 7AY, Avon, England. RP Sun, HB (reprint author), Tsinghua Univ, Beijing 100084, Peoples R China. NR 0 TC 0 Z9 0 U1 4 U2 4 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1949-3053 EI 1949-3061 J9 IEEE T SMART GRID JI IEEE Trans. Smart Grid PD MAR PY 2016 VL 7 IS 2 SI SI BP 971 EP 973 DI 10.1109/TSG.2016.2523818 PG 3 WC Engineering, Electrical & Electronic SC Engineering GA DG4BK UT WOS:000372014900042 ER PT J AU Baker, K Guo, JY Hug, G Li, X AF Baker, Kyri Guo, Junyao Hug, Gabriela Li, Xin TI Distributed MPC for Efficient Coordination of Storage and Renewable Energy Sources Across Control Areas SO IEEE TRANSACTIONS ON SMART GRID LA English DT Article DE Distributed optimization; model predictive control; storage; AC optimal power flow; approximate Newton direction method ID OPTIMAL POWER-FLOW; MODEL-PREDICTIVE CONTROL; WIND POWER; UNIT COMMITMENT; SYSTEMS; OPERATIONS AB In electric power systems, multiple entities are responsible for ensuring an economic and reliable way of delivering power from producers to consumers. With the increase of variable renewable generation it is becoming increasingly important to take advantage of the individual entities' (and their areas') capabilities for balancing variability. Hence, in this paper, we employ and extend the approximate Newton directions method to optimally coordinate control areas leveraging storage available in one area to balance variable resources in another area with only minimal information exchange among the areas. The problem to be decomposed is a model predictive control problem including generation constraints, energy storage constraints, and AC power flow constraints. Singularity issues encountered when formulating the respective Newton-Raphson steps due to intertemporal constraints are addressed and extensions to the original decomposition method are proposed to improve the convergence rate and required communication of the method. C1 [Baker, Kyri] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Guo, Junyao; Hug, Gabriela; Li, Xin] Carnegie Mellon Univ, Dept Elect & Comp Engn, Pittsburgh, PA 15213 USA. RP Baker, K (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA.; Guo, JY; Hug, G; Li, X (reprint author), Carnegie Mellon Univ, Dept Elect & Comp Engn, Pittsburgh, PA 15213 USA. EM kyri.baker@nrel.gov; junyaog@andrew.cmu.edu; ghug@ece.cmu.edu; xinli@ece.cmu.edu FU National Science Foundation [ECCS 1027576]; SYSU-CMU Joint Institute of Engineering FX This work was supported in part by the National Science Foundation under Grant ECCS 1027576, and in part by the SYSU-CMU Joint Institute of Engineering. Paper no. TSG-00644-2014. NR 26 TC 4 Z9 4 U1 2 U2 3 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1949-3053 EI 1949-3061 J9 IEEE T SMART GRID JI IEEE Trans. Smart Grid PD MAR PY 2016 VL 7 IS 2 SI SI BP 992 EP 1001 DI 10.1109/TSG.2015.2512503 PG 10 WC Engineering, Electrical & Electronic SC Engineering GA DG4BK UT WOS:000372014900045 ER PT J AU Xiang, Y Liu, JY Liu, YL AF Xiang, Yue Liu, Junyong Liu, Yilu TI Robust Energy Management of Microgrid With Uncertain Renewable Generation and Load SO IEEE TRANSACTIONS ON SMART GRID LA English DT Article DE Exchange electricity price; microgrid; optimization; orthogonal array (OA); scenarios ID UNIT COMMITMENT PROBLEM; POWER; STORAGE; SYSTEM AB A scenario-based robust energy management method accounting for the worst-case amount of renewable generation (RG) and load is developed in this paper. The economic and robust model is formulated to maximize the total exchange cost while getting the minimum social benefits cost at the same time. Uncertainty of RG and load is described as an uncertain set produced by interval prediction. Then, the Taguchi's orthogonal array (OA) testing method is used to provide possible testing scenarios. A simple, but practical, search strategy based on OA is designed for solving the optimization problem. By optimizing the worst-case scenario, the energy management solution of the proposed model is robust against most of the possible realizations of the modeled uncertain set by Monte Carlo verification. Numerical cases on the typical microgrid system show the effectiveness of the model and solution strategy. In addition, the influence of exchange electricity price and other parameters are also discussed in the cases. C1 [Xiang, Yue; Liu, Junyong] Sichuan Univ, Sch Elect Engn & Informat, Chengdu 610065, Peoples R China. [Xiang, Yue; Liu, Yilu] Univ Tennessee, Dept Elect Engn & Comp Sci, Knoxville, TN 37996 USA. [Liu, Yilu] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Xiang, Y (reprint author), Sichuan Univ, Sch Elect Engn & Informat, Chengdu 610065, Peoples R China.; Xiang, Y (reprint author), Univ Tennessee, Dept Elect Engn & Comp Sci, Knoxville, TN 37996 USA. EM exxyye@gmail.com FU National High Technology Research and Development Program of China [2014AA051901]; National Science Foundation of China [51377111]; Engineering Research Center by Engineering Research Center Program of the U.S. National Science Foundation; Department of Energy under National Science Foundation [EEC-1041877]; Center for Ultra-Wide-Area Resilient Electric Energy Transmission Networks Industry Partnership Program FX This work was supported in part by the National High Technology Research and Development Program of China under Grant 2014AA051901, in part by the National Science Foundation of China under Grant 51377111, in part by the Engineering Research Center shared facilities supported by the Engineering Research Center Program of the U.S. National Science Foundation, in part by the Department of Energy under National Science Foundation Award EEC-1041877, and in part by the Center for Ultra-Wide-Area Resilient Electric Energy Transmission Networks Industry Partnership Program. Paper no. TSG-00568-2014. NR 38 TC 5 Z9 5 U1 8 U2 14 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1949-3053 EI 1949-3061 J9 IEEE T SMART GRID JI IEEE Trans. Smart Grid PD MAR PY 2016 VL 7 IS 2 SI SI BP 1034 EP 1043 DI 10.1109/TSG.2014.2385801 PG 10 WC Engineering, Electrical & Electronic SC Engineering GA DG4BK UT WOS:000372014900049 ER PT J AU Wang, ZY Chen, BK Wang, JH Kim, J AF Wang, Zhaoyu Chen, Bokan Wang, Jianhui Kim, Jinho TI Decentralized Energy Management System for Networked Microgrids in Grid-Connected and Islanded Modes SO IEEE TRANSACTIONS ON SMART GRID LA English DT Article DE Distributed generator (DG); microgrids (MGs); power distribution system; stochastic optimization ID CONSTRAINED UNIT COMMITMENT; ACTIVE DISTRIBUTION GRIDS; OPTIMIZATION; GENERATION; SECURITY; OPERATION AB This paper proposes a decentralized energy management system for the coordinated operation of networked microgirds (MGs) in a distribution system. In the grid-connected mode, the distribution network operator and each MG are considered as distinct entities with individual objectives to minimize their own operation costs. It is assumed that both dispatchable and renewable energy source-based distributed generators (DGs) exist in the distribution network and the networked MGs. In order to coordinate the operation of all entities, we apply a decentralized bi-level algorithm to solve the problem with the first level to conduct negotiations among all entities and the second level to update the non-converging penalties. In the islanded mode, the objective of each MG is to maintain a reliable power supply to its customers. In order to take into account the uncertainties of DG outputs and load consumption, we formulate the problems as two-stage stochastic programs. The first stage is to determine base generation setpoints based on the forecasts and the second stage is to adjust the generation outputs based on the realized scenarios. Case studies of a distribution system with networked MGs demonstrate the effectiveness of the proposed methodology in both grid-connected and islanded modes. C1 [Wang, Zhaoyu] Georgia Inst Technol, Sch Elect & Comp Engn, Atlanta, GA 30332 USA. [Chen, Bokan] Iowa State Univ, Sch Ind & Mfg Syst Engn, Ames, IA 50014 USA. [Wang, Jianhui] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Kim, Jinho] Gachon Univ, Songnam 463777, South Korea. RP Wang, ZY (reprint author), Georgia Inst Technol, Sch Elect & Comp Engn, Atlanta, GA 30332 USA.; Chen, BK (reprint author), Iowa State Univ, Sch Ind & Mfg Syst Engn, Ames, IA 50014 USA.; Wang, JH (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA.; Kim, J (reprint author), Gachon Univ, Songnam 463777, South Korea. EM zhaoyuwang@gatech.edu; bokanc@iastate.edu; jianhui.wang@anl.gov; kimjh@gachon.ac.kr FU U.S. Department of Energy Office of Electricity Delivery and Energy Reliability FX This work was supported by the U.S. Department of Energy Office of Electricity Delivery and Energy Reliability. Paper no. TSG-00574-2014. NR 30 TC 5 Z9 5 U1 3 U2 6 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1949-3053 EI 1949-3061 J9 IEEE T SMART GRID JI IEEE Trans. Smart Grid PD MAR PY 2016 VL 7 IS 2 SI SI BP 1097 EP 1105 DI 10.1109/TSG.2015.2427371 PG 9 WC Engineering, Electrical & Electronic SC Engineering GA DG4BK UT WOS:000372014900055 ER PT J AU Grear, ME Crofts, SB Copping, AE Summers, AP Ditsche, P AF Grear, M. E. Crofts, S. B. Copping, A. E. Summers, A. P. Ditsche, P. TI Finite element material model of harbor seals' (Phoca vitulina) skin and blubber SO INTEGRATIVE AND COMPARATIVE BIOLOGY LA English DT Meeting Abstract CT Annual Meeting of the Society-for-Integrative-and-Comparative-Biology (SICB) CY JAN 03-07, 2016 CL Portland, OR SP Soc Integrat & Comparat Biol C1 Univ Washington, Seattle, WA 98195 USA. Pacific NW Natl Lab, Richland, WA 99352 USA. EM mgrear@uw.edu NR 0 TC 0 Z9 0 U1 2 U2 2 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 1540-7063 EI 1557-7023 J9 INTEGR COMP BIOL JI Integr. Comp. Biol. PD MAR PY 2016 VL 56 SU 1 MA 73-4 BP E79 EP E79 PG 1 WC Zoology SC Zoology GA DH0FJ UT WOS:000372457600316 ER PT J AU Haskins, DL Hamilton, MT Finger, JW Jones, AL Bringolf, RB Tuberville, TD AF Haskins, D. L. Hamilton, M. T. Finger, J. W. Jones, A. L. Bringolf, R. B. Tuberville, T. D. TI Immunological costs of trace element contaminants in Yellow-bellied sliders (Trachemys scripta scripta) SO INTEGRATIVE AND COMPARATIVE BIOLOGY LA English DT Meeting Abstract CT Annual Meeting of the Society-for-Integrative-and-Comparative-Biology (SICB) CY JAN 03-07, 2016 CL Portland, OR SP Soc Integrat & Comparat Biol C1 Univ Georgia, Savannah River Ecol Lab, Athens, GA 30602 USA. Auburn Univ, Auburn, AL 36849 USA. Univ S Carolina, Columbia, SC 29208 USA. Univ Georgia, Warnell Sch Forestry & Nat Resources, Savannah River Ecol Lab, Athens, GA 30602 USA. EM david.haskins@uga.edu NR 0 TC 0 Z9 0 U1 0 U2 0 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 1540-7063 EI 1557-7023 J9 INTEGR COMP BIOL JI Integr. Comp. Biol. PD MAR PY 2016 VL 56 SU 1 MA P2.51 BP E299 EP E299 PG 1 WC Zoology SC Zoology GA DH0FJ UT WOS:000372457601552 ER PT J AU Hope, SF Beck, ML Kennamer, RA Hopkin, WA AF Hope, S. F. Beck, M. L. Kennamer, R. A. Hopkin, W. A. TI The effect of incubation temperature on Wood Duck duckling behavior SO INTEGRATIVE AND COMPARATIVE BIOLOGY LA English DT Meeting Abstract CT Annual Meeting of the Society-for-Integrative-and-Comparative-Biology (SICB) CY JAN 03-07, 2016 CL Portland, OR SP Soc Integrat & Comparat Biol C1 Virginia Polytech Inst & State Univ, Blacksburg, VA 24061 USA. Univ Georgia, Athens, GA 30602 USA. Savannah River Ecol Lab, Aiken, SC 29802 USA. EM shope@vt.edu NR 0 TC 0 Z9 0 U1 2 U2 2 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 1540-7063 EI 1557-7023 J9 INTEGR COMP BIOL JI Integr. Comp. Biol. PD MAR PY 2016 VL 56 SU 1 MA P1.177 BP E303 EP E303 PG 1 WC Zoology SC Zoology GA DH0FJ UT WOS:000372457601569 ER PT J AU Kelley, JF Smith, T Davis, R Podar, M Raghavan, RE Stott, MB Reysenbach, AL AF Kelley, J. F. Smith, T. Davis, R. Podar, M. Raghavan, R. E. Stott, M. B. Reysenbach, A. -L TI Preliminary analysis of New Zealand hot spring Nanoarchaeota and Korarchaeota metagenomes SO INTEGRATIVE AND COMPARATIVE BIOLOGY LA English DT Meeting Abstract CT Annual Meeting of the Society-for-Integrative-and-Comparative-Biology (SICB) CY JAN 03-07, 2016 CL Portland, OR SP Soc Integrat & Comparat Biol C1 Portland State Univ, Portland, OR 97207 USA. Oak Ridge Natl Lab, Oak Ridge, TN USA. GNS Sci, Dunedin, New Zealand. EM jokelley@pdx.edu NR 0 TC 0 Z9 0 U1 1 U2 1 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 1540-7063 EI 1557-7023 J9 INTEGR COMP BIOL JI Integr. Comp. Biol. PD MAR PY 2016 VL 56 SU 1 MA P1.98 BP E313 EP E313 PG 1 WC Zoology SC Zoology GA DH0FJ UT WOS:000372457601608 ER PT J AU Kramer, SLB Boyce, BL AF Kramer, Sharlotte L. B. Boyce, Brad L. TI Preface to the special volume on the second Sandia Fracture Challenge SO INTERNATIONAL JOURNAL OF FRACTURE LA English DT Editorial Material C1 [Kramer, Sharlotte L. B.; Boyce, Brad L.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Kramer, SLB (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM slkrame@sandia.gov; blboyce@sandia.gov NR 0 TC 0 Z9 0 U1 1 U2 3 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0376-9429 EI 1573-2673 J9 INT J FRACTURE JI Int. J. Fract. PD MAR PY 2016 VL 198 IS 1-2 BP 1 EP 3 DI 10.1007/s10704-016-0087-9 PG 3 WC Materials Science, Multidisciplinary; Mechanics SC Materials Science; Mechanics GA DH4KV UT WOS:000372755800001 ER PT J AU Boyce, BL Kramer, SLB Bosiljevac, TR Corona, E Moore, JA Elkhodary, K Simha, CHM Williams, BW Cerrone, AR Nonn, A Hochhalter, JD Bomarito, GF Warner, JE Carter, BJ Warner, DH Ingraffea, AR Zhang, T Fang, X Lua, J Chiaruttini, V Maziere, M Feld-Payet, S Yastrebov, VA Besson, J Chaboche, JL Lian, J Di, Y Wu, B Novokshanov, D Vajragupta, N Kucharczyk, P Brinnel, V Dobereiner, B Munstermann, S Neilsen, MK Dion, K Karlson, KN Foulk, JW Brown, AA Veilleux, MG Bignell, JL Sanborn, SE Jones, CA Mattie, PD Pack, K Wierzbicki, T Chi, SW Lin, SP Mahdavi, A Predan, J Zadravec, J Gross, AJ Ravi-Chandar, K Xue, L AF Boyce, B. L. Kramer, S. L. B. Bosiljevac, T. R. Corona, E. Moore, J. A. Elkhodary, K. Simha, C. H. M. Williams, B. W. Cerrone, A. R. Nonn, A. Hochhalter, J. D. Bomarito, G. F. Warner, J. E. Carter, B. J. Warner, D. H. Ingraffea, A. R. Zhang, T. Fang, X. Lua, J. Chiaruttini, V. Maziere, M. Feld-Payet, S. Yastrebov, V. A. Besson, J. Chaboche, J. -L. Lian, J. Di, Y. Wu, B. Novokshanov, D. Vajragupta, N. Kucharczyk, P. Brinnel, V. Doebereiner, B. Muenstermann, S. Neilsen, M. K. Dion, K. Karlson, K. N. Foulk, J. W., III Brown, A. A. Veilleux, M. G. Bignell, J. L. Sanborn, S. E. Jones, C. A. Mattie, P. D. Pack, K. Wierzbicki, T. Chi, S. -W. Lin, S. -P. Mahdavi, A. Predan, J. Zadravec, J. Gross, A. J. Ravi-Chandar, K. Xue, L. TI The second Sandia Fracture Challenge: predictions of ductile failure under quasi-static and moderate-rate dynamic loading SO INTERNATIONAL JOURNAL OF FRACTURE LA English DT Article DE Fracture; Rupture; Tearing; Deformation; Plasticity; Metal; Alloy; Simulation; rediction; Modeling ID POLYCRYSTALLINE AL 6061-T6; KERNEL PARTICLE METHODS; STRENGTH STEEL SHEETS; HIGH-STRAIN-RATE; CRACK-PROPAGATION; ROOM-TEMPERATURE; DAMAGE; MODEL; BEHAVIOR; DEFORMATION AB Ductile failure of structural metals is relevant to a wide range of engineering scenarios. Computational methods are employed to anticipate the critical conditions of failure, yet they sometimes provide inaccurate and misleading predictions. Challenge scenarios, such as the one presented in the current work, provide an opportunity to assess the blind, quantitative predictive ability of simulation methods against a previously unseen failure problem. Rather than evaluate the predictions of a single simulation approach, the Sandia Fracture Challenge relies on numerous volunteer teams with expertise in computational mechanics to apply a broad range of computational methods, numerical algorithms, and constitutive models to the challenge. This exercise is intended to evaluate the state of health of technologies available for failure prediction. In the first Sandia Fracture Challenge, a wide range of issues were raised in ductile failure modeling, including a lack of consistency in failure models, the importance of shear calibration data, and difficulties in quantifying the uncertainty of prediction [see Boyce et al. (Int J Fract 186:5-68, 2014) for details of these observations]. This second Sandia Fracture Challenge investigated the ductile rupture of a Ti-6Al-4V sheet under both quasi-static and modest-rate dynamic loading (failure in 0.1 s). Like the previous challenge, the sheet had an unusual arrangement of notches and holes that added geometric complexity and fostered a competition between tensile- and shear-dominated failure modes. The teams were asked to predict the fracture path and quantitative far-field failure metrics such as the peak force and displacement to cause crack initiation. Fourteen teams contributed blind predictions, and the experimental outcomes were quantified in three independent test labs. Additional shortcomings were revealed in this second challenge such as inconsistency in the application of appropriate boundary conditions, need for a thermomechanical treatment of the heat generation in the dynamic loading condition, and further difficulties in model calibration based on limited real-world engineering data. As with the prior challenge, this work not only documents the 'state-of-the-art' in computational failure prediction of ductile tearing scenarios, but also provides a detailed dataset for non-blind assessment of alternative methods. C1 [Boyce, B. L.; Kramer, S. L. B.; Bosiljevac, T. R.; Corona, E.; Neilsen, M. K.; Bignell, J. L.; Sanborn, S. E.; Jones, C. A.; Mattie, P. D.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Moore, J. A.] Northwestern Univ, Evanston, IL USA. [Elkhodary, K.] Amer Univ Cairo, New Cairo, Egypt. [Simha, C. H. M.; Williams, B. W.] Nat Resources Canada, CanmetMAT, Hamilton, ON, Canada. [Cerrone, A. R.] GE Global Res Ctr, Niskayuna, NY USA. [Nonn, A.] Ostbayer Tech Hsch, Regensburg, Germany. [Hochhalter, J. D.; Bomarito, G. F.; Warner, J. E.] NASA, Langley Res Ctr, Hampton, VA 23665 USA. [Carter, B. J.; Warner, D. H.; Ingraffea, A. R.] Cornell Univ, Ithaca, NY USA. [Zhang, T.; Fang, X.; Lua, J.] Global Engn & Mat Inc, Princeton, NJ USA. [Chiaruttini, V.; Feld-Payet, S.; Chaboche, J. -L.] Univ Paris Saclay, Onera, Chatillon, France. [Maziere, M.; Yastrebov, V. A.; Besson, J.] PSL Res Univ, MINES ParisTech, Ctr Mat, CNRS UMR 7633, Evry, France. [Lian, J.; Di, Y.; Wu, B.; Novokshanov, D.; Vajragupta, N.; Kucharczyk, P.; Brinnel, V.; Doebereiner, B.; Muenstermann, S.] Rhein Westfal TH Aachen, Aachen, Germany. [Dion, K.; Karlson, K. N.; Foulk, J. W., III; Brown, A. A.; Veilleux, M. G.] Sandia Natl Labs, Livermore, CA USA. [Pack, K.; Wierzbicki, T.] MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Chi, S. -W.; Lin, S. -P.; Mahdavi, A.] Univ Illinois, Chicago, IL USA. [Predan, J.; Zadravec, J.] Univ Maribor, SLO-2000 Maribor, Slovenia. [Gross, A. J.; Ravi-Chandar, K.] Univ Texas Austin, Austin, TX 78712 USA. [Xue, L.] Thinkviewer LLC, Sugar Land, TX USA. RP Boyce, BL (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM blboyce@sandia.gov; slkrame@sandia.gov; trbosil@sandia.gov; ecorona@sandia.gov; johnallanmoore@gmail.com; khalile@aucegypt.edu; Hari.Simha@NRCan-RNCan.gc.ca; Bruce.Williams@NRCan-RNCan.gc.ca; albert.cerrone@ge.com; aida.nonn@oth-regensburg.de; jacob.d.hochhalter@nasa.gov; geoffrey.f.bomarito@nasa.gov; james.e.warner@nasa.gov; bjc21@cornell.edu; reddhw52@cornell.edu; ari1@cornell.edu; tzhang@gem-innovation.com; xfang@gem-innovation.com; jlua@gem-innovation.com; vincent.chiaruttini@onera.fr; matthieu.maziere@mines-paristech.fr; sylvia.feld-payet@onera.fr; vladislav.yastrebov@mines-paristech.fr; jacques.besson@mines-paristech.fr; jean-louis.chaboche@onera.fr; junhe.lian@iehk.rwth-aachen.de; yidu.di@iehk.rwth-aachen.de; bo.wu@iehk.rwth-aachen.de; denis.novokshanov@iehk.rwth-aachen.de; napat.vajragupta@iehk.rwth-aachen.de; pawel.kucharczyk@iehk.rwth-aachen.de; victoria.brinnel@iehk.rwth-aachen.de; benedikt.doebereiner@iehk.rwth-aachen.de; sebastian.muenstermann@iehk.rwth-aachen.de; mkneils@sandia.gov; kdion@sandia.gov; knkarls@sandia.gov; jwfoulk@sandia.gov; aabrown@sandia.gov; mgveill@sandia.gov; jbignel@sandia.gov; sesanbo@sandia.gov; cajone@sandia.gov; pdmatti@sandia.gov; kpack@mit.edu; wierz@mit.edu; swchi@uic.edu; slin46@ford.com; amahda2@uic.edu; jozef.predan@um.si; zadravec.jozef@gmail.com; andrew.gross@mail.utexas.edu; ravi@utexas.edu; xue@alum.mit.edu RI Besson, Jacques/A-4144-2008; Munstermann, Sebastian/E-5480-2012; Xue, Liang/A-1266-2007; Warner, Derek/A-2303-2012; Lian, Junhe/C-5492-2009 OI Besson, Jacques/0000-0003-1975-2408; Munstermann, Sebastian/0000-0002-6251-2429; Xue, Liang/0000-0003-0468-0624; Lian, Junhe/0000-0003-0323-3486 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Office of Naval Research: MURI [N00014-06-1-0505-A00001]; Office of Naval Research: FNC Project [N00014-08-1-0189]; Office of Naval Research [N00014-11-C-0487]; National Science Foundation [CMMI-1532528] FX BLB and HEF would like to thank Dr. James Redmond for managing Sandia's role in this work through the DOE Advanced Scientific Computing program. SLBK and TRB would like to thank Dr. Dennis Croessmann and Dr. David Epp for their management role supporting the experimental efforts at Sandia for this work through the NNSA Weapon System Engineering and Assessment Technology Engineering Campaign. JLB, SES, and CAJ would like to thank DOE/NE and Ryan Bechtel for partially supporting their participation in this challenge. The Sandia authors would like to thank the follow-ing individuals for providing laboratory support of the experiments: Thomas Crenshaw, John Laing, Jhana Gearhart, Mathew Ingraham, Artis Jackson, Darren Pendley, Jack Heister, and Alice Kilgo. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. The work of AJG and KRC at the University of Texas was performed during the course of an investigation into ductile failure under two related research programs funded by the Office of Naval Research: MURI Project N00014-06-1-0505-A00001 and FNC Project: N00014-08-1-0189; this support is gratefully acknowledged. The authors from GEM are grateful for the support provided by the Office of Naval Research (N00014-11-C-0487) for which Dr. Paul Hess and Dr. Ken Nahshon serve as the technical monitors. KP and TW are grateful to Dr. Borja Erice at Ecole Polytechnique for the development of the user material subroutine; thanks are also due to Dr. Christian C. Roth at MIT for a valuable discussion. The authors gratefully acknowledge financial support from the National Science Foundation (Grant Number CMMI-1532528, "Summit on Predictive Modeling of Ductile Failure") towards holding a Summit to discuss and distill the results reported in this article. NR 68 TC 8 Z9 8 U1 14 U2 30 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0376-9429 EI 1573-2673 J9 INT J FRACTURE JI Int. J. Fract. PD MAR PY 2016 VL 198 IS 1-2 BP 5 EP 100 DI 10.1007/s10704-016-0089-7 PG 96 WC Materials Science, Multidisciplinary; Mechanics SC Materials Science; Mechanics GA DH4KV UT WOS:000372755800002 ER PT J AU Dion, K Neilsen, MK AF Dion, Kristin Neilsen, Michael K. TI Coupled thermal stress simulations of ductile tearing SO INTERNATIONAL JOURNAL OF FRACTURE LA English DT Article DE Ductile tearing; Metals; Plasticity; Damage; Constitutive model ID PREDICTIONS AB Predictions for ductile tearing of a geometrically complex Ti-6Al-4V plate were generated using a Unified Creep Plasticity Damage model in fully coupled thermal stress simulations. Uniaxial tension and butterfly shear tests performed at displacement rates of 0.0254 and 25.4 mm/s were also simulated. Results from these simulations revealed that the material temperature increase due to plastic work can have a dramatic effect on material ductility predictions in materials that exhibit little strain hardening. This occurs because the temperature increase causes the apparent hardening of the material to decrease which leads to the initiation of deformation localization and subsequent ductile tearing earlier in the loading process. C1 [Dion, Kristin; Neilsen, Michael K.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Neilsen, MK (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM mkneils@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Sandia National Laboratories FX We are grateful for the opportunity to participate in the Sandia Fracture Challenge 2 and would like to thank Drs. B. Boyce and S. Kramer for their work and for inviting us to participate. Helpful comments from reviewers of this paper, Drs. W. Scherzinger and B. Reedlunn, Sandia National Laboratories, and external reviewers, significantly improved the quality of this paper. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. Sandia National Laboratories support of this work is gratefully acknowledged. NR 11 TC 0 Z9 0 U1 0 U2 0 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0376-9429 EI 1573-2673 J9 INT J FRACTURE JI Int. J. Fract. PD MAR PY 2016 VL 198 IS 1-2 BP 167 EP 178 DI 10.1007/s10704-016-0093-y PG 12 WC Materials Science, Multidisciplinary; Mechanics SC Materials Science; Mechanics GA DH4KV UT WOS:000372755800007 ER PT J AU Karlson, KN Foulk, JW Brown, AA Veilleux, MG AF Karlson, Kyle N. Foulk, James W., III Brown, Arthur A. Veilleux, Michael G. TI Sandia fracture challenge 2: Sandia California's modeling approach SO INTERNATIONAL JOURNAL OF FRACTURE LA English DT Article DE Titanium alloys; Ti-6Al-4V; Fracture; Failure; Localization; Anisotropy; Viscoplasticity; Void evolution; Thermomechanical; Regularization; Nonlocality; Surface elements ID STRAIN-LOCALIZATION; DUCTILE FRACTURE; DEFORMATION; PLASTICITY; FORMULATIONS; TI-6AL-4V; FAILURE; METALS AB The second Sandia Fracture Challenge illustrates that predicting the ductile fracture of Ti-6Al-4V subjected to moderate and elevated rates of loading requires thermomechanical coupling, elasto-thermo-poro-viscoplastic constitutive models with the physics of anisotropy and regularized numerical methods for crack initiation and propagation. We detail our initial approach with an emphasis on iterative calibration and systematically increasing complexity to accommodate anisotropy in the context of an isotropic material model. Blind predictions illustrate strengths and weaknesses of our initial approach. We then revisit our findings to illustrate the importance of including anisotropy in the failure process. Mesh-independent solutions of continuum damage models having both isotropic and anisotropic yields surfaces are obtained through nonlocality and localization elements. C1 [Karlson, Kyle N.; Foulk, James W., III; Brown, Arthur A.; Veilleux, Michael G.] Sandia Natl Labs, 7011 East Ave, Livermore, CA 94550 USA. RP Foulk, JW (reprint author), Sandia Natl Labs, 7011 East Ave, Livermore, CA 94550 USA. EM jwfoulk@sandia.gov FU Joint DoD/DOE Munitions Technology Development Program (JMP); JMP; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors are grateful for the support of our colleagues during the Sandia Fracture Challenge. We profited from fruitful discussions regarding the analysis and experiments from Lauren Beghini, Michael Chiesa, John Emery, Wei-Yang Lu, and Tracy Vogler. We would like to give special thanks to Alejandro Mota, Jake Ostien, and Bill Scherzinger for their contributions in constitutive modeling and methods for regularization. Finally, we could not have been successful without the support of Kendall Pierson and the Sierra SolidMechanics team. The authors would like to also acknowledge that this work was supported in part through the Joint DoD/DOE Munitions Technology Development Program (JMP). Funding from JMP has enabled improvements in robustness and guidelines for methods devoted to the prediction of ductile fracture. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 36 TC 0 Z9 0 U1 1 U2 2 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0376-9429 EI 1573-2673 J9 INT J FRACTURE JI Int. J. Fract. PD MAR PY 2016 VL 198 IS 1-2 BP 179 EP 195 DI 10.1007/s10704-016-0090-1 PG 17 WC Materials Science, Multidisciplinary; Mechanics SC Materials Science; Mechanics GA DH4KV UT WOS:000372755800008 ER PT J AU Abreu-Sepulveda, M Williams, DE Huq, A Dhital, C Li, YC Paranthaman, MP Zaghib, K Manivannan, A AF Abreu-Sepulveda, Maria Williams, Dominique E. Huq, Ashfia Dhital, Chetan Li, Yunchao Paranthaman, M. Parans Zaghib, Karim Manivannan, A. TI Synthesis and characterization of substituted garnet and perovskite-based lithium-ion conducting solid electrolytes SO IONICS LA English DT Article DE Solid electrolytes; Garnet; Perovskite; Lithium-ion conduction; Solid-state lithium-ion battery ID SOLUTION LA0.67-XLI3XTIO3; LANTHANUM TITANATES; OXIDES; LI7LA3ZR2O12 AB Titanium, tantalum-substituted Li(7)La(3)Zr(2-x)A(x)O(12) (LLZO, A=Ta, Ti) garnets, and chromium-substituted La(2/3)-xLi3xTi1-yCryO3 (LLTO) perovskites were prepared by a conventional solid-state reaction and the Pechini processes. The desired crystal phases were obtained by varying the calcination temperature and time, as well as the substitution concentration. All samples indicated decomposition of the precursors when heated above 750 degrees C and formation of the desired phase after heat treatment at higher temperatures. Neutron diffraction data shows the formation of a predominant cubic phase in the case of Ta-LLZO, and monoclinic phase with minor impurity phases for Cr-LLTO. Ionic conductivity for Ti-LLZO (Li7La3Zr1.Ti-4(0).O-6(12)), Ta-LLZO (Li6.03La3Zr1.533Ta0.46O12), and Cr-LLTO (La(2/3)-xLi3xTi0.9Cr0.1O3) at room temperature were found to be 5.21x10(-6), 1.01x10(-6), and 1.2x10(-4) S cm(-1), respectively. The activation energies of the compounds were determined from the Arrhenius plot and were 0.44 eV (Ti-0.6-LLZO), 0.54 eV (Ta-0.5-LLZO), and 0.20 eV (Cr-0.1-LLTO). C1 [Abreu-Sepulveda, Maria; Williams, Dominique E.; Manivannan, A.] US DOE, NETL, Morgantown, WV 26507 USA. [Huq, Ashfia; Dhital, Chetan] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Li, Yunchao; Paranthaman, M. Parans] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Zaghib, Karim] Hydro Quebec, Varennes, PQ J3X 1S1, Canada. [Manivannan, A.] W Virginia Univ, Mech & Aerosp Engn, Morgantown, WV 26507 USA. RP Manivannan, A (reprint author), US DOE, NETL, Morgantown, WV 26507 USA. EM manivana@netl.doe.gov RI Huq, Ashfia/J-8772-2013; Dhital, Chetan/O-5634-2016; OI Huq, Ashfia/0000-0002-8445-9649; Dhital, Chetan/0000-0001-8125-6048; Li, Yunchao/0000-0001-5460-5855; Paranthaman, Mariappan/0000-0003-3009-8531 FU Vehicle Technology Program (EERE); Oak Ridge Institute for Science and Education (ORISE) program; Mickey Leland Energy Fellowship (MLEF) program; US Department of Energy, Office of Basic Energy Sciences, Scientific User Facilities Division FX This work was supported by the Vehicle Technology Program (EERE), Oak Ridge Institute for Science and Education (ORISE), and Mickey Leland Energy Fellowship (MLEF) programs. A portion of this research at ORNL's Spallation Neutron Source was sponsored by the US Department of Energy, Office of Basic Energy Sciences, Scientific User Facilities Division. Support (MPP and YL) for Neutron characterizations and impedance measurements was provided by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences, and Engineering Division. NR 28 TC 0 Z9 0 U1 29 U2 80 PU SPRINGER HEIDELBERG PI HEIDELBERG PA TIERGARTENSTRASSE 17, D-69121 HEIDELBERG, GERMANY SN 0947-7047 EI 1862-0760 J9 IONICS JI Ionics PD MAR PY 2016 VL 22 IS 3 BP 317 EP 325 DI 10.1007/s11581-015-1556-2 PG 9 WC Chemistry, Physical; Electrochemistry; Physics, Condensed Matter SC Chemistry; Electrochemistry; Physics GA DH7ZC UT WOS:000373011800002 ER PT J AU Isselhardt, BH Prussin, SG Savina, MR Willingham, DG Knight, KB Hutcheon, ID AF Isselhardt, B. H. Prussin, S. G. Savina, M. R. Willingham, D. G. Knight, K. B. Hutcheon, I. D. TI Rate equation model of laser induced bias in uranium isotope ratios measured by resonance ionization mass spectrometry SO JOURNAL OF ANALYTICAL ATOMIC SPECTROMETRY LA English DT Article ID BROAD-BAND RADIATION; HYPERFINE-STRUCTURE; SPECTROSCOPIC DATA; ATOMIC URANIUM; EXCITATION; PRECISION; ABUNDANCES; BANDWIDTH; GRAINS; RIMS AB Resonance Ionization Mass Spectrometry (RIMS) has been developed as a method to measure uranium isotope abundances. In this approach, RIMS is used as an element-selective ionization process between uranium atoms and potential isobars without the aid of chemical purification and separation. The use of broad bandwidth lasers with automated feedback control of wavelength was applied to the measurement of the U-235/U-238 ratio to decrease laser-induced isotopic fractionation. In application, isotope standards are used to identify and correct bias in measured isotope ratios, but understanding laser-induced bias from first-principles can improve the precision and accuracy of experimental measurements. A rate equation model for predicting the relative ionization probability has been developed to study the effect of variations in laser parameters on the measured isotope ratio. The model uses atomic data and empirical descriptions of laser performance to estimate the laser-induced bias expected in experimental measurements of the U-235/U-238 ratio. Empirical corrections are also included to account for ionization processes that are difficult to calculate from first principles with the available atomic data. Development of this model has highlighted several important considerations for properly interpreting experimental results. C1 [Isselhardt, B. H.; Knight, K. B.; Hutcheon, I. D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Prussin, S. G.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Savina, M. R.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Willingham, D. G.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Isselhardt, BH (reprint author), Lawrence Livermore Natl Lab, Livermore, CA USA. EM isselhardtl@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division; U.S. Department of Homeland Security's National Technical Nuclear Forensics Center; Defense Threat Reduction Agency (DTRA) [HDTRA 135636-M]; Laboratory Directed Research and Development Program at LLNL [14-ERD-082. LLNL-JRNL-648449] FX This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. The CHARISMA facility at Argonne National Laboratory is supported by the U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division. The authors are grateful for support from the U.S. Department of Homeland Security's National Technical Nuclear Forensics Center, including funding for the experimental effort of B. H. I., K. B. K., M. R. S and D. G. W. This work was supported, in part, by the Defense Threat Reduction Agency (DTRA) through Award No. HDTRA 135636-M. Manuscript preparation at LLNL was funded by the Laboratory Directed Research and Development Program at LLNL under project tracking code 14-ERD-082. LLNL-JRNL-648449. NR 45 TC 0 Z9 0 U1 5 U2 9 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 0267-9477 EI 1364-5544 J9 J ANAL ATOM SPECTROM JI J. Anal. At. Spectrom. PD MAR PY 2016 VL 31 IS 3 BP 666 EP 678 DI 10.1039/c5ja00249d PG 13 WC Chemistry, Analytical; Spectroscopy SC Chemistry; Spectroscopy GA DH5UK UT WOS:000372857300006 ER PT J AU Bell, NS Monson, TC DiAntonio, C Wu, Y AF Bell, N. S. Monson, T. C. DiAntonio, C. Wu, Y. TI Practical Colloidal Processing of Multication Ceramics SO JOURNAL OF CERAMIC SCIENCE AND TECHNOLOGY LA English DT Review DE Colloids; ceramic processing; dispersions; spark plasma sintering ID STIRRED MEDIA MILL; RUTILE-WATER INTERFACE; BARIUM-TITANATE NANOPARTICLES; METAL-OXIDE NANOPARTICLES; DENSITY-FUNCTIONAL THEORY; TITANIUM-DIOXIDE NANOPARTICLES; AQUEOUS ALUMINA SUSPENSIONS; HYDROXIDE SOL-PRECIPITATION; COMB POLYMER ARCHITECTURE; PEROVSKITE-TYPE OXIDES AB The use of colloidal processing principles in the formation of ceramic materials is well appreciated for developing homogeneous material properties in sintered products, enabling novel forming techniques for porous ceramics or 3D printing, and controlling microstructure to enable optimized material properties. The solution processing of electronic ceramic materials often involves multiple cationic elements or dopants to affect microstructure and properties. Material stability must be considered through the steps of colloidal processing to optimize desired component properties. This review provides strategies for preventing material degradation in particle synthesis, milling processes, and dispersion, with case studies of consolidation using spark plasma sintering of these systems. The prevention of multi cation corrosion in colloidal dispersions can be achieved by utilizing conditions similar to the synthesis environment or by the development of surface passivation layers. The choice of dispersing surfactants can be related to these surface states, which are of special importance for nanoparticle systems. A survey of dispersant chemistries related to some common synthesis conditions is provided for perovskite systems as an example. These principles can be applied to many colloidal systems related to electronic and optical applications. C1 [Bell, N. S.] Sandia Natl Labs, 01815 Adv Mat Lab, POB 5800 MS1411, Albuquerque, NM 87185 USA. [Monson, T. C.] Sandia Natl Labs, 01124 Nanoscale Sci, POB 5800 MS1415, Albuquerque, NM 87185 USA. [DiAntonio, C.] Sandia Natl Labs, 02734 Ferroelect Neutron Generator & Tube Lifecyc, POB 5800 MS0958, Albuquerque, NM 87185 USA. [Wu, Y.] Alfred Univ, New York State Coll Ceram, Kazuo Inamori Sch Engn, 2 Pine St, Alfred, NY 14802 USA. RP Bell, NS (reprint author), Sandia Natl Labs, 01815 Adv Mat Lab, POB 5800 MS1411, Albuquerque, NM 87185 USA. EM nsbell@sandia.gov OI Monson, Todd/0000-0002-9782-7084 FU Air Force Research Laboratory, Directed Energy Directorate, High Power Microwave Division (AFRL/RDH); U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Lockheed Martin Corporation FX The authors sincerely thank Mike Winter, Pin Yang, Tom Chavez, Lonnie Haden, Julie Gibson, Lindsey Evans, Steve Lockwood, and Kevin Ewsuk. T.C.M. would like to acknowledge Jean L. Leger, Tyler E. Stevens, and David A. Vargas for assistance with nanoparticle synthesis and electron microscopy. T.C.M. acknowledges partial support from the Air Force Research Laboratory, Directed Energy Directorate, High Power Microwave Division (AFRL/RDH).r Sandia National Laboratories is a multi-program laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 283 TC 0 Z9 0 U1 14 U2 48 PU GOLLER VERLAG GMBH PI BADEN BADEN PA ASCHMATTSTRASSE 8, D-76532 BADEN BADEN, GERMANY SN 2190-9385 J9 J CERAM SCI TECHNOL JI J. Ceram. Sci. Technol. PD MAR PY 2016 VL 7 IS 1 BP 1 EP 28 DI 10.4416/JCST2015-00025 PG 28 WC Materials Science, Ceramics SC Materials Science GA DI2HK UT WOS:000373316100001 ER PT J AU Clark, DL AF Clark, David L. TI Malcolm H. Chisholm OBITUARY SO JOURNAL OF CLUSTER SCIENCE LA English DT Biographical-Item C1 [Clark, David L.] Los Alamos Natl Lab, Los Alamos, NM USA. RP Clark, DL (reprint author), Los Alamos Natl Lab, Los Alamos, NM USA. EM dlclark@lanl.gov NR 1 TC 0 Z9 0 U1 3 U2 3 PU SPRINGER/PLENUM PUBLISHERS PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1040-7278 EI 1572-8862 J9 J CLUST SCI JI J. Clust. Sci. PD MAR PY 2016 VL 27 IS 2 BP 417 EP 419 DI 10.1007/s10876-016-0975-1 PG 3 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DH7FC UT WOS:000372956500001 ER PT J AU Rao, XL Lu, N Li, GF Nakashima, J Tang, YH Dixon, RA AF Rao, Xiaolan Lu, Nan Li, Guifen Nakashima, Jin Tang, Yuhong Dixon, Richard A. TI Comparative cell-specific transcriptomics reveals differentiation of C-4 photosynthesis pathways in switchgrass and other C-4 lineages SO JOURNAL OF EXPERIMENTAL BOTANY LA English DT Article DE C-4 photosynthesis; carbon fixation; cell-specific transcriptomics; comparative transcriptomics; switchgrass ID PANICUM-VIRGATUM L.; RNA-SEQ DATA; NADP-MALIC ENZYME; GENE-EXPRESSION; FUNCTIONAL-DIFFERENTIATION; DEVELOPMENTAL DYNAMICS; LEAF DEVELOPMENT; REFERENCE GENOME; KRANZ ANATOMY; BUNDLE-SHEATH AB Almost all C-4 plants require the co-ordination of the adjacent and fully differentiated cell types, mesophyll (M) and bundle sheath (BS). The C-4 photosynthetic pathway operates through two distinct subtypes based on how malate is decarboxylated in BS cells; through NAD-malic enzyme (NAD-ME) or NADP-malic enzyme (NADP-ME). The diverse or unique cell-specific molecular features of M and BS cells from separate C-4 subtypes of independent lineages remain to be determined. We here provide an M/BS cell type-specific transcriptome data set from the monocot NAD-ME subtype switchgrass (Panicum virgatum). A comparative transcriptomics approach was then applied to compare the M/BS mRNA profiles of switchgrass, monocot NADP-ME subtype C-4 plants maize and Setaria viridis, and dicot NAD-ME subtype Cleome gynandra. We evaluated the convergence in the transcript abundance of core components in C-4 photosynthesis and transcription factors to establish Kranz anatomy, as well as gene distribution of biological functions, in these four independent C-4 lineages. We also estimated the divergence between NAD-ME and NADP-ME subtypes of C-4 photosynthesis in the two cell types within C-4 species, including differences in genes encoding decarboxylating enzymes, aminotransferases, and metabolite transporters, and differences in the cell-specific functional enrichment of RNA regulation and protein biogenesis/homeostasis. We suggest that C-4 plants of independent lineages in both monocots and dicots underwent convergent evolution to establish C-4 photosynthesis, while distinct C-4 subtypes also underwent divergent processes for the optimization of M and BS cell co-ordination. The comprehensive data sets in our study provide a basis for further research on evolution of C-4 species. C1 [Rao, Xiaolan; Lu, Nan; Dixon, Richard A.] Univ N Texas, Dept Biol Sci, 1155 Union Circle 305220, Denton, TX 76203 USA. [Rao, Xiaolan; Tang, Yuhong; Dixon, Richard A.] US DOE, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA. [Li, Guifen; Nakashima, Jin; Tang, Yuhong] Samuel Roberts Noble Fdn Inc, 2510 Sam Noble Pkwy, Ardmore, OK 73401 USA. RP Dixon, RA (reprint author), Univ N Texas, Dept Biol Sci, 1155 Union Circle 305220, Denton, TX 76203 USA.; Dixon, RA (reprint author), US DOE, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA. EM richard.dixon@unt.edu FU Advanced Research Projects Agency-Energy (ARPA-E); US Department of Energy Bioenergy Research Centers through the Office of Biological and Environmental Research in the DOE Office of Science FX This research was supported by grants to RAD from both The Advanced Research Projects Agency-Energy (ARPA-E) and the US Department of Energy Bioenergy Research Centers, through the Office of Biological and Environmental Research in the DOE Office of Science. Genome Panicum virgatum v1.1 sequence data were produced by the US Department of Energy Joint Genome Institute http://www.jgi.doe.gov/ in collaboration with the user community. Computational resources were provided by UNT's High Performance Computing Services. We thank Drs Rajeev Azad and Chenggang Liu for critical reading of the manuscript. NR 74 TC 5 Z9 5 U1 7 U2 27 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0022-0957 EI 1460-2431 J9 J EXP BOT JI J. Exp. Bot. PD MAR PY 2016 VL 67 IS 6 BP 1649 EP 1662 DI 10.1093/jxb/erv553 PG 14 WC Plant Sciences SC Plant Sciences GA DH7NV UT WOS:000372981800007 PM 26896851 ER PT J AU Zhang, X Hirsch, CN Sekhon, RS de Leon, N Kaeppler, SM AF Zhang, Xia Hirsch, Candice N. Sekhon, Rajandeep S. de Leon, Natalia Kaeppler, Shawn M. TI Evidence for maternal control of seed size in maize from phenotypic and transcriptional analysis SO JOURNAL OF EXPERIMENTAL BOTANY LA English DT Article DE Endosperm; gene expression; maize; maternal effect; seed development; seed size ID GENE-EXPRESSION; ENDOSPERM DEVELOPMENT; RNA-SEQ; ARABIDOPSIS SEEDS; NETWORK ANALYSIS; DNA METHYLATION; IMPRINTED GENES; GRAIN WEIGHT; HEAT-STRESS; PLANTS AB Seed size is an important component of grain yield and a key determinant trait for crop domestication. The Krug Yellow Dent long-term selection experiment for large and small seed provides a valuable resource to dissect genetic and phenotypic changes affecting seed size within a common genetic background. In this study, inbred lines derived from Krug Large Seed (KLS) and Krug Small Seed (KSS) populations and reciprocal F-1 crosses were used to investigate developmental and molecular mechanisms governing seed size. Seed morphological characteristics showed striking differences between KLS and KSS inbred lines, and the reciprocal cross experiment revealed a strong maternal influence on both seed weight and seed size. Quantification of endosperm area, starchy endosperm cell size, and kernel dry mass accumulation indicated a positive correlation between seed size, endosperm cell number, and grain filling rate, and patterns of grain filling in reciprocal crosses mirrored that of the maternal parent. Consistent with the maternal contribution to seed weight, transcriptome profiling of reciprocal F-1 hybrids showed substantial similarities to the maternal parent. A set of differentially expressed genes between KLS and KSS inbreds were found, which fell into a broad number of functional categories including DNA methylation, nucleosome assembly, and heat stress response. In addition, gene co-expression network analysis of parental inbreds and reciprocal F-1 hybrids identified co-expression modules enriched in ovule development and DNA methylation, implicating these two processes in seed size determination. These results expand our understanding of seed size regulation and help to uncover the developmental and molecular basis underlying maternal control of seed size in maize. C1 [Zhang, Xia; de Leon, Natalia; Kaeppler, Shawn M.] Univ Wisconsin, Dept Agron, 1575 Linden Dr, Madison, WI 53706 USA. [Hirsch, Candice N.] Univ Minnesota, Dept Agron & Plant Genet, St Paul, MN 55108 USA. [Sekhon, Rajandeep S.] Clemson Univ, Dept Biochem & Genet, Clemson, SC 29634 USA. [de Leon, Natalia; Kaeppler, Shawn M.] Univ Wisconsin, DOE Great Lakes Bioenergy Res Ctr, 1575 Linden Dr, Madison, WI 53706 USA. RP Kaeppler, SM (reprint author), Univ Wisconsin, Dept Agron, 1575 Linden Dr, Madison, WI 53706 USA.; Kaeppler, SM (reprint author), Univ Wisconsin, DOE Great Lakes Bioenergy Res Ctr, 1575 Linden Dr, Madison, WI 53706 USA. EM smkaeppl@wisc.edu NR 65 TC 1 Z9 1 U1 12 U2 31 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0022-0957 EI 1460-2431 J9 J EXP BOT JI J. Exp. Bot. PD MAR PY 2016 VL 67 IS 6 BP 1907 EP 1917 DI 10.1093/jxb/erw006 PG 11 WC Plant Sciences SC Plant Sciences GA DH7NV UT WOS:000372981800027 PM 26826570 ER PT J AU Baines, SB Chen, X Vogt, S Fisher, NS Twining, BS Landry, MR AF Baines, Stephen B. Chen, Xi Vogt, Stefan Fisher, Nicholas S. Twining, Benjamin S. Landry, Michael R. TI Microplankton trace element contents: implications for mineral limitation of mesozooplankton in an HNLC area SO JOURNAL OF PLANKTON RESEARCH LA English DT Article DE mineral limitation; diatoms; flagellates; mesozooplankton; zinc; iron; nickel; manganese; trace metals; SXRF ID X-RAY-FLUORESCENCE; RICA UPWELLING DOME; RNA-DNA RATIOS; MARINE-PHYTOPLANKTON; ZOOPLANKTON PRODUCTION; ACARTIA-TONSA; PACIFIC-OCEAN; SILICIC-ACID; FOOD QUALITY; IRON CONTENT AB Mesozooplankton production in high-nutrient low-chlorophyll regions of the ocean may be reduced if the trace element concentrations in their food are insufficient to meet growth and metabolic demands. We used elemental microanalysis (SXRF) of single-celled plankton to determine their trace metal contents during a series of semi-Lagrangian drift studies in an HNLC upwelling region, the Costa Rica Dome (CRD). Cells from the surface mixed layer had lower Fe: S but higher Zn: S and Ni: S than those from the subsurface chlorophyll maximum at 22-30 m. Diatom Fe: S values were typically 3-fold higher than those in flagellated cells. The ratios of Zn: C in flagellates and diatoms were generally similar to each other, and to co-occurring mesozooplankton. Estimated Fe: C ratios in flagellates were lower than those in co-occurring mesozooplankton, sometimes by more than 3-fold. In contrast, Fe: C in diatoms was typically similar to that in zooplankton. RNA: DNA ratios in the CRD were low compared with other regions, and were related to total autotrophic biomass and weakly to the discrepancy between Zn: C in flagellated cells and mesozooplankton tissues. Mesozooplankton may have been affected by the trace element content of their food, even though trace metal limitation of phytoplankton was modest at best. C1 [Baines, Stephen B.] SUNY Stony Brook, Dept Ecol & Evolut, Stony Brook, NY 11789 USA. [Chen, Xi; Fisher, Nicholas S.] SUNY Stony Brook, Sch Marine & Atmospher Sci, Stony Brook, NY 11789 USA. [Vogt, Stefan] Argonne Natl Lab, Adv Photon Source, 9700 S Cass Ave, Argonne, IL 60439 USA. [Twining, Benjamin S.] Bigelow Lab Ocean Sci, East Boothbay, ME 04544 USA. [Landry, Michael R.] Univ Calif San Diego, Scripps Inst Oceanog, 9500 Gilman Dr, La Jolla, CA 92093 USA. RP Baines, SB (reprint author), SUNY Stony Brook, Dept Ecol & Evolut, Stony Brook, NY 11789 USA. EM stephen.baines@stonybrook.edu RI Vogt, Stefan/J-7937-2013 OI Vogt, Stefan/0000-0002-8034-5513 FU US National Science Foundation [OCE-0962201, OCE-1131139, OCE-0826626] FX US National Science Foundation grants OCE-0962201 and OCE-1131139 to S.B.B. and OCE-0826626 to M.R.L. NR 64 TC 3 Z9 3 U1 3 U2 10 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0142-7873 EI 1464-3774 J9 J PLANKTON RES JI J. Plankton Res. PD MAR-APR PY 2016 VL 38 IS 2 BP 256 EP 270 DI 10.1093/plankt/fbv109 PG 15 WC Marine & Freshwater Biology; Oceanography SC Marine & Freshwater Biology; Oceanography GA DH6AV UT WOS:000372874300007 PM 27275029 ER PT J AU McCalley, S Wang, YD McMurray, C Vockley, J AF McCalley, Steve Wang, Yudong McMurray, Cynthia Vockley, Jerry TI COMPLEX I DEFICIENCY IN THE CORTEX OF HUNTINGTON'S DISEASE MICE SO MOLECULAR GENETICS AND METABOLISM LA English DT Meeting Abstract CT 39th Annual Meeting of the Society-for-Inherited-Metabolic-Disorders (SIMD) CY APR 03-06, 2016 CL Ponte Vedra Beach, FL SP Soc Inherited Metab Disorders C1 [McCalley, Steve] Univ Pittsburgh, Grad Sch Publ Hlth, Human Genet, Pittsburgh, PA USA. [McCalley, Steve; Wang, Yudong; Vockley, Jerry] Univ Pittsburgh, Childrens Hosp, Med Genet, Pediat, \, Pittsburgh, PA 15260 USA. [McMurray, Cynthia] Lawrence Berkeley Natl Lab, Berkeley, CA USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 1096-7192 EI 1096-7206 J9 MOL GENET METAB JI Mol. Genet. Metab. PD MAR PY 2016 VL 117 IS 3 MA 71 BP 270 EP 270 PG 1 WC Endocrinology & Metabolism; Genetics & Heredity; Medicine, Research & Experimental SC Endocrinology & Metabolism; Genetics & Heredity; Research & Experimental Medicine GA DH3JP UT WOS:000372683600090 ER PT J AU France, RM Dimroth, F Grassman, TJ King, RR AF France, Ryan M. Dimroth, Frank Grassman, Tyler J. King, Richard R. TI Metamorphic epitaxy for multijunction solar cells SO MRS BULLETIN LA English DT Article ID DISLOCATION DENSITIES; THREADING DISLOCATION; BUFFER LAYERS; EFFICIENCY; SI; SEMICONDUCTORS; RELAXATION; IMPACT AB Multijunction solar cells have proven to be capable of extremely high efficiencies by combining multiple semiconductor materials with bandgaps tuned to the solar spectrum. Reaching the optimum set of semiconductors often requires combining high-quality materials with different lattice constants into a single device, a challenge particularly suited for metamorphic epitaxy. In this article, we describe different approaches to metamorphic multijunction solar cells, including traditional upright metamorphic, state-of-the-art inverted metamorphic, and forward-looking multijunction designs on silicon. We also describe the underlying materials science of graded buffers that enables metamorphic subcells with low dislocation densities. Following nearly two decades of research, recent efforts have demonstrated high-quality lattice-mismatched multijunction solar cells with very little performance loss related to the mismatch, enabling solar-to-electric conversion efficiencies over 45%. C1 [France, Ryan M.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Dimroth, Frank] Fraunhofer Inst Solar Energy Syst ISE, Dept Epitaxy & Solar Cells 3 5, Berlin, Germany. [Grassman, Tyler J.] Ohio State Univ, Dept Mat Sci & Engn, Columbus, OH 43210 USA. [Grassman, Tyler J.] Ohio State Univ, Dept Elect & Comp Engn, Columbus, OH 43210 USA. [King, Richard R.] Arizona State Univ, Sch Elect Comp & Energy Engn, Tempe, AZ 85287 USA. RP France, RM (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA.; Dimroth, F (reprint author), Fraunhofer Inst Solar Energy Syst ISE, Dept Epitaxy & Solar Cells 3 5, Berlin, Germany.; Grassman, TJ (reprint author), Ohio State Univ, Dept Mat Sci & Engn, Columbus, OH 43210 USA.; Grassman, TJ (reprint author), Ohio State Univ, Dept Elect & Comp Engn, Columbus, OH 43210 USA.; King, RR (reprint author), Arizona State Univ, Sch Elect Comp & Energy Engn, Tempe, AZ 85287 USA. EM ryan.france@nrel.gov; frank.dimroth@ise.fraunhofer.de; grassman.5@osu.edu; richard.r.king@asu.edu NR 56 TC 1 Z9 1 U1 3 U2 9 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0883-7694 EI 1938-1425 J9 MRS BULL JI MRS Bull. PD MAR PY 2016 VL 41 IS 3 BP 202 EP 209 DI 10.1557/mrs.2016.25 PG 8 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA DH8AW UT WOS:000373016600006 ER PT J AU Chapman, KW AF Chapman, Karena W. TI Emerging operando and x-ray pair distribution function methods for energy materials development SO MRS BULLETIN LA English DT Article ID LITHIUM-ION BATTERY; ELECTRODES; DIFFRACTION; PDF AB Our energy needs drive widespread materials research. Advances in materials characterization are critical to this research effort. Using new characterization tools that allow us to probe the atomic structure of energy materials in situ as they operate, we can identify how their structure is linked to their functional properties and performance. These fundamental insights serve as a roadmap to enhance performance in the next generation of advanced materials. In the last decade, developments in synchrotron instrumentation have made the pair distribution function (PDF) method and operando x-ray studies more readily accessible tools capable of providing valuable insights into complex materials systems. Here, the emergence of the PDF method as a versatile structure characterization tool and the further enhancement of this method through developments in operando capabilities and multivariate data analytics are described. These advances in materials characterization are demonstrated by several highlighted studies focused on energy storage in batteries. C1 [Chapman, Karena W.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Chapman, KW (reprint author), Argonne Natl Lab, Argonne, IL 60439 USA. EM chapmank@aps.anl.gov FU US Department of Energy [DE-AC02-06CH11357]; NECCES, an Energy Frontier Research Center - US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001294, DE-SC0012583]; Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub - US Department of Energy, Office of Science, Basic Energy Sciences FX Contributions from P. Chupas, K. Wiaderek, O. Borkiewicz, S. Lapidus, B. Shyam, C. Kurtz, and collaborations with H. Liu, F. Strobridge, E. Castillo-Martinez, R. Robert, and C. Grey (University of Cambridge), N. Periera, G. Amatucci (Rutgers University), N. Rajput, and K. Persson (Lawrence Berkley National Laboratory) are gratefully acknowledged. Work done at Argonne and use of the Advanced Photon Source, an Office of Science User Facility operated for the US Department of Energy Office of Science by Argonne National Laboratory, were supported by the US Department of Energy under Contract No. DE-AC02-06CH11357. Work was supported as part of NECCES, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0001294 and DE-SC0012583, and as part of the Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub funded by the US Department of Energy, Office of Science, Basic Energy Sciences. NR 23 TC 3 Z9 3 U1 11 U2 34 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0883-7694 EI 1938-1425 J9 MRS BULL JI MRS Bull. PD MAR PY 2016 VL 41 IS 3 BP 231 EP 238 DI 10.1557/mrs.2016.26 PG 8 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA DH8AW UT WOS:000373016600010 ER PT J AU Liu, W Xie, SP Lu, J AF Liu, Wei Xie, Shang-Ping Lu, Jian TI Tracking ocean heat uptake during the surface warming hiatus SO NATURE COMMUNICATIONS LA English DT Article ID EARTHS ENERGY IMBALANCE; OBJECTIVE ANALYSES; TEMPERATURE; PACIFIC; ACCELERATION; UNCERTAINTY; VARIABILITY; MODEL; ENSO AB Ocean heat uptake is observed to penetrate deep into the Atlantic and Southern Oceans during the recent hiatus of global warming. Here we show that the deep heat penetration in these two basins is not unique to the hiatus but is characteristic of anthropogenic warming and merely reflects the depth of the mean meridional overturning circulation in the basin. We find, however, that heat redistribution in the upper 350m between the Pacific and Indian Oceans is closely tied to the surface warming hiatus. The Indian Ocean shows an anomalous warming below 50m during hiatus events due to an enhanced heat transport by the Indonesian throughflow in response to the intensified trade winds in the equatorial Pacific. Thus, the Pacific and Indian Oceans are the key regions to track ocean heat uptake during the surface warming hiatus. C1 [Liu, Wei; Xie, Shang-Ping] Univ Calif San Diego, Scripps Inst Oceanog, CASPO, 9500 Gilman Dr, La Jolla, CA 92093 USA. [Lu, Jian] Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99354 USA. RP Liu, W (reprint author), Univ Calif San Diego, Scripps Inst Oceanog, CASPO, 9500 Gilman Dr, La Jolla, CA 92093 USA. EM wel109@ucsd.edu FU NSF [AGS-1249145]; U.S. Department of Energy Office of Science Biological and Environmental Research (BER) as part of the Regional and Global Climate Modeling program FX This work is supported by NSF AGS-1249145. Jian Lu was supported by the U.S. Department of Energy Office of Science Biological and Environmental Research (BER) as part of the Regional and Global Climate Modeling program. The CESM model output data are publicly available on the Earth System Grid (ESG). For observational and reanalysis data, the EN4 data are publicly available at http://hadobs.metoffice.com/en4/, the Ishii data are publicly available at http://rda.ucar.edu/data sets/ds285.3/ and http://www.data.jma.go.jp/gmd/kaiyou/english/ohc/ohc_data_en.html, the WOA data are publicly available at https://www.nodc.noaa.gov/OC5/3M_HEAT_CONTENT/ and the ECMWF ORAS4 data are publicly available at https://climatedataguide.ucar.edu/climate-data/oras4-ecmwf-oceanreanalys is-and-derived-ocean-heat-content and Integrated Climate Data Center -ICDC. NR 38 TC 9 Z9 9 U1 5 U2 17 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD MAR PY 2016 VL 7 AR 10926 DI 10.1038/ncomms10926 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH9ZF UT WOS:000373153800001 PM 27025666 ER PT J AU Mefford, JT Rong, X Abakumov, AM Hardin, WG Dai, S Kolpak, AM Johnston, KP Stevenson, KJ AF Mefford, J. Tyler Rong, Xi Abakumov, Artem M. Hardin, William G. Dai, Sheng Kolpak, Alexie M. Johnston, Keith P. Stevenson, Keith J. TI Water electrolysis on La1-xSrxCoO3-delta perovskite electrocatalysts SO NATURE COMMUNICATIONS LA English DT Article ID ION DIFFUSION-COEFFICIENTS; TRANSITION-METAL OXIDES; OXYGEN EVOLUTION REACTION; ALKALINE-SOLUTION; REDOX REACTIONS; COBALT OXIDE; REDUCTION; ELECTRODES; CATALYSTS; OXIDATION AB Perovskite oxides are attractive candidates as catalysts for the electrolysis of water in alkaline energy storage and conversion systems. However, the rational design of active catalysts has been hampered by the lack of understanding of the mechanism of water electrolysis on perovskite surfaces. Key parameters that have been overlooked include the role of oxygen vacancies, B-O bond covalency, and redox activity of lattice oxygen species. Here we present a series of cobaltite perovskites where the covalency of the Co-O bond and the concentration of oxygen vacancies are controlled through Sr2+ substitution into La1 - xSrxCoO3 - delta. We attempt to rationalize the high activities of La1 - xSrxCoO3 - delta through the electronic structure and participation of lattice oxygen in the mechanism of water electrolysis as revealed through ab initio modelling. Using this approach, we report a material, SrCoO2.7, with a high, room temperature-specific activity and mass activity towards alkaline water electrolysis. C1 [Mefford, J. Tyler; Stevenson, Keith J.] Univ Texas Austin, Dept Chem, Austin, TX 78712 USA. [Rong, Xi; Kolpak, Alexie M.] MIT, Dept Mech Engn, Cambridge, MA 02139 USA. [Abakumov, Artem M.; Stevenson, Keith J.] Skolkovo Inst Sci & Technol, Ctr Electrochem Energy Storage, Moscow 143026, Russia. [Abakumov, Artem M.] Univ Antwerp, Electron Microscopy Mat Sci, Groenenborgerlaan 171, B-2020 Antwerp, Belgium. [Hardin, William G.; Johnston, Keith P.; Stevenson, Keith J.] Univ Texas Austin, Texas Mat Inst, Austin, TX 78712 USA. [Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Johnston, Keith P.] Univ Texas Austin, Dept Chem Engn, Austin, TX 78712 USA. [Stevenson, Keith J.] Univ Texas Austin, Ctr Nano & Mol Sci & Technol, Austin, TX 78712 USA. RP Stevenson, KJ (reprint author), Univ Texas Austin, Dept Chem, Austin, TX 78712 USA.; Stevenson, KJ (reprint author), Skolkovo Inst Sci & Technol, Ctr Electrochem Energy Storage, Moscow 143026, Russia.; Stevenson, KJ (reprint author), Univ Texas Austin, Texas Mat Inst, Austin, TX 78712 USA.; Stevenson, KJ (reprint author), Univ Texas Austin, Ctr Nano & Mol Sci & Technol, Austin, TX 78712 USA. EM K.Stevenson@skoltech.ru RI Dai, Sheng/K-8411-2015 OI Dai, Sheng/0000-0002-8046-3931 FU R.A. Welch Foundation [F-1529, F-1319]; Skoltech-MIT Center; Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences FX Financial support for this work was provided by the R.A. Welch Foundation (grants F-1529 and F-1319). X.R. and A.M.K. acknowledge support from the Skoltech-MIT Center for Electrochemical Energy Storage. Computations were performed using computational resources from XSEDE and NERSC. S.D. was supported as part of the Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences. We thank D.W. Redman for help with the RHE measurements. NR 62 TC 17 Z9 17 U1 49 U2 132 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD MAR PY 2016 VL 7 AR 11053 DI 10.1038/ncomms11053 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH3YC UT WOS:000372721700001 PM 27006166 ER PT J AU Shi, CZ Dubois, M Chen, Y Cheng, L Ramezani, H Wang, Y Zhang, X AF Shi, Chengzhi Dubois, Marc Chen, Yun Cheng, Lei Ramezani, Hamidreza Wang, Yuan Zhang, Xiang TI Accessing the exceptional points of parity-time symmetric acoustics SO NATURE COMMUNICATIONS LA English DT Article ID OPTICAL ISOLATION AB Parity-time (PT) symmetric systems experience phase transition between PT exact and broken phases at exceptional point. These PT phase transitions contribute significantly to the design of single mode lasers, coherent perfect absorbers, isolators, and diodes. However, such exceptional points are extremely difficult to access in practice because of the dispersive behaviour of most loss and gain materials required in PT symmetric systems. Here we introduce a method to systematically tame these exceptional points and control PT phases. Our experimental demonstration hinges on an active acoustic element that realizes a complex-valued potential and simultaneously controls the multiple interference in the structure. The manipulation of exceptional points offers new routes to broaden applications for PT symmetric physics in acoustics, optics, microwaves and electronics, which are essential for sensing, communication and imaging. C1 [Shi, Chengzhi; Dubois, Marc; Ramezani, Hamidreza; Wang, Yuan; Zhang, Xiang] Univ Calif Berkeley, NSF Nano Scale Sci & Engn Ctr NSEC, 3112 Etcheverry Hall, Berkeley, CA 94720 USA. [Chen, Yun; Cheng, Lei] Fudan Univ, Dept Microelect, State Key Lab ASIC & Syst, Shanghai 201203, Peoples R China. [Zhang, Xiang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Zhang, Xiang] King Abdulaziz Univ, Dept Phys, Jeddah 21589, Saudi Arabia. RP Zhang, X (reprint author), Univ Calif Berkeley, NSF Nano Scale Sci & Engn Ctr NSEC, 3112 Etcheverry Hall, Berkeley, CA 94720 USA.; Zhang, X (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA.; Zhang, X (reprint author), King Abdulaziz Univ, Dept Phys, Jeddah 21589, Saudi Arabia. EM xiang@berkeley.edu RI Wang, Yuan/F-7211-2011; Shi, Chengzhi/N-1485-2016 OI Shi, Chengzhi/0000-0003-0799-213X FU Office of Naval Research (ONR) MURI program [N00014-13-1-0631] FX This research was supported by the Office of Naval Research (ONR) MURI program under Grant No. N00014-13-1-0631. NR 31 TC 16 Z9 16 U1 13 U2 27 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD MAR PY 2016 VL 7 AR 11110 DI 10.1038/ncomms11110 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DI1XO UT WOS:000373290500001 PM 27025443 ER PT J AU van der Plas, F Manning, P Allan, E Scherer-Lorenzen, M Verheyen, K Wirth, C Zavala, MA Hector, A Ampoorter, E Baeten, L Barbaro, L Bauhus, J Benavides, R Benneter, A Berthold, F Bonal, D Bouriaud, O Bruelheide, H Bussotti, F Carnol, M Castagneyrol, B Charbonnier, Y Coomes, D Coppi, A Bastias, CC Dawud, SM De Wandeler, H Domisch, T Finer, L Gessler, A Granier, A Grossiord, C Guyot, V Hattenschwiler, S Jactel, H Jaroszewicz, B Joly, FX Jucker, T Koricheva, J Milligan, H Muller, S Muys, B Nguyen, D Pollastrini, M Raulund-Rasmussen, K Selvi, F Stenlid, J Valladares, F Vesterdal, L Zielinski, D Fischer, M AF van der Plas, Fons Manning, Peter Allan, Eric Scherer-Lorenzen, Michael Verheyen, Kris Wirth, Christian Zavala, Miguel A. Hector, Andy Ampoorter, Evy Baeten, Lander Barbaro, Luc Bauhus, Juergen Benavides, Raquel Benneter, Adam Berthold, Felix Bonal, Damien Bouriaud, Olivier Bruelheide, Helge Bussotti, Filippo Carnol, Monique Castagneyrol, Bastien Charbonnier, Yohan Coomes, David Coppi, Andrea Bastias, Cristina C. Dawud, Seid Muhie De Wandeler, Hans Domisch, Timo Finer, Leena Gessler, Arthur Granier, Andre Grossiord, Charlotte Guyot, Virginie Haettenschwiler, Stephan Jactel, Herve Jaroszewicz, Bogdan Joly, Francois-Xavier Jucker, Tommaso Koricheva, Julia Milligan, Harriet Mueller, Sandra Muys, Bart Nguyen, Diem Pollastrini, Martina Raulund-Rasmussen, Karsten Selvi, Federico Stenlid, Jan Valladares, Fernando Vesterdal, Lars Zielinski, Dawid Fischer, Markus TI Jack-of-all-trades effects drive biodiversity-ecosystem multifunctionality relationships in European forests SO NATURE COMMUNICATIONS LA English DT Article ID SOIL MICROBIAL BIOMASS; SPECIES RICHNESS; STATISTICAL INEVITABILITY; CURRENT KNOWLEDGE; EXTRACTION METHOD; PLANT DIVERSITY; SERVICES; NITROGEN; CARBON; CHALLENGES AB There is considerable evidence that biodiversity promotes multiple ecosystem functions (multifunctionality), thus ensuring the delivery of ecosystem services important for human well-being. However, the mechanisms underlying this relationship are poorly understood, especially in natural ecosystems. We develop a novel approach to partition biodiversity effects on multifunctionality into three mechanisms and apply this to European forest data. We show that throughout Europe, tree diversity is positively related with multifunctionality when moderate levels of functioning are required, but negatively when very high function levels are desired. For two well-known mechanisms, 'complementarity' and 'selection', we detect only minor effects on multifunctionality. Instead a third, so far overlooked mechanism, the 'jack-of-all-trades' effect, caused by the averaging of individual species effects on function, drives observed patterns. Simulations demonstrate that jack-of-all-trades effects occur whenever species effects on different functions are not perfectly correlated, meaning they may contribute to diversity-multifunctionality relationships in many of the world's ecosystems. C1 [van der Plas, Fons; Manning, Peter; Allan, Eric; Fischer, Markus] Univ Bern, Inst Plant Sci, Altenbergrain 21, CH-3013 Bern, Switzerland. [van der Plas, Fons; Manning, Peter] Biodivers & Climate Res Ctr, Senckenberg Gesell Naturforsch, Senckenberganlage 25, D-60325 Frankfurt, Germany. [Scherer-Lorenzen, Michael; Benavides, Raquel; Mueller, Sandra] Univ Freiburg, Fac Biol, Geobot, Schanzlestr 1, D-79104 Freiburg, Germany. [Verheyen, Kris; Ampoorter, Evy; Baeten, Lander] Univ Ghent, Dept Forest & Water Management, Forest & Nat Lab, Coupure Links 653, B-9000 Ghent, Belgium. [Wirth, Christian] Univ Leipzig, Systemat Bot & Funct Biodivers, Johannisallee 21, D-04103 Leipzig, Germany. [Wirth, Christian; Bruelheide, Helge] German Ctr Integrat Biodivers Res iDiv, Deutsch Pl 5e, D-04103 Leipzig, Germany. [Zavala, Miguel A.] Univ Alcala De Henares, Dept Life Sci, Forest Ecol & Restorat Grp, Madrid 28805, Spain. [Hector, Andy] Univ Oxford, Dept Plant Sci, S Parks Rd, Oxford OX1 3RB, England. [Baeten, Lander] Univ Ghent, Dept Biol, Terr Ecol Unit, KL Ledeganckstr 35, B-9000 Ghent, Belgium. [Barbaro, Luc; Castagneyrol, Bastien; Charbonnier, Yohan; Guyot, Virginie; Jactel, Herve] INRA, UMR BIOGECO 1202, F-33610 Cestas, France. [Barbaro, Luc; Castagneyrol, Bastien; Charbonnier, Yohan; Guyot, Virginie; Jactel, Herve] Univ Bordeaux, BIOGECO, UMR 1202, F-33600 Pessac, France. [Bauhus, Juergen; Benneter, Adam] Univ Freiburg, Fac Environm & Nat Resources, Chair Silviculture, Fahnenbergpl, D-79085 Freiburg, Germany. [Berthold, Felix; Bruelheide, Helge] Univ Halle Wittenberg, Inst Biol, Geobotany & Bot Garden, Kirchtor 1, D-06108 Halle, Germany. [Bonal, Damien; Granier, Andre] INRA, UMR EEF, Allee Arboretum, F-54280 Champenoux, France. [Bouriaud, Olivier] Stefan Cel Mare Univ Suceava, Fac Forestry, Univ St 13, Suceava 720229, Romania. [Bussotti, Filippo; Coppi, Andrea; Pollastrini, Martina; Selvi, Federico] Univ Florence, Dept Agrifood Prod & Environm Sci DISPAA, Lab Appl & Environm Bot, Via G La Pira 4, I-50121 Florence, Italy. [Carnol, Monique] Univ Liege, Lab Plant & Microbial Ecol, Bot B22,Chemin Vallee 4, B-4000 Liege, Belgium. [Coomes, David; Jucker, Tommaso] Univ Cambridge, Dept Plant Sci, Forest Ecol & Conservat, Downing St, Cambridge CB2 3EA, England. [Bastias, Cristina C.; Valladares, Fernando] CSIC, MNCN, Natl Museum Nat Sci, Dept Biogeog & Global Change, Serrano 115 Bis, Madrid 28006, Spain. [Dawud, Seid Muhie; Raulund-Rasmussen, Karsten; Vesterdal, Lars] Univ Copenhagen, Dept Geosci & Nat Resource Management, Rolighedsvej 23, DK-1958 Frederiksberg C, Denmark. [De Wandeler, Hans; Muys, Bart] Univ Leuven, Div Forest Nat & Landscape, Celestijnenlaan 200E, B-3001 Louvain, Belgium. [Domisch, Timo; Finer, Leena] Nat Resources Inst Finland, POB 68, FI-80101 Joensuu, Finland. [Gessler, Arthur] Swiss Fed Res Inst WSL, Zurcherstr 111, CH-8903 Birmensdorf, Switzerland. [Grossiord, Charlotte] Los Alamos Natl Lab, Earth & Environm Sci Div, POB 1663, Los Alamos, NM 87545 USA. [Guyot, Virginie] INRA, DYNAFOR, UMR 1201, F-31326 Castanet Tolosan, France. [Haettenschwiler, Stephan; Joly, Francois-Xavier] Univ Montpellier, Univ Paul Valery Montpellier EPHE, CEFE, UMR 5175, 1919 Route Mende, F-34293 Montpellier, France. [Jaroszewicz, Bogdan; Zielinski, Dawid] Univ Warsaw, Fac Biol, Bialowieza Geobotan Stn, Ilji Miecznikowa 1, PL-02096 Warsaw, Poland. [Koricheva, Julia; Milligan, Harriet] Royal Holloway Univ London, Sch Biol Sci, Egham TW20 0EX, Surrey, England. [Nguyen, Diem; Stenlid, Jan] Swedish Univ Agr Sci, Dept Forest Mycol & Plant Pathol, POB 7026, SE-75007 Uppsala, Sweden. [Valladares, Fernando] Univ Rey Juan Carlos, ESCET, Dept Biol & Geol, C Tulipan S-N, Mostoles 28933, Spain. RP van der Plas, F (reprint author), Univ Bern, Inst Plant Sci, Altenbergrain 21, CH-3013 Bern, Switzerland.; van der Plas, F (reprint author), Biodivers & Climate Res Ctr, Senckenberg Gesell Naturforsch, Senckenberganlage 25, D-60325 Frankfurt, Germany. EM fonsvanderplas@gmail.com RI Bauhus, Jurgen/G-4449-2013; Gessler, Arthur/C-7121-2008; Bouriaud, Olivier/C-4700-2011; Raulund-Rasmussen, Karsten/E-8424-2015; Fischer, Markus/C-6411-2008; Manning, Peter/I-6523-2012; Suceava, USV/E-8611-2011; Zavala, Miguel/H-3603-2015; Vesterdal, Lars/D-5227-2011; Pollastrini, Martina/N-7989-2014; Bastias, Cristina C. /C-3657-2017; Coppi, Andrea/D-2886-2016; OI Bauhus, Jurgen/0000-0002-9673-4986; Gessler, Arthur/0000-0002-1910-9589; Bouriaud, Olivier/0000-0002-8046-466X; Raulund-Rasmussen, Karsten/0000-0003-1573-1167; Fischer, Markus/0000-0002-5589-5900; Manning, Peter/0000-0002-7940-2023; Zavala, Miguel/0000-0003-1456-0132; Vesterdal, Lars/0000-0003-0309-3735; Pollastrini, Martina/0000-0003-0959-9489; Bastias, Cristina C. /0000-0002-2479-2001; Castagneyrol, Bastien/0000-0001-8795-7806; DAWUD, SEID MUHIE/0000-0002-5587-945X; Coppi, Andrea/0000-0003-4760-8403; Benavides, Raquel/0000-0003-2328-5371; Nguyen, Diem/0000-0002-9680-5772; Jucker, Tommaso/0000-0002-0751-6312; Baeten, Lander/0000-0003-4262-9221 FU European Union [265171] FX We thank Sophia Ratcliffe for managing the FunDivEurope database. The research leading to these results received funding from the European Union Seventh Framework Programme (FP7/2007-2013) under grant agreement no. 265171. NR 47 TC 5 Z9 6 U1 43 U2 87 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD MAR PY 2016 VL 7 AR 11109 DI 10.1038/ncomms11109 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH6GJ UT WOS:000372888700001 PM 27010076 ER PT J AU Zhang, L Lei, DS Smith, JM Zhang, M Tong, HM Zhang, X Lu, ZY Liu, JK Alivisatos, AP Ren, G AF Zhang, Lei Lei, Dongsheng Smith, Jessica M. Zhang, Meng Tong, Huimin Zhang, Xing Lu, Zhuoyang Liu, Jiankang Alivisatos, A. Paul Ren, Gang TI Three-dimensional structural dynamics and fluctuations of DNA-nanogold conjugates by individual-particle electron tomography SO NATURE COMMUNICATIONS LA English DT Article ID NEGATIVE-STAINING PROTOCOL; EMPIRICAL FORCE-FIELD; MOLECULAR-DYNAMICS; SINGLE-MOLECULE; NUCLEIC-ACIDS; MICROSCOPY; LIPOPROTEINS; SIMULATION; VISUALIZATION; NANOPARTICLES AB DNA base pairing has been used for many years to direct the arrangement of inorganic nanocrystals into small groupings and arrays with tailored optical and electrical properties. The control of DNA-mediated assembly depends crucially on a better understanding of three-dimensional structure of DNA-nanocrystal-hybridized building blocks. Existing techniques do not allow for structural determination of these flexible and heterogeneous samples. Here we report cryo-electron microscopy and negative-staining electron tomography approaches to image, and three-dimensionally reconstruct a single DNA-nanogold conjugate, an 84-bp double-stranded DNA with two 5-nm nanogold particles for potential substrates in plasmon-coupling experiments. By individual-particle electron tomography reconstruction, we obtain 14 density maps at similar to 2-nm resolution. Using these maps as constraints, we derive 14 conformations of dsDNA by molecular dynamics simulations. The conformational variation is consistent with that from liquid solution, suggesting that individual-particle electron tomography could be an expected approach to study DNA-assembling and flexible protein structure and dynamics. C1 [Zhang, Lei; Lei, Dongsheng; Zhang, Meng; Tong, Huimin; Zhang, Xing; Lu, Zhuoyang; Ren, Gang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Zhang, Lei; Zhang, Xing] Xi An Jiao Tong Univ, Sch Sci, Dept Appl Phys, Xian 710049, Peoples R China. [Smith, Jessica M.; Alivisatos, A. Paul] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Smith, Jessica M.; Alivisatos, A. Paul] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Smith, Jessica M.; Alivisatos, A. Paul] Univ Calif Berkeley, Dept Mat Sci, Berkeley, CA 94720 USA. [Lu, Zhuoyang; Liu, Jiankang] Xi An Jiao Tong Univ, Minist Educ, Key Lab Biomed Informat Engn, Ctr Mitochondrial Biol & Med, Xian 710049, Peoples R China. [Lu, Zhuoyang; Liu, Jiankang] Xi An Jiao Tong Univ, Sch Life Sci & Technol, Xian 710049, Peoples R China. [Lu, Zhuoyang; Liu, Jiankang] Xi An Jiao Tong Univ, Frontier Inst Sci & Technol, Xian 710049, Peoples R China. [Alivisatos, A. Paul] Univ Calif Berkeley, Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. RP Ren, G (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. EM gren@lbl.gov RI Alivisatos , Paul /N-8863-2015; Liu, Jiankang/A-1610-2011; Zhang, Lei/G-6427-2012 OI Alivisatos , Paul /0000-0001-6895-9048; Zhang, Lei/0000-0002-4880-824X FU National Science Foundation [DMR-1344290]; Office of Science, Office of Basic Energy Sciences of the US Department of Energy [DE-AC02-05CH11231]; National Heart, Lung, and Blood Institute of the National Institutes of Health [R01HL115153]; National Institute of General Medical Sciences of the National Institutes of Health [R01GM104427]; National Natural Science Foundation of China [11504287]; Young Talent Support Plan of Xi'an Jiaotong University; National Basic Research Program of Ministry of Science and Technology, China [2015CB553602] FX We thank Drs Qian Chen and Phillip Geissler for their discussion and comments, and Mr Matthew Rames for editing. This material is based upon work supported by the National Science Foundation under grant DMR-1344290. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences of the US Department of Energy under contract no. DE-AC02-05CH11231. G.R. is supported by the National Heart, Lung, and Blood Institute of the National Institutes of Health (no. R01HL115153) and the National Institute of General Medical Sciences of the National Institutes of Health (no. R01GM104427). L.Z. is partly supported by National Natural Science Foundation of China (no. 11504287) and Young Talent Support Plan of Xi'an Jiaotong University; Z.L. and J.L. are partly supported by the National Basic Research Program of Ministry of Science and Technology, China (no. 2015CB553602). NR 49 TC 2 Z9 2 U1 14 U2 34 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD MAR PY 2016 VL 7 AR 11083 DI 10.1038/ncomms11083 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DI0AS UT WOS:000373157800001 PM 27025159 ER PT J AU Nesaraja, CD McCutchan, EA AF Nesaraja, C. D. McCutchan, E. A. TI Nuclear Data Sheets for A=41 SO NUCLEAR DATA SHEETS LA English DT Article ID LOW-LYING STATES; THERMAL-NEUTRON CAPTURE; VECTOR ANALYZING POWER; HIGH-SPIN STATES; INELASTIC PROTON-SCATTERING; POSITIVE PION-PRODUCTION; BETA-DELAYED PROTONS; N=28 SHELL CLOSURE; CIRCULAR-POLARIZATION CORRELATION; ANGULAR-DISTRIBUTION MEASUREMENTS AB Available information pertaining to the nuclear structure of all nuclei with mass numbers A=41 ranging from Al (Z=13) to Ti (Z=22) are presented. The experimental reaction and decay data are evaluated and any inconsistencies or discrepancies are noted. The adopted values for various level properties (such as the spin, parity and and halflife) and gamma properties (energy, intensity and multipole character) are given. Since the prior evaluation several new measurements have expanded our knowledge of A=41 nuclides. The half-life of the ground state of Si-41 has been determined and a single excited state identified. Excited levels in P-41 have been observed for the firstt ime. In Cl-41, seven new excited states have been identified in deep inelastic and heavy ion transfer reactions. Half-lifes for four states in Ar-41 have been updated and additional levels with gammas have been included from a new measurement using the multiple ion transfer reaction. In Ca-41 via charge-exchange reaction measurements, several new excited states were observed. A number of new resonances in K-41 have been identified via the (p,gamma) reaction. There remains a significant discrepancy in the half-life of the first excited state (980 keV) in K-41, with measurements differing by more than an order of magnitude. Transfer reactions suggest that this M1 transition should be l-forbidden, however, several measurements yield a lifetime which suggests a sizable M1 strength. Further measurements to resolve the current conflicts would be beneficial. C1 [Nesaraja, C. D.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [McCutchan, E. A.] Brookhaven Natl Lab, Natl Nucl Data Ctr, Upton, NY 11973 USA. RP Nesaraja, CD (reprint author), Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. FU Office of Nuclear Physics, Office of Science, US Department of Energy [DE-AC02-98CH10946, DE-AC05-00OR22725] FX Research sponsored by Office of Nuclear Physics, Office of Science, US Department of Energy, under contract DE-AC02-98CH10946 (E.M.), DE-AC05-00OR22725 (C.N.). NR 528 TC 1 Z9 1 U1 3 U2 5 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD MAR-APR PY 2016 VL 133 BP 1 EP 219 DI 10.1016/j.nds.2016.02.001 PG 219 WC Physics, Nuclear SC Physics GA DH6GM UT WOS:000372889000001 ER PT J AU Perfetti, CM Rearden, BT Martin, WR AF Perfetti, Christopher M. Rearden, Bradley T. Martin, William R. TI SCALE Continuous-Energy Eigenvalue Sensitivity Coefficient Calculations SO NUCLEAR SCIENCE AND ENGINEERING LA English DT Article DE SCALE; TSUNAMI; eigenvalue sensitivity coefficients ID MONTE-CARLO METHOD AB The need to model geometrically complex systems with improved ease of use and fidelity and the desire to extend the Tools for Sensitivity and UNcertainty Analysis Methodology Implementation (TSUNAMI) analysis to advanced applications have motivated the development of a methodology for calculating sensitivity coefficients in continuous-energy (CE) Monte Carlo applications. The Contributon-Linked eigenvalue sensitivity/Uncertainty estimation via Track length importance CHaracterization (CLUTCH) and Iterated Fission Probability (IFP) eigenvalue sensitivity methods were recently implemented in the CE KENO framework of the SCALE code system to enable TSUNAMI-3D to perform eigenvalue sensitivity calculations using CE Monte Carlo methods. This paper provides a detailed description of the theory behind the CLUTCH method and describes in detail its implementation. This work also explores the improvements in eigenvalue sensitivity coefficient accuracy that can be gained through use of CE sensitivity methods and compares several sensitivity methods in terms of computational efficiency and memory requirements. The IFP and CLUTCH methods produced sensitivity coefficient estimates that matched, and in some cases exceeded, the accuracy of those produced using the multigroup TSUNAMI-3D approach. The CLUTCH method was found to calculate sensitivity coefficients with the highest degree of efficiency and the lowest computational memory footprint for the problems examined. C1 [Perfetti, Christopher M.; Rearden, Bradley T.] Oak Ridge Natl Lab, POB 2008,MS 6170, Oak Ridge, TN 37831 USA. [Martin, William R.] Univ Michigan, Dept Nucl Engn & Radiol Sci, 2355 Bonisteel Blvd, Ann Arbor, MI 48109 USA. RP Perfetti, CM (reprint author), Oak Ridge Natl Lab, POB 2008,MS 6170, Oak Ridge, TN 37831 USA. EM perfetticm@ornl.gov FU U.S. Department of Energy (DOE) Nuclear Criticality Safety Program; National Nuclear Security Administration FX This work was supported by the U.S. Department of Energy (DOE) Nuclear Criticality Safety Program, funded and managed by the National Nuclear Security Administration for DOE. The authors would like to thank L. M. Petrie, Jr., and K. B. Bekar for their assistance in implementing the CE TSUNAMI sequence. NR 19 TC 1 Z9 1 U1 0 U2 0 PU AMER NUCLEAR SOC PI LA GRANGE PK PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA SN 0029-5639 EI 1943-748X J9 NUCL SCI ENG JI Nucl. Sci. Eng. PD MAR PY 2016 VL 182 IS 3 BP 332 EP 353 PG 22 WC Nuclear Science & Technology SC Nuclear Science & Technology GA DH9DS UT WOS:000373097200005 ER PT J AU Perfetti, CM Rearden, BT AF Perfetti, Christopher M. Rearden, Bradley T. TI Development of a Generalized Perturbation Theory Method for Sensitivity Analysis Using Continuous-Energy Monte Carlo Methods SO NUCLEAR SCIENCE AND ENGINEERING LA English DT Article DE Generalized perturbation theory; sensitivity coefficients; Monte Carlo AB The sensitivity and uncertainty analysis tools of the Oak Ridge National Laboratory SCALE nuclear modeling and simulation code system that have been developed over the last decade have proven indispensable for numerous application and design studies for nuclear criticality safety and reactor physics. SCALE contains tools for analyzing the uncertainty in the eigenvalue of critical systems with realistic three-dimensional Monte Carlo simulations but currently can only quantify the uncertainty in important neutronic parameters such as multigroup cross sections, fuel fission rates, activation rates, and neutron fluence rates with one- or two-dimensional models. A more complete understanding of the sources of uncertainty in these design-limiting parameters using high-fidelity models could lead to improvements in process optimization and reactor safety and help inform regulators when setting operational safety margins. A novel approach for calculating eigenvalue sensitivity coefficients, known as the CLUTCH (Contributon-Linked eigenvalue sensitivity/Uncertainty estimation via Track length importance CHaracterization) method, was recently explored as academic research and has been found to accurately and rapidly calculate sensitivity coefficients in criticality safety applications. The work presented here describes an extension of the CLUTCH method, known as the GEneralized Adjoint Responses in Monte Carlo (GEAR MC) method, that enables the calculation of sensitivity coefficients and uncertainty analysis for a generalized set of neutronic responses using high-fidelity continuous-energy Monte Carlo calculations. Several criticality safety systems were examined to demonstrate proof of principle for the GEAR-MC method, and GEAR-MC produced response sensitivity coefficients that agreed well with reference direct perturbation sensitivity coefficients. C1 [Perfetti, Christopher M.; Rearden, Bradley T.] Oak Ridge Natl Lab, POB 2008,MS 6170, Oak Ridge, TN 37831 USA. RP Perfetti, CM (reprint author), Oak Ridge Natl Lab, POB 2008,MS 6170, Oak Ridge, TN 37831 USA. EM perfetticm@ornl.gov FU U.S. Department of Energy (DOE) Nuclear Criticality Safety Program; National Nuclear Security Administration FX The authors would like to thank M. Williams for his guidance regarding the theory of generalized response sensitivity calculations. This work was supported by the U.S. Department of Energy (DOE) Nuclear Criticality Safety Program, funded and managed by the National Nuclear Security Administration for DOE. NR 13 TC 1 Z9 1 U1 0 U2 0 PU AMER NUCLEAR SOC PI LA GRANGE PK PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA SN 0029-5639 EI 1943-748X J9 NUCL SCI ENG JI Nucl. Sci. Eng. PD MAR PY 2016 VL 182 IS 3 BP 354 EP 368 PG 15 WC Nuclear Science & Technology SC Nuclear Science & Technology GA DH9DS UT WOS:000373097200006 ER PT J AU Bardella, P Chow, WW Montrosset, I AF Bardella, Paolo Chow, Weng W. Montrosset, Ivo TI Design and Analysis of Enhanced Modulation Response in Integrated Coupled Cavities DBR Lasers Using Photon-Photon Resonance SO PHOTONICS LA English DT Article DE semiconductor laser diode; monolithically-integrated coupled-cavity DBR lasers; integrated optics; photonic integrated circuits (PICs); direct modulation; small-signal modulation bandwidth; eye diagram; DBR laser; optical injection-locking ID LOCKED SEMICONDUCTOR-LASERS; INJECTION-GRATING DESIGN; MU M WAVELENGTH; BANDWIDTH ENHANCEMENT; SPEED ENHANCEMENT; NOISE-REDUCTION; GHZ; DYNAMICS; MULTISECTION; IMPROVEMENT AB In the last few decades, various solutions have been proposed to increase the modulation bandwidth and, consequently, the transmission bit-rate of semiconductor lasers. In this manuscript, we discuss a design procedure for a recently proposed laser cavity realized with the monolithic integration of two distributed Bragg reflector (DBR) lasers allowing one to extend the modulation bandwidth. Such an extension is obtained introducing in the dynamic response a photon-photon resonance (PPR) at a frequency higher than the modulation bandwidth of the corresponding single-section laser. Design guidelines will be proposed, and dynamic small and large signal simulations results, calculated using a finite difference traveling wave (FDTW) numerical simulator, will be discussed to confirm the design results. The effectiveness of the design procedure is verified in a structure with PPR frequency at 35GHz allowing one to obtain an open eye diagram for a non-return-to-zero (NRZ) digital signal up to 80 GHz. Furthermore, the investigation of the rich dynamics of this structure shows that with proper bias conditions, it is possible to obtain also a tunable self-pulsating signal in a frequency range related to the PPR design. C1 [Bardella, Paolo; Montrosset, Ivo] Politecn Torino, Dipartimento Elettron & Telecomunicazioni, Corso Duca Abruzzi 24, I-10129 Turin, Italy. [Chow, Weng W.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Bardella, P (reprint author), Politecn Torino, Dipartimento Elettron & Telecomunicazioni, Corso Duca Abruzzi 24, I-10129 Turin, Italy. EM paolo.bardella@polito.it; wwchow@sandia.gov; ivo.montrosset@polito.it NR 34 TC 2 Z9 2 U1 1 U2 6 PU MDPI AG PI BASEL PA POSTFACH, CH-4005 BASEL, SWITZERLAND SN 2304-6732 J9 Photonics JI Photonics PD MAR PY 2016 VL 3 IS 1 AR 4 DI 10.3390/photonics3010004 PG 14 WC Optics SC Optics GA DI2FC UT WOS:000373310100004 ER PT J AU Freissinet, C Getty, SA Trainer, MG Glavin, DP Mahaffy, PR McLain, HL Benna, M AF Freissinet, C. Getty, S. A. Trainer, M. G. Glavin, D. P. Mahaffy, P. R. McLain, H. L. Benna, M. TI Evaluation of the robustness of chromatographic columns in a simulated highly radiative Jovian environment SO PLANETARY AND SPACE SCIENCE LA English DT Article DE Capillary columns stationary phases; Radiations; Electrons; Icy moons; Gas chromatography mass spectrometry; Organics ID IN-SITU ANALYSIS; GAS-CHROMATOGRAPHY; COMETARY NUCLEUS AB Gas chromatography mass spectrometry (GCMS) is currently the most widely used analytical method for in situ investigation of organic molecules in space environments. Various types of GC column stationary phases have been, are currently, or will be used at the different solar system bodies including Mars, the Moon, Titan and comets. However, GCMS use in highly radiative environments such as Jupiter and its moons has never been explored and raises questions on the robustness of GC columns and stationary phases to extreme radiation. In this study, several types of GC columns were irradiated by high-energy electrons and protons in order to simulate the harsh conditions of a journey through Jupiter's radiation belts. Post-irradiation characterization shows that the three types of columns investigated, DB-5MS, CP-Chirasil-Dex CB and GS-GasPro, maintained their peak resolution and general separation performance after the radiation exposure. These results demonstrate that GCMS techniques can be applied to study the space environment of Jupiter's icy moons with no need for substantial radiation shielding of the columns. (c) 2016 Elsevier Ltd. All rights reserved. C1 [Freissinet, C.; Getty, S. A.; Trainer, M. G.; Glavin, D. P.; Mahaffy, P. R.; McLain, H. L.; Benna, M.] NASA, Goddard Space Flight Ctr, Planetary Environm Lab, Greenbelt, MD 20771 USA. [Freissinet, C.] Oak Ridge Associated Univ, NASA, Postdoctoral Program, Oak Ridge, TN 37830 USA. [Benna, M.] Univ Maryland Baltimore Cty, Ctr Space Sci & Technol, Baltimore, MD 21250 USA. RP Freissinet, C (reprint author), NASA, Goddard Space Flight Ctr, Planetary Environm Lab, Greenbelt, MD 20771 USA. EM caroline.freissinet@nasa.gov RI Benna, Mehdi/F-3489-2012; Glavin, Daniel/D-6194-2012 OI Glavin, Daniel/0000-0001-7779-7765 NR 14 TC 1 Z9 1 U1 2 U2 7 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0032-0633 J9 PLANET SPACE SCI JI Planet Space Sci. PD MAR PY 2016 VL 122 BP 38 EP 45 DI 10.1016/j.pss.2016.01.004 PG 8 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DH4RS UT WOS:000372773700004 ER PT J AU Erbilgin, O Sutter, M Kerfeld, CA AF Erbilgin, Onur Sutter, Markus Kerfeld, Cheryl A. TI The Structural Basis of Coenzyme A Recycling in a Bacterial Organelle SO PLOS BIOLOGY LA English DT Article ID B-12-DEPENDENT 1,2-PROPANEDIOL DEGRADATION; SEROVAR TYPHIMURIUM LT2; MULTIPLE SEQUENCE ALIGNMENT; PROTEIN FAMILIES DATABASE; METHANOSARCINA-THERMOPHILA; CARBONIC-ANHYDRASE; SALMONELLA-TYPHIMURIUM; MOLECULAR GRAPHICS; BETA-LACTAMASE; MICROCOMPARTMENT AB Bacterial Microcompartments (BMCs) are proteinaceous organelles that encapsulate critical segments of autotrophic and heterotrophic metabolic pathways; they are functionally diverse and are found across 23 different phyla. The majority of catabolic BMCs (metabolosomes) compartmentalize a common core of enzymes to metabolize compounds via a toxic and/or volatile aldehyde intermediate. The core enzyme phosphotransacylase (PTAC) recycles Coenzyme A and generates an acyl phosphate that can serve as an energy source. The PTAC predominantly associated with metabolosomes (PduL) has no sequence homology to the PTAC ubiquitous among fermentative bacteria (Pta). Here, we report two high-resolution PduL crystal structures with bound substrates. The PduL fold is unrelated to that of Pta; it contains a dimetal active site involved in a catalytic mechanism distinct from that of the housekeeping PTAC. Accordingly, PduL and Pta exemplify functional, but not structural, convergent evolution. The PduL structure, in the context of the catalytic core, completes our understanding of the structural basis of cofactor recycling in the metabolosome lumen. C1 [Erbilgin, Onur; Kerfeld, Cheryl A.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Sutter, Markus; Kerfeld, Cheryl A.] Michigan State Univ, MSU DOE Plant Res Lab, E Lansing, MI 48824 USA. [Sutter, Markus; Kerfeld, Cheryl A.] Michigan State Univ, Dept Biochem & Mol Biol, E Lansing, MI 48824 USA. [Sutter, Markus; Kerfeld, Cheryl A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA. RP Kerfeld, CA (reprint author), Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA.; Kerfeld, CA (reprint author), Michigan State Univ, MSU DOE Plant Res Lab, E Lansing, MI 48824 USA.; Kerfeld, CA (reprint author), Michigan State Univ, Dept Biochem & Mol Biol, E Lansing, MI 48824 USA.; Kerfeld, CA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA. EM ckerfeld@lbl.gov OI erbilgin, onur/0000-0002-6122-6156 FU National Institutes of Health, National Institute of Allergy and Infectious Diseases (NIAID) [1R01AI114975-01] FX This work was funded by the National Institutes of Health, National Institute of Allergy and Infectious Diseases (NIAID) (http://www.niaid.nih.gov/) grant 1R01AI114975-01. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 61 TC 2 Z9 2 U1 1 U2 4 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1545-7885 J9 PLOS BIOL JI PLoS. Biol. PD MAR PY 2016 VL 14 IS 3 AR e1002399 DI 10.1371/journal.pbio.1002399 PG 20 WC Biochemistry & Molecular Biology; Biology SC Biochemistry & Molecular Biology; Life Sciences & Biomedicine - Other Topics GA DH8JB UT WOS:000373038200015 PM 26959993 ER PT J AU Hershey, DM Ren, XF Melnyk, RA Browne, PJ Ozyamak, E Jones, SR Chang, MCY Hurley, JH Komeili, A AF Hershey, David M. Ren, Xuefeng Melnyk, Ryan A. Browne, Patrick J. Ozyamak, Ertan Jones, Stephanie R. Chang, Michelle C. Y. Hurley, James H. Komeili, Arash TI MamO Is a Repurposed Serine Protease that Promotes Magnetite Biomineralization through Direct Transition Metal Binding in Magnetotactic Bacteria SO PLOS BIOLOGY LA English DT Article ID CUPRIAVIDUS-NECATOR H16; MAGNETOSPIRILLUM-MAGNETICUM; PHYLOGENETIC ANALYSIS; MAGNETOSOME MEMBRANE; CRYSTAL-STRUCTURE; HIGH-THROUGHPUT; STRAIN AMB-1; ION FRET; REVEALS; EVOLUTION AB Many living organisms transform inorganic atoms into highly ordered crystalline materials. An elegant example of such biomineralization processes is the production of nano-scale magnetic crystals in magnetotactic bacteria. Previous studies implicated the involvement of two putative serine proteases, MamE and MamO, during the early stages of magnetite formation in Magnetospirillum magneticum AMB-1. Here, using genetic analysis and X-ray crystallography, we show that MamO has a degenerate active site, rendering it incapable of protease activity. Instead, MamO promotes magnetosome formation through two genetically distinct, noncatalytic activities: activation of MamE-dependent proteolysis of biomineralization factors and direct binding to transition metal ions. By solving the structure of the protease domain bound to a metal ion, we identify a surface-exposed di-histidine motif in MamO that contributes to metal binding and show that it is required to initiate biomineralization in vivo. Finally, we find that pseudoproteases are widespread in magnetotactic bacteria and that they have evolved independently in three separate taxa. Our results highlight the versatility of protein scaffolds in accommodating new biochemical activities and provide unprecedented insight into the earliest stages of biomineralization. C1 [Hershey, David M.; Browne, Patrick J.; Ozyamak, Ertan; Komeili, Arash] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Ren, Xuefeng; Chang, Michelle C. Y.; Hurley, James H.; Komeili, Arash] Univ Calif Berkeley, Dept Mol & Cellular Biol, Berkeley, CA 94720 USA. [Ren, Xuefeng; Hurley, James H.; Komeili, Arash] Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. [Melnyk, Ryan A.; Chang, Michelle C. Y.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Jones, Stephanie R.; Chang, Michelle C. Y.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Hurley, James H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. RP Komeili, A (reprint author), Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA.; Komeili, A (reprint author), Univ Calif Berkeley, Dept Mol & Cellular Biol, Berkeley, CA 94720 USA.; Komeili, A (reprint author), Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. EM komeili@berkeley.edu FU National Institutes of Health [R01GM084122]; Office of Naval Research [N000141310421]; UC Office of the President, Multicampus Research Programs and Initiatives grant [MR-15-328599]; Program for Breakthrough Biomedical Research; Sandler Foundation; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX DMH and AK are supported by grants from the National Institutes of Health (www.nih.gov R01GM084122) and the Office of Naval Research (www.onr.navy.mil N000141310421). Beamline 8.3.1 at the Advanced Light Source, LBNL, is supported by the UC Office of the President, Multicampus Research Programs and Initiatives grant MR-15-328599 (http://www.ucop.edu/research-grantsprogram/programs/multi-campus-resear ch-programsand-initiatives.html) and the Program for Breakthrough Biomedical Research (http://pbbr.ucsf.edu/), which is partially funded by the Sandler Foundation. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy (http://science.energy.gov/bes/) under Contract No. DE-AC02-05CH11231. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 57 TC 4 Z9 4 U1 7 U2 15 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1545-7885 J9 PLOS BIOL JI PLoS. Biol. PD MAR PY 2016 VL 14 IS 3 AR e1002402 DI 10.1371/journal.pbio.1002402 PG 23 WC Biochemistry & Molecular Biology; Biology SC Biochemistry & Molecular Biology; Life Sciences & Biomedicine - Other Topics GA DH8JB UT WOS:000373038200018 PM 26981620 ER PT J AU Chen, M Bu, LT Alahuhta, M Brunecky, R Xu, Q Lunin, VV Brady, JW Crowley, MF Himmel, ME Bomble, YJ AF Chen, Mo Bu, Lintao Alahuhta, Markus Brunecky, Roman Xu, Qi Lunin, Vladimir V. Brady, John W. Crowley, Michael F. Himmel, Michael E. Bomble, Yannick J. TI Strategies to reduce end-product inhibition in family 48 glycoside hydrolases SO PROTEINS-STRUCTURE FUNCTION AND BIOINFORMATICS LA English DT Article DE glycoside hydrolases; product inhibition; biofuels; cellulose; molecular dynamics ID FREE-ENERGY DIFFERENCES; CLOSTRIDIUM-THERMOCELLUM CELLULOSOME; PROCESSIVE ENDOCELLULASE CELF; NONEQUILIBRIUM MEASUREMENTS; CRYSTAL-STRUCTURE; CELLULASE CE148F; FORCE-FIELDS; CELLULOLYTICUM; COMPONENT; DYNAMICS AB Family 48 cellobiohydrolases are some of the most abundant glycoside hydrolases in nature. They are able to degrade cellulosic biomass and therefore serve as good enzyme candidates for biofuel production. Family 48 cellulases hydrolyze cellulose chains via a processive mechanism, and produce end products composed primarily of cellobiose as well as other cellooligomers (dp <= 4). The challenge of utilizing cellulases in biofuel production lies in their extremely slow turnover rate. A factor contributing to the low enzyme activity is suggested to be product binding to enzyme and the resulting performance inhibition. In this study, we quantitatively evaluated the product inhibitory effect of four family 48 glycoside hydrolases using molecular dynamics simulations and product expulsion free-energy calculations. We also suggested a series of single mutants of the four family 48 glycoside hydrolases with theoretically reduced level of product inhibition. The theoretical calculations provide a guide for future experimental studies designed to produce mutant cellulases with enhanced activity. C1 [Chen, Mo; Brady, John W.] Cornell Univ, Dept Food Sci, Ithaca, NY 14853 USA. [Bu, Lintao; Alahuhta, Markus; Brunecky, Roman; Xu, Qi; Lunin, Vladimir V.; Crowley, Michael F.; Himmel, Michael E.; Bomble, Yannick J.] Natl Renewable Energy Lab, Golden, CO USA. RP Bomble, YJ (reprint author), Natl Renewable Energy Lab, Golden, CO USA. EM Yannick.bomble@nrel.gov FU BioEnergy Science Center; Office of Biological and Environmental Research in the DOE Office of Science FX We thank Gregg T. Beckham from the National Renewable Energy Laboratory for useful discussions at the inception of this project. We also thank the BioEnergy Science Center for funding. The BioEnergy Science Center is a U.S. Department of Energy Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science. NR 41 TC 0 Z9 0 U1 5 U2 12 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0887-3585 EI 1097-0134 J9 PROTEINS JI Proteins PD MAR PY 2016 VL 84 IS 3 BP 295 EP 304 DI 10.1002/prot.24965 PG 10 WC Biochemistry & Molecular Biology; Biophysics SC Biochemistry & Molecular Biology; Biophysics GA DI2TP UT WOS:000373352100001 PM 26572060 ER PT J AU Benioff, P AF Benioff, Paul TI Space- and time-dependent scaling of numbers in mathematical structures: effects on physical and geometric quantities SO QUANTUM INFORMATION PROCESSING LA English DT Article DE Number structure scaling; Fiber bundles; Gauge theory; Theory and experiment ID COHERENT THEORY; UNIVERSE AB The relationship between the foundations of mathematics and physics is a topic of of much interest. This paper continues this exploration by examination of the effect of space- and time- dependent number scaling on theoretical descriptions of some physical and geometric quantities. Fiber bundles provide a good framework to introduce a space- and time- or space-time-dependent number scaling field. The effect of the scaling field on a few nonlocal physical and geometric quantities is described. The effect on gauge theories is to introduce a new complex scalar field into the derivatives appearing in Lagrangians. U(1) invariance of Lagrangian terms does not affect the real part of the scaling field. For this field, any mass is possible. The scaling field is also shown to affect quantum wave packets and path lengths, and geodesic equations even on flat space. Scalar fields described so far in physics are possible candidates for the scaling field. The lack of direct evidence for the field in physics restricts the scaling field in that the gradient of the field must be close to zero in a local region of cosmological space and time. There are no restrictions outside the region. It is also seen that the scaling field does not affect comparisons of computation or measurements outputs with one another. However, it does affect the assignment of numerical values to the outputs of computations or measurements. These are needed because theory predictions are in terms of numerical values. C1 [Benioff, Paul] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RP Benioff, P (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. EM pbenioff@anl.gov FU US Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357] FX This material is based upon work supported by the US Department of Energy, Office of Science, Office of Nuclear Physics, under contract number DE-AC02-06CH11357. NR 34 TC 0 Z9 0 U1 1 U2 1 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1570-0755 EI 1573-1332 J9 QUANTUM INF PROCESS JI Quantum Inf. Process. PD MAR PY 2016 VL 15 IS 3 SI SI BP 1081 EP 1102 DI 10.1007/s11128-015-1084-z PG 22 WC Physics, Multidisciplinary; Physics, Mathematical SC Physics GA DH6BX UT WOS:000372877100006 ER PT J AU Carson, CG Stute, M Ji, YH Polle, R Reboul, A Lackner, KS AF Carson, Cantwell G. Stute, Martin Ji, Yinghuang Polle, Roseline Reboul, Arthur Lackner, Klaus S. TI Invalidation of the Intracavity Optogalvanic Method for Radiocarbon Detection SO RADIOCARBON LA English DT Article DE Intracavity optogalvanic spectroscopy (ICOGS); radiocarbon; laser spectroscopy; monitoring verification and accounting ID ABSOLUTE FREQUENCIES; LASING TRANSITIONS; MASS-SPECTROMETRY; C-14 ANALYSIS; SPECTROSCOPY; AMS; SENSITIVITY; LASER AB The intracavity optogalvanic spectroscopy (ICOGS) method has been reported to quantify radiocarbon at subambient levels (<1 part per trillion). ICOGS uses a gas sample that is ionized in a low-pressure glow discharge located inside a (CO2)-C-14 laser cavity to detect changes in the discharge current under periodic modulation of the laser power to determine the (CO2)-C-14 concentration of the sample. When claims of detection thresholds below ambient levels were not verified by other researchers, we constructed a theoretical analysis to resolve differences between these conflicting reports and built and tested an ICOGS system to establish a lower limit of detection. Using a linear absorbance model of the background contribution of (CO2)-C-12 and data from the HITRAN database, we estimate that the limit of detection (3 sigma(x)) is close to 1.5x10(4) Modern. By measuring a 1.5x10(4) Modern enriched CO2 sample in a cavity modulation ICOGS system without a clear signal, we conclude that for this system the limit of detection for ICOGS must be above 1.5x10(4). The implications for previous ICOGS reports are discussed. C1 [Carson, Cantwell G.; Ji, Yinghuang; Lackner, Klaus S.] Columbia Univ, Earth & Environm Engn Dept, New York, NY USA. [Carson, Cantwell G.] US DOE, Natl Energy Technol Lab, Pittsburgh, PA USA. [Stute, Martin] Barnard Coll, Dept Environm Sci, New York, NY USA. [Polle, Roseline; Reboul, Arthur] Ecole Polytech, Palaiseau, Ile De France, France. [Polle, Roseline] Univ London Imperial Coll Sci Technol & Med, London, England. [Reboul, Arthur] Neoen, Paris, Ile De France, France. [Lackner, Klaus S.] Arizona State Univ, Ctr Negat Carbon Emiss, Tempe, AZ USA. RP Carson, CG (reprint author), Columbia Univ, Earth & Environm Engn Dept, New York, NY USA.; Carson, CG (reprint author), US DOE, Natl Energy Technol Lab, Pittsburgh, PA USA. EM carsonc@netl.doe.gov FU National Energy Technology Laboratory at the U.S. Dept. of Energy [DE-FE0001535]; Columbia University Research Initiative for Science and Engineering; Alliance Program FX The authors thank The National Energy Technology Laboratory at the U.S. Dept. of Energy (Award DE-FE0001535) and the Columbia University Research Initiative for Science and Engineering for their generous support and Philipp Stoelting for technical consultation. Roseline Polle and Arthur Reboul also thank the Alliance Program for their sponsorship. NR 26 TC 2 Z9 2 U1 2 U2 2 PU UNIV ARIZONA DEPT GEOSCIENCES PI TUCSON PA RADIOCARBON 4717 E FORT LOWELL RD, TUCSON, AZ 85712 USA SN 0033-8222 EI 1945-5755 J9 RADIOCARBON JI Radiocarbon PD MAR PY 2016 VL 58 IS 1 BP 213 EP 225 DI 10.1017/RDC.2016.5 PG 13 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DH5LG UT WOS:000372829700019 ER PT J AU Carson, CG AF Carson, Cantwell G. TI Response to "Comment on "Invalidation of the Intracavity Optogalvanic Method for Radiocarbon Detection'" by Daniel E Murnick SO RADIOCARBON LA English DT Editorial Material ID SPECTROSCOPY AB Our results, when taken alongside those of two other research groups, appear to invalidate the early positive results for intracavity optogalvanic spectroscopy (ICOGS) and its detection of radiocarbon. Daniel Murnick, whose lab published those early results, has directed a comment setting out the perceived shortcomings of our article and the reasons that the results do not constitute invalidation, as our article claims. Absent support from his own findings or published literature, his various counterclaims regarding our experimental procedure appear to constitute only his considered professional opinion and the largest confounder highlighted by our research is not even mentioned. The preponderance of documented evidence regarding ICOGS clearly supports the null hypothesis and in our opinion, nothing in Murnick's comment indicates otherwise. C1 [Carson, Cantwell G.] Natl Energy Technol Lab, Pittsburgh, PA USA. RP Carson, CG (reprint author), Natl Energy Technol Lab, Pittsburgh, PA USA. EM carsonc@netl.doe.gov NR 10 TC 0 Z9 0 U1 1 U2 1 PU UNIV ARIZONA DEPT GEOSCIENCES PI TUCSON PA RADIOCARBON 4717 E FORT LOWELL RD, TUCSON, AZ 85712 USA SN 0033-8222 EI 1945-5755 J9 RADIOCARBON JI Radiocarbon PD MAR PY 2016 VL 58 IS 1 BP 231 EP 232 DI 10.1017/RDC.2016.11 PG 2 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DH5LG UT WOS:000372829700021 ER PT J AU Rivero, AJ Sathre, R Navarro, JG AF Jimenez Rivero, Ana Sathre, Roger Garcia Navarro, Justo TI Life cycle energy and material flow implications of gypsum plasterboard recycling in the European Union SO RESOURCES CONSERVATION AND RECYCLING LA English DT Article DE Gypsum plasterboard; European Union; Material flow analysis; Life cycle assessment (LCA); Primary energy; GHG emissions ID CONSTRUCTION; WASTE AB Turning waste into a resource is a way to increase resource use efficiency and close the material loop of a circular economy. Gypsum plasterboard is well suited for this, because the raw material calcium sulphate dihydrate (CaSO4 center dot 2H(2)O) can repeatedly change its properties through a reversible hydration reaction. The waste hierarchy is applied when plasterboard is recycled instead of landfilled, which contributes to the European 2020 target of 70% recovery of construction and demolition (C&D) waste, as defined in the Directive 2008/98/EC on Waste. This paper evaluates the energy and climate impacts of different levels of plasterboard recycling. First, we formulate a life cycle model of gypsum mass flows in the European Union (EU-27) in the reference year 2013. This model constitutes the basis of the quantitative scenario analysis. Secondly, we assess the material flows, energy use and greenhouse gas (GHG) emissions in different recycling scenarios. We compare the current situation ("2013 base case") to two scenarios: a worst case scenario of 0% recycled gypsum ("Zero recycling case"), and a best case scenario of zero gypsum waste sent to landfill, corresponding to 18.7% recycled gypsum in new plasterboard ("High recycling case"). We find no significant variation between scenarios in terms of life cycle energy use, as lower impacts from gypsum mining, transport of natural gypsum and final disposal in the best case scenario are balanced by the energy for the transport of plasterboard waste and recycled gypsum and for material pre-processing during manufacturing. In contrast, life cycle GHG emissions are lower as recycling increases, largely driven by the degradation of plasterboard lining paper in landfills. (C) 2016 Elsevier B.V. All rights reserved. C1 [Jimenez Rivero, Ana; Garcia Navarro, Justo] Univ Politecn Madrid, Res Grp Sustainabil Construct & Ind GiSCI, Ciudad Univ S-N, E-28040 Madrid, Spain. [Sathre, Roger] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Anal & Environm Impacts Div, Berkeley, CA 94720 USA. RP Rivero, AJ (reprint author), Univ Politecn Madrid, Res Grp Sustainabil Construct & Ind GiSCI, Ciudad Univ S-N, E-28040 Madrid, Spain. EM ana.jimenez@upm.es RI Jimenez-Rivero, Ana/M-1542-2014; GARCIA NAVARRO, JUSTO/L-9419-2014 OI Jimenez-Rivero, Ana/0000-0003-4013-2334; GARCIA NAVARRO, JUSTO/0000-0002-5268-1587 FU European Commission-DG Environment through the Life + programme [LIFE11 ENV/BE/001039]; US Department of Energy [DE-AC02-05CH11231] FX This study has been performed under the framework of the GtoG project, supported by the European Commission-DG Environment through the Life + programme; under contract number LIFE11 ENV/BE/001039. Lawrence Berkeley National Laboratory is supported by the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 46 TC 3 Z9 3 U1 10 U2 30 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0921-3449 EI 1879-0658 J9 RESOUR CONSERV RECY JI Resour. Conserv. Recycl. PD MAR-APR PY 2016 VL 108 BP 171 EP 181 DI 10.1016/j.resconrec.2016.01.014 PG 11 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA DH6YZ UT WOS:000372939300014 ER PT J AU Tonn, B Hawkins, B Rose, E AF Tonn, Bruce Hawkins, Beth Rose, Erin TI Assessment of the American Recovery and Reinvestment Act Upon the Department of Energy Weatherization Assistance Program SO REVIEW OF POLICY RESEARCH LA English DT Article DE energy; governance; civil society; national governance; low-income weatherization; American Recovery and Reinvestment Act (ARRA); United States ID DAVIS-BACON; COSTS AB The Department of Energy (DOE) administers the national low-income Weatherization Assistance Program (WAP). Under this program, DOE provides grants to states (grantees), which then provide grants to local weatherization agencies (subgrantees), to weatherize income-eligible homes for free. The American Recovery and Reinvestment Act (ARRA) of 2009 allocated $5 billion in funding to WAP, a very significant increase from an annual appropriation that ranged in the $200-250 million range for many years. As part of a major evaluation of WAP, states and local weatherization agencies were surveyed, in part, to assess their experiences during the ARRA period. The substantial funding increase created a number of issues for the national weatherization network: the political visibility of their programs increased significantly, organizational responsibilities were shifted, new laws and regulations were passed that impacted their programs, media attention of their programs increased, federal oversight of their programs increased; and programmatic costs increased because of the increased oversight and because ARRA required WAP to operate under the provisions of the Davis-Bacon Act of 1931. There was some concern within the national weatherization network that the influx of ARRA funds would permanently damage nonfederal funding leveraging relationships. However, two-thirds of grantees and over 40% of subgrantees stated that they believe that the long-term impacts of ARRA on leveraging relationships will be positive. C1 [Tonn, Bruce; Hawkins, Beth] Three3 Inc, Knoxville, TN USA. [Rose, Erin] Oak Ridge Natl Lab, Div Environm Sci, POB 2008, Oak Ridge, TN 37831 USA. RP Tonn, B (reprint author), Three3 Inc, Knoxville, TN USA. NR 26 TC 1 Z9 1 U1 0 U2 0 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1541-132X EI 1541-1338 J9 REV POLICY RES JI Rev. Policy Res. PD MAR PY 2016 VL 33 IS 2 SI SI BP 178 EP 200 DI 10.1111/ropr.12164 PG 23 WC Political Science; Public Administration SC Government & Law; Public Administration GA DH8QZ UT WOS:000373062300005 ER PT J AU Ginocchio, JN AF Ginocchio, Joseph N. TI Pseudospin Symmetry as a Bridge between Hadrons and Nuclei SO SYMMETRY-BASEL LA English DT Article DE quarks in nuclei; relatiistic symmetry in nuclei; pseuspin symmetry AB Atomic nuclei exhibit approximate pseudospin symmetry. We review the arguments that this symmetry is a relativistic symmetry. The condition for this symmetry is that the sum of the vector and scalar potentials in the Dirac Hamiltonian is a constant. We give the generators of pseudospin symmetry. We review some of the predictions that follow from the insight that pseudospin symmetry has relativistic origins . We show that approximate pseudospin symmetry in nuclei predicts approximate spin symmetry in anti-nucleon scattering from nuclei. Since QCD sum rules predict that the sum of the scalar and vector potentials is small, we discuss the quark origins of pseudospin symmetry in nuclei and spin symmetry in hadrons. C1 [Ginocchio, Joseph N.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87505 USA. RP Ginocchio, JN (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87505 USA. EM gino@lanl.gov FU US Department of Energy [W-7405-ENG-36] FX This research was supported by the US Department of Energy, Contract No. W-7405-ENG-36. NR 28 TC 0 Z9 0 U1 4 U2 8 PU MDPI AG PI BASEL PA POSTFACH, CH-4005 BASEL, SWITZERLAND SN 2073-8994 J9 SYMMETRY-BASEL JI Symmetry-Basel PD MAR PY 2016 VL 8 IS 3 DI 10.3390/sym8030016 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH8OD UT WOS:000373052700007 ER PT J AU Eschbaumer, M Stenfeldt, C Pacheco, JM Rekant, SI Arzt, J AF Eschbaumer, Michael Stenfeldt, Carolina Pacheco, Juan M. Rekant, Steven I. Arzt, Jonathan TI Effect of storage conditions on subpopulations of peripheral blood T lymphocytes isolated from naive cattle and cattle infected with foot-and-mouth disease virus SO VETERINARY CLINICAL PATHOLOGY LA English DT Article DE Cryopreservation; flow cytometry; immunophenotyping; peripheral blood mononuclear cells; storage ID MONONUCLEAR-CELLS; FLOW-CYTOMETRY; CRYOPRESERVATION; RESPONSES; FRESH; LIMITATIONS AB BackgroundImmunophenotyping of blood lymphocytes by flow cytometry is important in infectious disease research. In animal experiments and other longitudinal studies, the processing, prompt staining, and analysis of fresh samples is a logistical challenge and daily assay variation can confound data interpretation. ObjectiveThis study examined the feasibility of cryopreservation and deferred analysis of bovine peripheral blood T lymphocytes from normal or infected animals. MethodsPeripheral blood mononuclear cells were collected from 4 naive Holstein steers and 4 steers infected with foot-and-mouth-disease virus serotype Asia1. Identical aliquots were labeled and analyzed immediately, labeled for deferred analysis, or stored at -70 degrees C or over liquid nitrogen for up to 3 weeks before labeling. ResultsFreezing of unlabeled cells induced statistically significant changes in phenotypic recognition. In infected animals, the T-cell population increased by 28% and CD8(+) T cells by 32%, while total CD3(+) cells decreased by 16%, and CD4(+) T cells decreased by 12%. Subsequent storage of frozen cells for the duration of the study, however, had no significant effect. There was less than 20% relative change in subpopulation sizes, and storage at -70 degrees C or over liquid nitrogen was equivalent. ConclusionsDepending on the objectives and practical limitations of a study, deferred labeling of peripheral blood lymphocytes can be a viable option. Although frozen storage of lymphocytes can introduce some artifactual distortion of relative cell populations, frozen cells can be maintained in storage until all samples in a longitudinal study can be analyzed in batch under standardized conditions and without introducing further bias. C1 [Eschbaumer, Michael; Stenfeldt, Carolina; Pacheco, Juan M.; Rekant, Steven I.; Arzt, Jonathan] USDA ARS, Plum Isl Anim Dis Ctr, FADRU, POB 848, Greenport, NY 11944 USA. [Eschbaumer, Michael; Stenfeldt, Carolina; Rekant, Steven I.] Oak Ridge Inst Sci & Educ, PIADC Res Participat Program, Oak Ridge, TN USA. RP Arzt, J (reprint author), USDA ARS, Plum Isl Anim Dis Ctr, FADRU, POB 848, Greenport, NY 11944 USA. EM jonathan.arzt@ars.usda.gov OI Stenfeldt, Carolina/0000-0002-2074-3886; Pacheco, Juan/0000-0001-5477-0201; Arzt, Jonathan/0000-0002-7517-7893 FU CRIS project (USDA, Agricultural Research Service [ARS]) [1940-32000-057-00D]; Science and Technology Directorate of the U.S. Department of Homeland Security [HSHQPM-13-X-00131]; PIADC Research Participation Program fellowships FX This work was funded in part by CRIS project 1940-32000-057-00D (USDA, Agricultural Research Service [ARS]), as well as through an interagency agreement with the Science and Technology Directorate of the U.S. Department of Homeland Security under Award Number HSHQPM-13-X-00131. Michael Eschbaumer, Carolina Stenfeldt, and Steven Rekant are recipients of PIADC Research Participation Program fellowships, administered by the Oak Ridge Institute for Science and Education (ORISE) through an interagency agreement with the U.S. Department of Energy. The authors thank William Golde, Jared Patch, and Mary Kenney of USDA/ARS, PIADC, for their help with setting up the flow cytometry workflow, and the Animal Resource Branch at PIADC for assistance with animal procedures. The content is solely the responsibility of the authors and does not necessarily represent the official views of the USDA or any other federal entity. The sponsors had no involvement in the study design, in the collection, analysis, and interpretation of data; in the writing of the manuscript; and in the decision to submit the manuscript for publication. NR 16 TC 2 Z9 2 U1 0 U2 1 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0275-6382 EI 1939-165X J9 VET CLIN PATH JI Vet. Clin. Pathol. PD MAR PY 2016 VL 45 IS 1 BP 110 EP 115 DI 10.1111/vcp.12327 PG 6 WC Veterinary Sciences SC Veterinary Sciences GA DH6TW UT WOS:000372925900013 PM 26802284 ER PT J AU Robertson, EJ Battigelli, A Proulx, C Mannige, RV Haxton, TK Yun, LS Whitelam, S Zuckermann, RN AF Robertson, Ellen J. Battigelli, Alessia Proulx, Caroline Mannige, Ranjan V. Haxton, Thomas K. Yun, Lisa Whitelam, Stephen Zuckermann, Ronald N. TI Design, Synthesis, Assembly, and Engineering of Peptoid Nanosheets SO ACCOUNTS OF CHEMICAL RESEARCH LA English DT Review ID SOLID-PHASE SYNTHESIS; SECONDARY-STRUCTURE; CYCLIC PEPTOIDS; SIDE-CHAINS; OLIGOMERS; POLYMERS; GLYCINES); DISCOVERY; CRYSTALS; HELICES AB Two-dimensional (2D) atomically defined organic nanomaterials are an important material class with broad applications. However, few general synthetic methods exist to produce such materials in high yields and to precisely functionalize them. One strategy to form ordered 2D organic nanomaterials is through the supramolecular assembly of sequence-defined synthetic polymers. Peptoids, one such class of polymer, are designable bioinspired heteropolymers whose main-chain length and monomer sequence can be precisely controlled. We have recently discovered that individual peptoid polymers with a simple sequence of alternating hydrophobic and ionic monomers can self-assemble into highly ordered, free-floating nanosheets. A detailed understanding of their molecular structure and supramolecular assembly dynamics provides a robust platform for the discovery of new classes of nanosheets with tunable properties and novel applications. In this Account, we discuss the discovery, characterization, assembly, molecular modeling, and functionalization of peptoid nanosheets. The fundamental properties of peptoid nanosheets, their mechanism of formation, and their application as robust scaffolds for molecular recognition and as templates for the growth of inorganic minerals have been probed by an arsenal of experimental characterization techniques (e.g., scanning probe, electron, and optical microscopy, X-ray diffraction, surface-selective vibrational spectroscopy, and surface tensiometry) and computational techniques (coarse-grained and atomistic modeling). Peptoid nanosheets are supramolecular assemblies of 16-42-mer chains that form molecular bilayers. They span tens of microns in lateral dimensions and freely float in water. Their component chains are highly ordered, with chains nearly fully extended and packed parallel to one another as a result of hydrophobic and electrostatic interactions. Nanosheets form via a novel interface-catalyzed monolayer collapse mechanism. Peptoid chains first assemble into a monolayer at either an air water or oil water interface, on which peptoid chains extend, order, and pack into a brick-like pattern. Upon mechanical compression of the interface, the monolayer buckles into stable bilayer structures. Recent work has focused on the design of nanosheets with tunable properties and functionality. They are readily engineerable, as functional monomers can be readily incorporated onto the nanosheet surface or into the interior. For example, functional hydrophilic "loops" have been displayed on the surfaces of nanosheets. These loops can interact with specific protein targets, serving as a potentially general platform for molecular recognition. Nanosheets can also bind metal ions and serve as 2D templates for mineral growth. Through our understanding of the formation mechanism, along with predicted features ascertained from molecular modeling, we aim to further design and synthesize nanosheets as robust protein mimetics with the potential for unprecedented functionality and stability. C1 [Robertson, Ellen J.; Battigelli, Alessia; Proulx, Caroline; Mannige, Ranjan V.; Haxton, Thomas K.; Yun, Lisa; Whitelam, Stephen; Zuckermann, Ronald N.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Zuckermann, RN (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. EM rnzuckermann@lbl.gov FU Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC02-05CH11231]; Defense Threat Reduction Agency [IACRO-B0845281]; Natural Sciences and Engineering Research Council of Canada (NSERC PDF) FX This work was performed at the Molecular Foundry at Lawrence Berkeley National Laboratory, supported by the Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy, under Contract DE-AC02-05CH11231. R.V.M., T.K.H., E.J.R., A.B., R.N.Z., and S.W. were supported by the Defense Threat Reduction Agency under Contract IACRO-B0845281. C.P. was also supported by the Natural Sciences and Engineering Research Council of Canada (NSERC PDF). NR 33 TC 9 Z9 9 U1 33 U2 82 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0001-4842 EI 1520-4898 J9 ACCOUNTS CHEM RES JI Accounts Chem. Res. PD MAR PY 2016 VL 49 IS 3 BP 379 EP 389 DI 10.1021/acs.accounts.5b00439 PG 11 WC Chemistry, Multidisciplinary SC Chemistry GA DG9GV UT WOS:000372391700004 PM 26741294 ER PT J AU Hybertsen, MS Venkataraman, L AF Hybertsen, Mark S. Venkataraman, Latha TI Structure-Property Relationships in Atomic-Scale Junctions: Histograms and Beyond SO ACCOUNTS OF CHEMICAL RESEARCH LA English DT Review ID SINGLE-MOLECULE JUNCTIONS; ELECTRONIC TRANSPORT; CONDUCTANCE; THERMOELECTRICITY; CIRCUITS; LEVEL AB Over the past 10 years, there has been tremendous progress in the measurement, modeling and understanding of structure function relationships in single molecule junctions. Numerous research groups have addressed significant scientific questions, directed both to conductance phenomena at the single molecule level and to the fundamental chemistry that controls junction functionality. Many different functionalities have been demonstrated, including single-molecule diodes, optically and mechanically activated switches, and, significantly, physical phenomena with no classical analogues, such as those based on quantum interference effects. Experimental techniques for reliable and reproducible single molecule junction formation and characterization have led to this progress. In particular, the scanning tunneling microscope based break-junction (STM-BJ) technique has enabled rapid, sequential measurement of large numbers of nanoscale junctions allowing a statistical analysis to readily distinguish reproducible characteristics. Harnessing fundamental link chemistry has provided the necessary chemical control over junction formation, enabling measurements that revealed clear relationships between molecular structure and conductance characteristics. Such link groups (amines, methylsnflides, pyridines, etc.) maintain a stable lone pair configuration that selectively bonds to specific, undercoordinated transition metal atoms available following rupture of a metal point contact in the STM-BJ experiments. This basic chemical principle rationalizes the observation of highly reproducible conductance signatures. Subsequently, the method has been extended to probe a variety of physical phenomena ranging from basic I-V characteristics to more complex properties such as thermopower and electrochemical response. By adapting the technique to a conducting cantilever atomic force microscope (AFM-BJ), simultaneous measurement of the mechanical, characteristics of nanoscale junctions as they are pulled apart has given complementary information such as the stiffness and rupture force of the molecule-metal link bond. Overall, while the BJ technique does not produce a single molecule circuit for practical applications, it has proved remarkably versatile for fundamental studies. Measured data and analysis have been combined with atomic-scale theory and calculations, typically performed for representative junction structures, to provide fundamental physical understanding of structure function relationships. This Account integrates across an extensive series of our specific nanoscale junction studies which were carried out with the STM- and AFM-BJ techniques and supported by theoretical analysis and density functional theory based calculations, with emphasis on the physical characteristics of the measurement process and the rich data sets that emerge. Several examples illustrate the impact of measured trends based on the most probable values for key characteristics (obtained from ensembles of order 1000-10 000 individual junctions) to build a solid picture of conductance phenomena as well as attributes of the link bond chemistry. The key forward-looking question posed here is the extent to which the full data sets represented by the individual trajectories can be analyzed to address structure-function questions at the level of individual junctions. Initial progress toward physical modeling of conductance of individual junctions indicates trends consistent with physical junction structures. Analysis of junction mechanics reveals a scaling procedure that collapses existing data onto a universal force-extension curve. This research directed to understanding the distribution of structures and physical characteristics addresses fundamental questions concerning the interplay between chemical control and stochastically driven diversity. C1 [Hybertsen, Mark S.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Venkataraman, Latha] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. RP Hybertsen, MS (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA.; Venkataraman, L (reprint author), Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. EM mhyberts@bnl.gov; lv2117@columbia.edu OI Venkataraman, Latha/0000-0002-6957-6089 FU NSF [DMR-1507440]; Packard Foundation; U.S. DOE Office of Science User Facility, at Brookhaven National Laboratory [DE-SC0012704] FX We thank our collaborators who contributed to the work described here. This work was supported by the NSF DMR-1507440 and the Packard Foundation. A portion of this work was performed using facilities in the Center for Functional Nanomaterials, which is a U.S. DOE Office of Science User Facility, at Brookhaven National Laboratory under Contract No. DE-SC0012704. NR 41 TC 2 Z9 2 U1 20 U2 50 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0001-4842 EI 1520-4898 J9 ACCOUNTS CHEM RES JI Accounts Chem. Res. PD MAR PY 2016 VL 49 IS 3 BP 452 EP 460 DI 10.1021/acs.accounts.6b00004 PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA DG9GV UT WOS:000372391700011 PM 26938931 ER PT J AU Mondal, T Ashkar, R Butler, P Bhowmick, AK Krishnamoorti, R AF Mondal, Titash Ashkar, Rana Butler, Paul Bhowmick, Anil K. Krishnamoorti, Ramanan TI Graphene Nanocomposites with High Molecular Weight Poly(epsilon-caprolactone) Grafts: Controlled Synthesis and Accelerated Crystallization SO ACS MACRO LETTERS LA English DT Article ID POLYMER; OXIDE; NANOPARTICLES; TEMPERATURE; STRATEGIES; NANOSHEETS; GRAPHITE; KINETICS AB Grafting of high molecular weight polymers to graphitic nanoplatelets is a critical step toward the development of high performance graphene nanocomposites. However, designing such a grafting route has remained a major impediment. Herein, we report a "grafting to" synthetic pathway by which high molecular weight polymer, poly(e-caprolactone) (PCL), is tethered, at high grafting density, to highly anisotropic graphitic nanoplatelets. The efficacy of this tethering route and the resultant structural arrangements within the composite are confirmed by neutron and X-ray scattering measurements in the melt and solution phase. In the semicrystalline state, Xray analysis indicates that chain tethering onto the graphitic nanoplatelets results in conformational changes of the polymer chains, which enhance the nucleation process and aid formation of PCL crystallites. This is corroborated by the superior thermal properties of the composite, manifested in accelerated crystallization kinetics and a significant increase in the thermal degradation temperature. In principle, this synthesis route can be extended to a variety of high molecular weight polymers, which can open new avenues to solution-based processing of graphitic nanomaterials and the fabrication of complex 3D patterned graphitic nanocomposites. C1 [Mondal, Titash] Indian Inst Technol, Dept Chem, Patna 800013, Bihar, India. [Mondal, Titash; Krishnamoorti, Ramanan] Univ Houston, Dept Chem & Biomol Engn, Houston, TX 77204 USA. [Ashkar, Rana] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. [Ashkar, Rana; Butler, Paul] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Butler, Paul] Univ Delaware, Dept Chem & Biomol Engn, Newark, DE 19711 USA. [Mondal, Titash; Bhowmick, Anil K.] Indian Inst Technol, Ctr Rubber Technol, Kharagpur 721302, W Bengal, India. [Ashkar, Rana] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. RP Krishnamoorti, R (reprint author), Univ Houston, Dept Chem & Biomol Engn, Houston, TX 77204 USA.; Bhowmick, AK (reprint author), Indian Inst Technol, Ctr Rubber Technol, Kharagpur 721302, W Bengal, India. EM anilkb@rtc.iitkgp.ernet.in; ramanan@uh.edu RI Krishnamoorti, Ramanan/F-7914-2011; Butler, Paul/D-7368-2011 OI Krishnamoorti, Ramanan/0000-0001-5831-502X; FU U.S. Science and Technology Forum (IUSSTF; from Fundamentals to Applications of Nanoparticle Assemblies) [32-2012/2013-14]; National Science Foundation [DMR-0944772] FX The authors acknowledge the help of Dr. Viktor Hadjiev (Texas Center for Superconductivity, University of Houston) in the Raman spectroscopy measurements. The authors also thank Dr. David Mildner and Dr. Markus Bleuel for their help with the USANS experiments. T.M., A.K.B., and R.K. gratefully acknowledge the generous support of the Indo U.S. Science and Technology Forum (IUSSTF; from Fundamentals to Applications of Nanoparticle Assemblies//32-2012/2013-14). T.M. and A.K.B also acknowledge the partial support of Central Research, Bridgestone Corporation, Japan. This work utilized facilities at the NIST Center for Neutron Research (NCNR) supported in part by the National Science Foundation under Grant DMR-0944772. NR 33 TC 6 Z9 6 U1 7 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2161-1653 J9 ACS MACRO LETT JI ACS Macro Lett. PD MAR PY 2016 VL 5 IS 3 BP 278 EP 282 DI 10.1021/acsmacrolett.5600930 PG 5 WC Polymer Science SC Polymer Science GA DG9IL UT WOS:000372395900004 ER PT J AU Li, X Liu, YD Wan, L Li, ZL Suh, H Ren, JX Ocola, LE Hu, WB Ji, SX Nealey, PF AF Li, Xiao Liu, Yadong Wan, Lei Li, Zhaolei Suh, Hyoseon Ren, Jiaxing Ocola, Leonidas E. Hu, Wenbing Ji, Shengxiang Nealey, Paul F. TI Effect of Stereochemistry on Directed Self-Assembly of Poly(styrene-b-lactide) Films on Chemical Patterns SO ACS MACRO LETTERS LA English DT Article ID STEREOBLOCK POLY(LACTIC ACID)S; STEREOCOMPLEX FORMATION; BLOCK-COPOLYMERS; THIN-FILMS; PERPENDICULAR ORIENTATION; POLY(METHYL METHACRYLATE); MICRODOMAIN ORIENTATION; DENSITY MULTIPLICATION; INTERACTION PARAMETER; TRIBLOCK COPOLYMERS AB We demonstrated here for the first time that the stereochemistry of polylactide (PLA) blocks affected the assembly behaviors of PS-b-PLA on chemical patterns. Two PS-b-PLA block copolymers, where the PLA block is either racemic (PDLLA) or left-handed (PLLA), were synthesized and directed to assemble on chemical patterns with a wide range of L-s/L-o. PS-b-PDLLA was stretched up to 70% on chemical patterns, while PS-b-PLLA was only stretched by 20%. The assembly behavior of PS-b-PDLLA was different from AB diblock copolymer, but similar to that of ABA triblock copolymer. The high stretchability might be attributed to the formation of stereocomplexes in PDLLA blocks. Compared to ABA triblock copolymers, stereocomplexed diblock copolymers have much faster assembly kinetics. This observation provides a new concept to achieve large process windows by the introduction of specific interactions, for example, H-bonding, supramolecular interaction, and sterecomplexation, between polymer chains. C1 [Li, Xiao; Suh, Hyoseon; Ren, Jiaxing; Nealey, Paul F.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. [Liu, Yadong; Ji, Shengxiang] Chinese Acad Sci, Changchun Inst Appl Chem, Key Lab Polymer Ecomat, 5625 Renmin St, Changchun 130022, Peoples R China. [Wan, Lei] HGST, 3403 Yerba Buena Rd, San Jose, CA 95135 USA. [Li, Zhaolei; Hu, Wenbing] Nanjing Univ, Sch Chem & Chem Engn, Nanjing 210093, Jiangsu, Peoples R China. [Ocola, Leonidas E.] Argonne Natl Lab, Ctr Nanoscale Mat, Lemont, IL 60439 USA. RP Nealey, PF (reprint author), Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA.; Ji, SX (reprint author), Chinese Acad Sci, Changchun Inst Appl Chem, Key Lab Polymer Ecomat, 5625 Renmin St, Changchun 130022, Peoples R China. EM sji@ciac.ac.cn; nealey@uchicago.edu RI Ji, Shengxiang/A-7567-2015; OI Ji, Shengxiang/0000-0003-0336-0530; Ocola, Leonidas/0000-0003-4990-1064 FU DOE Office of Science [DE-AC02-06CH11357]; National Natural Science Foundation of China [51173181, 51373166]; Chinese Academy of Sciences; Department of Science and Technology of Jilin Province [20160414032GH] FX This research used resources of the Center for Nanoscale Materials, a U.S. Department of Energy (DOE) Office of Science User Facility, operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. S.J. gratefully thanks the funding from the National Natural Science Foundation of China (Nos. 51173181 and 51373166), "The Hundred Talents Program" from the Chinese Academy of Sciences and the International S&T Cooperation Program from Department of Science and Technology of Jilin Province (No. 20160414032GH). NR 49 TC 2 Z9 2 U1 13 U2 49 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2161-1653 J9 ACS MACRO LETT JI ACS Macro Lett. PD MAR PY 2016 VL 5 IS 3 BP 396 EP 401 DI 10.1021/acsmacrolett.6b00011 PG 6 WC Polymer Science SC Polymer Science GA DG9IL UT WOS:000372395900028 ER PT J AU Guo, R Rusak, E Staude, I Dominguez, J Decker, M Rockstuhl, C Brener, I Neshev, DN Kivshar, YS AF Guo, Rui Rusak, Evgenia Staude, Isabelle Dominguez, Jason Decker, Manuel Rockstuhl, Carsten Brener, Igal Neshev, Dragomir N. Kivshar, Yuri S. TI Multipolar Coupling in Hybrid Metal Dielectric Metasurfaces SO ACS PHOTONICS LA English DT Article DE metal-dielectric metasurfaces; subwavelength nanostructures; directional radiation properties; multipolar radiation ID NANOANTENNAS; EMISSION; ANTENNA AB We study functional hybrid metasurfaces consisting of metal-dielectric nanoantennas that direct light from an incident plane wave or from localized light sources into a preferential direction. The directionality is obtained by carefully balancing the multipolar contributions to the scattering response from the constituents of the metasurface. The hybrid nanoantennas are composed of a plasmonic gold nanorod acting as a feed element and a silicon nanodisk acting as a director element. In order to experimentally realize this design, we have developed a two-step electron-beam lithography process in combination with a precision alignment step. The optical response of the fabricated sample is measured and reveals distinct signatures of coupling between the plasmonic and the dielectric nanoantenna elements that ultimately leads to unidirectional radiation of light. C1 [Guo, Rui; Rusak, Evgenia; Staude, Isabelle; Decker, Manuel; Neshev, Dragomir N.; Kivshar, Yuri S.] Australian Natl Univ, Res Sch Phys & Engn, Nonlinear Phys Ctr, Canberra, ACT 2601, Australia. [Guo, Rui; Rusak, Evgenia; Staude, Isabelle; Decker, Manuel; Neshev, Dragomir N.; Kivshar, Yuri S.] Australian Natl Univ, Res Sch Phys & Engn, Ctr Ultrahigh Bandwidth Devices Opt Syst CUDOS, Canberra, ACT 2601, Australia. [Rusak, Evgenia; Rockstuhl, Carsten] Karlsruhe Inst Technol, Inst Theoret Solid State Phys, D-76131 Karlsruhe, Germany. [Staude, Isabelle] Univ Jena, Abbe Ctr Photon, Inst Appl Phys, D-07743 Jena, Germany. [Dominguez, Jason] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. [Rockstuhl, Carsten] Karlsruhe Inst Technol, Inst Nanotechnol, D-76021 Karlsruhe, Germany. RP Staude, I (reprint author), Australian Natl Univ, Res Sch Phys & Engn, Nonlinear Phys Ctr, Canberra, ACT 2601, Australia.; Staude, I (reprint author), Australian Natl Univ, Res Sch Phys & Engn, Ctr Ultrahigh Bandwidth Devices Opt Syst CUDOS, Canberra, ACT 2601, Australia.; Staude, I (reprint author), Univ Jena, Abbe Ctr Photon, Inst Appl Phys, D-07743 Jena, Germany. EM isabelle.staude@uni-jena.de RI Staude, Isabelle/N-4270-2015; Neshev, Dragomir/A-3759-2008; Rockstuhl, Carsten/S-5832-2016 OI Neshev, Dragomir/0000-0002-4508-8646; FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Australian National Fabrication Facility (ANFF) ACT node; Australian Research Council; Australian Research Council through DECRA Fellowship; Group of Eight: Australia Germany Joint Research Cooperation Scheme; German National Merit Foundation; Thuringian State Government within its ProExcellence initiative (ACP); German Science Foundation [RO 3640/7-1]; DAAD (PPP Australien); Erasmus Mundus NANOPHI project [2013 5659/002001] FX This work was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. The authors also acknowledge support from the Australian National Fabrication Facility (ANFF) ACT node, the Australian Research Council through Discovery Project and DECRA Fellowship grants, and the Group of Eight: Australia Germany Joint Research Cooperation Scheme and the German National Merit Foundation. I.S. gratefully acknowledges financial support by the Thuringian State Government within its ProExcellence initiative (ACP2020). C.R thanks the German Science Foundation (project RO 3640/7-1) for financial support. The work was further supported by the DAAD (PPP Australien). We acknowledge the support of the Erasmus Mundus NANOPHI project, contract number 2013 5659/002001. NR 25 TC 5 Z9 6 U1 19 U2 52 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2330-4022 J9 ACS PHOTONICS JI ACS Photonics PD MAR PY 2016 VL 3 IS 3 BP 349 EP 353 DI 10.1021/acsphotonics.6b00012 PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Optics; Physics, Applied; Physics, Condensed Matter SC Science & Technology - Other Topics; Materials Science; Optics; Physics GA DH0MY UT WOS:000372479500008 ER PT J AU Zarick, HF Erwin, WR Boulesbaa, A Hurd, OK Webb, JA Puretzky, AA Geohegan, DB Bardhan, R AF Zarick, Holly F. Erwin, William R. Boulesbaa, Abdelaziz Hurd, Olivia K. Webb, Joseph A. Puretzky, Alexander A. Geohegan, David B. Bardhan, Rizia TI Improving Light Harvesting in Dye-Sensitized Solar Cells Using Hybrid Bimetallic Nanostructures SO ACS PHOTONICS LA English DT Article DE dye-sensitized solar cell; plasmon-enhanced solar cell; bimetallic nanostructures; transient absorption spectroscopy; electron dynamics ID ALLOY POPCORN NANOPARTICLES; ENHANCED RAMAN-SCATTERING; SURFACE-PLASMON RESONANCE; HIGH-EFFICIENCY; AG NANOPARTICLES; TRANSIENT ABSORPTION; GOLD NANOSTRUCTURES; ELECTRON-TRANSFER; ENERGY-TRANSPORT; SILICON DIOXIDE AB In this work we demonstrate improved light trapping in dye-sensitized solar cells (DSSCs) with hybrid bimetallic gold core/silver shell nanostructures. Silica-coated bimetallic nanostructures (Au/Ag/SiO2 NSs) integrated in the active layer of DSSCs resulted in 7.51% power conversion efficiency relative to 5.97% for reference DSSCs, giving rise to 26% enhancement in device performance. DSSC efficiencies were governed by the particle density of Au/Ag/SiO2 NSs with best performing devices utilizing only 0.44 wt % of nanostructures. We performed transient absorption spectroscopy of DSSCs with variable concentrations of Au/Ag/SiO2 NSs and observed an increase in amplitude and decrease in lifetime with increasing particle density relative to reference. We attributed this trend to plasmon resonant energy transfer and population of the singlet excited states of the sensitizer molecules at the optimum concentration of NSs promoting enhanced exciton generation and rapid charge transfer into TiO2. C1 [Zarick, Holly F.; Erwin, William R.; Webb, Joseph A.; Bardhan, Rizia] Vanderbilt Univ, Dept Chem & Biomol Engn, 221 Kirkland Hall, Nashville, TN 37235 USA. [Hurd, Olivia K.] Vanderbilt Univ, Dept Mech Engn, 221 Kirkland Hall, Nashville, TN 37235 USA. [Boulesbaa, Abdelaziz; Puretzky, Alexander A.; Geohegan, David B.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Bardhan, R (reprint author), Vanderbilt Univ, Dept Chem & Biomol Engn, 221 Kirkland Hall, Nashville, TN 37235 USA. EM rizia.bardhan@vanderbilt.edu RI Boulesbaa, Abdelaziz/J-3314-2016; Geohegan, David/D-3599-2013 OI Boulesbaa, Abdelaziz/0000-0003-4519-4403; Geohegan, David/0000-0003-0273-3139 FU NSF [NSF EPS1004083, EEC 1342185]; Department of Education for a Graduate Assistance in Areas of National Need (GAANN) Fellowship [P0200A090323]; National Science Foundation [1445197] FX H.F.Z. acknowledges support from NSF EPSCOR (NSF EPS1004083), NSF BRIGE (EEC 1342185), and the Department of Education for a Graduate Assistance in Areas of National Need (GAANN) Fellowship under Grant No. P0200A090323. W.R.E. and J.A.W. acknowledge support from the National Science Foundation Graduate Research Fellowship Program under Grant No. 1445197. Ultrafast measurements were conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. NR 77 TC 10 Z9 10 U1 9 U2 55 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2330-4022 J9 ACS PHOTONICS JI ACS Photonics PD MAR PY 2016 VL 3 IS 3 BP 385 EP 394 DI 10.1021/acsphotonics.5b00552 PG 10 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Optics; Physics, Applied; Physics, Condensed Matter SC Science & Technology - Other Topics; Materials Science; Optics; Physics GA DH0MY UT WOS:000372479500013 ER PT J AU Simpson, MJ Doughty, B Yang, B Xiao, K Ma, YZ AF Simpson, Mary Jane Doughty, Benjamin Yang, Bin Xiao, Kai Ma, Ying-Zhong TI Separation of Distinct Photoexcitation Species in Femtosecond Transient Absorption Microscopy SO ACS PHOTONICS LA English DT Article DE perovskite; transient absorption microscopy; photoexcitation; dimension reduction; big data ID PEROVSKITE SOLAR-CELLS; ORGANOMETAL HALIDE PEROVSKITE; PUMP-PROBE MICROSCOPY; EXCITON BINDING-ENERGY; CARRIER DYNAMICS; THIN-FILMS; ELECTRONIC-PROPERTIES; CHARGE-CARRIERS; QUANTUM DOTS; RECOMBINATION AB Femtosecond transient absorption microscopy is a novel chemical imaging capability with simultaneous high spatial and temporal resolution. Although several powerful data analysis approaches have been developed and successfully applied to separate distinct chemical species in such images, the application of such analysis to distinguish different photoexcited species is rare. In this paper, we demonstrate a combined approach based on phasor and linear decomposition analysis on a microscopic level that allows us to separate the contributions of both the excitons and free charge carriers in the observed transient absorption response of a composite organometallic lead halide perovskite film. We found spatial regions where the transient absorption response was predominately a result of excitons and others where it was predominately due to charge carriers, and regions consisting of signals from both contributors. Quantitative decomposition of the transient absorption response curves further enabled us to reveal the relative contribution of each photoexcitation to the measured response at spatially resolved locations in the film. C1 [Simpson, Mary Jane; Doughty, Benjamin; Ma, Ying-Zhong] Oak Ridge Natl Lab, Chem Sci Div, Oak Ridge, TN 37831 USA. [Yang, Bin; Xiao, Kai] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Ma, YZ (reprint author), Oak Ridge Natl Lab, Chem Sci Div, Oak Ridge, TN 37831 USA. EM may1@ornl.gov RI Yang, Bin/P-8529-2014; Ma, Yingzhong/L-6261-2016; Doughty, Benjamin /M-5704-2016 OI Yang, Bin/0000-0002-5667-9126; Ma, Yingzhong/0000-0002-8154-1006; Doughty, Benjamin /0000-0001-6429-9329 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division FX M.J.S., B.D., and Y.-Z.M. were supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. Perovskite sample preparation by B.Y. and K.X. was performed at the Center for Nanophase Materials Sciences (CNMS), which is a DOE Office of Science User Facility. MJ.S. thanks Michael J. Simpson, Jesse W. Wilson, and Francisco E. Robles for sharing their data analysis expertise through helpful discussions and trouble-shooting Python scripts. NR 49 TC 3 Z9 3 U1 11 U2 51 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2330-4022 J9 ACS PHOTONICS JI ACS Photonics PD MAR PY 2016 VL 3 IS 3 BP 434 EP 442 DI 10.1021/acsphotonics.5b00638 PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Optics; Physics, Applied; Physics, Condensed Matter SC Science & Technology - Other Topics; Materials Science; Optics; Physics GA DH0MY UT WOS:000372479500019 ER PT J AU Ford, NR Hecht, KA Hu, DH Orr, G Xiong, YJ Squier, TC Rorrer, GL Roesijadi, G AF Ford, Nicole R. Hecht, Karen A. Hu, DeHong Orr, Galya Xiong, Yijia Squier, Thomas C. Rorrer, Gregory L. Roesijadi, Guritno TI Antigen Binding and Site-Directed Labeling of Biosilica-Immobilized Fusion Proteins Expressed in Diatoms SO ACS SYNTHETIC BIOLOGY LA English DT Article DE diatom; silica; biarsenical probe; biosensor; TNT; anthrax ID THALASSIOSIRA-PSEUDONANA BACILLARIOPHYCEAE; SILICA IMMOBILIZATION; FLUOROMETER; MICROSCOPY; PROBE AB The diatom Thalassiosira pseudonana was genetically modified to express biosilica-targeted fusion proteins comprising either enhanced green fluorescent protein (EGFP) or single chain antibodies engineered with a tetracysteine tagging sequence. Of interest were the site specific binding of (1) the fluorescent biarsenical probe AsCy3 and AsCy3e to the tetracysteine tagged fusion proteins and (2) high and low molecular mass antigens, the Bacillus anthracis surface layer protein EA1 or small molecule explosive trinitrotoluene (TNT), to biosilica-immobilized single chain antibodies. Analysis of biarsenical probe binding using fluorescence and structured illumination microscopy indicated differential colocalization with EGFP in nascent and mature biosilica, supporting the use of either EGFP or bound AsCy3 and AsCy3e in studying biosilica maturation. Large increases in the lifetime of a fluorescent analogue of TNT upon binding single chain antibodies provided a robust signal capable of discriminating binding to immobilized antibodies in the transformed frustule from nonspecific binding to the biosilica matrix. In conclusion, our results demonstrate an ability to engineer diatoms to create antibody-functionalized mesoporous silica able to selectively bind chemical and biological agents for the development of sensing platforms. C1 [Ford, Nicole R.; Hecht, Karen A.; Roesijadi, Guritno] Pacific NW Natl Lab, Marine Biotechnol, Sequim, WA 98382 USA. [Hu, DeHong; Orr, Galya] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Xiong, Yijia; Squier, Thomas C.] Western Univ Hlth Sci, Dept Basic Med Sci, Lebanon, OR 97355 USA. [Roesijadi, Guritno] Oregon State Univ, Dept Microbiol, Corvallis, OR 97331 USA. [Rorrer, Gregory L.] Oregon State Univ, Sch Chem Biol & Environm Engn, Corvallis, OR 97331 USA. RP Roesijadi, G (reprint author), Pacific NW Natl Lab, Marine Biotechnol, Sequim, WA 98382 USA.; Roesijadi, G (reprint author), Oregon State Univ, Dept Microbiol, Corvallis, OR 97331 USA. EM g.roesijadi@pnnl.gov RI Hu, Dehong/B-4650-2010 OI Hu, Dehong/0000-0002-3974-2963 FU Defense Threat Reduction Agency; Office of Naval Research; Environmental Molecular Sciences Laboratory (EMSL); DOE's OBER FX Drs. Nils Kroger and Nicole Poulsen (CUBE Center for Molecular Bioengineering, Dresden, DE) provided clones for Sil3 and its Sil3T8 derivative; Drs. Ellen Goldman and Igor Medintz (Naval Research Laboratory, Washington, D.C.) provided clones for scFvs and sdAbs, and assistance in preparing fluorescent TNT surrogate compounds, respectively. Drs. Li-Jung Kuo and Valerie Cullinan (Pacific Northwest National Laboratory) contributed to synthesis of AF555-TNB and statistical analysis, respectively. This research was supported by the Defense Threat Reduction Agency (G.R and T.C.S.), the Office of Naval Research (G.R. and G.L.R), and the Environmental Molecular Sciences Laboratory (EMSL) (G.R. and T.C.S). Part of the research was performed using EMSL, a national scientific user facility sponsored by the DOE's OBER and located at PNNL. NR 31 TC 2 Z9 2 U1 5 U2 11 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2161-5063 J9 ACS SYNTH BIOL JI ACS Synth. Biol. PD MAR PY 2016 VL 5 IS 3 BP 193 EP 199 DI 10.1021/acssynbio.5b00191 PG 7 WC Biochemical Research Methods SC Biochemistry & Molecular Biology GA DH3FI UT WOS:000372672500001 PM 26746113 ER PT J AU Akey, DL Terwilliger, TC Smith, JL AF Akey, David L. Terwilliger, Thomas C. Smith, Janet L. TI Efficient merging of data from multiple samples for determination of anomalous substructure SO ACTA CRYSTALLOGRAPHICA SECTION D-STRUCTURAL BIOLOGY LA English DT Article DE sulfur phasing; local scaling; anomalous scattering; data merging ID NATIVE BIOLOGICAL MACROMOLECULES; PHASE DETERMINATION; FLAVIVIRUS NS1; DIFFRACTION; REFINEMENT; RESOLUTION; SELECTION; CRYSTALS AB Merging of data from multiple crystals has proven to be useful for determination of the anomalously scattering atomic substructure for crystals with weak anomalous scatterers (e.g. S and P) and/or poor diffraction. Strategies for merging data from many samples, which require assessment of sample isomorphism, rely on metrics of variability in unit-cell parameters, anomalous signal correlation and overall data similarity. Local scaling, anomalous signal optimization and data-set weighting, implemented in phenix. scale_and_merge, provide an efficient protocol for merging data from many samples. The protein NS1 was used in a series of trials with data collected from 28 samples for phasing by single-wavelength anomalous diffraction of the native S atoms. The local-scaling, anomalous-optimization protocol produced merged data sets with higher anomalous signal quality indicators than did standard global-scaling protocols. The local-scaled data were also more successful in substructure determination. Merged data quality was assessed for data sets where the multiplicity was reduced in either of two ways: by excluding data from individual crystals (to reduce errors owing to non-isomorphism) or by excluding the last-recorded segments of data from each crystal (to minimize the effects of radiation damage). The anomalous signal was equivalent at equivalent multiplicity for the two procedures, and structure-determination success correlated with anomalous signal metrics. The quality of the anomalous signal was strongly correlated with data multiplicity over a range of 12-fold to 150-fold multiplicity. For the NS1 data, the local-scaling and anomalous-optimization protocol handled sample non-isomorphism and radiation-induced decay equally well. C1 [Akey, David L.; Smith, Janet L.] Univ Michigan, Inst Life Sci, 210 Washtenaw Ave, Ann Arbor, MI 48109 USA. [Terwilliger, Thomas C.] Los Alamos Natl Lab, Biosci Div, Mail Stop M888, Los Alamos, NM 87545 USA. RP Smith, JL (reprint author), Univ Michigan, Inst Life Sci, 210 Washtenaw Ave, Ann Arbor, MI 48109 USA. EM janetsmith@umich.edu RI Terwilliger, Thomas/K-4109-2012 OI Terwilliger, Thomas/0000-0001-6384-0320 FU US National Institutes of Health [P01AI055672, P01GM063210]; US Department of Energy [DE-AC02-05CH11231]; Martha L. Ludwig Professorship of Protein Structure and Function FX This work was supported by grants from the US National Institutes of Health (P01AI055672 to JLS and P01GM063210 to TCT), the US Department of Energy (contract DE-AC02-05CH11231) to TCT and the Martha L. Ludwig Professorship of Protein Structure and Function to JLS. The beamlines of GM/CA@APS were supported by the National Institute of General Medical Sciences ('GM'; Y1-GM-1104) and the National Cancer Institute ('CA'; Y1-CO-1020). NR 17 TC 0 Z9 0 U1 1 U2 1 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND EI 2059-7983 J9 ACTA CRYSTALLOGR D JI Acta Crystallogr. Sect. D-Struct. Biol. PD MAR PY 2016 VL 72 BP 296 EP 302 DI 10.1107/S2059798315021920 PN 3 PG 7 WC Biochemical Research Methods; Biochemistry & Molecular Biology; Biophysics; Crystallography SC Biochemistry & Molecular Biology; Biophysics; Crystallography GA DG8XJ UT WOS:000372366600003 PM 26960117 ER PT J AU Terwilliger, TC Bunkoczi, G Hung, LW Zwart, PH Smith, JL Akey, DL Adams, PD AF Terwilliger, Thomas C. Bunkoczi, Gabor Hung, Li-Wei Zwart, Peter H. Smith, Janet L. Akey, David L. Adams, Paul D. TI Can I solve my structure by SAD phasing? Anomalous signal in SAD phasing SO ACTA CRYSTALLOGRAPHICA SECTION D-STRUCTURAL BIOLOGY LA English DT Article DE SAD phasing; anomalous signal; anomalous phasing; solving structures ID MULTIPLE ISOMORPHOUS REPLACEMENT; X-RAY-DIFFRACTION; CRYSTAL-STRUCTURE; DENSITY-MODIFICATION; ELECTRON-DENSITY; DATA-COLLECTION; TRANSFER-RNA; MACROMOLECULAR CRYSTALLOGRAPHY; STRUCTURE REFINEMENT; RESOLUTION REVEALS AB A key challenge in the SAD phasing method is solving a structure when the anomalous signal-to-noise ratio is low. A simple theoretical framework for describing measurements of anomalous differences and the resulting useful anomalous correlation and anomalous signal in a SAD experiment is presented. Here, the useful anomalous correlation is defined as the correlation of anomalous differences with ideal anomalous differences from the anomalous substructure. The useful anomalous correlation reflects the accuracy of the data and the absence of minor sites. The useful anomalous correlation also reflects the information available for estimating crystallographic phases once the substructure has been determined. In contrast, the anomalous signal (the peak height in a model-phased anomalous difference Fourier at the coordinates of atoms in the anomalous substructure) reflects the information available about each site in the substructure and is related to the ability to find the substructure. A theoretical analysis shows that the expected value of the anomalous signal is the product of the useful anomalous correlation, the square root of the ratio of the number of unique reflections in the data set to the number of sites in the substructure, and a function that decreases with increasing values of the atomic displacement factor for the atoms in the substructure. This means that the ability to find the substructure in a SAD experiment is increased by high data quality and by a high ratio of reflections to sites in the substructure, and is decreased by high atomic displacement factors for the substructure. C1 [Terwilliger, Thomas C.] Los Alamos Natl Lab, Biosci Div, Mail Stop M888, Los Alamos, NM 87545 USA. [Bunkoczi, Gabor] Univ Cambridge, Dept Haematol, Cambridge Inst Med Res, Wellcome Trust MRC Bldg, Cambridge CB2 0XY, England. [Hung, Li-Wei] Los Alamos Natl Lab, Div Phys, Mail Stop D454, Los Alamos, NM 87545 USA. [Zwart, Peter H.; Adams, Paul D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Smith, Janet L.; Akey, David L.] Univ Michigan, Inst Life Sci, Ann Arbor, MI 48109 USA. [Smith, Janet L.] Univ Michigan, Dept Biol Chem, Ann Arbor, MI 48109 USA. RP Terwilliger, TC (reprint author), Los Alamos Natl Lab, Biosci Div, Mail Stop M888, Los Alamos, NM 87545 USA. EM terwilliger@lanl.gov RI Terwilliger, Thomas/K-4109-2012; OI Terwilliger, Thomas/0000-0001-6384-0320; Hung, Li-Wei/0000-0001-6690-8458 FU US National Institutes of Health [P01GM063210, P01AI055672]; US Department of Energy [DE-AC02-05CH11231] FX The authors appreciate the support received from the US National Institutes of Health (grant P01GM063210 to PDA, TCT, Jane S. Richardson and Randy J. Read, and grant P01AI055672 to JLS). This work was partially supported by the US Department of Energy under contract DE-AC02-05CH11231. NR 88 TC 3 Z9 3 U1 3 U2 6 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND EI 2059-7983 J9 ACTA CRYSTALLOGR D JI Acta Crystallogr. Sect. D-Struct. Biol. PD MAR PY 2016 VL 72 BP 346 EP 358 DI 10.1107/S2059798315019269 PN 3 PG 13 WC Biochemical Research Methods; Biochemistry & Molecular Biology; Biophysics; Crystallography SC Biochemistry & Molecular Biology; Biophysics; Crystallography GA DG8XJ UT WOS:000372366600008 PM 26960122 ER PT J AU Terwilliger, TC Bunkoczi, G Hung, LW Zwart, PH Smith, JL Akey, DL Adams, PD AF Terwilliger, Thomas C. Bunkoczi, Gabor Hung, Li-Wei Zwart, Peter H. Smith, Janet L. Akey, David L. Adams, Paul D. TI Can I solve my structure by SAD phasing? Planning an experiment, scaling data and evaluating the useful anomalous correlation and anomalous signal SO ACTA CRYSTALLOGRAPHICA SECTION D-STRUCTURAL BIOLOGY LA English DT Article DE SAD phasing; anomalous signal; experimental design ID CRYSTAL-STRUCTURE; DIFFRACTION DATA; TRANSFER-RNA; ISOMORPHOUS REPLACEMENT; RESPONSE REGULATOR; RESOLUTION REVEALS; BACILLUS-SUBTILIS; DATA QUALITY; COMPLEX; PROTEIN AB A key challenge in the SAD phasing method is solving a structure when the anomalous signal-to-noise ratio is low. Here, algorithms and tools for evaluating and optimizing the useful anomalous correlation and the anomalous signal in a SAD experiment are described. A simple theoretical framework [Terwilliger et al. (2016), Acta Cryst. D72, 346-358] is used to develop methods for planning a SAD experiment, scaling SAD data sets and estimating the useful anomalous correlation and anomalous signal in a SAD data set. The phenix. plan_sad_experiment tool uses a database of solved and unsolved SAD data sets and the expected characteristics of a SAD data set to estimate the probability that the anomalous substructure will be found in the SAD experiment and the expected map quality that would be obtained if the substructure were found. The phenix. scale_and_merge tool scales unmerged SAD data from one or more crystals using local scaling and optimizes the anomalous signal by identifying the systematic differences among data sets, and the phenix.anomalous_signal tool estimates the useful anomalous correlation and anomalous signal after collecting SAD data and estimates the probability that the data set can be solved and the likely figure of merit of phasing. C1 [Terwilliger, Thomas C.] Los Alamos Natl Lab, Biosci Div, Mail Stop M888, Los Alamos, NM 87545 USA. [Bunkoczi, Gabor] Univ Cambridge, Dept Haematol, Cambridge Inst Med Res, Wellcome Trust MRC Bldg, Cambridge CB2 0XY, England. [Hung, Li-Wei] Los Alamos Natl Lab, Div Phys, Mail Stop D454, Los Alamos, NM 87545 USA. [Zwart, Peter H.; Adams, Paul D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Smith, Janet L.; Akey, David L.] Univ Michigan, Inst Life Sci, Ann Arbor, MI 48109 USA. [Smith, Janet L.] Univ Michigan, Dept Biol Chem, Ann Arbor, MI 48109 USA. RP Terwilliger, TC (reprint author), Los Alamos Natl Lab, Biosci Div, Mail Stop M888, Los Alamos, NM 87545 USA. EM terwilliger@lanl.gov RI Terwilliger, Thomas/K-4109-2012; OI Terwilliger, Thomas/0000-0001-6384-0320; Hung, Li-Wei/0000-0001-6690-8458 FU US National Institutes of Health [P01GM063210, P01AI055672]; US Department of Energy [DE-AC02-05CH11231] FX The authors appreciate the support received from the US National Institutes of Health (grant P01GM063210 to PDA, TCT and Randy J. Read, and grant P01AI055672 to JLS). This work was partially supported by the US Department of Energy under contract DE-AC02-05CH11231. NR 93 TC 2 Z9 2 U1 1 U2 2 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND EI 2059-7983 J9 ACTA CRYSTALLOGR D JI Acta Crystallogr. Sect. D-Struct. Biol. PD MAR PY 2016 VL 72 BP 359 EP 374 DI 10.1107/S2059798315019403 PN 3 PG 16 WC Biochemical Research Methods; Biochemistry & Molecular Biology; Biophysics; Crystallography SC Biochemistry & Molecular Biology; Biophysics; Crystallography GA DG8XJ UT WOS:000372366600009 PM 26960123 ER PT J AU Jorda, J Sawaya, MR Yeates, TO AF Jorda, Julien Sawaya, Michael R. Yeates, Todd O. TI Progress in low-resolution ab initio phasing with CrowdPhase SO ACTA CRYSTALLOGRAPHICA SECTION D-STRUCTURAL BIOLOGY LA English DT Article DE crowdsourcing; phase problem; CrowdPhase; direct methods ID ELECTRON-DENSITY MAPS; FOLDING GAME PLAYERS; MACROMOLECULAR CRYSTALLOGRAPHY; ANGSTROM RESOLUTION; GENETIC ALGORITHM; ATOMIC-STRUCTURE; HIGH-SYMMETRY; PROTEIN; LIKELIHOOD; VIRUS AB Ab initio phasing by direct computational methods in low-resolution X-ray crystallography is a long-standing challenge. A common approach is to consider it as two subproblems: sampling of phase space and identification of the correct solution. While the former is amenable to a myriad of search algorithms, devising a reliable target function for the latter problem remains an open question. Here, recent developments in CrowdPhase, a collaborative online game powered by a genetic algorithm that evolves an initial population of individuals with random genetic make-up (i.e. random phases) each expressing a phenotype in the form of an electron-density map, are presented. Success relies on the ability of human players to visually evaluate the quality of these maps and, following a Darwinian survival-of-the-fittest concept, direct the search towards optimal solutions. While an initial study demonstrated the feasibility of the approach, some important crystallographic issues were overlooked for the sake of simplicity. To address these, the new CrowdPhase includes consideration of space-group symmetry, a method for handling missing amplitudes, the use of a map correlation coefficient as a quality metric and a solvent-flattening step. Performances of this installment are discussed for two low-resolution test cases based on bona fide diffraction data. C1 [Jorda, Julien; Sawaya, Michael R.; Yeates, Todd O.] UCLA DOE, Inst Genom & Prote, 611 Charles Young Dr East, Los Angeles, CA 90095 USA. [Yeates, Todd O.] Univ Calif Los Angeles, Inst Mol Biol, 611 Charles Young Dr East, Los Angeles, CA 90095 USA. [Yeates, Todd O.] Univ Calif Los Angeles, Dept Chem & Biochem, 611 Charles Young Dr East, Los Angeles, CA 90095 USA. RP Yeates, TO (reprint author), UCLA DOE, Inst Genom & Prote, 611 Charles Young Dr East, Los Angeles, CA 90095 USA.; Yeates, TO (reprint author), Univ Calif Los Angeles, Inst Mol Biol, 611 Charles Young Dr East, Los Angeles, CA 90095 USA.; Yeates, TO (reprint author), Univ Calif Los Angeles, Dept Chem & Biochem, 611 Charles Young Dr East, Los Angeles, CA 90095 USA. EM yeates@mbi.ucla.edu OI Sawaya, Michael/0000-0003-0874-9043; Yeates, Todd/0000-0001-5709-9839 FU DOE Office of Science FX The authors would like to thank the CCP4 Study Weekend organizers and attendees, the UCLA Biochemistry Molecular and Structural Biology graduate students, the Yeates, Bowie and Eisenberg laboratories at UCLA and the undergraduate students Jeff Wang, Duy Ngo and Peter Leung for their active participation in the games. This work was supported by the BER program of the DOE Office of Science. NR 46 TC 0 Z9 0 U1 4 U2 7 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND EI 2059-7983 J9 ACTA CRYSTALLOGR D JI Acta Crystallogr. Sect. D-Struct. Biol. PD MAR PY 2016 VL 72 BP 446 EP 453 DI 10.1107/S2059798316003405 PN 3 PG 8 WC Biochemical Research Methods; Biochemistry & Molecular Biology; Biophysics; Crystallography SC Biochemistry & Molecular Biology; Biophysics; Crystallography GA DG8XJ UT WOS:000372366600018 PM 26960132 ER PT J AU Cheng, XB Zhang, R Zhao, CZ Wei, F Zhang, JG Zhang, Q AF Cheng, Xin-Bing Zhang, Rui Zhao, Chen-Zi Wei, Fei Zhang, Ji-Guang Zhang, Qiang TI A Review of Solid Electrolyte Interphases on Lithium Metal Anode SO ADVANCED SCIENCE LA English DT Article ID LI-ION BATTERIES; ELECTROCHEMICAL IMPEDANCE SPECTROSCOPY; HIGH-ENERGY-DENSITY; RAY PHOTOELECTRON-SPECTROSCOPY; SURFACE-FILM FORMATION; PROPYLENE CARBONATE ELECTROLYTE; RECHARGEABLE LI-O-2 BATTERIES; ETHER-BASED ELECTROLYTES; IN-SITU; SULFUR BATTERIES AB Lithium metal batteries (LMBs) are among the most promising candidates of high-energy-density devices for advanced energy storage. However, the growth of dendrites greatly hinders the practical applications of LMBs in portable electronics and electric vehicles. Constructing stable and efficient solid electrolyte interphase (SEI) is among the most effective strategies to inhibit the dendrite growth and thus to achieve a superior cycling performance. In this review, the mechanisms of SEI formation and models of SEI structure are briefly summarized. The analysis methods to probe the surface chemistry, surface morphology, electrochemical property, dynamic characteristics of SEI layer are emphasized. The critical factors affecting the SEI formation, such as electrolyte component, temperature, current density, are comprehensively debated. The efficient methods to modify SEI layer with the introduction of new electrolyte system and additives, ex-situ-formed protective layer, as well as electrode design, are summarized. Although these works afford new insights into SEI research, robust and precise routes for SEI modification with well-designed structure, as well as understanding of the connection between structure and electrochemical performance, is still inadequate. A multidisciplinary approach is highly required to enable the formation of robust SEI for highly efficient energy storage systems. C1 [Cheng, Xin-Bing; Zhang, Rui; Zhao, Chen-Zi; Wei, Fei; Zhang, Qiang] Tsinghua Univ, Dept Chem Engn, Beijing Key Lab Green Chem React Engn & Technol, Beijing 100084, Peoples R China. [Zhang, Ji-Guang] Pacific NW Natl Lab, Joint Ctr Energy Storage Res Energy & Environm Di, Richland, WA 99354 USA. RP Zhang, Q (reprint author), Tsinghua Univ, Dept Chem Engn, Beijing Key Lab Green Chem React Engn & Technol, Beijing 100084, Peoples R China. EM zhang-qiang@mails.tsinghua.edu.cn RI Zhang, Qiang/B-1799-2012; Cheng, Xin-Bing/F-8448-2014; Zhang, Rui/B-3843-2015 OI Zhang, Qiang/0000-0002-3929-1541; Cheng, Xin-Bing/0000-0001-7567-1210; Zhang, Rui/0000-0003-3740-8352 FU Natural Scientific Foundation of China [21422604, 21561130151]; National Basic Research Program of China [2011CB932602, 2015CB932500]; Tsinghua University Initiative Scientific Research Program [2014z22076] FX This work was supported by the Natural Scientific Foundation of China (21422604 and 21561130151), National Basic Research Program of China (2011CB932602 and 2015CB932500), and Tsinghua University Initiative Scientific Research Program (2014z22076). NR 190 TC 46 Z9 46 U1 161 U2 381 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2198-3844 J9 ADV SCI JI Adv. Sci. PD MAR PY 2016 VL 3 IS 3 AR 1500213 DI 10.1002/advs.201500213 PG 20 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DH0XU UT WOS:000372508400006 PM 27774393 ER PT J AU Lu, XJ Howard, JW Chen, AP Zhu, JL Li, S Wu, G Dowden, P Xu, HW Zhao, YS Jia, QX AF Lu, Xujie Howard, John W. Chen, Aiping Zhu, Jinlong Li, Shuai Wu, Gang Dowden, Paul Xu, Hongwu Zhao, Yusheng Jia, Quanxi TI Antiperovskite Li3OCl Superionic Conductor Films for Solid-State Li-Ion Batteries SO ADVANCED SCIENCE LA English DT Article ID LITHIUM; ELECTROLYTE; STABILITY C1 [Lu, Xujie; Chen, Aiping; Dowden, Paul; Jia, Quanxi] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Howard, John W.; Zhu, Jinlong; Li, Shuai; Zhao, Yusheng] Univ Nevada, High Pressure Sci & Engn Ctr, Las Vegas, NV 89154 USA. [Wu, Gang] SUNY Buffalo, Dept Chem & Biol Engn, Buffalo, NY 14260 USA. [Xu, Hongwu] Los Alamos Natl Lab, Earth & Environm Sci Div, Los Alamos, NM 87545 USA. RP Lu, XJ; Jia, QX (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA.; Zhao, YS (reprint author), Univ Nevada, High Pressure Sci & Engn Ctr, Las Vegas, NV 89154 USA. EM xujie@lanl.gov; yusheng.zhao@unlv.edu; qxjia@lanl.gov RI Wu, Gang/E-8536-2010; Chen, Aiping/F-3212-2011; Lu, Xujie/L-9672-2014; OI Wu, Gang/0000-0003-4956-5208; Chen, Aiping/0000-0003-2639-2797; Lu, Xujie/0000-0001-8402-7160; Xu, Hongwu/0000-0002-0793-6923 FU Advanced Research Projects Agency-Energy (ARPA-E), U.S. Department of Energy (DOE) [DE-AR0000347] FX This work was funded, in part, by the Advanced Research Projects Agency-Energy (ARPA-E), U.S. Department of Energy (DOE), under Award Number DE-AR0000347. The work at Los Alamos National Laboratory was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy Office of Science. The authors thank Prof. John B. Goodenough, Prof. Jianshi Zhou, Dr. Yutao Li, Dr. Luke Daemen, and Dr. John Lemmon for their insightful suggestions. NR 26 TC 7 Z9 7 U1 32 U2 72 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA EI 2198-3844 J9 ADV SCI JI Adv. Sci. PD MAR PY 2016 VL 3 IS 3 AR 1500359 DI 10.1002/advs.201500359 PG 5 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DH0XU UT WOS:000372508400003 PM 27812460 ER PT J AU Stange, B McInerney, J Golden, A Benade, W Neill, B Mayer, A Witter, R Tenney, L Stinson, K Cragle, D Newman, LS AF Stange, Bill McInerney, John Golden, Ashley Benade, Wendy Neill, Barbara Mayer, Annyce Witter, Roxana Tenney, Liliana Stinson, Kaylan Cragle, Donna Newman, Lee S. TI Integrated Approach to Health Screening of Former Department of Energy Workers Detects Both Occupational and Non-Occupational Illness SO AMERICAN JOURNAL OF INDUSTRIAL MEDICINE LA English DT Article DE occupational; non-occupational; exposure-based; integrated; former worker; DOE ID TRADE-CENTER DISASTER; NUCLEAR SITES; BERYLLIUM SENSITIZATION; OLDER CONSTRUCTION; RISK; DISEASE; SYMPTOMS; COHORT; RECOMMENDATIONS; ABNORMALITIES AB Background The National Supplemental Screening Program ( NSSP) uses a Total Worker Health (TM) approach to address U.S. Department of Energy ( DOE) former worker health. This article provides the design of the integrated occupational health screening and promotion program. Methods The NSSP implemented a web-based relational health records system to process demographic, exposure, and clinical data. We present medical findings for 12,000 DOE former workers that completed an initial NSSP medical screening between October 1, 2005 and October 4, 2013. We discuss the DOE former worker participant population and the exposure- based and non-occupational medical screening tests used. Results The NSSP identified potential occupationally related health conditions in 40.5% of those screened. Notably, we identified 85.8% of participants with addressable non-occupational health conditions, many of which were previously undiagnosed. Conclusion The NSSP demonstrates that the identification of potential occupational health issues in conjunction with addressable non-occupational health conditions provides former workers with information to more effectively manage health. (C) 2016 Wiley Periodicals, Inc. C1 [Stange, Bill; McInerney, John; Benade, Wendy] Oak Ridge Associated Univ, Hlth Energy & Environm, 9950 West 80th Ave,Suite 17, Arvada, CO 80005 USA. [Golden, Ashley; Neill, Barbara; Cragle, Donna] Oak Ridge Associated Univ, Hlth Energy & Environm, Oak Ridge, TN USA. [Mayer, Annyce] Natl Jewish Hlth, Dept Med, Div Environm & Occupat Hlth Sci, Denver, CO USA. [Witter, Roxana; Tenney, Liliana; Newman, Lee S.] Univ Colorado, Ctr Worker Hlth & Environm, Colorado Sch Publ Hlth, Anschutz Med Campus, Aurora, CO USA. RP Stange, B (reprint author), Oak Ridge Associated Univ, 9950 West 80th Ave,Suite 17, Arvada, CO 80005 USA. EM bill.stange@orau.org FU Oak Ridge Associated Universities [DE-FC01-05EH04022]; U.S. Department of Energy [DE-FC01-05EH04022] FX The National Supplemental Screening Program is funded by Cooperative Agreement DE-FC01-05EH04022 between Oak Ridge Associated Universities and the U.S. Department of Energy. NR 43 TC 0 Z9 0 U1 1 U2 3 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0271-3586 EI 1097-0274 J9 AM J IND MED JI Am. J. Ind. Med. PD MAR PY 2016 VL 59 IS 3 BP 200 EP 211 DI 10.1002/ajim.22554 PG 12 WC Public, Environmental & Occupational Health SC Public, Environmental & Occupational Health GA DG7UW UT WOS:000372290200005 PM 26891339 ER PT J AU Troutman, VA Strand, CL Campbell, MF Tulgestke, AM Miller, VA Davidson, DF Hanson, RK AF Troutman, V. A. Strand, C. L. Campbell, M. F. Tulgestke, A. M. Miller, V. A. Davidson, D. F. Hanson, R. K. TI High-speed OH* chemiluminescence imaging of ignition through a shock tube end-wall SO APPLIED PHYSICS B-LASERS AND OPTICS LA English DT Article ID HIGH-PRESSURE; TEMPERATURE; ENGINE; WAVES AB A high-speed OH* chemiluminescence imaging diagnostic was developed to image the structure and homogeneity of combustion events behind reflected shock waves in the Stanford Constrained Reaction Volume Shock Tube. An intensified high-repetition-rate imaging system was used to acquire images of OH* chemiluminescence (near 308 nm) through a fused quartz shock tube end-wall window at 10-33 kHz during the combustion of n-heptane (21 % O-2/Ar, phi = 0.5). In general, the imaging technique enabled observation of the main ignition event in the core of the shock tube that corresponded to typical markers of ignition (e.g., pressure rise), as well as localized ignition near the wall that preceded the main core ignition event for some conditions. Case studies were performed to illustrate the utility of this novel imaging diagnostic. First, by comparing localized wall ignition events to the core ignition event, the temperature homogeneity of the post-reflected shock gas near the end-wall was estimated to be within 0.5 % for the test condition presented (T = 1159K, P = 0.25MPa). Second, the effect of a recession in the shock tube wall, created by an observation window, on the combustion event was visualized. Localized ignition was observed near the window, but this disturbance did not propagate to the core of the shock tube before the main ignition event. Third, the effect of shock tube cleanliness was investigated by conducting tests in which the shock tube was not cleaned for multiple consecutive runs. For tests after no cleaning was performed, ignition events were concentrated in the lower half of the shock tube. In contrast, when the shock tube was cleaned, the ignition event was distributed around the entire circumference of the shock tube; validating the cleaning procedure. C1 [Troutman, V. A.; Strand, C. L.; Tulgestke, A. M.; Miller, V. A.; Davidson, D. F.; Hanson, R. K.] Stanford Univ, High Temp Gasdynam Lab, Stanford, CA 94305 USA. [Campbell, M. F.] Sandia Natl Labs, Combust Res Facil, Livermore, CA USA. RP Troutman, VA (reprint author), Stanford Univ, High Temp Gasdynam Lab, Stanford, CA 94305 USA. EM vtrout@stanford.edu OI Troutman, Valerie/0000-0001-6306-6347 FU US Army Research Laboratory; US Army Research Office [W911NF1310206]; Gabilan Stanford Graduate Fellowship; National Science Foundation Graduate Research Fellowship Program [DGE-114747]; AFOSR; National Defense Science and Engineering Graduate Fellowship [32CFR168a] FX This material is based upon work supported by the US Army Research Laboratory and the US Army Research Office under Contract/Grant Number W911NF1310206, with Ralph Anthenien as contract monitor. We acknowledge loan of the intensified camera system from an AFOSR-sponsored research program. V.A.T. was supported by the Gabilan Stanford Graduate Fellowship and the National Science Foundation Graduate Research Fellowship Program (Grant No. DGE-114747). Any opinion, findings and conclusions or recommendations expressed in this material are those of the authors(s) and do not necessarily reflect the views of the National Science Foundation. M.F.C. was supported by a National Defense Science and Engineering Graduate Fellowship (32CFR168a). NR 19 TC 0 Z9 0 U1 3 U2 8 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0946-2171 EI 1432-0649 J9 APPL PHYS B-LASERS O JI Appl. Phys. B-Lasers Opt. PD MAR PY 2016 VL 122 IS 3 AR 56 DI 10.1007/s00340-016-6326-y PG 7 WC Optics; Physics, Applied SC Optics; Physics GA DG7RY UT WOS:000372282600011 ER PT J AU Skrodzki, PJ Becker, JR Diwakar, PK Harilal, SS Hassanein, A AF Skrodzki, Patrick J. Becker, Jason R. Diwakar, Prasoon K. Harilal, Sivanandan S. Hassanein, Ahmed TI A Comparative Study of Single-pulse and Double-pulse Laser-Induced Breakdown Spectroscopy with Uranium-containing Samples SO APPLIED SPECTROSCOPY LA English DT Article DE Double-pulse laser-induced breakdown spectroscopy; DPLIBS; Nuclear forensics; Uranium; Signal enhancement; Plasma diagnostics ID SIGNAL ENHANCEMENT; PLASMA; LIBS; WAVELENGTH; ABLATION; THORIUM AB Laser-induced breakdown spectroscopy (LIBS) holds potential advantages in special nuclear material (SNM) sensing and nuclear forensics, which require rapid analysis, minimal sample preparation, and stand-off distance capability. SNM, such as U, however, result in crowded emission spectra with LIBS, and characteristic emission lines are challenging to discern. It is well-known that double-pulse LIBS (DPLIBS) improves the signal intensity for analytes over conventional single-pulse LIBS (SPLIBS). This study investigates the U signal in a glass matrix using DPLIBS and compares it to signal obtained using SPLIBS. Double-pulse LIBS involves sequential firing of a 1.06 mu m Nd:YAG pre-pulse and 10.6 mu m TEA CO2 heating pulse in a near collinear geometry. Optimization of experimental parameters including inter-pulse delay and energy follows identification of characteristic lines for the bulk analyte Ca and the minor constituent analyte U for both DPLIBS and SPLIBS. Spatial and temporal coupling of the two pulses in the proposed DPLIBS technique yields improvements in analytical merits with a negligible increase in damage to the sample compared to SPLIBS. Subsequently, the study discusses optimum plasma emission conditions of U lines and relative figures of merit in both SPLIBS and DPLIBS. Investigation into plasma characteristics also addresses plausible mechanisms related to the observed U analyte signal variation between SPLIBS and DPLIBS. C1 [Skrodzki, Patrick J.; Becker, Jason R.; Diwakar, Prasoon K.; Hassanein, Ahmed] Purdue Univ, Ctr Mat Extreme Environm CMUXE, Sch Nucl Engn, 400 Cent Dr, W Lafayette, IN 47907 USA. [Harilal, Sivanandan S.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Diwakar, PK (reprint author), Purdue Univ, Ctr Mat Extreme Environm CMUXE, Sch Nucl Engn, 400 Cent Dr, W Lafayette, IN 47907 USA. EM pdiwakar@purdue.edu RI Harilal, Sivanandan/B-5438-2014 OI Harilal, Sivanandan/0000-0003-2266-7976 FU NSF-PIRE project; DOE/NNSA Office of Nonproliferation and Verification Research and Development [NA-22]; Purdue Summer Undergraduate Research Fellowship (SURF) program FX This work is partially supported by NSF-PIRE project and DOE/NNSA Office of Nonproliferation and Verification Research and Development (NA-22). PJ Skrodzki and JR Becker would like to acknowledge the Purdue Summer Undergraduate Research Fellowship (SURF) program for partial support. NR 25 TC 1 Z9 1 U1 9 U2 26 PU SAGE PUBLICATIONS INC PI THOUSAND OAKS PA 2455 TELLER RD, THOUSAND OAKS, CA 91320 USA SN 0003-7028 EI 1943-3530 J9 APPL SPECTROSC JI Appl. Spectrosc. PD MAR PY 2016 VL 70 IS 3 BP 467 EP 473 DI 10.1177/0003702815626670 PG 7 WC Instruments & Instrumentation; Spectroscopy SC Instruments & Instrumentation; Spectroscopy GA DH1OH UT WOS:000372554000006 PM 26810184 ER PT J AU Dolan, MM Mathews, GJ Lam, DD Lan, NQ Herczeg, GJ Dearborn, DSP AF Dolan, Michelle M. Mathews, Grant J. Doan Duc Lam Nguyen Quynh Lan Herczeg, Gregory J. Dearborn, David S. P. TI EVOLUTIONARY TRACKS FOR BETELGEUSE SO ASTROPHYSICAL JOURNAL LA English DT Article DE stars: evolution; stars: individual (Alpha Orionis); stars: late-type; stars: mass-loss; stars: oscillations; starspots; supergiants ID MASS-LOSS RATES; TURBULENT COMPRESSIBLE CONVECTION; CLOSE CIRCUMSTELLAR ENVIRONMENT; RED SUPERGIANT BETELGEUSE; STELLAR ASTROPHYSICS MESA; 1ST OVERTONE LINES; EQUATION-OF-STATE; ALPHA-ORIONIS; DYNAMICAL ATMOSPHERE; ANGULAR DIAMETER AB We have constructed a series of nonrotating quasi-hydrostatic evolutionary models for the M2 Iab supergiant Betelgeuse (alpha Orionis). Our models are constrained by multiple observed values for the temperature, luminosity, surface composition, and mass loss for this star, along with the parallax distance and high-resolution imagery that determines its radius. We have then applied our best-fit models to analyze the observed variations in surface luminosity and the size of detected surface bright spots as the result of up-flowing convective material from regions of high temperature in the surface convective zone. We also attempt to explain the intermittently observed periodic variability in a simple radial linear adiabatic pulsation model. Based on the best fit to all observed data, we suggest a best progenitor mass estimate of 20(-3)(+5) M-circle dot and a current age from the start of the zero-age main sequence of 8.0-8.5 Myr based on the observed ejected mass while on the giant branch. C1 [Dolan, Michelle M.; Mathews, Grant J.] Univ Notre Dame, Dept Phys, Ctr Astrophys, Notre Dame, IN 46656 USA. [Doan Duc Lam] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Nguyen Quynh Lan] Hanoi Natl Univ Educ, Dept Phys, Hanoi, Vietnam. [Herczeg, Gregory J.] Peking Univ, Kavli Inst Astron & Astrophys, Beijing 100871, Peoples R China. [Dearborn, David S. P.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Dolan, MM; Mathews, GJ (reprint author), Univ Notre Dame, Dept Phys, Ctr Astrophys, Notre Dame, IN 46656 USA.; Lam, DD (reprint author), Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden.; Lan, NQ (reprint author), Hanoi Natl Univ Educ, Dept Phys, Hanoi, Vietnam.; Herczeg, GJ (reprint author), Peking Univ, Kavli Inst Astron & Astrophys, Beijing 100871, Peoples R China.; Dearborn, DSP (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM velasnr@gmail.com; gmathews@nd.edu; lam.doan@physics.uu.se; nquynhlan@hnue.edu.vn; gherczeg1@gmail.com; ddearborn@llnl.gov OI Herczeg, Gregory/0000-0002-7154-6065 FU DoE Nuclear Theory grant [DE-FG02-95ER40934]; NSF Joint Institute for Nuclear Astrophysics FX Work at Notre Dame is supported by DoE Nuclear Theory grant number DE-FG02-95ER40934. One of the authors (N.Q. L.) acknowledges support from the NSF Joint Institute for Nuclear Astrophysics. NR 141 TC 2 Z9 2 U1 2 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 1 PY 2016 VL 819 IS 1 AR 7 DI 10.3847/0004-637X/819/1/7 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DG7ZY UT WOS:000372303400007 ER PT J AU MacLeod, M Guillochon, J Ramirez-Ruiz, E Kasen, D Rosswog, S AF MacLeod, Morgan Guillochon, James Ramirez-Ruiz, Enrico Kasen, Daniel Rosswog, Stephan TI OPTICAL THERMONUCLEAR TRANSIENTS FROM TIDAL COMPRESSION OF WHITE DWARFS AS TRACERS OF THE LOW END OF THE MASSIVE BLACK HOLE MASS FUNCTION SO ASTROPHYSICAL JOURNAL LA English DT Article DE accretion, accretion disks; black hole physics; methods: numerical; radiative transfer; white dwarfs ID GAMMA-RAY BURST; EARLY-TYPE GALAXIES; IA SUPERNOVAE; X-RAY; SWIFT J1644+57; GRAVITATIONAL-WAVES; DISRUPTION FLARES; GLOBULAR-CLUSTERS; STAR DISTRIBUTION; LIGHT CURVES AB In this paper, we model the observable signatures of tidal disruptions of white dwarf (WD) stars using massive black holes (MBHs) of moderate mass, approximate to 10(3)-10(5) M-circle dot. When the WD passes deep enough within the MBH's tidal field, these signatures include thermonuclear transients from burning during maximum compression. We combine a hydrodynamic simulation that includes nuclear burning of the disruption of a 0.6 M-circle dot C/O WD with a Monte Carlo radiative transfer calculation to synthesize the properties of a representative transient. The transient's emission emerges in the optical, with light. curves and spectra reminiscent of Type I supernovae. The properties are strongly viewing. angle dependent, and key spectral signatures are approximate to 10,000 km s(-1) doppler shifts, due to the orbital motion of the unbound ejecta. Disruptions of He WDs likely produce large quantities of intermediate-mass elements, offering a possible production mechanism for Ca-rich transients. Accompanying multi-wavelength transients are fueled by accretion and arise from the nascent accretion disk and relativistic jet. If MBHs of moderate mass exist with number densities similar to those of supermassive BHs, both high-energy wide-field monitors and upcoming optical surveys should detect tens to hundreds of WD tidal disruptions per year. The current best strategy for their detection may therefore be deep optical follow-up of high-energy transients of unusually long duration. The detection rate or the nondetection of these transients by current and upcoming surveys can thus be used to place meaningful constraints on the extrapolation of the MBH mass function to moderate masses. C1 [MacLeod, Morgan; Ramirez-Ruiz, Enrico] Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 95064 USA. [Guillochon, James] Harvard Smithsonian Ctr Astrophys, Inst Theory & Computat, 60 Garden St, Cambridge, MA 02138 USA. [Kasen, Daniel] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Kasen, Daniel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Rosswog, Stephan] Stockholm Univ, AlbaNova, Dept Astron, Oskar Klein Ctr, SE-10691 Stockholm, Sweden. RP MacLeod, M (reprint author), Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 95064 USA. OI Guillochon, James/0000-0002-9809-8215 FU UCSC; Packard Foundation; Radcliffe Institute for Advanced Study; NASA ATP grant [NNX14AH37G]; Einstein Grant [PF3-140108]; DFG [RO-3399/8-1, AOBJ-575415]; Swedish Research Council (VR) [621-2012-4870] FX We thank Maria Drout for guidance and data used in Figure 6, and Ryan Foley for helpful discussions and comments on an early version of this manuscript. We are grateful to Laura Chomiuk and Sjoert van Velzen for comments on radio afterglows of tidal disruption events and to Sjoert van Velzen for sharing code to estimate their properties. We further acknowledge helpful conversations with Roseanne Cheng, Lixin Dai, Julian Krolik, Tom Maccarone, Phillip Macias, Michela Mapelli, Cole Miller, Dheeraj Pasham, Martin Rees, Elena Rossi, and Michele Trenti. M.M. is grateful for the support of the Chancellor's Fellowship at UCSC. E.R.-R. acknowledges financial support from the Packard Foundation, Radcliffe Institute for Advanced Study, and NASA ATP grant NNX14AH37G. J.G. acknowledges support from Einstein Grant PF3-140108. S.R. was supported by the DFG under RO-3399/8-1, AOBJ-575415 and by the Swedish Research Council (VR) under grant 621-2012-4870. Part of the simulations have been performed at the facilities of the The North-German Supercomputing Alliance (HLRN). NR 119 TC 5 Z9 5 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 1 PY 2016 VL 819 IS 1 AR 3 DI 10.3847/0004-637X/819/1/3 PG 17 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DG7ZY UT WOS:000372303400003 ER PT J AU Nickels, JD Atkinson, J Papp-Szabo, E Stanley, C Diallo, SO Perticaroli, S Baylis, B Mahon, P Ehlers, G Katsaras, J Dutcher, JR AF Nickels, Jonathan D. Atkinson, John Papp-Szabo, Erzsebet Stanley, Christopher Diallo, Souleymane O. Perticaroli, Stefania Baylis, Benjamin Mahon, Perry Ehlers, Georg Katsaras, John Dutcher, John R. TI Structure and Hydration of Highly-Branched, Monodisperse Phytoglycogen Nanoparticles SO BIOMACROMOLECULES LA English DT Article ID WATER-PROTEIN FLUCTUATIONS; NEUTRON-SCATTERING; AQUEOUS-SOLUTIONS; LIGHT-SCATTERING; DIELECTRIC-RELAXATION; BIOLOGICAL-MEMBRANES; PHYSICAL CONSTRAINTS; GLYCOGEN STRUCTURE; SUPERCOOLED WATER; TIME SCALES AB Phytoglycogen is a naturally occurring polysaccharide nano particle made up of extensively branched glucose monomers. It has a number of unusual and advantageous properties, such as high water retention, low viscosity, and high stability in water, which make this biomaterial a promising candidate for a wide variety of applications. In this study, we have characterized the structure and hydration of aqueous dispersions of phytoglycogen nanoparticles using neutron scattering. Small angle neutron scattering results suggest that the phytoglycogen nanoparticles behave similar to hard sphere colloids and are hydrated by a large number of water molecules (each nanoparticle contains between 250% and 285% of its mass in water). This suggests that phytoglycogen is an ideal sample in which to study the dynamics of hydration water. To this end, we used quasielastic neutron scattering (QENS) to provide an independent and consistent measure of the hydration number, and to estimate the retardation factor (or degree of water slow-down) for hydration wafer translational motions. These data demonstrate a length-scale dependence in the measured retardation factors that clarifies the origin of discrepancies between retardation factor values reported for hydration water using different experimental techniques. The present approach can be generalized to other systems containing nanoconfined water. C1 [Nickels, Jonathan D.; Katsaras, John] Oak Ridge Natl Lab, Joint Inst Neutron Sci, Oak Ridge, TN 37831 USA. [Nickels, Jonathan D.; Katsaras, John] Univ Tennessee, Dept Phys, Knoxville, TN 37996 USA. [Atkinson, John; Papp-Szabo, Erzsebet; Perticaroli, Stefania; Baylis, Benjamin; Mahon, Perry; Dutcher, John R.] Univ Guelph, Dept Phys, Guelph, ON N1G 2W1, Canada. [Nickels, Jonathan D.; Stanley, Christopher; Katsaras, John] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. [Diallo, Souleymane O.] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Ehlers, Georg] Oak Ridge Natl Lab, Quantum Condensed Matter Div, POB 2008, Oak Ridge, TN 37831 USA. RP Dutcher, JR (reprint author), Univ Guelph, Dept Phys, Guelph, ON N1G 2W1, Canada. EM dutcher@uoguelph.ca RI Nickels, Jonathan/I-1913-2012; Ehlers, Georg/B-5412-2008; OI Nickels, Jonathan/0000-0001-8351-7846; Ehlers, Georg/0000-0003-3513-508X; Stanley, Christopher/0000-0002-4226-7710; Katsaras, John/0000-0002-8937-4177 FU Ontario Ministry of Agriculture (OMAF); Natural Sciences and Engineering Research Council (NSERC) of Canada; Senior Canada Research Chair in Soft Matter and Biological Physics; U.S. DOE BES through EPSCoR [DE-FG02-08ER46528]; US DOE [DE-AC05-00OR22725] FX The authors would like to thank Phil Whiting, Anton Korenevski, and Michael Grossutti for discussions that have greatly benefitted this work. Mirexus Biotechnologies, Inc. generously supplied the monodisperse phytoglycogen nano particles. This work was funded by grants from the Ontario Ministry of Agriculture (OMAF) and the Natural Sciences and Engineering Research Council (NSERC) of Canada (J.R.D.). J.R.D. is the recipient of a Senior Canada Research Chair in Soft Matter and Biological Physics. J.D.N. is partially supported by the U.S. DOE BES through EPSCoR Grant No. DE-FG02-08ER46528. J.K. is supported through the Scientific User Facilities Division of the DOE Office of Basic Energy Sciences under US DOE Contract No. DE-AC05-00OR22725. Facilities as the Spallation Neutron Source are managed by UT-Battelle, LLC under US DOE Contract No. DE-AC05-00OR22725. NR 61 TC 4 Z9 4 U1 5 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1525-7797 EI 1526-4602 J9 BIOMACROMOLECULES JI Biomacromolecules PD MAR PY 2016 VL 17 IS 3 BP 735 EP 743 DI 10.1021/acs.biomac.5b01393 PG 9 WC Biochemistry & Molecular Biology; Chemistry, Organic; Polymer Science SC Biochemistry & Molecular Biology; Chemistry; Polymer Science GA DG9GW UT WOS:000372391800004 PM 26866896 ER PT J AU VanDelinder, V Brener, S Bachand, GD AF VanDelinder, Virginia Brener, Stephanie Bachand, George D. TI Mechanisms Underlying the Active Self-Assembly of Microtubule Rings and Spools SO BIOMACROMOLECULES LA English DT Article ID COUNTERCLOCKWISE MOTION; RIGIDITY; SYSTEMS; ROTATIONS; NANOWIRES; TRANSPORT; FILAMENTS; BEHAVIOR; FORCE AB Active self-assembly offers a powerful route for the creation of dynamic multiscale structures that are presently inaccessible with standard microfabrication techniques. One such system uses the translation of microtubule filaments by surface-tethered kinesin to actively assemble nanocomposites with bundle, ring, and spool morphologies. Attempts to observe mechanisms involved in this active assembly system have been hampered by experimental difficulties with performing observation during buffer exchange and photodamage from fluorescent excitation. In the present work, we used a custom microfluidic device to remove these limitations and directly study ring/spool formation, including the earliest events (nucleation) that drive subsequent nanocomposite assembly. Three distinct formation events were observed: pinning, collisions, and induced curvature. Of these three, collisions accounted for the majority of event leading to ring/spool formation, while the rate of pinning was shown to be dependent on the amount of photodamage in the system. We further showed that formation mechanism directly affects the diameter and rotation direction of the resultant rings and spools. Overall, the fundamental understanding described in this work provides a foundation by which the properties of motor-driven, actively assembled nanocomposites may be tailored toward specific applications. C1 [VanDelinder, Virginia; Brener, Stephanie; Bachand, George D.] Sandia Natl Labs, Ctr Integrated Nanotechnol, POB 5800,MS 1303, Albuquerque, NM 87111 USA. RP Bachand, GD (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol, POB 5800,MS 1303, Albuquerque, NM 87111 USA. EM gdbacha@sandia.gov OI Bachand, George/0000-0002-3169-9980 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering (BES-MSE); U.S. Department of Energy (DOE), Office of Science [RA 2013A0021]; Lockheed Martin Corporation, for U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering (BES-MSE). This work was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE), Office of Science (user Project No. RA 2013A0021). Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 36 TC 1 Z9 1 U1 5 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1525-7797 EI 1526-4602 J9 BIOMACROMOLECULES JI Biomacromolecules PD MAR PY 2016 VL 17 IS 3 BP 1048 EP 1056 DI 10.1021/acs.biomac.5b01684 PG 9 WC Biochemistry & Molecular Biology; Chemistry, Organic; Polymer Science SC Biochemistry & Molecular Biology; Chemistry; Polymer Science GA DG9GW UT WOS:000372391800036 PM 26842978 ER PT J AU Lucius, M Falatach, R McGlone, C Makaroff, K Danielson, A Williams, C Nix, JC Konkolewicz, D Page, RC Berberich, JA AF Lucius, Melissa Falatach, Rebecca McGlone, Cameron Makaroff, Katherine Danielson, Alex Williams, Cameron Nix, Jay C. Konkolewicz, Dominik Page, Richard C. Berberich, Jason A. TI Investigating the Impact of Polymer Functional Groups on the Stability and Activity of Lysozyme-Polymer Conjugates SO BIOMACROMOLECULES LA English DT Article ID DIFFERENTIAL SCANNING FLUOROMETRY; GRAFTING-FROM; INDUCED INACTIVATION; RESPONSIVE POLYMERS; RAFT POLYMERIZATION; PROTEIN STABILITY; ENZYME-ACTIVITY; PEGYLATION; SURFACE; PEG AB Polymers are often conjugated to proteins to improve stability; however, the impact of polymer chain length and functional groups on protein structure and function is not Well understood. Here we use RAFT polymerization to grow polymers of different lengths and functionality from a short acrylamide oligomer with a RAFT end group conjugated to lysozyme. We show by X-ray crystallography that enzyme structure is minimally impacted by modification with the RAFT end group. Significant activity toward the negatively charged Micrococcus lysodeicticus cell wall was maintained when lysozyme was modified with cationic polymers. Thermal and chemical stability of the conjugates was characterized using differential scanning fluorimetry and tryptophan fluorescence. All conjugates had a lower melting temperature; however, conjugates containing ionic or substrate mimicking polymers were more resistant to denaturation by guanidine hydrochloride. Our results demonstrate that tailoring polymer functionality can improve conjugate activity and minimize enzymatic inactivation by denaturants. C1 [Lucius, Melissa; McGlone, Cameron; Makaroff, Katherine; Danielson, Alex; Williams, Cameron; Konkolewicz, Dominik] Miami Univ, Dept Chem & Biochem, Oxford, OH 45056 USA. [Page, Richard C.; Berberich, Jason A.] Miami Univ, Dept Chem Paper & Biomed Engn, Oxford, OH 45056 USA. [Nix, Jay C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biol Consortium, Adv Light Source, Beamline 4-2-2, Berkeley, CA 94720 USA. RP Konkolewicz, D (reprint author), Miami Univ, Dept Chem & Biochem, Oxford, OH 45056 USA.; Page, RC; Berberich, JA (reprint author), Miami Univ, Dept Chem Paper & Biomed Engn, Oxford, OH 45056 USA. EM d.konkolewicz@miamioh.edu; pagerc@miamioh.edu; berberj@miamioh.edu OI Page, Richard/0000-0002-3006-3171 FU Miami University Committee on Faculty Research; U.S. Department of Energy at Lawrence Berkeley National Laboratory [DE-AC03-76SF00098] FX We are grateful to M. Sameer Al-Abdul-Wahid for assistance with the mass spectrometry analysis. D.K., RC.P., and J.A.B. acknowledge institutional startup funds from Miami University. JA.B. acknowledges the Miami University Committee on Faculty Research for support. The Advanced Light Source is supported by the U.S. Department of Energy under contract number DE-AC03-76SF00098 at Lawrence Berkeley National Laboratory. NR 60 TC 9 Z9 9 U1 12 U2 45 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1525-7797 EI 1526-4602 J9 BIOMACROMOLECULES JI Biomacromolecules PD MAR PY 2016 VL 17 IS 3 BP 1123 EP 1134 DI 10.1021/acs.biomac.5b01743 PG 12 WC Biochemistry & Molecular Biology; Chemistry, Organic; Polymer Science SC Biochemistry & Molecular Biology; Chemistry; Polymer Science GA DG9GW UT WOS:000372391800045 PM 26866284 ER PT J AU Malfatti, MA Kuhn, EA Turteltaub, KW Vickers, SM Jensen, EH Strayer, L Anderson, KE AF Malfatti, Michael A. Kuhn, Edward A. Turteltaub, Kenneth W. Vickers, Selwyn M. Jensen, Eric H. Strayer, Lori Anderson, Kristin E. TI Disposition of the Dietary Mutagen 2-Amino-3,8-dimethylimidazo[4,5-f]quinoxaline in Healthy and Pancreatic Cancer Compromised Humans SO CHEMICAL RESEARCH IN TOXICOLOGY LA English DT Article ID ACCELERATOR MASS-SPECTROMETRY; MEAT INTAKE; HETEROCYCLIC AMINES; COLORECTAL-CANCER; COLON-CANCER; DNA-ADDUCT; RISK; EXPOSURE; ASSOCIATIONS; METABOLISM AB Pancreatic cancer is the fourth leading cause of cancer death in the U.S. Once diagnosed, prognosis is poor with a 5-year survival rate of less than 5%. Exposure to carcinogenic heterocyclic amines (HCAs) derived from cooked meat has been shown to be positively associated with pancreatic cancer risk. To evaluate the processes that determine the carcinogenic potential of HCAs for human pancreas, 14-carbon labeled 2-amino-3,8-dimethylimidazo [4,5-f]quinoxaline (MeIQx), a putative human carcinogenic HCA found in well-done cooked meat, was administered at a dietary relevant dose to human volunteers diagnosed with pancreatic cancer undergoing partial pancreatectomy and healthy control volunteers. After C-14-MeIQx exposure, blood and urine were collected for pharmacokinetic and metabolite analysis. MeIQx-DNA adducts levels were quantified by accelerator mass spectrometry from pancreatic tissue excised during surgery from the cancer patient group. Pharmacokinetic analysis of plasma revealed a rapid distribution of MeIQx with a plasma elimination half-life of approximately 3.5 h in 50%' of the cancer patients and all of the control volunteers. In 2 of the 4 cancer patients, very low levels of MeIQx were detected in plasma and urine suggesting low absorption from the gut into the plasma. Urinary, metabolite analysis revealed five MeIQx metabolites with 2-amino-3-methylimidazo[4,5-f]quinoxaline-8-carboxylic acid being the most abundant accounting for 25%-50% of the recovered 14-carbon/mL urine. There was no discernible difference in metabolite levels between the cancer patient volunteers and-the control group. MeIQx-DNA adduct analysis of pancreas and duodenum tissue revealed adduct levels indistinguishable from background levels. Although other meat derived HCA mutagens have been shown to bind DNA in pancreatic tissue, indicating that exposure to HCAs from cooked meat cannot be discounted as a risk factor for pancreatic cancer, the results from this current study show that exposure to a single dietary dose of MeIQx does not readily form measurable DNA adducts under the conditions of the experiment. C1 [Malfatti, Michael A.; Kuhn, Edward A.; Turteltaub, Kenneth W.] Lawrence Livermore Natl Lab, Biosci & Biotechnol Div, Phys & Life Sci Directorate, 7000 East Ave,L-452, Livermore, CA 94550 USA. [Vickers, Selwyn M.] Univ Alabama Birmingham, 1720 2nd Ave South, Birmingham, AL 35233 USA. [Jensen, Eric H.; Strayer, Lori; Anderson, Kristin E.] Univ Minnesota, Minneapolis, MN 55455 USA. RP Malfatti, MA (reprint author), Lawrence Livermore Natl Lab, Biosci & Biotechnol Div, Phys & Life Sci Directorate, 7000 East Ave,L-452, Livermore, CA 94550 USA. FU U.S. Department of Energy by Lawrence Livermore National Laboratory at the Research Resource for Biomedical AMS [DE-AC52-07NA27344]; National Institute of General Medical Sciences [2P41GM103483-16]; UAB/UMN SPORE in Pancreatic Cancer (NIH/NCI) [P50 CA101955-07] FX This work was performed under the auspices of the U.S. Department of Energy by, Lawrence Livermore National Laboratory at the Research Resource for Biomedical AMS under contract DE-AC52-07NA27344 and supported by a grant from the National Institute of General Medical Sciences (2P41GM103483-16). Support was also provided through a pilot funding mechanism from UAB/UMN SPORE in Pancreatic Cancer (NIH/NCI P50 CA101955-07). NR 40 TC 2 Z9 2 U1 2 U2 2 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0893-228X EI 1520-5010 J9 CHEM RES TOXICOL JI Chem. Res. Toxicol. PD MAR PY 2016 VL 29 IS 3 BP 352 EP 358 DI 10.1021/acs.chemrestox.5b00495 PG 7 WC Chemistry, Medicinal; Chemistry, Multidisciplinary; Toxicology SC Pharmacology & Pharmacy; Chemistry; Toxicology GA DH3HK UT WOS:000372677900012 PM 26918625 ER PT J AU Williams, TJ AF Williams, Timothy J. TI Delivering Science on Day One SO COMPUTING IN SCIENCE & ENGINEERING LA English DT Article C1 [Williams, Timothy J.] Argonne Natl Lab, Argonne Leadership Comp Facil, Early Sci Program, Argonne, IL 60439 USA. RP Williams, TJ (reprint author), Argonne Natl Lab, Argonne Leadership Comp Facil, Early Sci Program, Argonne, IL 60439 USA. EM tjwilliams@anl.gov FU DOE Office of Science User Facility [DE-AC02-06CH11357, DE-AC05-00OR22725] FX The Argonne Leadership Computing Facility is a DOE Office of Science User Facility supported under contract DE-AC02-06CH11357. The Oak Ridge Leadership Computing Facility is a DOE Office of Science User Facility supported under contract DE-AC05-00OR22725. I gratefully acknowledge the assistance of Laura Wolf, Argonne National Laboratory, in editing this article. NR 0 TC 0 Z9 0 U1 1 U2 1 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 1521-9615 EI 1558-366X J9 COMPUT SCI ENG JI Comput. Sci. Eng. PD MAR-APR PY 2016 VL 18 IS 2 BP 104 EP 107 DI 10.1109/MCSE.2016.22 PG 4 WC Computer Science, Interdisciplinary Applications SC Computer Science GA DH3MX UT WOS:000372692200012 ER PT J AU Iisa, K French, RJ Orton, KA Yung, MM Johnson, DK ten Dam, J Watson, MJ Nimlos, MR AF Iisa, Kristiina French, Richard J. Orton, Kellene A. Yung, Matthew M. Johnson, David K. ten Dam, Jeroen Watson, Michael J. Nimlos, Mark R. TI In Situ and ex Situ Catalytic Pyrolysis of Pine in a Bench-Scale Fluidized Bed Reactor System SO ENERGY & FUELS LA English DT Article ID MISCANTHUS X GIGANTEUS; BIOMASS PYROLYSIS; BIO-OIL; LIGNOCELLULOSIC BIOMASS; ZEOLITES; PRODUCTS; VAPORS; FUEL; HYDROCARBONS; PERFORMANCE AB In situ and ex situ catalytic pyrolysis were compared in a system with two 2-in. bubbling fluidized bed reactors. Pine was pyrolyzed in the system with a catalyst, HZSM-5 with a silica-to-alumina ratio of 30, placed either in the first (pyrolysis) reactor or the second (upgrading) reactor. Both the pyrolysis and upgrading temperatures were 500 degrees C, and the weight hourly space velocity was 1.1 h(-1). Five catalytic cycles were completed in each experiment. The catalytic cyder were continued until oxygenates in the vapors became dominant. The catalyst was then oxidized, after which a new catalytic cycle was begun. The in situ configuration gave slightly higher oil yield but also higher oxygen content than the ex situ configuration, which indicates that the catalyst deactivated faster in the in situ configuration than the ex situ configuration. Analysis of the spent catalysts confirmed higher accumulation of metals in the in situ experiment. In all experiments, the organic oil mass yields varied between 14 and 17% and the carbon efficiencies between 20 and 25%. The organic oxygen concentrations in the oils were 16-18%, which represented a 45% reduction compared to corresponding noncatalytic pyrolysis oils prepared in the same fluidized bed reactor system. GC/MS analysis showed the oils to contain one-to four-ring aromatic hydrocarbons and a variety of oxygenates (phenols, furans, benzofurans, methoxyphenols, naphthalenols, indenols). High fractions of oxygen were rejected as water, CO, and CO,, which indicates the importance of dehydration, decarbonylation, and decarboxylation reactions. Light gases were the major sources of carbon losses, followed by char and coke. C1 [Iisa, Kristiina; French, Richard J.; Orton, Kellene A.; Yung, Matthew M.; Johnson, David K.; Nimlos, Mark R.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [ten Dam, Jeroen; Watson, Michael J.] Johnson Matthey Technol Ctr, Billingham TS23 1LB, Cleveland, England. RP Iisa, K (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM kristiina.iisa@nrel.gov FU U.S. Department of Energy [DE-AC36-08GO28308]; National Renewable Energy Laboratory; U.S. DOE Office of Energy Efficiency and Renewable Energy Bioenergy Technologies Office FX This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08GO28308 with the National Renewable Energy Laboratory. Funding provided by U.S. DOE Office of Energy Efficiency and Renewable Energy Bioenergy Technologies Office is gratefully acknowledged. We wish to thank Scott Palmer, Michele Myers, Ming Pan, Alexander Stanton, Matt Plumb, Bill Michener, Stuart Black, Steve Deutch, Renee Happs, Dr. Erica Gjersing, Dr. Calvin Mukarakate, and Dr. Robert Baldwin for their technical assistance and discussions. NR 65 TC 3 Z9 3 U1 6 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0887-0624 EI 1520-5029 J9 ENERG FUEL JI Energy Fuels PD MAR PY 2016 VL 30 IS 3 BP 2144 EP 2157 DI 10.1021/acs.energyfuels.5b02165 PG 14 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DH1RO UT WOS:000372562800069 ER PT J AU Park, LKE Ren, SJ Yiacoumi, S Ye, XP Borole, AP Tsouris, C AF Park, Lydia Kyoung-Eun Ren, Shoujie Yiacoumi, Sotira Ye, X. Philip Borole, Abhijeet P. Tsouris, Costas TI Separation of Switchgrass Bio-Oil by Water/Organic Solvent Addition and pH Adjustment SO ENERGY & FUELS LA English DT Article ID FAST PYROLYSIS; AQUEOUS-PHASE; ACETIC-ACID; BIOMASS; EXTRACTION; RECOVERY; HYDRODEOXYGENATION; CONVERSION; FRACTION; GAS AB Applications of bio-oil are limited by its challenging properties including high moisture content, low pH, high viscosity, high oxygen content, and low heating value. Separation of switchgrass bio-oil components by adding water, organic solvents (hexadecane and octane), and sodium hydroxide may help to overcome these issues. Acetic acid and phenolic compounds were extracted in aqueous and organic phases, respectively. Polar chemicals, such as acetic acid, did not partition in the organic solvent phase. Acetic acid in the aqueous phase after extraction is beneficial for a microbial-electrolysis-cell application to produce hydrogen as an energy source for further hydrodeoxygenation of bio-oil. Organic solvents extracted more chemicals from bio-oil in combined than in sequential extraction; however, organic solvents partitioned into the aqueous phase in combined extraction. When sodium hydroxide was added to adjust the pH of aqueous bio-oil, organic-phase precipitation occurred. As the pH was increased, a biphasic aqueous/organic dispersion was formed, and phase separation was optimized at approximately pH 6. The neutralized organic bio-oil had approximately 37% less oxygen and 100% increased heating value than the initial centrifuged bio-oil. The less oxygen content and increased heating value indicated a significant improvement of the bio-oil quality through neutralization. C1 [Park, Lydia Kyoung-Eun; Yiacoumi, Sotira; Tsouris, Costas] Georgia Inst Technol, Atlanta, GA 30332 USA. [Ren, Shoujie; Ye, X. Philip] Univ Tennessee, Inst Agr, Knoxville, TN 37996 USA. [Borole, Abhijeet P.] Univ Tennessee, Bredesen Ctr Interdisciplinary Res & Educ, Knoxville, TN 37996 USA. [Borole, Abhijeet P.; Tsouris, Costas] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Tsouris, C (reprint author), Georgia Inst Technol, Atlanta, GA 30332 USA.; Tsouris, C (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM tsourisc@ornl.gov RI Tsouris, Costas/C-2544-2016; OI Tsouris, Costas/0000-0002-0522-1027; Borole, Abhijeet/0000-0001-8423-811X FU U.S. Department of Energy, BioEnergy Technologies Office, under the CHASE program; U.S. Department of Energy [DEAC05-00OR22725]; Department of Energy FX The authors are thankful to Niki Labbe and Pyongchung Kim of the University of Tennessee at Knoxville for providing pyrolysis oil, David Bostwick from the BioAnalytical Mass Spectrometry Facility at the Georgia Institute of Technology (GIT) for assistance with GC-MS analysis, and Xiaofei (Sophie) Zeng and Spyros G. Pavlostathis of GIT for assistance with HPLC analysis. The authors also thank ALS Environmental for analyzing the oxygen content and heating value of product samples. This work was funded by the U.S. Department of Energy, BioEnergy Technologies Office, under the CHASE program. The manuscript has been coauthored by UT-Battelle, LLC, under Contract No. DEAC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 31 TC 2 Z9 2 U1 10 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0887-0624 EI 1520-5029 J9 ENERG FUEL JI Energy Fuels PD MAR PY 2016 VL 30 IS 3 BP 2164 EP 2173 DI 10.1021/acs.energyfuels.5b02537 PG 10 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DH1RO UT WOS:000372562800071 ER PT J AU Lee, CW Zhao, YX Lu, SY Stevens, WR AF Lee, Chun Wai Zhao, Yongxin Lu, Shengyong Stevens, William R. TI Catalytic Destruction of a Surrogate Organic Hazardous Air Pollutant as a Potential Co-benefit for Coal-Fired Selective Catalytic Reduction Systems SO ENERGY & FUELS LA English DT Article ID MERCURY OXIDATION; FLUE-GAS; AROMATIC-HYDROCARBONS; COMBUSTION CONDITIONS; INCINERATION PLANTS; REAL-TIME; EMISSIONS; 1,2-DICHLOROBENZENE; PARTICLES; PYROLYSIS AB Catalytic destruction of benzene (C6H6), a surrogate for organic hazardous air pollutants (HAPs) produced from coal combustion, was investigated using a commercial selective catalytic reduction (SCR) catalyst for evaluating the potential co-benefit of the SCR technology for reducing organic HAP emissions. Bench-scale experiments were performed using simulated coal combustion flue gases under a broad range of SCR reaction conditions. C6H6 was added at 1 or 17 ppm into the flue gas mixtures with different concentrations of sulfur dioxide (SO2), nitrogen oxide (NO), hydrogen chloride (HCl), and ammonia (NH3) to simulate the combustion of bituminous and sub-bituminous coals. The destruction of the C6H6 across the catalyst was measured by a total hydrocarbon analyzer and a resonance-enhanced multiphoton ionization time-of-flight mass spectrometer (REMPI-TOFMS) for the experiments with high (17 ppm) and low (1 ppm) concentrations of C6H6, respectively. The operating parameters of the SCR process, including the space velocity, temperature, and concentration of C6H6, were found to have a significant impact on the destruction of C6H6. The constituents of the flue gas had very little impact on the destruction, suggesting that the significant additional co-benefit of destruction of trace organic HAPs provided by the SCR process may be applicable to a wide variety of coals under different firing conditions. Destruction of C6H6 with high efficiencies is likely to occur concurrently with the reduction of NO during the SCR process without indication of carbon deposition on the catalyst. C1 [Lee, Chun Wai] US EPA, Natl Risk Management Res Lab, Res Triangle Pk, NC 27711 USA. [Zhao, Yongxin] ARCADIS US Inc, Durham, NC 27713 USA. [Lu, Shengyong] Zhejiang Univ, Inst Thermal Power Engn, State Key Lab Clean Energy Utilizat, Hangzhou 310027, Zhejiang, Peoples R China. [Stevens, William R.] Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37830 USA. [Zhao, Yongxin] Albemarle Corp, Baton Rouge, LA 70805 USA. [Stevens, William R.] Kentucky Christian Univ, Coll Hlth Sci, Grayson, KY 41143 USA. RP Lee, CW (reprint author), US EPA, Natl Risk Management Res Lab, Res Triangle Pk, NC 27711 USA. EM lee.chun-wai@epa.gov FU Ministry of Education of China through the Program of Introducing Talents of Discipline to University [B08026] FX Jeremy Lecomte (Universite d'Orleans, Orleans, France, student intern at the U.S. EPA) provided support for the experimental testing and data analysis. The authors are thankful for the support provided to one of the authors (Shengyong Lu) by the Ministry of Education of China through the Program of Introducing Talents of Discipline to University (B08026). NR 24 TC 0 Z9 0 U1 8 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0887-0624 EI 1520-5029 J9 ENERG FUEL JI Energy Fuels PD MAR PY 2016 VL 30 IS 3 BP 2240 EP 2247 DI 10.1021/acs.energyfuels.5b02058 PG 8 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DH1RO UT WOS:000372562800080 ER PT J AU Moreland, K AF Moreland, Kenneth TI The Tensions of In Situ Visualization SO IEEE COMPUTER GRAPHICS AND APPLICATIONS LA English DT Editorial Material C1 [Moreland, Kenneth] Sandia Natl Labs, Livermore, CA 94550 USA. RP Moreland, K (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA. EM kmorel@sandia.gov NR 11 TC 2 Z9 2 U1 3 U2 4 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 0272-1716 EI 1558-1756 J9 IEEE COMPUT GRAPH JI IEEE Comput. Graph. Appl. PD MAR-APR PY 2016 VL 36 IS 2 BP 5 EP 9 PG 5 WC Computer Science, Software Engineering SC Computer Science GA DH1NA UT WOS:000372550200002 PM 26960023 ER PT J AU Wejnert, C Hess, KL Rose, CE Balaji, A Smith, JC Paz-Bailey, G AF Wejnert, Cyprian Hess, Kristen L. Rose, Charles E. Balaji, Alexandra Smith, Justin C. Paz-Bailey, Gabriela CA NHBS Study Grp TI Age-Specific Race and Ethnicity Disparities in HIV Infection and Awareness Among Men Who Have Sex With Men-20 US Cities, 2008-2014 SO JOURNAL OF INFECTIOUS DISEASES LA English DT Article DE HIV; MSM; health disparities; black MSM ID BEHAVIORAL SURVEILLANCE SYSTEM; YOUNG BLACK-MEN; WHITE MEN; UNITED-STATES; RISK; PREVENTION; ATLANTA; METAANALYSIS; PREVALENCE; GA AB Background. Over half of human immunodeficiency virus (HIV) infections in the United States occur among men who have sex with men (MSM). Among MSM, 16% of estimated new infections in 2010 occurred among black MSM <25 years old. Methodology. We analyzed National HIV Behavioral Surveillance data on MSM from 20 cities. Poisson models were used to test racial disparities, by age, in HIV prevalence, HIV awareness, and sex behaviors among MSM in 2014. Data from 2008, 2011, and 2014 were used to examine how racial/ethnic disparities changed across time. Results. While black MSM did not report greater sexual risk than other MSM, they were most likely to be infected with HIV and least likely to know it. Among black MSM aged 18-24 years tested in 2014, 26% were HIV positive. Among white MSM aged 18-24 years tested in 2014, 3% were HIV positive. The disparity in HIV prevalence between black and white MSM increased from 2008 to 2014, especially among young MSM. Conclusions. Disparities in HIV prevalence between black and white MSM continue to increase. Black MSM may be infected with HIV at younger ages than other MSM and may benefit from prevention efforts that address the needs of younger men. C1 [Wejnert, Cyprian; Rose, Charles E.; Balaji, Alexandra; Paz-Bailey, Gabriela] Ctr Dis Control & Prevent, Natl Ctr HIV Viral Hepatitis STD & TB Prevent, Div HIV AIDS Prevent, Atlanta, GA USA. [Hess, Kristen L.; Smith, Justin C.] Oak Ridge Inst Sci & Educ, Atlanta, GA USA. RP Wejnert, C (reprint author), 1600 Clifton Rd NE,MS E 46, Atlanta, GA 30329 USA. EM cwejnert@cdc.gov NR 28 TC 2 Z9 2 U1 1 U2 3 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 0022-1899 EI 1537-6613 J9 J INFECT DIS JI J. Infect. Dis. PD MAR 1 PY 2016 VL 213 IS 5 BP 776 EP 783 DI 10.1093/infdis/jiv500 PG 8 WC Immunology; Infectious Diseases; Microbiology SC Immunology; Infectious Diseases; Microbiology GA DG9XY UT WOS:000372438300014 PM 26486637 ER PT J AU Ouyang, GY Ray, PK Kramer, MJ Akinc, M AF Ouyang, Gaoyuan Ray, Pratik K. Kramer, Matthew J. Akinc, Mufit TI High-Temperature Oxidation of ZrB2-SiC-AlN Composites at 1600 degrees C SO JOURNAL OF THE AMERICAN CERAMIC SOCIETY LA English DT Article ID DIBORIDE-SILICON CARBIDE; ZIRCONIUM DIBORIDE; SINTERING AID; CERAMICS; ZRB2; 1500-DEGREES-C; POWDERS; OXYGEN; ALN AB The effect of AlN substitution on oxidation of ZrB2-SiC was evaluated at 1600 degrees C up to 5 h. Replacement of ZrB2 by AlN, with 30 vol% SiC resulted in improved oxidation resistance with a thinner scale and reduced oxygen affected area. On the other hand, substitution of AlN for SiC resulted in a deterioration of the oxidation resistance with an abnormal scale and significant recession. The effect of SiC content was also studied, and was found to be consistent with the literature for the composites without AlN additions. A similar effect was observed when AlN was added, with the higher SiC content materials showing improved oxidation resistance. X-ray photoelectron spectroscopy showed the presence of Al2O3 and SiO2 on the surface, which could possibly lead to a modification in the viscosity of the glassy oxide scale. Possibly, the oxidation behavior of ZrB2-SiC composites can be improved with controlled AlN additions by adjusting the Al:Si ratios. C1 [Ouyang, Gaoyuan; Ray, Pratik K.; Kramer, Matthew J.; Akinc, Mufit] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA USA. [Ouyang, Gaoyuan; Ray, Pratik K.; Kramer, Matthew J.; Akinc, Mufit] Ames Lab, Div Mat Sci & Engn, Ames, IA USA. RP Akinc, M (reprint author), Iowa State Univ, Dept Mat Sci & Engn, Ames, IA USA.; Akinc, M (reprint author), Ames Lab, Div Mat Sci & Engn, Ames, IA USA. EM makinc@iastate.edu RI Ray, Pratik/C-5383-2008 OI Ray, Pratik/0000-0002-0656-4566 FU AFOSRHTAM [FA9550-11-1-201] FX This work was supported by the AFOSRHTAM under contract # FA9550-11-1-201. The authors greatly acknowledge the support from this project. The authors thank Eric Neuman and Prof. William G. Fahrenholtz for their assistance regarding the pressureless sintering of ZrB2-SiC. The authors also thank Warren Straszheim for his help in the EDS mapping analyses and Jim Anderegg for the XPS analyses. NR 30 TC 2 Z9 2 U1 5 U2 13 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0002-7820 EI 1551-2916 J9 J AM CERAM SOC JI J. Am. Ceram. Soc. PD MAR PY 2016 VL 99 IS 3 BP 808 EP 813 DI 10.1111/jace.14039 PG 6 WC Materials Science, Ceramics SC Materials Science GA DG6JB UT WOS:000372189300012 ER PT J AU Meier, W Meyer, KE Sava Gallis, DF Blea-Kirby, MA Roth, J Felman, D Breuer, T Dension, GJ Zutavern, FJ Huebner, W Brennecka, GL AF Meier, William Meyer, Kelsey Elizabeth Sava Gallis, Dorina F. Blea-Kirby, Mia Angelica Roth, Joshua Felman, Daniel Breuer, Tim Dension, Gary J. Zutavern, Fred J. Huebner, Wayne Brennecka, Geoff L. TI Highly Textured BaTiO3 via Templated Grain Growth and Resulting Polarization Reversal Dynamics SO JOURNAL OF THE AMERICAN CERAMIC SOCIETY LA English DT Article ID 180-DEGREES DOMAIN-WALLS; LEAD-FREE PIEZOCERAMICS; BARIUM-TITANATE; SINGLE-CRYSTALS; SWITCHING TIME; ELECTROMECHANICAL PROPERTIES; PIEZOELECTRIC CERAMICS; DEPENDENCE; NUCLEATION; THICKNESS AB Samples of bulk textured polycrystalline BaTiO3 ceramics were fabricated using a templated grain growth (TGG) approach in order to investigate effects of polycrystallinity and texture related to ferroelectric domain reversal under high-power drive conditions. Barium titanate platelets were formed via two-step topochemical conversion of bismuth titanate platelets grown via molten salt synthesis, then aligned via tape casting within a matrix of fine BaTiO3 powder. The coarse-grained parts showed a high degree of crystallographic texture after sintering. Combined with ceramics of similar density and polycrystallinity, but random orientation and commercial single-crystal specimens, this sample set enabled direct isolation of crystallographic texture and polycrystallinity as the primary variables for high-power polarization reversal studies. These studies have also demonstrated a link between grain size and polarization reversal time that strongly suggests that grain boundaries serve effectively as nucleation sites during the ferroelectric switching process. C1 [Meier, William] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Meyer, Kelsey Elizabeth] Univ Virginia, Dept Mech & Aerosp Engn, Charlottesville, VA 22904 USA. [Sava Gallis, Dorina F.; Blea-Kirby, Mia Angelica; Dension, Gary J.; Zutavern, Fred J.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Roth, Joshua] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Felman, Daniel] Oregon State Univ, Dept Mech Ind & Mfg Engn, Corvallis, OR 97331 USA. [Breuer, Tim] EaglePicher Technol, Joplin, MO 64802 USA. [Huebner, Wayne] Missouri S&T, Dept Mat Sci & Engn, Rolla, MO 65409 USA. [Brennecka, Geoff L.] Colorado Sch Mines, Dept Met & Mat Engn, Golden, CO 80401 USA. RP Brennecka, GL (reprint author), Colorado Sch Mines, Dept Met & Mat Engn, Golden, CO 80401 USA. EM gbrennec@mines.edu RI Sava Gallis, Dorina/D-2827-2015; Brennecka, Geoff/J-9367-2012 OI Brennecka, Geoff/0000-0002-4476-7655 FU Laboratory Directed Research and Development (LDRD) program at Sandia National Laboratories; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors express their gratitude to Harlan Brown-Shaklee (SNL), Tom Chavez (SNL), and Dr. Eric Bohannan (Missouri S&T) for technical assistance with some of the measurements associated with this work, as well as to Gary Pena and Dr. Steve Glover (both SNL) for technical assistance in support of the high power test bed.16 The SEM imaging and associated EDS and EBSD analysis on the sintered parts would not have been possible without the significant expertise and contributions of Bonnie McKenzie and Dr. Joe Michael (both SNL). A portion of this work was supported by the Laboratory Directed Research and Development (LDRD) program at Sandia National Laboratories. Sandia is a multiprogram laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. The authors also note that this work is largely the result of work done carried out by W. M., J. R. R., D. F., and T. B. during their capstone senior design course at Missouri S& T, in collaboration with SNL. NR 42 TC 1 Z9 1 U1 21 U2 38 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0002-7820 EI 1551-2916 J9 J AM CERAM SOC JI J. Am. Ceram. Soc. PD MAR PY 2016 VL 99 IS 3 BP 922 EP 929 DI 10.1111/jace.14048 PG 8 WC Materials Science, Ceramics SC Materials Science GA DG6JB UT WOS:000372189300029 ER PT J AU McMurray, JW AF McMurray, Jacob Wesley TI Thermodynamic Assessment of the Pr-O System SO JOURNAL OF THE AMERICAN CERAMIC SOCIETY LA English DT Article ID R(N)O(2N-2) HOMOLOGOUS SERIES; PRASEODYMIUM OXIDES; OXYGEN SYSTEM; ELECTRICAL-CONDUCTIVITY; SIMULATIONS; PRESSURE; ELEMENTS AB The Calphad method was used to perform a thermodynamic assessment of the Pr-O system. Compound energy formalism representations were developed for the fluorite -PrO2-x and bixbyite sigma-Pr3O5 +/- x solid solutions while the two-sublattice liquid model was used to describe the binary melt. The series of phases between Pr2O3 and PrO2 were taken to be stoichiometric. Equilibrium oxygen pressure, phase equilibria, and enthalpy data were used to optimize the adjustable parameters of the models for a self-consistent representation of the thermodynamic behavior of the Pr-O system from 298K to melting. C1 [McMurray, Jacob Wesley] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP McMurray, JW (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM mcmurrayjw1@ornl.gov OI McMurray, Jacob/0000-0001-5111-3054 FU US Department of Energy, Office of Nuclear Energy Fuel Cycle Technology Program; U.S. Department of Energy [DE-AC05-00OR22725] FX The author thanks Allen Haynes, Dongwon Shin, and Dane Wilson of the Oak Ridge National Laboratory for helpful comments. The work was supported by the US Department of Energy, Office of Nuclear Energy Fuel Cycle Technology Program. This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for the United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doepublic-access-plan). NR 32 TC 0 Z9 0 U1 2 U2 10 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0002-7820 EI 1551-2916 J9 J AM CERAM SOC JI J. Am. Ceram. Soc. PD MAR PY 2016 VL 99 IS 3 BP 1092 EP 1099 DI 10.1111/jace.14049 PG 8 WC Materials Science, Ceramics SC Materials Science GA DG6JB UT WOS:000372189300050 ER PT J AU Alexander, A Moody, NA Bandaru, PR AF Alexander, Anna Moody, Nathan A. Bandaru, Prabhakar R. TI Enhanced quantum efficiency of photoelectron emission, through surface textured metal electrodes SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A LA English DT Article AB It is predicted that the quantum efficiency (QE) of photoelectron emission from metals may be enhanced, possibly by an order of magnitude, through optimized surface texture. Through extensive computational simulations, it is shown that the absorption enhancement in select surface groove geometries may be a dominant contributor to enhanced QE and corresponds to localized Fabry-Perot resonances. The inadequacy of extant analytical models in predicting the QE increase, and suggestions for further improvement, are discussed. (C) 2015 American Vacuum Society. C1 [Alexander, Anna; Bandaru, Prabhakar R.] Univ Calif San Diego, Dept Mech Engn, Mat Sci Program, La Jolla, CA 92130 USA. [Moody, Nathan A.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Bandaru, PR (reprint author), Univ Calif San Diego, Dept Mech Engn, Mat Sci Program, La Jolla, CA 92130 USA. EM pbandaru@ucsd.edu FU LANL-UCSD initiative FX The authors are grateful for financial support from the LANL-UCSD initiative. The authors appreciate discussions with H. Yamada on the EM modeling. NR 20 TC 1 Z9 1 U1 2 U2 7 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 0734-2101 EI 1520-8559 J9 J VAC SCI TECHNOL A JI J. Vac. Sci. Technol. A PD MAR PY 2016 VL 34 IS 2 AR 021401 DI 10.1116/1.4936082 PG 5 WC Materials Science, Coatings & Films; Physics, Applied SC Materials Science; Physics GA DG8RW UT WOS:000372352300020 ER PT J AU Burton, MC Beebe, MR Yang, KD Lukaszew, RA Valente-Feliciano, AM Reece, C AF Burton, Matthew C. Beebe, Melissa R. Yang, Kaida Lukaszew, Rosa A. Valente-Feliciano, Anne-Marie Reece, Charles TI Superconducting NbTiN thin films for superconducting radio frequency accelerator cavity applications SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A LA English DT Article AB Current superconducting radio frequency technology, used in various particle accelerator facilities across the world, is reliant upon bulk niobium superconducting cavities. Due to technological advancements in the processing of bulk Nb cavities, the facilities have reached accelerating fields very close to a material-dependent limit, which is close to 50 MV/m for bulk Nb. One possible solution to improve upon this fundamental limitation was proposed a few years ago by Gurevich [Appl. Phys. Lett. 88, 012511 (2006)], consisting of the deposition of alternating thin layers of superconducting and insulating materials on the interior surface of the cavities. The use of type-II superconductors with Tc > Tc-Nb and H-c > Hc(Nb), (e.g., Nb3Sn, NbN, or NbTiN) could potentially greatly reduce the surface resistance (Rs) and enhance the accelerating field, if the onset of vortex penetration is increased above Hc(Nb), thus enabling higher field gradients. Although Nb3Sn may prove superior, it is not clear that it can be grown as a suitable thin film for the proposed multilayer approach, since very high temperature is typically required for its growth, hindering achieving smooth interfaces and/or surfaces. On the other hand, since NbTiN has a smaller lower critical field (H-c1) and higher critical temperature (T-c) than Nb and increased conductivity compared to NbN, it is a promising candidate material for this new scheme. Here, the authors present experimental results correlating film microstructure with superconducting properties on NbTiN thin film coupon samples while also comparing films grown with targets of different stoichiometry. It is worth mentioning that the authors have achieved thin films with bulk-like lattice parameter and transition temperature while also achieving H-c1 values larger than bulk for films thinner than their London penetration depths. (C) 2016 American Vacuum Society. C1 [Burton, Matthew C.; Beebe, Melissa R.; Yang, Kaida; Lukaszew, Rosa A.] Coll William & Mary, Dept Phys, Small Hall,300 Ukrop Way, Williamsburg, VA 23185 USA. [Valente-Feliciano, Anne-Marie; Reece, Charles] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. RP Burton, MC (reprint author), Coll William & Mary, Dept Phys, Small Hall,300 Ukrop Way, Williamsburg, VA 23185 USA. EM mcburton@email.wm.edu RI Yang, Kaida/K-7916-2012 OI Yang, Kaida/0000-0003-2018-2625 FU Defense Threat Reduction Agency [HDTRA1-10-1-0072] FX The authors would like to thank the SRF Institute at Jefferson Lab and acknowledge support from the Defense Threat Reduction Agency under Grant No. HDTRA1-10-1-0072. NR 11 TC 0 Z9 0 U1 8 U2 14 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 0734-2101 EI 1520-8559 J9 J VAC SCI TECHNOL A JI J. Vac. Sci. Technol. A PD MAR PY 2016 VL 34 IS 2 AR 021518 DI 10.1116/1.4941735 PG 6 WC Materials Science, Coatings & Films; Physics, Applied SC Materials Science; Physics GA DG8RW UT WOS:000372352300040 ER PT J AU Mamun, MAA Elmustafa, AA Hernandez-Garcia, C Mammei, R Poelker, M AF Mamun, Md Abdullah A. Elmustafa, Abdelmageed A. Hernandez-Garcia, Carlos Mammei, Russell Poelker, Matthew TI Effect of Sb thickness on the performance of bialkali-antimonide photocathodes SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A LA English DT Article ID FILMS; CRYSTALLIZATION; VACUUM AB The alkali species Cs and K were codeposited using an effusion source, onto relatively thick layers of Sb (50 nm to similar to 7 mu m) grown on GaAs and Ta substrates inside a vacuum chamber that was baked and not-vented, and also baked and vented with clean dry nitrogen but not rebaked. The characteristics of the Sb films, including sticking probability, surface roughness, grain size, and crystal properties were very different for these conditions, yet comparable values of photocathode yield [or quantum efficiency (QE)] at 284V were obtained following codeposition of the alkali materials. Photocathodes manufactured with comparatively thick Sb layers exhibited the highest QE and the best 1/e lifetime. The authors speculate that the alkali codeposition enabled optimized stoichiometry for photocathodes manufactured using thick Sb layers, which could serve as a reservoir for the alkali materials. (C) 2016 American Vacuum Society. C1 [Mamun, Md Abdullah A.; Elmustafa, Abdelmageed A.] Old Dominion Univ, Dept Mech & Aerosp Engn, Norfolk, VA 23529 USA. [Mamun, Md Abdullah A.; Elmustafa, Abdelmageed A.] Thomas Jefferson Natl Accelerator Facil, Appl Res Ctr, Newport News, VA 23606 USA. [Hernandez-Garcia, Carlos; Mammei, Russell; Poelker, Matthew] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. RP Mamun, MAA (reprint author), Old Dominion Univ, Dept Mech & Aerosp Engn, Norfolk, VA 23529 USA. EM mmamu001@odu.edu FU U.S. Department of Energy, Division of Material Sciences [DE-FG02-97ER45625]; National Science Foundation [DMR-0420304] FX This material is based on work supported by the U.S. Department of Energy, Division of Material Sciences, under Grant No. DE-FG02-97ER45625, and the National Science Foundation Grant No. DMR-0420304. The authors thank Kai Zhang of ODU and the College of William & Mary for the use of FESEM to obtain the microscopic images. NR 53 TC 3 Z9 3 U1 6 U2 14 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 0734-2101 EI 1520-8559 J9 J VAC SCI TECHNOL A JI J. Vac. Sci. Technol. A PD MAR PY 2016 VL 34 IS 2 AR 021509 DI 10.1116/1.4939563 PG 14 WC Materials Science, Coatings & Films; Physics, Applied SC Materials Science; Physics GA DG8RW UT WOS:000372352300031 ER PT J AU Peshek, TJ Burst, JM Coutts, TJ Gessert, TA AF Peshek, Timothy J. Burst, James M. Coutts, Timothy J. Gessert, Timothy A. TI Zero added oxygen for high quality sputtered ITO: A data science investigation of reduced Sn-content and added Zr SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A LA English DT Article ID IN2O3 THIN-FILMS; PULSED-LASER DEPOSITION; DOPED INDIUM OXIDE; TRANSPARENT CONDUCTING OXIDE; LIGHT-EMITTING-DIODES; HIGH-MOBILITY; ELECTRICAL-PROPERTIES; ROOM-TEMPERATURE; ATMOSPHERE AB The authors demonstrate mobilities of >45 cm(2)/V s for sputtered tin-doped indium oxide (ITO) films at zero added oxygen. All films were deposited with 5 wt. % SnO2, instead of the more conventional 8-10 wt. %, and had varying ZrO2 content from 0 to 3 wt. %, with a subsequent reduction in In2O3 content. These films were deposited by radio-frequency magnetron sputtering from nominally stoichiometric targets with varying oxygen partial pressure in the sputter ambient. Anomalous behavior was discovered for films with no Zr-added, where a bimodality of high and low mobilities was discovered for nominally similar growth conditions. However, all films showed the lowest resistivity and highest mobilities when the oxygen partial pressure in the sputter ambient was zero. This result is contrasted with several other reports of ITO transport performance having a maximum for small but nonzero oxygen partial pressure. This result is attributed to the reduced concentration of SnO2. The addition of ZrO2 yielded the highest mobilities at >55 cm(2)/V s and the films showed a modest increase in optical transmission with increasing Zr-content. (C) 2016 American Vacuum Society. C1 [Peshek, Timothy J.] Arizona State Univ, Sch Engn Matter Transport & Energy, Tempe, AZ 85287 USA. [Peshek, Timothy J.; Burst, James M.; Coutts, Timothy J.; Gessert, Timothy A.] Natl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USA. [Peshek, Timothy J.] Case Western Reserve Univ, Dept Mat Sci & Engn, Cleveland, OH 44106 USA. RP Gessert, TA (reprint author), Natl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USA. EM tjp3@case.edu FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory FX The authors would like to thank Yifan Xu for helpful discussions of data analytics. This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. NR 36 TC 0 Z9 0 U1 3 U2 11 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 0734-2101 EI 1520-8559 J9 J VAC SCI TECHNOL A JI J. Vac. Sci. Technol. A PD MAR PY 2016 VL 34 IS 2 AR 021201 DI 10.1116/1.4939830 PG 10 WC Materials Science, Coatings & Films; Physics, Applied SC Materials Science; Physics GA DG8RW UT WOS:000372352300013 ER PT J AU Biner, SB AF Biner, S. B. TI Pore and grain boundary migration under a temperature gradient: a phase-field model study SO MODELLING AND SIMULATION IN MATERIALS SCIENCE AND ENGINEERING LA English DT Article DE phase-field model; pore and grain boundary migration; temperature gradient ID MICROSTRUCTURE DEVELOPMENT; 2 DIMENSIONS; GROWTH; SIMULATION; DRAG; EQUATIONS AB The collective migration behavior of pores and grain boundaries under a temperature gradient is studied for simple single crystal, bi-crystal and polycrystal configurations with a phase-field model formulism. For simulation of the microstructure of solids, composed of pores and grain boundaries, the results indicate that not only the volume fraction of pores, but also its spatial partitioning between the grain boundary junctions and the grain boundary segments appears to be important. In addition to various physical properties, the evolution kinetics, under given temperature gradients, will be strongly influenced with the initial morphology of a poly-crystalline microstructure. C1 [Biner, S. B.] Idaho Natl Lab, Fuel Modeling & Simulat, Idaho Falls, ID 83415 USA. RP Biner, SB (reprint author), Idaho Natl Lab, Fuel Modeling & Simulat, Idaho Falls, ID 83415 USA. EM bulent.biner@inl.gov FU DOE Nuclear Energy Advanced Modeling and Simulation program; US DOE [DE-AC07-05ID14517] FX This work was funded by DOE Nuclear Energy Advanced Modeling and Simulation program. This manuscript has been authored by Battelle Energy Alliance, LLC under Contract No. DE-AC07-05ID14517 with US DOE. The US government retains, and the publisher, by accepting the article for publication, acknowledges that the US government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for US government purposes. NR 24 TC 0 Z9 0 U1 5 U2 11 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0965-0393 EI 1361-651X J9 MODEL SIMUL MATER SC JI Model. Simul. Mater. Sci. Eng. PD MAR PY 2016 VL 24 IS 3 AR 035019 DI 10.1088/0965-0393/24/3/035019 PG 10 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA DG8QD UT WOS:000372347800019 ER PT J AU Kumar, A Nguyen, L DeGraef, M Sundararaghavan, V AF Kumar, A. Nguyen, L. DeGraef, M. Sundararaghavan, V. TI A Markov random field approach for microstructure synthesis SO MODELLING AND SIMULATION IN MATERIALS SCIENCE AND ENGINEERING LA English DT Article DE reconstruction; microstructure; finite element analysis; simulation; probability ID POLYCRYSTALS; DEFORMATION; ALUMINUM AB We test the notion that many microstructures have an underlying stationary probability distribution. The stationary probability distribution is ubiquitous: we know that different windows taken from a polycrystalline microstructure are generally 'statistically similar'. To enable computation of such a probability distribution, microstructures are represented in the form of undirected probabilistic graphs called Markov Random Fields (MRFs). In the model, pixels take up integer or vector states and interact with multiple neighbors over a window. Using this lattice structure, algorithms are developed to sample the conditional probability density for the state of each pixel given the known states of its neighboring pixels. The sampling is performed using reference experimental images. 2D microstructures are artificially synthesized using the sampled probabilities. Statistical features such as grain size distribution and autocorrelation functions closely match with those of the experimental images. The mechanical properties of the synthesized microstructures were computed using the finite element method and were also found to match the experimental values. C1 [Sundararaghavan, V.] Univ Michigan, Aerosp Engn, Ann Arbor, MI 48109 USA. [Kumar, A.] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Nguyen, L.; DeGraef, M.] Carnegie Mellon Univ, Mat Sci & Engn, Pittsburgh, PA 15213 USA. RP Kumar, A (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN USA. EM veeras@umich.edu FU Air Force Office of Scientific Research (AFOSR) [FA9550-12-1-0475, FA9550-12-1-0458] FX The work presented here was funded by Air Force Office of Scientific Research (AFOSR) grant number FA9550-12-1-0475 and FA9550-12-1-0458 NR 34 TC 2 Z9 2 U1 2 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0965-0393 EI 1361-651X J9 MODEL SIMUL MATER SC JI Model. Simul. Mater. Sci. Eng. PD MAR PY 2016 VL 24 IS 3 AR 035015 DI 10.1088/0965-0393/24/3/035015 PG 13 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA DG8QD UT WOS:000372347800015 ER PT J AU O'Connor, DT Welland, MJ Liu, WK Voorhees, PW AF O'Connor, Devin T. Welland, Michael J. Liu, Wing Kam Voorhees, Peter W. TI Phase transformation and fracture in single LixFePO4 cathode particles: a phase-field approach to Li-ion intercalation and fracture SO MODELLING AND SIMULATION IN MATERIALS SCIENCE AND ENGINEERING LA English DT Article DE phase-field; fracture; chemo-mechanics; Bulter-Volmer Kinetics; Li-ion batteries ID ENERGY-LOSS SPECTROSCOPY; LIFEPO4 NANOPARTICLES; ELECTRODE PARTICLES; BATTERY ELECTRODES; CRACK-PROPAGATION; STRESS GENERATION; COHERENCY STRAIN; MODEL; DIFFUSION; INSTABILITY AB Modern Li-ion batteries with LiFePO4 cathodes have been shown to be low cost, non-toxic, have a high theoretical capacity, and high (dis) charging rates. Although LiFePO4 has advantageous properties for electrical energy storage, it can lose some of its charging capacity when cycled. Researchers have found cracks that develop in LiFePO4 cathode particles during cycling, and it has been suggested that this is the main cause of the capacity loss. The work presented here develops a multi-physics computational model to investigate the possible causes of fracture in single LiFePO4 particles. The model combines the recently developed reaction-limited phase-field model for Li-ion intercalation with the phase-field model for brittle fracture. We use our numerical model to simulate single LiFePO4 cathode particles during galvanostatic discharging as well as under no charging. It was found that because of the phase transformation and two-phase coexistence of LiFePO4, cracks were able to grow due to large stresses at coherent phase boundaries. Phase nucleation at particle side facets was also examined and we show that pre-cracks grow that follow the high stresses at the coherent interface during charging. C1 [O'Connor, Devin T.; Liu, Wing Kam] Northwestern Univ, Dept Mech Engn, Evanston, IL 60208 USA. [Welland, Michael J.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Voorhees, Peter W.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [O'Connor, Devin T.] Exponent Failure Anal Associates, 2595 Canyon Blvd Suite 440, Boulder, CO 80302 USA. RP O'Connor, DT (reprint author), Northwestern Univ, Dept Mech Engn, Evanston, IL 60208 USA.; O'Connor, DT (reprint author), Exponent Failure Anal Associates, 2595 Canyon Blvd Suite 440, Boulder, CO 80302 USA. EM devin.t.oconnor@gmail.com RI Voorhees, Peter /B-6700-2009; Liu, Wing/B-7599-2009 FU National Physical Sciences Consortium; Argonne National Laboratory; Department of Energy, Office of Science, Division of Materials Science and Engineering FX We gratefully acknowledge the computing resources provided on Blues, a high-performance computing cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory. DT O'Connor would like acknowledge the National Physical Sciences Consortium and Argonne National Laboratory for their partial support. Part of the work at Argonne by M J Welland was funded by the Department of Energy, Office of Science, Division of Materials Science and Engineering. NR 51 TC 2 Z9 2 U1 6 U2 15 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0965-0393 EI 1361-651X J9 MODEL SIMUL MATER SC JI Model. Simul. Mater. Sci. Eng. PD MAR PY 2016 VL 24 IS 3 AR 035020 DI 10.1088/0965-0393/24/3/035020 PG 17 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA DG8QD UT WOS:000372347800020 ER PT J AU Schultz, PA Snow, CS AF Schultz, Peter A. Snow, Clark S. TI Mechanical properties of metal dihydrides SO MODELLING AND SIMULATION IN MATERIALS SCIENCE AND ENGINEERING LA English DT Article DE metal hydrides; density functional theory; computational uncertainty; elastic constants; phase stability ID TOTAL-ENERGY CALCULATIONS; ELECTRONIC-STRUCTURE; AB-INITIO; DISLOCATION LOOP; ZIRCONIUM HYDRIDES; BLISTER FORMATION; BUBBLE EVOLUTION; 1ST PRINCIPLES; HELIUM RELEASE; TRANSITION AB First-principles calculations are used to characterize the bulk elastic properties of cubic and tetragonal phase metal dihydrides, MH2 {M = Sc, Y, Ti, Zr, Hf, lanthanides} to gain insight into the mechanical properties that govern the aging behavior of rare-earth di-tritides as the constituent H-3, tritium, decays into He-3. As tritium decays, helium is inserted in the lattice, the helium migrates and collects into bubbles, that then can ultimately create sufficient internal pressure to rupture the material. The elastic properties of the materials are needed to construct effective mesoscale models of the process of bubble growth and fracture. Dihydrides of the scandium column and most of the rare-earths crystalize into a cubic phase, while dihydrides from the next column, Ti, Zr, and Hf, distort instead into the tetragonal phase, indicating incipient instabilities in the phase and potentially significant changes in elastic properties. We report the computed elastic properties of these dihydrides, and also investigate the off-stoichiometric phases as He or vacancies accumulate. As helium builds up in the cubic phase, the shear moduli greatly soften, converting to the tetragonal phase. Conversely, the tetragonal phases convert very quickly to cubic with the removal of H from the lattice, while the cubic phases show little change with removal of H. The source and magnitude of the numerical and physical uncertainties in the modeling are analyzed and quantified to establish the level of confidence that can be placed in the computational results, and this quantified confidence is used to justify using the results to augment and even supplant experimental measurements. C1 [Schultz, Peter A.] Sandia Natl Labs, Multiscale Sci Dept, POB 5800, Albuquerque, NM 87185 USA. [Snow, Clark S.] Sandia Natl Labs, Appl Sci & Technol Maturat Dept, POB 5800, Albuquerque, NM 87185 USA. RP Schultz, PA (reprint author), Sandia Natl Labs, Multiscale Sci Dept, POB 5800, Albuquerque, NM 87185 USA. EM paschul@sandia.gov FU United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 67 TC 0 Z9 0 U1 9 U2 14 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0965-0393 EI 1361-651X J9 MODEL SIMUL MATER SC JI Model. Simul. Mater. Sci. Eng. PD MAR PY 2016 VL 24 IS 3 AR 035005 DI 10.1088/0965-0393/24/3/035005 PG 23 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA DG8QD UT WOS:000372347800005 ER PT J AU Sokolov, A Aranson, IS AF Sokolov, Andrey Aranson, Igor S. TI Rapid expulsion of microswimmers by a vortical flow SO NATURE COMMUNICATIONS LA English DT Article ID SUSPENSIONS; BACTERIA; CHEMOTAXIS; TRANSPORT; SHEAR; MODEL AB Interactions of microswimmers with their fluid environment are exceptionally complex. Macroscopic shear flow alters swimming trajectories in a highly nontrivial way and results in dramatic reduction of viscosity and heterogeneous bacterial distributions. Here we report on experimental and theoretical studies of rapid expulsion of microswimmers, such as motile bacteria, by a vortical flow created by a rotating microparticle. We observe a formation of a macroscopic depletion area in a high-shear region, in the vicinity of a microparticle. The rapid migration of bacteria from the shear-rich area is caused by a vortical structure of the flow rather than intrinsic random fluctuations of bacteria orientations, in stark contrast to planar shear flow. Our mathematical model reveals that expulsion is a combined effect of motility and alignment by a vortical flow. Our findings offer a novel approach for manipulation of motile microorganisms and shed light on bacteria-flow interactions. C1 [Sokolov, Andrey; Aranson, Igor S.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Aranson, Igor S.] Northwestern Univ, Dept Engn Sci & Appl Math, 2145 Sheridan Rd, Evanston, IL 60202 USA. RP Sokolov, A; Aranson, IS (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA.; Aranson, IS (reprint author), Northwestern Univ, Dept Engn Sci & Appl Math, 2145 Sheridan Rd, Evanston, IL 60202 USA. EM sokolov@anl.gov; aronson@anl.gov FU US Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Science and Engineering Division; NIH [1R01GM104978-01] FX The research was supported by the US Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Science and Engineering Division (experiment), and by the NIH, grant 1R01GM104978-01 (analysis). NR 38 TC 2 Z9 2 U1 4 U2 13 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD MAR PY 2016 VL 7 AR 11114 DI 10.1038/ncomms11114 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH4DO UT WOS:000372735900001 PM 27005581 ER PT J AU Zlotnik, A Nagao, R Kiss, IZ Li, JS AF Zlotnik, Anatoly Nagao, Raphael Kiss, Istvan Z. Li, Jr-Shin TI Phase-selective entrainment of nonlinear oscillator ensembles SO NATURE COMMUNICATIONS LA English DT Article ID COUPLED OSCILLATORS; COMPLEX NETWORKS; SYNCHRONIZATION; MODEL; AMPLITUDE AB The ability to organize and finely manipulate the hierarchy and timing of dynamic processes is important for understanding and influencing brain functions, sleep and metabolic cycles, and many other natural phenomena. However, establishing spatiotemporal structures in biological oscillator ensembles is a challenging task that requires controlling large collections of complex nonlinear dynamical units. In this report, we present a method to design entrainment signals that create stable phase patterns in ensembles of heterogeneous nonlinear oscillators without using state feedback information. We demonstrate the approach using experiments with electrochemical reactions on multielectrode arrays, in which we selectively assign ensemble subgroups into spatiotemporal patterns with multiple phase clusters. The experimentally confirmed mechanism elucidates the connection between the phases and natural frequencies of a collection of dynamical elements, the spatial and temporal information that is encoded within this ensemble, and how external signals can be used to retrieve this information. C1 [Zlotnik, Anatoly] Los Alamos Natl Lab, Ctr Nonlinear Studies, MS B258, Los Alamos, NM 87545 USA. [Nagao, Raphael; Kiss, Istvan Z.] St Louis Univ, Dept Chem, 3501 Laclede Ave, St Louis, MO 63103 USA. [Li, Jr-Shin] Washington Univ, Dept Elect & Syst Engn, CB 1042,1 Brookings Dr, St Louis, MO 63130 USA. RP Li, JS (reprint author), Washington Univ, Dept Elect & Syst Engn, CB 1042,1 Brookings Dr, St Louis, MO 63130 USA. EM jsli@wustl.edu RI Nagao, Raphael/J-9148-2013; Kiss, Istvan/C-1801-2008 OI Nagao, Raphael/0000-0001-8400-9093; Kiss, Istvan/0000-0003-0993-3184 FU U.S. National Science Foundation [CMMI-1301148, CMMI-1462796, ECCS-1509342, CHE-1465013]; CNPq [229171/2013-3]; U.S. Department of Energy [DE-AC52-06NA25396] FX This work was supported by the U.S. National Science Foundation under the awards CMMI-1301148, CMMI-1462796, ECCS-1509342, and CHE-1465013, the CNPq Award 229171/2013-3, and the U.S. Department of Energy under contract DE-AC52-06NA25396. NR 47 TC 2 Z9 2 U1 2 U2 10 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD MAR PY 2016 VL 7 AR 10788 DI 10.1038/ncomms10788 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DG9MQ UT WOS:000372407500001 PM 26988313 ER PT J AU Cristini, A Meakin, C Hirschi, R Arnett, D Georgy, C Viallet, M AF Cristini, A. Meakin, C. Hirschi, R. Arnett, D. Georgy, C. Viallet, M. TI Linking 1D evolutionary to 3D hydrodynamical simulations of massive stars SO PHYSICA SCRIPTA LA English DT Article DE turbulence; stellar evolution; convection; convective boundary mixing; massive stars; carbon burning ID STELLAR TURBULENT CONVECTION; EQUATION-OF-STATE; WHITE-DWARFS; SHEAR-FREE; MODELS; INTERIORS; ENTRAINMENT; ROTATION; FLASH; CODE AB Stellar evolution models of massive stars are important for many areas of astrophysics, for example nucleosynthesis yields, supernova progenitor models and understanding physics under extreme conditions. Turbulence occurs in stars primarily due to nuclear burning at different mass coordinates within the star. The understanding and correct treatment of turbulence and turbulent mixing at convective boundaries in stellar models has been studied for decades but still lacks a definitive solution. This paper presents initial results of a study on convective boundary mixing (CBM) in massive stars. The 'stiffness' of a convective boundary can be quantified using the bulk Richardson number (Ri(B)), the ratio of the potential energy for restoration of the boundary to the kinetic energy of turbulent eddies. A 'stiff' boundary (Ri(B) similar to 10(4)) will suppress CBM, whereas in the opposite case a 'soft' boundary (Ri(B) similar to 10) will be more susceptible to CBM. One of the key results obtained so far is that lower convective boundaries (closer to the centre) of nuclear burning shells are 'stiffer' than the corresponding upper boundaries, implying limited CBM at lower shell boundaries. This is in agreement with 3D hydrodynamic simulations carried out by Meakin and Arnett (2007 Astrophys. J. 667 448-75). This result also has implications for new CBM prescriptions in massive stars as well as for nuclear burning flame front propagation in super-asymptotic giant branch stars and also the onset of novae. C1 [Cristini, A.; Hirschi, R.; Georgy, C.] Keele Univ, Astrophys Grp, Lennard Jones Labs, Keele ST5 5BG, Staffs, England. [Meakin, C.; Arnett, D.] Univ Arizona, Dept Astron, Tucson, AZ 85721 USA. [Meakin, C.] New Mexico Consortium, Los Alamos, NM 87544 USA. [Meakin, C.] Los Alamos Natl Lab, Div Theoret, POB 1663, Los Alamos, NM 87545 USA. [Hirschi, R.] Univ Tokyo, WPI, Kavli IPMU, Kashiwa, Chiba 2778583, Japan. [Georgy, C.] Univ Geneva, Observ Geneva, CH-1290 Versoix, Switzerland. [Viallet, M.] Max Planck Inst Astrophys, Karl Schwarzschild Str 1, D-85741 Garching, Germany. RP Cristini, A (reprint author), Keele Univ, Astrophys Grp, Lennard Jones Labs, Keele ST5 5BG, Staffs, England. EM a.j.cristini@keele.ac.uk FU EU [306901]; World Premier International Research Center Initiative (WPI Initiative); MEXT, Japan; National Science Foundation [OCI-1053575]; NSF grant at University of Arizona [1107445]; European Research Council through grant [341157-COCO2CASA]; BIS National E-infrastructure capital grant [ST/K00042X/1]; STFC capital [ST/H008519/1, ST/K00087X/1]; STFC DiRAC Operations grant [ST/K003267/1]; Durham University FX The authors acknowledge support from EU-FP7-ERC-2012-St Grant 306901. RH acknowledges support from the World Premier International Research Center Initiative (WPI Initiative), MEXT, Japan. This work used the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by National Science Foundation grant number OCI-1053575. CM and WDA acknowledge support from NSF grant 1107445 at the University of Arizona. MV acknowledges support from the European Research Council through grant ERC-AdG No. 341157-COCO2CASA. This work used the DiRAC Data Centric system at Durham University, operated by the Institute for Computational Cosmology on behalf of the STFC DiRAC HPC Facility (www.dirac.ac.uk. This equipment was funded by BIS National E-infrastructure capital grant ST/K00042X/1, STFC capital grants ST/H008519/1 and ST/K00087X/1, STFC DiRAC Operations grant ST/K003267/1 and Durham University. DiRAC is part of the National E-Infrastructure. AC acknowledges Clare Carson, Matteo Millington, Josef Dymnicki and Aaron Wainwright for their support in the production of this work. NR 51 TC 3 Z9 3 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0031-8949 EI 1402-4896 J9 PHYS SCRIPTA JI Phys. Scr. PD MAR PY 2016 VL 91 IS 3 AR 034006 DI 10.1088/0031-8949/91/3/034006 PG 12 WC Physics, Multidisciplinary SC Physics GA DH0IF UT WOS:000372466700017 ER PT J AU Ward, D Waddington, JC Svensson, CE AF Ward, D. Waddington, J. C. Svensson, C. E. TI Inspirations from the theories of Bohr and Mottelson: a Canadian perspective SO PHYSICA SCRIPTA LA English DT Article DE nuclear structure; collective excitations; high angular momentum ID FUSION-EVAPORATION REACTIONS; SUPERDEFORMED ROTATIONAL BANDS; EVEN-EVEN NUCLEI; HIGH-SPIN STATES; SHELL-MODEL; RESPONSE CHARACTERISTICS; DEFORMED-NUCLEI; COULOMB-EXCITATION; VIBRATIONAL-STATES; QUADRUPOLE-MOMENT AB The theories developed by Bohr and Mottelson have inspired much of the world-wide experimental investigation into the structure of the atomic nucleus. On the occasion of the 40th anniversary of the awarding of their Nobel prize, we reflect on some of the experimental developments made in understanding the structure of nuclei. We have chosen to focus on experiments performed in Canada, or having strong ties to Canada, and the work included here spans virtually the whole of the second half of the 20th century. The 8 pi Spectrometer, which figures prominently in this story, was a novel departure for funding science in Canada that involved an intimate collaboration between a Crown Corporation (Atomic Energy of Canada Ltd) and University research, and enabled many of the insights discussed here. C1 [Waddington, J. C.] McMaster Univ, Dept Phys & Astron, Hamilton, ON L8S 4M1, Canada. [Svensson, C. E.] Univ Guelph, Dept Phys, Guelph, ON N1G 2W1, Canada. [Ward, D.] AECL Res, Chalk River Labs, Chalk River, ON K0J 1J0, Canada. [Ward, D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Svensson, CE (reprint author), Univ Guelph, Dept Phys, Guelph, ON N1G 2W1, Canada. EM sven@uoguelph.ca FU Natural Sciences and Engineering Research Council of Canada (NSERC); Canada Research Chairs program FX The authors would like to thank D J Hinde, T L Khoo, A O Macchiavelli, and J Simpson for helpful discussions. This work has been partially supported by the Natural Sciences and Engineering Research Council of Canada (NSERC) and the Canada Research Chairs program. NR 123 TC 2 Z9 2 U1 2 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0031-8949 EI 1402-4896 J9 PHYS SCRIPTA JI Phys. Scr. PD MAR PY 2016 VL 91 IS 3 AR 033002 DI 10.1088/0031-8949/91/3/033002 PG 22 WC Physics, Multidisciplinary SC Physics GA DH0IF UT WOS:000372466700003 ER PT J AU Claudio, T Stein, N Petermann, N Stroppa, DG Koza, MM Wiggers, H Klobes, B Schierning, G Hermann, RP AF Claudio, Tania Stein, Niklas Petermann, Nils Stroppa, Daniel G. Koza, Michael Marek Wiggers, Hartmut Klobes, Benedikt Schierning, Gabi Hermann, Raphael P. TI Lattice dynamics and thermoelectric properties of nanocrystalline silicon-germanium alloys SO PHYSICA STATUS SOLIDI A-APPLICATIONS AND MATERIALS SCIENCE LA English DT Article DE inelastic neutron scattering; lattice dynamics; phosphorus doping; Si-Ge alloys; specific heat; thermoelectric transport ID QUANTUM-WELL STRUCTURES; COMPUTER-SIMULATION; BULK SILICON; PHONONS; FIGURE; MERIT; PRESSURE AB The lattice dynamics and thermoelectric properties of sintered phosphorus-doped nanostructured silicon-germanium alloys obtained by gas-phase synthesis were studied. Measurements of the density of phonon states by inelastic neutron scattering were combined with measurements of the elastic constants and the low-temperature heat capacity. A strong influence of nanostructuring and alloying on the lattice dynamics was observed. The thermoelectric transport properties of samples with different doping as well as samples sintered at different temperature were characterized between room temperature and 1000 degrees C. A peak figure of merit zT = 0.88 at 900 degrees C is observed and is comparatively insensitive to the aforementioned parameter variations. (C) 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim C1 [Claudio, Tania; Klobes, Benedikt; Hermann, Raphael P.] Forschungszentrum Julich, Julich Ctr Neutron Sci, D-52425 Julich, Germany. [Claudio, Tania; Klobes, Benedikt; Hermann, Raphael P.] Forschungszentrum Julich, Peter Grunberg Inst, JARA FIT, D-52425 Julich, Germany. [Claudio, Tania; Hermann, Raphael P.] Univ Liege, Fac Sci, B-4000 Liege, Belgium. [Stein, Niklas; Petermann, Nils; Wiggers, Hartmut; Schierning, Gabi] Univ Duisburg Essen, Fac Engn, D-47057 Duisburg, Germany. [Stein, Niklas; Petermann, Nils; Wiggers, Hartmut; Schierning, Gabi] Univ Duisburg Essen, Ctr Nanointegrat Duisburg Essen CENIDE, D-47057 Duisburg, Germany. [Stroppa, Daniel G.] Forschungszentrum Julich, Peter Grunberg Inst PGI 5, D-52425 Julich, Germany. [Koza, Michael Marek] Inst Laue Langevin, 71 Ave Martyrs, F-38000 Grenoble, France. [Hermann, Raphael P.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Hermann, RP (reprint author), Forschungszentrum Julich, Julich Ctr Neutron Sci, D-52425 Julich, Germany.; Hermann, RP (reprint author), Forschungszentrum Julich, Peter Grunberg Inst, JARA FIT, D-52425 Julich, Germany.; Hermann, RP (reprint author), Univ Liege, Fac Sci, B-4000 Liege, Belgium.; Hermann, RP (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM hermannrp@ornl.gov RI Hermann, Raphael/F-6257-2013 OI Hermann, Raphael/0000-0002-6138-5624 FU Helmholtz Gemeinschaft Deutscher Forschungszentren [VH NG-407]; German Science Foundation (DFG) within the priority program on nanoscaled thermoelectrics, SPP 1386; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division FX The Institute Laue-Langevin (ILL Grenoble, France) and the Advanced Photon Source (APS) at Argonne National Laboratory are acknowledged for neutron and synchrotron radiation beam time at IN6 and 6-ID-D, respectively. The Helmholtz Gemeinschaft Deutscher Forschungszentren is acknowledged for funding VH NG-407 "Lattice dynamics in emerging functional materials." Funding by the German Science Foundation (DFG) within the priority program on nanoscaled thermoelectrics, SPP 1386, is gratefully acknowledged. D. Meertens is kindly acknowledged for TEM sample preparation, D. Weber for scientific input, and K. Friese for input on XRD refinement, and T. Watkins for helpful discussions. This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 41 TC 0 Z9 0 U1 11 U2 23 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1862-6300 EI 1862-6319 J9 PHYS STATUS SOLIDI A JI Phys. Status Solidi A-Appl. Mat. PD MAR PY 2016 VL 213 IS 3 SI SI BP 515 EP 523 DI 10.1002/pssa.201532500 PG 9 WC Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Materials Science; Physics GA DH3XJ UT WOS:000372719800003 ER PT J AU Issenmann, D Eon, S Bracht, H Hettich, M Dekorsy, T Buth, G Steininger, R Baumbach, T Hansen, JL Larsen, AN Ager, JW Haller, EE Plech, A AF Issenmann, Daniel Eon, Soizic Bracht, Hartmut Hettich, Mike Dekorsy, Thomas Buth, Gernot Steininger, Ralph Baumbach, Tilo Hansen, John Lundsgaard Larsen, Arne Nylandsted Ager, Joel W., III Haller, Eugene E. Plech, Anton TI Ultrafast study of phonon transport in isotopically controlled semiconductor nanostructures SO PHYSICA STATUS SOLIDI A-APPLICATIONS AND MATERIALS SCIENCE LA English DT Article DE femtosecond spectroscopy; Ge; multilayers; Si; thermal conductivity; ultrafast X-ray scattering; zone folding ID THERMAL-CONDUCTIVITY; GAAS/ALAS SUPERLATTICES; ACOUSTIC PHONONS; HEAT-CONDUCTION; SCATTERING; LINE AB Isotopically modulated silicon and germanium multilayers are analyzed by means of femtosecond spectroscopy and pulsed X-ray scattering for determining thermal conductivity and phonon modes. Isotopic modulation decreases thermal conductivity stronger than expected from a band bending model in the coherent phonon transport regime, in particular for silicon. Femtosecond spectroscopy and X-ray scattering resolve zone folded vibration modes, which are located at the edge of the new, smaller Brillouin zone due to the multilayer periodicity. These modes can contribute to the reduction of thermal conductivity by Uniklapp processes within the zone-folded mini-bands. [GRAPHICS] Color-coded increase in ultrafast X-ray scattering in vicinity to the mini-zone boundary of a germanium multilayer. (C) 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim C1 [Issenmann, Daniel; Buth, Gernot; Steininger, Ralph; Baumbach, Tilo; Plech, Anton] Karlsruhe Inst Technol, Inst Photon Sci & Synchrotron Radiat ANKA, POB 3640, D-76021 Karlsruhe, Germany. [Eon, Soizic; Bracht, Hartmut] Univ Munster, Inst Mat Phys, Wilhelm Klemm Str 10, D-48149 Munster, Germany. [Hettich, Mike; Dekorsy, Thomas] Univ Konstanz, Ctr Appl Photon, Univ Str 10, D-78262 Constance, Germany. [Hettich, Mike; Dekorsy, Thomas] Univ Konstanz, Dept Phys, Univ Str 10, D-78262 Constance, Germany. [Baumbach, Tilo] Karlsruhe Inst Technol, Lab Applicat Synchrotron Radiat, POB 3640, D-76021 Karlsruhe, Germany. [Hansen, John Lundsgaard; Larsen, Arne Nylandsted] Univ Aarhus, Dept Phys & Astron, Ny Munkegade 120, DK-8000 Aarhus, Denmark. [Ager, Joel W., III; Haller, Eugene E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Plech, A (reprint author), Karlsruhe Inst Technol, Inst Photon Sci & Synchrotron Radiat ANKA, POB 3640, D-76021 Karlsruhe, Germany. EM anton.plech@kit.edu RI Plech, Anton/E-4895-2010; OI Plech, Anton/0000-0002-6290-9303; Dekorsy, Thomas/0000-0003-2257-2854 FU German Science Foundation DFG [SPP 1386]; German Science Foundation DFG within the Heisenberg fellowship of A. Plech and H. Bracht; German Science Foundation DFG Helmholtz-Association topic "Research with photons, ions and neutrons"; Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy [DE-AC02-05CH11231]; [SFB 767] FX This project is supported by German Science Foundation DFG under contract "Isotherm" within the priority program SPP 1386, within the Heisenberg fellowship of A. Plech and H. Bracht and within the Helmholtz-Association topic "Research with photons, ions and neutrons." We acknowledge beamtime and support by ESRF (beamline ID09b) and ANKA (beamlines SCD, SUL-X) and the Difflab at ANKA. Partial support by the SFB 767 is also acknowledged. We are grateful for profound help and support by N. Hiller, S. Ibrahimkutty, D. Khakhulin, N. Smale, S. Stankov, M. Wulff, and M. Zakharova. E. E. Haller and J. W. Ager were supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 46 TC 1 Z9 1 U1 2 U2 7 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1862-6300 EI 1862-6319 J9 PHYS STATUS SOLIDI A JI Phys. Status Solidi A-Appl. Mat. PD MAR PY 2016 VL 213 IS 3 SI SI BP 541 EP 548 DI 10.1002/pssa.201532462 PG 8 WC Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Materials Science; Physics GA DH3XJ UT WOS:000372719800006 ER PT J AU Bessas, D Winkler, M Sergueev, I Konig, JD Bottner, H Hermann, RP AF Bessas, D. Winkler, M. Sergueev, I. Koenig, J. D. Boettner, H. Hermann, R. P. TI Lattice dynamics in elemental modulated Sb2Te3 films SO PHYSICA STATUS SOLIDI A-APPLICATIONS AND MATERIALS SCIENCE LA English DT Article DE elemental modulated films; lattice dynamics; nuclear inelastic scattering; Sb2Te3; synchrotron radiation diffraction ID NUCLEAR; ABSORPTION; BI2TE3 AB The crystallinity and the lattice dynamics in elemental modulated Sb2Te3 films are investigated microscopically using high energy synchrotron radiation diffraction combined with Sb-121 nuclear inelastic scattering. The correlation length is found to be finite but less than 100 A. The element specific density of phonon states is extracted. A comparison with the element specific density of phonon states in bulk Sb2Te3 confirms that the main features in the density of phonon states arise from the layered structure. The average speed of sound at 40 K, 1.74(2)km s(-1), is almost the same compared to bulk Sb2Te3 at 20 K. 1.78(2)km s(-1). Similarly, the change in the acoustic cut-off energy is within the experimental detection limit. Thus, we suggest that the lattice thermal conductivity in elemental modulated Sb2Te3 films should not be significantly changed from its bulk value. (C) 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim C1 [Bessas, D.; Hermann, R. P.] Forschungszentrum Julich, JARA FIT, Julich Ctr Neutron Sci, D-52425 Julich, Germany. [Bessas, D.; Hermann, R. P.] Forschungszentrum Julich, JARA FIT, Peter Grunberg Inst PGI, D-52425 Julich, Germany. [Bessas, D.; Hermann, R. P.] Univ Liege, Fac Sci, B-4000 Liege, Belgium. [Winkler, M.; Koenig, J. D.; Boettner, H.] Fraunhofer Inst Phys Measurement Tech IPM, Heidenhofstr 8, D-79110 Freiburg, Germany. [Bessas, D.; Sergueev, I.] European Synchrotron Radiat Facil, BP 220, F-38043 Grenoble, France. [Hermann, R. P.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Sergueev, I.] DESY, D-22607 Hamburg, Germany. [Boettner, H.] Seilerweg 5, D-79108 Freiburg, Germany. RP Bessas, D (reprint author), Forschungszentrum Julich, JARA FIT, Julich Ctr Neutron Sci, D-52425 Julich, Germany.; Bessas, D (reprint author), Forschungszentrum Julich, JARA FIT, Peter Grunberg Inst PGI, D-52425 Julich, Germany.; Bessas, D (reprint author), Univ Liege, Fac Sci, B-4000 Liege, Belgium. EM bessas@esrf.fr RI Hermann, Raphael/F-6257-2013 OI Hermann, Raphael/0000-0002-6138-5624 FU DFG [SPP1386]; Helmholtz University Young Investigator Group "Lattice Dynamics in Emerging Functional Materials"; Materials Sciences and Engineering Division, Office of Basic Energy Sciences, US Department of Energy FX The DFG priority program SPP1386 "Nanostructured Thermoelectrics" and the Helmholtz University Young Investigator Group "Lattice Dynamics in Emerging Functional Materials" are acknowledged for the financial support of this study. RPH acknowledges support from the Materials Sciences and Engineering Division, Office of Basic Energy Sciences, US Department of Energy. RPH and DB acknowledge the European Synchrotron Radiation Facility and the Advanced Photon Source for provision of synchrotron radiation beam time and the helpful discussions with Dr. A. Chumakov and Dr. R. Ruffer at ID-18 and the help of Dr. D. Robinson during data acquisition at 6-ID-D, respectively. NR 26 TC 1 Z9 1 U1 6 U2 17 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1862-6300 EI 1862-6319 J9 PHYS STATUS SOLIDI A JI Phys. Status Solidi A-Appl. Mat. PD MAR PY 2016 VL 213 IS 3 SI SI BP 694 EP 698 DI 10.1002/pssa.201532431 PG 5 WC Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Materials Science; Physics GA DH3XJ UT WOS:000372719800021 ER PT J AU Peranio, N Eibl, O Bassler, S Nielsch, K Klobes, B Hermann, RP Daniel, M Albrecht, M Gorlitz, H Pacheco, V Bedoya-Martinez, N Hashibon, A Elsasser, C AF Peranio, N. Eibl, O. Bassler, S. Nielsch, K. Klobes, B. Hermann, R. P. Daniel, M. Albrecht, M. Goerlitz, H. Pacheco, V. Bedoya-Martinez, N. Hashibon, A. Elsaesser, C. TI From thermoelectric bulk to nanomaterials: Current progress for Bi2Te3 and CoSb3 SO PHYSICA STATUS SOLIDI A-APPLICATIONS AND MATERIALS SCIENCE LA English DT Article DE Bi2Te3; CoSb3; lattice dynamics; nanomaterials; point defects; thermoelectric effects; transmission electron microscopy ID SKUTTERUDITE THIN-FILMS; TEMPERATURE MBE DEPOSITION; PULSED-LASER DEPOSITION; STRUCTURAL-PROPERTIES; THERMAL-CONDUCTIVITY; BISMUTH TELLURIDE; LATTICE-DYNAMICS; SB2TE3; SUPERLATTICES; STABILITY AB Bi2Te3 and CoSb3 based nanomaterials were synthesized and their thermoelectric, structural, and vibrational properties analyzed to assess and reduce ZT-limiting mechanisms. The same preparation and/or characterization methods were applied in the different materials systems. Single-crystalline, ternary p-type Bi15Sb29Te56, and n-type Bi38Te55Se7 nanowires with power factors comparable to nanostructured bulk materials were prepared by potential-pulsed electrochemical deposition in a nanostructured Al2O3 matrix. p-type Sb2Te3, n-type Bi2Te3, and n-type CoSb3 thin films were grown at room temperature using molecular beam epitaxy and were subsequently annealed at elevated temperatures. This yielded polycrystalline, single phase thin films with optimized charge carrier densities. In CoSb3 thin films the speed of sound could be reduced by filling the cage structure with Yb and alloying with Fe yielded p-type material. Bi-2(Te0.91Se0.09)(3)/SiC and (Bi0.26Sb0.74)(2)Te-3/SiC nanocomposites with low thermal conductivities and ZT values larger than 1 were prepared by spark plasma sintering. Nanostructure, texture, chemical composition, as well as electronic and phononic excitations were investigated by X-ray diffraction, nuclear resonance scattering, inelastic neutron scattering, Mossbauer spectroscopy, and transmission electron microscopy. For Bi2Te3 materials, ab-initio calculations together with equilibrium and non-equilibrium molecular dynamics simulations for point defects yielded their formation energies and their effect on lattice thermal conductivity, respectively. [GRAPHICS] Current advances in thermoelectric Bi2Te3 and CoSb3 based nanomaterials are summarized. Advanced synthesis and characterization methods and theoretical modeling were combined to assess and reduce ZT-limiting mechanisms in these materials. (C) 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim C1 [Peranio, N.; Eibl, O.] Univ Tubingen, Inst Appl Phys, Morgenstelle 10, D-72076 Tubingen, Germany. [Bassler, S.; Nielsch, K.] Univ Hamburg, Inst Nanostruct & Solid State Phys, Jungiusstr 11, D-20355 Hamburg, Germany. [Nielsch, K.; Klobes, B.] Forschungszentrum Julich, Julich Ctr Neutron Sci, Leo Brandt Str 1, D-52425 Julich, Germany. [Klobes, B.; Hermann, R. P.] Forschungszentrum Julich, Peter Grunberg Inst, JARA FIT, Leo Brandt Str 1, D-52425 Julich, Germany. [Hermann, R. P.] Univ Liege, Fac Sci, B-4000 Liege, Belgium. [Hermann, R. P.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Daniel, M.; Albrecht, M.] Tech Univ Chemnitz, Inst Phys, Reichenhainer Str 70, D-09107 Chemnitz, Germany. [Albrecht, M.] Univ Augsburg, Inst Phys, Univ Str 1 Nord, D-86159 Augsburg, Germany. [Goerlitz, H.; Pacheco, V.] Fraunhofer Inst Mfg Technol & Adv Mat IFAM, Branch Lab Dresden, Winterbergstr 28, D-01277 Dresden, Germany. [Bedoya-Martinez, N.; Hashibon, A.; Elsaesser, C.] Fraunhofer Inst Werkstoffmech IWM, Wohlerstr 11, D-79108 Freiburg, Germany. RP Peranio, N (reprint author), Univ Tubingen, Inst Appl Phys, Morgenstelle 10, D-72076 Tubingen, Germany. EM nicola.peranio@uni-tuebingen.de; oliver.eibl@uni-tuebingen.de RI Bedoya Martinez, Natalia/G-8477-2016; Hermann, Raphael/F-6257-2013; Pacheco, Vicente/O-4062-2016; Nielsch, Kornelius/S-3196-2016 OI Bedoya Martinez, Natalia/0000-0001-9824-6129; Hermann, Raphael/0000-0002-6138-5624; FU German Research Foundation (DFG) [1386]; Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. Department of Energy; Ministry of Science, Research and the Arts Baden-Wurttemberg; DFG FX Financial support by the German Research Foundation (DFG) via the Priority Programme 1386 "Nanostructured Thermoelectric Materials: Theory, Model Systems and Controlled Synthesis" is gratefully acknowledged. R.P. Hermann acknowledges support from the Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. Department of Energy. N. Bedoya-Martinez acknowledges funding by the Ministry of Science, Research and the Arts Baden-Wurttemberg and DFG for calculations performed on the computational resource ForHLR Phase I. NR 74 TC 5 Z9 5 U1 34 U2 108 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1862-6300 EI 1862-6319 J9 PHYS STATUS SOLIDI A JI Phys. Status Solidi A-Appl. Mat. PD MAR PY 2016 VL 213 IS 3 SI SI BP 739 EP 749 DI 10.1002/pssa.201532614 PG 11 WC Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Materials Science; Physics GA DH3XJ UT WOS:000372719800026 ER PT J AU Sesselmann, A Klobes, B Dasgupta, T Gourdon, O Hermann, R Mueller, E AF Sesselmann, Andreas Klobes, Benedikt Dasgupta, Titas Gourdon, Olivier Hermann, Raphael Mueller, Eckhard TI Neutron diffraction and thermoelectric properties of indium filled InxCo4Sb12 (x=0.05, 0.2) and indium cerium filled Ce0.05In0.1Co4Sb12 skutterudites SO PHYSICA STATUS SOLIDI A-APPLICATIONS AND MATERIALS SCIENCE LA English DT Article DE neutron diffraction; Sb deficiency; skutterudites; thermoelectrics ID N-TYPE SKUTTERUDITES; CRYSTAL-STRUCTURE AB The thermoelectric properties on polycrystalline single (In) and double filled (Ce, In) skuttemdites are characterized between 300 and 700 K. Powder neutron diffraction measurements of the skutterudite compositions In,Co4Sb12 (x = 0.05, 0.2) and Ce0.05In0.1Ca4Sb12 as a function of temperature (12-300 K) were carried out, which gives more insight into the structural data of single and double-filled skutterudites. Results show that due to the annealing treatment, a Sb deficiency is detectable and thus verifies defects at the Sb lattice site of the skutterudite. Furthermore, we show by electron microprobe analysis that a considerable amount of indium is lost during synthesis and post-processing for the single indium filled samples, but not for the double cerium and indium skuttenidite sample. In our experiments, the double-filled skuttenidite is superior to the single-filled skutterudite composition due to a higher charge carrier density, a comparable lattice thermal resistivity, and a higher density of states effective mass. Furthermore, we obtained a significantly higher Einstein temperature for the double-filled skuttenidite composition in comparison to the single-filled species, which reflects the high sensitivity due to filling of the void lattice position within the skutterudite crystal. (C) 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim C1 [Sesselmann, Andreas; Mueller, Eckhard] German Aerosp Ctr DLR, Inst Mat Res, D-51147 Cologne, Germany. [Klobes, Benedikt; Hermann, Raphael] Forschungszentrum Julich, Julich Ctr Neutron Sci, D-52425 Julich, Germany. [Klobes, Benedikt; Hermann, Raphael] Forschungszentrum Julich, Peter Grunberg Inst, JARA FIT, D-52425 Julich, Germany. [Dasgupta, Titas] Indian Inst Technol, Dept Met Engn & Mat Sci, Bombay 400076, Maharashtra, India. [Gourdon, Olivier] Los Alamos Natl Lab, LANSCE, POB 1663, Los Alamos, NM 87545 USA. [Hermann, Raphael] Univ Liege, Fac Sci, B-4000 Liege, Belgium. [Hermann, Raphael] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Mueller, Eckhard] Univ Giessen, Inst Inorgan & Analyt Chem, Heinrich Buff Ring 58, D-35392 Giessen, Germany. RP Sesselmann, A (reprint author), German Aerosp Ctr DLR, Inst Mat Res, D-51147 Cologne, Germany. EM andreas.sesselmann@dlr.de RI Hermann, Raphael/F-6257-2013 OI Hermann, Raphael/0000-0002-6138-5624 FU Helmholtz Association of German [VH NG-407]; US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; DFG [SPP-1386] FX The Helmholtz Association of German research centers is acknowledged for funding VH NG-407 "Lattice dynamics in emerging functional materials." The Spallation Neutron Source is acknowledged for provision of neutron beam time at POWGEN under the JCNS access program. Work at Oak Ridge National Laboratory was supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. Support from the DFG priority program SPP-1386 "Nanostructured Thermoelectries" is gratefully acknowledged. We are also grateful to Dr. B. Chakoumakos for support in the diffraction data analysis and furthermore we thank G. Skomedal for performing the EPMA. Endnotes NR 40 TC 2 Z9 2 U1 1 U2 8 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1862-6300 EI 1862-6319 J9 PHYS STATUS SOLIDI A JI Phys. Status Solidi A-Appl. Mat. PD MAR PY 2016 VL 213 IS 3 SI SI BP 766 EP 773 DI 10.1002/pssa.201532589 PG 8 WC Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Materials Science; Physics GA DH3XJ UT WOS:000372719800029 ER PT J AU Kieslich, G Cerretti, G Veremchuk, I Hermann, RP Panthofer, M Grin, J Tremel, W AF Kieslich, Gregor Cerretti, Giacomo Veremchuk, Igor Hermann, Raphael P. Panthofer, Martin Grin, Juri Tremel, Wolfgang TI A chemists view: Metal oxides with adaptive structures for thermoelectric applications SO PHYSICA STATUS SOLIDI A-APPLICATIONS AND MATERIALS SCIENCE LA English DT Article DE crystallographic shear; Magneli phases; metal oxides; thermal conductivity; thermoelectrics ID DOPED ZNO CERAMICS; LOW THERMAL-CONDUCTIVITY; PERFORMANCE BULK THERMOELECTRICS; RESOLUTION ELECTRON-MICROSCOPY; REDUCED TUNGSTEN TRIOXIDE; CRYSTALLOGRAPHIC SHEAR; CRYSTAL-STRUCTURE; MAGNELI PHASES; X-RAY; TITANIUM-OXIDES AB Thermoelectric devices can help to tackle future challenges in the energy sector through the conversion of waste heat directly into usable electric energy. For a wide applicability low-cost materials with reasonable thermoelectric performances and cost-efficient preparation techniques are required. In this context metal oxides are an interesting class of materials because of their inherenthigh-temperature stability and relative high sustainability. Their thermoelectric performance, however, needs to be improved for wide application. Compounds with adaptive structures are a very interesting class of materials. A slight reduction of early transition metal oxides generates electrons as charge carriers and crystallographic shear planes as structure motif. The crystallographic shear planes lead to a reduction of intrinsic thermal conductivity. At the same time, the electronic transport properties can be tuned by the degree of reduction. So far only a few transition metal oxides with adaptive structures have been investigated with respect to their thermoelectric properties, leaving much room for improvement. This review gives an overview of thermoelectric oxides, highlights the structural aspects of the crystallographic shear planes and the resulting thermoelectric properties. (C) 2016 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim C1 [Kieslich, Gregor; Tremel, Wolfgang] Univ Cambridge, Funct Inorgan & Hybrid Mat Grp, Dept Mat Sci & Met, 27 Charles Babbage Rd, Cambridge CB3 0FS, England. [Cerretti, Giacomo; Panthofer, Martin; Tremel, Wolfgang] Johannes Gutenberg Univ Mainz, Inst Anorgan Chem & Analyt Chem, Duesbergweg 10-14, D-55099 Mainz, Germany. [Veremchuk, Igor; Grin, Juri] Max Planck Inst Chem Phys Fester Stoffe, D-01187 Dresden, Germany. [Hermann, Raphael P.] Forschungszentrum Julich, JARA FIT, JCNS, D-52425 Julich, Germany. [Hermann, Raphael P.] Forschungszentrum Julich, JARA FIT, PGI, D-52425 Julich, Germany. [Hermann, Raphael P.] Univ Liege, Fac Sci, B-4000 Liege, Belgium. [Hermann, Raphael P.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Tremel, W (reprint author), Univ Cambridge, Funct Inorgan & Hybrid Mat Grp, Dept Mat Sci & Met, 27 Charles Babbage Rd, Cambridge CB3 0FS, England.; Tremel, W (reprint author), Johannes Gutenberg Univ Mainz, Inst Anorgan Chem & Analyt Chem, Duesbergweg 10-14, D-55099 Mainz, Germany. EM tremel@uni-mainz.de RI Mainz, EMZ-M/E-3619-2016; Hermann, Raphael/F-6257-2013; Tremel, Wolfgang/D-8125-2011; Kieslich, Gregor/D-7443-2017 OI Hermann, Raphael/0000-0002-6138-5624; Tremel, Wolfgang/0000-0002-4536-994X; Kieslich, Gregor/0000-0003-2038-186X FU Deutsche Forschungsgemeinschaft [1386]; Konrad-Adenauer Stiftung FX This research was supported by the Deutsche Forschungsgemeinschaft within the priority programm 1386 Nanostructured Thermoelectrics. G.K. was supported by a fellowship from the Konrad-Adenauer Stiftung. NR 242 TC 1 Z9 1 U1 21 U2 63 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1862-6300 EI 1862-6319 J9 PHYS STATUS SOLIDI A JI Phys. Status Solidi A-Appl. Mat. PD MAR PY 2016 VL 213 IS 3 SI SI BP 808 EP 823 DI 10.1002/pssa.201532702 PG 16 WC Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Materials Science; Physics GA DH3XJ UT WOS:000372719800033 ER PT J AU Dippon, M Babiniec, SM Ding, HP Ricote, S Sullivan, NP AF Dippon, Michael Babiniec, Sean M. Ding, Hanping Ricote, Sandrine Sullivan, Neal P. TI Exploring electronic conduction through BaCexZr0.9-xY0.1O3-d proton-conducting ceramics SO SOLID STATE IONICS LA English DT Article DE Solid-solution barium cerate and; barium zirconate; Thin membrane; Electrolysis; Cerium reduction; Electronic leakage; Ceramic proton conductor ID SOLID OXIDE ELECTROLYZER; DOPED BARIUM CERATE; STEAM ELECTROLYSIS; FUEL-CELLS; CHEMICAL-STABILITY; TRANSPORT-PROPERTIES; BACE0.2ZR0.7Y0.1O3-DELTA AB This work explores the formation of undesirable electronic leakage in BaCe,Zr0.9 xYo.103 a (BCZY) proton conducting ceramic thin membranes used in H2O-electrolysis and hydrogen -pumping applications. Very low hydrogen fluxes (hydrogen transport number below 0.4) through thin BCZY membranes during electrolysis operation were recently reported. These poor performances were explained by the presence of an undesirable electronic leakage that forms due to reduction of cerium in the BCZY material. In this paper, we investigate the influence of the cerium content in the BCZY membranes on the magnitude of this electronic leakage. Three compositions were fabricated with x = 0, 0.1, and 0.2 (BZY10, BCZY18, and BCZY27, respectively). Unique gas conditions were chosen to isolate specific charge carriers present in the thin membranes, and decouple the electronic -conduction effects. While significant electronic leakage was observed in the BCZY27 material under these well-defined conditions, minimal leakage was detected in BCZY18 and BZY10. These results confirm that the presence of the electronic leakage is linked to the cerium content and is most probably due to the reduction of cerium ions under bias. Additionally, BCZY18 is the preferred composition for electrolysis applications due to its relative lack of electronic conductivity, reasonable protonic conductivity, and affinity for high -density sintering. (C) 2016 Elsevier B.V. All rights reserved. C1 [Dippon, Michael] Karlsruhe Inst Technol, Inst Mat Elect & Elect Engn, D-76021 Karlsruhe, Germany. [Babiniec, Sean M.; Ding, Hanping; Ricote, Sandrine; Sullivan, Neal P.] Colorado Sch Mines, Dept Mech Engn, Colorado Fuel Cell Ctr, Golden, CO 80401 USA. [Babiniec, Sean M.] Sandia Natl Labs, Mat Devices & Energy Technol, POB 5800, Albuquerque, NM 87185 USA. RP Sullivan, NP (reprint author), Colorado Sch Mines, Dept Mech Engn, Colorado Fuel Cell Ctr, Golden, CO 80401 USA. EM nsulliva@mines.edu RI Ding, Hanping/G-2029-2016 OI Ding, Hanping/0000-0002-8734-7933 FU Colorado School of Mines Foundation, Protonic Capital Funds FX The authors acknowledge the Colorado School of Mines Foundation, Protonic Capital Funds for support of this work. The authors would like to thank Dr. Grant Hudish and Steve Govorchin from CoorsTek for performing the ICP-OES measurements and Drs. W. Grover Coors and Anthony Manerbino from CoorsTek, Inc. (Golden, CO, USA) for insightful discussions. NR 43 TC 2 Z9 2 U1 15 U2 35 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-2738 EI 1872-7689 J9 SOLID STATE IONICS JI Solid State Ion. PD MAR PY 2016 VL 286 BP 117 EP 121 DI 10.1016/j.ssi.2016.01.029 PG 5 WC Chemistry, Physical; Physics, Condensed Matter SC Chemistry; Physics GA DG9FO UT WOS:000372388400018 ER PT J AU Weaver, BP Williams, BJ Anderson-Cook, CM Higdon, DM AF Weaver, Brian P. Williams, Brian J. Anderson-Cook, Christine M. Higdon, David M. TI Computational Enhancements to Bayesian Design of Experiments Using Gaussian Processes SO BAYESIAN ANALYSIS LA English DT Article DE Bayesian design of experiments; Gaussian processes; accelerated life tests; preposterior expectation; expected quantile improvement ID SEQUENTIAL MONTE-CARLO; COMPUTER EXPERIMENTS; GLOBAL OPTIMIZATION; RESOURCE-ALLOCATION; ALGORITHM; SYSTEMS; MODELS AB Bayesian design of experiments is a methodology for incorporating prior information into the design phase of an experiment. Unfortunately, the typical Bayesian approach to designing experiments is both numerically and analytically intractable without additional assumptions or approximations. In this paper, we discuss how Gaussian processes can be used to help alleviate the numerical issues associated with Bayesian design of experiments. We provide an example based on accelerated life tests and compare our results with large-sample methods. C1 [Weaver, Brian P.; Williams, Brian J.; Anderson-Cook, Christine M.; Higdon, David M.] Los Alamos Natl Lab, Stat Sci Grp, CCS 6, Los Alamos, NM 87545 USA. RP Weaver, BP (reprint author), Los Alamos Natl Lab, Stat Sci Grp, CCS 6, Los Alamos, NM 87545 USA. EM theguz@lanl.gov OI Williams, Brian/0000-0002-3465-4972 NR 30 TC 1 Z9 1 U1 3 U2 3 PU INT SOC BAYESIAN ANALYSIS PI PITTSBURGH PA CARNEGIE MELLON UNIV, DEPT STTISTICS, PITTSBURGH, PA 15213 USA SN 1931-6690 EI 1936-0975 J9 BAYESIAN ANAL JI Bayesian Anal. PD MAR PY 2016 VL 11 IS 1 BP 191 EP 213 DI 10.1214/15-BA945 PG 23 WC Mathematics, Interdisciplinary Applications; Statistics & Probability SC Mathematics GA DG4UM UT WOS:000372068400008 ER PT J AU He, J Du, SY Tan, XH Arefin, A Han, CS AF He, Jian Du, Shiyu Tan, Xiaohua Arefin, Ayesha Han, Cliff S. TI Improved lysis of single bacterial cells by a modified alkaline-thermal shock procedure SO BIOTECHNIQUES LA English DT Article DE cell lysis; single-cell genomics; genome recovery; unculturable microbiology; genome sequencing ID SP-NOV.; AMPLIFICATION; DIVERSITY; RESISTANCE; GENOMICS; SAMPLES; SOIL AB Single-cell genomics (SCG) is a recently developed tool to study the genomes of unculturable bacterial species. SCG relies on multiple-strand displacement amplification (MDA), PCR, and next-generation sequencing (NGS); however, obtaining sufficient amounts of high-quality DNA from samples is a major challenge when performing this technique. Here we present an improved bacterial cell lysing procedure that combines incubation in an alkaline buffer with a thermal shock (freezing/heating) treatment to yield highly intact genomic DNA with high efficiency. This procedure is more efficient in lysing Bacillus subtilis and Synechocystis cells compared with two other frequently used lysis methods. Furthermore, 16S ribosomal RNA gene and overall genome recovery were found to be improved by this method using single cells from a Utah desert soil community or Escherichia coli single cells, respectively. The efficiency of genome recovery for E. coli single cells using our procedure is comparable with that of the REPLI-g Single Cell (SC) Kit, but our method is much more economical. By providing high-quality genome templates suitable for downstream applications, our procedure will be a promising improvement for SCG research. C1 [He, Jian] Chinese Acad Sci, Dalian Inst Chem Phys, Ctr Translat Med, Dept Biotechnol, Dalian, Liaoning, Peoples R China. [He, Jian; Arefin, Ayesha; Han, Cliff S.] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM USA. [Du, Shiyu] Chinese Acad Sci, Engn Lab Specialty Fibers & Nucl Energy Mat, Ningbo Inst Mat Technol & Engn, Ningbo, Zhejiang, Peoples R China. [Tan, Xiaohua] Wenzhou Med Univ, Key Lab Biotechnol & Pharmaceut Engn, Mol Pharmacol Res Ctr, Sch Pharm, Wenzhou, Zhejiang, Peoples R China. RP He, J (reprint author), Chinese Acad Sci, Dalian Inst Chem Phys, Ctr Translat Med, Dept Biotechnol, Dalian, Liaoning, Peoples R China.; Han, CS (reprint author), Los Alamos Natl Lab, Biosci Div, Los Alamos, NM USA. EM jih003@dicp.ac.cn; han_cliff@lanl.gov FU China Scholarship Council [2010617090]; Department of Energy Los Alamos National Laboratory LDRD program FX We thank Armand Dichosa, Blaire Stevens, and Cheryl Kuske for providing the soil sample. This work was supported in part by a scholarship from China Scholarship Council (No 2010617090) and funding provided by the Department of Energy Los Alamos National Laboratory LDRD program. NR 23 TC 0 Z9 0 U1 3 U2 10 PU BIOTECHNIQUES OFFICE PI NEW YORK PA 52 VANDERBILT AVE, NEW YORK, NY 10017 USA SN 0736-6205 EI 1940-9818 J9 BIOTECHNIQUES JI Biotechniques PD MAR PY 2016 VL 60 IS 3 BP 129 EP 135 DI 10.2144/000114389 PG 6 WC Biochemical Research Methods; Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DG5FS UT WOS:000372102200005 PM 26956090 ER PT J AU Barnes, T Thiruvathukal, GK AF Barnes, Tiffany Thiruvathukal, George K. TI The Need for Research in Broadening Participation SO COMMUNICATIONS OF THE ACM LA English DT Editorial Material C1 [Barnes, Tiffany] N Carolina State Univ, Comp Sci, Raleigh, NC 27695 USA. [Thiruvathukal, George K.] Loyola Univ Chicago, Comp Sci, Chicago, IL 60660 USA. [Thiruvathukal, George K.] Argonne Natl Lab, Div Math & Comp Sci, Argonne Leadership Comp Facil, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Barnes, T (reprint author), N Carolina State Univ, Comp Sci, Raleigh, NC 27695 USA.; Thiruvathukal, GK (reprint author), Loyola Univ Chicago, Comp Sci, Chicago, IL 60660 USA.; Thiruvathukal, GK (reprint author), Argonne Natl Lab, Div Math & Comp Sci, Argonne Leadership Comp Facil, 9700 S Cass Ave, Argonne, IL 60439 USA. EM tiffany.barnes@gmail.com; gkt@cs.luc.edu NR 7 TC 0 Z9 0 U1 0 U2 0 PU ASSOC COMPUTING MACHINERY PI NEW YORK PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA SN 0001-0782 EI 1557-7317 J9 COMMUN ACM JI Commun. ACM PD MAR PY 2016 VL 59 IS 3 BP 33 EP 34 DI 10.1145/2880177 PG 2 WC Computer Science, Hardware & Architecture; Computer Science, Software Engineering; Computer Science, Theory & Methods SC Computer Science GA DG3MM UT WOS:000371973700019 ER PT J AU Qi, YF Jo, S Im, W AF Qi, Yifei Jo, Sunhwan Im, Wonpil TI Roles of glycans in interactions between gp120 and HIV broadly neutralizing antibodies SO GLYCOBIOLOGY LA English DT Article DE PG9; PGT128; protein-glycan interaction ID MOLECULAR-DYNAMICS SIMULATION; ENVELOPE GLYCOPROTEIN GP120; CRYSTAL-STRUCTURE; VACCINE DESIGN; USER-INTERFACE; POTENT; GLYCOSYLATION; RECOGNITION; CONSTRAINTS; DATABASE AB Many novel broadly neutralizing antibodies against human immunodeficiency virus (HIV) have been identified during the past decade, providing promising templates for the development of an effective HIV-1 vaccine. Structural studies reveal that the epitopes of some of these antibodies involve one or more crucial glycans, without which the binding is completely abolished. In this study, we have investigated the critical roles of glycans in interactions between HIV-1 gp120 and two broadly neutralizing antibodies PG9 (targeting V1/V2) and PGT128 (targeting V3) that are able to neutralize more than 70% of HIV-1 isolates. We have performed molecular dynamics simulations of a number of systems including antibody-gp120 complex with and without glycans, antibody, gp120 with and without glycans, and glycan-only systems. The simulation results show that the complex structures are stabilized by the glycans, and the multivalent interactions between the antibody and gp120 promote cooperativities to further enhance the binding. In the free gp120, the glycans increase the flexibility of the V1/V2 and V3 loops, which likely increases the entropy cost of the antibody recognition. However, the antibodies are able to bind the flexible interface by recognizing the preexisting glycan conformation, and penetrating the glycan shield with flexible complementarity determining region loops that sample the bound conformations occasionally. C1 [Qi, Yifei; Im, Wonpil] Univ Kansas, Dept Mol Biosci, 2030 Becker Dr, Lawrence, KS 66047 USA. [Qi, Yifei; Im, Wonpil] Univ Kansas, Ctr Computat Biol, 2030 Becker Dr, Lawrence, KS 66047 USA. [Jo, Sunhwan] Argonne Natl Lab, Leadership Comp Facil, 9700 Cass Ave Bldg 240, Argonne, IL 60439 USA. RP Im, W (reprint author), Univ Kansas, Dept Mol Biosci, 2030 Becker Dr, Lawrence, KS 66047 USA.; Im, W (reprint author), Univ Kansas, Ctr Computat Biol, 2030 Becker Dr, Lawrence, KS 66047 USA. EM wonpil@ku.edu FU University of Kansas General Research Fund [2301552]; National Institutes of Health and the Pittsburgh Supercomputing Center (PSC) [P41GM103712-S1]; [NSF IIA-1359530]; [NIH U54GM087519]; [XSEDE MCB070009] FX This work was supported by the University of Kansas General Research Fund allocation #2301552, NSF IIA-1359530, NIH U54GM087519 and XSEDE MCB070009. Anton computer time was provided by the National Center for Multiscale Modeling of Biological Systems (MMBioS) through Grant P41GM103712-S1 from the National Institutes of Health and the Pittsburgh Supercomputing Center (PSC). NR 56 TC 1 Z9 1 U1 3 U2 13 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 0959-6658 EI 1460-2423 J9 GLYCOBIOLOGY JI Glycobiology PD MAR PY 2016 VL 26 IS 3 BP 251 EP 260 DI 10.1093/glycob/cwv101 PG 10 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DG4BA UT WOS:000372013700004 PM 26537503 ER PT J AU France, RM Geisz, JF Garcia, I Steiner, MA McMahon, WE Friedman, DJ Moriarty, TE Osterwald, C Ward, JS Duda, A Young, M Olavarria, WJ AF France, Ryan M. Geisz, John F. Garcia, Ivan Steiner, Myles A. McMahon, William E. Friedman, Daniel J. Moriarty, Tom E. Osterwald, Carl Ward, J. Scott Duda, Anna Young, Michelle Olavarria, Waldo J. TI Design Flexibility of Ultrahigh Efficiency Four-Junction Inverted Metamorphic Solar Cells SO IEEE JOURNAL OF PHOTOVOLTAICS LA English DT Article DE Four-junction solar cells; inverted metamorphic multijunction ID OPTIMIZATION AB The inverted metamorphic solar cell has highly tunable bandgaps, in part due to the metamorphic subcells. Using phosphide-based compositionally graded buffers, we show a wide variety of GaInAs solar cells, ranging in bandgap from 1.2 to 0.7 eV. These metamorphic subcells are all high quality and can be used for a wide variety of multijunction designs. GaInAs solar cells with 0.70 eV bandgaps are developed using an InAsP buffer that extends beyond the InP lattice constant, allowing access to an additional 2 mA/cm(2) of photocurrent at AM1.5D and 25 degrees C. This subcell is implemented into a four-junction inverted metamorphic solar cell combined with an appropriate antireflective coating, which increases the series-connected multijunction current by 0.5 mA/cm(2) with respect to designs using 0.74-eV GaInAs. However, the optimal design depends on the spectrum and operating temperature. We show how the device flexibility can be used to fine-tune the design for various spectra in order to maximize energy yield for a given operating condition. One-sun devices achieve 35.3 +/- 1.2% efficiency under the AM0 spectra and 37.8 +/- 1.2% efficiency under the global spectra at 25 degrees C. Concentrator devices designed for elevated operating temperature achieve 45.6 +/- 2.3% peak efficiency under 690x the direct spectrum and 45.2 +/- 2.3% efficiency at 1000x and 25 degrees C. Device optimization is performed for the direct spectrum on 1 sun devices with 2% shadowing, which achieve 39.8 +/- 1.2% efficiency under the direct spectrum at 1 sun, highlighting the excellent performance and bandgap tunability of the four-junction inverted metamorphic solar cell. C1 [France, Ryan M.; Geisz, John F.; Garcia, Ivan; Steiner, Myles A.; McMahon, William E.; Friedman, Daniel J.; Moriarty, Tom E.; Osterwald, Carl; Ward, J. Scott; Duda, Anna; Young, Michelle; Olavarria, Waldo J.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Garcia, Ivan] Univ Politecn Madrid, Inst Energia Solar, E-28040 Madrid, Spain. RP France, RM; Geisz, JF; Garcia, I; Steiner, MA; McMahon, WE; Friedman, DJ; Moriarty, TE; Osterwald, C; Ward, JS; Duda, A; Young, M; Olavarria, WJ (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA.; Garcia, I (reprint author), Univ Politecn Madrid, Inst Energia Solar, E-28040 Madrid, Spain. EM ryan.france@nrel.gov; john.geisz@nrel.gov; ivan.garcia@nrel.gov; myles.steiner@nrel.gov; bill.mcmahon@nrel.gov; daniel.friedman@nrel.gov; Tom.Moriarty@nrel.gov; Carl.Osterwald@nrel.gov; scott.ward@nrel.gov; anna.duda@nrel.gov; michelle.young@nrel.gov; waldo.olavarria@nrel.gov RI Garcia, Ivan/L-1547-2014 OI Garcia, Ivan/0000-0002-9895-2020 FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory; IOF grant from the People Program (Marie Curie Actions) of the European Union under REA [299878] FX This work was supported by the U.S. Department of Energy under Contract DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. The work of I. Garcia was supported by an IOF grant from the People Program (Marie Curie Actions) of the European Union's Seventh Framework Program (FP7/2007-2013) under REA Grant 299878. NR 23 TC 6 Z9 6 U1 3 U2 6 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2156-3381 J9 IEEE J PHOTOVOLT JI IEEE J. Photovolt. PD MAR PY 2016 VL 6 IS 2 BP 578 EP 583 DI 10.1109/JPHOTOV.2015.2505182 PG 6 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA DG4AK UT WOS:000372012100029 ER PT J AU Malikopoulos, AA AF Malikopoulos, Andreas A. TI A Multiobjective Optimization Framework for Online Stochastic Optimal Control in Hybrid Electric Vehicles SO IEEE TRANSACTIONS ON CONTROL SYSTEMS TECHNOLOGY LA English DT Article DE Hybrid electric vehicles (HEVs); multiobjective optimization; Pareto control policy; power management control; stochastic optimal control ID ENERGY MANAGEMENT; AVERAGE COST; STRATEGY; ALGORITHMS; SIMULATION AB The increasing urgency to extract additional efficiency from hybrid propulsion systems has led to the development of advanced power management control algorithms. In this paper, we address the problem of online optimization of the supervisory power management control in parallel hybrid electric vehicles (HEVs). We model HEV operation as a controlled Markov chain and show that the control policy yielding the Pareto optimal solution minimizes online the long-run expected average cost per unit time criterion. The effectiveness of the proposed solution is validated through simulation and compared with the solution derived with dynamic programming using the average cost criterion. Both solutions achieved the same cumulative fuel consumption demonstrating that the online Pareto control policy is an optimal control policy. C1 [Malikopoulos, Andreas A.] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. RP Malikopoulos, AA (reprint author), Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. EM andreas@ornl.gov FU US Department of Energy [DE-AC05-00OR22725] FX This manuscript has been authored by UT-Battelle, LLC, under contract DE-AC05-00OR22725 with the US Department of Energy. The US government retains and the publisher, by accepting the article for publication, acknowledges that the US government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for US government purposes. Recommended by Associate Editor K. Butts. NR 43 TC 2 Z9 2 U1 5 U2 22 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1063-6536 EI 1558-0865 J9 IEEE T CONTR SYST T JI IEEE Trans. Control Syst. Technol. PD MAR PY 2016 VL 24 IS 2 BP 440 EP 450 DI 10.1109/TCST.2015.2454444 PG 11 WC Automation & Control Systems; Engineering, Electrical & Electronic SC Automation & Control Systems; Engineering GA DG3WY UT WOS:000372002500006 ER PT J AU Gangammanavar, H Sen, S Zavala, VM AF Gangammanavar, Harsha Sen, Suvrajeet Zavala, Victor M. TI Stochastic Optimization of Sub-Hourly Economic Dispatch With Wind Energy SO IEEE TRANSACTIONS ON POWER SYSTEMS LA English DT Article DE Economic dispatch; stochastic decomposition; sub-hourly dispatch ID UNIT COMMITMENT; DECOMPOSITION; VARIABILITY; CONSTRAINTS; UNCERTAINTY; GENERATION; SECURITY; CAPACITY; MARKET AB We present a stochastic programming framework for a multiple timescale economic dispatch problem to address integration of renewable energy resources into power systems. This framework allows certain slow-response energy resources to be controlled at an hourly timescale, while fast-response resources, including renewable resources, and related network decisions can be controlled at a sub-hourly timescale. To this end, we study two models motivated by actual scheduling practices of system operators. Using an external simulator as driver for sub-hourly wind generation, we optimize these economic dispatch models using stochastic decomposition, a sample-based approach for stochastic programming. Computational experiments, conducted on the IEEE-RTS96 system and the Illinois system, reveal that optimization with sub-hourly dispatch not only results in lower expected operational costs, but also predicts these costs with far greater accuracy than with models allowing only hourly dispatch. Our results also demonstrate that when compared with standard approaches using the extensive formulation of stochastic programming, the sequential sampling approach of stochastic decomposition provides better predictions with much less computational time. C1 [Gangammanavar, Harsha; Sen, Suvrajeet] Univ So Calif, Daniel J Epstein Dept Ind & Syst Engn, Los Angeles, CA 90089 USA. [Zavala, Victor M.] Argonne Natl Lab, Div Math & Comp Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Gangammanavar, H; Sen, S (reprint author), Univ So Calif, Daniel J Epstein Dept Ind & Syst Engn, Los Angeles, CA 90089 USA.; Zavala, VM (reprint author), Argonne Natl Lab, Div Math & Comp Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM gangamma@usc.edu; s.sen@usc.edu; vzavala@mcs.anl.gov FU U.S. Department of Energy, Office of Science [DE-AC02-06CH11357]; NSF [CMMI: 0900070]; AFOSR [FA9550-13-1-0015] FX The work of V. M. Zavala was supported by the U.S. Department of Energy, Office of Science, under contract number DE-AC02-06CH11357. This work was supported by NSF (CMMI: 0900070) and AFOSR (FA9550-13-1-0015). Paper no. TPWRS-00790-2014. NR 33 TC 5 Z9 5 U1 1 U2 8 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8950 EI 1558-0679 J9 IEEE T POWER SYST JI IEEE Trans. Power Syst. PD MAR PY 2016 VL 31 IS 2 BP 949 EP 959 DI 10.1109/TPWRS.2015.2410301 PG 11 WC Engineering, Electrical & Electronic SC Engineering GA DG4CH UT WOS:000372017600010 ER PT J AU Ozdemir, O Munoz, FD Ho, JL Hobbs, BF AF Ozdemir, Ozge Munoz, Francisco D. Ho, Jonathan L. Hobbs, Benjamin F. TI Economic Analysis of Transmission Expansion Planning With Price-Responsive Demand and Quadratic Losses by Successive LP SO IEEE TRANSACTIONS ON POWER SYSTEMS LA English DT Article DE Demand response; nonlinear optimization; successive linear programming; transmission planning ID DECOMPOSITION APPROACH; ELECTRICITY MARKETS; POWER; NETWORK; GENERATION; MODELS; PENETRATION; ALGORITHM; COST AB The growth of demand response programs and renewable generation is changing the economics of transmission. Planners and regulators require tools to address the implications of possible technology, policy, and economic developments for the optimal configuration of transmission grids. We propose a model for economic evaluation and optimization of inter-regional transmission expansion, as well as the optimal response of generators' investments to locational incentives, that accounts for Kirchhoff's laws and three important nonlinearities. The first is consumer response to energy prices, modeled using elastic demand functions. The second is resistance losses. The third is the product of line susceptance and flows in the linearized DC load flow model. We develop a practical method combining Successive Linear Programming with Gauss-Seidel iteration to co-optimize AC and DC transmission and generation capacities in a linearized DC network while considering hundreds of hourly realizations of renewable supply and load. We test our approach for a European electricity market model including 33 countries. The examples indicate that demand response can be a valuable resource that can significantly affect the economics, location, and amounts of transmission and generation investments. Further, representing losses and Kirchhoff's laws is also important in transmission policy analyses. C1 [Ozdemir, Ozge] Energy Res Ctr Netherlands ECN, Unit Policy Studies, NL-1043 NT Amsterdam, Netherlands. [Munoz, Francisco D.] Univ Adolfo Ibanez, Ind Engn & Operat Grp IE&O, Santiago, Chile. [Munoz, Francisco D.] Sandia Natl Labs, Dept Complex Math & Algorithms, POB 5800, Albuquerque, NM 87185 USA. [Ho, Jonathan L.] Johns Hopkins Univ, Dept Geog & Environm Engn, Baltimore, MD 21218 USA. [Hobbs, Benjamin F.] Johns Hopkins Univ, Dept Geog & Environm Engn DoGEE, Environm Management, Baltimore, MD 21218 USA. RP Ozdemir, O (reprint author), Energy Res Ctr Netherlands ECN, Unit Policy Studies, NL-1043 NT Amsterdam, Netherlands.; Munoz, FD (reprint author), Univ Adolfo Ibanez, Ind Engn & Operat Grp IE&O, Santiago, Chile.; Ho, JL (reprint author), Johns Hopkins Univ, Dept Geog & Environm Engn, Baltimore, MD 21218 USA.; Hobbs, BF (reprint author), Johns Hopkins Univ, Dept Geog & Environm Engn DoGEE, Environm Management, Baltimore, MD 21218 USA. EM ozdemir@ecn.nl; fdmunoz@sandia.gov; jho19@jhu.edu; bhobbs@jhu.edu FU U.S. DOE CERTS Reliability and Markets program; NSF [IIA 1243482, ECCS 1230788]; Fulbright Foundation; U.S. DOE, Office of Science, Office of Advanced Scientific Computing Research, Applied Mathematics program through Project "Multifaceted Mathematics for Complex Energy Systems" [KJ0401000] FX This work was supported in part by U.S. DOE CERTS Reliability and Markets program, NSF grants IIA 1243482 and ECCS 1230788, the Fulbright Foundation, and the U.S. DOE, Office of Science, Office of Advanced Scientific Computing Research, Applied Mathematics program under contract number KJ0401000 through the Project "Multifaceted Mathematics for Complex Energy Systems". Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94-AL85000 Paper no. TPWRS-01060-2014. NR 65 TC 4 Z9 4 U1 2 U2 6 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8950 EI 1558-0679 J9 IEEE T POWER SYST JI IEEE Trans. Power Syst. PD MAR PY 2016 VL 31 IS 2 BP 1096 EP 1107 DI 10.1109/TPWRS.2015.2427799 PG 12 WC Engineering, Electrical & Electronic SC Engineering GA DG4CH UT WOS:000372017600023 ER PT J AU Muratori, M Rizzoni, G AF Muratori, Matteo Rizzoni, Giorgio TI Residential Demand Response: Dynamic Energy Management and Time-Varying Electricity Pricing SO IEEE TRANSACTIONS ON POWER SYSTEMS LA English DT Article DE Demand response; electricity pricing; rebound peaks; residential energy management; TOU and CPP ID LOAD CONTROL; CONSUMPTION; MARKETS; IMPACTS AB Demand response programs are currently being proposed as a solution to deal with issues related to peak demand and to improve the operation of the electric power system. In the demand response paradigm, electric utilities provide incentives and benefits to private consumers as a compensation for their flexibility in the timing of their electricity consumption. In this paper, a dynamic energy management framework, based on highly resolved energy consumption models, is used to simulate automated residential demand response. The models estimate the residential demand using a novel bottom-up approach that quantifies consumer energy use behavior, thus providing an accurate estimation of the actual amount of controllable resources. The optimal schedule of all of the controllable appliances, including plug-in electric vehicles, is found by minimizing consumer electricity-related expenditures. Recently, time-varying electricity rate plans have been proposed by electric utilities as an incentive to their customers with the objective of re-shaping the aggregate demand. Large-scale simulations are performed to analyze and quantitatively assess the impact of demand response programs using different electricity price structures. Results show that simple time-varying electricity price structures, coupled with large-scale adoption of automated energy management systems, might create pronounced rebound peaks in the aggregate residential demand. To cope with the rebound peaks created by the synchronization of the individual residential demands, innovative electricity price structures-called Multi-TOU and Multi-CPP-are proposed. C1 [Muratori, Matteo] Pacific NW Natl Lab, Joint Glogal Change Res Inst, College Pk, MD 20740 USA. [Rizzoni, Giorgio] Ohio State Univ, Dept Mech Engn, Columbus, OH 43212 USA. RP Muratori, M (reprint author), Pacific NW Natl Lab, Joint Glogal Change Res Inst, College Pk, MD 20740 USA.; Rizzoni, G (reprint author), Ohio State Univ, Dept Mech Engn, Columbus, OH 43212 USA. EM matteo.muratori@pnnl.gov; rizzoni.1@osu.edu RI Rizzoni, Giorgio/D-2961-2016 OI Rizzoni, Giorgio/0000-0002-8397-7241 FU National Science Foundation [1029337] FX This work was performed at The Ohio State University-Center for Automotive Research supported by the National Science Foundation under Grant 1029337. Paper no. TPWRS-01072-2014. NR 33 TC 7 Z9 7 U1 8 U2 17 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8950 EI 1558-0679 J9 IEEE T POWER SYST JI IEEE Trans. Power Syst. PD MAR PY 2016 VL 31 IS 2 BP 1108 EP 1117 DI 10.1109/TPWRS.2015.2414880 PG 10 WC Engineering, Electrical & Electronic SC Engineering GA DG4CH UT WOS:000372017600024 ER PT J AU Xu, Y Liu, CC Schneider, KP Ton, DT AF Xu, Yin Liu, Chen-Ching Schneider, Kevin P. Ton, Dan T. TI Placement of Remote-Controlled Switches to Enhance Distribution System Restoration Capability SO IEEE TRANSACTIONS ON POWER SYSTEMS LA English DT Article DE Distribution automation (DA); reliability; remote controlled switch; self-healing; service restoration ID ALGORITHM; SEARCH; DAS AB A smart distribution system should restore service to interrupted customers as quickly as possible after an outage. Upgrading manual switches to remote-controlled switches (RCSs) enhances restoration capability. The placement of RCSs should consider both functional and economic requirements. This paper presents a systematic method to determine the set of switches to be upgraded for an existing distribution system. The maximum restoration capability is achieved by upgrading a near-minimum number of manual switches to RCSs. The RCS placement problem is formulated as a weighed set cover (WSC) problem. A greedy algorithm with a polynomial-time computational efficiency is designed to generate a near-optimal solution for the WSC problem. A 3-feeder 9-node test system and a 4-feeder 1069-node unbalanced test system with microgrids are used to validate the effectiveness of the proposed method. C1 [Xu, Yin; Liu, Chen-Ching] Washington State Univ, Sch Elect Engn & Comp Sci, Pullman, WA 99163 USA. [Liu, Chen-Ching] Univ Coll Dublin, Sch Mech & Mat Engn, Dublin 2, Ireland. [Schneider, Kevin P.] Pacific NW Natl Lab, Battelle Seattle Res Ctr, Seattle, WA 98109 USA. [Ton, Dan T.] US DOE, Smart Grid R&D, Washington, DC 20585 USA. RP Xu, Y; Liu, CC (reprint author), Washington State Univ, Sch Elect Engn & Comp Sci, Pullman, WA 99163 USA.; Schneider, KP (reprint author), Pacific NW Natl Lab, Battelle Seattle Res Ctr, Seattle, WA 98109 USA.; Ton, DT (reprint author), US DOE, Smart Grid R&D, Washington, DC 20585 USA. EM yxu2@eecs.wsu.edu; liu@eecs.wsu.edu; kevin.schneider@pnnl.gov; dan.ton@hq.doe.gov FU U.S. Department of Energy (DOE); Pacific Northwest National Laboratory (PNNL) FX This work was supported in part by the U.S. Department of Energy (DOE) and Pacific Northwest National Laboratory (PNNL). Paper no. TPWRS-01106-2014. NR 25 TC 4 Z9 4 U1 2 U2 5 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8950 EI 1558-0679 J9 IEEE T POWER SYST JI IEEE Trans. Power Syst. PD MAR PY 2016 VL 31 IS 2 BP 1139 EP 1150 DI 10.1109/TPWRS.2015.2419616 PG 12 WC Engineering, Electrical & Electronic SC Engineering GA DG4CH UT WOS:000372017600027 ER PT J AU Li, S Zhang, W Lian, JM Kalsi, K AF Li, Sen Zhang, Wei Lian, Jianming Kalsi, Karanjit TI Market-Based Coordination of Thermostatically Controlled Loads-Part I: A Mechanism Design Formulation SO IEEE TRANSACTIONS ON POWER SYSTEMS LA English DT Article DE Demand response; market-based coordination; mechanism design; thermostatically controlled loads ID DEMAND-SIDE MANAGEMENT; REGULATION SERVICE; ELECTRIC VEHICLES; DATA CENTERS; ENERGY AB This paper focuses on the coordination of a population of thermostatically controlled loads (TCLs) with unknown parameters to achieve group objectives. The problem involves designing the device bidding and market clearing strategies to motivate self-interested users to realize efficient energy allocation subject to a peak energy constraint. This coordination problem is formulated as a mechanism design problem, and we propose a mechanism to implement the social choice function in dominant strategy equilibrium. The proposed mechanism consists of a novel bidding and clearing strategy that incorporates the internal dynamics of TCLs in the market mechanism design, and we show it can realize the team optimal solution. This paper is divided into two parts. Part I presents a mathematical formulation of the problem and develops a coordination framework using the mechanism design approach. Part II presents a learning scheme to account for the unknown load model parameters, and evaluates the proposed framework through realistic simulations. C1 [Li, Sen; Zhang, Wei] Ohio State Univ, Dept Elect & Comp Engn, Columbus, OH 43210 USA. [Lian, Jianming; Kalsi, Karanjit] Pacific NW Natl Lab, Elect Infrastruct Grp, Richland, WA 99354 USA. RP Li, S; Zhang, W (reprint author), Ohio State Univ, Dept Elect & Comp Engn, Columbus, OH 43210 USA.; Lian, JM; Kalsi, K (reprint author), Pacific NW Natl Lab, Elect Infrastruct Grp, Richland, WA 99354 USA. EM li.2886@osu.edu; zhang.491@osu.edu; jianming.lian@pnnl.gov; karanjit.Kalsi@pnnl.gov RI Zhang, Wei/B-3219-2013; Zhang, Wei/L-2407-2016 OI Zhang, Wei/0000-0002-7511-2870 NR 37 TC 3 Z9 3 U1 1 U2 5 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8950 EI 1558-0679 J9 IEEE T POWER SYST JI IEEE Trans. Power Syst. PD MAR PY 2016 VL 31 IS 2 BP 1170 EP 1178 DI 10.1109/TPWRS.2015.2432057 PG 9 WC Engineering, Electrical & Electronic SC Engineering GA DG4CH UT WOS:000372017600030 ER PT J AU Li, S Zhang, W Lian, JM Kalsi, K AF Li, Sen Zhang, Wei Lian, Jianming Kalsi, Karanjit TI Market-Based Coordination of Thermostatically Controlled Loads-Part II: Unknown Parameters and Case Studies SO IEEE TRANSACTIONS ON POWER SYSTEMS LA English DT Article DE Demand response; joint state-parameter estimation; mechanism design; thermostatically controlled loads AB This two-part paper considers the coordination of a population of thermostatically controlled loads (TCLs) with unknown parameters to achieve group objectives. The problem involves designing the bidding and market clearing strategy to motivate self-interested users to realize efficient energy allocation subject to a peak energy constraint. The companion paper (Part I) formulates the problem and proposes a load coordination framework using the mechanism design approach. To address the unknown parameters, Part II of this paper presents a joint state and parameter estimation framework based on the expectation maximization algorithm. The overall framework is then validated using real-world weather data and price data, and is compared with other approaches in terms of aggregated load response. Simulation results indicate that our coordination framework can effectively improve the operational efficiency of the distribution system and reduce power congestion at key times. C1 [Li, Sen; Zhang, Wei] Ohio State Univ, Dept Elect & Comp Engn, Columbus, OH 43210 USA. [Lian, Jianming; Kalsi, Karanjit] Pacific NW Natl Lab, Elect Infrastruct Grp, Richland, WA 99354 USA. RP Li, S; Zhang, W (reprint author), Ohio State Univ, Dept Elect & Comp Engn, Columbus, OH 43210 USA.; Lian, JM; Kalsi, K (reprint author), Pacific NW Natl Lab, Elect Infrastruct Grp, Richland, WA 99354 USA. EM li.2886@osu.edu; zhang.491@osu.edu; jianming.lian@pnnl.gov; karanjit.Kalsi@pnnl.gov RI Zhang, Wei/B-3219-2013; Zhang, Wei/L-2407-2016 OI Zhang, Wei/0000-0002-7511-2870 NR 15 TC 0 Z9 0 U1 0 U2 2 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8950 EI 1558-0679 J9 IEEE T POWER SYST JI IEEE Trans. Power Syst. PD MAR PY 2016 VL 31 IS 2 BP 1179 EP 1187 DI 10.1109/TPWRS.2015.2432060 PG 9 WC Engineering, Electrical & Electronic SC Engineering GA DG4CH UT WOS:000372017600031 ER PT J AU Bucher, MA Chatzivasileiadis, S Andersson, G AF Bucher, Matthias A. Chatzivasileiadis, Spyridon Andersson, Goeran TI Managing Flexibility in Multi-Area Power Systems SO IEEE TRANSACTIONS ON POWER SYSTEMS LA English DT Article DE Computational geometry; inter-TSO coordination; operational flexibility AB In this paper we present a framework to efficiently characterize the available operational flexibility in a multi-area power system. We focus on the available reserves and the tie-line flows. The proposed approach is an alternative to the current calculation of the available transfer capacity (ATC), as it considers location and availability of reserves, transmission constraints, and interdependencies of tie-line flows between different areas, while it takes into account the N - 1 security criterion. The method is based on computational geometry using polytopic projections. It requires only a limited amount of information exchange and does not need central coordination. The method has two versions: a passive approach, and an active approach where neighboring areas can share reserves. In that respect we also introduce the term "exportable flexibility". Case studies demonstrate the improved tie-line utilization, especially if reserves are shared, and the visualization benefits. C1 [Bucher, Matthias A.; Andersson, Goeran] ETH, Dept Informat Technol & Elect Engn, EEH Power Syst Lab, Zurich, Switzerland. [Chatzivasileiadis, Spyridon] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Bucher, MA; Andersson, G (reprint author), ETH, Dept Informat Technol & Elect Engn, EEH Power Syst Lab, Zurich, Switzerland.; Chatzivasileiadis, S (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM mb@eeh.ee.ethz.ch; andersson@eeh.ee.ethz.ch; schatzivasileiadis@lb1.gov FU Swiss Federal Office of Energy (SFOE); Swissgrid FX This work was carried out within the project Balancing Power in the European System (BPES) and supported by the Swiss Federal Office of Energy (SFOE) and Swissgrid. Paper no. TPWRS-01174-2014. NR 13 TC 3 Z9 3 U1 2 U2 4 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8950 EI 1558-0679 J9 IEEE T POWER SYST JI IEEE Trans. Power Syst. PD MAR PY 2016 VL 31 IS 2 BP 1218 EP 1226 DI 10.1109/TPWRS.2015.2413387 PG 9 WC Engineering, Electrical & Electronic SC Engineering GA DG4CH UT WOS:000372017600035 ER PT J AU Pan, K Guan, YP Watson, JP Wang, JH AF Pan, Kai Guan, Yongpei Watson, Jean-Paul Wang, Jianhui TI Strengthened MILP Formulation for Certain Gas Turbine Unit Commitment Problems SO IEEE TRANSACTIONS ON POWER SYSTEMS LA English DT Article DE Gas turbines; mixed-integer linear programming; unit commitment ID COORDINATION; TERM AB In this paper, we derive a strengthened MILP formulation for certain gas turbine unit commitment problems, in which the ramping rates are no smaller than the minimum generation amounts. This type of gas turbines can usually start-up faster and have a larger ramping rate, as compared to the traditional coalfired power plants. Recently, the number of this type of gas turbines increases significantly due to affordable gas prices and their scheduling flexibilities to accommodate intermittent renewable energy generation. In this study, several new families of strong valid inequalities are developed to help reduce the computational time to solve these types of problems. Meanwhile, the validity and facet-defining proofs are provided for certain inequalities. Finally, numerical experiments on a modified IEEE 118-bus system and the power system data based on recent studies verify the effectiveness of applying our formulation to model and solve this type of gas turbine unit commitment problems, including reducing the computational time to obtain an optimal solution or obtaining a much smaller optimality gap, as compared to the default CPLEX, when the time limit is reached with no optimal solutions obtained. C1 [Pan, Kai; Guan, Yongpei] Univ Florida, Dept Ind & Syst Engn, Gainesville, FL 32611 USA. [Watson, Jean-Paul] Sandia Natl Labs, Discrete Math & Complex Syst Dept, POB 5800, Albuquerque, NM 87185 USA. [Wang, Jianhui] Argonne Natl Lab, Div Energy Syst, Lemont, IL 60439 USA. RP Pan, K; Guan, YP (reprint author), Univ Florida, Dept Ind & Syst Engn, Gainesville, FL 32611 USA.; Watson, JP (reprint author), Sandia Natl Labs, Discrete Math & Complex Syst Dept, POB 5800, Albuquerque, NM 87185 USA.; Wang, JH (reprint author), Argonne Natl Lab, Div Energy Syst, Lemont, IL 60439 USA. EM kpan@ufl.edu; guan@ise.ufl.edu; jwatson@sandia.gov; jianhui.wang@anl.gov FU U.S. Department of Energy Office of Electricity Delivery and Energy Reliability; Sandia National Laboratories' Laboratory-Directed Research and Development Program; Lockheed Martin Corporation, for U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The work of J. Wang was supported in part by the U.S. Department of Energy Office of Electricity Delivery and Energy Reliability. The work of J.-P. Watson was supported by Sandia National Laboratories' Laboratory-Directed Research and Development Program. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. Paper no. TPWRS-01445-2014. NR 18 TC 0 Z9 0 U1 2 U2 3 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8950 EI 1558-0679 J9 IEEE T POWER SYST JI IEEE Trans. Power Syst. PD MAR PY 2016 VL 31 IS 2 BP 1440 EP 1448 DI 10.1109/TPWRS.2015.2426139 PG 9 WC Engineering, Electrical & Electronic SC Engineering GA DG4CH UT WOS:000372017600056 ER PT J AU Wang, YZ Chen, C Wang, JH Baldick, R AF Wang, Yezhou Chen, Chen Wang, Jianhui Baldick, Ross TI Research on Resilience of Power Systems Under Natural Disasters-A Review SO IEEE TRANSACTIONS ON POWER SYSTEMS LA English DT Review DE Blackout restoration; natural disasters; power systems operation ID SERVICE RESTORATION; MULTIAGENT SYSTEM; EXPERT-SYSTEM; MICROGRIDS; METHODOLOGY; RELIABILITY; CHALLENGES; HURRICANES; STRATEGIES; ALLOCATION AB Natural disasters can cause large blackouts. Research into natural disaster impacts on electric power systems is emerging to understand the causes of the blackouts, explore ways to prepare and harden the grid, and increase the resilience of the power grid under such events. At the same time, new technologies such as smart grid, micro grid, and wide area monitoring applications could increase situational awareness as well as enable faster restoration of the system. This paper aims to consolidate and review the progress of the research field towards methods and tools of forecasting natural disaster related power system disturbances, hardening and pre-storm operations, and restoration models. Challenges and future research opportunities are also presented in the paper. C1 [Wang, Yezhou; Baldick, Ross] Univ Texas Austin, Austin, TX 78712 USA. [Chen, Chen; Wang, Jianhui] Argonne Natl Lab, CEEESA, Argonne, IL 60439 USA. RP Wang, YZ; Baldick, R (reprint author), Univ Texas Austin, Austin, TX 78712 USA.; Chen, C; Wang, JH (reprint author), Argonne Natl Lab, CEEESA, Argonne, IL 60439 USA. EM nickncwang@utexas.edu; morningchen@anl.gov; jianhui.wang@anl.gov; baldick@ece.utexas.edu FU U.S. Department of Energy Office of Electricity Delivery and Energy Reliability; Defense Threat Reduction Agency FX This work was supported by the U.S. Department of Energy Office of Electricity Delivery and Energy Reliability. The work of Y. Wang and R. Baldick was supported in part by the Defense Threat Reduction Agency. Paper no. TPWRS-01666-2014. NR 84 TC 10 Z9 10 U1 12 U2 24 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8950 EI 1558-0679 J9 IEEE T POWER SYST JI IEEE Trans. Power Syst. PD MAR PY 2016 VL 31 IS 2 BP 1604 EP 1613 DI 10.1109/TPWRS.2015.2429656 PG 10 WC Engineering, Electrical & Electronic SC Engineering GA DG4CH UT WOS:000372017600072 ER PT J AU Li, ZS Guo, QL Sun, HB Wang, JH AF Li, Zhengshuo Guo, Qinglai Sun, Hongbin Wang, Jianhui TI Sufficient Conditions for Exact Relaxation of Complementarity Constraints for Storage-Concerned Economic Dispatch SO IEEE TRANSACTIONS ON POWER SYSTEMS LA English DT Article DE Complementarity constraint; economic dispatch; relaxation; storage ID ENERGY-STORAGE; GENERATION; CAPACITY AB Storage-concerned economic dispatch (ED) problems with complementarity constraints are strongly non-convex and hard to solve. In this letter, an exact relaxation method is proposed to relax the non-convex ED to a convex form under two sufficient conditions, which can be further generalized for other problems of similar structures. A mathematical proof is provided, and the numerical tests verify the effect of this method. C1 [Li, Zhengshuo; Guo, Qinglai; Sun, Hongbin] Tsinghua Univ, Dept Elect Engn, State Key Lab Power Syst, Beijing 100084, Peoples R China. [Wang, Jianhui] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Sun, HB (reprint author), Tsinghua Univ, Dept Elect Engn, State Key Lab Power Syst, Beijing 100084, Peoples R China. EM shb@tsinghua.edu.cn FU National Key Basic Research Program of China (973 Program) [2013CB228202]; Innovative Research Groups of NSFC [51321005]; NSFC-RCUK_EPSRC [51361135703] FX This work was supported in part by National Key Basic Research Program of China (973 Program) (2013CB228202), Innovative Research Groups of NSFC (51321005), and NSFC-RCUK_EPSRC (51361135703). Paper no. PESL-00093-2014. NR 4 TC 1 Z9 1 U1 1 U2 2 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8950 EI 1558-0679 J9 IEEE T POWER SYST JI IEEE Trans. Power Syst. PD MAR PY 2016 VL 31 IS 2 BP 1653 EP 1654 DI 10.1109/TPWRS.2015.2412683 PG 2 WC Engineering, Electrical & Electronic SC Engineering GA DG4CH UT WOS:000372017600079 ER PT J AU Li, ZS Wang, JH Sun, HB Guo, QL AF Li, Zhengshuo Wang, Jianhui Sun, Hongbin Guo, Qinglai TI Transmission Contingency Screening Considering Impacts of Distribution Grids SO IEEE TRANSACTIONS ON POWER SYSTEMS LA English DT Article DE Contingency analysis; contingency selection; contingency screening; network equivalencing; global power flow AB As traditional transmission contingency screening (TCS) methods neglect impacts of distribution grids, the contingency selection result may not be always satisfactory, especially when distribution networks are more frequently looped in a smart grid. Two new contingency screening methods considering impacts of distribution grids are proposed in this letter. The first one is based on global power flow, and the second only utilizes distribution network equivalencing. Numerical tests show both new methods can give more reliable results than TCS. C1 [Li, Zhengshuo; Sun, Hongbin; Guo, Qinglai] Tsinghua Univ, Dept Elect Engn, Beijing 100084, Peoples R China. [Wang, Jianhui] Argonne Natl Lab, Argonne, IL 60439 USA. RP Sun, HB (reprint author), Tsinghua Univ, Dept Elect Engn, Beijing 100084, Peoples R China.; Wang, JH (reprint author), Argonne Natl Lab, Argonne, IL 60439 USA. EM jianhui.wang@anl.gov; shb@tsinghua.edu.cn FU National Key Basic Research Program of China (973 Program) [2013CB228203]; Innovative Research Groups of NSFC [51321005]; U.S. Department of Energy Office of Electricity Delivery and Energy Reliability FX This work was supported in part by the National Key Basic Research Program of China (973 Program) (2013CB228203) and in part by Innovative Research Groups of NSFC (51321005). The work of J. Wang was supported by the U.S. Department of Energy Office of Electricity Delivery and Energy Reliability. Paper no. PESL-00121-2014. NR 4 TC 1 Z9 1 U1 1 U2 1 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8950 EI 1558-0679 J9 IEEE T POWER SYST JI IEEE Trans. Power Syst. PD MAR PY 2016 VL 31 IS 2 BP 1659 EP 1660 DI 10.1109/TPWRS.2015.2412692 PG 2 WC Engineering, Electrical & Electronic SC Engineering GA DG4CH UT WOS:000372017600082 ER PT J AU Kim, HS Madavali, B Hong, SJ Kim, TS AF Kim, Hyo-Seob Madavali, Babu Hong, Soon-Jik Kim, Taek-Soo TI Effect of Milling Time on the Microstructure and Thermoelectric Properties of P-type TAGS-90 Alloys by HEM and SPS SO INTERNATIONAL JOURNAL OF APPLIED CERAMIC TECHNOLOGY LA English DT Article ID MECHANICAL-PROPERTIES; TRANSPORT; HARDNESS AB In this study, p-type TAGS-90 powders were fabricated using high-energy milling (HEM), subsequently sintered by spark plasma sintering (SPS). And then, the effects of milling time on the microstructure, mechanical, and thermoelectric properties were investigated. The powders were quickly decreased to fine particles of similar to 1 m in size and uniformly agglomerated with the increasing of milling time. XRD results indicated that all milled powders and SPSed samples showed single GeTe phase. Also, EDX results showed almost no contamination and exact composition after milling. The maximum figure of merit, ZT = 1.08, was obtained for 30-min-milled sample at 723 K. C1 [Kim, Hyo-Seob] Iowa State Univ, Ames Lab, 208 Met Dev, Ames, IA 50011 USA. [Madavali, Babu; Hong, Soon-Jik] Kongju Natl Univ, Div Adv Mat Engn, Cheonan 331717, South Korea. [Madavali, Babu; Hong, Soon-Jik] Kongju Natl Univ, Inst Rare Met, Cheonan 331717, South Korea. [Kim, Taek-Soo] Korea Inst Ind Technol KITECH, Korea Inst Rare Met KIRAM, 7-47 Songdo Dong, Inchon 406130, South Korea. RP Hong, SJ (reprint author), Kongju Natl Univ, Div Adv Mat Engn, Cheonan 331717, South Korea.; Hong, SJ (reprint author), Kongju Natl Univ, Inst Rare Met, Cheonan 331717, South Korea.; Kim, TS (reprint author), Korea Inst Ind Technol KITECH, Korea Inst Rare Met KIRAM, 7-47 Songdo Dong, Inchon 406130, South Korea. EM hongsj@kongju.ac.kr; tskim@kitech.re.kr RI Madavali, Babu/A-1486-2014 OI Madavali, Babu/0000-0002-8486-701X FU Korea Institute of Energy Technology Evaluation and Planning (KETEP) - Korea government Ministry of Knowledge Economy [20115010100020] FX This work was supported by the Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant funded by the Korea government Ministry of Knowledge Economy (No. 20115010100020). NR 25 TC 1 Z9 1 U1 2 U2 8 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1546-542X EI 1744-7402 J9 INT J APPL CERAM TEC JI Int. J. Appl. Ceram. Technol. PD MAR-APR PY 2016 VL 13 IS 2 BP 239 EP 244 DI 10.1111/ijac.12476 PG 6 WC Materials Science, Ceramics SC Materials Science GA DG4JA UT WOS:000372037300004 ER PT J AU Song, JH Chan, SW Rodenbough, PP Zhang, LH AF Song, Junhua Chan, Siu-Wai Rodenbough, Philip P. Zhang, Lihua TI Size-Dependent Crystal Properties of Nanocuprite SO INTERNATIONAL JOURNAL OF APPLIED CERAMIC TECHNOLOGY LA English DT Article ID CUPROUS-OXIDE; NANOPARTICLES; CU2O; OXIDATION; COPPER; SPECTROSCOPY; NANOCUBES AB Cuprite nanoparticles from 9 nm to 1 m with narrow size distribution (+/- 7%) are prepared by two different methods. The lattice parameter increases up to 0.2% as the crystallite size decreases to 9 nm from micron size. X-ray Absorption Near Edge Spectroscope study of our copper oxide nanoparticles shows mostly Cu (I) with increasing concentration of Cu (II) as decreasing crystal sizes. The size effect in Cu(II)/Cu(I) ratio indicates that at smaller crystal size, the Cu2O tends to be more oxidized at higher charge state with Cu(I)-O bond. Thus, the lattice expansion can be explained by the presence of longer Cu (II)-O bond than Cu (I)-O bond and/or oxygen interstitials in nanocuprite. C1 [Song, Junhua; Chan, Siu-Wai; Rodenbough, Philip P.] Columbia Univ, Dept Appl Phys & Appl Math, Mat Sci & Engn Program, New York, NY 10027 USA. [Rodenbough, Philip P.] Columbia Univ, Dept Chem, New York, NY 10027 USA. [Zhang, Lihua] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Chan, SW (reprint author), Columbia Univ, Dept Appl Phys & Appl Math, Mat Sci & Engn Program, New York, NY 10027 USA. EM sc174@columbia.edu FU National Science Foundation-DMR [1206764]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work is primarily supported by National Science Foundation-DMR 1206764. Research at National Synchrotron Light Source, Center for Functional Nanomaterials, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. We would like to acknowledge SWC's former student Jenna Pike for her investigation in cuprite nanoparticle synthesis. We would like to thank Nebojsa Marinkovic for the experimental setup at BNL NSLS beamline X19A. NR 22 TC 2 Z9 2 U1 5 U2 11 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1546-542X EI 1744-7402 J9 INT J APPL CERAM TEC JI Int. J. Appl. Ceram. Technol. PD MAR-APR PY 2016 VL 13 IS 2 BP 389 EP 394 DI 10.1111/ijac.12486 PG 6 WC Materials Science, Ceramics SC Materials Science GA DG4JA UT WOS:000372037300025 ER PT J AU Dongol, R Chambliss, K Sundaram, SK Diwan, MV AF Dongol, Ruhil Chambliss, Kameron Sundaram, Shanmugavelayutham K. Diwan, Milind V. TI Mechanical Properties of Photomultiplier Tube Glasses for Neutrino Detection SO INTERNATIONAL JOURNAL OF APPLIED GLASS SCIENCE LA English DT Article AB Photomultiplier tubes (PMT) are one of the primary components of water Cherenkov neutrino detection for the Long Baseline Neutrino Experiment (LBNE). Thousands of 10- to 12-inch diameter PMT bulbs are placed in the inner wall of a detection tank or a reservoir (e.g., deep mine) filled with 10,000 gallons of high purity water with a resistivity of 11-18.24M-cm. Long-term service of PMTs is vital to the success of neutrino detection projects. We report our results of our investigation on mechanical properties of PMT glasses from two vendors and the effect of ion exchange on their mechanical strength. Vickers indentation, four-point bend test, and ring-on-ring biaxial flexural strength test were used for evaluation of the mechanical strength. Chemical (potassium-sodium ion exchange) strengthening results show increased strength of 46% in one vendor glass and a 57% increase in the other, with no significant reduction in optical transmission in the ultraviolet-visible range of the electromagnetic spectrum that is critical to neutrino detection. Our results also show narrowing of the distribution of strength calculated using Weibull statistics with chemical strengthening for comparable exchange depths of 22-28m. C1 [Dongol, Ruhil; Chambliss, Kameron; Sundaram, Shanmugavelayutham K.] Alfred Univ, New York State Coll Ceram, Kazuo Inamori Sch Engn, Multifunct Mat Lab M&M Lab, Alfred, NY 14802 USA. [Diwan, Milind V.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Dongol, R; Sundaram, SK (reprint author), Alfred Univ, New York State Coll Ceram, Kazuo Inamori Sch Engn, Multifunct Mat Lab M&M Lab, Alfred, NY 14802 USA. EM sundaram@alfred.edu FU Brookhaven National Laboratory (BNL); BNL; Kyocera Corporation FX Brookhaven National Laboratory (BNL) supported this work under the advisory of Dr. Diwan and Mr. Rahul Sharma and a subcontract to Alfred University. We are grateful for their guidance and BNL's financial support for the project. SKS acknowledges the Inamori Professorship supported by the Kyocera Corporation. NR 21 TC 0 Z9 0 U1 0 U2 0 PU WILEY PERIODICALS, INC PI SAN FRANCISCO PA ONE MONTGOMERY ST, SUITE 1200, SAN FRANCISCO, CA 94104 USA SN 2041-1286 EI 2041-1294 J9 INT J APPL GLASS SCI JI Int. J. Appl. Glass Sci. PD MAR PY 2016 VL 7 IS 1 SI SI BP 94 EP 103 DI 10.1111/ijag.12140 PG 10 WC Materials Science, Ceramics SC Materials Science GA DG4AQ UT WOS:000372012700009 ER PT J AU Nguyen, BN Hou, ZS Bacon, DH Murray, CJ White, MD AF Ba Nghiep Nguyen Hou, Zhangshuan Bacon, Diana H. Murray, Christopher J. White, Mark D. TI Three-dimensional modeling of the reactive transport of CO2 and its impact on geomechanical properties of reservoir rocks and seals SO INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL LA English DT Article DE CO2 reservoir; Reactive transport; Geochemistry; Geomechanics; Geomechanical modeling; Mineral composition; Homogenization; Fault; Hydraulic fracture; Elastic modulus ID GEOLOGICAL STORAGE; HYDROTHERMAL SYSTEMS; AQUIFER DISPOSAL; SALINE AQUIFERS; INJECTION; FLOW; SITE; FIELD; SEQUESTRATION; GEOCHEMISTRY AB This article develops a model to analyze CO2 reservoirs using the STOMP-CO2-R code that is interfaced with the ABAQUS (R) finite element package. The STOMP-CO2-R/ABAQUS (R) simulator accounts for the reactive transport of CO2 causing changes in mineralogy that modify the geomechanical properties of reservoir rocks and seals. Rocks' elastic properties that vary during CO2 injection and govern the poroelastic behavior of rocks are modeled by an Eshelby-Mori-Tanka approach. A three-dimensional (3D) STOMP-CO2-R model for a CO2 reservoir containing a vertical fault was built to analyze a formation containing a reaction network with 5 minerals: albite, anorthite, calcite, kaolinite and quartz. A 3D ABAQUS (R) model that maps this STOMP-CO2-R model was built for the analysis using STOMP-CO2-R/ABAQUS (R). The results show that after a long period of CO2 injection the mineralogical changes significantly reduced the permeability and elastic modulus of the reservoir in front of the fault leading to a reduction of the pressure margin to fracture at and beyond the injection location. The impact of reactive transport of CO2 on the geomechanical properties of reservoir rocks and seals are studied in terms of mineral composition changes that affect the rock stiffness, stress and strain distributions, and pressure margin to fracture. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Ba Nghiep Nguyen; Hou, Zhangshuan; Bacon, Diana H.; Murray, Christopher J.; White, Mark D.] Pacific NW Natl Lab, POB 999,MSIN J4-55, Richland, WA 99352 USA. RP Nguyen, BN (reprint author), Pacific NW Natl Lab, POB 999,MSIN J4-55, Richland, WA 99352 USA. EM Ba.Nguyen@pnnl.gov RI Hou, Zhangshuan/B-1546-2014; OI Hou, Zhangshuan/0000-0002-9388-6060; Bacon, Diana/0000-0001-9122-5333 FU U.S. Department of Energy (DOE) [DE-AC05-RL01830]; National Energy Technology Laboratory; U.S. DOE, Office of Fossil Energy, National Risk Assessment Partnership; U.S. DOE Office of Vehicle Technologies FX This study was conducted at Pacific Northwest National Laboratory, operated by Battelle for the U.S. Department of Energy (DOE) under Contract DE-AC05-RL01830. Funding for this project was provided by the National Energy Technology Laboratory and U.S. DOE, Office of Fossil Energy as part of the National Risk Assessment Partnership. The initial EMTA development was funded by the U.S. DOE Office of Vehicle Technologies. STOMP-CO2/ABAQUS (R) and STOMP-CO2-R/ABAQUS (R) analyses were performed using PNNL Institutional Computing at Pacific Northwest National Laboratory. NR 64 TC 1 Z9 2 U1 3 U2 11 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1750-5836 EI 1878-0148 J9 INT J GREENH GAS CON JI Int. J. Greenh. Gas Control PD MAR PY 2016 VL 46 BP 100 EP 115 DI 10.1016/j.ijggc.2016.01.004 PG 16 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels; Engineering, Environmental SC Science & Technology - Other Topics; Energy & Fuels; Engineering GA DG1OI UT WOS:000371837000010 ER PT J AU Ma, JL Eason, JP Dowling, AW Biegler, LT Miller, DC AF Ma, Jinliang Eason, John P. Dowling, Alexander W. Biegler, Lorenz T. Miller, David C. TI Development of a first-principles hybrid boiler model for oxy-combustion power generation system SO INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL LA English DT Article DE Boiler model; Oxy-combustion; Pulverized coal combustion; System optimization; Carbon capture; Discrete ordinates method ID COAL COMBUSTION; FLUE-GAS; HEAT INTEGRATION; FUEL COMBUSTION; OPTIMIZATION; PLANTS; COMPRESSION; SIMULATION; SEPARATION; CAPTURE AB The design of an oxy-combustion system for CO2 capture involves the integration of multiple devices including air separation unit, coal-fired boiler, steam turbine, flue gas cleanup, recycle, and compression units. Thousands of design parameters for the entire system need to be optimized to achieve the lowest cost per kilowatt-hour of electricity generated. An appropriate first-principles based boiler model with short computer execution time but yet reasonable accuracy in both air-fired and oxy-fired configurations is highly desired. To this end, a hybrid boiler model with 1-D resolution for main flow and reaction related calculations and 3-D resolution for radiative heat transfer was developed as a part of the oxy-combustion subtask of the Carbon Capture and Simulation Initiative (CCSI) sponsored by U.S. Department of Energy. The developed model is able to automatically generate a 3-D mesh based on user-specified furnace shape for the calculation of radiative heat transfer using discrete ordinates method. The 3-D cells are assigned to individual regions along the furnace height, forming 1-D zones in which conservations of mass and energy in both gas and particle phases are enforced. The kinetics of heterogeneous reactions between char particles and gas reactants are modeled zone by zone in Lagrangian framework. Gas phase chemistry in each zone is simplified based on chemical equilibrium. The submodels for calculating the radiative properties of the gas and particle phases and those for calculating the heterogeneous char reactions are suitable for both air-fired and oxy-fired conditions. A typical boiler model can be converged in approximately 1 min on a personal computer and, therefore, is suitable for the generation of reduced order models in algebraic form which could be used for the large-scale multivariable optimization of the oxy-combustion systems. By modeling a utility boiler in both air-fired and oxy-fired configurations and comparing the results to those from computational fluid dynamics simulations, the hybrid boiler model was found to give very comparable predictions in major boiler performance parameters such as furnace exit gas temperature, heat losses to walls, and unburned carbon in fly ash. By modeling a small test furnace, it was found that with the adjustments on a "mixedness" related effectiveness factor for the char combustion and gasification reactions, the boiler model is able to correctly predict the trends of incident radiation heat flux profile along the furnace axial length as well as the trend of the unburned carbon in both air-fired and oxy-fired configurations. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Ma, Jinliang; Miller, David C.] Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. [Ma, Jinliang] AECOM, 3610 Collins Ferry Rd, Morgantown, WV 26505 USA. [Eason, John P.; Dowling, Alexander W.; Biegler, Lorenz T.] Carnegie Mellon Univ, Dept Chem Engn, Pittsburgh, PA 15289 USA. RP Ma, JL (reprint author), AECOM, 3610 Collins Ferry Rd, Morgantown, WV 26505 USA. EM jinliang.ma@netl.doe.gov FU U.S. Department of Energy, Office of Fossil Energy, Carbon Capture Simulation Initiative (CCSI); National Energy Technology Laboratory's ongoing research under the RES [DE-FE0004000]; agency of the United States Government FX This work was supported by the U.S. Department of Energy, Office of Fossil Energy as part of the Carbon Capture Simulation Initiative (CCSI). This technical effort was performed in support of the National Energy Technology Laboratory's ongoing research under the RES contract DE-FE0004000. This report was prepared as an account of work sponsored by an agency of the United States Government. Neither the United States Government nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof. NR 43 TC 1 Z9 1 U1 8 U2 16 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1750-5836 EI 1878-0148 J9 INT J GREENH GAS CON JI Int. J. Greenh. Gas Control PD MAR PY 2016 VL 46 BP 136 EP 157 DI 10.1016/j.ijggc.2015.12.036 PG 22 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels; Engineering, Environmental SC Science & Technology - Other Topics; Energy & Fuels; Engineering GA DG1OI UT WOS:000371837000012 ER PT J AU Keating, EH Harp, DH Dai, ZX Pawar, RJ AF Keating, Elizabeth H. Harp, Dylan H. Dai, Zhenxue Pawar, Rajesh J. TI Reduced order models for assessing CO2 impacts in shallow unconfined aquifers SO INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL LA English DT Article DE Response surface; CO2 leakage impact; Shallow groundwater quality ID ADAPTIVE REGRESSION SPLINES; CARBON SEQUESTRATION; NEURAL-NETWORK; OPTIMIZATION; LEAKAGE; DESIGN; SITE AB Risk assessment studies of potential CO2 sequestration projects consider many factors, including the possibility of brine and/or CO2 leakage from the storage reservoir. Detailed multiphase reactive transport simulations have been developed to predict the impact of such leaks on shallow groundwater quality; however, these simulations are computationally expensive and thus difficult to directly embed in a probabilistic risk assessment analysis. Here we present a process for developing computationally fast reduced-order models which emulate key features of the more detailed reactive transport simulations. A large ensemble of simulations that take into account uncertainty in aquifer characteristics and CO2/brine leakage scenarios were performed. Twelve simulation outputs of interest were used to develop response surfaces (RSs) using a MARS (multivariate adaptive regression splines) algorithm (Milborrow, 2015). A key part of this study is to compare different measures of ROM accuracy. We show that for some computed outputs, MARS performs very well in matching the simulation data. The capability of the RS to predict simulation outputs for parameter combinations not used in RS development was tested using cross-validation. Again, for some outputs, these results were quite good. For other outputs, however, the method performs relatively poorly. Performance was best for predicting the volume of depressed-pH-plumes, and was relatively poor for predicting organic and trace metal plume volumes. We believe several factors, including the non-linearity of the problem, complexity of the geochemistry, and granularity in the simulation results, contribute to this varied performance. The reduced order models were developed principally to be used in probabilistic performance analysis where a large range of scenarios are considered and ensemble performance is calculated. We demonstrate that they effectively predict the ensemble behavior. However, the performance of the RSs is much less accurate when used to predict time-varying outputs from a single simulation. If an analysis requires only a small number of scenarios to be investigated, computationally expensive physics-based simulations would likely provide more reliable results. If the aggregate behavior of a large number of realizations is the focus, as will be the case in probabilistic quantitative risk assessment, the methodology presented here is relatively robust. Published by Elsevier Ltd. C1 [Keating, Elizabeth H.; Harp, Dylan H.; Dai, Zhenxue; Pawar, Rajesh J.] Los Alamos Natl Lab, Computat Geosci Grp, Earth & Environm Sci Div, MS T003, Los Alamos, NM 87545 USA. RP Keating, EH (reprint author), Los Alamos Natl Lab, Computat Geosci Grp, Earth & Environm Sci Div, MS T003, Los Alamos, NM 87545 USA. EM ekeating@lanl.gov OI Harp, Dylan/0000-0001-9777-8000; Dai, Zhenxue/0000-0002-0805-7621 FU DOE Office of Fossil Energy's Crosscutting Research program FX This research was conducted as part of the Department of Energy's National Risk Assessment Partnership (NRAP). Support for this project came from the DOE Office of Fossil Energy's Crosscutting Research program. We appreciate the very helpful contributions of two anonymous reviewers. NR 33 TC 5 Z9 5 U1 0 U2 5 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1750-5836 EI 1878-0148 J9 INT J GREENH GAS CON JI Int. J. Greenh. Gas Control PD MAR PY 2016 VL 46 BP 187 EP 196 DI 10.1016/j.ijggc.2016.01.008 PG 10 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels; Engineering, Environmental SC Science & Technology - Other Topics; Energy & Fuels; Engineering GA DG1OI UT WOS:000371837000015 ER PT J AU Sun, AY Lu, JM Freifeld, BM Hovorka, SD Islam, A AF Sun, Alexander Y. Lu, Jiemin Freifeld, Barry M. Hovorka, Susan D. Islam, Akand TI Using pulse testing for leakage detection in carbon storage reservoirs: A field demonstration SO INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL LA English DT Article DE Leakage detection; Geological carbon sequestration; Pulse testing; Frequency domain analysis ID GEOLOGIC CO2 STORAGE; SEQUESTRATION SITES; PRESSURE; BRINE; FLOW; CONNECTIVITY; INJECTION; AQUIFER; DESIGN; WELL AB Monitoring techniques capable of deep subsurface detection are desirable for early warning and leakage pathway identification in geologic carbon storage formations. This work demonstrates the feasibility of a pulse-testing-based leakage detection procedure, in which the storage reservoir is stimulated using periodic injection patterns and the acquired pressure perturbation signals are analyzed in the frequency domain to detect potential deviations in the reservoir's frequency domain responses. Unlike the traditional well testing and associated time domain analyses, pulse testing aims to minimize the interference of reservoir operations and other ambient noise by selecting appropriate pulsing frequencies such that reservoir responses to coded injection patterns can be uniquely determined in frequency domain. Field demonstration of this pulse-testing leakage detection technique was carried out at a CO2 enhanced oil recovery site-the Cranfield site located in Mississippi, USA, which has long been used as a carbon storage research site. During the demonstration, two sets of pulsing experiments (baseline and leak tests) were performed using 90-min and 150-min pulsing periods to demonstrate feasibility of time-lapse leakage detection. For leak tests, an artificial leakage source was created through rate-controlled venting of CO2 from one of the monitoring wells because of the lack of known leakage pathways at the site. Our results show that leakage events caused a significant deviation in the amplitude of the frequency response function, indicating that pulse testing may be deployed as a cost-effective active monitoring technique, with a great potential for site-wide automated monitoring. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Sun, Alexander Y.; Lu, Jiemin; Hovorka, Susan D.; Islam, Akand] Univ Texas Austin, Bur Econ Geol, Jackson Sch Geosci, Austin, TX USA. [Freifeld, Barry M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Sun, AY (reprint author), Univ Texas Austin, Bur Econ Geol, Jackson Sch Geosci, Austin, TX USA. EM alex.sun@beg.utexas.edu RI Sun, Alexander/A-9959-2011; Freifeld, Barry/F-3173-2010 FU U.S. Department of Energy, National Energy Technology Laboratory [DE-FE0012231] FX This work was supported by the U.S. Department of Energy, National Energy Technology Laboratory under grant DE-FE0012231. The authors are grateful to the following individuals for their help during the field experiments: Denbury field technicians; Mr. Ramon Trevino, the SECARB project manager at the Bureau of Economic Geology; Mr.Paul Cook and Alex Morales at Lawrence Berkeley National Lab; Mr. Kirk Delaune at Sandia Technologies, LLC; and NETL project manager Mr. Brian Dressel. The authors are thankful to the two reviewers (Drs. Michael Cardiff and Peter Fokker) for their constructive comments during the review of the original manuscript. NR 42 TC 2 Z9 2 U1 3 U2 3 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1750-5836 EI 1878-0148 J9 INT J GREENH GAS CON JI Int. J. Greenh. Gas Control PD MAR PY 2016 VL 46 BP 215 EP 227 DI 10.1016/j.ijggc.2016.01.015 PG 13 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels; Engineering, Environmental SC Science & Technology - Other Topics; Energy & Fuels; Engineering GA DG1OI UT WOS:000371837000018 ER PT J AU Bianchi, M Zheng, LE Birkholzer, JT AF Bianchi, Marco Zheng, Liange Birkholzer, Jens T. TI Combining multiple lower-fidelity models for emulating complex model responses for CCS environmental risk assessment SO INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL LA English DT Article DE Risk assessment; Model; Reduced order model; Groundwater; Surrogate modeling ID GLOBAL OPTIMIZATION; NEURAL-NETWORK; DESIGN OPTIMIZATION; SURROGATE FUNCTIONS; ENGINEERING DESIGN; COMPUTER CODE; SIMULATION; MANAGEMENT; APPROXIMATIONS; CALIBRATION AB Numerical modeling is essential to support natural resource management and environmental policy making. In the context of CO2 geological sequestration, these models are indispensible parts of risk assessment tools. However, because of increasing complexity, modern numerical models require a great computational effort, which in some cases may be infeasible. An increasingly popular approach to overcome computational limitations is the use of surrogate models. This paper presents a new surrogate modeling approach to reduce the computational cost of running a complex, high-fidelity model. The approach is based on the simplification the high-fidelity model into computationally efficient, lower fidelity models and on linking them with a mathematical function (linking function) that addresses the discrepancies between outputs from models with different levels of fidelity. The resulting linking function model, which can be developed with small computational effort, can be efficiently used in numerical applications where multiple runs of the original high-fidelity model are required, such as for uncertainty quantification or sensitivity analysis. The proposed approach was then applied to the development of a reduced order model for the prediction of groundwater quality impacts from CO2 and brine leakage for the National Risk Assessment Partnership (NRAP) project. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Bianchi, Marco; Zheng, Liange; Birkholzer, Jens T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Geosci Div, Berkeley, CA 94720 USA. [Bianchi, Marco] British Geol Survey, Ctr Environm Sci, Keyworth NG12 5GG, Notts, England. RP Zheng, LE (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Geosci Div, Berkeley, CA 94720 USA. EM LZheng@lbl.gov RI Birkholzer, Jens/C-6783-2011; zheng, liange/B-9748-2011 OI Birkholzer, Jens/0000-0002-7989-1912; zheng, liange/0000-0002-9376-2535 FU Assistant Secretary for Fossil Energy of the U.S. Department of Energy; National Energy Technology Laboratory of the U.S. Department of Energy; National Risk Assessment Partnership of the U.S. Department of Energy [DEACO2-05CH11231] FX This work was funded by the Assistant Secretary for Fossil Energy, National Energy Technology Laboratory, National Risk Assessment Partnership, of the U.S. Department of Energy under Contract No. DEACO2-05CH11231. The Guest Editor Susan Carrot and two anonymous reviewers are grateful acknowledged for their comments, which helped improving the final version of the manuscript. NR 69 TC 3 Z9 3 U1 4 U2 15 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1750-5836 EI 1878-0148 J9 INT J GREENH GAS CON JI Int. J. Greenh. Gas Control PD MAR PY 2016 VL 46 BP 248 EP 258 DI 10.1016/j.ijggc.2016.01.009 PG 11 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels; Engineering, Environmental SC Science & Technology - Other Topics; Energy & Fuels; Engineering GA DG1OI UT WOS:000371837000021 ER PT J AU Cotton, SJ Miller, WH AF Cotton, Stephen J. Miller, William H. TI The Symmetrical Quasi-Classical Model for Electronically Non-Adiabatic Processes Applied to Energy Transfer Dynamics in Site-Exciton Models of Light-Harvesting Complexes SO JOURNAL OF CHEMICAL THEORY AND COMPUTATION LA English DT Article ID QUANTUM COHERENCE AB In a recent series of papers, "it has been illustrated that a symmetrical quasi-classical (SQC) windowing model applied to the Meyer Miller (MM) classical vibronic Hamiltonian provides an excellent description of a variety of electronically non-adiabatic benchmark model systems for which exact quantum results are available for comparison. In this paper, the SQC/MM approach is used to treat energy transfer dynamics in site-exciton models of light-harvesting complexes, and in particular, the well-known 7-state Fenna Mathews-Olson (FMO) complex. Again, numerically "exact" results are available for comparison, here via the hierarchical equation of motion (HEOM) approach of Ishizaki and Fleming, and it is seen that the simple SQC/MM pproach provides very reasonable agreement with the "previous HEOM results. It is noted, however, that unlike most (if not all) simple approaches for treating these systems, because the SQC/MM approach presents a fully atomistic simulation based on classical trajectory simulation, it places no restrictions on the characteristics of the thermal baths coupled to each two-level site, e.g., bath spectral densities (SD) of any analytic functional form may be employed as well as discrete SD determined experimentally or from MD simulation (nor is there any restriction that the baths be harmonic), opening up the possibility of simulating more realistic variations on the basic site-exciton framework for describing the non-adiabatic dynamics of photosynthetic pigment complexes. C1 [Cotton, Stephen J.; Miller, William H.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Cotton, Stephen J.; Miller, William H.] Univ Calif Berkeley, Kenneth S Pitzer Ctr Theoret Chem, Berkeley, CA 94720 USA. [Cotton, Stephen J.; Miller, William H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Cotton, SJ; Miller, WH (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Cotton, SJ; Miller, WH (reprint author), Univ Calif Berkeley, Kenneth S Pitzer Ctr Theoret Chem, Berkeley, CA 94720 USA.; Cotton, SJ; Miller, WH (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM StephenJCotton47@gmail.com; MillerWH@berkeley.edu FU National Science Foundation [CHE-1464647]; Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division, U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX S.J.C. thanks Dr. Jan Roden of the Whaley Research Group at Berkeley for useful and inspiring discussions relating to the site-exciton model of the FMO complex as well as other site-exciton models, and moreover, the types of questions one may begin to ask and answer with trajectory-based methods for treating these systems. S.J.C. also thanks Professor Akihito Ishizaki for providing the HEOM results from refs 8 and 9. This work was supported by the National Science Foundation under Grant No. CHE-1464647 and by the Director, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division, U.S. Department of Energy under Contract No. DE-AC02-05CH11231. In addition, this research utilized computation resources provided by the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 14 TC 7 Z9 7 U1 8 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1549-9618 EI 1549-9626 J9 J CHEM THEORY COMPUT JI J. Chem. Theory Comput. PD MAR PY 2016 VL 12 IS 3 BP 983 EP 991 DI 10.1021/acs.jctc.5b01178 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DG1UF UT WOS:000371852300008 PM 26761191 ER PT J AU Apra, E Kowalski, K AF Apra, E. Kowalski, K. TI Implementation of High-Order Multireference Coupled-Cluster Methods on Intel Many Integrated Core Architecture SO JOURNAL OF CHEMICAL THEORY AND COMPUTATION LA English DT Article ID GRAPHICAL PROCESSING UNITS; MOLECULAR-DYNAMICS SIMULATIONS; QUANTUM-CHEMISTRY CALCULATIONS; DENSITY-FUNCTIONAL THEORY; WAVE-FUNCTION ANSATZ; BRILLOUIN-WIGNER; CONFIGURATION-INTERACTION; CONTINUOUS TRANSITION; EXCITED-STATES; MODEL SYSTEMS AB In this paper we discuss the implementation of multireference coupled-cluster formalism with singles, doubles, and noniterative triples (MRCCSD(T)), which is capable of taking advantage of the processing power of the Intel Xeon Phi coprocessor. We discuss the integration of two levels of parallelism underlying the MRCCSD(T) implementation with computational kernels designed to offload the computationally intensive parts of the MRCCSD(T) formalism to Intel Xeon Phi coprocessors. Special attention is given to the enhancement of the parallel performance by task reordering that has improved load balancing in the noniterative part of the MRCCSD(T) calculations. We also discuss aspects regarding efficient optimization and vectorization strategies. C1 [Apra, E.; Kowalski, K.] Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, K8-91,POB 999, Richland, WA 99352 USA. RP Apra, E; Kowalski, K (reprint author), Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, K8-91,POB 999, Richland, WA 99352 USA. EM edoardo.apra@pnnl.gov; karol.kowalski@pnnl.gov RI Apra, Edoardo/F-2135-2010 OI Apra, Edoardo/0000-0001-5955-0734 FU Intel Parallel Computational Centers program; Department of Energy's Office of Biological and Environmental Research; US Department of Energy [DE-AC06.76RLO-1830] FX This work has been supported by the Intel Parallel Computational Centers program. All calculations have been performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. The Pacific Northwest National Laboratory is operated for the US Department of Energy by the Battelle Memorial Institute under Contract No. DE-AC06.76RLO-1830. NR 103 TC 1 Z9 1 U1 3 U2 10 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1549-9618 EI 1549-9626 J9 J CHEM THEORY COMPUT JI J. Chem. Theory Comput. PD MAR PY 2016 VL 12 IS 3 BP 1129 EP 1138 DI 10.1021/acs.jctc.5b00957 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DG1UF UT WOS:000371852300020 PM 26808463 ER PT J AU Collier, SM Dean, AP Oates, LG Ruark, MD Jackson, RD AF Collier, Sarah M. Dean, Andrew P. Oates, Lawrence G. Ruark, Matthew D. Jackson, Randall D. TI Does Plant Biomass Manipulation in Static Chambers Affect Nitrous Oxide Emissions from Soils? SO JOURNAL OF ENVIRONMENTAL QUALITY LA English DT Article ID FLUX; DENITRIFICATION; NITRIFICATION; N2O AB One of the most widespread approaches for measurement of greenhouse gas emissions from soils involves the use of static chambers. This method is relatively inexpensive, is easily replicated, and is ideally suited to plot-based experimental systems. Among its limitations is the loss of detection sensitivity with increasing chamber height, which creates challenges for deployment in systems including tall vegetation. It is not always possible to avoid inclusion of plants within chambers or to extend chamber height to fully accommodate plant growth. Thus, in many systems, such as perennial forages and biomass crops, plants growing within static chambers must either be trimmed or folded during lid closure. Currently, data on how different types of biomass manipulation affect measured results is limited. Here, we compare the effects of cutting vs. folding of biomass on nitrous oxide measurements in switchgrass (Panicum virgatum L.) and alfalfa (Medicago sativa L.) systems. We report only limited evidence of treatment effects during discrete sampling events and little basis for concern that effects may intensify over time as biomass manipulation is repeatedly imposed. However, nonsignificant treatment effects that were consistently present amounted to significant overall trends in three out of the four systems studied. Such minor disparities in flux could amount to considerable quantities over time, suggesting that caution should be exercised when comparing cumulative emission values from studies using different biomass manipulation strategies. C1 [Collier, Sarah M.] Univ Wisconsin, Off Sustainabil, Madison, WI 53706 USA. [Collier, Sarah M.; Ruark, Matthew D.] Univ Wisconsin, Dept Soil Sci, Madison, WI 53706 USA. [Dean, Andrew P.; Oates, Lawrence G.; Jackson, Randall D.] Univ Wisconsin, DOE Great Lakes Bioenergy Res Ctr, Madison, WI 53706 USA. [Oates, Lawrence G.; Jackson, Randall D.] Univ Wisconsin, Dept Agron, 1575 Linden Dr, Madison, WI 53706 USA. RP Oates, LG (reprint author), Univ Wisconsin, DOE Great Lakes Bioenergy Res Ctr, Madison, WI 53706 USA.; Oates, LG (reprint author), Univ Wisconsin, Dept Agron, 1575 Linden Dr, Madison, WI 53706 USA. EM oates@wisc.edu OI Oates, Lawrence/0000-0003-4829-7600; Collier, Sarah/0000-0002-8834-5075 FU National Science Foundation [1215858]; USDA [2013-68002-20525]; US Department of Energy Great Lakes Bioenergy Research Center-DOE BER Office of Science [DE-FC02-07ER64494]; DOE OBP Office of Energy Efficiency and Renewable Energy [DE-AC05-76RL01830] FX This material is based on work supported by the National Science Foundation under Grant Number 1215858, by the USDA under Grant Number 2013-68002-20525, and by the US Department of Energy Great Lakes Bioenergy Research Center-DOE BER Office of Science (DE-FC02-07ER64494) and DOE OBP Office of Energy Efficiency and Renewable Energy (DE-AC05-76RL01830). The authors thank Nicholas Keuler at the University of Wisconsin-Madison CALS Statistical Consulting Group and David Duncan for statistical consultation and two anonymous reviewers for input that greatly improved this manuscript. NR 24 TC 0 Z9 0 U1 6 U2 16 PU AMER SOC AGRONOMY PI MADISON PA 677 S SEGOE RD, MADISON, WI 53711 USA SN 0047-2425 EI 1537-2537 J9 J ENVIRON QUAL JI J. Environ. Qual. PD MAR-APR PY 2016 VL 45 IS 2 BP 751 EP 756 DI 10.2134/jeq2015.07.0377 PG 6 WC Environmental Sciences SC Environmental Sciences & Ecology GA DG1AR UT WOS:000371797900040 PM 27065424 ER PT J AU Batlle, JVI Beresford, NA Beaugelin-Seiller, K Bezhenar, R Brown, J Cheng, JJ Cujic, M Dragovic, S Duffa, C Fievet, B Hosseini, A Jung, KT Kamboj, S Keum, DK Kryshev, A LePoire, D Maderich, V Min, BI Perianez, R Sazykina, T Suh, KS Yu, C Wang, C Heling, R AF Vives i Batlle, J. Beresford, N. A. Beaugelin-Seiller, K. Bezhenar, R. Brown, J. Cheng, J. -J. Cujic, M. Dragovic, S. Duffa, C. Fievet, B. Hosseini, A. Jung, K. T. Kamboj, S. Keum, D. -K. Kryshev, A. LePoire, D. Maderich, V. Min, B. -I. Perianez, R. Sazykina, T. Suh, K-S. Yu, C. Wang, C. Heling, R. TI Inter-comparison of dynamic models for radionuclide transfer to marine biota in a Fukushima accident scenario SO JOURNAL OF ENVIRONMENTAL RADIOACTIVITY LA English DT Article DE Dynamic model; Dose rate; Fukushima; Marine biota; Radionuclide transfer; MODARIA ID ABSORBED DOSE-RATES; NONHUMAN BIOTA; NUCLEAR ACCIDENT; DISPERSION; CS-137; PLANT; ENVIRONMENT; EXPOSURE; WILDLIFE; PACIFIC AB We report an inter-comparison of eight models designed to predict the radiological exposure of radionuclides in marine biota. The models were required to simulate dynamically the uptake and turnover of radionuclides by marine organisms. Model predictions of radionuclide uptake and turnover using kinetic calculations based on biological half-life (T-B1/2) and/or more complex metabolic modelling approaches were used to predict activity concentrations and, consequently, dose rates of Sr-90, I-131 and Cs-137 to fish, crustaceans, macroalgae and molluscs under circumstances where the water concentrations are changing with time. For comparison, the ERICA Tool, a model commonly used in environmental assessment, and which uses equilibrium concentration ratios, was also used. As input to the models we used hydrodynamic forecasts of water and sediment activity concentrations using a simulated scenario reflecting the Fukushima accident releases. Although model variability is important, the intercomparison gives logical results, in that the dynamic models predict consistently a pattern of delayed rise of activity concentration in biota and slow decline instead of the instantaneous equilibrium with the activity concentration in seawater predicted by the ERICA Tool. The differences between ERICA and the dynamic models increase the shorter the T-B1/2 becomes; however, there is significant variability between models, underpinned by parameter and methodological differences between them. The need to validate the dynamic models used in this intercomparison has been highlighted, particularly in regards to optimisation of the model biokinetic parameters. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Vives i Batlle, J.] Belgian Nucl Res Ctr SCK CEN, Boeretang 200, B-2400 Mol, Belgium. [Beresford, N. A.] NERC Ctr Ecol & Hydrol, Lib Ave, Lancaster LA1 4AP, England. [Beaugelin-Seiller, K.; Duffa, C.; Fievet, B.] PRP ENV, IRSN, Paris, France. [Bezhenar, R.; Maderich, V.] Inst Math Machine & Syst Problems, Glushkov Ave 42, UA-03187 Kiev, Ukraine. [Brown, J.; Hosseini, A.] Norwegian Radiat Protect Author, Grini Naeringspk 13,POB 55, NO-1332 Osteras, Norway. [Cheng, J. -J.; Kamboj, S.; LePoire, D.; Yu, C.; Wang, C.] Argonne Natl Lab, Div Environm Sci, 9700 South Cass Ave,EVS Bldg 240, Argonne, IL 60439 USA. [Cujic, M.] Univ Belgrade, Inst Applicat Nucl Energy, Banatska 31b, Belgrade 11080, Serbia. [Dragovic, S.] Univ Belgrade, Vinca Inst Nucl Sci, POB 522, Belgrade, Serbia. [Jung, K. T.] Korea Inst Ocean Sci & Technol, 787 Haean Ro, Ansan 426744, South Korea. [Keum, D. -K.; Min, B. -I.; Suh, K-S.] Korea Atom Energy Res Inst, 150 Deokjindong,POB 105, Daejeon 305353, South Korea. [Kryshev, A.; Sazykina, T.] Res & Prod Assoc Typhoon, 4 Pobedy Str, Obninsk 249038, Kaluga Region, Russia. [Perianez, R.] Univ Seville, Dept Fis Aplicada 1, Carretera Utrera Km 1, Seville 41013, Spain. [Heling, R.] NRG, Utrechtseweg 310, NL-6800 ES Arnhem, Netherlands. RP Batlle, JVI (reprint author), Belgian Nucl Res Ctr SCK CEN, Boeretang 200, B-2400 Mol, Belgium. EM jordi.vives.i.batlle@sckcen.be RI Beresford, Nicholas/I-6188-2012; Perianez, Raul/F-5710-2010; OI Maderich, Vladimir/0000-0003-3143-0727 NR 54 TC 4 Z9 4 U1 7 U2 25 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0265-931X EI 1879-1700 J9 J ENVIRON RADIOACTIV JI J. Environ. Radioact. PD MAR PY 2016 VL 153 BP 31 EP 50 DI 10.1016/j.jenvrad.2015.12.006 PG 20 WC Environmental Sciences SC Environmental Sciences & Ecology GA DG3BO UT WOS:000371944700005 ER PT J AU Xu, C Zhang, S Sugiyama, Y Ohte, N Ho, YF Fujitake, N Kaplan, DI Yeager, CM Schwehr, K Santschi, PH AF Xu, Chen Zhang, Saijin Sugiyama, Yuko Ohte, Nobuhito Ho, Yi-Fang Fujitake, Nobuhide Kaplan, Daniel I. Yeager, Chris M. Schwehr, Kathleen Santschi, Peter H. TI Role of natural organic matter on iodine and (PU)-P-239,240 distribution and mobility in environmental samples from the northwestern Fukushima Prefecture, Japan SO JOURNAL OF ENVIRONMENTAL RADIOACTIVITY LA English DT Article DE Fukushima Prefecture; Iodine; Iodide; Iodate; Organo-iodine; Speciation; Plutonium; Isotopic ratio; Cesium; pH; Eh; Soil organic matter (SOM); Nitrogen-containing organic compounds; Deciduous forest; Coniferous forest; Urban; Paddy; Stemwater; Throughfall; Bulk deposition ID NUCLEAR-POWER-PLANT; SAVANNA RIVER SITE; K-EDGE XANES; HYDROXAMATE SIDEROPHORES; RADIOIODINE I-129; MASS-SPECTROMETRY; STABLE IODINE; SPECIATION; SOILS; ACCIDENT AB In order to assess how environmental factors are affecting the distribution and migration of radioiodine and plutonium that were emitted from the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) accident, we quantified iodine and Pu-239,Pu-240 concentration changes in soil samples with different land uses (urban, paddy, deciduous forest and coniferous forest), as well as iodine speciation in surface water and rainwater. Sampling locations were 53-63 km northwest of the FDNPP within a 75-km radius, in close proximity of each other. A ranking of the land uses by their surface soil (<4 cm) stable I-127 concentrations was coniferous forest > deciduous forest > urban > paddy, and Pu-239,Pu-240 concentrations ranked as deciduous forest > coniferous forest > paddy > urban. Both were quite distinct from that of Cs-134 and Cs-137: urban > coniferous forest > deciduous forest > paddy, indicating differences in their sources, deposition phases, and biogeochemical behavior in these soil systems. Although stable I-127 might not have fully equilibrated with Fukushima-derived I-129, it likely still works as a proxy for the long-term fate of I-129. Surficial soil I-127 content was well correlated to soil organic matter (SOM) content, regardless of land use type, suggesting that SOM might be an important factor affecting iodine biogeochemistry. Other soil chemical properties, such as Eh and pH, had strong correlations to soil I-127 content, but only within a given land use (e.g., within urban soils). Organic carbon (OC) concentrations and Eh were positively, and pH was negatively correlated to I-127 concentrations in surface water and rain samples. It is also noticeable that I-127 in the wet deposition was concentrated in both the deciduous and coniferous forest throughfall and stemfall water, respectively, comparing to the bulk rainwater. Further, both forest throughfall and stemflow water consisted exclusively of organo-iodine, suggesting all inorganic iodine in the original bulk deposition (similar to 28.6% of total iodine) have been completely converted to organo-iodine. Fukushima-derived Pu-239,Pu-240 was detectable at a distance similar to 61 km away, NW of FDNPP. However, it is confined to the litter layer, even three years after the FDNPP accident-derived emissions. Plutonium-239,240 activities were significantly correlated with soil OC and nitrogen contents, indicating Pu may be associated with nitrogen-containing SOM, similar to what has been observed at other locations in the United States. Together, these finding suggest that natural organic matter (NOM) plays a key role in affecting the fate and transport of I and Pu and may warrant greater consideration for predicting long-term stewardship of contaminated areas and evaluating various remediation options in Japan. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Xu, Chen; Zhang, Saijin; Ho, Yi-Fang; Schwehr, Kathleen; Santschi, Peter H.] Texas A&M Univ, Lab Environm & Oceanog Res, Dept Marine Sci, Bldg 3029, Galveston, TX 77551 USA. [Sugiyama, Yuko] Univ Hyogo, Sch Human Sci & Environm, 1-1-12 Shinzaike Honcho, Himeji, Hyogo 6700092, Japan. [Ohte, Nobuhito] Kyoto Univ, Grad Sch Informat, Dept Social Informat, Kyoto 6068501, Japan. [Fujitake, Nobuhide] Kobe Univ, Grad Sch Agr Sci, Div Agroenvironm Biol, Nada Ku, 1-1 Rokkodai, Kobe, Hyogo 6578501, Japan. [Kaplan, Daniel I.] Savannah River Natl Lab, Aiken, SC 29808 USA. [Yeager, Chris M.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Xu, C (reprint author), Texas A&M Univ, Lab Environm & Oceanog Res, Dept Marine Sci, Bldg 3029, Galveston, TX 77551 USA. EM xuchen66@tamu.edu FU U.S. Department of Energy (DOE) Office of Science - Subsurface Biogeochemistry Research program [ER65222-1038426-0017532]; DOE [DE-ER64567-1031562-0014364, DE-SC0014152, DE-AD09-96SR18500]; JSPS; River Foundation (Kasen Zaidan, Japan); [24248027] FX This work was funded by the U.S. Department of Energy (DOE) Office of Science - Subsurface Biogeochemistry Research program (ER65222-1038426-0017532), DOE SBR grant #DE-ER64567-1031562-0014364, DOE SBR award # DE-SC0014152, and DOE contract DE-AD09-96SR18500. Yuko Sugiyama was supported by JSPS Bilateral Joint Research Projects with USA and Grants-in-Aid for Scientific Research #24248027. Nobuhito Ohte was partly supported by a grant for River Management Research (FY2014, 2015) from the River Foundation (Kasen Zaidan, Japan). We really appreciate the Associate Editor Prof. Dr. Shun-ichi Hisamatsu and two anonymous reviewers for their constructive comments that have greatly improved the manuscript. NR 78 TC 1 Z9 1 U1 11 U2 33 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0265-931X EI 1879-1700 J9 J ENVIRON RADIOACTIV JI J. Environ. Radioact. PD MAR PY 2016 VL 153 BP 156 EP 166 PG 11 WC Environmental Sciences SC Environmental Sciences & Ecology GA DG3BO UT WOS:000371944700019 PM 26773510 ER PT J AU Burnett, JL Miley, HS Milbrath, BD AF Burnett, Jonathan L. Miley, Harry S. Milbrath, Brian D. TI Radionuclide observables during the Integrated Field Exercise of the Comprehensive Nuclear-Test-Ban Treaty SO JOURNAL OF ENVIRONMENTAL RADIOACTIVITY LA English DT Article DE Integrated Field Exercise; OSI; CTBT ID GAMMA-SPECTROMETRY; IN-SITU; VALIDATION; CS-137; SOIL AB In 2014 the Preparatory Commission for the Comprehensive Nuclear-Test-Ban Treaty Organization (CTBTO) undertook an Integrated Field Exercise (IFE14) in Jordan. The exercise consisted of a simulated 0.5-2 kT underground nuclear explosion triggering an On-site Inspection (OSI) to search for evidence of a Treaty violation. This research paper evaluates two of the OSI techniques used during the IFE14, laboratory-based gamma-spectrometry of soil samples and in-situ gamma-spectrometry, both of which were implemented to search for 17 OSI relevant particulate radionuclides indicative of nuclear explosions. The detection sensitivity is evaluated using real IFE and model data. It indicates that higher sensitivity laboratory measurements are the optimum technique during the IFE and within the Treaty/Protocol-specified OSI timeframes. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Burnett, Jonathan L.; Miley, Harry S.; Milbrath, Brian D.] Pacific NW Natl Lab, POB 999, Richland, WA 99352 USA. RP Burnett, JL (reprint author), Pacific NW Natl Lab, POB 999, Richland, WA 99352 USA. EM jonathan.burnett@pnnl.gov FU U.S. Department of Energy [DE-AC05-76RL01830] FX The authors thank the IFE14 host country, the Hashemite Kingdom of Jordan, for making this data available, and the Provisional Technical Secretariat (PTS) for providing IFE data and support, and particularly Dr. Xavier Blanchard of the PTS staff for detailed explanations on how to interpret the in-situ reported values. Further, the authors thank the National Oceanic and Atmospheric Administration (NOAA) Air Resources Laboratory (ARL) for the provision of the HYSPLIT transport and dispersion model and Real-time Environmental Applications and Display sYstem (READY) website (http://www.ready.noaa.gov) used in this research. The views expressed here do not necessarily reflect the opinion of the United States Government, the United States Department of Energy, or the Pacific Northwest National Laboratory. Pacific Northwest National Laboratory is operated for the U.S. Department of Energy by Battelle under Contract DE-AC05-76RL01830. NR 31 TC 1 Z9 1 U1 2 U2 3 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0265-931X EI 1879-1700 J9 J ENVIRON RADIOACTIV JI J. Environ. Radioact. PD MAR PY 2016 VL 153 BP 195 EP 200 DI 10.1016/j.jenvrad.2016.01.002 PG 6 WC Environmental Sciences SC Environmental Sciences & Ecology GA DG3BO UT WOS:000371944700023 PM 26802699 ER PT J AU Fahey, AJ Perea, DE Bartrand, J Arey, BW Thevuthasan, S AF Fahey, Albert J. Perea, Daniel E. Bartrand, Jonah Arey, Bruce W. Thevuthasan, Suntharampillai TI Uranium isotopic ratio measurements of U3O8 reference materials by atom probe tomography SO JOURNAL OF ENVIRONMENTAL RADIOACTIVITY LA English DT Article DE Atom probe tomography; Uranium; Isotopic ratios ID DEPLETED URANIUM AB We report results of measurements of isotopic ratios obtained with atom probe tomography on U3O8 reference materials certified for their isotopic abundances of uranium. The results show good agreement with the certified values. High backgrounds due to tails from adjacent peaks complicate the measurement of the integrated peak areas as well as the fact that only oxides of uranium appear in the spectrum, the most intense of which is doubly charged. In addition, lack of knowledge of other instrumental parameters, such as the dead time, may bias the results. Isotopic ratio measurements can be performed at the nanometer-scale with the expectation of sensible results. The abundance sensitivity and mass resolving power of the mass spectrometer are not sufficient to compete with magnetic-sector instruments but are not far from measurements made by ToF-SIMS of other isotopic systems. The agreement of the major isotope ratios is more than sufficient to distinguish most anthropogenic compositions from natural. Published by Elsevier Ltd. C1 [Fahey, Albert J.] Naval Res Lab, 4555 Overlook Ave SW, Washington, DC 20375 USA. [Perea, Daniel E.; Bartrand, Jonah; Arey, Bruce W.; Thevuthasan, Suntharampillai] Pacific NW Natl Lab, Environm Mol Sci Lab, 902 Battelle Blvd,POB 999,MS J4-70, Richland, WA 99352 USA. RP Fahey, AJ (reprint author), Naval Res Lab, 4555 Overlook Ave SW, Washington, DC 20375 USA. EM albert.fahey@nrl.navy.mil NR 17 TC 1 Z9 1 U1 3 U2 9 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0265-931X EI 1879-1700 J9 J ENVIRON RADIOACTIV JI J. Environ. Radioact. PD MAR PY 2016 VL 153 BP 206 EP 213 DI 10.1016/j.jenvrad.2015.12.018 PG 8 WC Environmental Sciences SC Environmental Sciences & Ecology GA DG3BO UT WOS:000371944700025 PM 26774651 ER PT J AU Xie, XJ Liu, YQ Pi, KF Liu, CX Li, JX Duan, MY Wang, YX AF Xie, Xianjun Liu, Yaqing Pi, Kunfu Liu, Chongxuan Li, Junxia Duan, Mengyu Wang, Yanxin TI In situ Fe-sulfide coating for arsenic removal under reducing conditions SO JOURNAL OF HYDROLOGY LA English DT Article DE Iron sulfides; Arsenic contamination; Groundwater; In situ remediation; Reducing conditions ID CONTAMINATED GROUNDWATER; BANGLADESH GROUNDWATER; AQUEOUS-SOLUTION; IRON-OXIDES; REMEDIATION; WATER; SORPTION; HEALTH; MACKINAWITE; PYRITE AB An in situ Fe-sulfide coating approach has been developed for As-contaminated groundwater remediation. Alternate injection of Fe(II), O-2-free water and S2- can realize Fe-sulfide coating onto quartz sands with minor changes in porosity. As(III) uptake experiment indicated that the retardation factor for As(III) was 37 and dynamic retention capacity was 44.94 mg As(III)/g Fe, which was much higher than the maximum adsorption capacity for As(III) by FeS and FeS2. This result indicated that adsorption cannot be the only mechanism for As(III) uptake by Fe-sulfide coating layer. The SEM image and FTIR spectra results suggested that interaction between As(III) and Fe-sulfides and formation of As-sulfide precipitates could significantly contribute to As(III) uptake by Fe-sulfide coating layer. Alternate injection of Fe(II) + As (III) and S2- was conducted to simulate in situ As immobilization from real groundwater. The SEM image showed that the quartz sands were mainly covered by crystalline framboidal pyrite after such amendment. The breakthrough of As(III) was not observed during this experiment and the removal capacity for As(III) was 109.7 mg As/g Fe. The As(III) immobilization mechanism during alternate injection of Fe (II) + As(III) and S2- was significantly different from that of As(III) uptake by Fe-sulfide coating. The direct interaction between As(III) and S2- produced As-iulfides contributed to the high As(III) removal capacity during alternate injection of Fe(II) + As(III) and S2-. This result indicated that alternate injection of Fe(II) and S-2-approach has an attractive application for As-contaminated groundwater remediation under strongly reducing environment. 2016 Elsevier B.V. All rights reserved. C1 [Xie, Xianjun; Liu, Yaqing; Pi, Kunfu; Liu, Chongxuan; Li, Junxia; Duan, Mengyu; Wang, Yanxin] China Univ Geosci, State Key Lab Biogeol & Environm Geol, Wuhan 430074, Peoples R China. [Xie, Xianjun; Liu, Yaqing; Pi, Kunfu; Liu, Chongxuan; Li, Junxia; Duan, Mengyu; Wang, Yanxin] China Univ Geosci, Sch Environm Studies, Wuhan 430074, Peoples R China. [Liu, Chongxuan] Pacific NW Natl Lab, Richland, WA 99354 USA. RP Xie, XJ; Wang, YX (reprint author), China Univ Geosci, State Key Lab Biogeol & Environm Geol, Wuhan 430074, Peoples R China.; Xie, XJ; Wang, YX (reprint author), China Univ Geosci, Sch Environm Studies, Wuhan 430074, Peoples R China. EM xjxie@cug.edu.cn; yx.wang@cug.edu.cn RI Liu, Chongxuan/C-5580-2009 FU National Natural Science Foundation of China [41521001, 41202168, 41372254]; Ministry of Science and Technology of China [2012AA062602]; Fundamental Research Fund for National Universities, China University of Geosciences (Wuhan) FX This research was financially supported by the National Natural Science Foundation of China (Nos. 41521001, 41202168 and 41372254), the Ministry of Science and Technology of China (2012AA062602), and the Fundamental Research Fund for National Universities, China University of Geosciences (Wuhan). NR 44 TC 3 Z9 3 U1 21 U2 52 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-1694 EI 1879-2707 J9 J HYDROL JI J. Hydrol. PD MAR PY 2016 VL 534 BP 42 EP 49 DI 10.1016/j.jhydrol.2015.12.057 PG 8 WC Engineering, Civil; Geosciences, Multidisciplinary; Water Resources SC Engineering; Geology; Water Resources GA DG3AC UT WOS:000371940900005 ER PT J AU Harms, PA Visser, A Moran, JE Esser, BK AF Harms, Patrick A. Visser, Ate Moran, Jean E. Esser, Brad K. TI Distribution of tritium in precipitation and surface water in California SO JOURNAL OF HYDROLOGY LA English DT Article DE Tritium; Precipitation; Surface water; Residence time ID MODIFIED GLOBAL-MODEL; GROUNDWATER RECHARGE; RESIDENCE TIMES; FLOW; AGE AB The tritium concentration in the surface hydrosphere throughout California was characterized to examine the reasons for spatial variability and to enhance the applicability of tritium in hydrological investigations. Eighteen precipitation samples were analyzed and 148 samples were collected from surface waters across California in the Summer and Fall of 2013, with repeat samples from some locations collected in Winter and Spring of 2014 to examine seasonal variation. The concentration of tritium in present day precipitation varied from 4.0 pCi/L near the California coast to 17.8 pCi/L in the Sierra Nevada Mountains. Concentrations in precipitation increase in spring due to the 'Spring Leak' phenomenon. The average coastal concentration (6.3 +/- 1.2 pCi/L) in precipitation matches estimated pre-nuclear levels. Surface water samples show a trend of increasing tritium with inland distance. Superimposed on that trend, elevated tritium concentrations are found in the San Francisco Bay area compared to other coastal areas, resulting from municipal water imported from inland mountain sources and local anthropogenic sources. Tritium concentrations in most surface waters decreased between Summer/Fall 2013 and Winter/Spring 2014 likely due to an increased groundwater signal as a result of drought conditions in 2014. A relationship between tritium and electrical conductivity in surface water was found to be indicative of water provenance and anthropogenic influences such as agricultural runoff. Despite low initial concentrations in precipitation, tritium continues to be a valuable tracer in a post nuclear bomb pulse world. (C) 2016 Elsevier B.V. All rights reserved. C1 [Harms, Patrick A.; Visser, Ate; Esser, Brad K.] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. [Moran, Jean E.] Calif State Univ East Bay, 25800 Carlos Bee Blvd, Hayward, CA 94542 USA. RP Visser, A (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. EM visser3@llnl.gov RI Visser, Ate/G-8826-2012; OI Harms, Patrick/0000-0003-0716-0026; Moran, Jean/0000-0002-1749-804X FU Lawrence Livermore National Laboratory [DE-AC52-07NA27344. LLNL-JRNL-676467] FX This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. LLNL-JRNL-676467. NR 34 TC 4 Z9 4 U1 9 U2 23 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-1694 EI 1879-2707 J9 J HYDROL JI J. Hydrol. PD MAR PY 2016 VL 534 BP 63 EP 72 DI 10.1016/j.jhydrol.2015.12.046 PG 10 WC Engineering, Civil; Geosciences, Multidisciplinary; Water Resources SC Engineering; Geology; Water Resources GA DG3AC UT WOS:000371940900007 ER PT J AU Du, EH Jackson, CR Klaus, J McDonnell, JJ Griffiths, NA Williamson, MF Greco, JL Bitew, M AF Du, Enhao Jackson, C. Rhett Klaus, Julian McDonnell, Jeffrey J. Griffiths, Natalie A. Williamson, Margaret F. Greco, James L. Bitew, Menberu TI Interflow dynamics on a low relief forested hillslope: Lots of fill, little spill SO JOURNAL OF HYDROLOGY LA English DT Article DE Interflow; Argillic layer; Low relief; Fill-and-spill ID GENERATION PROCESSES; RUNOFF GENERATION; SUBSURFACE FLOW; SOIL-LAYER; CATCHMENT; HYDROLOGY; WATER; TOPOGRAPHY; STREAMFLOW; STORAGE AB We evaluated the occurrence of perching and interflow over and within a sandy clay loam argillic horizon within first-order, low-relief, forested catchments at the Savannah River Site (SRS) in the Upper Coastal Plain of South Carolina. We measured soil hydraulic properties, depths to the argillic layer, soil moisture, shallow groundwater behavior, interflow interception trench flows, and streamflow over a 4-year period to explore the nature and variability of soil hydraulic characteristics, the argillic "topography", and their influence on interflow generation. Perching occurred frequently within and above the restricting argillic horizons during our monitoring period, but interflow was infrequent due to microtopographic relief and associated depression storage on the argillic layer surface. High percolation rates through the argillic horizon, particularly through soil anomalies, also reduced the importance of interflow. Interflow generation was highly variable across eleven segments of a 121 m interception trench. Hillslopes were largely disconnected from stream behavior during storms. Hillslope processes were consistent with the fill-and-spill hypothesis and featured a sequence of distinct thresholds: vertical wetting front propagation to the argillic layer; saturation of the argillic followed by local perching; filling of argillic layer depressions; and finally connectivity of depressions leading to interflow generation. Analysis of trench flow data indicated a cumulative rainfall threshold of 60 mm to generate interflow, a value at the high end of the range of thresholds reported elsewhere. Published by Elsevier B.V. C1 [Du, Enhao; Jackson, C. Rhett; Williamson, Margaret F.; Greco, James L.; Bitew, Menberu] Univ Georgia, Warnell Sch Forestry & Nat Resources, Athens, GA 30602 USA. [Klaus, Julian; McDonnell, Jeffrey J.] Univ Saskatchewan, Global Inst Water Secur, Saskatoon, SK S7N 0W0, Canada. [McDonnell, Jeffrey J.] Univ Aberdeen, Sch Geosci, Aberdeen AB9 1FX, Scotland. [Griffiths, Natalie A.] Oak Ridge Natl Lab, Climate Change Sci Inst, Oak Ridge, TN 37831 USA. [Griffiths, Natalie A.] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Du, Enhao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Climate Sci Dept, Berkeley, CA 94720 USA. [Klaus, Julian] Luxembourg Inst Sci & Technol, Catchment & Ecohydrol Res Grp, Esch Sur Alzette, Luxembourg. [Williamson, Margaret F.] Peace Corps, Washington, DC 20526 USA. [Greco, James L.] ADA Engn, Tampa, FL 33606 USA. RP Du, EH (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Climate Sci Dept, Berkeley, CA 94720 USA. EM enhaodu@gmail.com OI Griffiths, Natalie/0000-0003-0068-7714 FU Department of Energy - Bioenergy Technologies Office through the U.S. Forest Service Savannah River under Interagency Agreement [DE-A109-00SR22188]; U.S. DOE Bioenergy Technologies Office; U.S. Department of Energy [DE-AC05-00OR22725]; Department of Energy - Savannah River Operations Office through the U.S. Forest Service Savannah River under Interagency Agreement [DE-A109-00SR22188] FX Support was provided by the Department of Energy - Bioenergy Technologies Office and Savannah River Operations Office through the U.S. Forest Service Savannah River under Interagency Agreement DE-A109-00SR22188. SRS is a National Environmental Research Park. John Blake of the USDA Forest Service was instrumental in project coordination. Benjamin Morris managed the field data collection. Bob Bahn, Shelly Robertson, Erin Harris, Damion Drover, Louise Jacques and several undergraduates from the University of Georgia assisted with fieldwork. Kellie Vache of Oregon State University and Luisa Hopp of the University of Bayreuth provided valuable advice and discussions of the data. Support to Natalie Griffiths was provided by U.S. DOE Bioenergy Technologies Office. Oak Ridge National Laboratory is managed by UT-Battelle, LLC for the U.S. Department of Energy under contract DE-AC05-00OR22725. NR 42 TC 1 Z9 1 U1 6 U2 18 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-1694 EI 1879-2707 J9 J HYDROL JI J. Hydrol. PD MAR PY 2016 VL 534 BP 648 EP 658 DI 10.1016/j.jhydrol.2016.01.039 PG 11 WC Engineering, Civil; Geosciences, Multidisciplinary; Water Resources SC Engineering; Geology; Water Resources GA DG3AC UT WOS:000371940900052 ER PT J AU An, FP An, GP An, Q Antonelli, V Baussan, E Beacom, J Bezrukov, L Blyth, S Brugnera, R Avanzini, MB Busto, J Cabrera, A Cai, H Cai, X Cammi, A Cao, GF Cao, J Chang, Y Chen, SM Chen, SJ Chen, YX Chiesa, D Clemenza, M Clerbaux, B Conrad, J D'Angelo, D De Kerret, H Deng, Z Deng, ZY Ding, YY Djurcic, Z Dornic, D Dracos, M Drapier, O Dusini, S Dye, S Enqvist, T Fan, DH Fang, J Favart, L Ford, R Goeger-Neff, M Gan, H Garfagnini, A Giammarchi, M Gonchar, M Gong, GH Gong, H Gonin, M Grassi, M Grewing, C Guan, MY Guarino, V Guo, G Guo, WL Guo, XH Hagner, C Han, R He, M Heng, YK Hsiung, Y Hu, J Hu, SY Hu, T Huang, HX Huang, XT Huo, L Ioannisian, A Jeitler, M Ji, XD Jiang, XS Jollet, C Kang, L Karagounis, M Kazarian, N Krumshteyn, Z Kruth, A Kuusiniemi, P Lachenmaier, T Leitner, R Li, C Li, JX Li, WD Li, WG Li, XM Li, XN Li, Y Li, YF Li, ZB Liang, H Lin, GL Lin, T Lin, YH Ling, JJ Lippi, I Liu, DW Liu, HB Liu, H Liu, JL Liu, JL Liu, JC Liu, Q Liu, SB Liu, SL Lombardi, P Long, YB Lu, HQ Lu, JS Lu, JB Lu, JG Lubsandorzhiev, B Ludhova, L Luo, S Lyashuk, V Mollenberg, R Ma, XB Mantovani, F Mao, YJ Mari, SM McDonough, WF Meng, G Meregaglia, A Meroni, E Mezzetto, M Miramonti, L Mueller, T Naumov, D Oberauer, L Ochoa-Ricoux, JP Olshevskiy, A Ortica, F Paoloni, A Peng, HP Peng, JC Previtali, E Qi, M Qian, S Qian, X Qian, YZ Qin, ZH Raffelt, G Ranucci, G Ricci, B Robens, M Romani, A Ruan, XD Ruan, XC Salamanna, G Shaevitz, M Sinev, V Sirignano, C Sisti, M Smirnov, O Soiron, M Stahl, A Stanco, L Steinmann, J Sun, XL Sun, YJ Taichenachev, D Tang, J Tkachev, I Trzaska, W Van Waasen, S Volpe, C Vorobel, V Votano, L Wang, CH Wang, GL Wang, H Wang, M Wang, RG Wang, SG Wang, W Wang, Y Wang, Y Wang, YF Wang, Z Wang, Z Wang, ZG Wang, ZM Wei, W Wen, LJ Wiebusch, C Wonsak, B Wu, Q Wulz, CE Wurm, M Xi, YF Xia, DM Xie, YG Xing, ZZ Xu, JL Yan, BJ Yang, CG Yang, CW Yang, G Yang, L Yang, YF Yao, Y Yegin, U Yermia, F You, ZY Yu, BX Yu, CX Yu, ZY Zavatarelli, S Zhan, L Zhang, C Zhang, HH Zhang, JW Zhang, JB Zhang, QM Zhang, YM Zhang, ZY Zhao, ZH Zheng, YH Zhong, WL Zhou, GR Zhou, J Zhou, L Zhou, R Zhou, S Zhou, WX Zhou, X Zhou, YL Zhou, YF Zou, JH AF An, Fengpeng An, Guangpeng An, Qi Antonelli, Vito Baussan, Eric Beacom, John Bezrukov, Leonid Blyth, Simon Brugnera, Riccardo Avanzini, Margherita Buizza Busto, Jose Cabrera, Anatael Cai, Hao Cai, Xiao Cammi, Antonio Cao, Guofu Cao, Jun Chang, Yun Chen, Shaomin Chen, Shenjian Chen, Yixue Chiesa, Davide Clemenza, Massimiliano Clerbaux, Barbara Conrad, Janet D'Angelo, Davide De Kerret, Herve Deng, Zhi Deng, Ziyan Ding, Yayun Djurcic, Zelimir Dornic, Damien Dracos, Marcos Drapier, Olivier Dusini, Stefano Dye, Stephen Enqvist, Timo Fan, Donghua Fang, Jian Favart, Laurent Ford, Richard Goeger-Neff, Marianne Gan, Haonan Garfagnini, Alberto Giammarchi, Marco Gonchar, Maxim Gong, Guanghua Gong, Hui Gonin, Michel Grassi, Marco Grewing, Christian Guan, Mengyun Guarino, Vic Guo, Gang Guo, Wanlei Guo, Xin-Heng Hagner, Caren Han, Ran He, Miao Heng, Yuekun Hsiung, Yee Hu, Jun Hu, Shouyang Hu, Tao Huang, Hanxiong Huang, Xingtao Huo, Lei Ioannisian, Ara Jeitler, Manfred Ji, Xiangdong Jiang, Xiaoshan Jollet, Cecile Kang, Li Karagounis, Michael Kazarian, Narine Krumshteyn, Zinovy Kruth, Andre Kuusiniemi, Pasi Lachenmaier, Tobias Leitner, Rupert Li, Chao Li, Jiaxing Li, Weidong Li, Weiguo Li, Xiaomei Li, Xiaonan Li, Yi Li, Yufeng Li, Zhi-Bing Liang, Hao Lin, Guey-Lin Lin, Tao Lin, Yen-Hsun Ling, Jiajie Lippi, Ivano Liu, Dawei Liu, Hongbang Liu, Hu Liu, Jianglai Liu, Jianli Liu, Jinchang Liu, Qian Liu, Shubin Liu, Shulin Lombardi, Paolo Long, Yongbing Lu, Haoqi Lu, Jiashu Lu, Jingbin Lu, Junguang Lubsandorzhiev, Bayarto Ludhova, Livia Luo, Shu Lyashuk, Vladimir Moellenberg, Randolph Ma, Xubo Mantovani, Fabio Mao, Yajun Mari, Stefano M. McDonough, William F. Meng, Guang Meregaglia, Anselmo Meroni, Emanuela Mezzetto, Mauro Miramonti, Lino Mueller, Thomas Naumov, Dmitry Oberauer, Lothar Ochoa-Ricoux, Juan Pedro Olshevskiy, Alexander Ortica, Fausto Paoloni, Alessandro Peng, Haiping Peng, Jen-Chieh Previtali, Ezio Qi, Ming Qian, Sen Qian, Xin Qian, Yongzhong Qin, Zhonghua Raffelt, Georg Ranucci, Gioacchino Ricci, Barbara Robens, Markus Romani, Aldo Ruan, Xiangdong Ruan, Xichao Salamanna, Giuseppe Shaevitz, Mike Sinev, Valery Sirignano, Chiara Sisti, Monica Smirnov, Oleg Soiron, Michael Stahl, Achim Stanco, Luca Steinmann, Jochen Sun, Xilei Sun, Yongjie Taichenachev, Dmitriy Tang, Jian Tkachev, Igor Trzaska, Wladyslaw Van Waasen, Stefan Volpe, Cristina Vorobel, Vit Votano, Lucia Wang, Chung-Hsiang Wang, Guoli Wang, Hao Wang, Meng Wang, Ruiguang Wang, Siguang Wang, Wei Wang, Yi Wang, Yi Wang, Yifang Wang, Zhe Wang, Zheng Wang, Zhigang Wang, Zhimin Wei, Wei Wen, Liangjian Wiebusch, Christopher Wonsak, Bjoern Wu, Qun Wulz, Claudia-Elisabeth Wurm, Michael Xi, Yufei Xia, Dongmei Xie, Yuguang Xing, Zhi-Zhong Xu, Jilei Yan, Baojun Yang, Changgen Yang, Chaowen Yang, Guang Yang, Lei Yang, Yifan Yao, Yu Yegin, Ugur Yermia, Frederic You, Zhengyun Yu, Boxiang Yu, Chunxu Yu, Zeyuan Zavatarelli, Sandra Zhan, Liang Zhang, Chao Zhang, Hong-Hao Zhang, Jiawen Zhang, Jingbo Zhang, Qingmin Zhang, Yu-Mei Zhang, Zhenyu Zhao, Zhenghua Zheng, Yangheng Zhong, Weili Zhou, Guorong Zhou, Jing Zhou, Li Zhou, Rong Zhou, Shun Zhou, Wenxiong Zhou, Xiang Zhou, Yeling Zhou, Yufeng Zou, Jiaheng TI Neutrino physics with JUNO SO JOURNAL OF PHYSICS G-NUCLEAR AND PARTICLE PHYSICS LA English DT Article DE reactor neutrino experiments; large scintillator detectors; neutrino physics; neutrino astronomy ID CORE-COLLAPSE SUPERNOVAE; WATER CHERENKOV DETECTOR; REACTOR ANTINEUTRINO EXPERIMENTS; SOLAR CHEMICAL-COMPOSITION; DARK-MATTER CANDIDATES; STAR-FORMATION RATE; GAMMA-RAY BURSTS; MASS HIERARCHY; GALACTIC SUPERNOVA; NUCLEON DECAY AB The Jiangmen Underground Neutrino Observatory (JUNO), a 20 kton multipurpose underground liquid scintillator detector, was proposed with the determination of the neutrino mass hierarchy (MH) as a primary physics goal. The excellent energy resolution and the large fiducial volume anticipated for the JUNO detector offer exciting opportunities for addressing many important topics in neutrino and astro-particle physics. In this document, we present the physics motivations and the anticipated performance of the JUNO detector for various proposed measurements. Following an introduction summarizing the current status and open issues in neutrino physics, we discuss how the detection of antineutrinos generated by a cluster of nuclear power plants allows the determination of the neutrino MH at a 3-4 sigma significance with six years of running of JUNO. The measurement of antineutrino spectrum with excellent energy resolution will also lead to the precise determination of the neutrino oscillation parameters sin(2) theta(12), Delta m(21)(2), and vertical bar Delta m(ee)(2)vertical bar to an accuracy of better than 1%, which will play a crucial role in the future unitarity test of the MNSP matrix. The JUNO detector is capable of observing not only antineutrinos from the power plants, but also neutrinos/antineutrinos from terrestrial and extra-terrestrial sources, including supernova burst neutrinos, diffuse supernova neutrino background, geoneutrinos, atmospheric neutrinos, and solar neutrinos. As a result of JUNO's large size, excellent energy resolution, and vertex reconstruction capability, interesting new data on these topics can be collected. For example, a neutrino burst from a typical core-collapse supernova at a distance of 10 kpc would lead to similar to 5000 inverse-beta-decay events and similar to 2000 all-flavor neutrino-proton ES events in JUNO, which are of crucial importance for understanding the mechanism of supernova explosion and for exploring novel phenomena such as collective neutrino oscillations. Detection of neutrinos from all past core-collapse supernova explosions in the visible universe with JUNO would further provide valuable information on the cosmic star-formation rate and the average core-collapse neutrino energy spectrum. Antineutrinos originating from the radioactive decay of uranium and thorium in the Earth can be detected in JUNO with a rate of similar to 400 events per year, significantly improving the statistics of existing geoneutrino event samples. Atmospheric neutrino events collected in JUNO can provide independent inputs for determining the MH and the octant of the theta(23) mixing angle. Detection of the Be-7 and B-8 solar neutrino events at JUNO would shed new light on the solar metallicity problem and examine the transition region between the vacuum and matter dominated neutrino oscillations. Regarding light sterile neutrino topics, sterile neutrinos with 10-(5) eV(2) < Delta m(41)(2) < 10(-2) and a sufficiently large mixing angle theta(14) could be identified through a precise measurement of the reactor antineutrino energy spectrum. Meanwhile, JUNO can also provide us excellent opportunities to test the eV-scale sterile neutrino hypothesis, using either the radioactive neutrino sources or a cyclotron-produced neutrino beam. The JUNO detector is also sensitive to several other beyondthe-standard-model physics. Examples include the search for proton decay via the p -> K++ <(v)over bar> decay channel, search for neutrinos resulting from dark-matter annihilation in the Sun, search for violation of Lorentz invariance via the sidereal modulation of the reactor neutrino event rate, and search for the effects of non-standard interactions. The proposed construction of the JUNO detector will provide a unique facility to address many outstanding crucial questions in particle and astrophysics in a timely and cost-effective fashion. It holds the great potential for further advancing our quest to understanding the fundamental properties of neutrinos, one of the building blocks of our Universe. C1 [An, Fengpeng] E China Univ Sci & Technol, Shanghai 200237, Peoples R China. [An, Guangpeng; Cai, Xiao; Cao, Guofu; Cao, Jun; Deng, Ziyan; Ding, Yayun; Fang, Jian; Grassi, Marco; Guan, Mengyun; Guo, Wanlei; He, Miao; Heng, Yuekun; Hu, Jun; Hu, Tao; Jiang, Xiaoshan; Li, Weidong; Li, Weiguo; Li, Xiaonan; Li, Yufeng; Lin, Tao; Liu, Jinchang; Liu, Shulin; Lu, Haoqi; Lu, Jiashu; Lu, Junguang; Qian, Sen; Qin, Zhonghua; Sun, Xilei; Wang, Ruiguang; Wang, Yifang; Wang, Zheng; Wang, Zhigang; Wang, Zhimin; Wei, Wei; Wen, Liangjian; Xie, Yuguang; Xing, Zhi-Zhong; Xu, Jilei; Yan, Baojun; Yang, Changgen; Yu, Boxiang; Yu, Zeyuan; Zhan, Liang; Zhang, Jiawen; Zhao, Zhenghua; Zhong, Weili; Zhou, Li; Zhou, Shun; Zhou, Yeling; Zou, Jiaheng] Inst High Energy Phys, Beijing 100039, Peoples R China. [An, Qi; Liang, Hao; Liu, Shubin; Peng, Haiping; Sun, Yongjie] Univ Sci & Technol China, Hefei 230026, Peoples R China. 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[Ochoa-Ricoux, Juan Pedro] Pontificia Univ Catolica Chile, Inst Fis, Alameda 340, Santiago, Chile. [Ortica, Fausto; Romani, Aldo] Ist Nazl Fis Nucl, I-06100 Perugia, Italy. [Ortica, Fausto; Romani, Aldo] Univ Perugia, Dept Chem Biol & Biotechnol, I-06100 Perugia, Italy. [Paoloni, Alessandro; Votano, Lucia] Ist Nazl Fis Nucl, Lab Nazl Frascati, Rome, Italy. [Qian, Xin; Zhang, Chao] Brookhaven Natl Lab, Upton, NY 11973 USA. [Qian, Yongzhong] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Raffelt, Georg] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shaevitz, Mike] Columbia Univ, New York, NY USA. [Soiron, Michael; Stahl, Achim; Steinmann, Jochen; Wiebusch, Christopher] Rhein Westfal TH Aachen, Phys Inst B3, Aachen, Germany. [Trzaska, Wladyslaw] Univ Jyvaskyla, Dept Phys, Jyvaskyla, Finland. [Wurm, Michael] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Wurm, Michael] Johannes Gutenberg Univ Mainz, EC PRISMA, D-55122 Mainz, Germany. [Yang, Chaowen; Zhou, Rong] Sichuan Univ, Chengdu 610064, Peoples R China. [Yermia, Frederic] Univ Nantes, Ecole Mines Nantes, CNRS, SUBATECH,IN2P3, Nantes, France. [Yu, Chunxu] Nankai Univ, Tianjin 300071, Peoples R China. [Zavatarelli, Sandra] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Zhang, Qingmin] Xi An Jiao Tong Univ, Xian 710049, Peoples R China. [Zhou, Yufeng] Acad Sinica, Beijing, Peoples R China. RP Cao, J; Guo, WL; He, M; Li, YF; Wen, LJ; Xing, ZZ; Zhan, L; Zhong, WL; Zhou, S (reprint author), Inst High Energy Phys, Beijing 100039, Peoples R China.; Ludhova, L; Meroni, E (reprint author), Ist Nazl Fis Nucl, Sez Milano, Via Celoria 16, I-20133 Milan, Italy.; Ludhova, L; Meroni, E (reprint author), Univ Milan, Dipartimento Fis, Milan, Italy.; Han, R (reprint author), North China Elect Power Univ, Beijing, Peoples R China.; Oberauer, L (reprint author), Tech Univ Munich, Garching, Germany.; Lin, GL (reprint author), Natl Chiao Tung Univ, Inst Phys, Hsinchu, Taiwan.; Peng, JC (reprint author), Univ Illinois, Dept Phys, Urbana, IL USA.; McDonough, WF (reprint author), Univ Maryland, Dept Geol, College Pk, MD 20742 USA.; Zhang, C (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA.; Raffelt, G (reprint author), Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany.; Wiebusch, C (reprint author), Rhein Westfal TH Aachen, Phys Inst B3, Aachen, Germany.; Wurm, M (reprint author), Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany.; Wurm, M (reprint author), Johannes Gutenberg Univ Mainz, EC PRISMA, D-55122 Mainz, Germany. EM caoj@ihep.ac.cn; guowl@ihep.ac.cn; hanran@ncepu.edu.cn; hem@ihep.ac.cn; liyufeng@ihep.ac.cn; glin@mail.nctu.edu.tw; ludhova@gmail.com; mcdonoug@umd.edu; emanuela.meroni@mi.infn.it; lothar.oberauer@tum.de; jcpeng@illinois.edu; raffelt@mpp.mpg.de; wenlj@ihep.ac.cn; wiebusch@physik.rwth-aachen.de; michael.wurm@uni-mainz.de; xingzz@ihep.ac.cn; zhanl@ihep.ac.cn; chao@bnl.gov; zhongwl@ihep.ac.cn; zhoush@ihep.ac.cn RI Zhou, Shun/K-7083-2014; Cao, Jun/G-8701-2012; Lyashuk, Vladimir/R-9766-2016; Ortica, Fausto/C-1001-2013; Wiebusch, Christopher/G-6490-2012; dusini, stefano/J-3686-2012; Chiesa, Davide/H-7240-2014; Olshevskiy, Alexander/I-1580-2016; Romani, Aldo/G-8103-2012; McDonough, William/I-7720-2012; Stahl, Achim/E-8846-2011; Antonelli, Vito/B-7901-2013; Ling, Jiajie/I-9173-2014; DAngelo, Davide/K-9164-2013 OI Paoloni, Alessandro/0000-0002-4141-7799; Kruth, Andre/0000-0002-6273-8778; Zhou, Shun/0000-0003-4572-9666; Tang, Jian/0000-0002-2926-2560; Cao, Jun/0000-0002-3586-2319; HSIUNG, YEE/0000-0003-4801-1238; Clemenza, Massimiliano/0000-0002-8064-8936; Qian, Xin/0000-0002-7903-7935; Lu, Jiashu/0000-0003-4308-4665; Zhang, Chao/0000-0003-2298-6272; Beacom, John/0000-0002-0005-2631; Ochoa-Ricoux, Juan Pedro/0000-0001-7376-5555; Lin, Tao/0000-0002-6450-9629; Lyashuk, Vladimir/0000-0002-8192-797X; Ortica, Fausto/0000-0001-8276-452X; Wiebusch, Christopher/0000-0002-6418-3008; dusini, stefano/0000-0002-1128-0664; Chiesa, Davide/0000-0003-1978-1727; Olshevskiy, Alexander/0000-0002-8902-1793; Romani, Aldo/0000-0002-7338-0097; McDonough, William/0000-0001-9154-3673; Stahl, Achim/0000-0002-8369-7506; Antonelli, Vito/0000-0001-9680-0149; Ling, Jiajie/0000-0003-2982-0670; DAngelo, Davide/0000-0001-9857-8107 FU Chinese Academy of Sciences; Ministry of Science and Technology of China; National Natural Science Foundation of China; Shanghai Jiao Tong University; Tsinghua University in China; Belgian Fonds de la Recherche Scientifique; FNRS in Belgium; Charles University in Prague; Czech Republic; CNRS National Institute of Nuclear and Particle Physics (IN2P3) in France; Deutsche Forschungsgemeinschaft (DFG); Helmholtz Alliance for Astroparticle Physics (HAP) in Germany; Helmholtz Gemeinschaft (HGF) in Germany; Istituto Nazionale di Fisica Nucleare (INFN) in Italy; Joint Institute for Nuclear Research (JINR) in Russia; NSFC-RFBR joint research program; Guangdong provincial government; Jiangmen and Kaiping Municipal Government FX The JUNO Experiment is supported by the Chinese Academy of Sciences, the Ministry of Science and Technology of China, the National Natural Science Foundation of China, Shanghai Jiao Tong University, and Tsinghua University in China, the Belgian Fonds de la Recherche Scientifique, FNRS in Belgium, the Charles University in Prague, Czech Republic, the CNRS National Institute of Nuclear and Particle Physics (IN2P3) in France, the Deutsche Forschungsgemeinschaft (DFG), Helmholtz Alliance for Astroparticle Physics (HAP), and Helmholtz Gemeinschaft (HGF) in Germany, the Istituto Nazionale di Fisica Nucleare (INFN) in Italy, the Joint Institute for Nuclear Research (JINR) in Russia, and the NSFC-RFBR joint research program. We acknowledge the generous support of the Guangdong provincial government and the Jiangmen and Kaiping Municipal Government. We are grateful for the ongoing cooperation from the China General Nuclear Power Group (CGNPC). NR 456 TC 45 Z9 45 U1 46 U2 77 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0954-3899 EI 1361-6471 J9 J PHYS G NUCL PARTIC JI J. Phys. G-Nucl. Part. Phys. PD MAR PY 2016 VL 43 IS 3 AR 030401 DI 10.1088/0954-3899/43/3/030401 PG 188 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA DG4SZ UT WOS:000372064200001 ER PT J AU LaMont, SP Glover, SE AF LaMont, Stephen P. Glover, Samuel E. TI 10th International Conference on Methods and Applications of Radioanalytical Chemistry (MARC X) Introduction SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Editorial Material C1 [LaMont, Stephen P.] Los Alamos Natl Lab, Nucl & Radiochem, POB 1663,MS J514, Los Alamos, NM 87545 USA. [Glover, Samuel E.] Natl Inst Occupat Safety & Hlth, Div Appl Res & Technol, Biomonitoring & Hlth Assessment Branch, 1090 Tusculum Ave,MS C26, Cincinnati, OH 45226 USA. RP Glover, SE (reprint author), Natl Inst Occupat Safety & Hlth, Div Appl Res & Technol, Biomonitoring & Hlth Assessment Branch, 1090 Tusculum Ave,MS C26, Cincinnati, OH 45226 USA. EM lamont@lanl.gov FU Intramural CDC HHS [CC999999] NR 0 TC 0 Z9 0 U1 0 U2 1 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD MAR PY 2016 VL 307 IS 3 BP 1567 EP 1568 DI 10.1007/s10967-016-4716-6 PG 2 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA DG1ER UT WOS:000371808900001 PM 27546944 ER PT J AU Clark, RA Barinaga, CJ McNamara, BK Schwantes, JM Ballou, NE AF Clark, Richard A. Barinaga, Charles J. McNamara, Bruce K. Schwantes, Jon M. Ballou, Nathan E. TI Selective fluorination and separation of metals with NF3 for mass spectrometry SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article; Proceedings Paper CT 10th International Conference on Methods and Applications of Radioanalytical Chemistry (MARC) CY APR 12-17, 2015 CL Kailua Kona, HI DE Mass spectrometry; Fluorination; Nitrogen trifluoride; Nuclear forensics ID TEMPERATURE FLUORINATION; URANIUM TETRAFLUORIDE; ENVIRONMENTAL-SAMPLES; BROMINE TRIFLUORIDE; THERMAL NF3; OXIDES; U3O8; HEXAFLUORIDE; DIFLUORIDE; FLUORIDES AB We report recent progress on the development of a new methodology based on the generation of volatile metal fluorides through the use of nitrogen trifluoride (NF3) and the measurement of these metal fluorides by electron ionization mass spectrometry. Though unreactive under ambient conditions, NF3 reacts selectively at specified temperatures with various metal-containing species to form volatile metal fluorides. Utilizing these species-dependent traits, elements of a sample may be sequentially produced and thus separated on-line. Tellurium was reacted inside a thermogravimetric analyzer, the gas outlet of which was directly coupled to a quadrupole mass spectrometer with an electron impact ionization source. C1 [Clark, Richard A.; Barinaga, Charles J.; McNamara, Bruce K.; Schwantes, Jon M.; Ballou, Nathan E.] Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99352 USA. RP Clark, RA (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99352 USA. EM richard.clark@pnnl.gov NR 27 TC 0 Z9 0 U1 2 U2 9 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD MAR PY 2016 VL 307 IS 3 BP 1587 EP 1590 DI 10.1007/s10967-015-4392-y PG 4 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA DG1ER UT WOS:000371808900004 ER PT J AU Eslinger, PW Schrom, BT AF Eslinger, Paul W. Schrom, Brian T. TI Multi-detection events, probability density functions, and reduced location area SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article; Proceedings Paper CT 10th International Conference on Methods and Applications of Radioanalytical Chemistry (MARC) CY APR 12-17, 2015 CL Kailua Kona, HI DE Source-term estimation; Atmospheric modeling; Nuclear explosion detection; CTBTO ID INTERNATIONAL MONITORING-SYSTEM; MEASURED AIR CONCENTRATIONS; NUCLEAR-TEST; BAYESIAN-INFERENCE; NORTH-KOREA; XENON; DISPERSION AB Several efforts have been made in the Comprehensive Nuclear-Test-Ban Treaty (CTBT) community to assess the benefits of combining detections of radionuclides to improve the location estimates available from atmospheric transport modeling (ATM) backtrack calculations. We present a Bayesian estimation approach rather than a simple dilution field of regard approach to allow xenon detections and non-detections to be combined mathematically. This system represents one possible probabilistic approach to radionuclide event formation. Application of this method to a recent interesting radionuclide event shows a substantial reduction in the location uncertainty of that event. C1 [Eslinger, Paul W.] Pacific NW Natl Lab, 902 Battelle Blvd,MSIN K7-76,POB 999, Richland, WA 99352 USA. [Schrom, Brian T.] Pacific NW Natl Lab, 902 Battelle Blvd,MSIN J4-65,POB 999, Richland, WA 99352 USA. RP Eslinger, PW (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd,MSIN K7-76,POB 999, Richland, WA 99352 USA. EM paul.w.eslinger@pnnl.gov; brian.schrom@pnnl.gov NR 24 TC 0 Z9 0 U1 2 U2 2 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD MAR PY 2016 VL 307 IS 3 BP 1599 EP 1605 DI 10.1007/s10967-015-4339-3 PG 7 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA DG1ER UT WOS:000371808900007 ER PT J AU Velazquez, M Dreyer, J Drury, OB Salaymeh, S Friedrich, S AF Velazquez, Miguel Dreyer, Jonathan Drury, Owen B. Salaymeh, Saleem Friedrich, Stephan TI Cryogenic gamma detectors enable direct detection of U-236 and minor actinides for non-destructive assay SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article; Proceedings Paper CT 10th International Conference on Methods and Applications of Radioanalytical Chemistry (MARC) CY APR 12-17, 2015 CL Kailua Kona, HI DE Superconducting gamma detectors; Transition edge sensors; Non-destructive analysis; Uranium isotopic analysis; Minor actinides AB We demonstrate the utility of a superconducting transition edge sensor (TES) gamma-ray detector with high energy resolution and low Compton background for non-destructive assay (NDA) of a uranium sample from reprocessed nuclear fuel. We show that TES gamma-detectors can separate low-energy actinide gamma-emissions from the background and nearby lines, even from minor isotopes whose signals are often obscured in NDA with conventional Ge detectors. Superconducting gamma-detectors may therefore bridge the gap between high-accuracy destructive assay (DA) and easier-to-use NDA. C1 [Velazquez, Miguel; Dreyer, Jonathan; Drury, Owen B.; Friedrich, Stephan] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. [Salaymeh, Saleem] Savannah River Natl Lab, Bldg 737-A, Aiken, SC 29802 USA. [Velazquez, Miguel] INAOE, Santa Maria Tonatzintla 72840, Puebla, Mexico. RP Friedrich, S (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. EM friedrich1@llnl.gov NR 10 TC 0 Z9 0 U1 3 U2 4 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD MAR PY 2016 VL 307 IS 3 BP 1607 EP 1610 DI 10.1007/s10967-015-4409-6 PG 4 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA DG1ER UT WOS:000371808900008 ER PT J AU Tamasi, AL Cash, LJ Eley, C Porter, RB Pugmire, DL Ross, AR Ruggiero, CE Tandon, L Wagner, GL Walensky, JR Wall, AD Wilkerson, MP AF Tamasi, Alison L. Cash, Leigh J. Eley, Christopher Porter, Reid B. Pugmire, David L. Ross, Amy R. Ruggiero, Christy E. Tandon, Lav Wagner, Gregory L. Walensky, Justin R. Wall, Angelique D. Wilkerson, Marianne P. TI A lexicon for consistent description of material images for nuclear forensics SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article; Proceedings Paper CT 10th International Conference on Methods and Applications of Radioanalytical Chemistry (MARC) CY APR 12-17, 2015 CL Kailua Kona, HI DE Image; Morphology; Nuclear forensics; Scanning electron microscopy; Terminology; Texture ID URANIUM-DIOXIDE; AMMONIUM DIURANATE; PRECIPITATION; MORPHOLOGY; POWDER; PARAMETERS; PARTICLES; PRODUCTS; URANYL; OXIDE AB We have developed a lexicon to consistently and objectively describe morphological features observed in scanning electron microscopy (SEM) images. Here we provide the lexicon flowsheet, define the terminology, and detail step-by-step characterization of SEM images collected from a set of actinide oxides. We conclude that this lexicon can be used to characterize texture and surface features, particle structure and size, and grain boundaries in an image of a material. The lexicon should be applicable to characterization of images collected from other techniques for measuring morphology, as well. LA-UR-15-26746. C1 [Tamasi, Alison L.; Cash, Leigh J.; Porter, Reid B.; Pugmire, David L.; Ross, Amy R.; Ruggiero, Christy E.; Tandon, Lav; Wagner, Gregory L.; Wall, Angelique D.; Wilkerson, Marianne P.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. [Tamasi, Alison L.; Walensky, Justin R.] Univ Missouri, Dept Chem, Columbia, MO 65211 USA. [Eley, Christopher] South Carolina State Univ, Dept Chem, Orangeburg, SC 29117 USA. RP Wilkerson, MP (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM mpw@lanl.gov OI Wagner, Gregory/0000-0002-7852-7529 NR 22 TC 3 Z9 3 U1 4 U2 12 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD MAR PY 2016 VL 307 IS 3 BP 1611 EP 1619 DI 10.1007/s10967-015-4455-0 PG 9 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA DG1ER UT WOS:000371808900009 ER PT J AU Mathew, KJ Haoszbek, A AF Mathew, K. J. Haoszbek, A. TI Comparison of mass spectrometric methods (TE, MTE and conventional) for uranium isotope ratio measurements SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article; Proceedings Paper CT 10th International Conference on Methods and Applications of Radioanalytical Chemistry (MARC) CY APR 12-17, 2015 CL Kailua Kona, HI DE Uranium isotope ratios; Thermal ionization mass spectrometry; Total evaporation; Certified reference materials ID METAL ASSAY; PLUTONIUM; CERTIFICATION; STANDARD AB The isotope ratio measurement techniques-total evaporation (TE), modified total evaporation (MTE), and conventional-used for characterization measurements of certified reference materials by thermal ionization mass spectrometer instruments are compared. The advantages of each method, the fractionation profiles resulting from the measurement techniques, and factors affecting systematic components of bias in the isotope ratio measurements are discussed. The TE and MTE techniques yield major ratios and the conventional and MTE techniques yield minor ratios of comparable quality (in terms of precision and accuracy). C1 [Mathew, K. J.; Haoszbek, A.] US DOE, NBL, 9800 S Cass Ave, Argonne, IL 60439 USA. [Mathew, K. J.] Savannah River Natl Lab, FH Area Analyt Labs, Bldg 707-F, Aiken, SC 29808 USA. [Haoszbek, A.] Dokuz Eylul Univ, Izmir, Turkey. RP Mathew, KJ (reprint author), US DOE, NBL, 9800 S Cass Ave, Argonne, IL 60439 USA.; Mathew, KJ (reprint author), Savannah River Natl Lab, FH Area Analyt Labs, Bldg 707-F, Aiken, SC 29808 USA. EM kattathu.mathew@srs.gov NR 14 TC 3 Z9 3 U1 3 U2 8 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD MAR PY 2016 VL 307 IS 3 BP 1681 EP 1687 DI 10.1007/s10967-015-4484-8 PG 7 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA DG1ER UT WOS:000371808900020 ER PT J AU Mathew, KJ Hasozbek, A AF Mathew, K. J. Hasozbek, A. TI Comparison of mass spectrometric methods (TE, MTE and conventional) for uranium isotope ratio measurements (vol 307, pg 1681, 2016) SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Correction C1 [Mathew, K. J.; Hasozbek, A.] US DOE, NBL, 9800 S Cass Ave, Argonne, IL 60439 USA. [Mathew, K. J.] Savannah River Natl Lab, FH Area Analyt Labs, Bldg 707-F, Aiken, SC 29808 USA. [Hasozbek, A.] Dokuz Eylul Univ, Izmir, Turkey. RP Mathew, KJ (reprint author), US DOE, NBL, 9800 S Cass Ave, Argonne, IL 60439 USA.; Mathew, KJ (reprint author), Savannah River Natl Lab, FH Area Analyt Labs, Bldg 707-F, Aiken, SC 29808 USA. EM kattathu.mathew@srs.gov NR 1 TC 0 Z9 0 U1 0 U2 0 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD MAR PY 2016 VL 307 IS 3 BP 1689 EP 1689 DI 10.1007/s10967-015-4562-y PG 1 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA DG1ER UT WOS:000371808900021 ER PT J AU Seiner, BN King, AR Finn, E Greenwood, LR Metz, LA Friese, J Marsden, O Davies, AV Scivier, P AF Seiner, Brienne N. King, Andy R. Finn, Erin Greenwood, Lawrence R. Metz, Lori A. Friese, Judah Marsden, Olivia Davies, Ashley V. Scivier, Philip TI Fission product analysis of HEU irradiated within a boron carbide capsule: comparison of detection methodology at PNNL and AWE SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article; Proceedings Paper CT 10th International Conference on Methods and Applications of Radioanalytical Chemistry (MARC) CY APR 12-17, 2015 CL Kailua Kona, HI DE Compton suppression; High-purity gamma spectroscopy; Fission product analysis ID EXTRACTION CHROMATOGRAPHY; SEQUENTIAL DETERMINATION; SEPARATION; PRECONCENTRATION; ACTINIDES; SAMPLES AB The fission products from HEU formed under a fast-pooled neutron spectrum generated using a boron carbide shield were analyzed at Pacific Northwest National Laboratory and the Atomic Weapons Establishment. The results from each laboratory using chemical separation, high-purity germanium gamma spectroscopy and/or Compton suppression gamma spectroscopy are compared with the potential benefits and limitations of the different gamma spectroscopy methods discussed. C1 [Seiner, Brienne N.; Finn, Erin; Greenwood, Lawrence R.; Metz, Lori A.; Friese, Judah] Pacific NW Natl Lab, 902 Battelle Blvd,POB 999, Richland, WA 99354 USA. [King, Andy R.; Marsden, Olivia; Davies, Ashley V.; Scivier, Philip] AWE, Reading RG7 4PR, Berks, England. RP Seiner, BN (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd,POB 999, Richland, WA 99354 USA. EM brienne.seiner@pnnl.gov RI Greenwood, Lawrence/H-9539-2016 OI Greenwood, Lawrence/0000-0001-6563-0650 NR 20 TC 1 Z9 1 U1 2 U2 5 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD MAR PY 2016 VL 307 IS 3 BP 1729 EP 1734 DI 10.1007/s10967-015-4395-8 PG 6 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA DG1ER UT WOS:000371808900029 ER PT J AU Seiner, BN Burnett, JL King, AR Finn, E Greenwood, LR Metz, LA Friese, J Marsden, O Davies, AV Scivier, P AF Seiner, Brienne N. Burnett, Jonathan L. King, Andy R. Finn, Erin Greenwood, Lawrence R. Metz, Lori A. Friese, Judah Marsden, Olivia Davies, Ashley V. Scivier, Philip TI Fission product analysis in HEU irradiated within a boron carbide capsule: comparison of detection methodology at PNNL and AWE (vol 307, pg 1729, 2016) SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Correction C1 [Seiner, Brienne N.; Finn, Erin; Greenwood, Lawrence R.; Metz, Lori A.; Friese, Judah] Pacific NW Natl Lab, 902 Battelle Blvd,POB 999, Richland, WA 99354 USA. [Burnett, Jonathan L.; King, Andy R.; Marsden, Olivia; Davies, Ashley V.; Scivier, Philip] AWE, Reading RG7 4PR, Berks, England. RP Seiner, BN (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd,POB 999, Richland, WA 99354 USA. EM brienne.seiner@pnnl.gov RI Greenwood, Lawrence/H-9539-2016 OI Greenwood, Lawrence/0000-0001-6563-0650 NR 2 TC 0 Z9 0 U1 1 U2 1 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD MAR PY 2016 VL 307 IS 3 BP 1735 EP 1735 DI 10.1007/s10967-015-4539-x PG 1 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA DG1ER UT WOS:000371808900030 ER PT J AU Haney, MM Seiner, BN Finn, EC Friese, JI AF Haney, Morgan M. Seiner, Brienne N. Finn, Erin C. Friese, Judah I. TI Rapid quantitation of uranium from mixed fission product samples SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article; Proceedings Paper CT 10th International Conference on Methods and Applications of Radioanalytical Chemistry (MARC) CY APR 12-17, 2015 CL Kailua Kona, HI DE UTEVA; Uranium-235; Gamma spectroscopy; Rapid chemical separations ID EXTRACTION CHROMATOGRAPHY; SEPARATION; ELECTRODEPOSITION; PRECONCENTRATION; ACTINIDES AB Chemical similarities between uranium(VI) and molybdenum(VI) create challenges for separation and quantitation of uranium isotopes from a mixed fission product sample. The purpose of this work was to demonstrate an improved chemical separation for the detection of U-235 using gamma spectroscopy. The optimized method, which included extraction and anion exchange chromatography, demonstrated a consistent chemical yield of 74 +/- A 3 % for uranium. Using a fresh fission product sample the minimum detectable activity for U-235, U-237, and U-238 was reduced by a factor of two. The chemical isolation of uranium was achieved in less than 4 h, with a separation factor of 1.41 x 10(5) from molybdenum. C1 [Haney, Morgan M.; Seiner, Brienne N.; Finn, Erin C.; Friese, Judah I.] Pacific NW Natl Lab, 902 Battelle Blvd,POB 999, Richland, WA 99352 USA. RP Haney, MM; Seiner, BN (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd,POB 999, Richland, WA 99352 USA. EM Morgan.Haney@pnnl.gov; Brienne.Seiner@pnnl.gov NR 12 TC 0 Z9 0 U1 2 U2 4 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD MAR PY 2016 VL 307 IS 3 BP 1737 EP 1742 DI 10.1007/s10967-015-4617-0 PG 6 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA DG1ER UT WOS:000371808900031 ER PT J AU Liezers, M Farmer, OT Thomas, ML Hager, GJ Eiden, GC AF Liezers, Martin Farmer, Orville T., III Thomas, May L. Hager, George J. Eiden, Gregory C. TI A new bench-top approach to the isotopic purification of Pu-244 SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article; Proceedings Paper CT 10th International Conference on Methods and Applications of Radioanalytical Chemistry (MARC) CY APR 12-17, 2015 CL Kailua Kona, HI DE Isotope enrichment; Isotope purification; Pu-244; Nuclear forensics; High purity isotopes ID MASS-SPECTROMETRY; ICP-MS; CALUTRON AB A new approach to isotopic purification has been developed and applied to the production of a small quantity of Pu-244 with an isotopic purity > 99.996 %, as compared against the standard Pu-244 available that displays an isotopic purity of 97.87 %. The presence of Pu isotopes Pu-239, Pu-240, Pu-241 and Pu-242 have been greatly reduced, allowing for higher spiking levels of the isotopically purified Pu-244 tracer to be used in environmental level sample analysis. Details of the isotopic purification process will be described along with the effect this improved Pu tracer could have on analytical Pu mass spectrometry measurements. C1 [Liezers, Martin; Farmer, Orville T., III; Thomas, May L.; Hager, George J.; Eiden, Gregory C.] Pacific NW Natl Lab, J4-60, Richland, WA 99352 USA. RP Liezers, M (reprint author), Pacific NW Natl Lab, J4-60, Richland, WA 99352 USA. EM martin.liezers@pnnl.gov NR 11 TC 1 Z9 1 U1 3 U2 3 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD MAR PY 2016 VL 307 IS 3 BP 1795 EP 1800 DI 10.1007/s10967-015-4341-9 PG 6 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA DG1ER UT WOS:000371808900040 ER PT J AU Liezers, M Carman, AJ Eiden, GC AF Liezers, Martin Carman, April J. Eiden, Gregory C. TI The preparation of non-radioactive glassy surrogate nuclear explosion debris (SNED) loaded with isotopically altered Xe SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article; Proceedings Paper CT 10th International Conference on Methods and Applications of Radioanalytical Chemistry (MARC) CY APR 12-17, 2015 CL Kailua Kona, HI DE Trinitite; Nuclear forensics; Fission Xe; Surrogate nuclear explosion debris; Laser melting; Laser ablation ID XENON; FALLOUT; SYSTEM AB The measurement of Kr and Xe isotope ratios in nuclear explosion debris can be performed requiring little sample preparation. Fragments of debris are simply crushed or heated to release trapped gases Kr and Xe arising from fission product decay. As a suitable test material for this measurement, we have been investigating a method to incorporate isotopically enriched Xe-129 in glassy materials that mimic nuclear explosion debris. The approach used to prepare these materials will be described along with some of the example results obtained. C1 [Liezers, Martin; Carman, April J.; Eiden, Gregory C.] Pacific NW Natl Lab, J4-60, Richland, WA 99352 USA. RP Liezers, M (reprint author), Pacific NW Natl Lab, J4-60, Richland, WA 99352 USA. EM martin.liezers@pnnl.gov NR 15 TC 0 Z9 0 U1 8 U2 12 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD MAR PY 2016 VL 307 IS 3 BP 1811 EP 1817 DI 10.1007/s10967-015-4396-7 PG 7 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA DG1ER UT WOS:000371808900043 ER PT J AU Zickefoose, JK Bronson, FL Ilie, G Jaderstrom, H Venkataraman, R AF Zickefoose, James K. Bronson, Frazier L. Ilie, Gabriela Jaederstroem, Henrik Venkataraman, Ram TI Performance of a low activity beta-sensitive Sr-90 water monitor SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article; Proceedings Paper CT 10th International Conference on Methods and Applications of Radioanalytical Chemistry (MARC) CY APR 12-17, 2015 CL Kailua Kona, HI DE Fukushima; Sr-90; Water contamination; Minimum detectable concentration; Beta sensitive detector ID NUCLEAR-POWER-PLANT; ACCIDENT; RADIONUCLIDES AB A continuous on-line beta sensitive water monitor was developed to determine the Sr-90 activity levels in water after processing at the Fukushima nuclear power plants. The sensitivity required by the customer, 10 Bq kg(-1), posed issues for any existing continuous on-line technology. The developed water monitor has maximized the efficiency to beta radiation while minimizing gamma background, and achieves a minimum detectable concentration of 6.3 Bq kg(-1) in a 1 h measurement. C1 [Zickefoose, James K.; Bronson, Frazier L.; Ilie, Gabriela; Jaederstroem, Henrik] Canberra Ind, 800 Res Pkwy, Merida, CT 06450 USA. [Venkataraman, Ram] Oak Ridge Natl Lab, One Bethel Valley Rd, Oak Ridge, TN 37831 USA. RP Zickefoose, JK (reprint author), Canberra Ind, 800 Res Pkwy, Merida, CT 06450 USA. EM james.zickefoose@canberra.com NR 11 TC 0 Z9 0 U1 1 U2 3 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD MAR PY 2016 VL 307 IS 3 BP 1819 EP 1824 DI 10.1007/s10967-015-4487-5 PG 6 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA DG1ER UT WOS:000371808900044 ER PT J AU McLain, DR Mertz, CJ Sudowe, R AF McLain, Derek R. Mertz, Carol J. Sudowe, Ralf TI A performance comparison of commercially available strontium extraction chromatography columns SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article; Proceedings Paper CT 10th International Conference on Methods and Applications of Radioanalytical Chemistry (MARC) CY APR 12-17, 2015 CL Kailua Kona, HI DE Extraction chromatography; Strontium; Elution comparison AB Extraction chromatographic separations following a nuclear event will require both speed and accuracy. Ideally these separations will be carried out using commercially available products. Because Sr-90 is a likely material to be used in a radioactivity dispersal device, commercially available products for the separation of strontium were tested to evaluate differences in their elution profiles that may affect elution procedures. Gravity flow columns show better resolution, but vacuum flow columns allow rapid processing and are still adequate for purification if multiple aqueous conditions can be employed in the elution strategy. C1 [McLain, Derek R.; Sudowe, Ralf] Univ Nevada, HRC 102,4505 S Maryland Pkwy,Box 454009, Las Vegas, NV 89154 USA. [Mertz, Carol J.] Argonne Natl Lab, 9700 S Cass Ave B109, Lemont, IL 60439 USA. RP McLain, DR (reprint author), Univ Nevada, HRC 102,4505 S Maryland Pkwy,Box 454009, Las Vegas, NV 89154 USA. EM mclaind@unlv.nevada.edu NR 8 TC 0 Z9 0 U1 3 U2 3 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD MAR PY 2016 VL 307 IS 3 BP 1825 EP 1831 DI 10.1007/s10967-015-4634-z PG 7 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA DG1ER UT WOS:000371808900045 ER PT J AU Mincher, BJ Tillotson, RD Garn, T Rutledge, V Law, J Schmitt, NC AF Mincher, Bruce J. Tillotson, Richard D. Garn, Troy Rutledge, Veronica Law, Jack Schmitt, Nicholas C. TI The solvent extraction of Am(VI) using centrifugal contactors SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article; Proceedings Paper CT 10th International Conference on Methods and Applications of Radioanalytical Chemistry (MARC) CY APR 12-17, 2015 CL Kailua Kona, HI DE Americium(VI); Centrifugal contactors; Minor actinides; Sodium bismuthate; Solvent extraction ID AMERICIUM AB An engineering-scale centrifugal contactor test bed was built at Idaho National Laboratory to perform solvent extraction testing for the partitioning of hexavalent americium. The raffinate simulant feed was spiked with Am-243 and Ce-139 and treated with sodium bismuthate to oxidize americium to Am(VI), filtered and contacted with 1 M DAAP/dodecane using centrifugal contactors. Extraction efficiency comparable to batch contacts was obtained, indicating for the first time that Am(VI) can be maintained under process conditions. Contrary to expectations, stripping was not as effective as expected. However, this result may actually be advantageous to process design, since a scrub step, previously thought to be impossible due to rapid Am(VI) reduction, may now be considered for future flowsheet tests. C1 [Mincher, Bruce J.; Tillotson, Richard D.; Garn, Troy; Rutledge, Veronica; Law, Jack; Schmitt, Nicholas C.] Idaho Natl Lab, Aqueous Separat & Radiochem Dept, POB 1625, Idaho Falls, ID 83415 USA. RP Mincher, BJ (reprint author), Idaho Natl Lab, Aqueous Separat & Radiochem Dept, POB 1625, Idaho Falls, ID 83415 USA. EM bruce.mincher@inl.gov RI Mincher, Bruce/C-7758-2017; OI Law, Jack/0000-0001-7085-7542 NR 7 TC 3 Z9 3 U1 1 U2 5 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD MAR PY 2016 VL 307 IS 3 BP 1833 EP 1836 DI 10.1007/s10967-015-4397-6 PG 4 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA DG1ER UT WOS:000371808900046 ER PT J AU Byerly, B Tandon, L Hayes-Sterbenz, A Martinez, P Keller, R Stanley, F Spencer, K Thomas, M Xu, N Schappert, M Fulwyler, J AF Byerly, Benjamin Tandon, Lav Hayes-Sterbenz, Anna Martinez, Patrick Keller, Russ Stanley, Floyd Spencer, Khalil Thomas, Mariam Xu, Ning Schappert, Michael Fulwyler, James TI Determination of initial fuel state and number of reactor shutdowns in archived low-burnup uranium targets SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article; Proceedings Paper CT 10th International Conference on Methods and Applications of Radioanalytical Chemistry (MARC) CY APR 12-17, 2015 CL Kailua Kona, HI DE Irradiation; Targets; Uranium; Plutonium; Ruthenium; Cesium ID ACCIDENT CONDITIONS; EXTRACTION; VOLATILE AB This study presents a method for destructive analysis of irradiated uranium (U) targets, with a focus on collection and measurement of long-lived (t (1/2) > similar to 10 years) and stable fission product isotopes of ruthenium and cesium. Long-lived and stable isotopes of these elements can provide information on reactor conditions (e.g. flux, irradiation time, cooling time) in old samples (> 5-10 years) whose short-lived fission products have decayed away. The separation and analytical procedures were tested on archived U reactor targets at Los Alamos National Laboratory as part of an effort to evaluate reactor models at low-burnup. C1 [Byerly, Benjamin; Tandon, Lav; Hayes-Sterbenz, Anna; Martinez, Patrick; Keller, Russ; Stanley, Floyd; Spencer, Khalil; Thomas, Mariam; Xu, Ning; Schappert, Michael; Fulwyler, James] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Byerly, B (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM byerly@lanl.gov OI Byerly, Benjamin/0000-0003-0165-8122 NR 19 TC 0 Z9 0 U1 0 U2 0 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD MAR PY 2016 VL 307 IS 3 BP 1871 EP 1876 DI 10.1007/s10967-015-4538-y PG 6 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA DG1ER UT WOS:000371808900053 ER PT J AU Arnquist, IJ Thomas, MLP Grate, JW Bliss, M Hoppe, EW AF Arnquist, Isaac J. Thomas, May-Lin P. Grate, Jay W. Bliss, Mary Hoppe, Eric W. TI A dry ashing assay method for the trace determination of Th and U in polymers using inductively coupled plasma mass spectrometry SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article; Proceedings Paper CT 10th International Conference on Methods and Applications of Radioanalytical Chemistry (MARC) CY APR 12-17, 2015 CL Kailua Kona, HI DE Polymers; Uranium; Thorium; Radiopurity assay; Inductively coupled plasma mass spectrometry ID DARK-MATTER DETECTOR; SAMPLE PREPARATION; RADIOACTIVITY; ELEMENTS; XENON; LEAD AB This paper discusses the methods developed for determining the radiopurity of high density polyethylene and polyetherketone ketone materials to be considered for use in ultralow background physics experiments. This work focuses on the processes used to render the polymeric samples acid soluble for subsequent ultratrace analysis using inductively coupled plasma mass spectrometry. High density polyethylene was determined to contain 2.19 +/- A 0.42 pg Th/g and 2.81 +/- A 0.52 pg U/g. The method provided very low absolute detection limits of 17.2 and 38.1 fg for Th and U, respectively. However, the polyetherketone ketone sample etched or devitrified the quartz, causing determined values to be a factor of 2-4 higher for Th and 5-9 higher for U from dissolution assay results. C1 [Arnquist, Isaac J.; Thomas, May-Lin P.; Grate, Jay W.; Bliss, Mary; Hoppe, Eric W.] Pacific NW Natl Lab, MSIN J4-60,POB 999, Richland, WA 99352 USA. RP Arnquist, IJ (reprint author), Pacific NW Natl Lab, MSIN J4-60,POB 999, Richland, WA 99352 USA. EM isaac.arnquist@pnnl.gov RI Bliss, Mary/G-2240-2012 OI Bliss, Mary/0000-0002-7565-4813 NR 38 TC 2 Z9 2 U1 2 U2 2 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD MAR PY 2016 VL 307 IS 3 BP 1883 EP 1890 DI 10.1007/s10967-015-4343-7 PG 8 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA DG1ER UT WOS:000371808900055 ER PT J AU Klingberg, FJ Biegalski, SR Prinke, A Haas, DA Lowrey, JD AF Klingberg, Franziska J. Biegalski, Steven R. Prinke, Amanda Haas, Derek A. Lowrey, Justin D. TI Analysis of Xe-125 electron-photon coincidence decay SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article; Proceedings Paper CT 10th International Conference on Methods and Applications of Radioanalytical Chemistry (MARC) CY APR 12-17, 2015 CL Kailua Kona, HI DE Radioxenon; Neutron activation; CTBT; Treaty verification AB As part of the verification component of the Comprehensive Nuclear-Test-Ban Treaty (CTBT), environmental gas samples originating from nuclear fission are analyzed for the presence of Xe-131m, Xe-133m, Xe-133, and Xe-135. In this work, the non-traditional radioxenon isotope Xe-125 was investigated. The isotope was produced as an isotopically pure sample via neutron activation of Xe-124 at the University of Texas at Austin Nuclear Engineering Teaching Lab's TRIGA MARK II Reactor. The sample was then measured using a HPGe detector as well as an ARSA-style beta-gamma coincidence detector. Potential sources and sensitivities for production of Xe-125 are also considered for relevance to the CTBT verification mission. C1 [Klingberg, Franziska J.; Biegalski, Steven R.] Univ Texas Austin, Nucl Engn Teaching Lab, 10100 Burnet Rd Bldg 159, Austin, TX 78758 USA. [Prinke, Amanda; Haas, Derek A.; Lowrey, Justin D.] Pacific NW Natl Lab, 902 Battelle Blvd,POB 999, Richland, WA 99352 USA. RP Klingberg, FJ (reprint author), Univ Texas Austin, Nucl Engn Teaching Lab, 10100 Burnet Rd Bldg 159, Austin, TX 78758 USA. EM klingberg@utexas.edu NR 12 TC 0 Z9 0 U1 2 U2 2 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD MAR PY 2016 VL 307 IS 3 BP 1933 EP 1939 DI 10.1007/s10967-015-4519-1 PG 7 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA DG1ER UT WOS:000371808900061 ER PT J AU Fujii, T Hori, JI Du, M Fukutani, S Takamiya, K Yamana, H Kiyanagi, Y AF Fujii, Toshiyuki Hori, Jun-ichi Du, Miting Fukutani, Satoshi Takamiya, Koichi Yamana, Hajimu Kiyanagi, Yoshiaki TI Isotopic composition of a sample enriched in Zr-93 SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article; Proceedings Paper CT 10th International Conference on Methods and Applications of Radioanalytical Chemistry (MARC) CY APR 12-17, 2015 CL Kailua Kona, HI DE Zirconium; Long lived fission product; Isotopic analysis; Nuclear data; J-PARC ID J-PARC/MLF/ANNRI; NUCLEAR-DATA; J-PARC AB A project to determine the neutron-capture cross section of long lived fission products and minor actinides has been started by using a beam-line at Japan Proton Accelerator Research Complex (J-PARC). One of the target nuclides is Zr-93, which was prepared in Oak Ridge National Laboratory. Qualitative and quantitative analyses on the sample were performed at Kyoto University. The isotopic composition of (m) Zr (m 90, 91, 92, 93, 94, and 96) was precisely determined by multi-collector thermal ionization mass spectrometry with < 0.1 % of 2 sigma uncertainty. The atomic abundance of Zr-93 in the sample was determined to be 18.86 +/- A 0.05 %. C1 [Fujii, Toshiyuki; Hori, Jun-ichi; Fukutani, Satoshi; Takamiya, Koichi; Yamana, Hajimu] Kyoto Univ, Inst Res Reactor, 2-1010 Asashiro Nishi, Sennan, Osaka 5900494, Japan. [Du, Miting] Oak Ridge Natl Lab, Nucl Secur & Isotope Technol Div, Oak Ridge, TN 37831 USA. [Kiyanagi, Yoshiaki] Hokkaido Univ, Grad Sch Engn, Sapporo, Hokkaido 0608628, Japan. RP Fujii, T (reprint author), Kyoto Univ, Inst Res Reactor, 2-1010 Asashiro Nishi, Sennan, Osaka 5900494, Japan. EM tosiyuki@rri.kyoto-u.ac.jp NR 12 TC 0 Z9 0 U1 3 U2 8 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD MAR PY 2016 VL 307 IS 3 BP 1945 EP 1948 DI 10.1007/s10967-015-4540-4 PG 4 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA DG1ER UT WOS:000371808900063 ER PT J AU Abir, M Islam, F Wachs, D Lee, HK AF Abir, Muhammad Islam, Fahima Wachs, Daniel Lee, Hyoung-Koo TI Sparse-view neutron CT reconstruction of irradiated fuel assembly using total variation minimization with Poisson statistics SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article; Proceedings Paper CT 10th International Conference on Methods and Applications of Radioanalytical Chemistry (MARC) CY APR 12-17, 2015 CL Kailua Kona, HI DE CT reconstruction; Sparse-view; Total variation minimization; Poisson statistics; Irradiated fuel assembly ID BEAM COMPUTED-TOMOGRAPHY; COMPRESSED SENSING PICCS; IMAGE-RECONSTRUCTION; VARIATION REGULARIZATION; ALGORITHM; PROJECTION; RESTORATION; NOISE AB We inspect the nuclear fuel assembly by demonstrating the potential use of sparse-view neutron computed tomography. The projection images of the fuel assembly were collected at the Idaho National Laboratory hot fuel examination facility using indirect foil-film transfer technique. The radiographs were digitized using a commercial film digitizer and registered spatially for reconstruction. Digitized data were reconstructed using simultaneous algebraic reconstruction technique (SART) with total variation minimization using a dual approach for numerical solution assuming the projection data are corrupted by Poisson noise. To validate and evaluate the performance of the algorithm, visual inspections, as well as quantitative evaluation studies using a computer simulation data and the experimental data of the fuel assembly were carried out. The proposed method provides better reconstruction for both simulated and experimental case in terms of artifact reduction, higher SNR, and better spatial resolution compared to the reconstruction yielded by filtered back projection and SART reconstruction. C1 [Abir, Muhammad; Wachs, Daniel] Idaho Natl Lab, Mat & Fuel Complex,POB 1625, Idaho Falls, ID 83415 USA. [Islam, Fahima; Lee, Hyoung-Koo] Missouri Univ Sci & Technol, Dept Min & Nucl Engn, 301 W 14th St, Rolla, MO 65409 USA. RP Lee, HK (reprint author), Missouri Univ Sci & Technol, Dept Min & Nucl Engn, 301 W 14th St, Rolla, MO 65409 USA. EM muhammad.abir@inl.gov; leehk@mst.edu NR 45 TC 0 Z9 0 U1 5 U2 9 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD MAR PY 2016 VL 307 IS 3 BP 1967 EP 1979 DI 10.1007/s10967-015-4542-2 PG 13 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA DG1ER UT WOS:000371808900067 ER EF